FN Thomson Reuters Web of Science™
VR 1.0
PT J
AU Ruffing, AM
AF Ruffing, Anne M.
TI RNA-Seq analysis and targeted mutagenesis for improved free fatty acid
production in an engineered cyanobacterium
SO BIOTECHNOLOGY FOR BIOFUELS
LA English
DT Article
DE Free fatty acid biosynthesis; FFA biosynthesis; Cyanobacterial biofuels;
Algal biofuels; Cyanobacteria; Free fatty acid; RNA-seq; FFA toxicity
ID SYNECHOCYSTIS SP PCC-6803; GENE-EXPRESSION; ESCHERICHIA-COLI; OXIDATIVE
STRESS; OSMOTIC-STRESS; HIGH LIGHT; IDENTIFICATION; CHLOROPLAST;
ACTIVATION; BIODIESEL
AB Background: High-energy-density biofuels are typically derived from the fatty acid pathway, thus establishing free fatty acids (FFAs) as important fuel precursors. FFA production using photosynthetic microorganisms like cyanobacteria allows for direct conversion of carbon dioxide into fuel precursors. Recent studies investigating cyanobacterial FFA production have demonstrated the potential of this process, yet FFA production was also shown to have negative physiological effects on the cyanobacterial host, ultimately limiting high yields of FFAs.
Results: Cyanobacterial FFA production was shown to generate reactive oxygen species (ROS) and lead to increased cell membrane permeability. To identify genetic targets that may mitigate these toxic effects, RNA-seq analysis was used to investigate the host response of Synechococcus elongatus PCC 7942. Stress response, nitrogen metabolism, photosynthesis, and protein folding genes were up-regulated during FFA production while genes involved in carbon and hydrogen metabolisms were down-regulated. Select genes were targeted for mutagenesis to confirm their role in mitigating FFA toxicity. Gene knockout of two porins and the overexpression of ROS-degrading proteins and hypothetical proteins reduced the toxic effects of FFA production, allowing for improved growth, physiology, and FFA yields. Comparative transcriptomics, analyzing gene expression changes associated with FFA production and other stress conditions, identified additional key genes involved in cyanobacterial stress response.
Conclusions: A total of 15 gene targets were identified to reduce the toxic effects of FFA production. While single-gene targeted mutagenesis led to minor increases in FFA production, the combination of these targeted mutations may yield additional improvement, advancing the development of high-energy-density fuels derived from cyanobacteria.
C1 Sandia Natl Labs, Dept Bioenergy & Def Technol, Albuquerque, NM 87185 USA.
RP Ruffing, AM (reprint author), Sandia Natl Labs, Dept Bioenergy & Def Technol, MS 1413,POB 5800, Albuquerque, NM 87185 USA.
EM aruffin@sandia.gov
FU Harry S. Truman Fellowship in National Security Science and Engineering;
Laboratory Directed Research and Development program; United States
Department of Energy [DE-ACO4-94AL85000]
FX This work was supported by the Harry S. Truman Fellowship in National
Security Science and Engineering and the Laboratory Directed Research
and Development program. Sandia is a multi-program laboratory operated
by Sandia Corporation, a Lockheed Martin Company, for the United States
Department of Energy under Contract DE-ACO4-94AL85000. Next-gen
sequencing for the RNA-seq analysis was performed at Los Alamos National
Laboratory. The author is grateful to Dr. James Laio (University of
California, Los Angeles) and Dr. Susan Golden (University of California,
San Diego) for providing plasmids pSA126 and pAM2991. The author would
also like to acknowledge Bryan Carson for the use of laboratory
equipment.
NR 42
TC 22
Z9 22
U1 3
U2 40
PU BIOMED CENTRAL LTD
PI LONDON
PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND
SN 1754-6834
J9 BIOTECHNOL BIOFUELS
JI Biotechnol. Biofuels
PD AUG 6
PY 2013
VL 6
AR 113
DI 10.1186/1754-6834-6-113
PG 15
WC Biotechnology & Applied Microbiology; Energy & Fuels
SC Biotechnology & Applied Microbiology; Energy & Fuels
GA 198EZ
UT WOS:000322906200001
PM 23919451
ER
PT J
AU Gerrish, PJ
Colato, A
Sniegowski, PD
AF Gerrish, Philip J.
Colato, Alexandre
Sniegowski, Paul D.
TI Genomic mutation rates that neutralize adaptive evolution and natural
selection
SO JOURNAL OF THE ROYAL SOCIETY INTERFACE
LA English
DT Article
DE population genetics; mutagenesis; error threshold; Fisher's fundamental
theorem; beneficial mutations
ID SINGLE-NUCLEOTIDE SUBSTITUTIONS; IMMUNODEFICIENCY-VIRUS TYPE-1; DYNAMIC
FITNESS LANDSCAPES; DEPENDENT RNA-POLYMERASE; QUASI-SPECIES MODEL;
ERROR-THRESHOLD; MULLERS RATCHET; LETHAL MUTAGENESIS; ASEXUAL
POPULATIONS; SACCHAROMYCES-CEREVISIAE
AB When mutation rates are low, natural selection remains effective, and increasing the mutation rate can give rise to an increase in adaptation rate. When mutation rates are high to begin with, however, increasing the mutation rate may have a detrimental effect because of the overwhelming presence of deleterious mutations. Indeed, if mutation rates are high enough: (i) adaptive evolution may be neutralized, resulting in a zero (or negative) adaptation rate despite the continued availability of adaptive and/or compensatory mutations, or (ii) natural selection may be neutralized, because the fitness of lineages bearing adaptive and/or compensatory mutations-whether established or newly arising-is eroded by excessive mutation, causing such lineages to decline in frequency. We apply these two criteria to a standard model of asexual adaptive evolution and derive mathematical expressions-some new, some old in new guise-delineating the mutation rates under which either adaptive evolution or natural selection is neutralized. The expressions are simple and require no a priori knowledge of organism- and/or environment-specific parameters. Our discussion connects these results to each other and to previous theory, showing convergence or equivalence of the different results in most cases.
C1 [Gerrish, Philip J.] Univ New Mexico, Dept Biol, Ctr Evolutionary & Theoret Immunol, Albuquerque, NM 87131 USA.
[Gerrish, Philip J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Colato, Alexandre] Fed Univ Sao Carlos UFSCar, Dept Ciencias Nat Matemat & Educ, Araras, Brazil.
[Sniegowski, Paul D.] Univ Penn, Dept Biol, Leidy Labs 213, Philadelphia, PA 19104 USA.
RP Gerrish, PJ (reprint author), Univ New Mexico, Dept Biol, Ctr Evolutionary & Theoret Immunol, 230 Castetter Hall,MSC03-2020, Albuquerque, NM 87131 USA.
EM pgerrish@unm.edu
RI Colato, Alexandre/G-6818-2012;
OI Colato, Alexandre/0000-0003-0076-007X; Gerrish,
Philip/0000-0001-6393-0553
FU US National Institutes of Health [R01 GM079843-01, R01 GM079483-02S1,
1P20RR18754, UM1-AI100645-01]; European Commission [FP7 231807]
FX Special thanks to Cristian Batista for insightful explanations of the
error threshold as a phase transition, to Isabel Gordo for helping make
connections among the different theories and to Claus Wilke for helpful
comments and clarifications. We also thank Michael Lassig, Paul Joyce,
Alan Perelson, Boris Shraiman, Sidhartha Goyal, Daniel Balick, Nico
Stollenwerk, Gabriela Gomes, Ana Margarida Sousa, Jorge Carneiro and
Josep Sardanyes for helpful discussions, and two anonymous reviewers for
helpful comments. Much of this research was developed thanks to fertile
environments provided by two institutes: the Kavli Institute for
Theoretical Physics in Santa Barbara, CA (2011 Microbial and Viral
Evolution workshop), and the Instituto Gulbenkian de Ciencias in Oeiras,
Portugal. This work was supported by the US National Institutes of
Health grants: R01 GM079843-01 (P.J.G./P.D.S.), R01 GM079483-02S1
(P.J.G./P.D.S.), a seed grant through 1P20RR18754 (Center for
Evolutionary and Theoretical Immunology) (P.J.G.), UM1-AI100645-01
(Center for HIV/AIDS Vaccine Immunology-Immunogen Design; P.J.G.); and
European Commission grant no. FP7 231807 (P.J.G.).
NR 86
TC 4
Z9 4
U1 2
U2 31
PU ROYAL SOC
PI LONDON
PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND
SN 1742-5689
J9 J R SOC INTERFACE
JI J. R. Soc. Interface
PD AUG 6
PY 2013
VL 10
IS 85
AR 20130329
DI 10.1098/rsif.2013.0329
PG 12
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 167DL
UT WOS:000320610700017
PM 23720539
ER
PT J
AU Aaltonen, T
Amerio, S
Amidei, D
Anastassov, A
Annovi, A
Antos, J
Apollinari, G
Appel, JA
Arisawa, T
Artikov, A
Asaadi, J
Ashmanskas, W
Auerbach, B
Aurisano, A
Azfar, F
Badgett, W
Bae, T
Barbaro-Galtieri, A
Barnes, VE
Barnett, BA
Barria, P
Bartos, P
Bauce, M
Bedeschi, F
Behari, S
Bellettini, G
Bellinger, J
Benjamin, D
Beretvas, A
Bhatti, A
Bland, KR
Blumenfeld, B
Bocci, A
Bodek, A
Boisvert, V
Bortoletto, D
Boudreau, J
Boveia, A
Brigliadori, L
Bromberg, C
Brucken, E
Budagov, J
Budd, HS
Burkett, K
Busetto, G
Bussey, P
Butti, P
Buzatu, A
Calamba, A
Camarda, S
Campanelli, M
Canelli, F
Carls, B
Carlsmith, D
Carosi, R
Carrillo, S
Casal, B
Casarsa, M
Castro, A
Catastin, P
Cauz, D
Cavaliere, V
Cavalli-Sforza, M
Cerri, A
Cerrito, L
Chen, YC
Chertok, M
Chiarelli, G
Chlachidze, G
Cho, K
Chokheli, D
Ciocci, MA
Clark, A
Clarke, C
Convery, ME
Conway, J
Corbo, M
Cordelli, M
Cox, CA
Cox, DJ
Cremonesi, M
Cruz, D
Cuevas, J
Culbertson, R
d'Ascenzo, N
Datta, M
De Barbaro, P
Demortier, L
Deninno, M
d'Errico, M
Devoto, F
Di Canto, A
Di Ruzza, B
Dittmann, JR
D'Onofrio, M
Donati, S
Dorigo, M
Driutti, A
Ebina, K
Edgar, R
Elagin, A
Erbacher, R
Errede, S
Esham, B
Eusebi, R
Farrington, S
Ramos, JPF
Field, R
Flanagan, G
Forrest, R
Franklin, M
Freeman, JC
Frisch, H
Funakoshi, Y
Garfinkel, AF
Garosi, P
Gerberich, H
Gerchtein, E
Giagu, S
Giakoumopoulou, V
Gibson, K
Ginsburg, CM
Giokaris, N
Giromini, P
Giurgiu, G
Glagolev, V
Glenzinski, D
Gold, M
Goldin, D
Golossanov, A
Gomez, G
Gomez-Ceballos, G
Goncharov, M
Lopez, OG
Gorelov, I
Goshaw, AT
Goulianos, K
Gramellini, E
Grinstein, S
Grosso-Pilcher, C
Group, RC
da Costa, JG
Hahn, SR
Han, JY
Happacher, F
Hara, K
Hare, M
Harr, RF
Harrington-Taber, T
Hatakeyama, K
Hays, C
Heinrich, J
Herndon, M
Hocker, A
Hong, Z
Hopkins, W
Hou, S
Hughes, RE
Husemann, U
Hussein, M
Huston, J
Introzzi, G
Iori, M
Ivanov, A
James, E
Jang, D
Jayatilaka, B
Jeon, EJ
Jindariani, S
Jones, M
Joo, KK
Jun, SY
Junk, TR
Kambeitz, M
Kamon, T
Karchin, PE
Kasmi, A
Kato, Y
Ketchum, W
Keung, J
Kilminster, B
Kim, DH
Kim, HS
Kim, JE
Kim, MJ
Kim, SB
Kim, SH
Kim, YJ
Kim, YK
Kimura, N
Kirby, M
Knoepfel, K
Kondo, K
Kong, DJ
Konigsberg, J
Kotwal, AV
Kreps, M
Kroll, J
Kruse, M
Kuhr, T
Kurata, M
Laasanen, AT
Lammel, S
Lancaster, M
Lannon, K
Latino, G
Lee, HS
Lee, JS
Leo, S
Leone, S
Lewis, JD
Limosani, A
Lipeles, E
Lister, A
Liu, H
Liu, Q
Liu, T
Lockwitz, S
Loginov, A
Luca, A
Lucchesi, D
Lueck, J
Lujan, P
Lukens, P
Lungu, G
Lys, J
Lysak, R
Madrak, R
Maestro, P
Malik, S
Manca, G
Manousakis-Katsikakis, A
Margaroli, F
Marino, P
Martinez, M
Matera, K
Mattson, ME
Mazzacane, A
Mazzanti, P
McFarland, KS
McNulty, R
Mehta, A
Mehtala, P
Mesropian, C
Miao, T
Mietlicki, D
Mitra, A
Miyake, H
Moed, S
Moggi, N
Moon, CS
Moore, R
Morello, MJ
Mukherjee, A
Muller, T
Murat, P
Mussini, M
Nachtman, J
Nagai, Y
Naganoma, J
Nakano, I
Napier, A
Nett, J
Neu, C
Nigmanov, T
Nodulman, L
Noh, SY
Norniella, O
Oakes, L
Oh, SH
Oh, YD
Oksuzian, I
Okusawa, T
Orava, R
Ortolan, L
Pagliarone, C
Palencia, E
Palni, P
Papadimitriou, V
Parker, W
Pauletta, G
Paulini, M
Paus, C
Phillips, TJ
Piacentino, G
Pianori, E
Pilot, J
Pitts, K
Plager, C
Pondrom, L
Poprocki, S
Potamianos, K
Pranko, A
Prokoshin, F
Ptohos, F
Punzi, G
Ranjan, N
Fernandez, IR
Renton, P
Rescigno, M
Rimondi, F
Ristori, L
Robson, A
Rodriguez, T
Rolli, S
Ronzani, M
Roser, R
Rosner, JL
Ruffini, F
Ruiz, A
Russ, J
Rusu, V
Sakumoto, WK
Sakurai, Y
Santi, L
Sato, K
Saveliev, V
Savoy-Navarro, A
Schlabach, P
Schmidt, EE
Schwarz, T
Scodellaro, L
Scuri, F
Seidel, S
Seiya, Y
Semenov, A
Sforza, F
Shalhout, SZ
Shears, T
Shepard, PF
Shimojima, M
Shochet, M
Shreyber-Tecker, I
Simonenko, A
Sinervo, P
Sliwa, K
Smith, JR
Snider, FD
Song, H
Sorin, V
Stancari, M
St Denis, R
Stelzer, B
Stelzer-Chilton, O
Stentz, D
Strologas, J
Sudo, Y
Sukhanov, A
Suslov, I
Takemasa, K
Takeuchi, Y
Tang, J
Tecchio, M
Teng, PK
Thom, J
Thomson, E
Thukral, V
Toback, D
Tokar, S
Tollefson, K
Tomura, T
Tonelli, D
Torre, S
Torretta, D
Totaro, P
Trovato, M
Ukegawa, F
Uozumi, S
Vazquez, F
Velev, G
Vellidis, C
Vernieri, C
Vidal, M
Vilar, R
Vizan, J
Vogel, M
Volpi, G
Wagner, P
Wallny, R
Wang, SM
Warburton, A
Waters, D
Wester, WC
Whiteson, D
Wicklund, AB
Wilbur, S
Williams, HH
Wilson, JS
Wilson, P
Winer, BL
Wittich, P
Wolbers, S
Wolfe, H
Wright, T
Wu, X
Wu, Z
Yamamoto, K
Yamato, D
Yang, T
Yang, UK
Yang, YC
Yao, WM
Yeh, GP
Yi, K
Yoh, J
Yorita, K
Yoshida, T
Yu, GB
Yu, I
Zanetti, AM
Zeng, Y
Zhou, C
Zucchelli, S
AF Aaltonen, T.
Amerio, S.
Amidei, D.
Anastassov, A.
Annovi, A.
Antos, J.
Apollinari, G.
Appel, J. A.
Arisawa, T.
Artikov, A.
Asaadi, J.
Ashmanskas, W.
Auerbach, B.
Aurisano, A.
Azfar, F.
Badgett, W.
Bae, T.
Barbaro-Galtieri, A.
Barnes, V. E.
Barnett, B. A.
Barria, P.
Bartos, P.
Bauce, M.
Bedeschi, F.
Behari, S.
Bellettini, G.
Bellinger, J.
Benjamin, D.
Beretvas, A.
Bhatti, A.
Bland, K. R.
Blumenfeld, B.
Bocci, A.
Bodek, A.
Boisvert, V.
Bortoletto, D.
Boudreau, J.
Boveia, A.
Brigliadori, L.
Bromberg, C.
Brucken, E.
Budagov, J.
Budd, H. S.
Burkett, K.
Busetto, G.
Bussey, P.
Butti, P.
Buzatu, A.
Calamba, A.
Camarda, S.
Campanelli, M.
Canelli, F.
Carls, B.
Carlsmith, D.
Carosi, R.
Carrillo, S.
Casal, B.
Casarsa, M.
Castro, A.
Catastin, P.
Cauz, D.
Cavaliere, V.
Cavalli-Sforza, M.
Cerri, A.
Cerrito, L.
Chen, Y. C.
Chertok, M.
Chiarelli, G.
Chlachidze, G.
Cho, K.
Chokheli, D.
Ciocci, M. A.
Clark, A.
Clarke, C.
Convery, M. E.
Conway, J.
Corbo, M.
Cordelli, M.
Cox, C. A.
Cox, D. J.
Cremonesi, M.
Cruz, D.
Cuevas, J.
Culbertson, R.
d'Ascenzo, N.
Datta, M.
De Barbaro, P.
Demortier, L.
Deninno, M.
d'Errico, M.
Devoto, F.
Di Canto, A.
Di Ruzza, B.
Dittmann, J. R.
D'Onofrio, M.
Donati, S.
Dorigo, M.
Driutti, A.
Ebina, K.
Edgar, R.
Elagin, A.
Erbacher, R.
Errede, S.
Esham, B.
Eusebi, R.
Farrington, S.
Fernandez Ramos, J. P.
Field, R.
Flanagan, G.
Forrest, R.
Franklin, M.
Freeman, J. C.
Frisch, H.
Funakoshi, Y.
Garfinkel, A. F.
Garosi, P.
Gerberich, H.
Gerchtein, E.
Giagu, S.
Giakoumopoulou, V.
Gibson, K.
Ginsburg, C. M.
Giokaris, N.
Giromini, P.
Giurgiu, G.
Glagolev, V.
Glenzinski, D.
Gold, M.
Goldin, D.
Golossanov, A.
Gomez, G.
Gomez-Ceballos, G.
Goncharov, M.
Gonzalez Lopez, O.
Gorelov, I.
Goshaw, A. T.
Goulianos, K.
Gramellini, E.
Grinstein, S.
Grosso-Pilcher, C.
Group, R. C.
da Costa, J. Guimaraes
Hahn, S. R.
Han, J. Y.
Happacher, F.
Hara, K.
Hare, M.
Harr, R. F.
Harrington-Taber, T.
Hatakeyama, K.
Hays, C.
Heinrich, J.
Herndon, M.
Hocker, A.
Hong, Z.
Hopkins, W.
Hou, S.
Hughes, R. E.
Husemann, U.
Hussein, M.
Huston, J.
Introzzi, G.
Iori, M.
Ivanov, A.
James, E.
Jang, D.
Jayatilaka, B.
Jeon, E. J.
Jindariani, S.
Jones, M.
Joo, K. K.
Jun, S. Y.
Junk, T. R.
Kambeitz, M.
Kamon, T.
Karchin, P. E.
Kasmi, A.
Kato, Y.
Ketchum, W.
Keung, J.
Kilminster, B.
Kim, D. H.
Kim, H. S.
Kim, J. E.
Kim, M. J.
Kim, S. B.
Kim, S. H.
Kim, Y. J.
Kim, Y. K.
Kimura, N.
Kirby, M.
Knoepfel, K.
Kondo, K.
Kong, D. J.
Konigsberg, J.
Kotwal, A. V.
Kreps, M.
Kroll, J.
Kruse, M.
Kuhr, T.
Kurata, M.
Laasanen, A. T.
Lammel, S.
Lancaster, M.
Lannon, K.
Latino, G.
Lee, H. S.
Lee, J. S.
Leo, S.
Leone, S.
Lewis, J. D.
Limosani, A.
Lipeles, E.
Lister, A.
Liu, H.
Liu, Q.
Liu, T.
Lockwitz, S.
Loginov, A.
Luca, A.
Lucchesi, D.
Lueck, J.
Lujan, P.
Lukens, P.
Lungu, G.
Lys, J.
Lysak, R.
Madrak, R.
Maestro, P.
Malik, S.
Manca, G.
Manousakis-Katsikakis, A.
Margaroli, F.
Marino, P.
Martinez, M.
Matera, K.
Mattson, M. E.
Mazzacane, A.
Mazzanti, P.
McFarland, K. S.
McNulty, R.
Mehta, A.
Mehtala, P.
Mesropian, C.
Miao, T.
Mietlicki, D.
Mitra, A.
Miyake, H.
Moed, S.
Moggi, N.
Moon, C. S.
Moore, R.
Morello, M. J.
Mukherjee, A.
Muller, Th.
Murat, P.
Mussini, M.
Nachtman, J.
Nagai, Y.
Naganoma, J.
Nakano, I.
Napier, A.
Nett, J.
Neu, C.
Nigmanov, T.
Nodulman, L.
Noh, S. Y.
Norniella, O.
Oakes, L.
Oh, S. H.
Oh, Y. D.
Oksuzian, I.
Okusawa, T.
Orava, R.
Ortolan, L.
Pagliarone, C.
Palencia, E.
Palni, P.
Papadimitriou, V.
Parker, W.
Pauletta, G.
Paulini, M.
Paus, C.
Phillips, T. J.
Piacentino, G.
Pianori, E.
Pilot, J.
Pitts, K.
Plager, C.
Pondrom, L.
Poprocki, S.
Potamianos, K.
Pranko, A.
Prokoshin, F.
Ptohos, F.
Punzi, G.
Ranjan, N.
Redondo Fernandez, I.
Renton, P.
Rescigno, M.
Rimondi, F.
Ristori, L.
Robson, A.
Rodriguez, T.
Rolli, S.
Ronzani, M.
Roser, R.
Rosner, J. L.
Ruffini, F.
Ruiz, A.
Russ, J.
Rusu, V.
Sakumoto, W. K.
Sakurai, Y.
Santi, L.
Sato, K.
Saveliev, V.
Savoy-Navarro, A.
Schlabach, P.
Schmidt, E. E.
Schwarz, T.
Scodellaro, L.
Scuri, F.
Seidel, S.
Seiya, Y.
Semenov, A.
Sforza, F.
Shalhout, S. Z.
Shears, T.
Shepard, P. F.
Shimojima, M.
Shochet, M.
Shreyber-Tecker, I.
Simonenko, A.
Sinervo, P.
Sliwa, K.
Smith, J. R.
Snider, F. D.
Song, H.
Sorin, V.
Stancari, M.
St Denis, R.
Stelzer, B.
Stelzer-Chilton, O.
Stentz, D.
Strologas, J.
Sudo, Y.
Sukhanov, A.
Suslov, I.
Takemasa, K.
Takeuchi, Y.
Tang, J.
Tecchio, M.
Teng, P. K.
Thom, J.
Thomson, E.
Thukral, V.
Toback, D.
Tokar, S.
Tollefson, K.
Tomura, T.
Tonelli, D.
Torre, S.
Torretta, D.
Totaro, P.
Trovato, M.
Ukegawa, F.
Uozumi, S.
Vazquez, F.
Velev, G.
Vellidis, C.
Vernieri, C.
Vidal, M.
Vilar, R.
Vizan, J.
Vogel, M.
Volpi, G.
Wagner, P.
Wallny, R.
Wang, S. M.
Warburton, A.
Waters, D.
Wester, W. C., III
Whiteson, D.
Wicklund, A. B.
Wilbur, S.
Williams, H. H.
Wilson, J. S.
Wilson, P.
Winer, B. L.
Wittich, P.
Wolbers, S.
Wolfe, H.
Wright, T.
Wu, X.
Wu, Z.
Yamamoto, K.
Yamato, D.
Yang, T.
Yang, U. K.
Yang, Y. C.
Yao, W. -M.
Yeh, G. P.
Yi, K.
Yoh, J.
Yorita, K.
Yoshida, T.
Yu, G. B.
Yu, I.
Zanetti, A. M.
Zeng, Y.
Zhou, C.
Zucchelli, S.
CA CDF Collaboration
TI Exclusion of exotic top-like quarks with-4/3 electric charge using
jet-charge tagging in single-lepton t(t)over-bar events at CDF
SO PHYSICAL REVIEW D
LA English
DT Article
ID PARTON DISTRIBUTIONS; COLLIDER DETECTOR; CALORIMETER; COLLISIONS;
FERMILAB
AB We report on a measurement of the top-quark electric charge in t (t) over bar events in which one W boson originating from the top-quark pair decays into leptons and the other into hadrons. The event sample was collected by the CDF II detector in root s = 1.96 TeV proton-antiproton collisions and corresponds to 5.6 fb(-1). We find the data to be consistent with the standard model and exclude the existence of an exotic quark with -4/3 electric charge and mass of the conventional top quark at the 99% confidence level.
C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan.
[Auerbach, B.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Giakoumopoulou, V.; Giokaris, N.; Manousakis-Katsikakis, A.] Univ Athens, GR-15771 Athens, Greece.
[Camarda, S.; Cavalli-Sforza, M.; Grinstein, S.; Martinez, M.; Ortolan, L.; Sorin, V.] Univ Autonoma Barcelona, ICREA, Inst Fis Altes Energies, E-08193 Bellaterra, Barcelona, Spain.
[Bland, K. R.; Dittmann, J. R.; Hatakeyama, K.; Kasmi, A.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA.
[Brigliadori, L.; Castro, A.; Deninno, M.; Gramellini, E.; Mazzanti, P.; Moggi, N.; Mussini, M.; Rimondi, F.; Zucchelli, S.] Ist Nazl Fis Nucl Bologna, I-40127 Bologna, Italy.
[Brigliadori, L.; Castro, A.; Mussini, M.; Zucchelli, S.] Univ Bologna, I-40127 Bologna, Italy.
[Chertok, M.; Conway, J.; Cox, C. A.; Cox, D. J.; Erbacher, R.; Forrest, R.; Ivanov, A.; Shalhout, S. Z.; Smith, J. R.] Univ Calif Davis, Davis, CA 95616 USA.
[Plager, C.; Wallny, R.] Univ Calif Los Angeles, Los Angeles, CA 90024 USA.
[Cuevas, J.; Gomez, G.; Palencia, E.; Ruiz, A.; Scodellaro, L.; Vilar, R.; Vizan, J.] Univ Cantabria, CSIC, Inst Fis Cantabria, E-39005 Santander, Spain.
[Calamba, A.; Jang, D.; Jun, S. Y.; Paulini, M.; Russ, J.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA.
[Boveia, A.; Canelli, F.; Frisch, H.; Grosso-Pilcher, C.; Ketchum, W.; Kim, Y. K.; Rosner, J. L.; Shochet, M.; Tang, J.; Wilbur, S.; Yang, U. K.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA.
[Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Comenius Univ, Bratislava 84248, Slovakia.
[Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Inst Expt Phys, Kosice 04001, Slovakia.
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[Anastassov, A.; Apollinari, G.; Appel, J. A.; Ashmanskas, W.; Badgett, W.; Behari, S.; Beretvas, A.; Burkett, K.; Canelli, F.; Chlachidze, G.; Convery, M. E.; Corbo, M.; Culbertson, R.; d'Ascenzo, N.; Datta, M.; Di Ruzza, B.; Flanagan, G.; Freeman, J. C.; Gerchtein, E.; Ginsburg, C. M.; Glenzinski, D.; Golossanov, A.; Group, R. C.; Hahn, S. R.; Harrington-Taber, T.; Hocker, A.; Hopkins, W.; James, E.; Jayatilaka, B.; Jindariani, S.; Junk, T. R.; Kilminster, B.; Kirby, M.; Knoepfel, K.; Lammel, S.; Lewis, J. D.; Liu, T.; Lukens, P.; Madrak, R.; Mazzacane, A.; Miao, T.; Moed, S.; Moon, C. S.; Moore, R.; Mukherjee, A.; Murat, P.; Nachtman, J.; Papadimitriou, V.; Poprocki, S.; Ristori, L.; Roser, R.; Rusu, V.; Saveliev, V.; Savoy-Navarro, A.; Schlabach, P.; Schmidt, E. E.; Snider, F. D.; Stancari, M.; Stentz, D.; Sukhanov, A.; Thom, J.; Tonelli, D.; Torretta, D.; Velev, G.; Vellidis, C.; Wester, W. C., III; Wilson, P.; Wittich, P.; Wolbers, S.; Yang, T.; Yeh, G. P.; Yi, K.; Yoh, J.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
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[Clark, A.; Lister, A.; Wu, X.] Univ Geneva, CH-1211 Geneva 4, Switzerland.
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[Aaltonen, T.; Brucken, E.; Devoto, F.; Mehtala, P.; Orava, R.] Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland.
[Aaltonen, T.; Brucken, E.; Devoto, F.; Mehtala, P.; Orava, R.] Helsinki Inst Phys, FIN-00014 Helsinki, Finland.
[Carls, B.; Cavaliere, V.; Errede, S.; Esham, B.; Gerberich, H.; Matera, K.; Norniella, O.; Pitts, K.] Univ Illinois, Urbana, IL 61801 USA.
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[Kambeitz, M.; Kreps, M.; Kuhr, T.; Lueck, J.; Muller, Th.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany.
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[Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, Y. C.; Yu, I.] Sungkyunkwan Univ, Suwon 440746, South Korea.
[Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, Y. C.; Yu, I.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea.
[Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, Y. C.; Yu, I.] Chonnam Natl Univ, Kwangju 500757, South Korea.
[Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, Y. C.; Yu, I.] Chonbuk Natl Univ, Jeonju 561756, South Korea.
[Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, Y. C.; Yu, I.] Ewha Womans Univ, Seoul 120750, South Korea.
[Barbaro-Galtieri, A.; Cerri, A.; Lujan, P.; Lys, J.; Potamianos, K.; Pranko, A.; Yao, W. -M.] Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[D'Onofrio, M.; Manca, G.; McNulty, R.; Mehta, A.; Shears, T.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England.
[Campanelli, M.; Cerrito, L.; Lancaster, M.; Waters, D.] UCL, London WC1E 6BT, England.
[Fernandez Ramos, J. P.; Gonzalez Lopez, O.; Redondo Fernandez, I.] Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain.
[Gomez-Ceballos, G.; Goncharov, M.; Paus, C.] MIT, Cambridge, MA 02139 USA.
[Sinervo, P.; Stelzer, B.; Stelzer-Chilton, O.; Warburton, A.] McGill Univ, Inst Particle Phys, Montreal, PQ H3A 2T8, Canada.
[Sinervo, P.; Stelzer, B.; Stelzer-Chilton, O.; Warburton, A.] Simon Fraser Univ, Burnaby, BC V5A 1S6, Canada.
[Sinervo, P.; Stelzer, B.; Stelzer-Chilton, O.; Warburton, A.] Univ Toronto, Toronto, ON M5S 1A7, Canada.
[Sinervo, P.; Stelzer, B.; Stelzer-Chilton, O.; Warburton, A.] TRIUMF, Vancouver, BC V6T 2A3, Canada.
[Amidei, D.; Edgar, R.; Mietlicki, D.; Schwarz, T.; Tecchio, M.; Wilson, J. S.; Wright, T.] Univ Michigan, Ann Arbor, MI 48109 USA.
[Bromberg, C.; Hussein, M.; Huston, J.; Tollefson, K.] Michigan State Univ, E Lansing, MI 48824 USA.
[Shreyber-Tecker, I.] ITEP, Moscow 117259, Russia.
[Gold, M.; Gorelov, I.; Palni, P.; Seidel, S.; Strologas, J.; Vogel, M.] Univ New Mexico, Albuquerque, NM 87131 USA.
[Hughes, R. E.; Lannon, K.; Pilot, J.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA.
[Nakano, I.] Okayama Univ, Okayama 7008530, Japan.
[Kato, Y.; Okusawa, T.; Seiya, Y.; Yamamoto, K.; Yamato, D.; Yoshida, T.] Osaka City Univ, Osaka 588, Japan.
[Azfar, F.; Farrington, S.; Hays, C.; Oakes, L.; Renton, P.] Univ Oxford, Oxford OX1 3RH, England.
[Amerio, S.; Bauce, M.; Busetto, G.; d'Errico, M.; Lucchesi, D.; Totaro, P.] Ist Nazl Fis Nucl, Sez Padova Trento, I-35131 Padua, Italy.
[Bauce, M.; Busetto, G.; d'Errico, M.; Lucchesi, D.] Univ Padua, I-35131 Padua, Italy.
[Heinrich, J.; Keung, J.; Kroll, J.; Lipeles, E.; Pianori, E.; Ristori, L.; Rodriguez, T.; Thomson, E.; Wagner, P.; Whiteson, D.; Williams, H. H.] Univ Penn, Philadelphia, PA 19104 USA.
[Barria, P.; Bedeschi, F.; Bellettini, G.; Butti, P.; Carosi, R.; Chiarelli, G.; Ciocci, M. A.; Cremonesi, M.; Di Canto, A.; Donati, S.; Garosi, P.; Introzzi, G.; Latino, G.; Leo, S.; Leone, S.; Maestro, P.; Marino, P.; Morello, M. J.; Piacentino, G.; Punzi, G.; Ronzani, M.; Ruffini, F.; Scuri, F.; Sforza, F.; Trovato, M.; Vernieri, C.] Ist Nazl Fis Nucl, I-56127 Pisa, Italy.
[Bellettini, G.; Butti, P.; Di Canto, A.; Donati, S.; Punzi, G.; Ronzani, M.; Sforza, F.] Univ Pisa, I-56127 Pisa, Italy.
[Barria, P.; Ciocci, M. A.; Garosi, P.; Latino, G.; Maestro, P.; Ruffini, F.] Univ Siena, I-56127 Pisa, Italy.
[Marino, P.; Morello, M. J.; Trovato, M.; Vernieri, C.] Scuola Normale Super Pisa, I-56127 Pisa, Italy.
[Introzzi, G.] INFN Pavia, I-27100 Pavia, Italy.
[Introzzi, G.] Univ Pavia, I-27100 Pavia, Italy.
[Boudreau, J.; Gibson, K.; Nigmanov, T.; Shepard, P. F.; Song, H.] Univ Pittsburgh, Pittsburgh, PA 15260 USA.
[Barnes, V. E.; Bortoletto, D.; Garfinkel, A. F.; Jones, M.; Laasanen, A. T.; Liu, Q.; Ranjan, N.; Vidal, M.] Purdue Univ, W Lafayette, IN 47907 USA.
[Bodek, A.; Boisvert, V.; Budd, H. S.; De Barbaro, P.; Han, J. Y.; McFarland, K. S.; Sakumoto, W. K.] Univ Rochester, Rochester, NY 14627 USA.
[Bhatti, A.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10065 USA.
[Giagu, S.; Iori, M.; Margaroli, F.; Rescigno, M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy.
[Iori, M.] Univ Roma La Sapienza, I-00185 Rome, Italy.
[Asaadi, J.; Aurisano, A.; Cruz, D.; Elagin, A.; Eusebi, R.; Goldin, D.; Hong, Z.; Kamon, T.; Nett, J.; Thukral, V.; Toback, D.] Texas A&M Univ, Mitchell Inst Fundamental Phys & Astron, College Stn, TX 77843 USA.
[Casarsa, M.; Cauz, D.; Dorigo, M.; Driutti, A.; Pagliarone, C.; Pauletta, G.; Santi, L.; Zanetti, A. M.] Ist Nazl Fis Nucl Trieste Udine, I-34127 Trieste, Italy.
[Dorigo, M.] Univ Trieste, I-34127 Trieste, Italy.
[Pauletta, G.; Santi, L.] Univ Udine, I-33100 Udine, Italy.
[Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan.
[Group, R. C.; Hare, M.; Napier, A.; Rolli, S.; Sliwa, K.] Tufts Univ, Medford, MA 02155 USA.
[Liu, H.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA.
[Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan.
[Clarke, C.; Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA.
[Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA.
[Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA.
RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland.
RI ciocci, maria agnese /I-2153-2015; Cavalli-Sforza, Matteo/H-7102-2015;
Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015;
Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov,
Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; Martinez, Mario
/I-3549-2015; Warburton, Andreas/N-8028-2013; Kim, Soo-Bong/B-7061-2014;
Robson, Aidan/G-1087-2011; maestro, paolo/E-3280-2010; Chiarelli,
Giorgio/E-8953-2012; Lysak, Roman/H-2995-2014; Russ, James/P-3092-2014;
vilar, rocio/P-8480-2014; Moon, Chang-Seong/J-3619-2014; Scodellaro,
Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein,
Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014
OI Brucken, Jens Erik/0000-0001-6066-8756; ciocci, maria agnese
/0000-0003-0002-5462; Introzzi, Gianluca/0000-0002-1314-2580;
Piacentino, Giovanni/0000-0001-9884-2924; Marino,
Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov,
Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399;
Warburton, Andreas/0000-0002-2298-7315; maestro,
paolo/0000-0002-4193-1288; Chiarelli, Giorgio/0000-0001-9851-4816; Russ,
James/0000-0001-9856-9155; Moon, Chang-Seong/0000-0001-8229-7829;
Scodellaro, Luca/0000-0002-4974-8330; Punzi,
Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694;
Paulini, Manfred/0000-0002-6714-5787
FU U.S. Department of Energy; National Science Foundation; Italian Istituto
Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports,
Science and Technology of Japan; Natural Sciences and Engineering
Research Council of Canada; National Science Council of the Republic of
China; Swiss National Science Foundation; A. P. Sloan Foundation;
Bundesministerium fur Bildung und Forschung, Germany; Korean World Class
University Program; National Research Foundation of Korea; Royal
Society, UK; Russian Foundation for Basic Research; Ministerio de
Ciencia e Innovacion, Spain; Programa Consolider-Ingenio, Spain; Slovak
RD Agency; Academy of Finland; Australian Research Council (ARC);
Science and Technology Facilities Council, UK
FX We thank the Fermilab staff and the technical staffs of the
participating institutions for their vital contributions. This work was
supported by the U.S. Department of Energy and National Science
Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the
Ministry of Education, Culture, Sports, Science and Technology of Japan;
the Natural Sciences and Engineering Research Council of Canada; the
National Science Council of the Republic of China; the Swiss National
Science Foundation; the A. P. Sloan Foundation; the Bundesministerium
fur Bildung und Forschung, Germany; the Korean World Class University
Program, the National Research Foundation of Korea; the Science and
Technology Facilities Council and the Royal Society, UK; the Russian
Foundation for Basic Research; the Ministerio de Ciencia e Innovacion,
and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the
Academy of Finland; and the Australian Research Council (ARC).
NR 38
TC 10
Z9 10
U1 3
U2 20
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 2470-0010
EI 2470-0029
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 5
PY 2013
VL 88
IS 3
AR 032003
DI 10.1103/PhysRevD.88.032003
PG 13
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 196SU
UT WOS:000322797500005
ER
PT J
AU Yang, YG
Xu, MY
He, ZL
Guo, J
Sun, GP
Zhou, JZ
AF Yang, Yonggang
Xu, Meiying
He, Zhili
Guo, Jun
Sun, Guoping
Zhou, Jizhong
TI Microbial Electricity Generation Enhances Decabromodiphenyl Ether
(BDE-209) Degradation
SO PLOS ONE
LA English
DT Article
ID POLYBROMINATED DIPHENYL ETHERS; IN-SITU BIOREMEDIATION; FUNCTIONAL GENE
MICROARRAYS; ANAEROBIC DEGRADATION; FUEL-CELLS; REDUCTIVE DEBROMINATION;
CONTAMINATED SEDIMENTS; ELEVATED CO2; COMMUNITIES; GROUNDWATER
AB Due to environmental persistence and biotoxicity of polybrominated diphenyl ethers (PBDEs), it is urgent to develop potential technologies to remediate PBDEs. Introducing electrodes for microbial electricity generation to stimulate the anaerobic degradation of organic pollutants is highly promising for bioremediation. However, it is still not clear whether the degradation of PBDEs could be promoted by this strategy. In this study, we hypothesized that the degradation of PBDEs (e. g., BDE-209) would be enhanced under microbial electricity generation condition. The functional compositions and structures of microbial communities in closed-circuit microbial fuel cell (c-MFC) and open-circuit microbial fuel cell (o-MFC) systems for BDE-209 degradation were detected by a comprehensive functional gene array, GeoChip 4.0, and linked with PBDE degradations. The results indicated that distinctly different microbial community structures were formed between c-MFCs and o-MFCs, and that lower concentrations of BDE-209 and the resulting lower brominated PBDE products were detected in c-MFCs after 70-day performance. The diversity and abundance of a variety of functional genes in c-MFCs were significantly higher than those in o-MFCs. Most genes involved in chlorinated solvent reductive dechlorination, hydroxylation, methoxylation and aromatic hydrocarbon degradation were highly enriched in c-MFCs and significantly positively correlated with the removal of PBDEs. Various other microbial functional genes for carbon, nitrogen, phosphorus and sulfur cycling, as well as energy transformation process, were also significantly increased in c-MFCs. Together, these results suggest that PBDE degradation could be enhanced by introducing the electrodes for microbial electricity generation and by specifically stimulating microbial functional genes.
C1 [Yang, Yonggang; Xu, Meiying; Guo, Jun; Sun, Guoping] Guangdong Inst Microbiol, Guangdong Prov Key Lab Microbial Culture Collect, Guangzhou, Guangdong, Peoples R China.
[He, Zhili; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA.
[He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Bot & Microbiol, Norman, OK 73019 USA.
[Yang, Yonggang; Xu, Meiying; Guo, Jun; Sun, Guoping] South China Minist Prov Joint Dev, State Key Lab Appl Microbiol, Guangzhou, Guangdong, Peoples R China.
[Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
RP Xu, MY (reprint author), Guangdong Inst Microbiol, Guangdong Prov Key Lab Microbial Culture Collect, Guangzhou, Guangdong, Peoples R China.
EM xumy@gdim.cn
FU National Basic Research Program of China (973 Program) [2012CB22307];
Natural Science Foundation of Guangdong, China [9351007002000001];
National Natural Science Foundation [31200096]; National Postdoctoral
Foundation [2012M521578]; Postdoctoral Foundation of Guangdong Academy
of Sciences [20120001]; Natural Science Foundation of Guangdong Province
[S2011010004267]; Guangdong-Hongkong Technology Cooperation Funding
[2009A030902003]; Guangdong Province - Chinese Academy of Sciences
strategic cooperative project [2009B091300023, 2010B090301048];
International Cooperation Projects of Guangdong Province
[2011B050400005]; ENIGMA - Ecosystems and Networks Integrated with Genes
and Molecular Assemblies through the Office of Science, Office of
Biological and Environmental Research, the United States Department of
Energy [DE-AC02-05CH11231]
FX This research was supported by the National Basic Research Program of
China (973 Program) (2012CB22307), the Team Project of the Natural
Science Foundation of Guangdong, China (9351007002000001), the National
Natural Science Foundation (31200096), the National Postdoctoral
Foundation (2012M521578), the Postdoctoral Foundation of Guangdong
Academy of Sciences (20120001), the Natural Science Foundation of
Guangdong Province (S2011010004267), the Guangdong-Hongkong Technology
Cooperation Funding (2009A030902003), the Guangdong Province - Chinese
Academy of Sciences strategic cooperative project (2009B091300023,
2010B090301048), and the International Cooperation Projects of Guangdong
Province (2011B050400005). The development of the GeoChip and associated
computational pipelines used in this study was funded by ENIGMA -
Ecosystems and Networks Integrated with Genes and Molecular Assemblies
through the Office of Science, Office of Biological and Environmental
Research, the United States Department of Energy under Contract No.
DE-AC02-05CH11231. The funders had no role in study design, data
collection and analysis, decision to publish, or preparation of the
manuscript.
NR 33
TC 4
Z9 5
U1 11
U2 116
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1932-6203
J9 PLOS ONE
JI PLoS One
PD AUG 5
PY 2013
VL 8
IS 8
AR e70686
DI 10.1371/journal.pone.0070686
PG 10
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 218XC
UT WOS:000324465000119
PM 23940625
ER
PT J
AU Yeon, J
Smith, MD
Sefat, AS
Tran, TT
Halasyamani, PS
zur Loye, HC
AF Yeon, Jeongho
Smith, Mark D.
Sefat, Athena S.
Tran, T. Thao
Halasyamani, P. Shiv
zur Loye, Hans-Conrad
TI U3F12(H2O), a Noncentrosymmetric Uranium(IV) Fluoride Prepared via a
Convenient In Situ Route That Creates U4+ under Mild Hydrothermal
Conditions
SO INORGANIC CHEMISTRY
LA English
DT Article
ID MAGNETIC-PROPERTIES; STRUCTURE-PROPERTY; CRYSTAL-GROWTH; GERMANATE;
ZN2+; UF4
AB A new noncentrosymmetric U4+-containing fluoride, U3F12(H2O), has been synthesized via a mild hydrothermal route and its crystal structure determined by single-crystal X-ray diffraction. The material exhibits a complex three-dimensional structure that is based on [U8F33(H2O)(2))](9-) hexanuclear building units consisting of corner- and edge-shared UF8, UF9, and UOF7 polyhedra. Powder second-harmonic generation (SHG) measurements revealed that the SHG efficiency for U3F12(H2O) is comparable to that of alpha-SiO2. Magnetic susceptibility measurements indicated that the U4+(f(2))-containing material exhibits a singlet ground state at low temperature. IR and UV-vis reflectance spectra were obtained, and the thermal behavior was investigated by thermogravimetric analysis.
C1 [Yeon, Jeongho; Smith, Mark D.; zur Loye, Hans-Conrad] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA.
[Sefat, Athena S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
[Tran, T. Thao; Halasyamani, P. Shiv] Univ Houston, Dept Chem, Houston, TX 77204 USA.
RP zur Loye, HC (reprint author), Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA.
EM zurloye@mailbox.sc.edu
RI Halasyamani, P. Shiv/A-8620-2009; Halasyamani, Shiv/J-3438-2014; Sefat,
Athena/R-5457-2016;
OI Halasyamani, Shiv/0000-0003-1787-1040; Sefat,
Athena/0000-0002-5596-3504; zur Loye, Hans-Conrad/0000-0001-7351-9098
FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of
Materials Sciences and Engineering; DOE [DE-SC0008664]; Welch Foundation
[E-1457]
FX Research supported by the U.S. Department of Energy, Office of Basic
Energy Sciences, Division of Materials Sciences and Engineering. J.Y.,
M.D.S., and H.-C.z.L. acknowledge DOE Award DE-SC0008664 for support.
P.S.H. and T.T.T., who performed the SHG measurements, thank the Welch
Foundation for support (Grant E-1457).
NR 30
TC 16
Z9 16
U1 1
U2 10
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
EI 1520-510X
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 8303
EP 8305
DI 10.1021/ic401412t
PG 3
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300007
PM 23834284
ER
PT J
AU Barry, BM
Dickie, DA
Murphy, LJ
Clyburne, JAC
Kemp, RA
AF Barry, Brian M.
Dickie, Diane A.
Murphy, Luke J.
Clyburne, Jason A. C.
Kemp, Richard A.
TI NH/PH Isomerization and a Lewis Pair for Carbon Dioxide Capture
SO INORGANIC CHEMISTRY
LA English
DT Article
ID STRUCTURAL-CHARACTERIZATION; N BONDS; CO2; COMPLEXES; CHEMISTRY;
INSERTION; ACTIVATION; REACTIVITY; BORANES; MAGNESIUM
AB Bis(di-i-propylphosphino)amine 1 reacts with B(C6F5)(3) to form an adduct with concomitant N/P H-isomerization. This species reacts smoothly with carbon dioxide. An attempt to prepare an anionic derivative resulted in the formation of a novel heterocycle derived from the PNP ligand and B(C6F5)(3).
C1 [Barry, Brian M.; Dickie, Diane A.; Kemp, Richard A.] Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA.
[Murphy, Luke J.; Clyburne, Jason A. C.] St Marys Univ, Dept Chem, Atlantic Ctr Green Chem, Halifax, NS B3H 3C3, Canada.
[Kemp, Richard A.] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA.
RP Clyburne, JAC (reprint author), St Marys Univ, Dept Chem, Atlantic Ctr Green Chem, Halifax, NS B3H 3C3, Canada.
EM jason.clyburne@smu.ca; rakemp@unm.edu
RI Dickie, Diane/B-1647-2010
OI Dickie, Diane/0000-0003-0939-3309
FU NSF [CHE09-11110, CHE12-13529, CHE08-40523, CHE09-46690]; Laboratory
Directed Research and Development program at Sandia National
Laboratories [LDRD 151300]; NSERC of Canada; Canada Research Chairs
Program; CFI; NSRIT; SMU; NSF CRIF:MU award [CHE04-43580]; United States
Department of Energy [DE-AC04-94AL85000]
FX This work was financially supported by the NSF (Grants CHE09-11110 and
CHE12-13529), the Laboratory Directed Research and Development program
at Sandia National Laboratories (LDRD 151300), and NSERC of Canada.
J.A.C.C. acknowledges support from the Canada Research Chairs Program,
CFI, and NSRIT. L.J.M. thanks SMU for a graduate fellowship. The Bruker
X-ray diffractometer was purchased via a NSF CRIF:MU award to UNM
(CHE04-43580), and the NMR spectrometers were upgraded via grants from
the NSF (CHE08-40523 and CHE09-46690). High resolution mass spectrometry
data were obtained by UNM Mass Spectrometry Facility. Sandia is a
multiprogram laboratory operated by Sandia Corporation, a Lockheed
Martin Company, for the United States Department of Energy under
Contract No. DE-AC04-94AL85000.
NR 35
TC 15
Z9 15
U1 1
U2 43
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 8312
EP 8314
DI 10.1021/ic401498r
PG 3
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300010
PM 23879626
ER
PT J
AU Reinert, AA
Payne, C
Wang, LM
Ciston, J
Zhu, YM
Khalifah, PG
AF Reinert, Alexandra A.
Payne, Candace
Wang, Limin
Ciston, James
Zhu, Yimei
Khalifah, Peter G.
TI Synthesis and Characterization of Visible Light Absorbing
(GaN)(1-x)(ZnO)(x) Semiconductor Nanorods
SO INORGANIC CHEMISTRY
LA English
DT Article
ID (GA1-XZNX)(N1-XOX) SOLID-SOLUTION; HOMOLOGOUS COMPOUNDS;
HYDROGEN-PRODUCTION; PHOTOCATALYTIC ACTIVITY; INFRARED ABSORPTION;
WATER; ZNO; GA2O3(ZNO)(M); GAN; IRRADIATION
AB Although the (GaN)(1-x)(ZnO)(x) solid solution is one of the most effective systems for driving overall solar water splitting with visible light, its quantum yield for overall water splitting using visible light photons has not yet reached ten percent. Understanding and controlling the nanoscale morphology of this system may allow its overall conversion efficiency to be raised to technologically relevant levels. We describe the use a Ga2O3(ZnO)(16) precursor phase in the synthesis of this phase which naturally results in the production of arrays of nanorods with favorable diameters (similar to 100 nm) and band gaps (similar to 2.5 eV). Substantial absorption within the band gap is observed, part of which is found to follow the E-3 scaling characteristic of free carriers scattered by ionized impurity sites. Compositional analysis suggests that a substantial quantity of cation vacancies (similar to 3%) may be present in some samples. The typical nanorod growth direction and dominant {10 (1) over bar1} facet for powders in this system have been identified through electron microscopy methods, leading to the conclusion that polarity may play an important role in the high photoactivity of this family of wurtzite semiconductors.
C1 [Reinert, Alexandra A.; Payne, Candace; Khalifah, Peter G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
[Wang, Limin; Khalifah, Peter G.] Brookhaven Natl Labs, Dept Chem, Upton, NY 11973 USA.
[Ciston, James] Brookhaven Natl Labs, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Zhu, Yimei] Brookhaven Natl Labs, CMPMSD, Upton, NY 11973 USA.
RP Khalifah, PG (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
EM Limin.Wang@ge.com; JCiston@lbl.gov; kpete@bnl.gov
FU U.S. Department of Energy [DEAC02-98CH10886]; Department of Energy via a
Hydrogen Fuel Initiative; Scientific User Facilities Division, Office of
Basic Energy Sciences, U.S. Department of Energy; DOE
[DE-AC02-98CH10886]
FX This work was in part carried out at BNL under Contract DEAC02-98CH10886
with the U.S. Department of Energy. Funding was provided by the
Department of Energy via a Hydrogen Fuel Initiative grant through the
Solar Photochemistry program (P.K.); interactions with HFI collaborators
E. Fujita, J. Muckerman, and J. Rodriguez are gratefully acknowledged.
We also acknowledge M. Dawber and P. Allen at Stony Brook University for
many insightful discussions on the physics of polar materials. Portions
of this research were carried out at the Oak Ridge National Laboratory's
Spallation Neutron Source sponsored by the Scientific User Facilities
Division, Office of Basic Energy Sciences, U.S. Department of Energy.
Optical data and electron microscopy data were collected at Brookhaven
National Laboratory's Center for Functional Nanomaterials supported by
the DOE under grant DE-AC02-98CH10886.
NR 49
TC 12
Z9 12
U1 4
U2 101
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
EI 1520-510X
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 8389
EP 8398
DI 10.1021/ic400011n
PG 10
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300019
PM 23829594
ER
PT J
AU Cabana, J
Chernova, NA
Xiao, J
Roppolo, M
Aldi, KA
Whittingham, MS
Grey, CP
AF Cabana, Jordi
Chernova, Natasha A.
Xiao, Jie
Roppolo, Megan
Aldi, Kellie A.
Whittingham, M. Stanley
Grey, Clare P.
TI Study of the Transition Metal Ordering in Layered NaxNix/2Mn1-x/2O2 (2/3
<= x <= 1) and Consequences of Na/Li Exchange
SO INORGANIC CHEMISTRY
LA English
DT Article
ID RECHARGEABLE LITHIUM BATTERIES; POSITIVE ELECTRODE MATERIAL; PAIR
DISTRIBUTION FUNCTION; CATHODE MATERIAL; O2 STRUCTURE; RAY-DIFFRACTION;
ION-EXCHANGE; NMR-SPECTROSCOPY; MANGANESE OXIDES; LOCAL-STRUCTURE
AB A series of layered oxides within the NaxNix/2Mn1-x/2O2 (2/3 <= x <= 1) system were synthesized by classical solid-state methodologies. A study of their long and short-range structure was undertaken by combining X-ray diffraction and NMR spectroscopy. A transition from P2 to O-3 stacking was observed at x > 0.8 when samples were made at 900 degrees C, which was accompanied by disordering of ions in the transition metal layer. The magnetic properties of the materials were consistent with this picture of ordering, with all samples showing antiferromagnetic character. At x = 2/3, competition between a P2 and a P3 structure, with different degrees of transition metal ordering, was found depending on the synthesis temperature. Na/Li exchange led to structures with octahedral or tetrahedral coordination of the alkali metal, and Li/Ni crystallographic exchange, in the resulting O-3 phases. The transition from alkali metal prismatic coordination to octahedral/tetrahedral coordination involves [TMO6](infinity) layer shearing that induces some structural disorder through the formation of stacking faults.
C1 [Cabana, Jordi; Aldi, Kellie A.; Grey, Clare P.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
[Cabana, Jordi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
[Cabana, Jordi] Univ Illinois, Dept Chem, Chicago, IL 60607 USA.
[Chernova, Natasha A.; Xiao, Jie; Roppolo, Megan; Whittingham, M. Stanley] SUNY Binghamton, Inst Mat Res, Binghamton, NY 13902 USA.
RP Cabana, J (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
EM jcabana@uic.edu; cpg27@cam.ac.uk
RI Cabana, Jordi/G-6548-2012
OI Cabana, Jordi/0000-0002-2353-5986
FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office
of Vehicle Technologies of the U.S. Department of Energy, Batteries for
Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231];
National Science Foundation [0549370]; [6807148]; [6517749]
FX This work was supported by the Assistant Secretary for Energy Efficiency
and Renewable Energy, Office of Vehicle Technologies of the U.S.
Department of Energy, under Contract DE-AC02-05CH11231, as part of the
Batteries for Advanced Transportation Technologies (BATT) Program. The
program is managed by LBNL for the Department of Energy. Binghamton and
Stony Brook were supported under Subcontracts 6807148 and 6517749,
respectively. J.C. is indebted to Generalitat de Catalunya (Spain) for a
Beatriu de Pinos fellowship covering his work at Stony Brook. K.A.A.
thanks the National Science Foundation for support via the Integrated
Graduate Education and Research Training fellowship (Award No. 0549370).
NR 48
TC 22
Z9 24
U1 5
U2 100
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 8540
EP 8550
DI 10.1021/ic400579w
PG 11
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300035
PM 23909957
ER
PT J
AU Wang, SM
Zhang, JZ
Zhang, Y
Alvarado, A
Attapattu, J
He, DW
Wang, LP
Chen, CF
Zhao, YS
AF Wang, Shanmin
Zhang, Jianzhong
Zhang, Yi
Alvarado, Andrew
Attapattu, Jeevake
He, Duanwei
Wang, Liping
Chen, Changfeng
Zhao, Yusheng
TI Phase-Transition Induced Elastic Softening and Band Gap Transition in
Semiconducting PbS at High Pressure
SO INORGANIC CHEMISTRY
LA English
DT Article
ID LEAD CHALCOGENIDES; THERMAL-EXPANSION; PBTE; DIFFRACTION; GPA;
POLYMORPHISM; TEMPERATURE; NAH
AB We have investigated the crystal structure and phase stability, elastic incompressibility, and electronic properties of PbS based on high-pressure neutron diffraction, in-situ electrical resistance measurements, and first-principles calculations. The refinements show that the orthorhombic phase is structurally isotypic with indium iodide (In adopting a Cmcm structure (B33). The cubic-to-orthorhombic transition occurs at,similar to 2.1(1) GPa with a 3.8% volume collapse and a positive Clausius-Clapeyron slope. Phase-transition induced elastic softening is also observed, which is presumably attributed to the enhanced metallic bonding in the B33 phase. On the basis of band structure simulations, the cubic and orthorhombic phases are typical of direct and indirect semiconductors with band gaps of 0.47(1) and 1.04(1) eV, respectively, which supports electrical resistivity measurements of an abrupt jump at the structural transition. On the basis of the resolved structure for B33, the phase transition paths for B1 -> B33 -> B2 involve translation of a trigonal prism in B1 and motion of the next-nearest neighbor Pb atom into (SPb7) coordination and subsequent lattice distortion in the B33 phase.
C1 [Wang, Shanmin; Zhang, Jianzhong; Zhao, Yusheng] Los Alamos Natl Lab, LANSCE Div, Los Alamos, NM 87545 USA.
[Wang, Shanmin; He, Duanwei] Sichuan Univ, Inst Atom & Mol Phys, Chengdu 610065, Peoples R China.
[Wang, Shanmin; Zhang, Yi; Alvarado, Andrew; Attapattu, Jeevake; Wang, Liping; Chen, Changfeng; Zhao, Yusheng] Univ Nevada, HiPSEC, Las Vegas, NV 89154 USA.
[Wang, Shanmin; Zhang, Yi; Alvarado, Andrew; Attapattu, Jeevake; Wang, Liping; Chen, Changfeng; Zhao, Yusheng] Univ Nevada, Dept Phys, Las Vegas, NV 89154 USA.
RP He, DW (reprint author), Sichuan Univ, Inst Atom & Mol Phys, Chengdu 610065, Peoples R China.
EM DuanweiHe@scu.edu.cn; Yusheng.Zhao@unlv.edu
RI Zhang, Yi/C-9291-2011;
OI Zhang, Jianzhong/0000-0001-5508-1782
FU U.S. Department of Energy's Office of Basic Energy Sciences; UNLV High
Pressure Science and Engineering Center (HiPSEC); DOE NNSA Center of
Excellence [DE-FC52-06NA27684]; UNLV; China 973 Program [2011CB808205];
National Natural Science Foundation of China [11027405]
FX This work has partly benefited from the use of the Lujan Neutron
Scattering Center at Los Alamos Neutron Science Center, which is funded
by the U.S. Department of Energy's Office of Basic Energy Sciences. This
work is also supported by UNLV High Pressure Science and Engineering
Center (HiPSEC), which is a DOE NNSA Center of Excellence operated under
Cooperative Agreement DE-FC52-06NA27684, and UNLV start-up funding to
Y.Z. We thank support from the China 973 Program (Grant 2011CB808205),
and the National Natural Science Foundation of China (Grant 11027405).
We thank X. Zhou for the electrical resistance measurements.
NR 49
TC 11
Z9 11
U1 5
U2 52
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 8638
EP 8643
DI 10.1021/ic400801s
PG 6
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300045
PM 23909959
ER
PT J
AU Deblonde, GJP
Sturzbecher-Hoehne, M
Abergel, RJ
AF Deblonde, Gauthier J-P.
Sturzbecher-Hoehne, Manuel
Abergel, Rebecca J.
TI Solution Thermodynamic Stability of Complexes Formed with the
Octadentate Hydroxypyridinonate Ligand 3,4,3-LI(1,2-HOPO): A Critical
Feature for Efficient Chelation of Lanthanide(IV) and Actinide(IV) Ions
SO INORGANIC CHEMISTRY
LA English
DT Article
ID NITRILOTRIACETIC ACID; SEQUESTERING AGENTS; TECHNICAL REPORT;
DECORPORATION; 5-LIO(ME-3,2-HOPO); EQUILIBRIA; PLUTONIUM; CONSTANTS;
THORIUM; PROGRAM
AB The solution thermodynamics of water-soluble complexes formed between Ce(III), Ce(IV), Th(IV) and the octadentate chelating agent 3,4,3-LI(1,2-HOPO) were investigated. Several techniques including spectrofluorirnetric and automated spectrophotometric titrations were used to overcome the slow spontaneous oxidation of Ce(III) complexes yielding to stability constants of log beta(110) = 17.4 +/- 0.5, log beta(11-1) = 8.3 +/- 0.4 and log beta(111)= 21.2 +/- 0.4 for [Ce(III)(3,4,3-LI(1,2-HOPO))](-), [Ce(III)(3,4,3-LI(1,2-HOPO)(OH)(2-), and [Ce-(III)(3,4,3-LI(1,2-HOPO)H), respectively. Using the spectral properties of the hydrowyridinonate chelator in ligand competition titrations against nitrilotriacetic acid, the stability constant log beta(110) = 41.5 0.5 was determined for [Ce(IV)(3,4,3-LI(1,2-HOPO)]. Finally, the extraordinarily stable complex [Ce(IV)(3,4,3-LI(1,2-HOPO))] was used in Th(IV) competition titrations, resulting in a stability constant of log Am = 40.1 0.5 for [Th(IV)3,4,3-LI(1,2-HOPO))). These experimental values are in excellent agreement with previous estimates, they are discussed with respect to the ionic radius and oxidation state of each cationic metal, and allow predictions on the stability of other actinide complexes including ([Ce(IV)(3,4,3-LI(1,2-HOPO], and [Pu(IV)(3,4,3-LI(1,2-HOPO))], [Np(IV)(3,4,3-LI(1,2-HOPO] and [Pu(IV)(3,4,3-LI(1,2-HOPO]. Comparisons with the standard ligand diethylenetriamine pentaacetic acid (DTPA) provide a thermodynamic basis for the observed significantly higher efficacy of 3,4,3-LI(1,2-HOPO) as an in vivo actinide ciecorporation agent
C1 [Deblonde, Gauthier J-P.; Sturzbecher-Hoehne, Manuel; Abergel, Rebecca J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Glenn T Seaborg Ctr, Div Chem Sci, Berkeley, CA 94720 USA.
RP Abergel, RJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Glenn T Seaborg Ctr, Div Chem Sci, Berkeley, CA 94720 USA.
EM rjabergel@lbl.gov
RI Deblonde, Gauthier/O-3881-2014
OI Deblonde, Gauthier/0000-0002-0825-8714
FU National Institutes of Health (National Institute of Allergy and
Infectious Diseases) [RAI087604Z]; U.S. Department of Energy
[DE-ACO205CH11231]
FX We thank Prof. Kenneth N. Raymond for helpful discussions, and Tiffany
Pham for assistance with the cyclic voltammetry experimental setup. This
research was supported by the National Institutes of Health (National
Institute of Allergy and Infectious Diseases, RAI087604Z) through the
U.S. Department of Energy under Contract No. DE-ACO205CH11231.
NR 24
TC 14
Z9 14
U1 2
U2 54
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 8805
EP 8811
DI 10.1021/ic4010246
PG 7
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300064
PM 23855806
ER
PT J
AU Badiei, YM
Polyansky, DE
Muckerman, JT
Szalda, DJ
Haberdar, R
Zong, RF
Thummel, RP
Fujita, E
AF Badiei, Yosra M.
Polyansky, Dmitry E.
Muckerman, James T.
Szalda, David J.
Haberdar, Rubabe
Zong, Ruifa
Thummel, Randolph P.
Fujita, Etsuko
TI Water Oxidation with Mononuclear Ruthenium(II) Polypyridine Complexes
Involving a Direct Ru-IV=O Pathway in Neutral and Alkaline Media
SO INORGANIC CHEMISTRY
LA English
DT Article
ID COUPLED ELECTRON-TRANSFER; PHOTOSYSTEM-II; SINGLE-SITE; REDOX
PROPERTIES; PROTON-TRANSFER; CATALYSTS; LIGANDS
AB The catalytic water oxidation mechanism proposed for many single-site ruthenium complexes proceeds via the nucleophilic attack of a water molecule on the Ru-V=O species. In contrast, Ru(II) complexes containing 4-t-buty1-2,6-di- 1',8'-(naphthyrid-2'-y1)-pyridine (and its bisbenzo-derivafive), an equatorial water, and two axial 4-picolines follow the thermodynamically more favorable "direct pathway via [Ru-IV=O](2+), which avoids the higher oxidation state [Ru-V=O](3+) in neutral and basic media. Our experimental and theoretical results that focus on the pH dependent onset catalytic potentials indicative of a PCET driven low energy pathway for the formation of products with an O-O bond (such as [Ru-III-OOH](2+) and [Ru-IV-OO](2+) at an applied potential below the Ru-V=O/Ru-IV=O couple clearly support such a mechanism. However, in the cases of [Ru(tpy)(bpy)(OH2))(2+) and [Ru(tpy)(bpm)(OH2))(2+), the formation of the Ru-V=O species appears to be required before O-O bond formation. The complexes under discussion provide a unique functional model for water oxidation that proceeds by four consecutive PCET steps in neutral and alkaline media.
C1 [Badiei, Yosra M.; Polyansky, Dmitry E.; Muckerman, James T.; Fujita, Etsuko] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Szalda, David J.] CUNY Bernard M Baruch Coll, Dept Nat Sci, New York, NY 10010 USA.
[Haberdar, Rubabe; Zong, Ruifa; Thummel, Randolph P.] Univ Houston, Dept Chem, Houston, TX 77204 USA.
RP Polyansky, DE (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM dmitriyp@bnl.gov; fujita@bnl.gov
RI Polyansky, Dmitry/C-1993-2009
OI Polyansky, Dmitry/0000-0002-0824-2296
FU Brookhaven National Laboratory (BNL) [DE-AC02-98CH10886]; U.S.
Department of Energy [DE-FG0207-ER15888]; Division of Chemical Sciences,
Geosciences, & Biosciences, Office of Basic Energy Sciences; U.S.
Department of Energy for funding under the BES Hydrogen Fuel Initiative;
Robert A. Welch Foundation [E-621]
FX We thank Natawutt Kaveevivitchai for TON measurements by Method 1. The
work at Brookhaven National Laboratory (BNL) is funded under contract
DE-AC02-98CH10886 and the work at Houston is funded under contract
DE-FG0207-ER15888 with the U.S. Department of Energy and supported by
its Division of Chemical Sciences, Geosciences, & Biosciences, Office of
Basic Energy Sciences. The BNL authors also thank the U.S. Department of
Energy for funding under the BES Hydrogen Fuel Initiative. R.H., R.Z.,
and R.P.T. also thank the Robert A. Welch Foundation (E-621).
NR 45
TC 36
Z9 36
U1 5
U2 64
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
EI 1520-510X
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 8845
EP 8850
DI 10.1021/ic401023w
PG 6
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300068
PM 23837911
ER
PT J
AU Jin, GB
Hu, YJ
Bellott, B
Skanthakumar, S
Haire, RG
Soderholm, L
Ibers, JA
AF Jin, Geng Bang
Hu, Yung-Jin
Bellott, Brian
Skanthakumar, S.
Haire, Richard G.
Soderholm, L.
Ibers, James A.
TI Reinvestigation of Np2Se5: A Clear Divergence from Th2S5 and Th2Se5 in
Chalcogen-Chalcogen and Metal-Chalcogen Interactions
SO INORGANIC CHEMISTRY
LA English
DT Article
ID X-RAY-ABSORPTION; CHARGE-DENSITY-WAVE; CRYSTAL-STRUCTURE;
ELECTRONIC-STRUCTURE; OPTICAL-PROPERTIES; URANIUM CHALCOGENIDES;
FINE-STRUCTURE; NEPTUNIUM; SE; ACTINIDE
AB Single crystals of Np2Se5 have been prepared through the reactions of Np and Se at 1223 K in an Sb2Se3 flux. The structure of Np2Se5, which has been characterized by single-crystal X-ray diffraction methods, crystallizes in the tetragonal space group P4(2)/nmc. The crystallographic unit cell includes one unique Np and two Se positions. Se(1) atoms form one-dimensional infinite chains along the a and b axes with alternating intermediate Se-Se distances of 2.6489 (8) and 2.7999 (8) angstrom, whereas Se(2) is a discrete Se2- anion. Each Np is coordinated to 10 Se atoms and every NpSe10 polyhedron shares faces, edges, or vertices with 14 other identical metal polyhedra to form a complex three-dimensional structure. Np L-III-edge X-ray Absorption Near Edge Structure ()CANES) measurements show a clear shift in edge position to higher energies for Np2Se5 compared to Np3Se5 (Np23+Np4+Se52-). Magnetic susceptibility measurements indicate that Np2Se5 undergoes a ferromagnetic type ordering below 18(1) K. Above the transition temperature, Np2Se5 behaves as a paramagnet with an effective moment of 1.98(5) mu(B)/Np, given by a best fit of susceptibilities to a modified Curie-Weiss law over the temperature range 50-320 K.
C1 [Jin, Geng Bang; Hu, Yung-Jin; Skanthakumar, S.; Soderholm, L.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Jin, Geng Bang; Bellott, Brian; Ibers, James A.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
[Haire, Richard G.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
RP Jin, GB (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM gjin@anl.gov
FU U.S. Department of Energy, Basic Energy Sciences, Chemical Sciences,
Biosciences [DEAC02-06CH11357]; U.S. DOE, OBES, Materials Sciences
[DEAC02-06CH11357]; U.S. Department of Energy, Basic Energy Sciences,
Chemical Sciences, Biosciences, and Geosciences Division and Division of
Materials Sciences and Engineering [ER-15522]
FX The research at Argonne National Laboratory was supported by the U.S.
Department of Energy, Basic Energy Sciences, Chemical Sciences,
Biosciences, under contract DEAC02-06CH11357. X-ray absorption
spectroscopy data were obtained at the Advanced Photon Source, which is
supported by the U.S. DOE, OBES, Materials Sciences under the same
contract number. The work at Northwestern University was supported by
the U.S. Department of Energy, Basic Energy Sciences, Chemical Sciences,
Biosciences, and Geosciences Division and Division of Materials Sciences
and Engineering Grant ER-15522.
NR 71
TC 0
Z9 0
U1 1
U2 18
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
EI 1520-510X
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 9111
EP 9118
DI 10.1021/ic401384t
PG 8
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300094
PM 23883193
ER
PT J
AU Guo, YR
Wu, Q
Odoh, SO
Schreckenbach, G
Pan, QJ
AF Guo, Yuan-Ru
Wu, Qian
Odoh, Samuel O.
Schreckenbach, Georg
Pan, Qing-Jiang
TI Theoretical Study of Structural, Spectroscopic and Reaction Properties
of trans-bis(imido) Uranium(VI) Complexes
SO INORGANIC CHEMISTRY
LA English
DT Article
ID DENSITY-FUNCTIONAL THEORY; ORDER REGULAR APPROXIMATION; CATION-CATION
INTERACTIONS; RAY CRYSTAL-STRUCTURE; URANYL-ION; CARBENE COMPLEXES;
ORGANOMETALLIC COMPLEX; ELECTRONIC-STRUCTURE; MACROCYCLIC LIGANDS; IMIDO
ANALOGS
AB To advance the understanding of the chemical behavior of actinides, a series of trans-bis(imido) uranium(VI) complexes, U(NR)(2)(THF)(2)(cis-I-2) (2R; R = H, Me, Bu-t, Cy, and Ph), U(NR)(2)(THF)(3)(trans-I-2) (3R; R = H, Me, Bu-t Cy, and Ph) and U((NBu)-Bu-t)(2)(THF)(3)(cis-I-2) (3(t)Bu'), were investigated using relativistic density functional theory. The axial U=N bonds in these complexes have partial triple bonding character. The calculated bond lengths, bond orders, and stretching vibrational frequencies reveal that the U=N bonds of the bis-imido complexes can be tuned by the variation of their axial substituents. This has been evidenced by the analysis of electronic structures. 2H, for instance, was calculated to show iodine based high lying occupied orbitals and U(f)-type low-lying unoccupied orbitals. Its U=N bonding orbitals, formed by U(f) and N(p), occur in a region of the relatively low energy. Upon varying the axial substituent from H to Bu-t and Ph, the U=N bonding orbitals of 2(t)Bu and 2Ph are greatly destabilized. We further compared the U=E (E = N and 0) bonds of 2H with 3H and their uranyl analogues, to address effects of the equatorial tetrahydrofuran (THF) ligand and the E group. It is found that the U=N bonds are slightly weaker than the U=O bonds of their uranyl analogues. This is in line with the finding that cis-UNR2 isomers, although energetically unfavorable, are more accessible than cis-UO2 would be It is also evident that 2H and 3H display lower U=(NH) stretching vibrations at 740 cm(-1) than the U=O at 820 cm(-1) of uranyl complexes. With the inclusion of both solvation and spin-orbit coupling, the free energies of the formation reactions of the bis-imido uranium complexes were calculated. The formation of the experimentally synthesized 3Me, 3Ph, and 2tBu are found to be thermodynamically favorable. Finally, the absorption bands previously obtained from experimental studies were well reproduced by time dependent density functional theory calculations.
C1 [Wu, Qian; Pan, Qing-Jiang] Heilongjiang Univ, Key Lab Funct Inorgan Mat Chem, Educ Minist, Sch Chem & Mat Sci, Harbin 150080, Peoples R China.
[Guo, Yuan-Ru] Northeast Forestry Univ, Coll Mat Sci & Engn, Educ Minist, Key Lab Biobased Mat Sci & Technol, Harbin 150040, Peoples R China.
[Odoh, Samuel O.; Schreckenbach, Georg] Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada.
[Odoh, Samuel O.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
RP Pan, QJ (reprint author), Heilongjiang Univ, Key Lab Funct Inorgan Mat Chem, Educ Minist, Sch Chem & Mat Sci, Harbin 150080, Peoples R China.
EM panqjitc@163.com
FU Fundamental Research Funds for the Central Universities [DL11CB07];
National Natural Science Foundation of China [21273063, 30901136];
Program for New Century Excellent Talents in University [NCET-11-0958];
Key Project of Chinese Ministry of Education [211048]; Natural Sciences
and Engineering Research Council of Canada (NSERC)
FX Q.-J.P. is grateful to Dr. Dimitri Laikov for providing the Priroda
code. This work is supported by Fundamental Research Funds for the
Central Universities (DL11CB07), National Natural Science Foundation of
China (21273063, 30901136), Program for New Century Excellent Talents in
University (NCET-11-0958), and Key Project of Chinese Ministry of
Education (211048). Foundations for the Returned Overseas Chinese
Scholars of Heilongjiang Province (LC2011C22) and State Education
Ministry are greatly acknowledged. G.S. acknowledges funding from the
Natural Sciences and Engineering Research Council of Canada (NSERC).
NR 99
TC 6
Z9 6
U1 2
U2 50
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 5
PY 2013
VL 52
IS 15
BP 9143
EP 9152
DI 10.1021/ic401440w
PG 10
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 197PO
UT WOS:000322863300097
PM 23834342
ER
PT J
AU Yuan, SW
Shui, JL
Grabstanowicz, L
Chen, C
Commet, S
Reprogle, B
Xu, T
Yu, LP
Liu, DJ
AF Yuan, Shengwen
Shui, Jiang-Lan
Grabstanowicz, Lauren
Chen, Chen
Commet, Sean
Reprogle, Briana
Xu, Tao
Yu, Luping
Liu, Di-Jia
TI A Highly Active and Support-Free Oxygen Reduction Catalyst Prepared from
Ultrahigh-Surface-Area Porous Polyporphyrin
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE electrocatalysis; fuel cells; oxygen reduction catalysts; polyporphyrin;
porous organic polymers
ID PEM FUEL-CELLS; CATHODE CATALYST; METAL ELECTROCATALYSTS; HYDROGEN
STORAGE; CARBON NANOTUBES; IRON; PRECURSOR; POLYANILINE; PYROLYSIS;
DIOXYGEN
C1 [Yuan, Shengwen; Shui, Jiang-Lan; Chen, Chen; Commet, Sean; Reprogle, Briana; Liu, Di-Jia] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Grabstanowicz, Lauren; Xu, Tao] No Illinois Univ, Dept Chem & Biochem, De Kalb, IL 60115 USA.
[Yu, Luping] Univ Chicago, Dept Chem, Chicago, IL 60637 USA.
RP Yu, LP (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA.
EM djliu@anl.gov
FU U.S. Department of Energy's the Office of Science; Office of Energy
Efficiency and Renewable Energy Fuel Cell Technologies program
FX This work was supported by the U.S. Department of Energy's the Office of
Science and the Office of Energy Efficiency and Renewable Energy Fuel
Cell Technologies program. The authors are grateful to Dr. Jiangbin Xia,
Dr. Jun Lu, Dr. Deborah J. Myers, and Alex Mason for their support with
experiments.
NR 46
TC 60
Z9 61
U1 14
U2 181
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PD AUG 5
PY 2013
VL 52
IS 32
BP 8349
EP 8353
DI 10.1002/anie.201302924
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA 194KK
UT WOS:000322631600032
PM 23804418
ER
PT J
AU Fernandez-Martinez, A
Kalkan, B
Clark, SM
Waychunas, GA
AF Fernandez-Martinez, Alejandro
Kalkan, Bora
Clark, Simon M.
Waychunas, Glenn A.
TI Pressure-Induced Polyamorphism and Formation of 'Aragonitic' Amorphous
Calcium Carbonate
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE amorphous materials; calcium carbonate; phase transitions; Raman
spectroscopy; X-ray diffraction
ID BIOMPHALARIA-GLABRATA; DOLOMITE FORMATION; MAGNESIAN CALCITE;
PHASE-TRANSITIONS; BIOMINERALIZATION; CRYSTALLIZATION; TRANSFORMATION;
REFINEMENTS; TEMPERATURE; GROWTH
C1 [Fernandez-Martinez, Alejandro] CNRS, Inst Sci Terre, F-38041 Grenoble 9, France.
[Fernandez-Martinez, Alejandro] Univ Grenoble 1, F-38041 Grenoble 9, France.
[Kalkan, Bora; Clark, Simon M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Clark, Simon M.] Macquarie Univ, Dept Earth & Planetary Sci, N Ryde, NSW 2109, Australia.
[Fernandez-Martinez, Alejandro; Waychunas, Glenn A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
RP Fernandez-Martinez, A (reprint author), CNRS, Inst Sci Terre, BP 53X, F-38041 Grenoble 9, France.
EM Alex.Fernandez-Martinez@ujf-grenoble.fr
RI Fernandez-Martinez, Alejandro/B-4042-2010; Clark, Simon/B-2041-2013
OI Fernandez-Martinez, Alejandro/0000-0001-5073-9629; Clark,
Simon/0000-0002-7488-3438
FU Office of Science, Office of Basic Energy Sciences, of the U.S.
Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S.
Department of Energy [DE-AC02-05CH11231]; Center for Nanoscale Control
of Geologic CO2, an Energy Frontier Research Center; U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences
[DE-AC02-05CH11231]; IAEA [TUR/10006]
FX The Advanced Light Source is supported by the Director, Office of
Science, Office of Basic Energy Sciences, of the U.S. Department of
Energy under Contract No. DE-AC02-05CH11231. This research used
resources of the National Energy Research Scientific Computing Center,
which is supported by the Office of Science of the U.S. Department of
Energy under Contract No. DE-AC02-05CH11231. A.F.-M. and G. A. W. were
partially supported as part of the Center for Nanoscale Control of
Geologic CO2, an Energy Frontier Research Center funded by
the U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences under Award Number DE-AC02-05CH11231. B. K. acknowledges
support from IAEA, fellowship Code No.: TUR/10006. We thank Adam F.
Wallace for fruitful discussions.
NR 36
TC 21
Z9 21
U1 3
U2 81
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
EI 1521-3773
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PD AUG 5
PY 2013
VL 52
IS 32
BP 8354
EP 8357
DI 10.1002/anie.201302974
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA 194KK
UT WOS:000322631600033
PM 23818278
ER
PT J
AU Lohn, AJ
Stevens, JE
Mickel, PR
Marinella, MJ
AF Lohn, Andrew J.
Stevens, James E.
Mickel, Patrick R.
Marinella, Matthew J.
TI Optimizing TaOx memristor performance and consistency within the
reactive sputtering "forbidden region"
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID RRAM
AB Standard deposition processes for depositing ReRAM oxides utilize mass flow of reactive gas to control stoichiometry and have difficulty depositing a precisely defined sub-stoichiometry within a "forbidden region" where film properties are discontinuous with mass flow. We show that by maintaining partial pressure within this discontinuous "forbidden region," instead of by maintaining mass flow, we can optimize tantalum oxide device properties and reduce or eliminate the electroforming step. We also show that defining the partial pressure set point as a fraction of the "forbidden region" instead of as an absolute value can be used to improve wafer-to-wafer consistency with minimal recalibration efforts. (C) 2013 AIP Publishing LLC.
C1 [Lohn, Andrew J.; Stevens, James E.; Mickel, Patrick R.; Marinella, Matthew J.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Lohn, AJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
FU U.S. Department of Energy's National Nuclear Security Administration
[DE-AC0494AL85000]
FX Sandia National Laboratories is a multi-program laboratory managed and
operated by Sandia Corporation, a wholly owned subsidiary of Lockheed
Martin Corporation, for the U.S. Department of Energy's National Nuclear
Security Administration under Contract No. DE-AC0494AL85000.
NR 15
TC 20
Z9 20
U1 1
U2 60
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 5
PY 2013
VL 103
IS 6
AR 063502
DI 10.1063/1.4817927
PG 4
WC Physics, Applied
SC Physics
GA 198FT
UT WOS:000322908300077
ER
PT J
AU Mun, BS
Yoon, J
Mo, SK
Chen, K
Tamura, N
Dejoie, C
Kunz, M
Liu, Z
Park, C
Moon, K
Ju, H
AF Mun, Bongjin Simon
Yoon, Joonseok
Mo, Sung-Kwan
Chen, Kai
Tamura, Nobumichi
Dejoie, Catherine
Kunz, Martin
Liu, Zhi
Park, Changwoo
Moon, Kyungsun
Ju, Honglyoul
TI Role of joule heating effect and bulk-surface phases in voltage-driven
metal-insulator transition in VO2 crystal
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID VANADIUM DIOXIDE; MOTT TRANSITION
AB We report the characteristics of a voltage-induced metal-insulator transition (MIT) in macro-sized VO2 crystals. The square of MIT onset voltage (V-2(CMIT)) value shows a linear dependence with the ambient temperature, suggesting that the Joule heating effect is the likely cause to the voltage-induced MIT. The combination of optical microscope images and Laue microdiffraction patterns show the simultaneous presence of a metallic phase in the bulk of the crystal with partially insulating surface layers even after the MIT occurs. A large asymmetry in the heating power just before and after the MIT reflects the sudden exchange of Joule heat to its environment. (C) 2013 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.
C1 [Mun, Bongjin Simon] Gwangju Inst Sci & Technol, Dept Phys & Photon Sci, Sch Phys & Chem, Ertl Ctr Electrochem & Catalyst, Kwangju 500712, South Korea.
[Yoon, Joonseok; Moon, Kyungsun; Ju, Honglyoul] Yonsei Univ, Dept Phys, Seoul 120749, South Korea.
[Mo, Sung-Kwan; Chen, Kai; Tamura, Nobumichi; Dejoie, Catherine; Kunz, Martin; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Chen, Kai] Xi An Jiao Tong Univ, Ctr Adv Mat Performance Nanoscale CAMP Nano, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China.
[Park, Changwoo] Hanbat Natl Univ, Div Appl Chem & Biotechnol, Taejon 305719, South Korea.
[Park, Changwoo] Adv Nano Prod, Chungwon 363942, Chungbuk, South Korea.
RP Mun, BS (reprint author), Gwangju Inst Sci & Technol, Dept Phys & Photon Sci, Sch Phys & Chem, Ertl Ctr Electrochem & Catalyst, Kwangju 500712, South Korea.
EM bsmun@gist.ac.kr; tesl@yonsei.ac.kr
RI Chen, Kai/O-5662-2014; Liu, Zhi/B-3642-2009; Mo, Sung-Kwan/F-3489-2013;
xjtu, campnano/Q-1904-2015;
OI Chen, Kai/0000-0002-4917-4445; Liu, Zhi/0000-0002-8973-6561; Mo,
Sung-Kwan/0000-0003-0711-8514; Yoon, Joonseok/0000-0001-5937-1787
FU Basic Science Research Program through the National Research Foundation
of Korea (NRF); Ministry of Education, Science and Technology
[2012R1A1A2006948, 2012R1A1A2001745]; Office of Science, Office of Basic
Energy Sciences, Materials Science Division, of the US Department of
Energy [DE-AC02-05CH11231]; NSF [0416243]; GIST College's GUP Research
Fund
FX H. L. Ju and B. S. Mun would like to thank the support by Basic Science
Research Program through the National Research Foundation of Korea (NRF)
funded by the Ministry of Education, Science and Technology
(2012R1A1A2006948 and 2012R1A1A2001745). The Advanced Light Source is
supported by the Director, Office of Science, Office of Basic Energy
Sciences, Materials Science Division, of the US Department of Energy
under Contract No. DE-AC02-05CH11231 at LBNL. The microdiffraction
program at the ALS on BL 12.3.2 was made possible by NSF Grant No.
0416243. This paper was supported by GIST College's 2013 GUP Research
Fund.
NR 17
TC 16
Z9 16
U1 1
U2 63
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 5
PY 2013
VL 103
IS 6
AR 061902
DI 10.1063/1.4817727
PG 5
WC Physics, Applied
SC Physics
GA 198FT
UT WOS:000322908300026
ER
PT J
AU Singh, R
Chowdhury, DR
Xiong, J
Yang, H
Azad, AK
Taylor, AJ
Jia, QX
Chen, HT
AF Singh, Ranjan
Chowdhury, Dibakar Roy
Xiong, Jie
Yang, Hao
Azad, Abul K.
Taylor, Antoinette J.
Jia, Q. X.
Chen, Hou-Tong
TI Influence of film thickness in THz active metamaterial devices: A
comparison between superconductor and metal split-ring resonators
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID NEGATIVE-INDEX METAMATERIALS; TERAHERTZ METAMATERIALS; REFRACTION;
ELECTRODYNAMICS; PERMITTIVITY; TUNABILITY
AB We experimentally demonstrate thickness-dependent resonance tuning in planar terahertz superconducting metamaterials. Inductive-capacitive resonance of arrays of split-ring resonators fabricated from 50, 100, and 200 nm thick YBa2Cu3O7-delta (YBCO) and gold films were characterized and compared as a function of temperature. In the YBCO metamaterials the resonance frequency strongly depends on the thickness, and they show high thermal tunability in both resonance strength and frequency below the superconducting transition temperature, where the imaginary conductivity varies by three orders of magnitude. In contrast, the resonance in the gold metamaterials exhibits little thickness-dependence and very small tunability. (C) 2013 AIP Publishing LLC.
C1 [Singh, Ranjan; Chowdhury, Dibakar Roy; Xiong, Jie; Yang, Hao; Azad, Abul K.; Taylor, Antoinette J.; Jia, Q. X.; Chen, Hou-Tong] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.
[Singh, Ranjan] Los Alamos Natl Lab, AOT HPE, Los Alamos, NM 87545 USA.
RP Singh, R (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA.
EM ranjan@lanl.gov; chenht@lanl.gov
RI Singh, Ranjan/B-4091-2010; Chen, Hou-Tong/C-6860-2009; Jia, Q.
X./C-5194-2008;
OI Singh, Ranjan/0000-0001-8068-7428; Chen, Hou-Tong/0000-0003-2014-7571;
Azad, Abul/0000-0002-7784-7432
FU Los Alamos National Laboratory LDRD Program; National Nuclear Security
Administration of the US Department of Energy [DE-AC52-06NA25396]
FX We acknowledge partial support from the Los Alamos National Laboratory
LDRD Program. This work was performed, in part, at the Center for
Integrated Nanotechnologies, a US Department of Energy, Office of Basic
Energy Sciences Nanoscale Science Research Center operated jointly by
Los Alamos and Sandia National Laboratories. Los Alamos National
Laboratory, an affirmative action/equal opportunity employer, is
operated by Los Alamos National Security, LLC, for the National Nuclear
Security Administration of the US Department of Energy under contract
DE-AC52-06NA25396.
NR 41
TC 11
Z9 11
U1 3
U2 91
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 5
PY 2013
VL 103
IS 6
AR 061117
DI 10.1063/1.4817814
PG 5
WC Physics, Applied
SC Physics
GA 198FT
UT WOS:000322908300017
ER
PT J
AU Lampimaki, M
Zelenay, V
Krepelova, A
Liu, Z
Chang, R
Bluhm, H
Ammann, M
AF Lampimaeki, Markus
Zelenay, Veronika
Krepelova, Adela
Liu, Zhi
Chang, Rui
Bluhm, Hendrik
Ammann, Markus
TI Ozone-Induced Band Bending on Metal-Oxide Surfaces Studied under
Environmental Conditions
SO CHEMPHYSCHEM
LA English
DT Article
DE band bending; metal oxides; ozone; surface chemistry; x-ray
photoelectron spectroscopy
ID RAY PHOTOELECTRON-SPECTROSCOPY; TITANIUM-DIOXIDE; OXYGEN; TIO2(110);
DECOMPOSITION; ADSORPTION; WATER; DUST; TEMPERATURE; ABSORPTION
AB Ozone adsorption and decomposition on metal oxides is of wide interest in technology and in atmospheric chemistry. Here, ozone-adsorption-induced band bending is observed on Ti-and Fe-oxide model surfaces under dry and humid conditions. Photoelectron spectroscopic studies indicate the effect of charge transfer to O-3, which limits the surface coverage of the precursor to decomposition reactions. This is also consistent with the negative pressure dependence observed in previous studies. These results contribute to our fundamental understanding of ozone adsorption and decomposition mechanisms on metal oxides of environmental and technological relevance.
C1 [Lampimaeki, Markus; Zelenay, Veronika; Krepelova, Adela; Ammann, Markus] Paul Scherrer Inst, Lab Radiochem & Environm Chem, CH-5232 Villigen, Switzerland.
[Liu, Zhi; Chang, Rui] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
RP Ammann, M (reprint author), Paul Scherrer Inst, Lab Radiochem & Environm Chem, CH-5232 Villigen, Switzerland.
EM markus.ammann@psi.ch
RI Liu, Zhi/B-3642-2009; Ammann, Markus/E-4576-2011;
OI Liu, Zhi/0000-0002-8973-6561; Ammann, Markus/0000-0001-5922-9000;
Lampimaki, Markus/0000-0003-1990-6155
FU Swiss National Science Foundation [130175]; Office of Science, Office of
Basic Energy Sciences, and by the Division of Chemical Sciences,
Geosciences, and Biosciences of the U.S. Department of Energy at
Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]
FX This work was supported by the Swiss National Science Foundation (grant
no. 130175) (M. L. and M. A.). The Advanced Light Source and beamline
9.3.2 are supported by the Director, Office of Science, Office of Basic
Energy Sciences, and by the Division of Chemical Sciences, Geosciences,
and Biosciences of the U.S. Department of Energy at Lawrence Berkeley
National Laboratory under Contract No. DE-AC02-05CH11231.
NR 35
TC 9
Z9 9
U1 3
U2 41
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1439-4235
EI 1439-7641
J9 CHEMPHYSCHEM
JI ChemPhysChem
PD AUG 5
PY 2013
VL 14
IS 11
BP 2419
EP 2425
DI 10.1002/cphc.201300418
PG 7
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 190KP
UT WOS:000322339100012
PM 23740601
ER
PT J
AU Doll, T
Velasco-Velez, JJ
Rosenthal, D
Avila, J
Fuenzalida, V
AF Doll, Theodor
Velasco-Velez, Juan J.
Rosenthal, Dirk
Avila, Jonathan
Fuenzalida, Victor
TI Direct Observation of the Electroadsorptive Effect on Ultrathin Films
for Microsensor and Catalytic-Surface Control
SO CHEMPHYSCHEM
LA English
DT Article
DE adsorption; electroadsorptive effect; semiconductors; sensors; thin
films
ID SEMICONDUCTOR GAS SENSORS; THIN-FILMS; SNO2; NO2; OXIDE; TEMPERATURE;
OXYGEN; FIELD; CHEMISORPTION
AB Microchemical sensors and catalytic reactors make use of gases during adsorption in specific ways on selected materials. Fine-tuning is normally achieved by morphological control and material doping. The latter relates surface properties to the electronic structure of the bulk, and this suggests the possibility of electronic control. Although unusual for catalytic surfaces, such phenomena are sometimes reported for microsensors, but with little understanding of the underlying mechanisms. Herein, direct observation of the electroadsorptive effect by a combination of X-ray photoelectron spectroscopy and con-ductivity analysis on nanometre-thick semiconductor films on buried control electrodes is reported. For the SnO2/NO2 model system, NO3 surface species, which normally decay at the latest within minutes, can be kept stable for 1.5 h with a high coverage of 15% under appropriate electric fields. This includes uncharged states, too, and implies that nanoelectronic structures provide control over the predominant adsorbate conformation on exterior surfaces and thus opens the field for chemically reactive interfaces with in situ tunability.
C1 [Doll, Theodor; Velasco-Velez, Juan J.] Johannes Gutenberg Univ Mainz, D-55128 Mainz, Germany.
[Rosenthal, Dirk] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany.
[Velasco-Velez, Juan J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Avila, Jonathan] Univ Fed Santa Catarina, CFM, Lab Filmes Finos & Superficies LFFS, BR-88040900 Florianopolis, SC, Brazil.
[Avila, Jonathan; Fuenzalida, Victor] Univ Chile, Dept Fis, Santiago, Chile.
RP Doll, T (reprint author), Hannover Med Sch, VIANNA, Feodor Lynen Str 35, D-30625 Hannover, Germany.
EM doll.theodor@mh-hannover.de; dirkrose@fhi-berlin.mpg.de
RI Fuenzalida, Victor/A-5244-2013
OI Fuenzalida, Victor/0000-0002-5481-4646
FU DAAD/CONICYT [ALECHILE 2009-193]; Chilean government [FONDECYT 1110168]
FX Partial funding of this work by DAAD/CONICYT ALECHILE 2009-193 and Grant
FONDECYT 1110168 of the Chilean government is acknowledged. The authors
gratefully acknowledge layer preparation (dev.1) by FhG IPM, Freiburg,
Germany.
NR 36
TC 0
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U1 1
U2 11
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1439-4235
J9 CHEMPHYSCHEM
JI ChemPhysChem
PD AUG 5
PY 2013
VL 14
IS 11
BP 2505
EP 2510
DI 10.1002/cphc.201201013
PG 6
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 190KP
UT WOS:000322339100022
PM 23687010
ER
PT J
AU Santarnecchi, E
Polizzotto, NR
Godone, M
Giovannelli, F
Feurra, M
Matzen, L
Rossi, A
Rossi, S
AF Santarnecchi, Emiliano
Polizzotto, Nicola Riccardo
Godone, Marco
Giovannelli, Fabio
Feurra, Matteo
Matzen, Laura
Rossi, Alessandro
Rossi, Simone
TI Frequency-Dependent Enhancement of Fluid Intelligence Induced by
Transcranial Oscillatory Potentials
SO CURRENT BIOLOGY
LA English
DT Article
ID CURRENT STIMULATION TACS; WORKING-MEMORY; CORTICAL EXCITABILITY; BRAIN
EXCITABILITY; PREFRONTAL CORTEX; SYNCHRONIZATION; PERFORMANCE;
COGNITION; HUMANS; RATS
AB Everyday problem solving requires the ability to go beyond experience by efficiently encoding and manipulating new information, i.e., fluid intelligence (Gf) [1]. Performance in tasks involving Gf, such as logical and abstract reasoning, has been shown to rely on distributed neural networks, with a crucial role played by prefrontal regions [2]. Synchronization of neuronal activity in the gamma band is a ubiquitous phenomenon within the brain; however, no evidence of its causal involvement in cognition exists to date [3]. Here, we show an enhancement of Gf ability in a cognitive task induced by exogenous rhythmic stimulation within the gamma band. Imperceptible alternating current [4] delivered through the scalp over the left middle frontal gyrus resulted in a frequency-specific shortening of the time required to find the correct solution in a visuospatial abstract reasoning task classically employed to measure Gf abilities (i.e., Raven's matrices) [5]. Crucially, gamma-band stimulation (gamma-tACS) selectively enhanced performance only on more complex trials involving conditional/logical reasoning. The present finding supports a direct involvement of gamma oscillatory activity in the mechanisms underlying higher-order human cognition.
C1 [Santarnecchi, Emiliano; Godone, Marco; Feurra, Matteo; Rossi, Alessandro; Rossi, Simone] Univ Siena, Dept Med Surg & Neurosci, I-53100 Siena, Italy.
[Polizzotto, Nicola Riccardo] Univ Pittsburgh, Dept Psychiat, Pittsburgh, PA 15213 USA.
[Giovannelli, Fabio] Florence Hosp, Complex Unit Neurol, I-50134 Florence, Italy.
[Matzen, Laura] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Santarnecchi, E (reprint author), Univ Siena, Dept Med Surg & Neurosci, Via Laterina 8, I-53100 Siena, Italy.
EM emilianosantarnecchi@gmail.com
RI Feurra, Matteo/K-4448-2013;
OI Feurra, Matteo/0000-0003-0934-6764; rossi, simone/0000-0001-6697-9459
NR 39
TC 56
Z9 56
U1 1
U2 21
PU CELL PRESS
PI CAMBRIDGE
PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA
SN 0960-9822
J9 CURR BIOL
JI Curr. Biol.
PD AUG 5
PY 2013
VL 23
IS 15
BP 1449
EP 1453
DI 10.1016/j.cub.2013.06.022
PG 5
WC Biochemistry & Molecular Biology; Cell Biology
SC Biochemistry & Molecular Biology; Cell Biology
GA 198NS
UT WOS:000322930200022
PM 23891115
ER
PT J
AU Brown, EW
DuBois, JL
Holzmann, M
Ceperley, DM
AF Brown, Ethan W.
DuBois, Jonathan L.
Holzmann, Markus
Ceperley, David M.
TI Exchange-correlation energy for the three-dimensional homogeneous
electron gas at arbitrary temperature
SO PHYSICAL REVIEW B
LA English
DT Article
ID ONE-COMPONENT PLASMA; DENSE IONIZED MATTER; GROUND-STATE; EQUILIBRIUM
PROPERTIES; STATISTICAL-MECHANICS; QUANTUM CORRECTIONS;
FINITE-TEMPERATURE; LIQUID; FUNCTIONALS; ACCURATE
AB We fit finite-temperature path integral Monte Carlo calculations of the exchange-correlation energy of the 3D finite-temperature homogeneous electron gas in the warm-dense regime [r(s) = (3/4 pi n)(1/3)a(B)(-1) < 40 and Theta = T/T-F > 0.0625]. In doing so, we construct a Pade approximant which collapses to Debye-Huckel theory in the high-temperature, low-density limit. Likewise, the zero-temperature limit matches the numerical results of ground-state quantum Monte Carlo, as well as analytical results in the high-density limit.
C1 [Brown, Ethan W.; Ceperley, David M.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA.
[Brown, Ethan W.; DuBois, Jonathan L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Holzmann, Markus] Univ Paris 06, CNRS, LPTMC, UMR 7600, F-75005 Paris, France.
[Holzmann, Markus] Univ Grenoble 1, CNRS, LPMMC, UMR 5493, F-38042 Grenoble, France.
[Holzmann, Markus] European Theoret Spect Facil, Grenoble, France.
RP Brown, EW (reprint author), Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA.
EM brown122@illinois.edu
OI DuBois, Jonathan/0000-0003-3154-4273
FU US Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]; LDRD [10-ERD-058]; Lawrence Scholar program;
[DE-FG52-09NA29456]
FX The authors would like to thank Jeremy McMinis and Miguel Morales for
useful discussions. This work was supported by Grant No.
DE-FG52-09NA29456. In addition, the work of E.B. and J.D. was performed
under the auspices of the US Department of Energy by Lawrence Livermore
National Laboratory under Contract No. DE-AC52-07NA27344 with support
from LDRD 10-ERD-058 and the Lawrence Scholar program. Computational
resources included LC machines at Lawrence Livermore National Laboratory
through the institutional computation Grand Challenge program.
NR 43
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U1 1
U2 19
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 5
PY 2013
VL 88
IS 8
AR 081102
DI 10.1103/PhysRevB.88.081102
PG 5
WC Physics, Condensed Matter
SC Physics
GA 196SK
UT WOS:000322796300002
ER
PT J
AU Jansen, GR
AF Jansen, G. R.
TI Spherical coupled-cluster theory for open-shell nuclei
SO PHYSICAL REVIEW C
LA English
DT Article
ID CONNECTED TRIPLE EXCITATIONS; EXCITED-STATES; ENERGY-LEVELS; FULL
INCLUSION; EOM-CCSDT; SYSTEMS
AB Background: A microscopic description of nuclei is important to understand the nuclear shell model from fundamental principles. This is difficult to achieve for more than the lightest nuclei without an effective approximation scheme.
Purpose: Define and evaluate an approximation scheme that can be used to study nuclei that are described as two particles attached to a closed (sub-) shell nucleus.
Methods: The equation-of-motion coupled-cluster formalism has been used to obtain ground- and excited-state energies. This method is based on the diagonalization of a non-Hermitian matrix obtained from a similarity transformation of the many-body nuclear Hamiltonian. A chiral interaction at the next-to-next-to-next-to leading order (N-3 LO) using a cutoff at 500 MeV was used.
Results: The ground- state energies of Li-6 and He-6 were in good agreement with a no-core shell-model calculation using the same interaction. Several excited states were also produced with overall good agreement. Only the J(pi) = 3(+) excited state in Li-6 showed a sizable deviation. The ground- state energies of O-18, F-18, and Ne-18 were converged but underbound compared to experiment. Moreover, the calculated spectra were converged and comparable to both experiment and shell-model studies in this region. Some excited states in O-18 were high or missing in the spectrum. It was also shown that the wave function for both ground and excited states separates into an intrinsic part and a Gaussian for the center-of-mass coordinate. Spurious center-of-mass excitations are clearly identified.
Conclusions: Results are converged with respect to the size of the model space and the method can be used to describe nuclear states with simple structure. Especially the ground-state energies were very close to what has been achieved by exact diagonalization. To obtain a closer match with experimental data, effects of three-nucleon forces, the scattering continuum, as well as additional configurations in the coupled-cluster approximations are necessary.
C1 [Jansen, G. R.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
[Jansen, G. R.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA.
[Jansen, G. R.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway.
[Jansen, G. R.] Univ Oslo, Ctr Math Applicat, N-0316 Oslo, Norway.
RP Jansen, GR (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
EM gustav.jansen@utk.edu
OI Jansen, Gustav R./0000-0003-3558-0968
FU Office of Nuclear Physics, US Department of Energy (Oak Ridge National
Laboratory) [DE-FG02-96ER40963, DE-SC0008499]; Office of Science of the
Department of Energy [DE-AC05-00OR22725]
FX I thank M. Hjorth-Jensen and T. Papenbrock for valuable comments on the
manuscript. In addition I thank G. Hagen and A. Ekstrom for very useful
discussions. This work was partly supported by the Office of Nuclear
Physics, US Department of Energy (Oak Ridge National Laboratory), under
Contracts No. DE-FG02-96ER40963 (University of Tennessee) and No.
DE-SC0008499 (NUCLEI SciDAC-3 Collaboration). An award of computer time
was provided by the Innovative and Novel Computational Impact on Theory
and Experiment (INCITE) program. This research used resources of the Oak
Ridge Leadership Computing Facility located in the Oak Ridge National
Laboratory, which is supported by the Office of Science of the
Department of Energy under Contract No. DE-AC05-00OR22725 and used
computational resources of the National Center for Computational
Sciences, the National Institute for Computational Sciences, and the
Notur project in Norway.
NR 51
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U1 1
U2 6
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 2469-9985
EI 2469-9993
J9 PHYS REV C
JI Phys. Rev. C
PD AUG 5
PY 2013
VL 88
IS 2
AR 024305
DI 10.1103/PhysRevC.88.024305
PG 20
WC Physics, Nuclear
SC Physics
GA 196SP
UT WOS:000322796900005
ER
PT J
AU Alexandrou, C
Negele, JW
Petschlies, M
Strelchenko, A
Tsapalis, A
AF Alexandrou, C.
Negele, J. W.
Petschlies, M.
Strelchenko, A.
Tsapalis, A.
TI Determination of Delta-resonance parameters from lattice QCD
SO PHYSICAL REVIEW D
LA English
DT Article
ID QUANTUM-FIELD THEORIES; VOLUME DEPENDENCE; ENERGY-SPECTRUM; STATES
AB A method suitable for extracting resonance parameters of unstable baryons in lattice QCD is examined. The method is applied to the strong decay of the Delta to a pion-nucleon state, extracting the pi N Delta coupling constant and Delta decay width.
C1 [Alexandrou, C.] Univ Cyprus, Dept Phys, CY-1678 Nicosia, Cyprus.
[Alexandrou, C.; Petschlies, M.] Cyprus Inst, Computat Based Sci & Technol Res Ctr, CY-2121 Nicosia, Cyprus.
[Negele, J. W.] MIT, Ctr Theoret Phys, Nucl Sci Lab, Cambridge, MA 02139 USA.
[Negele, J. W.] MIT, Ctr Theoret Phys, Dept Phys, Cambridge, MA 02139 USA.
[Strelchenko, A.] Fermilab Natl Accelerator Lab, Div Comp Sci, Batavia, IL 60510 USA.
[Tsapalis, A.] Hellen Naval Acad, Piraeus 18539, Greece.
[Tsapalis, A.] Natl Tech Univ Athens, Dept Phys, Athens 15780, Greece.
RP Alexandrou, C (reprint author), Univ Cyprus, Dept Phys, POB 20537, CY-1678 Nicosia, Cyprus.
FU Research Executive Agency of the European Union [PITN-GA-2009-238353];
DOE Office of Nuclear Physics [DE-FG02-94ER40818]; Cyprus Research
Promotion Foundation [NEA YPiODeltaOMH/SigmaTPATH/0308/31]; National
Energy Research Scientific Computing Center; Office of Science of the
DOE [DE-AC02-05CH11231]; Julich Supercomputing Center under the PRACE EU
FP7 Project [2011040546]; PRACE [RI-211528, FP7-261557]
FX We would like to thank C. Michael for valuable discussions. This
research was in part supported by the Research Executive Agency of the
European Union under Grant Agreement No. PITN-GA-2009-238353 (ITN
STRONGnet) and in part by the DOE Office of Nuclear Physics under Grant
No. DE-FG02-94ER40818. The GPU computing resources were provided by the
Cy-Tera machine at the Cyprus Institute, supported in part by the Cyprus
Research Promotion Foundation under Contract No. NEA Y Pi O Delta
OMH/Sigma TPATH/0308/31, the National Energy Research Scientific
Computing Center supported by the Office of Science of the DOE under
Grant No. DE-AC02-05CH11231, and by the Julich Supercomputing Center,
awarded under the PRACE EU FP7 Project No. 2011040546. The multi-GPU
domain wall inverter code [19] is based on the QUDA library [20,21], and
its development has been supported by PRACE Grants No. RI-211528 and No.
FP7-261557.
NR 21
TC 5
Z9 5
U1 0
U2 0
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1550-7998
EI 1550-2368
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 5
PY 2013
VL 88
IS 3
AR 031501
DI 10.1103/PhysRevD.88.031501
PG 5
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 196SU
UT WOS:000322797500002
ER
PT J
AU Latimer, ML
Berdiyorov, GR
Xiao, ZL
Peeters, FM
Kwok, WK
AF Latimer, M. L.
Berdiyorov, G. R.
Xiao, Z. L.
Peeters, F. M.
Kwok, W. K.
TI Realization of Artificial Ice Systems for Magnetic Vortices in a
Superconducting MoGe Thin Film with Patterned Nanostructures
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID SPIN-ICE; FRUSTRATION; FERROELECTRICITY; DEFECTS
AB We report an anomalous matching effect in MoGe thin films containing pairs of circular holes arranged in such a way that four of those pairs meet at each vertex point of a square lattice. A remarkably pronounced fractional matching was observed in the magnetic field dependences of both the resistance and the critical current. At the half matching field the critical current can be even higher than that at zero field. This has never been observed before for vortices in superconductors with pinning arrays. Numerical simulations within the nonlinear Ginzburg-Landau theory reveal a square vortex ice configuration in the ground state at the half matching field and demonstrate similar characteristic features in the field dependence of the critical current, confirming the experimental realization of an artificial ice system for vortices for the first time.
C1 [Latimer, M. L.; Xiao, Z. L.; Kwok, W. K.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Latimer, M. L.; Xiao, Z. L.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.
[Berdiyorov, G. R.; Peeters, F. M.] Univ Antwerp, Dept Fys, B-2020 Antwerp, Belgium.
RP Latimer, ML (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM xiao@anl.gov; francois.peeters@ua.ac.be
RI CMT, UAntwerpen Group/A-5523-2016
FU US Department of Energy DOE BES [DE-AC02-06CH11357]; Flemish Science
Foundation (FWO-Vl); Methusalem Foundation of the Flemish Government;
FWO-Vl; DOE BES [DE-AC02-06CH11357, DE-FG02-06ER46334]; NIU/ANL
Distinguished Graduate Fellowship grant
FX This work was supported by the US Department of Energy DOE BES under
Contract No. DE-AC02-06CH11357 (transport measurements), the Flemish
Science Foundation (FWO-Vl) and the Methusalem Foundation of the Flemish
Government (numerical simulations). G. R. B. acknowledges an individual
grant from FWO-Vl. The nanopatterning and morphological analysis were
performed at Argonne's Center for Nanoscale Materials (CNM) which is
funded by DOE BES under Contract No. DE-AC02-06CH11357. We are grateful
to Dr. Charles Reichhardt in Los Alamos National Laboratory for
stimulating discussions and critical comments. Z. L. X. acknowledges DOE
BES Grant No. DE-FG02-06ER46334 (sample fabrication and imaging). M. L.
L. was a recipient of the NIU/ANL Distinguished Graduate Fellowship
grant.
NR 36
TC 20
Z9 20
U1 5
U2 39
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 5
PY 2013
VL 111
IS 6
AR 067001
DI 10.1103/PhysRevLett.111.067001
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196TJ
UT WOS:000322799200013
PM 23971602
ER
PT J
AU Ping, Y
Coppari, F
Hicks, DG
Yaakobi, B
Fratanduono, DE
Hamel, S
Eggert, JH
Rygg, JR
Smith, RF
Swift, DC
Braun, DG
Boehly, TR
Collins, GW
AF Ping, Y.
Coppari, F.
Hicks, D. G.
Yaakobi, B.
Fratanduono, D. E.
Hamel, S.
Eggert, J. H.
Rygg, J. R.
Smith, R. F.
Swift, D. C.
Braun, D. G.
Boehly, T. R.
Collins, G. W.
TI Solid Iron Compressed Up to 560 GPa
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID EARTHS INNER-CORE; ABSORPTION FINE-STRUCTURE; AB-INITIO CALCULATIONS;
X-RAY-DIFFRACTION; SPECTROSCOPY; ELASTICITY; FE; TEMPERATURE; PRESSURE;
FACILITY
AB Dynamic compression by multiple shocks is used to compress iron up to 560 GPa (5.6 Mbar), the highest solid-state pressure yet attained for iron in the laboratory. Extended x-ray absorption fine structure (EXAFS) spectroscopy offers simultaneous density, temperature, and local-structure measurements for the compressed iron. The data show that the close-packed structure of iron is stable up to 560 GPa, the temperature at peak compression is significantly higher than expected from pure compressive work, and the dynamic strength of iron is many times greater than the static strength based on lower pressure data. The results provide the first constraint on the melting line of iron above 400 GPa.
C1 [Ping, Y.; Coppari, F.; Hicks, D. G.; Fratanduono, D. E.; Hamel, S.; Eggert, J. H.; Rygg, J. R.; Smith, R. F.; Swift, D. C.; Braun, D. G.; Collins, G. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Yaakobi, B.; Boehly, T. R.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA.
RP Ping, Y (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
EM ping2@LLNL.gov
RI Hicks, Damien/B-5042-2015
OI Hicks, Damien/0000-0001-8322-9983
FU U.S. DOE HEDLP program; U.S. DOE by LLNL [DEAC52-07NA27344]; LDRD
program at LLNL
FX We wish to thank the OMEGA team at LLE for laser operation and technical
support. We also would like to thank W. Unites, T. Uphaus, S. Uhlich,
and R. Wallace for target fabrication. We appreciate helpful discussion
with R. E. Rudd and R. Kraus. Y. P. acknowledges support from the U.S.
DOE HEDLP program. This work was performed under the auspices of the
U.S. DOE by LLNL under Contract No. DEAC52-07NA27344 and the LDRD
program at LLNL.
NR 49
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U1 4
U2 70
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 5
PY 2013
VL 111
IS 6
AR 065501
DI 10.1103/PhysRevLett.111.065501
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196TJ
UT WOS:000322799200007
PM 23971582
ER
PT J
AU Van Schelt, J
Lascar, D
Savard, G
Clark, JA
Bertone, PF
Caldwell, S
Chaudhuri, A
Levand, AF
Li, G
Morgan, GE
Orford, R
Segel, RE
Sharma, KS
Sternberg, MG
AF Van Schelt, J.
Lascar, D.
Savard, G.
Clark, J. A.
Bertone, P. F.
Caldwell, S.
Chaudhuri, A.
Levand, A. F.
Li, G.
Morgan, G. E.
Orford, R.
Segel, R. E.
Sharma, K. S.
Sternberg, M. G.
TI First Results from the CARIBU Facility: Mass Measurements on the
r-Process Path
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID FRS-ESR FACILITY; PENNING TRAP; ADJUSTMENT PROCEDURES; GAS CATCHERS;
INPUT DATA; NUCLEAR; SPECTROMETER; ISOTOPES; ION; RESOLUTION
AB The Canadian Penning Trap mass spectrometer has made mass measurements of 33 neutron-rich nuclides provided by the new Californium Rare Isotope Breeder Upgrade facility at Argonne National Laboratory. The studied region includes the Sn-132 double shell closure and ranges in Z from In to Cs, with Sn isotopes measured out to A = 135, and the typical measurement precision is at the 100 ppb level or better. The region encompasses a possible major waiting point of the astrophysical r process, and the impact of the masses on the r process is shown through a series of simulations. These first-ever simulations with direct mass information on this waiting point show significant increases in waiting time at Sn and Sb in comparison with commonly used mass models, demonstrating the inadequacy of existing models for accurate r-process calculations.
C1 [Van Schelt, J.; Lascar, D.; Savard, G.; Clark, J. A.; Bertone, P. F.; Caldwell, S.; Chaudhuri, A.; Levand, A. F.; Li, G.; Segel, R. E.; Sternberg, M. G.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.
[Van Schelt, J.; Savard, G.; Caldwell, S.; Sternberg, M. G.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA.
[Lascar, D.; Segel, R. E.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA.
[Chaudhuri, A.; Morgan, G. E.; Sharma, K. S.] Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada.
[Li, G.; Orford, R.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada.
RP Van Schelt, J (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.
RI Chaudhuri, Ankur/G-2940-2013
FU NSERC, Canada [216974]; U.S. DOE, Office of Nuclear Physics
[DE-AC02-06CH11357]
FX The authors acknowledge J. W. Truran and C. Ugalde for their helpful
discussions regarding the simulations. This work was performed under the
auspices of NSERC, Canada, Application No. 216974, and the U.S. DOE,
Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357.
NR 44
TC 24
Z9 24
U1 1
U2 18
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 5
PY 2013
VL 111
IS 6
AR 061102
DI 10.1103/PhysRevLett.111.061102
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196TJ
UT WOS:000322799200002
PM 23971550
ER
PT J
AU Wang, XN
Zhu, Y
AF Wang, Xin-Nian
Zhu, Yan
TI Medium Modification of gamma Jets in High-Energy Heavy-Ion Collisions
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID NUCLEI; PHOTON; PP
AB Two puzzling features in the experimental study of jet quenching in central Pb + Pb collisions at the LHC are explained within a linearized Boltzmann transport model for jet propagation. A gamma-tagged jet is found to lose about 15% of its initial energy while its azimuthal angle remains almost unchanged due to rapid cooling of the medium. The reconstructed jet fragmentation function is found to have some modest enhancement at both small and large fractional momenta as compared to that in the vacuum because of the increased contribution of leading particles to the reconstructed jet energy and induced gluon radiation and recoiled partons. A gamma-tagged jet fragmentation function is proposed that is more sensitive to jet-medium interaction and the jet transport parameter in the medium. The effects of recoiled medium partons on the reconstructed jets are also discussed.
C1 [Wang, Xin-Nian] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China.
[Wang, Xin-Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.
[Zhu, Yan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA.
[Zhu, Yan] Univ Bielefeld, Fac Phys, D-33501 Bielefeld, Germany.
RP Wang, XN (reprint author), Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China.
OI Wang, Xin-Nian/0000-0002-9734-9967
FU NSFC [11221504]; U.S. DOE [DE-AC02-05CH11231]; German Research
Foundation DFG (ITRG) [GRK 881]; Humboldt Foundation
FX We thank M. Cacciari for providing a modified version of FASTJET for use
in this study. This work is supported by the NSFC under Grant No.
11221504, the U.S. DOE under Contract No. DE-AC02-05CH11231, and within
the framework of the JET Collaboration. Y. Z. is also supported by the
German Research Foundation DFG (ITRG) GRK 881 and the Humboldt
Foundation.
NR 22
TC 31
Z9 31
U1 0
U2 2
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 5
PY 2013
VL 111
IS 6
AR 062301
DI 10.1103/PhysRevLett.111.062301
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196TJ
UT WOS:000322799200003
PM 23971567
ER
PT J
AU Woo, SJ
Lee, ES
Yoon, M
Kim, YH
AF Woo, Sung-Jae
Lee, Eui-Sup
Yoon, Mina
Kim, Yong-Hyun
TI Finite-Temperature Hydrogen Adsorption and Desorption Thermodynamics
Driven by Soft Vibration Modes
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID ADSORBED MOLECULES; STORAGE; ENTROPIES; SITES; METAL
AB It has been widely accepted that enhanced dihydrogen adsorption is required for room-temperature hydrogen storage on nanostructured porous materials. Here we report, based on results of first-principles total energy and vibrational spectrum calculations, finite-temperature adsorption and desorption thermodynamics of hydrogen molecules that are adsorbed on the metal center of metal-porphyrin-incorporated graphene. We have revealed that the room-temperature hydrogen storage is achievable not only with the enhanced adsorption enthalpy, but also with soft-mode driven vibrational entropy of the adsorbed dihydrogen molecule. The soft vibration modes mostly result from multiple orbital coupling between the hydrogen molecule and the buckled metal center, for example, in Ca-porphyrin-incorporated graphene. Our study suggests that the current design strategy for room-temperature hydrogen storage materials should be modified with explicitly taking the finite-temperature vibration thermodynamics into account.
C1 [Woo, Sung-Jae; Lee, Eui-Sup; Kim, Yong-Hyun] Korea Adv Inst Sci & Technol, Grad Sch Nanosci & Technol WCU, Taejon 305701, South Korea.
[Yoon, Mina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
RP Kim, YH (reprint author), Korea Adv Inst Sci & Technol, Grad Sch Nanosci & Technol WCU, Taejon 305701, South Korea.
EM yong.hyun.kim@kaist.ac.kr
RI Kim, Yong-Hyun/C-2045-2011; Yoon, Mina/A-1965-2016
OI Kim, Yong-Hyun/0000-0003-4255-2068; Yoon, Mina/0000-0002-1317-3301
FU WCU [R31-2008-000-10071-0]; NRF [2012R1A2A2A01046191, 2010-0006922];
Global Frontier RD [2011-0031566]; Korea government (MEST); National
Energy Research Scientific Computing Center [DE-AC02-05CH11231]
FX We thank J. Kang and Y. Ihm for reading the manuscript. This work was
supported by the WCU (R31-2008-000-10071-0), NRF (2012R1A2A2A01046191
and 2010-0006922), and Global Frontier R&D (2011-0031566: Center for
Multiscale Energy Systems) programs funded by the Korea government
(MEST). M. Y. was supported by the U.S. Department of Energy, Office of
Basic Energy Sciences, Materials Sciences and Engineering Division for
structural configurations of the metal-incorporated graphene; the
Scientific User Facilities Division for explorations of the catalytic
functionality in theme research at the Center for Nanophase Materials
Sciences; and the National Energy Research Scientific Computing Center
for computing resource under Contract No. DE-AC02-05CH11231. S-J. W. and
E-S. L. contributed equally to this work.
NR 32
TC 9
Z9 9
U1 7
U2 45
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 5
PY 2013
VL 111
IS 6
AR 066102
DI 10.1103/PhysRevLett.111.066102
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196TJ
UT WOS:000322799200009
PM 23971592
ER
PT J
AU Li, KY
Eres, G
Howe, J
Chuang, YJ
Li, XF
Gu, ZJ
Zhang, LT
Xie, SS
Pan, ZW
AF Li, Kaiyuan
Eres, Gyula
Howe, Jane
Chuang, Yen-Jun
Li, Xufan
Gu, Zhanjun
Zhang, Litong
Xie, Sishen
Pan, Zhengwei
TI Self-Assembly of Graphene on Carbon Nanotube Surfaces
SO SCIENTIFIC REPORTS
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; PYROLYTIC CARBON; LARGE-AREA; FILMS;
NANORIBBONS; MECHANISMS; GRAPHITE; GROWTH
AB The rolling up of a graphene sheet into a tube is a standard visualization tool for illustrating carbon nanotube (CNT) formation. However, the actual processes of rolling up graphene sheets into CNTs in laboratory syntheses have never been demonstrated. Here we report conformal growth of graphene by carbon self-assembly on single-wall and multi-wall CNTs using chemical vapor deposition (CVD) of methane without the presence of metal catalysts. The new graphene layers roll up into seamless coaxial cylinders encapsulating the existing CNTs, but their adhesion to the primary CNTs is weak due to the existence of lattice misorientation. Our study shows that graphene nucleation and growth by self-assembly of carbon on the inactive carbon basal plane of CNTs occurs by a new mechanism that is markedly different from epitaxial growth on metal surfaces, opening up the possibility of graphene growth on many other non-metal substrates by simple methane CVD.
C1 [Li, Kaiyuan; Chuang, Yen-Jun; Li, Xufan; Gu, Zhanjun; Pan, Zhengwei] Univ Georgia, Coll Engn, Athens, GA 30602 USA.
[Li, Kaiyuan; Chuang, Yen-Jun; Li, Xufan; Gu, Zhanjun; Pan, Zhengwei] Univ Georgia, Dept Phys & Astron, Athens, GA 30602 USA.
[Li, Kaiyuan; Zhang, Litong] Northwestern Polytech Univ, Sci & Technol Thermostruct Composite Mat Lab, Xian 710072, Shaanxi, Peoples R China.
[Eres, Gyula; Howe, Jane] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
[Gu, Zhanjun] Chinese Acad Sci, Inst High Energy Phys, Lab Bioenvironm Effects Nanomat & Nanosafety, Beijing 100049, Peoples R China.
[Xie, Sishen] Chinese Acad Sci, Inst Phys, Beijing 100080, Peoples R China.
RP Eres, G (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
EM eresg@ornl.gov; panz@uga.edu
RI Gu, Zhanjun/A-7592-2013; Li, Xufan/A-8292-2013; Eres, Gyula/C-4656-2017;
OI Gu, Zhanjun/0000-0003-3717-2423; Li, Xufan/0000-0001-9814-0383; Eres,
Gyula/0000-0003-2690-5214; Pan, Zhengwei/0000-0002-3854-958X
FU U.S. NSF [CAREER DMR-0955908]; China Scholarship Council; Materials
Sciences and Engineering Division, Office of Basic Energy Science, U.S.
Department of Energy; National Basic Research Programs of China (973
program) [2012CB932504]; Oak Ridge National Laboratory's Shared Research
Equipment (ShaRE) User Program; Scientific User Facilities Division of
the Office of Basic Energy Science
FX Z.W.P. acknowledges funding by U.S. NSF (CAREER DMR-0955908). K.Y.L.
thanks the financial support from the China Scholarship Council. G.E.
acknowledges funding by the Materials Sciences and Engineering Division,
Office of Basic Energy Science, U.S. Department of Energy. Z.J.G.
acknowledges support by the National Basic Research Programs of China
(973 program, No. 2012CB932504). The microscopy work was sponsored by
Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User
Program, which is sponsored by the Scientific User Facilities Division
of the Office of Basic Energy Science.
NR 31
TC 6
Z9 6
U1 2
U2 145
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2045-2322
J9 SCI REP-UK
JI Sci Rep
PD AUG 5
PY 2013
VL 3
AR 2353
DI 10.1038/srep02353
PG 4
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 195JR
UT WOS:000322698700003
PM 23912638
ER
PT J
AU Shvedova, AA
Yanamala, N
Murray, AR
Kisin, ER
Khaliullin, T
Hatfield, MK
Tkach, AV
Krantz, QT
Nash, D
King, C
Gilmour, MI
Gavett, SH
AF Shvedova, Anna A.
Yanamala, Naveena
Murray, Ashley R.
Kisin, Elena R.
Khaliullin, Timur
Hatfield, Meghan K.
Tkach, Alexey V.
Krantz, Q. T.
Nash, David
King, Charly
Gilmour, M. Ian
Gavett, Stephen H.
TI OXIDATIVE STRESS, INFLAMMATORY BIOMARKERS, AND TOXICITY IN MOUSE LUNG
AND LIVER AFTER INHALATION EXPOSURE TO 100% BIODIESEL OR PETROLEUM
DIESEL EMISSIONS
SO JOURNAL OF TOXICOLOGY AND ENVIRONMENTAL HEALTH-PART A-CURRENT ISSUES
LA English
DT Article
ID FAILURE-PRONE RATS; EXHAUST INHALATION; ENGINE EXHAUST; PARTICLES;
PARTICULATE; OILS; ACROLEIN; IMPACT; CELLS; FUEL
AB Over the past decade, soy biodiesel (BD) has become a first alternative energy source that is economically viable and meets requirements of the Clean Air Act. Due to lower mass emissions and reduced hazardous compounds compared to diesel combustion emissions (CE), BD exposure is proposed to produce fewer adverse health effects. However, considering the broad use of BD and its blends in different industries, this assertion needs to be supported and validated by mechanistic and toxicological data. Here, adverse effects were compared in lungs and liver of BALB/cJ mice after inhalation exposure (0, 50, 150, or 500 g/m(3); 4 h/d, 5 d/wk, for 4 wk) to CE from 100% biodiesel (B100) and diesel (D100). Compared to D100, B100 CE produced a significant accumulation of oxidatively modified proteins (carbonyls), an increase in 4-hydroxynonenal (4-HNE), a reduction of protein thiols, a depletion of antioxidant gluthatione (GSH), a dose-related rise in the levels of biomarkers of tissue damage (lactate dehydrogenase, LDH) in lungs, and inflammation (myeloperoxidase, MPO) in both lungs and liver. Significant differences in the levels of inflammatory cytokines interleukin (IL)-6, IL-10, IL-12p70, monocyte chemoattractant protein (MCP)-1, interferon (IFN) , and tumor necrosis factor (TNF)- were detected in lungs and liver upon B100 and D100 CE exposures. Overall, the tissue damage, oxidative stress, inflammation, and cytokine response were more pronounced in mice exposed to BD CE. Further studies are required to understand what combustion products in BD CE accelerate oxidative and inflammatory responses.
C1 [Shvedova, Anna A.; Yanamala, Naveena; Murray, Ashley R.; Kisin, Elena R.; Khaliullin, Timur; Hatfield, Meghan K.; Tkach, Alexey V.] NIOSH, Hlth Effects Lab Div, Pathol & Physiol Res Branch, Morgantown, WV USA.
[Shvedova, Anna A.; Murray, Ashley R.] W Virginia Univ, Sch Med, Dept Physiol & Pharmacol, Morgantown, WV 26506 USA.
[Krantz, Q. T.; King, Charly; Gilmour, M. Ian; Gavett, Stephen H.] US EPA, Environm Publ Hlth Div, Natl Hlth & Environm Effects Res Lab, Durham, NC USA.
[Nash, David] ORISE, Oak Ridge, TN USA.
[Nash, David] US EPA, Natl Risk Management Res Lab, Res Triangle Pk, NC 27711 USA.
RP Shvedova, AA (reprint author), Pathol & Physiol Res Branch MS 2015, 1095 Willowdale Rd, Morgantown, WV 26505 USA.
EM ats1@cdc.gov
FU NIOSH [2927ZKCY]
FX The authors are grateful to Bill Linak (U.S. EPA) for assistance in
inhalation engineering and to Mary Daniels and Liz Boykin (U.S. EPA) for
laboratory work. They also thank Dr. Vince Castranova and Dr. Teh-hsun
B. Chen (CDC/NIOSH/HELD) and Dr. Mark Higuchi (U.S. EPA) for their
discussion, comments, and feedback. This work was supported by NIOSH,
2927ZKCY.
NR 53
TC 17
Z9 17
U1 0
U2 11
PU TAYLOR & FRANCIS INC
PI PHILADELPHIA
PA 325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA
SN 1528-7394
EI 1087-2620
J9 J TOXICOL ENV HEAL A
JI J. Toxicol. Env. Health Part A
PD AUG 3
PY 2013
VL 76
IS 15
BP 907
EP 921
DI 10.1080/15287394.2013.825217
PG 15
WC Environmental Sciences; Public, Environmental & Occupational Health;
Toxicology
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Toxicology
GA 240BK
UT WOS:000326069500002
PM 24156694
ER
PT J
AU Modreanu, M
Durand, O
Jellison, GE
Salviati, G
Fried, M
AF Modreanu, Mircea
Durand, Olivier
Jellison, Gerald E.
Salviati, Giancarlo
Fried, Miklos
TI Special issue on "Current Trends in Optical and X-Ray Metrology of
Advanced Materials for Nanoscale Devices III", E-MRS Spring
2012-Symposium W, held in Strasbourg, France, May 14-18, 2012
SO THIN SOLID FILMS
LA English
DT Editorial Material
C1 [Modreanu, Mircea] Natl Univ Ireland Univ Coll Cork, Tyndall Natl Inst, Cork, Ireland.
[Durand, Olivier] Univ Europeenne Bretagne, FOTON OHM, UMR CNRS 6082, INSA Rennes, Bretagne, France.
[Jellison, Gerald E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN USA.
[Salviati, Giancarlo] Univ Parma, CNR, I-43100 Parma, Italy.
RP Modreanu, M (reprint author), Natl Univ Ireland Univ Coll Cork, Tyndall Natl Inst, Cork, Ireland.
RI Modreanu, Mircea/A-7181-2008; Salviati, Giancarlo/F-4947-2016
OI Modreanu, Mircea/0000-0003-0334-2439; Salviati,
Giancarlo/0000-0002-9828-6371
NR 0
TC 0
Z9 0
U1 0
U2 10
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0040-6090
J9 THIN SOLID FILMS
JI Thin Solid Films
PD AUG 3
PY 2013
VL 541
SI SI
BP 1
EP 2
DI 10.1016/j.tsf.2013.07.027
PG 2
WC Materials Science, Multidisciplinary; Materials Science, Coatings &
Films; Physics, Applied; Physics, Condensed Matter
SC Materials Science; Physics
GA 201KN
UT WOS:000323140600001
ER
PT J
AU Bonanno, PL
Gautier, S
El Gmili, Y
Moudakir, T
Sirenko, AA
Kazimirov, A
Cai, ZH
Martin, J
Goh, WH
Martinez, A
Ramdane, A
Le Gratiet, L
Maloufi, N
Assouar, MB
Ougazzaden, A
AF Bonanno, P. L.
Gautier, S.
El Gmili, Y.
Moudakir, T.
Sirenko, A. A.
Kazimirov, A.
Cai, Z-H.
Martin, J.
Goh, W. H.
Martinez, A.
Ramdane, A.
Le Gratiet, L.
Maloufi, N.
Assouar, M. B.
Ougazzaden, A.
TI Nondestructive mapping of chemical composition and structural qualities
of group III-nitride nanowires using submicron beam synchrotron-based
X-ray diffraction
SO THIN SOLID FILMS
LA English
DT Article; Proceedings Paper
CT Symposium W on Current Trends in Optical and X-Ray Metrology of Advanced
Materials for Nanoscale Devices III / Spring Meeting of the
European-Materials-Research-Society (E-MRS)
CY MAY 14-18, 2012
CL Strasbourg, FRANCE
SP European Mat Res Soc (E MRS), Hinds Instruments Inc, Horiba
DE Nondestructive; GaN; Synchrotron; X-ray diffraction; Nano; Nanowire;
RSM; MQW
ID QUANTUM DOTS; GROWTH
AB Submicron beam synchrotron-based X-ray diffraction (XRD) techniques have been developed and used to accurately and nondestructively map chemical composition and material quality of selectively grown group nanowires. GaN, AlGaN, and InGaN multi-quantum-well nanowires have been selectively grown on lattice matched and mismatched substrates, and the challenges associated with obtaining and interpreting submicron beam XRD results are addressed and solved. Nanoscale cathodoluminescence is used to examine exciton behavior, and energy-dispersive X-ray spectroscopy is used to verify chemical composition. Scanning transmission electron microscopy is later used to paint a more complete picture. The advantages of submicron beam XRD over other techniques are discussed in the context of this challenging material system. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Bonanno, P. L.; Goh, W. H.; Ougazzaden, A.] UMI 2958 Georgia Tech CNRS, Georgia Inst Technol GTL, F-57070 Metz, France.
[Gautier, S.; Martin, J.] Univ Metz, UMR CNRS 7132, LMOPS UMI Lab Mat Opt Photon & Micronano Syst, F-57070 Metz, France.
[Gautier, S.; Martin, J.] SUPELEC, F-57070 Metz, France.
[Gautier, S.; El Gmili, Y.; Moudakir, T.; Martin, J.] UMI 2958 Georgia Tech CNRS, F-57070 Metz, France.
[Sirenko, A. A.] New Jersey Inst Technol, Dept Phys, Newark, NJ 07102 USA.
[Kazimirov, A.] Cornell Univ, CHESS, Ithaca, NY 14853 USA.
[Cai, Z-H.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Martinez, A.; Ramdane, A.; Le Gratiet, L.] UPR CNRS 20, Lab Photon & Nanostruct, F-91460 Marcoussis, France.
[Maloufi, N.] Lab Etud Textures & Applicat Mat UMR CNRS 7078 Il, F-57045 Metz 1, France.
[Assouar, M. B.] Nancy Univ, CNRS, Lab Phys Milieux Ionises & Applicat, F-54506 Vandoeuvre Les Nancy, France.
RP Bonanno, PL (reprint author), UMI 2958 Georgia Tech CNRS, Georgia Inst Technol GTL, F-57070 Metz, France.
EM plb2@njit.edu
RI Assouar, Badreddine/A-7849-2011
OI Assouar, Badreddine/0000-0002-5823-3320
NR 14
TC 1
Z9 1
U1 0
U2 38
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0040-6090
J9 THIN SOLID FILMS
JI Thin Solid Films
PD AUG 3
PY 2013
VL 541
SI SI
BP 46
EP 50
DI 10.1016/j.tsf.2012.12.099
PG 5
WC Materials Science, Multidisciplinary; Materials Science, Coatings &
Films; Physics, Applied; Physics, Condensed Matter
SC Materials Science; Physics
GA 201KN
UT WOS:000323140600011
ER
PT J
AU Aithal, SM
AF Aithal, S. M.
TI Prediction of Voltage Signature in a Homogeneous Charge Compression
Ignition (HCCI) Engine Fueled with Propane and Acetylene
SO COMBUSTION SCIENCE AND TECHNOLOGY
LA English
DT Article
DE Alternative fuels; Charged species; Equilibrium; Equivalence ratio; HCCI
engine; Ionization
ID COMBUSTION; REDUCTION; NOX
AB Ion sensors work on the principle that the ion current in a combusting mixture is proportional to the electrical conductivity of the mixture. Ion sensors can thus provide direct in-cylinder combustion information to the engine controller in order to optimize engine performance and reduce emissions. Electrical conductivity of the combusting mixture depends on the mixture composition (fuel and equivalence ratio) along with the temperature and pressure. A previously developed equilibrium chemistry model consisting of 20 neutral species and seven charged species was shown to correctly predict the temporal variation of current in a constant-volume, spark-ignited methane/air mixture in a constant volume chamber, for various air/fuel ratios. The current study explores the use of this equilibrium chemistry model for predicting the voltage signatures in a homogeneous charge compression ignition (HCCI) engine fueled with alternative fuels such as propane and acetylene operating at low temperatures and equivalence ratios. Temporal variation of the current signal is compared with experimental data for various equivalence ratios for propane and acetylene. The contribution of various charged species to the current signal is also analyzed. It was seen that the equilibrium chemistry model captures the experimentally observed voltage signal trends correctly for both propane and acetylene for a range of equivalence ratios. The ability of the model to correctly correlate the voltage signal with equivalence ratio for various fuels shows its potential for diagnostics and control of next-generation engines.
C1 Argonne Natl Lab, Argonne, IL 60439 USA.
RP Aithal, SM (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM aithal@mcs.anl.gov
FU Office of Science, U.S. Department of Energy [DE-AC02-06CH11357]; U.S.
Department of Energy Office of Science laboratory [DE-AC02-06CH11357];
U.S. Government
FX This work was supported by the Office of Science, U.S. Department of
Energy, under Contract No. DE-AC02-06CH11357.; The submitted manuscript
has been created by UChicago Argonne, LLC, Operator of Argonne National
Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of
Science laboratory, is operated under Contract No. DE-AC02-06CH11357.
The U.S. Government retains for itself, and others acting on its behalf,
a paid-up nonexclusive, irrevocable worldwide license in said article to
reproduce, prepare derivative works, distribute copies to the public,
and perform publicly and display publicly, by or on behalf of the
Government.
NR 26
TC 4
Z9 4
U1 0
U2 10
PU TAYLOR & FRANCIS INC
PI PHILADELPHIA
PA 325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA
SN 0010-2202
J9 COMBUST SCI TECHNOL
JI Combust. Sci. Technol.
PD AUG 3
PY 2013
VL 185
IS 8
BP 1184
EP 1201
DI 10.1080/00102202.2013.781593
PG 18
WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary;
Engineering, Chemical
SC Thermodynamics; Energy & Fuels; Engineering
GA 188SG
UT WOS:000322213300003
ER
PT J
AU Breshears, DD
Adams, HD
Eamus, D
McDowell, NG
Law, DJ
Will, RE
Williams, AP
Zou, CB
AF Breshears, David D.
Adams, Henry D.
Eamus, Derek
McDowell, Nate G.
Law, Darin J.
Will, Rodney E.
Williams, A. Park
Zou, Chris B.
TI The critical amplifying role of increasing atmospheric moisture demand
on tree mortality and associated regional die-off
SO FRONTIERS IN PLANT SCIENCE
LA English
DT Editorial Material
ID CHANGE-TYPE DROUGHT; VEGETATION MORTALITY; CARBON METABOLISM;
UNITED-STATES; CLIMATE; MECHANISMS; TEMPERATURE; CONDUCTANCE; RESPONSES;
DYNAMICS
C1 [Breshears, David D.; Law, Darin J.] Univ Arizona, Sch Nat Resources & Environm, Tucson, AZ 85721 USA.
[Breshears, David D.] Univ Arizona, Dept Ecol & Evolutionary Biol, Tucson, AZ USA.
[Adams, Henry D.; McDowell, Nate G.; Williams, A. Park] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA.
[Eamus, Derek] Univ Technol Sydney, Sch Environm, Sydney, NSW 2007, Australia.
[Will, Rodney E.; Zou, Chris B.] Oklahoma State Univ, Dept Nat Resource Ecol & Management, Stillwater, OK 74078 USA.
RP Law, DJ (reprint author), Univ Arizona, Sch Nat Resources & Environm, Tucson, AZ 85721 USA.
EM dlaw@email.arizona.edu
RI Adams, Henry/A-8742-2010; Will, Rodney/G-8111-2011; Williams,
Park/B-8214-2016; Zou, Chris/A-5039-2010;
OI Adams, Henry/0000-0002-6403-5304; Williams, Park/0000-0001-8176-8166;
Zou, Chris/0000-0003-0080-2866; Eamus, Derek/0000-0003-2765-8040
NR 38
TC 30
Z9 30
U1 5
U2 57
PU FRONTIERS RESEARCH FOUNDATION
PI LAUSANNE
PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND
SN 1664-462X
J9 FRONT PLANT SCI
JI Front. Plant Sci.
PD AUG 2
PY 2013
VL 4
AR 266
DI 10.3389/fpls.2013.00266
PG 4
WC Plant Sciences
SC Plant Sciences
GA AA0DJ
UT WOS:000330765000001
PM 23935600
ER
PT J
AU Riley, LM
Weadge, JT
Baker, P
Robinson, H
Codee, JDC
Tipton, PA
Ohman, DE
Howell, PL
AF Riley, Laura M.
Weadge, Joel T.
Baker, Perrin
Robinson, Howard
Codee, Jeroen D. C.
Tipton, Peter A.
Ohman, Dennis E.
Howell, P. Lynne
TI Structural and Functional Characterization of Pseudomonas aeruginosa
AlgX ROLE OF AlgX IN ALGINATE ACETYLATION
SO JOURNAL OF BIOLOGICAL CHEMISTRY
LA English
DT Article
ID BIOSYNTHETIC GENE-CLUSTER; CARBOHYDRATE-BINDING MODULES; GRAM-NEGATIVE
BACTERIA; BIOFILM FORMATION; ACETYLPEPTIDOGLYCAN ESTERASE; EVOLUTIONARY
CONSERVATION; NEISSERIA-GONORRHOEAE; INDUCED DISPERSION;
PROTEIN-STRUCTURE; CYSTIC-FIBROSIS
AB The exopolysaccharide alginate, produced by mucoid Pseudomonas aeruginosa in the lungs of cystic fibrosis patients, undergoes two different chemical modifications as it is synthesized that alter the properties of the polymer and hence the biofilm. One modification, acetylation, causes the cells in the biofilm to adhere better to lung epithelium, form microcolonies, and resist the effects of the host immune system and/or antibiotics. Alginate biosynthesis requires 12 proteins encoded by the algD operon, including AlgX, and although this protein is essential for polymer production, its exact role is unknown. In this study, we present the X-ray crystal structure of AlgX at 2.15 angstrom resolution. The structure reveals that AlgX is a two-domain protein, with an N-terminal domain with structural homology to members of the SGNH hydrolase superfamily and a C-terminal carbohydrate-binding module. A number of residues in the carbohydrate-binding module form a substrate recognition "pinch point" that we propose aids in alginate binding and orientation. Although the topology of the N-terminal domain deviates from canonical SGNH hydrolases, the residues that constitute the Ser-His-Asp catalytic triad characteristic of this family are structurally conserved. In vivo studies reveal that site-specific mutation of these residues results in non-acetylated alginate. This catalytic triad is also required for acetylesterase activity in vitro. Our data suggest that not only does AlgX protect the polymer as it passages through the periplasm but that it also plays a role in alginate acetylation. Our results provide the first structural insight for a wide group of closely related bacterial polysaccharide acetyltransferases.
C1 [Howell, P. Lynne] Hosp Sick Children, Program Mol Struct & Funct, Toronto, ON M5G 1X8, Canada.
[Robinson, Howard] Brookhaven Natl Lab, Photon Sci Div, Upton, NY 11973 USA.
[Codee, Jeroen D. C.] Leiden Univ, Leiden Inst Chem, NL-2300 RA Leiden, Netherlands.
[Tipton, Peter A.] Univ Missouri, Dept Biochem, Columbia, MO 65211 USA.
[Ohman, Dennis E.] Virginia Commonwealth Univ, Med Ctr, Dept Microbiol & Immunol, Richmond, VA 23298 USA.
[Ohman, Dennis E.] Virginia Commonwealth Univ, Med Ctr, McGuire Vet Affairs Med Ctr, Richmond, VA 23298 USA.
[Howell, P. Lynne] Univ Toronto, Dept Biochem, Toronto, ON M5S 1A8, Canada.
RP Howell, PL (reprint author), Hosp Sick Children, Program Mol Struct & Funct, 555 Univ Ave, Toronto, ON M5G 1X8, Canada.
EM howell@sickkids.ca
FU United States Department of Energy Office of Biological and
Environmental Research; National Institutes of Health National Center
for Research Resources
FX We thank Yura Lobsanov, Francis Wolfram, Dustin J. Little, Jason Koo,
John C. C. Whitney, and G. David Smith for helpful discussions and
Patrick Yip for technical assistance. National Synchrotron Light Source
beamline X29 is supported by the United States Department of Energy
Office of Biological and Environmental Research and the National
Institutes of Health National Center for Research Resources.
NR 94
TC 15
Z9 18
U1 3
U2 19
PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC
PI BETHESDA
PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA
SN 0021-9258
EI 1083-351X
J9 J BIOL CHEM
JI J. Biol. Chem.
PD AUG 2
PY 2013
VL 288
IS 31
BP 22299
EP 22314
DI 10.1074/jbc.M113.484931
PG 16
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 302HY
UT WOS:000330596300012
PM 23779107
ER
PT J
AU Glockner, C
Kern, J
Broser, M
Zouni, A
Yachandra, V
Yano, J
AF Gloeckner, Carina
Kern, Jan
Broser, Matthias
Zouni, Athina
Yachandra, Vittal
Yano, Junko
TI Structural Changes of the Oxygen-evolving Complex in Photosystem II
during the Catalytic Cycle
SO JOURNAL OF BIOLOGICAL CHEMISTRY
LA English
DT Article
ID X-RAY-ABSORPTION; PHOTOSYNTHETIC WATER OXIDATION; MN4CA CLUSTER;
CRYSTAL-STRUCTURE; MN CLUSTER; MANGANESE COMPLEX; ELECTRONIC-STRUCTURE;
S-2 STATES; THERMOSYNECHOCOCCUS-ELONGATUS; ANGSTROM RESOLUTION
AB The oxygen-evolving complex (OEC) in the membrane-bound protein complex photosystem II (PSII) catalyzes the water oxidation reaction that takes place in oxygenic photosynthetic organisms. We investigated the structural changes of the Mn4CaO5 cluster in the OEC during the S state transitions using x-ray absorption spectroscopy (XAS). Overall structural changes of the Mn4CaO5 cluster, based on the manganese ligand and Mn-Mn distances obtained from this study, were incorporated into the geometry of the Mn4CaO5 cluster in the OEC obtained from a polarized XAS model and the 1.9-angstrom high resolution crystal structure. Additionally, we compared the S-1 state XAS of the dimeric and monomeric form of PSII from Thermosynechococcus elongatus and spinach PSII. Although the basic structures of the OEC are the same for T. elongatus PSII and spinach PSII, minor electronic structural differences that affect the manganese K-edge XAS between T. elongatus PSII and spinach PSII are found and may originate from differences in the second sphere ligand atom geometry.
C1 [Gloeckner, Carina; Broser, Matthias; Zouni, Athina] Tech Univ Berlin, Inst Chem, Max Volmer Lab Biophys Chem, D-10623 Berlin, Germany.
[Kern, Jan; Yachandra, Vittal; Yano, Junko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
RP Zouni, A (reprint author), Tech Univ Berlin, Inst Chem, Max Volmer Lab Biophys Chem, Str 17 Juni 135, D-10623 Berlin, Germany.
EM zouni@mailbox.tu-berlin.de; vkyachandra@lbl.gov; jyano@lbl.gov
RI Kern, Jan/G-2586-2013
OI Kern, Jan/0000-0002-7272-1603
FU National Institutes of Health; NCCR; Department of Energy, Office of
Biological and Environmental Research
FX We thank Prof. Johannes Messinger for many useful discussions, D.
DiFiore for technical assistance with sample preparation and the staff
at Stanford Synchrotron Radiation Lightsource, Stanford, CA, for support
of the EXAFS measurements. Synchrotron facilities were provided by the
Stanford Synchrotron Radiation Lightsource operated by the Department of
Energy, Office of Basic Energy Sciences. The Stanford Synchrotron
Radiation Lightsource Biomedical Technology program is supported by the
National Institutes of Health, the NCCR, and the Department of Energy,
Office of Biological and Environmental Research.
NR 74
TC 52
Z9 53
U1 6
U2 60
PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC
PI BETHESDA
PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA
SN 0021-9258
EI 1083-351X
J9 J BIOL CHEM
JI J. Biol. Chem.
PD AUG 2
PY 2013
VL 288
IS 31
BP 22607
EP 22620
DI 10.1074/jbc.M113.476622
PG 14
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 302HY
UT WOS:000330596300041
PM 23766513
ER
PT J
AU Chavan, H
Khan, MMT
Tegos, G
Krishnamurthy, P
AF Chavan, Hemantkumar
Khan, Mohiuddin Md Taimur
Tegos, George
Krishnamurthy, Partha
TI Efficient Purification and Reconstitution of ATP Binding Cassette
Transporter B6 (ABCB6) for Functional and Structural Studies
SO JOURNAL OF BIOLOGICAL CHEMISTRY
LA English
DT Article
ID GLYCOPROTEIN MULTIDRUG TRANSPORTER; P-GLYCOPROTEIN;
HEPATOCELLULAR-CARCINOMA; LIPID FLIPPASE; MECHANISM; EXPRESSION;
PROTEOLIPOSOMES; RESISTANCE; LOCALIZES; MUTATIONS
AB The mitochondrial ATP binding cassette transporter ABCB6 has been associated with a broad range of physiological functions, including growth and development, therapy-related drug resistance, and the new blood group system Langereis. ABCB6 has been proposed to regulate heme synthesis by shuttling coproporphyrinogen III from the cytoplasm into the mitochondria. However, direct functional information of the transport complex is not known. To understand the role of ABCB6 in mitochondrial transport, we developed an in vitro system with pure and active protein. ABCB6 overexpressed in HEK293 cells was solubilized from mitochondrial membranes and purified to homogeneity. Purified ABCB6 showed a high binding affinity for MgATP (K-d = 0.18 mu M) and an ATPase activity with a K-m of 0.99 mM. Reconstitution of ABCB6 into liposomes allowed biochemical characterization of the ATPase including (i) substrate-stimulated ATPase activity, (ii) transport kinetics of its proposed endogenous substrate coproporphyrinogen III, and (iii) transport kinetics of substrates identified using a high throughput screening assay. Mutagenesis of the conserved lysine to alanine (K629A) in the Walker A motif abolished ATP hydrolysis and substrate transport. These results suggest a direct interaction between mitochondrial ABCB6 and its transport substrates that is critical for the activity of the transporter. Furthermore, the simple immunoaffinity purification of ABCB6 to near homogeneity and efficient reconstitution of ABCB6 into liposomes might provide the basis for future studies on the structure/function of ABCB6.
C1 [Chavan, Hemantkumar; Krishnamurthy, Partha] Univ Kansas, Med Ctr, Dept Pharmacol Toxicol & Therapeut, Kansas City, KS 66160 USA.
[Khan, Mohiuddin Md Taimur] Washington State Univ, Dept Chem Engn & Bioengn, Pullman, WA 99146 USA.
[Khan, Mohiuddin Md Taimur] Pacific NW Natl Lab, Div Bioenergy & Biotechnol, Richland, WA 99352 USA.
[Tegos, George] Univ New Mexico, Ctr Mol Discovery, Albuquerque, NM 87131 USA.
[Tegos, George] Univ New Mexico, Sch Med, Albuquerque, NM 87131 USA.
[Chavan, Hemantkumar; Krishnamurthy, Partha] Massachusetts Gen Hosp, Wellman Ctr Photomed, Boston, MA 02114 USA.
[Tegos, George] Harvard Univ, Sch Med, Dept Dermatol, Boston, MA 02114 USA.
RP Krishnamurthy, P (reprint author), Univ Kansas, Med Ctr, Dept Pharmacol Toxicol & Therapeut, 3901 Rainbow Blvd, Kansas City, KS 66160 USA.
EM pkasturi@kumc.edu
OI Chavan, Hemantkumar/0000-0002-9963-6230
FU National Institutes of Health [P20RR021940, R03MH093193]
FX This work was supported, in whole or in part, by National Institutes of
Health Grants P20RR021940 and R03MH093193.
NR 50
TC 9
Z9 10
U1 0
U2 10
PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC
PI BETHESDA
PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA
SN 0021-9258
EI 1083-351X
J9 J BIOL CHEM
JI J. Biol. Chem.
PD AUG 2
PY 2013
VL 288
IS 31
BP 22658
EP 22669
DI 10.1074/jbc.M113.485284
PG 12
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 302HY
UT WOS:000330596300045
PM 23792964
ER
PT J
AU Grant, CD
Kang, SO
Hay, BP
AF Grant, Christopher D.
Kang, Sung Ok
Hay, Benjamin P.
TI Synthesis of a Hydrophilic Naphthalimidedioxime
SO JOURNAL OF ORGANIC CHEMISTRY
LA English
DT Article
ID TRANSFER HYDROGENATION; REDUCTIVE AMINATION; ACID-DERIVATIVES;
CONVENIENT
AB Imidedioximes are formed in hydroxylamine-treated polyacrylonitrile adsorbents used in the extraction of uranium from seawater. Although known to be a good uranophile, the glutarimidedioxime model compound 1 is rapidly hydrolyzed under acidic conditions used to elute metals from the adsorbent. This work reports the synthesis of a hydrophilic naphthalimidedioxime derivative 14, which is stable under acidic elution conditions. The synthesis starts from simple acenaphthenequinone 7 and converts it to a functional group dense imidedioxime 14 in 7 steps.
C1 [Grant, Christopher D.; Kang, Sung Ok; Hay, Benjamin P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
RP Hay, BP (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
EM haybp@ornl.gov
FU Fuel Resources Campaign in the Fuel Cycle Research and Development
Program, Office of Nuclear Energy, U.S. Department of Energy (DOE)
FX This work was supported by the Fuel Resources Campaign in the Fuel Cycle
Research and Development Program, Office of Nuclear Energy, U.S.
Department of Energy (DOE).
NR 20
TC 6
Z9 6
U1 1
U2 25
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0022-3263
EI 1520-6904
J9 J ORG CHEM
JI J. Org. Chem.
PD AUG 2
PY 2013
VL 78
IS 15
BP 7735
EP 7740
DI 10.1021/jo4009386
PG 6
WC Chemistry, Organic
SC Chemistry
GA 197LQ
UT WOS:000322853100037
PM 23786218
ER
PT J
AU Gudavalli, RKP
Katsenovich, YP
Wellman, DM
Idarraga, M
Lagos, LE
Tansel, B
AF Gudavalli, Ravi K. P.
Katsenovich, Yelena P.
Wellman, Dawn M.
Idarraga, Melina
Lagos, Leonel E.
Tansel, Berrin
TI Comparison of the kinetic rate law parameters for the dissolution of
natural and synthetic autunite in the presence of aqueous bicarbonate
ions
SO CHEMICAL GEOLOGY
LA English
DT Article
DE Autunite; Dissolution; Uranium; Activation energy; Enthalpy; Bicarbonate
ID CRYSTAL-STRUCTURE; COMPLEX-FORMATION; META-AUTUNITE; CARBONATE; URANIUM;
URANYL; MINERALS; PH; TEMPERATURE; CHEMISTRY
AB This research evaluated the effect of aqueous hydrogen carbonate solutions on the uranium rate of release from natural Ca-autunite and quantified the process kinetic rate law for a better prediction of the stability of autunite-group minerals. Testing was accomplished via a single-pass flow-through (SPFT) apparatus using buffered aqueous bicarbonate solutions (0.0005 to 0.003 M) at temperatures of 23-90 degrees C and pH values of 7-11. The release rate of uranium from Ca-autunite was directly correlated to increasing concentrations of hydrogen carbonate solutions and showed strong pH dependency. Ca-autunite kinetic rate law parameters were compared to the values obtained for synthetic Na-autunite. The power law coefficient and intrinsic rate constant were higher at pH 9-11 for Ca-autunite than for Na-autunite. The lower stability of Ca-autunite was attributed to the high Ca-autunite surface cracking, fractures and basal plane cleavages as compared to Na-autunite and the combined effect of the formation of aqueous uranyl-carbonate and calcium uranyl carbonate species as a driving force for uranium(VI) detachment and the formation of secondary Ca-P hydroxyapatite and uranyl phosphate mineral phases as a driving force for phosphate and calcium detachment controlling the net release of elements. Published by Elsevier B.V.
C1 [Gudavalli, Ravi K. P.; Katsenovich, Yelena P.; Idarraga, Melina; Lagos, Leonel E.] Florida Int Univ, Appl Res Ctr, Miami, FL 33174 USA.
[Gudavalli, Ravi K. P.; Tansel, Berrin] Florida Int Univ, Dept Civil & Environm Engn, Miami, FL 33174 USA.
[Wellman, Dawn M.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Katsenovich, YP (reprint author), Florida Int Univ, Appl Res Ctr, 10555 W Flagler St,Suite 2100, Miami, FL 33174 USA.
EM katsenov@fiu.edu
FU U.S. Department of Energy Office of Environmental Management
[DE-EM0000598]; Department of Energy (DOE) [DE-AC05-76RL01830]
FX Funding for this work was provided by the U.S. Department of Energy
Office of Environmental Management under grant DE-EM0000598. This
manuscript was prepared in collaboration with the Deep Vadose Zone -
Applied Field Research Initiative at the Pacific Northwest National
Laboratory. The Pacific Northwest National Laboratory is operated by
Battelle Memorial Institute for the Department of Energy (DOE) under
Contract DE-AC05-76RL01830. We gratefully acknowledge the efforts of K.
Parker from Pacific Northwest National Laboratory for his help with the
surface area analysis of synthetic autunite; and A. Henao for his
assistance in conducting KPA and ICP-OES analysis. The authors also
acknowledge Dr. Y. Liu from the FIU Advanced Materials Engineering
Research Institute (AMERI) and R. Lapierre and T. Beasley from FCAEM for
their assistance with the SEM/EDS analysis.
NR 45
TC 1
Z9 1
U1 0
U2 18
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0009-2541
J9 CHEM GEOL
JI Chem. Geol.
PD AUG 2
PY 2013
VL 351
BP 299
EP 309
DI 10.1016/j.chemgeo.2013.05.038
PG 11
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 197NI
UT WOS:000322857500024
ER
PT J
AU Aguilar-Arevalo, AA
Brown, BC
Bugel, L
Cheng, G
Church, ED
Conrad, JM
Dharmapalan, R
Djurcic, Z
Finley, DA
Ford, R
Garcia, FG
Garvey, GT
Grange, J
Huelsnitz, W
Ignarra, C
Imlay, R
Johnson, RA
Karagiorgi, G
Katori, T
Kobilarcik, T
Louis, WC
Mariani, C
Marsh, W
Mills, GB
Mirabal, J
Moore, CD
Mousseau, J
Nienaber, P
Osmanov, B
Pavlovic, Z
Perevalov, D
Polly, CC
Ray, H
Roe, BP
Russell, AD
Shaevitz, MH
Spitz, J
Stancu, I
Tayloe, R
Van de Water, RG
Wascko, MO
White, DH
Wickremasinghe, DA
Zeller, GP
Zimmerman, ED
AF Aguilar-Arevalo, A. A.
Brown, B. C.
Bugel, L.
Cheng, G.
Church, E. D.
Conrad, J. M.
Dharmapalan, R.
Djurcic, Z.
Finley, D. A.
Ford, R.
Garcia, F. G.
Garvey, G. T.
Grange, J.
Huelsnitz, W.
Ignarra, C.
Imlay, R.
Johnson, R. A.
Karagiorgi, G.
Katori, T.
Kobilarcik, T.
Louis, W. C.
Mariani, C.
Marsh, W.
Mills, G. B.
Mirabal, J.
Moore, C. D.
Mousseau, J.
Nienaber, P.
Osmanov, B.
Pavlovic, Z.
Perevalov, D.
Polly, C. C.
Ray, H.
Roe, B. P.
Russell, A. D.
Shaevitz, M. H.
Spitz, J.
Stancu, I.
Tayloe, R.
Van de Water, R. G.
Wascko, M. O.
White, D. H.
Wickremasinghe, D. A.
Zeller, G. P.
Zimmerman, E. D.
CA MiniBooNE Collaboration
TI First measurement of the muon antineutrino double-differential
charged-current quasielastic cross section
SO PHYSICAL REVIEW D
LA English
DT Article
ID ELECTRON-SCATTERING; PION ABSORPTION; NEGATIVE MUONS; CAPTURE RATES;
NEUTRINO; MINIBOONE; DETECTOR; STATES; SIMULATION; RESONANCE
AB The largest sample ever recorded of (nu) over bar (mu) charged-current quasielastic (CCQE, (nu) over bar (mu) + p -> mu(+) + n) candidate events is used to produce the minimally model-dependent, flux-integrated double-differential cross section d(2)sigma/dT(mu) d cos theta(mu) for (nu) over bar (mu) CCQE for a mineral oil target. This measurement exploits the large statistics of the MiniBooNE antineutrino mode sample and provides the most complete information of this process to date. In order to facilitate historical comparisons, the flux-unfolded total cross section sigma(E-nu) and single-differential cross section d sigma/dQ(2) on both mineral oil and on carbon are also reported. The observed cross section is somewhat higher than the predicted cross section from a model assuming independently acting nucleons in carbon with canonical form factor values. The shape of the data are also discrepant with this model. These results have implications for intranuclear processes and can help constrain signal and background processes for future neutrino oscillation measurements.
C1 [Dharmapalan, R.; Stancu, I.] Univ Alabama, Tuscaloosa, AL 35487 USA.
[Djurcic, Z.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Johnson, R. A.; Wickremasinghe, D. A.] Univ Cincinnati, Cincinnati, OH 45221 USA.
[Zimmerman, E. D.] Univ Colorado, Boulder, CO 80309 USA.
[Cheng, G.; Karagiorgi, G.; Shaevitz, M. H.] Columbia Univ, New York, NY 10027 USA.
[Brown, B. C.; Finley, D. A.; Ford, R.; Garcia, F. G.; Kobilarcik, T.; Marsh, W.; Moore, C. D.; Perevalov, D.; Polly, C. C.; Russell, A. D.; Zeller, G. P.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Grange, J.; Mousseau, J.; Osmanov, B.; Ray, H.] Univ Florida, Gainesville, FL 32611 USA.
[Tayloe, R.] Indiana Univ, Bloomington, IN 47405 USA.
[Garvey, G. T.; Huelsnitz, W.; Louis, W. C.; Mills, G. B.; Mirabal, J.; Pavlovic, Z.; Van de Water, R. G.; White, D. H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Imlay, R.] Louisiana State Univ, Baton Rouge, LA 70803 USA.
[Bugel, L.; Conrad, J. M.; Ignarra, C.; Katori, T.; Spitz, J.] MIT, Cambridge, MA 02139 USA.
[Aguilar-Arevalo, A. A.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico.
[Roe, B. P.] Univ Michigan, Ann Arbor, MI 48109 USA.
[Nienaber, P.] St Marys Univ Minnesota, Winona, MN 55987 USA.
[Church, E. D.] Yale Univ, New Haven, CT 06520 USA.
[Mariani, C.] Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA 24061 USA.
[Wascko, M. O.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England.
RP Aguilar-Arevalo, AA (reprint author), Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico.
RI Mariani, Camillo/J-6070-2015;
OI Mariani, Camillo/0000-0003-3284-4681; Louis,
William/0000-0002-7579-3709; Aguilar-Arevalo, Alexis
A./0000-0001-9279-3375; Spitz, Joshua/0000-0002-6288-7028; Wascko,
Morgan/0000-0002-8348-4447; Van de Water, Richard/0000-0002-1573-327X;
Katori, Teppei/0000-0002-9429-9482
NR 84
TC 71
Z9 71
U1 1
U2 5
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1550-7998
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 2
PY 2013
VL 88
IS 3
AR 032001
DI 10.1103/PhysRevD.88.032001
PG 31
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 196LU
UT WOS:000322777800001
ER
PT J
AU Gando, A
Gando, Y
Hanakago, H
Ikeda, H
Inoue, K
Ishidoshiro, K
Ishikawa, H
Koga, M
Matsuda, R
Matsuda, S
Mitsui, T
Motoki, D
Nakamura, K
Obata, A
Oki, A
Oki, Y
Otani, M
Shimizu, I
Shirai, J
Suzuki, A
Takemoto, Y
Tamae, K
Ueshima, K
Watanabe, H
Xu, BD
Yamada, S
Yamauchi, Y
Yoshida, H
Kozlov, A
Yoshida, S
Piepke, A
Banks, TI
Fujikawa, BK
Han, K
O'Donnell, T
Berger, BE
Learned, JG
Matsuno, S
Sakai, M
Efremenko, Y
Karwowski, HJ
Markoff, DM
Tornow, W
Detwiler, JA
Enomoto, S
Decowski, MP
AF Gando, A.
Gando, Y.
Hanakago, H.
Ikeda, H.
Inoue, K.
Ishidoshiro, K.
Ishikawa, H.
Koga, M.
Matsuda, R.
Matsuda, S.
Mitsui, T.
Motoki, D.
Nakamura, K.
Obata, A.
Oki, A.
Oki, Y.
Otani, M.
Shimizu, I.
Shirai, J.
Suzuki, A.
Takemoto, Y.
Tamae, K.
Ueshima, K.
Watanabe, H.
Xu, B. D.
Yamada, S.
Yamauchi, Y.
Yoshida, H.
Kozlov, A.
Yoshida, S.
Piepke, A.
Banks, T. I.
Fujikawa, B. K.
Han, K.
O'Donnell, T.
Berger, B. E.
Learned, J. G.
Matsuno, S.
Sakai, M.
Efremenko, Y.
Karwowski, H. J.
Markoff, D. M.
Tornow, W.
Detwiler, J. A.
Enomoto, S.
Decowski, M. P.
CA KamLAND Collaboration
TI Reactor on-off antineutrino measurement with KamLAND
SO PHYSICAL REVIEW D
LA English
DT Article
ID NEUTRON FISSION-PRODUCTS; GEO-NEUTRINOS; EARTH; FLUX; SPECTRUM; MODELS
AB The recent long-term shutdown of Japanese nuclear reactors has resulted in a significantly reduced reactor (nu) over bar (e) flux at KamLAND. This running condition provides a unique opportunity to confirm and constrain backgrounds for the reactor (nu) over bar (e) oscillation analysis. The data set also has improved sensitivity for other (nu) over bar (e) signals, in particular (nu) over bar (e)'s produced in beta-decays from U-238 and Th-232 within the Earth's interior, whose energy spectrum overlaps with that of reactor (nu) over bar (e)'s. Including constraints on theta(13) from accelerator and short-baseline reactor neutrino experiments, a combined three-flavor analysis of solar and KamLAND data gives fit values for the oscillation parameters of tan (2)theta(12) = 0.436(-0.025)(+0.029), Delta m(21)(2) = 7.53(-0.18)(+0.18) x 10(-5) eV(2), and sin (2)theta(13) = 0.023(-0.002)(+0.002). Assuming a chondritic Th/U mass ratio, we obtain 116(-27)(+28) (nu) over bar (e) events from U-238 and Th-232, corresponding to a geo (nu) over bar (e) flux of 3.4(-0.8)(+0.8) x 10(6) cm(-2) s(-1) at the KamLAND location. We evaluate various bulk silicate Earth composition models using the observed geo (nu) over bar (e) rate.
C1 [Gando, A.; Gando, Y.; Hanakago, H.; Ikeda, H.; Inoue, K.; Ishidoshiro, K.; Ishikawa, H.; Koga, M.; Matsuda, R.; Matsuda, S.; Mitsui, T.; Motoki, D.; Nakamura, K.; Obata, A.; Oki, A.; Oki, Y.; Otani, M.; Shimizu, I.; Shirai, J.; Suzuki, A.; Takemoto, Y.; Tamae, K.; Ueshima, K.; Watanabe, H.; Xu, B. D.; Yamada, S.; Yamauchi, Y.; Yoshida, H.] Tohoku Univ, Res Ctr Neutrino Sci, Sendai, Miyagi 9808578, Japan.
[Inoue, K.; Koga, M.; Nakamura, K.; Kozlov, A.; Piepke, A.; Fujikawa, B. K.; Berger, B. E.; Efremenko, Y.; Tornow, W.; Enomoto, S.; Decowski, M. P.] Univ Tokyo, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan.
[Yoshida, S.] Osaka Univ, Grad Sch Sci, Toyonaka, Osaka 5600043, Japan.
[Piepke, A.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA.
[Banks, T. I.; Fujikawa, B. K.; Han, K.; O'Donnell, T.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Banks, T. I.; Fujikawa, B. K.; Han, K.; O'Donnell, T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Berger, B. E.] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA.
[Learned, J. G.; Matsuno, S.; Sakai, M.] Univ Hawaii Manoa, Dept Phys & Astron, Honolulu, HI 96822 USA.
[Efremenko, Y.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
[Karwowski, H. J.; Markoff, D. M.; Tornow, W.] Triangle Univ Nucl Lab, Durham, NC 27708 USA.
[Karwowski, H. J.; Markoff, D. M.; Tornow, W.] Duke Univ, Dept Phys, Durham, NC 27705 USA.
[Karwowski, H. J.; Markoff, D. M.; Tornow, W.] N Carolina Cent Univ, Durham, NC 27701 USA.
[Karwowski, H. J.; Markoff, D. M.; Tornow, W.] Univ N Carolina, Chapel Hill, NC 27599 USA.
[Detwiler, J. A.; Enomoto, S.] Univ Washington, Ctr Expt Nucl Phys & Astrophys, Seattle, WA 98195 USA.
[Decowski, M. P.] Nikhef, NL-1019 XG Amsterdam, Netherlands.
[Decowski, M. P.] Univ Amsterdam, NL-1019 XG Amsterdam, Netherlands.
RP Gando, A (reprint author), Tohoku Univ, Res Ctr Neutrino Sci, Sendai, Miyagi 9808578, Japan.
RI Han, Ke/D-3697-2017
OI Han, Ke/0000-0002-1609-7367
FU Japanese Ministry of Education, Culture, Sports, Science and Technology
[21000001]; World Premier International Research Center Initiative (WPI
Initiative), MEXT, Japan; Stichting FOM in the Netherlands; US
Department of Energy (DOE) [DE-AC02-05CH11231]
FX The KamLAND experiment is supported by the Grant-in-Aid for Specially
Promoted Research under Grant No. 21000001 of the Japanese Ministry of
Education, Culture, Sports, Science and Technology; the World Premier
International Research Center Initiative (WPI Initiative), MEXT, Japan;
Stichting FOM in the Netherlands; and under the US Department of Energy
(DOE) Grant No. DE-AC02-05CH11231, as well as other DOE grants to
individual institutions. The Kamioka Mining and Smelting Company has
provided service for activities in the mine.
NR 38
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U1 2
U2 15
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1550-7998
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 2
PY 2013
VL 88
IS 3
AR 033001
DI 10.1103/PhysRevD.88.033001
PG 10
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 196LU
UT WOS:000322777800002
ER
PT J
AU Li, JZ
Ma, YQ
Chao, KT
AF Li, Jin-Zhao
Ma, Yan-Qing
Chao, Kuang-Ta
TI QCD and relativistic O(alpha(s)v(2)) corrections to hadronic decays of
spin-singlet heavy quarkonia h(c), h(b) and eta(b)
SO PHYSICAL REVIEW D
LA English
DT Article
ID P-1(1) STATE; PARTON DISTRIBUTIONS; CHARMONIUM; AMPLITUDES
AB We calculate the annihilation decay widths of spin-singlet heavy quarkonia h(c), h(b) and eta(b) into light hadrons with both QCD and relativistic corrections at order O(alpha(s)v(2)) in nonrelativistic QCD. With appropriate estimates for the long-distance matrix elements by using the potential model and operator evolution method, we find that our predictions of these decay widths are consistent with recent experimental measurements. We also find that the O(alpha(s)v(2)) corrections are small for b (b) over bar states but substantial for c (c) over bar states. In particular, the negative contribution of O(alpha(s)v(2)) correction to the h(c) decay can lower the decay width, as compared with previous predictions without the O(alpha(s)v(2)) correction, and thus result in a good agreement with the recent BESIII measurement.
C1 [Li, Jin-Zhao; Chao, Kuang-Ta] Peking Univ, Dept Phys, Beijing 100871, Peoples R China.
[Li, Jin-Zhao; Chao, Kuang-Ta] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China.
[Ma, Yan-Qing] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
[Chao, Kuang-Ta] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China.
RP Li, JZ (reprint author), Peking Univ, Dept Phys, Beijing 100871, Peoples R China.
EM lijinzhao86@gmail.com; yqma@bnl.gov; ktchao@pku.edu.cn
FU National Natural Science Foundation of China [11021092, 11075002];
Ministry of Science and Technology of China [2009CB825200]; U.S.
Department of Energy [DE-AC02-98CH10886]
FX We are grateful to B. Q. Li, C. Meng, J. W. Qiu, and M. Stratmann for
many helpful discussions. This work was supported in part by the
National Natural Science Foundation of China (No. 11021092 and No.
11075002), and the Ministry of Science and Technology of China (No.
2009CB825200). Y. Q. M is supported by the U.S. Department of Energy,
Contract No. DE-AC02-98CH10886.
NR 46
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PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 2470-0010
EI 2470-0029
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 2
PY 2013
VL 88
IS 3
AR 034002
DI 10.1103/PhysRevD.88.034002
PG 15
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 196LU
UT WOS:000322777800005
ER
PT J
AU Adamczyk, L
Adkins, JK
Agakishiev, G
Aggarwal, MM
Ahammed, Z
Alekseev, I
Alford, J
Anson, CD
Aparin, A
Arkhipkin, D
Aschenauer, E
Averichev, GS
Balewski, J
Banerjee, A
Barnovska, Z
Beavis, DR
Bellwied, R
Betancourt, MJ
Betts, RR
Bhasin, A
Bhati, AK
Bhattarai, P
Bichsel, H
Bielcik, J
Bielcikova, J
Bland, LC
Bordyuzhin, IG
Borowski, W
Bouchet, J
Brandin, AV
Brovko, SG
Bruna, E
Bultmann, S
Bunzarov, I
Burton, TP
Butterworth, J
Cai, XZ
Caines, H
Sanchez, MCD
Cebra, D
Cendejas, R
Cervantes, MC
Chaloupka, P
Chang, Z
Chattopadhyay, S
Chen, HF
Chen, JH
Chen, JY
Chen, L
Cheng, J
Cherney, M
Chikanian, A
Christie, W
Chung, P
Chwastowski, J
Codrington, MJM
Corliss, R
Cramer, JG
Crawford, HJ
Cui, X
Das, S
Leyva, AD
De Silva, LC
Debbe, RR
Dedovich, TG
Deng, J
de Souza, RD
Dhamija, S
Di Ruzza, B
Didenko, L
Ding, F
Dion, A
Djawotho, P
Dong, X
Drachenberg, JL
Draper, JE
Du, CM
Dunkelberger, LE
Dunlop, JC
Efimov, LG
Elnimr, M
Engelage, J
Eppley, G
Eun, L
Evdokimov, O
Fatemi, R
Fazio, S
Fedorisin, J
Fersch, RG
Filip, P
Finch, E
Fisyak, Y
Flores, E
Gagliardi, CA
Gangadharan, DR
Garand, D
Geurts, F
Gibson, A
Gliske, S
Grebenyuk, OG
Grosnick, D
Gupta, A
Gupta, S
Guryn, W
Haag, B
Hajkova, O
Hamed, A
Han, LX
Harris, JW
Hays-Wehle, JP
Heppelmann, S
Hirsch, A
Hoffmann, GW
Hofman, DJ
Horvat, S
Huang, B
Huang, HZ
Huck, P
Humanic, TJ
Igo, G
Jacobs, WW
Jena, C
Judd, EG
Kabana, S
Kang, K
Kapitan, J
Kauder, K
Ke, HW
Keane, D
Kechechyan, A
Kesich, A
Kikola, DP
Kiryluk, J
Kisel, I
Kisiel, A
Klein, SR
Koetke, DD
Kollegger, T
Konzer, J
Koralt, I
Korsch, W
Kotchenda, L
Kravtsov, P
Krueger, K
Kulakov, I
Kumar, L
Lamont, MAC
Landgraf, JM
Landry, KD
LaPointe, S
Lauret, J
Lebedev, A
Lednicky, R
Lee, JH
Leight, W
LeVine, MJ
Li, C
Li, W
Li, X
Li, X
Li, Y
Li, ZM
Lima, LM
Lisa, MA
Liu, F
Ljubicic, T
Llope, WJ
Longacre, RS
Lu, Y
Luo, X
Luszczak, A
Ma, GL
Ma, YG
Don, DMMDM
Mahapatra, DP
Majka, R
Margetis, S
Markert, C
Masui, H
Matis, HS
McDonald, D
McShane, TS
Mioduszewski, S
Mitrovski, MK
Mohammed, Y
Mohanty, B
Mondal, MM
Munhoz, MG
Mustafa, MK
Naglis, M
Nandi, BK
Nasim, M
Nayak, TK
Nelson, JM
Nogach, LV
Novak, J
Odyniec, G
Ogawa, A
Oh, K
Ohlson, A
Okorokov, V
Oldag, EW
Oliveira, RAN
Olson, D
Pachr, M
Page, BS
Pal, SK
Pan, YX
Pandit, Y
Panebratsev, Y
Pawlak, T
Pawlik, B
Pei, H
Perkins, C
Peryt, W
Pile, P
Planinic, M
Pluta, J
Poljak, N
Porter, J
Poskanzer, AM
Powell, CB
Pruneau, C
Pruthi, NK
Przybycien, M
Pujahari, PR
Putschke, J
Qiu, H
Ramachandran, S
Raniwala, R
Raniwala, S
Ray, RL
Riley, CK
Ritter, HG
Roberts, JB
Rogachevskiy, OV
Romero, JL
Ross, JF
Ruan, L
Rusnak, J
Sahoo, NR
Sahu, PK
Sakrejda, I
Salur, S
Sandacz, A
Sandweiss, J
Sangaline, E
Sarkar, A
Schambach, J
Scharenberg, RP
Schmah, AM
Schmidke, B
Schmitz, N
Schuster, TR
Seger, J
Seyboth, P
Shah, N
Shahaliev, E
Shao, M
Sharma, B
Sharma, M
Shi, SS
Shou, QY
Sichtermann, EP
Singaraju, RN
Skoby, MJ
Smirnov, D
Smirnov, N
Solanki, D
Sorensen, P
Desouza, UG
Spinka, HM
Srivastava, B
Stanislaus, TDS
Stevens, JR
Stock, R
Strikhanov, M
Stringfellow, B
Suaide, AAP
Suarez, MC
Sumbera, M
Sun, XM
Sun, Y
Sun, Z
Surrow, B
Svirida, DN
Symons, TJM
de Toledo, AS
Takahashi, J
Tang, AH
Tang, Z
Tarini, LH
Tarnowsky, T
Thomas, JH
Tian, J
Timmins, AR
Tlusty, D
Tokarev, M
Trentalange, S
Tribble, RE
Tribedy, P
Trzeciak, BA
Tsai, OD
Turnau, J
Ullrich, T
Underwood, DG
Van Buren, G
Van Nieuwenhuizen, G
Vanfossen, JA
Varma, R
Vasconcelos, GMS
Videbaek, F
Viyogi, YP
Vokal, S
Voloshin, SA
Vossen, A
Wada, M
Wang, F
Wang, G
Wang, H
Wang, JS
Wang, Q
Wang, XL
Wang, Y
Webb, G
Webb, JC
Westfall, GD
Whitten, C
Wieman, H
Wissink, SW
Witt, R
Wu, YF
Xiao, Z
Xie, W
Xin, K
Xu, H
Xu, N
Xu, QH
Xu, W
Xu, Y
Xu, Z
Xue, L
Yang, Y
Yang, Y
Yepes, P
Yi, L
Yip, K
Yoo, IK
Zawisza, M
Zbroszczyk, H
Zhang, JB
Zhang, S
Zhang, XP
Zhang, Y
Zhang, ZP
Zhao, F
Zhao, J
Zhong, C
Zhu, X
Zhu, YH
Zoulkarneeva, Y
Zyzak, M
AF Adamczyk, L.
Adkins, J. K.
Agakishiev, G.
Aggarwal, M. M.
Ahammed, Z.
Alekseev, I.
Alford, J.
Anson, C. D.
Aparin, A.
Arkhipkin, D.
Aschenauer, E.
Averichev, G. S.
Balewski, J.
Banerjee, A.
Barnovska, Z.
Beavis, D. R.
Bellwied, R.
Betancourt, M. J.
Betts, R. R.
Bhasin, A.
Bhati, A. K.
Bhattarai, P.
Bichsel, H.
Bielcik, J.
Bielcikova, J.
Bland, L. C.
Bordyuzhin, I. G.
Borowski, W.
Bouchet, J.
Brandin, A. V.
Brovko, S. G.
Bruna, E.
Bueltmann, S.
Bunzarov, I.
Burton, T. P.
Butterworth, J.
Cai, X. Z.
Caines, H.
De la Barca Sanchez, M. Calderon
Cebra, D.
Cendejas, R.
Cervantes, M. C.
Chaloupka, P.
Chang, Z.
Chattopadhyay, S.
Chen, H. F.
Chen, J. H.
Chen, J. Y.
Chen, L.
Cheng, J.
Cherney, M.
Chikanian, A.
Christie, W.
Chung, P.
Chwastowski, J.
Codrington, M. J. M.
Corliss, R.
Cramer, J. G.
Crawford, H. J.
Cui, X.
Das, S.
Leyva, A. Davila
De Silva, L. C.
Debbe, R. R.
Dedovich, T. G.
Deng, J.
Derradi de Souza, R.
Dhamija, S.
di Ruzza, B.
Didenko, L.
Ding, F.
Dion, A.
Djawotho, P.
Dong, X.
Drachenberg, J. L.
Draper, J. E.
Du, C. M.
Dunkelberger, L. E.
Dunlop, J. C.
Efimov, L. G.
Elnimr, M.
Engelage, J.
Eppley, G.
Eun, L.
Evdokimov, O.
Fatemi, R.
Fazio, S.
Fedorisin, J.
Fersch, R. G.
Filip, P.
Finch, E.
Fisyak, Y.
Flores, E.
Gagliardi, C. A.
Gangadharan, D. R.
Garand, D.
Geurts, F.
Gibson, A.
Gliske, S.
Grebenyuk, O. G.
Grosnick, D.
Gupta, A.
Gupta, S.
Guryn, W.
Haag, B.
Hajkova, O.
Hamed, A.
Han, L-X.
Harris, J. W.
Hays-Wehle, J. P.
Heppelmann, S.
Hirsch, A.
Hoffmann, G. W.
Hofman, D. J.
Horvat, S.
Huang, B.
Huang, H. Z.
Huck, P.
Humanic, T. J.
Igo, G.
Jacobs, W. W.
Jena, C.
Judd, E. G.
Kabana, S.
Kang, K.
Kapitan, J.
Kauder, K.
Ke, H. W.
Keane, D.
Kechechyan, A.
Kesich, A.
Kikola, D. P.
Kiryluk, J.
Kisel, I.
Kisiel, A.
Klein, S. R.
Koetke, D. D.
Kollegger, T.
Konzer, J.
Koralt, I.
Korsch, W.
Kotchenda, L.
Kravtsov, P.
Krueger, K.
Kulakov, I.
Kumar, L.
Lamont, M. A. C.
Landgraf, J. M.
Landry, K. D.
LaPointe, S.
Lauret, J.
Lebedev, A.
Lednicky, R.
Lee, J. H.
Leight, W.
LeVine, M. J.
Li, C.
Li, W.
Li, X.
Li, X.
Li, Y.
Li, Z. M.
Lima, L. M.
Lisa, M. A.
Liu, F.
Ljubicic, T.
Llope, W. J.
Longacre, R. S.
Lu, Y.
Luo, X.
Luszczak, A.
Ma, G. L.
Ma, Y. G.
Don, D. M. M. D. Madagodagettige
Mahapatra, D. P.
Majka, R.
Margetis, S.
Markert, C.
Masui, H.
Matis, H. S.
McDonald, D.
McShane, T. S.
Mioduszewski, S.
Mitrovski, M. K.
Mohammed, Y.
Mohanty, B.
Mondal, M. M.
Munhoz, M. G.
Mustafa, M. K.
Naglis, M.
Nandi, B. K.
Nasim, Md.
Nayak, T. K.
Nelson, J. M.
Nogach, L. V.
Novak, J.
Odyniec, G.
Ogawa, A.
Oh, K.
Ohlson, A.
Okorokov, V.
Oldag, E. W.
Oliveira, R. A. N.
Olson, D.
Pachr, M.
Page, B. S.
Pal, S. K.
Pan, Y. X.
Pandit, Y.
Panebratsev, Y.
Pawlak, T.
Pawlik, B.
Pei, H.
Perkins, C.
Peryt, W.
Pile, P.
Planinic, M.
Pluta, J.
Poljak, N.
Porter, J.
Poskanzer, A. M.
Powell, C. B.
Pruneau, C.
Pruthi, N. K.
Przybycien, M.
Pujahari, P. R.
Putschke, J.
Qiu, H.
Ramachandran, S.
Raniwala, R.
Raniwala, S.
Ray, R. L.
Riley, C. K.
Ritter, H. G.
Roberts, J. B.
Rogachevskiy, O. V.
Romero, J. L.
Ross, J. F.
Ruan, L.
Rusnak, J.
Sahoo, N. R.
Sahu, P. K.
Sakrejda, I.
Salur, S.
Sandacz, A.
Sandweiss, J.
Sangaline, E.
Sarkar, A.
Schambach, J.
Scharenberg, R. P.
Schmah, A. M.
Schmidke, B.
Schmitz, N.
Schuster, T. R.
Seger, J.
Seyboth, P.
Shah, N.
Shahaliev, E.
Shao, M.
Sharma, B.
Sharma, M.
Shi, S. S.
Shou, Q. Y.
Sichtermann, E. P.
Singaraju, R. N.
Skoby, M. J.
Smirnov, D.
Smirnov, N.
Solanki, D.
Sorensen, P.
DeSouza, U. G.
Spinka, H. M.
Srivastava, B.
Stanislaus, T. D. S.
Stevens, J. R.
Stock, R.
Strikhanov, M.
Stringfellow, B.
Suaide, A. A. P.
Suarez, M. C.
Sumbera, M.
Sun, X. M.
Sun, Y.
Sun, Z.
Surrow, B.
Svirida, D. N.
Symons, T. J. M.
de Toledo, A. Szanto
Takahashi, J.
Tang, A. H.
Tang, Z.
Tarini, L. H.
Tarnowsky, T.
Thomas, J. H.
Tian, J.
Timmins, A. R.
Tlusty, D.
Tokarev, M.
Trentalange, S.
Tribble, R. E.
Tribedy, P.
Trzeciak, B. A.
Tsai, O. D.
Turnau, J.
Ullrich, T.
Underwood, D. G.
Van Buren, G.
Van Nieuwenhuizen, G.
Vanfossen, J. A., Jr.
Varma, R.
Vasconcelos, G. M. S.
Videbaek, F.
Viyogi, Y. P.
Vokal, S.
Voloshin, S. A.
Vossen, A.
Wada, M.
Wang, F.
Wang, G.
Wang, H.
Wang, J. S.
Wang, Q.
Wang, X. L.
Wang, Y.
Webb, G.
Webb, J. C.
Westfall, G. D.
Whitten, C., Jr.
Wieman, H.
Wissink, S. W.
Witt, R.
Wu, Y. F.
Xiao, Z.
Xie, W.
Xin, K.
Xu, H.
Xu, N.
Xu, Q. H.
Xu, W.
Xu, Y.
Xu, Z.
Xue, L.
Yang, Y.
Yang, Y.
Yepes, P.
Yi, L.
Yip, K.
Yoo, I-K.
Zawisza, M.
Zbroszczyk, H.
Zhang, J. B.
Zhang, S.
Zhang, X. P.
Zhang, Y.
Zhang, Z. P.
Zhao, F.
Zhao, J.
Zhong, C.
Zhu, X.
Zhu, Y. H.
Zoulkarneeva, Y.
Zyzak, M.
CA STAR Collaboration
TI Measurement of J/psi Azimuthal Anisotropy in Au plus Au Collisions at
root s(NN)=200 GeV
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID HEAVY-ION COLLISIONS; QUARK COALESCENCE; STAR; MODELS; FLOW
AB The measurement of J/psi azimuthal anisotropy is presented as a function of transverse momentum for different centralities in Au + Au collisions at root s(NN) = 200 GeV. The measured J/psi elliptic flow is consistent with zero within errors for transverse momentum between 2 and 10 GeV/c. Our measurement suggests that J/psi particles with relatively large transverse momenta are not dominantly produced by coalescence from thermalized charm quarks, when comparing to model calculations.
C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, Krakow, Poland.
[Gliske, S.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Nelson, J. M.] Univ Birmingham, Birmingham, W Midlands, England.
[Arkhipkin, D.; Aschenauer, E.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dion, A.; Dunlop, J. C.; Fazio, S.; Fisyak, Y.; Guryn, W.; Huang, B.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Mitrovski, M. K.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Wang, H.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Brovko, S. G.; De la Barca Sanchez, M. Calderon; Cebra, D.; Ding, F.; Draper, J. E.; Flores, E.; Haag, B.; Kesich, A.; Romero, J. L.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA.
[Dunkelberger, L. E.; Huang, H. Z.; Igo, G.; Landry, K. D.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Whitten, C., Jr.; Xu, W.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA.
[Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, Sao Paulo, Brazil.
[Chen, J. Y.; Chen, L.; Huck, P.; Ke, H. W.; Li, Z. M.; Liu, F.; Luo, X.; Shi, S. S.; Wu, Y. F.; Yang, Y.; Zhang, J. B.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China.
[Betts, R. R.; Evdokimov, O.; Hofman, D. J.; Kauder, K.; Pandit, Y.; Pei, H.; Suarez, M. C.] Univ Illinois, Chicago, IL 60607 USA.
[Chwastowski, J.; Luszczak, A.] Cracow Univ Technol, Krakow, Poland.
[Cherney, M.; Don, D. M. M. D. Madagodagettige; McShane, T. S.; Ross, J. F.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA.
[Bielcik, J.; Chaloupka, P.; Hajkova, O.; Pachr, M.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic.
[Barnovska, Z.; Bielcikova, J.; Chung, P.; Kapitan, J.; Rusnak, J.; Sumbera, M.; Tlusty, D.] Nucl Phys Inst CR, Rez 25068, Czech Republic.
[Kollegger, T.; Schuster, T. R.; Stock, R.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany.
[Das, S.; Mahapatra, D. P.; Sahu, P. K.] Inst Phys, Bhubaneswar 751005, Orissa, India.
[Nandi, B. K.; Pujahari, P. R.; Sarkar, A.; Varma, R.] Indian Inst Technol, Bombay 400076, Maharashtra, India.
[Dhamija, S.; Jacobs, W. W.; Page, B. S.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA.
[Alekseev, I.; Bordyuzhin, I. G.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow, Russia.
[Bhasin, A.; Gupta, A.; Gupta, S.] Univ Jammu, Jammu 180001, India.
[Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia.
[Alford, J.; Bouchet, J.; Keane, D.; Kumar, L.; Margetis, S.; Vanfossen, J. A., Jr.] Kent State Univ, Kent, OH 44242 USA.
[Adkins, J. K.; Fatemi, R.; Fersch, R. G.; Korsch, W.; Ramachandran, S.; Webb, G.] Univ Kentucky, Lexington, KY 40506 USA.
[Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.] Inst Modern Phys, Lanzhou, Peoples R China.
[Dong, X.; Eun, L.; Grebenyuk, O. G.; Kiryluk, J.; Kisel, I.; Klein, S. R.; Kulakov, I.; Masui, H.; Matis, H. S.; Naglis, M.; Odyniec, G.; Olson, D.; Porter, J.; Poskanzer, A. M.; Powell, C. B.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Sichtermann, E. P.; Sun, X. M.; Symons, T. J. M.; Thomas, J. H.; Wieman, H.; Xu, N.; Zyzak, M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Balewski, J.; Betancourt, M. J.; Corliss, R.; Hays-Wehle, J. P.; Leight, W.; Stevens, J. R.; Van Nieuwenhuizen, G.] MIT, Cambridge, MA 02139 USA.
[Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, Munich, Germany.
[Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA.
[Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia.
[Jena, C.; Mohanty, B.] Natl Inst Sci & Educ & Res, Bhubaneswar 751005, Orissa, India.
[Anson, C. D.; Gangadharan, D. R.; Humanic, T. J.; Lisa, M. A.] Ohio State Univ, Columbus, OH 43210 USA.
[Bueltmann, S.; Koralt, I.] Old Dominion Univ, Norfolk, VA 23529 USA.
[Pawlik, B.; Turnau, J.] Inst Nucl Phys PAN, Krakow, Poland.
[Aggarwal, M. M.; Bhati, A. K.; Pruthi, N. K.; Sharma, B.] Panjab Univ, Chandigarh 160014, India.
[Cendejas, R.; Heppelmann, S.] Penn State Univ, University Pk, PA 16802 USA.
[Nogach, L. V.] Inst High Energy Phys, Protvino, Russia.
[Garand, D.; Hirsch, A.; Kikola, D. P.; Konzer, J.; Li, X.; Mustafa, M. K.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Wang, Q.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA.
[Oh, K.; Yoo, I-K.] Pusan Natl Univ, Pusan 609735, South Korea.
[Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India.
[Butterworth, J.; Eppley, G.; Geurts, F.; Llope, W. J.; McDonald, D.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA.
[Lima, L. M.; Munhoz, M. G.; Oliveira, R. A. N.; DeSouza, U. G.; Suaide, A. A. P.; de Toledo, A. Szanto] Univ Sao Paulo, Sao Paulo, Brazil.
[Chen, H. F.; Cui, X.; Li, C.; Lu, Y.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Zhang, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China.
[Deng, J.; Xu, Q. H.] Shandong Univ, Jinan 250100, Shandong, Peoples R China.
[Cai, X. Z.; Chen, J. H.; Han, L-X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shou, Q. Y.; Tian, J.; Xue, L.; Zhang, S.; Zhao, J.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
[Borowski, W.; Kabana, S.] SUBATECH, Nantes, France.
[Li, X.; Surrow, B.] Temple Univ, Philadelphia, PA 19122 USA.
[Cervantes, M. C.; Chang, Z.; Djawotho, P.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mohammed, Y.; Mondal, M. M.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA.
[Bhattarai, P.; Codrington, M. J. M.; Leyva, A. Davila; Hoffmann, G. W.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA.
[Bellwied, R.; De Silva, L. C.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA.
[Cheng, J.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China.
[Witt, R.] US Naval Acad, Annapolis, MD 21402 USA.
[Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA.
[Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nasim, Md.; Nayak, T. K.; Pal, S. K.; Sahoo, N. R.; Singaraju, R. N.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India.
[Kisiel, A.; Pawlak, T.; Peryt, W.; Pluta, J.; Sandacz, A.; Trzeciak, B. A.; Zawisza, M.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland.
[Bichsel, H.; Cramer, J. G.] Univ Washington, Seattle, WA 98195 USA.
[Elnimr, M.; LaPointe, S.; Pruneau, C.; Putschke, J.; Sharma, M.; Tarini, L. H.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA.
[Bruna, E.; Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Horvat, S.; Majka, R.; Ohlson, A.; Riley, C. K.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA.
[Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia.
RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, Krakow, Poland.
RI Lednicky, Richard/K-4164-2013; Takahashi, Jun/B-2946-2012; Alekseev,
Igor/J-8070-2014; Sumbera, Michal/O-7497-2014; Strikhanov,
Mikhail/P-7393-2014; XIAO, Zhigang/C-3788-2015; Aparecido Negrao de
Oliveira, Renato/G-9133-2015; Tang, Zebo/A-9939-2014; Fazio, Salvatore
/G-5156-2010; Yang, Yanyun/B-9485-2014; Rusnak, Jan/G-8462-2014;
Bielcikova, Jana/G-9342-2014; Xu, Wenqin/H-7553-2014; Bruna,
Elena/C-4939-2014; Chaloupka, Petr/E-5965-2012; Huang,
Bingchu/H-6343-2015; Derradi de Souza, Rafael/M-4791-2013; Suaide,
Alexandre/L-6239-2016; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016;
Svirida, Dmitry/R-4909-2016; Inst. of Physics, Gleb
Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma,
Yu-Gang/M-8122-2013
OI Takahashi, Jun/0000-0002-4091-1779; Alekseev, Igor/0000-0003-3358-9635;
Sumbera, Michal/0000-0002-0639-7323; Strikhanov,
Mikhail/0000-0003-2586-0405; Tang, Zebo/0000-0002-4247-0081; Yang,
Yanyun/0000-0002-5982-1706; Xu, Wenqin/0000-0002-5976-4991; Bruna,
Elena/0000-0001-5427-1461; Huang, Bingchu/0000-0002-3253-3210; Derradi
de Souza, Rafael/0000-0002-2084-7001; Suaide,
Alexandre/0000-0003-2847-6556; Xin, Kefeng/0000-0003-4853-9219; Yi,
Li/0000-0002-7512-2657; Okorokov, Vitaly/0000-0002-7162-5345; Ma,
Yu-Gang/0000-0002-0233-9900
FU Office of NP within the U.S. DOE Office of Science; Office of HEP within
the U.S. DOE Office of Science; U.S. NSF; Sloan Foundation; CNRS/IN2P3;
FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian
Federation; NNSFC; CAS; MoST; MoE of China; GA of Czech Republic; FOM of
Netherlands; NWO of the Netherlands; DAE; DST; CSIR of India; Polish
Ministry of Science and Higher Education; National Research Foundation
[NRF-2012004024]; Ministry of Science, Education, and Sports of the
Republic of Croatia; RosAtom of Russia; RHIC Operations Group; RCF at
BNL; NERSC Center at LBNL; Open Science Grid consortium; MSMT of Czech
Republic
FX We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at
LBNL and the Open Science Grid consortium for providing resources and
support. This work was supported in part by the Offices of NP and HEP
within the U.S. DOE Office of Science, the U.S. NSF, the Sloan
Foundation; CNRS/IN2P3, FAPESP CNPq of Brazil; Ministry of Education and
Science of the Russian Federation; NNSFC, CAS, MoST, and MoE of China;
GA and MSMT of the Czech Republic; FOM and NWO of the Netherlands; DAE,
DST, and CSIR of India; Polish Ministry of Science and Higher Education;
National Research Foundation (NRF-2012004024), Ministry of Science,
Education, and Sports of the Republic of Croatia; and RosAtom of Russia.
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PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 2
PY 2013
VL 111
IS 5
AR 052301
DI 10.1103/PhysRevLett.111.052301
PG 7
WC Physics, Multidisciplinary
SC Physics
GA 196MM
UT WOS:000322779700006
PM 23952389
ER
PT J
AU Farhan, A
Derlet, PM
Kleibert, A
Balan, A
Chopdekar, RV
Wyss, M
Perron, J
Scholl, A
Nolting, F
Heyderman, LJ
AF Farhan, A.
Derlet, P. M.
Kleibert, A.
Balan, A.
Chopdekar, R. V.
Wyss, M.
Perron, J.
Scholl, A.
Nolting, F.
Heyderman, L. J.
TI Direct Observation of Thermal Relaxation in Artificial Spin Ice
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID FRUSTRATION
AB We study the thermal relaxation of artificial spin ice with photoemission electron microscopy, and are able to directly observe how such a system finds its way from an energetically excited state to the ground state. On plotting vertex-type populations as a function of time, we can characterize the relaxation, which occurs in two stages, namely a string and a domain regime. Kinetic Monte Carlo simulations agree well with the temporal evolution of the magnetic state when including disorder, and the experimental results can be explained by considering the effective interaction energy associated with the separation of pairs of vertex excitations.
C1 [Farhan, A.; Chopdekar, R. V.; Wyss, M.; Perron, J.; Heyderman, L. J.] Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.
[Farhan, A.; Perron, J.; Heyderman, L. J.] Swiss Fed Inst Technol, Dept Mat, Lab Mesoscop Syst, CH-8093 Zurich, Switzerland.
[Derlet, P. M.] Paul Scherrer Inst, NUM, Condensed Matter Theory Grp, CH-5232 Villigen, Switzerland.
[Kleibert, A.; Balan, A.; Chopdekar, R. V.; Nolting, F.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.
[Wyss, M.] Univ Basel, Swiss Nanosci Inst, CH-4056 Basel, Switzerland.
[Perron, J.] Univ Paris 06, Lab Chim Phys Matiere & Rayonnement UMR UPMC CNRS, F-75231 Paris 05, France.
[Scholl, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Farhan, A (reprint author), Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.
EM laura.heyderman@psi.ch
RI Chopdekar, Rajesh/D-2067-2009; Kleibert, Armin/P-6775-2014; Scholl,
Andreas/K-4876-2012; Heyderman, Laura/E-7959-2015; Farhan,
Alan/N-7288-2016
OI Chopdekar, Rajesh/0000-0001-6727-6501; Kleibert,
Armin/0000-0003-3630-9360; Farhan, Alan/0000-0002-2384-2249
FU Swiss National Science Foundation; Swiss Nanoscience Institute, Basel,
Switzerland
FX The authors would like to thank Juri Honegger for technical support.
This work was supported by the Swiss National Science Foundation and the
Swiss Nanoscience Institute, Basel, Switzerland. Part of this work was
performed at the Swiss Light Source, Paul Scherrer Institute, Villigen,
Switzerland and the Advanced Light Source, Lawrence Berkeley National
Laboratory (LBNL), Berkeley, California.
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J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 2
PY 2013
VL 111
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DI 10.1103/PhysRevLett.111.057204
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196MM
UT WOS:000322779700024
PM 23952441
ER
PT J
AU Sayre, DB
Brune, CR
Caggiano, JA
Glebov, VY
Hatarik, R
Bacher, AD
Bleuel, DL
Casey, DT
Cerjan, CJ
Eckart, MJ
Fortner, RJ
Frenje, JA
Friedrich, S
Gatu-Johnson, M
Grim, GP
Hagmann, C
Knauer, JP
Kline, JL
McNabb, DP
McNaney, JM
Mintz, JM
Moran, MJ
Nikroo, A
Phillips, T
Pino, JE
Remington, BA
Rowley, DP
Schneider, DH
Smalyuk, VA
Stoeffl, W
Tipton, RE
Weber, SV
Yeamans, CB
AF Sayre, D. B.
Brune, C. R.
Caggiano, J. A.
Glebov, V. Y.
Hatarik, R.
Bacher, A. D.
Bleuel, D. L.
Casey, D. T.
Cerjan, C. J.
Eckart, M. J.
Fortner, R. J.
Frenje, J. A.
Friedrich, S.
Gatu-Johnson, M.
Grim, G. P.
Hagmann, C.
Knauer, J. P.
Kline, J. L.
McNabb, D. P.
McNaney, J. M.
Mintz, J. M.
Moran, M. J.
Nikroo, A.
Phillips, T.
Pino, J. E.
Remington, B. A.
Rowley, D. P.
Schneider, D. H.
Smalyuk, V. A.
Stoeffl, W.
Tipton, R. E.
Weber, S. V.
Yeamans, C. B.
TI Measurement of the T plus T Neutron Spectrum Using the National Ignition
Facility
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID DECAY; SCATTERING; FUSION; T&T
AB Neutron time-of-flight spectra from inertial confinement fusion experiments with tritium-filled targets have been measured at the National Ignition Facility. These spectra represent a significant improvement in energy resolution and statistics over previous measurements, and afford the first definitive observation of a peak resulting from sequential decay through the ground state of He-5 at low reaction energies E-c.m. less than or similar to 100 keV. To describe the spectrum, we have developed an R-matrix model that accounts for interferences from fermion symmetry and intermediate states, and show these effects to be non-negligible. We also find the spectrum can be described by sequential decay through l = 1 states in He-5, which differs from previous interpretations.
C1 [Sayre, D. B.; Caggiano, J. A.; Hatarik, R.; Bleuel, D. L.; Casey, D. T.; Cerjan, C. J.; Eckart, M. J.; Fortner, R. J.; Friedrich, S.; Hagmann, C.; McNabb, D. P.; McNaney, J. M.; Mintz, J. M.; Moran, M. J.; Phillips, T.; Pino, J. E.; Remington, B. A.; Rowley, D. P.; Schneider, D. H.; Smalyuk, V. A.; Stoeffl, W.; Tipton, R. E.; Weber, S. V.; Yeamans, C. B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Brune, C. R.] Ohio Univ, Athens, OH 45701 USA.
[Glebov, V. Y.; Knauer, J. P.] Univ Rochester, Rochester, NY 14623 USA.
[Bacher, A. D.] Indiana Univ, Bloomington, IN 47405 USA.
[Frenje, J. A.; Gatu-Johnson, M.] MIT, Cambridge, MA 02139 USA.
[Grim, G. P.; Kline, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Nikroo, A.] Gen Atom Co, San Diego, CA 92121 USA.
RP Sayre, DB (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
EM sayre4@llnl.gov
RI Pino, Jesse/C-9183-2014;
OI Kline, John/0000-0002-2271-9919
FU Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]
FX We thank the operation teams at the National Ignition Facility and
Lawrence Livermore National Laboratory Tritium Facility for enabling the
current investigation. This work was performed under the auspices of
Lawrence Livermore National Security, LLC, under Contract No.
DE-AC52-07NA27344.
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J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 2
PY 2013
VL 111
IS 5
AR 052501
DI 10.1103/PhysRevLett.111.052501
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196MM
UT WOS:000322779700007
PM 23952390
ER
PT J
AU Yin, WG
Liu, X
Tsvelik, AM
Dean, MPM
Upton, MH
Kim, J
Casa, D
Said, A
Gog, T
Qi, TF
Cao, G
Hill, JP
AF Yin, Wei-Guo
Liu, X.
Tsvelik, A. M.
Dean, M. P. M.
Upton, M. H.
Kim, Jungho
Casa, D.
Said, A.
Gog, T.
Qi, T. F.
Cao, G.
Hill, J. P.
TI Ferromagnetic Exchange Anisotropy from Antiferromagnetic Superexchange
in the Mixed 3d-5d Transition-Metal Compound Sr3CuIrO6
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID MAGNETIC-PROPERTIES; CRYSTAL-STRUCTURE; EXCITATIONS; ORBITALS; OXIDES;
CHAIN
AB We report a combined experimental and theoretical study of the unusual ferromagnetism in the one-dimensional copper-iridium oxide Sr3CuIrO6. Utilizing Ir L-3 edge resonant inelastic x-ray scattering, we reveal a large gap magnetic excitation spectrum. We find that it is caused by an unusual exchange anisotropy generating mechanism, namely, strong ferromagnetic anisotropy arising from antiferromagnetic superexchange, driven by the alternating strong and weak spin-orbit coupling on the 5d Ir and 3d Cu magnetic ions, respectively. From symmetry consideration, this novel mechanism is generally present in systems with edge-sharing Cu2+O4 plaquettes and Ir4+O6 octahedra. Our results point to unusual magnetic behavior to be expected in mixed 3d - 5d transition-metal compounds via exchange pathways that are absent in pure 3d or 5d compounds.
C1 [Yin, Wei-Guo; Liu, X.; Tsvelik, A. M.; Dean, M. P. M.; Hill, J. P.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
[Liu, X.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.
[Liu, X.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.
[Upton, M. H.; Kim, Jungho; Casa, D.; Said, A.; Gog, T.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Qi, T. F.; Cao, G.] Univ Kentucky, Ctr Adv Mat, Lexington, KY 40506 USA.
[Qi, T. F.; Cao, G.] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA.
RP Yin, WG (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
EM wyin@bnl.gov
RI Dean, Mark/B-4541-2011; Qi, Tongfei/A-7226-2013; Casa,
Diego/F-9060-2016; Yin, Weiguo/A-9671-2014
OI Dean, Mark/0000-0001-5139-3543; Yin, Weiguo/0000-0002-4965-5329
FU U.S. Department of Energy (DOE), Division of Materials Science
[DE-AC02-98CH10886]; DOE, Office of Science, Office of Basic Energy
Sciences [DE-AC02-06CH11357]; NSF [DMR-0856234]
FX The work at Brookhaven National Laboratory was supported by the U.S.
Department of Energy (DOE), Division of Materials Science, under
Contract No. DE-AC02-98CH10886. Use of the Advanced Photon Source was
supported by DOE, Office of Science, Office of Basic Energy Sciences,
under Contract No. DE-AC02-06CH11357. T. F. Q. and G. C. were supported
by the NSF through Grant No. DMR-0856234.
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SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 2
PY 2013
VL 111
IS 5
AR 057202
DI 10.1103/PhysRevLett.111.057202
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196MM
UT WOS:000322779700022
PM 23952439
ER
PT J
AU McGrath, WJ
Graziano, V
Zabrocka, K
Mangel, WF
AF McGrath, William J.
Graziano, Vito
Zabrocka, Katarzyna
Mangel, Walter F.
TI First generation inhibitors of the adenovirus proteinase
SO FEBS LETTERS
LA English
DT Article
DE Adenovirus proteinase; Inhibitors; Structure-based drug design
ID 11-AMINO-ACID PEPTIDE COFACTOR; PROMISCUOUS INHIBITORS; SERINE
PROTEINASES; VIRAL PROTEINASES; ACID COFACTOR; AMINO-ACID; RESOLUTION;
RHODAMINE; MECHANISM; PROTEASE
AB As there are more than 50 adenovirus serotypes, the likelihood of developing an effective vaccine is low. Here we describe inhibitors of the adenovirus proteinase (AVP) with the ultimate objective of developing anti-adenovirus agents. Inhibitors were identified via structure-based drug design using as druggable sites the active site and a conserved cofactor pocket in the crystal structures of AVP. A lead compound was identified that had an IC50 of 18 mu M. One of eight structural derivatives of the lead compound had an IC50 of 140 nM against AVP and an IC50 of 490 nM against the AVP with its cofactor bound. (C) 2013 Federation of European Biochemical Societies. Published by Elsevier B.V. All rights reserved.
C1 [McGrath, William J.; Graziano, Vito; Zabrocka, Katarzyna; Mangel, Walter F.] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA.
RP Mangel, WF (reprint author), Brookhaven Natl Lab, Dept Biosci, 50 Bell Ave, Upton, NY 11973 USA.
EM mangel@bnl.gov
FU office of Biological and Environmental Research of the U.S. Department
of Energy [DE-AC0298CH10886]; Brookhaven National Laboratory; National
Institutes of Health [AI R0141599]; U.S. Department of Energy, Office of
Science, Office of Workforce Development for Teachers and Scientists
(WDTS) under the Science Undergraduate Laboratory Internship (SULI)
program
FX We thank Dr. R. Rizzo at Stony Brook University for access to his NCI
database formatted for use with DOCK and for helpful discussions. We
thank Jeff Aube at the University of Kansas for useful suggestions and
discussions. +Research supported by the office of Biological
and Environmental Research of the U.S. Department of Energy under Prime
Contract DE-AC0298CH10886 with Brookhaven National Laboratory and by
National Institutes of Health Grant AI R0141599 to W.F.M. K.Z. was
supported by the U.S. Department of Energy, Office of Science, Office of
Workforce Development for Teachers and Scientists (WDTS) under the
Science Undergraduate Laboratory Internship (SULI) program.
NR 25
TC 3
Z9 3
U1 0
U2 4
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0014-5793
J9 FEBS LETT
JI FEBS Lett.
PD AUG 2
PY 2013
VL 587
IS 15
BP 2332
EP 2339
DI 10.1016/j.febslet.2013.05.033
PG 8
WC Biochemistry & Molecular Biology; Biophysics; Cell Biology
SC Biochemistry & Molecular Biology; Biophysics; Cell Biology
GA 194BM
UT WOS:000322606000007
PM 23711373
ER
PT J
AU Czaplewski, DA
Holt, MV
Ocola, LE
AF Czaplewski, David A.
Holt, Martin V.
Ocola, Leonidas E.
TI The range and intensity of backscattered electrons for use in the
creation of high fidelity electron beam lithography patterns
SO NANOTECHNOLOGY
LA English
DT Article
ID SPIN QUBIT; SCATTERING; CRYSTAL; FABRICATION; MATTER; LIGHT
AB We present a set of universal curves that predict the range and intensity of backscattered electrons which can be used in conjunction with electron beam lithography to create high fidelity nanoscale patterns. The experimental method combines direct write dose, backscattered dose, and a self-reinforcing pattern geometry to measure the dose provided by backscattered electrons to a nanoscale volume on the substrate surface at various distances from the electron source. Electron beam lithography is used to precisely control the number and position of incident electrons on the surface of the material. Atomic force microscopy is used to measure the height of the negative electron beam lithography resist. Our data shows that the range and the intensity of backscattered electrons can be predicted using the density and the atomic number of any solid material, respectively. The data agrees with two independent Monte Carlo simulations without any fitting parameters. These measurements are the most accurate electron range measurements to date.
C1 [Czaplewski, David A.; Holt, Martin V.; Ocola, Leonidas E.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
RP Czaplewski, DA (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave Bldg 440, Argonne, IL 60439 USA.
OI Ocola, Leonidas/0000-0003-4990-1064
FU Center for Nanoscale Materials, a US Department of Energy, Office of
Science, Office of Basic Energy Sciences User Facility
[DE-AC02-06CH11357]
FX This work was performed at the Center for Nanoscale Materials, a US
Department of Energy, Office of Science, Office of Basic Energy Sciences
User Facility under Contract No. DE-AC02-06CH11357. The authors would
like to thank Tijana Rajh for discussions on the interaction of
radiation with matter. The authors would like to thank Tijana Rajh,
Alyssa Pasquale, and Daniel Lopez for help in constructing and editing
the manuscript.
NR 31
TC 5
Z9 5
U1 0
U2 19
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0957-4484
J9 NANOTECHNOLOGY
JI Nanotechnology
PD AUG 2
PY 2013
VL 24
IS 30
AR 305302
DI 10.1088/0957-4484/24/30/305302
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA 181WG
UT WOS:000321700100004
PM 23817998
ER
PT J
AU Stash, AI
Chen, YS
Kovalchukova, OV
Tsirelson, VG
AF Stash, A. I.
Chen, Yu-Sheng
Kovalchukova, O. V.
Tsirelson, V. G.
TI Electron density, electrostatic potential, and spatial organization of
ammonium hydrooxalate oxalic acid dihydrate heteromolecular crystal from
data of diffraction experiment at 15 K using synchrotron radiation and
theoretical calculations
SO RUSSIAN CHEMICAL BULLETIN
LA English
DT Article
DE electron density; chemical bond; electrostatic interaction
ID COVALENT BOND ORDERS; CHARGE-DENSITY; ENERGY; MOLECULES; COMPLEXES;
INSIGHTS; SALTS; ANION; DFT
AB A high-precision diffraction study at 15 K using synchrotron radiation and theoretical calculation of a heteromolecular crystal ammonium hydrooxalate oxalic acid dihydrate NH4 (+)center dot C2HO4 (-)center dot C2H2O4 center dot 2H(2)O (1) were carried out. The calculation was performed with the Kohn-Sham method taking into account periodic boundary conditions. The joint experimental and theoretical study allowed one to locate positions of hydrogen atoms and to reliably establish peculiar features of the electron density and electrostatic potential distributions in 1. Interatomic and molecular interactions were characterized based on the electron density properties within the framework of a quantum topological theory. The bond order indices were calculated from the experimental electron density without using the orbital notions. A new approach based on visualization of the ellipsoids whose semiaxes depend on the principal values of the electron density curvature at the bond critical points was used. It was found that charge transfer between ammonium cation and hydrooxalate anion in 1 dominates other electrostatic interactions in the crystal. Based on analysis of peculiar features of the electron density and electrostatic potential distributions in the crystal of 1, it was found that spatial organization of the crystal in hand is also governed by one more, weaker, electrostatic factor that originated from the presence of well-localized regions behind protons on the extensions of the lines of covalent bonds at the periphery of the molecules. In those regions, the electrostatic potential is higher than in other directions due to anisotropy of the electron density distribution. This feature mainly ensures directed complementary electrostatic interaction between corresponding fragments with negatively charged regions of neighboring molecules, such as the lone electron pairs and p-electrons.
C1 [Stash, A. I.] L Ya Karpov Phys & Chem Res Inst, Moscow 105064, Russia.
[Chen, Yu-Sheng] Univ Chicago, Adv Photon Source, ChemMatCARS Beamline, Argonne, IL 60439 USA.
[Kovalchukova, O. V.] Peoples Friendship Univ Russia, Moscow 117198, Russia.
[Tsirelson, V. G.] DI Mendeleev Univ Chem Technol Russia, Moscow 125047, Russia.
RP Tsirelson, VG (reprint author), DI Mendeleev Univ Chem Technol Russia, 9 Miusskaya Pl, Moscow 125047, Russia.
EM astas@yandex.ru; yschen@cars.uchicago.edu; okovalchukova@mail.ru;
tsirel@muctr.ru
FU Russian Foundation for Basic Research [13-03-00767-a]; US Department of
Energy, Office of Science, Office of Basic Energy Sciences
[DE-AC02-06CH11357]; National Science Foundation/US Department of Energy
[NSF/CHE-0822838]
FX This work was financially supported by the Russian Foundation for Basic
Research (Project No. 13-03-00767-a). Use of the Advanced Photon Source
was financially supported by the US Department of Energy, Office of
Science, Office of Basic Energy Sciences, under Contract No.
DE-AC02-06CH11357. ChemMatCARS Sector 15 is principally supported by the
National Science Foundation/US Department of Energy under Grant No.
NSF/CHE-0822838.
NR 55
TC 4
Z9 4
U1 3
U2 10
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1066-5285
EI 1573-9171
J9 RUSS CHEM B+
JI Russ. Chem. Bull.
PD AUG
PY 2013
VL 62
IS 8
BP 1752
EP 1763
DI 10.1007/s11172-013-0252-5
PG 12
WC Chemistry, Multidisciplinary
SC Chemistry
GA AG3PI
UT WOS:000335331400007
ER
PT J
AU Feng, Q
Blythe, HJ
Jiang, FX
Xu, XH
Heald, SM
Fox, AM
Gehring, GA
AF Feng, Qi
Blythe, Harry J.
Jiang, Feng-Xian
Xu, Xiao-Hong
Heald, Steve M.
Fox, A. Mark
Gehring, Gillian A.
TI Contrasting behavior of the structural and magnetic properties in Mn-
and Fe-doped In2O3 films
SO APL MATERIALS
LA English
DT Article
ID SPINTRONICS; (IN1-XFEX)(2)O3-SIGMA; FERROMAGNETISM; SEMICONDUCTOR; OXIDE
AB We have observed room temperature ferromagnetism in In2O3 thin films doped with either 5 at.% Mn or Fe, prepared by pulsed laser deposition at substrate temperatures ranging from 300 to 600 degrees C. The dependence of saturation magnetization on grain size was investigated for both types of In2O3 films. It is revealed that, for the Mn-doped films, the magnetization was largest with small grains, indicating the importance of grain boundaries. In contrast, for Fe-doped films, the largest magnetization was observed with large grains. (C) 2013 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.
C1 [Feng, Qi; Blythe, Harry J.; Fox, A. Mark; Gehring, Gillian A.] Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England.
[Jiang, Feng-Xian; Xu, Xiao-Hong] Shanxi Normal Univ, Sch Chem & Mat Sci, Linfen 041004, Peoples R China.
[Heald, Steve M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Gehring, GA (reprint author), Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England.
EM g.gehring@sheffield.ac.uk
RI Fox, Mark/F-1096-2010
OI Fox, Mark/0000-0002-9025-2441
FU U.S. DOE [DE-AC02-06CH11357]
FX Use of the Advanced Photon Source, an Office of Science User Facility
operated for the U.S. Department of Energy (DOE) Office of Science by
Argonne National Laboratory, was also supported by the U.S. DOE under
Contract No. DE-AC02-06CH11357. We thank Dr. Xiufang Qin for help with
the XRD measurements.
NR 22
TC 5
Z9 5
U1 1
U2 8
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 2166-532X
J9 APL MATER
JI APL Mater.
PD AUG
PY 2013
VL 1
IS 2
AR 022107
DI 10.1063/1.4818169
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA AC1RD
UT WOS:000332272800011
ER
PT J
AU Marezio, M
Chmaissem, O
Bougerol, C
Karppinen, M
Yamauchi, H
Geballe, TH
AF Marezio, M.
Chmaissem, O.
Bougerol, C.
Karppinen, M.
Yamauchi, H.
Geballe, T. H.
TI Overdoped cuprates with high-temperature superconducting transitions
SO APL MATERIALS
LA English
DT Article
ID T-C SUPERCONDUCTORS; COPPER OXIDES
AB Evidence for high-T-c cuprate superconductivity is found in a region of the phase diagram where non-superconducting Fermi liquid metals are expected. Cu valences estimated independently from both x-ray absorption near-edge spectroscopy and bond valence sum measurements are >2.3, and are in close agreement with each other for structures in the homologous series (Cu0.75Mo0.25)Sr-2(Y,Ce)sCu2O(5+2s+delta) with s = 1, 2, 3, and 4. The record short apical oxygen distance, at odds with current theory, suggests the possibility of a new pairing mechanism. The possibility that the charge reservoir layers are able to screen long range coulomb interactions and thus enhance T-c is discussed. (C) 2013 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.
C1 [Marezio, M.] CRETA CNRS, F-38042 Grenoble 9, France.
[Chmaissem, O.] Univ Illinois, Dept Phys, De Kalb, IL 60115 USA.
[Chmaissem, O.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Bougerol, C.] CEA CNRS, Inst Neel, F-38042 Grenoble 9, France.
[Karppinen, M.; Yamauchi, H.] Aalto Univ, Dept Chem, FI-00076 Aalto, Finland.
[Geballe, T. H.] Stanford Univ, Dept Appl Phys & Mat Sci, Stanford, CA 94305 USA.
RP Marezio, M (reprint author), CRETA CNRS, F-38042 Grenoble 9, France.
EM marezio@grenoble.cnrs.fr
RI Karppinen, Maarit/G-8035-2012; Bougerol, Catherine/M-6980-2015
OI Bougerol, Catherine/0000-0002-4823-0919
FU U.S. Department of Energy, Office of Science, Materials Science and
Engineering Division [DE-AC02-06CH11357]; Academy of Finland [126528,
255562]; Tekes [1726/31/07]; Airforce Office of Scientific Research
(AFOSR) [FA9550-09-1-0583]
FX Work at Argonne was supported by the U.S. Department of Energy, Office
of Science, Materials Science and Engineering Division, under Contract
No. DE-AC02-06CH11357. The work at Aalto University was supported by
Academy of Finland (Nos. 126528 and 255562) and Tekes (No. 1726/31/07).
The work at Stanford was supported in part by the Airforce Office of
Scientific Research (AFOSR) under Grant No. FA9550-09-1-0583. T.H.G.
would like to acknowledge helpful comments from Sri Raghu, Steve
Kivelson, and Aharon Kapitulnik.
NR 22
TC 4
Z9 4
U1 1
U2 15
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 2166-532X
J9 APL MATER
JI APL Mater.
PD AUG
PY 2013
VL 1
IS 2
AR 021103
DI 10.1063/1.4817895
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA AC1RD
UT WOS:000332272800004
ER
PT J
AU Jacobus, JA
Duda, CG
Coleman, MC
Martin, SM
Mapuskar, K
Mao, G
Smith, BJ
Aykin-Burns, N
Guida, P
Gius, D
Domann, FE
Knudson, CM
Spitz, DR
AF Jacobus, James A.
Duda, Chester G.
Coleman, Mitchell C.
Martin, Sean M.
Mapuskar, Kranti
Mao, Gaowei
Smith, Brian J.
Aykin-Burns, Nukhet
Guida, Peter
Gius, David
Domann, Frederick E.
Knudson, C. Michael
Spitz, Douglas R.
TI Low-Dose Radiation-Induced Enhancement of Thymic Lymphomagenesis in
Lck-Bax Mice is Dependent on LET and Gender
SO RADIATION RESEARCH
LA English
DT Article
ID MANGANESE SUPEROXIDE-DISMUTASE; DEHYDROGENASE SUBUNIT-C;
IONIZING-RADIATION; GENOMIC INSTABILITY; HEPATOCELLULAR-CARCINOMA;
MITOCHONDRIAL ROS; TUMOR-SUPPRESSOR; OXIDATIVE STRESS; MAMMALIAN-CELLS;
CANCER-CELLS
AB The hypothesis thatmitochondrial dysfunction and increased superoxide levels in thymocytes over expressing Bax (Lck-Bax1 and Lck-Bax38&1) contributes to lymphomagenesis after low-dose radiation was tested. Lck-Bax1 single-transgenic and Lck-Bax38&1 double-transgenic mice were exposed to single whole-body doses of 10 or 100 cGy of Cs-137 or iron ions (1,000 MeV/n, 150 keV/lm) or silicon ions (300 MeV/n, 67 keV/lm). A 10 cGy dose of Cs-137 significantly increased the incidence and onset of thymic lymphomas in female Lck-Bax1 mice. In Lck-Bax38&1 mice, a 100 cGy dose of high-LET iron ions caused a significant dose dependent acceleration of lymphomagenesis in both males and females that was not seen with silicon ions. To determine the contribution of mitochondrial oxidative metabolism, Lck-Bax38&1 over expressing mice were crossed with knockouts of the mitochondrial protein deacetylase, Sirtuin 3 (Sirt3), which regulates superoxide metabolism. Sirt3(-/-)/Lck-Bax38&1 mice demonstrated significant increases in thymocyte superoxide levels and acceleration of lymphomagenesis (P < 0.001). These results show that lymphomagenesis in Bax over expressing animals is enhanced by radiation exposure in both an LET and gender dependent fashion. These findings support the hypothesis that mitochondrial dysfunction leads to increased superoxide levels and accelerates lymphomagenesis in Lck-Bax transgenic mice. (C) 2013 by Radiation Research Society
C1 [Jacobus, James A.; Coleman, Mitchell C.; Mapuskar, Kranti; Mao, Gaowei; Domann, Frederick E.; Spitz, Douglas R.] Univ Iowa, Dept Radiat Oncol, Free Radical & Radiat Biol Program, Holden Comprehens Canc Ctr, Iowa City, IA 52242 USA.
[Duda, Chester G.; Mapuskar, Kranti] Univ Iowa, Interdisciplinary Grad Program Human Toxicol, Iowa City, IA 52242 USA.
[Martin, Sean M.; Knudson, C. Michael] Univ Iowa, Dept Pathol, Iowa City, IA 52242 USA.
[Smith, Brian J.] Univ Iowa, Coll Publ Hlth, Dept Biostat, Iowa City, IA 52242 USA.
[Aykin-Burns, Nukhet] Univ Arkansas Med Sci, Dept Pharmaceut Sci, Div Radiat Hlth, Little Rock, AR 72205 USA.
[Guida, Peter] Brookhaven Natl Lab, Dept Med, Upton, NY 11973 USA.
[Gius, David] Northwestern Univ, Feinberg Sch Med, Dept Radiat Oncol, Chicago, IL 60611 USA.
RP Spitz, DR (reprint author), Univ Iowa, Dept Radiat Oncol, Free Radical & Radiat Biol Program, B180 Med Labs, Iowa City, IA 52242 USA.
EM douglas-spitz@uiowa.edu
RI mao, gaowei/A-8142-2015;
OI mao, gaowei/0000-0001-6090-8131; Domann, Frederick/0000-0002-0489-2179
FU Department of Energy/NASA [DE-SC0000830]; [NIH T32 CA078586];
[R01CA152601]; [R01CA152799]; [R01CA168292]; [3 P30 CA086862]
FX The authors would like to thank Amanda Kalen from the Radiation and Free
Radical Research Core in the Holden Comprehensive Cancer Center for
assistance with low-LET irradiations, The University of Iowa Flow
Cytometry Facility located in the Carver College of Medicine Core
Research Facilities/Holden Comprehensive Cancer Center Core Laboratory,
and Gareth Smith for his editorial assistance. We also thank the
scientists and staff at Brookhaven National Laboratory Medical
Department and NASA Space Radiation Laboratory for their assistance with
our high-LET exposures. Finally, we wish to extend our gratitude to the
Office of Animal Resources at the University of Iowa and especially our
primary caretaker during these studies, Gary Duder. This work was
supported by Department of Energy/NASA grant DE-SC0000830, as well as
grants NIH T32 CA078586, R01CA152601, R01CA152799, R01CA168292 and 3 P30
CA086862.
NR 50
TC 2
Z9 2
U1 0
U2 3
PU RADIATION RESEARCH SOC
PI LAWRENCE
PA 810 E TENTH STREET, LAWRENCE, KS 66044 USA
SN 0033-7587
EI 1938-5404
J9 RADIAT RES
JI Radiat. Res.
PD AUG
PY 2013
VL 180
IS 2
BP 156
EP 165
DI 10.1667/RR3293.1
PG 10
WC Biology; Biophysics; Radiology, Nuclear Medicine & Medical Imaging
SC Life Sciences & Biomedicine - Other Topics; Biophysics; Radiology,
Nuclear Medicine & Medical Imaging
GA AA3KG
UT WOS:000330990700006
PM 23819597
ER
PT J
AU Pavlova, IV
Lewis, KC
AF Pavlova, Iglika V.
Lewis, Kayla C.
TI An Easy & Fun Way to Teach about How Science "Works": Popularizing
Haack's Crossword-Puzzle Analogy
SO AMERICAN BIOLOGY TEACHER
LA English
DT Article
DE Active learning; scientific reasoning; ad hoc hypotheses; pseudoscience;
evolution
AB Science is a complex process, and we must not teach our students overly simplified versions of "the" scientific method. We propose that students can uncover the complex realities of scientific thinking by exploring the similarities and differences between solving the familiar crossword puzzles and scientific "puzzles." Similarly to solving a crossword puzzle, solving puzzles in science is a complex and creative process in which hypotheses and theories evolve through the accumulation of many pieces of independent, yet interlocking, lines of evidence. We discuss the important lessons from Haack's crossword-puzzle analogy and how it applies to teaching science.
C1 [Pavlova, Iglika V.] Univ Chicago, Coll Biol Sci, Chicago, IL 60637 USA.
[Lewis, Kayla C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Pavlova, IV (reprint author), Univ Chicago, Coll Biol Sci, 924 E 57th St,BSLC,Rm 208, Chicago, IL 60637 USA.
EM iglikap@uchicago.edu
NR 14
TC 1
Z9 1
U1 0
U2 2
PU NATL ASSOC BIOLOGY TEACHERS INC
PI RESTON
PA 12030 SUNRISE VALLEY DR, #110, RESTON, VA 20191 USA
SN 0002-7685
EI 1938-4211
J9 AM BIOL TEACH
JI Am. Biol. Teach.
PD AUG
PY 2013
VL 75
IS 6
BP 397
EP 401
DI 10.1525/abt.2013.75.6.7
PG 5
WC Biology; Education, Scientific Disciplines
SC Life Sciences & Biomedicine - Other Topics; Education & Educational
Research
GA 301YR
UT WOS:000330568700007
ER
PT J
AU Kerr, GD
Egbert, SD
Al-Nabulsi, I
Beck, HL
Cullings, HM
Endo, S
Hoshi, M
Imanaka, T
Kaul, DC
Maruyama, S
Reeves, GI
Ruehm, W
Sakaguchi, A
Simon, SL
Spriggs, GD
Stram, DO
Tonda, T
Weiss, JF
Weitz, RL
Young, RW
AF Kerr, George D.
Egbert, Stephen D.
Al-Nabulsi, Isaf
Beck, Harold L.
Cullings, Harry M.
Endo, Satoru
Hoshi, Masaharu
Imanaka, Tetsuji
Kaul, Dean C.
Maruyama, Satoshi
Reeves, Glen I.
Ruehm, Werner
Sakaguchi, Aya
Simon, Steven L.
Spriggs, Gregory D.
Stram, Daniel O.
Tonda, Tetsuji
Weiss, Joseph F.
Weitz, Ronald L.
Young, Robert W.
TI WORKSHOP REPORT ON ATOMIC BOMB DOSIMETRY-RESIDUAL RADIATION EXPOSURE:
RECENT RESEARCH AND SUGGESTIONS FOR FUTURE STUDIES
SO HEALTH PHYSICS
LA English
DT Article
DE atomic bomb; atomic bomb survivors; fallout; radiation effects
ID FALLOUT DEPOSITION; BLACK RAIN; HIROSHIMA; U-235/U-238; SURVIVORS;
NAGASAKI; RATIOS
AB There is a need for accurate dosimetry for studies of health effects in the Japanese atomic bomb survivors because of the important role that these studies play in worldwide radiation protection standards. International experts have developed dosimetry systems, such as the Dosimetry System 2002 (DS02), which assess the initial radiation exposure to gamma rays and neutrons but only briefly consider the possibility of some minimal contribution to the total body dose by residual radiation exposure. In recognition of the need for an up-to-date review of the topic of residual radiation exposure in Hiroshima and Nagasaki, recently reported studies were reviewed at a technical session at the 57th Annual Meeting of the Health Physics Society in Sacramento, California, 22-26 July 2012. A one-day workshop was also held to provide time for detailed discussion of these newer studies and to evaluate their potential use in clarifying the residual radiation exposures to the atomic-bomb survivors at Hiroshima and Nagasaki. Suggestions for possible future studies are also included in this workshop report.
C1 [Kerr, George D.] Kerr Consulting, Knoxville, TN USA.
[Kerr, George D.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA.
[Egbert, Stephen D.] Sci Applicat Int Corp, San Diego, CA 92121 USA.
[Al-Nabulsi, Isaf; Weiss, Joseph F.] US DOE, Washington, DC 20585 USA.
[Beck, Harold L.] US DOE, New York, NY USA.
[Cullings, Harry M.] Radiat Effects Res Fdn, Hiroshima, Japan.
[Endo, Satoru] Prefectural Univ Hiroshima, Hiroshima, Japan.
[Hoshi, Masaharu; Sakaguchi, Aya; Tonda, Tetsuji] Hiroshima Univ, Hiroshima 730, Japan.
[Imanaka, Tetsuji] Kyoto Univ, Kyoto 6068501, Japan.
[Kaul, Dean C.] SAIC, Park City, UT USA.
[Maruyama, Satoshi] Minist Hlth Labour & Welf, Tokyo, Japan.
[Reeves, Glen I.] Appl Res Associates, Arlington, VA USA.
[Ruehm, Werner] Helmholtz Zentrum Muenchen, German Res Ctr Environm Hlth, Neuherberg, Germany.
[Simon, Steven L.] NCI, NIH, Bethesda, MD 20892 USA.
[Spriggs, Gregory D.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Stram, Daniel O.] Univ So Calif, Los Angeles, CA USA.
[Weitz, Ronald L.] SAIC, Albuquerque, NM USA.
[Young, Robert W.] Def Nucl Agcy, Winter Pk, FL USA.
RP Kerr, GD (reprint author), Oak Ridge Associated Univ, POB 117, Oak Ridge, TN 37831 USA.
EM George.Kerr@orau.org
RI Sakaguchi, Aya/E-8134-2015; Endo, Satoru/D-9091-2012;
OI Endo, Satoru/0000-0001-5961-681X; Hoshi, Masaharu/0000-0001-6978-0883
FU U.S. Department of Energy (DOE)
FX We wish to thank David Landguth, Oak Ridge National Laboratory, for his
organizational expertise that resulted in a highly successful workshop.
The help and advice of the Health Physics Society meeting organizers and
the staff of Burk and Associates are greatly appreciated. We would also
like to thank John Boice for his excellent presentation at the start of
the technical session, although he was not able to participate in the
workshop. The participation of George D. Kerr, Steve D. Egbert, Harold
L. Beck, Harry M. Cullings, Satoru Endo, Masaharu Hoshi, Tetsuji
Imanaka, Dean C. Kaul, Aya Sakaguchi, Gregory D. Springs, Daniel O.
Stram, and R. L. Weitz in the workshop was financially supported by the
U.S. Department of Energy (DOE). The views of the authors do not
necessarily reflect those of the DOE, the U.S. government, or the
authors' institutions.
NR 24
TC 8
Z9 8
U1 0
U2 8
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
BP 140
EP 149
DI 10.1097/HP.0b013e31828ca73a
PG 10
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AT
UT WOS:000330367400004
PM 23799498
ER
PT J
AU Torii, T
Sugita, T
Okada, CE
Reed, MS
Blumenthal, DJ
AF Torii, Tatsuo
Sugita, Takeshi
Okada, Colin E.
Reed, Michael S.
Blumenthal, Daniel J.
TI ENHANCED ANALYSIS METHODS TO DERIVE THE SPATIAL DISTRIBUTION OF I-131
DEPOSITION ON THE GROUND BY AIRBORNE SURVEYS AT AN EARLY STAGE AFTER THE
FUKUSHIMA DAIICHI NUCLEAR POWER PLANT ACCIDENT
SO HEALTH PHYSICS
LA English
DT Article
DE accident; reactor; environmental assessment; I-131; monitoring;
environmental
ID SYSTEM; JAPAN
AB This paper applies both new and well tested analysis methods to aerial radiological surveys to extract the I-131 ground concentrations present after the March 2011 Fukushima Daiichi nuclear power plant (NPP) accident. The analysis provides a complete map of I-131 deposition, an important quantity incalculable at the time of the accident due to the short half-life of I-131 and the complexity of the analysis. A map of I-131 deposition is the first step in conducting internal exposure assessments, population dose reconstruction, and follow-up epidemiological studies. The short half-life of I-131 necessitates the use of aerial radiological surveys to cover the large area quickly, thoroughly, and safely. Teams from the U. S. Department of Energy National Nuclear Security Administration (DOE/NNSA) performed aerial radiological surveys to provide initial maps of the dispersal of radioactive material in Japan. This work reports on analyses performed on a subset of the initial survey data by a joint Japan-U.S. collaboration to determine I-131 ground concentrations. The analytical results show a high concentration of I-131 northwest of the NPP, consistent with the previously reported radioactive cesium deposition, but also shows a significant I-131 concentration south of the plant, which was not observed in the original cesium analysis. The difference in the radioactive iodine and cesium patterns is possibly the result of differences in the ways these materials settle out of the air.
C1 [Torii, Tatsuo; Sugita, Takeshi] JAEA, Fukushima Environm Safety Ctr, Tokyo 1008577, Japan.
[Okada, Colin E.; Reed, Michael S.] US DOE, Remote Sensing Lab, Las Vegas, NV USA.
[Blumenthal, Daniel J.] US DOE, Natl Nucl Secur Adm, Washington, DC 20585 USA.
RP Torii, T (reprint author), JAEA, Chiyoda Ku, 2-2-2 Uchisaiwai Cho, Tokyo 1008577, Japan.
EM torii.tatsuo@jaea.go.jp
FU U.S. Department of Energy [DE-AC52-06NA25946]
FX The authors are grateful to collaborators from JAEA/Headquarters of
Fukushima Partnership Operations, U.S. DOE/RSL, and NNSA for their
cooperation and assistance. We also thank H. Hirayama (KEK, Japan) for
his useful suggestion and discussion on the Monte Carlo simulation.
Moreover, we would like to acknowledge that this work was performed in
part under Contract No. DE-AC52-06NA25946 with the U.S. Department of
Energy.
NR 17
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U1 2
U2 15
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
BP 192
EP 200
DI 10.1097/HP.0b013e318294444e
PG 9
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AT
UT WOS:000330367400010
PM 23799504
ER
PT J
AU Farfan, E
Jannik, GT
Lee, P
Powell, A
AF Farfan, Eduardo
Jannik, G. Timothy
Lee, Patricia
Powell, Aaron
TI Comparison of CAP88 PC Ver. 3.0 and MAXDOSE Dose Assessment Models
Involving Co-located Stack Releases at the Savannah River Site
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; computer calculations; dose assessment; dosimetry
AB The Savannah River National Laboratory's Environmental Dosimetry Group performs dosimetry assessments for Savannah River Site (SRS) radionuclide air emissions utilizing the Clean Air Act Assessment Package-1988 (CAP88) code (CAP88 PC Ver. 3.0) and the MAXDOSE-SR Ver. 2011 code, which is an SRS-specific version of the Nuclear Regulatory Commission's MAXIGASP code. CAP88 PC and MAXDOSE-SR are used at SRS for demonstrating compliance with Environmental Protection Agency dose standards for radionuclide emissions to the atmosphere and Department of Energy Order 458.1 dose standards, respectively. During a routine comparison of these two assessment models, it was discovered that CAP88 PC Ver. 3.0 was not producing the expected results when using multiple co-located stacks in a single run. Specifically, if the stack heights are considered separately, the results for several radionuclides (but not all) differ from the combined run [i.e., 1 + 2 does not equal (1+2)]. Additionally, when two or more stack heights are considered in a run, the results depend on the order of the selected stack heights. For example, for a two stack-height run of 0 meter and 61 m input produces different results from a 61 m and 0 m input run. This study presents a comparison of CAP88 PC Ver. 3.0 and MAXDOSE-SR Ver. 2011 based on SRS input data and on two-stack release scenarios. The selected radionuclides for this study included gases/vapors (H-3, C-14, Kr-85, and I-131) and particulates (Sr-190, Cs-137, Pu-239, and Am-241) commonly encountered at SRS.
C1 [Farfan, Eduardo; Jannik, G. Timothy; Lee, Patricia] Savannah River Natl Lab, Aiken, SC 29808 USA.
[Powell, Aaron] Univ N Carolina, Charlotte, NC 28223 USA.
RP Farfan, E (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA.
EM eduardo.farfan@srnl.doe.gov
FU U.S. Department of Energy [DE-AC09-08SR22470]
FX This manuscript has been co-authored by Savannah River Nuclear
Solutions, LLC under Contract No. DE-AC09-08SR22470 with the U.S.
Department of Energy. The United States Government retains and the
publisher, by accepting this article for publication, acknowledges that
the United States Government retains a non-exclusive, paid-up,
irrevocable, worldwide license to publish or reproduce the published
form of this work, or allow others to do so, for United States
Government purposes. Mention of trade names or commercial products does
not constitute endorsement or recommendation for use by the authors or
their corresponding organizations.
NR 11
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U1 0
U2 2
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S158
EP S163
PG 6
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300008
PM 23803669
ER
PT J
AU Jelinski, J
Wahl, L
Donovan, T
AF Jelinski, John
Wahl, Linnea
Donovan, Thomas
TI Assessment of an Improved Stack Sample Collection System for H-3 and
C-14
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; C-14; air sampling; tritium
AB Lawrence Berkeley National Laboratory developed a simple, efficient, and cost-effective replacement for the traditional glass column system used to monitor H-3 and C-14 emissions from rooftop stacks. The primary goals in developing a replacement (the modified jar system) were to 1) maintain or improve collection efficiency while keeping leakage to less than 5%, 2) simplify the set-up process, and 3) reduce costs. Both the traditional glass column assembly and the modified jar system were operated in tandem for a 13-mo period. Results showed that the modified sample jar system provided equivalent or improved collection efficiency for both H-3 and C-14. Additional advantages included reduced leak-test errors, quicker and simpler set-up, and material costs that were reduced by nearly an order of magnitude.
C1 [Jelinski, John; Wahl, Linnea; Donovan, Thomas] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Jelinski, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM jajelinski@lbl.gov
NR 4
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U1 0
U2 1
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S119
EP S124
PG 6
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300004
PM 23803665
ER
PT J
AU Leggett, R
Scofield, P
Eckerman, K
AF Leggett, Richard
Scofield, Patricia
Eckerman, Keith
TI Basis and Implications of the CAP88 Age-Specific Dose Coefficients
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; modeling, biological factors; modeling, dose
assessment; modeling, environmental
AB Recent versions of CAP88 incorporate age-specific dose coefficients based on biokinetic and dosimetric models applied in Federal Guidance Report 13, "Cancer Risk Coefficients for Environmental Exposure to Radionuclides." With a few exceptions the models are those recommended in a series of reports by the International Commission on Radiological Protection (ICRP) on estimation of doses to the public from environmental radionuclides. This paper describes the basis for the ICRP's age-specific biokinetic and dosimetric models and examines differences with age in dose coefficients derived from those models.
C1 [Leggett, Richard; Scofield, Patricia; Eckerman, Keith] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Leggett, R (reprint author), Oak Ridge Natl Lab, MS 6113,POB 2008, Oak Ridge, TN 37831 USA.
EM scofieldpa@ornl.gov
FU Office of Radiation and Indoor Air, U. S. Environmental Protection
Agency (EPA) [1824-S581-A1, DE-AC05-00OR22725]; UT-Battelle; U.S.
Government [DE-AC05-00OR22725]
FX The work described in this manuscript was sponsored by the Office of
Radiation and Indoor Air, U. S. Environmental Protection Agency (EPA),
under Interagency Agreement DOE No. 1824-S581-A1, under contract No.
DE-AC05-00OR22725 with UT-Battelle. The submitted manuscript has been
authored by a contractor of the U.S. Government under contract
DE-AC05-00OR22725. Accordingly, the U.S. Government retains a
nonexclusive, royalty-free license to publish or reproduce the published
form of this contribution, or allow others to do so, for U.S. Government
purposes.
NR 19
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U1 0
U2 1
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S149
EP S157
PG 9
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300007
PM 23803668
ER
PT J
AU MacQueen, D
Bertoldo, N
Wegrecki, A
AF MacQueen, Donald
Bertoldo, Nicholas
Wegrecki, Anthony
TI A Best Fit Approach to Estimating Multiple Diffuse Source Terms Using
Ambient Air Monitoring Data and an Air Dispersion Model
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; modeling, dose assessment; monitoring, air;
regulations
ID TRITIUM
AB Lawrence Livermore National Laboratory uses CAP88-PC Version 1.0 modeling software to demonstrate compliance with the Code of Federal Regulations Title 40 Part 61 Subpart H (National Emission Standards for Emissions of Radionuclides Other Than Radon From Department of Energy Facilities). Annual air emissions from both well characterized stack sources and difficult to characterize diffuse sources must be assessed. This paper describes a process that uses a mathematical optimization routine to find a set of estimated diffuse source terms that together with the measured stack source terms provides a best fit of modeled air concentrations to measured air concentrations at available sampling locations. The estimated and measured source terms may then be used in subsequent CAP88-PC modeling to estimate dose at the off-site maximally exposed individual. LLNL has found this process to be an effective way to deal with the required assessment of diffuse sources that have otherwise been difficult to assess.
C1 [MacQueen, Donald; Bertoldo, Nicholas; Wegrecki, Anthony] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
RP MacQueen, D (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave L-627, Livermore, CA 94550 USA.
EM macqueen1@llnl.gov
FU U.S. Department of Energy by Lawrence Livermore National Laboratory
[W-7405-Eng-48, DE-AC52-07NA27344]
FX The authors would like to thank LLNL staff members Gary Bear, Steve
Hall, Terrance Poole, and Kent Wilson for their work designing,
operating, and maintaining the environmental sampling and meteorological
monitoring equipment that provide the information necessary for this
work. The authors also thank the reviewers for their helpful and
thought-provoking comments. This work was performed under the auspices
of the U.S. Department of Energy by Lawrence Livermore National
Laboratory in part under Contract W-7405-Eng-48 and in part under
Contract DE-AC52-07NA27344.
NR 10
TC 0
Z9 0
U1 0
U2 1
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S140
EP S148
PG 9
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300006
PM 23803667
ER
PT J
AU McNaughton, M
Brock, B
Eisele, W
Fuehne, D
Green, A
Whicker, J
AF McNaughton, Michael
Brock, Burgandy
Eisele, William, Jr.
Fuehne, David
Green, Andrew
Whicker, Jeffrey
TI Addressing Nuclides Not in the CAP88-PC Version-3 Library
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; dose assessment; emissions, atmospheric; monitoring,
air
AB Versions of the computer program, CAP88, are widely used to calculate the radiological doses from radionuclides emitted into the air. CAP88-PC Version-3 includes an extensive library of radionuclides, but there are many more that are not included. Surrogates are often used to substitute for nuclides not in the library, though the results are usually overestimates. This paper addresses nuclides that are not in the library and describes methods to obtain more accurate results.
C1 [McNaughton, Michael; Brock, Burgandy; Eisele, William, Jr.; Fuehne, David; Green, Andrew; Whicker, Jeffrey] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP McNaughton, M (reprint author), Los Alamos Natl Lab, MS J978, Los Alamos, NM 87545 USA.
EM mcnaught@lanl.gov
NR 5
TC 0
Z9 0
U1 0
U2 0
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S182
EP S188
PG 7
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300012
PM 23803673
ER
PT J
AU Michelotti, E
Green, A
Whicker, J
Eisele, W
Fuehne, D
McNaughton, M
AF Michelotti, Erika
Green, Andrew
Whicker, Jeffrey
Eisele, William
Fuehne, David
McNaughton, Michael
TI Validation Test for CAP88 Predictions of Tritium Dispersion at Los
Alamos National Laboratory
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; dose assessment; emissions; atmospheric; monitoring;
air
AB Gaussian plume models, such as CAP88, are used regularly for estimating downwind concentrations from stack emissions. At many facilities, the U. S. Environmental Protection Agency (U. S. EPA) requires that CAP88 be used to demonstrate compliance with air quality regulations for public protection from emissions of radionuclides. Gaussian plume models have the advantage of being relatively simple and their use pragmatic; however, these models are based on simplifying assumptions and generally they are not capable of incorporating dynamic meteorological conditions or complex topography. These limitations encourage validation tests to understand the capabilities and limitations of the model for the specific application. Los Alamos National Laboratory (LANL) has complex topography but is required to use CAP88 for compliance with the Clean Air Act Subpart H. The purpose of this study was to test the accuracy of the CAP88 predictions against ambient air measurements using released tritium as a tracer. Stack emissions of tritium from two LANL stacks were measured and the dispersion modeled with CAP88 using local meteorology. Ambient air measurements of tritium were made at various distances and directions from the stacks. Model predictions and ambient air measurements were compared over the course of a full year's data. Comparative results were consistent with other studies and showed the CAP88 predictions of downwind tritium concentrations were on average about three times higher than those measured, and the accuracy of the model predictions were generally more consistent for annual averages than for bi-weekly data.
C1 [Michelotti, Erika; Green, Andrew; Whicker, Jeffrey; Eisele, William; Fuehne, David; McNaughton, Michael] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Whicker, J (reprint author), Los Alamos Natl Lab, Mail Stop J978, Los Alamos, NM 87545 USA.
EM jjwhicker@lanl.gov
NR 15
TC 1
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U1 0
U2 4
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S176
EP S181
PG 6
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300011
PM 23803672
ER
PT J
AU Rhoads, K
Snyder, S
Staven, L
AF Rhoads, Kathleen
Snyder, Sandra
Staven, Lissa
TI A Comparison of Dose Results from the Clean Air Act Assessment
Package-1988, Personal Computer (CAP88-PC), Version 3 to Previous
Versions
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; dose assessment; emissions, atmospheric; regulations
AB Computer software packages approved by the U.S. Environmental Protection Agency (U.S. EPA), including CAP88-PC, are used by U.S. Department of Energy (U.S. DOE) sites to demonstrate compliance with the radionuclide air emission standard under the Clean Air Act. CAP88-PC version 3, was approved by the U.S. EPA in February 2006 for use by U.S. DOE facilities. Version 3 incorporates several major changes that have the potential to affect calculated doses relative to calculations using earlier versions. This analysis examined the types and magnitudes of changes to dose estimates for specific radionuclides calculated using the version 3 software compared with the previous versions. For parent radionuclides and for the total dose from radionuclide chains, total effective dose calculated with version 3 was compared to effective dose equivalent calculated with previous versions. Various comparisons were also performed to determine which of the updates in version 3 accounted for changes in overall dose estimates. CAP88-PC version 3 would produce substantially different results relative to previous versions of the code for a number of radionuclides, including some isotopes that may be present at U.S. DOE facilities, as well as those used for industrial and medical applications. In general, doses for many radionuclides were lower using version 3 but doses for a few key radionuclides increased relative to the previous versions.
C1 [Rhoads, Kathleen; Snyder, Sandra; Staven, Lissa] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Rhoads, K (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM sandra.snyder@pnnl.gov
FU U.S. Department of Energy [DE-AC05-76RL01830]
FX Pacific Northwest National Laboratory is operated by Battelle Memorial
Institute for the U.S. Department of Energy under Contract No.
DE-AC05-76RL01830. This work was supported by the U.S. Department of
Energy.
NR 24
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U1 0
U2 2
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S125
EP S139
PG 15
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300005
PM 23803666
ER
PT J
AU Snyder, S
Vazquez, G
Hay, T
AF Snyder, Sandra
Vazquez, Gustavo
Hay, Tristan
TI Use of CAP88 at Department of Energy Sites
SO HEALTH PHYSICS
LA English
DT Article
DE operational topics; dose assessment; emissions, atmospheric; regulations
AB The U.S. Department of Energy is committed to protecting the public and environment against undue risk from radiation associated with radiological activities conducted under its control. Some U.S. Department of Energy Site activities result in emissions of radioactive materials to the air. CAP88 codes are used to model these emissions and the subsequent maximum estimated dose to a member of the public in the vicinity of the U.S. Department of Energy Site. This paper reviews the use of the CAP88 code at the variety of U.S. Department of Energy sites that use it for compliance reporting under Title 40 of the Code of Federal Regulations Part 61, Subpart H.
C1 [Snyder, Sandra; Hay, Tristan] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Vazquez, Gustavo] US DOE, Off Hlth Safety & Secur, Washington, DC 20585 USA.
RP Snyder, S (reprint author), Pacific NW Natl Lab, POB 999,K3-54, Richland, WA 99352 USA.
EM sandra.snyder@pnnl.gov
OI Snyder, Sandra/0000-0001-5826-1324
FU U.S. Department of Energy [DE-AC05-76RL01830]
FX The Pacific Northwest National Laboratory is operated by Battelle
Memorial Institute for the U.S. Department of Energy under Contract No.
DE-AC05-76RL01830. This work was supported by the U.S. Department of
Energy.
NR 7
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U2 3
PU LIPPINCOTT WILLIAMS & WILKINS
PI PHILADELPHIA
PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA
SN 0017-9078
EI 1538-5159
J9 HEALTH PHYS
JI Health Phys.
PD AUG
PY 2013
VL 105
IS 2
SU 2
BP S164
EP S168
PG 5
WC Environmental Sciences; Public, Environmental & Occupational Health;
Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical
Imaging
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA 299AJ
UT WOS:000330366300009
PM 23803670
ER
PT J
AU Bounoua, L
Kahime, K
Houti, L
Blakey, T
Ebi, KL
Zhang, P
Imhoff, ML
Thome, KJ
Dudek, C
Sahabi, SA
Messouli, M
Makhlouf, B
El Laamrani, A
Boumezzough, A
AF Bounoua, Lahouari
Kahime, Kholoud
Houti, Leila
Blakey, Tara
Ebi, Kristie L.
Zhang, Ping
Imhoff, Marc L.
Thome, Kurtis J.
Dudek, Claire
Sahabi, Salah A.
Messouli, Mohammed
Makhlouf, Baghdad
El Laamrani, Abderrahmane
Boumezzough, Ali
TI Linking Climate to Incidence of Zoonotic Cutaneous Leishmaniasis (L.
major) in Pre-Saharan North Africa
SO INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH
LA English
DT Article
DE cutaneous leishmaniasis; surface climate indicators; incidence; climate;
NDVI; North Africa
ID PHLEBOTOMUS-PAPATASI DIPTERA; SEASONAL DISTRIBUTION; LUTZOMYIA-OVALLESI;
TEMPORAL DYNAMICS; SOUTHWEST ASIA; SAND FLIES; PSYCHODIDAE; MOROCCO;
TRANSMISSION; POPULATIONS
AB Shifts in surface climate may have changed the dynamic of zoonotic cutaneous leishmaniasis (ZCL) in the pre-Saharan zones of North Africa. Caused by Leishmania major, this form multiplies in the body of rodents serving as reservoirs of the disease. The parasite is then transmitted to human hosts by the bite of a Phlebotomine sand fly (Diptera: Psychodidae) that was previously fed by biting an infected reservoir. We examine the seasonal and interannual dynamics of the incidence of this ZCL as a function of surface climate indicators in two regions covering a large area of the semi-arid Pre-Saharan North Africa. Results suggest that in this area, changes in climate may have initiated a trophic cascade that resulted in an increase in ZCL incidence. We find the correlation between the rainy season precipitation and the same year Normalized Difference Vegetation Index (NDVI) to be strong for both regions while the number of cases of ZCL incidence lags the precipitation and NDVI by 2 years. The zoonotic cutaneous leishmaniasis seasonal dynamic appears to be controlled by minimum temperatures and presents a 2-month lag between the reported infection date and the presumed date when the infection actually occurred. The decadal increase in the number of ZCL occurrence in the region suggests that changes in climate increased minimum temperatures sufficiently and created conditions suitable for endemicity that did not previously exist. We also find that temperatures above a critical range suppress ZCL incidence by limiting the vector's reproductive activity.
C1 [Bounoua, Lahouari; Zhang, Ping; Thome, Kurtis J.] NASA, Goddard Space Flight Ctr, Biospher Sci Lab, Greenbelt, MD 20771 USA.
[Kahime, Kholoud; Boumezzough, Ali] Cadi Ayyad Univ, Lab Ecol & Environm, Marrakech 40000, Morocco.
[Houti, Leila] Fac Med, Sidi Bel Abbes 22000, Algeria.
[Blakey, Tara] Florida Int Univ, Miami, FL 33199 USA.
[Ebi, Kristie L.] ClimAdapt LLC, Los Altos, CA 94022 USA.
[Zhang, Ping] Earth Resources Technol Inc, Laurel, MD 20707 USA.
[Imhoff, Marc L.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA.
[Dudek, Claire] Bethesda Chevy Chase High Sch, Bethesda, MD 20814 USA.
[Sahabi, Salah A.] Hydrometeorol Inst Training & Res, Oran 31025, Algeria.
[Messouli, Mohammed] Cadi Ayyad Univ, Lab Hydrobiol Ecotoxicol & Sanitat, Marrakech 40000, Morocco.
[Makhlouf, Baghdad] Estab Local Publ Hlth, Saida 20000, Algeria.
[El Laamrani, Abderrahmane] Minist Hlth, Directorate Epidemiol & Dis Control, Rabat 10010, Morocco.
RP Bounoua, L (reprint author), NASA, Goddard Space Flight Ctr, Biospher Sci Lab, Code 618, Greenbelt, MD 20771 USA.
EM Lahouari.Bounoua-1@nasa.gov; kahimkholoud@gmail.com;
leilahouti@yahoo.fr; tblakey@fiu.edu; krisebi@essllc.org;
ping.zhang@nasa.gov; marc.imhoff@pnnl.gov; kurtis.thome@nasa.gov;
cdudek@smith.edu; salah_sahabi@yahoo.com; messouli@gmail.com;
makhloufbaghdad@yahoo.fr; laamrani55@gmail.com; aboumezzough@gmail.com
FU International START Secretariat; U.S. National Science Foundation
[GEO-0627839]; IDRC-Canada (Leila Houti) [105738-001]; NASA summer
fellowships
FX This article is based on research partially supported by a sub-award
2013-01 (to Kholoud Kahime) from the International START Secretariat
with funds supplied by the U. S. Global Change Research Program
administered by the U.S. National Science Foundation under Grant Number
GEO-0627839, and by the IDRC-Canada (Leila Houti) through project#
105738-001. Tara Blakey and Claire Dudek were supported by NASA summer
fellowships. Warm thanks are due to Haj Haddou (DELM, Rabat) and Ismail
Chichaoui (SIAAP, Errachidia) for help with the epidemiological data.
NR 48
TC 11
Z9 12
U1 4
U2 13
PU MDPI AG
PI BASEL
PA POSTFACH, CH-4005 BASEL, SWITZERLAND
SN 1660-4601
J9 INT J ENV RES PUB HE
JI Int. J. Environ. Res. Public Health
PD AUG
PY 2013
VL 10
IS 8
BP 3172
EP 3191
DI 10.3390/ijerph10083172
PG 20
WC Environmental Sciences; Public, Environmental & Occupational Health
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health
GA 301IT
UT WOS:000330526700006
PM 23912199
ER
PT J
AU Williams, KP
Kelly, DP
AF Williams, Kelly P.
Kelly, Donovan P.
TI Proposal for a new class within the phylum Proteobacteria,
Acidithiobacillia classis nov., with the type order Acidithiobacillales,
and emended description of the class Gammaproteobacteria
SO INTERNATIONAL JOURNAL OF SYSTEMATIC AND EVOLUTIONARY MICROBIOLOGY
LA English
DT Article
ID PURPLE BACTERIA; PHYLOGENY; SUBDIVISION; THIOBACILLUS; ALIGNMENTS;
SULFUR; TREE
AB The order Acidithiobacillales was previously assigned to the class Gammaproteobacteria. Recent analyses have indicated that this order actually lies outside all the proteobacterial classes, as a sister group to the combined classes Betaproteobacteria and Gamma proteobacteria. We now confirm this result with multiprotein phylogenetic analysis of all the available genomes of members of the order Acidithiobacillales and representatives of all available bacterial orders, and propose the new proteobacterial class, Acidithiobacillia, with the type order Acidithiobacillales, comprising the families Acidithiobacillaceae and Thermithiobacillaceae with the type genus Acidithiobacillus.
C1 [Williams, Kelly P.] Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94551 USA.
[Kelly, Donovan P.] Univ Warwick, Sch Life Sci, Coventry CV4 7AL, W Midlands, England.
RP Kelly, DP (reprint author), Univ Warwick, Sch Life Sci, Coventry CV4 7AL, W Midlands, England.
EM D.P.Kelly@warwick.ac.uk
FU DOE Early Career Laboratory Directed Research and Development award; US
Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]
FX K. P. W. was supported by a DOE Early Career Laboratory Directed
Research and Development award. Sandia National Laboratories is a
multi-program laboratory managed and operated by Sandia Corporation, a
wholly owned subsidiary of Lockheed Martin Corporation, for the US
Department of Energy's National Nuclear Security Administration under
contract DE-AC04-94AL85000. We are grateful to editors of the IJSEM for
advice on the Bacteriological Code and the correct etymology to describe
the new class.
NR 28
TC 42
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U1 1
U2 9
PU SOC GENERAL MICROBIOLOGY
PI READING
PA MARLBOROUGH HOUSE, BASINGSTOKE RD, SPENCERS WOODS, READING RG7 1AG,
BERKS, ENGLAND
SN 1466-5026
EI 1466-5034
J9 INT J SYST EVOL MICR
JI Int. J. Syst. Evol. Microbiol.
PD AUG
PY 2013
VL 63
BP 2901
EP 2906
DI 10.1099/ijs.0.049270-0
PN 8
PG 6
WC Microbiology
SC Microbiology
GA 297RA
UT WOS:000330271400023
PM 23334881
ER
PT J
AU Li, G
Li, XS
Zhang, KN
Li, B
Zhang, Y
AF Li, Gang
Li, Xiao-Sen
Zhang, Keni
Li, Bo
Zhang, Yu
TI Effects of Impermeable Boundaries on Gas Production from Hydrate
Accumulations in the Shenhu Area of the South China Sea
SO ENERGIES
LA English
DT Article
DE natural gas hydrate; gas production; simulation; horizontal well; Shenhu
area
ID METHANE HYDRATE; PRODUCTION BEHAVIOR; MARINE-SEDIMENTS; NATURAL-GAS;
SIMULATION; DEPOSITS; ZONE; WELL
AB Based on currently available data from site measurements and the preliminary estimates of the gas production potential from the hydrate accumulations at the SH7 site in the Shenhu Area using the depressurization method with a single horizontal well placed in the middle of the Hydrate-Bearing Layer (HBL), the dependence of production performance on the permeabilities of the overburden (OB) and underburden (UB) layers was investigated in this modeling study. The simulation results indicated that the temperature and the pressure of the HBL were affected by the permeabilities of OB and UB and the effect of depressurization with impermeable OB and UB was significantly stronger than that with permeable boundaries. Considering the percentage of hydrate dissociation, the gas production rate and the gas-to-water ratio, the hydrate deposit with impermeable OB and UB was expected to be the potential gas production target.
C1 [Li, Gang; Li, Xiao-Sen; Li, Bo; Zhang, Yu] Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China.
[Zhang, Keni] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Li, XS (reprint author), Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China.
EM ligang@ms.giec.ac.cn; lixs@ms.giec.ac.cn; kzhang@lbl.gov;
libo@ms.giec.ac.cn; zhangyu1@ms.giec.ac.cn
FU National Science Fund for Distinguished Young Scholars of China
[51225603]; National Natural Science Foundation of China [51076155,
51004089, 51106160]; Science & Technology Program of Guangzhou
[2012J5100012]
FX This work was supported by National Science Fund for Distinguished Young
Scholars of China (Grant 51225603), National Natural Science Foundation
of China (51076155, 51004089 and 51106160), and Science & Technology
Program of Guangzhou (2012J5100012), which are gratefully acknowledged.
NR 35
TC 2
Z9 2
U1 3
U2 14
PU MDPI AG
PI BASEL
PA POSTFACH, CH-4005 BASEL, SWITZERLAND
SN 1996-1073
J9 ENERGIES
JI Energies
PD AUG
PY 2013
VL 6
IS 8
BP 4078
EP 4096
DI 10.3390/en6084078
PG 19
WC Energy & Fuels
SC Energy & Fuels
GA 297VC
UT WOS:000330282200022
ER
PT J
AU Alam, TM
AF Alam, Todd M.
TI Ab Initio Calculations of Possible gamma-Gauche Effects in the C-13-NMR
for Methine and Carbonyl Carbons in Precise Polyethylene Acrylic Acid
Copolymers
SO MOLECULES
LA English
DT Article
DE ab initio; C-13-NMR; chemical shift; trans-gauche; gamma-gauche;
methine; carbonyl
ID CHEMICAL-SHIFTS; NMR-SPECTRA; IGLO; DEPENDENCIES; SUBSTITUENT; PROTEINS;
POLYMERS
AB The impacts of local polymer chain conformations on the methine and carbonyl C-13-NMR chemical shifts for polyethylene acrylic acid p(E-AA) copolymers were predicted using ab initio methods. Using small molecular cluster models, the magnitude and sign of the.-gauche torsional angle effect, along with the impact of local tetrahedral structure distortions near the carbonyl group, on the C-13-NMR chemical shifts were determined. These C-13-NMR chemical shift variations were compared to the experimental trends observed for precise p(E-AA) copolymers as a function acid group spacing and degree of zinc-neutralization in the corresponding p(E-AA) ionomers. These ab initio calculations address the future ability of C-13-NMR chemical shift variations to provide information about the local chain conformations in p(E-AA) copolymer materials.
C1 Sandia Natl Labs, Dept Nanostruct & Elect Mat, Albuquerque, NM 87185 USA.
RP Alam, TM (reprint author), Sandia Natl Labs, Dept Nanostruct & Elect Mat, POB 5800, Albuquerque, NM 87185 USA.
EM tmalam@sandia.gov
FU USA Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]; Sandia Laboratory Directed Research Development
(LDRD) program
FX Sandia National Laboratories is a multi-program laboratory managed and
operated by Sandia Corporation, a wholly owned subsidiary of Lockheed
Martin Corporation, for the USA Department of Energy's National Nuclear
Security Administration under contract DE-AC04-94AL85000. This research
was supported by funding from the Sandia Laboratory Directed Research
Development (LDRD) program. The authors would also like to thank Janelle
Jenkins for initial calculations and stimulating discussions concerning
these investigations.
NR 15
TC 0
Z9 0
U1 1
U2 5
PU MDPI AG
PI BASEL
PA POSTFACH, CH-4005 BASEL, SWITZERLAND
SN 1420-3049
J9 MOLECULES
JI Molecules
PD AUG
PY 2013
VL 18
IS 8
BP 9010
EP 9020
DI 10.3390/molecules18089010
PG 11
WC Chemistry, Organic
SC Chemistry
GA 298DL
UT WOS:000330304100022
PM 23899834
ER
PT J
AU Ramanathan, M
Darling, SB
AF Ramanathan, Muruganathan
Darling, Seth B.
TI Nanofabrication with metallopolymers - recent developments and future
perspectives
SO POLYMER INTERNATIONAL
LA English
DT Review
DE metallopolymers; metal-containing polymer; nanofabrication; patterning;
self-assembly; amphiphilic; pyrolysis; calcination
ID BLOCK-COPOLYMER LITHOGRAPHY; ATOMIC LAYER DEPOSITION; RING-OPENING
POLYMERIZATION; SEQUENTIAL INFILTRATION SYNTHESIS; METAL-CONTAINING
POLYMERS; ABC TRIBLOCK TERPOLYMER; HIGH-MOLECULAR-WEIGHT; STAR-SHAPED
POLYMERS; SALT-LOADED MICELLES; DIBLOCK COPOLYMER
AB Synthetic polymers containing metals and metal centers have experienced rapid growth in the last two decades. Metal-containing polymers have an unprecedented role to play in modern high-tech applications including nanomanufacturing, sensing, separation and catalysis. Advancement in synthetic strategies for macromolecules has enabled the synthesis of novel, exotic and use-inspired metallopolymers. Using state-of-the-art design strategies, it is now possible to perform targeted synthesis of macromolecules with varied complexity that contain a range of metal centers either in the backbone or in the side chains of the organic moiety. The presence of an inorganic element (metals and metal centers) in organic moieties has led to a number of new physicochemical properties while implementing novel functionality to the polymer matrix. This review covers nanotechnology influenced by distinctive features of metal-containing macromolecular systems, particularly in developing flexible, functionalmaterials. (C) 2013 Society of Chemical industry
C1 [Ramanathan, Muruganathan] Oak Ridge Natl Lab, CNMS, Oak Ridge, TN 37831 USA.
[Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
[Darling, Seth B.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA.
RP Ramanathan, M (reprint author), Oak Ridge Natl Lab, CNMS, Oak Ridge, TN 37831 USA.
EM nmr@ornl.gov
FU Center for Nanoscale Materials, a US Department of Energy, Office of
Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Scientific
User Facilities Division, Office of Basic Energy Sciences, US Department
of Energy
FX This research was conducted at the Center for Nanophase Materials
Sciences, which is sponsored at Oak Ridge National Laboratory by the
Scientific User Facilities Division, Office of Basic Energy Sciences, US
Department of Energy. This work was performed, in part, at the Center
for Nanoscale Materials, a US Department of Energy, Office of Science,
Office of Basic Energy Sciences User Facility under Contract No.
DE-AC02-06CH11357.
NR 189
TC 11
Z9 11
U1 3
U2 39
PU WILEY
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0959-8103
EI 1097-0126
J9 POLYM INT
JI Polym. Int.
PD AUG
PY 2013
VL 62
IS 8
BP 1123
EP 1134
DI 10.1002/pi.4541
PG 12
WC Polymer Science
SC Polymer Science
GA 296NE
UT WOS:000330191000001
ER
PT J
AU Schneider, CM
Fadley, CS
AF Schneider, Claus M.
Fadley, Charles S.
TI Magnetic spectroscopies Introduction
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Editorial Material
ID MAGNETORESISTANCE; FERROMAGNETISM
C1 [Schneider, Claus M.] Peter Gruenberg Inst PGI 6, Res Ctr, D-52425 Julich, Germany.
[Schneider, Claus M.] Univ Duisburg Essen, Fac Phys, D-47057 Duisburg, Germany.
[Fadley, Charles S.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA.
[Fadley, Charles S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Schneider, CM (reprint author), Peter Gruenberg Inst PGI 6, Res Ctr, D-52425 Julich, Germany.
EM c.m.schneider@fz-juelich.de; fadley@physics.ucdavis.edu
RI Schneider, Claus/H-7453-2012
OI Schneider, Claus/0000-0002-3920-6255
NR 10
TC 0
Z9 0
U1 1
U2 5
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2013
VL 189
BP 127
EP 128
DI 10.1016/j.elspec.2013.05.002
PG 2
WC Spectroscopy
SC Spectroscopy
GA 285VL
UT WOS:000329423000022
ER
PT J
AU Tober, ED
Palomares, FJ
Ynzunza, RX
Denecke, R
Morais, J
Liesegang, J
Hussain, Z
Shick, AB
Pickett, WE
Fadley, CS
AF Tober, Eric D.
Palomares, F. Javier
Ynzunza, Ramon X.
Denecke, Reinhard
Morais, Jonder
Liesegang, John
Hussain, Zahid
Shick, Alexander B.
Pickett, Warren E.
Fadley, Charles S.
TI Observation of dynamical spin-dependent electron interactions and
screening in magnetic transitions via core-level multiplet-energy
separations
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Article
DE Photoemission; Multiplet splittings; Magnetic transitions; Screening,
Free-electron lasers
ID POLARIZED PHOTOELECTRON DIFFRACTION; BINDING ENERGIES; GD(0001) SURFACE;
PHOTOEMISSION; GD; METALS; ORDER; FILMS
AB The magnetic phase transitions for Gd(0 0 0 1) grown on W(1 1 0) - a bulk transition at 293 K and a surface transition about 85 K above this - are found to influence the energy separation of the Gd 5s and 4s core-photoelectron doublets. The 5s doublet separation Delta E-5s changes over a range of temperatures spanning these transitions, and decreases by a maximum of 60 meV in this region, but then recovers its original value; the 4s doublet shows a smaller change in the reverse direction, which does not recover at high temperature. Some of these effects are semi-quantitatively understood from free-atom multiplet theory and from theoretical calculations based on all-electron LDA+U calculations including 4f electron correlation effects. However, the high-temperature behavior of the data also suggest a dynamical nature to these effects via spin-dependent electron screening that is influenced by magnetic fluctuations. Several avenues for studying such effects in a time-resolved manner in future experiments are discussed. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Tober, Eric D.; Palomares, F. Javier; Ynzunza, Ramon X.; Denecke, Reinhard; Shick, Alexander B.; Pickett, Warren E.; Fadley, Charles S.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA.
[Tober, Eric D.; Palomares, F. Javier; Ynzunza, Ramon X.; Denecke, Reinhard; Morais, Jonder; Liesegang, John; Fadley, Charles S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Liesegang, John] La Trobe Univ, Dept Phys, Melbourne, Vic 3086, Australia.
[Hussain, Zahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
RP Fadley, CS (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA.
EM fadley@lbl.gov
RI Morais, Jonder/E-5022-2013; Shick, Alexander/C-1420-2013; Register,
CMSS/G-7191-2015; Palomares, Francisco Javier/C-4605-2011
OI Morais, Jonder/0000-0002-4143-1208; Shick,
Alexander/0000-0003-2700-5517; Palomares, Francisco
Javier/0000-0002-4768-2219
FU Office of Energy Research, Mat. Sci. Div., of the U.S. Dept. of Energy
[DE-AC03-76SF00098, DE-AC02-05CH11231]; DGICyT MEC, Spain
[PB94-0022-C02-02]; DOE [DE-FG03-03NA00071]
FX Support was provided by the Director, Office of Energy Research, Mat.
Sci. Div., of the U.S. Dept. of Energy, under Contracts No.
DE-AC03-76SF00098 and DE-AC02-05CH11231, and the DGICyT (Grant No.
PB94-0022-C02-02) MEC, Spain. Work at UC Davis (W.E.P.) was supported in
part by DOE grant No. DE-FG03-03NA00071.
NR 42
TC 1
Z9 1
U1 1
U2 11
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2013
VL 189
BP 152
EP 156
DI 10.1016/j.elspec.2012.12.009
PG 5
WC Spectroscopy
SC Spectroscopy
GA 285VL
UT WOS:000329423000026
ER
PT J
AU Kortright, JB
AF Kortright, Jeffrey B.
TI Resonant soft X-ray and extreme ultraviolet magnetic scattering in
nanostructured magnetic materials: Fundamentals and directions
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Article
DE Resonant soft X-ray magnetic scattering; Nanostructured magnetic
materials; Energy spectra; Polarization dependence; Kerr rotation
ID DEPTH-SENSITIVE PROBE; CIRCULAR-DICHROISM; EXCHANGE SCATTERING;
FARADAY-ROTATION; RECORDING MEDIA; THIN-FILMS; FE; MULTILAYER;
POLARIZATION; EDGES
AB Theoretical and practical aspects of resonant magnetic and charge scattering in the soft X-ray and extreme ultraviolet spectral ranges are reviewed. Intensity-only measurements are considered because they are more efficient than polarization-resolving measurements. Two very different approaches are discussed and compared; transmission small-angle scattering described by a simple kinematical scattering model and specular reflection described by more complex yet standard magneto-optical formalisms. In both cases the scattered intensity is seen to contain distinct terms resulting from pure-charge scattering, pure-magnetic scattering, and charge-magnetic cross-terms, and emphasis is placed on distinguishing these contributions via their energy spectra and its dependence on incident polarization. Combined with measurements vs. scattering vector q, both approaches provide significant capability to resolve magnetic and chemical structure down to nanometer length scales. The role of and need for modeling to obtain reliable information from data is discussed, as are current directions and opportunities. (C) 2013 Elsevier B.V. All rights reserved.
C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Kortright, JB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM JBKortright@lbl.gov
FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of
Materials Science [DE-AC02-05CH11231]
FX This work, including measurements conducted at beamlines 8.0.1, 4.0.2,
and 6.3.2 at the Advanced Light Source (LBNL), was supported by the U.S.
Department of Energy, Office of Basic Energy Sciences, Division of
Materials Science under Contract no. DE-AC02-05CH11231.
NR 76
TC 3
Z9 3
U1 0
U2 10
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2013
VL 189
BP 178
EP 186
DI 10.1016/j.elspec.2013.01.019
PG 9
WC Spectroscopy
SC Spectroscopy
GA 285VL
UT WOS:000329423000030
ER
PT J
AU Fischer, P
Im, MY
Baldasseroni, C
Bordel, C
Hellman, F
Lee, JS
Fadley, CS
AF Fischer, Peter
Im, Mi-Young
Baldasseroni, Chloe
Bordel, Catherine
Hellman, Frances
Lee, Jong-Soo
Fadley, Charles S.
TI Magnetic imaging with full-field soft X-ray microscopies
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Article
DE X-ray magnetic dichroism; Soft X-ray spectromicroscopy; Spin dynamics;
Fresnel zone plates; Mesoscale magnetism; Photoelectron microscopy;
X-PEEM
ID CIRCULAR-DICHROISM; ELECTRON-MICROSCOPY; ANTIFERROMAGNETIC DOMAINS;
MAGNETORESISTANCE; MEMORY; FILMS
AB Progress toward a fundamental understanding of magnetism continues to be of great scientific interest and high technological relevance. To control magnetization on the nanoscale, external magnetic fields and spin polarized currents are commonly used. In addition, novel concepts based on spin manipulation by electric fields or photons are emerging which benefit from advances in tailoring complex magnetic materials. Although the nanoscale is at the very origin of magnetic behavior, there is a new trend toward investigating mesoscale magnetic phenomena, thus adding complexity and functionality, both of which will become crucial for future magnetic devices.
Advanced analytical tools are thus needed for the characterization of magnetic properties spanning the nano- to the meso-scale. Imaging magnetic structures with high spatial and temporal resolution over a large field of view and in three dimensions is therefore a key challenge. A variety of spectromicroscopic techniques address this challenge by taking advantage of variable-polarization soft X-rays, thus enabling X-ray dichroism effects provide magnetic contrast. These techniques are also capable of quantifying in an element-, valence- and site-sensitive way the basic properties of ferro(i)- and antiferro-magnetic systems, such as spin and orbital moments, spin configurations from the nano- to the meso-scale and spin dynamics with sub-ns time resolution.
This paper reviews current achievements and outlines future trends with one of these spectromicroscopies, magnetic full field transmission soft X-ray microscopy (MTXM) using a few selected examples of recent research on nano- and meso-scale magnetic phenomena. The complementarity of MTXM to X-ray photoemission electron microscopy (X-PEEM) is also emphasized. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Fischer, Peter; Im, Mi-Young] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA.
[Baldasseroni, Chloe] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Bordel, Catherine; Hellman, Frances] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Bordel, Catherine; Hellman, Frances; Fadley, Charles S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94270 USA.
[Lee, Jong-Soo] DGIST, Dept Energy Syst Engn, Taegu 711873, South Korea.
[Fadley, Charles S.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA.
RP Fischer, P (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM PJFischer@lbl.gov
RI Fischer, Peter/A-3020-2010; Lee, Jong-Soo /F-7461-2010
OI Fischer, Peter/0000-0002-9824-9343; Lee, Jong-Soo /0000-0002-3045-2206
FU Office of Science, Office of Basic Energy Sciences, Materials Sciences
and Engineering Division, of the U.S. Department of Energy
[DE-AC02-05-CH11231]; Leading Foreign Research Institute Recruitment
Program through the National Research Foundation (NRF) of Korea;
Ministry of Education, Science and Technology (MEST) [2012K1A4A3053565]
FX This work was supported by the Director, Office of Science, Office of
Basic Energy Sciences, Materials Sciences and Engineering Division, of
the U.S. Department of Energy under contract no. DE-AC02-05-CH11231 and
by Leading Foreign Research Institute Recruitment Program through the
National Research Foundation (NRF) of Korea funded by the Ministry of
Education, Science and Technology (MEST) (2012K1A4A3053565).
NR 52
TC 4
Z9 4
U1 4
U2 32
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2013
VL 189
BP 196
EP 205
DI 10.1016/j.elspec.2013.03.012
PG 10
WC Spectroscopy
SC Spectroscopy
GA 285VL
UT WOS:000329423000032
ER
PT J
AU Ruan, LL
Robertson, GP
AF Ruan, Leilei
Robertson, G. Philip
TI Initial nitrous oxide, carbon dioxide, and methane costs of converting
conservation reserve program grassland to row crops under no-till vs.
conventional tillage
SO GLOBAL CHANGE BIOLOGY
LA English
DT Article
DE carbon dioxide; conservation reserve program; global warming impact;
greenhouse gas balance; methane; nitrous oxide; no-till; tillage
ID GREENHOUSE-GAS FLUXES; SOIL ORGANIC-CARBON; LONG-TERM; N2O EMISSIONS;
MANAGEMENT; SYSTEMS; CO2; SEQUESTRATION; ROTATION; MATTER
AB Around 4.4 millionha of land in USDA Conservation Reserve Program (CRP) contracts will expire between 2013 and 2018 and some will likely return to crop production. No-till (NT) management offers the potential to reduce the global warming costs of CO2, CH4, and N2O emissions during CRP conversion, but to date there have been no CRP conversion tillage comparisons. In 2009, we converted portions of three 9-21ha CRP fields in Michigan to conventional tillage (CT) or NT soybean production and reserved a fourth field for reference. Both CO2 and N2O fluxes increased following herbicide application in all converted fields, but in the CT treatment substantial and immediate N2O and CO2 fluxes occurred after tillage. For the initial 201-day conversion period, average daily N2O fluxes (g N2O-Nha(-1)d(-1)) were significantly different in the order: CT (47.5 +/- 6.31, n=6)>> NT (16.7 +/- 2.45, n=6)>> reference (2.51 +/- 0.73, n=4). Similarly, soil CO2 fluxes in CT were 1.2 times those in NT and 3.1 times those in the unconverted CRP reference field. All treatments were minor sinks for CH4 (-0.69 +/- 0.42 to -1.86 +/- 0.37g CH4-Cha(-1)d(-1)) with no significant differences among treatments. The positive global warming impact (GWI) of converted soybean fields under both CT (11.5 Mg CO(2)eha(-1)) and NT (2.87 Mg CO(2)eha(-1)) was in contrast to the negative GWI of the unconverted reference field (-3.5 Mg CO(2)eha(-1)) with on-going greenhouse gas (GHG) mitigation. N2O contributed 39.3% and 55.0% of the GWI under CT and NT systems with the remainder contributed by CO2 (60.7% and 45.0%, respectively). Including foregone mitigation, we conclude that NT management can reduce GHG costs by 60% compared to CT during initial CRP conversion.
C1 [Ruan, Leilei; Robertson, G. Philip] Michigan State Univ, WK Kellogg Biol Stn, Dept Plant Soil & Microbial Sci, Great Lakes Bioenergy Res Ctr, Hickory Corners, MI 49060 USA.
RP Ruan, LL (reprint author), Michigan State Univ, WK Kellogg Biol Stn, Dept Plant Soil & Microbial Sci, Great Lakes Bioenergy Res Ctr, Hickory Corners, MI 49060 USA.
EM ruanleil@msu.edu
OI Robertson, G/0000-0001-9771-9895
FU US DOE Office of Science [DE-FCO2-07ER64494]; Office of Energy
Efficiency and Renewable Energy [DE-ACO5-76RL01830]; US National Science
Foundation LTER Program [DEB 1027253]; MSU AgBioResearch
FX We thank P. Jasrotia, S. VanderWulp, E. Robertson, K. Kahmark, C.
McMinn, S. Sippel, S. Bohm and many others for assistance in the field
and laboratory. We thank T. Zenone for help with the Eddy Covariances
data. We also thank A.N. Kravchenko and S.K Hamilton for many helpful
suggestions and insightful comments. Financial support was provided by
the US DOE Office of Science (DE-FCO2-07ER64494) and Office of Energy
Efficiency and Renewable Energy (DE-ACO5-76RL01830), the US National
Science Foundation LTER Program (DEB 1027253), and MSU AgBioResearch.
NR 50
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U1 7
U2 69
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1354-1013
EI 1365-2486
J9 GLOBAL CHANGE BIOL
JI Glob. Change Biol.
PD AUG
PY 2013
VL 19
IS 8
BP 2478
EP 2489
DI 10.1111/gcb.12216
PG 12
WC Biodiversity Conservation; Ecology; Environmental Sciences
SC Biodiversity & Conservation; Environmental Sciences & Ecology
GA 276IV
UT WOS:000328744900015
PM 23553929
ER
PT J
AU Liu, HY
Williams, AP
Allen, CD
Guo, DL
Wu, XC
Anenkhonov, OA
Liang, EY
Sandanov, DV
Yin, Y
Qi, ZH
Badmaeva, NK
AF Liu, Hongyan
Williams, A. Park
Allen, Craig D.
Guo, Dali
Wu, Xiuchen
Anenkhonov, Oleg A.
Liang, Eryuan
Sandanov, Denis V.
Yin, Yi
Qi, Zhaohuan
Badmaeva, Natalya K.
TI Rapid warming accelerates tree growth decline in semi-arid forests of
Inner Asia
SO GLOBAL CHANGE BIOLOGY
LA English
DT Article
DE drought; forest die-off; Inner Asia; semi-arid; semi-humid; tree growth
decline; tree ring
ID CHANGE-TYPE DROUGHT; CLIMATE SYSTEM; GLOBAL DATASET; CHINESE PINE;
DIE-OFF; MORTALITY; VEGETATION; MONGOLIA; RECONSTRUCTION; VARIABILITY
AB Forests around the world are subject to risk of high rates of tree growth decline and increased tree mortality from combinations of climate warming and drought, notably in semi-arid settings. Here, we assess how climate warming has affected tree growth in one of the world's most extensive zones of semi-arid forests, in Inner Asia, a region where lack of data limits our understanding of how climate change may impact forests. We show that pervasive tree growth declines since 1994 in Inner Asia have been confined to semi-arid forests, where growing season water stress has been rising due to warming-induced increases in atmospheric moisture demand. A causal link between increasing drought and declining growth at semi-arid sites is corroborated by correlation analyses comparing annual climate data to records of tree-ring widths. These ring-width records tend to be substantially more sensitive to drought variability at semi-arid sites than at semi-humid sites. Fire occurrence and insect/pathogen attacks have increased in tandem with the most recent (2007-2009) documented episode of tree mortality. If warming in Inner Asia continues, further increases in forest stress and tree mortality could be expected, potentially driving the eventual regional loss of current semi-arid forests.
C1 [Liu, Hongyan; Wu, Xiuchen; Yin, Yi; Qi, Zhaohuan] Peking Univ, Coll Urban & Environm Sci, Beijing 100871, Peoples R China.
[Williams, A. Park] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA.
[Allen, Craig D.] US Geol Survey, Jemez Mt Field Stn, Ft Collins Sci Ctr, Los Alamos, NM 87544 USA.
[Guo, Dali] Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China.
[Anenkhonov, Oleg A.; Sandanov, Denis V.; Badmaeva, Natalya K.] Russian Acad Sci, Siberian Branch, Inst Gen & Expt Biol, Ulan Ude 670047, Russia.
[Liang, Eryuan] Chinese Acad Sci, Inst Tibetan Plateau Res, Beijing 100085, Peoples R China.
RP Liu, HY (reprint author), Peking Univ, Coll Urban & Environm Sci, Beijing 100871, Peoples R China.
EM lhy@urban.pku.edu.cn; craig_allen@usgs.gov
RI Guo, Dali/G-2158-2014; Liang, Eryuan/A-1435-2010; Guo, Dali/C-3498-2012;
Williams, Park/B-8214-2016; Anenkhonov, Oleg/J-8690-2016
OI Liang, Eryuan/0000-0002-8003-4264; Williams, Park/0000-0001-8176-8166;
Anenkhonov, Oleg/0000-0001-8633-7154
FU National Natural Science Foundation of China [NSFC 41071124,
40711120173, 41011120251]; Russian Foundation of Basic Research [RFBR
13-04-91180, 10-04-91159]; US Geological Survey Climate and Land Use
Change Program; LANL-LDRD; DOE-BER
FX This study was supported by grants from the National Natural Science
Foundation of China (NSFC 41071124, 40711120173 and 41011120251) and the
Russian Foundation of Basic Research (RFBR 13-04-91180 and 10-04-91159);
CDA was supported by the US Geological Survey Climate and Land Use
Change Program, and APW was supported by LANL-LDRD and DOE-BER. We thank
Y. Guo, J. Ren, and S. He for their helps in tree-ring sampling, and J.
Dai for providing the Liupan Mt. raw ring-width data. The authors stated
no conflict of interest.
NR 55
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U1 15
U2 107
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1354-1013
EI 1365-2486
J9 GLOBAL CHANGE BIOL
JI Glob. Change Biol.
PD AUG
PY 2013
VL 19
IS 8
BP 2500
EP 2510
DI 10.1111/gcb.12217
PG 11
WC Biodiversity Conservation; Ecology; Environmental Sciences
SC Biodiversity & Conservation; Environmental Sciences & Ecology
GA 276IV
UT WOS:000328744900017
PM 23564688
ER
PT J
AU Hanson, D
Schmalzer, D
AF Hanson, Donald
Schmalzer, David
TI An adoption scenario for carbon capture in pulverized coal power plants
in the USA
SO GREENHOUSE GASES-SCIENCE AND TECHNOLOGY
LA English
DT Article
DE carbon capture; CO2 reduction; electric generation; energy scenario;
energy policy; ESIM; greenhouse gases
AB In this paper we use the Electricity Supply and Investment Model (ESIM) power system model to examine the energy market effects of incentivized adoption of carbon capture and storage (CCS), with a primary focus on retrofitting existing pulverized coal plants. In the presence of a medium' carbon charge and least-cost dispatch, units with CCS are operated with higher utilization rates than fossil energy plants without carbon capture, hence lowering CO2 emissions. This path helps to lower the capital outlays that will be necessary to make a transition to a full portfolio of advanced low-carbon technologies. Required research, development and demonstration can be financed by a portion of the carbon charge revenue. (C) 2013 Society of Chemical Industry and John Wiley & Sons, Ltd
C1 [Hanson, Donald; Schmalzer, David] Argonne Natl Lab, Lemont, IL 60439 USA.
RP Hanson, D (reprint author), Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA.
EM dhanson@anl.gov
FU US National Energy Technology Laboratory (NETL)
FX The authors would like to thank the US National Energy Technology
Laboratory (NETL) for support.
NR 4
TC 1
Z9 1
U1 0
U2 3
PU WILEY PERIODICALS, INC
PI SAN FRANCISCO
PA ONE MONTGOMERY ST, SUITE 1200, SAN FRANCISCO, CA 94104 USA
SN 2152-3878
J9 GREENH GASES
JI Greenh. Gases
PD AUG
PY 2013
VL 3
IS 4
BP 303
EP 308
DI 10.1002/ghg.1359
PG 6
WC Energy & Fuels; Engineering, Environmental; Environmental Sciences
SC Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 267ZV
UT WOS:000328138100007
ER
PT J
AU Sepsova, V
Karasova, JZ
Korabecny, J
Dolezal, R
Zemek, F
Bennion, BJ
Kuca, K
AF Sepsova, Vendula
Karasova, Jana Zdarova
Korabecny, Jan
Dolezal, Rafael
Zemek, Filip
Bennion, Brian J.
Kuca, Kamil
TI Oximes: Inhibitors of Human Recombinant Acetylcholinesterase. A
Structure-Activity Relationship (SAR) Study
SO INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
LA English
DT Article
DE oximes; acetylcholinesterase; inhibitors; SAR study
ID BISPYRIDINIUM COMPOUNDS BEARING; REACTIVATION ACTIVITY;
THERAPEUTIC-EFFICACY; PYRIDINIUM OXIMES; DIAGNOSIS; AGENTS; BRAIN;
TABUN; LINKER
AB Acetylcholinesterase (AChE) reactivators were developed for the treatment of organophosphate intoxication. Standard care involves the use of anticonvulsants (e.g., diazepam), parasympatolytics (e.g., atropine) and oximes that restore AChE activity. However, oximes also bind to the active site of AChE, simultaneously acting as reversible inhibitors. The goal of the present study is to determine how oxime structure influences the inhibition of human recombinant AChE (hrAChE). Therefore, 24 structurally different oximes were tested and the results compared to the previous eel AChE (EeAChE) experiments. Structural factors that were tested included the number of pyridinium rings, the length and structural features of the linker, and the number and position of the oxime group on the pyridinium ring.
C1 [Sepsova, Vendula; Korabecny, Jan; Zemek, Filip] Univ Def, Fac Mil Hlth Sci, Dept Toxicol, Hradec Kralove 50001, Czech Republic.
[Karasova, Jana Zdarova] Univ Def, Fac Mil Hlth Sci, Dept Publ Hlth, Hradec Kralove 50001, Czech Republic.
[Karasova, Jana Zdarova; Korabecny, Jan; Dolezal, Rafael; Kuca, Kamil] Univ Hosp, Biomed Res Ctr, Hradec Kralove 50005, Czech Republic.
[Bennion, Brian J.] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Livermore, CA 94550 USA.
[Kuca, Kamil] Univ Def, Fac Mil Hlth Sci, Ctr Adv Studies, Hradec Kralove 50001, Czech Republic.
RP Kuca, K (reprint author), Univ Hosp, Biomed Res Ctr, Sokolska 581, Hradec Kralove 50005, Czech Republic.
EM sepsova@pmfhk.cz; karasova@pmfhk.cz; korabecny@pmfhk.cz;
rafael.dolezal@fnhk.cz; zemek.filip@gmail.com; Bennion1@llnl.gov;
kamil.kuca@fnhk.cz
RI Dolezal, Rafael/B-3956-2017
FU Ministry of Defence; Ministry of Education, Youth and Sports
[SV/FVZ201104]; MH CZ-DRO (University Hospital Hradec Kralove)
[00179906]; U.S. Department of Energy, National Nuclear Security
Administration [DE-AC52-07NA27344]; [CZ.1.07/2.3.00/30.0044]
FX This work was supported by the project of Ministry of Defence, A
long-term organization development plan 1011, by project of Ministry of
Education, Youth and Sports, SV/FVZ201104, by MH CZ-DRO (University
Hospital Hradec Kralove, No. 00179906) and by Post-doctoral project (No.
CZ.1.07/2.3.00/30.0044). Lawrence Livermore National Laboratory is
operated by Lawrence Livermore National Security, LLC, for the U.S.
Department of Energy, National Nuclear Security Administration under
Contract DE-AC52-07NA27344. The access to computing and storage
facilities owned by parties and projects contributing to the National
Grid Infrastructure MetaCentrum, provided under the program "Projects of
Large Infrastructure for Research, Development, and Innovations"
(LM2010005) is highly appreciated.
NR 34
TC 12
Z9 12
U1 1
U2 25
PU MDPI AG
PI BASEL
PA POSTFACH, CH-4005 BASEL, SWITZERLAND
SN 1422-0067
J9 INT J MOL SCI
JI Int. J. Mol. Sci.
PD AUG
PY 2013
VL 14
IS 8
BP 16882
EP 16900
DI 10.3390/ijms140816882
PG 19
WC Biochemistry & Molecular Biology; Chemistry, Multidisciplinary
SC Biochemistry & Molecular Biology; Chemistry
GA 272ZE
UT WOS:000328501300086
PM 23959117
ER
PT J
AU Nakayasu, ES
Brown, RN
Ansong, C
Sydor, MA
Imtiaz, S
Mihai, C
Sontag, R
Hixson, KK
Monroe, ME
Sobreira, TJP
Orr, G
Petyuk, VA
Yang, F
Smith, RD
Adkins, JN
AF Nakayasu, Ernesto S.
Brown, Roslyn N.
Ansong, Charles
Sydor, Michael A.
Imtiaz, Sayed
Mihai, Cosmin
Sontag, Ryan
Hixson, Kim K.
Monroe, Matthew E.
Sobreira, Tiago J. P.
Orr, Galya
Petyuk, Vladislav A.
Yang, Feng
Smith, Richard D.
Adkins, Joshua N.
TI Multi-omic Data Integration Links Deleted in Breast Cancer 1 (DBC1)
Degradation to Chromatin Remodeling in Inflammatory Response
SO MOLECULAR & CELLULAR PROTEOMICS
LA English
DT Article
ID NF-KAPPA-B; INNATE IMMUNE-RESPONSES; GENE-EXPRESSION; SIGNALING PATHWAY;
BINDING PROTEIN; MACROPHAGES; ACTIVATION; PROTEASOME; ALPHA;
PHOSPHORYLATION
AB This study investigated the dynamics of ubiquitinated proteins after the inflammatory stimulation of RAW 264.7 macrophage-like cells with bacterial lipopolysaccharide. Ubiquitination is a common protein post-translational modification that regulates many key cellular functions. We demonstrated that levels of global ubiquitination and K48 and K63 polyubiquitin chains change after lipopolysaccharide stimulation. Quantitative proteomic analysis identified 1199 ubiquitinated proteins, 78 of which exhibited significant changes in ubiquitination levels following stimulation. Integrating the ubiquitinome data with global proteomic and transcriptomic results allowed us to identify a subset of 88 proteins that were targeted for degradation after lipopolysaccharide stimulation. Using cellular assays and Western blot analyses, we biochemically validated DBC1 (a histone deacetylase inhibitor) as a degradation substrate that is targeted via an orchestrated mechanism utilizing caspases and the proteasome. The degradation of DBC1 releases histone deacetylase activity, linking lipopolysaccharide activation to chromatin remodeling in caspase- and proteasome-mediated signaling.
C1 [Nakayasu, Ernesto S.; Ansong, Charles; Sydor, Michael A.; Imtiaz, Sayed; Sontag, Ryan; Monroe, Matthew E.; Petyuk, Vladislav A.; Yang, Feng; Smith, Richard D.; Adkins, Joshua N.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
[Brown, Roslyn N.] Washington State Univ, Ctr Bioprod & Bioenergy, Richland, WA 99354 USA.
[Mihai, Cosmin; Hixson, Kim K.; Orr, Galya] Pacific NW Natl Lab, Environm & Mol Sci Lab, Richland, WA 99352 USA.
[Sobreira, Tiago J. P.] Natl Ctr Res Energy & Mat, Natl Lab Biosci LN Bio, BR-13083970 Campinas, SP, Brazil.
RP Adkins, JN (reprint author), Pacific NW Natl Lab, Div Biol Sci, POB 999,MSIN K8-98, Richland, WA 99352 USA.
EM Joshua.Adkins@pnnl.gov
RI Smith, Richard/J-3664-2012; Sobreira, Tiago/C-1276-2008;
OI Smith, Richard/0000-0002-2381-2349; Sobreira, Tiago/0000-0002-0217-0084;
Petyuk, Vladislav/0000-0003-4076-151X
FU NIAID (National Institutes of Health/DHHS) [Y1-AI-8494-01]; NIGMS,
National Institutes of Health [GM094623]; NIH [5P41RR018522-10]; NIGMS
[8 P41 GM103493-10]; U.S. Department of Energy Office of Biological and
Environmental Research (DOE/BER); DOE [DE-AC05-76RLO1830]
FX This work was supported by NIAID (National Institutes of Health/DHHS)
through interagency agreement The proper number is: Y1-AI-8494-01 and
NIGMS, National Institutes of Health (GM094623). This work used
instrumentation and capabilities developed with support from NIH Grant
No. 5P41RR018522-10, NIGMS Grant No. 8 P41 GM103493-10, and the U.S.
Department of Energy Office of Biological and Environmental Research
(DOE/BER). Significant portions of this work were performed in the EMSL,
a DOE/BER national scientific user facility located at Pacific Northwest
National Laboratory. The Pacific Northwest National Laboratory is
operated for the DOE by Battelle under Contract DE-AC05-76RLO1830.
NR 53
TC 2
Z9 2
U1 0
U2 7
PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC
PI BETHESDA
PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA
SN 1535-9476
EI 1535-9484
J9 MOL CELL PROTEOMICS
JI Mol. Cell. Proteomics
PD AUG
PY 2013
VL 12
IS 8
BP 2136
EP 2147
DI 10.1074/mcp.M112.026138
PG 12
WC Biochemical Research Methods
SC Biochemistry & Molecular Biology
GA 277SH
UT WOS:000328839100009
PM 23639857
ER
PT J
AU Dunagan, SE
Johnson, R
Zavaleta, J
Russell, PB
Schmid, B
Flynn, C
Redemann, J
Shinozuka, Y
Livingston, J
Segal-Rosenhaimer, M
AF Dunagan, Stephen E.
Johnson, Roy
Zavaleta, Jhony
Russell, Philip B.
Schmid, Beat
Flynn, Connor
Redemann, Jens
Shinozuka, Yohei
Livingston, John
Segal-Rosenhaimer, Michal
TI Spectrometer for Sky-Scanning Sun-Tracking Atmospheric Research (4STAR):
Instrument Technology
SO REMOTE SENSING
LA English
DT Article
DE atmosphere; climate; pollution; radiometry; technology; hyperspectral;
fiber optic
ID AEROSOL OPTICAL DEPTH; VERTICAL PROFILES; AIRBORNE; RETRIEVAL
AB The Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) combines airborne sun tracking and sky scanning with diffraction spectroscopy to improve knowledge of atmospheric constituents and their links to air-pollution/climate. Direct beam hyper-spectral measurement of optical depth improves retrievals of gas constituents and determination of aerosol properties. Sky scanning enhances retrievals of aerosol type and size distribution. 4STAR measurements will tighten the closure between satellite and ground-based measurements. 4STAR incorporates a modular sun-tracking/sky-scanning optical head with fiber optic signal transmission to rack mounted spectrometers, permitting miniaturization of the external optical head, and future detector evolution. Technical challenges include compact optical collector design, radiometric dynamic range and stability, and broad spectral coverage. Test results establishing the performance of the instrument against the full range of operational requirements are presented, along with calibration, engineering flight test, and scientific field campaign data and results.
C1 [Dunagan, Stephen E.; Johnson, Roy; Zavaleta, Jhony; Russell, Philip B.; Redemann, Jens; Segal-Rosenhaimer, Michal] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA.
[Schmid, Beat; Flynn, Connor] Pacific NW Natl Lab, Richland, WA 99325 USA.
[Shinozuka, Yohei] NASA, Ames Cooperat Res Earth Sci & Technol ARC CREST, Moffett Field, CA 94035 USA.
[Shinozuka, Yohei] Bay Area Environm Res Inst, Sonoma, CA 95476 USA.
[Livingston, John] SRI Int, Menlo Pk, CA 94025 USA.
RP Dunagan, SE (reprint author), NASA, Ames Res Ctr, MS 245-4, Moffett Field, CA 94035 USA.
EM Stephen.E.Dunagan@nasa.gov; Roy.R.Johnson@nasa.gov;
Jhony.R.Zavaleta@nasa.gov; Philip.B.Russell@nasa.gov;
beat.schmid@pnnl.gov; connor.flynn@pnnl.gov; Jens.Redemann-1@nasa.gov;
Yohei.Shinozuka@nasa.gov; John.M.Livingston@nasa.gov;
Michal.Segalrozenhaimer@nasa.gov
FU NASA Radiation Science Program; Ames Instrument Working Group; DOE
Atmospheric Radiation Measurement Program, Battelle's Pacific Northwest
Division; NOAA Office of Global Programs
FX 4STAR design, development, and testing were supported by the NASA
Radiation Science Program, the Ames Instrument Working Group, the DOE
Atmospheric Radiation Measurement Program, Battelle's Pacific Northwest
Division, and the NOAA Office of Global Programs. Instrument conceptual
advice and scientific data analysis software were provided by the NASA
Goddard AERONET group under the leadership of Brent Holben.
NR 18
TC 10
Z9 10
U1 0
U2 8
PU MDPI AG
PI BASEL
PA POSTFACH, CH-4005 BASEL, SWITZERLAND
SN 2072-4292
J9 REMOTE SENS-BASEL
JI Remote Sens.
PD AUG
PY 2013
VL 5
IS 8
BP 3872
EP 3895
DI 10.3390/rs5083872
PG 24
WC Remote Sensing
SC Remote Sensing
GA 274SI
UT WOS:000328626100011
ER
PT J
AU Jiang, N
Zhu, WQ
Zheng, ZT
Chen, GS
Fan, DQ
AF Jiang, Nan
Zhu, Wenquan
Zheng, Zhoutao
Chen, Guangsheng
Fan, Deqin
TI A Comparative Analysis between GIMSS NDVIg and NDVI3g for Monitoring
Vegetation Activity Change in the Northern Hemisphere during 1982-2008
SO REMOTE SENSING
LA English
DT Article
DE GIMMS; NDVI; vegetation; climate change; Northern Hemisphere
ID TERRESTRIAL CARBON SINK; SATELLITE DATA; TIME-SERIES; DATA SETS;
GREEN-UP; LAND; TRENDS; GROWTH; INDEX; PRODUCTIVITY
AB The long-term Normalized Difference Vegetation Index (NDVI) time-series data set generated from the Advanced Very High Resolution Radiometers (AVHRR) has been widely used to monitor vegetation activity change. The third version of NDVI (NDVI3g) produced by the Global Inventory Modeling and Mapping Studies (GIMMS) group was released recently. The comparisons between the new and old versions should be conducted for linking existing studies with future applications of NDVI3g in monitoring vegetation activity change. Based on simple and piecewise linear regression methods, this study made a comparative analysis between NDVIg and NDVI3g for monitoring vegetation activity change and its responses to climate change in the middle and high latitudes of the Northern Hemisphere during 1982-2008. Our results indicated that there were large differences between NDVIg and NDVI3g in the spatial patterns for both the overall changing trends and the timing of Turning Points (TP) in NDVI time series, which spread over almost the entire study region. The average NDVI trend from NDVI3g was almost twice as great as that from NDVIg and the detected average timing of TP from NDVI3g was about one year later. Although the general spatial patterns were consistent between two data sets for detecting the responses of growing-season NDVI to temperature and precipitation changes, there were large differences in the response magnitude, with a higher response magnitude to temperature in NDVI3g and an opposite response to precipitation change for the two data sets. These results demonstrated that the NDVIg data set may underestimate the vegetation activity change trend and its response to climate change in the middle and high latitudes of the Northern Hemisphere during the past three decades.
C1 [Jiang, Nan; Zhu, Wenquan; Zheng, Zhoutao; Fan, Deqin] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China.
[Jiang, Nan; Zhu, Wenquan; Zheng, Zhoutao; Fan, Deqin] Beijing Normal Univ, Coll Resources Sci & Technol, Beijing 100875, Peoples R China.
[Chen, Guangsheng] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA.
RP Zhu, WQ (reprint author), Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China.
EM jiangnan@mail.bnu.edu.cn; zhuwq75@bnu.edu.cn;
zhengzhoutao90@mail.bnu.edu.cn; kinly129@163.com; cheng@ornl.gov
FU National Basic Research Program of China [2011CB952001]; State Key
Laboratory of Earth Surface Processes and Resource Ecology [2013-ZY-14];
Fundamental Research Funds for the Central University
FX This work was supported by the National Basic Research Program of China
(Grant No. 2011CB952001), the State Key Laboratory of Earth Surface
Processes and Resource Ecology (Grant No. 2013-ZY-14), and the
Fundamental Research Funds for the Central University. We thank C. J.
Tucker, J. Pinzon, and R. B. Myneni for providing GIMMS NDVI3g data set
and valuable suggestions.
NR 35
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Z9 26
U1 3
U2 28
PU MDPI AG
PI BASEL
PA POSTFACH, CH-4005 BASEL, SWITZERLAND
SN 2072-4292
J9 REMOTE SENS-BASEL
JI Remote Sens.
PD AUG
PY 2013
VL 5
IS 8
BP 4031
EP 4044
DI 10.3390/rs5084031
PG 14
WC Remote Sensing
SC Remote Sensing
GA 274SI
UT WOS:000328626100017
ER
PT J
AU Nadziejka, DE
AF Nadziejka, David E.
TI What Editors Want: An Author's Guide to Scientific Journal Publishing
SO TECHNICAL COMMUNICATION
LA English
DT Book Review
C1 [Nadziejka, David E.] Van Andel Res Inst, Grand Rapids, MI USA.
[Nadziejka, David E.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Nadziejka, David E.] IIT, Chicago, IL 60616 USA.
RP Nadziejka, DE (reprint author), Van Andel Res Inst, Grand Rapids, MI USA.
NR 1
TC 0
Z9 0
U1 0
U2 0
PU SOC TECHNICAL COMMUNICATION
PI FAIRFAX
PA 9401 LEE HIGHWAY, STE 300, FAIRFAX, VA 22031 USA
SN 0049-3155
J9 TECH COMMUN-STC
JI Tech. Commun.
PD AUG
PY 2013
VL 60
IS 3
BP 248
EP 248
PG 1
WC Communication
SC Communication
GA 270OS
UT WOS:000328328700026
ER
PT J
AU Xie, JR
Kelley, S
Szymanski, BK
AF Xie, Jierui
Kelley, Stephen
Szymanski, Boleslaw K.
TI Overlapping Community Detection in Networks: The State-of-the-Art and
Comparative Study
SO ACM COMPUTING SURVEYS
LA English
DT Article
DE Algorithms; Performance; Overlapping community detection; social
networks
ID FUZZY C-MEANS; COMPLEX NETWORKS; MIXTURE-MODELS; RAND INDEX; ALGORITHM;
GRAPHS
AB This article reviews the state-of-the-art in overlapping community detection algorithms, quality measures, and benchmarks. A thorough comparison of different algorithms (a total of fourteen) is provided. In addition to community-level evaluation, we propose a framework for evaluating algorithms' ability to detect overlapping nodes, which helps to assess overdetection and underdetection. After considering community-level detection performance measured by normalized mutual information, the Omega index, and node-level detection performance measured by F-score, we reached the following conclusions. For low overlapping density networks, SLPA, OSLOM, Game, and COPRA offer better performance than the other tested algorithms. For networks with high overlapping density and high overlapping diversity, both SLPA and Game provide relatively stable performance. However, test results also suggest that the detection in such networks is still not yet fully resolved. A common feature observed by various algorithms in real-world networks is the relatively small fraction of overlapping nodes (typically less than 30%), each of which belongs to only 2 or 3 communities.
C1 [Xie, Jierui; Szymanski, Boleslaw K.] Rensselaer Polytech Inst, Dept Comp Sci, Troy, NY 12180 USA.
[Kelley, Stephen] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Xie, JR (reprint author), Rensselaer Polytech Inst, Dept Comp Sci, 110 8th St, Troy, NY 12180 USA.
EM jierui.xie@gmail.com
RI Szymanski, Boleslaw/A-9121-2009
OI Szymanski, Boleslaw/0000-0002-0307-6743
FU Army Research Laboratory [W911NF-09-2-0053]; Office of Naval Research
Grant [N00014-09-1-0607]
FX The work of J. Xie and B. K. Szymanski was supported in part by the Army
Research Laboratory under Cooperative Agreement Number W911NF-09-2-0053
and by the Office of Naval Research Grant No. N00014-09-1-0607. The
views and conclusions contained in this document are those of the
authors and should not be interpreted as representing the official
policies either expressed of implied of the Army Research Laboratory,
the Office of Naval Research, or the U.S. Government.
NR 99
TC 131
Z9 136
U1 9
U2 48
PU ASSOC COMPUTING MACHINERY
PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0360-0300
EI 1557-7341
J9 ACM COMPUT SURV
JI ACM Comput. Surv.
PD AUG
PY 2013
VL 45
IS 4
AR 43
DI 10.1145/2501654.2501657
PG 35
WC Computer Science, Theory & Methods
SC Computer Science
GA 265FA
UT WOS:000327934000003
ER
PT J
AU Miller, DJ
Proff, C
Wen, JG
Abraham, DP
Bareno, J
AF Miller, Dean J.
Proff, Christian
Wen, J. G.
Abraham, Daniel P.
Bareno, Javier
TI Observation of Microstructural Evolution in Li Battery Cathode Oxide
Particles by In Situ Electron Microscopy
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
ID LITHIUM-ION CELLS; STRUCTURAL-CHANGES; ELECTROCHEMICAL LITHIATION;
LITHIUM/POLYMER CELLS; DENDRITIC GROWTH; SNO2 NANOWIRE; POWER;
LINI0.8CO0.15AL0.05O2; SPECTROSCOPY; PERFORMANCE
AB We developed a simple approach to carry out in situ electron microscopy of single Li-ion battery cathode particles during electrochemical cycling. We focused on Li(Ni0.8Co0.15Al0.05)O-2-based cathode materials because life-cycle tests suggest a strong contribution of the cathode material to changes in cell impedance. In situ scanning electron microscopy was carried out operando during cycling and at various stages by interrupted cycling. Our work revealed several important aspects of cathode oxide particle dynamics: significant separations develop between grains even during the very first charge (oxide delithiation) and electrolyte penetration through that crack network all the way into the particle interior. Comparing these results to post-test microstructural characterization of oxide particles subjected to extensive cycling confirms the occurrence of these processes in practical cells and suggests that the physical separation and isolation of grains may contribute to performance degradation of lithium-ion cells.
C1 [Miller, Dean J.; Proff, Christian; Wen, J. G.] Argonne Natl Lab, Elect Microscopy Ctr, Argonne, IL 60439 USA.
[Miller, Dean J.; Proff, Christian; Wen, J. G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Abraham, Daniel P.; Bareno, Javier] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
RP Miller, DJ (reprint author), Argonne Natl Lab, Elect Microscopy Ctr, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM miller@anl.gov
OI Bareno, Javier/0000-0003-1230-9278
FU U.S. DOE EERE-Vehicle Technologies Program; Argonne Laboratory Directed
Research and Development [DE-AC02-06CH11357]; Office of Science - Basic
Energy Sciences
FX The valuable discussions and suggestions of Martin Bettge (ANL-CSE) are
gratefully acknowledged. The assistance of Nancy Miller, Christine
Miller, and Darren Miller in carrying out initial in situ measurements
is also gratefully acknolwedged. This research was supported by the U.S.
DOE EERE-Vehicle Technologies Program and by Argonne Laboratory Directed
Research and Development funding under contract DE-AC02-06CH11357. The
Electron Microscopy Center at Argonne is supported by the Office of
Science - Basic Energy Sciences.
NR 40
TC 47
Z9 47
U1 15
U2 132
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD AUG
PY 2013
VL 3
IS 8
BP 1098
EP 1103
DI 10.1002/aenm.201300015
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA 263FY
UT WOS:000327793600021
ER
PT J
AU Yakal-Kremski, K
Cronin, JS
Chen-Wiegart, YCK
Wang, J
Barnett, SA
AF Yakal-Kremski, K.
Cronin, J. S.
Chen-Wiegart, Y. -C. K.
Wang, J.
Barnett, S. A.
TI Studies of Solid Oxide Fuel Cell Electrode Evolution Using 3D Tomography
SO FUEL CELLS
LA English
DT Article; Proceedings Paper
CT 10th European SOFC Forum
CY JUN 26-29, 2012
CL Lucerne, SWITZERLAND
SP European Fuel Cell Forum
DE Degradation; Electrode; SOFC; Solid Oxide Fuel Cell; Three Dimensional
Tomography
ID MICROSTRUCTURE DEGRADATION; SOFC CATHODES; 3-DIMENSIONAL RECONSTRUCTION;
ELECTROCHEMICAL PROPERTIES; FIRING TEMPERATURE; ANODE DEGRADATION; YSZ;
PERFORMANCE; POLARIZATION; IMPURITIES
AB This paper describes 3D tomographic investigations of the structural evolution of Ni-yttria-stabilized zirconia (Ni-YSZ) and (La,Sr)MnO3-YSZ (LSM-YSZ) composite solid oxide fuel cell (SOFC) electrodes. Temperatures higher than normally used in SOFC operation are utilized to accelerate electrode evolution. Quantitative 3D FIB-SEM and X-ray tomographic imaging contributes to development of mechanistic evolution models needed to accurately predict long-term durability. Ni-YSZ anode functional layers annealed in humidified hydrogen at 900-1,100 degrees C exhibited microstructural coarsening leading to a decrease in three-phase boundary (TPB) density. There was also a change in the fraction of pores that were isolated, which impacted the density of electrochemically active TPBs. The polarization resistance of optimally fired LSM-YSZ electrodes increased upon thermal aging at 1,000 degrees C, whereas that of under-fired electrodes decreased upon aging. These results are explained in terms of observed 3D microstructural changes.
C1 [Yakal-Kremski, K.; Cronin, J. S.; Barnett, S. A.] Northwestern Univ, Dept Mat Sci, Evanston, IL 60208 USA.
[Chen-Wiegart, Y. -C. K.; Wang, J.] Brookhaven Natl Lab, Photon Source Directorate, Upton, NY 11973 USA.
RP Yakal-Kremski, K (reprint author), Northwestern Univ, Dept Mat Sci, Evanston, IL 60208 USA.
EM kkremski@u.northwestern.edu
RI Barnett, Scott/B-7502-2009
NR 40
TC 7
Z9 7
U1 5
U2 61
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1615-6846
EI 1615-6854
J9 FUEL CELLS
JI Fuel Cells
PD AUG
PY 2013
VL 13
IS 4
SI SI
BP 449
EP 454
DI 10.1002/fuce.201200177
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 262AO
UT WOS:000327706700001
ER
PT J
AU Zheng, BL
Li, Y
Xu, WZ
Zhou, YZ
Mathaudhu, SN
Zhu, YT
Lavernia, EJ
AF Zheng, Baolong
Li, Ying
Xu, Weizong
Zhou, Yizhang
Mathaudhu, Suveen N.
Zhu, Yuntian
Lavernia, Enrique J.
TI Twinning in cryomilled nanocrystalline Mg powder
SO PHILOSOPHICAL MAGAZINE LETTERS
LA English
DT Article
DE twinning; magnesium; nanocrystalline; cryomilling
ID HIGH-PRESSURE TORSION; DEFORMATION TWINS; SINGLE-CRYSTALS; ALLOY; AL;
METALS; MAGNESIUM; MECHANISMS; STRENGTH; SLIP
AB Nanocrystalline (nc) Mg powder was synthesized via cryomilling. Extension twins were identified with high-resolution transmission electron microscopy in the cryomilled powders and the study presents the first evidence of twinning in unalloyed nc Mg. The formation of twins in the nc Mg is attributed to a high strain rate, the low (cryogenic) temperature and high local shear stresses present around the grain boundaries during deformation by cryomilling.
C1 [Zheng, Baolong; Zhou, Yizhang; Lavernia, Enrique J.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA.
[Li, Ying] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Xu, Weizong; Zhu, Yuntian] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA.
[Mathaudhu, Suveen N.] US Army Res Lab, Aberdeen Proving Ground, MD 21005 USA.
RP Lavernia, EJ (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA.
EM lavernia@ucdavis.edu
RI Zhu, Yuntian/B-3021-2008; Xu, Weizong/G-3328-2014; Li, Ying/G-3908-2010;
Mathaudhu, Suveen/B-4192-2009
OI Zhu, Yuntian/0000-0002-5961-7422; Xu, Weizong/0000-0003-0030-8606; Li,
Ying/0000-0003-3738-9307;
FU US Army Research Office [W911NF-10-1-0512]
FX The authors acknowledge the financial support provided by the US Army
Research Office (Grant No W911NF-10-1-0512). The authors would like to
express their appreciation to Professor S. Mahajan for constructive
discussion and suggestions.
NR 35
TC 2
Z9 2
U1 5
U2 20
PU TAYLOR & FRANCIS LTD
PI ABINGDON
PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND
SN 0950-0839
EI 1362-3036
J9 PHIL MAG LETT
JI Philos. Mag. Lett.
PD AUG 1
PY 2013
VL 93
IS 8
BP 457
EP 464
DI 10.1080/09500839.2013.801567
PG 8
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering; Physics, Applied; Physics, Condensed Matter
SC Materials Science; Metallurgy & Metallurgical Engineering; Physics
GA 263XF
UT WOS:000327840600003
ER
PT J
AU Wang, ZG
Williams, RT
Grim, JQ
Gao, F
Kerisit, S
AF Wang, Zhiguo
Williams, Richard T.
Grim, Joel Q.
Gao, Fei
Kerisit, Sebastien
TI Kinetic Monte Carlo simulations of excitation density dependent
scintillation in CsI and CsI(TI)
SO PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS
LA English
DT Article
DE inorganic scintillators; kinetic Monte Carlo; nonlinear quenching;
non-proportionality; scintillation mechanisms
ID FAST INTRINSIC LUMINESCENCE; GAMMA-RAY INTERACTION; ELECTRON-HOLE PAIRS;
NON-PROPORTIONALITY; ALKALI HALIDES; TEMPERATURE-DEPENDENCE; ENERGY
RESOLUTION; LIGHT YIELD; VK CENTERS; PURE CSI
AB Nonlinear quenching of electron-hole pairs in the denser regions of ionization tracks created by -ray and high-energy electrons is a likely cause of the light yield non-proportionality of many inorganic scintillators. Therefore, kinetic Monte Carlo (KMC) simulations were carried out to investigate the scintillation properties of pure and thallium-doped CsI as a function of electron-hole pair density. The availability of recent experimental data on the excitation density dependence of the light yield of CsI following ultraviolet excitation allowed for an improved parameterization of the interactions between self-trapped excitons (STE) in the KMC model via dipole-dipole Forster transfer. The KMC simulations reveal that nonlinear quenching occurs very rapidly (within a few picoseconds) in the early stages of the scintillation process. In addition, the simulations predict that the concentration of thallium activators can affect the extent of nonlinear quenching as it has a direct influence on the STE density through STE dissociation and electron scavenging. This improved model will enable more realistic simulations of the non-proportional -ray and electron response of inorganic scintillators.
C1 [Wang, Zhiguo; Gao, Fei; Kerisit, Sebastien] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
[Williams, Richard T.; Grim, Joel Q.] Wake Forest Univ, Dept Phys, Winston Salem, NC 27109 USA.
RP Kerisit, S (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
EM sebastien.kerisit@pnnl.gov
RI Wang, Zhiguo/B-7132-2009; Melcher, Charles/E-9818-2012
OI Melcher, Charles/0000-0002-4586-4764
FU National Nuclear Security Administration, Office of Nuclear
Nonproliferation Research and Engineering [NA-22]; U.S. Department of
Energy (DOE)
FX The authors acknowledge Drs. Luke W. Campbell, Micah Prange, Renee M.
Van Ginhoven, and YuLong Xie for insightful discussions. This research
was supported by the National Nuclear Security Administration, Office of
Nuclear Nonproliferation Research and Engineering (NA-22), of the U.S.
Department of Energy (DOE).
NR 52
TC 12
Z9 12
U1 2
U2 10
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0370-1972
EI 1521-3951
J9 PHYS STATUS SOLIDI B
JI Phys. Status Solidi B-Basic Solid State Phys.
PD AUG
PY 2013
VL 250
IS 8
BP 1532
EP 1540
DI 10.1002/pssb.201248587
PG 9
WC Physics, Condensed Matter
SC Physics
GA 262BG
UT WOS:000327708500013
ER
PT J
AU Patel, AP
Stanek, CR
Grimes, RW
AF Patel, Ankoor P.
Stanek, Chris R.
Grimes, Robin W.
TI Comparison of defect processes in REAlO3 perovskites and RE3Al5O12
garnets
SO PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS
LA English
DT Article
DE defect volumes; garnet; optical ceramics; pair potential; perovskite;
point defects; scintillators
ID BAND-GAP SCINTILLATORS; ENERGY-TRANSFER; INORGANIC SCINTILLATORS;
SINGLE-CRYSTAL; LUMINESCENCE; ALUMINUM; YAG; LUALO3-CE; CREATION; OXIDES
AB Defects can decrease the efficiency of scintillators by trapping electrons. Here, point defects in REAlO3 and RE3Al5O12 are predicted with pair potential simulations, where RE is yttrium or a trivalent rare earth cation. It was found that REAlO3 shows a preference for Al2O3-excess whereas RE3Al5O12 most readily exhibits RE2O3-excess. Also, lattice volume changes for the energetically favorable intrinsic mechanisms are relatively invariant as a function of RE cation size in RE3Al5O12, but not in REAlO3. However, in non-stoichiometric RE3Al5O12, the energetically preferred disorder mechanism results in an increasing lattice expansion with increasing RE radius whereas, in non-stoichiometric perovskites, a relatively small, radius independent, lattice contraction is predicted. These results illustrate that defect behavior in REAlO3 perovskites and RE3Al5O12 garnets is quite disimilar. (C) 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
C1 [Patel, Ankoor P.; Grimes, Robin W.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England.
[Stanek, Chris R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Patel, AP (reprint author), Univ London Imperial Coll Sci Technol & Med, Prince Consort Rd, London SW7 2AZ, England.
EM ankoor.patel@imperial.ac.uk
NR 53
TC 9
Z9 9
U1 4
U2 36
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0370-1972
EI 1521-3951
J9 PHYS STATUS SOLIDI B
JI Phys. Status Solidi B-Basic Solid State Phys.
PD AUG
PY 2013
VL 250
IS 8
BP 1624
EP 1631
DI 10.1002/pssb.201248583
PG 8
WC Physics, Condensed Matter
SC Physics
GA 262BG
UT WOS:000327708500027
ER
PT J
AU Crease, RP
AF Crease, Robert P.
TI Just-in-time physics
SO PHYSICS WORLD
LA English
DT Editorial Material
C1 [Crease, Robert P.] SUNY Stony Brook, Dept Philosophy, Stony Brook, NY USA.
[Crease, Robert P.] Brookhaven Natl Lab, Upton, NY 11973 USA.
RP Crease, RP (reprint author), SUNY Stony Brook, Dept Philosophy, Stony Brook, NY USA.
EM robert.crease@stonybrook.edu
NR 0
TC 0
Z9 0
U1 0
U2 1
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0953-8585
J9 PHYS WORLD
JI Phys. World
PD AUG
PY 2013
VL 26
IS 8
BP 19
EP 19
PG 1
WC Physics, Multidisciplinary
SC Physics
GA 266ZL
UT WOS:000328063200013
ER
PT J
AU Peuker, JM
Lynch, P
Krier, H
Glumac, N
AF Peuker, Jennifer Mott
Lynch, Patrick
Krier, Herman
Glumac, Nick
TI On AlO Emission Spectroscopy as a Diagnostic in Energetic Materials
Testing
SO PROPELLANTS EXPLOSIVES PYROTECHNICS
LA English
DT Article
DE AlO Emission; Aluminum combustion; Energetics; Explosives
ID ALUMINUM PARTICLE COMBUSTION; SOLID-ROCKET MOTOR;
TEMPERATURE-MEASUREMENTS; ELEVATED PRESSURE; CARBON-DIOXIDE;
LASER-ABLATION; SHOCK-TUBE; IGNITION; TIME; NANOALUMINUM
AB The emission of AlO is commonly observed in tests involving aluminum combustion in propellants and explosives. Such emission has been used as a signature of combustion, as a tool for measuring ignition and reaction times, and as a thermometer. This paper provides a critical review of methodologies exploiting AlO emission spectroscopy as a quantitative tool in energetics testing. Controlled tests involving aluminized explosives, as well as those using added alumina, are conducted, in which AlO emission is quantified and compared to total oxidation in the final residue. Experimental parameters such as optical depth and fireball confinement are systematically varied to examine the effect on AlO emission. We find that thermometry using AlO remains valid, and a new approach to using low resolution spectra is proposed. However, AlO emission spectroscopy or photometry can be quantitatively correlated to ignition and burning time, or used to infer the presence or absence of aluminum combustion, only under a limited set of circumstances. Factors that limit the ability to use AlO emission quantitatively are discussed in depth.
C1 [Peuker, Jennifer Mott; Krier, Herman; Glumac, Nick] Univ Illinois, Urbana, IL 61801 USA.
[Lynch, Patrick] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
RP Peuker, JM (reprint author), Univ Illinois, 1206 W Green St, Urbana, IL 61801 USA.
EM glumac@illinois.edu
RI Glumac, Nick/C-1730-2015
OI Glumac, Nick/0000-0001-6673-0573
FU ONR [N00014-01-1-0899, N00014-08-1-0772]; DTRA [HDTRA1-07-1-0011,
HDTRA-1-10-1-0003]
FX This work, which was performed over a period of several years, received
funding from several sources including ONR contracts N00014-01-1-0899
and N00014-08-1-0772 under Dr. Judah Gold-wasser and Mr. Dan Tam. In
addition, DTRA funding from Dr. William Wilson and Dr. Suhithi Peiris
(Contracts HDTRA1-07-1-0011 and HDTRA-1-10-1-0003) supported work in
explosive systems. Finally, we wish to thank Dr. Kibong Kim for advice
and support during the conduct of this project. His suggestions led
directly to our investigation of barrier layer effects on AlO emission.
NR 67
TC 8
Z9 8
U1 0
U2 23
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0721-3115
EI 1521-4087
J9 PROPELL EXPLOS PYROT
JI Propellants Explos. Pyrotech.
PD AUG
PY 2013
VL 38
IS 4
BP 577
EP 585
DI 10.1002/prep.201200144
PG 9
WC Chemistry, Applied; Engineering, Chemical
SC Chemistry; Engineering
GA 261KS
UT WOS:000327664500017
ER
PT J
AU Zhou, JY
Krovvidi, RK
Gao, YQ
Gao, H
Petritis, BO
De, AK
Miller-Graziano, CL
Bankey, PE
Petyuk, VA
Nicora, CD
Clauss, TR
Moore, RJ
Shi, TJ
Brown, JN
Kaushal, A
Xiao, WZ
Davis, RW
Maier, RV
Tompkins, RG
Qian, WJ
Camp, DG
Smith, RD
AF Zhou, Jian-Ying
Krovvidi, Ravi K.
Gao, Yuqian
Gao, Hong
Petritis, Brianne O.
De, Asit K.
Miller-Graziano, Carol L.
Bankey, Paul E.
Petyuk, Vladislav A.
Nicora, Carrie D.
Clauss, Therese R.
Moore, Ronald J.
Shi, Tujin
Brown, Joseph N.
Kaushal, Amit
Xiao, Wenzhong
Davis, Ronald W.
Maier, Ronald V.
Tompkins, Ronald G.
Qian, Wei-Jun
Camp, David G., II
Smith, Richard D.
CA Inflammation Host Response Injury
TI Trauma-associated human neutrophil alterations revealed by comparative
proteomics profiling
SO PROTEOMICS CLINICAL APPLICATIONS
LA English
DT Article
DE Genomics; Human neutrophil; LC-MS; MS; Trauma
ID NF-KAPPA-B; TANDEM MASS-SPECTROMETRY; INFLAMMATORY RESPONSE; SHOTGUN
PROTEOMICS; CELL-PROLIFERATION; PROTEIN-SYNTHESIS; GENE-EXPRESSION;
CANCER-CELLS; APOPTOSIS; ACTIVATION
AB PurposePolymorphonuclear neutrophils (PMNs) play an important role in mediating the innate immune response after severe traumatic injury; however, the cellular proteome response to traumatic condition is still largely unknown.
Experimental designWe applied 2D-LC-MS/MS-based shotgun proteomics to perform comparative proteome profiling of human PMNs from severe trauma patients and healthy controls.
ResultsA total of 197 out of approximate to 2500 proteins (being identified with at least two peptides) were observed with significant abundance changes following the injury. The proteomics data were further compared with transcriptomics data for the same genes obtained from an independent patient cohort. The comparison showed that the protein abundance changes for the majority of proteins were consistent with the mRNA abundance changes in terms of directions of changes. Moreover, increased protein secretion was suggested as one of the mechanisms contributing to the observed discrepancy between protein and mRNA abundance changes. Functional analyses of the altered proteins showed that many of these proteins were involved in immune response, protein biosynthesis, protein transport, NRF2-mediated oxidative stress response, the ubiquitin-proteasome system, and apoptosis pathways.
Conclusions and clinical relevanceOur data suggest increased neutrophil activation and inhibited neutrophil apoptosis in response to trauma. The study not only reveals an overall picture of functional neutrophil response to trauma at the proteome level, but also provides a rich proteomics data resource of trauma-associated changes in the neutrophil that will be valuable for further studies of the functions of individual proteins in PMNs.
C1 [Zhou, Jian-Ying; Krovvidi, Ravi K.; Gao, Yuqian; Petritis, Brianne O.; Petyuk, Vladislav A.; Nicora, Carrie D.; Clauss, Therese R.; Moore, Ronald J.; Shi, Tujin; Brown, Joseph N.; Qian, Wei-Jun; Camp, David G., II; Smith, Richard D.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
[Zhou, Jian-Ying; Krovvidi, Ravi K.; Gao, Yuqian; Petritis, Brianne O.; Petyuk, Vladislav A.; Nicora, Carrie D.; Clauss, Therese R.; Moore, Ronald J.; Shi, Tujin; Brown, Joseph N.; Qian, Wei-Jun; Camp, David G., II; Smith, Richard D.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
[De, Asit K.; Miller-Graziano, Carol L.; Bankey, Paul E.] Univ Rochester, Sch Med, Dept Surg, Rochester, NY USA.
[Gao, Hong; Kaushal, Amit; Xiao, Wenzhong; Davis, Ronald W.] Stanford Univ, Sch Med, Stanford Genome Technol Ctr, Palo Alto, CA 94304 USA.
[Xiao, Wenzhong; Maier, Ronald V.] Univ Washington, Harborview Med Ctr, Dept Surg, Seattle, WA 98104 USA.
[Tompkins, Ronald G.] Harvard Univ, Sch Med, Dept Surg, Shriners Burn Ctr, Boston, MA 02115 USA.
[Tompkins, Ronald G.] Harvard Univ, Massachusetts Gen Hosp, Sch Med, Boston, MA USA.
RP Smith, RD (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999,MSIN K8-98, Richland, WA 99352 USA.
EM rds@pnnl.gov
RI Smith, Richard/J-3664-2012; Shi, Tujin/O-1789-2014;
OI Smith, Richard/0000-0002-2381-2349; Baker, Henry/0000-0002-8273-5320;
Petyuk, Vladislav/0000-0003-4076-151X
FU NIH [U54 GM-62119-02, T32 GM-008256, P41 GM103493, DP2OD006668]; EMSL
(Environmental Molecular Science Laboratory); US Department of Energy
(DOE) Office of Biological and Environmental Research on the Pacific
Northwest National Laboratory (PNNL) campus in Richland, Washington; DOE
[DE-AC05-76RLO-1830]
FX Portions of this research were supported by NIH grants U54 GM-62119-02
(to R.G.T.) and T32 GM-008256 (to R.G.T.), P41 GM103493 (to R.D.S.),
DP2OD006668 (to W.J.Q.), and EMSL (Environmental Molecular Science
Laboratory). EMSL is a national scientific user facility sponsored by
the US Department of Energy (DOE) Office of Biological and Environmental
Research on the Pacific Northwest National Laboratory (PNNL) campus in
Richland, Washington. PNNL is operated by Battelle for the DOE under
contract DE-AC05-76RLO-1830.
NR 81
TC 4
Z9 4
U1 0
U2 3
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1862-8346
EI 1862-8354
J9 PROTEOM CLIN APPL
JI Proteom. Clin. Appl.
PD AUG
PY 2013
VL 7
IS 7-8
SI SI
BP 571
EP 583
DI 10.1002/prca.201200109
PG 13
WC Biochemical Research Methods; Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 263FQ
UT WOS:000327792800011
PM 23589343
ER
PT J
AU Ruszkowski, M
Brzezinski, K
Jedrzejczak, R
Dauter, M
Dauter, Z
Sikorski, M
Jaskolski, M
AF Ruszkowski, Milosz
Brzezinski, Krzysztof
Jedrzejczak, Robert
Dauter, Miroslawa
Dauter, Zbigniew
Sikorski, Michal
Jaskolski, Mariusz
TI Medicago truncatula histidine-containing phosphotransfer protein
Structural and biochemical insights into the cytokinin transduction
pathway in plants
SO FEBS JOURNAL
LA English
DT Article
DE cytokinin hormone receptor; histidine-aspartate two-component
phosphorelay; HPt; phytohormone signal transduction; MtCRE1
ID SECONDARY-STRUCTURE; CRYSTAL-STRUCTURES; PHOSPHORYLATION; COMPLEX;
DICTYOSTELIUM; ARABIDOPSIS; REFINEMENT; FEATURES; BINDING; SYSTEMS
AB Histidine-containing phosphotransfer proteins (HPts) take part in hormone signal transduction in higher plants. The overall pathway of this process is reminiscent of the two-component system initially identified in prokaryotes. HPts function in histidine-aspartate phosphorelays in which they mediate the signal from sensory kinases (usually membrane proteins) to RRs in the nucleus. Here, we report the crystal structure of an HPt protein from Medicagotruncatula (MtHPt1) determined at 1.45 angstrom resolution and refined to an R-factor of 16.7% using low-temperature synchrotron-radiation X-ray diffraction data. There is one MtHPt1 molecule in the asymmetric unit of the crystal lattice with P2(1)2(1)2(1) symmetry. The protein fold consists of six helices, four of which form a C-terminal helix bundle. The coiled-coil structure of the bundle is stabilized by a network of S-aromatic interactions involving highly conserved sulfur-containing residues. The structure reveals a solvent-exposed side chain of His79, which is the phosphorylation site, as demonstrated by autoradiography combined with site-directed mutation. It is surrounded by highly conserved residues present in all plant HPts. These residues form a putative docking interface for either the receiver domain of the sensory kinase, or for the RR. The biological activity of MtHPt1 was tested by autoradiography. It demonstrated phosphorylation by the intracellular kinase domain of the cytokinin receptor MtCRE1. Complex formation between MtHPt1 and the intracellular fragment of MtCRE1 was confirmed by thermophoresis, with a dissociation constant K-d of 14m.
DatabaseThe atomic coordinates and structure factors for the crystal structure of histidine-containing phosphotransfer protein MtHPt1 from Medicagotruncatula have been deposited with the RCSB Protein Data Bank under the accession code 3us6.
C1 [Ruszkowski, Milosz; Brzezinski, Krzysztof; Sikorski, Michal; Jaskolski, Mariusz] Polish Acad Sci, Inst Bioorgan Chem, Ctr Biocrystallog Res, Poznan, Poland.
[Jedrzejczak, Robert] Argonne Natl Lab, Midwest Ctr Struct Genom, Argonne, IL 60439 USA.
[Dauter, Miroslawa] Argonne Natl Lab, SAIC Frederick Inc, Basic Res Program, Argonne, IL 60439 USA.
[Jaskolski, Mariusz] Adam Mickiewicz Univ, Fac Chem, Dept Crystallog, PL-60780 Poznan, Poland.
RP Jaskolski, M (reprint author), Adam Mickiewicz Univ, Fac Chem, Dept Crystallog, Grunwaldzka 6, PL-60780 Poznan, Poland.
EM mariuszj@amu.edu.pl
FU European Union within the European Regional Developmental Fund; Polish
Ministry of Science and Higher Education [NN 301 003739]; NIH [P41
RR001081]; U.S. Department of Energy, Office of Science, Office of Basic
Energy Sciences [W-31-109-Eng-38]
FX We are grateful to Dr Stephen Blanke and Dr Stefan Duhr (NanoTemper
Technologies) for making the thermophoresis equipment available to us
and to Prof. Jan Wrzesinski (IBCh, PAS, Poznan, Poland) for help with
the autoradiography experiment. Financial support of the project was
provided by the European Union within the European Regional
Developmental Fund and by the Polish Ministry of Science and Higher
Education (grant No. NN 301 003739). The pMCSG9 vector was acquired from
the Midwest Center for Structural Genomics. X-Ray diffraction data were
collected at the Southeast Regional Collaborative Access Team (SER-CAT)
beamline of the APS/ANL. Use of the Advanced Photon Source was supported
by the U.S. Department of Energy, Office of Science, Office of Basic
Energy Sciences, under Contract No. W-31-109-Eng-38. The CHIMERA package
from the Resource for Biocomputing, Visualization, and Informatics at
the University of California, San Francisco, is supported by an NIH
grant P41 RR001081.
NR 42
TC 3
Z9 3
U1 1
U2 15
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1742-464X
EI 1742-4658
J9 FEBS J
JI FEBS J.
PD AUG
PY 2013
VL 280
IS 15
BP 3709
EP 3720
DI 10.1111/febs.12363
PG 12
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 253ZK
UT WOS:000327129100021
PM 23721763
ER
PT J
AU Johnston-Peck, AC
Cullen, DA
Tracy, JB
AF Johnston-Peck, Aaron C.
Cullen, David A.
Tracy, Joseph B.
TI Composition-Mediated Order-Disorder Transformation in FePt Nanoparticles
SO PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION
LA English
DT Article
DE electron microscopy; intermetallic phases; iron; magnetic materials;
platinum
ID BIT-PATTERNED MEDIA; OXYGEN REDUCTION; CDSE NANOCRYSTALS; IRON-PLATINUM;
PHASE; SUPERLATTICES; MECHANISM; COBALT; ALLOYS
C1 [Johnston-Peck, Aaron C.; Tracy, Joseph B.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA.
[Cullen, David A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RP Johnston-Peck, AC (reprint author), N Carolina State Univ, Dept Mat Sci & Engn, Box 7907, Raleigh, NC 27695 USA.
EM jbtracy@ncsu.edu
RI Cullen, David/A-2918-2015
OI Cullen, David/0000-0002-2593-7866
FU GAANN fellowship; National Science Foundation [CHE-0943975]; Oak Ridge
National Laboratory's SHaRE User Facility; Scientific User Facilities
Division, Office of Basic Energy Sciences, U.S. Department of Energy
FX The authors thank Giovanna Scarel and Gregory N. Parsons (NCSU) for
providing assistance with atomic layer deposition. A.C.J.-P.
acknowledges support from a GAANN fellowship. This research was
supported by the National Science Foundation (CHE-0943975) and Oak Ridge
National Laboratory's SHaRE User Facility, which is sponsored by the
Scientific User Facilities Division, Office of Basic Energy Sciences,
U.S. Department of Energy.
NR 51
TC 2
Z9 2
U1 2
U2 18
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA POSTFACH 101161, 69451 WEINHEIM, GERMANY
SN 0934-0866
EI 1521-4117
J9 PART PART SYST CHAR
JI Part. Part. Syst. Charact.
PD AUG
PY 2013
VL 30
IS 8
BP 678
EP 682
DI 10.1002/ppsc.201300028
PG 5
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 255OT
UT WOS:000327250400008
ER
PT J
AU Masciola, M
Nahon, M
Driscoll, F
AF Masciola, Marco
Nahon, Meyer
Driscoll, Frederick
TI Preliminary Assessment of the Importance of Platform-Tendon Coupling in
a Tension Leg Platform
SO JOURNAL OF OFFSHORE MECHANICS AND ARCTIC ENGINEERING-TRANSACTIONS OF THE
ASME
LA English
DT Article
ID DYNAMICS; TLP
AB This paper presents performance metrics that can be used to evaluate the response sensitivity of a tension leg platform (TLP) to its tendons. An uncoupled TLP model ignores the intrinsic dynamics and environmental loads on the cables by treating each tendon as an ideal massless spring. A coupled TLP system, in contrast, considers the effects of distributed mass and drag along the tendon. Under certain operating conditions, an uncoupled dynamics model can produce results comparable to its coupled counterpart. This paper defines the conditions under which it is acceptable to model a TLP tendon as a linear spring, as opposed to one that considers the cable dynamics. The analysis is performed in the frequency domain and, for generality, the results are nondimensionalized. The findings indicate that a more elaborate set of conditions than the platform-to-cable mass ratio must be satisfied for the two models to provide similar results. To conclude this study, two simulations are performed and compared against the performance metrics derived in this paper.
C1 [Masciola, Marco; Nahon, Meyer] McGill Univ, Dept Mech Engn, Montreal, PQ H3A 2K6, Canada.
[Driscoll, Frederick] Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Masciola, M (reprint author), McGill Univ, Dept Mech Engn, Montreal, PQ H3A 2K6, Canada.
NR 27
TC 1
Z9 1
U1 1
U2 5
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0892-7219
EI 1528-896X
J9 J OFFSHORE MECH ARCT
JI J. Offshore Mech. Arct. Eng. Trans. ASME
PD AUG
PY 2013
VL 135
IS 3
AR 031901
DI 10.1115/1.4023795
PG 11
WC Engineering, Ocean; Engineering, Mechanical
SC Engineering
GA 240QV
UT WOS:000326113000022
ER
PT J
AU Kajimoto, M
Priddy, CMO
Ledee, DR
Xu, C
Isern, N
Olson, AK
Des Rosiers, C
Portman, MA
AF Kajimoto, Masaki
Priddy, Colleen M. O'Kelly
Ledee, Dolena R.
Xu, Chun
Isern, Nancy
Olson, Aaron K.
Des Rosiers, Christine
Portman, Michael A.
TI Myocardial Reloading After Extracorporeal Membrane Oxygenation Alters
Substrate Metabolism While Promoting Protein Synthesis
SO JOURNAL OF THE AMERICAN HEART ASSOCIATION
LA English
DT Article
DE amino acids; congenital heart disease; extracorporeal circulation;
metabolism; pediatrics
ID CITRIC-ACID CYCLE; CARDIOPULMONARY BYPASS; RAT-HEART;
OXIDATIVE-METABOLISM; PYRUVATE; ANAPLEROSIS; CHILDREN; SUPPORT;
REPERFUSION
AB Background-Extracorporeal membrane oxygenation (ECMO) unloads the heart, providing a bridge to recovery in children after myocardial stunning. ECMO also induces stress which can adversely affect the ability to reload or wean the heart from the circuit. Metabolic impairments induced by altered loading and/or stress conditions may impact weaning. However, cardiac substrate and amino acid requirements upon weaning are unknown. We assessed the hypothesis that ventricular reloading with ECMO modulates both substrate entry into the citric acid cycle (CAC) and myocardial protein synthesis.
Methods and Results-Sixteen immature piglets (7.8 to 15.6 kg) were separated into 2 groups based on ventricular loading status: 8-hour ECMO (UNLOAD) and postwean from ECMO (RELOAD). We infused into the coronary artery [2-C-13]-pyruvate as an oxidative substrate and [C-13(6)]-L-leucine as an indicator for amino acid oxidation and protein synthesis. Upon RELOAD, each functional parameter, which were decreased substantially by ECMO, recovered to near-baseline level with the exclusion of minimum dP/dt. Accordingly, myocardial oxygen consumption was also increased, indicating that overall mitochondrial metabolism was reestablished. At the metabolic level, when compared to UNLOAD, RELOAD altered the contribution of various substrates/pathways to tissue pyruvate formation, favoring exogenous pyruvate versus glycolysis, and acetyl-CoA formation, shifting away from pyruvate decarboxylation to endogenous substrate, presumably fatty acids. Furthermore, there was also a significant increase of tissue concentrations for all CAC intermediates (approximate to 80%), suggesting enhanced anaplerosis, and of fractional protein synthesis rates (>70%).
Conclusions-RELOAD alters both cytosolic and mitochondrial energy substrate metabolism, while favoring leucine incorporation into protein synthesis rather than oxidation in the CAC. Improved understanding of factors governing these metabolic perturbations may serve as a basis for interventions and thereby improve success rate from weaning from ECMO.
C1 [Kajimoto, Masaki; Priddy, Colleen M. O'Kelly; Ledee, Dolena R.; Xu, Chun; Olson, Aaron K.; Portman, Michael A.] Seattle Childrens Res Inst, Ctr Dev Therapeut, Seattle, WA 98101 USA.
[Priddy, Colleen M. O'Kelly] Univ Washington, Dept Surg, Seattle, WA 98195 USA.
[Isern, Nancy] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
[Des Rosiers, Christine] Univ Montreal, Dept Nutr, Montreal, PQ H3C 3J7, Canada.
[Des Rosiers, Christine] Montreal Heart Inst, Montreal, PQ H1T 1C8, Canada.
[Olson, Aaron K.; Portman, Michael A.] Univ Washington, Dept Pediat, Div Cardiol, Seattle, WA 98195 USA.
RP Portman, MA (reprint author), Seattle Childrens Res Inst, 1900 9th Ave, Seattle, WA 98101 USA.
EM michael.portman@seattlechildrens.org
RI Des Rosiers, Christine/O-6285-2014
FU National Heart Lung and Blood Institute of the National Institutes of
Health [R01HL60666]; Department of Energy's Office of Biological and
Environmental Research
FX Research reported in this publication was supported the National Heart
Lung and Blood Institute of the National Institutes of Health under
award number R01HL60666. The content is solely the responsibility of the
authors and does not necessarily represent the official views of the
National Institutes of Health. A portion of the research was performed
using Environmental Molecular Sciences Laboratory (EMSL), a national
scientific user facility sponsored by the Department of Energy's Office
of Biological and Environmental Research and located at Pacific
Northwest National Laboratory.
NR 23
TC 10
Z9 10
U1 0
U2 2
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 2047-9980
J9 J AM HEART ASSOC
JI J. Am. Heart Assoc.
PD AUG
PY 2013
VL 2
IS 4
AR e000106
DI 10.1161/JAHA.113.000106
PG 10
WC Cardiac & Cardiovascular Systems
SC Cardiovascular System & Cardiology
GA 243TP
UT WOS:000326340900016
PM 23959443
ER
PT J
AU Morgan, B
D'Mello, S
Abbott, R
Radvansky, G
Haass, M
Tamplin, A
AF Morgan, Brent
D'Mello, Sidney
Abbott, Robert
Radvansky, Gabriel
Haass, Michael
Tamplin, Andrea
TI Individual Differences in Multitasking Ability and Adaptability
SO HUMAN FACTORS
LA English
DT Article
DE cognitive abilities; spatial manipulation; working memory; MATB; task
switching
ID GENERAL FLUID INTELLIGENCE; WORKING-MEMORY; MENTAL ROTATION; TASK;
PERFORMANCE; ENVIRONMENT
AB Objective: The aim of this study was to identify the cognitive factors that predictability and adaptability during multitasking with a flight simulator.
Background: Multitasking has become increasingly prevalent as most professions require individuals to perform multiple tasks simultaneously. Considerable research has been undertaken to identify the characteristics of people (i.e., individual differences) that predict multitasking ability. Although working memory is a reliable predictor of general multitasking ability (i.e., performance in normal conditions), there is the question of whether different cognitive faculties are needed to rapidly respond to changing task demands (adaptability).
Method: Participants first completed a battery of cognitive individual differences tests followed by multitasking sessions with a flight simulator. After a baseline condition, difficulty of the flight simulator was incrementally increased via four experimental manipulations, and performance metrics were collected to assess multitasking ability and adaptability.
Results: Scholastic aptitude and working memory predicted general multitasking ability (i.e., performance at baseline difficulty), but spatial manipulation (in conjunction with working memory) was a major predictor of adaptability (performance in difficult conditions after accounting for baseline performance).
Conclusion: Multitasking ability and adaptability may be overlapping but separate constructs that draw on overlapping (but not identical) sets of cognitive abilities.
Application: The results of this study are applicable to practitioners and researchers in human factors to assess multitasking performance in real-world contexts and with realistic task constraints. We also present a framework for conceptualizing multitasking adaptability on the basis of five adaptability profiles derived from performance on tasks with consistent versus increased difficulty.
C1 [Morgan, Brent] Univ Memphis, Memphis, TN 38152 USA.
[D'Mello, Sidney; Radvansky, Gabriel] Univ Notre Dame, Dept Psychol, Notre Dame, IN 46556 USA.
[D'Mello, Sidney] Univ Notre Dame, Dept Comp Sci, Notre Dame, IN 46556 USA.
[Abbott, Robert; Haass, Michael] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Tamplin, Andrea] Univ Notre Dame, Cognit Brain & Behav Program, Notre Dame, IN 46556 USA.
RP Morgan, B (reprint author), Univ Memphis, 202 Psychol Bldg,400 Innovat Dr, Memphis, TN 38152 USA.
EM brent.morgan@memphis.edu
FU Sandia National Laboratories' Laboratory-Directed Research and
Development (LDRD) [130787]; U.S. Department of Energy
[DE-AC04-94AL85000]
FX This work was supported by Sandia National Laboratories'
Laboratory-Directed Research and Development (LDRD) Project 130787.
Sandia is a multiprogram laboratory operated by Sandia Corporation, a
Lockheed Martin Company, for the U.S. Department of Energy under
Contract DE-AC04-94AL85000.
NR 41
TC 8
Z9 9
U1 1
U2 23
PU SAGE PUBLICATIONS INC
PI THOUSAND OAKS
PA 2455 TELLER RD, THOUSAND OAKS, CA 91320 USA
SN 0018-7208
EI 1547-8181
J9 HUM FACTORS
JI Hum. Factors
PD AUG
PY 2013
VL 55
IS 4
BP 776
EP 788
DI 10.1177/0018720812470842
PG 13
WC Behavioral Sciences; Engineering, Industrial; Ergonomics; Psychology,
Applied; Psychology
SC Behavioral Sciences; Engineering; Psychology
GA 245ER
UT WOS:000326444200006
PM 23964417
ER
PT J
AU Kim, I
Kihm, K
AF Kim, Iltai
Kihm, Kenneth
TI Progressive Dryout of Nanofluids on the Hydrophilic and Hydrophobic
Surfaces
SO JOURNAL OF HEAT TRANSFER-TRANSACTIONS OF THE ASME
LA English
DT Editorial Material
C1 [Kim, Iltai] Sandia Natl Labs, Nanophoton Grp, Ctr Integrated Nanotechnol, Livermore, CA 94550 USA.
[Kihm, Kenneth] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA.
RP Kim, I (reprint author), Sandia Natl Labs, Nanophoton Grp, Ctr Integrated Nanotechnol, Livermore, CA 94550 USA.
NR 0
TC 1
Z9 1
U1 1
U2 3
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0022-1481
EI 1528-8943
J9 J HEAT TRANS-T ASME
JI J. Heat Transf.-Trans. ASME
PD AUG
PY 2013
VL 135
IS 8
AR 080911
PG 1
WC Thermodynamics; Engineering, Mechanical
SC Thermodynamics; Engineering
GA 241LH
UT WOS:000326167900011
ER
PT J
AU Kirchoff, E
Kihm, KD
Rosenfeld, J
Rawal, S
Bilheux, H
Walker, L
Voisin, S
Pratt, D
Swanson, A
AF Kirchoff, E.
Kihm, K. D.
Rosenfeld, J.
Rawal, S.
Bilheux, H.
Walker, L.
Voisin, S.
Pratt, D.
Swanson, A.
TI Neutron Tomography of Lithium (Li) Menisci inside a Molybdenum (Mo) Heat
Pipe
SO JOURNAL OF HEAT TRANSFER-TRANSACTIONS OF THE ASME
LA English
DT Editorial Material
C1 [Kirchoff, E.; Kihm, K. D.] Univ Tennessee, Knoxville, TN 37996 USA.
[Rosenfeld, J.] Thermacore Inc, Lancaster, PA USA.
[Rawal, S.] Lockheed Martin Space Syst Co, Denver, CO USA.
[Bilheux, H.; Walker, L.; Voisin, S.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Pratt, D.; Swanson, A.] Air Force Res Lab, Wright Patterson AFB, OH USA.
RP Kirchoff, E (reprint author), Univ Tennessee, Knoxville, TN 37996 USA.
RI Bilheux, Hassina/H-4289-2012
OI Bilheux, Hassina/0000-0001-8574-2449
NR 0
TC 0
Z9 0
U1 0
U2 8
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0022-1481
EI 1528-8943
J9 J HEAT TRANS-T ASME
JI J. Heat Transf.-Trans. ASME
PD AUG
PY 2013
VL 135
IS 8
AR 080902
PG 1
WC Thermodynamics; Engineering, Mechanical
SC Thermodynamics; Engineering
GA 241LH
UT WOS:000326167900002
ER
PT J
AU Dongarra, J
Tourancheau, B
AF Dongarra, Jack
Tourancheau, Bernard
TI Introduction for August Special Issue CCDSC
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Editorial Material
C1 [Dongarra, Jack] Univ Tennessee, Knoxville, TN 37996 USA.
[Dongarra, Jack] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Tourancheau, Bernard] Univ Grenoble, UMR LIG, Grenoble, France.
RP Dongarra, J (reprint author), Univ Tennessee, Knoxville, TN 37996 USA.
RI Dongarra, Jack/E-3987-2014
NR 0
TC 0
Z9 0
U1 0
U2 1
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2013
VL 27
IS 3
SI SI
BP 231
EP 231
DI 10.1177/1094342013497990
PG 1
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA 239AI
UT WOS:000325993400001
ER
PT J
AU Spafford, K
Vetter, JS
Benson, T
Parker, M
AF Spafford, Kyle
Vetter, Jeffrey S.
Benson, Thomas
Parker, Mike
TI Modeling synthetic aperture radar computation with Aspen
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Article
DE performance modeling; Aspen; workload characterization; Echelon;
synthetic aperture radar; FFT
ID PARALLEL COMPUTATION
AB This case study presents an analytical performance model for the DARPA UHPC streaming sensor challenge problem developed using Aspen, a domain-specific language for performance modeling. The model focuses on the exploration of algorithmic tradeoffs, data structures and storage, and the impact of an important tiling factor in the image formation kernel of a synthetic aperture radar image-processing computation.
C1 [Spafford, Kyle; Vetter, Jeffrey S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Benson, Thomas] Georgia Tech Res Inst, Atlanta, GA 30332 USA.
[Parker, Mike] NVIDIA, Santa Clara, CA USA.
RP Vetter, JS (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.
EM vetter@ornl.gov
FU Office of Advanced Scientific Computing Research in the U.S. Department
of Energy; DARPA [HR0011-10-90008]; Oak Ridge National Laboratory
[AC05-00OR22725]
FX This research is sponsored by the Office of Advanced Scientific
Computing Research in the U.S. Department of Energy and DARPA (contract
number HR0011-10-90008). The paper has been authored by Oak Ridge
National Laboratory, which is managed by UT-Battelle, LLC under Contract
DE-AC05-00OR22725 to the U.S. Government. Accordingly, the U.S.
Government retains a non-exclusive, royalty-free license to publish or
reproduce the published form of this contribution, or allow others to do
so, for U.S. Government purposes.
NR 14
TC 1
Z9 1
U1 0
U2 6
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2013
VL 27
IS 3
SI SI
BP 255
EP 262
DI 10.1177/1094342013488262
PG 8
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA 239AI
UT WOS:000325993400004
ER
PT J
AU Saltz, JH
Teodoro, G
Pan, T
Cooper, LAD
Kong, J
Klasky, S
Kurc, TM
AF Saltz, Joel H.
Teodoro, George
Pan, Tony
Cooper, Lee A. D.
Kong, Jun
Klasky, Scott
Kurc, Tahsin M.
TI Feature-based analysis of large-scale spatio-temporal sensor data on
hybrid architectures
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Article
DE Sensor data; imaging data; data analysis and management; cluster
computing; GPGPU
ID HIGH-PERFORMANCE
AB The analysis of large sensor datasets for structural and functional features has applications in many domains, including weather and climate modeling, characterization of subsurface reservoirs, and biomedicine. The vast amount of data obtained from state-of-the-art sensors and the computational cost of analysis operations create a barrier to such analyses. In this paper, we describe middleware system support to take advantage of large clusters of hybrid CPU-GPU nodes to address the data and compute-intensive requirements of feature-based analyses of large spatio-temporal datasets.
C1 [Saltz, Joel H.; Teodoro, George; Pan, Tony; Cooper, Lee A. D.; Kong, Jun; Kurc, Tahsin M.] Emory Univ, Ctr Comprehens Informat, Atlanta, GA 30322 USA.
[Saltz, Joel H.; Teodoro, George; Pan, Tony; Cooper, Lee A. D.; Kong, Jun; Kurc, Tahsin M.] Emory Univ, Biomed Informat Dept, Atlanta, GA 30322 USA.
[Klasky, Scott; Kurc, Tahsin M.] Oak Ridge Natl Lab, Sci Data Grp, Oak Ridge, TN 37831 USA.
RP Saltz, JH (reprint author), Biomed Informat Dept, 36 Eagle Row,Suite 566, Atlanta, GA 30322 USA.
EM jhsaltz@emory.edu
FU NCI [HHSN261200 800001E]; NLM [5R01LM009239-04, 1R01LM011119-01]; NHLBI
[R24HL085343]; NIH [NIH P20EB000591, RC4MD005964]; CTSA Program, NIH,
NCATS [UL1TR000454]; NSF [OCI-0910735]
FX This work was funded, in part, by contract HHSN261200 800001E by the
NCI; and grants 5R01LM009239-04 and 1R01LM011119-01 from the NLM,
R24HL085343 from the NHLBI, NIH P20EB000591, RC4MD005964 from NIH, and
PHS grant UL1TR000454 from the CTSA Program, NIH, NCATS. This research
used resources of the Keeneland Computing Facility at the Georgia
Institute of Technology, which is supported by the NSF under contract
OCI-0910735.
NR 27
TC 1
Z9 1
U1 0
U2 7
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2013
VL 27
IS 3
SI SI
BP 263
EP 272
DI 10.1177/1094342013488260
PG 10
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA 239AI
UT WOS:000325993400005
ER
PT J
AU Gainaru, A
Cappello, F
Snir, M
Kramer, W
AF Gainaru, Ana
Cappello, Franck
Snir, Marc
Kramer, William
TI Failure prediction for HPC systems and applications: Current situation
and open issues
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Article
DE failure prediction; fault tolerance; signal analysis
AB As large-scale systems evolve towards post-petascale computing, it is crucial to focus on providing fault-tolerance strategies that aim to minimize fault's effects on applications. By far the most popular technique is the checkpoint-restart strategy. A complement to this classical approach is failure avoidance, by which the occurrence of a fault is predicted and proactive measures are taken. This requires a reliable prediction system to anticipate failures and their locations. One way of offering prediction is by the analysis of system logs generated during production by large-scale systems. Current research in this field presents a number of limitations that make them unusable for running on real production high-performance computing (HPC) systems. Based on our observations that different failures have different distributions and behaviours, we propose a novel hybrid approach that combines signal analysis with data mining in order to overcome current limitations. We show that by analysing each event according to its specific behaviour, our prediction provides a precision of over 90% and its able to discover about 50% of all failures in a system, result which allows its integration in proactive fault tolerance protocols.
C1 [Gainaru, Ana; Kramer, William] Natl Ctr Supercomp Applicat, Urbana, IL USA.
[Gainaru, Ana; Snir, Marc] Univ Illinois, Dept Comp Sci, Urbana, IL 61801 USA.
[Cappello, Franck] Univ Illinois, Urbana, IL 61801 USA.
[Cappello, Franck] INRIA, Le Chesnay, France.
[Snir, Marc] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA.
RP Gainaru, A (reprint author), Univ Illinois, Off NCSA 4017, Natl Ctr Supercomp Aplicat, 1205 W Clark St, Urbana, IL 61801 USA.
EM againaru@illinois.edu
FU National Science Foundation [OCI 07-25070]; state of Illinois; U.S.
Department of Energy, Office of Science [DE-AC02-06CH11357]
FX This research is part of the Blue Waters sustained-petascale computing
project, which is supported by the National Science Foundation (award
number OCI 07-25070) and the state of Illinois. Blue Waters is a joint
effort of the University of Illinois at Urbana-Champaign and its
National Center for Supercomputing Applications. This research was done
in the context of the INRIA-Illinois Joint Laboratory for Petascale
Computing. This work was also supported by the U.S. Department of
Energy, Office of Science, under Contract No. DE-AC02-06CH11357.
NR 35
TC 5
Z9 5
U1 0
U2 5
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2013
VL 27
IS 3
SI SI
BP 273
EP 282
DI 10.1177/1094342013488258
PG 10
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA 239AI
UT WOS:000325993400006
ER
PT J
AU Carpenter, I
Archibald, RK
Evans, KJ
Larkin, J
Micikevicius, P
Norman, M
Rosinski, J
Schwarzmeier, J
Taylor, MA
AF Carpenter, I.
Archibald, R. K.
Evans, K. J.
Larkin, J.
Micikevicius, P.
Norman, M.
Rosinski, J.
Schwarzmeier, J.
Taylor, M. A.
TI Progress towards accelerating HOMME on hybrid multi-core systems
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Article
DE CAM; HOMME; GPU; scalability; tracer
ID DYNAMICAL CORE; MODELS; SCHEME
AB The suitability of a spectral element based dynamical core (HOMME) within the Community Atmospheric Model (CAM) for GPU-based architectures is examined and initial performance results are reported. This work was done within a project to enable CAM to run at high resolution on next-generation, multi-petaflop systems. The dynamical core is the present focus because it dominates the performance profile of our target problem. HOMME enjoys good scalability due to its underlying cubed-sphere mesh with full two-dimensional decomposition and the localization of all computational work within each element. The thread blocking and code changes that allow HOMME to effectively use GPUs are described along with a rewritten vertical remapping scheme, which improves performance on both CPUs and GPUs. Validation of results in the full HOMME model is also described. We demonstrate that the most expensive kernel in the model executes more than three times faster on the GPU than the CPU. These improvements are expected to provide improved efficiency when incorporated into the full model that has been configured for the target problem. Remaining issues affecting performance include optimizing the boundary exchanges for the case of multiple spectral elements being computed on the GPU.
C1 [Carpenter, I.] Natl Renewable Energy Lab, Computat Sci Grp, Golden, CO 80401 USA.
[Archibald, R. K.; Norman, M.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Evans, K. J.] Oak Ridge Natl Lab, Computat Earth Sci Grp, Oak Ridge, TN USA.
[Larkin, J.] Cray Inc, Oak Ridge, TN USA.
[Micikevicius, P.] NVIDIA, Santa Clara, CA USA.
[Rosinski, J.] NOAA, ESRL, Boulder, CO USA.
[Schwarzmeier, J.] Cray Inc, Chippewa Falls, WI USA.
[Taylor, M. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Carpenter, I (reprint author), Natl Renewable Energy Lab, Computat Sci Ctr, 1617 Cole Blvd,MS 1622, Golden, CO 80401 USA.
EM Ilene.Carpenter@nrel.gov
RI Archibald, Rick/I-6238-2016;
OI Archibald, Rick/0000-0002-4538-9780; Evans,
Katherine/0000-0001-8174-6450
FU Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]
FX MAT and KJE have been supported by the DOE BER SciDAC project, 'A
Scalable and Extensible Earth System'. This research used resources of
the Oak Ridge Leadership Computing Facility at the Oak Ridge National
Laboratory, which is supported by the Office of Science of the U.S.
Department of Energy under Contract Number DE-AC05-00OR22725.
NR 19
TC 5
Z9 5
U1 0
U2 17
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2013
VL 27
IS 3
SI SI
BP 335
EP 347
DI 10.1177/1094342012462751
PG 13
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA 239AI
UT WOS:000325993400011
ER
PT J
AU Dubey, A
Calder, AC
Daley, C
Fisher, RT
Graziani, C
Jordan, GC
Lamb, DQ
Reid, LB
Townsley, DM
Weide, K
AF Dubey, Anshu
Calder, Alan C.
Daley, Christopher
Fisher, Robert T.
Graziani, C.
Jordan, George C.
Lamb, Donald Q.
Reid, Lynn B.
Townsley, Dean M.
Weide, Klaus
TI Pragmatic optimizations for better scientific utilization of large
supercomputers
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Article
DE FLASH; supercomputer; optimizations; SN Ia; GCD model
ID GRAVITATIONALLY CONFINED DETONATION; ASTROPHYSICAL THERMONUCLEAR
FLASHES; ADAPTIVE MESH REFINEMENT; IA-SUPERNOVAE; DEFLAGRATION PHASE;
CARBON IGNITION; WHITE-DWARF; MODEL; HYDRODYNAMICS; SIMULATIONS
AB Advances in modeling and algorithms, combined with growth in computing resources, have enabled simulations of multiphysics-multiscale phenomena that can greatly enhance our scientific understanding. However, on currently available high-performance computing (HPC) resources, maximizing the scientific outcome of simulations requires many trade-offs. In this paper we describe our experiences in running simulations of the explosion phase of Type Ia supernovae on the largest available platforms. The simulations use FLASH, a modular, adaptive mesh, parallel simulation code with a wide user base. The simulations use multiple physics components: hydrodynamics, gravity, a sub-grid flame model, a three-stage burning model, and a degenerate equation of state. They also use Lagrangian tracer particles, which are then post-processed to determine the nucleosynthetic yields. We describe the simulation planning process, and the algorithmic optimizations and trade-offs that were found to be necessary. Several of the optimizations and trade-offs were made during the course of the simulations as our understanding of the challenges evolved, or when simulations went into previously unexplored physical regimes. We also briefly outline the anticipated challenges of, and our preparations for, the next-generation computing platforms.
C1 [Dubey, Anshu; Daley, Christopher; Graziani, C.; Jordan, George C.; Lamb, Donald Q.; Weide, Klaus] Univ Chicago, Computat Inst, Flash Ctr Computat Sci Astron & Astrophys, Chicago, IL 60637 USA.
[Dubey, Anshu; Daley, Christopher; Graziani, C.; Lamb, Donald Q.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Calder, Alan C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY USA.
[Reid, Lynn B.] NTEC Environm Technol, Subiaco, WA, Australia.
[Reid, Lynn B.] Univ Western Australia, Crawley, WA, Australia.
[Townsley, Dean M.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA.
RP Dubey, A (reprint author), Univ Chicago, Computat Inst, Flash Ctr Computat Sci Astron & Astrophys, 5747 South Ellis Ave, Chicago, IL 60637 USA.
EM dubey@flash.uchicago.edu
RI Fisher, Robert/J-8667-2014;
OI Fisher, Robert/0000-0001-8077-7255; Weide, Klaus/0000-0001-9869-9750
FU ASC/Alliance Program NNSA, US Department of Energy [B523820]
FX This work was supported by the ASC/Alliance Program NNSA, US Department
of Energy (grant number B523820) to the Flash Center at the University
of Chicago.
NR 38
TC 5
Z9 5
U1 0
U2 5
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2013
VL 27
IS 3
SI SI
BP 360
EP 373
DI 10.1177/1094342012464404
PG 14
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA 239AI
UT WOS:000325993400013
ER
PT J
AU Kerr, M
Prime, MB
Swenson, H
Buechler, MA
Steinzig, M
Clausen, B
Sisneros, T
AF Kerr, Matthew
Prime, Michael B.
Swenson, Hunter
Buechler, Miles A.
Steinzig, Michael
Clausen, Bjorn
Sisneros, Thomas
TI Residual Stress Characterization in a Dissimilar Metal Weld Nuclear
Reactor Piping System Mock Up
SO JOURNAL OF PRESSURE VESSEL TECHNOLOGY-TRANSACTIONS OF THE ASME
LA English
DT Article
ID CONTOUR METHOD; DIFFRACTION
AB Time-of-flight neutron diffraction, contour method, and surface hole drilling residual stress measurements were conducted at Los Alamos National Lab (LANL) on a lab sized plate specimen (P4) from phase 1 of the joint U. S. Nuclear Regulatory Commission and Electric Power Research Institute Weld Residual Stress (NRC/EPRI WRS) program. The specimen was fabricated from a 304L stainless steel plate containing a seven pass alloy 82 groove weld, restrained during welding and removed from the restraint for residual stress characterization. This paper presents neutron diffraction and contour method results, and compares these experimental stress measurements to a WRS finite element (FE) model. Finally, details are provided on the procedure used to calculate the residual stress distribution in the restrained or as welded condition in order to allow comparison to other residual stress data collected as part of phase 1 of the WRS program.
C1 [Kerr, Matthew] US Nucl Regulatory Commiss, Off Nucl Regulatory Res, Washington, DC 20555 USA.
[Prime, Michael B.; Swenson, Hunter; Buechler, Miles A.; Steinzig, Michael] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Clausen, Bjorn; Sisneros, Thomas] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA.
RP Kerr, M (reprint author), Knolls Atom Power Lab, Schenectady, NY 12301 USA.
EM matthew.kerr.contractor@unnpp.gov
RI Clausen, Bjorn/B-3618-2015;
OI Clausen, Bjorn/0000-0003-3906-846X; Prime, Michael/0000-0002-4098-5620
NR 32
TC 0
Z9 0
U1 0
U2 8
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0094-9930
EI 1528-8978
J9 J PRESS VESS-T ASME
JI J. Press. Vessel Technol.-Trans. ASME
PD AUG
PY 2013
VL 135
IS 4
AR 041205
DI 10.1115/1.4024446
PG 8
WC Engineering, Mechanical
SC Engineering
GA 239JS
UT WOS:000326019500006
ER
PT J
AU Clifton, A
Schreck, S
Scott, G
Kelley, N
Lundquist, JK
AF Clifton, Andrew
Schreck, Scott
Scott, George
Kelley, Neil
Lundquist, Julie K.
TI Turbine Inflow Characterization at the National Wind Technology Center
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
ID LOW-LEVEL JET; SOUTHERN GREAT-PLAINS; STABLE BOUNDARY-LAYER;
SURFACE-LAYER; TURBULENCE MEASUREMENTS; CLIMATOLOGY; TERRAIN; SITE
AB Utility-scale wind turbines operate in dynamic flows that can vary significantly over time scales from less than a second to several years. To better understand the inflow to utility-scale turbines on time scales from seconds to minutes, the National Renewable Energy Laboratory installed and commissioned two inflow measurement towers at the National Wind Technology Center near Boulder, Colorado, in 2011. These towers are 135 m tall and instrumented with sonic anemometers, cup anemometers, wind vanes, and temperature measurements to characterize the inflow wind speed and direction, turbulence, stability and thermal stratification for two utility-scale turbines. In this paper, we present variations in mean and turbulent wind parameters with height, atmospheric stability, and as a function of wind direction that could be important for turbine operation, and for the persistence of turbine wakes. Wind speed, turbulence intensity, and dissipation are all factors that affect turbine performance. Our results show that these all vary with height across the rotor disk, demonstrating the importance of measuring atmospheric conditions that influence wind turbine performance at multiple heights in the rotor disk, rather than relying on extrapolation from conditions measured at lower levels.
C1 [Clifton, Andrew; Schreck, Scott; Scott, George; Lundquist, Julie K.] Natl Wind Technol Ctr, Natl Renewable Energy Lab NREL, Golden, CO 80401 USA.
[Lundquist, Julie K.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA.
RP Clifton, A (reprint author), Natl Wind Technol Ctr, Natl Renewable Energy Lab NREL, Golden, CO 80401 USA.
OI Clifton, Andrew/0000-0001-9698-5083; LUNDQUIST,
JULIE/0000-0001-5490-2702
FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy
Laboratory
FX This work was supported by the U.S. Department of Energy under Contract
No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory.
NR 37
TC 8
Z9 8
U1 0
U2 13
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2013
VL 135
IS 3
AR 031017
DI 10.1115/1.4024068
PG 11
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA 239IV
UT WOS:000326017000017
ER
PT J
AU Ermanoski, I
Siegel, NP
Stechel, EB
AF Ermanoski, Ivan
Siegel, Nathan P.
Stechel, Ellen B.
TI A New Reactor Concept for Efficient Solar-Thermochemical Fuel Production
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
DE solar fuels; thermochemical; hydrogen; carbon dioxide; synthesis gas;
concentrating solar power
ID WATER-SPLITTING CYCLE; HYDROGEN-PRODUCTION; NONSTOICHIOMETRIC CERIA;
REDOX REACTIONS; CO2; HEAT; COMPOSITES; REDUCTION; SYSTEMS; ZN/ZNO
AB We describe and analyze the efficiency of a new solar-thermochemical reactor concept, which employs a moving packed bed of reactive particles produce of H-2 or CO from solar energy and H2O or CO2. The packed bed reactor incorporates several features essential to achieving high efficiency: spatial separation of pressures, temperature, and reaction products in the reactor; solid-solid sensible heat recovery between reaction steps; continuous on-sun operation; and direct solar illumination of the working material. Our efficiency analysis includes material thermodynamics and a detailed accounting of energy losses, and demonstrates that vacuum pumping, made possible by the innovative pressure separation approach in our reactor, has a decisive efficiency advantage over inert gas sweeping. We show that in a fully developed system, using CeO2 as a reactive material, the conversion efficiency of solar energy into H-2 and CO at the design point can exceed 30%. The reactor operational flexibility makes it suitable for a wide range of operating conditions, allowing for high efficiency on an annual average basis. The mixture of H-2 and CO, known as synthesis gas, is not only usable as a fuel but is also a universal starting point for the production of synthetic fuels compatible with the existing energy infrastructure. This would make it possible to replace petroleum derivatives used in transportation in the U. S., by using less than 0.7% of the U. S. land area, a roughly two orders of magnitude improvement over mature biofuel approaches. In addition, the packed bed reactor design is flexible and can be adapted to new, better performing reactive materials.
C1 [Ermanoski, Ivan] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Siegel, Nathan P.] Bucknell Univ, Dept Mech Engn, Lewisburg, PA 17837 USA.
[Stechel, Ellen B.] Arizona State Univ, LightWorks, Tempe, AZ 85287 USA.
RP Ermanoski, I (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM iermano@sandia.gov; nate.siegel@bucknell.edu; Ellen.Stechel@asu.edu
FU Laboratory Directed Research and Development program at Sandia National
Laboratories; U.S. Department of Energy Fuel Cell Technologies Program
via the Solar Thermochemical Hydrogen (STCH) directive; United States
Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]
FX The authors would like to gratefully acknowledge the contributions of
James E. Miller, Brian D. Ehrhart, Richard B. Diver, Anthony McDaniel,
and Andrea Ambrosini. This work was supported by the Laboratory Directed
Research and Development program at Sandia National Laboratories, in the
form of a Grand Challenge project entitled "Reimagining Liquid
Transportation Fuels: Sunshine to Petrol.," and the U.S. Department of
Energy Fuel Cell Technologies Program via the Solar Thermochemical
Hydrogen (STCH) directive. Sandia is a multiprogram laboratory operated
by Sandia Corporation, a Lockheed Martin Company, for the United States
Department of Energy's National Nuclear Security Administration under
Contract No. DE-AC04-94AL85000.
NR 43
TC 60
Z9 60
U1 7
U2 56
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2013
VL 135
IS 3
AR 031002
DI 10.1115/1.4023356
PG 10
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA 239IV
UT WOS:000326017000002
ER
PT J
AU Florita, AR
Brackney, LJ
Otanicar, TP
Robertson, J
AF Florita, Anthony R.
Brackney, Larry J.
Otanicar, Todd P.
Robertson, Jeffrey
TI Classification of Commercial Building Electrical Demand Profiles for
Energy Storage Applications
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
ID RENEWABLE ENERGY; THERMAL MASS; SYSTEMS
AB Commercial buildings have a significant impact on energy and the environment, being responsible for more than 18% of the annual primary energy consumption in the United States. Analyzing their electrical demand profiles is necessary for the assessment of supply-demand interactions and potential; of particular importance are supply- or demand-side energy storage assets and the value they bring to various stakeholders in the smart grid context. This research developed and applied unsupervised classification of commercial buildings according to their electrical demand profile. A Department of Energy (DOE) database was employed, containing electrical demand profiles representing the United States commercial building stock as detailed in the 2003 Commercial Buildings Consumption Survey (CBECS) and as modeled in the EnergyPlus building energy simulation tool. The essence of the approach was: (1) discrete wavelet transformation of the electrical demand profiles, (2) energy and entropy feature extraction (absolute and relative) from the wavelet levels at definitive time frames, and (3) Bayesian probabilistic hierarchical clustering of the features to classify the buildings in terms of similar patterns of electrical demand. The process yielded a categorized and more manageable set of representative electrical demand profiles, inference of the characteristics influencing supply-demand interactions, and a test bed for quantifying the impact of applying energy storage technologies.
C1 [Florita, Anthony R.; Brackney, Larry J.] Natl Renewable Energy Lab, Elect Resources & Bldg Syst Integrat Ctr, Golden, CO 80401 USA.
[Otanicar, Todd P.] Univ Tulsa, Dept Mech Engn, Tulsa, OK 74104 USA.
[Robertson, Jeffrey] Loyola Marymount Univ, Dept Mech Engn, Los Angeles, CA 90045 USA.
RP Florita, AR (reprint author), Natl Renewable Energy Lab, Elect Resources & Bldg Syst Integrat Ctr, Golden, CO 80401 USA.
EM anthony.florita@nrel.gov
NR 16
TC 3
Z9 3
U1 0
U2 3
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2013
VL 135
IS 3
AR 031020
DI 10.1115/1.4024029
PG 10
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA 239IV
UT WOS:000326017000020
ER
PT J
AU Kragh, KA
Fleming, PA
Scholbrock, AK
AF Kragh, Knud A.
Fleming, Paul A.
Scholbrock, Andrew K.
TI Increased Power Capture by Rotor Speed-Dependent Yaw Control of Wind
Turbines
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
AB When extracting energy from the wind using upwind, horizontal-axis wind turbines, a primary condition for ensuring maximum power yield is the ability to align the rotor axis with the dominating wind direction. Attempts have been made to improve the yaw alignment of wind turbines by applying advanced measurement technologies, such as light detection and ranging systems. However, application of advanced measurement equipment is associated with additional costs and increased system complexity. This study is focused on assessing the current performance of an operating turbine and exploring how the yaw alignment can be improved using measurements from the existing standard measurements system. By analyzing data from a case turbine and a corresponding meteorological mast, a correction scheme for the original yaw control system is suggested. The correction scheme is applied to the case turbine and tested. Results show that, with the correction scheme in place, the yaw alignment of the case turbine is improved and the yaw error is reduced to the vicinity of zero degrees. As a result of the improved yaw alignment, an increased power capture is observed for below-rated wind speeds.
C1 [Kragh, Knud A.] Tech Univ Denmark, Dept Wind Energy, DK-4000 Roskilde, Denmark.
[Fleming, Paul A.; Scholbrock, Andrew K.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Kragh, KA (reprint author), Tech Univ Denmark, Dept Wind Energy, DK-4000 Roskilde, Denmark.
EM knkr@dtu.dk; Paul.fleming@nrel.gov
FU Wind and Water Power Program, Office of Energy Efficiency and Renewable
Energy of the U.S. Department of Energy [DE-AC02-05CH11231]
FX Invaluable support for this work was provided by Lee Jay Fingersh, Garth
Johnson, Scott Wilde, Mark Murphy, Jerry Hur, Syhoune Thao, and Don
Baker of NREL. NREL's contributions to this study were funded by the
Wind and Water Power Program, Office of Energy Efficiency and Renewable
Energy of the U.S. Department of Energy, under Contract No.
DE-AC02-05CH11231. The authors are solely responsible for any omission
or errors contained herein.
NR 13
TC 4
Z9 4
U1 1
U2 8
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2013
VL 135
IS 3
AR 031018
DI 10.1115/1.4023971
PG 7
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA 239IV
UT WOS:000326017000018
ER
PT J
AU Lee, S
Churchfield, MJ
Moriarty, PJ
Jonkman, J
Michalakes, J
AF Lee, S.
Churchfield, M. J.
Moriarty, P. J.
Jonkman, J.
Michalakes, J.
TI A Numerical Study of Atmospheric and Wake Turbulence Impacts on Wind
Turbine Fatigue Loadings
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
ID BOUNDARY-LAYER; SIMULATIONS
AB Large-eddy simulations of atmospheric boundary layers under various stability and surface roughness conditions are performed to investigate the turbulence impact on wind turbines. In particular, the aeroelastic responses of the turbines are studied to characterize the fatigue loading of the turbulence present in the boundary layer and in the wake of the turbines. Two utility-scale 5 MW turbines that are separated by seven rotor diameters are placed in a 3 km by 3 km by 1 km domain. They are subjected to atmospheric turbulent boundary layer flow and data are collected on the structural response of the turbine components. The surface roughness was found to increase the fatigue loads while the atmospheric instability had a small influence. Furthermore, the downstream turbines yielded higher fatigue loads indicating that the turbulent wakes generated from the upstream turbines have significant impact.
C1 [Lee, S.; Churchfield, M. J.; Moriarty, P. J.; Jonkman, J.; Michalakes, J.] Natl Renewable Energy Lab, Natl Wind Technol Ctr, Golden, CO 80401 USA.
RP Lee, S (reprint author), Natl Renewable Energy Lab, Natl Wind Technol Ctr, 15013 Denver West Pkwy,MS 3811, Golden, CO 80401 USA.
EM Sang.Lee@nrel.gov
FU National Renewable Energy Laboratory's LDRD program
FX The authors gratefully acknowledge the financial support provided by the
National Renewable Energy Laboratory's LDRD program. All of the
computations were performed on the Red Mesa high-performance computing
system of the National Renewable Energy Laboratory. Discussions and
guidance by Marshall Buhl has been greatly appreciated.
NR 31
TC 7
Z9 7
U1 0
U2 17
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2013
VL 135
IS 3
AR 031001
DI 10.1115/1.4023319
PG 10
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA 239IV
UT WOS:000326017000001
ER
PT J
AU Zhu, GD
AF Zhu, Guangdong
TI Study of the Optical Impact of Receiver Position Error on Parabolic
Trough Collectors
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
AB A newly developed analytical optical approach-first-principle OPTical intercept calculation (FirstOPTIC)-is employed to study the optical impact of receiver position error on parabolic trough collectors. The FirstOPTIC method treats optical error sources the way they are typically characterized in laboratory measurements using a geometrical or optical interpretation. By analyzing a large number of cases with varying system parameters, such as overall system optical error and the collector's geometrical parameters, a practical correlation between actual measurement data and its corresponding error-convolution approximation for receiver position error is established from parametric study; the correlation enables a direct comparison of receiver position error to the sun shape and other optical error sources (such as mirror specularity and slope error) with respect to the collector optical performance. The effective coefficients that define the correlation of actual measurement data and its error-convolution approximation for receiver position error are also summarized for several existing trough collectors; these make it convenient to characterize the relative impact of receiver position error compared with other optical error sources, which was not straightforward in the past. It is shown that FirstOPTIC is a suitable tool for in-depth optical analysis and fast collector design optimization, which otherwise require computationally intensive ray-tracing simulations.
C1 Natl Renewable Energy Lab, Concentrating Solar Power Program, Golden, CO 80401 USA.
RP Zhu, GD (reprint author), Natl Renewable Energy Lab, Concentrating Solar Power Program, 15013 Denver West Pkwy, Golden, CO 80401 USA.
EM Guangdong.Zhu@nrel.gov
FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy
Laboratory (NREL)
FX This work was supported by the U.S. Department of Energy under the
Contract No. DE-AC36-08GO28308 with the National Renewable Energy
Laboratory (NREL). Thanks to Allan Lewandowski, Mike Wagner, Ty Neises,
and Chuck Kutscher in the NREL's Thermal Systems Group for their
valuable comments on this work.
NR 13
TC 2
Z9 3
U1 1
U2 7
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2013
VL 135
IS 3
AR 031021
DI 10.1115/1.4024247
PG 5
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA 239IV
UT WOS:000326017000021
ER
PT J
AU Kita, NT
Yin, QZ
MacPherson, GJ
Ushikubo, T
Jacobsen, B
Nagashima, K
Kurahashi, E
Krot, AN
Jacobsen, SB
AF Kita, Noriko T.
Yin, Qing-Zhu
MacPherson, Glenn J.
Ushikubo, Takayuki
Jacobsen, Benjamin
Nagashima, Kazuhide
Kurahashi, Erika
Krot, Alexander N.
Jacobsen, Stein B.
TI 26Al-26Mg isotope systematics of the first solids in the early solar
system
SO METEORITICS & PLANETARY SCIENCE
LA English
DT Article
ID ALUMINUM-RICH INCLUSIONS; REFRACTORY INCLUSIONS; CARBONACEOUS-CHONDRITE;
AL-26-MG-26 SYSTEMATICS; INITIAL AL-26/AL-27; HETEROGENEOUS
DISTRIBUTION; CONTEMPORANEOUS FORMATION; CA,AL-RICH INCLUSIONS;
PROTOPLANETARY DISKS; ALLENDE METEORITE
AB High-precision bulk aluminum-magnesium isotope measurements of calcium-aluminum-rich inclusions (CAIs) from CV carbonaceous chondrites in several laboratories define a bulk 26Al-26Mg isochron with an inferred initial 26Al/27Al ratio of approximately 5.25x10-5, named the canonical ratio. Nonigneous CV CAIs yield well-defined internal 26Al-26Mg isochrons consistent with the canonical value. These observations indicate that the canonical 26Al/27Al ratio records initial Al/Mg fractionation by evaporation and condensation in the CV CAI-forming region. The internal isochrons of igneous CV CAIs show a range of inferred initial 26Al/27Al ratios, (4.2-5.2)x10-5, indicating that CAI melting continued for at least 0.2Ma after formation of their precursors. A similar range of initial 26Al/27Al ratios is also obtained from the internal isochrons of many CAIs (igneous and nonigneous) in other groups of carbonaceous chondrites. Some CAIs and refractory grains (corundum and hibonite) from unmetamorphosed or weakly metamorphosed chondrites, including CVs, are significantly depleted in 26Al. At least some of these refractory objects may have formed prior to injection of 26Al into the protosolar molecular cloud and its subsequent homogenization in the protoplanetary disk. Bulk aluminum and magnesium-isotope measurements of various types of chondrites plot along the bulk CV CAI isochron, suggesting homogeneous distribution of 26Al and magnesium isotopes in the protoplanetary disk after an epoch of CAI formation. The inferred initial 26Al/27Al ratios of chondrules indicate that most chondrules formed 1-3Ma after CAIs with the canonical 26Al/27Al ratio.
C1 [Kita, Noriko T.; Ushikubo, Takayuki] Univ Wisconsin, Dept Geosci, WiscSIMS, Madison, WI 53706 USA.
[MacPherson, Glenn J.] Smithsonian Inst, US Natl Museum Nat Hist, Dept Mineral Sci, Washington, DC 20560 USA.
[Jacobsen, Benjamin] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
[Nagashima, Kazuhide; Krot, Alexander N.] Univ Hawaii Manoa, Sch Ocean Earth Sci & Technol, Hawaii Inst Geophys & Planetol, Honolulu, HI 96822 USA.
[Kurahashi, Erika] Univ Munster, Inst Mineral, D-48149 Munster, Germany.
[Jacobsen, Stein B.] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA.
RP Kita, NT (reprint author), Univ Wisconsin, Dept Geosci, WiscSIMS, Madison, WI 53706 USA.
EM noriko@geology.wisc.edu
RI Yin, Qing-Zhu/B-8198-2009; Kita, Noriko/H-8035-2016
OI Yin, Qing-Zhu/0000-0002-4445-5096; Kita, Noriko/0000-0002-0204-0765
FU NASA [NNX09AB88G, NNX11AJ51G, NNX11AD43G, NNX11 AK82G, NNX10AH76G]; UC
Laboratory Fees Research Program [12_LR-237921]
FX The authors acknowledge the organizing committee of the Workshop on
"Formation of the First Solid in the Solar System" for the opportunity
of this article. The constructive comments by Joel Baker and James
Connelly and the careful handling by associate editor Edward Scott
improved clarity of the manuscript significantly. This work is supported
by NASA programs (NNX09AB88G, NK; NNX11AJ51G, QZY; NNX11AD43G, GJM;
NNX11 AK82G, SBJ; NNX10AH76G, ANK) and UC Laboratory Fees Research
Program 12_LR-237921 to QZY.
NR 99
TC 40
Z9 40
U1 1
U2 28
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1086-9379
EI 1945-5100
J9 METEORIT PLANET SCI
JI Meteorit. Planet. Sci.
PD AUG
PY 2013
VL 48
IS 8
BP 1383
EP 1400
DI 10.1111/maps.12141
PG 18
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 237KC
UT WOS:000325867500002
ER
PT J
AU Bullock, ES
Knight, KB
Richter, FM
Kita, NT
Ushikubo, T
MacPherson, GJ
Davis, AM
Mendybaev, RA
AF Bullock, Emma S.
Knight, Kim B.
Richter, Frank M.
Kita, Noriko T.
Ushikubo, Takayuki
MacPherson, Glenn J.
Davis, Andrew M.
Mendybaev, Ruslan A.
TI Mg and Si isotopic fractionation patterns in types B1 and B2 CAIs:
Implications for formation under different nebular conditions
SO METEORITICS & PLANETARY SCIENCE
LA English
DT Article
ID AL-RICH INCLUSIONS; REFRACTORY INCLUSIONS; CRYSTALLIZATION SEQUENCES;
ALLENDE METEORITE; MELILITE; CONDENSATION; EVAPORATION; LIQUIDS;
CHONDRITES; EVOLUTION
AB Magnesium and silicon isotopic profiles across melilite grains in two type B1 and two type B2 calcium-aluminum-rich inclusions (CAIs) reveal differing but constant enrichments in heavy isotopes everywhere except 1000m from the CAI margins. There is no close correlation in the B1s or the B2s between isotopic composition and akermanite content of the melilite, a measure of progressive igneous crystallization, yet such a correlation might be expected in a type B2: without a melilite mantle (as in B1s) to seal the interior off and prevent further evaporation, the melt would have maintained communication with the external gas. These observations indicate a model in which B1s and B2s solidified under differing conditions. The B2s solidified under lower hydrogen pressures (PH210-4-10-5 bars) than did B1s (PH2>10-4 bars), so surface volatilization was slower in the B2s and internal chemical and isotopic equilibrium was maintained over the interval of melilite crystallization. The outermost zones of the CAIs (1000m from the edge) are not consistently enriched in heavy isotopes relative to the interiors, as might be expected from diffusion-limited surface evaporation of the melt. In all cases, the magnesium in the CAI margins is lighter than in the interiors. In one case, silicon in the margin also is lighter, but locally in some CAIs, it is isotopically heavier near the surface. If melt evaporation played a role in the formation of these outer zones, a later event in many cases caused isotopic re-equilibration with an external and isotopically near-normal reservoir.
C1 [Bullock, Emma S.; MacPherson, Glenn J.] Smithsonian Inst, US Natl Museum Nat Hist, Washington, DC 20560 USA.
[Knight, Kim B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Richter, Frank M.; Davis, Andrew M.; Mendybaev, Ruslan A.] Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA.
[Kita, Noriko T.; Ushikubo, Takayuki] Univ Wisconsin, Dept Geosci, Madison, WI 53706 USA.
[Davis, Andrew M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA.
RP Bullock, ES (reprint author), Smithsonian Inst, US Natl Museum Nat Hist, Washington, DC 20560 USA.
EM bullockE@si.edu
RI Kita, Noriko/H-8035-2016;
OI Kita, Noriko/0000-0002-0204-0765; Davis, Andrew/0000-0001-7955-6236
FU NASA [NNX09AG39G, NNX09AB88G, NNX11AD43G, NNX09AG38G]; NSF [EAR03-19230,
EAR07-44079]
FX The manuscript was greatly improved by careful and thoughtful reviews by
Drs. Christine Floss (Assoc. Ed.), Yunbin Guan, Julie Paque, and Steve
Simon. This work was supported by NASA grants NNX09AG39G (A. M. D., PI),
NNX09AB88G (N. K., PI), NNX11AD43G (G. J. M., PI), and NNX09AG38G (F.
R., PI). WiscSIMS is partly supported by NSF (EAR03-19230, EAR07-44079).
NR 34
TC 7
Z9 7
U1 2
U2 15
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1086-9379
EI 1945-5100
J9 METEORIT PLANET SCI
JI Meteorit. Planet. Sci.
PD AUG
PY 2013
VL 48
IS 8
BP 1440
EP 1458
DI 10.1111/maps.12158
PG 19
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 237KC
UT WOS:000325867500006
ER
PT J
AU Rebel, B
Mufson, S
AF Rebel, B.
Mufson, S.
TI The search for neutrino-antineutrino mixing resulting from Lorentz
invariance violation using neutrino interactions in MINOS
SO ASTROPARTICLE PHYSICS
LA English
DT Article
DE Neutrino; Lorentz invariance; CPT
AB We searched for a sidereal modulation in the rate of neutrinos produced by the NuMI beam and observed by the MINOS far detector. The detection of such harmonic signals could be a signature of neutrino-anti-neutrino mixing due to Lorentz and CPT violation as described by the Standard-Model Extension framework. We found no evidence for these sidereal signals and we placed limits on the coefficients in this theory describing the effect. This is the first report of limits on these neutrino-anti-neutrino mixing coefficients. (c) 2013 Elsevier B.V. All rights reserved.
C1 [Rebel, B.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Mufson, S.] Indiana Univ, Bloomington, IN 47405 USA.
RP Rebel, B (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA.
EM brebel@fnal.gov; mufson@astro.indiana.edu
FU Indiana University Center for Spacetime Symmetries (IUCSS); U.S.
Department of Energy Office of Science [DE-FG02-91ER40661]
FX We gratefully acknowledge our many valuable conversations with Alan
Kostelecky and Jorge Diaz during the course of this work. This work was
supported in part by the Indiana University Center for Spacetime
Symmetries (IUCSS) and by the U.S. Department of Energy Office of
Science through grant DE-FG02-91ER40661 to Indiana University. We thank
the MINOS collaboration for releasing the timestamp information for the
neutrino interactions used in this analysis. We are grateful to the
Minnesota Department of Natural Resources, the crew of the Soudan
Underground Laboratory, and the staff of Fermilab for their
contributions to this effort.
NR 21
TC 15
Z9 15
U1 0
U2 0
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0927-6505
EI 1873-2852
J9 ASTROPART PHYS
JI Astropart Phys.
PD AUG
PY 2013
VL 48
BP 78
EP 81
DI 10.1016/j.astropartphys.2013.07.006
PG 4
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 234VK
UT WOS:000325672200010
ER
PT J
AU Wang, XM
Whitehead, JP
AF Wang, Xiaoming
Whitehead, Jared P.
TI A bound on the vertical transport of heat in the 'ultimate' state of
slippery convection at large Prandtl numbers
SO JOURNAL OF FLUID MECHANICS
LA English
DT Article
DE Benard convection; mantle convection; turbulent convection
ID RAYLEIGH-BENARD CONVECTION; THERMAL-CONVECTION; TURBULENT CONVECTION;
ENERGY-DISSIPATION; BOUSSINESQ SYSTEM; UNIFYING THEORY; BEHAVIOR; FLUID;
LAYER
AB An upper bound on the rate of vertical heat transport is established in three dimensions for stress-free velocity boundary conditions on horizontally periodic plates. A variation of the background method is implemented that allows negative values of the quadratic form to yield 'small' (O (1/Pr)) corrections to the subsequent bound. For large (but finite) Prandtl numbers this bound is an improvement over the 'ultimate' Ra-1/2 scaling and, in the limit of infinite Pr, agrees with the bound of Ra-5/12 recently derived in that limit for stress-free boundaries.
C1 [Wang, Xiaoming] Florida State Univ, Dept Math, Tallahassee, FL 32306 USA.
[Whitehead, Jared P.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.
RP Whitehead, JP (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.
EM whitehead@lanl.gov
FU National Science Foundation [DMS1008852]; US Department of Energy
through the LANL/LDRD Program
FX We thank R. Wittenberg for careful comments and criticism of this
manuscript as well as the thoughtful insights of three anonymous
reviewers. This work is supported in part by the National Science
Foundation through DMS1008852, and the US Department of Energy through
the LANL/LDRD Program.
NR 49
TC 3
Z9 3
U1 1
U2 2
PU CAMBRIDGE UNIV PRESS
PI NEW YORK
PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA
SN 0022-1120
EI 1469-7645
J9 J FLUID MECH
JI J. Fluid Mech.
PD AUG
PY 2013
VL 729
BP 103
EP 122
DI 10.1017/jfm.2013.289
PG 20
WC Mechanics; Physics, Fluids & Plasmas
SC Mechanics; Physics
GA 190YK
UT WOS:000322379400006
ER
PT J
AU Morgan, B
Duraisamy, K
Nguyen, N
Kawai, S
Lele, SK
AF Morgan, Brandon
Duraisamy, K.
Nguyen, N.
Kawai, S.
Lele, S. K.
TI Flow physics and RANS modelling of oblique shock/turbulent boundary
layer interaction
SO JOURNAL OF FLUID MECHANICS
LA English
DT Article
DE turbulence modelling; turbulence simulation; wave-turbulence
interactions
ID DIRECT NUMERICAL-SIMULATION; SHOCK-INDUCED SEPARATION; LARGE-EDDY
SIMULATION; TURBULENCE; UNSTEADINESS; MOTIONS; REGION
AB Large-eddy simulation (LES) is utilized to investigate flow physics and lower-fidelity modelling assumptions in the simulation of an oblique shock impinging on a supersonic turbulent boundary layer (OSTBLI). A database of LES solutions is presented, covering a range of shock strengths and Reynolds numbers, that is utilized as a surrogate-truth model to explore three topics. First, detailed conservation budgets are extracted within the framework of parametric investigation to identify trends that might be used to mitigate statistical (aleatory) uncertainties in inflow conditions. It is found, for instance, that an increase in Reynolds number does not significantly affect length of separation. Additionally, it is found that variation in the shock-generating wedge angle has the effect of increasing the intensity of low-frequency oscillations and moving these motions towards longer time scales, even when scaled by interaction length. Next, utilizing the LES database, a detailed analysis is performed of several existing models describing the low-frequency unsteady motion of the OSTBLI system. Most significantly, it is observed that the length scale of streamwise coherent structures appears to be dependent on Reynolds number, and at the Reynolds number of the present simulations, these structures do not exist on time scales long enough to be the primary cause of low-frequency unsteadiness. Finally, modelling errors associated with turbulence closures using eddy-viscosity and stress-transport-based Reynolds-averaged Navier-Stokes (RANS) simulations are investigated. It is found that while the stress-transport models offer improved predictions, inadequacies in modelling the turbulence transport terms and the isotropic treatment of the dissipation is seen to limit their accuracy.
C1 [Morgan, Brandon; Duraisamy, K.; Nguyen, N.; Kawai, S.; Lele, S. K.] Stanford Univ, Dept Aeronaut & Astronaut, Stanford, CA 94305 USA.
RP Morgan, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
EM bmorgan1@stanford.edu
FU DoD; AFOSR; NDSEG; DoE PSAAP Program; 32 CFR 168a
FX This research was conducted with government support under and awarded by
DoD, AFOSR, NDSEG Fellowship, 32 CFR 168a and by the DoE PSAAP Program.
Computer time has been provided by NASA NAS, HPCC at LLNL, and HPC at
LANL. We would also like to recognize Dr M. R. Visbal at AFRL for
providing the FDL3DI code that has been extended and used in the present
study.
NR 68
TC 11
Z9 12
U1 1
U2 31
PU CAMBRIDGE UNIV PRESS
PI NEW YORK
PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA
SN 0022-1120
EI 1469-7645
J9 J FLUID MECH
JI J. Fluid Mech.
PD AUG
PY 2013
VL 729
BP 231
EP 284
DI 10.1017/jfm.2013.301
PG 54
WC Mechanics; Physics, Fluids & Plasmas
SC Mechanics; Physics
GA 190YK
UT WOS:000322379400011
ER
PT J
AU Sundriyal, V
Sosonkina, M
Gaenko, A
Zhang, Z
AF Sundriyal, Vaibhav
Sosonkina, Masha
Gaenko, Alexander
Zhang, Zhao
TI Energy saving strategies for parallel applications with point-to-point
communication phases
SO JOURNAL OF PARALLEL AND DISTRIBUTED COMPUTING
LA English
DT Article
DE Dynamic voltage and frequency scaling; Point-to-point communications;
Multicore platforms; GAMESS
ID DISTRIBUTED DATA INTERFACE
AB Although high-performance computing traditionally focuses on the efficient execution of large-scale applications, both energy and power have become critical concerns when approaching exascale. Drastic increases in the power consumption of supercomputers affect significantly their operating costs and failure rates. In modern microprocessor architectures, equipped with dynamic voltage and frequency scaling (DVFS) and CPU clock modulation (throttling), the power consumption may be controlled in software. Additionally, network interconnect, such as Infiniband, may be exploited to maximize energy savings while the application performance loss and frequency switching overheads must be carefully balanced. This paper advocates for a runtime assessment of such overheads by means of characterizing point-to-point communications into phases followed by analyzing the time gaps between the communication calls. Certain communication and architectural parameters are taken into consideration in the three proposed frequency scaling strategies, which differ with respect to their treatment of the time gaps. The experimental results are presented for NAS parallel benchmark problems as well as for the realistic parallel electronic structure calculations performed by the widely used quantum chemistry package GAMESS. For the latter, three different process-to-core mappings were studied as to their energy savings under the proposed frequency scaling strategies and under the existing state-of-the-art techniques. Close to the maximum energy savings were obtained with a low performance loss of 2% on the given platform. (C) 2013 Elsevier Inc. All rights reserved.
C1 [Sundriyal, Vaibhav; Sosonkina, Masha; Gaenko, Alexander] Iowa State Univ, Ames Lab, Ames, IA 50011 USA.
[Sundriyal, Vaibhav; Zhang, Zhao] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA.
[Sosonkina, Masha] Old Dominion Univ, Dept Modeling Simulat & Visualizat Engn, Norfolk, VA 23529 USA.
RP Sundriyal, V (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA.
EM vaibhavs@iastate.edu; masha@scl.ameslab.gov;
alex@si.msg.chem.iastate.edu; zzhang@iastate.edu
FU Ames Laboratory; Iowa State University [DE-AC02-07CH11358]; U.S.
Department of Energy; Air Force Office of Scientific Research
[FA9550-12-1-0476]; National Science Foundation [NSF/OCI-0941434,
0904782, 1047772]
FX This work was supported in part by Ames Laboratory and Iowa State
University under the contract DE-AC02-07CH11358 with the U.S. Department
of Energy, by the Air Force Office of Scientific Research under the
AFOSR award FA9550-12-1-0476, and by the National Science Foundation
grants NSF/OCI-0941434, 0904782, 1047772.
NR 37
TC 3
Z9 3
U1 0
U2 3
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0743-7315
EI 1096-0848
J9 J PARALLEL DISTR COM
JI J. Parallel Distrib. Comput.
PD AUG
PY 2013
VL 73
IS 8
BP 1157
EP 1169
DI 10.1016/j.jpdc.2013.03.006
PG 13
WC Computer Science, Theory & Methods
SC Computer Science
GA 230AI
UT WOS:000325308600013
ER
PT J
AU Dimitrov, IK
Si, WD
Ku, W
Han, SJ
Jaroszynski, J
AF Dimitrov, I. K.
Si, W. D.
Ku, W.
Han, S. J.
Jaroszynski, J.
TI Unusual persistence of superconductivity against high magnetic fields in
the strongly-correlated iron-chalcogenide film FeTe:O-x
SO LOW TEMPERATURE PHYSICS
LA English
DT Article
ID HEAVY-FERMION; STATE; TEMPERATURE; PNICTIDES; SPIN
AB We report an unusual persistence of superconductivity against high magnetic fields in the iron-chalcogenide film FeTe:O-x below approximate to 2.5 K. Instead of saturating, like mean-field behavior with a single order parameter, the measured low-temperature upper critical field increases progressively, suggesting a large supply of superconducting states accessible via magnetic field or low-energy thermal fluctuations. We demonstrate that superconducting states of finite momenta can be realized within the conventional theory, despite its questionable applicability. Our findings reveal a fundamental characteristic of superconductivity and electronic structure in the strongly correlated iron-based superconductors. (C) 2013 AIP Publishing LLC.
C1 [Dimitrov, I. K.; Si, W. D.; Ku, W.; Han, S. J.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
[Jaroszynski, J.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA.
RP Dimitrov, IK (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
EM idimitrov@bnl.gov; wds@bnl.gov
FU Office of Science, U.S. Department of Energy, Materials Sciences and
Engineering Division [DE-AC02-98CH10886]; NSF by the State of Florida
[DMR-1157490]; DOE
FX The work at Brookhaven National Laboratory was supported by the Office
of Science, U.S. Department of Energy, Materials Sciences and
Engineering Division, under Contract No. DE-AC02-98CH10886. A portion of
this work was performed at the National High Magnetic Field Laboratory,
which is supported by NSF Cooperative Agreement No. DMR-1157490 by the
State of Florida, and by the DOE. I. K. D. wishes to thank Vyacheslav
Solovyov and Silvia Haindl for critical reading of the manuscript and
helpful suggestions.
NR 39
TC 3
Z9 3
U1 4
U2 18
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1063-777X
EI 1090-6517
J9 LOW TEMP PHYS+
JI Low Temp. Phys.
PD AUG
PY 2013
VL 39
IS 8
BP 680
EP 684
DI 10.1063/1.4818790
PG 5
WC Physics, Applied
SC Physics
GA 223OO
UT WOS:000324815900003
ER
PT J
AU McNulty, NP
Wu, M
Erickson, AR
Pan, CL
Erickson, BK
Martens, EC
Pudlo, NA
Muegge, BD
Henrissat, B
Hettich, RL
Gordon, JI
AF McNulty, Nathan P.
Wu, Meng
Erickson, Alison R.
Pan, Chongle
Erickson, Brian K.
Martens, Eric C.
Pudlo, Nicholas A.
Muegge, Brian D.
Henrissat, Bernard
Hettich, Robert L.
Gordon, Jeffrey I.
TI Effects of Diet on Resource Utilization by a Model Human Gut Microbiota
Containing Bacteroides cellulosilyticus WH2, a Symbiont with an
Extensive Glycobiome
SO PLOS BIOLOGY
LA English
DT Article
ID PROTEIN IDENTIFICATIONS; MASS-SPECTROMETRY; ESCHERICHIA-COLI;
GNOTOBIOTIC MICE; HUMAN INTESTINE; METABOLISM; GENE; THETAIOTAOMICRON;
POLYSACCHARIDE; EXPRESSION
AB The human gut microbiota is an important metabolic organ, yet little is known about how its individual species interact, establish dominant positions, and respond to changes in environmental factors such as diet. In this study, gnotobiotic mice were colonized with an artificial microbiota comprising 12 sequenced human gut bacterial species and fed oscillating diets of disparate composition. Rapid, reproducible, and reversible changes in the structure of this assemblage were observed. Time-series microbial RNA-Seq analyses revealed staggered functional responses to diet shifts throughout the assemblage that were heavily focused on carbohydrate and amino acid metabolism. High-resolution shotgun metaproteomics confirmed many of these responses at a protein level. One member, Bacteroides cellulosilyticus WH2, proved exceptionally fit regardless of diet. Its genome encoded more carbohydrate active enzymes than any previously sequenced member of the Bacteroidetes. Transcriptional profiling indicated that B. cellulosilyticus WH2 is an adaptive forager that tailors its versatile carbohydrate utilization strategy to available dietary polysaccharides, with a strong emphasis on plant-derived xylans abundant in dietary staples like cereal grains. Two highly expressed, diet-specific polysaccharide utilization loci (PULs) in B. cellulosilyticus WH2 were identified, one with characteristics of xylan utilization systems. Introduction of a B. cellulosilyticus WH2 library comprising >90,000 isogenic transposon mutants into gnotobiotic mice, along with the other artificial community members, confirmed that these loci represent critical diet-specific fitness determinants. Carbohydrates that trigger dramatic increases in expression of these two loci and many of the organism's 111 other predicted PULs were identified by RNA-Seq during in vitro growth on 31 distinct carbohydrate substrates, allowing us to better interpret in vivo RNA-Seq and proteomics data. These results offer insight into how gut microbes adapt to dietary perturbations at both a community level and from the perspective of a well-adapted symbiont with exceptional saccharolytic capabilities, and illustrate the value of artificial communities.
C1 [McNulty, Nathan P.; Wu, Meng; Muegge, Brian D.; Gordon, Jeffrey I.] Washington Univ, Sch Med, Ctr Genome Sci & Syst Biol, St Louis, MO 63130 USA.
[Erickson, Alison R.; Hettich, Robert L.] Univ Tennessee, Grad Sch Genome Sci & Technol, Oak Ridge Natl Lab, Knoxville, TN USA.
[Erickson, Alison R.; Pan, Chongle; Erickson, Brian K.; Hettich, Robert L.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA.
[Martens, Eric C.; Pudlo, Nicholas A.] Univ Michigan, Sch Med, Dept Microbiol & Immunol, Ann Arbor, MI 48109 USA.
[Henrissat, Bernard] CNRS, Marseille, France.
[Henrissat, Bernard] Aix Marseille Univ, Marseille, France.
RP McNulty, NP (reprint author), Washington Univ, Sch Med, Ctr Genome Sci & Syst Biol, St Louis, MO 63130 USA.
EM jgordon@wustl.edu
RI Henrissat, Bernard/J-2475-2012; Hettich, Robert/N-1458-2016
OI Hettich, Robert/0000-0001-7708-786X
FU NIH [DK30292, DK70977]; Crohn's and Colitis Foundation of America;
European Research Council under European Union [322820]; ORNL Laboratory
FX The majority of this work was supported by grants from the NIH (DK30292,
DK70977). Other sources of support included the Crohn's and Colitis
Foundation of America, the European Research Council under the European
Union's Seventh Framework Programme (FP/2007-2013)/ERC Grant Agreement
no. 322820, and an ORNL Laboratory Director's Exploratory Seed Money
grant (for metaproteomics). The funders had no role in study design,
data collection and analysis, decision to publish, or preparation of the
manuscript.
NR 67
TC 63
Z9 64
U1 8
U2 55
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1545-7885
J9 PLOS BIOL
JI PLoS. Biol.
PD AUG
PY 2013
VL 11
IS 8
AR e1001637
DI 10.1371/journal.pbio.1001637
PG 20
WC Biochemistry & Molecular Biology; Biology
SC Biochemistry & Molecular Biology; Life Sciences & Biomedicine - Other
Topics
GA 209PR
UT WOS:000323771900015
PM 23976882
ER
PT J
AU Zhang, DZ
Jackson, JM
Chen, B
Sturhahn, W
Zhao, JY
Yan, JY
Caracas, R
AF Zhang, Dongzhou
Jackson, Jennifer M.
Chen, Bin
Sturhahn, Wolfgang
Zhao, Jiyong
Yan, Jinyuan
Caracas, Razvan
TI Elasticity and lattice dynamics of enstatite at high pressure
SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH
LA English
DT Article
DE enstatite; elasticity; lattice dynamics; upper mantle; sound velocities;
equation of state
ID NUCLEAR RESONANT SCATTERING; FUNCTIONAL PERTURBATION-THEORY; MANTLE
SHEAR STRUCTURE; EQUATION-OF-STATE; ORTHO-PYROXENE; MGSIO3
ORTHOENSTATITE; SOUND VELOCITIES; PHASE-TRANSITION; SEISMIC VELOCITIES;
1073 K
AB The behavior of synthetic-powdered Fe-57-enriched enstatite (Mg0.980Fe0.020(5))(Mg0.760Fe0.240)Si2O6 has been explored by X-ray diffraction (XRD) and nuclear resonant inelastic X-ray scattering (NRIXS). The Pbca-structured enstatite sample was compressed in fine pressure increments for our independent XRD measurements. One structural transition between 10.1 and 12.2GPa has been identified from the XRD data. The XRD reflections observed for the high-pressure phase are best matched with space group P2(1)/c. We combine density functional theory with Mossbauer spectroscopy and NRIXS to understand the local site symmetry of the Fe atoms in our sample. A third-order Birch-Murnaghan (BM3) equation of state fitting gives K-T0=1035GPa and KT0=132 for the Pbca phase. At 12GPa, a BM3 fitting gives K-T12=22010GPa with KT12=84 for the P2(1)/c phase. NRIXS measurements were performed with in situ XRD up to 17GPa. The partial phonon density of states (DOS) was derived from the raw NRIXS data, and from the low-energy region of the DOS, the Debye sound velocity was determined. We use the equation of state determined from XRD and Debye sound velocity to compute the isotropic compressional (V-P) and shear (V-S) wave velocities of enstatite at different pressures. Our results help constrain the high-pressure properties of Pbca-structured enstatite in the Earth's upper mantle. We find that candidate upper mantle phase assemblages containing Pbca-structured enstatite are associated with shear velocity gradients that are higher than the average Earth model PREM but lower than regional studies down to about 250km depth.
C1 [Zhang, Dongzhou; Jackson, Jennifer M.; Chen, Bin; Sturhahn, Wolfgang] CALTECH, Div Geol & Planetary Sci, Seismol Lab, Pasadena, CA 91125 USA.
[Zhao, Jiyong] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Yan, Jinyuan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Caracas, Razvan] Univ Lyon 1, Ecole Normale Super Lyon, CNRS, F-69365 Lyon, France.
RP Zhang, DZ (reprint author), CALTECH, Div Geol & Planetary Sci, Seismol Lab, 1200 E Calif Blvd, Pasadena, CA 91125 USA.
EM dzzhang@caltech.edu
RI Chen, Bin/A-5980-2008; Caracas, Razvan/C-8115-2012; Zhang,
Dongzhou/D-9604-2017
OI Zhang, Dongzhou/0000-0002-6679-892X
FU NSF [CAREER EAR-0956166]; Tectonics Observatory at Caltech through the
Gordon and Betty Moore Foundation; COMPRES under NSF Cooperative
Agreement [EAR 06-49658]
FX We thank C. A. Murphy, J. K. Wicks, and A. S. Wolf for help in
conducting experiments and Y. Fei for synthesizing the sample. We thank
the NSF (CAREER EAR-0956166) and the Tectonics Observatory at Caltech
(funded through the Gordon and Betty Moore Foundation) for support of
this research. Use of the Advanced Photon Source was supported by the
U.S. D.O.E., O.S., and O.B.E.S. (DE-AC02-06CH11357). Use of the Advanced
Light Source was supported by the U.S. D.O.E., O.S., and O.B.E.S.
(DE-AC02-05CH11231). Sector 3 operations, the gas-loading system at
GSECARS, and beamline 12.2.2 are supported in part by COMPRES under NSF
Cooperative Agreement EAR 06-49658.
NR 73
TC 8
Z9 8
U1 2
U2 25
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 2169-9313
EI 2169-9356
J9 J GEOPHYS RES-SOL EA
JI J. Geophys. Res.-Solid Earth
PD AUG
PY 2013
VL 118
IS 8
BP 4071
EP 4082
DI 10.1002/jgrb.50303
PG 12
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 225VH
UT WOS:000324991900013
ER
PT J
AU Coates, AJ
Wellbrock, A
Jones, GH
Waite, JH
Schippers, P
Thomsen, MF
Arridge, CS
Tokar, RL
AF Coates, A. J.
Wellbrock, A.
Jones, G. H.
Waite, J. H.
Schippers, P.
Thomsen, M. F.
Arridge, C. S.
Tokar, R. L.
TI Photoelectrons in the Enceladus plume
SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS
LA English
DT Article
DE Enceladus; photoelectrons; plume; ionosphere; Saturn; magnetosphere
ID IONOSPHERIC PHOTOELECTRONS; ELECTRON SPECTROMETER; MAGNETOSPHERE;
PLASMA; SATURN; ATMOSPHERE; VENUS
AB The plume of Enceladus is a remarkable plasma environment containing several charged particle species. These include cold magnetospheric electrons, negative and positive water clusters, charged nanograins, and magnetospheric photoelectrons produced from ionization of neutrals throughout the magnetosphere near Enceladus. Here we discuss observations of a population newly identified by the Cassini Plasma Spectrometer (CAPS) electron spectrometer instrumentphotoelectrons produced in the plume ionosphere itself. These were found during the E19 encounter, in the energetic particle shadow where penetrating particles are absent. Throughout E19, CAPS was oriented away from the ram direction where the clusters and nanograins are observed during other encounters. Plume photoelectrons are also clearly observed during the E9 encounter and are also seen at all other Enceladus encounters where electron spectra are available. This new population, warmer than the ambient plasma population, is distinct from, but adds to, the magnetospheric photoelectrons. Here we discuss the observations and examine the implications, including the ionization source these electrons provide.
C1 [Coates, A. J.; Wellbrock, A.; Jones, G. H.; Arridge, C. S.] Univ Coll London, Mullard Space Sci Lab, Dorking RH5 6NT, Surrey, England.
[Coates, A. J.; Wellbrock, A.; Jones, G. H.; Arridge, C. S.] UCL Birkbeck, Ctr Planetary Sci, London, England.
[Waite, J. H.] SW Res Inst, San Antonio, TX USA.
[Schippers, P.] Observ Paris, LESIA, Meudon, France.
[Thomsen, M. F.; Tokar, R. L.] Planetary Sci Inst, Tucson, AZ USA.
[Thomsen, M. F.; Tokar, R. L.] Los Alamos Natl Lab, Los Alamos, NM USA.
RP Coates, AJ (reprint author), Univ Coll London, Mullard Space Sci Lab, Holmbury St Mary, Dorking RH5 6NT, Surrey, England.
EM a.coates@ucl.ac.uk
RI Jones, Geraint/C-1682-2008; Arridge, Christopher/A-2894-2009; Coates,
Andrew/C-2396-2008;
OI Arridge, Christopher/0000-0002-0431-6526; Coates,
Andrew/0000-0002-6185-3125; Jones, Geraint/0000-0002-5859-1136
FU CAPS ELS science by STFC; CAPS ELS operations and software team by ESA
via the UK Space Agency; Royal Society; NASA JPL [1243218, 1405851];
U.S. Department of Energy; NASA's Cassini project
FX We thank L. K. Gilbert and G. R. Lewis for software support. We
acknowledge support of CAPS ELS science by STFC and of the CAPS ELS
operations and software team by ESA via the UK Space Agency (from 2011).
C. S. A. was supported by a Royal Society research fellowship. Work in
the U. S. was supported by NASA JPL contracts 1243218 and 1405851 to the
Southwest Research Institute. Work at Los Alamos was conducted under the
auspices of the U.S. Department of Energy, with support from NASA's
Cassini project.
NR 39
TC 5
Z9 5
U1 1
U2 9
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 2169-9380
EI 2169-9402
J9 J GEOPHYS RES-SPACE
JI J. Geophys. Res-Space Phys.
PD AUG
PY 2013
VL 118
IS 8
BP 5099
EP 5108
DI 10.1002/jgra.50495
PG 10
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 225VK
UT WOS:000324992300033
ER
PT J
AU Farina, M
Pappadopulo, D
Strumia, A
AF Farina, Marco
Pappadopulo, Duccio
Strumia, Alessandro
TI A modified naturalness principle and its experimental tests
SO JOURNAL OF HIGH ENERGY PHYSICS
LA English
DT Article
DE Beyond Standard Model; Standard Model
ID RENORMALIZATION-GROUP EQUATIONS; DOUBLY-CHARGED HIGGS; QUANTUM-FIELD
THEORY; MINIMAL DARK-MATTER; HIERARCHY PROBLEM; INVISIBLE AXION;
NEUTRINO MASSES; STANDARD MODEL; HARMLESS AXION; CP INVARIANCE
AB Motivated by LHC results, we modify the usual criterion for naturalness by ignoring the uncomputable power divergences. The Standard Model satisfies the modified criterion ('finite naturalness') for the measured values of its parameters. Extensions of the SM motivated by observations (Dark Matter, neutrino masses, the strong CP problem, vacuum instability, inflation) satisfy finite naturalness in special ranges of their parameter spaces which often imply new particles below a few TeV. Finite naturalness bounds are weaker than usual naturalness bounds because any new particle with SM gauge interactions gives a finite contribution to the Higgs mass at two loop order.
C1 [Farina, Marco] Cornell Univ, Dept Phys, LEPP, Ithaca, NY 14853 USA.
[Pappadopulo, Duccio] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Pappadopulo, Duccio] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA.
[Strumia, Alessandro] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy.
[Strumia, Alessandro] Ist Nazl Fis Nucl, I-56127 Pisa, Italy.
[Strumia, Alessandro] NICPB, EE-10143 Tallinn, Estonia.
RP Farina, M (reprint author), Cornell Univ, Dept Phys, LEPP, Ithaca, NY 14853 USA.
EM mf627@cornell.edu; pappadopulo@berkeley.edu; astrumia@mail.df.unipi.it
FU ESF [8090, 8499, MTT8]; SF0690030s09 project; NSF [PHY-0757868]
FX We thank Savas Dimopoulos, Gian Giudice and Mikhail Shaposhnikov for
discussions. This work was supported by the ESF grants 8090, 8499, MTT8
and by SF0690030s09 project. The work of MF was supported in part by the
NSF grant PHY-0757868.
NR 86
TC 48
Z9 48
U1 0
U2 1
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1029-8479
J9 J HIGH ENERGY PHYS
JI J. High Energy Phys.
PD AUG
PY 2013
IS 8
AR 022
DI 10.1007/JHEP08(2013)022
PG 21
WC Physics, Particles & Fields
SC Physics
GA 214EL
UT WOS:000324113700022
ER
PT J
AU Kim, B
Olsson, RH
Wojciechowski, KE
AF Kim, Bongsang
Olsson, Roy H., III
Wojciechowski, Ken E.
TI AlN Microresonator-Based Filters With Multiple Bandwidths at Low
Intermediate Frequencies
SO JOURNAL OF MICROELECTROMECHANICAL SYSTEMS
LA English
DT Article
DE Aluminum nitride (AlN) resonators; filters; microresonators; RF
microelectromechanical systems (MEMS)
ID CONTOUR-MODE RESONATORS; ACOUSTIC RESONATORS
AB Filters with various bandwidths at low intermediate frequency (IF) have been demonstrated using aluminum nitride (AlN) microresonator technology. Specifically, at 13 MHz, 6 kHz, and 25 kHz bandwidth filters were implemented using a single resonator topology, and 250 kHz and 500 kHz bandwidth filters were constructed via the parallel lattice topology using four sub-resonators and L-matching networks. The bandwidths of these filters are from 0.046% to 3.8%, and particularly the 500 kHz bandwidth filter at 13 MHz is >12x wider than that of the resonator k(t)(2) limit (40 kHz). The 100x variations in filter percent bandwidth were realized in a 1700 nm-thick aluminum nitride film on the same wafer through CMOS-compatible fabrication processes. Changes in the filter termination for proper filter matching were implemented in the Agilent Genesys RF and microwave design simulation software using actual measured filter responses with 50 Omega termination. The great flexibility in filter bandwidths and resonant frequencies, as well as other benefits such as size, manufacturing cost, isolation, and insertion loss provided by AlN microresonators will enable next generation multi-band, multi-waveform, and cognitive radios for defense and consumer wireless applications. [2012-0217]
C1 [Kim, Bongsang] Bosch Res & Technol Ctr, Palo Alto, CA 94304 USA.
[Olsson, Roy H., III; Wojciechowski, Ken E.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Kim, B (reprint author), Bosch Res & Technol Ctr, Palo Alto, CA 94304 USA.
EM bongsang.kim@us.bosch.com; rholsso@sandia.gov; kwojcie@sandia.gov
FU U.S. Department of Energy's National Nuclear Security Administration
[DE-AC04-4AL85000]
FX The views expressed are those of the author and do not reflect the
official policy or position of the Department of Defense or the U.S.
Government. The authors would like to thank Dr. S. Raman from DARPA, and
R. Newgard, Dr. R. Potter, and C. Conway from Rockwell Collins for their
support and guidance. They would like to acknowledge the staff of the
Microelectronics Develop Laboratory, Sandia National Laboratories, for
fabrication of the devices and C. Nordquist and M. Balance for the use
of RF characterization resources. Also, a special thanks is given to J.
Nguyen for the help and support in measurement. Sandia National
Laboratories is a multiprogram laboratory managed and operated by Sandia
Corporation, a wholly owned subsidiary of Lockheed Martin Corporation,
for the U.S. Department of Energy's National Nuclear Security
Administration, under Contract DE-AC04-4AL85000.
NR 31
TC 7
Z9 7
U1 0
U2 9
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 1057-7157
J9 J MICROELECTROMECH S
JI J. Microelectromech. Syst.
PD AUG
PY 2013
VL 22
IS 4
BP 949
EP 961
DI 10.1109/JMEMS.2013.2251414
PG 13
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Instruments & Instrumentation; Physics, Applied
SC Engineering; Science & Technology - Other Topics; Instruments &
Instrumentation; Physics
GA 231HW
UT WOS:000325408100015
ER
PT J
AU Freeman, CM
Moridis, G
Ilk, D
Blasingame, TA
AF Freeman, C. M.
Moridis, G.
Ilk, D.
Blasingame, T. A.
TI A numerical study of performance for tight gas and shale gas reservoir
systems
SO JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING
LA English
DT Article
DE shale; tight gas; shale gas; well performance; linear flow; fracture
interference; stimulated reservoir volume
ID FLOW
AB Various analytical, semi-analytical, and empirical models have been proposed to characterize rate and pressure behavior as a function of time in tight gas and shale gas systems featuring horizontal wells with multiple hydraulic fractures. Despite a few analytical models, as well as a small number of published numerical studies, there is currently little consensus regarding the large-scale flow behavior over time in such systems, particularly regarding the dominant flow regimes and whether or not reservoir properties or volumes can be estimated from well performance data.
We constructed a fit-for-purpose numerical simulator which accounts for a variety of production features pertinent to these systems-specifically ultra-tight matrix permeability, hydraulically fractured horizontal wells with induced fractures of various configurations, multiple porosity and permeability fields, and desorption. These features cover the production mechanisms which are currently believed to be most relevant in tight gas and shale gas systems.
We employ the numerical simulator to examine various tight gas and shale gas systems and to identify and illustrate the various flow regimes which progressively occur over time. We perform this study at fine grid discretization on the order of 1 mm near fractures to accurately capture flow effects at all time periods. We visualize the flow regimes using specialized plots of rate and pressure functions, as well as maps of pressure and sorption distributions.
We use pressure maps to visualize the various flow regimes and their transitions in tight gas systems. In a typical tight gas system, we illustrate the initial linear flow into the hydraulic fractures (i.e., formation linear flow), transitioning to compound formation linear flow, and eventually transforming into elliptical flow. We explore variations of possible shale gas system models. Based on diffusive flow (with and without desorption), we show that due to the extremely low permeability of shale matrix (a few nanodarcies), the flow behavior is dominated by the extent of and configuration of the fractures.
This work expands our understanding of flow behavior in tight gas and shale gas systems, where such an understanding may ultimately be used to estimate reservoir properties and reserves in these types of reservoirs. Published by Elsevier B.V.
C1 [Freeman, C. M.; Moridis, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Ilk, D.] DeGolyer & McNaughton, Houston, TX 77056 USA.
[Blasingame, T. A.] Texas A&M Univ, College Stn, TX 77843 USA.
RP Freeman, CM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS 90-1116, Berkeley, CA 94720 USA.
EM cmfreeman@lbl.gov; gjmoridis@lbl.gov; dilk@demac.com;
t-blasingame@tamu.edu
FU RPSEA through the Ultra-Deepwater and Unconventional Natural Gas and
Other Petroleum Resources Research and Development Program [07122-23]
FX This work was supported by RPSEA (Contract no. 07122-23) through the
Ultra-Deepwater and Unconventional Natural Gas and Other Petroleum
Resources Research and Development Program as authorized by the US
Energy Policy Act (EPAct) of 2005.
NR 19
TC 22
Z9 28
U1 4
U2 56
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0920-4105
J9 J PETROL SCI ENG
JI J. Pet. Sci. Eng.
PD AUG
PY 2013
VL 108
BP 22
EP 39
DI 10.1016/j.petrol.2013.05.007
PG 18
WC Energy & Fuels; Engineering, Petroleum
SC Energy & Fuels; Engineering
GA 228ZS
UT WOS:000325232200004
ER
PT J
AU Moridis, GJ
Kim, J
Reagan, MT
Kim, SJ
AF Moridis, George J.
Kim, Jihoon
Reagan, Matthew T.
Kim, Se-Joon
TI Feasibility of gas production from a gas hydrate accumulation at the
UBGH2-6 site of the Ulleung basin in the Korean East Sea
SO JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING
LA English
DT Article
DE gas production; hydrates; Ulleung basin; simulation; flow; geomechanics
ID COUPLED FLOW; SEQUENTIAL-METHODS; BEARING SEDIMENTS; FLUID-FLOW;
STABILITY; DEPOSITS; GEOMECHANICS; DEPRESSURIZATION; DECOMPOSITION;
ALASKA
AB We investigate the feasibility of production from a marine hydrate accumulation that has the properties and conditions of the UBGH2-6 site at the Ulleung basin in the Korean East Sea. The 20 m-thick system is in deep water (2160 m) but close to the ocean floor (with its top at 140 mbsf), and is characterized by alternating mud (near hydrate-free) and sand (hydrate-rich) layers. The layered stratigraphy and the presence of mud layers preclude the use of horizontal wells and necessitate vertical wells. The analysis indicates that production from such a hydrate accumulation is feasible, but the production rates are generally modest. The production rate Q(p) peaks at about 1.45 ST m(3)/s = 4.4 MMSCFD at about t = 1 year, and continuously declines afterward. Sensitivity analysis indicates that cumulative production increases with a declining initial hydrate saturation, an increasing intrinsic permeability of the sand layers and an increasing thermal conductivity of the porous media, while the effect of porosity is non-monotonic: production initially increases with a decreasing porosity, but the trend is later reversed. However, the sensitivity to these parameters is limited, and does not alter the overall predictions of modest production potential. The geomechanical situation appears challenging, as significant subsidence (exceeding 3.5 m at a depth of 20 m below the sea floor, and 1.5 m at the top of the hydrate deposit) is estimated to occur along a large part of the wellbore, and yielding and failure within the 20 m-thick system are possible early in the production process. However, there is significant uncertainty in the predictions of the geomechanical system behavior because they are not based on measured system properties but only on estimates/assumptions from analogs. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Moridis, George J.; Kim, Jihoon; Reagan, Matthew T.] Div Earth Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Kim, Se-Joon] Korea Inst Geosci & Mineral Resources, Petr & Marine Res Div, Taejon, South Korea.
RP Moridis, GJ (reprint author), Div Earth Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM gjmoridis@lbl.gov
RI Reagan, Matthew/D-1129-2015
OI Reagan, Matthew/0000-0001-6225-4928
FU Korea Institute of Geoscience and Mineral Resources; Office of Natural
Gas and Petroleum Technology, through the National Energy Technology
Laboratory, under the U.S. Department of Energy [DE-AC02-05CH11231]
FX This work was supported by the Korea Institute of Geoscience and Mineral
Resources, and by the Assistant Secretary for Fossil Energy, Office of
Natural Gas and Petroleum Technology, through the National Energy
Technology Laboratory, under the U.S. Department of Energy, Contract no.
DE-AC02-05CH11231.
NR 48
TC 7
Z9 7
U1 2
U2 22
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0920-4105
J9 J PETROL SCI ENG
JI J. Pet. Sci. Eng.
PD AUG
PY 2013
VL 108
BP 180
EP 210
DI 10.1016/j.petrol.2013.03.002
PG 31
WC Energy & Fuels; Engineering, Petroleum
SC Energy & Fuels; Engineering
GA 228ZS
UT WOS:000325232200018
ER
PT J
AU Tokunaga, TK
Wan, JM
Jung, JW
Kim, TW
Kim, Y
Dong, WM
AF Tokunaga, Tetsu K.
Wan, Jiamin
Jung, Jong-Won
Kim, Tae Wook
Kim, Yongman
Dong, Wenming
TI Capillary pressure and saturation relations for supercritical CO2 and
brine in sand: High-pressure P-c(S-w) controller/meter measurements and
capillary scaling predictions
SO WATER RESOURCES RESEARCH
LA English
DT Article
DE capillary pressure; geologic carbon sequestration; capillary scaling;
wettability
ID CONTACT-ANGLE MEASUREMENTS; POROUS-MEDIA; CARBON-DIOXIDE; FRACTIONAL
WETTABILITY; HYDRAULIC CONDUCTIVITY; INTERFACIAL-TENSIONS;
SURFACE-ROUGHNESS; SILICA SURFACES; SALINE AQUIFERS; HYDROXYL-GROUPS
AB In geologic carbon sequestration, reliable predictions of CO2 storage require understanding the capillary behavior of supercritical (sc) CO2. Given the limited availability of measurements of the capillary pressure (P-c) dependence on water saturation (S-w) with scCO(2) as the displacing fluid, simulations of CO2 sequestration commonly rely on modifying more familiar air/H2O and oil/H2O P-c(S-w) relations, adjusted to account for differences in interfacial tensions. In order to test such capillary scaling-based predictions, we developed a high-pressure P-c(S-w) controller/meter, allowing accurate P-c and S-w measurements. Drainage and imbibition processes were measured on quartz sand with scCO(2)-brine at pressures of 8.5 and 12.0MPa (45 degrees C), and air-brine at 21 degrees C and 0.1MPa. Drainage and rewetting at intermediate S-w levels shifted to P-c values that were from 30% to 90% lower than predicted based on interfacial tension changes. Augmenting interfacial tension-based predictions with differences in independently measured contact angles from different sources led to more similar scaled P-c(S-w) relations but still did not converge onto universal drainage and imbibition curves. Equilibrium capillary trapping of the nonwetting phases was determined for P-c=0 during rewetting. The capillary-trapped volumes for scCO(2) were significantly greater than for air. Given that the experiments were all conducted on a system with well-defined pore geometry (homogeneous sand), and that scCO(2)-brine interfacial tensions are fairly well constrained, we conclude that the observed deviations from scaling predictions resulted from scCO(2)-induced decreased wettability. Wettability alteration by scCO(2) makes predicting hydraulic behavior more challenging than for less reactive fluids.
Key Points equilibrium between CO2 and brine in reservoirs differs from nonreactive fluids wettability alteration from CO2 exposure is important residual trapping of CO2 can be higher than expected
C1 [Tokunaga, Tetsu K.; Wan, Jiamin; Jung, Jong-Won; Kim, Tae Wook; Kim, Yongman; Dong, Wenming] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
RP Tokunaga, TK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM tktokunaga@lbl.gov
RI Kim, Tae Wook/E-5954-2011; Tokunaga, Tetsu/H-2790-2014; Wan,
Jiamin/H-6656-2014; Kim, Yongman/D-1130-2015; Dong, Wenming/G-3221-2015
OI Tokunaga, Tetsu/0000-0003-0861-6128; Kim, Yongman/0000-0002-8857-1291;
Dong, Wenming/0000-0003-2074-8887
FU ZERT; NCGC; NRAP; Office of Sequestration, Hydrogen, and Clean Coal
Fuels, through the National Energy Technology Laboratory (NETL), U.S.
Department of Energy [DE-AC02-05CH11231]; Center for Nanoscale Control
of Geologic CO2, an Energy Frontier Research Center; U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences
[DE-AC02-05CH11231]; DOE Office of Fossil Energy's Cross Cutting
Research program; NRAP under U.S. Department of Energy
[DE-AC02-05CH11231]
FX This work was carried out under funding support from the ZERT, NCGC, and
NRAP. The ZERT project was funded by the Assistant Secretary for Fossil
Energy, Office of Sequestration, Hydrogen, and Clean Coal Fuels, through
the National Energy Technology Laboratory (NETL), U.S. Department of
Energy under contract DE-AC02-05CH11231. This material is also based on
work supported as part of the Center for Nanoscale Control of Geologic
CO2, an Energy Frontier Research Center funded by the U.S.
Department of Energy, Office of Science, Office of Basic Energy Sciences
under award DE-AC02-05CH11231. Portions of this work were completed as
part of National Risk Assessment Partnership (NRAP) project. Support for
this project came from the DOE Office of Fossil Energy's Cross Cutting
Research program. The authors wish to acknowledge Robert Romanosky (NETL
Strategic Center for Coal) and Regis Conrad (DOE Office of Fossil
Energy) for programmatic guidance, direction, and support. NRAP is a
multilab effort that leverages broad technical capabilities across the
DOE complex. NRAP involves five DOE national laboratories: NETL,
Lawrence Berkeley National Laboratory, Lawrence Livermore National
Laboratory, Los Alamos National Laboratory, and Pacific Northwest
National Laboratory. This team is working together to develop a
science-based method for quantifying the likelihood of risks (and
associated potential liabilities) for CO2 storage sites. The
work in this paper was reviewed by members of the NRAP Technical
Leadership Team, including Jens Birkholzer. NRAP funding was provided to
Lawrence Berkeley National Laboratory under U.S. Department of Energy
contract DE-AC02-05CH11231. The authors thank Christopher Pentland and
the anonymous reviewers for their helpful suggestions that lead to
improved presentation.
NR 81
TC 19
Z9 19
U1 0
U2 30
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 0043-1397
J9 WATER RESOUR RES
JI Water Resour. Res.
PD AUG
PY 2013
VL 49
IS 8
BP 4566
EP 4579
DI 10.1002/wrcr.20316
PG 14
WC Environmental Sciences; Limnology; Water Resources
SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water
Resources
GA 223VA
UT WOS:000324838300003
ER
PT J
AU Grate, JW
Warner, MG
Pittman, JW
Dehoff, KJ
Wietsma, TW
Zhang, CY
Oostrom, M
AF Grate, Jay W.
Warner, Marvin G.
Pittman, Jonathan W.
Dehoff, Karl J.
Wietsma, Thomas W.
Zhang, Changyong
Oostrom, Mart
TI Silane modification of glass and silica surfaces to obtain equally
oil-wet surfaces in glass-covered silicon micromodel applications
SO WATER RESOURCES RESEARCH
LA English
DT Article
DE wettability; contact angle; silanization; glass; silica; surface
modification; micromodel; porous media; pore network; immiscible
displacement
ID POROUS-MEDIA; INTERFACIAL PROPERTIES; CONTACT-ANGLE; WETTABILITY; WATER;
VISUALIZATION; INFILTRATION; DISPLACEMENT; DISSOLUTION; SATURATION
AB Wettability is a key parameter influencing capillary pressures, permeabilities, fingering mechanisms, and saturations in multiphase flow processes within porous media. Glass-covered silicon micromodels provide precise structures in which pore-scale displacement processes can be visualized. The wettability of silicon and glass surfaces can be modified by silanization. However, similar treatments of glass and silica surfaces using the same silane do not necessarily yield the same wettability as determined by the oil-water contact angle. In this study, surface cleaning pretreatments were investigated to determine conditions that yield oil-wet surfaces on glass with similar wettability to silica surfaces treated with the same silane, and both air-water and oil-water contact angles were determined. Borosilicate glass surfaces cleaned with standard cleaning solution 1 (SC1) yield intermediate-wet surfaces when silanized with hexamethyldisilazane (HMDS), while the same cleaning and silanization yields oil-wet surfaces on silica. However, cleaning glass in boiling concentrated nitric acid creates a surface that can be silanized to obtain oil-wet surfaces using HMDS. Moreover, this method is effective on glass with prior thermal treatment at an elevated temperature of 400 degrees C. In this way, silica and glass can be silanized to obtain equally oil-wet surfaces using HMDS. It is demonstrated that pretreatment and silanization is feasible in silicon-silica/glass micromodels previously assembled by anodic bonding, and that the change in wettability has a significant observable effect on immiscible fluid displacements in the pore network.
C1 [Grate, Jay W.; Warner, Marvin G.; Pittman, Jonathan W.; Dehoff, Karl J.; Wietsma, Thomas W.; Zhang, Changyong; Oostrom, Mart] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Grate, JW (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA.
EM jwgrate@pnnl.gov
RI Zhang, Changyong/A-8012-2013
FU The Carbon Sequestration Initiative of the Laboratory Directed Research
and Development Program at the Pacific Northwest National Laboratory
(PNNL); Department of Energy's Office of Biological and Environmental
Research
FX The Carbon Sequestration Initiative of the Laboratory Directed Research
and Development Program at the Pacific Northwest National Laboratory
(PNNL) supported this research. A portion of this research was carried
out in the William R. Wiley Environmental Molecular Sciences Laboratory
(EMSL), a national scientific user facility sponsored by the Department
of Energy's Office of Biological and Environmental Research and located
at PNNL. PNNL is a multiprogram national laboratory operated for the DOE
by Battelle Memorial Institute.
NR 45
TC 9
Z9 9
U1 5
U2 59
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 0043-1397
J9 WATER RESOUR RES
JI Water Resour. Res.
PD AUG
PY 2013
VL 49
IS 8
BP 4724
EP 4729
DI 10.1002/wrcr.20367
PG 6
WC Environmental Sciences; Limnology; Water Resources
SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water
Resources
GA 223VA
UT WOS:000324838300015
ER
PT J
AU Revil, A
Wu, Y
Karaoulis, M
Hubbard, SS
Watson, DB
Eppehimer, JD
AF Revil, A.
Wu, Y.
Karaoulis, M.
Hubbard, S. S.
Watson, D. B.
Eppehimer, J. D.
TI Geochemical and geophysical responses during the infiltration of fresh
water into the contaminated saprolite of the Oak Ridge Integrated Field
Research Challenge site, Tennessee
SO WATER RESOURCES RESEARCH
LA English
DT Article
DE induced polarization; resistivity; ERT; complex conductivity; flow
through experiment; saprolite
ID SPECTRAL INDUCED POLARIZATION; COMPLEX CONDUCTIVITY; SHALY SANDS;
POROUS-MEDIA; PERMEABILITY; TRANSPORT; SOIL
AB At the Oak Ridge Integrated Field Research Challenge (IFRC) site, Tennessee, the saprolitic aquifer was contaminated by leaks from the former S-3 disposal ponds between 1951 and 1983. The chemistry of the contaminant plume is also episodically impacted by fresh meteoritic water infiltrating vertically from a shallow variably saturated perched zone and the ditch surrounding the former S-3 ponds. We performed a column experiment using saprolite from the contaminated aquifer to understand the geochemical and complex electrical conductivity signatures associated with such events. The changes in the pH and pore water ionic strength are responsible for measurable changes in both the in-phase and quadrature conductivities. The pore water conductivity can be related to the nitrate concentration (the main ionic species in the plume) while the release of uranium is controlled by the pH. We developed a simple model to determine the pore water conductivity and pH from the recorded complex conductivity. This model is applied to time-lapse resistivity data at the IFRC site. Time-lapse inversion of resistivity data, performed with an active time constrain approach, shows the occurrence of an infiltration event during the winter of 2008-2009 with a dilution of the pore water chemistry and an increase of the pH. A simple numerical simulation of the infiltration of fresh water into the unconfined contaminated aquifer is consistent with this scenario.
Key Points Complex conductivity is related to pore water and interfacial chemistry Surface conductivity cannot be neglected in ERT Time-lapse ERT is used to monitor an infiltration event.
C1 [Revil, A.; Eppehimer, J. D.] Colorado Sch Mines, Dept Geophys, Golden, CO 80401 USA.
[Revil, A.; Karaoulis, M.] Univ Savoie, ISTerre, CNRS, UMR 5275, Le Bourget Du Lac, France.
[Wu, Y.; Hubbard, S. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Watson, D. B.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
RP Revil, A (reprint author), Colorado Sch Mines, Dept Geophys, Golden, CO 80401 USA.
EM arevil@mines.edu
RI Hubbard, Susan/E-9508-2010; Watson, David/C-3256-2016; Wu,
Yuxin/G-1630-2012
OI Watson, David/0000-0002-4972-4136; Wu, Yuxin/0000-0002-6953-0179
FU Environment Remediation Science Program (ERSP), U.S. Department of
Energy (DOE) [DE-FG02-08ER646559]
FX We thank the Environment Remediation Science Program (ERSP), U.S.
Department of Energy (DOE, award DE-FG02-08ER646559) for funding. The
authors appreciate the efforts of Davis Lesmes, the ERSP program
manager. We thank Marcella Mueller for her help in getting the Oak Ridge
data and samples, Jennifer Earles for the Water levels, Kevin Birdwell
for the precipitation data from the ORNL Meteorological Program, and
Magnus Skold for his help with the experimental data. We thank the three
referees and the Associate Editor for their constructive reviews.
NR 30
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U1 1
U2 21
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 0043-1397
J9 WATER RESOUR RES
JI Water Resour. Res.
PD AUG
PY 2013
VL 49
IS 8
BP 4952
EP 4970
DI 10.1002/wrcr.20380
PG 19
WC Environmental Sciences; Limnology; Water Resources
SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water
Resources
GA 223VA
UT WOS:000324838300032
ER
PT J
AU Kim, TW
Tokunaga, TK
Bargar, JR
Latimer, MJ
Webb, SM
AF Kim, Tae Wook
Tokunaga, Tetsu K.
Bargar, John R.
Latimer, Matthew J.
Webb, Samuel M.
TI Brine film thicknesses on mica surfaces under geologic CO2 sequestration
conditions and controlled capillary pressures
SO WATER RESOURCES RESEARCH
LA English
DT Article
DE brine film; CO2 sequestration; capillary pressure; mica; roughness;
synchrotron X-ray fluorescence (XRF)
ID DISJOINING PRESSURE; SUPERCRITICAL CO2; WETTING PHENOMENA;
REFRACTIVE-INDEX; MUSCOVITE MICA; CARBON-DIOXIDE; SOLID-SURFACES;
PORE-SCALE; WATER; CONDENSATION
AB Brine films remaining on mineral surfaces in deep reservoirs during CO2 sequestration are expected to influence multiphase flow, diffusion, and reactions, but little is known about their behavior. Using synchrotron X-ray fluorescence (XRF), we measured thicknesses of KCsI2 brine films on two difference roughness mica surfaces under conditions representative of geological CO2 sequestration (7.8 MPa and 40 degrees C) to understand the influences of mineral surface roughness and capillary potential. Brine thicknesses measured on the Mica 1 (smooth) and Mica 2 (rough) mica surfaces ranged from 23 to 8 nm and 491 to 412 nm, respectively, over the small range of tested capillary potentials (0.18-3.7 kPa). Within these potentials, brine film thicknesses on mica were governed by surface roughness and only weakly influenced by capillary potentials. In comparing drainage and rewetting isotherms, some film thickness hysteresis was observed, possibly indicative of changes in mica wettability.
Key Points
Influences of surface roughness and capillary pressure on brine films on mica The hysteresis on both mica surfaces may be related to contact angle hysteresis The comparisons between experimental data and DLVO theory
C1 [Kim, Tae Wook; Tokunaga, Tetsu K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Kim, Tae Wook] Stanford Univ, Dept Energy Resources Engn, Sch Earth Sci, Stanford, CA 94583 USA.
[Bargar, John R.; Latimer, Matthew J.; Webb, Samuel M.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Stanford, CA USA.
RP Kim, TW (reprint author), Stanford Univ, Dept Energy Resources Engn, Sch Earth Sci, 367 Panama St, Stanford, CA 94583 USA.
EM taewkim@stanford.edu
RI Kim, Tae Wook/E-5954-2011; Tokunaga, Tetsu/H-2790-2014; Webb,
Samuel/D-4778-2009
OI Tokunaga, Tetsu/0000-0003-0861-6128; Webb, Samuel/0000-0003-1188-0464
FU Center for Nanoscale Control of Geologic CO2, an Energy Frontier
Research Center; U.S. Department of Energy (DOE), Office of Science;
U.S. DOE [DE-AC02-05CH11231]; DOE Office of Biological and Environmental
Research; National Institutes of Health, National Institute of General
Medical Sciences [P41GM103393]; National Center for Research Resources
[P41RR001209]
FX This research is supported as part of the Center for Nanoscale Control
of Geologic CO2, an Energy Frontier Research Center funded by
the U.S. Department of Energy (DOE), Office of Science. This research
was carried out under U.S. DOE contract DE-AC02-05CH11231. Portions of
this study were carried out at the Stanford Synchrotron Radiation
Lightsource (SSRL), a Directorate of SLAC National Accelerator
Laboratory and an Office of Science User Facility operated for the U.S.
DOE, Office of Science by Stanford University. The SSRL Structural
Molecular Biology Program is supported by the DOE Office of Biological
and Environmental Research, and by the National Institutes of Health,
National Institute of General Medical Sciences (including P41GM103393)
and the National Center for Research Resources (P41RR001209). In
addition, we thank Kevin Knauss for use of the AFM, and the anonymous
reviewers for their valuable comments.
NR 35
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Z9 5
U1 1
U2 22
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 0043-1397
J9 WATER RESOUR RES
JI Water Resour. Res.
PD AUG
PY 2013
VL 49
IS 8
BP 5071
EP 5076
DI 10.1002/wrcr.20404
PG 6
WC Environmental Sciences; Limnology; Water Resources
SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water
Resources
GA 223VA
UT WOS:000324838300041
ER
PT J
AU Sawada, D
Nishiyama, Y
Petridis, L
Parthasarathi, R
Gnanakaran, S
Forsyth, VT
Wada, M
Langan, P
AF Sawada, Daisuke
Nishiyama, Yoshiharu
Petridis, Loukas
Parthasarathi, R.
Gnanakaran, S.
Forsyth, V. Trevor
Wada, Masahisa
Langan, Paul
TI Structure and dynamics of a complex of cellulose with EDA: insights into
the action of amines on cellulose
SO CELLULOSE
LA English
DT Article
DE Neutron diffraction; Computational simulation; Cellulose amino complex;
Ethylene diamine; Crystal transition; Hydrogen-bond
ID NEUTRON FIBER DIFFRACTION; SYNCHROTRON X-RAY; AMMONIA-SOLVENT
COMBINATIONS; HYDROGEN-BONDING SYSTEM; PARTICLE MESH EWALD;
MOLECULAR-DYNAMICS; LIQUID-AMMONIA; CRYSTALLINE CELLULOSE;
ENZYMATIC-HYDROLYSIS; ELECTRON-DIFFRACTION
AB The neutron structure of a complex of EDA with cellulose has been determined to reveal the location of hydrogen atoms involved in hydrogen-bonding. EDA disrupts the hydrogen-bonding pattern of naturally occurring cellulose by accepting a strong hydrogen-bond from the O6 hydroxymethyl group as the conformation of this group is rotated from tg to gt. The O3-H center dot O5 intrachain hydrogen-bond commonly found in cellulose allomorphs is observed to be disordered in the neutron structure, and quantum chemistry and molecular dynamics calculations show that O3 prefers to donate to EDA. The hydrogen-bonding arrangement is highly dynamic with bonds continually being formed and broken thus explaining the difficulty in locating all of the hydrogen atoms in the neutron scattering density maps. Comparison with other polysaccharide-amino complexes supports a common underlying mechanism for amine disruption of cellulose.
C1 [Sawada, Daisuke; Langan, Paul] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.
[Nishiyama, Yoshiharu] Univ Grenoble 1, Ctr Rech Macromol Vegetales, CNRS, F-38041 Grenoble 9, France.
[Petridis, Loukas] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA.
[Parthasarathi, R.; Gnanakaran, S.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM 87545 USA.
[Forsyth, V. Trevor] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 5, France.
[Forsyth, V. Trevor] Keele Univ, EPSAM, Keele ST5 5BG, Staffs, England.
[Forsyth, V. Trevor] Keele Univ, ISTM, Keele ST5 5BG, Staffs, England.
[Wada, Masahisa] Univ Tokyo, Dept Biomat Sci, Grad Sch Agr & Life Sci, Tokyo 1138657, Japan.
[Wada, Masahisa] Kyung Hee Univ, Dept Plant & Environm New Resources, Coll Life Sci, Yongin 446701, Gyeonggi Do, South Korea.
RP Sawada, D (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.
EM sawadad@ornl.gov
RI Parthasarathi, Ramakrishnan/C-2093-2008; Forsyth, V. Trevor/A-9129-2010;
Nishiyama, Yoshiharu/A-3492-2012; Langan, Paul/N-5237-2015; Petridis,
Loukas/B-3457-2009;
OI Parthasarathi, Ramakrishnan/0000-0001-5417-5867; Forsyth, V.
Trevor/0000-0003-0380-3477; Nishiyama, Yoshiharu/0000-0003-4069-2307;
Langan, Paul/0000-0002-0247-3122; Petridis, Loukas/0000-0001-8569-060X;
Gnanakaran, S/0000-0002-9368-3044
FU French Agence Nationale de la Reserche; Genomic Science Program, Office
of Biological and Environmental Research, US Department of Energy [FWP
ERKP752]; Center for Structural Molecular Biology (CSMB); Office of
Biological and Environmental Research; U.S. Department of Energy
[DE-AC05-00OR22725]; Office of Science of DOE [DE-AC02-05CH11231]; UK
Engineering and Physical Sciences Research Council (EPSRC)
[GR/R47950/01]; [18780131]
FX We thank beam line D19 at the Institute Laue Langevin for use of
facilities, John Allibon, John Archer and Sax Mason for support with
data collection, and Thomas Rosenau for helpful discussions and advice.
MW was supported by a Grant-in-Aid for Scientific Research (18780131).
This study was partly funded by the French Agence Nationale de la
Reserche. PL and LP were partly funded by the Genomic Science Program,
Office of Biological and Environmental Research, US Department of
Energy, under FWP ERKP752. PL was partly support by the Center for
Structural Molecular Biology (CSMB) which is supported by the Office of
Biological and Environmental Research, using facilities supported by the
U.S. Department of Energy, managed by UT-Battelle, LLC under contract
No. DE-AC05-00OR22725. This research used resources of the Hopeper
supercomputer at NERSC, supported by the Office of Science of DOE under
Contract No. DE-AC02-05CH11231. VTF acknowledges support from the UK
Engineering and Physical Sciences Research Council (EPSRC) for the
construction of the D19 diffractometer at the ILL under grant
GR/R47950/01
NR 56
TC 2
Z9 2
U1 6
U2 33
PU SPRINGER
PI DORDRECHT
PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS
SN 0969-0239
EI 1572-882X
J9 CELLULOSE
JI Cellulose
PD AUG
PY 2013
VL 20
IS 4
BP 1563
EP 1571
DI 10.1007/s10570-013-9974-7
PG 9
WC Materials Science, Paper & Wood; Materials Science, Textiles; Polymer
Science
SC Materials Science; Polymer Science
GA 195AE
UT WOS:000322673000003
ER
PT J
AU Watkins, JM
Nielsen, LC
Ryerson, FJ
DePaolo, DJ
AF Watkins, James M.
Nielsen, Laura C.
Ryerson, Frederick J.
DePaolo, Donald J.
TI The influence of kinetics on the oxygen isotope composition of calcium
carbonate
SO EARTH AND PLANETARY SCIENCE LETTERS
LA English
DT Article
DE calcite; oxygen isotopes; equilibrium; kinetic; carbonic anhydrase;
paleothermometry
ID CA-44/CA-40 FRACTIONATION; EQUILIBRIUM FRACTIONATION; ZEEBE,R.E. 1999;
TRACE-ELEMENT; CA ISOTOPES; IN-SITU; EXPLANATION; BICARBONATE;
ANHYDRASE; SYSTEM
AB Paleotemperature reconstructions rely on knowledge of the equilibrium separation of oxygen isotopes between aqueous solution and calcium carbonate. Although oxygen isotope separation is expected on theoretical grounds, the temperature-dependence remains uncertain because other factors, such as slow exchange of isotopes between dissolved CO2-species and water, can obscure the temperature signal. This is problematic for crystal growth experiments on laboratory timescales and for interpreting the oxygen isotope composition of crystals formed in natural settings. We present results from experiments in which inorganic calcite is precipitated in the presence of 0.25 mu M dissolved bovine carbonic anhydrase (CA). The presence of dissolved CA accelerates oxygen isotope equilibration between the dissolved carbon species CO2, H2CO3, HCO3-, CO32- and water, thereby eliminating this source of isotopic disequilibrium during calcite growth. The experimental results allow us to isolate, for the first time, kinetic oxygen isotope effects occurring at the calcite water interface. We present a framework of ion-by-ion growth of calcite that reconciles our new measurements with measurements of natural cave calcites that are the best candidate for having precipitated under near-equilibrium conditions. Our findings suggest that isotopic equilibrium between calcite and water is unlikely to have been established in laboratory experiments or in many natural settings. The use of CA in carbonate precipitation experiments offers new opportunities to refine oxygen isotope-based geothermometers and to interrogate environmental variables other than temperature that influence calcite growth rates. Published by Elsevier B.V.
C1 [Watkins, James M.] Univ Oregon, Dept Geol Sci, Eugene, OR 97403 USA.
[Nielsen, Laura C.] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA.
[Ryerson, Frederick J.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[DePaolo, Donald J.] Lawrence Livermore Natl Lab, Div Earth Sci, Livermore, CA USA.
[DePaolo, Donald J.] Univ Calif Berkeley, Berkeley, CA 94720 USA.
RP Watkins, JM (reprint author), Univ Oregon, Dept Geol Sci, Eugene, OR 97403 USA.
EM watkins4@uoregon.edu
FU U.S. Depailinent of Energy, Office of Basic Energy Sciences, Division of
Chemical, Biological and Geological Sciences through Lawrence Berkeley
National Laboratory; Center for Nanoscale Control of Geologic
CO2, an Energy Frontier Research Center [DE-AC02-05CH11231,
DE-AC52-07NA27344]
FX Alexander Gagnon is credited for suggesting we use carbonic anhydrase in
our experiments. Wenbo Yang made the oxygen isotope measurements. Dave
Ruddle and Matthew Gonzales helped build the experimental apparatus. We
are grateful for discussions with Mariette Wolthers, Aradhna Tripati,
Shaun Brown, and Amanda Thomas, as well as comments from two anonymous
reviewers. This research was supported by the U.S. Depailinent of
Energy, Office of Basic Energy Sciences, Division of Chemical,
Biological and Geological Sciences through Lawrence Berkeley National
Laboratory and as part of the Center for Nanoscale Control of Geologic
CO2, an Energy Frontier Research Center under contract No.
DE-AC02-05CH11231 (LBNL) and Contract No. DE-AC52-07NA27344 (LLNL).
NR 37
TC 35
Z9 35
U1 3
U2 42
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0012-821X
J9 EARTH PLANET SC LETT
JI Earth Planet. Sci. Lett.
PD AUG 1
PY 2013
VL 375
BP 349
EP 360
DI 10.1016/j.epsl.2013.05.054
PG 12
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 223YB
UT WOS:000324847300032
ER
PT J
AU Best, MG
Christiansen, EH
Deino, AL
Gromme, S
Hart, GL
Tingey, DG
AF Best, Myron G.
Christiansen, Eric H.
Deino, Alan L.
Gromme, Sherman
Hart, Garret L.
Tingey, David G.
TI The 36-18 Ma Indian Peak-Caliente ignimbrite field and calderas,
southeastern Great Basin, USA: Multicyclic super-eruptions
SO GEOSPHERE
LA English
DT Article
ID SNAKE RANGE DECOLLEMENT; DUCTILE-BRITTLE TRANSITION; SILICIC MAGMA
CHAMBERS; ASH-FLOW CALDERAS; NORTH-AMERICA; SOUTHWESTERN UTAH; EASTERN
NEVADA; VOLCANIC FIELD; LINCOLN COUNTY; GRANITIC-ROCKS
AB The Indian Peak-Caliente caldera complex and its surrounding ignimbrite field were a major focus of explosive silicic activity in the eastern sector of the subduction-related southern Great Basin ignimbrite province during the middle Cenozoic (36-18 Ma) ignimbrite flareup. Caldera-forming activity migrated southward through time in response to rollback of the subducting lithosphere. Nine partly exposed, separate to partly overlapping source calderas and an equal number of concealed sources compose the Indian Peak-Caliente caldera complex. Calderas have diameters to as much as 60 km and are filled with as much as 5000 m of intracaldera tuff and wall-collapse breccias.
More than 50 ignimbrite cooling units, including 22 of regional (> 100 km(3)) extent, are distinguished on the basis of stratigraphic position, chemical and modal composition, Ar-40/Ar-39 age, and paleomagnetic direction. The most voluminous ash flows spread as far as 150 km from the caldera complex across a high plateau of limited relief-the Great Basin altiplano, which was created by late Paleozoic through Mesozoic orogenic deformation and crustal thickening. The resulting ignimbrite field covers a present area of similar to 60,000 km(2) in east-central Nevada and southwestern Utah. Before post-volcanic extension, ignimbrites had an estimated aggregate volume of similar to 33,000 km(3). At least seven of the largest cooling units were produced by super-eruptions of more than 1000 km(3). The largest, at 5900 km(3), originally covered an area of 32,000 km(2) to outflow depths of hundreds of meters. Outflow ignimbrite sequences comprise as many as several cooling units from different sources with an aggregate thickness locally reaching a kilometer; sequences are almost everywhere conformable and lack substantial intervening erosional debris and angular discordances, thus manifesting a lack of synvolcanic crustal extension. Fallout ash in the mid-continent is associated with two of the super-eruptions.
Ignimbrites are mostly calc-alkalic and high-K, a reflection of the unusually thick crust in which the magmas were created. They have a typical arc chemical signature and define a spectrum of compositions that ranges from high-silica (78 wt%) rhyolite to andesite (61 wt% silica). Rhyolite magmas were erupted in relatively small volumes more or less throughout the history of activity, but in a much larger volume after 24 Ma in the southern part of the caldera complex, creating 10,000 km3 of ignimbrite. The field has some rhyolite ignimbrites, the largest of which are in the south and were emplaced after 24 Ma. But the most distinctive attributes of the Indian Peak-Caliente field are two distinct classes of ignimbrite:
1. Super-eruptive monotonous intermediates. More or less uniform and unzoned deposits of dacitic ignimbrite that are phenocryst rich (to as much as similar to 50%) with plagioclase > biotite approximate to quartz approximate to hornblende > Fe-Ti oxides +/- sanidine, pyroxene, and titanite; apatite and zircon are ubiquitous accessory phases. These tuffs were deposited at 31.13, 30.06, and 29.20 Ma in volumes of 2000, 5900, and 4400 km(3), respectively, from overlapping, multicyclic calderas. A unique, and pos-sibly kindred, phenocryst-rich latiteandesite ignimbrite with an outflow volume of 1100 km(3) was erupted at 22.56 Ma from a concealed source caldera to the south.
2. Trachydacitic Isom-type tuffs. Also relatively uniform but phenocryst poor (< 20%) with plagioclase >> clinopyroxene approximate to orthopyroxene approximate to Fe-Ti oxides >> apatite. These alkali-calcic tuffs are enriched in TiO2, K2O, P2O5, Ba, Nb, and Zr and depleted in CaO, MgO, Ni, and Cr, and have an arc chemical signature. Magmas were erupted from a concealed source immediately after and just to the southeast of the multicyclic monotonous intermediates. Most of their aggregate outflow volume of 1800 km3 was erupted from 27.90 to 27.25 Ma. Nothing like this couplet of distinct ignimbrites, in such volumes, have been documented in other middle Cenozoic volcanic fields in the southwestern U. S. where the ignimbrite flareup is manifest. Magmas were created in unusually thick crust (as thick as 70 km) where large-scale inputs of mantle-derived basaltic magma powered partial melting, assimilation, mixing, and differentiation processes. Dacite and some rhyolite ignimbrites were derived from relatively low-temperature (700-800 C), water-rich magmas that were a couple of log units more oxidized than the quartz-fayalite-magnetite (QFM) oxygen buffer at depths of similar to 8-12 km. In contrast to these "main-trend" magmas, trachydacitic Isom-type magmas were derived from drier and hotter (similar to 950 degrees C) magmas originating deeper in the crust (to as deep as 30 km) by fractionation processes in andesitic differentiates of the mantle magma. "Off-trend" rhyolitic magmas that are both younger and older than the Isom type but possessed some of their same chemical characteristics possibly reflect an ancestry involving Isom-type magmas as well as main-trend rhyolitic magmas.
Andesitic lavas extruded during the flareup but mostly after 25 Ma constitute a roughly estimated 12% of the volume of silicic ignimbrite, in contrast to major volcanic fields to the east, e. g., the Southern Rocky Mountain field, where the volume of intermediate-composition lavas exceeds that of silicic ignimbrites.
C1 [Best, Myron G.; Christiansen, Eric H.; Tingey, David G.] Brigham Young Univ, Dept Geol Sci, Provo, UT 84602 USA.
[Deino, Alan L.] Berkeley Geochronol Ctr, Berkeley, CA 94709 USA.
[Hart, Garret L.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Best, MG (reprint author), Brigham Young Univ, Dept Geol Sci, Provo, UT 84602 USA.
OI Christiansen, Eric/0000-0002-1108-5260
FU National Science Foundation [EAR-8604195, 8618323, 8904245, 9104612,
9706906, 0923495]; Brigham Young University
FX Financial support for the Great Basin project was provided by the
National Science Foundation through grants EAR-8604195, 8618323,
8904245, 9104612, 9706906, and 0923495 to M. G. Best and E. H.
Christiansen. The U.S. Geological Survey and Nevada Bureau of Mines and
Geology supported quadrangle mapping. The continuing financial and
material assistance of Brigham Young University is gratefully
acknowledged.
NR 143
TC 13
Z9 13
U1 1
U2 17
PU GEOLOGICAL SOC AMER, INC
PI BOULDER
PA PO BOX 9140, BOULDER, CO 80301-9140 USA
SN 1553-040X
J9 GEOSPHERE
JI Geosphere
PD AUG
PY 2013
VL 9
IS 4
BP 864
EP 950
DI 10.1130/GES00902.1
PG 87
WC Geosciences, Multidisciplinary
SC Geology
GA 221SM
UT WOS:000324679200009
ER
PT J
AU Maloney, JM
Noble, PJ
Driscoll, NW
Kent, GM
Smith, SB
Schmauder, GC
Babcock, JM
Baskin, RL
Karlin, R
Kell, AM
Seitz, GG
Zimmerman, S
Kleppe, JA
AF Maloney, Jillian M.
Noble, Paula J.
Driscoll, Neal W.
Kent, Graham M.
Smith, Shane B.
Schmauder, Gretchen C.
Babcock, Jeffrey M.
Baskin, Robert L.
Karlin, Robert
Kell, Annie M.
Seitz, Gordon G.
Zimmerman, Susan
Kleppe, John A.
TI Paleoseismic history of the Fallen Leaf segment of the West Tahoe-Dollar
Point fault reconstructed from slide deposits in the Lake Tahoe Basin,
California-Nevada
SO GEOSPHERE
LA English
DT Article
ID SIERRA-NEVADA; RANGE PROVINCE; EASTERN CALIFORNIA; YR BP; DEFORMATION;
EARTHQUAKES; GLACIATION; BOUNDARY; SYSTEM; COAST
AB The West Tahoe-Dollar Point fault (WTDPF) extends along the western margin of the Lake Tahoe Basin (northern Sierra Nevada, western United States) and is characterized as its most hazardous fault. Fallen Leaf Lake, Cascade Lake, and Emerald Bay are three subbasins of the Lake Tahoe Basin, located south of Lake Tahoe, and provide an opportunity to image primary earthquake deformation along the WTDPF and associated landslide deposits. Here we present results from high-resolution seismic Chirp (compressed high intensity radar pulse) surveys in Fallen Leaf Lake and Cascade Lake, multibeam bathymetry coverage of Fallen Leaf Lake, onshore Lidar (light detection and ranging) data for the southern Lake Tahoe Basin, and radiocarbon dates from piston cores in Fallen Leaf Lake and Emerald Bay. Slide deposits imaged beneath Fallen Leaf Lake appear to be synchronous with slides in Lake Tahoe, Emerald Bay, and Cascade Lake. The temporal correlation of slides between multiple basins suggests triggering by earthquakes on the WTDPF system. If this correlation is correct, we postulate a recurrence interval of similar to 3-4 k.y. for large earthquakes on the Fallen Leaf Lake segment of the WTDPF, and the time since the most recent event (similar to 4.5 k.y. ago) exceeds this recurrence time. In addition, Chirp data beneath Cascade Lake image strands of the WTDPF offsetting the lake floor as much as similar to 7.5 m. The Cascade Lake data combined with onshore Lidar allow us to map the WTDPF continuously between Fallen Leaf Lake and Cascade Lake. This improved mapping of the WTDPF reveals the fault geometry and architecture south of Lake Tahoe and improves the geohazard assessment of the region.
C1 [Maloney, Jillian M.; Driscoll, Neal W.; Babcock, Jeffrey M.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA.
[Noble, Paula J.; Smith, Shane B.; Karlin, Robert] Univ Nevada, Dept Geol Sci & Engn, Reno, NV 89557 USA.
[Kent, Graham M.; Schmauder, Gretchen C.; Kell, Annie M.] Univ Nevada, Nevada Seismol Lab, Reno, NV 89557 USA.
[Baskin, Robert L.] US Geol Survey, West Valley City, UT 84119 USA.
[Seitz, Gordon G.] Calif Geol Survey, Menlo Pk, CA 94025 USA.
[Zimmerman, Susan] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA.
[Kleppe, John A.] Univ Nevada, Coll Engn, Reno, NV 89557 USA.
RP Maloney, JM (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, 9500 Gilman Dr, La Jolla, CA 92093 USA.
RI Zimmerman, Susan/A-3351-2013
FU National Science Foundation [OCE-0649410, EAR-127499]; U.S. Geological
Survey National Earthquake Hazards Reduction Program [10HQPA1000,
06HQGR0064, 02HQGR0072]; Exxon-Mobil student grant; Lawrence Livermore
National Laboratory Laboratory Directed Research and Development grant
[09-ERI-003]
FX This research was supported by National Science Foundation grants
OCE-0649410 and EAR-127499, U.S. Geological Survey National Earthquake
Hazards Reduction Program grants 10HQPA1000, 06HQGR0064, and 02HQGR0072,
and an Exxon-Mobil student grant. This manuscript was greatly enhanced
through thoughtful reviews from Cathy Busby, Paul Umhoefer, Mike Oskin,
and Rich Briggs. Radiocarbon ages for the 2010 Fallen Leaf Lake cores
were funded by Lawrence Livermore National Laboratory Laboratory
Directed Research and Development grant 09-ERI-003. We thank Brig
Ebright for his permission to allow us to conduct research on Cascade
Lake and Paul Baker for access to a boat ramp on his property. We are
indebted to Fire Chief Gary Gerren for access to the Fallen Leaf Lake
boat ramp and invasive species boat wash. Generous support from Bill
Craven and access to his boat allowed collection of the 2010 multibeam
survey. We also thank Shane Romsos and the Tahoe Regional Planning
Agency for access to the critical airborne Lidar (light detection and
ranging) data collected in 2010. We thank Anders Noren and Kristina
Brady from LacCore for adding Fallen Leaf Lake to their busy 2010 coring
schedule and for helping us get a high-quality suite of piston cores.
Initial core processing, logging, and sampling of the 2010 Fallen Leaf
Lake cores were conducted at LacCore. We thank Laurel Stratton for her
logistical role in initiating the 2010 coring program and for helping
with initial core processing, and Danny Brothers for conversations
regarding previously collected Chirp (compressed high intensity radar
pulse) profiles and sediment cores.
NR 45
TC 6
Z9 6
U1 0
U2 13
PU GEOLOGICAL SOC AMER, INC
PI BOULDER
PA PO BOX 9140, BOULDER, CO 80301-9140 USA
SN 1553-040X
J9 GEOSPHERE
JI Geosphere
PD AUG
PY 2013
VL 9
IS 4
BP 1065
EP 1090
DI 10.1130/GES00877.1
PG 26
WC Geosciences, Multidisciplinary
SC Geology
GA 221SM
UT WOS:000324679200014
ER
PT J
AU Kamireddy, SR
Li, JB
Abbina, S
Berti, M
Tucker, M
Ji, Y
AF Kamireddy, Srinivas Reddy
Li, Jinbao
Abbina, Srinivas
Berti, Marisol
Tucker, Melvin
Ji, Yun
TI Converting forage sorghum and sunn hemp into biofuels through dilute
acid pretreatment
SO INDUSTRIAL CROPS AND PRODUCTS
LA English
DT Article
DE Acid pretreatment; Sunn hemp; Sorghum Brown-mid rib (BMR); Sorghum Non
Brown-mid rib; Enzymatic hydrolysis; NMR; FTIR
ID ENZYMATIC-HYDROLYSIS; CORN STOVER; LIGNOCELLULOSIC BIOMASS; HERBACEOUS
CROPS; SUGAR PRODUCTION; WHEAT-STRAW; RICE STRAW; ETHANOL; FERMENTATION;
FEEDSTOCK
AB Forage sorghum [Sorghum bicolor (L.) Moench], Brown Mid-Rib (SBMR) and non-BMR (SNBMR) types, and sunn hemp (Crotalaria juncea L) are primarily used as forage and fiber crops, respectively. In this study, these crops were evaluated as feedstocks for biofuels and value added chemicals. This was achieved using dilute acid pretreatment and enzymatic hydrolysis using commercial cellulase enzymes. The highest xylose yield was observed was for SNBMR 95 wt%, followed by SBMR with 91 wt% at combined severity factor (CSF) 1.56 and 1.44. However, for sunn hemp the maximum xylose yield was observed at 72 wt% at CSF 1.48. At harsher pretreatment conditions the xylose yield decreased in all the biomasses due to degradation. In similar fashion, the overall glucan saccharification yield after enzymatic hydrolysis for SNBMR was found to be 90 wt% followed by SBMR 84 wt% at CSF 1.47, and 1.24. For sunn hemp it was observed to be 68 wt% at CSF 2.06. This was mainly due to the high crystallinity index of sunn hemp as compared with that of sorghum. In addition the FTIR and H-1 NMR, C-13 NMR analysis did not prove any major variation in the individual functional groups or chemical structures in these raw and pretreated biomasses. Overall, from the results it can be concluded that SBMR and SNBMR have better potential for biofuel production as compared with sunn hemp biomass. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Kamireddy, Srinivas Reddy; Ji, Yun] Univ N Dakota, Dept Chem Engn, Grand Fork, ND 58202 USA.
[Li, Jinbao] Shaanxi Univ Sci & Technol, Coll Light Ind & Energy Sources, Xian, Shaanxi, Peoples R China.
[Abbina, Srinivas] Univ N Dakota, Dept Chem, Grand Fork, ND 58202 USA.
[Berti, Marisol] N Dakota State Univ, Dept Plant Sci, Fargo, ND 58108 USA.
[Tucker, Melvin] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA.
RP Ji, Y (reprint author), Univ N Dakota, Dept Chem Engn, 241 Centennial Dr, Grand Fork, ND 58202 USA.
EM yun.ji@engr.und.edu
NR 45
TC 10
Z9 10
U1 4
U2 28
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0926-6690
EI 1872-633X
J9 IND CROP PROD
JI Ind. Crop. Prod.
PD AUG
PY 2013
VL 49
BP 598
EP 609
DI 10.1016/j.indcrop.2013.06.018
PG 12
WC Agricultural Engineering; Agronomy
SC Agriculture
GA 220EZ
UT WOS:000324566600082
ER
PT J
AU Buckley, MR
Plehn, T
Takeuchi, M
AF Buckley, Matthew R.
Plehn, Tilman
Takeuchi, Michihisa
TI Buckets of tops
SO JOURNAL OF HIGH ENERGY PHYSICS
LA English
DT Article
DE QCD Phenomenology; Jets
ID HADRON COLLIDERS; MEASURING MASSES; PARTICLE; BOSON; LHC
AB Reconstructing hadronically decaying top quarks is a key challenge at the LHC, affecting a long list of Higgs analyses and new physics searches. We propose a new method of collecting jets in buckets, corresponding to top quarks and initial state radiation. This method is particularly well suited for moderate transverse momenta of the top quark, closing the gap between top taggers and traditional top reconstruction. Applying it to searches for supersymmetric top squarks we illustrate the power of buckets.
C1 [Buckley, Matthew R.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA.
[Plehn, Tilman] Heidelberg Univ, Inst Theoret Phys, Heidelberg, Germany.
[Takeuchi, Michihisa] Kings Coll London, Dept Phys, Theoret Phys & Cosmol Grp, London WC2R 2LS, England.
RP Buckley, MR (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA.
EM mbuckley@fnal.gov; Plehn@uni-heidelberg.de; michihisa.takeuchi@kclac.uk
OI Buckley, Matthew/0000-0003-1109-3460
FU United States Department of Energy [DE-AC02-07CH11359]
FX We would like to thank the Aspen Center of Physics because the idea for
this paper was born on a Snowmass ski lift. Fermilab is operated by
Fermi Research Alliance, LLC, under contract DE-AC02-07CH11359 with the
United States Department of Energy. MRB would like to thank Joseph
Lykken and Maria Spiropulu for useful advice. MT would like to thank
Bobby Acharya for helpful discussions.
NR 61
TC 14
Z9 14
U1 0
U2 1
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1029-8479
J9 J HIGH ENERGY PHYS
JI J. High Energy Phys.
PD AUG
PY 2013
IS 8
AR 086
DI 10.1007/JHEP08(2013)086
PG 22
WC Physics, Particles & Fields
SC Physics
GA 214EL
UT WOS:000324113700086
ER
PT J
AU Campbell, JM
Ellis, RK
Nason, P
Zanderighi, G
AF Campbell, John M.
Ellis, R. Keith
Nason, Paolo
Zanderighi, Giulia
TI W and Z bosons in association with two jets using the POWHEG method
SO JOURNAL OF HIGH ENERGY PHYSICS
LA English
DT Article
DE Monte Carlo Simulations; NLO Computations
AB In this work we present the implementation of generators for W and Z bosons in association with two jets interfaced to parton showers using the POWHEG BOX method. We incorporate matrix elements from the parton-level Monte Carlo program MCFM in the POWHEG-BOX, allowing for a considerable improvement in speed compared to previous implementations. We address certain problems that arise when processes that are singular at the Born level are implemented in a shower framework using either a generation cut or a Born suppression factor to yield weighted events. In such a case, events with very large weights can be generated after the shower through a number of mechanisms. Events with very small transverse momentum at the Born level can develop large transverse momentum either after the hardest emission, after the shower, or after the inclusion of multi-parton interactions. We present a solution to this problem that can be easily implemented in the POWHEG BOX. We also show that a full solution to this problem can only be achieved if the generator maintains physical validity also when the transverse momentum of the emitted partons becomes unresolved. One such scheme is the recently-proposed MiNLO method for the choice of scale and the exponentiation of Sudakov form factors in NLO computations. We present a validation study of our generators, by comparing their output to available LHC data. Furthermore, we suggest an observable that is very sensitive to the modeling of multi-parton interactions, that may be studied in both W and Z production in association with two jets.
C1 [Campbell, John M.; Ellis, R. Keith] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Nason, Paolo] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy.
[Zanderighi, Giulia] Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford OX1 2JD, England.
RP Campbell, JM (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
EM johnmc@fnal.gov; ellis@fnal.gov; paolo.nason@mib.infn.it;
g.zanderighi1@physics.ox.ac.uk
OI Nason, Paolo/0000-0001-9250-246X
NR 54
TC 11
Z9 11
U1 0
U2 4
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1029-8479
J9 J HIGH ENERGY PHYS
JI J. High Energy Phys.
PD AUG
PY 2013
IS 8
AR 005
DI 10.1007/JHEP08(2013)005
PG 33
WC Physics, Particles & Fields
SC Physics
GA 214EL
UT WOS:000324113700005
ER
PT J
AU Carena, M
Gori, S
Shah, NR
Wagner, CEM
Wang, LT
AF Carena, Marcela
Gori, Stefania
Shah, Nausheen R.
Wagner, Carlos E. M.
Wang, Lian-Tao
TI Light stops, light staus and the 125 GeV Higgs
SO JOURNAL OF HIGH ENERGY PHYSICS
LA English
DT Article
DE Supersymmetry Phenomenology
ID SUPERSYMMETRIC STANDARD MODEL; EXPLICIT CP VIOLATION; ROOT-S=7 TEV;
E(+)E(-) COLLISIONS; PP COLLISIONS; TOP-QUARK; COMPUTATIONAL TOOL;
SCALAR LEPTONS; ATLAS DETECTOR; CROSS-SECTION
AB The ATLAS and CMS experiments have recently announced the discovery of a Higgs-like resonance with mass close to 125 GeV. Overall, the data is consistent with a Standard Model (SM)-like Higgs boson. Such a particle may arise in the minimal supersymmetric extension of the SM with average stop masses of the order of the TeV scale and a sizable stop mixing parameter. In this article we discuss properties of the SM-like Higgs production and decay rates induced by the possible presence of light staus and light stops. Light staus can affect the decay rate of the Higgs into di-photons and, in the case of sizable left-right mixing, induce an enhancement in this production channel up to similar to 50% of the Standard Model rate. Light stops may induce sizable modifications of the Higgs gluon fusion production rate and correlated modifications to the Higgs diphoton decay. Departures from SM values of the bottom-quark and tau-lepton couplings to the Higgs can be obtained due to Higgs mixing effects triggered by light third generation scalar superpartners. We describe the phenomenological implications of light staus on searches for light stops and non-standard Higgs bosons. Finally, we discuss the current status of the search for light staus produced in association with sneutrinos, in final states containing a W gauge boson and a pair of tau s.
C1 [Carena, Marcela] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Carena, Marcela; Gori, Stefania; Wagner, Carlos E. M.; Wang, Lian-Tao] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA.
[Carena, Marcela; Wagner, Carlos E. M.; Wang, Lian-Tao] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA.
[Gori, Stefania; Wagner, Carlos E. M.] Argonne Natl Lab, Div High Energy Phys, Lemont, IL 60439 USA.
[Shah, Nausheen R.] Univ Michigan, Dept Phys, Michigan Ctr Theoret Phys, Ann Arbor, MI 48109 USA.
RP Carena, M (reprint author), Fermilab Natl Accelerator Lab, POB 500,Kirk Rd, Batavia, IL 60510 USA.
EM carena@fnal.gov; goris@uchicago.edu; naushah@umich.edu;
cwagner@hep.anl.gov; liantaow@uchicago.edu
FU NSF [PHY-0756966]; DOE Early Career Award [de-sc0003930]; U.S.
Department of Energy [DE-AC02-07CH11359, DE-AC02-06CH11357]; DoE
[DE-SC0007859]
FX We would like to thank Felix Yu for useful discussions. SG thanks the
Galileo Galilei Institute for Theoretical Physics for its hospitality
during some part of this work. L.T.W. is supported by the NSF under
grant PHY-0756966 and the DOE Early Career Award under grant
de-sc0003930. Fermilab is operated by Fermi Research Alliance, LLC under
Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. Work
at ANL is supported in part by the U.S. Department of Energy under
Contract No. DE-AC02-06CH11357. N.R.S is supported by the DoE grant No.
DE-SC0007859. We would also like to thank the Aspen Center for Physics
and the KITP, Santa Barbara, where part of the work has been done.
NR 141
TC 21
Z9 21
U1 0
U2 4
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1029-8479
J9 J HIGH ENERGY PHYS
JI J. High Energy Phys.
PD AUG
PY 2013
IS 8
AR 087
DI 10.1007/JHEP08(2013)087
PG 32
WC Physics, Particles & Fields
SC Physics
GA 214EL
UT WOS:000324113700087
ER
PT J
AU Zhou, R
Behunin, RO
Lin, SY
Hu, BL
AF Zhou, Rong
Behunin, Ryan O.
Lin, Shih-Yuin
Hu, B. L.
TI Boundary effects on quantum entanglement and its dynamics in a
detector-field system
SO JOURNAL OF HIGH ENERGY PHYSICS
LA English
DT Article
DE Boundary Quantum Field Theory; Quantum Dissipative Systems
ID BROWNIAN-MOTION; BLACK-HOLES; DISSIPATION; TOPOLOGY
AB In this paper we analyze an exactly solvable model consisting of an inertial Unruh-DeWitt detector which interacts linearly with a massless quantum field in Minkowski spacetime with a perfectly reflecting flat plane boundary. Firstly a set of coupled equations for the detector's and the field's Heisenberg operators are derived. Then we introduce the linear entropy as a measure of entanglement between the detector and the quantum field under mirror reflection, and solve the early-time detector-field entanglement dynamics. After coarse-graining the field, the dynamics of the detector's internal degree of freedom is described by a quantum Langevin equation, where the dissipation and noise kernels respectively correspond to the retarded Green's functions and Hadamard elementary functions of the free quantum field in a half space. At late times when the combined system is in a stationary state, we obtain exact expressions for the detector's covariance matrix and show that the detector-field entanglement decreases for smaller separation between the detector and the mirror. We explain the behavior of detector-field entanglement qualitatively with the help of a detector's mirror image, compare them with the case of two real detectors and explain the differences.
C1 [Zhou, Rong; Hu, B. L.] Univ Maryland, Joint Quantum Inst, College Pk, MD 20742 USA.
[Zhou, Rong; Hu, B. L.] Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA.
[Behunin, Ryan O.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.
[Behunin, Ryan O.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Lin, Shih-Yuin] Natl Changhua Univ Educ, Dept Phys, Changhua 50007, Taiwan.
RP Zhou, R (reprint author), Univ Maryland, Joint Quantum Inst, College Pk, MD 20742 USA.
EM zhour@umd.edu; rbehunin@lanl.gov; sylin@cc.ncue.edu.tw; blhu@umd.edu
FU NSF [PHY-0801368]; Nation Science Council of Taiwan [NSC
99-2112-M-018-001-MY3]; National Center for Theoretical Sciences,
Taiwan; NSF-NSC U.S.-East Asia Ph.D student grant
FX This work is supported in part by the NSF Grant No. PHY-0801368 and the
Nation Science Council of Taiwan under the Grant No. NSC
99-2112-M-018-001-MY3 and in part by the National Center for Theoretical
Sciences, Taiwan. ROB is aided by an NSF-NSC U.S.-East Asia Ph.D student
grant award to spend a summer in Taiwan in 2010.
NR 52
TC 4
Z9 4
U1 1
U2 5
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1029-8479
J9 J HIGH ENERGY PHYS
JI J. High Energy Phys.
PD AUG
PY 2013
IS 8
AR 040
DI 10.1007/JHEP08(2013)040
PG 23
WC Physics, Particles & Fields
SC Physics
GA 214EL
UT WOS:000324113700040
ER
PT J
AU Guyader, A
Hengartner, N
AF Guyader, Arnaud
Hengartner, Nick
TI On the Mutual Nearest Neighbors Estimate in Regression
SO JOURNAL OF MACHINE LEARNING RESEARCH
LA English
DT Article
DE nonparametric estimation; nearest neighbor methods; mathematical
statistics
ID NONPARAMETRIC REGRESSION; CONVERGENCE; RATES
AB Motivated by promising experimental results, this paper investigates the theoretical properties of a recently proposed nonparametric estimator, called the Mutual Nearest Neighbors rule, which estimates the regression function m(x) = E[Y vertical bar X = x] as follows: first identify the k nearest neighbors of x in the sample D-n, then keep only those for which x is itself one of the k nearest neighbors, and finally take the average over the corresponding response variables. We prove that this estimator is consistent and that its rate of convergence is optimal. Since the estimate with the optimal rate of convergence depends on the unknown distribution of the observations, we also present adaptation results by data-splitting.
C1 [Guyader, Arnaud] Univ Rennes 2, IRMAR, F-35043 Rennes, France.
[Guyader, Arnaud] Univ Rennes 2, INRIA Rennes, F-35043 Rennes, France.
[Hengartner, Nick] Los Alamos Natl Lab, Informat Sci Grp, Los Alamos, NM 87545 USA.
RP Guyader, A (reprint author), Univ Rennes 2, IRMAR, Campus Villejean,Pl Recteur Henri Le Moal,CS 2430, F-35043 Rennes, France.
EM ARNAUD.GUYADER@UHB.FR; NICKH@LANL.GOV
NR 26
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U1 3
U2 3
PU MICROTOME PUBL
PI BROOKLINE
PA 31 GIBBS ST, BROOKLINE, MA 02446 USA
SN 1532-4435
J9 J MACH LEARN RES
JI J. Mach. Learn. Res.
PD AUG
PY 2013
VL 14
BP 2361
EP 2376
PG 16
WC Automation & Control Systems; Computer Science, Artificial Intelligence
SC Automation & Control Systems; Computer Science
GA 223JD
UT WOS:000324799600007
ER
PT J
AU Huggel, C
Stone, D
Auffhammer, M
Hansen, G
AF Huggel, Christian
Stone, Daithi
Auffhammer, Maximilian
Hansen, Gerrit
TI Loss and damage attribution
SO NATURE CLIMATE CHANGE
LA English
DT Editorial Material
ID CLIMATE-CHANGE; DISASTER LOSSES
C1 [Huggel, Christian] Univ Zurich, Dept Geog, CH-8057 Zurich, Switzerland.
[Stone, Daithi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Auffhammer, Maximilian] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Auffhammer, Maximilian] Natl Bur Econ Res, Cambridge, MA 02138 USA.
[Hansen, Gerrit] Potsdam Inst Climate Impact Res PIK, D-14412 Potsdam, Germany.
RP Huggel, C (reprint author), Univ Zurich, Dept Geog, Winterthurerstr 190, CH-8057 Zurich, Switzerland.
EM christian.huggel@geo.uzh.ch
NR 17
TC 26
Z9 28
U1 2
U2 13
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 1758-678X
J9 NAT CLIM CHANGE
JI Nat. Clim. Chang.
PD AUG
PY 2013
VL 3
IS 8
BP 694
EP 696
PG 4
WC Environmental Sciences; Environmental Studies; Meteorology & Atmospheric
Sciences
SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences
GA 219EB
UT WOS:000324487400006
ER
PT J
AU Morozov, D
Weber, GH
AF Morozov, Dmitriy
Weber, Gunther H.
TI Distributed Merge Trees
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE topological data analysis; feature extraction; merge tree computation;
parallelization; hybrid parallelization approaches
ID COMPUTATION
AB Improved simulations and sensors are producing datasets whose increasing complexity exhausts our ability to visualize and comprehend them directly. To cope with this problem, we can detect and extract significant features in the data and use them as the basis for subsequent analysis. Topological methods are valuable in this context because they provide robust and general feature definitions.
As the growth of serial computational power has stalled, data analysis is becoming increasingly dependent on massively parallel machines. To satisfy the computational demand created by complex datasets, algorithms need to effectively utilize these computer architectures. The main strength of topological methods, their emphasis on global information, turns into an obstacle during parallelization.
We present two approaches to alleviate this problem. We develop a distributed representation of the merge tree that avoids computing the global tree on a single processor and lets us parallelize subsequent queries. To account for the increasing number of cores per processor, we develop a new data structure that lets us take advantage of multiple shared-memory cores to parallelize the work on a single node. Finally, we present experiments that illustrate the strengths of our approach as well as help identify future challenges.
C1 [Morozov, Dmitriy; Weber, Gunther H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA.
[Weber, Gunther H.] Univ Calif Davis, Dept Comp Sci, Davis, CA 95616 USA.
RP Morozov, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, 1 Cyclotron Rd,MS 50F-1650, Berkeley, CA 94720 USA.
EM dmitriy@mrzv.org; GHWeber@lbl.gov
OI Weber, Gunther/0000-0002-1794-1398
FU Office of Science, Advanced Scientific Computing Research, of the U.S.
Department of Energy [DE-AC02-05CH11231]
FX This work was supported by the Director, Office of Science, Advanced
Scientific Computing Research, of the U.S. Department of Energy under
Contract No. DE-AC02-05CH11231 through the grant "Topology-based
Visualization and Analysis of High-dimensional Data and Time-varying
Data at the Extreme Scale," program manager Lucy Nowell, and by the use
resources of the National Energy Research Scientific Computing Center
(NERSC). The authors wish to thank Hank Childs, Terry Ligocki, Zarija
Lukic, Peter Nugent, Casey Stark, and Matthew Turk for their
encouragement and help.
NR 23
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PU ASSOC COMPUTING MACHINERY
PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
EI 1558-1160
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2013
VL 48
IS 8
BP 93
EP 102
DI 10.1145/2517327.2442526
PG 10
WC Computer Science, Software Engineering
SC Computer Science
GA 214TO
UT WOS:000324158900009
ER
PT J
AU Friedley, A
Hoefler, T
Bronevetsky, G
Lumsdaine, A
Ma, CC
AF Friedley, Andrew
Hoefler, Torsten
Bronevetsky, Greg
Lumsdaine, Andrew
Ma, Ching-Chen
TI Ownership Passing: Efficient Distributed Memory Programming on
Multi-core Systems
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE Ownership Passing; Distributed Memory; Shared Memory; Message Passing;
Multi-core
AB The number of cores in multi- and many-core high-performance processors is steadily increasing. MPI, the de-facto standard for programming high-performance computing systems offers a distributed memory programming model. MPI's semantics force a copy from one process' send buffer to another process' receive buffer. This makes it difficult to achieve the same performance on modern hardware than shared memory programs which are arguably harder to maintain and debug. We propose generalizing MPI's communication model to include ownership passing, which make it possible to fully leverage the shared memory hardware of multi-and many-core CPUs to stream communicated data concurrently with the receiver's computations on it. The benefits and simplicity of message passing are retained by extending MPI with calls to send (pass) ownership of memory regions, instead of their contents, between processes. Ownership passing is achieved with a hybrid MPI implementation that runs MPI processes as threads and is mostly transparent to the user. We propose an API and a static analysis technique to transform legacy MPI codes automatically and transparently to the programmer, demonstrating that this scheme is easy to use in practice. Using the ownership passing technique, we see up to 51% communication speedups over a standard message passing implementation on state-of-the art multicore systems. Our analysis and interface will lay the groundwork for future development of MPI-aware optimizing compilers and multi-core specific optimizations, which will be key for success in current and next-generation computing platforms.
C1 [Friedley, Andrew; Lumsdaine, Andrew] Indiana Univ, Bloomington, IN 47405 USA.
[Hoefler, Torsten] ETH, Zurich, Switzerland.
[Bronevetsky, Greg] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Ma, Ching-Chen] Rose Hulman Inst Technol, Terre Haute, IN 47803 USA.
RP Friedley, A (reprint author), Indiana Univ, Bloomington, IN 47405 USA.
EM afriedle@indiana.edu; htor@inf.ethz.ch; bronevetsky@llnl.gov;
lums@indiana.edu; mac@rose-hulman.edu
FU Department of Energy X-Stack program; Early Career award program; U.S.
Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]
FX This work was supported in part by the Department of Energy X-Stack
program and the Early Career award program. It was partially performed
under the auspices of the U.S. Department of Energy by Lawrence
Livermore National Laboratory under Contract DE-AC52-07NA27344.
(LLNL-CONF-609538)
NR 25
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U1 0
U2 4
PU ASSOC COMPUTING MACHINERY
PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
EI 1558-1160
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2013
VL 48
IS 8
BP 177
EP 186
DI 10.1145/2517327.2442534
PG 10
WC Computer Science, Software Engineering
SC Computer Science
GA 214TO
UT WOS:000324158900017
ER
PT J
AU Park, CS
Sen, K
Iancu, C
AF Park, Chang-Seo
Sen, Koushik
Iancu, Costin
TI Scaling Data Race Detection for Partitioned Global Address Space
Programs
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE scalable data race detection; hierarchical sampling
C1 [Park, Chang-Seo; Sen, Koushik] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Iancu, Costin] Lawrence Berkeley Natl Lab, Berkeley, CA USA.
RP Park, CS (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA.
EM parkcs@eecs.berkeley.edu; ksen@eecs.berkeley.edu; cciancu@lbl.gov
NR 5
TC 0
Z9 0
U1 0
U2 1
PU ASSOC COMPUTING MACHINERY
PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2013
VL 48
IS 8
BP 305
EP 306
DI 10.1145/2517327.2442557
PG 2
WC Computer Science, Software Engineering
SC Computer Science
GA 214TO
UT WOS:000324158900039
ER
PT J
AU Wozniak, JM
Armstrong, TG
Wilde, M
Katz, DS
Lusk, E
Foster, IT
AF Wozniak, Justin M.
Armstrong, Timothy G.
Wilde, Michael
Katz, Daniel S.
Lusk, Ewing
Foster, Ian T.
TI Swift/T: Scalable Data Flow Programming for Many-Task Applications
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE Languages; MPI; ADLB; Swift; Turbine; exascale; concurrency; dataflow;
futures
AB Swift/T, a novel programming language implementation for highly scalable data flow programs, is presented.
C1 [Wozniak, Justin M.; Wilde, Michael; Katz, Daniel S.; Lusk, Ewing; Foster, Ian T.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Wozniak, Justin M.; Armstrong, Timothy G.; Wilde, Michael; Katz, Daniel S.; Foster, Ian T.] Univ Chicago, Chicago, IL 60637 USA.
RP Wozniak, JM (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA.
EM wozniak@mcs.anl.gov; tga@uchicago.edu; wilde@mcs.anl.gov;
d.katz@ieee.org; lusk@mcs.anl.gov; foster@mcs.anl.gov
FU U.S. DOE Office of Science [DE-AC02-06CH11357, FWP-57810]; National
Science Foundation
FX This research is supported by the U.S. DOE Office of Science under
contract DE-AC02-06CH11357, FWP-57810. Computing resources were provided
by the Argonne Leadership Computing Facility. This material was based on
work (by DSK) supported by the National Science Foundation, while
working at the Foundation. Any opinion, finding, and conclusions or
recommendations expressed in this material are those of the authors and
do not necessarily reflect the views of the National Science Foundation.
NR 7
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PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2013
VL 48
IS 8
BP 309
EP 310
DI 10.1145/2517327.2442559
PG 2
WC Computer Science, Software Engineering
SC Computer Science
GA 214TO
UT WOS:000324158900041
ER
PT J
AU Jiang, S
Ding, XN
Xu, YH
Davis, K
AF Jiang, Song
Ding, Xiaoning
Xu, Yuehai
Davis, Kei
TI A Prefetching Scheme Exploiting both Data Layout and Access History on
Disk
SO ACM TRANSACTIONS ON STORAGE
LA English
DT Article
DE Algorithms; Performance; Design; Experimentation; Prefetching; spatial
locality; hard disk; buffer cache
AB Prefetching is an important technique for improving effective hard disk performance. A prefetcher seeks to accurately predict which data will be requested and load it ahead of the arrival of the corresponding requests. Current disk prefetch policies in major operating systems track access patterns at the level of file abstraction. While this is useful for exploiting application-level access patterns, for two reasons file-level prefetching cannot realize the full performance improvements achievable by prefetching. First, certain prefetch opportunities can only be detected by knowing the data layout on disk, such as the contiguous layout of file metadata or data from multiple files. Second, nonsequential access of disk data (requiring disk head movement) is much slower than sequential access, and the performance penalty for mis-prefetching a randomly located block, relative to that of a sequential block, is correspondingly greater.
To overcome the inherent limitations of prefetching at logical file level, we propose to perform prefetching directly at the level of disk layout, and in a portable way. Our technique, called DiskSeen, is intended to be supplementary to, and to work synergistically with, any present file-level prefetch policies. DiskSeen tracks the locations and access times of disk blocks and, based on analysis of their temporal and spatial relationships, seeks to improve the sequentiality of disk accesses and overall prefetching performance. It also implements a mechanism to minimize mis-prefetching, on a per-application basis, to mitigate the corresponding performance penalty.
Our implementation of the DiskSeen scheme in the Linux 2.6 kernel shows that it can significantly improve the effectiveness of prefetching, reducing execution times by 20%-60% for microbenchmarks and real applications such as grep, CVS, and TPC-H. Even for workloads specifically designed to expose its weaknesses, DiskSeen incurs only minor performance loss.
C1 [Jiang, Song; Xu, Yuehai] Wayne State Univ, Dept Elect & Comp Engn, Detroit, MI 48202 USA.
[Ding, Xiaoning] New Jersey Inst Technol, Dept Comp Sci, Newark, NJ 07102 USA.
[Davis, Kei] Los Alamos Natl Lab, CCS Div, Los Alamos, NM 87545 USA.
RP Jiang, S (reprint author), Wayne State Univ, Dept Elect & Comp Engn, Detroit, MI 48202 USA.
EM sjiang@wayne.edu
RI Ding, Xiaoning/C-9933-2014
OI Ding, Xiaoning/0000-0002-9947-0437
FU National Science Foundation [CCF-0702500, CCF-0845711, CNS-1117772,
CNS-1217948]
FX This research was supported in part by National Science Foundation
grants CCF-0702500, CCF-0845711, CAREER CCF-0845711, CNS-1117772, and
CNS-1217948.
NR 34
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U1 0
U2 7
PU ASSOC COMPUTING MACHINERY
PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 1553-3077
J9 ACM T STORAGE
JI ACM Trans. Storage
PD AUG
PY 2013
VL 9
IS 3
AR 10
DI 10.1145/2508010
PG 23
WC Computer Science, Hardware & Architecture; Computer Science, Software
Engineering
SC Computer Science
GA 216XX
UT WOS:000324321200004
ER
PT J
AU Tello, C
Villela, T
Torres, S
Bersanelli, M
Smoot, GF
Ferreira, IS
Cingoz, A
Lamb, J
Barbosa, D
Perez-Becker, D
Ricciardi, S
Currivan, JA
Platania, P
Maino, D
AF Tello, C.
Villela, T.
Torres, S.
Bersanelli, M.
Smoot, G. F.
Ferreira, I. S.
Cingoz, A.
Lamb, J.
Barbosa, D.
Perez-Becker, D.
Ricciardi, S.
Currivan, J. A.
Platania, P.
Maino, D.
TI The 2.3 GHz continuum survey of the GEM project
SO ASTRONOMY & ASTROPHYSICS
LA English
DT Article
DE surveys; Galaxy: structure; radio continuum: general; radio continuum:
ISM
ID MICROWAVE-ANISOTROPY-PROBE; GALACTIC SYNCHROTRON EMISSION; ATACAMA
COSMOLOGY TELESCOPE; BACKGROUND POWER SPECTRUM; SOUTH-POLE TELESCOPE; 11
CM WAVELENGTH; COMPONENT SEPARATION; FOREGROUND EMISSION; WMAP
OBSERVATIONS; RADIO-EMISSION
AB Context. Determining the spectral and spatial characteristics of the radio continuum of our Galaxy is an experimentally challenging endeavour for improving our understanding of the astrophysics of the interstellar medium. This knowledge has also become of paramount significance for cosmology, since Galactic emission is the main source of astrophysical contamination in measurements of the cosmic microwave background (CMB) radiation on large angular scales.
Aims. We present a partial-sky survey of the radio continuum at 2.3 GHz within the scope of the Galactic Emission Mapping (GEM) project, an observational program conceived and developed to reveal the large-scale properties of Galactic synchrotron radiation through a set of self-consistent surveys of the radio continuum between 408 MHz and 10 GHz.
Methods. The GEM experiment uses a portable and double-shielded 5.5-m radiotelescope in altazimuthal configuration to map 60-degree-wide declination bands from different observational sites by circularly scanning the sky at zenithal angles of 30 degrees from a constantly rotating platform. The observations were accomplished with a total power receiver, whose front-end high electron mobility transistor (HEMT) amplifier was matched directly to a cylindrical horn at the prime focus of the parabolic reflector. The Moon was used to calibrate the antenna temperature scale and the preparation of the map required direct subtraction and destriping algorithms to remove ground contamination as the most significant source of systematic error.
Results. We used 484 h of total intensity observations from two locations in Colombia and Brazil to yield 66% sky coverage from delta = -51 degrees.73 to delta = +34 degrees.78. The observations in Colombia were obtained with a horizontal HPBW of 2 degrees.30 +/- 0 degrees.13 and a vertical HPBW of 1 degrees.92 +/- 0 degrees.18. The pointing accuracy was 6 '.84 and the RMS sensitivity was 11.42 mK. The observations in Brazil were obtained with a horizontal HPBW of 2 degrees.31 +/- 0 degrees.03 and a vertical HPBW of 1 degrees.82 +/- 0 degrees.12. The pointing accuracy was 5 '.26 and the RMS sensitivity was 8.24 mK. The zero-level uncertainty of the combined survey is 103 mK with a temperature scale error of 5% after direct correlation with the Rhodes/HartRAO survey at 2326 MHz on a T-T plot.
Conclusions. The sky brightness distribution into regions of low and high emission in the GEM survey is consistent with the appearance of a transition region as seen in the Haslam 408 MHz and WMAP K-band surveys. Preliminary results also show that the temperature spectral index between 408 MHz and the 2.3 GHz band of the GEM survey has a weak spatial correlation with these regions; but it steepens significantly from high to low emission regions with respect to the WMAP K-band survey.
C1 [Tello, C.; Villela, T.] Inst Nacl Pesquisas Espaciais, Div Astrofis, BR-12201970 Sao Jose Dos Campos, SP, Brazil.
[Torres, S.] Ctr Int Fis, Bogota, Colombia.
[Bersanelli, M.; Maino, D.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy.
[Smoot, G. F.; Ricciardi, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Smoot, G. F.; Cingoz, A.; Perez-Becker, D.; Currivan, J. A.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Ferreira, I. S.] Univ Brasilia, Inst Fis, BR-70919970 Brasilia, DF, Brazil.
[Lamb, J.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA.
[Barbosa, D.] Inst Telecomunicacoes, Grp RadioAstron, Aveiro, Portugal.
[Perez-Becker, D.] Univ Nacl Autonoma Mexico, Fac Ciencias, Dept Fis, Mexico City 04510, DF, Mexico.
[Ricciardi, S.] Osserv Astron Padova, INAF, I-35122 Padua, Italy.
[Platania, P.] CNR ENEA EURATOM Assoc, Ist Fis Plasma, I-20125 Milan, Italy.
RP Tello, C (reprint author), Inst Nacl Pesquisas Espaciais, Div Astrofis, CP 515, BR-12201970 Sao Jose Dos Campos, SP, Brazil.
OI Ricciardi, Sara/0000-0002-3807-4043
FU FAPESP in Brazil [97/03861-2, 97/06794-4, 00/06770-2]; CNPq
[305219/2004-9, 303637/2007-2, 484378/2007-4, 308113/2010-1,
506269/2010-8]; NATO [CRG960175]; Colciencias funding of the GEM project
in Colombia [2228-05-103-96, 221-96]; FCT - Portugal; POCI through an
SFRH/BPD; POCI [POCTI/FNU/42263/2001, POCI/CTE-AST/57209/2004]
FX We are enormously grateful to several generations of students and
technicians at LBNL and INPE, for whom GEM was a rich learning
experience. We are particularly indebted to John Gibson, Alexandre M. R.
Alves, Luiz Arantes, and Luiz Antonio Reitano for their dedicated
commitment; to Jon Aymon, Tony Banday, Justin Jonas, and Andrew Jaffe
for helpful advice and to SLB/INPE for logistics support in Cachoeira
Paulista. The destriped version of the Rhodes/HartRAO map was reproduced
courtesy of Tony Banday. The GEM project in Brazil was supported by
FAPESP through grants 97/03861-2, 97/06794-4 and 00/06770-2. T. V.
acknowledges support from CNPq through grants 305219/2004-9,
303637/2007-2, 484378/2007-4, 308113/2010-1, 506269/2010-8. M. B.
acknowledges the support of the NATO Collaborative Grant CRG960175. S.
T. acknowledges the support provided by Colciencias funding of the GEM
project in Colombia through project 2228-05-103-96, contract No. 221-96.
D. B. acknowledges support from FCT - Portugal and POCI through an
SFRH/BPD grant and project grants POCTI/FNU/42263/2001 and
POCI/CTE-AST/57209/2004. Last, but not least, we would like to
acknowledge the referee's comments, without which the significance of
this article would not have been fully appreciated.
NR 129
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PU EDP SCIENCES S A
PI LES ULIS CEDEX A
PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A,
FRANCE
SN 0004-6361
EI 1432-0746
J9 ASTRON ASTROPHYS
JI Astron. Astrophys.
PD AUG
PY 2013
VL 556
AR A1
DI 10.1051/0004-6361/20079306
PG 20
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 211GH
UT WOS:000323893500001
ER
PT J
AU West, TO
Brown, ME
Duren, RM
Ogle, SM
Moss, RH
AF West, Tristram O.
Brown, Molly E.
Duren, Riley M.
Ogle, Stephen M.
Moss, Richard H.
TI Definition, capabilities and components of a terrestrial carbon
monitoring system
SO CARBON MANAGEMENT
LA English
DT Article
ID UNITED-STATES; WOOD HARVEST; LAND-USE; INVENTORY; CLIMATE; UNCERTAINTY;
RESOLUTION; FLUXES; MODEL; CYCLE
AB Research efforts for effectively and consistently monitoring terrestrial carbon are increasing in number. As such, there is a need to define carbon monitoring and how it relates to carbon cycle science and carbon management. There is also a need to identify capabilities of a carbon monitoring system and the system components needed to develop the capabilities. Capabilities that enable the effective application of a carbon monitoring system for monitoring and management purposes may include: reconciling carbon stocks and fluxes, developing consistency across spatial and temporal scales, tracking horizontal movement of carbon, attribution of emissions to originating sources, cross-sectoral accounting, uncertainty quantification, redundancy and policy relevance. Focused research is needed to integrate these capabilities for sustained estimates of carbon stocks and fluxes. Additionally, if monitoring is intended to inform management decisions, management priorities should be considered prior to development of a monitoring system.
C1 [West, Tristram O.; Moss, Richard H.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA.
[Brown, Molly E.] NASA, Goddard Space Flight Ctr, Biospher Sci Lab, Greenbelt, MD 20771 USA.
[Duren, Riley M.] NASA, Jet Prop Lab, Pasadena, CA 91109 USA.
[Duren, Riley M.] CALTECH, Pasadena, CA 91109 USA.
[Ogle, Stephen M.] Colorado State Univ, Nat Resource Ecol Lab, Ft Collins, CO 80523 USA.
RP West, TO (reprint author), Pacific NW Natl Lab, Joint Global Change Res Inst, 5825 Univ Res Court, College Pk, MD 20740 USA.
EM tristram.west@pnnl.gov
RI West, Tristram/C-5699-2013; Brown, Molly/M-5146-2013; Brown,
Molly/E-2724-2010;
OI West, Tristram/0000-0001-7859-0125; Brown, Molly/0000-0001-7384-3314;
Brown, Molly/0000-0001-7384-3314; Ogle, Stephen/0000-0003-1899-7446;
Moss, Richard/0000-0001-5005-0063
FU National Aeronautics and Space Administration under Carbon Monitoring
System Phase 2 Project [NNH12AU35I]; Jet Propulsion Laboratory, a
division of the California Institute of Technology
FX Support for TO West is from the National Aeronautics and Space
Administration under Carbon Monitoring System Phase 2 Project
#NNH12AU35I. Support for Rill Duren is from the Jet Propulsion
Laboratory, a division of the California Institute of Technology under
contract to the National Aeronautics and Space Administration. The
authors have no other relevant affiliations or financial involvement
with any organization or entity with a financial interest in or
financial conflict with the subject matter or materials discussed in the
manuscript apart from those disclosed.
NR 59
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U1 1
U2 17
PU FUTURE SCI LTD
PI LONDON
PA UNITED HOUSE, 2 ALBERT PL, LONDON, N3 1QB, ENGLAND
SN 1758-3004
J9 CARBON MANAG
JI Carbon Manag.
PD AUG
PY 2013
VL 4
IS 4
BP 413
EP 422
DI 10.4155/CMT.13.36
PG 10
WC Environmental Sciences; Environmental Studies
SC Environmental Sciences & Ecology
GA 198RR
UT WOS:000322940500015
ER
PT J
AU Aad, G
Abajyan, T
Abbott, B
Abdallah, J
Khalek, SA
Abdelalim, AA
Abdinov, O
Aben, R
Abi, B
Abolins, M
AbouZeid, OS
Abramowicz, H
Abreu, H
Acerbia, E
Acharya, BS
Adamczyk, L
Adams, DL
Addy, TN
Adelman, J
Adomeit, S
Adragna, P
Adye, T
Aefsky, S
Aguilar-Saavedra, JA
Agustoni, M
Aharrouche, M
Ahlen, SP
Ahles, F
Ahmad, A
Ahsan, M
Aielli, G
Akdogan, T
Akesson, TP
Akimoto, G
Akimov, AV
Alam, MS
Alam, MA
Albert, J
Albrand, S
Aleksa, M
Aleksandrov, IN
Alessandria, F
Alexa, C
Alexander, G
Alexandre, G
Alexopoulos, T
Alhroob, M
Aliev, M
Alimonti, G
Alison, J
Allbrooke, BMM
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CA ATLAS Collaboration
TI Improved luminosity determination in pp collisions at root s=7 TeV using
the ATLAS detector at the LHC
SO EUROPEAN PHYSICAL JOURNAL C
LA English
DT Article
ID INTERACTION-POINT; SENSORS; BEAM
AB The luminosity calibration for the ATLAS detector at the LHC during pp collisions at root s = 7 TeV in 2010 and 2011 is presented. Evaluation of the luminosity scale is performed using several luminosity-sensitive detectors, and comparisons are made of the long-term stability and accuracy of this calibration applied to the pp collisions at root s = 7 TeV. A luminosity uncertainty of delta L/L = +/- 3.5 % is obtained for the 47 pb(-1) of data delivered to ATLAS in 2010, and an uncertainty of delta L/L = +/- 1.8 % is obtained for the 5.5 fb(-1) delivered in 2011.
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[Abdallah, J.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Nadal, J.; Osuna, C.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain.
[Abdallah, J.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Nadal, J.; Osuna, C.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] ICREA, Barcelona, Spain.
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[do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil.
[Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil.
[Adams, D. L.; Assamagan, K.; Baker, M. D.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Debbe, R.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M-A.; Poblaguev, A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rahm, D.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Sircar, A.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
[Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C-M.; Dinuta, F.; Dita, P.; Dita, S.; Micu, L.; Olariu, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania.
[Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania.
West Univ Timisoara, Timisoara, Romania.
[Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina.
[Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England.
[Gillberg, D.; Koffas, T.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada.
[Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellina, F.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Byszewski, M.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Cerri, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Di Micco, B.; Dittus, F.; Dobinson, R.; Dobos, D.; Dobson, E.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Dunford, M.; Dydak, F.; Ellis, N.; Elsing, M.; Fabre, C.; Farthouat, P.; Fassnacht, P.; Francis, D.; Franz, S.; Froeschl, R.; Froidevaux, D.; Torregrosa, E. Fullana; Gabaldon, C.; Garelli, N.; Garonne, V.; Gianotti, F.; Gibson, S. M.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hahn, F.; Haider, S.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Inigo-Golfin, J.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Joram, C.; Jungst, R. M.; Kaneda, M.; Kaplon, J.; Kerschen, N.; Klioutchnikova, T.; Koeneke, K.; Lamanna, M.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Meyer, T. C.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Torchiani, I.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zajacova, Z.; Zwalinski, L.] CERN, Geneva, Switzerland.
[Anderson, K. J.; Boveia, A.; Canelli, F.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA.
[Diaz, M. A.; Pino, S. A. Olivares; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile.
[Brooks, W. K.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile.
[Bai, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China.
[Han, L.; Jiang, Y.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wang, H.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China.
[Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China.
[Feng, C.; Ge, P.; He, M.; Li, H.; Meng, Z.; Miao, J.; Zhan, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China.
Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China.
[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France.
[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France.
[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France.
[Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA.
[Alonso, A.; Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark.
[Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Arcavacata Di Rende, Italy.
[Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy.
[Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland.
[Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland.
[Yagci, K. Dindar; Firan, A.; Hadavand, H. K.; Hoffman, J.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA.
[Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA.
[Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Husemann, U.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Hamburg, Germany.
[Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Husemann, U.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany.
[Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany.
[Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany.
[Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Kotwal, A.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA.
[Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland.
[Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy.
[Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Glatzer, J.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kollefrath, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Lumb, D.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Wiik-Fuchs, L. A. M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany.
[Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland.
[Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy.
[Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy.
[Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia.
[Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia.
[Duren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany.
[Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland.
[Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Hamer, M.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany.
[Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France.
[Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] CNRS IN2P3, Grenoble, France.
[Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France.
[Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA.
[da Costa, J. Barreiro Guimaraes; Belloni, A.; Brandenburg, G. W.; Catastini, P.; Conti, G.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA.
[Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E-E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany.
[Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany.
[Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany.
[Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan.
[Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA.
[Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria.
[Behera, P. K.; Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA.
[Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA.
[Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia.
[Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan.
[Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan.
[Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan.
[Takashima, R.] Kyoto Univ, Kyoto 612, Japan.
[Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan.
[Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina.
[Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina.
[Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; De Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England.
[Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy.
[Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy.
[Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England.
[Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia.
[Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia.
[Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England.
[Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England.
[Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England.
[Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France.
[Akesson, T. P.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.] Lund Univ, Fys Inst, Lund, Sweden.
[Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; March, L.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain.
[Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Maettig, S.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany.
[Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klemetti, M.; Klinger, J. A.; Lane, J. L.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England.
[Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France.
[Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France.
[Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA.
[Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Guler, H.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada.
[Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia.
[Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA.
[Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.
[Acerbia, E.; Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy.
[Acerbia, E.; Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy.
[Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus.
[Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus.
[Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA.
[Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Guler, H.; Leroy, C.; Martin, J. P.; Mehdiyev, R.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada.
[Akimov, A. V.; Baranov, P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia.
[Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia.
[Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst, Moscow, Russia.
[Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Calfayan, P.; De Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.] Univ Munich, Fak Phys, Munich, Germany.
[Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Seuster, R.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany.
[Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan.
[Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan.
[Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan.
[Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundisa, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy.
[Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy.
[Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA.
[Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koetsveld, F.; Koenig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands.
[Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands.
[Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands.
[Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.
[Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. S.; Bogdanchikov, A.; Kazanin, V. F.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia.
[Budick, B.; Casadei, D.; Cranmer, K.; Van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA.
[Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA.
[Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan.
[Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA.
[Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA.
[Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic.
[Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA.
[Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France.
[Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France.
[Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan.
[Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway.
[Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England.
[Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy.
[Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy.
[Alison, J.; Brendlinger, K.; Degenhardt, J.; Dressnandt, N.; Fratina, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA.
[Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia.
[Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy.
[Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy.
[Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA.
[Aguilar-Saavedra, J. A.; Amor Dos Santosa, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle We-Mansa, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal.
[Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain.
[Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain.
[Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic.
[Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic.
[Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic.
[Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia.
[Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England.
[Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada.
[Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan.
[Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; Pedis, D. De; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy.
[Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy.
[Aielli, G.; Albert, J.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy.
[Aielli, G.; Albert, J.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy.
[Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy.
[Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy.
[Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco.
[Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco.
[El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco.
[Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco.
[Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco.
[Cherkaoui El Mourslie, R.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco.
[Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J-B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondament Univers, Gif Sur Yvette, France.
[Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA.
[Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA.
[Booth, N.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Formica, A.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mc-fayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England.
[Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan.
[Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany.
[Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada.
[Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA.
[Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia.
[Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia.
[Assamagan, K.; Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa.
[Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa.
[Asman, B.; Bendtz, K.; Bohma, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden.
[Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden.
[Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden.
[Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA.
[Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
[Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England.
[Bangert, A.; Cuthbert, C.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia.
[Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, H.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, D.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan.
[Harpaz, S. Behar; Kajomovitz, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel.
[Harpaz, S. Behar; Kajomovitz, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Haifa, Israel.
[Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel.
[Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece.
[Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan.
[Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan.
[Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan.
[Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan.
[AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Knecht, N. S.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada.
[Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortina, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada.
[Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada.
[Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan.
[Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA.
[Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia.
[Avolio, G.; Deng, J.; Farrell, S.; Eschrich, I. Gough; Hawkins, D.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA.
[Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy.
[Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy.
[Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy.
[Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA.
[Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden.
[Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain.
[Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain.
[Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain.
[Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain.
[Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] CSIC, Valencia, Spain.
[Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada.
[Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada.
[Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England.
[Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan.
[Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel.
[Asfandiyarov, R.; Banerjee, Sw; Carrillo-Montoya, G. D.; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Fang, Y.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Li, H.; Ma, L. L.; Garcia, B. R. Mellado; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA.
[Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany.
[Barisonzi, M.; Becker, K.; Becks, K. H.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schultes, J.; Sturm, P.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany.
[Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Lagouri, T.; Lee, L.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA.
[Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia.
[Biscarat, C.; Cogneras, E.; Rahal, G.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France.
[Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England.
[Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal.
[Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal.
[Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA.
[Beloborodova, O.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia.
[Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal.
[Hernandez, A. M. Castaneda] UASLP, Dept Phys, San Luis Potosi, Mexico.
[Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy.
[Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey.
[Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA.
[Do Valle We-Mansa, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal.
[Do Valle We-Mansa, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal.
[Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa.
[Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany.
[Konoplich, R.] Manhattan Coll, New York, NY USA.
[Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China.
[Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan.
[Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal.
[Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA.
[Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary.
[Perez, K.] CALTECH, Pasadena, CA 91125 USA.
[Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy.
[Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland.
[Smirnova, L. N.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia.
[Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa.
RP Fortina, D (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany.
EM atlas.publications@cern.ch
RI Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin,
Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Mashinistov,
Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz,
Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan
Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones,
Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Della
Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015;
Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer,
Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo,
Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva,
Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko,
Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov,
Vladimir/M-6194-2015; Wolters, Helmut/M-4154-2013; Dawson,
Ian/K-6090-2013; Moraes, Arthur/F-6478-2010; Solfaroli Camillocci,
Elena/J-1596-2012; Ferrando, James/A-9192-2012; Boyko, Igor/J-3659-2013;
Brooks, William/C-8636-2013; Tudorache, Alexandra/L-3557-2013;
Tudorache, Valentina/D-2743-2012; Doyle, Anthony/C-5889-2009;
Marti-Garcia, Salvador/F-3085-2011; Shabalina, Elizaveta/M-2227-2013;
Castro, Nuno/D-5260-2011; Fassi, Farida/F-3571-2016; la rotonda,
laura/B-4028-2016; Santamarina Rios, Cibran/K-4686-2014; Bosman,
Martine/J-9917-2014; Wemans, Andre/A-6738-2012; Demirkoz,
Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; Ventura,
Andrea/A-9544-2015; Livan, Michele/D-7531-2012; Mitsou,
Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Riu,
Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose
/H-6339-2015; Nemecek, Stanislav/G-5931-2014; Lokajicek,
Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Staroba,
Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot,
Nicolo/A-2675-2009; Marcisovsky, Michal/H-1533-2014; Mikestikova,
Marcela/H-1996-2014; Kuday, Sinan/C-8528-2014; Tomasek,
Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba,
Jiri/G-7737-2014; Moorhead, Gareth/B-6634-2009; Peleganchuk,
Sergey/J-6722-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe
Francesco/A-5629-2016; Booth, Christopher/B-5263-2016; Solodkov,
Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario
/I-3549-2015; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017;
Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014;
Karyukhin, Andrey/J-3904-2014; SULIN, VLADIMIR/N-2793-2015; Nechaeva,
Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia,
Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria
Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin,
Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo,
Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; De, Kaushik/N-1953-2013;
Snesarev, Andrey/H-5090-2013; Warburton, Andreas/N-8028-2013; Sukharev,
Andrey/A-6470-2014; Fazio, Salvatore /G-5156-2010; Lee,
Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Smirnova,
Oxana/A-4401-2013; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009;
Carvalho, Joao/M-4060-2013; Nozka, Libor/G-5550-2014; Kepka,
Oldrich/G-6375-2014
OI Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636;
Andreazza, Attilio/0000-0001-5161-5759; Mashinistov,
Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz,
Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar
Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton,
Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes
Milosavljevic, Marija/0000-0003-4477-9733; Della Pietra,
Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206;
Negrini, Matteo/0000-0003-0101-6963; Ferrer,
Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543;
Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo,
stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645;
Tikhomirov, Vladimir/0000-0002-9634-0581; Wolters,
Helmut/0000-0002-9588-1773; Moraes, Arthur/0000-0002-5157-5686;
Solfaroli Camillocci, Elena/0000-0002-5347-7764; Ferrando,
James/0000-0002-1007-7816; Boyko, Igor/0000-0002-3355-4662; Brooks,
William/0000-0001-6161-3570; Doyle, Anthony/0000-0001-6322-6195; Castro,
Nuno/0000-0001-8491-4376; Fassi, Farida/0000-0002-6423-7213; la rotonda,
laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X;
Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291;
Coccaro, Andrea/0000-0003-2368-4559; Santamarina Rios,
Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Wemans,
Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan,
Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886;
Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582;
Mir, Lluisa-Maria/0000-0002-4276-715X; Mikestikova,
Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Tomasek,
Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Moorhead,
Gareth/0000-0002-9299-9549; Peleganchuk, Sergey/0000-0003-0907-7592;
Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736;
Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed
Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco,
Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe
Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649;
Veloso, Filipe/0000-0002-5956-4244; Booth,
Christopher/0000-0002-6051-2847; Gomes, Agostinho/0000-0002-5940-9893;
Solodkov, Alexander/0000-0002-2737-8674; Zaitsev,
Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207;
Grancagnolo, Francesco/0000-0002-9367-3380; Korol,
Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009;
Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin,
Andrey/0000-0001-9087-4315; SULIN, VLADIMIR/0000-0003-3943-2495;
Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia,
Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora
Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira,
Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399;
KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo,
Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; De,
Kaushik/0000-0002-5647-4489; Warburton, Andreas/0000-0002-2298-7315;
Lee, Jason/0000-0002-2153-1519; Smirnova, Oxana/0000-0003-2517-531X;
Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048;
Carvalho, Joao/0000-0002-3015-7821;
FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF,
Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil;
NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS,
China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech
Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark;
DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union;
ERC, European Union; NSRF, European Union; IN2P3-CNRS, France;
CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF,
Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF,
Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo
Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco;
FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW,
Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of
Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia;
ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain;
SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF,
Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland;
NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United
Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of
America; NSF, United States of America
FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC,
Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq
and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile;
CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and
VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark;
EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France;
GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and
NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN,
Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands;
BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS
(MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR;
MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South
Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF
and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey;
STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and
NSF, United States of America.
NR 24
TC 167
Z9 165
U1 16
U2 181
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1434-6044
EI 1434-6052
J9 EUR PHYS J C
JI Eur. Phys. J. C
PD AUG
PY 2013
VL 73
IS 8
AR 2518
DI 10.1140/epjc/s10052-013-2518-3
PG 39
WC Physics, Particles & Fields
SC Physics
GA 211IY
UT WOS:000323901300010
ER
PT J
AU Aad, G
Abajyan, T
Abbott, B
Abdallah, J
Abdel Khalek, S
Abdelalim, AA
Abdinov, O
Aben, R
Abi, B
Abolins, M
AbouZeid, OS
Abramowicz, H
Abreu, H
Acharya, BS
Adamczyk, L
Adams, DL
Addy, TN
Adelman, J
Adomeit, S
Adragna, P
Adye, T
Aefsky, S
Aguilar-Saavedra, JA
Agustoni, M
Aharrouche, M
Ahlen, SP
Ahles, F
Ahmad, A
Ahsan, M
Aielli, G
Akesson, TPA
Akimoto, G
Akimov, AV
Alam, MS
Alam, MA
Albert, J
Albrand, S
Aleksa, M
Aleksandrov, IN
Alessandria, F
Alexa, C
Alexander, G
Alexandre, G
Alexopoulos, T
Alhroob, M
Aliev, M
Alimonti, G
Alison, J
Allbrooke, BMM
Allport, PP
Allwood-Spiers, SE
Almond, J
Aloisio, A
Alon, R
Alonso, A
Alonso, F
Altheimer, A
Gonzalez, BA
Alviggi, MG
Amako, K
Amelung, C
Ammosov, VV
Dos Santos, SPA
Amorim, A
Amram, N
Anastopoulos, C
Ancu, LS
Andari, N
Andeen, T
Anders, CF
Anders, G
Anderson, KJ
Andreazza, A
Andrei, V
Andrieux, ML
Anduaga, XS
Angelidakis, S
Anger, P
Angerami, A
Anghinolfi, F
Anisenkov, AV
Anjos, N
Annovi, A
Antonaki, A
Antonelli, M
Antonov, A
Antos, J
Anulli, F
Aoki, M
Aoun, S
Bella, LA
Apolle, R
Arabidze, G
Aracena, I
Arai, Y
Arce, ATH
Arfaoui, S
Arguin, JF
Argyropoulos, S
Arik, E
Arik, M
Armbruster, AJ
Arnaez, O
Arnal, V
Arnault, C
Artamonov, A
Artoni, G
Arutinov, D
Asai, S
Ask, S
Asman, B
Asquith, L
Assamagan, K
Astbury, A
Atkinson, M
Aubert, B
Auge, E
Augsten, K
Aurousseau, M
Avolio, G
Avramidou, R
Axen, D
Azuelos, G
Azuma, Y
Baak, MA
Baccaglioni, G
Bacci, C
Bach, AM
Bachacou, H
Bachas, K
Backes, M
Backhaus, M
Mayes, JB
Badescu, E
Bagnaia, P
Bahinipati, S
Bai, Y
Bailey, DC
Bain, T
Baines, JT
Baker, OK
Baker, MD
Baker, S
Balek, P
Banas, E
Banerjee, P
Banerjee, S
Banfi, D
Bangert, A
Bansal, V
Bansil, HS
Barak, L
Baranov, SP
Galtieri, AB
Barber, T
Barberio, EL
Barberis, D
Barbero, M
Bardin, DY
Barillari, T
Barisonzi, M
Barklow, T
Barlow, N
Barnett, BM
Barnett, RM
Baroncelli, A
Barone, G
Barr, AJ
Barreiro, F
da Costa, JBG
Barrillon, P
Bartoldus, R
Barton, AE
Bartsch, V
Basye, A
Bates, RL
Batkova, L
Batley, JR
Battaglia, A
Battistin, M
Bauer, F
Bawa, HS
Beale, S
Beau, T
Beauchemin, PH
Beccherle, R
Bechtle, P
Beck, HP
Becker, K
Becker, S
Beckingham, M
Becks, KH
Beddall, AJ
Beddall, A
Bedikian, S
Bednyakov, VA
Bee, CP
Beemster, LJ
Begel, M
Harpaz, SB
Behera, PK
Beimforde, M
Belanger-Champagne, C
Bell, PJ
Bell, WH
Bella, G
Bellagamba, L
Bellomo, M
Belloni, A
Beloborodova, OL
Belotskiy, K
Beltramello, O
Benary, O
Benchekroun, D
Bendtz, K
Benekos, N
Benhammou, Y
Noccioli, EB
Garcia, JAB
Benjamin, DP
Benoit, M
Bensinger, JR
Benslama, K
Bentvelsen, S
Berge, D
Kuutmann, EB
Berger, N
Berghaus, F
Berglund, E
Beringer, J
Bernat, P
Bernhard, R
Bernius, C
Berry, T
Bertella, C
Bertin, A
Bertolucci, F
Besana, MI
Besjes, GJ
Besson, N
Bethke, S
Bhimji, W
Bianchi, RM
Bianchini, L
Bianco, M
Biebel, O
Bieniek, SP
Bierwagen, K
Biesiada, J
Biglietti, M
Bilokon, H
Bindi, M
Binet, S
Bingul, A
Bini, C
Bittner, B
Black, CW
Black, KM
Blair, RE
Blanchard, JB
Blanchot, G
Blazek, T
Bloch, I
Blocker, C
Blocki, J
Blondel, A
Blum, W
Blumenschein, U
Bobbink, GJ
Bobrovnikov, VS
Bocchetta, SS
Bocci, A
Boddy, CR
Boehler, M
Boek, J
Boek, TT
Boelaert, N
Bogaerts, JA
Bogdanchikov, AG
Bogouch, A
Bohm, C
Bohm, J
Boisvert, V
Bold, T
Boldea, V
Bolnet, NM
Bomben, M
Bona, M
Bondioli, M
Boonekamp, M
Bordoni, S
Borer, C
Borisov, A
Borissov, G
Borjanovic, I
Borri, M
Borroni, S
Bortfeldt, J
Bortolotto, V
Bos, K
Boscherini, D
Bosman, M
Boterenbrood, H
Bouchami, J
Boudreau, J
Bouhova-Thacker, EV
Boumediene, D
Bourdarios, C
Bousson, N
Boveia, A
Boyd, J
Boyko, IR
Bozovic-Jelisavcic, I
Bracinik, J
Branchini, P
Brandt, A
Brandt, G
Brandt, O
Bratzler, U
Brau, B
Brau, JE
Braun, HM
Brazzale, SF
Brelier, B
Bremer, J
Brendlinger, K
Brenner, R
Bressler, S
Britton, D
Brochu, FM
Brock, I
Brock, R
Broggi, F
Bromberg, C
Bronner, J
Brooijmans, G
Brooks, T
Brooks, WK
Brown, G
Brown, H
de Renstrom, PAB
Bruncko, D
Bruneliere, R
Brunet, S
Bruni, A
Bruni, G
Bruschi, M
Buanes, T
Buat, Q
Bucci, F
Buchanan, J
Buchholz, P
Buckingham, RM
Buckley, AG
Buda, SI
Budagov, IA
Budick, B
Bugge, L
Bulekov, O
Bundock, AC
Bunse, M
Buran, T
Burckhart, H
Burdin, S
Burgess, T
Burke, S
Busato, E
Buscher, V
Bussey, P
Buszello, CP
Butler, B
Butler, JM
Buttar, CM
Butterworth, JM
Buttinger, W
Byszewski, M
Urban, SC
Caforio, D
Cakir, O
Calafiura, P
Calderini, G
Calfayan, P
Calkins, R
Caloba, LP
Caloi, R
Calvet, D
Calvet, S
Toro, RC
Camarri, P
Cameron, D
Caminada, LM
Armadans, RC
Campana, S
Campanelli, M
Canale, V
Canelli, F
Canepa, A
Cantero, J
Cantrill, R
Capasso, L
Garrido, MDMC
Caprini, I
Caprini, M
Capriotti, D
Capua, M
Caputo, R
Cardarelli, R
Carli, T
Carlino, G
Carminati, L
Caron, B
Caron, S
Carquin, E
Carrillo-Montoya, GD
Carter, AA
Carter, JR
Carvalho, J
Casadei, D
Casado, MP
Cascella, M
Caso, C
Hernandez, AMC
Castaneda-Miranda, E
Gimenez, VC
Castro, NF
Cataldi, G
Catastini, P
Catinaccio, A
Catmore, JR
Cattai, A
Cattani, G
Caughron, S
Cavaliere, V
Cavalli, D
Cavalli-Sforza, M
Cavasinni, V
Ceradini, F
Cerqueira, AS
Cerri, A
Cerrito, L
Cerutti, F
Cetin, SA
Chafaq, A
Chakraborty, D
Chalupkova, I
Chan, K
Chang, P
Chapleau, B
Chapman, JD
Chapman, JW
Chareyre, E
Charlton, DG
Chavda, V
Barajas, CAC
Cheatham, S
Chekanov, S
Chekulaev, SV
Chelkov, GA
Chelstowska, MA
Chen, C
Chen, H
Chen, S
Chen, X
Chen, Y
Cheng, Y
Cheplakov, A
El Moursli, RC
Chernyatin, V
Cheu, E
Cheung, SL
Chevalier, L
Chiefari, G
Chikovani, L
Childers, JT
Chilingarov, A
Chiodini, G
Chisholm, AS
Chislett, RT
Chitan, A
Chizhov, MV
Choudalakis, G
Chouridou, S
Christidi, IA
Christov, A
Chromek-Burckhart, D
Chu, ML
Chudoba, J
Ciapetti, G
Ciftci, AK
Ciftci, R
Cinca, D
Cindro, V
Ciocio, A
Cirilli, M
Cirkovic, P
Citron, ZH
Citterio, M
Ciubancan, M
Clark, A
Clark, PJ
Clarke, RN
Cleland, W
Clemens, JC
Clement, B
Clement, C
Coadou, Y
Cobal, M
Coccaro, A
Cochran, J
Coelli, S
Coffey, L
Cogan, JG
Coggeshall, J
Cogneras, E
Colas, J
Cole, S
Colijn, AP
Collins, NJ
Collins-Tooth, C
Collot, J
Colombo, T
Colon, G
Compostella, G
Muino, PC
Coniavitis, E
Conidi, MC
Consonni, SM
Consorti, V
Constantinescu, S
Conta, C
Conti, G
Conventi, F
Cooke, M
Cooper, BD
Cooper-Sarkar, AM
Copic, K
Cornelissen, T
Corradi, M
Corriveau, F
Corso-Radu, A
Cortes-Gonzalez, A
Cortiana, G
Costa, G
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CA ATLAS Collaboration
TI Measurement of the inclusive jet cross-section in pp collisions at root
s=2.76 TeV and comparison to the inclusive jet cross-section at root s=7
TeV using the ATLAS detector
SO EUROPEAN PHYSICAL JOURNAL C
LA English
DT Article
ID DEEP-INELASTIC SCATTERING; CERN PBARP COLLIDER; (P)OVER-BAR-P
COLLISIONS; PERTURBATION-THEORY; PARTON DISTRIBUTIONS; EP SCATTERING;
FRAGMENTATION; SHOWERS; MODEL
AB The inclusive jet cross-section has been measured in proton-proton collisions at root s = 2.76 TeV in a dataset corresponding to an integrated luminosity of 0.20 pb(-1) collected with the ATLAS detector at the Large Hadron Collider in 2011. Jets are identified using the anti-k(t) algorithm with two radius parameters of 0.4 and 0.6. The inclusive jet double-differential cross-section is presented as a function of the jet transverse momentum p(T) and jet rapidity y, covering a range of 20 <= p(T) < 430 GeV and vertical bar y vertical bar < 4.4. The ratio of the cross-section to the inclusive jet cross-section measurement at root s = 7 TeV, published by the ATLAS Collaboration, is calculated as a function of both transverse momentum and the dimensionless quantity x(T) = 2p(T)/root s, in bins of jet rapidity. The systematic uncertainties on the ratios are significantly reduced due to the cancellation of correlated uncertainties in the two measurements. Results are compared to the prediction from next-to-leading order perturbative QCD calculations corrected for non-perturbative effects, and next-to-leading order Monte Carlo simulation. Furthermore, the ATLAS jet cross-section measurements at root s = 2.76 TeV and root s = 7 TeV are analysed within a framework of next-to-leading order perturbative QCD calculations to determine parton distribution functions of the proton, taking into account the correlations between the measurements.
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[Abajyan, T.; Ahmad, A.; Arutinov, D.; Backhaus, M.; Barbero, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Karagounis, M.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Limbach, C.; Loddenkoetter, T.; Mazur, M.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Sarrazin, B.; Schaepe, S.; Schmieden, K.; Schultens, M. J.; Schwindt, T.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany.
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[Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina.
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[Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Wang, J.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China.
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[Alonso, A.; Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark.
[Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN, Grp Collegato Cosenza, Arcavacata Di Rende, Italy.
[Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy.
[Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland.
[Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland.
[Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA.
[Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA.
[Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Gomez Fajardo, L. S.; Firmino Da Costa, J. Goncalves Pinto; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Jimenez Belenguer, M.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Perez Cavalcanti, T.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Hamburg, Germany.
[Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Gomez Fajardo, L. S.; Firmino Da Costa, J. Goncalves Pinto; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Jimenez Belenguer, M.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Perez Cavalcanti, T.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany.
[Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany.
[Anger, P.; Ciftci, R.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany.
[Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA.
[Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland.
[Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy.
[Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany.
[Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Mora Herrera, C.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland.
[Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Ferretto Parodi, A.; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy.
[Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Ferretto Parodi, A.; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy.
[Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia.
[Djobava, T.; Khubuab, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia.
[Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany.
[Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; Ferreira de Lima, D. E.; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Oropeza Barrera, C.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland.
[Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Hamer, M.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany.
[Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France.
[Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Weydert, C.] CNRS, IN2P3, Grenoble, France.
[Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France.
[Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA.
[da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Lopez Mateos, D.; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA.
[Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Henke, M.; Hofmann, J. I.; Khomicha, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany.
[Anders, C. F.; Kasieczkab, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany.
[Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany.
[Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan.
[Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA.
[Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria.
[Behera, P. K.; Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA.
[Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA.
[Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia.
[Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan.
[Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan.
[Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan.
[Takashima, R.] Kyoto Univ, Kyoto 612, Japan.
[Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan.
[Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina.
[Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina.
[Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England.
[Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy.
[Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy.
[Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England.
[Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia.
[Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia.
[Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England.
[Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Panduro Vazquez, J. G.; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England.
[Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England.
[Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA.
[Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Chareyre, E.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France.
[Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Chareyre, E.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France.
[Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Chareyre, E.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France.
[Akesson, T. P. A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjrnmark, J. U.; Smirnova, O.] Lund Univ, Inst Fys, Lund, Sweden.
[Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain.
[Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany.
[Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England.
[Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France.
[Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France.
[Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA.
[Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada.
[Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Nunes Hanninger, G.; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia.
[Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA.
[Abolins, M.; Alvarez Gonzalez, B.; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.
[Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy.
[Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy.
[Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus.
[Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus.
[Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA.
[Arguin, J-F.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada.
[Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia.
[Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia.
[Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia.
[Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany.
[Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany.
[Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan.
[Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan.
[Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan.
[Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy.
[Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy.
[Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA.
[Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koetsveld, F.; Koenig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands.
[Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Doxiadis, A. D.; Ferrari, P.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands.
[Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Doxiadis, A. D.; Ferrari, P.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands.
[Calkins, R.; Chakraborty, D.; Cole, S.; Rocha De Lima, J. G.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.
[Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I. O.; Peleganchuk, S. V.; Shamov, A. G.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia.
[Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA.
[Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA.
[Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan.
[Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA.
[Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA.
[Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic.
[Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA.
[Abdel Khalek, S.; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; DeRegie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lorenzo Martinez, N.; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France.
[Abdel Khalek, S.; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; DeRegie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lorenzo Martinez, N.; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France.
[Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan.
[Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway.
[Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England.
[Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy.
[Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy.
[Alison, J.; Brendlinger, K.; Degenhardt, J.; Dressnandt, N.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA.
[Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia.
[Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy.
[Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy.
[Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA.
[Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorgea, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal.
[Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain.
[Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain.
[Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic.
[Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic.
[Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic.
[Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] Inst High Energy Phys, State Res Ctr, Protvino, Russia.
[Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Conventi, F.; Dewhurst, A.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England.
[Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada.
[Tanaka, S.] Ritsumeikan Univ, Shiga, Japan.
[Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminaria, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy.
[Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy.
[Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy.
[Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy.
[Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy.
[Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy.
[Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Res Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco.
[Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco.
[El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco.
[Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier & LPTPM, Fac Sci, Oujda, Morocco.
[El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco.
[Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Engelmann, R.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Manjarres Ramos, J. A.; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France.
[Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA.
[Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA.
[Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England.
[Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan.
[Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany.
[Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada.
[Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA.
[Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia.
[Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia.
Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa.
[Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa.
[Carrillo-Montoya, G. D.; Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa.
[Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Elmsheuser, J.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden.
[Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden.
[Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden.
[Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA.
[Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
[Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Santoyo Castillo, I.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England.
[Bangert, A.; Black, C. W.; Cuthbert, C.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia.
[Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan.
[Harpaz, S. Behar; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel.
[Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel.
[Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece.
[Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan.
[Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan.
[Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan.
[Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan.
[AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Cheung, S. L.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada.
[Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oram, C. J.; Perez Codina, E.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada.
[Benitez Garcia, J. A.; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada.
[Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan.
[Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA.
[Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia.
[Bondioli, M.; Corso-Radu, A.; Farrell, S.; Gough Eschrich, I.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA.
[Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] INFN, Grp Collegato Udine, Udine, Italy.
[Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy.
[Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy.
[Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA.
[Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden.
[Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain.
[Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain.
[Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain.
[Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain.
[Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain.
[Axen, D.; Gay, C.; Gecse, Z.; Kind, O.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada.
[Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada.
[Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England.
[Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan.
[Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel.
[Banerjee, Sw.; Castaneda Hernandez, A. M.; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Ma, L. L.; Mellado Garcia, B. R.; Ming, Y.; Pan, Y. B.; Pedraza Morales, M. I.; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA.
[Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany.
[Barisonzi, M.; Becker, K.; Becks, K. H.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany.
[Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA.
[Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia.
[Cogneras, E.; Kohlmann, S.; Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France.
[Acharya, B. S.; Ruan, X.] Kings Coll London, Dept Phys, London, England.
[Amorim, A.; Gomes, A.; Maio, A.; Pina, J.; Savard, P.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal.
[Amorim, A.; Gomes, A.; Maio, A.; Pina, J.; Savard, P.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal.
[Apolle, R.; Davies, E.; Mattravers, C.; Nash, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England.
[Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada.
[Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA.
[Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia.
[Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal.
[Castaneda Hernandez, A. M.] UASLP, Dept Phys, San Luis Potosi, Mexico.
[Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy.
[Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey.
[Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA.
[Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, Dep Fis, Caparica, Portugal.
[Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal.
[Dobson, E.] UCL, Dept Phys & Astron, London, England.
[Ge, P.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.
[Grinstein, S.; Martinez, M.] ICREA, Barcelona, Spain.
[Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa.
[Huseynov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan.
[Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany.
Manhattan Coll, New York, NY USA.
[Li, B.; Zhang, D.] Acad Sinica, Inst Phys, Taipei, Taiwan.
[Li, S.] Aix Marseille Univ, CPPM, Marseille, France.
[Li, S.] CNRS, IN2P3, Marseille, France.
[Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China.
[Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan.
[Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India.
[Meng, Z.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China.
[Messina, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy.
[Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia.
[Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland.
[Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal.
[Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA.
[Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary.
[Perez, K.] CALTECH, Pasadena, CA 91125 USA.
[Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy.
[Ruan, X.] Univ Paris 11, LAL, Orsay, France.
[Ruan, X.] CNRS, IN2P3, F-91405 Orsay, France.
[Smirnova, L. N.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia.
[Spousta, M.] Columbia Univ, Nevis Lab, Irvington, NY USA.
[Tamsett, M. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
[Tsionou, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England.
[Vickey, T.] Univ Oxford, Dept Phys, Oxford, England.
[Wu, Y.; Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA.
[Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa.
RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany.
RI Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek,
Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco,
Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Marcisovsky,
Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Kuday,
Sinan/C-8528-2014; Tomasek, Lukas/G-6370-2014; Svatos,
Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Moorhead,
Gareth/B-6634-2009; Peleganchuk, Sergey/J-6722-2014; De,
Kaushik/N-1953-2013; Snesarev, Andrey/H-5090-2013; Warburton,
Andreas/N-8028-2013; Sukharev, Andrey/A-6470-2014; Fazio, Salvatore
/G-5156-2010; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011;
Smirnova, Oxana/A-4401-2013; Fabbri, Laura/H-3442-2012; Villa,
Mauro/C-9883-2009; Carvalho, Joao/M-4060-2013; Nozka, Libor/G-5550-2014;
Nemecek, Stanislav/G-5931-2014; Capua, Marcella/A-8549-2015; Tartarelli,
Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda,
laura/B-4028-2016; Dawson, Ian/K-6090-2013; Moraes, Arthur/F-6478-2010;
Solfaroli Camillocci, Elena/J-1596-2012; Ferrando, James/A-9192-2012;
Boyko, Igor/J-3659-2013; Brooks, William/C-8636-2013; Tudorache,
Alexandra/L-3557-2013; Tudorache, Valentina/D-2743-2012; Doyle,
Anthony/C-5889-2009; Marti-Garcia, Salvador/F-3085-2011; Shabalina,
Elizaveta/M-2227-2013; Castro, Nuno/D-5260-2011; Wolters,
Helmut/M-4154-2013; Yang, Haijun/O-1055-2015; Monzani,
Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol,
Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Olshevskiy,
Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito,
Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira,
Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV,
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Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev,
Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Gladilin,
Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Mashinistov,
Ruslan/M-8356-2015; Fullana Torregrosa, Esteban/A-7305-2016; Buttar,
Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo,
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Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Bosman,
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Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose
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OI Mikestikova, Marcela/0000-0003-1277-2596; Kuday,
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Peleganchuk, Sergey/0000-0003-0907-7592; De,
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Carvalho, Joao/0000-0002-3015-7821; Coccaro, Andrea/0000-0003-2368-4559;
Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua,
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Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria,
Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244;
Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213;
la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca
Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos,
Helena/0000-0003-1710-9291; Moraes, Arthur/0000-0002-5157-5686;
Solfaroli Camillocci, Elena/0000-0002-5347-7764; Ferrando,
James/0000-0002-1007-7816; Boyko, Igor/0000-0002-3355-4662; Brooks,
William/0000-0001-6161-3570; Doyle, Anthony/0000-0001-6322-6195; Castro,
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Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380;
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Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira,
Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399;
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Alexandre/0000-0002-4961-8368; Gladilin, Leonid/0000-0001-9422-8636;
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Ruslan/0000-0001-7925-4676; Fullana Torregrosa,
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Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar
Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton,
Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes
Milosavljevic, Marija/0000-0003-4477-9733; SULIN,
VLADIMIR/0000-0003-3943-2495; Petrucci, Fabrizio/0000-0002-5278-2206;
Negrini, Matteo/0000-0003-0101-6963; Ferrer,
Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543;
Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo,
stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645;
Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov,
Igor/0000-0001-5570-0133; Bosman, Martine/0000-0002-7290-643X; Wemans,
Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan,
Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886;
Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582;
Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra,
Massimo/0000-0003-4446-3368
FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF,
Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil;
NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS,
China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech
Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark;
DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union;
ERC, European Union; NSRF, European Union; IN2P3-CNRS, France;
CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF,
Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF,
Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo
Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco;
FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW,
Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of
Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia;
ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain;
SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF,
Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland;
NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United
Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of
America; NSF, United States of America
FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC,
Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq
and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile;
CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and
VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark;
EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France;
GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and
NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN,
Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands;
BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS
(MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR;
MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South
Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF
and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey;
STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and
NSF, United States of America.
NR 92
TC 24
Z9 24
U1 9
U2 158
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1434-6044
EI 1434-6052
J9 EUR PHYS J C
JI Eur. Phys. J. C
PD AUG
PY 2013
VL 73
IS 8
AR 2509
DI 10.1140/epjc/s10052-013-2509-4
PG 56
WC Physics, Particles & Fields
SC Physics
GA 211IY
UT WOS:000323901300004
ER
PT J
AU Xing, YL
Chou, CS
Shu, CW
AF Xing, Yulong
Chou, Ching-Shan
Shu, Chi-Wang
TI ENERGY CONSERVING LOCAL DISCONTINUOUS GALERKIN METHODS FOR WAVE
PROPAGATION PROBLEMS
SO INVERSE PROBLEMS AND IMAGING
LA English
DT Article
DE Wave propagation; local discontinuous Calerkin method; energy
conservation; error estimate; superconvergence
ID FINITE-ELEMENT-METHOD; CONSERVATION-LAWS; HYPERBOLIC SYSTEMS; EQUATION
AB Wave propagation problems arise in a wide range of applications. The energy conserving property is one of the guiding principles for numerical algorithms, in order to minimize the phase or shape errors after long time integration. In this paper, we develop and analyze a local discontinuous Calerkin (LDC) method for solving the wave equation. We prove optimal error estimates, superconvergence toward a particular projection of the exact solution, and the energy conserving property for the semi-discrete formulation. The analysis is extended to the fully discrete LDC scheme, with the centered second-order time discretization (the leap-frog scheme). Our numerical experiments demonstrate optimal rates of convergence and superconvergence. We also show that the shape of the solution, after long time integration, is well preserved due to the energy conserving property.
C1 [Xing, Yulong] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.
[Xing, Yulong] Univ Tennessee, Dept Math, Oak Ridge, TN 37831 USA.
[Chou, Ching-Shan] Ohio State Univ, Dept Math, Columbus, OH 43221 USA.
[Shu, Chi-Wang] Brown Univ, Div Appl Math, Providence, RI 02912 USA.
RP Xing, YL (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.
EM xingy@math.utk.edu; chou@math.ohio-state.edu; shu@dam.brown.edu
FU NSF [DMS-1216454, DMS-1020625, DMS-1112700]; ORNL's Laboratory Directed
Research and Development funds; DOE Office of Advanced Scientific
Computing Research; DOE [DE-FG02-08ER25863]; UT-Battelle, LLC
[DE-AC05-00OR22725]
FX The work of the first author was partially performed at ORNL, which is
managed by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725.
NR 23
TC 12
Z9 12
U1 1
U2 5
PU AMER INST MATHEMATICAL SCIENCES-AIMS
PI SPRINGFIELD
PA PO BOX 2604, SPRINGFIELD, MO 65801-2604 USA
SN 1930-8337
EI 1930-8345
J9 INVERSE PROBL IMAG
JI Inverse Probl. Imaging
PD AUG
PY 2013
VL 7
IS 3
SI SI
BP 967
EP 986
DI 10.3934/ipi.2013.7.967
PG 20
WC Mathematics, Applied; Physics, Mathematical
SC Mathematics; Physics
GA 218AO
UT WOS:000324405200018
ER
PT J
AU Akl, TJ
Wilson, MA
Ericson, MN
Cote, GL
AF Akl, Tony J.
Wilson, Mark A.
Ericson, M. Nance
Cote, Gerard L.
TI Intestinal perfusion monitoring using photoplethysmography
SO JOURNAL OF BIOMEDICAL OPTICS
LA English
DT Article
DE photoplethysmography; spectroscopy; oximetry; perfusion monitoring;
trauma
ID NEAR-INFRARED SPECTROSCOPY; BLOOD-FLOW; IMPLANTABLE SENSOR;
OXYGEN-SATURATION; TISSUE; SHOCK; RESUSCITATION; PENETRATION;
HEMOGLOBIN; PRESSURE
AB In abdominal trauma patients, monitoring intestinal perfusion and oxygen consumption is essential during the resuscitation period. Photoplethysmography is an optical technique potentially capable of monitoring these changes in real time to provide the medical staff with a timely and quantitative measure of the adequacy of resuscitation. The challenges for using optical techniques in monitoring hemodynamics in intestinal tissue are discussed, and the solutions to these challenges are presented using a combination of Monte Carlo modeling and theoretical analysis of light propagation in tissue. In particular, it is shown that by using visible wavelengths (i.e., 470 and 525 nm), the perfusion signal is enhanced and the background contribution is decreased compared with using traditional near-infrared wavelengths leading to an order of magnitude enhancement in the signal-to-background ratio. It was further shown that, using the visible wavelengths, similar sensitivity to oxygenation changes could be obtained (over 50% compared with that of near-infrared wavelengths). This is mainly due to the increased contrast between tissue and blood in that spectral region and the confinement of the photons to the thickness of the small intestine. Moreover, the modeling results show that the source to detector separation should be limited to roughly 6 mm while using traditional near-infrared light, with a few centimeters source to detector separation leads to poor signal-to-background ratio. Finally, a visible wavelength system is tested in an in vivo porcine study, and the possibility of monitoring intestinal perfusion changes is showed. (C) 2013 Society of Photo-Optical Instrumentation Engineers (SPIE)
C1 [Akl, Tony J.; Cote, Gerard L.] Texas A&M Univ, Dept Biomed Engn, College Stn, TX 77843 USA.
[Wilson, Mark A.] Univ Pittsburgh, Dept Surg, Pittsburgh, PA 15213 USA.
[Wilson, Mark A.] Vet Affairs Healthcare Syst, Pittsburgh, PA 15240 USA.
[Ericson, M. Nance] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Akl, TJ (reprint author), Texas A&M Univ, Dept Biomed Engn, 5045 Emerging Technol Bldg, College Stn, TX 77843 USA.
EM takl@tamu.edu
RI Ericson, Milton/H-9880-2016
OI Ericson, Milton/0000-0002-6628-4865
FU NIH [5R01-GM077150]
FX This research was funded by a bioengineering research partnership (BRP)
grant from NIH (#5R01-GM077150).
NR 53
TC 0
Z9 0
U1 0
U2 5
PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS
PI BELLINGHAM
PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA
SN 1083-3668
EI 1560-2281
J9 J BIOMED OPT
JI J. Biomed. Opt.
PD AUG
PY 2013
VL 18
IS 8
AR 087005
DI 10.1117/1.JBO.18.8.087005
PG 12
WC Biochemical Research Methods; Optics; Radiology, Nuclear Medicine &
Medical Imaging
SC Biochemistry & Molecular Biology; Optics; Radiology, Nuclear Medicine &
Medical Imaging
GA 216MN
UT WOS:000324287700022
PM 23942635
ER
PT J
AU El Hedri, S
Hook, A
Jankowiak, M
Wacker, JG
AF El Hedri, Sonia
Hook, Anson
Jankowiak, Martin
Wacker, Jay G.
TI Learning how to count: a high multiplicity search for the LHC
SO JOURNAL OF HIGH ENERGY PHYSICS
LA English
DT Article
DE QCD Phenomenology; Jets
ID ALGORITHMS
AB We introduce a search technique that is sensitive to a broad class of signals with large final state multiplicities. Events are clustered into large radius jets and jet substructure techniques are used to count the number of subjets within each jet. The search consists of a cut on the total number of subjets in the event as well as the summed jet mass and missing energy. Two different techniques for counting subjets are described and expected sensitivities are presented for eight benchmark signals. These signals exhibit diverse phenomenology, including 2-step cascade decays, direct three body decays, and multi-top final states. We find improved sensitivity to these signals as compared to previous high multiplicity searches as well as a reduced reliance on missing energy requirements. One benefit of this approach is that it allows for natural data driven estimates of the QCD background.
C1 [El Hedri, Sonia; Wacker, Jay G.] Stanford Univ, SLAC, Menlo Pk, CA 94025 USA.
[Hook, Anson] Princeton Univ, Inst Adv Studies, Princeton, NJ 08544 USA.
[Jankowiak, Martin] Heidelberg Univ, Inst Theoret Phys, Heidelberg, Germany.
RP El Hedri, S (reprint author), Stanford Univ, SLAC, Menlo Pk, CA 94025 USA.
EM soniaeh@slac.stanford.edu; hook@ias.edu;
jankowiak@thphys.uni-heidelberg.de; jgwacker@slac.stanford.edu
FU US DOE [DE-AC02-76-SF00515, DE-FG02-90ER40542]; Stanford Graduate
Fellowship
FX We thank Timothy Cohen, Eder Izaguirre, Mariangela Lisanti, Jesse
Thaler, Gavin Salam, Stefan Hoche, Steffen Schumann, Ariel Schwartzman,
Ken Van Tilburg, and Xinlu Huang for helpful discussions. MJ would like
to thank Michael Spannowsky for interesting conversations. Special
thanks to Timothy Cohen for having provided Monte Carlo data for the QCD
background. SE and JW are supported by the US DOE under contract number
DE-AC02-76-SF00515. SE is supported by a Stanford Graduate Fellowship.
All is supported by the US DOE under contract number DE-FG02-90ER40542.
NR 59
TC 14
Z9 14
U1 0
U2 0
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1029-8479
J9 J HIGH ENERGY PHYS
JI J. High Energy Phys.
PD AUG
PY 2013
IS 8
AR 136
DI 10.1007/JHEP08(2013)136
PG 38
WC Physics, Particles & Fields
SC Physics
GA 214EN
UT WOS:000324114000037
ER
PT J
AU Acciarri, R
Adams, C
Asaadi, J
Baller, B
Bolton, T
Bromberg, C
Cavanna, F
Church, E
Edmunds, D
Ereditato, A
Farooq, S
Fleming, B
Greenlee, H
Horton-Smith, G
James, C
Klein, E
Lang, K
Laurens, P
McKee, D
Mehdiyev, R
Page, B
Palamara, O
Partyka, K
Rameika, G
Rebel, B
Soderberg, M
Spitz, J
Szelc, AM
Weber, M
Wojcik, M
Yang, T
Zeller, GP
AF Acciarri, R.
Adams, C.
Asaadi, J.
Baller, B.
Bolton, T.
Bromberg, C.
Cavanna, F.
Church, E.
Edmunds, D.
Ereditato, A.
Farooq, S.
Fleming, B.
Greenlee, H.
Horton-Smith, G.
James, C.
Klein, E.
Lang, K.
Laurens, P.
McKee, D.
Mehdiyev, R.
Page, B.
Palamara, O.
Partyka, K.
Rameika, G.
Rebel, B.
Soderberg, M.
Spitz, J.
Szelc, A. M.
Weber, M.
Wojcik, M.
Yang, T.
Zeller, G. P.
TI A study of electron recombination using highly ionizing particles in the
ArgoNeuT Liquid Argon TPC
SO JOURNAL OF INSTRUMENTATION
LA English
DT Article
DE Cryogenic detectors; Analysis and statistical methods; Time projection
chambers
ID THERMALIZATION; MATTER; XENON
AB Electron recombination in highly ionizing stopping protons and deuterons is studied in the ArgoNeuT detector. The data are well modeled by either a Birks model or a modified form of the Box model. The dependence of recombination on the track angle with respect to the electric field direction is much weaker than the predictions of the Jaffe columnar theory and by theoretical-computational simulations.
C1 [Acciarri, R.; Baller, B.; Greenlee, H.; James, C.; Rameika, G.; Rebel, B.; Soderberg, M.; Yang, T.; Zeller, G. P.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Adams, C.; Cavanna, F.; Church, E.; Fleming, B.; Klein, E.; Palamara, O.; Partyka, K.; Spitz, J.; Szelc, A. M.] Yale Univ, New Haven, CT 06520 USA.
[Asaadi, J.; Soderberg, M.] Syracuse Univ, Syracuse, NY 13244 USA.
[Bolton, T.; Farooq, S.; Horton-Smith, G.; McKee, D.] Kansas State Univ, Manhattan, KS 66506 USA.
[Bromberg, C.; Edmunds, D.; Laurens, P.; Page, B.] Michigan State Univ, E Lansing, MI 48824 USA.
[Cavanna, F.] Univ Aquila, I-67100 Laquila, Italy.
[Cavanna, F.] Ist Nazl Fis Nucl, Laquila, Italy.
[Ereditato, A.; Weber, M.] Univ Bern, Bern, Switzerland.
[Lang, K.; Mehdiyev, R.] Univ Texas Austin, Austin, TX 78712 USA.
[Palamara, O.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, Italy.
[Wojcik, M.] Lodz Univ Technol, Lodz, Poland.
RP Baller, B (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA.
EM baller@fnal.gov
RI Horton-Smith, Glenn/A-4409-2011;
OI Horton-Smith, Glenn/0000-0001-9677-9167; Spitz,
Joshua/0000-0002-6288-7028; Weber, Michele/0000-0002-2770-9031; Cavanna,
Flavio/0000-0002-5586-9964
FU Fermilab; U.S. Department of Energy; National Science foundation; United
States Department of Energy [DE-AC02-07CH11359]
FX We gratefully acknowledge the support of Fermilab, the U.S. Department
of Energy and the National Science foundation. Fermilab is operated by
Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with
the United States Department of Energy.
NR 18
TC 11
Z9 11
U1 0
U2 10
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 1748-0221
J9 J INSTRUM
JI J. Instrum.
PD AUG
PY 2013
VL 8
AR P08005
DI 10.1088/1748-0221/8/08/P08005
PG 18
WC Instruments & Instrumentation
SC Instruments & Instrumentation
GA 212XZ
UT WOS:000324017400010
ER
PT J
AU Bassignana, D
Li, Z
Lozano, M
Pellegrini, G
Quirion, D
Tuuva, T
AF Bassignana, D.
Li, Z.
Lozano, M.
Pellegrini, G.
Quirion, D.
Tuuva, T.
TI Design, fabrication and characterization of the first dual-column 3D
stripixel detectors
SO JOURNAL OF INSTRUMENTATION
LA English
DT Article
DE Solid state detectors; Radiation-hard detectors; Particle tracking
detectors (Solid-state detectors)
ID RESISTIVITY SILICON DETECTORS; N-EFF; SIMULATION
AB This paper presents design, fabrication and the first characterization of the new 3D stripixel detector. The device has dual-column electrodes (both n(+)- and p(+)-type) arranged in a quincunx configuration and processed in a single-sided process on n-type silicon bulk. Double-metal technology allows to connect the electrodes by two sets of perpendicular strips providing a X-Y projective read-out. The design of the sensor has been optimized with the use of TCAD Sentaurus simulations. TCT measurements were performed to study the active area of the detector. Finally, 2D position sensitivity was investigated reconstructing the position of a laser beam within a 80x80 mu m(2) pixel, defined by two neighbouring p(+)-type strips crossing two neighbouring n(+)-type strips.
C1 [Bassignana, D.; Lozano, M.; Pellegrini, G.; Quirion, D.] CSIC, CNM, IMB, Barcelona 08193, Spain.
[Li, Z.] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Tuuva, T.] Lappeenranta Univ, Lappeenranta 53850, Finland.
RP Pellegrini, G (reprint author), CSIC, CNM, IMB, Campus Univ Autonoma Barcelona, Barcelona 08193, Spain.
EM giulio.pellegrini@csic.es
RI Bassignana, Daniela/J-7266-2012; Quirion, David/K-7597-2014; Lozano,
Manuel/C-3445-2011; Pellegrini, Giulio/F-4921-2011
OI Bassignana, Daniela/0000-0001-7582-9161; Quirion,
David/0000-0002-5309-0535; Lozano, Manuel/0000-0001-5826-5544;
Pellegrini, Giulio/0000-0002-1606-3546
FU Spanish Ministry of Education and Science through Particle Physics
National Program [FPA2010-22060-C02-02, FPA2010-22163-C02-02]; GICSERV
program "Access to ICTS integrated nano-and micro electronics clean
room" of Spanish Ministry of Education and Science
FX This work has been financed by the Spanish Ministry of Education and
Science through the Particle Physics National Program
(FPA2010-22060-C02-02 and FPA2010-22163-C02-02) and through the GICSERV
program "Access to ICTS integrated nano-and micro electronics clean
room" of the same Ministry. This work was done in the framework of CERN
RD50 Radiation hard semiconductor devices for very high luminosity
colliders.
NR 13
TC 2
Z9 2
U1 0
U2 4
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 1748-0221
J9 J INSTRUM
JI J. Instrum.
PD AUG
PY 2013
VL 8
AR P08014
DI 10.1088/1748-0221/8/08/P08014
PG 18
WC Instruments & Instrumentation
SC Instruments & Instrumentation
GA 212XZ
UT WOS:000324017400019
ER
PT J
AU Shin, S
Kim, D
Hwang, I
Kim, M
Choi, J
Liu, G
Hou, J
Chunjarean, S
Kim, KR
Huang, J
Nam, S
AF Shin, S.
Kim, D.
Hwang, I.
Kim, M.
Choi, J.
Liu, G.
Hou, J.
Chunjarean, S.
Kim, K-R
Huang, J.
Nam, S.
TI Lattice design and beam dynamics studies for the PLS-II
SO JOURNAL OF INSTRUMENTATION
LA English
DT Article
DE Accelerator modelling and simulations (multi-particle dynamics;
single-particle dynamics); Beam dynamics; Accelerator Subsystems and
Technologies
AB Pohang Light Source (PLS) [1] had operated for 14 year successfully. To meet the request of the increasing user community, the PLS-II that is the upgrade project of PLS have been carried out. Main design goals of the PLS-II lattice are to increase beam energy to 3 GeV, to increase number of insertion devices by factor of two (20 IDs), to increase beam current to 400 mA and to reduce beam emittance below 10 nm with existing PLS tunnel and injection system. Following the desired design criteria, DBA lattice had been chosen such that the full storage ring includes 12 long straight sections and 12 short straight sections for installation of insertion devices with keeping beam emittance as small as possible. Through the six months of commissioning in the later half of 2011 and user operation in full period of 2012, we have successfully operated 14 insertion devices operation and top-up operation with 200 mA beam current and 5.8 nm beam emittance. It is especially important that good understanding of the machine operation and limitations can be achieved by comparison of experimental and simulation data during realizing final PLS-II goal and stable operation. Therefore, this paper describes the results of lattice design and beam dynamics studies for the PLS-II [2, 3].
C1 [Shin, S.; Kim, D.; Hwang, I.; Kim, M.; Kim, K-R; Huang, J.; Nam, S.] POSTECH, Pohang Accelerator Lab, Pohang 790784, Kyungbuk, South Korea.
[Choi, J.] Brookhaven Natl Lab, NSLS 2, Upton, NY 11973 USA.
[Liu, G.; Hou, J.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
[Chunjarean, S.] Chiang Mai Univ, Chiang Mai 50200, Thailand.
RP Shin, S (reprint author), POSTECH, Pohang Accelerator Lab, Pohang 790784, Kyungbuk, South Korea.
EM tlssh@postech.ac.kr
FU Converging Research Center Program through Ministry of Science, ICT and
Future Planning [2013K000306]
FX We thank Prof. Helmut Wiedemann (SLAC), W. Wan (ALS), M. Boege (SLS), L.
Nadolski (SOLEIL) and T. Shaftan (NSLS-II) for their graceful comments.
This research was supported by the Converging Research Center Program
through the Ministry of Science, ICT and Future Planning (2013K000306).
NR 11
TC 0
Z9 0
U1 1
U2 1
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 1748-0221
J9 J INSTRUM
JI J. Instrum.
PD AUG
PY 2013
VL 8
AR P08008
DI 10.1088/1748-0221/8/08/P08008
PG 23
WC Instruments & Instrumentation
SC Instruments & Instrumentation
GA 212XZ
UT WOS:000324017400013
ER
PT J
AU Tao, GH
Miller, WH
AF Tao, Guohua
Miller, William H.
TI Time-dependent importance sampling in semi-classical initial value
representation calculations for time correlation functions. III. A
state-resolved implementation to electronically non-adiabatic dynamics
SO MOLECULAR PHYSICS
LA English
DT Article
DE non-adiabatic; semi-classical (SC); time-dependent (TD); correlation
function
ID MOLECULAR-DYNAMICS; QUANTUM DYNAMICS
AB The recently developed time-dependent (TD) Monte Carlo (MC) importance sampling method [Tao and Miller; JCP 135, 024104 (2011)] provides an efficient implementation of the semi-classical (SC) initial value representation (IVR) methodology for the evaluation of time correlation functions. The key idea in this TD-SC-IVR method is to perform importance sampling of trajectories for the MC averages in the SC calculations with a sampling function that includes information about the final (time-evolved) values of the coordinates and momenta of trajectories in addition to (the usual) information of their initial values. This paper shows how this approach deals with electronically non-adiabatic dynamics, i.e. dynamics that involves coupled multiple electronic states. We suggest that a state-resolved sampling function may facilitate the efficient implementation of TD-SC-IVR for such processes. This is illustrated by application to the calculation of the nuclear momentum distribution function (i.e. the nuclear energy-loss spectrum) for a benchmark non-adiabatic scattering problem.
C1 [Tao, Guohua; Miller, William H.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Tao, Guohua; Miller, William H.] Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA.
[Tao, Guohua; Miller, William H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
RP Miller, WH (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
EM millerwh@berkeley.edu
FU National Science Foundation [CHE-1148645]; Office of Science, Office of
Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences
Division, U.S. Department of Energy [DE-AC02-05CH11231]
FX This work was supported by the National Science Foundation Grant No.
CHE-1148645 and by the Director, Office of Science, Office of Basic
Energy Sciences, Chemical Sciences, Geosciences, and Biosciences
Division, U.S. Department of Energy under Contract No.
DE-AC02-05CH11231. We also acknowledge a generous allocation of
supercomputing time from the National Energy Research Scientific
Computing Center (NERSC) and the use of the Lawrencium computational
cluster resource provided by the IT Division at the Lawrence Berkeley
National Laboratory.
NR 20
TC 5
Z9 5
U1 0
U2 8
PU TAYLOR & FRANCIS LTD
PI ABINGDON
PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND
SN 0026-8976
J9 MOL PHYS
JI Mol. Phys.
PD AUG 1
PY 2013
VL 111
IS 14-15
SI SI
BP 1987
EP 1993
DI 10.1080/00268976.2013.776712
PG 7
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 211BR
UT WOS:000323879600006
ER
PT J
AU von Lilienfeld, OA
AF von Lilienfeld, O. Anatole
TI Force correcting atom centred potentials for generalised gradient
approximated density functional theory: Approaching hybrid functional
accuracy for geometries and harmonic frequencies in small
chlorofluorocarbons
SO MOLECULAR PHYSICS
LA English
DT Article
DE vibrational spectroscopy; atom centered potentials; plane-wave and
pseudopotentials; high-performance computing
ID SPACE GAUSSIAN PSEUDOPOTENTIALS; DER-WAALS INTERACTIONS; CAPPING
POTENTIALS; 1ST PRINCIPLES; NONCOVALENT INTERACTIONS;
ELECTRONIC-STRUCTURE; MOLECULAR-PROPERTIES; LIQUID WATER; SOFT ACIDS;
AB-INITIO
AB Generalised gradient approximated (GGA) density functional theory (DFT) typically overestimates polarisability and bond-lengths, and underestimates force constants of covalent bonds. To overcome this problem we show that one can use empirical force correcting atom centred potentials (FCACPs), parametrised for every nuclear species. Parameters are obtained through minimisation of a penalty functional that explicitly encodes hybrid DFT forces and static polarisabilities of reference molecules. For hydrogen, fluorine, chlorine and carbon the respective reference molecules consist of H-2, F-2, Cl-2 and CH4. The transferability of this approach is assessed for harmonic frequencies in a small set of chlorofluorocarbon molecules. Numerical evidence, gathered for CF4, CCl4, CCl3F, CCl2F2, CClF3, ClF, HF, HCl, CFH3, CF2H2, CF3H, CHCl3, CH2Cl2 and CH3Cl indicates that the GGA+FCACP level of theory yields harmonic frequencies that are significantly more consistent with hybrid DFT values, as well as slightly reduced molecular polarisability.
C1 [von Lilienfeld, O. Anatole] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA.
[von Lilienfeld, O. Anatole] Univ Basel, Dept Chem, CH-4056 Basel, Switzerland.
RP von Lilienfeld, OA (reprint author), Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM anatole@alcf.anl.gov
RI von Lilienfeld, O. Anatole/D-8529-2011
FU Office of Science of the U.S. DOE [DE-AC02-06CH11357]
FX This article is dedicated to Prof. M. Quack, the author's Diplomvater at
ETH Zurich in 2001, and co-author of the resulting paper [14]. The
author is thankful for many technical discussions with P.J. Feibelman,
A. E. Mattsson and A. G. Taube at Sandia National Laboratories. This
research used resources of the Argonne Leadership Computing Facility at
Argonne National Laboratory, which is supported by the Office of Science
of the U.S. DOE under contract DE-AC02-06CH11357.
NR 77
TC 4
Z9 4
U1 0
U2 6
PU TAYLOR & FRANCIS LTD
PI ABINGDON
PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND
SN 0026-8976
J9 MOL PHYS
JI Mol. Phys.
PD AUG 1
PY 2013
VL 111
IS 14-15
SI SI
BP 2147
EP 2153
DI 10.1080/00268976.2013.793834
PG 7
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 211BR
UT WOS:000323879600024
ER
PT J
AU Pfeiffer, AN
Sayres, SG
Leone, SR
AF Pfeiffer, Adrian N.
Sayres, Scott G.
Leone, Stephen R.
TI Calculation of valence electron motion induced by sequential
strong-field ionisation
SO MOLECULAR PHYSICS
LA English
DT Article
DE sequential double ionisation; valence electron motion; circular
polarisation
ID ATOMS
AB Strong-field ionisation leads to the formation of electron wave packets in the valence shell of the resulting ion under appropriate experimental conditions. Ab-initio calculations of the population and coherence dynamics are challenging and are usually limited to single ionisation of simple systems by linearly polarised fields. Here, a calculation based on static-field rate equations is presented to obtain the density matrix for sequential double ionisation. The results for single ionisation of neon and xenon by linearly polarised pulses are in satisfactory agreement with ab-initio calculations. For double ionisation of neon and xenon by elliptically polarised fields, five coherence channels with recurrence times between 1.1 fs and 51.9 fs are predicted to exhibit a significant degree of coherence. The degree of coherence is affected by the polarisation of the laser pulse and decreases in general for elliptical polarisation, but for the investigated cases a significant degree of coherence is predicted to occur up to the regime of close-to-circular polarisation.
C1 [Pfeiffer, Adrian N.; Sayres, Scott G.; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Pfeiffer, Adrian N.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA.
RP Pfeiffer, AN (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
EM apfeiffer@lbl.gov
RI Pfeiffer, Adrian/J-7671-2016
FU Laboratory Directed Research and Development Program at Lawrence
Berkeley National Laboratory; National Science Foundation Chemistry
Division [CHE-1049946]; office of Science, office of Basic Energy
Sciences, of the US Department of Energy [DE-AC02-05CH11231]; National
Science Foundation Engineering Research Center for Extreme Ultraviolet
Science and Technology; W.M. Keck Foundation; Department of Defense
National Security Science and Engineering Faculty Fellowship
FX A.N.P. is supported by the Laboratory Directed Research and Development
Program at Lawrence Berkeley National Laboratory. S. G. S. is supported
by the National Science Foundation Chemistry Division CHE-1049946. S. R.
L. acknowledges additional support that contributed to the intellectual
content of this project: The Director, office of Science, office of
Basic Energy Sciences, of the US Department of Energy under Contract No.
DE-AC02-05CH11231; National Science Foundation Engineering Research
Center for Extreme Ultraviolet Science and Technology; W.M. Keck
Foundation; Department of Defense National Security Science and
Engineering Faculty Fellowship.
NR 28
TC 3
Z9 3
U1 3
U2 27
PU TAYLOR & FRANCIS LTD
PI ABINGDON
PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND
SN 0026-8976
J9 MOL PHYS
JI Mol. Phys.
PD AUG 1
PY 2013
VL 111
IS 14-15
SI SI
BP 2283
EP 2291
DI 10.1080/00268976.2013.801527
PG 9
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 211BR
UT WOS:000323879600037
ER
PT J
AU Pyka, K
Keller, J
Partner, HL
Nigmatullin, R
Burgermeister, T
Meier, DM
Kuhlmann, K
Retzker, A
Plenio, MB
Zurek, WH
del Campo, A
Mehlstaubler, TE
AF Pyka, K.
Keller, J.
Partner, H. L.
Nigmatullin, R.
Burgermeister, T.
Meier, D. M.
Kuhlmann, K.
Retzker, A.
Plenio, M. B.
Zurek, W. H.
del Campo, A.
Mehlstaeubler, T. E.
TI Topological defect formation and spontaneous symmetry breaking in ion
Coulomb crystals
SO NATURE COMMUNICATIONS
LA English
DT Article
ID TRAPPED IONS; LIQUID-CRYSTALS; TRANSITION; DYNAMICS
AB Symmetry breaking phase transitions play an important role in nature. When a system traverses such a transition at a finite rate, its causally disconnected regions choose the new broken symmetry state independently. Where such local choices are incompatible, topological defects can form. The Kibble-Zurek mechanism predicts the defect densities to follow a power law that scales with the rate of the transition. Owing to its ubiquitous nature, this theory finds application in a wide field of systems ranging from cosmology to condensed matter. Here we present the successful creation of defects in ion Coulomb crystals by a controlled quench of the confining potential, and observe an enhanced power law scaling in accordance with numerical simulations and recent predictions. This simple system with well-defined critical exponents opens up ways to investigate the physics of non-equilibrium dynamics from the classical to the quantum regime.
C1 [Pyka, K.; Keller, J.; Partner, H. L.; Burgermeister, T.; Meier, D. M.; Kuhlmann, K.; Mehlstaeubler, T. E.] Phys Tech Bundesanstalt, D-38116 Braunschweig, Germany.
[Nigmatullin, R.; Plenio, M. B.] Univ Ulm, Inst Theoret Phys, D-89069 Ulm, Germany.
[Nigmatullin, R.; Plenio, M. B.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England.
[Retzker, A.] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Givat Ram, Israel.
[Plenio, M. B.] Univ Ulm, Ctr Integrated Quantum Sci & Technol, D-89069 Ulm, Germany.
[Zurek, W. H.; del Campo, A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[del Campo, A.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.
RP Mehlstaubler, TE (reprint author), Phys Tech Bundesanstalt, Bundesallee 100, D-38116 Braunschweig, Germany.
EM tanja.mehlstaeubler@ptb.de
RI del Campo, Adolfo/B-8439-2009; Plenio, Martin/I-7895-2013;
OI del Campo, Adolfo/0000-0003-2219-2851; Nigmatullin,
Ramil/0000-0003-2577-6561; Keller, Jonas/0000-0002-3596-995X
FU NSF [PHY11-25915]; United States Department of Energy through the
LANL/LDRD Program; LANL J. Robert Oppenheimer fellowship; EU STREP PICC;
Alexander von Humboldt Foundation; Career Integration Grant (CIG)
[321798]; EPSRC; DFG through QUEST
FX We thank B. Damski and R. Rivers for suggestions and comments on the
manuscript, L. Yi for his contributions to the detection software, E.
Passemar for providing statistics codes and K. Thirumalai for assistance
in the lab. This work was supported by NSF PHY11-25915, the United
States Department of Energy through the LANL/LDRD Program and a LANL J.
Robert Oppenheimer fellowship (A.d.C.), the EU STREP PICC, the Alexander
von Humboldt Foundation (M.B.P.), Career Integration Grant (CIG) no.
321798 (A.R.), by EPSRC (R.N.) and by DFG through QUEST. A.d.C. and
W.H.Z. are grateful to KITP for hospitality.
NR 42
TC 78
Z9 78
U1 5
U2 29
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2291
DI 10.1038/ncomms3291
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209JN
UT WOS:000323752000007
PM 23921564
ER
PT J
AU Xu, WZ
Zhang, YF
Cheng, GM
Jian, WW
Millett, PC
Koch, CC
Mathaudhu, SN
Zhu, YT
AF Xu, Weizong
Zhang, Yongfeng
Cheng, Guangming
Jian, Weiwei
Millett, Paul C.
Koch, Carl C.
Mathaudhu, Suveen N.
Zhu, Yuntian
TI In-situ atomic-scale observation of irradiation-induced void formation
SO NATURE COMMUNICATIONS
LA English
DT Article
ID VOLTAGE ELECTRON-MICROSCOPE; NEUTRON-IRRADIATION; RADIATION-DAMAGE;
DISLOCATION LOOPS; GAS-BUBBLES; HCP METALS; NUCLEATION; EVOLUTION;
ZIRCONIUM; ALLOYS
AB The formation of voids in an irradiated material significantly degrades its physical and mechanical properties. Void nucleation and growth involve discrete atomic-scale processes that, unfortunately, are not yet well understood due to the lack of direct experimental examination. Here we report an in-situ atomic-scale observation of the nucleation and growth of voids in hexagonal close-packed magnesium under electron irradiation. The voids are found to first grow into a plate-like shape, followed by a gradual transition to a nearly equiaxial geometry. Using atomistic simulations, we show that the initial growth in length is controlled by slow nucleation kinetics of vacancy layers on basal facets and anisotropic vacancy diffusivity. The subsequent thickness growth is driven by thermodynamics to reduce surface energy. These experiments represent unprecedented resolution and characterization of void nucleation and growth under irradiation, and might help with understanding the irradiation damage of other hexagonal close-packed materials.
C1 [Xu, Weizong; Cheng, Guangming; Jian, Weiwei; Koch, Carl C.; Zhu, Yuntian] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA.
[Zhang, Yongfeng] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Millett, Paul C.] Univ Arkansas, Dept Mech Engn, Fayetteville, AR 72701 USA.
[Mathaudhu, Suveen N.] US Army, Res Off, Div Mat Sci, Res Triangle Pk, NC 27709 USA.
RP Zhu, YT (reprint author), N Carolina State Univ, Dept Mat Sci & Engn, Box 7907, Raleigh, NC 27695 USA.
EM ytzhu@ncsu.edu
RI Zhu, Yuntian/B-3021-2008; Cheng, Guangming/F-8999-2010; Mathaudhu,
Suveen/B-4192-2009; Xu, Weizong/G-3328-2014
OI Zhu, Yuntian/0000-0002-5961-7422; Cheng, Guangming/0000-0001-5852-1341;
Xu, Weizong/0000-0003-0030-8606
FU Laboratory Directed Research and Development Program Office of the Idaho
National Laboratory [00042959-00032]; US Army Research Office
[W911NF-12-1-0009]
FX We thank Dr M.-H. Tsai for constructive discussions. We acknowledge
financial support from the Laboratory Directed Research and Development
Program Office of the Idaho National Laboratory (00042959-00032), and US
Army Research Office (W911NF-12-1-0009).
NR 53
TC 17
Z9 17
U1 9
U2 89
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2288
DI 10.1038/ncomms3288
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209JN
UT WOS:000323752000004
PM 23912894
ER
PT J
AU Zhu, JH
Zhang, SY
Zhang, K
Wang, XJ
Mays, JW
Wooley, KL
Pochan, DJ
AF Zhu, Jiahua
Zhang, Shiyi
Zhang, Ke
Wang, Xiaojun
Mays, Jimmy W.
Wooley, Karen L.
Pochan, Darrin J.
TI Disk-cylinder and disk-sphere nanoparticles via a block copolymer blend
solution construction
SO NATURE COMMUNICATIONS
LA English
DT Article
ID MULTICOMPARTMENT MICELLES; DIBLOCK COPOLYMERS; INTRACELLULAR DELIVERY;
SOLUTION-STATE; ASSEMBLIES; POLYMERIZATION; MORPHOLOGY; CELLS; SHAPE
AB Researchers strive to produce nanoparticles with complexity in composition and structure. Although traditional spherical, cylindrical and membranous, or planar, nanostructures are ubiquitous, scientists seek more complicated geometries for potential functionality. Here we report the simple solution construction of multigeometry nanoparticles, disk-sphere and disk-cylinder, through a straightforward, molecular-level, blending strategy with binary mixtures of block copolymers. The multigeometry nanoparticles contain disk geometry in the core with either spherical patches along the disk periphery in the case of disk-sphere particles or cylindrical edges and handles in the case of the disk-cylinder particles. The portions of different geometry in the same nanoparticles contain different core block chemistry, thus also defining multicompartments in the nanoparticles. Although the block copolymers chosen for the blends are important for the definition of the final hybrid particles, the control of the kinetic pathway of assembly is critical for successful multigeometry particle construction.
C1 [Zhu, Jiahua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Zhang, Shiyi; Wooley, Karen L.] Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA.
[Zhang, Shiyi; Wooley, Karen L.] Texas A&M Univ, Dept Chem Engn, College Stn, TX 77843 USA.
[Zhang, Shiyi] Washington Univ, Dept Chem, St Louis, MO 63130 USA.
[Zhang, Ke] Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA.
[Wang, Xiaojun; Mays, Jimmy W.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
[Pochan, Darrin J.] Univ Delaware, Dept Mat Sci & Engn, Newark, DE 19716 USA.
RP Wooley, KL (reprint author), Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA.
EM wooley@chem.tamu.edu; pochan@udel.edu
RI Wooley, Karen/D-4399-2015; Zhu, Jiahua/F-3204-2012
OI Wooley, Karen/0000-0003-4086-384X; Zhu, Jiahua/0000-0003-2889-3421
FU National Science Foundation [DMR-0906815, DMR-1105304]; W.T.
Doherty-Welch Chair in Chemistry [A-0001]; Materials Science and
Engineering Division, US Department of Energy (DoE), Office of Basic
Energy Sciences (BES) [DEAC05-00OR22725]
FX This material is based upon work supported by the National Science
Foundation under Grants DMR-0906815 (D.J.P. and K.L.W.) and DMR-1105304
(K.L.W.) and the W.T. Doherty-Welch Chair in Chemistry, Grant No. A-0001
(K.L.W.). A portion of work was supported by the Materials Science and
Engineering Division, US Department of Energy (DoE), Office of Basic
Energy Sciences (BES) under Contract No. DEAC05-00OR22725. We thank the
Keck Electron Microscopy lab at University of Delaware, Professor
Chaoying Ni and Mr Frank Kriss for electron microscopy assistance. We
thank Mr Sameer Sathaye, Ms Yingchao Chen and Mr Ngoc Nguyen for the
atomic force microscopy assistance.
NR 38
TC 54
Z9 54
U1 11
U2 159
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2297
DI 10.1038/ncomms3297
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209JN
UT WOS:000323752000013
PM 23921650
ER
PT J
AU Sorenson, KB
Hanson, B
AF Sorenson, Ken B.
Hanson, Brady
TI MAKING THE CASE FOR SAFE STORAGE OF USED NUCLEAR FUEL FOR EXTENDED
PERIODS OF TIME: COMBINING NEAR-TERM EXPERIMENTS AND ANALYSES WITH
LONGER-TERM CONFIRMATORY DEMONSTRATIONS
SO NUCLEAR ENGINEERING AND TECHNOLOGY
LA English
DT Article
DE Used Nuclear Fuel; Extended Storage; High Burnup; Confirmatory
Demonstration
AB The need for extended storage of used nuclear fuel is increasing globally as disposition schedules for used fuel are pushed further into the future. This is creating a situation where dry storage of used fuel may need to be extended beyond normal regulatory licensing periods. While it is generally accepted that used fuel in dry storage will remain in a safe condition, there is little data that demonstrate used fuel performance in dry storage environments for long periods of time. This is especially true for high burnup used fuel. This paper discusses a technical approach that defines a process that develops the technical basis for demonstrating the safety of used fuel over extended periods of time.
C1 [Sorenson, Ken B.] Sandia Natl Labs, Adv Nucl Fuel Cycle Technol, Albuquerque, NM 87185 USA.
[Hanson, Brady] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Sorenson, KB (reprint author), Sandia Natl Labs, Adv Nucl Fuel Cycle Technol, Box 5800, Albuquerque, NM 87185 USA.
EM kbsoren@sandia.gov
NR 7
TC 3
Z9 3
U1 0
U2 8
PU KOREAN NUCLEAR SOC
PI DAEJEON
PA NUTOPIA BLDG, 342-1 JANGDAE-DONG, DAEJEON, 305-308, SOUTH KOREA
SN 1738-5733
J9 NUCL ENG TECHNOL
JI Nucl. Eng. Technol.
PD AUG
PY 2013
VL 45
IS 4
BP 421
EP 426
DI 10.5516/NET.06.2013.707
PG 6
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 215RC
UT WOS:000324227000001
ER
PT J
AU Chen, S
Baker, I
Frost, HJ
AF Chen, Si
Baker, Ian
Frost, Harold J.
TI Surface instability and mass transfer during the bonding of ice spheres
SO PHILOSOPHICAL MAGAZINE
LA English
DT Article
DE ice; X-ray topography; microstructural characterization
ID SCANNING-ELECTRON-MICROSCOPY; TEMPERATURE-GRADIENT METAMORPHISM; SNOW
CRYSTALS; DRY SNOW; MICROSTRUCTURAL EVOLUTION; ISOTHERMAL CONDITIONS;
AREA; GRAINS; COVER; MORPHOLOGY
AB The morphological changes occurring in a vertically aligned, one-dimensional ice sphere array under quasi-isothermal conditions were investigated as a geometrically simplified model of snow aggregates, in order to understand the mechanisms operating during the bonding of ice crystals. Time-lapse three-dimensional images of the specimen were obtained using computed X-ray micro-tomography, in order to characterize the time-dependent structural evolution of the specimen. Fine-scale structural features were examined immediately after the time-lapse observations using a scanning electron microscope equipped with a cryo-system. Porous necks between adjacent ice spheres were observed to develop via the growth of small protrusions on the surface of the ice spheres. The instability of the specimen surface, i.e. the initially smooth surface breaking down into small protrusions, was analysed using the model proposed by Mullins and Sekerka. The analysis indicates the strong influence of the wavelength of the protrusions on surface stability and the important role of vapour transfer during the bonding process of the ice spheres. The grain boundaries that formed between the protrusions and the small mass build-ups on the surfaces of the ice spheres provide evidence for grain boundary migration.
C1 [Chen, Si; Baker, Ian; Frost, Harold J.] Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA.
[Chen, Si] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Chen, S (reprint author), Dartmouth Coll, Thayer Sch Engn, 8000 Cummings Hall, Hanover, NH 03755 USA.
EM sichen@aps.anl.gov
FU US Army Research Office [51065-EV]
FX This work was supported by the US Army Research Office Contact 51065-EV.
The views and conclusions contained herein are those of the authors and
should not be interpreted as necessarily representing official policies,
either expressed or implied of the ARO or the US Government.
NR 47
TC 2
Z9 2
U1 1
U2 16
PU TAYLOR & FRANCIS LTD
PI ABINGDON
PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND
SN 1478-6435
EI 1478-6443
J9 PHILOS MAG
JI Philos. Mag.
PD AUG 1
PY 2013
VL 93
IS 23
BP 3177
EP 3193
DI 10.1080/14786435.2013.805274
PG 17
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering; Physics, Applied; Physics, Condensed Matter
SC Materials Science; Metallurgy & Metallurgical Engineering; Physics
GA 202XX
UT WOS:000323255300008
ER
PT J
AU Arrington, CL
McKay, KS
Baca, ED
Coleman, JJ
Colombe, Y
Finnegan, P
Hite, DA
Hollowell, AE
Jordens, R
Jost, JD
Leibfried, D
Rowen, AM
Warring, U
Weides, M
Wilson, AC
Wineland, DJ
Pappas, DP
AF Arrington, Christian L.
McKay, Kyle S.
Baca, Ehren D.
Coleman, Jonathan J.
Colombe, Yves
Finnegan, Patrick
Hite, Dustin A.
Hollowell, Andrew E.
Joerdens, Robert
Jost, John D.
Leibfried, Dietrich
Rowen, Adam M.
Warring, Ulrich
Weides, Martin
Wilson, Andrew C.
Wineland, David J.
Pappas, David P.
TI Micro-fabricated stylus ion trap
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID LITHOGRAPHY
AB An electroformed, three-dimensional stylus Paul trap was designed to confine a single atomic ion for use as a sensor to probe the electric-field noise of proximate surfaces. The trap was microfabricated with the UV-LIGA technique to reduce the distance of the ion from the surface of interest. We detail the fabrication process used to produce a 150 mu m tall stylus trap with feature sizes of 40 mu m. We confined single, laser-cooled, Mg-25(+) ions with lifetimes greater than 2 h above the stylus trap in an ultra-high-vacuum environment. After cooling a motional mode of the ion at 4 MHz close to its ground state (< n > = 0.34 +/- 0.07), the heating rate of the trap was measured with Raman side-band spectroscopy to be 387 +/- 15 quanta/s at an ion height of 62 mu m above the stylus electrodes. (C) 2013 AIP Publishing LLC.
C1 [Arrington, Christian L.; Baca, Ehren D.; Coleman, Jonathan J.; Finnegan, Patrick; Hollowell, Andrew E.; Rowen, Adam M.] Sandia Natl Labs, Albuquerque, NM 87123 USA.
[McKay, Kyle S.; Colombe, Yves; Hite, Dustin A.; Joerdens, Robert; Jost, John D.; Leibfried, Dietrich; Warring, Ulrich; Weides, Martin; Wilson, Andrew C.; Wineland, David J.; Pappas, David P.] NIST, Boulder, CO 80305 USA.
RP Arrington, CL (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA.
EM clarrin@sandia.gov; kyle.mckay@nist.gov
RI Weides, Martin/C-1470-2009;
OI Weides, Martin/0000-0002-2718-6795; Jordens, Robert/0000-0001-5333-0562
FU IARPA under ARO [DNI-017389]; ONR; NIST Quantum Information program
FX This work was supported by IARPA under ARO Contract No. DNI-017389, ONR,
and the NIST Quantum Information program.
NR 19
TC 7
Z9 7
U1 1
U2 22
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 085001
DI 10.1063/1.4817304
PG 6
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400052
PM 24007096
ER
PT J
AU Beer, SK
Lawson, SA
AF Beer, S. K.
Lawson, S. A.
TI Note: Thermal imaging enhancement algorithm for gas turbine aerothermal
characterization
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
AB An algorithm was developed to convert radiation intensity images acquired using a black and white CCD camera to thermal images without requiring knowledge of incident background radiation. This unique infrared (IR) thermography method was developed to determine aerothermal characteristics of advanced cooling concepts for gas turbine cooling application. Compared to IR imaging systems traditionally used for gas turbine temperature monitoring, the system developed for the current study is relatively inexpensive and does not require calibration with surface mounted thermocouples.
C1 [Beer, S. K.; Lawson, S. A.] US DOE, Off Sci & Technol, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
RP Beer, SK (reprint author), US DOE, Off Sci & Technol, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA.
FU U.S. Department of Energy (DOE) Postgraduate Research Program at the
National Energy Technology Laboratory
FX This research was supported in part by an appointment to the U.S.
Department of Energy (DOE) Postgraduate Research Program at the National
Energy Technology Laboratory administered by the Oak Ridge Institute for
Science and Education (ORISE).
NR 4
TC 0
Z9 0
U1 1
U2 6
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 086108
DI 10.1063/1.4819318
PG 3
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400084
PM 24007128
ER
PT J
AU Bolme, CA
Ramos, KJ
AF Bolme, C. A.
Ramos, K. J.
TI Line-imaging velocimetry for observing spatially heterogeneous
mechanical and chemical responses in plastic bonded explosives during
impact
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID INTERFEROMETER
AB A line-imaging velocity interferometer was implemented on a single-stage light gas gun to probe the spatial heterogeneity of mechanical response, chemical reaction, and initiation of detonation in explosives. The instrument is described in detail, and then data are presented on several shock-compressed materials to demonstrate the instrument performance on both homogeneous and heterogeneous samples. The noise floor of this diagnostic was determined to be 0.24 rad with a shot on elastically compressed sapphire. The diagnostic was then applied to two heterogeneous plastic bonded explosives: 3,3'-diaminoazoxyfurazan (DAAF) and PBX 9501, where significant spatial velocity heterogeneity was observed during the build up to detonation. In PBX 9501, the velocity heterogeneity was consistent with the explosive grain size, however in DAAF, we observed heterogeneity on a much larger length scale than the grain size that was similar to the imaging resolution of the instrument. (C) 2013 AIP Publishing LLC.
C1 [Bolme, C. A.; Ramos, K. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Bolme, CA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM cbolme@lanl.gov
OI Bolme, Cynthia/0000-0002-1880-271X
FU National Nuclear Security Administration Science Campaign 2 (High
Explosives Science); National Nuclear Security Administration of the
U.S. Department of Energy [DE-AC52-06NA25396]
FX The authors would like to thank Dr. Peter Celliers, Dr. David Erskine,
and Dr. Rick Gustavsen for participating in helpful discussion, Tim
Pierce, Adam Pacheco, and Ben Hollowell for their assistance in fielding
the experiments, and Elizabeth Francois for providing the DAAF PBX. This
work was performed at Los Alamos National Laboratory and was funded by
the National Nuclear Security Administration Science Campaign 2 (High
Explosives Science). Los Alamos National Laboratory is operated by Los
Alamos National Security, LLC, for the National Nuclear Security
Administration of the U.S. Department of Energy under Contract No.
DE-AC52-06NA25396.
NR 20
TC 4
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U1 2
U2 15
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 083903
DI 10.1063/1.4817307
PG 7
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400031
PM 24007075
ER
PT J
AU Feng, J
Nasiatka, J
Wong, J
Chen, XM
Hidalgo, S
Vecchione, T
Zhu, H
Palomares, FJ
Padmore, HA
AF Feng, Jun
Nasiatka, J.
Wong, Jared
Chen, Xumin
Hidalgo, Sergio
Vecchione, T.
Zhu, H.
Javier Palomares, F.
Padmore, H. A.
TI A stigmatic ultraviolet-visible monochromator for use with a high
brightness laser driven plasma light source
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID CZERNY-TURNER SPECTROMETER; ASTIGMATISM; SPECTROGRAPH
AB Laser driven plasma light sources offer highly intense output in the UV-visible region combined with a source size as small as 100 mu m. In order to effectively use the small source size in high brightness applications, a stigmatic monochromator and focusing system must be used. Here we describe a simple brightness preserving optical system that should be useful across a broad range of applications. The output flux of this system is between 6 x 10(11) ph/s and 4 x 10(12) ph/s with a spectra resolution of 1.7 nm and field spot size of 0.1 mm from the UV to the VIS spectra range. (C) 2013 AIP Publishing LLC.
C1 [Feng, Jun; Nasiatka, J.; Wong, Jared; Chen, Xumin; Hidalgo, Sergio; Padmore, H. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Vecchione, T.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA.
[Zhu, H.] Energetiq Technol Inc, Woburn, MA 01801 USA.
[Javier Palomares, F.] Inst Ciencia Mat Madrid CSIC, Madrid 28049, Spain.
RP Feng, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RI Palomares, Francisco Javier/C-4605-2011
OI Palomares, Francisco Javier/0000-0002-4768-2219
FU Office of Science, Office of Basic Energy Sciences, of the U.S.
Department of Energy [DE-AC02-05CH11231]; Spanish MINECO [MAT2010-18432,
Consolider FUNCOAT CSD-2008-0023]
FX This work was performed at Lawrence Berkeley National Laboratory under
the auspices of the Office of Science, Office of Basic Energy Sciences,
of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231.
F.J.P. thanks the financial support from the Spanish MINECO (grants
MAT2010-18432 and Consolider FUNCOAT CSD-2008-0023).
NR 16
TC 5
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U1 2
U2 12
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 085114
DI 10.1063/1.4817587
PG 6
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400070
PM 24007114
ER
PT J
AU Jones, AM
Kelly, JF
Severtsen, RH
McCloy, JS
AF Jones, A. Mark
Kelly, James F.
Severtsen, Ronald H.
McCloy, John S.
TI Regenerative feedback resonant circuit to detect transient changes in
electromagnetic properties of semi-insulating materials
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID DEEP-LEVEL SPECTROSCOPY; REFRACTIVE-INDEX CHANGE; PHASE-NOISE;
SILICON-WAFERS; PHOTOCONDUCTIVITY MEASUREMENTS; MICROWAVE-OSCILLATORS;
LIFETIME MEASUREMENT; LOSS TANGENT; SEMICONDUCTORS; RESISTIVITY
AB A prototype regenerative feedback resonant circuit has been developed for measuring the transient spectral response due to perturbations in properties of various electromagnetic materials. The circuit can accommodate a variety of cavity resonators, shown here in the 8 GHz range, with passive quality factors (Q(stat)) as high as 7000 depending upon material loading. The positive feedback enhanced dynamic quality factors (Q(dyn)) of resonator/material combinations in the regenerative circuit are on the order of 107-108. The theory, design, and implementation of the circuit is discussed along with real-time monitored example measurements of effects due to photon-induced charge carriers in high-resistivity silicon wafers and magnetic-field induced perturbations of yttrium-iron garnet. (C) 2013 AIP Publishing LLC.
C1 [Jones, A. Mark; Kelly, James F.; Severtsen, Ronald H.; McCloy, John S.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP McCloy, JS (reprint author), Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA.
EM john.mccloy@wsu.edu
RI McCloy, John/D-3630-2013
OI McCloy, John/0000-0001-7476-7771
FU Defense Threat Reduction Agency IACRO [11-4485I]; Laboratory Directed
Research and Development; U.S. Department of Energy (DOE)
[DE-AC05-76RL01830]
FX This work was supported in part by the Defense Threat Reduction Agency
IACRO 11-4485I and in part by Laboratory Directed Research and
Development. Pacific Northwest National Laboratory is operated for the
U.S. Department of Energy (DOE) by Battelle under Contract NO.
DE-AC05-76RL01830. The authors thank Justin Fernandes and Jonathan
Tedeschi for their assistance with some of the measurements.
NR 59
TC 4
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U1 1
U2 3
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 084703
DI 10.1063/1.4817537
PG 11
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400040
PM 24007084
ER
PT J
AU Mortensen, DR
Seidler, GT
Bradley, JA
Lipp, MJ
Evans, WJ
Chow, P
Xiao, YM
Boman, G
Bowden, ME
AF Mortensen, D. R.
Seidler, G. T.
Bradley, J. A.
Lipp, M. J.
Evans, W. J.
Chow, P.
Xiao, Y. -M.
Boman, G.
Bowden, M. E.
TI A versatile medium-resolution x-ray emission spectrometer for diamond
anvil cell applications
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID ELECTRONIC EXCITATIONS; HIGH-PRESSURE; SCATTERING; SPECTROSCOPY
AB We present design and performance details for a polycapillary-coupled x-ray spectrometer that provides very high collection efficiency at a moderate energy resolution suitable for many studies of nonresonant x-ray emission spectroscopy, especially for samples of heavy elements under high pressures. Using a single Bragg analyzer operating close to backscattering geometry so as to minimize the effect of the weak divergence of the quasicollimated exit beam from the polycapillary optic, this instrument can maintain a typical energy resolution of 5 eV over photon energies from 5 keV to 10 keV. We find dramatically improved count rates as compared to a traditional higher-resolution instrument based on a single spherically bent crystal analyzer. (C) 2013 AIP Publishing LLC.
C1 [Mortensen, D. R.; Seidler, G. T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA.
[Bradley, J. A.; Lipp, M. J.; Evans, W. J.] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA.
[Chow, P.; Xiao, Y. -M.; Boman, G.] Carnegie Inst Sci, HPCAT, Argonne, IL 60439 USA.
[Bowden, M. E.] Pacific NW Natl Lab, Richland, WA 99354 USA.
RP Seidler, GT (reprint author), Univ Washington, Dept Phys, Seattle, WA 98195 USA.
EM seidler@uw.edu
FU US Department of Energy, Basic Energy Sciences [DE-FG02-09ER16106];
DOE-NNSA [DE-NA0001974]; DOE-BES [DE-FG02-99ER45775, DE-AC02-06CH11357];
National Science Foundation (NSF); LDRD at LLNL under US Department of
Energy by Lawrence Livermore National Laboratory [12-LW-014,
DE-AC52-07NA27344]; Chemical Imaging Initiative at PNNL
FX G.T.S. acknowledges support of this research program by the US
Department of Energy, Basic Energy Sciences, under Award No.
DE-FG02-09ER16106. HPCAT operations are supported by DOE-NNSA under
Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775,
with partial instrumentation funding by National Science Foundation
(NSF). APS is supported by DOE-BES, under Contract No.
DE-AC02-06CH11357. Part of this work was supported by the LDRD 12-LW-014
at LLNL and performed under the auspices of the US Department of Energy
by Lawrence Livermore National Laboratory under Contract No.
DE-AC52-07NA27344. Additional support was provided by the Chemical
Imaging Initiative at PNNL, operated by Battelle for the US Department
of Energy.
NR 25
TC 4
Z9 4
U1 1
U2 13
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 083908
DI 10.1063/1.4819257
PG 4
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400036
PM 24007080
ER
PT J
AU Siddiqui, SF
Knipe, K
Manero, A
Meid, C
Wischek, J
Okasinski, J
Almer, J
Karlsson, AM
Bartsch, M
Raghavan, S
AF Siddiqui, Sanna F.
Knipe, Kevin
Manero, Albert
Meid, Carla
Wischek, Janine
Okasinski, John
Almer, Jonathan
Karlsson, Anette M.
Bartsch, Marion
Raghavan, Seetha
TI Synchrotron X-ray measurement techniques for thermal barrier coated
cylindrical samples under thermal gradients
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID FATIGUE CRACKS; COATINGS; STRAIN; CREEP
AB Measurement techniques to obtain accurate in situ synchrotron strain measurements of thermal barrier coating systems (TBCs) applied to hollow cylindrical specimens are presented in this work. The Electron Beam Physical Vapor Deposition coated specimens with internal cooling were designed to achieve realistic temperature gradients over the TBC coated material such as that occurring in the turbine blades of aeroengines. Effects of the circular cross section on the x-ray diffraction (XRD) measurements in the various layers, including the thermally grown oxide, are investigated using high-energy synchrotron x-rays. Multiple approaches for beam penetration including collection, tangential, and normal to the layers, along with variations in collection parameters are compared for their ability to attain high-resolution XRD data from the internal layers. This study displays the ability to monitor in situ, the response of the internal layers within the TBC, while implementing a thermal gradient across the thickness of the coated sample. The thermal setup maintained coating surface temperatures in the range of operating conditions, while monitoring the substrate cooling, for a controlled thermal gradient. Through variation in measurement location and beam parameters, sufficient intensities are obtained from the internal layers which can be used for depth resolved strain measurements. Results are used to establish the various techniques for obtaining XRD measurements through multi-layered coating systems and their outcomes will pave the way towards goals in achieving realistic in situ testing of these coatings. (C) 2013 AIP Publishing LLC.
C1 [Siddiqui, Sanna F.; Knipe, Kevin; Manero, Albert; Raghavan, Seetha] Univ Cent Florida, Dept Mech & Aerosp Engn, Orlando, FL 32816 USA.
[Meid, Carla; Wischek, Janine; Bartsch, Marion] German Aerosp Ctr DLR, Inst Mat Res, D-51147 Cologne, Germany.
[Okasinski, John; Almer, Jonathan] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA.
[Karlsson, Anette M.] Cleveland State Univ, Cleveland, OH 44115 USA.
RP Siddiqui, SF (reprint author), Univ Cent Florida, Dept Mech & Aerosp Engn, Orlando, FL 32816 USA.
EM seetha.raghavan@ucf.edu
RI Bartsch, Marion/B-9501-2012
OI Bartsch, Marion/0000-0002-3952-2928
FU National Science Foundation [OISE 1157619, CMMI 1125696, 1144246];
German Science Foundation (DFG) [SFB-TRR103]; U.S. DOE
[DE-AC02-06CH11357]
FX This material is based upon work supported by the National Science
Foundation grants (Grant Nos. OISE 1157619 and CMMI 1125696) and by the
German Science Foundation (DFG) grant (Grant No. SFB-TRR103), Project
A3. This material is additionally based upon work supported by the
National Science Foundation Graduate Research Fellowship Program under
Grant No. 1144246 awarded to Sanna F. Siddiqui. Use of the Advanced
Photon Source, an Office of Science User Facility operated for the U.S.
Department of Energy (DOE) Office of Science by Argonne National
Laboratory, was supported by the U.S. DOE under Contract No.
DE-AC02-06CH11357.
NR 15
TC 5
Z9 5
U1 1
U2 16
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 083904
DI 10.1063/1.4817543
PG 7
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400032
PM 24007076
ER
PT J
AU Stoschus, H
Thomas, DM
Hudson, B
Watkins, M
Finkenthal, DF
Moyer, RA
Osborne, TH
AF Stoschus, H.
Thomas, D. M.
Hudson, B.
Watkins, M.
Finkenthal, D. F.
Moyer, R. A.
Osborne, T. H.
TI Status and characterization of the lithium beam diagnostic on DIII-D
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID ARBITRARY COLLISIONALITY; BOOTSTRAP CURRENT; TOKAMAKS; PLASMAS; LI
AB The 30 keV lithium beam diagnostic on DIII-D is suitable to measure both the radial electron density and poloidal magnetic field profiles in the pedestal. The refurbished system features a new setup to measure the Doppler shift allowing accurate alignment of the spectral filters. The injector has been optimized to generate a stable lithium neutral beam with a current of I = 15-20mA and a diameter of 1.9 +/- 0.1 cm measured by beam imaging. The typical temporal resolution is Delta t = 1-10 ms and the radial resolution of Delta R = 5mm is given by the optical setup. A new analysis technique based on fast Fourier transform avoids systematic error contributions from the digital lock-in analysis and accounts intrinsically for background light correction. Latest upgrades and a detailed characterization of the system are presented. Proof-of-principle measurements of the poloidal magnetic field with a statistical error of typically 2% show a fair agreement with the predictions modeled with the Grad-Shafranov equilibrium solver EFIT within 4%. (C) 2013 AIP Publishing LLC.
C1 [Stoschus, H.; Hudson, B.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA.
[Thomas, D. M.; Watkins, M.; Osborne, T. H.] Gen Atom Co, San Diego, CA 92186 USA.
[Finkenthal, D. F.] Palomar Coll, San Marcos, CA 92069 USA.
[Moyer, R. A.] Univ Calif San Diego, La Jolla, CA 92093 USA.
RP Stoschus, H (reprint author), Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA.
EM stoschus@fusion.gat.com
FU U.S. Department of Energy [DE-AC05-06OR23100, DE-FC02-04ER54698,
DE-FG02-07ER54917]
FX This work was supported in part by the U.S. Department of Energy under
DE-AC05-06OR23100, DE-FC02-04ER54698, and DE-FG02-07ER54917. The authors
acknowledge greatly N. H. Brooks, A. G. McLean, A. W. Leonard, R. L.
Boivin, and the DIII-D team.
NR 24
TC 2
Z9 2
U1 0
U2 8
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 083503
DI 10.1063/1.4816824
PG 7
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400016
PM 24007061
ER
PT J
AU Xu, GY
Xu, ZJ
Tranquada, JM
AF Xu, Guangyong
Xu, Zhijun
Tranquada, J. M.
TI Absolute cross-section normalization of magnetic neutron scattering data
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
AB We discuss various methods to obtain the resolution volume for neutron scattering experiments, in order to perform absolute normalization on inelastic magnetic neutron scattering data. Examples from previous experiments are given. We also try to provide clear definitions of a number of physical quantities which are commonly used to describe neutron magnetic scattering results, including the dynamic spin correlation function and the imaginary part of the dynamic susceptibility. Formulas that can be used for general purposes are provided and the advantages of the different normalization processes are discussed. (C) 2013 AIP Publishing LLC.
C1 [Xu, Guangyong; Xu, Zhijun; Tranquada, J. M.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
RP Xu, GY (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
RI xu, zhijun/A-3264-2013; Tranquada, John/A-9832-2009; Xu,
Guangyong/A-8707-2010; BL18, ARCS/A-3000-2012
OI xu, zhijun/0000-0001-7486-2015; Tranquada, John/0000-0003-4984-8857; Xu,
Guangyong/0000-0003-1441-8275;
FU Office of Basic Energy Sciences, U.S. Department of Energy (DOE)
[DE-AC02-98CH10886]
FX We would like to thank S. M. Shapiro and I. Zaliznyak for useful
discussions. Technical support from instrument scientists M. Stone, D.
Singh, and Y. Zhao is also gratefully acknowledged. Financial support by
Office of Basic Energy Sciences, U.S. Department of Energy (DOE) under
Contract No. DE-AC02-98CH10886 is acknowledged.
NR 9
TC 17
Z9 17
U1 1
U2 11
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2013
VL 84
IS 8
AR 083906
DI 10.1063/1.4818323
PG 5
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA 211YC
UT WOS:000323947400034
PM 24007078
ER
PT J
AU Lumsdaine, A
AF Lumsdaine, Arnold
TI PREFACE
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Editorial Material
C1 Oak Ridge Natl Lab, Oak Ridge, TN USA.
RP Lumsdaine, A (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN USA.
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP V
EP V
PG 1
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200001
ER
PT J
AU Fischer, CR
Bowen, BP
Pan, CL
Northen, TR
Banfield, JF
AF Fischer, Curt R.
Bowen, Benjamin P.
Pan, Chongle
Northen, Trent R.
Banfield, Jillian F.
TI Stable-Isotope Probing Reveals That Hydrogen Isotope Fractionation in
Proteins and Lipids in a Microbial Community Are Different and
Species-Specific
SO ACS CHEMICAL BIOLOGY
LA English
DT Article
ID ACID-MINE DRAINAGE; FATTY-ACIDS; PROTEOMICS; BACTERIA; GROWTH;
DISTRIBUTIONS; REQUIREMENT; VARIABILITY; GENOMES
AB The fractionation of hydrogen stable isotopes during lipid biosynthesis is larger in autotrophic than in heterotrophic microorganisms, possibly due to selective incorporation of hydrogen from water into NAD(P)H, resulting in D-depleted lipids. An analogous fractionation should occur during amino acid biosynthesis. Whereas these effects are traditionally measured using gas-phase isotope ratio on 1H-1H and 1H-2H, using an electrospray mass spectrometry-based technique on the original biomolecular structure and fitting of isotopic patterns we measured the hydrogen isotope compositions of proteins from an acidophilic microbial community with organism specificity and compared values with those for lipids. We showed that lipids were isotopically light by -260 parts per thousand relative to water in the growth solution; alternatively protein isotopic composition averaged -370 parts per thousand. This difference suggests that steps in addition to NAD(P)H formation contribute to D/H fractionation. Further, autotrophic bacteria sharing 94% 16S rRNA gene sequence identity displayed statistically significant differences in protein hydrogen isotope fractionation, suggesting different metabolic traits consistent with distinct ecological niches or incorrectly annotated gene function. In addition, it was found that heterotrophic, archaeal members of the community had isotopically light protein (-323 parts per thousand) relative to growth water and were significantly different from coexisting bacteria. This could be attributed to metabolite transfer from autotrophs and unknown aspects of fractionation associated with iron reduction. Differential fractionation of hydrogen stable isotopes into metabolites and proteins may reveal trophic levels of members of microbial communities. The approach developed here provided insights into the metabolic characteristics of organisms in natural communities and may be applied to analyze other systems.
C1 [Fischer, Curt R.; Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.
[Banfield, Jillian F.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA.
[Bowen, Benjamin P.; Northen, Trent R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
[Pan, Chongle] Oak Ridge Natl Lab, BioSci Div, Oak Ridge, TN 37831 USA.
[Pan, Chongle] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.
RP Banfield, JF (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.
EM jbanfield@berkeley.edu
OI Northen, Trent/0000-0001-8404-3259
FU U.S. Department of Energy, Office of Biological and Environmental
Research Carbon-Cycling Program [DE-SC0004665]; DOE Genomics:GTL Program
[DE-FG02-05ER64134]; ENIGMA Scientific Focus Area [DE-AC02-05CH11231]
FX This research was funded by the U.S. Department of Energy, Office of
Biological and Environmental Research Carbon-Cycling Program
(DE-SC0004665), the DOE Genomics:GTL Program grant number
DE-FG02-05ER64134 and ENIGMA Scientific Focus Area No.
DE-AC02-05CH11231. The authors thank Banfield lab members for assistance
with biofilm sampling in the field, and JM Hayes for valuable technical
discussions.
NR 31
TC 6
Z9 6
U1 1
U2 36
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1554-8929
J9 ACS CHEM BIOL
JI ACS Chem. Biol.
PD AUG
PY 2013
VL 8
IS 8
BP 1755
EP 1763
DI 10.1021/cb400210q
PG 9
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 204KA
UT WOS:000323363000015
PM 23713674
ER
PT J
AU Bagriantsev, SN
Ang, KH
Gallardo-Godoy, A
Clark, KA
Arkin, MR
Renslo, AR
Minor, DL
AF Bagriantsev, Sviatoslav N.
Ang, Kean-Hooi
Gallardo-Godoy, Alejandra
Clark, Kimberly A.
Arkin, Michelle R.
Renslo, Adam R.
Minor, Daniel L., Jr.
TI A High-Throughput Functional Screen Identifies Small Molecule Regulators
of Temperature- and Mechano-Sensitive K-2P Channels
SO ACS CHEMICAL BIOLOGY
LA English
DT Article
ID DOMAIN K+ CHANNELS; POTASSIUM CHANNELS; SACCHAROMYCES-CEREVISIAE;
TREK-1; PORE; INHIBITION; TRAAK; YEAST; BLOCK; SELECTIVITY
AB K-2P (KCNK) potassium channels generate "leak" potassium currents that strongly influence cellular excitability and contribute to pain, somatosensation, anesthesia, and mood. Despite their physiological importance, K(2P)s lack specific pharmacology. Addressing this issue has been complicated by the challenges that the leak nature of K-2P currents poses for electrophysiology-based high-throughput screening strategies. Here, we present a yeast-based high-throughput screening assay that avoids this problem. Using a simple growth-based functional readout, we screened a library of 106,281 small molecules and identified two new inhibitors and three new activators of the mammalian K-2P channel K(2P)2.1 (KCNK2, TREK-1). By combining biophysical, structure-activity, and mechanistic analysis, we developed a dihydroacridine analogue, ML67-33, that acts as a low micromolar, selective activator of temperature- and mechano-sensitive K-2P channels. Biophysical studies show that ML67-33 reversibly increases channel currents by activating the extracellular selectivity filter-based C-type gate that forms the core gating apparatus on which a variety of diverse modulatory inputs converge. The new K-2P modulators presented here, together with the yeast-based assay, should enable both mechanistic and physiological studies of K-2P activity and facilitate the discovery and development of other K-2P small molecule modulators.
C1 [Bagriantsev, Sviatoslav N.; Clark, Kimberly A.; Minor, Daniel L., Jr.] Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 94158 USA.
[Ang, Kean-Hooi; Gallardo-Godoy, Alejandra; Arkin, Michelle R.; Renslo, Adam R.] Univ Calif San Francisco, Small Mol Discovery Ctr, San Francisco, CA 94158 USA.
[Ang, Kean-Hooi; Gallardo-Godoy, Alejandra; Arkin, Michelle R.; Renslo, Adam R.] Univ Calif San Francisco, Dept Pharmaceut Chem, San Francisco, CA 94158 USA.
[Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA.
[Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Cellular & Mol Pharmacol, San Francisco, CA 94158 USA.
[Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, San Francisco, CA 94158 USA.
[Minor, Daniel L., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
RP Minor, DL (reprint author), Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 94158 USA.
EM daniel.minor@ucsf.edu
RI Gallardo-Godoy, Alejandra/E-7870-2013;
OI Bagriantsev, Sviatoslav/0000-0002-6661-3403; Renslo,
Adam/0000-0002-1240-2846
FU NIH [R01-MH093603]; American Heart Association [0740019N]; Life Sciences
Research Foundation
FX This work was supported by grants to D.L.M. from NIH R01-MH093603 and
American Heart Association 0740019N and to S.N.B. from the Life Sciences
Research Foundation. D.L.M. is an AHA Established Investigator. We thank
E. Gracheva and Minor lab members for comments on the manuscript. S.N.B.
is a Genentech Fellow of the Life Sciences Research Foundation.
NR 50
TC 23
Z9 23
U1 2
U2 12
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1554-8929
J9 ACS CHEM BIOL
JI ACS Chem. Biol.
PD AUG
PY 2013
VL 8
IS 8
BP 1841
EP 1851
DI 10.1021/cb400289x
PG 11
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 204KA
UT WOS:000323363000024
PM 23738709
ER
PT J
AU Scheele, M
Engel, JH
Ferry, VE
Hanifi, D
Liu, Y
Alivisatos, AP
AF Scheele, Marcus
Engel, Jesse H.
Ferry, Vivian E.
Hanifi, David
Liu, Yi
Alivisatos, A. Paul
TI Nonmonotonic Size Dependence in the Hole Mobility of
Methoxide-Stabilized PbSe Quantum Dot Solids
SO ACS NANO
LA English
DT Article
DE quantum dot solids; electrical transport; optical properties; coupling
ID ELECTRICAL-PROPERTIES; NANOCRYSTAL ARRAYS; CHARGE-TRANSPORT; FILMS;
LIGANDS; ENERGY
AB We present a facile procedure to fabricate p-type PbSe-based quantum dot solids with mobilities as large as 0.3 cm(2) V-1 s(-1). Upon partial ligand exchange of oleate-capped PbSe quantum dots with the methoxide ion, we observe a pronounced red shift in the excitonic transition in conjunction with a large increase in conductivity. We show that there is little correlation between these two phenomena and that the electronic coupling energy in PbSe quantum dot solids is much smaller than often assumed. However, we observe for the Hist time a nonmonotonic size dependence of the hole mobility, illustrating that coupling can nonetheless be dominant in determining the transport characteristics. We attribute these effects to a decrease in charging energy and interparticle spacing leading to enhanced electronic coupling on one hand and enhanced dipole interactions on the other hand, which is held responsible for the majority of the red shift.
C1 [Scheele, Marcus; Engel, Jesse H.; Ferry, Vivian E.; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Scheele, Marcus; Engel, Jesse H.; Ferry, Vivian E.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Hanifi, David; Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM alivis@berkeley.edu
RI Foundry, Molecular/G-9968-2014; Alivisatos , Paul /N-8863-2015
OI Alivisatos , Paul /0000-0001-6895-9048
FU Self-Assembly of Organic/Inorganic Nanocomposite Materials program
[DE-AC02-05CH11231]; Director, Office of Science, Office of Basic Energy
Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]
FX Nanoparticle synthesis and characterization, ligand exchange, sample
preparation, and transport measurements were funded by the Self-Assembly
of Organic/Inorganic Nanocomposite Materials program (Grant
DE-AC02-05CH11231 to A.P.A), photoelectron spectroscopy experiments were
carried out within the Helios Solar Energy Research Center, and FT-IR
spectroscopy was performed as a User Project at the Molecular Foundry,
Lawrence Berkeley National Laboratory, all of which are supported by the
Director, Office of Science, Office of Basic Energy Sciences of the U.S.
Department of Energy under Contract No. DE-AC02-05CH11231. MS. would
like to thank the Alexander von Humboldt Foundation for a Feodor Lynen
Fellowship. David K. Britt is acknowledged for providing the 5.3 nm
nanoparticle sample and Waqas Khalid for fabricating the FET substrates
used in this work.
NR 36
TC 15
Z9 15
U1 3
U2 48
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD AUG
PY 2013
VL 7
IS 8
BP 6774
EP 6781
DI 10.1021/nn401657n
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 210DX
UT WOS:000323810600036
PM 23859499
ER
PT J
AU Strelcov, E
Jesse, S
Huang, YL
Teng, YC
Kravchenko, II
Chu, YH
Kalinin, SV
AF Strelcov, Evgheni
Jesse, Stephen
Huang, Yen-Lin
Teng, Yung-Chun
Kravchenko, Ivan I.
Chu, Ying-Hao
Kalinin, Sergei V.
TI Space- and Time-Resolved Mapping of Ionic Dynamic and Electroresistive
Phenomena in Lateral Devices
SO ACS NANO
LA English
DT Article
DE KPFM; ionic dynamics; Ca-BFO; surface potential distribution; oxygen
vacancy
ID ATOMIC-FORCE MICROSCOPY; KELVIN PROBE MICROSCOPY; SCANNING IMPEDANCE
MICROSCOPY; ELECTRIC-FIELD; OXIDE; SURFACE; SEMICONDUCTOR; RESOLUTION;
CHALLENGES; BATTERIES
AB A scanning probe microscopy-based technique for probing local ionic and electronic transport and their dynamic behavior on the 10 ms to 10 s scale is presented. The time-resolved Kelvin probe force microscopy (tr-KPFM) allows mapping of surface potential in both space and time domains, visualizing electronic and ionic charge dynamics and separating underlying processes based on their time responses. Here, tr-KPFM is employed to explore the interplay of the adsorbed surface ions and bulk oxygen vacancies and their role in the resistive switching in a Ca-substituted bismuth ferrite thin film.
C1 [Strelcov, Evgheni; Jesse, Stephen; Kravchenko, Ivan I.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Huang, Yen-Lin; Teng, Yung-Chun; Chu, Ying-Hao] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan.
RP Strelcov, E (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM strelcove@ornl.gov; sergei2@ornl.gov
RI Ying-Hao, Chu/A-4204-2008; Strelcov, Evgheni/H-1654-2013; Kravchenko,
Ivan/K-3022-2015; Kalinin, Sergei/I-9096-2012; Jesse,
Stephen/D-3975-2016
OI Ying-Hao, Chu/0000-0002-3435-9084; Kravchenko, Ivan/0000-0003-4999-5822;
Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483
FU Scientific User Facilities Division, Office of Basic Energy Sciences,
U.S. Department of Energy at Oak Ridge National Laboratory; National
Science Council of Republic of China [NSC-101-2119-M-009-003-MY2];
Ministry of Education [MOE-ATU 101W961]; Center for Interdisciplinary
Science at National Chiao Tung University
FX This research was conducted at the Center for Nanophase Materials
Sciences, which is sponsored at Oak Ridge National Laboratory by the
Scientific User Facilities Division, Office of Basic Energy Sciences,
U.S. Department of Energy. The work in National Chiao Tung University
was supported by the National Science Council of Republic of China
(under Contract No. NSC-101-2119-M-009-003-MY2), Ministry of Education
(Grant No. MOE-ATU 101W961), and Center for Interdisciplinary Science at
National Chiao Tung University.
NR 75
TC 11
Z9 11
U1 3
U2 89
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD AUG
PY 2013
VL 7
IS 8
BP 6806
EP 6815
DI 10.1021/nn4017873
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 210DX
UT WOS:000323810600039
PM 23837694
ER
PT J
AU Kodali, V
Littke, MH
Tilton, SC
Teeguarden, JG
Shi, L
Frevert, CW
Wang, W
Pounds, JG
Thrall, BD
AF Kodali, Vamsi
Littke, Matthew H.
Tilton, Susan C.
Teeguarden, Justin G.
Shi, Liang
Frevert, Charles W.
Wang, Wei
Pounds, Joel G.
Thrall, Brian D.
TI Dysregulation of Macrophage Activation Profiles by Engineered
Nanoparticles
SO ACS NANO
LA English
DT Article
DE nanotoxicology; macrophage; iron oxide; amorphous silica; Streptococcus
pneumoniae; lipopolysaccharide; scavenger receptor
ID SCAVENGER RECEPTOR CD204; AIR-POLLUTION; INFLAMMATORY RESPONSE; CLASS-A;
STREPTOCOCCUS-PNEUMONIAE; ALVEOLAR MACROPHAGES; SILICA NANOPARTICLES;
HOSPITAL ADMISSIONS; AMORPHOUS SILICA; GENE-EXPRESSION
AB Although the potential human health impacts from exposure to engineered nanoparticles (ENPs) are uncertain, past epidemiological studies have established correlations between exposure to ambient air pollution particulates and the incidence of pneumonia and lung infections. Using amorphous silica and superparamagnetic iron oxide (SPIO) as model high production volume ENPs, we examined how macrophage activation by bacterial lipopolysaccharide (LPS) or the lung pathogen Streptococcus pneumoniae is altered by ENP pretreatment. Neither silica nor SPIO treatment elicited direct cytotoxic or pro-inflammatory effects in bone marrow-derived macrophages However pretreatment of macrophages with SPIO caused extensive reprogramming of nearly 500 genes regulated in response to,LPS challenge, hallmarked by exaggerated activation of oxidative stress response pathways and suppressed activation of both pro- and anti-inflammatory pathways Silica pretreatment altered regulation of only 67 genes but there was strong correlation with gene sets affected by SPIO. Macrophages exposed to SPIO displayed a phenotype suggesting an impaired ability to transition from an M1 to M2-like activation state, characterized by suppressed IL-10 induction, enhanced TNF alpha production, and diminished phagocytic activity toward S. pneumonia. Studies in macrophages deficient in scavenger receptor A (SR-A) showed SR-A participates in cell uptake of both the ENPs and S. pneumonia and co-regulates the anti-inflammatory IL-10 pathway. Thus, mechanisms for dysregulation of innate immunity exist by virtue that common receptor recognition pathways are used by some ENPs and pathogenic bacteria, although the extent of transcriptional reprogramming of macrophage function depends on the physicochemical properties of the ENP after internalization. Our results also illustrate that biological effects of ENPs may be indirectly manifested only after challenging normal cell function. Nanotoxicology screening strategies should therefore consider how exposure to these materials alters susceptibility to other environmental exposures.
C1 [Kodali, Vamsi; Littke, Matthew H.; Teeguarden, Justin G.; Shi, Liang; Pounds, Joel G.; Thrall, Brian D.] Pacific NW Natl Lab, Ctr Nanotoxicol, Richland, WA 99352 USA.
[Kodali, Vamsi; Littke, Matthew H.; Teeguarden, Justin G.; Shi, Liang; Pounds, Joel G.; Thrall, Brian D.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
[Tilton, Susan C.] Pacific NW Natl Lab, Computat Sci Div, Richland, WA 99352 USA.
[Frevert, Charles W.] Univ Washington, Dept Comparat Med, Seattle, WA 98195 USA.
[Wang, Wei] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA.
RP Thrall, BD (reprint author), Pacific NW Natl Lab, Ctr Nanotoxicol, Richland, WA 99352 USA.
EM brian.thrall@pnnl.gov
RI Wang, Wei/B-5924-2012; Kodali, Vamsi/D-2497-2009; Geracitano,
Laura/E-6926-2013;
OI Pounds, Joel/0000-0002-6616-1566; Teeguarden,
Justin/0000-0003-3817-4391; Kodali, Vamsi/0000-0001-6177-0568
FU National Institute of Environmental Health Sciences [U19 ES019544, RO1
ES016212]
FX The authors thank Drs. Norman Karin and Cosmin Mihai for technical
assistance. Support for this research was provided by the National
Institute of Environmental Health Sciences through grants U19 ES019544
and RO1 ES016212.
NR 55
TC 29
Z9 29
U1 5
U2 44
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD AUG
PY 2013
VL 7
IS 8
BP 6997
EP 7010
DI 10.1021/nn402145t
PG 14
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 210DX
UT WOS:000323810600061
PM 23808590
ER
PT J
AU Bult, JB
Crisp, R
Perkins, CL
Blackburn, JL
AF Bult, Justin B.
Crisp, Ryan
Perkins, Craig L.
Blackburn, Jeffrey L.
TI Role of Dopants in Long-Range Charge Carrier Transport for p-Type and
n-Type Graphene Transparent Conducting Thin Films
SO ACS NANO
LA English
DT Article
DE graphene; transparent conductor; charged impurity; scattering;
photovoltalcs; conductivity; mobility; transport; temperature-dependent
ID CHEMICAL-VAPOR-DEPOSITION; CARBON NANOTUBE NETWORKS; RAMAN-SPECTROSCOPY;
LARGE-AREA; ELECTRODES; SCATTERING; OXIDES; PHOTOVOLTAICS; PERFORMANCE;
DEFECTS
AB Monolayer to few-layer graphene thin films have several attractive properties such as high transparency, exceptional electronic transport, mechanical durability, and environmental stability, which are required in transparent conducting electrodes (TCs). The successful incorporation of graphene TCs into demanding applications such as thin film photovoltaics requires a detailed understanding of the factors controlling long-range charge transport. In this study, we use spectroscopic and electrical transport measurements to provide a self-consistent understanding of the macroscopic (centimeter, many-grain scale) transport properties of chemically doped p-type and n-type graphene TCs. We demonstrate the first large-area n-type graphene TCs through the use of hydrazine or polyethyleneimine as dopants. The n-type graphene TCs utilizing PEI, either as the sole dopant or as an overcoat, have good stability in air compared to TCs only doped with hydrazine. We demonstrate a shift in Fermi energy of well over 1 V between the n- and p-type graphene TCs and a sheet resistance of similar to 50 Omega/sq at 89% visible transmittance. The carrier density is increased by 2 orders of magnitude in heavily doped graphene TCs, while the mobility is reduced by a factor of similar to 7 due to charged impurity scattering. Temperature-dependent measurements demonstrate that the molecular dopants also help to suppress processes associated with carrier localization that may limit the potential of intrinsic graphene TCs. These results suggest that properly doped graphene TCs may be well-suited as anodes or cathodes for a variety of opto-electronic applications.
C1 [Bult, Justin B.; Crisp, Ryan; Perkins, Craig L.; Blackburn, Jeffrey L.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Blackburn, JL (reprint author), Natl Renewable Energy Lab, 16253 Denver West Pkwy, Golden, CO 80401 USA.
EM jeffrey.blackburn@nrel.gov
RI Crisp, Ryan/C-9944-2014
OI Crisp, Ryan/0000-0002-3703-9617
FU NREL's Laboratory Directed Research and Development (LORD) program
FX We gratefully acknowledge NREL's Laboratory Directed Research and
Development (LORD) program for funding. We thank Kevin Mistry for
helpful discussions regarding n-type doping.
NR 46
TC 30
Z9 31
U1 4
U2 134
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD AUG
PY 2013
VL 7
IS 8
BP 7251
EP 7261
DI 10.1021/nn402673z
PG 11
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 210DX
UT WOS:000323810600090
PM 23859709
ER
PT J
AU He, XW
Wang, X
Nanot, S
Cong, K
Jiang, QJ
Kane, AA
Goldsmith, JEM
Hauge, RH
Leonard, F
Kono, J
AF He, Xiaowei
Wang, Xuan
Nanot, Sebastien
Cong, Kankan
Jiang, Qijia
Kane, Alexander A.
Goldsmith, John E. M.
Hauge, Robert H.
Leonard, Francois
Kono, Junichiro
TI Photothermoelectric p-n Junction Photodetector with Intrinsic Broadband
Polarimetry Based on Macroscopic Carbon Nanotube Films
SO ACS NANO
LA English
DT Article
DE SWCNTs; photothermoelectric effect; intrinsic polarimetry; photodetector
ID SOLAR-CELLS
AB Light polarization is used in the animal kingdom for communication, navigation, and enhanced scene interpretation and also plays an important role in astronomy, remote sensing, and military applications. To date, there have been few photodetector materials demonstrated to have direct polarization sensitivity, as is usually the case in nature. Here, we report the realization of a carbon-based broadband photodetector, where the polarimetry is intrinsic to the active photodetector material. The detector is based on pn junctions formed between two macroscopic films of single-wall carbon nanotubes. A responsivity up to similar to 1 V/W was observed in these devices, with a broadband spectral response spanning the visible to the mid-infrared. This responsivity is about 35 times larger than previous devices without pn junctions. A combination of experiment and theory is used to demonstrate the photothermoelectric origin of the responsivity and to discuss the performance attributes of such devices.
C1 [He, Xiaowei; Wang, Xuan; Nanot, Sebastien; Cong, Kankan; Jiang, Qijia; Kono, Junichiro] Rice Univ, Dept Elect & Comp Engn, Houston, TX 77005 USA.
[Cong, Kankan; Kono, Junichiro] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA.
[Kane, Alexander A.; Goldsmith, John E. M.; Leonard, Francois] Sandia Natl Labs, Livermore, CA 94551 USA.
[Hauge, Robert H.] Rice Univ, Dept Chem, Houston, TX 77005 USA.
[Hauge, Robert H.] King Abdulaziz Univ, Jeddah 21589, Saudi Arabia.
RP Leonard, F (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA.
EM fleonar@sandia.gov; kono@rice.edu
RI Hauge, Robert/A-7008-2011;
OI Hauge, Robert/0000-0002-3656-0152; Nanot, Sebastien/0000-0002-3185-1583
FU Lockheed-Martin Rice University LANCER Program; National Science
Foundation [OISE-0968405, EEC-0540832]; Department of Energy BES Program
[DE-FG02-06ER46308]; Robert A. Welch Foundation [C-1509]; U.S.
Department of Energy, Office of Science, through the National Institute
for Nano-Engineering (NINE) at Sandia National Laboratories; Laboratory
Directed Research and Development Program at Sandia National
Laboratories; United States Department of Energy [DEAC01-94-AL85000];
Intelligence Community Postdoctoral Fellowship Program
FX This work was supported by the Lockheed-Martin Rice University LANCER
Program, the National Science Foundation (through Grant Nos.
OISE-0968405 and EEC-0540832), the Department of Energy BES Program
(through Grant No. DE-FG02-06ER46308), the Robert A. Welch Foundation
(through Grant No. C-1509), the U.S. Department of Energy, Office of
Science, through the National Institute for Nano-Engineering (NINE) at
Sandia National Laboratories, and the Laboratory Directed Research and
Development Program at Sandia National Laboratories, a multiprogram
laboratory operated by Sandia Corporation, a Lockheed Martin Co, for the
United States Department of Energy under Contract No. DEAC01-94-AL85000.
AAK acknowledges support from the Intelligence Community Postdoctoral
Fellowship Program. We thank Nick Thompson for his help with editing and
proofreading the manuscript
NR 23
TC 25
Z9 25
U1 7
U2 91
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD AUG
PY 2013
VL 7
IS 8
BP 7271
EP 7277
DI 10.1021/nn402679u
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 210DX
UT WOS:000323810600092
PM 23808567
ER
PT J
AU Morris, CL
Bacon, J
Borozdin, K
Miyadera, H
Perry, J
Rose, E
Watson, S
White, T
Aberle, D
Green, JA
McDuff, GG
Lukic, Z
Milner, EC
AF Morris, C. L.
Bacon, Jeffrey
Borozdin, Konstantin
Miyadera, Haruo
Perry, John
Rose, Evan
Watson, Scott
White, Tim
Aberle, Derek
Green, J. Andrew
McDuff, George G.
Lukic, Zarija
Milner, Edward C.
TI A new method for imaging nuclear threats using cosmic ray muons
SO AIP ADVANCES
LA English
DT Article
AB Muon tomography is a technique that uses cosmic ray muons to generate three dimensional images of volumes using information contained in the Coulomb scattering of the muons. Advantages of this technique are the ability of cosmic rays to penetrate significant overburden and the absence of any additional dose delivered to subjects under study above the natural cosmic ray flux. Disadvantages include the relatively long exposure times and poor position resolution and complex algorithms needed for reconstruction. Here we demonstrate a new method for obtaining improved position resolution and statistical precision for objects with spherical symmetry. C (C) 2013 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.
C1 [Morris, C. L.; Bacon, Jeffrey; Borozdin, Konstantin; Miyadera, Haruo; Perry, John; Rose, Evan; Watson, Scott; White, Tim] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Aberle, Derek; Green, J. Andrew; McDuff, George G.] Natl Secur Technol, Los Alamos, NM 87544 USA.
[Lukic, Zarija] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Milner, Edward C.] So Methodist Univ, Dallas, TX 75205 USA.
RP Morris, CL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
OI Watson, Scott/0000-0003-1318-5924; Morris,
Christopher/0000-0003-2141-0255; Perry, John/0000-0003-3639-5617
FU United States Department of Energy; United States Department of State;
Defense Threat Reduction Agency of the United States Department of
Defense
FX We would like to acknowledge help from Dave Schwellenbach and Wendi
Dreesen setting up the hardware and software that has enabled these
measurements. This work was supported in part by the United States
Department of Energy, the United States Department of State, and the
Defense Threat Reduction Agency of the United States Department of
Defense.
NR 8
TC 2
Z9 3
U1 1
U2 11
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 2158-3226
J9 AIP ADV
JI AIP Adv.
PD AUG
PY 2013
VL 3
IS 8
AR 082128
DI 10.1063/1.4820349
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA 210PA
UT WOS:000323845000028
ER
PT J
AU Zhang, SF
Li, YK
Fathololoumi, S
Nguyen, HPT
Wang, Q
Mi, ZT
Li, QM
Wang, GT
AF Zhang, Shaofei
Li, Yukun
Fathololoumi, Saeed
Hieu Pham Trung Nguyen
Wang, Qi
Mi, Zetian
Li, Qiming
Wang, George T.
TI On the efficiency droop of top-down etched InGaN/GaN nanorod light
emitting diodes under optical pumping
SO AIP ADVANCES
LA English
DT Article
ID QUANTUM-WELLS; SEMICONDUCTORS; PERFORMANCE; EMISSION; ORIGIN; FIELDS;
ARRAYS; GAN
AB The optical performance of top-down etched InGaN/GaN nanorod light emitting diodes (LEDs) was studied using temperature variable photoluminescence spectroscopy with a 405 nm pump laser. Efficiency droop is measured from such nanorod structures, which is further enhanced with decreasing temperature. Through detailed rate equation analysis of the temperature-dependent carrier distribution and modeling of the quantum efficiency, this unique phenomenon can be largely explained by the interplay and dynamics between carrier radiative recombination in localized states and nonradiative recombination via surface states/defects. (C) 2013 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.
C1 [Zhang, Shaofei; Li, Yukun; Fathololoumi, Saeed; Hieu Pham Trung Nguyen; Wang, Qi; Mi, Zetian] McGill Univ, Dept Elect & Comp Engn, Montreal, PQ H3A 0E9, Canada.
[Li, Qiming; Wang, George T.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Zhang, SF (reprint author), McGill Univ, Dept Elect & Comp Engn, 3480 Univ St, Montreal, PQ H3A 0E9, Canada.
FU Natural Sciences and Engineering Research Council of Canada; Fonds de
recherchsur la nature et les technologies; Solid-State-Lighting Science
Energy Frontier Research Center; U.S. DOE Office of Basic Energy
Sciences; U.S. Department of Energy National Nuclear Security
Administration [DE-AC04-94AL85000]
FX This work was supported by the Natural Sciences and Engineering Research
Council of Canada and the Fonds de recherchsur la nature et les
technologies. The nanorod fabrication was performed at Sandia and funded
by the Solid-State-Lighting Science Energy Frontier Research Center,
funded by the U.S. DOE Office of Basic Energy Sciences. Sandia National
Laboratories is a multi-program laboratory managed and operated by
Sandia Corporation, a wholly owned subsidiary of Lockheed Martin
Corporation, for the U.S. Department of Energy National Nuclear Security
Administration under contract DE-AC04-94AL85000.
NR 39
TC 6
Z9 6
U1 1
U2 41
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 2158-3226
J9 AIP ADV
JI AIP Adv.
PD AUG
PY 2013
VL 3
IS 8
AR 082103
DI 10.1063/1.4817834
PG 8
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA 210PA
UT WOS:000323845000003
ER
PT J
AU Zhang, JB
Tang, LY
Zhang, J
Qin, ZX
Zeng, XJ
Liu, J
Wen, JS
Xu, ZJ
Gu, GD
Chen, XJ
AF Zhang Jian-Bo
Tang Ling-Yun
Zhang Jiang
Qin Zhen-Xing
Zeng Xiao-Jing
Liu Jing
Wen Jin-Sheng
Xu Zhi-Jun
Gu Genda
Chen Xiao-Jia
TI Pressure-induced isostructural phase transition in Bi2Sr2CaCu2O8+delta
SO CHINESE PHYSICS C
LA English
DT Article
DE cuprate superconductors; structural properties; high pressure;
synchrotron X-ray diffraction
ID SINGLE-CRYSTAL; SUPERCONDUCTIVITY; TEMPERATURE; DEPENDENCE
AB The high-pressure structures of an underdoped cuprate superconductor Bi2Sr2CaCu2O8+delta have been studied by synchrotron X-ray diffraction at pressures up to 36.5 GPa. We find that this superconductor retains its orthogonal structure with the space group Amaa in the pressure range studied. Upon compression, both the a and b axes first shrink monotonically up to 17.4 GPa from their ambient pressure values and keep these behaviors with positive compressibilities up to 36.5 GPa after experiencing expansion with negative compressibilities in the pressure regime between 17.4 and 23.7 GPa. However, the c axis decreases continuously with increasing pressure with a slow change at about 23.7 GPa. The results indicate an isostructural phase transition starting at 17.4 GPa and a structural collapse at around 23.7 GPa.
C1 [Zhang Jian-Bo; Tang Ling-Yun; Zhang Jiang; Qin Zhen-Xing; Zeng Xiao-Jing; Chen Xiao-Jia] S China Univ Technol, Dept Phys, Guangzhou 510640, Guangdong, Peoples R China.
[Liu Jing] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China.
[Wen Jin-Sheng; Xu Zhi-Jun; Gu Genda] Brookhaven Natl Lab, Upton, NY 11973 USA.
RP Zhang, JB (reprint author), S China Univ Technol, Dept Phys, Guangzhou 510640, Guangdong, Peoples R China.
RI Wen, Jinsheng/F-4209-2010; Zhang, Jiang/B-6158-2008; xu,
zhijun/A-3264-2013
OI Wen, Jinsheng/0000-0001-5864-1466; xu, zhijun/0000-0001-7486-2015
FU Cultivation Fund of the Key Scientific and Technical Innovation Project,
Ministry of Education of China [708070]; U.S. DOE BES
[DE-AC02-98CH10886]
FX Supported by Cultivation Fund of the Key Scientific and Technical
Innovation Project, Ministry of Education of China (708070), and U.S.
DOE BES (DE-AC02-98CH10886)
NR 29
TC 0
Z9 0
U1 1
U2 21
PU CHINESE PHYSICAL SOC
PI BEIJING
PA P O BOX 603, BEIJING 100080, PEOPLES R CHINA
SN 1674-1137
J9 CHINESE PHYS C
JI Chin. Phys. C
PD AUG
PY 2013
VL 37
IS 8
AR UNSP 088003
DI 10.1088/1674-1137/37/8/088003
PG 4
WC Physics, Nuclear; Physics, Particles & Fields
SC Physics
GA 198QQ
UT WOS:000322937800018
ER
PT J
AU Li, H
Zhang, HS
Zhang, Y
AF Li Hui
Zhang Hong-Sheng
Zhang Yi
TI A Generalized Semi-Holographic Universe
SO CHINESE PHYSICS LETTERS
LA English
DT Article
ID UNIFIED 1ST LAW; DARK ENERGY; PHANTOM THERMODYNAMICS; BLACK-HOLES;
MODEL; CONSTRAINTS; PRINCIPLE; DYNAMICS; VACUUM
AB We study the semi-holographic idea in the context of decaying dark components. The energy flow between dark energy and the compensating dark matter is thermodynamically generalized to involve a particle number variable dark component with non-zero chemical potential. It is found that, unlike the original semi-holographic model, no cosmological constant is needed for a dynamical evolution of the universe. A transient phantom phase appears while a non-trivial dark energy-dark matter scaling solution stays at a later time, which evades the big-rip and helps to resolve the coincidence problem. For reasonable parameters, the deceleration parameter is well consistent with current observations. The original semi-holographic model is extended and it also suggests that the concordance model may be reconstructed from the semi-holographic idea.
C1 [Li Hui] Yantai Univ, Dept Phys, Yantai 264005, Peoples R China.
[Zhang Hong-Sheng] Shanghai Normal Univ, SUCA, Shanghai 200234, Peoples R China.
[Zhang Yi] Chongqing Univ Posts & Telecommun, Coll Math & Phys, Chongqing 400065, Peoples R China.
[Zhang Hong-Sheng; Zhang Yi] Chinese Acad Sci, Inst Theoret Phys, State Key Lab Theoret Phys, Beijing 100190, Peoples R China.
[Zhang Yi] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA.
RP Li, H (reprint author), Yantai Univ, Dept Phys, 30 Qingquan Rd, Yantai 264005, Peoples R China.
EM lihui@ytu.edu.cn
FU National Natural Science Foundation of China [10747155, 11205131,
11075106, 11005164, 11175270, 10935013]; Program for Professor of
Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher
Learning, Shanghai Municipal Pujiang [10PJ1408100]; CQ CSTC
[2010BB0408]; Argonne National Laboratory
FX Supported by the National Natural Science Foundation of China under
Grant Nos 10747155, 11205131, 11075106, 11005164, 11175270 and 10935013,
the Program for Professor of Special Appointment (Eastern Scholar) at
Shanghai Institutions of Higher Learning, Shanghai Municipal Pujiang
under Grant No 10PJ1408100, CQ CSTC under Grant No 2010BB0408, and the
Argonne National Laboratory.
NR 53
TC 1
Z9 1
U1 0
U2 1
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0256-307X
J9 CHINESE PHYS LETT
JI Chin. Phys. Lett.
PD AUG
PY 2013
VL 30
IS 8
AR 089801
DI 10.1088/0256-307X/30/8/089801
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 209DH
UT WOS:000323733900056
ER
PT J
AU Gallagher, KG
Croy, JR
Balasubramanian, M
Bettge, M
Abraham, DP
Burrell, AK
Thackeray, MM
AF Gallagher, Kevin G.
Croy, Jason R.
Balasubramanian, Mahalingam
Bettge, Martin
Abraham, Daniel P.
Burrell, Anthony K.
Thackeray, Michael M.
TI Correlating hysteresis and voltage fade in lithium- and manganese-rich
layered transition-metal oxide electrodes
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Lithium-ion; Cathode; Decay mechanism; Destabilization; Tetrahedral
site; Intercalation
ID X-RAY-DIFFRACTION; ION BATTERIES; STRUCTURAL-CHARACTERIZATION;
NEUTRON-DIFFRACTION; DELITHIATED LIVO2; CATHODE MATERIAL; CAPACITY;
LIMNO2; ELECTROCHEMISTRY; TRANSFORMATION
AB Electrochemical studies demonstrate a strong correlation between the phenomena of hysteresis and voltage fade in lithium- and manganese-rich layered transition-metal oxide electrodes. A mechanism is proposed that entails both the reversible and irreversible migration of transition metal ions. Their reversible migration to a metastable configuration, suggested to involve the occupation of tetrahedral sites in the lithium layer, is manifested as a 1 V hysteresis in site energy for 10-15% of the lithium content. The irreversible migration of the transition metal ions through the metastable 'hysteresis' sites to localized and lower energy cubic environments results in the observed voltage fade phenomenon. (c) 2013 Elsevier B.V. All rights reserved.
C1 [Gallagher, Kevin G.; Croy, Jason R.; Bettge, Martin; Abraham, Daniel P.; Burrell, Anthony K.; Thackeray, Michael M.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
[Balasubramanian, Mahalingam] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Lemont, IL 60439 USA.
RP Gallagher, KG (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
EM kevin.gallagher@anl.gov
FU Vehicle Technologies Program, Hybrid and Electric Systems; Argonne, a
U.S. Department of Energy Office of Science Laboratory
[DE-AC02-06CH11357]
FX Support from the Vehicle Technologies Program, Hybrid and Electric
Systems, in particular David Howell, Peter Faguy, and Tien Duong at the
U.S. Department of Energy, Office of Energy Efficiency and Renewable
Energy, is gratefully acknowledged. The submitted manuscript has been
created by UChicago Argonne, LLC, Operator of Argonne National
Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of
Science Laboratory, is operated under Contract No. DE-AC02-06CH11357.
The U.S. Government retains for itself, and others acting on its behalf,
a paid-up nonexclusive, irrevocable worldwide license in said article to
reproduce, prepare derivative works, distribute copies to the public,
and perform publicly and display publicly, by or on behalf of the
Government.
NR 27
TC 76
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U1 8
U2 174
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD AUG
PY 2013
VL 33
BP 96
EP 98
DI 10.1016/j.elecom.2013.04.022
PG 3
WC Electrochemistry
SC Electrochemistry
GA 199VW
UT WOS:000323024600024
ER
PT J
AU Krasko, VA
Doris, E
AF Krasko, Vitaliy A.
Doris, Elizabeth
TI State distributed PV policies: Can low cost (to government) policies
have a market impact?
SO ENERGY POLICY
LA English
DT Article
DE State policy; Distributed generation; Photovoltaics
ID DEPLOYMENT; ENERGY
AB This analysis examines the use of state policy as a tool to support the development of distributed generation photovoltaic (PV) markets. The focus is on low-cost market opening policies instead of various forms of government subsidies aimed at reducing installation costs. The ideas tested in this work are: (1) low-cost market opening policies can be effective in facilitating PV market growth without subsidizing projects, and (2) policies can be made more effective if states and localities stage their enactment in a particular order. The policies selected for evaluation emerge from a policy stacking theory outlined in Doris (2012), NREL/CP-7A30-54801, Golden, CO: National Renewable Energy Laboratory. A cross-section econometric analysis that takes into account the quality of interconnection standards, net metering standards, Renewable Portfolio Standards (RPS), RPS set-asides, and a non-policy determinant (population) explains about 70% of the variation in newly installed PV capacity across states and indicates that all of the selected policies are significant. Nonparametric statistical tests confirm the regression results. Qualitative evidence is also presented indicating that effective policy ordering starts with improving interconnection standards, closely followed by improvements in net metering standards, and eventually strengthened by the enactment of an RPS and set-asides. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Krasko, Vitaliy A.; Doris, Elizabeth] Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Krasko, Vitaliy A.] Colorado Sch Mines, Div Econ & Business, Golden, CO 80401 USA.
RP Krasko, VA (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA.
EM vitaliy.krasko@nrel.gov; Elizabeth.Doris@nrel.gov
NR 27
TC 7
Z9 7
U1 1
U2 18
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
J9 ENERG POLICY
JI Energy Policy
PD AUG
PY 2013
VL 59
BP 172
EP 181
DI 10.1016/j.enpol.2013.03.015
PG 10
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 202QW
UT WOS:000323235700016
ER
PT J
AU Park, WY
Phadke, A
Shah, N
Letschert, V
AF Park, Won Young
Phadke, Amol
Shah, Nihar
Letschert, Virginie
TI Efficiency improvement opportunities in TVs: Implications for market
transformation programs
SO ENERGY POLICY
LA English
DT Article
DE TV energy efficiency; Cost effectiveness; Market transformation
AB Televisions (TVs) account for a significant portion of residential electricity consumption and global TV shipments are expected to continue to increase. We assess the market trends in the energy efficiency of TVs that are likely to occur without any additional policy intervention and estimate that TV efficiency will likely improve by over 60% by 2015 with savings potential of 45 terawatt-hours [TW h] per year in 2015, compared to today's technology. We discuss various energy-efficiency improvement options and evaluate the cost effectiveness of three of them. At least one of these options improves efficiency by at least 20% cost effectively beyond ongoing market trends. We provide insights for policies and programs that can be used to accelerate the adoption of efficient technologies to further capture global energy savings potential from TVs which we estimate to be up to 23 TW h per year in 2015. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Park, Won Young; Phadke, Amol; Shah, Nihar; Letschert, Virginie] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Park, WY (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM wypark@lbl.gov
FU Bureau of Oceans and International Environmental and Scientific Affairs,
U.S. Department of State; U.S. Department of Energy [DE-AC02-05CH11231]
FX We wish to thank the reviewers of this article as well as the report, TV
Energy Consumption Trends and Energy-Efficiency Improvement Options
(LBNL5024-E), on which this paper is based. This work was funded by the
Bureau of Oceans and International Environmental and Scientific Affairs,
U.S. Department of State, and administered by the U.S. Department of
Energy in support of the Super-efficient Equipment and Appliance
Deployment (SEAD) Initiative through the U.S. Department of Energy under
Contract No. DE-AC02-05CH11231. Any errors or omissions are the authors'
own.
NR 39
TC 6
Z9 6
U1 1
U2 5
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
J9 ENERG POLICY
JI Energy Policy
PD AUG
PY 2013
VL 59
BP 361
EP 372
DI 10.1016/j.enpol.2013.03.048
PG 12
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 202QW
UT WOS:000323235700033
ER
PT J
AU Vine, E
AF Vine, Edward
TI Transforming the energy efficiency market in California: Key findings,
lessons learned and future directions from California's market effects
studies
SO ENERGY POLICY
LA English
DT Article
DE Evaluation; Market effects; Market transformation
AB In the last three years, the California Institute for Energy and Environment (CIEE), along with the California Public Utilities Commission (CPUC), managed three market effects studies that were funded by the CPUC. This paper summarizes the key findings from these studies that focused on compact fluorescent lamps (CFLs), residential new construction (RNC), and high bay lighting (HBL),(1) with a particular focus on changes to California's market effects evaluation protocol and lessons learned during the evaluation of market effects. This paper also summarizes the key results from a survey that was conducted by CIEE in February 2011 to determine what additional studies should be conducted in the evaluation of market effects. Published by Elsevier Ltd.
C1 [Vine, Edward] Calif Inst Energy & Environm, Berkeley, CA 94720 USA.
[Vine, Edward] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Vine, E (reprint author), Calif Inst Energy & Environm, Bldg 90-4000, Berkeley, CA 94720 USA.
EM elvine@lbl.gov
NR 7
TC 1
Z9 1
U1 4
U2 11
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
J9 ENERG POLICY
JI Energy Policy
PD AUG
PY 2013
VL 59
BP 702
EP 709
DI 10.1016/j.enpol.2013.04.030
PG 8
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 202QW
UT WOS:000323235700062
ER
PT J
AU Coniglio, N
Cross, CE
AF Coniglio, N.
Cross, C. E.
TI Initiation and growth mechanisms for weld solidification cracking
SO INTERNATIONAL MATERIALS REVIEWS
LA English
DT Review
DE Weld solidification cracking; Crack initiation; Crack growth; Liquid
fracture; Strain partitioning; Stress and strain around moving weld pool
ID HOT-TEARING CRITERION; ALUMINUM-ALLOYS; POROSITY FORMATION;
GRAIN-REFINEMENT; HIGH-STRENGTH; MUSHY ZONES; MODEL; SUSCEPTIBILITY;
PARAMETERS; MICROPOROSITY
AB Solidification cracking is a weld defect common to certain susceptible alloys rendering many of them unweldable. It forms and grows continuously behind a moving weld pool within the two phase mushy zone and involves a complex interaction between thermal, metallurgical and mechanical factors. Despite decades long efforts to investigate weld solidification cracking, there remains a significant lack of understanding regarding its underlying mechanisms. Criteria developed to evaluate alloy weldability will be examined in terms of proposed solidification cracking models. Crack initiation is discussed in terms of different criteria: critical stress to fracture the interdendritic liquid, critical strain to exceed the mushy zone ductility and critical hydrogen content to nucleate and grow a pore. Crack growth has been characterised in terms of a critical stress to fracture the liquid film surrounding a grain and critical strain rate interdependent with liquid feeding of the mushy zone opening. Experimental data to form a weld solidification crack are compiled, revealing the considerable amount of information available in the literature on this topic.
C1 [Coniglio, N.] IUT Le Creusot, Le Creusot, France.
[Cross, C. E.] LANL, Los Alamos, NM USA.
RP Coniglio, N (reprint author), IUT Le Creusot, Le Creusot, France.
EM nicolas.coniglio@u-bourgogne.fr
FU Federal Institute for Materials and Research Testing (BAM), Berlin
FX The authors are grateful to the Federal Institute for Materials and
Research Testing (BAM), Berlin, for supporting research on this topic
leading to the earned doctorate of one of the authors (Coniglio) from
which this work was compiled. The reviewers are gratefully acknowledged
for their useful comments.
NR 146
TC 9
Z9 9
U1 2
U2 38
PU MANEY PUBLISHING
PI LEEDS
PA STE 1C, JOSEPHS WELL, HANOVER WALK, LEEDS LS3 1AB, W YORKS, ENGLAND
SN 0950-6608
J9 INT MATER REV
JI Int. Mater. Rev.
PD AUG
PY 2013
VL 58
IS 7
BP 375
EP 397
DI 10.1179/1743280413Y.0000000020
PG 23
WC Materials Science, Multidisciplinary
SC Materials Science
GA 211VO
UT WOS:000323939700001
ER
PT J
AU Kerisit, S
Liu, CX
AF Kerisit, Sebastien
Liu, Chongxuan
TI Structure, Kinetics, and Thermodynamics of the Aqueous Uranyl(VI) Cation
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID MOLECULAR-DYNAMICS SIMULATION; WATER-EXCHANGE MECHANISM; SOLVATION
FREE-ENERGIES; ELECTRON CORRELATION; PROPER TREATMENT; HANFORD-SITE;
FORCE-FIELD; COORDINATION ENVIRONMENT; ADSORPTION EQUILIBRIA; SURFACE
COMPLEXATION
AB In this work, molecular simulation techniques were employed to gain insight into the structural, kinetic, and thermodynamic properties of the uranyl(VI) cation (UO22+) in aqueous solution. The simulations made use of an atomistic potential model (force field) derived in this work and based on the model of Guilbaud and Wipff [J. Mol. Struct. (THEOCHEM) 1996, 366, 55-63]. Reactive flux and thermodynamic integration calculations show that the derived potential model yields predictions for the water exchange rate and free energy of hydration, respectively, that are in agreement with experimental data. The water binding energies, hydration shell structure, and self diffusion coefficient were also calculated and analyzed. Finally, a combination of metadynamics and transition path sampling simulations was employed to probe the mechanisms of water exchange reactions in the first hydration shell of the uranyl ion. These atomistic simulations indicate, based on two-dimensional free energy surfaces, that water exchanges follow an associative interchange mechanism. The nature and structure of the water exchange transition states were also determined. The improved potential model is expected to lead to more accurate predictions of uranyl adsorption energies at mineral surfaces using potential-based molecular dynamics simulations.
C1 [Kerisit, Sebastien; Liu, Chongxuan] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA.
RP Kerisit, S (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA.
EM sebastien.kerisit@pnnl.gov
RI Liu, Chongxuan/C-5580-2009
FU U.S. Department of Energy (DOE) Biological and Environmental Research
(BER) Division through the Subsurface Biogeochemistry Research (SBR)
Program of the Science Focus Area (SFA) at Pacific Northwest National
Laboratory (PNNL); DOE's Office of Biological and Environmental Research
(OBER); Battelle Memorial Institute [DE-ACO5-76RL01830]
FX The authors acknowledge Dr. Patrick Nichols for providing the radial
distribution functions from his ab initio molecular dynamics simulation
of the uranyl(VI) cation in water. This research was supported by the
U.S. Department of Energy (DOE) Biological and Environmental Research
(BER) Division through the Subsurface Biogeochemistry Research (SBR)
Program of the Science Focus Area (SFA) at Pacific Northwest National
Laboratory (PNNL). The computer simulations were performed in part using
the Molecular Science Computing (MSC) facilities in the William R. Wiley
Environmental Molecular Sciences Laboratory (EMSL), a national
scientific user facility sponsored by the DOE's Office of Biological and
Environmental Research (OBER) and located at Pacific Northwest National
Laboratory (PNNL). PNNL is operated for the DOE by Battelle Memorial
Institute under Contract DE-ACO5-76RL01830.
NR 97
TC 23
Z9 23
U1 7
U2 61
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 1
PY 2013
VL 117
IS 30
BP 6421
EP 6432
DI 10.1021/jp404594p
PG 12
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 196WE
UT WOS:000322807300004
PM 23815284
ER
PT J
AU Poutsma, ML
AF Poutsma, Marvin L.
TI Evolution of Structure-Reactivity Correlations for the Hydrogen
Abstraction Reaction by Hydroxyl Radical and Comparison with That by
Chlorine Atom
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID GAS-PHASE REACTIONS; BOND-DISSOCIATION ENTHALPIES; TRANSITION-STATE
THEORY; MOLECULAR-ORBITAL CALCULATIONS; PREDICTING RATE CONSTANTS;
FREE-ENERGY CORRELATIONS; OH RADICALS; ATMOSPHERIC CHEMISTRY;
ORGANIC-COMPOUNDS; RATE COEFFICIENTS
AB A structure-reactivity correlation for the reaction (HO. + HCR3 -> HOH + CR3.) has been formulated: log k(298)(per H, cm(3)/molecule.s) = -0.000630 Delta H-r(2) -0.151 Delta H-r-1.056 Sigma F-1.053 Sigma R-21.26 (r(2) = 0.885; n = 70; mean unsigned deviation = 0.29 log units), where Delta H-r is the reaction enthalpy (kJ/mol) and F and R represent the dissection of Hammetts sigma(para) constant into its field/inductive and resonance effects, and compared for the analogous case for Cl. (ref 1). Although more exothermic, the dependence of HO. on Delta H-r is somewhat greater than Cl.. However the dependence on F and R is much less, suggestive of less charge separation in the transition state for the less electronegative HO. The range of k(OH) is significantly less than that of Cl., i.e., it is less dependent on substrate structure. Yet a crossover exists such that k(Cl) > k(HO) predominates for more reactive cases whereas k(Cl) < k(OH) characterizes the less reactive. The Arrhenius parameters reveal that this crossover results from a change in {E(Cl) - E(OH)} from negative to positive. In contrast, whereas the A factors for both increase significantly as reactivity increases, {A(Cl)/A(OH)} always exceeds unity.
C1 Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
RP Poutsma, ML (reprint author), Oak Ridge Natl Lab, Div Chem Sci, POB 2008, Oak Ridge, TN 37831 USA.
EM poutsmaml@ornl.gov
FU Division of Chemical Sciences, Geosciences and Biosciences, Office of
Basic Energy Sciences, U.S. Department of Energy; UT-Battelle, LLC
[DE-AC05-000R22725]; U.S. Department of Energy
FX This research was sponsored by the Division of Chemical Sciences,
Geosciences and Biosciences, Office of Basic Energy Sciences, U.S.
Department of Energy. This manuscript has been authored by UT-Battelle,
LLC, under Contract No. DE-AC05-000R22725 with the U.S. Department of
Energy. The United States Government retains and the publisher, by
accepting the article for publication, acknowledges that the United
States Government retains a nonexclusive, paid-up, irrevocable,
worldwide license to publish or reproduce the published form of this
manuscript, or allow others to do so, for United States Government
purposes.
NR 115
TC 5
Z9 6
U1 5
U2 47
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 1
PY 2013
VL 117
IS 30
BP 6433
EP 6449
DI 10.1021/jp404749z
PG 17
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 196WE
UT WOS:000322807300005
PM 23844551
ER
PT J
AU Trevitt, AJ
Prendergast, MB
Goulay, F
Savee, JD
Osborn, DL
Taatjes, CA
Leone, SR
AF Trevitt, Adam J.
Prendergast, Matthew B.
Goulay, Fabien
Savee, John D.
Osborn, David L.
Taatjes, Craig A.
Leone, Stephen R.
TI Product Branching Fractions of the CH plus Propene Reaction from
Synchrotron Photoionization Mass Spectrometry
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID SET MODEL CHEMISTRY; COUPLING PHOTOCHEMISTRY; CHEMICAL-DYNAMICS; TITANS
ATMOSPHERE; CROSS-SECTIONS; HAZE FORMATION; COMBUSTION; DISSOCIATION;
HYDROCARBONS; MECHANISM
AB The CH(X-2 pi) + propene reaction is studied in the gas phase at 298 K and 4 Torr (533.3 Pa) using VUV synchrotron photoionization mass spectrometry. The dominant product channel is the formation of C4H6 (m/z 54) + H. By fitting experimental photoionization spectra to measured spectra of known C4H6 isomers, the following relative branching fractions are obtained: 1,3-butadiene (0.63 +/- 0.13), 1,2-butadiene (0.25 +/- 0.05), and 1-butyne (0.12 0.03) with no detectable contribution from 2-butyne. The CD + propene reaction is also studied and two product channels are observed that correspond to C4H6 (m/z 54) + D and C4H5D (m/z 55) + H, formed at a ratio of 0.4 (m/z 54) to 1.0 (m/z 55). The D elimination channel forms almost exclusively 1,2-butadiene (0.97 +/- 0.20) whereas the H elimination channel leads to the formation of deuterated 1,3-butadiene (0.89 +/- 0.18) and 1-butyne (0.11 +/- 0.02); photoionization spectra of undeuterated species are used in the fitting of the measured m/z 55 (C4H5D) spectrum. The results are generally consistent with a CH cycloaddition mechanism to the C=C bond of propene, forming 1-methylallyl followed by elimination of a H atom via several competing processes. The direct detection of 1,3-butadiene as a reaction product is an important validation of molecular weight growth schemes implicating the CH + propene reaction, for example, those reported recently for the formation of benzene in the interstellar medium.
C1 [Trevitt, Adam J.; Prendergast, Matthew B.] Univ Wollongong, Sch Chem, Wollongong, NSW 2522, Australia.
[Goulay, Fabien] W Virginia Univ, Dept Chem, Morgantown, WV 26506 USA.
[Savee, John D.; Osborn, David L.; Taatjes, Craig A.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA.
[Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Trevitt, AJ (reprint author), Univ Wollongong, Sch Chem, Wollongong, NSW 2522, Australia.
EM adamt@uow.edu.au
RI Prendergast, Matthew/D-3955-2013; Trevitt, Adam/A-2915-2009
OI Trevitt, Adam/0000-0003-2525-3162
FU Australian Research Council [DP1094135]; International Synchrotron
Access Program (ISAP); National Collaborative Research Infrastructure
Strategy; Federal Government of Australia; Director, Office of Science,
Office of Basic Energy Sciences of the U.S. Department of Energy (DOE)
[DE-ACO2-05CH11231]; National Aeronautics and Space Administration
[NAGS-13339]; Division of Chemical Sciences, Geosciences, and
Biosciences, the Office of Basic Energy Sciences, the U.S. Department of
Energy; National Nuclear Security Administration [DE-AC04-94-AL85000]
FX We thank Dr. Oliver Welz for insightful discussions and Mr. Howard
Johnsen for technical support. A.J.T. acknowledges funding support from
the Australian Research Council (DP1094135) and travel funding provided
by the International Synchrotron Access Program (ISAP) managed by the
Australian Synchrotron. The ISAP is funded by a National Collaborative
Research Infrastructure Strategy grant provided by the Federal
Government of Australia. The Chemical Dynamics Beamline at the Advanced
Light Source is supported by the Director, Office of Science, Office of
Basic Energy Sciences of the U.S. Department of Energy (DOE) under
Contract No. DE-ACO2-05CH11231 at Lawrence Berkeley National Laboratory.
S.RL is also supported by the Gas Phase Physical Chemistry program of
DOE under Contract No. DEACO2-05CH11231. F.G. was supported by the
National Aeronautics and Space Administration (Grant NAGS-13339) while
at UCB and from West Virginia University (start up package). Sandia
authors (J.D.S., D.L.O., CAT.) and the instrumentation for this work are
supported by the Division of Chemical Sciences, Geosciences, and
Biosciences, the Office of Basic Energy Sciences, the U.S. Department of
Energy. Sandia is a multiprogram laboratory operated by Sandia Corp., a
Lockheed Martin Co., for the National Nuclear Security Administration
under contract DE-AC04-94-AL85000.
NR 38
TC 8
Z9 8
U1 9
U2 42
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 1
PY 2013
VL 117
IS 30
BP 6450
EP 6457
DI 10.1021/jp404965k
PG 8
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 196WE
UT WOS:000322807300006
PM 23829558
ER
PT J
AU Iwata, S
Bandyopadhyay, P
Xantheas, SS
AF Iwata, Suehiro
Bandyopadhyay, Pradipta
Xantheas, Sotiris S.
TI Cooperative Roles of Charge Transfer and Dispersion Terms in
Hydrogen-Bonded Networks of (H2O)(n), n=6, 11, and 16
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID SET SUPERPOSITION ERROR; PROJECTED MOLECULAR-ORBITALS; PLESSET
PERTURBATION-THEORY; AB-INITIO CALCULATIONS; LOW-ENERGY STRUCTURES;
WATER CLUSTERS; BINDING-ENERGIES; THERMOCHEMICAL KINETICS;
ELECTRONIC-STRUCTURE; EXCITED ORBITALS
AB The perturbation expansion based on the locally-projected molecular orbital (LPMO PT) was applied to the study of the hydrogen-bonded networks of water clusters with up to 16 molecules. Utilizing the local nature of the occupied and excited MOs on each monomer, the charge-transfer and dispersion terms are evaluated for every pair of molecules. The two terms are strongly correlated with each other for the hydrogen-bonded pairs. The strength of the hydrogen bonds in the clusters is further classified by the types of the hydrogen donor and acceptor water molecules. The relative energies evaluated with the LPMO PT among the isomers of (H2O)(6), (H2O)(11), and (H2O)(16) agree very well with those obtained from CCSD(T) calculations with large basis sets. The binding energy of the LPMO PT is approximately free of the basis set superposition errors caused both by the orbital basis inconsistency and by the configuration basis inconsistency.
C1 [Iwata, Suehiro] Keio Univ, Fac Sci & Technol, Dept Chem, Kohoku Ku, Yokohama, Kanagawa 2238522, Japan.
[Iwata, Suehiro] Toyota Phys & Chem Res Inst, Nagakute, Aichi 4801192, Japan.
[Bandyopadhyay, Pradipta] Jawaharlal Nehru Univ, Sch Computat & Integrat Sci, New Delhi 110067, India.
[Xantheas, Sotiris S.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA.
RP Iwata, S (reprint author), Keio Univ, Fac Sci & Technol, Dept Chem, Kohoku Ku, Yokohama, Kanagawa 2238522, Japan.
EM iwatasuehiro@gmail.com
RI Xantheas, Sotiris/L-1239-2015
FU JSPS [23550031]; U.S. Department of Energy, Office of Basic Energy
Sciences, Division of Chemical Sciences, Geosciences Biosciences; DST
[SR/S1/PC-45/2009]
FX One of the authors (S.I.) acknowledges the late Dr. Takeshi Nagata for
his essential contribution in the development of LPMO perturbation
theories. The work is partially supported by the Grant-in-Aid for
Science Research (No. 23550031) of JSPS (S.I.). Part of this work was
supported by the U.S. Department of Energy, Office of Basic Energy
Sciences, Division of Chemical Sciences, Geosciences & Biosciences.
Pacific Northwest National Laboratory (PNNL) is a multiprogram national
laboratory operated for DOE by Battelle (S.S.X.). This work is partly
supported by a grant awarded to P.B. by DST (No. SR/S1/PC-45/2009).
NR 56
TC 13
Z9 13
U1 1
U2 21
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 1
PY 2013
VL 117
IS 30
BP 6641
EP 6651
DI 10.1021/jp403837z
PG 11
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 196WE
UT WOS:000322807300023
PM 23805893
ER
PT J
AU Foley, JJ
Mazziotti, DA
AF Foley, Jonathan J.
Mazziotti, David A.
TI Cage versus Prism: Electronic Energies of the Water Hexamer
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID OH-STRETCH SPECTROSCOPY; DENSITY-MATRIX METHOD; RELATIVE ENERGIES;
ISOMERS; HYDROGEN; CONVERGENCE; GEOMETRIES; SYSTEMS; LIQUID; ICE
AB Recent experiments show that the cage isomer of the water hexamer is lower in energy than the prism isomer near 0 K, and yet state-of-the-art electronic structure calculations predict the prism to be lower in energy than the cage at 0 K. Here, we study the relative energies of the water hexamers from the parametric two-electron reduced density matrix (2-RDM) method in which the 2-RDM rather than the wave function is the basic variable of the calculations. In agreement with experiment and in contrast with traditional wave function methods, the 2-RDM calculations predict the cage to be more stable than the prism after vibrational zero-point correction. Multiple configurations from the hydrogen bonding are captured by the method. More generally, the results are consistent with our previous 2-RDM applications in that they reveal how multireference correlation in molecular systems is important for resolving small energy differences from hydrogen bonding as well as other types of intermolecular forces, even in systems that are not conventionally considered strongly correlated.
C1 [Foley, Jonathan J.; Mazziotti, David A.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA.
[Foley, Jonathan J.; Mazziotti, David A.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA.
[Foley, Jonathan J.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
RP Mazziotti, DA (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA.
EM damazz@uchicago.edu
FU NSF [CHE-1152425]; ARO [W91 INF-1 1-504 1-0085]; Keck Foundation;
Microsoft Corporation
FX DAM. gratefully acknowledges the NSF under Grant No. CHE-1152425, the
ARO under Grant No. W91 INF-1 1-504 1-0085, the Keck Foundation, and
Microsoft Corporation for their support.
NR 36
TC 9
Z9 10
U1 0
U2 11
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 1
PY 2013
VL 117
IS 30
BP 6712
EP 6716
DI 10.1021/jp405739d
PG 5
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 196WE
UT WOS:000322807300032
PM 23841757
ER
PT J
AU Yu, J
Phelan, D
Rodriguez-Rivera, JA
Podlesnyak, A
Louca, D
AF Yu, J.
Phelan, D.
Rodriguez-Rivera, J. A.
Podlesnyak, A.
Louca, Despina
TI Magneto-Polaron Formation and Field-Induced Effects with Dilute Doping
in LaCo1-yNiyO3
SO JOURNAL OF SUPERCONDUCTIVITY AND NOVEL MAGNETISM
LA English
DT Article
DE Magnetic excitations; Local distortions; Polaron melting
ID MAGNETIC SEMICONDUCTORS; SPIN; TRANSITION; CLUSTERS; LACOO3
AB Dilute magnetic ion doping in LaCo1-yNiyO3 with y <= 1 % leads to the formation of isotropic magnetic clusters that exhibit intracluster interactions which are ferromagnetic in nature. The clusters are comprised of Ni ions surrounded by six magnetically polarized Co ions. The Ni spin is delocalized from the Ni3+ ion but is confined in the vicinity of the six Co coordinated environment forming small magneto-polarons. The cluster ground state is estimated from bulk magnetization to be about g S similar to 10, in contrast to LaCoO3, which is not magnetic. Using neutron spectroscopy, transitions are observed between the lowest energy levels indicating that the cluster ground state is split. Under a magnetic field of 1 Tesla, the transitions are suppressed while with increasing temperature, the intracluster transitions are overshadowed by the activation of the Co3+ ions to the intermediate spin state.
C1 [Yu, J.; Phelan, D.; Louca, Despina] Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA.
[Phelan, D.; Rodriguez-Rivera, J. A.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA.
[Rodriguez-Rivera, J. A.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA.
[Podlesnyak, A.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA.
RP Louca, D (reprint author), Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA.
EM Louca@virginia.edu
RI Instrument, CNCS/B-4599-2012; Rodriguez-Rivera, Jose/A-4872-2013;
Podlesnyak, Andrey/A-5593-2013
OI Rodriguez-Rivera, Jose/0000-0002-8633-8314; Podlesnyak,
Andrey/0000-0001-9366-6319
FU US Department of Energy at the University of Virginia
[DE-FG02-01ER45927]; National Science Foundation [DMR-0944772]
FX The authors would like to acknowledge valuable discussions with C.
Leighton and D. Khomskii. They also express their gratitude to K. Yamada
for providing them with the opportunity to grow some of the single
crystals at the Institute of Materials Research of Tohoku University.
This work is supported by the US Department of Energy under contracts
DE-FG02-01ER45927 at the University of Virginia. This work additionally
utilized facilities supported in part by the National Science Foundation
under Agreement No. DMR-0944772.
NR 25
TC 0
Z9 0
U1 0
U2 8
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1557-1939
J9 J SUPERCOND NOV MAGN
JI J. Supercond. Nov. Magn
PD AUG
PY 2013
VL 26
IS 8
BP 2627
EP 2632
DI 10.1007/s10948-013-2148-x
PG 6
WC Physics, Applied; Physics, Condensed Matter
SC Physics
GA 211QU
UT WOS:000323925500012
ER
PT J
AU Castelle, CJ
Hug, LA
Wrighton, KC
Thomas, BC
Williams, KH
Wu, DY
Tringe, SG
Singer, SW
Eisen, JA
Banfield, JF
AF Castelle, Cindy J.
Hug, Laura A.
Wrighton, Kelly C.
Thomas, Brian C.
Williams, Kenneth H.
Wu, Dongying
Tringe, Susannah G.
Singer, Steven W.
Eisen, Jonathan A.
Banfield, Jillian F.
TI Extraordinary phylogenetic diversity and metabolic versatility in
aquifer sediment
SO NATURE COMMUNICATIONS
LA English
DT Article
ID MULTIPLE SEQUENCE ALIGNMENT; ALTERNATIVE COMPLEX-III;
PYROBACULUM-AEROPHILUM; RHODOTHERMUS-MARINUS; MAXIMUM-LIKELIHOOD;
REDUCING BACTERIA; NITROGEN-FIXATION; HYDROTHERMAL VENT;
ELECTRON-TRANSFER; ESCHERICHIA-COLI
AB Microorganisms in the subsurface represent a substantial but poorly understood component of the Earth's biosphere. Subsurface environments are complex and difficult to characterize; thus, their microbiota have remained as a 'dark matter' of the carbon and other biogeochemical cycles. Here we deeply sequence two sediment-hosted microbial communities from an aquifer adjacent to the Colorado River, CO, USA. No single organism represents more than similar to 1% of either community. Remarkably, many bacteria and archaea in these communities are novel at the phylum level or belong to phyla lacking a sequenced representative. The dominant organism in deeper sediment, RBG-1, is a member of a new phylum. On the basis of its reconstructed complete genome, RBG-1 is metabolically versatile. Its wide respiration-based repertoire may enable it to respond to the fluctuating redox environment close to the water table. We document extraordinary microbial novelty and the importance of previously unknown lineages in sediment biogeochemical transformations.
C1 [Castelle, Cindy J.; Hug, Laura A.; Wrighton, Kelly C.; Thomas, Brian C.; Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.
[Williams, Kenneth H.; Singer, Steven W.; Banfield, Jillian F.] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Wu, Dongying; Eisen, Jonathan A.] Univ Calif Davis, UC Davis Genome Ctr, Davis, CA 95616 USA.
[Tringe, Susannah G.] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA.
[Tringe, Susannah G.] Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA.
[Eisen, Jonathan A.] Univ Calif Davis, Dept Ecol & Evolut, Davis, CA 95616 USA.
[Eisen, Jonathan A.] Univ Calif Davis, Dept Med Microbiol & Immunol, Davis, CA 95616 USA.
RP Banfield, JF (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.
EM jbanfield@berkeley.edu
RI Williams, Kenneth/O-5181-2014;
OI Williams, Kenneth/0000-0002-3568-1155; Tringe,
Susannah/0000-0001-6479-8427; Eisen, Jonathan A./0000-0002-0159-2197
FU Integrated Field Research Challenge, Subsurface Biogeochemical Research
Program, Office of Science, Biological and Environmental Research, the
US Department of Energy (DOE) [DE-AC02-05CH11231, DE-SC0004733]
FX Funding was provided through the Integrated Field Research Challenge,
Subsurface Biogeochemical Research Program, Office of Science,
Biological and Environmental Research, the US Department of Energy (DOE)
grants DE-AC02-05CH11231 to the Lawrence Berkeley National Laboratory
(operated by the University of California) and DE-SC0004733. Sequencing
was performed at the DOE Joint Genome Institute under the CSP Program.
NR 60
TC 62
Z9 62
U1 3
U2 69
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2120
DI 10.1038/ncomms3120
PG 10
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209IL
UT WOS:000323749100001
PM 23979677
ER
PT J
AU Chien, TY
Kourkoutis, LF
Chakhalian, J
Gray, B
Kareev, M
Guisinger, NP
Muller, DA
Freeland, JW
AF Chien, Te Yu
Kourkoutis, Lena F.
Chakhalian, Jak
Gray, Benjamin
Kareev, Michael
Guisinger, Nathan P.
Muller, David A.
Freeland, John W.
TI Visualizing short-range charge transfer at the interfaces between
ferromagnetic and superconducting oxides
SO NATURE COMMUNICATIONS
LA English
DT Article
ID ANDREEV REFLECTION; HETEROSTRUCTURES; SUPERLATTICES; JUNCTIONS
AB The interplay between antagonistic superconductivity and ferromagnetism has been a interesting playground to explore the interaction between competing ground states. Although this effect in systems of conventional superconductors is better understood, the framework of the proximity effect at complex-oxide-based superconductor/ferromagnet interfaces is not so clear. The main difficulty originates from the lack of experimental tools capable of probing the interfaces directly with high spatial resolution. Here we harness cross-sectional scanning tunnelling microscopy and spectroscopy together with atomic-resolution electron microscopy to understand the buried interfaces between cuprate and manganite layers. The results show that the fundamental length scale of the electronic evolution between YBa2Cu3O7-delta (YBCO) and La2/3Ca1/3MnO3 (LCMO) is confined to the subnanometre range. Our findings provide a complete and direct microscopic picture of the electronic transition across the YBCO/LCMO interfaces, which is an important step towards understanding the competition between ferromagnetism and superconductivity in complex-oxide heterostructures.
C1 [Chien, Te Yu; Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Kourkoutis, Lena F.; Muller, David A.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA.
[Kourkoutis, Lena F.; Muller, David A.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA.
[Chakhalian, Jak; Gray, Benjamin; Kareev, Michael] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA.
[Guisinger, Nathan P.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
RP Chien, TY (reprint author), Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA.
EM tchien@uwyo.edu; freeland@anl.gov
RI Chakhalian, Jak/F-2274-2015;
OI Muller, David/0000-0003-4129-0473; Kourkoutis, Lena/0000-0002-1303-1362
FU US Department of Energy, Office of Science, Office of Basic Energy
Sciences [DE-AC02-06CH11357]; NSF [DMR-0747808]; DOD-ARO
[W911NF-11-1-0200]; Army Research Office [W911NF0910415]; National
Science Foundation Materials Research Science and Engineering Centers
(MRSEC) program [DMR 1120296]
FX Work at Argonne, including the Center for Nanoscale Materials, is
supported by the US Department of Energy, Office of Science, Office of
Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The
majority of the research at the University of Arkansas was supported by
the grant from the NSF (DMR-0747808) and partially by DOD-ARO
(W911NF-11-1-0200). Work at Cornell is supported by the Army Research
Office under award W911NF0910415, and made use of the Cornell Center for
Materials Research (CCMR) electron microscopy facility supported by the
National Science Foundation Materials Research Science and Engineering
Centers (MRSEC) program (DMR 1120296).
NR 41
TC 27
Z9 27
U1 4
U2 108
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2336
DI 10.1038/ncomms3336
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209JV
UT WOS:000323752900003
PM 23939385
ER
PT J
AU Browne, E
Tuli, JK
AF Browne, E.
Tuli, J. K.
TI Nuclear Data Sheets for A=251-259(odd)
SO NUCLEAR DATA SHEETS
LA English
DT Article
ID NEUTRON-DEFICIENT ISOTOPES; ALPHA-GAMMA-DECAY; PRODUCTION
CROSS-SECTIONS; COLD-FUSION REACTIONS; FISSION HALF-LIVES;
SUPER-HEAVY-NUCLEI; ATOMIC MASS EVALUATION; UNIFIED THEORETICAL
FRAMEWORK; PARTICLE-EMITTING ISOTOPES; DINUCLEAR SYSTEM CONCEPT
AB The evaluators present in this publication spectroscopic data and level schemes from radioactive decay and nuclear reaction studies for all known nuclei with mass numbers A=251, 253, 255, 257, and 259.
C1 [Browne, E.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Lawrence Berkeley Natl Lab, Upton, NY 11973 USA.
[Tuli, J. K.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA.
RP Browne, E (reprint author), Brookhaven Natl Lab, Natl Nucl Data Ctr, Lawrence Berkeley Natl Lab, Upton, NY 11973 USA.
NR 357
TC 6
Z9 6
U1 1
U2 10
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0090-3752
J9 NUCL DATA SHEETS
JI Nucl. Data Sheets
PD AUG-SEP
PY 2013
VL 114
IS 8-9
BP 1041
EP 1185
DI 10.1016/j.nds.2013.08.002
PG 145
WC Physics, Nuclear
SC Physics
GA 210WH
UT WOS:000323865000002
ER
PT J
AU Menendez, D
Nguyen, TA
Freudenberg, JM
Mathew, VJ
Anderson, CW
Jothi, R
Resnick, MA
AF Menendez, Daniel
Thuy-Ai Nguyen
Freudenberg, Johannes M.
Mathew, Viju J.
Anderson, Carl W.
Jothi, Raja
Resnick, Michael A.
TI Diverse stresses dramatically alter genome-wide p53 binding and
transactivation landscape in human cancer cells
SO NUCLEIC ACIDS RESEARCH
LA English
DT Article
ID EMBRYONIC STEM-CELLS; TUMOR-SUPPRESSOR; DNA RECOGNITION; TRANSCRIPTIONAL
NETWORK; P53-BINDING SITES; RESPONSE ELEMENT; GENE; MUTATIONS; PROMOTER;
PROTEIN
AB The effects of diverse stresses on promoter selectivity and transcription regulation by the tumor suppressor p53 are poorly understood. We have taken a comprehensive approach to characterizing the human p53 network that includes p53 levels, binding, expression and chromatin changes under diverse stresses. Human osteosarcoma U2OS cells treated with anti-cancer drugs Doxorubicin (DXR) or Nutlin-3 (Nutlin) led to strikingly different p53 gene binding patterns based on chromatin immunoprecipitation with high-throughput sequencing experiments. Although two contiguous RRRCWWGYYY decamers is the consensus binding motif, p53 can bind a single decamer and function in vivo. Although the number of sites bound by p53 was six times greater for Nutlin than DXR, expression changes induced by Nutlin were much less dramatic compared with DXR. Unexpectedly, the solvent dimethylsulphoxide (DMSO) alone induced p53 binding to many sites common to DXR; however, this binding had no effect on target gene expression. Together, these data imply a two-stage mechanism for p53 transactivation where p53 binding only constitutes the first stage. Furthermore, both p53 binding and transactivation were associated with increased active histone modification histone H3 lysine 4 trimethylation. We discovered 149 putative new p53 target genes including several that are relevant to tumor suppression, revealing potential new targets for cancer therapy and expanding our understanding of the p53 regulatory network.
C1 [Menendez, Daniel; Thuy-Ai Nguyen; Anderson, Carl W.; Resnick, Michael A.] NIEHS, Chromosome Stabil Grp, Mol Genet Lab, NIH, Res Triangle Pk, NC 27709 USA.
[Freudenberg, Johannes M.; Mathew, Viju J.; Jothi, Raja] NIEHS, Syst Biol Grp, Mol Carcinogenesis Lab, NIH, Res Triangle Pk, NC 27709 USA.
[Mathew, Viju J.] William G Enloe High Sch, Raleigh, NC 27610 USA.
[Anderson, Carl W.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA.
RP Jothi, R (reprint author), NIEHS, Syst Biol Grp, Mol Carcinogenesis Lab, NIH, POB 12233, Res Triangle Pk, NC 27709 USA.
EM jothi@mail.nih.gov; resnick@niehs.nih.gov
RI Jothi, Raja/G-3780-2015
FU NIH, National Institute of Environmental Health Sciences [Z01-ES065079,
1ZIAES102625-04]
FX Funding for open access charge: Supported by the Intramural Research
Program of the NIH, National Institute of Environmental Health Sciences
[Z01-ES065079 to M. A. R., 1ZIAES102625-04 to R.J.].
NR 68
TC 52
Z9 52
U1 1
U2 12
PU OXFORD UNIV PRESS
PI OXFORD
PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND
SN 0305-1048
EI 1362-4962
J9 NUCLEIC ACIDS RES
JI Nucleic Acids Res.
PD AUG
PY 2013
VL 41
IS 15
BP 7286
EP 7301
DI 10.1093/nar/gkt504
PG 16
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 212GL
UT WOS:000323970700017
PM 23775793
ER
PT J
AU Sun, CM
Querol-Audi, J
Mortimer, SA
Arias-Palomo, E
Doudna, JA
Nogales, E
Cate, JHD
AF Sun, Chaomin
Querol-Audi, Jordi
Mortimer, Stefanie A.
Arias-Palomo, Ernesto
Doudna, Jennifer A.
Nogales, Eva
Cate, Jamie H. D.
TI Two RNA-binding motifs in eIF3 direct HCV IRES-dependent translation
SO NUCLEIC ACIDS RESEARCH
LA English
DT Article
ID HEPATITIS-C VIRUS; INITIATION-FACTOR 3; 40S RIBOSOMAL-SUBUNIT;
ELECTRON-MICROSCOPY; NEW-GENERATION; SHAPE CHEMISTRY; CODON SELECTION;
ENTRY SITE; MECHANISM; PARTICLE
AB The initiation of protein synthesis plays an essential regulatory role in human biology. At the center of the initiation pathway, the 13-subunit eukaryotic translation initiation factor 3 (eIF3) controls access of other initiation factors and mRNA to the ribosome by unknown mechanisms. Using electron microscopy (EM), bioinformatics and biochemical experiments, we identify two highly conserved RNA-binding motifs in eIF3 that direct translation initiation from the hepatitis C virus internal ribosome entry site (HCV IRES) RNA. Mutations in the RNA-binding motif of subunit eIF3a weaken eIF3 binding to the HCV IRES and the 40S ribosomal subunit, thereby suppressing eIF2-dependent recognition of the start codon. Mutations in the eIF3c RNA-binding motif also reduce 40S ribosomal subunit binding to eIF3, and inhibit eIF5B-dependent steps downstream of start codon recognition. These results provide the first connection between the structure of the central translation initiation factor eIF3 and recognition of the HCV genomic RNA start codon, molecular interactions that likely extend to the human transcriptome.
C1 [Sun, Chaomin; Querol-Audi, Jordi; Mortimer, Stefanie A.; Arias-Palomo, Ernesto; Doudna, Jennifer A.; Nogales, Eva; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA.
[Doudna, Jennifer A.; Cate, Jamie H. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
[Doudna, Jennifer A.; Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.
[Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
[Cate, Jamie H. D.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
RP Cate, JHD (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.
EM jcate@lbl.gov
FU National Institutes of Health (NIH) [R56-AI095687, P50-GM102706];
Spanish Ministry of Education through the Programa Nacional de Movilidad
de Recursos Humanos del Plan Nacional de I-D+i
FX National Institutes of Health (NIH) [R56-AI095687 to J.H.D.C.;
P50-GM102706 to J.A.D. and J.H.D.C.]; Spanish Ministry of Education
through the Programa Nacional de Movilidad de Recursos Humanos del Plan
Nacional de I-D+i 2008-2011 (to E. A.-P.). J.A.D. and E.N. are Howard
Hughes Medical Institute Investigators. Funding for open access charge:
NIH [P50-GM102706].
NR 52
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PU OXFORD UNIV PRESS
PI OXFORD
PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND
SN 0305-1048
J9 NUCLEIC ACIDS RES
JI Nucleic Acids Res.
PD AUG
PY 2013
VL 41
IS 15
BP 7512
EP 7521
DI 10.1093/nar/gkt510
PG 10
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 212GL
UT WOS:000323970700035
PM 23766293
ER
PT J
AU Baylor, LR
Commaux, N
Jernigan, TC
Meitner, SJ
Combs, SK
Isler, RC
Unterberg, EA
Brooks, NH
Evans, TE
Leonard, AW
Osborne, TH
Parks, PB
Snyder, PB
Strait, EJ
Fenstermacher, ME
Lasnier, CJ
Moyer, RA
Loarte, A
Huijsmans, GTA
Futatani, S
AF Baylor, L. R.
Commaux, N.
Jernigan, T. C.
Meitner, S. J.
Combs, S. K.
Isler, R. C.
Unterberg, E. A.
Brooks, N. H.
Evans, T. E.
Leonard, A. W.
Osborne, T. H.
Parks, P. B.
Snyder, P. B.
Strait, E. J.
Fenstermacher, M. E.
Lasnier, C. J.
Moyer, R. A.
Loarte, A.
Huijsmans, G. T. A.
Futatani, S.
TI Reduction of edge localized mode intensity on DIII-D by on-demand
triggering with high frequency pellet injection and implications for
ITER
SO PHYSICS OF PLASMAS
LA English
DT Article
ID D TOKAMAK; PLASMA; TRANSPORT; STABILITY; DYNAMICS; PEDESTAL
AB The injection of small deuterium pellets at high repetition rates up to 12x the natural edge localized mode (ELM) frequency has been used to trigger high-frequency ELMs in otherwise low natural ELM frequency H-mode deuterium discharges in the DIII-D tokamak [J. L. Luxon and L. G. Davis, Fusion Technol. 8, 441 (1985)]. The resulting pellet-triggered ELMs result in up to 12x lower energy and particle fluxes to the divertor than the natural ELMs. The plasma global energy confinement and density are not strongly affected by the pellet perturbations. The plasma core impurity density is strongly reduced with the application of the pellets. These experiments were performed with pellets injected from the low field side pellet in plasmas designed to match the ITER baseline configuration in shape and normalized beta operation with input heating power just above the H-mode power threshold. Nonlinear MHD simulations of the injected pellets show that destabilization of ballooning modes by a local pressure perturbation is responsible for the pellet ELM triggering. This strongly reduced ELM intensity shows promise for exploitation in ITER to control ELM size while maintaining high plasma purity and performance. (C) 2013 AIP Publishing LLC.
C1 [Baylor, L. R.; Commaux, N.; Jernigan, T. C.; Meitner, S. J.; Combs, S. K.; Isler, R. C.; Unterberg, E. A.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA.
[Brooks, N. H.; Evans, T. E.; Leonard, A. W.; Osborne, T. H.; Parks, P. B.; Snyder, P. B.; Strait, E. J.] Gen Atom Co, San Diego, CA 92186 USA.
[Fenstermacher, M. E.; Lasnier, C. J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Moyer, R. A.] Univ Calif San Diego, La Jolla, CA 92093 USA.
[Loarte, A.; Huijsmans, G. T. A.; Futatani, S.] ITER Org, F-13115 St Paul Les Durance, France.
RP Baylor, LR (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37830 USA.
FU Oak Ridge National Laboratory; US Department of Energy
[DE-AC05-00OR22725, DE-FC02-04ER54698, DE-AC52-07NA27344,
DE-FG02-07ER54917]
FX This work was supported by the Oak Ridge National Laboratory managed by
UT-Battelle, LLC for the US Department of Energy under
DE-AC05-00OR22725, and the US Department of Energy under
DE-FC02-04ER54698, DE-AC52-07NA27344, and DE-FG02-07ER54917. The views
and opinions expressed herein do not necessarily reflect those of the
ITER Organization. The authors also thank S. L. Milora, J. H. Harris, P.
T. Lang, and T. S. Taylor for enlightening discussions and support and
the DIII-D Team for operating the experiment.
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PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082513
DI 10.1063/1.4818772
PG 8
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800064
ER
PT J
AU Chung, M
Qin, H
Gilson, EP
Davidson, RC
AF Chung, Moses
Qin, Hong
Gilson, Erik P.
Davidson, Ronald C.
TI Analysis of continuously rotating quadrupole focusing channels using
generalized Courant-Snyder theory
SO PHYSICS OF PLASMAS
LA English
DT Article
ID FIELDS
AB By extending the recently developed generalized Courant-Snyder theory for coupled transverse beam dynamics, we have constructed the Gaussian beam distribution and its projections with arbitrary mode emittance ratios. The new formulation has been applied to a continuously rotating quadrupole focusing channel because the basic properties of this channel are known theoretically and could also be investigated experimentally in a compact setup such as the linear Paul trap configuration. The new formulation retains a remarkably similar mathematical structure to the original Courant-Snyder theory, and thus, provides a powerful theoretical tool to investigate coupled transverse beam dynamics in general and more complex linear focusing channels. (C) 2013 AIP Publishing LLC.
C1 [Chung, Moses] Fermilab Natl Accelerator Lab, Accelerator Phys Ctr, Batavia, IL 60510 USA.
[Qin, Hong; Gilson, Erik P.; Davidson, Ronald C.] Princeton Univ, Plasma Phys Lab, Princeton, NJ 08543 USA.
[Qin, Hong] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China.
RP Chung, M (reprint author), Fermilab Natl Accelerator Lab, Accelerator Phys Ctr, Batavia, IL 60510 USA.
FU U.S. Department of Energy [DE-AC02-09CH11466]; United States Department
of Energy [DE-AC02-07CH11359]
FX This research was supported by the U.S. Department of Energy (Contract
Number DE-AC02-09CH11466). Fermilab is operated by Fermi Research
Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United
States Department of Energy.
NR 25
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U1 1
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PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 083121
DI 10.1063/1.4819830
PG 6
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800097
ER
PT J
AU Clark, SE
Winske, D
Schaeffer, DB
Everson, ET
Bondarenko, AS
Constantin, CG
Niemann, C
AF Clark, S. E.
Winske, D.
Schaeffer, D. B.
Everson, E. T.
Bondarenko, A. S.
Constantin, C. G.
Niemann, C.
TI Hybrid simulation of shock formation for super-Alfvenic expansion of
laser ablated debris through an ambient, magnetized plasma
SO PHYSICS OF PLASMAS
LA English
DT Article
ID COLLISIONLESS-SHOCK; FIELD; WAVELENGTHS; DYNAMICS; DESIGN; MODEL
AB Two-dimensional hybrid simulations of perpendicular collisionless shocks are modeled after potential laboratory conditions that are attainable in the LArge Plasma Device (LAPD) at the University of California, Los Angeles Basic Plasma Science Facility. The kJ class 1053nm Nd:Glass Raptor laser will be used to ablate carbon targets in the LAPD with on-target energies of 100-500 J. The ablated debris ions will expand into ambient, partially ionized hydrogen or helium. A parameter study is performed via hybrid simulation to determine possible conditions that could lead to shock formation in future LAPD experiments. Simulation results are presented along with a comparison to an analytical coupling parameter. (C) 2013 AIP Publishing LLC.
C1 [Clark, S. E.; Schaeffer, D. B.; Everson, E. T.; Bondarenko, A. S.; Constantin, C. G.; Niemann, C.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA.
[Winske, D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Clark, SE (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA.
EM clarkse@physics.ucla.edu
FU Defense Threat Reduction Agency (DTRA) [HDTRA1-12-1-0024]; DOE Office of
Science Early Career Research Program [DE-FOA-0000395]
FX This work was supported by the Defense Threat Reduction Agency (DTRA)
under Contract No. HDTRA1-12-1-0024 and by the DOE Office of Science
Early Career Research Program (DE-FOA-0000395).
NR 31
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PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082129
DI 10.1063/1.4819251
PG 8
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800032
ER
PT J
AU Dewar, RL
Bhattacharjee, A
Kulsrud, RM
Wright, AM
AF Dewar, R. L.
Bhattacharjee, A.
Kulsrud, R. M.
Wright, A. M.
TI Plasmoid solutions of the Hahm-Kulsrud-Taylor equilibrium model
SO PHYSICS OF PLASMAS
LA English
DT Article
ID MAGNETIC RECONNECTION; TEARING INSTABILITY; CURRENT SHEETS; FIELD; LAYER
AB The Hahm-Kulsrud (HK) [T.S. Hahm and R. M. Kulsrud, Phys. Fluids 28, 2412 (1985)] solutions for a magnetically sheared plasma slab driven by a resonant periodic boundary perturbation illustrate fully shielded (current sheet) and fully reconnected (magnetic island) responses. On the global scale, reconnection involves solving a magnetohydrodynamic (MHD) equilibrium problem. In systems with a continuous symmetry, such MHD equilibria are typically found by solving the Grad-Shafranov equation, and in slab geometry the elliptic operator in this equation is the 2-D Laplacian. Thus, assuming appropriate pressure and poloidal current profiles, a conformal mapping method can be used to transform one solution into another with different boundary conditions, giving a continuous sequence of solutions in the form of partially reconnected magnetic islands (plasmoids) separated by Syrovatsky current sheets. The two HK solutions appear as special cases. (C) 2013 AIP Publishing LLC.
C1 [Dewar, R. L.] Australian Natl Univ, Plasma Res Lab, Res Sch Phys & Engn, Canberra, ACT 0200, Australia.
[Dewar, R. L.] Univ Tokyo, Grad Sch Frontier Sci, Kashiwa, Chiba 2778561, Japan.
[Bhattacharjee, A.; Kulsrud, R. M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Wright, A. M.] Australian Natl Univ, Canberra, ACT 0200, Australia.
RP Dewar, RL (reprint author), Australian Natl Univ, Plasma Res Lab, Res Sch Phys & Engn, GPO Box 4, Canberra, ACT 0200, Australia.
EM robert.dewar@anu.edu.au; abhattac@pppl.gov; rkulsrud@pppl.gov
RI Dewar, Robert/B-1300-2008
OI Dewar, Robert/0000-0002-9518-7087
FU Australian Research Council; U.S. National Science Foundation;
Department of Energy
FX One of the authors (RLD) would like to thank the hospitality of and
stimulating conversations with Roger Hosking, as the idea behind this
paper was conceived during work on our book, still in preparation,
"Fundamentals of Fluid Mechanics and MHD." He would also like to thank
the hospitality of Princeton Plasma Physics Laboratory where the first
draft was written and of Zensho Yoshida at the University of Tokyo where
the work was completed. This research has been supported by the
Australian Research Council and the U.S. National Science Foundation and
Department of Energy. The plots were made using Mathematica
9.31
NR 31
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U1 0
U2 8
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082103
DI 10.1063/1.4817276
PG 7
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800006
ER
PT J
AU Dorf, MA
Cohen, RH
Simakov, AN
Joseph, I
AF Dorf, M. A.
Cohen, R. H.
Simakov, A. N.
Joseph, I.
TI On the applicability of the standard approaches for evaluating a
neoclassical radial electric field in a tokamak edge region
SO PHYSICS OF PLASMAS
LA English
DT Article
ID PLASMA EDGE; TRANSPORT
AB The use of the standard approaches for evaluating a neoclassical radial electric field Er, i.e., the Ampere (or gyro-Poisson) equation, requires accurate calculation of the difference between the gyroaveraged electron and ion particle fluxes (or densities). In the core of a tokamak, the nontrivial difference appears only in high-order corrections to a local Maxwellian distribution due to the intrinsic ambipolarity of particle transport. The evaluation of such high-order corrections may be inconsistent with the accuracy of the standard long wavelength gyrokinetic equation (GKE), thus imposing limitations on the applicability of the standard approaches. However, in the edge of a tokamak, charge-exchange collisions with neutrals and prompt ion orbit losses can drive non-intrinsically ambipolar particle fluxes for which a nontrivial (Er-dependent) difference between the electron and ion fluxes appears already in a low order and can be accurately predicted by the long wavelength GKE. The parameter regimes, where the radial electric field dynamics in the tokamak edge region is dominated by the non-intrinsically ambipolar processes, thus allowing for the use of the standard approaches, are discussed. (C) 2013 AIP Publishing LLC.
C1 [Dorf, M. A.; Cohen, R. H.; Joseph, I.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Simakov, A. N.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA.
RP Dorf, MA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
OI Simakov, Andrei/0000-0001-7064-9153
FU U.S. Department of Energy [DE-AC52-07NA27344, DE-AC52-06NA-25396]
FX The authors are grateful to A. Dimits, M. Umansky, T. Rognlien, B.
Cohen, and D. Ryutov for fruitful discussions. This research was
supported by the U.S. Department of Energy under contracts
DE-AC52-07NA27344 and DE-AC52-06NA-25396.
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U2 8
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082515
DI 10.1063/1.4818777
PG 6
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800066
ER
PT J
AU Farmer, WA
Morales, GJ
AF Farmer, W. A.
Morales, G. J.
TI Propagation of shear Alven waves in two-ion species plasmas confined by
a nonuniform magnetic field
SO PHYSICS OF PLASMAS
LA English
DT Article
ID ION-CYCLOTRON; CONVERSION; TOKAMAK; ALFVEN
AB Ray tracing calculations are performed for shear Alfven waves in two-ion species plasmas in which the magnetic field varies with position. Three different magnetic topologies of contemporary interest are explored: a linear magnetic mirror, a pure toroidal field, and a tokamak field. The wave frequency is chosen to lie in the upper propagation band, so that reflection at the ion-ion hybrid frequency can occur for waves originally propagating along the magnetic field direction. Calculations are performed for a magnetic well configuration used in recent experiments [S. T. Vincena et al., Geophys. Res. Lett. 38, L11101 (2011) and S. T. Vincena et al., Phys. Plasmas 20, 012111 (2013)] in the Large Plasma Device (LAPD) related to the ion-ion hybrid resonator. It is found that radial spreading cannot explain the relatively low values of the resonator quality factor (Q) measured in those experiments, even when finite ion temperature is considered. This identifies that a damping mechanism is present that is at least an order of magnitude larger than dissipation due to radial energy loss. Calculations are also performed for a magnetic field with pure toroidal geometry, without a poloidal field, as in experiments being planned for the Enormous Toroidal Plasma Device. In this case, the effects of field-line curvature cause radial reflections. A poloidal field is included to explore a tokamak geometry with plasma parameters expected in ITER. When ion temperature is ignored, it is found that the ion-ion hybrid resonator can exist and trap waves for multiples bounces. The effects of finite ion temperature combine with field line curvature to cause the reflection point to move towards the tritium cyclotron frequency when electron temperature is negligible. However, for ITER parameters, it is shown that the electrons must be treated in the adiabatic limit to properly describe resonator phenomena. (C) 2013 AIP Publishing LLC.
C1 [Farmer, W. A.; Morales, G. J.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA.
[Farmer, W. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
RP Farmer, WA (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA.
FU DOE [DE-SC0007791]; U.S. Department of Energy by Lawrence Livermore
National Laboratory [DE-AC52-07NA27344]
FX The work at UCLA was sponsored by DOE Grant DE-SC0007791. W. A. F. is a
Lawrence scholar and his work was performed under the auspices of the
U.S. Department of Energy by Lawrence Livermore National Laboratory
under Contract DE-AC52-07NA27344.
NR 24
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PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082132
DI 10.1063/1.4819776
PG 16
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800035
ER
PT J
AU French, DM
Shiffler, D
Cartwright, K
AF French, David M.
Shiffler, Don
Cartwright, Keith
TI Electron beam coupling to a metamaterial structure
SO PHYSICS OF PLASMAS
LA English
DT Article
ID CERENKOV; PERMITTIVITY; PERMEABILITY; RADIATION; MASER
AB Microwave metamaterials have shown promise in numerous applications, ranging from strip lines and antennas to metamaterial-based electron beam driven devices. In general, metamaterials allow microwave designers to obtain electromagnetic characteristics not typically available in nature. High Power Microwave (HPM) sources have in the past drawn inspiration from work done in the conventional microwave source community. In this article, the use of metamaterials in an HPM application is considered by using an effective medium model to determine the coupling of an electron beam to a metamaterial structure in a geometry similar to that of a dielectric Cerenkov maser. Use of the effective medium model allows for the analysis of a wide range of parameter space, including the "mu-negative," "epsilon-negative," and "double negative" regimes of the metamaterial. The physics of such a system are modeled analytically and by utilizing the particle-in-cell code ICEPIC. For this geometry and effective medium representation, optimum coupling of the electron beam to the metamaterial, and thus the optimum microwave or RF production, occurs in the epsilon negative regime of the metamaterial. Given that HPM tubes have been proposed that utilize a metamaterial, this model provides a rapid method of characterizing a source geometry that can be used to quickly understand the basic physics of such an HPM device. (C) 2013 AIP Publishing LLC.
C1 [French, David M.; Shiffler, Don] Air Force Res Lab, Directed Energy Directorate, Albuquerque, NM 87117 USA.
[Cartwright, Keith] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP French, DM (reprint author), Air Force Res Lab, Directed Energy Directorate, Albuquerque, NM 87117 USA.
FU Air Force Office of Scientific Research
FX The authors wish to thank the Air Force Office of Scientific Research
for supporting this project and would also like to thank Dr. Wilkin
Tang, Professor Y. Y. Lau, and Dr. John Luginsland for useful
discussions as well as Dr. Andrew Greenwood for his computational
support.
NR 31
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U1 2
U2 27
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 083116
DI 10.1063/1.4817021
PG 8
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800092
ER
PT J
AU Gee, A
Shin, YM
AF Gee, Anthony
Shin, Young-Min
TI Gain analysis of higher-order-mode amplification in a
dielectric-implanted multi-beam traveling wave structure (vol 20,
073106, 2013)
SO PHYSICS OF PLASMAS
LA English
DT Correction
C1 [Gee, Anthony; Shin, Young-Min] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.
[Shin, Young-Min] Fermilab Natl Accelerator Lab, Accelerator Phys Ctr, Batavia, IL 60510 USA.
RP Gee, A (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.
NR 1
TC 0
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U1 0
U2 9
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 089901
DI 10.1063/1.4818504
PG 1
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800129
ER
PT J
AU Heidbrink, WW
Austin, ME
Spong, DA
Tobias, BJ
Van Zeeland, MA
AF Heidbrink, W. W.
Austin, M. E.
Spong, D. A.
Tobias, B. J.
Van Zeeland, M. A.
TI Measurements of the eigenfunction of reversed shear Alfven eigenmodes
that sweep downward in frequency
SO PHYSICS OF PLASMAS
LA English
DT Article
ID DIII-D; WAVE CASCADES; JET TOKAMAK; SPECTROSCOPY; DISCHARGES; JT-60U;
PLASMAS; DRIVEN
AB Reversed shear Alfven eigenmodes (RSAEs) usually sweep upward in frequency when the minimum value of the safety factor q(min) decreases in time. On rare occasions, RSAEs sweep downward prior to the upward sweep. Electron cyclotron emission measurements show that the radial eigenfunction during the downsweeping phase is similar to the eigenfunction of normal, upsweeping RSAEs. (C) 2013 AIP Publishing LLC.
C1 [Heidbrink, W. W.] Univ Calif Irvine, Irvine, CA 92697 USA.
[Austin, M. E.] Univ Texas Austin, Austin, TX 78712 USA.
[Spong, D. A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Tobias, B. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Van Zeeland, M. A.] Gen Atom Co, San Diego, CA 92186 USA.
RP Heidbrink, WW (reprint author), Univ Calif Irvine, Irvine, CA 92697 USA.
EM heidbrink@fusion.gat.com
FU U.S. Department of Energy [SC-G903402, DE-FG03-97ER54415,
DE-AC05-0000R22725, DE-AC02-09CH11466, DE-FC02-04ER54698]
FX This work was supported by the U.S. Department of Energy under
SC-G903402, DE-FG03-97ER54415, DE-AC05-0000R22725, DE-AC02-09CH11466,
and DE-FC02-04ER54698. We thank the DIII-D Team for their support and E.
M. Bass, B. Breizman, W. Deng, and E. J. Strait for helpful discussions.
NR 54
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PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082504
DI 10.1063/1.4817950
PG 7
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800055
ER
PT J
AU Huang, YM
Bhattacharjee, A
Forbes, TG
AF Huang, Yi-Min
Bhattacharjee, A.
Forbes, Terry G.
TI Magnetic reconnection mediated by hyper-resistive plasmoid instability
SO PHYSICS OF PLASMAS
LA English
DT Article
ID EJECTION CURRENT SHEETS; NUMERICAL EXPERIMENTS; KINETIC SIMULATIONS;
SOLAR CORONA; TEARING MODE; MECHANISM; TEMPERATURE; ISLANDS; THICKNESS
AB Magnetic reconnection mediated by the hyper-resistive plasmoid instability is studied with both linear analysis and nonlinear simulations. The linear growth rate is found to scale as S-H(1/6) with respect to the hyper-resistive Lundquist number S-H equivalent to (LVA)-V-3/eta(H), where L is the system size, V-A is the Alfven velocity, and eta(H) is the hyper-resistivity. In the nonlinear regime, reconnection rate becomes nearly independent of S-H, the number of plasmoids scales as S-H(1/2), and the secondary current sheet length and width both scale as S-H(-1/2). These scalings are consistent with a heuristic argument assuming secondary current sheets are close to marginal stability. The distribution of plasmoids as a function of the enclosed flux psi is found to obey a psi (1) power law over an extended range, followed by a rapid fall off for large plasmoids. These results are compared with those from resistive magnetohydrodynamic studies. (C) 2013 AIP Publishing LLC.
C1 [Huang, Yi-Min; Bhattacharjee, A.] Ctr Integrated Computat & Anal Reconnect & Turbul, Princeton, NJ 08543 USA.
[Huang, Yi-Min; Bhattacharjee, A.] Ctr Magnet Self Org Lab & Astrophys Plasmas, Princeton, NJ 08543 USA.
[Huang, Yi-Min; Bhattacharjee, A.] Max Planck Princeton Ctr Plasma Phys, Princeton, NJ 08543 USA.
[Huang, Yi-Min; Bhattacharjee, A.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Forbes, Terry G.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA.
RP Huang, YM (reprint author), Ctr Integrated Computat & Anal Reconnect & Turbul, Princeton, NJ 08543 USA.
EM yiminh@princeton.edu
RI Huang, Yi-Min/G-6926-2011
OI Huang, Yi-Min/0000-0002-4237-2211
FU Department of Energy under the Center for Integrated Computation and
Analysis of Reconnection and Turbulence (CICART) [DE-FG02-07ER46372];
National Science Foundation [PHY-0215581]; NASA [NNX09AJ86G, NNX10AC04G,
NNM07AA02C]; NSF [ATM-0802727, ATM-090315, AGS-0962698]
FX This work was supported by the Department of Energy, Grant No.
DE-FG02-07ER46372, under the auspice of the Center for Integrated
Computation and Analysis of Reconnection and Turbulence (CICART), the
National Science Foundation, Grant No. PHY-0215581 (PFC: Center for
Magnetic Self-Organization in Laboratory and Astrophysical Plasmas),
NASA Grant Nos. NNX09AJ86G and NNX10AC04G, and NSF Grant Nos.
ATM-0802727, ATM-090315 and AGS-0962698. Y.M.H. is partially supported
by a NASA subcontract to the Smithsonian Astrophysical Observatory's
Center of Astrophysics, Grant No. NNM07AA02C. Computations were
performed on facilities at National Energy Research Scientific Computing
Center.
NR 60
TC 7
Z9 7
U1 1
U2 7
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082131
DI 10.1063/1.4819715
PG 9
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800034
ER
PT J
AU Jung, D
Yin, L
Gautier, DC
Wu, HC
Letzring, S
Dromey, B
Shah, R
Palaniyappan, S
Shimada, T
Johnson, RP
Schreiber, J
Habs, D
Fernandez, JC
Hegelich, BM
Albright, BJ
AF Jung, D.
Yin, L.
Gautier, D. C.
Wu, H. -C.
Letzring, S.
Dromey, B.
Shah, R.
Palaniyappan, S.
Shimada, T.
Johnson, R. P.
Schreiber, J.
Habs, D.
Fernandez, J. C.
Hegelich, B. M.
Albright, B. J.
TI Laser-driven 1 GeV carbon ions from preheated diamond targets in the
break-out afterburner regime
SO PHYSICS OF PLASMAS
LA English
DT Article
ID ACCELERATION; BEAMS
AB Experimental data are presented for laser-driven carbon C6+ ion-acceleration, verifying 2D-PIC studies for multi-species targets in the Break-Out Afterburner regime. With Trident's ultra-high contrast at relativistic intensities of 5 x 10(20) W/cm(2) and nm-scale diamond targets, acceleration of carbon ions has been optimized by using target laser-preheating for removal of surface proton contaminants. Using a high-resolution wide angle spectrometer, carbon C6+ ion energies exceeding 1 GeV or 83 MeV/amu have been measured, which is a 40% increase in maximum ion energy over uncleaned targets. These results are consistent with kinetic plasma modeling and analytic theory. (C) 2013 AIP Publishing LLC.
C1 [Jung, D.; Yin, L.; Gautier, D. C.; Wu, H. -C.; Letzring, S.; Shah, R.; Palaniyappan, S.; Shimada, T.; Johnson, R. P.; Fernandez, J. C.; Hegelich, B. M.; Albright, B. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Jung, D.; Schreiber, J.; Habs, D.] Univ Munich, Dept Phys, D-85748 Garching, Germany.
[Jung, D.; Schreiber, J.; Habs, D.] Max Planck Inst Quantum Opt, D-85748 Garching, Germany.
[Dromey, B.] Queens Univ Belfast, Belfast BT7 1NN, Antrim, North Ireland.
RP Jung, D (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM daniel.jung@outlook.com
RI Hegelich, Bjorn/J-2689-2013; Fernandez, Juan/H-3268-2011; palaniyappan,
sasikumar/A-7791-2015;
OI Fernandez, Juan/0000-0002-1438-1815; Albright,
Brian/0000-0002-7789-6525; Yin, Lin/0000-0002-8978-5320; Palaniyappan,
sasi/0000-0001-6377-1206
FU DOE OFES; Deutsche Forschungsgemeinschaft (DFG) [Transregio SFB TR18];
DFG Cluster of Excellence Munich-Center for Advanced Photonics (MAP);
DFG LMU-Excellence; U.S. Department of Energy by the Los Alamos National
Security, LLC, Los Alamos National Laboratory
FX We are grateful for the support of the Trident laser team in conducting
the experiments. The simulations were run on the LANL ASC Roadrunner and
Cielo supercomputers. Work was supported by DOE OFES, Deutsche
Forschungsgemeinschaft (DFG) through Transregio SFB TR18, DFG Cluster of
Excellence Munich-Center for Advanced Photonics (MAP), and DFG
LMU-Excellence. Work performed under the auspices of the U.S. Department
of Energy by the Los Alamos National Security, LLC, Los Alamos National
Laboratory.
NR 41
TC 29
Z9 29
U1 2
U2 36
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 083103
DI 10.1063/1.4817287
PG 9
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800079
ER
PT J
AU Ni, PA
Lund, SM
McGuffey, C
Alexander, N
Aurand, B
Barnard, JJ
Beg, FN
Bellei, C
Bieniosek, FM
Brabetz, C
Cohen, RH
Kim, J
Neumayer, P
Roth, M
Logan, BG
AF Ni, P. A.
Lund, S. M.
McGuffey, C.
Alexander, N.
Aurand, B.
Barnard, J. J.
Beg, F. N.
Bellei, C.
Bieniosek, F. M.
Brabetz, C.
Cohen, R. H.
Kim, J.
Neumayer, P.
Roth, M.
Logan, B. G.
TI Initial experimental evidence of self-collimation of
target-normal-sheath-accelerated proton beam in a stack of conducting
foils
SO PHYSICS OF PLASMAS
LA English
DT Article
ID PLASMA; LENS
AB Phenomena consistent with self-collimation (or weak self-focusing) of laser target-normal-sheath-accelerated protons was experimentally observed for the first time, in a specially engineered structure ("lens") consisting of a stack of 300 thin aluminum foils separated by 50 mu m vacuum gaps. The experiments were carried out in a "passive environment," i.e., no external fields applied, neutralization plasma or injection of secondary charged particles was imposed. Experiments were performed at the petawatt "PHELIX" laser user facility (E = 100 J, Delta t = 400 fs, lambda = 1062 nm) at the "Helmholtzzentrum fur Schwerionenforschung-GSI" in Darmstadt, Germany. The observed rms beam spot reduction depends inversely on energy, with a focusing degree decreasing monotonically from 2 at 5.4 MeV to 1.5 at 18.7 MeV. The physics inside the lens is complex, resulting in a number of different mechanisms that can potentially affect the particle dynamics within the structure. We present a plausible simple interpretation of the experiment in which the combination of magnetic self-pinch forces generated by the beam current together with the simultaneous reduction of the repulsive electrostatic forces due to the foils are the dominant mechanisms responsible for the observed focusing/collimation. This focusing technique could be applied to a wide variety of space-charge dominated proton and heavy ion beams and impact fields and applications, such as HEDP science, inertial confinement fusion in both fast ignition and heavy ion fusion approaches, compact laser-driven injectors for a Linear Accelerator (LINAC) or synchrotron, medical therapy, materials processing, etc. (C) 2013 AIP Publishing LLC.
C1 [Ni, P. A.; Bieniosek, F. M.; Logan, B. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Lund, S. M.; Barnard, J. J.; Bellei, C.; Cohen, R. H.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
[McGuffey, C.; Beg, F. N.; Kim, J.] Univ Calif San Diego, La Jolla, CA 92093 USA.
[Alexander, N.] Gen Atom Co, San Diego, CA 92121 USA.
[Aurand, B.; Brabetz, C.; Neumayer, P.] GSI Darmstadt, D-64291 Darmstadt, Germany.
[Roth, M.] Tech Univ Darmstadt, D-64289 Darmstadt, Germany.
RP Ni, PA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
OI Brabetz, Christian/0000-0003-2009-0982
FU U.S. Department of Energy at the Lawrence Berkeley and Lawrence
Livermore and National Laboratories [DE-AC02-05CH11231,
DE-AC52-07NA27344]; US DOE, OFES, under HEDLP [DE-FOA-0000583]
FX The authors would like to thank Joe Kwan (LBNL), Alex Friedman (LLNL),
Harry McLean (LLNL), Prav Patel (LLNL), and Gabriel Schaumann
(TU-Darmstadt) for fruitful technical discussions. We also want to thank
the technical team of PHELIX for support of the experiments and General
Atomics for providing the targets for the experiments. The authors sadly
note the untimely passing of our friend, colleague, and co-author Frank
Bieniosek. His clarity of scientific vision, his energy and enthusiasm,
guidance, and companionship are missed. This research was performed
under the auspices of the U.S. Department of Energy at the Lawrence
Berkeley and Lawrence Livermore and National Laboratories under contract
numbers DE-AC02-05CH11231 and DE-AC52-07NA27344 and was partially
supported by the US DOE, OFES, under HEDLP proposal #DE-FOA-0000583.
NR 31
TC 3
Z9 4
U1 0
U2 11
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 083111
DI 10.1063/1.4818147
PG 6
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800087
ER
PT J
AU Podesta, M
Gorelenkov, NN
White, RB
Fredrickson, ED
Gerhardt, SP
Kramer, GJ
AF Podesta, M.
Gorelenkov, N. N.
White, R. B.
Fredrickson, E. D.
Gerhardt, S. P.
Kramer, G. J.
TI Properties of Alfven eigenmodes in the Toroidal Alfven Eigenmode range
on the National Spherical Torus Experiment-Upgrade
SO PHYSICS OF PLASMAS
LA English
DT Article
ID PLASMAS; EXCITATION; STABILITY; PHYSICS
AB A second Neutral Beam (NB) injection line is being installed on the NSTX Upgrade device, resulting in six NB sources with different tangency radii that will be available for heating and current drive. This work explores the properties of instabilities in the frequency range of the Toroidal Alfven Eigenmode (TAE) for NSTX-U scenarios with various NB injection geometries, from more perpendicular to more tangential, and with increased toroidal magnetic field with respect to previous NSTX scenarios. Predictions are based on analysis through the ideal MHD code NOVA-K. For the scenarios considered in this work, modifications of the Alfven continuum result in a frequency up-shift and a broadening of the radial mode structure. The latter effect may have consequences for fast ion transport and loss. Preliminary stability considerations indicate that TAEs are potentially unstable with ion Landau damping representing the dominant damping mechanism. (C) 2013 AIP Publishing LLC.
C1 [Podesta, M.; Gorelenkov, N. N.; White, R. B.; Fredrickson, E. D.; Gerhardt, S. P.; Kramer, G. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Podesta, M (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
RI White, Roscoe/D-1773-2013
OI White, Roscoe/0000-0002-4239-2685
FU US-DoE [DE-AC02-09CH11466]
FX Work supported by US-DoE Contract DE-AC02-09CH11466.
NR 28
TC 3
Z9 3
U1 0
U2 8
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082502
DI 10.1063/1.4817277
PG 11
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800053
ER
PT J
AU Qin, H
Zhang, SX
Xiao, JY
Liu, J
Sun, YJ
Tang, WM
AF Qin, Hong
Zhang, Shuangxi
Xiao, Jianyuan
Liu, Jian
Sun, Yajuan
Tang, William M.
TI Why is Boris algorithm so good?
SO PHYSICS OF PLASMAS
LA English
DT Article
AB Due to its excellent long term accuracy, the Boris algorithm is the de facto standard for advancing a charged particle. Despite its popularity, up to now there has been no convincing explanation why the Boris algorithm has this advantageous feature. In this paper, we provide an answer to this question. We show that the Boris algorithm conserves phase space volume, even though it is not symplectic. The global bound on energy error typically associated with symplectic algorithms still holds for the Boris algorithm, making it an effective algorithm for the multi-scale dynamics of plasmas. (C) 2013 AIP Publishing LLC.
C1 [Qin, Hong; Zhang, Shuangxi; Xiao, Jianyuan; Liu, Jian] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China.
[Qin, Hong; Zhang, Shuangxi; Xiao, Jianyuan; Liu, Jian] Univ Sci & Technol China, Collaborat Innovat Ctr Adv Fus Energy & Plasma Sc, Hefei 230026, Anhui, Peoples R China.
[Qin, Hong; Tang, William M.] Princeton Univ, Plasma Phys Lab, Princeton, NJ 08543 USA.
[Sun, Yajuan] Chinese Acad Sci, Acad Math & Syst Sci, LSEC, Beijing 100190, Peoples R China.
RP Qin, H (reprint author), Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China.
RI Liu, Jian/E-5857-2010
FU ITER-China Program [2010GB107001, 2011GB106000, 2011GB105003]; National
Natural Science Foundation of China [NSFC-11075162]; U.S. Department of
Energy [DE-AC02-09CH111466]
FX This research was supported by the ITER-China Program (2010GB107001,
2011GB106000, and 2011GB105003), National Natural Science Foundation of
China (NSFC-11075162), and U.S. Department of Energy
(DE-AC02-09CH111466). We thank Professor Yifa Tang and Professor Zaijiu
Shang for fruitful discussion on symplectic and volume-preserving
algorithms.
NR 12
TC 30
Z9 31
U1 0
U2 14
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 084503
DI 10.1063/1.4818428
PG 4
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800128
ER
PT J
AU Restante, AL
Markidis, S
Lapenta, G
Intrator, T
AF Restante, A. L.
Markidis, S.
Lapenta, G.
Intrator, T.
TI Geometrical investigation of the kinetic evolution of the magnetic field
in a periodic flux rope
SO PHYSICS OF PLASMAS
LA English
DT Article
ID QUASI-SEPARATRIX LAYERS; CORONAL MASS EJECTIONS; SOLAR CORONA; NONLINEAR
EVOLUTION; KINK INSTABILITY; POINCARE MAPS; RECONNECTION; PLASMA; MODEL;
TUBES
AB Flux ropes are bundles of magnetic field wrapped around an axis. Many laboratory, space, and astrophysics processes can be represented using this idealized concept. Here, a massively parallel 3D kinetic simulation of a periodic flux rope undergoing the kink instability is studied. The focus is on the topology of the magnetic field and its geometric structures. The analysis considers various techniques such as Poincare maps and the quasi-separatrix layer (QSL). These are used to highlight regions with expansion or compression and changes in the connectivity of magnetic field lines and consequently to outline regions where heating and current may be generated due to magnetic reconnection. The present study is, to our knowledge, the first QSL analysis of a fully kinetic 3D particle in cell simulation and focuses the existing QSL method of analysis to periodic systems. (C) 2013 AIP Publishing LLC.
C1 [Restante, A. L.; Lapenta, G.] Univ Louvain, KULeuven, Dept Wiskunde, Afdeling Plasma Astrofys, Louvain, Belgium.
[Markidis, S.] KTH Royal Inst Technol, High Performance Comp & Visualizat HPCViz Dept, Stockholm, Sweden.
[Intrator, T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Restante, AL (reprint author), Univ Louvain, KULeuven, Dept Wiskunde, Afdeling Plasma Astrofys, Louvain, Belgium.
FU European Commission [2633430]
FX The research leading to these results has received funding from the
European Commission's Seventh Framework Programme (FP7/2007-2013) inside
the Grant agreement SWIFF (Project No. 2633430, www.swiff.eu).
NR 64
TC 5
Z9 5
U1 0
U2 4
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082501
DI 10.1063/1.4817167
PG 9
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800052
ER
PT J
AU Schroeder, CB
Esarey, E
Benedetti, C
Leemans, WP
AF Schroeder, C. B.
Esarey, E.
Benedetti, C.
Leemans, W. P.
TI Control of focusing forces and emittances in plasma-based accelerators
using near-hollow plasma channels
SO PHYSICS OF PLASMAS
LA English
DT Article
ID WAKEFIELD ACCELERATOR; BEAM; ELECTRONS
AB A near-hollow plasma channel, where the plasma density in the channel is much less than the plasma density in the walls, is proposed to provide independent control over the focusing and accelerating forces in a plasma accelerator. In this geometry the low density in the channel contributes to the focusing forces, while the accelerating fields are determined by the high density in the channel walls. The channel also provides guiding for intense laser pulses used for wakefield excitation. Both electron and positron beams can be accelerated in a nearly symmetric fashion. Near-hollow plasma channels can effectively mitigate emittance growth due to Coulomb scattering for high-energy physics applications. (C) 2013 AIP Publishing LLC.
C1 [Schroeder, C. B.; Esarey, E.; Benedetti, C.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Schroeder, CB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
FU Office of Science, Office of High Energy Physics, of the U.S. Department
of Energy [DE-AC02-05CH11231]
FX This work was supported by the Director, Office of Science, Office of
High Energy Physics, of the U.S. Department of Energy under Contract No.
DE-AC02-05CH11231.
NR 25
TC 17
Z9 17
U1 2
U2 25
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 080701
DI 10.1063/1.4817799
PG 4
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800001
ER
PT J
AU Stoltzfus-Dueck, T
Scott, BD
Krommes, JA
AF Stoltzfus-Dueck, T.
Scott, B. D.
Krommes, J. A.
TI Nonadiabatic electron response in the Hasegawa-Wakatani equations
SO PHYSICS OF PLASMAS
LA English
DT Article
ID DRIFT-WAVE TURBULENCE; TOKAMAK EDGE TURBULENCE; PLASMA TURBULENCE;
SELF-ORGANIZATION; MODE TURBULENCE; ASDEX UPGRADE; ZONAL FLOWS;
TRANSPORT; INSTABILITY; CONFINEMENT
AB Tokamak edge turbulence is strongly influenced by parallel electron physics, which relaxes density and potential fluctuations towards electron adiabatic response. Beginning with the paradigmatic Hasegawa-Wakatani equations (HWEs) for resistive tokamak edge turbulence, a unique decomposition of the electric potential (phi) into adiabatic (a) and nonadiabatic (b) portions is derived, based on the requirement that a neither drive nor respond to the parallel current j(parallel to). The form of the decomposition clarifies that, at perpendicular scales large relative to the sound radius, the electron adiabatic response controls the nonzonal phi, not the fluctuating density n. Simple energy balance arguments allow one to rigorously bound the ratio of rms nonzonal nonadiabatic fluctuations ((b) over tilde) relative to adiabatic ones ((a) over tilde). The role of the vorticity nonlinearity in transferring energy between adiabatic and nonadiabatic fluctuations aids intuitive understanding of selfs-ustained turbulence in the HWEs. When the normalized parallel resistivity is weak, (b) over tilde becomes effectively slaved, allowing the reduction to an approximate one-field model that remains valid for strong turbulence. In addition to guiding physical intuition, the one-field reduction should greatly ease further analytical manipulations. Direct numerical simulation of the 2D HWEs confirms the convergence of the asymptotic formula for (b) over tilde.
C1 [Stoltzfus-Dueck, T.] Teilinst Greifswald, EURATOM Assoc, Max Planck Inst Plasmaphys, D-17491 Greifswald, Germany.
[Scott, B. D.] EURATOM, Max Planck Inst Plasmaphys, D-85748 Garching, Germany.
[Krommes, J. A.] Princeton Univ, PPPL, Princeton, NJ 08543 USA.
RP Stoltzfus-Dueck, T (reprint author), Teilinst Greifswald, EURATOM Assoc, Max Planck Inst Plasmaphys, Wendelsteinstr 1, D-17491 Greifswald, Germany.
EM tstoltzf@ipp.mpg.de
FU Department of Energy Fusion Energy Sciences Fellowship; National Science
Foundation Graduate Research Fellowship; U.S. Department of Energy
[DE-AC02-76-CHO-3073]; Humboldt Research Fellowship for Postdoctoral
Researchers; European Atomic Energy Community; European Fusion
Development Agreement
FX Helpful discussions with Greg Hammett, Jim Myra, and Stewart Zweben are
gratefully acknowledged. This work was performed in part at PPPL
(supported by a Department of Energy Fusion Energy Sciences Fellowship,
a National Science Foundation Graduate Research Fellowship, and the U.S.
Department of Energy Contract No. DE-AC02-76-CHO-3073) and in part at
the Max-Planck-Institut fur Plasmaphysik, both in Garching (supported by
a Humboldt Research Fellowship for Postdoctoral Researchers) and in
Greifswald (funded by the European Atomic Energy Community, with the
work therefore subject to the provisions of the European Fusion
Development Agreement).
NR 56
TC 5
Z9 5
U1 0
U2 7
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082314
DI 10.1063/1.4816807
PG 13
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800050
ER
PT J
AU Thoma, C
Welch, DR
Hsu, SC
AF Thoma, C.
Welch, D. R.
Hsu, S. C.
TI Particle-in-cell simulations of collisionless shock formation via
head-on merging of two laboratory supersonic plasma jets
SO PHYSICS OF PLASMAS
LA English
DT Article
ID MAGNETIC FIELD; WAVES; BEAM
AB We describe numerical simulations, using the particle-in-cell (PIC) and hybrid-PIC code LSP [T. P. Hughes et al., Phys. Rev. ST Accel. Beams 2, 110401 (1999)], of the head-on merging of two laboratory supersonic plasma jets. The goals of these experiments are to form and study astrophysically relevant collisionless shocks in the laboratory. Using the plasma jet initial conditions (density similar to 10(14)-10(16) cm(-3), temperature similar to few eV, and propagation speed similar to 20-150 km/s), large-scale simulations of jet propagation demonstrate that interactions between the two jets are essentially collisionless at the merge region. In highly resolved one-and two-dimensional simulations, we show that collisionless shocks are generated by the merging jets when immersed in applied magnetic fields (B similar to 0.1-1 T). At expected plasma jet speeds of up to 150 km/s, our simulations do not give rise to unmagnetized collisionless shocks, which require much higher velocities. The orientation of the magnetic field and the axial and transverse density gradients of the jets have a strong effect on the nature of the interaction. We compare some of our simulation results with those of previously published PIC simulation studies of collisionless shock formation. (C) 2013 AIP Publishing LLC.
C1 [Thoma, C.; Welch, D. R.] Voss Sci LLC, Albuquerque, NM 87108 USA.
[Hsu, S. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Thoma, C (reprint author), Voss Sci LLC, Albuquerque, NM 87108 USA.
OI Hsu, Scott/0000-0002-6737-4934
FU Laboratory Directed Research and Development (LDRD) Program at LANL
through U.S. Department of Energy [DE-AC52-06NA25396]
FX This work was supported by the Laboratory Directed Research and
Development (LDRD) Program at LANL through U.S. Department of Energy
Contract No. DE-AC52-06NA25396. The authors also acknowledge useful
discussions with Dr. D. V. Rose and Dr. N. L. Bennett of Voss Scientific
and Dr. A. L. Moser of LANL.
NR 42
TC 6
Z9 6
U1 0
U2 8
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 082128
DI 10.1063/1.4819063
PG 16
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800031
ER
PT J
AU Welch, DR
Rose, DV
Thoma, C
Clark, RE
Miller, C
Madrid, EA
Zimmerman, WR
Rambo, PK
Schwarz, J
Savage, M
Atherton, BW
AF Welch, D. R.
Rose, D. V.
Thoma, C.
Clark, R. E.
Miller, C.
Madrid, E. A.
Zimmerman, W. R.
Rambo, P. K.
Schwarz, J.
Savage, M.
Atherton, B. W.
TI Kinetic simulation studies of laser-triggering in the Z gas switch
SO PHYSICS OF PLASMAS
LA English
DT Article
ID MONTE-CARLO; PIC-MCC
AB Advanced z-pinch accelerators require precise timing of multiple mega-ampere drivers to deliver terawatt power. The triggering of these drivers is now largely initiated by laser ionization of gas switches. In this paper, we discuss detailed fully kinetic simulation of the Z laser-triggered gas switch involving detailed finite-difference time-domain particle-in-cell Monte Carlo modeling of the trigger section of the switch. Other components of the accelerator from the Marx bank through the pulse-forming line are described as circuit elements. The simulations presented here build on a recently developed model of electro-negative gas breakdown and streamer propagation that included photons produced from de-excited neutrals. New effects include multi-photon ionization of the gas in a prescribed laser field. The simulations show the sensitivity of triggering to laser parameters including focal plane within the anode-cathode gap of the trigger section of the switch, intensity at focus, and laser pulse length. Detailed electromagnetic simulations of the trigger section with circuit modeling of the upstream and downstream components are largely in agreement with Z data and demonstrate a new capability. (C) 2013 AIP Publishing LLC.
C1 [Welch, D. R.; Rose, D. V.; Thoma, C.; Clark, R. E.; Miller, C.; Madrid, E. A.; Zimmerman, W. R.] Voss Sci LLC, Albuquerque, NM 87108 USA.
[Rambo, P. K.; Schwarz, J.; Savage, M.; Atherton, B. W.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Welch, DR (reprint author), Voss Sci LLC, Albuquerque, NM 87108 USA.
FU U.S. Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]
FX Sandia National Laboratories is a multi-program laboratory operated by
Sandia Corporation, a wholly owned subsidiary of Lockheed Martin
Company, for the U.S. Department of Energy's National Nuclear Security
Administration under Contract No. DE-AC04-94AL85000.
NR 19
TC 2
Z9 3
U1 0
U2 12
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2013
VL 20
IS 8
AR 083108
DI 10.1063/1.4818146
PG 8
WC Physics, Fluids & Plasmas
SC Physics
GA 211XY
UT WOS:000323946800084
ER
PT J
AU Shankaran, H
Zhang, Y
Tan, YB
Resat, H
AF Shankaran, Harish
Zhang, Yi
Tan, Yunbing
Resat, Haluk
TI Model-Based Analysis of HER Activation in Cells Co-Expressing EGFR, HER2
and HER3
SO PLOS COMPUTATIONAL BIOLOGY
LA English
DT Article
ID GROWTH-FACTOR RECEPTOR; HUMAN-BREAST-CANCER; MAMMARY EPITHELIAL-CELLS;
ERBB SIGNALING NETWORK; EXTRACELLULAR REGION; QUANTITATIVE-ANALYSIS;
TYROSINE KINASES; SYSTEMS BIOLOGY; LUNG-CANCER; LIGAND
AB The HER/ErbB family of receptor tyrosine kinases drives critical responses in normal physiology and cancer, and the expression levels of the various HER receptors are critical determinants of clinical outcomes. HER activation is driven by the formation of various dimer complexes between members of this receptor family. The HER dimer types can have differential effects on downstream signaling and phenotypic outcomes. We constructed an integrated mathematical model of HER activation, and trafficking to quantitatively link receptor expression levels to dimerization and activation. We parameterized the model with a comprehensive set of HER phosphorylation and abundance data collected in a panel of human mammary epithelial cells expressing varying levels of EGFR/HER1, HER2 and HER3. Although parameter estimation yielded multiple solutions, predictions for dimer phosphorylation were in agreement with each other. We validated the model using experiments where pertuzumab was used to block HER2 dimerization. We used the model to predict HER dimerization and activation patterns in a panel of human mammary epithelial cells lines with known HER expression levels in response to stimulations with ligands EGF and HRG. Simulations over the range of expression levels seen in various cell lines indicate that: i) EGFR phosphorylation is driven by HER1-HER1 and HER1-HER2 dimers, and not HER1-HER3 dimers, ii) HER1-HER2 and HER2-HER3 dimers both contribute significantly to HER2 activation with the EGFR expression level determining the relative importance of these species, and iii) the HER2-HER3 dimer is largely responsible for HER3 activation. The model can be used to predict phosphorylated dimer levels for any given HER expression profile. This information in turn can be used to quantify the potencies of the various HER dimers, and can potentially inform personalized therapeutic approaches.
C1 [Shankaran, Harish; Zhang, Yi; Resat, Haluk] Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA 99352 USA.
[Tan, Yunbing] Washington State Univ, Sch Elect Engn & Comp Sci, Pullman, WA 99164 USA.
RP Shankaran, H (reprint author), Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA 99352 USA.
EM haluk.resat@wsu.edu
FU National Institutes of Health [5R01GM072821-07]; U.S. Department of
Energy [DE-AC06-76RL01830]
FX The research described in this paper was funded by the National
Institutes of Health Grant 5R01GM072821-07 to H. R. Pacific Northwest
National Laboratory is a multiprogram national laboratory operated by
Battelle for the U.S. Department of Energy under Contract
DE-AC06-76RL01830. The funders had no role in study design, data
collection and analysis, decision to publish, or preparation of the
manuscript.
NR 73
TC 6
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U1 1
U2 12
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1553-7358
J9 PLOS COMPUT BIOL
JI PLoS Comput. Biol.
PD AUG
PY 2013
VL 9
IS 8
AR e1003201
DI 10.1371/journal.pcbi.1003201
PG 15
WC Biochemical Research Methods; Mathematical & Computational Biology
SC Biochemistry & Molecular Biology; Mathematical & Computational Biology
GA 211DQ
UT WOS:000323885400034
PM 23990774
ER
PT J
AU Cheng, Q
Kazemian, M
Pham, H
Blatti, C
Celniker, SE
Wolfe, SA
Brodsky, MH
Sinha, S
AF Cheng, Qiong
Kazemian, Majid
Hannah Pham
Blatti, Charles
Celniker, Susan E.
Wolfe, Scot A.
Brodsky, Michael H.
Sinha, Saurabh
TI Computational Identification of Diverse Mechanisms Underlying
Transcription Factor-DNA Occupancy
SO PLOS GENETICS
LA English
DT Article
ID GENOME-WIDE BINDING; GAGA FACTOR; IN-VITRO; DROSOPHILA-MELANOGASTER;
CHROMATIN-STRUCTURE; BIOPHYSICAL MODEL; RINGER GENE; PROTEIN;
NUCLEOSOME; COMPLEX
AB ChIP-based genome-wide assays of transcription factor (TF) occupancy have emerged as a powerful, high-throughput method to understand transcriptional regulation, especially on a global scale. This has led to great interest in the underlying biochemical mechanisms that direct TF-DNA binding, with the ultimate goal of computationally predicting a TF's occupancy profile in any cellular condition. In this study, we examined the influence of various potential determinants of TF-DNA binding on a much larger scale than previously undertaken. We used a thermodynamics-based model of TF-DNA binding, called "STAP," to analyze 45 TF-ChIP data sets from Drosophila embryonic development. We built a cross-validation framework that compares a baseline model, based on the ChIP'ed ("primary") TF's motif, to more complex models where binding by secondary TFs is hypothesized to influence the primary TF's occupancy. Candidates interacting TFs were chosen based on RNA-SEQ expression data from the time point of the ChIP experiment. We found widespread evidence of both cooperative and antagonistic effects by secondary TFs, and explicitly quantified these effects. We were able to identify multiple classes of interactions, including (1) long-range interactions between primary and secondary motifs (separated by <= 150 bp), suggestive of indirect effects such as chromatin remodeling, (2) short-range interactions with specific inter-site spacing biases, suggestive of direct physical interactions, and (3) overlapping binding sites suggesting competitive binding. Furthermore, by factoring out the previously reported strong correlation between TF occupancy and DNA accessibility, we were able to categorize the effects into those that are likely to be mediated by the secondary TF's effect on local accessibility and those that utilize accessibility-independent mechanisms. Finally, we conducted in vitro pull-down assays to test model-based predictions of short-range cooperative interactions, and found that seven of the eight TF pairs tested physically interact and that some of these interactions mediate cooperative binding to DNA.
C1 [Cheng, Qiong; Kazemian, Majid; Blatti, Charles; Sinha, Saurabh] Univ Illinois, Dept Comp Sci, Urbana, IL 61801 USA.
[Hannah Pham; Wolfe, Scot A.; Brodsky, Michael H.] Univ Massachusetts, Sch Med, Program Gene Funct & Express, Worcester, MA USA.
[Celniker, Susan E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Drosophila Genome Project, Dept Genome Dynam, Berkeley, CA 94720 USA.
[Wolfe, Scot A.] Univ Massachusetts, Sch Med, Dept Biochem & Mol Pharmacol, Worcester, MA USA.
[Brodsky, Michael H.] Univ Massachusetts, Sch Med, Dept Mol Med, Worcester, MA USA.
[Sinha, Saurabh] Univ Illinois, Inst Genom Biol, Urbana, IL USA.
RP Cheng, Q (reprint author), Univ Illinois, Dept Comp Sci, Urbana, IL 61801 USA.
EM Michael.brodsky@umassmed.edu; sinhas@illinois.edu
OI Kazemian, Majid/0000-0001-7080-8820
FU NIH [GM085233]; NSF [DBI-0746303, EFRI-1136913]; National Human Genome
Research Institute of the National Institutes of Health [R01
HG004744-01]; NHGRI [P41HG3487]; Department of Energy
[DE-AC02-05CH11231]
FX This work was performed with support from the NIH (GM085233) and the NSF
(DBI-0746303, EFRI-1136913) to SS, from the National Human Genome
Research Institute of the National Institutes of Health (R01 HG004744-01
to MHB and SAW), and by NHGRI grant P41HG3487 (SEC) through the
Department of Energy under contract no DE-AC02-05CH11231. The funders
had no role in study design, data collection and analysis, decision to
publish, or preparation of the manuscript.
NR 68
TC 21
Z9 21
U1 0
U2 13
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1553-7404
J9 PLOS GENET
JI PLoS Genet.
PD AUG
PY 2013
VL 9
IS 8
AR e1003571
DI 10.1371/journal.pgen.1003571
PG 23
WC Genetics & Heredity
SC Genetics & Heredity
GA 210KB
UT WOS:000323830300002
PM 23935523
ER
PT J
AU Rosu, S
Zawadzki, KA
Stamper, EL
Libuda, DE
Reese, AL
Dernburg, AF
Villeneuve, AM
AF Rosu, Simona
Zawadzki, Karl A.
Stamper, Ericca L.
Libuda, Diana E.
Reese, Angela L.
Dernburg, Abby F.
Villeneuve, Anne M.
TI The C-elegans DSB-2 Protein Reveals a Regulatory Network that Controls
Competence for Meiotic DSB Formation and Promotes Crossover Assurance
SO PLOS GENETICS
LA English
DT Article
ID DOUBLE-STRAND BREAKS; CAENORHABDITIS-ELEGANS; CROSSING-OVER; DNA-DAMAGE;
CHROMOSOME SEGREGATION; CHIASMA FORMATION; MEIOSIS; RECOMBINATION;
SYNAPSIS; HOMOLOG
AB For most organisms, chromosome segregation during meiosis relies on deliberate induction of DNA double-strand breaks (DSBs) and repair of a subset of these DSBs as inter-homolog crossovers (COs). However, timing and levels of DSB formation must be tightly controlled to avoid jeopardizing genome integrity. Here we identify the DSB-2 protein, which is required for efficient DSB formation during C. elegans meiosis but is dispensable for later steps of meiotic recombination. DSB-2 localizes to chromatin during the time of DSB formation, and its disappearance coincides with a decline in RAD-51 foci marking early recombination intermediates and precedes appearance of COSA-1 foci marking CO-designated sites. These and other data suggest that DSB-2 and its paralog DSB-1 promote competence for DSB formation. Further, immunofluorescence analyses of wild-type gonads and various meiotic mutants reveal that association of DSB-2 with chromatin is coordinated with multiple distinct aspects of the meiotic program, including the phosphorylation state of nuclear envelope protein SUN-1 and dependence on RAD-50 to load the RAD-51 recombinase at DSB sites. Moreover, association of DSB-2 with chromatin is prolonged in mutants impaired for either DSB formation or formation of downstream CO intermediates. These and other data suggest that association of DSB-2 with chromatin is an indicator of competence for DSB formation, and that cells respond to a deficit of CO-competent recombination intermediates by prolonging the DSB-competent state. In the context of this model, we propose that formation of sufficient CO-competent intermediates engages a negative feedback response that leads to cessation of DSB formation as part of a major coordinated transition in meiotic prophase progression. The proposed negative feedback regulation of DSB formation simultaneously (1) ensures that sufficient DSBs are made to guarantee CO formation and (2) prevents excessive DSB levels that could have deleterious effects.
C1 [Rosu, Simona; Zawadzki, Karl A.; Libuda, Diana E.; Reese, Angela L.; Villeneuve, Anne M.] Stanford Univ, Dept Dev Biol, Sch Med, Stanford, CA 94305 USA.
[Rosu, Simona; Zawadzki, Karl A.; Libuda, Diana E.; Reese, Angela L.; Villeneuve, Anne M.] Stanford Univ, Dept Genet, Sch Med, Stanford, CA 94305 USA.
[Stamper, Ericca L.; Dernburg, Abby F.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA.
[Stamper, Ericca L.; Dernburg, Abby F.] Univ Calif Berkeley, Calif Inst Quantitat Biosci QB3, Berkeley, CA 94720 USA.
[Dernburg, Abby F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
[Dernburg, Abby F.] Howard Hughes Med Inst, Chevy Chase, MD USA.
RP Rosu, S (reprint author), Stanford Univ, Dept Dev Biol, Sch Med, Stanford, CA 94305 USA.
EM annev@stanford.edu
OI Dernburg, Abby/0000-0001-8037-1079
FU NIH [T32 GM07790, R01 GM067268, P40 OD010440]; Leukemia and Lymphoma
Society Fellowship; Helen Hay Whitney Foundation Postdoctoral
Fellowship; HHMI
FX This work was supported by NIH Training Grant T32 GM07790 to SR and ALR,
by a Leukemia and Lymphoma Society Fellowship to KAZ, by a Helen Hay
Whitney Foundation Postdoctoral Fellowship to DEL, by the HHMI to AFD
and by NIH R01 GM067268 to AMV. Some strains were provided by the
Caenorhabditis Genetics Center (funded by NIH P40 OD010440). The funders
had no role in study design, data collection and analysis, decision to
publish, or preparation of the manuscript.
NR 58
TC 28
Z9 33
U1 0
U2 6
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1553-7404
J9 PLOS GENET
JI PLoS Genet.
PD AUG
PY 2013
VL 9
IS 8
AR e1003674
DI 10.1371/journal.pgen.1003674
PG 23
WC Genetics & Heredity
SC Genetics & Heredity
GA 210KB
UT WOS:000323830300025
PM 23950729
ER
PT J
AU Stamper, EL
Rodenbusch, SE
Rosu, S
Ahringer, J
Villeneuve, AM
Dernburg, AF
AF Stamper, Ericca L.
Rodenbusch, Stacia E.
Rosu, Simona
Ahringer, Julie
Villeneuve, Anne M.
Dernburg, Abby F.
TI Identification of DSB-1, a Protein Required for Initiation of Meiotic
Recombination in Caenorhabditis elegans, Illuminates a Crossover
Assurance Checkpoint
SO PLOS GENETICS
LA English
DT Article
ID DOUBLE-STRAND BREAKS; C-ELEGANS; SACCHAROMYCES-CEREVISIAE; CHROMOSOME
SYNAPSIS; HOMOLOG ALIGNMENT; DNA-REPLICATION; CROSSING-OVER;
NONDISJUNCTION MUTANTS; NUCLEAR REORGANIZATION; CHIASMA FORMATION
AB Meiotic recombination, an essential aspect of sexual reproduction, is initiated by programmed DNA double-strand breaks (DSBs). DSBs are catalyzed by the widely-conserved Spo11 enzyme; however, the activity of Spo11 is regulated by additional factors that are poorly conserved through evolution. To expand our understanding of meiotic regulation, we have characterized a novel gene, dsb-1, that is specifically required for meiotic DSB formation in the nematode Caenorhabditis elegans. DSB-1 localizes to chromosomes during early meiotic prophase, coincident with the timing of DSB formation. DSB-1 also promotes normal protein levels and chromosome localization of DSB-2, a paralogous protein that plays a related role in initiating recombination. Mutations that disrupt crossover formation result in prolonged DSB-1 association with chromosomes, suggesting that nuclei may remain in a DSB-permissive state. Extended DSB-1 localization is seen even in mutants with defects in early recombination steps, including spo-11, suggesting that the absence of crossover precursors triggers the extension. Strikingly, failure to form a crossover precursor on a single chromosome pair is sufficient to extend the localization of DSB-1 on all chromosomes in the same nucleus. Based on these observations we propose a model for crossover assurance that acts through DSB-1 to maintain a DSB-permissive state until all chromosome pairs acquire crossover precursors. This work identifies a novel component of the DSB machinery in C. elegans, and sheds light on an important pathway that regulates DSB formation for crossover assurance.
C1 [Stamper, Ericca L.; Rodenbusch, Stacia E.; Dernburg, Abby F.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA.
[Stamper, Ericca L.; Rodenbusch, Stacia E.; Dernburg, Abby F.] Univ Calif Berkeley, Calif Inst Quantitat Biosci QB3, Berkeley, CA 94720 USA.
[Rosu, Simona; Villeneuve, Anne M.] Stanford Univ, Dept Dev Biol & Genet, Sch Med, Stanford, CA 94305 USA.
[Ahringer, Julie] Univ Cambridge, Gurdon Inst, Cambridge, England.
[Ahringer, Julie] Univ Cambridge, Dept Genet, Cambridge CB2 3EH, England.
[Dernburg, Abby F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Div Life Sci, Berkeley, CA 94720 USA.
[Dernburg, Abby F.] Howard Hughes Med Inst, Chevy Chase, MD USA.
RP Stamper, EL (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.
EM AFDernburg@lbl.gov
OI Dernburg, Abby/0000-0001-8037-1079
FU Department of Energy Office of Science Graduate Fellowship (DOE SCGF);
National Science Foundation Graduate Research Fellowship (GRFP); NIH
[R01 GM067268, R01 GM065591]; Howard Hughes Medical Institute; NIH
Office of Research Infrastructure Programs [P40 OD010440]
FX This study was supported by a Department of Energy Office of Science
Graduate Fellowship (DOE SCGF, http://scgf.orau.gov/) to ELS, a National
Science Foundation Graduate Research Fellowship (GRFP,
http://www.nsfgrfp.org/) to SER, and by research funds from the NIH
(http://grants.nih.gov/grants/oer.htm) (R01 GM067268 to AMV and R01
GM065591 to AFD) and the Howard Hughes Medical Institute
(http://www.hhmi.org/). Some strains were provided by the CGC
(http://www.cbs.umn.edu/cgc), which is funded by NIH Office of Research
Infrastructure Programs (P40 OD010440). The funders had no role in study
design, data collection and analysis, decision to publish, or
preparation of the manuscript.
NR 94
TC 22
Z9 25
U1 0
U2 7
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1553-7404
J9 PLOS GENET
JI PLoS Genet.
PD AUG
PY 2013
VL 9
IS 8
AR e1003679
DI 10.1371/journal.pgen.1003679
PG 18
WC Genetics & Heredity
SC Genetics & Heredity
GA 210KB
UT WOS:000323830300030
PM 23990794
ER
PT J
AU Xu, PG
Tomota, Y
Vogel, SC
Suzuki, T
Yonemura, M
Kamiyama, T
AF Xu, P. G.
Tomota, Y.
Vogel, S. C.
Suzuki, T.
Yonemura, M.
Kamiyama, T.
TI TRANSFORMATION STRAIN AND TEXTURE EVOLUTION DURING DIFFUSIONAL PHASE
TRANSFORMATION OF LOW ALLOY STEELS STUDIED BY NEUTRON DIFFRACTION
SO REVIEWS ON ADVANCED MATERIALS SCIENCE
LA English
DT Article; Proceedings Paper
CT 6th International Conference on Physical and Numerical Simulation of
Materials Processing (ICPNS)
CY NOV 16-19, 2010
CL Guilin Univ Elect Technol, Guilin, PEOPLES R CHINA
SP Wollongong Univ, Chinese Mech Engn Soc, Minerals, Met & Mat Soc, Dynam Syst Inc, Harbin Inst Technol, Huaqiao Univ, Henan Polytechn Univ, Graz Univ Technol, Univ Sao Paulo, McGill Univ, Beijing Aviat Mfg Engn Inst, Univ Rijeka, Univ W Bohemia, Univ Oulu, GKSS Res Ctr, Hong Kong Polytechn Univ, Univ Delhi, Univ Osaka, JWRI, Univ Electro Commun, Chungnam Natl Univ, Korea Inst Machinery & Mat, Pusan Natl Univ, Riga Tech Univ, Delft Univ Technol, Moscow State Univ, RAS, Inst Phys & Mat Sci, Moscow State Inst Elect & Math, Moscow State Inst Steel & Alloys, Nanyang Technol Univ, Natl Taiwan Univ, Ege Univ, Univ Cambridge, Dept Mat & Matallurgy, EO Paton Elect Weld Inst, BATTELLE
HO Guilin Univ Elect Technol
ID LATTICE-PARAMETERS; RIETVELD-ANALYSIS; AUSTENITE; SELECTION; FERRITE;
DIFFRACTOMETER; TEMPERATURE; PREDICTION
AB The ferrite-to-austenite transformation during heating and the austenite-to-ferrite transformation during cooling were in situ investigated by KEK/SIRIUS and LANSCE/HIPPO neutron diffractometers under the stress-free condition. The deviation of ferrite lattice parameter from the linear thermal expansion and contraction during heating and cooling suggested the compressive strain occurred in ferrite phase. The texture memory effect between the cold compression texture of initial martensite and the final texture of ferrite after alpha -> gamma -> alpha phase transformation was interrupted by the static recrystallization of martensite during step-by-step heating, revealing that the occurrence of texture memory effect was not directly related to the deformation stored energy but related to the transformation strain and the strong variant selection for nucleation.
C1 [Xu, P. G.] Japan Atom Energy Agcy, Quantum Beam Sci Directorate, Ibaraki 3191195, Japan.
[Xu, P. G.; Tomota, Y.; Suzuki, T.; Yonemura, M.] Ibaraki Univ, Grad Sch Sci & Engn, Ibaraki 3168511, Japan.
[Vogel, S. C.] Los Alamos Natl Lab, Los Alamos Neutron Scattering Ctr, Los Alamos, NM 87545 USA.
RP Xu, PG (reprint author), Japan Atom Energy Agcy, Quantum Beam Sci Directorate, Ibaraki 3191195, Japan.
EM xu.pingguang@jaea.go.jp
RI Xu, Pingguang/F-6347-2011;
OI Xu, Pingguang/0000-0001-6547-0167; Vogel, Sven C./0000-0003-2049-0361
FU Japan Society for the Promotion of Science (JSPS: KAKENHI) [21860090]
FX The bulk texture evaluation research was financially supported by the
Grant-in-Aid for Young Scientists (No.21860090) of Japan Society for the
Promotion of Science (JSPS: KAKENHI). The authors thank to Dr. Y. Adachi
at National Institute for Materials Science, Japan for providing the
investigated steel.
NR 18
TC 2
Z9 2
U1 0
U2 12
PU INST PROBLEMS MECHANICAL ENGINEERING-RUSSIAN ACAD SCIENCES
PI ST PTERSBURG
PA BOLSHOJ 61, VAS OSTROV, ST PTERSBURG, 199178, RUSSIA
SN 1606-5131
J9 REV ADV MATER SCI
JI Rev. Adv. Mater. Sci.
PD AUG
PY 2013
VL 33
IS 5
BP 389
EP 395
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 210WL
UT WOS:000323865400003
ER
PT J
AU Bernert, T
Winkler, B
Haussuhl, E
Trouw, F
Vogel, SC
Hurd, AJ
Smilowitz, L
Henson, BF
Merrill, FE
Morris, CL
Mariam, FG
Saunders, A
Juarez-Arellano, EA
AF Bernert, T.
Winkler, B.
Haussuehl, E.
Trouw, F.
Vogel, S. C.
Hurd, A. J.
Smilowitz, L.
Henson, B. F.
Merrill, F. E.
Morris, C. L.
Mariam, F. G.
Saunders, A.
Juarez-Arellano, E. A.
TI In situ observation of self-propagating high temperature syntheses of
Ta5Si3, Ti5Si3 and TiB2 by proton and X-ray radiography
SO SOLID STATE SCIENCES
LA English
DT Article
DE Proton radiography; X-ray radiography; Self-propagating high-temperature
synthesis; Solid state kinetics
ID ANGLE NEUTRON-SCATTERING; COMBUSTION SYNTHESIS; TEXTURE ANALYSIS;
DIFFRACTION DATA; SHS; TRANSITION; ALLOYS; GROWTH; ENERGY; ROCKS
AB Self-propagating high temperature reactions of tantalum and titanium with silicon and titanium with boron were studied using proton and X-ray radiography, small-angle neutron scattering, neutron time-of-flight, X-ray and neutron diffraction, dilatometry and video recording. We show that radiography allows the observation of the propagation of the flame front in all investigated systems and the determination of the widths of the burning zones. X-ray and neutron diffraction showed that the reaction products consisted of approximate to 90 wt% of the main phase and one or two secondary phases. For the reaction 5Ti + 3Si -> Ti5Si3 flame front velocities of 7.1(3)-34.2(4) mm/s were determined depending on the concentration of a retardant added to the starting material, the geometry and the green density of the samples. The flame front width was determined to be 117(4)-1.82(8) mm and depends exponentially on the flame front velocity. Similarly, for the reaction Ti + 2B -> TiB2 flame front velocities of 15(2)-26.6(4) mm/s were determined, while for a 5Ta + 3Si -> Ta5Si3 reaction the flame front velocity was 7.05(4) mm/s. The micro structure of the product phase Ta5Si3 shows no texture. From SANS measurements the dependence of the specific surface of the product phase on the particle sizes of the starting materials was studied. (C) 2013 Elsevier Masson SAS. All rights reserved.
C1 [Bernert, T.; Winkler, B.; Haussuehl, E.] Goethe Univ Frankfurt, Inst Geowissensch, Abt Kristallog, D-60438 Frankfurt, Germany.
[Trouw, F.; Vogel, S. C.; Hurd, A. J.; Smilowitz, L.; Henson, B. F.; Merrill, F. E.; Morris, C. L.; Mariam, F. G.; Saunders, A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Juarez-Arellano, E. A.] Univ Papaloapan, Mexico City 68301, DF, Mexico.
RP Bernert, T (reprint author), Goethe Univ Frankfurt, Inst Geowissensch, Abt Kristallog, Altenhoferallee 1, D-60438 Frankfurt, Germany.
EM b.winkler@kristall.uni-frankfurt.de
OI Juarez-Arellano, Erick/0000-0003-4844-8317
FU German Science Foundation [Wi 1232-35]
FX We are grateful to the German Science Foundation for support within
project Wi 1232-35.
NR 38
TC 2
Z9 2
U1 0
U2 27
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1293-2558
EI 1873-3085
J9 SOLID STATE SCI
JI Solid State Sci.
PD AUG
PY 2013
VL 22
BP 33
EP 42
DI 10.1016/j.solidstatesciences.2013.05.007
PG 10
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical; Physics, Condensed
Matter
SC Chemistry; Physics
GA 204HP
UT WOS:000323356500006
ER
PT J
AU Gilbert, B
Erbs, JJ
Penn, RL
Petkov, V
Spagnoli, D
Waychunas, GA
AF Gilbert, Benjamin
Erbs, Jasmine J.
Penn, R. Lee
Petkov, Valeri
Spagnoli, Dino
Waychunas, Glenn A.
TI A disordered nanoparticle model for 6-line ferrihydrite
SO AMERICAN MINERALOGIST
LA English
DT Article
DE Nanoparticle structure; reverse Monte Carlo; total X-ray scattering;
pair distribution function
ID PAIR DISTRIBUTION FUNCTION; X-RAY-DIFFRACTION; BOND-VALENCE PARAMETERS;
2-LINE FERRIHYDRITE; STRUCTURAL MODEL; ELECTRON NANODIFFRACTION;
NANOCRYSTALLINE MATERIAL; ORIENTED AGGREGATION; IRON OXYHYDROXIDES;
LOCAL-STRUCTURE
AB Much of the bioavailable and geochemically reactive iron in aerobic, circumneutral settings is frequently found in the form of nanoscale particles of a hydrated iron(III) oxyhydroxide phase known as ferrihydrite. Developing useful structural descriptions of defective nanophases such as ferrihydrite has long posed significant challenges. Recently, Michel et al. (2007, 2010) proposed a structural model for ferrihydrite in place of the long-accepted model of Drits et al. (1993). Both models reproduce to high accuracy certain forms of X-ray scattering data from powdered ferrihydrite. However, discrepancies remain that we hypothesized are due to forms of structural disorder not easily represented by existing models. To test this hypothesis, we performed a novel structural analysis of total X-ray scattering data acquired from 6-line ferrihydrite. We generated three candidate whole-nanoparticle models of ferrihydrite composed of a two-phase Drits model, the Michel model, and a hybrid phase based on a single-phase Drits model that incorporated tetrahedral Fe sites, creating a lattice in which the Michel model was one of many possible topologies. We implemented a reverse Monte Carlo (RMC) approach to explore alternative configurations of iron occupancies plus structural disorder, and to refine the nanoparticle structure using both the reciprocal and real-space forms of the X-ray scattering data. We additionally used oxygen K-edge X-ray absorption spectroscopy to semi-quantitatively assess the ratio of protonated:non-protonated oxygen sites in an iron(III) oxides. This analysis provides independent evidence for a significantly lower OH:O stoichiometric ratio for ferrihydrite than for goethite, further constraining the RMC models.
The hybrid structure model gave better agreement to the experimental total scattering data than nanoparticles based upon either the Michel or Drits models. Models that incorporated tetrahedrally coordinated iron sites consistently achieved better matches to the data than models containing face-sharing octahedra. Long-range vacancy disorder was essential for optimum fits to the scattering data, highlighting the utility of whole-nanoparticle models in place of unit-cell models with random distributions of iron vacancies. The RMC-derived structures do not satisfy all experimental constraints on composition and structure. Nevertheless this work illustrates that a suitably constrained RMC method applied to whole-nanoparticle models can be an effective approach for exploring disorder in nanocrystalline materials.
C1 [Gilbert, Benjamin; Waychunas, Glenn A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Erbs, Jasmine J.; Penn, R. Lee] Univ Minnesota, Dept Chem, Minneapolis, MN 55455 USA.
[Petkov, Valeri] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48848 USA.
[Spagnoli, Dino] Univ Western Australia, Sch Chem & Biochem, Crawley, WA 6009, Australia.
RP Gilbert, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, MS 74R316C,1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM bgilbert@lbl.gov
RI Spagnoli, Dino/F-8641-2011; Gilbert, Benjamin/E-3182-2010
OI Spagnoli, Dino/0000-0001-6367-4748;
FU Office of Science, Office of Basic Energy Sciences, of the U.S.
Department of Energy [DE-AC02-05CH11231]; IGERT Program of the National
Science Foundation [DGE-0114372]; National Science Foundation [0346385];
NSF through the National Nanotechnology Infrastructure Network; DOE-BES
[DE-AC02-05CH11231, W-31-109-ENG-38]
FX Thanks to Pupa Gilbert for numerous valuable discussions, Sirine Fakra
for acquiring preliminary X-ray absorption spectroscopy data, and four
anonymous referees for their constructive comments. High-energy
X-ray-scattering data were acquired at beamline 11-ID-C at the Advanced
Photon Source (APS). Oxygen K-edge soft-X-ray absorption spectroscopy
was performed at ALS beamline 7.0.1 and we thank Per-Anders Glans and
Jinghua Guo. High-resolution synchrotron powder diffraction data were
acquired at ALS beamline 11.3.1 and we thank Simon Teat. B.G. and G.A.W.
were supported by the Director, Office of Science, Office of Basic
Energy Sciences, of the U.S. Department of Energy, hereby abbreviated to
DOE-BES, under Contract No. DE-AC02-05CH11231. J.J.E. and R.L.P. were
supported by the IGERT Program of the National Science Foundation under
award no. DGE-0114372 (fellowship to J.J.E.) and the National Science
Foundation Career Grant 0346385. TEM characterization was carried out at
the Characterization Facility, University of Minnesota, which receives
support from NSF through the National Nanotechnology Infrastructure
Network. Use of the ALS and the APS is supported by DOE-BES under
Contract Numbers DE-AC02-05CH11231 and W-31-109-ENG-38, respectively.
NR 84
TC 11
Z9 11
U1 6
U2 65
PU MINERALOGICAL SOC AMER
PI CHANTILLY
PA 3635 CONCORDE PKWY STE 500, CHANTILLY, VA 20151-1125 USA
SN 0003-004X
J9 AM MINERAL
JI Am. Miner.
PD AUG-SEP
PY 2013
VL 98
IS 8-9
BP 1465
EP 1476
DI 10.2138/am.2013.4421
PG 12
WC Geochemistry & Geophysics; Mineralogy
SC Geochemistry & Geophysics; Mineralogy
GA 207FJ
UT WOS:000323584000011
ER
PT J
AU Volkow, ND
Wang, GJ
Tomasi, D
Baler, RD
AF Volkow, Nora D.
Wang, Gen-Jack
Tomasi, Dardo
Baler, Ruben D.
TI Unbalanced neuronal circuits in addiction
SO CURRENT OPINION IN NEUROBIOLOGY
LA English
DT Article
ID NORMALIZES CINGULATE ACTIVITY; DEEP BRAIN-STIMULATION; SALIENT COGNITIVE
TASK; VENTRAL TEGMENTAL AREA; MEDIUM SPINY NEURONS; DRUG-ADDICTION;
SUBTHALAMIC NUCLEUS; COCAINE ADDICTION; LATERAL HABENULA; DOPAMINE
NEURONS
AB Through sequential waves of drug-induced neurochemical stimulation, addiction co-opts the brain's neuronal circuits that mediate reward, motivation to behavioral inflexibility and a severe disruption of self-control and compulsive drug intake. Brain imaging technologies have allowed neuroscientists to map out the neural landscape of addiction in the human brain and to understand how drugs modify it.
C1 [Volkow, Nora D.; Baler, Ruben D.] NIDA, NIH, Bethesda, MD 20892 USA.
[Wang, Gen-Jack; Tomasi, Dardo] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA.
RP Volkow, ND (reprint author), NIDA, NIH, Bethesda, MD 20892 USA.
EM nvokowl@nida.nih.gov
RI Tomasi, Dardo/J-2127-2015
FU Intramural NIH HHS [Z99 DA999999]
NR 100
TC 34
Z9 36
U1 4
U2 34
PU CURRENT BIOLOGY LTD
PI LONDON
PA 84 THEOBALDS RD, LONDON WC1X 8RR, ENGLAND
SN 0959-4388
J9 CURR OPIN NEUROBIOL
JI Curr. Opin. Neurobiol.
PD AUG
PY 2013
VL 23
IS 4
BP 639
EP 648
DI 10.1016/j.conb.2013.01.002
PG 10
WC Neurosciences
SC Neurosciences & Neurology
GA 204XJ
UT WOS:000323404300026
PM 23434063
ER
PT J
AU Zhang, P
Qiu, JX
Zheng, ZF
Liu, G
Ling, M
Martens, W
Wang, HH
Zhao, HJ
Zhang, SQ
AF Zhang, Peng
Qiu, Jingxia
Zheng, Zhanfeng
Liu, Gao
Ling, Min
Martens, Wayde
Wang, Haihui
Zhao, Huijun
Zhang, Shanqing
TI Free-standing and bendable carbon nanotubes/TiO2 nanofibres composite
electrodes for flexible lithium ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Flexible electrode; Carbon nanotubes; TiO2; Lithium ion batteries
ID ELECTROCHEMICAL ENERGY-STORAGE; PAPER; PERFORMANCE; ANODES
AB Carbon nanotube (CNT) and TiO2 nanofibre composite films are prepared and used as anode materials for lithium ion batteries (LIBs) without the use of binders and conventional copper current collector. The preliminary experimental results from X-ray diffraction, scanning electron microscopy and transmission electron microscopy suggest that the TiO2 nanofibres were well-dispersed and interwoven by the CNTs, forming freestanding, bendable and light weighted composite. In comparison with TiO2 nanofibre based LIBs, the CNTs could significantly improve the battery performance due to their high conductivity property and 3D network morphology. In both 1-3 V and 0.01-3 V testing voltage ranges, the as-prepared composites show excellent reversible capacity and capacity retention. The superior lithium storage capacity of the CNT/TiO2 composite was mainly attributed to dual functions of the CNTs the CNTs not only provide conductive networks to assist the electron transfer but also facilitate lithium ion diffusion between the electrolyte and the TiO2 active materials by preventing agglomeration of TiO2 nanofibres. This work demonstrates that the CNT TiO2 composite film could be one type of potential electrode material for large-scale LIB applications. Crown Copyright (C) 2013 Published by Elsevier Ltd. All rights reserved.
C1 [Zhang, Peng; Qiu, Jingxia; Ling, Min; Zhao, Huijun; Zhang, Shanqing] Griffith Univ, Griffith Sch Environm, Ctr Clean Environm & Energy, Environm Futures Ctr, Gold Coast, Qld 4222, Australia.
[Zheng, Zhanfeng; Martens, Wayde] Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, Australia.
[Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
[Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou, Guangdong, Peoples R China.
RP Zhang, SQ (reprint author), Griffith Univ, Griffith Sch Environm, Ctr Clean Environm & Energy, Environm Futures Ctr, Gold Coast Campus, Gold Coast, Qld 4222, Australia.
EM s.zhang@griffith.edu.au
RI Martens, Wayde/I-9848-2012; Zheng, Zhanfeng/A-6247-2010; Zhao,
Huijun/H-5882-2015; Zhang, Shanqing/C-2590-2008
OI Martens, Wayde/0000-0002-0959-6838; Zheng, Zhanfeng/0000-0001-9167-936X;
Zhao, Huijun/0000-0002-3028-0459;
FU Australia Research Council; Assistant Secretary for Energy Efficiency,
Office of Vehicle Technologies of the U.S. DOE under the Batteries for
Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231];
University of California, Office of the President through the University
of California
FX S. Zhang thanks to financial support from Australia Research Council
Future Fellowship Grant. G. Liu was funded by the Assistant Secretary
for Energy Efficiency, Office of Vehicle Technologies of the U.S. DOE
under contract number DE-AC02-05CH11231 under the Batteries for Advanced
Transportation Technologies (BATT) Program, and by the University of
California, Office of the President through the University of California
Discovery Grant. The authors also acknowledge the facilities and the
scientific and technical assistance of the Australian Microscopy &
Microanalysis Research Facility at the Centre for Microscopy and
Microanalysis at the University of Queensland.
NR 30
TC 34
Z9 34
U1 14
U2 164
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD AUG 1
PY 2013
VL 104
BP 41
EP 47
PG 7
WC Electrochemistry
SC Electrochemistry
GA 180NF
UT WOS:000321601200006
ER
PT J
AU Li, M
Zhou, WP
Marinkovic, NS
Sasaki, K
Adzic, RR
AF Li, M.
Zhou, W. -P.
Marinkovic, N. S.
Sasaki, K.
Adzic, R. R.
TI The role of rhodium and tin oxide in the platinum-based electrocatalysts
for ethanol oxidation to CO2
SO ELECTROCHIMICA ACTA
LA English
DT Article; Proceedings Paper
CT 3rd International Symposium on Surface Imaging/Spectroscopy at the
Solid/Liquid Interface (ISSIS)
CY MAY 27-JUN 01, 2012
CL Polish Acad Sci, J Haber Inst Catalysis & Surface Chem, Krakow, POLAND
SP Univ Warsaw, Fac Chem, Electrochem Soc, Shim Pol, KGHM, ECOREN, Azoty Tarnow, nLab
HO Polish Acad Sci, J Haber Inst Catalysis & Surface Chem
DE Rh(111); Pt-Rh-SnO2; Ethanol electrooxidation; EOR; In situ IRRAS
ID IN-SITU FTIR; PT-RH; ELECTROOXIDATION; ELECTRODES; CATALYSTS; DEMS;
SPECTROSCOPY; ADSORPTION
AB Our recent efforts in developing electrocatalysts for ethanol oxidation reaction are focused on the ternary Pt-Rh-SnO2 catalysts due to their superior performance in splitting C-C bond and the ability to fully oxidize ethanol to CO2. This work reports on the role of Rh from studies of the well-defined Rh(1 1 1) single-crystal and a series of carbon-supported nanoparticle catalysts for the electrooxidation of ethanol. A comparative study of supported nanocatalysts was carried out and their activity for ethanol oxidation decreased in the order of PtRhSnO2 >PtSnO2 > Pt> PtRh > Rh > RhSnO2. In situ infrared reflection-absorption spectroscopy studies showed that the catalysts' selectivity toward ethanol total oxidation to CO2 decreased in the order of: PtRhSnO2 RhSnO2 > PtRh > Pt> PtSnO2 Rh, verifying the role of Rh in breaking the C-C bond, and the roles of the two other constituents, SnO2 and Pt, that facilitate the oxidation of the reaction intermediates and lessen their bonding to Rh. These results help understanding the role of Rh and SnO2 in the catalytic oxidation of ethanol and provide insights for designing catalysts with improved propeties. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Li, M.; Zhou, W. -P.; Sasaki, K.; Adzic, R. R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Marinkovic, N. S.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA.
RP Marinkovic, NS (reprint author), Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA.
EM marinkov@bnl.gov
RI Li, Meng/L-8507-2013; Marinkovic, Nebojsa/A-1137-2016
OI Marinkovic, Nebojsa/0000-0003-3579-3453
NR 28
TC 35
Z9 35
U1 7
U2 83
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD AUG 1
PY 2013
VL 104
BP 454
EP 461
DI 10.1016/j.electacta.2012.10.046
PG 8
WC Electrochemistry
SC Electrochemistry
GA 180NF
UT WOS:000321601200055
ER
PT J
AU Miller, CL
Watson, DB
Lester, BP
Lowe, KA
Pierce, EM
Liang, LY
AF Miller, Carrie L.
Watson, David B.
Lester, Brian P.
Lowe, Kenneth A.
Pierce, Eric M.
Liang, Liyuan
TI Characterization of soils from an industrial complex contaminated with
elemental mercury
SO ENVIRONMENTAL RESEARCH
LA English
DT Article; Proceedings Paper
CT 10th International Conference on Mercury as a Global Pollutant
CY JUL 24-28, 2011
CL Halifax, CANADA
DE Analytical methods; Elemental mercury; Industrial contamination; Soil
ID RAY-FLUORESCENCE SPECTROMETRY; FORK POPLAR CREEK; OAK-RIDGE; REDUCED
SULFUR; ORGANIC-MATTER; CHEMICAL EXTRACTIONS; ATMOSPHERIC MERCURY;
SPATIAL-PATTERNS; SPECIATION; SEDIMENTS
AB Historical use of liquid elemental mercury (Hg(0)(I)) at the Y-12 National Security Complex in Oak Ridge, TN, USA, resulted in large deposits of Hg(0)(I) in the soils. The fate and distribution of the spilled Hg(0) are not well characterized. In this study we evaluated analytical tools for characterizing the speciation of Hg in the contaminated soils and then used the analytical techniques to examine the speciation of Hg in two soil cores collected at the site. These include x-ray fluorescence (XRF), soil Hg(0) headspace analysis, and total Hg determination by acid digestion coupled with cold vapor atomic absorption (HgT). XRF was not found to be suitable for evaluating Hg concentrations in heterogeneous soils containing low concentration of Hg or Hg(0) because Hg concentrations determined using this method were lower than those determined by HgT analysis and the XRF detection limit is 20 mg/kg. Hg(0)(g) headspace analysis coupled with HgT measurements yielded good results for examining the presence of Hg(0)(I) in soils and the speciation of Hg. The two soil cores are highly heterogeneous in both the depth and extent of Hg contamination, with Hg concentrations ranging from 0.05 to 8400 mg/kg. In the first core, Hg(0)(I) was distributed throughout the 3.2 m depth, whereas the second core, from a location 12 m away, contained Hg(0)(I) in a 0.3 m zone only. Sequential extractions showed organically associated Hg dominant at depths with low Hg concentration. Soil from the zone of groundwater saturation showed reducing conditions and the Hg is likely present as Hg-sulfide species. At this depth, lateral Hg transport in the groundwater may be a source of Hg detected in the soil at the deeper soil depths. Overall, characterization of soils containing Hg(0)(I) is difficult because of the heterogeneous distribution of Hg within the soils. This is exacerbated in industrial facilities where fill materials make up much of the soils and historical and continued reworking of the subsurface has remobilized the Hg. (C) 2013 Elsevier Inc. All rights reserved.
C1 [Miller, Carrie L.; Watson, David B.; Lester, Brian P.; Lowe, Kenneth A.; Pierce, Eric M.; Liang, Liyuan] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA.
RP Miller, CL (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008,MS 6038, Oak Ridge, TN 37831 USA.
EM millercl@ornl.gov
RI Miller, Carrie/B-8943-2012; Liang, Liyuan/O-7213-2014; Watson,
David/C-3256-2016; Pierce, Eric/G-1615-2011
OI Liang, Liyuan/0000-0003-1338-0324; Watson, David/0000-0002-4972-4136;
Pierce, Eric/0000-0002-4951-1931
NR 62
TC 16
Z9 16
U1 10
U2 75
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0013-9351
J9 ENVIRON RES
JI Environ. Res.
PD AUG
PY 2013
VL 125
SI SI
BP 20
EP 29
DI 10.1016/j.envres.2013.03.013
PG 10
WC Environmental Sciences; Public, Environmental & Occupational Health
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health
GA 204XQ
UT WOS:000323405000004
PM 23809204
ER
PT J
AU DeWoskin, RS
Sweeney, LM
Teeguarden, JG
Sams, R
Vandenberg, J
AF DeWoskin, R. S.
Sweeney, L. M.
Teeguarden, J. G.
Sams, R., II
Vandenberg, J.
TI Comparison of PBTK model and biomarker based estimates of the internal
dosimetry of acrylamide
SO FOOD AND CHEMICAL TOXICOLOGY
LA English
DT Article
DE PBTK model; Biomarkers of exposure; Hemoglobin adducts; Acrylamide;
Glycidamide; Dosimetry
ID HEMOGLOBIN ADDUCTS; FISCHER-344 RATS; MAILLARD REACTION;
RISK-ESTIMATION; ETHYLENE-OXIDE; B6C3F(1) MICE; GLYCIDAMIDE; EXPOSURE;
FOOD; HUMANS
AB Estimates of internal dosimetry for acrylamide (AA, 2-propenamide; CASRN: 79-06-1) and its active metabolite glycidamide (GA) were compared using either biomarkers of internal exposure (hemoglobin adduct levels in rats and humans) or a PBTK model (Sweeney et al., 2010). The resulting impact on the human equivalent dose (HED, oral exposures), the human equivalent concentration (HEC, inhalation), and final reference values was also evaluated. Both approaches yielded similar AA HEDs and HECs for the most sensitive noncancer effect of neurotoxicity, identical oral reference doses (RID) of 2 x 10(-3) mg AA/kg bw/d, and nearly identical inhalation reference concentrations (RfC = 0.006 mg/m(3) and 0.007 mg/m(3), biomarker and PBTK results, respectively). HED and HEC values for carcinogenic potential were very similar, resulting in identical inhalation unit risks of 0.1/(mg AA/m(3)), and nearly identical oral cancer slope factors (0.4 and 0.5/mg AA/kg bw/d), biomarker and PBTK results, respectively. The concordance in estimated HEDs, HECs, and reference values from these two diverse methods increases confidence in those values. Advantages and specific application of each approach are discussed.
(Note: Reference values derived with the PBPK model were part of this research, and do not replace values currently posted on IRIS: http://www.epa.gov/iris/toxreviews/0286tr.pdf.) Published by Elsevier Ltd.
C1 [DeWoskin, R. S.; Sams, R., II; Vandenberg, J.] US EPA, Natl Ctr Environm Assessment, Off Res & Dev, Res Triangle Pk, NC 27711 USA.
[Sweeney, L. M.] SAIC, Naval Med Res Unit Dayton, Kettering, OH 45440 USA.
[Teeguarden, J. G.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP DeWoskin, RS (reprint author), US EPA, Natl Ctr Environm Assessment, Off Res & Dev, MD-B243-01, Res Triangle Pk, NC 27711 USA.
EM dewoskin.rob@epa.gov; lmsweeney@aol.com; jt@pnl.gov
RI Sweeney, Lisa/K-5114-2012;
OI Sweeney, Lisa/0000-0002-4672-7358; Teeguarden,
Justin/0000-0003-3817-4391; Vandenberg, John/0000-0003-2619-9460
FU U.S. EPA; Grocery Manufacturers Association (GMA), Washington, DC
FX The Toxicological review for Acrylamide was funded by the U.S. EPA. The
development of the Sweeney et al. PBTK model (published in 2010) was
funded by the Grocery Manufacturers Association (GMA), Washington, DC.
The author's use of this model to generate the results presented here
was independent of the GMA.
NR 51
TC 1
Z9 2
U1 2
U2 20
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0278-6915
J9 FOOD CHEM TOXICOL
JI Food Chem. Toxicol.
PD AUG
PY 2013
VL 58
BP 506
EP 521
DI 10.1016/j.fct.2013.05.008
PG 16
WC Food Science & Technology; Toxicology
SC Food Science & Technology; Toxicology
GA 187EG
UT WOS:000322099100066
PM 23707562
ER
PT J
AU Woods, J
Kozubal, E
AF Woods, Jason
Kozubal, Eric
TI Combining liquid desiccant dehumidification with a dew-point evaporative
cooler: A design analysis
SO HVAC&R RESEARCH
LA English
DT Article
ID AIR-CONDITIONER; HEAT; PERFORMANCE; SYSTEM
AB This article uses a numerical model to analyze a concept combining a liquid desiccant dehumidifier with a dew-point indirect evaporative cooler. Each of these components, or stages, consists of an array of channel pairs, where a channel pair is two air channels separated by a thin plastic plate. In the first stage, a liquid desiccant film lining one side of the plates removes moisture from the process (supply-side) air through a membrane. An evaporatively cooled exhaust airstream on the other side of the plastic plate cools the desiccant. The second stage sensibly cools the dried process air with a dew-point evaporative cooler. This article uses a parametric analysis to illustrate the key design tradeoff for this concept: device size (a surrogate for cost) versus energy efficiency. The analysis finds the design parameters with the largest effect on this tradeoff and finds the combinations of design parameters giving near-optimal designs, which are designs with the highest efficiency for a given device size. The results indicate that there are two key parameters contributing to this tradeoff: the supply-side air channel thickness and the exhaust-air flow rate in the evaporative cooler.
C1 [Woods, Jason; Kozubal, Eric] Natl Renewable Energy Lab, Golden, CO USA.
RP Woods, J (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO USA.
EM jason.woods@nrel.gov
OI Woods, Jason/0000-0002-7661-2658
FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable
Energy Laboratory
FX This work was supported by the U.S. Department of Energy under Contract
No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory.
NR 17
TC 6
Z9 6
U1 3
U2 18
PU TAYLOR & FRANCIS INC
PI PHILADELPHIA
PA 325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA
SN 1078-9669
J9 HVAC&R RES
JI HVAC&R Res.
PD AUG 1
PY 2013
VL 19
IS 6
BP 663
EP 675
DI 10.1080/10789669.2013.797861
PG 13
WC Thermodynamics; Construction & Building Technology; Engineering,
Mechanical
SC Thermodynamics; Construction & Building Technology; Engineering
GA 205VZ
UT WOS:000323474200003
ER
PT J
AU Derr, K
Manic, M
AF Derr, Kurt
Manic, Milos
TI Wireless Sensor Network Configuration-Part I: Mesh Simplification for
Centralized Algorithms
SO IEEE TRANSACTIONS ON INDUSTRIAL INFORMATICS
LA English
DT Article
DE Delaunay triangulation; mesh generation; mesh simplification; sensor
node; wireless sensor network (WSN)
ID COMPUTING DIRICHLET TESSELLATIONS; DEPLOYMENT
AB This is the first of a two-part investigation of centralized and decentralized approaches for determining the optimal configuration of a sensor network. In this first part, we present a centralized approach for the generation of mesh (wireless sensor) network configurations that provide complete sensing coverage and communication connectivity of a domain. A challenging problem in deploying wireless sensor networks is maximizing coverage in irregular shaped polygonal areas while maintaining a high degree of node connectivity. The novelties presented in this paper are: 1) a centralized mesh simplification technique, the Iterative Node Removal with Constrained Delaunay Triangulation and Smoothing (INRCDTS) algorithm, and 2) a centralized mesh generation approach with INRCDTS that may be used for any nonintersecting closed polygonal area. Additionally, we provide a comparison of two centralized mesh generation techniques. The INRCDTS was built and tested as an enhancement of two traditional mesh generation techniques: advancing front technique and MATLAB partial differential equation toolbox. The INCRCDTS introduces the ability to tune the generated mesh configuration to the number of nodes and nodal spacing. The INRCDTS enhancement has proven to increase the uniformity of the mesh in an irregular shaped polygonal area relative to advancing front and MATLAB partial differential equation algorithms by 23% and 41%, respectively.
C1 [Derr, Kurt] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Manic, Milos] Univ Idaho, Idaho Falls, ID 83402 USA.
RP Derr, K (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA.
EM kurt.derr@inl.gov; misko@ieee.org
NR 33
TC 7
Z9 7
U1 1
U2 9
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 1551-3203
J9 IEEE T IND INFORM
JI IEEE Trans. Ind. Inform.
PD AUG
PY 2013
VL 9
IS 3
BP 1717
EP 1727
DI 10.1109/TII.2013.2245906
PG 11
WC Automation & Control Systems; Computer Science, Interdisciplinary
Applications; Engineering, Industrial
SC Automation & Control Systems; Computer Science; Engineering
GA 207AX
UT WOS:000323569900053
ER
PT J
AU Derr, K
Manic, M
AF Derr, Kurt
Manic, Milos
TI Wireless Sensor Network Configuration-Part II: Adaptive Coverage for
Decentralized Algorithms
SO IEEE TRANSACTIONS ON INDUSTRIAL INFORMATICS
LA English
DT Article
DE Adaptive algorithm; distributed algorithm; Extended Virtual Spring Mesh
(EVSM); self-organizing network; un-manned vehicle; wireless sensor
network (WSN)
ID DEPLOYMENT
AB This is the second of a two-part investigation of the generation of wireless sensor network (WSN) configurations that: 1) maximize coverage of irregular shaped polygonal areas and 2) maintain a high degree of node connectivity. The first-part of the investigation presented centralized algorithms for the generation of mesh (wireless sensor) network configurations that maximize coverage and connectivity. In this second part, we present a decentralized and distributed approach using an Extended Virtual Spring Mesh (EVSM)-Adaptive Coverage Algorithm and Protocol (ACAP) algorithm. The EVSM-ACAP algorithm represents an extension of EVSM algorithm with the newly developed ACAP. ACAP provides adaptive coverage and configuration of the mesh network by dynamically adjusting the sensing range of sensor nodes. EVSM-ACAP is compared to centralized mesh generation algorithms (described in the part one of the investigation), as well as other decentralized algorithms from artificial physics, for the control of large numbers of physical agents in sensor networks. EVSM-ACAP is shown to produce a sensor network deployment with an average sensor spacing within 1.6% of the desired spacing, versus 5.75% for the best centralized algorithmic approach. To the best of our knowledge, this is the first time that these centralized mesh network configuration algorithms have been contrasted with the scalable, robust, decentralized algorithms of artificial physics and EVSM.
C1 [Derr, Kurt] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Manic, Milos] Univ Idaho, Idaho Falls, ID 83402 USA.
RP Derr, K (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA.
EM kurt.derr@inl.gov; misko@ieee.org
NR 31
TC 12
Z9 12
U1 1
U2 18
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 1551-3203
EI 1941-0050
J9 IEEE T IND INFORM
JI IEEE Trans. Ind. Inform.
PD AUG
PY 2013
VL 9
IS 3
BP 1728
EP 1738
DI 10.1109/TII.2013.2245907
PG 11
WC Automation & Control Systems; Computer Science, Interdisciplinary
Applications; Engineering, Industrial
SC Automation & Control Systems; Computer Science; Engineering
GA 207AX
UT WOS:000323569900054
ER
PT J
AU Gomez, ME
Campillo, GE
Diez, S
Hoffmann, A
Lopera, W
AF Gomez, Maria E.
Campillo, Gloria E.
Diez, Sandra
Hoffmann, Axel
Lopera, Wilson
TI Influence of the Thickness of the Ferro- and Antiferromagnetic Phases on
Magnetic Properties in Epitaxial Heterostructures Based on Exchange
Biased La-Ca-Mn-O System
SO IEEE TRANSACTIONS ON MAGNETICS
LA English
DT Article; Proceedings Paper
CT 10th Latin American Workshop on Magnetism, Magnetic Materials and their
Applications (LAW3M)
CY APR 08-12, 2013
CL Univ Buenos Aires, Facultad Derecho, Buenos Aires, ARGENTINA
SP IEEE Magnet Soc
HO Univ Buenos Aires, Facultad Derecho
DE Ca-doped lanthanum manganite system; exchange biased oxide materials;
ferromagnetic/antiferromagnetic superlattices
ID LA2/3CA1/3MNO3/LA1/3CA2/3MNO3 SUPERLATTICES; MAGNETOTRANSPORT
PROPERTIES; MULTILAYERS; FILMS
AB Metal oxides show fascinating physical properties such as ferromagnetism, antiferromagnetism, high temperature superconductivity, ferroelectricity, or even multiferroicity. For many possible electronic applications as well as fundamental studies, it is essential to fabricate epitaxial layered films and multilayers of these materials having complex lattice structures with sharp interfaces, preserving epitaxiallity through the whole structure. We have grown these kind of oxide heterostructures on single crystal (001) oriented SrTiO3 substrates by using an in-situ DC sputtering technique at high oxygen pressures. Specifically, we report the study of magnetic and transport properties in ferromagnetic/antiferromagnetic, F/AF, heterostructures based on the Ca-doped lanthanum manganite system. We artificially grew La2/3Ca1/3MnO3/La1/3Ca2/3MnO3 heterostructures, maintaining constant the total thickness of the sample and systematically varying the thicknesses of the antiferromagnetic layer (t(AF)) and ferromagnetic layer (t(F)). Magnetization measurements indicate a dependence of Curie temperature, exchange bias field, and magnetoresistance behavior with the t(AF)/t(F) ratio.
C1 [Gomez, Maria E.; Diez, Sandra; Lopera, Wilson] Univ Valle, Dept Phys, Thin Film Grp, Cali 25360, Colombia.
[Campillo, Gloria E.] Univ Medellin, Dept Ciencias Basicas, Medellin, Colombia.
[Hoffmann, Axel] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
RP Gomez, ME (reprint author), Univ Valle, Dept Phys, Thin Film Grp, Cali 25360, Colombia.
EM maria.gomez@correounivalle.edu.co
RI Hoffmann, Axel/A-8152-2009
OI Hoffmann, Axel/0000-0002-1808-2767
NR 17
TC 0
Z9 0
U1 2
U2 20
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9464
J9 IEEE T MAGN
JI IEEE Trans. Magn.
PD AUG
PY 2013
VL 49
IS 8
BP 4576
EP 4581
DI 10.1109/TMAG.2013.2257711
PN 1
PG 6
WC Engineering, Electrical & Electronic; Physics, Applied
SC Engineering; Physics
GA 207ZE
UT WOS:000323642800024
ER
PT J
AU Mardegan, JRL
Aliouane, N
Coelho, LN
Aguero, O
Bittar, EM
Lang, JC
Pagliuso, PG
Torriani, IL
Giles, C
AF Mardegan, Jose R. L.
Aliouane, Nadir
Coelho, Leticia N.
Agueero, Oscar
Bittar, Eduardo M.
Lang, Jonathan C.
Pagliuso, Pascoal G.
Torriani, Iris L.
Giles, Carlos
TI Structural Distortion and Magnetic Order in the Intermetallic Eu3Ir4Sn13
Compound
SO IEEE TRANSACTIONS ON MAGNETICS
LA English
DT Article; Proceedings Paper
CT 10th Latin American Workshop on Magnetism, Magnetic Materials and their
Applications (LAW3M)
CY APR 08-12, 2013
CL Univ Buenos Aires, Facultad Derecho, Buenos Aires, ARGENTINA
SP IEEE Magnet Soc
HO Univ Buenos Aires, Facultad Derecho
DE Antiferromagnetic materials; crystallography; intermetallic; magnetic
properties
ID CRYSTAL-STRUCTURE; TRANSPORT-PROPERTIES; SNYB3RH4SN12; STANNIDES; EU
AB In this work, we have investigated the low temperature structural distortion and magnetic properties of the Eu3Ir4Sn13 Remeika cubic phase compound using X-ray powder diffraction (XRD), X-ray resonant magnetic scattering (XRMS) and neutron diffraction. X-ray scattering revealed that the peak observed in electrical resistivity and heat capacity measurements is related to a structural distortion at T* = 57.1 K. This crystallographic distortion characterized by the arising of a propagation vector (q) over right arrow = (0, (1/2), (1/2)) is due to a displacement of the Sn ions at the Sn1Sn2(12) polyhedron. In addition, the neutron diffraction experiments performed on a single crystal of Eu3Ir4Sn13 exhibit an antiferromagnetic coupling below T-N = 10.1 K where we observe a commensurate magnetic propagation vector (tau) over right arrow = (0, (1/2), (1/2)) identical to the one observed for the structural distortion.
C1 [Mardegan, Jose R. L.; Agueero, Oscar; Pagliuso, Pascoal G.; Torriani, Iris L.; Giles, Carlos] Univ Estadual Campinas, Inst Fis Gleb Wataghin, UNICAMP, BR-13083859 Campinas, SP, Brazil.
[Aliouane, Nadir] Paul Scherrer Inst, Neutron Scattering Lab, CH-5232 Villigen, Switzerland.
[Coelho, Leticia N.] Univ Brasilia, Inst Fis, BR-70919970 Brasilia, DF, Brazil.
[Bittar, Eduardo M.] Lab Nacl Luz Sincrotron, BR-13083970 Sao Paulo, Brazil.
[Lang, Jonathan C.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Mardegan, JRL (reprint author), Univ Estadual Campinas, Inst Fis Gleb Wataghin, UNICAMP, BR-13083859 Campinas, SP, Brazil.
EM jrlmardegan@gmail.com
RI Bittar, Eduardo/B-6266-2008; Inst. of Physics, Gleb
Wataghin/A-9780-2017; Torriani, Iris/E-5686-2010
OI Bittar, Eduardo/0000-0002-2762-1312;
NR 19
TC 5
Z9 5
U1 1
U2 27
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9464
J9 IEEE T MAGN
JI IEEE Trans. Magn.
PD AUG
PY 2013
VL 49
IS 8
BP 4652
EP 4655
DI 10.1109/TMAG.2013.2255589
PN 1
PG 4
WC Engineering, Electrical & Electronic; Physics, Applied
SC Engineering; Physics
GA 207ZE
UT WOS:000323642800042
ER
PT J
AU Schwank, J
Brown, D
Girard, S
Gouker, P
Gerardin, S
Quinn, H
Barnaby, H
AF Schwank, Jim
Brown, Dennis
Girard, Sylvain
Gouker, Pascale
Gerardin, Simone
Quinn, Heather
Barnaby, Hugh
TI SELECTED PAPERS FROM THE 2012 RADIATION AND ITS EFFECTS ON COMPONENTS
AND SYSTEMS (RADECS) CONFERENCE, Biarritz, France, September 24-28, 2012
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Editorial Material
C1 [Schwank, Jim] Sandia Natl Labs, Livermore, CA 94550 USA.
[Girard, Sylvain] Univ St Etienne, St Etienne, France.
[Gouker, Pascale] MIT Lincoln Lab, Cambridge, MA USA.
[Gerardin, Simone] Univ Padua, I-35100 Padua, Italy.
[Quinn, Heather] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Barnaby, Hugh] Arizona State Univ, Tempe, AZ 85287 USA.
RP Schwank, J (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA.
NR 0
TC 0
Z9 0
U1 0
U2 2
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2383
EP 2383
DI 10.1109/TNS.2013.2274257
PN 1
PG 1
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NJ
UT WOS:000323450700002
ER
PT J
AU Dodds, NA
Hooten, NC
Reed, RA
Schrimpf, RD
Warner, JH
Roche, NJH
McMorrow, D
Buchner, S
Jordan, S
Pellish, JA
Bennett, WG
Gaspard, NJ
King, MP
AF Dodds, N. A.
Hooten, N. C.
Reed, R. A.
Schrimpf, R. D.
Warner, J. H.
Roche, N. J. -H.
McMorrow, D.
Buchner, S.
Jordan, S.
Pellish, J. A.
Bennett, W. G.
Gaspard, N. J.
King, M. P.
TI SEL-Sensitive Area Mapping and the Effects of Reflection and Diffraction
From Metal Lines on Laser SEE Testing
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article; Proceedings Paper
CT European Conference on Radiation and its Effects on Components and
Systems (RADECS)
CY SEP 24-28, 2012
CL Biarritz, FRANCE
SP Univ Bordeaux, IMS Labs, RADECS Org, IEEE, Nucl & Plasma Sci Soc (NPSS), French Minist Higher Educ & Res, Conseil Reg Aquitaine, French Natl Ctr Sci Res (CNRS), Univ Bordeaux
DE Laser testing; sensitive volume; single-event latchup; single-photon
absorption (SPA); two-photon absorption (TPA)
ID PARTICLE-INDUCED LATCHUP; CMOS TEST STRUCTURES; CHARGE COLLECTION;
2-PHOTON ABSORPTION; CARRIER GENERATION; PULSED-LASER; SINGLE; DEVICES;
TECHNOLOGY
AB Laser and heavy-ion data reveal the areas and shapes of single-event latchup (SEL)-sensitive regions in CMOS test structures and their positions relative to the affected p-n-p-n paths. Contrary to previous two-dimensional studies, this three-dimensional study shows that the position of maximum SEL sensitivity in these structures is not centered on a p-n-p-n region, but between two neighboring p-n-p-n regions, suggesting that synergistic triggering increases SEL sensitivity.
The SEL-sensitivity maps suggest that laser light scattered from metal lines toward the silicon can contribute to the SEE response, for both back-side-incident two-photon absorption and front-side-incident single-photon absorption laser tests. We describe the metallization configurations and laser pulse energies for which reflected and/or diffracted laser light may contribute to the single-event effect (SEE) response.
C1 [Dodds, N. A.; Hooten, N. C.; Reed, R. A.; Schrimpf, R. D.; Bennett, W. G.; Gaspard, N. J.; King, M. P.] Vanderbilt Univ, Nashville, TN 37203 USA.
[Warner, J. H.; Roche, N. J. -H.; McMorrow, D.; Buchner, S.] Naval Res Lab, Washington, DC 20375 USA.
[Jordan, S.] Jazz Semicond, Newport Beach, CA 92660 USA.
[Pellish, J. A.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA.
RP Dodds, NA (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA.
EM nadodds@sandia.gov
RI Schrimpf, Ronald/L-5549-2013
OI Schrimpf, Ronald/0000-0001-7419-2701
NR 30
TC 7
Z9 8
U1 2
U2 15
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2550
EP 2558
DI 10.1109/TNS.2013.2246189
PN 1
PG 9
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NJ
UT WOS:000323450700026
ER
PT J
AU Javanainen, A
Ferlet-Cavrois, V
Jaatinen, J
Kettunen, H
Muschitiello, M
Pintacuda, F
Rossi, M
Schwank, JR
Shaneyfelt, MR
Virtanen, A
AF Javanainen, Arto
Ferlet-Cavrois, Veronique
Jaatinen, Jukka
Kettunen, Heikki
Muschitiello, Michele
Pintacuda, Francesco
Rossi, Mikko
Schwank, James R.
Shaneyfelt, Marty R.
Virtanen, Ari
TI Semi-Empirical Model for SEGR Prediction
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article; Proceedings Paper
CT European Conference on Radiation and its Effects on Components and
Systems (RADECS)
CY SEP 24-28, 2012
CL Biarritz, FRANCE
SP Univ Bordeaux, IMS Labs, RADECS Org, IEEE, Nucl & Plasma Sci Soc (NPSS), French Minist Higher Educ & Res, Conseil Reg Aquitaine, French Natl Ctr Sci Res (CNRS), Univ Bordeaux
DE Modeling; MOS; SEGR; semi-empirical
ID EVENT GATE RUPTURE; VERTICAL POWER MOSFETS; DIELECTRIC-BREAKDOWN;
HEAVY-IONS; CONDUCTION; EXPRESSION
AB The underlying physical mechanisms in single event gate rupture (SEGR) are not known precisely. SEGR is expected to occur when the energy deposition due to a heavy ion strike exceeds a certain threshold simultaneously with sufficient electric field across the gate dielectric. Typically the energy deposition is described by using the linear energy transfer (LET) of the given ion. Previously the LET has been demonstrated not to describe the SEGR sufficiently. The work presented here introduces a semi-empirical model for the SEGR prediction based on statistical variations in the energy deposition which are described theoretically.
C1 [Javanainen, Arto; Jaatinen, Jukka; Kettunen, Heikki; Rossi, Mikko; Virtanen, Ari] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland.
[Ferlet-Cavrois, Veronique; Muschitiello, Michele] European Space Agcy, Estec, NL-2200 AG Noordwijk, Netherlands.
[Pintacuda, Francesco] STMicroelectronics Srl, Catania, Italy.
[Schwank, James R.; Shaneyfelt, Marty R.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Javanainen, A (reprint author), Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland.
EM arto.javanainen@jyu.fi
RI Javanainen, Arto/P-6355-2016;
OI Javanainen, Arto/0000-0001-7906-3669; Virtanen, Ari/0000-0002-6591-6787
NR 14
TC 2
Z9 2
U1 0
U2 4
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2660
EP 2665
DI 10.1109/TNS.2012.2236105
PN 1
PG 6
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NJ
UT WOS:000323450700042
ER
PT J
AU Quinn, H
Graham, P
Morgan, K
Baker, Z
Caffrey, M
Smith, D
Wirthlin, M
Bell, R
AF Quinn, Heather
Graham, Paul
Morgan, Keith
Baker, Zachary
Caffrey, Michael
Smith, Dave
Wirthlin, Mike
Bell, Randy
TI Flight Experience of the Xilinx Virtex-4
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article; Proceedings Paper
CT European Conference on Radiation and its Effects on Components and
Systems (RADECS)
CY SEP 24-28, 2012
CL Biarritz, FRANCE
SP Univ Bordeaux, IMS Labs, RADECS Org, IEEE, Nucl & Plasma Sci Soc (NPSS), French Minist Higher Educ & Res, Conseil Reg Aquitaine, French Natl Ctr Sci Res (CNRS), Univ Bordeaux
DE Emulation; fault tolerance; field programmable gate arrays
ID FPGAS
AB This paper provides information regarding the use of the Xilinx Virtex-4 field-programmable gate array (FPGA) in a spacecraft deployed to low-earth orbit. The results are compared to pre-deployment accelerated single-event effects (SEEs) and fault-injection testing.
C1 [Quinn, Heather; Graham, Paul; Morgan, Keith; Baker, Zachary; Caffrey, Michael; Smith, Dave] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Wirthlin, Mike] Brigham Young Univ, Provo, UT 84602 USA.
[Bell, Randy] US DOE, Washington, DC 20585 USA.
RP Quinn, H (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM hquinn@lanl.gov
NR 11
TC 8
Z9 9
U1 0
U2 6
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2682
EP 2690
DI 10.1109/TNS.2013.2246581
PN 1
PG 9
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NJ
UT WOS:000323450700045
ER
PT J
AU Willis, JD
Collins, AG
Jurat-Fuentes, JL
Stewart, CN
AF Willis, Jonathan D.
Collins, A. Grace
Jurat-Fuentes, Juan-Luis
Stewart, C. Neal
TI Overexpression of TcEG1, an Insect Endoglucanase, in Switchgrass for
Improved Sugar Release
SO IN VITRO CELLULAR & DEVELOPMENTAL BIOLOGY-PLANT
LA English
DT Meeting Abstract
CT In Vitro Biology Meeting
CY JUN 15-19, 2013
CL Providence, RI
SP Soc In Vitro Biol
C1 [Willis, Jonathan D.; Collins, A. Grace; Stewart, C. Neal] Univ Tennessee, Dept Plant Sci, Knoxville, TN USA.
[Jurat-Fuentes, Juan-Luis] Univ Tennessee, Dept Entomol & Plant Pathol, Knoxville, TN 37901 USA.
[Willis, Jonathan D.; Stewart, C. Neal] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN USA.
EM jdwillis@utk.edu
NR 0
TC 0
Z9 0
U1 1
U2 5
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1054-5476
J9 IN VITRO CELL DEV-PL
JI In Vitro Cell. Dev. Biol.-Plant
PD AUG
PY 2013
VL 49
IS 4
BP 472
EP 473
PG 2
WC Plant Sciences; Cell Biology; Developmental Biology
SC Plant Sciences; Cell Biology; Developmental Biology
GA 206JG
UT WOS:000323515500018
ER
PT J
AU Fu, CX
Hernandez, T
Tudor, S
Wang, ZY
AF Fu, Chunxiang
Hernandez, Tim
Tudor, Steven
Wang, Zeng-Yu
TI Development of High Throughput Genetic Transformation Systems for Forage
and Biofuel Crops
SO IN VITRO CELLULAR & DEVELOPMENTAL BIOLOGY-PLANT
LA English
DT Meeting Abstract
CT In Vitro Biology Meeting
CY JUN 15-19, 2013
CL Providence, RI
SP Soc In Vitro Biol
C1 [Fu, Chunxiang; Hernandez, Tim; Tudor, Steven; Wang, Zeng-Yu] Samuel Roberts Noble Fdn Inc, Forage Improvement Div, Ardmore, OK 73401 USA.
[Wang, Zeng-Yu] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA.
EM cfu@noble.org
NR 0
TC 0
Z9 0
U1 0
U2 2
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1054-5476
J9 IN VITRO CELL DEV-PL
JI In Vitro Cell. Dev. Biol.-Plant
PD AUG
PY 2013
VL 49
IS 4
BP 475
EP 475
PG 1
WC Plant Sciences; Cell Biology; Developmental Biology
SC Plant Sciences; Cell Biology; Developmental Biology
GA 206JG
UT WOS:000323515500024
ER
PT J
AU Grant, JN
Willis, JD
Stewart, CN
AF Grant, Joshua N.
Willis, Jonathan D.
Stewart, C. Neal
TI Comparisons of Switchgrass Cell Wall Components Containing an
Overexpression of a Putative Switchgrass Endoglucanase
SO IN VITRO CELLULAR & DEVELOPMENTAL BIOLOGY-PLANT
LA English
DT Meeting Abstract
CT In Vitro Biology Meeting
CY JUN 15-19, 2013
CL Providence, RI
SP Soc In Vitro Biol
C1 [Grant, Joshua N.; Willis, Jonathan D.; Stewart, C. Neal] Univ Tennessee, Dept Plant Sci, Knoxville, TN USA.
[Willis, Jonathan D.; Stewart, C. Neal] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN USA.
EM jgrant2@utk.edu
NR 0
TC 0
Z9 0
U1 0
U2 5
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1054-5476
J9 IN VITRO CELL DEV-PL
JI In Vitro Cell. Dev. Biol.-Plant
PD AUG
PY 2013
VL 49
IS 4
BP 475
EP 475
PG 1
WC Plant Sciences; Cell Biology; Developmental Biology
SC Plant Sciences; Cell Biology; Developmental Biology
GA 206JG
UT WOS:000323515500025
ER
PT J
AU Austin, KG
Carvey, CE
Farina, EK
Lieberman, HR
AF Austin, Krista G.
Carvey, Christina E.
Farina, Emily K.
Lieberman, Harris R.
TI Predictors of the Relationships Between Nutritional Supplement Use and
Weight-Modification Goals of U.S. Army Soldiers
SO INTERNATIONAL JOURNAL OF SPORT NUTRITION AND EXERCISE METABOLISM
LA English
DT Article
DE dietary supplement; health behavior; weight management
ID EATING DISORDER BEHAVIORS; DIETARY-SUPPLEMENTS; BODY-IMAGE; CONTRIBUTING
FACTORS; MEAL-REPLACEMENT; UNITED-STATES; WOMEN; PREVALENCE; MEN;
PERFORMANCE
AB Background: U.S. Army Soldiers must meet body weight and composition standards and consequently may use nutritional supplements (NS) purported to assist in weight modification (WM). Nutritional supplements are dietary supplements (DS) and foods intended to supplement the diet. Purpose: This study assessed relationships between NS use, demographic characteristics, health-related behaviors, and WM goals among U.S. Army personnel. Methods: Participants (N = 990) self-reported NS use, categorized as energy drinks, sport nutrition products, or DS, and WM goal (lose, gain, or maintain) was ascertained by survey. DS were sub-categorized as health, weight-loss, weight-gain, or other DS. Chi-square and logistic regression were used to assess relationships between predictors, NS use, and WM goal. Most respondents (70.3% +/- 1.7%) consumed some NS; however, overall NS use was not related to WM goal. Significant relationships were observed between predictors (tobacco use, age, body-mass index, fitness score, general health, and eating habits) and both WM goal and NS use. Respondents attempting to lose or maintain weight were less likely to consume energy drinks and weight-gain DS. Conclusion: WM goal is related to multiple health behaviors including tobacco use, physical fitness score, and self-perception of health and eating behavior. NS are consumed in this population regardless of WM goal.
C1 [Austin, Krista G.; Farina, Emily K.] Oak Ridge Inst Sci & Educ, Belcamp, MD USA.
[Carvey, Christina E.; Lieberman, Harris R.] US Army Res Inst Environm Med, Natick, MA USA.
RP Austin, KG (reprint author), Oak Ridge Inst Sci & Educ, Belcamp, MD USA.
FU U.S. Army Medical Research and Materiel Command (USAMRMC); Department of
Defense Center Alliance for Dietary Supplement Research
FX This work was supported by the U.S. Army Medical Research and Materiel
Command (USAMRMC) and the Department of Defense Center Alliance for
Dietary Supplement Research. The opinions contained herein are the
private views of the authors and are not to be construed as official or
as reflecting the views of the Army or the Department of Defense.
Citations of commercial organizations and trade names in this report do
not constitute an official Department of the Army endorsement or
approval of the products or services of these organizations. Approved
for public release; distribution is unlimited.
NR 37
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U1 2
U2 26
PU HUMAN KINETICS PUBL INC
PI CHAMPAIGN
PA 1607 N MARKET ST, PO BOX 5076, CHAMPAIGN, IL 61820-2200 USA
SN 1526-484X
J9 INT J SPORT NUTR EXE
JI Int. J. Sport Nutr. Exerc. Metab.
PD AUG
PY 2013
VL 23
IS 4
BP 322
EP 335
PG 14
WC Nutrition & Dietetics; Sport Sciences
SC Nutrition & Dietetics; Sport Sciences
GA 208BE
UT WOS:000323649500003
PM 23239674
ER
PT J
AU Haight, TJ
Landau, SM
Carmichael, O
Schwarz, C
DeCarli, C
Jagust, WJ
AF Haight, Thaddeus J.
Landau, Susan M.
Carmichael, Owen
Schwarz, Christopher
DeCarli, Charles
Jagust, William J.
CA Alzheimer's Dis Neuroimaging
TI Dissociable Effects of Alzheimer Disease and White Matter
Hyperintensities on Brain Metabolism
SO JAMA NEUROLOGY
LA English
DT Article
ID MILD COGNITIVE IMPAIRMENT; EXECUTIVE DYSFUNCTION; GLUCOSE-METABOLISM;
DEMENTIA; BIOMARKERS; DECLINE; ASSOCIATION; PATHOLOGY; SYMPTOMS;
INFARCTS
AB IMPORTANCE Cerebrovascular disease and Alzheimer disease (AD) frequently co-occur and seem to act through different pathways in producing dementia.
OBJECTIVE To examine cerebrovascular disease and AD markers in relation to brain glucose metabolism in patients with mild cognitive impairment.
DESIGN AND SETTING Cohort study among the Alzheimer Disease Neuroimaging Initiative clinical sites in the United States and Canada.
PARTICIPANTS Two hundred three patients having amnestic mild cognitive impairment (74 of whom converted to AD) with serial imaging during a 3-year follow-up period.
MAIN OUTCOMES AND MEASURES Quantified white matter hyperintensities (WMHs) represented cerebrovascular disease, and cerebrospinal fluid beta-amyloid represented AD pathology. Brain glucose metabolism in temporoparietal and frontal brain regions was measured using positron emission tomography with fluorodeoxyglucose F18.
RESULTS In converters, greater WMHs were associated with decreased frontal metabolism (-0.048; 95% CI, -0.067 to -0.029) but not temporoparietal metabolism (0.010; 95% CI, -0.010 to 0.030). Greater cerebrospinal fluid beta-amyloid (per 10-pg/mL increase) was associated with increased temporoparietal metabolism (0.005; 95% CI, 0.000-0.010) but not frontal metabolism (0.002; 95% CI, -0.004 to 0.007) in the same patients. In nonconverters, similar relationships were observed except for a positive association of greater WMHs with increased temporoparietal metabolism (0.051; 95% CI, 0.027-0.076).
CONCLUSIONS AND RELEVANCE The dissociation of WMHs and cerebrospinal fluid beta-amyloid in relation to regional glucose metabolism suggests that these pathologic conditions operate through different and independent pathways in AD that reflect dysfunction in different brain systems. The positive association of greater WMHs with temporoparietal metabolism suggests that these pathologic processes do not co-occur in nonconverters.
C1 [Haight, Thaddeus J.; Landau, Susan M.; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA.
[Landau, Susan M.; Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
[Jagust, William J.] Univ Calif Berkeley, Sch Publ Hlth, Div Epidemiol, Berkeley, CA 94720 USA.
[Carmichael, Owen; Schwarz, Christopher; DeCarli, Charles] Univ Calif Davis, Dept Neurol, Davis, CA 95616 USA.
RP Haight, TJ (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, 118 Barker Hall,Mail Code 3190 Jagust Lab, Berkeley, CA 94720 USA.
EM tad@berkeley.edu
OI Schwarz, Christopher/0000-0002-1466-8357
FU ADNI from the National Institutes of Health [U01 AG024904]; National
Institute on Aging; National Institute of Biomedical Imaging and
Bioengineering; Canadian Institutes of Health Research; National
Institutes of Health [P30 AG010129, K01 AG030514]; Dana Foundation
FX Data collection and sharing for this project were funded by the ADNI
(grant U01 AG024904 from the National Institutes of Health). ADNI is
funded by the National Institute on Aging and the National Institute of
Biomedical Imaging and Bioengineering, as well as through generous
contributions from the following: Abbott, Alzheimer's Association,
Alzheimer's Drug Discovery Foundation, Amorfix Life Sciences Ltd,
AstraZeneca, Bayer HealthCare, BioClinica Inc, Biogen Idec Inc,
Bristol-Myers Squibb Company, Eisai Inc, Elan Pharmaceuticals Inc, Eli
Lilly and Company, F. Hoffmann-La Roche Ltd and its affiliated company
Genentech Inc, GE Healthcare, Innogenetics NV, Janssen Alzheimer
Immunotherapy, Johnson & Johnson Pharmaceutical Research & Development
LLC, Medpace Inc, Merck & Co, Meso Scale Diagnostics LLC, Novartis
Pharmaceuticals Corporation, Pfizer Inc, Servier, Synarc, and Takeda
Pharmaceutical Company. The Canadian Institutes of Health Research is
providing funds to support ADNI clinical sites in Canada. Private sector
contributions are facilitated by the Foundation for the National
Institutes of Health (http://www.fnih.org). The grantee organization is
the Northern California Institute for Research and Education, and the
study is coordinated by the Alzheimer's Disease Cooperative Study at the
University of California, San Diego. ADNI data are disseminated by the
Laboratory of Neuro Imaging at the University of California, Los
Angeles. This research was also supported by grants P30 AG010129 and K01
AG030514 from the National Institutes of Health and by the Dana
Foundation.
NR 38
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U1 1
U2 2
PU AMER MEDICAL ASSOC
PI CHICAGO
PA 330 N WABASH AVE, STE 39300, CHICAGO, IL 60611-5885 USA
SN 2168-6149
EI 2168-6157
J9 JAMA NEUROL
JI JAMA Neurol.
PD AUG
PY 2013
VL 70
IS 8
BP 1039
EP 1045
DI 10.1001/jamaneurol.2013.1878
PG 7
WC Clinical Neurology
SC Neurosciences & Neurology
GA 206ZO
UT WOS:000323565900013
PM 23779022
ER
PT J
AU Colotelo, AH
Cooke, SJ
Blouin-Demers, G
Murchie, KJ
Haxton, T
Smokorowski, KE
AF Colotelo, Alison H.
Cooke, Steven J.
Blouin-Demers, Gabriel
Murchie, Karen J.
Haxton, Tim
Smokorowski, Karen E.
TI Influence of water temperature and net tending frequency on the
condition of fish bycatch in a small-scale inland commercial fyke net
fishery
SO JOURNAL FOR NATURE CONSERVATION
LA English
DT Article
DE Bycatch; Inland commercial fisheries; Physiology; Injury
ID RELEASE ANGLING TOURNAMENTS; BONEFISH ALBULA-VULPES; LARGEMOUTH BASS;
MORTALITY; STRESS; SURVIVAL; BEHAVIOR; PHYSIOLOGY; EXERCISE; GEARS
AB To date, most studies of commercial fisheries bycatch have focused on mortality at time of capture as an endpoint. However, sub-lethal indicators of organismal condition have the potential to reveal mechanisms associated with mortality (both at time of capture and post-release) and opportunities for improving fish welfare. In this study, we simulated commercial fishing efforts in inland lakes with fyke nets during a typical fishing season (early April to late June) in southeastern Ontario, Canada, where bycatch of non-target fish species had previously been documented. Using non-target gamefish (i.e., largemouth bass [Micropterus salmoides, Lacepede], northern pike [Esox Lucius, L.]), as well as a target species (i.e., bluegill [Lepomis macrochirus, Rafinesque]), we examined the sub-lethal consequences of capture (e.g., blood physiology, reflex impairment, and injury) and compared the effects of being retained in the net for two different durations (i.e., two or six days) over a range of water temperatures (i.e., 3-28 degrees C). Sublethal physiological disturbances (i.e., blood glucose and lactate) in largemouth bass and bluegill tended to be greater at higher water temperatures. However, fish retained for six days generally did not exhibit greater stress than those retained for two days, with the exception of plasma glucose in largemouth bass. Reflex impairment was similar among temperature and retention periods. Fish retained in nets experienced a range of injuries (including fin frays, scale loss, and mouth damage) that had the potential to facilitate the development of opportunistic pathogenic infections. Greater incidences of injury on fish bycatch tended to be associated with higher temperatures and longer retention. To reduce physiological disturbances and injury that could lead to delayed mortality, we suggest that regulations for inland commercial fishers require them to check their nets more frequently as water temperatures increase. We suggest that future studies of bycatch incorporate sub-lethal endpoints given that they serve as an objective measure of fish welfare and can provide quantitative mechanistic information to support management actions. (C) 2013 Elsevier GmbH. All rights reserved.
C1 [Colotelo, Alison H.; Cooke, Steven J.; Murchie, Karen J.] Carleton Univ, Fish Ecol & Conservat Physiol Lab, Dept Biol, Ottawa, ON K1S 5B6, Canada.
[Cooke, Steven J.] Carleton Univ, Inst Environm Sci, Ottawa, ON K1S 5B6, Canada.
[Blouin-Demers, Gabriel] Univ Ottawa, Dept Biol, Ottawa, ON K1N 6N5, Canada.
[Haxton, Tim] Ontario Minist Nat Resources, Southern Sci & Informat Sect, Peterborough, ON K9L 8M5, Canada.
[Smokorowski, Karen E.] Fisheries & Oceans Canada, Great Lakes Lab Fisheries & Aquat Sci, Sault Ste Marie, ON P6A 2E5, Canada.
RP Colotelo, AH (reprint author), Pacific NW Natl Lab, POB 999,MSIN K6-85, Richland, WA 99352 USA.
EM Alison.Colotelo@pnnl.gov
RI Cooke, Steven/F-4193-2010;
OI Cooke, Steven/0000-0002-5407-0659; Haxton, Tim/0000-0002-9767-3986
FU Ontario Ministry of Natural Resources, Fisheries and Oceans Canada;
Canadian Wildlife Federation; World Wildlife Fund; Bob Jaquith of the
Ontario Commercial Fisheries Association; Canada Research Chair Program;
NSERC
FX All procedures used in this study were developed with approvals and
guidance from the Canadian Council on Animal Care administered by
Carleton University and Queen's University. Funding was provided by the
Ontario Ministry of Natural Resources, Fisheries and Oceans Canada, the
Canadian Wildlife Federation, and the World Wildlife Fund. We thank Bob
Jaquith of the Ontario Commercial Fisheries Association for providing
support for the project. Michael Davis kindly provided input on design
of the RAMP component. We also thank Cooke lab members for the
assistance with field work and data collection. Thank you to Keith
Stamplecoskie for formatting the manuscript. Cooke was supported by the
Canada Research Chair Program. Cooke and Blouin-Demers were also
supported by the NSERC Discovery Grant Program.
NR 47
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Z9 1
U1 2
U2 24
PU ELSEVIER GMBH, URBAN & FISCHER VERLAG
PI JENA
PA OFFICE JENA, P O BOX 100537, 07705 JENA, GERMANY
SN 1617-1381
J9 J NAT CONSERV
JI J. Nat. Conserv.
PD AUG
PY 2013
VL 21
IS 4
BP 217
EP 224
DI 10.1016/j.jnc.2013.01.001
PG 8
WC Biodiversity Conservation; Ecology
SC Biodiversity & Conservation; Environmental Sciences & Ecology
GA 207IQ
UT WOS:000323592500005
ER
PT J
AU Newsom, RK
Turner, DD
Goldsmith, JEM
AF Newsom, Rob K.
Turner, David D.
Goldsmith, John E. M.
TI Long-Term Evaluation of Temperature Profiles Measured by an Operational
Raman Lidar
SO JOURNAL OF ATMOSPHERIC AND OCEANIC TECHNOLOGY
LA English
DT Article
DE Instrumentation; sensors; Lidars; Lidar observations; Profilers;
atmospheric; Remote sensing
ID ATMOSPHERIC-TEMPERATURE; WATER-VAPOR; EXTINCTION; RADIOSONDE; AEROSOLS;
CLOUDS
AB This study investigates the accuracy and calibration stability of temperature profiles derived from an operational Raman lidar over a 2-yr period from 1 January 2009 to 31 December 2010. The lidar, which uses the rotational Raman technique for temperature measurement, is located at the U.S. Department of Energy's Atmospheric Radiation Measurement site near Billings, Oklahoma. The lidar performance specifications, data processing algorithms, and the results of several test runs are described. Calibration and overlap correction of the lidar is achieved using simultaneous and collocated radiosonde measurements. Results show that the calibration coefficients exhibit no significant long-term or seasonal variation but do show a distinct diurnal variation. When the diurnal variation in the calibration is not resolved the lidar temperature bias exhibits a significant diurnal variation. Test runs in which only nighttime radiosonde measurements are used for calibration show that the lidar exhibits a daytime warm bias that is correlated with the strength of the solar background signal. This bias, which reaches a maximum of similar to 2.4 K near solar noon, is reduced through the application of a correction scheme in which the calibration coefficients are parameterized in terms of the solar background signal. Comparison between the corrected lidar temperatures and the noncalibration radiosonde temperatures show a negligibly small median bias of -0.013 K for altitudes below 10 km AGL. The corresponding root-mean-square difference profile is roughly constant at similar to 2 K below 6 km AGL and increases to about 4.5 K at 10 km AGL.
C1 [Newsom, Rob K.] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Turner, David D.] NOAA, Natl Severe Storms Lab, Norman, OK 73069 USA.
[Goldsmith, John E. M.] Sandia Natl Labs, Livermore, CA USA.
RP Newsom, RK (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999,MSIN K9-30, Richland, WA 99352 USA.
EM rob.newsom@pnnl.gov
FU Office of Biological and Environmental Research of the U.S. Department
of Energy as part of the Atmospheric Radiation Measurement Climate
Research Facility
FX We wish to thank the staff at the ARM SGP site and Chris Martin in
particular for maintaining the operation of the Raman lidar. This
research was supported by the Office of Biological and Environmental
Research of the U.S. Department of Energy as part of the Atmospheric
Radiation Measurement Climate Research Facility.
NR 26
TC 19
Z9 19
U1 5
U2 18
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0739-0572
J9 J ATMOS OCEAN TECH
JI J. Atmos. Ocean. Technol.
PD AUG
PY 2013
VL 30
IS 8
BP 1616
EP 1634
DI 10.1175/JTECH-D-12-00138.1
PG 19
WC Engineering, Ocean; Meteorology & Atmospheric Sciences
SC Engineering; Meteorology & Atmospheric Sciences
GA 207XM
UT WOS:000323638000003
ER
PT J
AU Luke, EP
Kollias, P
AF Luke, Edward P.
Kollias, Pavlos
TI Separating Cloud and Drizzle Radar Moments during Precipitation Onset
Using Doppler Spectra
SO JOURNAL OF ATMOSPHERIC AND OCEANIC TECHNOLOGY
LA English
DT Article
DE Dynamics; Drizzle; Marine boundary layer; Stratiform clouds; Cloud
retrieval; Radars; Radar observations
ID VERTICAL AIR VELOCITIES; DROP-SIZE DISTRIBUTION; PARAMETERS; PROFILER;
DISTRIBUTIONS; SCATTERING; TURBULENCE; MOTION; GHZ; MIE
AB The retrieval of cloud, drizzle, and turbulence parameters using radar Doppler spectra is challenged by the convolution of microphysical and dynamical influences and the overall uncertainty introduced by turbulence. A new technique that utilizes recorded radar Doppler spectra from profiling cloud radars is presented here. The technique applies to areas in clouds where drizzle is initially produced by the autoconversion process and is detected by a positive skewness in the radar Doppler spectrum. Using the Gaussian-shape property of cloud Doppler spectra, the cloud-only radar Doppler spectrum is estimated and used to separate the cloud and drizzle contributions. Once separated, the cloud spectral peak can be used to retrieve vertical air motion and eddy dissipation rates, while the drizzle peak can be used to estimate the three radar moments of the drizzle particle size distribution. The technique works for nearly 50% of spectra found near cloud top, with efficacy diminishing to roughly 15% of spectra near cloud base. The approach has been tested on a large dataset collected in the Azores during the Atmospheric Radiation Measurement Program (ARM) Mobile Facility deployment on Graciosa Island from May 2009 through December 2010. Validation of the proposed technique is achieved using the cloud base as a natural boundary between radar Doppler spectra with and without cloud droplets. The retrieval algorithm has the potential to characterize the dynamical and microphysical conditions at cloud scale during the transition from cloud to precipitation. This has significant implications for improving the understanding of drizzle onset in liquid clouds and for improving model parameterization schemes of autoconversion of cloud water into drizzle.
C1 [Luke, Edward P.] Brookhaven Natl Lab, Div Atmospher Sci, Upton, NY 11973 USA.
[Kollias, Pavlos] McGill Univ, Dept Atmospher & Ocean Sci, Montreal, PQ, Canada.
RP Luke, EP (reprint author), Brookhaven Natl Lab, Div Atmospher Sci, Bldg 490D,Bell Ave, Upton, NY 11973 USA.
EM eluke@bnl.gov
FU Atmospheric System Research program of the Office of Biological and
Environmental Research of the U.S. Department of Energy
[DE-AC02-98CH10886]
FX This research was supported under Contract DE-AC02-98CH10886 by the
Atmospheric System Research program of the Office of Biological and
Environmental Research of the U.S. Department of Energy. Data were
obtained from the ARM Climate Research Facility of the U.S. Department
of Energy.
NR 29
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Z9 17
U1 2
U2 27
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0739-0572
J9 J ATMOS OCEAN TECH
JI J. Atmos. Ocean. Technol.
PD AUG
PY 2013
VL 30
IS 8
BP 1656
EP 1671
DI 10.1175/JTECH-D-11-00195.1
PG 16
WC Engineering, Ocean; Meteorology & Atmospheric Sciences
SC Engineering; Meteorology & Atmospheric Sciences
GA 207XM
UT WOS:000323638000005
ER
PT J
AU Giangrande, SE
McGraw, R
Lei, L
AF Giangrande, Scott E.
McGraw, Robert
Lei, Lei
TI An Application of Linear Programming to Polarimetric Radar Differential
Phase Processing
SO JOURNAL OF ATMOSPHERIC AND OCEANIC TECHNOLOGY
LA English
DT Article
DE Hydrometeorology; Algorithms; Radars; Radar observations; Remote sensing
ID DUAL-POLARIZATION RADAR; ENSEMBLE KALMAN FILTER; X-BAND; PART II;
REFLECTIVITY; CALIBRATION; RAINFALL; ATTENUATION; ASSIMILATION;
SIMULATION
AB Differential phase and its range derivative K-DP are of interest to several hydrological applications from weather radar systems. Despite the attractive qualities of polarimetric differential phase measurements, the usefulness of these radar measurements is potentially undermined as a consequence of measurement fluctuations and physical or beam geometry artifacts. This paper presents an application of linear programming for physical retrievals, here designed to improve estimates of differential propagation phase by allowing realistic physical constraints of monotonicity and polarimetric radar self-consistency. Results of the linear programming methods to the phase-processing problem are demonstrated at several common weather radar wavelengths (10, 5, and 3 cm).
C1 [Giangrande, Scott E.; McGraw, Robert] Brookhaven Natl Lab, Div Atmospher Sci, Upton, NY 11973 USA.
[Lei, Lei] Univ Oklahoma, Norman, OK 73019 USA.
RP Giangrande, SE (reprint author), Brookhaven Natl Lab, Div Atmospher Sci, Bldg 490D,POB 5000, Upton, NY 11973 USA.
EM scott.giangrande@bnl.gov
RI Giangrande, Scott/I-4089-2016
OI Giangrande, Scott/0000-0002-8119-8199
FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; Climate Science
for a Sustainable Energy Future project of the Earth System Modeling
(ESM) program in the DOE Office of Science; FASTER project; DOE ESM
program; U.S. Department of Energy
FX This paper has been authored by employees of Brookhaven Science
Associates, LLC, under Contract DE-AC02-98CH10886 with the U.S.
Department of Energy. The publisher by accepting the manuscript for
publication acknowledges that the U.S. government retains a
nonexclusive, paid-up, irrevocable, worldwide license to publish or
reproduce the published form of this manuscript, or allow others to do
so, for U.S. government purposes. Doctor Giangrande's work is supported
by the Climate Science for a Sustainable Energy Future project of the
Earth System Modeling (ESM) program in the DOE Office of Science. Doctor
McGraw's support is from the FASTER project (http://www.bnl.gov/faster/)
supported by the DOE ESM program. The authors thank Drs. Alexander
Ryzhkov (OU-NSSL), Michele Galletti (BNL), and Guifu Zhang (OU) for
critical discussions throughout the writing process as well as the
comments of several anonymous reviewers. Additional ARM radar dataset
support and operational implementation were assisted by Dr. Scott Collis
(ANL). A version of the LP-based method described by this manuscript and
all associated datasets are freely available online (http://www.arm.gov)
and as part of the open-source Python ARM Radar Toolkit.
NR 42
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Z9 11
U1 0
U2 8
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0739-0572
EI 1520-0426
J9 J ATMOS OCEAN TECH
JI J. Atmos. Ocean. Technol.
PD AUG
PY 2013
VL 30
IS 8
BP 1716
EP 1729
DI 10.1175/JTECH-D-12-00147.1
PG 14
WC Engineering, Ocean; Meteorology & Atmospheric Sciences
SC Engineering; Meteorology & Atmospheric Sciences
GA 207XM
UT WOS:000323638000009
ER
PT J
AU Dimitrijevic, NM
Tepavcevic, S
Liu, YZ
Rajh, T
Silver, SC
Tiede, DM
AF Dimitrijevic, Nada M.
Tepavcevic, Sanja
Liu, Yuzi
Rajh, Tijana
Silver, Sunshine C.
Tiede, David M.
TI Nanostructured TiO2/Polypyrrole for Visible Light Photocatalysis
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID TIO2 NANOPARTICLES; DEGRADATION; OLIGOMERS; NANOCOMPOSITES; POLYPYRROLE;
COMPOSITES; POLYMERS; DYNAMICS; CHARGES; PHENOL
AB Stable TiO2/polypyrrole nanocomposites have been synthesized by a simple one-step hydrothermal method. The nanocomposites are capable of efficient visible-light photocatalysis driven by their morphology that utilizes a high concentration of 4.5 nm TiO2 nanoparticles electronically coupled to 200-300 nm polypyrrole granules. The polypyrrole acts as visible-light photosensitizer, and the photoactivity of nanocomposite arises from the electron transfer from excited polypyrrole to TiO2 nanopartides and further across nanocomposite interface. The visible-light photocatalysis is demonstrated by methylene blue degradation and by the production of H-2 from water with efficiency of 1 mmol H-2 g(catalyst)(-1) h(-1)wt %(Pt)(-1).
C1 [Dimitrijevic, Nada M.; Silver, Sunshine C.; Tiede, David M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Dimitrijevic, Nada M.; Tepavcevic, Sanja; Liu, Yuzi; Rajh, Tijana] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA.
RP Dimitrijevic, NM (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM Dimitrijevic@anl.gov
RI Liu, Yuzi/C-6849-2011
FU Department of Energy, Office of Science, Office of Basic Energy Sciences
[DE-AC02-06CH11357]
FX This work was supported by Department of Energy, Office of Science,
Office of Basic Energy Sciences, under Contract No. DE-ACO2-06CH11357.
NR 27
TC 34
Z9 34
U1 10
U2 86
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 1
PY 2013
VL 117
IS 30
BP 15540
EP 15544
DI 10.1021/jp405562b
PG 5
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 196WG
UT WOS:000322807500010
ER
PT J
AU Savara, A
AF Savara, Aditya
TI Standard States for Adsorption on Solid Surfaces: 2D Gases, Surface
Liquids, and Langmuir Adsorbates
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID THIN-FILMS; N-ALKANES; THERMODYNAMICS; SPECTROSCOPY; ENTROPIES;
MGO(100); KINETICS; OXIDE; IR
AB Standard states are utilized to compare thermodynamic data obtained from different experiments and calculations, and this ability to compare thermodynamic data plays an important role in science and society. For molecules adsorbed on surfaces, there are currently no universally accepted standard states. Here, standard states are proposed for the different types of molecular adsorbate phases, with the intent to enable physical insight to be gained by tabulating experimental/calculated values, such that comparison between different systems and existing societal tabulations of chemical standard state tabulated values can be done directly. A "density based" standard state is proposed for 2D gases, and a "relative coverage based" standard state is proposed for immobile adsorbates and nonislanding 2D liquids. These units are chosen based upon the units which the activity depends on. The standard states recommended here are chosen due to the entropies associated with them, such that physical insight can be gained by direct comparison to existing tabulated data. For 2D gases adsorbed on solid surfaces, the recommended standard state is sigma(o) = 1.39 X 10(-7) mol m(-2). For immobile adsorbates and nonislanding liquid states on solid surfaces, the recommended standard state is theta(o)(A) = 0.5 (which implies a standard state for the surface sites of of theta(o)(s) = 1 - theta(o)(A) = 0.5). With the standard states recommended here, tabulated values at a common temperature are expected to display the following approximate hierarchy for decreasing entropy: 3D gas > 2D gas > liquid > surface liquid > solid > lattice confined. Recommended standard states are also provided in the Supporting Information for cases with dissociative adsorption.
C1 Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA.
RP Savara, A (reprint author), Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37830 USA.
EM savaraa@ornl.gov
RI Savara, Aditya (Ashi)/A-8831-2010
OI Savara, Aditya (Ashi)/0000-0002-1937-2571
FU Laboratory Directed Research and Development Program of Oak Ridge
National Laboratory
FX Research sponsored by the Laboratory Directed Research and Development
Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC,
for the U.S. Department of Energy. A.S. thanks James Kindt for useful
discussions regarding the configurational entropy of immobile
adsorbates.
NR 28
TC 10
Z9 10
U1 3
U2 23
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 1
PY 2013
VL 117
IS 30
BP 15710
EP 15715
DI 10.1021/jp404398z
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 196WG
UT WOS:000322807500029
ER
PT J
AU Sheridan, LB
Kim, YG
Perdue, BR
Jagannathan, K
Stickney, JL
Robinson, DB
AF Sheridan, Leah B.
Kim, Youn-Geun
Perdue, Brian R.
Jagannathan, Kaushik
Stickney, John L.
Robinson, David B.
TI Hydrogen Adsorption, Absorption, and Desorption at Palladium Nanofilms
formed on Au(111) by Electrochemical Atomic Layer Deposition (E-ALD):
Studies using Voltammetry and In Situ Scanning Tunneling Microscopy
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID SULFURIC-ACID-SOLUTION; LIMITED REDOX REPLACEMENT;
ENERGY-ELECTRON-DIFFRACTION; SINGLE-CRYSTAL ELECTRODES; ONE-CELL
CONFIGURATION; WELL-DEFINED SURFACES; PD DEPOSITION; UNDERPOTENTIAL
DEPOSITION; EPITAXIAL-GROWTH; COMPOUND SEMICONDUCTORS
AB Pd nanofilms were grown on Au(111) using the electrochemical form of atomic layer deposition (E-ALD). Deposits were formed by repeated cycles of surface-limited redox replacement (SLRR). Each cycle produced an atomic layer of Pd, allowing the reproducible formation of Pd nanofilms, with thicknesses proportional to the number of cycles performed. Pd deposits were formed with up to 30 cycles, in the present study, and used as a platform for studies of hydrogen sorption/desorption as a function of thickness. The SLRR cycle involved the initial formation of an atomic layer of Cu by underpotential deposition, followed by its galvanic exchange with PdCl42- ions at open circuit. The first three cycles were studied using in situ electrochemical scanning tunneling microscopy (EC-STM), which showed a consistent morphology from cycle to cycle and the monatomic steps indicative of layer-by-layer growth. Cyclic voltammetry was used to study the hydrogen sorption/desorption properties as a function of thickness in 0.1 M H2SO4. The results indicated that the underlying Au structure greatly influenced hydrogen adsorption, as did film thickness for deposits formed with fewer than five cycles. No hydrogen absorption occurred for the thinnest films, although it increased linearly for thicker films, producing an average H/Pd molar ratio of 0.6. Electrochemical annealing was shown to improve surface order, producing CVs that strongly resembled those characteristic of bulk Pd(111).
C1 [Sheridan, Leah B.; Kim, Youn-Geun; Perdue, Brian R.; Jagannathan, Kaushik; Stickney, John L.] Univ Georgia, Dept Chem, Athens, GA 30602 USA.
[Robinson, David B.] Sandia Natl Labs, Energy Nanomat Dept, Livermore, CA 94550 USA.
RP Stickney, JL (reprint author), Univ Georgia, Dept Chem, Athens, GA 30602 USA.
EM Stickney@uga.edu
RI Kim, Youn-Geun/C-3461-2008
OI Kim, Youn-Geun/0000-0002-5936-6520
FU National Science Foundation, Division of Materials Research [1006747];
Laboratory Directed Research and Development program at Sandia National
Laboratories; U.S. Department of Energy's National Nuclear Security
Administration [DE-AC04-94AL85000]
FX We acknowledge the support of the National Science Foundation, Division
of Materials Research #1006747 as well as the Laboratory Directed
Research and Development program at Sandia National Laboratories, a
multiprogram laboratory managed and operated by Sandia Corporation, a
wholly owned subsidiary of Lockheed Martin Corporation, for the U.S.
Department of Energy's National Nuclear Security Administration under
contract DE-AC04-94AL85000.
NR 91
TC 5
Z9 5
U1 2
U2 60
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 1
PY 2013
VL 117
IS 30
BP 15728
EP 15740
DI 10.1021/jp404723a
PG 13
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 196WG
UT WOS:000322807500031
ER
PT J
AU Han, KS
Wang, XQ
Dai, S
Hagaman, EW
AF Han, Kee Sung
Wang, Xiqing
Dai, Sheng
Hagaman, Edward W.
TI Distribution of 1-Butyl-3-methylimidazolium
Bistrifluoromethylsulfonimide in Mesoporous Silica As a Function of Pore
Filling
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID TEMPERATURE IONIC LIQUIDS; MAGNETIC-FIELD GRADIENTS; POROUS SILICA;
DIFFUSION MEASUREMENTS; NMR DIFFUSION; TRANSLATIONAL DYNAMICS;
IMIDAZOLIUM; SPECTROSCOPY; CONFINEMENT; SUPPRESSION
AB Rotational dynamics of the ionic liquid (IL) 1-butyl-3-methylimidazolium bistrifluoromethylsulfonimide, [C(4)mim][Tf2N], 1, as a neat liquid, and confined in mesoporous silica were investigated by spin-spin (T-2) and spin-lattice (TO relaxation measurements and C-13 NMR spectroscopy. Translational dynamics (self-diffusion) were monitored via the diffusion coefficient, D, obtained with pulsed field gradient NMR measurements. These data were used to determine the distribution of 1 in the pores of KIT-6, a mesoporous silica with a bicontinuous gyroid pore structure, as a function of filling fraction. Relaxation studies performed as a function of filling factor and temperature reveal a dynamic heterogeneity in both translational and rotational motions for 1 at filling factors, f = 0.2-1.0 (f = 1 corresponds to fully filled pores). Spin-lattice and spin-spin relaxation times reveal that the motion of 1 in silica mesopores conforms to that expected for a two-dimensional relaxation model. The relaxation dynamics are interpreted using a two-state, fast exchange model for all motions; a slow rotation (and translation) of molecules in contact with the surface and a faster motion approximated by the values for bulk relaxation and diffusion. Compound 1 retains liquid-like behavior at all filling factors and temperatures that extend to ca. 50 degrees below the bulk melting point. Translational motion in these systems, interpreted with MD-simulated diffusivity limits, confirms the high propensity of 1 to form a monolayer film on the silica surface at low filling factors. The attractive interaction of 1 with the surface is greater than that for self-association of 1. The trends in diffusion data at short and long diffusion time suggest that the population of surface-bound 1 is in intimate contact with 1 in the pores. This condition is most easily met at higher filling fractions with successive additions of 1 increasing the layer thickness built up on the surface layer.
C1 [Han, Kee Sung; Wang, Xiqing; Dai, Sheng; Hagaman, Edward W.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
RP Hagaman, EW (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
EM hagamanew@ornl.gov
RI Wang, Xiqing/E-3062-2010; Dai, Sheng/K-8411-2015;
OI Wang, Xiqing/0000-0002-1843-008X; Dai, Sheng/0000-0002-8046-3931; Han,
Kee Sung/0000-0002-3535-1818
FU Fluid Interface Reactions, Structures, and Transport (FIRST) Center;
U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences; Energy Frontier Research Center
FX This work was supported by the Fluid Interface Reactions, Structures,
and Transport (FIRST) Center, an Energy Frontier Research Center funded
by the U.S. Department of Energy, Office of Science, Office of Basic
Energy Sciences.
NR 45
TC 10
Z9 10
U1 2
U2 63
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 1
PY 2013
VL 117
IS 30
BP 15754
EP 15762
DI 10.1021/jp404990q
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 196WG
UT WOS:000322807500034
ER
PT J
AU Nakayasu, ES
Ansong, C
Brown, JN
Yang, F
Lopez-Ferrer, D
Qian, WJ
Smith, RD
Adkins, JN
AF Nakayasu, Ernesto S.
Ansong, Charles
Brown, Joseph N.
Yang, Feng
Lopez-Ferrer, Daniel
Qian, Wei-Jun
Smith, Richard D.
Adkins, Joshua N.
TI Evaluation of Selected Binding Domains for the Analysis of Ubiquitinated
Proteomes
SO JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY
LA English
DT Article
DE Ubiquitination; Post-translation modification; Affinity purification;
Proteomics; Mass spectrometry
ID PROTEASOMAL DEGRADATION; PROTEIN UBIQUITINATION; MASS-SPECTROMETRY; UBA
DOMAIN; POLYUBIQUITIN; IDENTIFICATION; PATHWAY; CHAINS; CELLS;
QUANTIFICATION
AB Ubiquitination is an abundant post-translational modification that consists of covalent attachment of ubiquitin to lysine residues or the N-terminus of proteins. Mono- and polyubiquitination have been shown to be involved in many critical eukaryotic cellular functions and are often disrupted by intracellular bacterial pathogens. Affinity enrichment of ubiquitinated proteins enables global analysis of this key modification. In this context, the use of ubiquitin-binding domains is a promising but relatively unexplored alternative to more broadly used immunoaffinity or tagged affinity enrichment methods. In this study, we evaluated the application of eight ubiquitin-binding domains that have differing affinities for ubiquitination states. Small-scale proteomics analysis identified similar to 200 ubiquitinated protein candidates per ubiquitin-binding domain pull-down experiment. Results from subsequent Western blot analyses that employed anti-ubiquitin or monoclonal antibodies against polyubiquitination at lysine 48 and 63 suggest that ubiquitin-binding domains from Dsk2 and ubiquilin-1 have the broadest specificity in that they captured most types of ubiquitination, whereas the binding domain from NBR1 was more selective to polyubiquitination. These data demonstrate that with optimized purification conditions, ubiquitin-binding domains can be an alternative tool for proteomic applications. This approach is especially promising for the analysis of tissues or cells resistant to transfection, of which the overexpression of tagged ubiquitin is a major hurdle.
C1 [Nakayasu, Ernesto S.; Ansong, Charles; Brown, Joseph N.; Yang, Feng; Lopez-Ferrer, Daniel; Qian, Wei-Jun; Smith, Richard D.; Adkins, Joshua N.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
[Lopez-Ferrer, Daniel] Capr Prote US LLC, Menlo Pk, CA 94025 USA.
RP Adkins, JN (reprint author), Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
EM Joshua.Adkins@pnnl.gov
RI Smith, Richard/J-3664-2012;
OI Smith, Richard/0000-0002-2381-2349; Adkins, Joshua/0000-0003-0399-0700
FU National Institute of Allergy and Infectious Diseases (NIH/DHHS)
[Y1-AI-4894-01]; National Institute for General Medical Sciences
[GM094623]; U.S. Department of Energy (DOE) Office of Biological and
Environmental Research (BER); NIH [5P41RR018522-10]; National Institute
of General Medical Sciences [8 P41 GM103493-10]; DOE by Battelle
[DE-AC05-76RLO1830]
FX The authors thank Drs. Matthew Monroe, Brooke Deatherage-Kaiser, and
Alexandra Rutledge for comments, input, and suggestions. This work was
supported by the National Institute of Allergy and Infectious Diseases
(NIH/DHHS through interagency agreement Y1-AI-4894-01; project website
www.SysBEP.org) and the National Institute for General Medical Sciences
(GM094623). Proteomics capabilities were developed under support from
the U.S. Department of Energy (DOE) Office of Biological and
Environmental Research (BER), NIH grant 5P41RR018522-10 and National
Institute of General Medical Sciences grant 8 P41 GM103493-10.
Significant portions of this work were performed using EMSL, a DOE/BER
national scientific user facility located at Pacific Northwest National
Laboratory. The Pacific Northwest National Laboratory is operated for
the DOE by Battelle under Contract DE-AC05-76RLO1830.
NR 59
TC 5
Z9 5
U1 0
U2 18
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1044-0305
EI 1879-1123
J9 J AM SOC MASS SPECTR
JI J. Am. Soc. Mass Spectrom.
PD AUG
PY 2013
VL 24
IS 8
BP 1214
EP 1223
DI 10.1007/s13361-013-0619-8
PG 10
WC Biochemical Research Methods; Chemistry, Analytical; Chemistry,
Physical; Spectroscopy
SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy
GA 184VZ
UT WOS:000321923100008
PM 23649778
ER
PT J
AU Kobayashi, R
Kaneko, K
Wakimoto, S
Chi, SX
Sanada, N
Watanuki, R
Suzuki, K
AF Kobayashi, Riki
Kaneko, Koji
Wakimoto, Shuichi
Chi, Songxue
Sanada, Naoyuki
Watanuki, Ryuta
Suzuki, Kazuya
TI Powder neutron diffraction study of HoCoGa5
SO JOURNAL OF THE KOREAN PHYSICAL SOCIETY
LA English
DT Article; Proceedings Paper
CT 19th International Conference on Magnetism (ICM)
CY JUL 08-12, 2012
CL Busan, SOUTH KOREA
DE HoCoGa5; TbCoGa5; Powder neutron diffraction; First-order transition;
Successive transitions; WAND
ID TRIANGULAR LATTICE; PHASE-TRANSITIONS; SUPERCONDUCTIVITY;
ANTIFERROMAGNETS; SCATTERING; CERHIN5; CSNICL3; CECOIN5
AB We have studied successive magnetic transitions of HoCoGa5 at T (N1) = 9.6 K and T (N2) = 7.5 K by using powder neutron diffraction. Apparent superlattice peaks were observed at temperatures below T (N1). With further decreases temperature, the patterns exhibit a substantial change at temperatures below T (N2). The observed magnetic peaks at 8 K (AntiFerromagnetic InCommensurate (AFIC) phase: T (N2) aOE (c) T < T (N1)) can be represented by the propagation vector q (L) = (1/2 0 tau) with tau = 0.35(2). In contrast, the magnetic structure becomes commensurate with q (C) = (1/2 0 1/2) at 4 K (AntiFerromagnetic Commensurate (AFC) phase: T < T (N2)). The temperature dependence of magnetic intensity shows an apparent temperature hysteresis at T (N2), indicates a first-order transition at T (N2). Analysis of the integrated intensity at 4 K reveals that the Ho moment with a size of 8.6(2) A mu(B), oriented parallel to the c-axis in the AFC phase. While the successive transitions of HoCoGa5 are different from those of TbCoGa5, the magnetic structure in the AFC phase of HoCoGa5 is the same as the AF (I) (Tb) of TbCoGa5, and may indicate an additional transition at a lower temperature in HoCoGa5.
C1 [Kobayashi, Riki; Kaneko, Koji; Wakimoto, Shuichi] Japan Atom Energy Agcy, Quantum Beam Sci Directorate, Ibaraki 3191195, Japan.
[Chi, Songxue] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA.
[Sanada, Naoyuki; Watanuki, Ryuta; Suzuki, Kazuya] Yokohama Natl Univ, Dept Adv Mat Chem, Hodogaya ku, Yokohama, Kanagawa 240, Japan.
RP Kobayashi, R (reprint author), Japan Atom Energy Agcy, Quantum Beam Sci Directorate, Ibaraki 3191195, Japan.
EM kobayashi.riki@jaea.go.jp
RI Chi, Songxue/A-6713-2013;
OI Chi, Songxue/0000-0002-3851-9153; Suzuki, Kazuya/0000-0002-2231-4225;
Watanuki, Ryuta/0000-0002-5331-923X
FU Ministry of Education, Culture, Sports, Science, and Technology, Japan
[23740247, 2454036]; Division of Scientific User Facilities, Department
of Energy (DOE) Basic Energy Sciences (BES); Japan Society for the
Promotion of Science (JSPS) for Young Scientists
FX This work was supported by a Grant-in-Aid for Young Scientists (B) (No.
23740247) and for Scientific Research (C) (No. 2454036) of The Ministry
of Education, Culture, Sports, Science, and Technology, Japan. The work
at Oak Ridge National Laboratory (ORNL) was supported by the Division of
Scientific User Facilities, Department of Energy (DOE) Basic Energy
Sciences (BES). Wide-Angle Neutron Diffractometer (WAND) is operated
jointly by ORNL and Japan Atomic Energy Agency (JAEA) under the
U.S.-Japan Cooperative Program in Neutron Scattering. One of the authors
(N.S.) acknowledges the support from the Research Fellowship of the
Japan Society for the Promotion of Science (JSPS) for Young Scientists.
NR 26
TC 2
Z9 2
U1 0
U2 13
PU KOREAN PHYSICAL SOC
PI SEOUL
PA 635-4, YUKSAM-DONG, KANGNAM-KU, SEOUL 135-703, SOUTH KOREA
SN 0374-4884
EI 1976-8524
J9 J KOREAN PHYS SOC
JI J. Korean Phys. Soc.
PD AUG
PY 2013
VL 63
IS 3
SI SI
BP 337
EP 340
DI 10.3938/jkps.63.337
PG 4
WC Physics, Multidisciplinary
SC Physics
GA 206FE
UT WOS:000323502800015
ER
PT J
AU Haga, Y
Bauer, ED
Tobash, PH
Mitchell, JN
Ayala-Valenzuela, O
McDonald, RD
Mielke, CH
Fisk, Z
AF Haga, Yoshinori
Bauer, Eric D.
Tobash, Paul H.
Mitchell, Jeremy N.
Ayala-Valenzuela, Oscar
McDonald, Ross D.
Mielke, Charles H.
Fisk, Zachary
TI Shubnikov-de Haas oscillation in PuIn3
SO JOURNAL OF THE KOREAN PHYSICAL SOCIETY
LA English
DT Article; Proceedings Paper
CT 19th International Conference on Magnetism (ICM)
CY JUL 08-12, 2012
CL Busan, SOUTH KOREA
AB The Fermi surface of PuIn3 is investigated using flux-grown single crystals. Shubnikov-de Haas (SdH) oscillations were detected by means of the skin-depth measurement using a proximity-detector-oscillator circuit. Angular dependence of the SdH frequency which corresponds to the extremal cross-sectional area of Fermi surface agrees well with the previous magnetic susceptibility measurement using conventional field-modulation method. The SdH oscillation suddenly vanishes when the magnetic field is tilted from the cubic [111] direction.
C1 [Haga, Yoshinori; Fisk, Zachary] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan.
[Bauer, Eric D.; Tobash, Paul H.; Mitchell, Jeremy N.; Ayala-Valenzuela, Oscar; McDonald, Ross D.; Mielke, Charles H.; Fisk, Zachary] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Fisk, Zachary] Univ Calif Irvine, Irvine, CA 92697 USA.
RP Haga, Y (reprint author), Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan.
EM haga.yoshinori@jaea.go.jp
RI Mitchell, Jeremy/E-2875-2010; Mielke, Charles/S-6827-2016;
OI Mitchell, Jeremy/0000-0001-7109-3505; Mielke,
Charles/0000-0002-2096-5411; Bauer, Eric/0000-0003-0017-1937; Mcdonald,
Ross/0000-0002-5819-4739
FU Ministry of Education, Culture, Sports, Science and Technology (MEXT)
[20102002, 20224015]; Japan Society of the Promotion of Science (JSPS)
FX This work was supported by a Grant-in-Aid for Scientific Research on
Innovative Areas: Heavy Electrons (No. 20102002), Scientific Research S
(No. 20224015) from the Ministry of Education, Culture, Sports, Science
and Technology (MEXT) and Japan Society of the Promotion of Science
(JSPS).
NR 5
TC 2
Z9 2
U1 2
U2 17
PU KOREAN PHYSICAL SOC
PI SEOUL
PA 635-4, YUKSAM-DONG, KANGNAM-KU, SEOUL 135-703, SOUTH KOREA
SN 0374-4884
EI 1976-8524
J9 J KOREAN PHYS SOC
JI J. Korean Phys. Soc.
PD AUG
PY 2013
VL 63
IS 3
SI SI
BP 380
EP 382
DI 10.3938/jkps.63.380
PG 3
WC Physics, Multidisciplinary
SC Physics
GA 206FE
UT WOS:000323502800026
ER
PT J
AU Bisig, A
Stark, M
Mawass, MA
Moutafis, C
Rhensius, J
Heidler, J
Buttner, F
Noske, M
Weigand, M
Eisebitt, S
Tyliszczak, T
Van Waeyenberge, B
Stoll, H
Schutz, G
Klaul, M
AF Bisig, Andre
Staerk, Martin
Mawass, Mohamad-Assaad
Moutafis, Christoforos
Rhensius, Jan
Heidler, Jakoba
Buettner, Felix
Noske, Matthias
Weigand, Markus
Eisebitt, Stefan
Tyliszczak, Tolek
Van Waeyenberge, Bartel
Stoll, Hermann
Schuetz, Gisela
Klaeul, Mathias
TI Correlation between spin structure oscillations and domain wall
velocities
SO NATURE COMMUNICATIONS
LA English
DT Article
ID MAGNETIC-FIELDS; MOTION; NANOWIRES; DYNAMICS; STATE
AB Magnetic sensing and logic devices based on the motion of magnetic domain walls rely on the precise and deterministic control of the position and the velocity of individual magnetic domain walls in curved nanowires. Varying domain wall velocities have been predicted to result from intrinsic effects such as oscillating domain wall spin structure transformations and extrinsic pinning due to imperfections. Here we use direct dynamic imaging of the nanoscale spin structure that allows us for the first time to directly check these predictions. We find a new regime of oscillating domain wall motion even below the Walker breakdown correlated with periodic spin structure changes. We show that the extrinsic pinning from imperfections in the nanowire only affects slow domain walls and we identify the magneto-static energy, which scales with the domain wall velocity, as the energy reservoir for the domain wall to overcome the local pinning potential landscape.
C1 [Bisig, Andre; Staerk, Martin; Moutafis, Christoforos; Rhensius, Jan; Heidler, Jakoba; Klaeul, Mathias] Univ Konstanz, Dept Phys, D-78457 Constance, Germany.
[Bisig, Andre; Mawass, Mohamad-Assaad; Noske, Matthias; Weigand, Markus; Stoll, Hermann; Schuetz, Gisela] Max Planck Inst Intelligent Syst, D-70569 Stuttgart, Germany.
[Bisig, Andre; Staerk, Martin; Moutafis, Christoforos; Heidler, Jakoba; Buettner, Felix; Klaeul, Mathias] Paul Scherrer Inst, SwissFEL, CH-5232 Villigen, Switzerland.
[Bisig, Andre; Staerk, Martin; Moutafis, Christoforos; Heidler, Jakoba; Buettner, Felix; Klaeul, Mathias] Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland.
[Bisig, Andre; Mawass, Mohamad-Assaad; Heidler, Jakoba; Buettner, Felix; Klaeul, Mathias] Johannes Gutenberg Univ Mainz, Inst Phys, D-55128 Mainz, Germany.
[Moutafis, Christoforos] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.
[Rhensius, Jan; Heidler, Jakoba] Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.
[Buettner, Felix; Eisebitt, Stefan] Tech Univ Berlin, Inst Opt & Atom Phys, D-10623 Berlin, Germany.
[Eisebitt, Stefan] Helmholtz Zentrum Berlin Mat & Energie GmbH, D-14109 Berlin, Germany.
[Tyliszczak, Tolek] LBNL, Adv Light Source, Berkeley, CA 94720 USA.
[Van Waeyenberge, Bartel] Univ Ghent, Dept Solid State Sci, B-9000 Ghent, Belgium.
RP Klaul, M (reprint author), Univ Konstanz, Dept Phys, Univ Str 10, D-78457 Constance, Germany.
EM Klaeui@Uni-Mainz.de
RI Buttner, Felix/J-9286-2012; Klaui, Mathias/B-6972-2009;
OI Buttner, Felix/0000-0002-6204-9948; Klaui, Mathias/0000-0002-4848-2569;
Moutafis, Christoforos/0000-0002-2006-9203
FU German Science Foundation [DFG SFB 767, KL1811, MAINZ GSC 266]; ERC
[2007-Stg 208162]; EU [RTN Spinswitch, MRTN CT-2006-035327, MAGWIRE
FP7-ICT-2009-5 257707]; COMATT; Swiss National Science Foundation;
Office of Science, Office of Basic Energy Sciences, of the US Department
of Energy [DE-AC02-05CH11231]
FX We acknowledge support by the German Science Foundation (DFG SFB 767,
KL1811, MAINZ GSC 266), the ERC (2007-Stg 208162), the EU (RTN
Spinswitch, MRTN CT-2006-035327, MAGWIRE FP7-ICT-2009-5 257707), COMATT
and the Swiss National Science Foundation. Part of this work was carried
out at the MAXYMUS scanning X-ray microscope at HZB, BESSY II in Berlin.
The Advanced Light Source is supported by the Director, Office of
Science, Office of Basic Energy Sciences, of the US Department of Energy
under Contract No. DE-AC02-05CH11231.
NR 35
TC 20
Z9 20
U1 3
U2 48
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2328
DI 10.1038/ncomms3328
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209JR
UT WOS:000323752400001
PM 23978905
ER
PT J
AU Lu, J
Lei, Y
Lau, KC
Luo, XY
Du, P
Wen, JG
Assary, RS
Das, U
Miller, DJ
Elam, JW
Albishri, HM
Abd El-Hady, D
Sun, YK
Curtiss, LA
Amine, K
AF Lu, Jun
Lei, Yu
Lau, Kah Chun
Luo, Xiangyi
Du, Peng
Wen, Jianguo
Assary, Rajeev S.
Das, Ujjal
Miller, Dean J.
Elam, Jeffrey W.
Albishri, Hassan M.
Abd El-Hady, D.
Sun, Yang-Kook
Curtiss, Larry A.
Amine, Khalil
TI A nanostructured cathode architecture for low charge overpotential in
lithium-oxygen batteries
SO NATURE COMMUNICATIONS
LA English
DT Article
ID ATOMIC LAYER DEPOSITION; RECHARGEABLE LI-O-2 BATTERIES; AIR BATTERIES;
ELECTROLYTES; NANOPARTICLES; CHALLENGES; NANOPORES; CATALYST
AB The lithium-oxygen battery, of much interest because of its very high-energy density, presents many challenges, one of which is a high-charge overpotential that results in large inefficiencies. Here we report a cathode architecture based on nanoscale components that results in a dramatic reduction in charge overpotential to similar to 0.2 V. The cathode utilizes atomic layer deposition of palladium nanoparticles on a carbon surface with an alumina coating for passivation of carbon defect sites. The low charge potential is enabled by the combination of palladium nanoparticles attached to the carbon cathode surface, a nanocrystalline form of lithium peroxide with grain boundaries, and the alumina coating preventing electrolyte decomposition on carbon. High-resolution transmission electron microscopy provides evidence for the nanocrystalline form of lithium peroxide. The new cathode material architecture provides the basis for future development of lithium-oxygen cathode materials that can be used to improve the efficiency and to extend cycle life.
C1 [Lu, Jun; Luo, Xiangyi; Du, Peng; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Lei, Yu; Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA.
[Lau, Kah Chun; Assary, Rajeev S.; Das, Ujjal; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Wen, Jianguo; Miller, Dean J.] Argonne Natl Lab, Electron Microscopy Ctr, Argonne, IL 60439 USA.
[Albishri, Hassan M.; Abd El-Hady, D.; Amine, Khalil] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah 80203, Saudi Arabia.
[Sun, Yang-Kook] Hanyang Univ, Dept Energy Engn, Seoul 133791, South Korea.
RP Sun, YK (reprint author), Hanyang Univ, Dept Energy Engn, Seoul 133791, South Korea.
EM yksun@hanyang.ac.kr; curtiss@anl.gov; amine@anl.gov
RI Amine, Khalil/K-9344-2013; Du, Peng/F-8336-2013; Lau, Kah
Chun/A-9348-2013; BM, MRCAT/G-7576-2011; Luo, Xiangyi/N-4709-2014; Luo,
Xiangyi/K-6058-2015; Surendran Assary, Rajeev/E-6833-2012; Faculty of,
Sciences, KAU/E-7305-2017;
OI Lau, Kah Chun/0000-0002-4925-3397; Luo, Xiangyi/0000-0002-4817-1461;
Luo, Xiangyi/0000-0002-4817-1461; Surendran Assary,
Rajeev/0000-0002-9571-3307; Lei, Yu/0000-0002-4161-5568
FU U.S. Department of Energy [DE-AC02-06CH11357]; Vehicle Technologies
Office, Department of Energy (DOE) Office of Energy Efficiency and
Renewable Energy (EERE); Department of Energy (DOE) Office of Energy
Efficiency and Renewable Energy (EERE) Postdoctoral Research Award under
the EERE Vehicles Technology Program; Tailored Interfaces for Energy
Storage, an Energy Frontier Research Center, Office of Basic Energy
Sciences Research; Human Resources Development of the Korea Institute of
Energy Technology Evaluation and Planning (KETEP) grant; Korean
government, Ministry of Knowledge and Economy [20114010203150]; National
Research Foundation of Korea (NRF) grant; Korea government (MEST)
[2009-0092780]; INCITE award; ALCC award; U.S. Department of Energy,
Office of Basic Energy Sciences [DE-AC02-06CH11357]
FX This work was supported by the U.S. Department of Energy under Contract
DE-AC02-06CH11357 with the main support provided by the Vehicle
Technologies Office, Department of Energy (DOE) Office of Energy
Efficiency and Renewable Energy (EERE). J.Lu was supported by the
Department of Energy (DOE) Office of Energy Efficiency and Renewable
Energy (EERE) Postdoctoral Research Award under the EERE Vehicles
Technology Program administered by the Oak Ridge Institute for Science
and Education (ORISE) for the DOE. This work was also partially
supported from the Tailored Interfaces for Energy Storage, an Energy
Frontier Research Center, Office of Basic Energy Sciences Research. This
work was also supported by the Human Resources Development of the Korea
Institute of Energy Technology Evaluation and Planning (KETEP) grant
funded by the Korean government, Ministry of Knowledge and Economy (No.
20114010203150) and by the National Research Foundation of Korea (NRF)
grant funded by the Korea government (MEST; No. 2009-0092780). We
acknowledge grants of computer time through INCITE and ALCC awards for
BlueGene/P computer at Argonne National Laboratory and allocations on
the CNM Carbon Cluster at Argonne National Laboratory, the ALCF Fusion
Cluster at Argonne National Laboratory, and the EMSL Chinook Cluster at
Pacific Northwest National Laboratory. Use of the Advanced Photon Source
and the Electron Microscopy Center at Argonne National Laboratory was
supported by the U.S. Department of Energy, Office of Basic Energy
Sciences, under contract No. DE-AC02-06CH11357.
NR 41
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U1 27
U2 303
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2383
DI 10.1038/ncomms3383
PG 9
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209KG
UT WOS:000323754400001
PM 23986151
ER
PT J
AU Shui, JL
Okasinski, JS
Kenesei, P
Dobbs, HA
Zhao, D
Almer, JD
Liu, DJ
AF Shui, Jiang-Lan
Okasinski, John S.
Kenesei, Peter
Dobbs, Howard A.
Zhao, Dan
Almer, Jonathan D.
Liu, Di-Jia
TI Reversibility of anodic lithium in rechargeable lithium-oxygen batteries
SO NATURE COMMUNICATIONS
LA English
DT Article
ID LI-AIR BATTERIES; NONAQUEOUS LI-O-2 BATTERIES; ETHER-BASED ELECTROLYTES;
X-RAY; CARBONATE ELECTROLYTES; REDUCTION; CATHODE; PERFORMANCE;
ELECTRODES; CATALYST
AB Non-aqueous lithium-air batteries represent the next-generation energy storage devices with very high theoretical capacity. The benefit of lithium-air batteries is based on the assumption that the anodic lithium is completely reversible during the discharge-charge process. Here we report our investigation on the reversibility of the anodic lithium inside of an operating lithium-air battery using spatially and temporally resolved synchrotron X-ray diffraction and three-dimensional micro-tomography technique. A combined electrochemical process is found, consisting of a partial recovery of lithium metal during the charging cycle and a constant accumulation of lithium hydroxide under both charging and discharging conditions. A lithium hydroxide layer forms on the anode separating the lithium metal from the separator. However, numerous microscopic 'tunnels' are also found within the hydroxide layer that provide a pathway to connect the metallic lithium with the electrolyte, enabling sustained ion-transport and battery operation until the total consumption of lithium.
C1 [Shui, Jiang-Lan; Dobbs, Howard A.; Zhao, Dan; Liu, Di-Jia] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Okasinski, John S.; Kenesei, Peter; Almer, Jonathan D.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA.
RP Liu, DJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM djliu@anl.gov
RI Zhao, Dan/D-5975-2011
OI Zhao, Dan/0000-0002-4427-2150
FU Office of Science, U. S. Department of Energy [DE-AC02-06CH11357]; Grand
Challenge program of Argonne National Laboratory
FX This work and the use of Advanced Photon Source are supported by Office
of Science, U. S. Department of Energy under Contract DE-AC02-06CH11357.
The financial support from the Grand Challenge program of Argonne
National Laboratory is gratefully acknowledged.
NR 55
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PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2255
DI 10.1038/ncomms3255
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209JF
UT WOS:000323751100006
PM 23929396
ER
PT J
AU Sokolov, AN
Yap, FL
Liu, N
Kim, K
Ci, LJ
Johnson, OB
Wang, HL
Vosgueritchian, M
Koh, AL
Chen, JH
Park, J
Bao, ZN
AF Sokolov, Anatoliy N.
Yap, Fung Ling
Liu, Nan
Kim, Kwanpyo
Ci, Lijie
Johnson, Olasupo B.
Wang, Huiliang
Vosgueritchian, Michael
Koh, Ai Leen
Chen, Jihua
Park, Jinseong
Bao, Zhenan
TI Direct growth of aligned graphitic nanoribbons from a DNA template by
chemical vapour deposition
SO NATURE COMMUNICATIONS
LA English
DT Article
ID GRAPHENE NANORIBBONS; AMORPHOUS-CARBON; RAMAN-SPECTROSCOPY; FILMS;
FABRICATION; MOLECULES; ARRAYS; NANOLITHOGRAPHY; CONDUCTIVITY;
ADSORPTION
AB Graphene, laterally confined within narrow ribbons, exhibits a bandgap and is envisioned as a next-generation material for high-performance electronics. To take advantage of this phenomenon, there is a critical need to develop methodologies that result in graphene ribbons <10 nm in width. Here we report the use of metal salts infused within stretched DNA as catalysts to grow nanoscopic graphitic nanoribbons. The nanoribbons are termed graphitic as they have been determined to consist of regions of sp(2) and sp(3) character. The nanoscopic graphitic nanoribbons are micrometres in length, <10 nm in width, and take on the shape of the DNA template. The DNA strand is converted to a graphitic nanoribbon by utilizing chemical vapour deposition conditions. Depending on the growth conditions, metallic or semiconducting graphitic nanoribbons are formed. Improvements in the growth method have potential to lead to bottom-up synthesis of pristine single-layer graphene nanoribbons.
C1 [Sokolov, Anatoliy N.; Yap, Fung Ling; Liu, Nan; Kim, Kwanpyo; Johnson, Olasupo B.; Vosgueritchian, Michael; Bao, Zhenan] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA.
[Sokolov, Anatoliy N.] Dow Chem Co USA, Midland, MI 48640 USA.
[Yap, Fung Ling] ASTAR, IMRE, Singapore 17602, Singapore.
[Ci, Lijie; Park, Jinseong] Samsung Cheil Ind Inc, Corp Res Inst, San Jose Lab, San Jose, CA 95131 USA.
[Wang, Huiliang] Stanford Univ, Stanford, CA 94305 USA.
[Koh, Ai Leen] Stanford Univ, Stanford Nano Shared Facil, Stanford, CA 94305 USA.
[Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
RP Bao, ZN (reprint author), Stanford Univ, Dept Chem Engn, Stauffer 3,381 North South Mall, Stanford, CA 94305 USA.
EM zbao@stanford.edu
RI Kim, Kwanpyo/D-9121-2011; Wang, Huiliang/C-6949-2014; Chen,
Jihua/F-1417-2011; 慈, 立杰/E-3485-2014
OI Kim, Kwanpyo/0000-0001-8497-2330; Chen, Jihua/0000-0001-6879-5936;
FU Agency for Science, Technology and Research (A*STAR); National Science
Foundation [DMR-EPS 1006989]; Stanford Global Climate and Energy
Program; David Filo and Jerry Yang Faculty; Scientific User Facilities
Division, Office of Basic Energy Sciences, US Department of Energy
FX F.L.Y. thanks the Agency for Science, Technology and Research (A*STAR)
for her postdoctoral fellowship. Z.B. acknowledge partial support from
the National Science Foundation (DMR-EPS 1006989), the Stanford Global
Climate and Energy Program and the David Filo and Jerry Yang Faculty
Fellow. We thank M.R. Dokmeci at Northeastern University for providing
the parylene-C masks. A portion of this research was conducted at the
Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge
National Laboratory by the Scientific User Facilities Division, Office
of Basic Energy Sciences, US Department of Energy. We acknowledge
Professor Hari Manoharan, Alex Contryman, Luckshihta Suriyasena
Liyanage, Peng Wei, Steve Park, Alex Azyner, Ying Diao and Sangwon Lee
for experimental support and discussions.
NR 47
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PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2402
DI 10.1038/ncomms3402
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209KM
UT WOS:000323755000001
PM 23989553
ER
PT J
AU Wadley, P
Novak, V
Campion, RP
Rinaldi, C
Marti, X
Reichlova, H
Zelezny, J
Gazquez, J
Roldan, MA
Varela, M
Khalyavin, D
Langridge, S
Kriegner, D
Maca, F
Masek, J
Bertacco, R
Holy, V
Rushforth, AW
Edmonds, KW
Gallagher, BL
Foxon, CT
Wunderlich, J
Jungwirth, T
AF Wadley, P.
Novak, V.
Campion, R. P.
Rinaldi, C.
Marti, X.
Reichlova, H.
Zelezny, J.
Gazquez, J.
Roldan, M. A.
Varela, M.
Khalyavin, D.
Langridge, S.
Kriegner, D.
Maca, F.
Masek, J.
Bertacco, R.
Holy, V.
Rushforth, A. W.
Edmonds, K. W.
Gallagher, B. L.
Foxon, C. T.
Wunderlich, J.
Jungwirth, T.
TI Tetragonal phase of epitaxial room-temperature antiferromagnet CuMnAs
SO NATURE COMMUNICATIONS
LA English
DT Article
ID TRIPLE-CRYSTAL DIFFRACTOMETRY; MAGNETIC-PROPERTIES; NEUTRON-DIFFRACTION;
SEMICONDUCTORS; SYSTEM; LAYERS; SB
AB Recent studies have demonstrated the potential of antiferromagnets as the active component in spintronic devices. This is in contrast to their current passive role as pinning layers in hard disk read heads and magnetic memories. Here we report the epitaxial growth of a new high-temperature antiferromagnetic material, tetragonal CuMnAs, which exhibits excellent crystal quality, chemical order and compatibility with existing semiconductor technologies. We demonstrate its growth on the III-V semiconductors GaAs and GaP, and show that the structure is also lattice matched to Si. Neutron diffraction shows collinear antiferromagnetic order with a high Neel temperature. Combined with our demonstration of room-temperature-exchange coupling in a CuMnAs/Fe bilayer, we conclude that tetragonal CuMnAs films are suitable candidate materials for antiferromagnetic spintronics.
C1 [Wadley, P.; Novak, V.; Rinaldi, C.; Marti, X.; Reichlova, H.; Zelezny, J.; Wunderlich, J.; Jungwirth, T.] Inst Phys ASCR, VVI, Prague 16253 6, Czech Republic.
[Wadley, P.; Campion, R. P.; Rushforth, A. W.; Edmonds, K. W.; Gallagher, B. L.; Foxon, C. T.; Jungwirth, T.] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England.
[Rinaldi, C.; Bertacco, R.] Politecn Milan, LNESS Dipartimento Fis, I-22100 Como, Italy.
[Marti, X.; Reichlova, H.; Holy, V.] Charles Univ Prague, Fac Math & Phys, Prague 12116 2, Czech Republic.
[Marti, X.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Gazquez, J.] ICMAB CSIC, Inst Cincia Mat Barcelona, E-08193 Bellaterra, Spain.
[Roldan, M. A.; Varela, M.] Univ Compluense Madrid, Dept Fis Aplicada 3, Madrid 28040, Spain.
[Roldan, M. A.; Varela, M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
[Khalyavin, D.; Langridge, S.] Rutherford Appleton Lab, ISIS, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England.
[Kriegner, D.] Univ Linz, Inst Semicond & Solid State Phys, A-4040 Linz, Austria.
[Maca, F.; Masek, J.] Inst Phys ASCR, VVI, Prague 18221 8, Czech Republic.
[Wunderlich, J.] Hitachi Cambridge Lab, Cambridge CB3 0HE, England.
RP Wadley, P (reprint author), Inst Phys ASCR, VVI, Cukrovarnicka 10, Prague 16253 6, Czech Republic.
EM peter.wadley@nottingham.ac.uk
RI Gallagher, Bryan/B-8116-2013; Khalyavin, Dmitry/E-4335-2017; Kriegner,
Dominik/C-6225-2013; Gazquez, Jaume/C-5334-2012; Marti,
Xavier/E-1103-2014; Varela, Maria/E-2472-2014; Maca,
Frantisek/G-4467-2014; Zelezny, Jakub/G-5276-2014; Masek,
Jan/G-5813-2014; Novak, Vit/G-6844-2014; Wunderlich, Joerg/G-6918-2014;
Jungwirth, Tomas/G-8952-2014; Varela, Maria/H-2648-2012; Reichlova,
Helena/H-4629-2014; Holy, Vaclav/E-1508-2017
OI Edmonds, Kevin/0000-0002-9793-4170; Gallagher,
Bryan/0000-0001-8310-0899; Campion, Richard/0000-0001-8990-8987;
Bertacco, Riccardo/0000-0002-8109-9166; Rinaldi,
Christian/0000-0001-6930-211X; Rushforth, Andrew/0000-0001-8774-6662;
Langridge, Sean/0000-0003-1104-0772; Khalyavin,
Dmitry/0000-0002-6724-7695; Kriegner, Dominik/0000-0001-6961-6581;
Gazquez, Jaume/0000-0002-2561-328X; Marti, Xavier/0000-0003-1653-5619;
Varela, Maria/0000-0002-6582-7004; Zelezny, Jakub/0000-0001-9471-0078;
Jungwirth, Tomas/0000-0002-9910-1674; Holy, Vaclav/0000-0002-0370-6928
FU ERC [23973]; Materials Sciences and Engineering Division of the U.S.
DOE; ORNLs Shared Research Equipment (ShaRE) User Facility; Office of
BES, U.S. DOE; Spanish Ministerio de Ciencia e Innovacin Tecnolgica
[MAT2009-07967, CSD2007-00041]; Generalitat de Catalunya; Czech Science
Foundation [P204/11/P339]; Austrian Academy of Sciences (DOC-Program);
EU ERC Advanced Grant [268066]; Ministry of Education of the Czech
Republic [LM2011026]; Academy of Sciences of the Czech Republic Preamium
Academiae; Fondazione Cariplo via the project EcoMag [2010-0584];
Science and Technology Facilities Council; EPSRC [EP/K027808/1]
FX Research at UCM (M.A.R.) was supported by the ERC Starting Grant No.
23973. Research at ORNL was supported by the Materials Sciences and
Engineering Division of the U.S. DOE (M.V.) and by ORNLs Shared Research
Equipment (ShaRE) User Facility, which is sponsored by the Office of
BES, U.S. DOE. J.R. C.F. acknowledges financial support from Spanish
Ministerio de Ciencia e Innovacin Tecnolgica (Projects MAT2009-07967,
Consolider NANOSELECT CSD2007-00041) and the Generalitat de Catalunya.
X.M. acknowledges the Czech Science Foundation (Project P204/11/P339).
D.Kriegner acknowledges the support by the Austrian Academy of Sciences
(DOC-Program). T.J. and V.N acknowledge the support from EU ERC Advanced
Grant No. 268066 and from the Ministry of Education of the Czech
Republic Grants No. LM2011026, and from the Academy of Sciences of the
Czech Republic Preamium Academiae. R.B. and C.R. acknowledge financial
support from Fondazione Cariplo via the project EcoMag (Project No.
2010-0584). Experiments at the ISIS Pulsed Neutron and Muon Source were
supported by a beamtime allocation from the Science and Technology
Facilities Council. Research at the University of Nottingham was funded
by EPSRC grant EP/K027808/1.
NR 35
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PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2322
DI 10.1038/ncomms3322
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209JQ
UT WOS:000323752300007
PM 23959149
ER
PT J
AU Wang, YS
Yu, XQ
Xu, SY
Bai, JM
Xiao, RJ
Hu, YS
Li, H
Yang, XQ
Chen, LQ
Huang, XJ
AF Wang, Yuesheng
Yu, Xiqian
Xu, Shuyin
Bai, Jianming
Xiao, Ruijuan
Hu, Yong-Sheng
Li, Hong
Yang, Xiao-Qing
Chen, Liquan
Huang, Xuejie
TI A zero-strain layered metal oxide as the negative electrode for
long-life sodium-ion batteries
SO NATURE COMMUNICATIONS
LA English
DT Article
ID RECHARGEABLE NA BATTERIES; ENERGY-STORAGE; HIGH-CAPACITY; CYCLE LIFE;
LOW-COST; ELECTROCHEMICAL INTERCALATION; CATHODE MATERIAL; ANODE
MATERIALS; INSERTION; PERFORMANCE
AB Room-temperature sodium-ion batteries have shown great promise in large-scale energy storage applications for renewable energy and smart grid because of the abundant sodium resources and low cost. Although many interesting positive electrode materials with acceptable performance have been proposed, suitable negative electrode materials have not been identified and their development is quite challenging. Here we introduce a layered material, P2-Na-0.66[Li0.22Ti0.78]O-2, as the negative electrode, which exhibits only similar to 0.77% volume change during sodium insertion/extraction. The zero-strain characteristics ensure a potentially long cycle life. The electrode material also exhibits an average storage voltage of 0.75V, a practical usable capacity of ca. 100 mAh g(-1), and an apparent Na+ diffusion coefficient of 1 x 10(-10) cm(-2) s(-1) as well as the best cyclability for a negative electrode material in a half-cell reported to date. This contribution demonstrates that P2-Na-0.66 [Li0.22Ti0.78]O-2 is a promising negative electrode material for the development of rechargeable long-life sodium-ion batteries.
C1 [Wang, Yuesheng; Xu, Shuyin; Xiao, Ruijuan; Hu, Yong-Sheng; Li, Hong; Chen, Liquan; Huang, Xuejie] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing Key Lab New Energy Mat & Devices, Key Lab Renewable Energy,Inst Phys, Beijing 100190, Peoples R China.
[Yu, Xiqian; Bai, Jianming; Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
RP Hu, YS (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing Key Lab New Energy Mat & Devices, Key Lab Renewable Energy,Inst Phys, Beijing 100190, Peoples R China.
EM rjxiao@aphy.iphy.ac.cn; yshu@aphy.iphy.ac.cn
RI Li, Hong/C-4643-2008; Xiao, Ruijuan/B-4739-2010; Hu,
Yong-Sheng/H-1177-2011; Bai, Jianming/O-5005-2015; Yu,
Xiqian/B-5574-2014; wang, yuesheng/D-2631-2015
OI Li, Hong/0000-0002-8659-086X; Hu, Yong-Sheng/0000-0002-8430-6474; Yu,
Xiqian/0000-0001-8513-518X; wang, yuesheng/0000-0001-7269-9015
FU '863' Project [2011AA11A235, 2009AA03310]; '973' Projects [2009CB220104,
2010CB833102, 2012CB932900]; NSFC [51222210, 11234013]; CAS project
[KJCX2-YW-W26]; One Hundred Talent Project of the Chinese Academy of
Sciences; Office of Vehicle Technologies [DEAC02-98CH10886]; US
Department of Energy
FX We thank Professor C. Delmas for the helpful and valuable discussions on
the structure evolution during sodium insertion. This work was supported
by funding from the '863' Project (2011AA11A235, 2009AA03310), '973'
Projects (2009CB220104, 2010CB833102, 2012CB932900), NSFC (51222210,
11234013), CAS project (KJCX2-YW-W26) and One Hundred Talent Project of
the Chinese Academy of Sciences. The work at Brookhaven National
Laboratory is supported by the US Department of Energy, the Assistant
Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle
Technologies under Contract Number DEAC02-98CH10886. We also acknowledge
beamline X14A and X18A at NSLS (BNL) and Shanghai Synchrotron Radiation
Facility (SSRF) BL14B1.
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PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD AUG
PY 2013
VL 4
AR 2365
DI 10.1038/ncomms3365
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 209KB
UT WOS:000323753600001
PM 23978932
ER
PT J
AU Hanson, JD
Anderson, DT
Cianciosa, M
Franz, P
Harris, JH
Hartwell, GH
Hirshman, SP
Knowlton, SF
Lao, LL
Lazarus, EA
Marrelli, L
Maurer, DA
Schmitt, JC
Sontag, AC
Stevenson, BA
Terranova, D
AF Hanson, J. D.
Anderson, D. T.
Cianciosa, M.
Franz, P.
Harris, J. H.
Hartwell, G. H.
Hirshman, S. P.
Knowlton, S. F.
Lao, L. L.
Lazarus, E. A.
Marrelli, L.
Maurer, D. A.
Schmitt, J. C.
Sontag, A. C.
Stevenson, B. A.
Terranova, D.
TI Non-axisymmetric equilibrium reconstruction for stellarators, reversed
field pinches and tokamaks
SO NUCLEAR FUSION
LA English
DT Article
AB Axisymmetric equilibrium reconstruction using magnetohydrodynamic equilibrium solutions to the Grad-Shafranov equation has long been an important tool for interpreting tokamak experiments. This paper describes recent results in non-axisymmetric (three-dimensional) equilibrium reconstruction of nominally axisymmetric plasmas (tokamaks and reversed field pinches (RFPs)), and fully non-axisymmetric plasmas (stellarators). Results from applying the V3FIT code to CTH and HSX stellarator plasmas, RFX-mod RFP plasmas and the DIII-D tokamak are presented.
C1 [Hanson, J. D.; Cianciosa, M.; Hartwell, G. H.; Knowlton, S. F.; Maurer, D. A.; Stevenson, B. A.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA.
[Anderson, D. T.] Univ Wisconsin, Dept Elect & Comp Engn, Madison, WI 53706 USA.
[Franz, P.; Marrelli, L.; Terranova, D.] EURATOM ENEA Assoc, Consorzio RFX, Padua, Italy.
[Harris, J. H.; Hirshman, S. P.; Lazarus, E. A.; Sontag, A. C.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Lao, L. L.] Gen Atom, San Diego, CA USA.
[Schmitt, J. C.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Hanson, JD (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA.
EM jdhanson@auburn.edu
RI Marrelli, Lionello/G-4451-2013
OI Marrelli, Lionello/0000-0001-5370-080X
FU U.S. DOE [DE-AC05-00OR22725, DE-FC02-04ER54698, DE-FG02-95ER54309]; UT
Battelle, LLC; European Communities
FX This work was supported by: the U.S. DOE under Contract
DE-AC05-00OR22725 with UT Battelle, LLC; U.S. DOE under Grant
DE-FC02-04ER54698 and Contract DE-FG02-95ER54309; U.S. DOE under other
contracts and grants; and the European Communities under contract of
Association between Euratom/ENEA. The views and opinions expressed
herein do not necessarily reflect those of the European Commission or
the U.S. DOE.
NR 11
TC 10
Z9 10
U1 0
U2 16
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083016
DI 10.1088/0029-5515/53/8/083016
PG 5
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000018
ER
PT J
AU Holland, C
Kinsey, JE
DeBoo, JC
Burrell, KH
Luce, TC
Smith, SP
Petty, CC
White, AE
Rhodes, TL
Schmitz, L
Doyle, EJ
Hillesheim, JC
McKee, GR
Yan, Z
Wang, G
Zeng, L
Grierson, BA
Marinoni, A
Mantica, P
Snyder, PB
Waltz, RE
Staebler, GM
Candy, J
AF Holland, C.
Kinsey, J. E.
DeBoo, J. C.
Burrell, K. H.
Luce, T. C.
Smith, S. P.
Petty, C. C.
White, A. E.
Rhodes, T. L.
Schmitz, L.
Doyle, E. J.
Hillesheim, J. C.
McKee, G. R.
Yan, Z.
Wang, G.
Zeng, L.
Grierson, B. A.
Marinoni, A.
Mantica, P.
Snyder, P. B.
Waltz, R. E.
Staebler, G. M.
Candy, J.
TI Validation studies of gyrofluid and gyrokinetic predictions of transport
and turbulence stiffness using the DIII-D tokamak
SO NUCLEAR FUSION
LA English
DT Article
AB A series of carefully designed validation experiments conducted on DIII-D to rigorously test gyrofluid and gyrokinetic predictions of transport and turbulence stiffness in both the ion and electron channels have provided an improved assessment of the experimental fidelity of those models over a range of plasma parameters. The first set of experiments conducted was designed to test predictions of H-mode core transport stiffness at fixed pedestal density and temperature. In low triangularity lower single null plasmas, a factor of 3 variation in neutral beam injection (NBI) heating was obtained, with modest changes to pedestal conditions that slowly increased with applied heating. The measurements and trends with increased NBI heating at both low and high injected torque are generally well-reproduced by the quasilinear trapped gyro-Landau fluid (TGLF) transport model at the lowest heating levels, but with decreasing fidelity (particularly in the electron profiles) as the heating power is increased. Complementing these global stiffness studies, a second set of experiments was performed to quantify the relationship between the local electron energy flux Q(e) and electron temperature gradient by varying the deposition profile of electron cyclotron heating about a specified reference radius in low density, low current L-mode plasmas. Modelling of these experiments using both the TGLF model and the nonlinear gyrokinetic GYRO code yields systematic underpredictions of the measured fluxes and fluctuation levels.
C1 [Holland, C.] Univ Calif San Diego, Energy Res Ctr, La Jolla, CA 92093 USA.
[Kinsey, J. E.; DeBoo, J. C.; Burrell, K. H.; Luce, T. C.; Smith, S. P.; Petty, C. C.; Snyder, P. B.; Waltz, R. E.; Staebler, G. M.; Candy, J.] Gen Atom Co, San Diego, CA 92186 USA.
[White, A. E.; Marinoni, A.] MIT, Cambridge, MA 02139 USA.
[Rhodes, T. L.; Schmitz, L.; Doyle, E. J.; Wang, G.; Zeng, L.] Univ Calif Los Angeles, Dept Phys, Los Angeles, CA 90095 USA.
[Rhodes, T. L.; Schmitz, L.; Doyle, E. J.; Wang, G.; Zeng, L.] Univ Calif Los Angeles, PSTI, Los Angeles, CA 90095 USA.
[Hillesheim, J. C.] Culham Sci Ctr, EURATOM CCFE Fus Assoc, Abingdon OX14 3DB, Oxon, England.
[McKee, G. R.; Yan, Z.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA.
[Grierson, B. A.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Mantica, P.] Assoc Euratom ENEA CNR, Ist Fis Plasma P Caldirola, Milan, Italy.
RP Holland, C (reprint author), Univ Calif San Diego, Energy Res Ctr, 9500 Gilman Dr, La Jolla, CA 92093 USA.
RI Mantica, Paola/K-3033-2012
FU US Department of Energy [DE-FG02-07ER54917, DE-FG02-06ER54871,
DE-FC02-04ER54698, DE-FC02-99ER54512, DE-FG02-08ER54984,
DE-FG02-89ER53296, DE-FG020-8ER54999]; Office of Science of the
Department of Energy [DE-AC05-00OR22725]; Office of Science of the US
Department of Energy [DE-AC02-05CH11231]
FX This work was supported by the US Department of Energy under
DE-FG02-07ER54917, DE-FG02-06ER54871, DE-FC02-04ER54698,
DE-FC02-99ER54512, DE-FG02-08ER54984, DE-FG02-89ER53296 and
DE-FG020-8ER54999. The authors wish to thank E. Bass, D. Pace, M. Van
Zeeland and W.W. Heidbrink for useful discussions of energetic particle
physics. The numerical simulations were performed as part of the
research program of the Center for the Simulation of Plasma
Microturbulence. This research used resources at the National Center for
Computational Sciences at Oak Ridge National Laboratory, which is
supported by the Office of Science of the Department of Energy under
Contract DE-AC05-00OR22725. Additional simulations were performed which
used resources of the National Energy Research Scientific Computing
Center, which is supported by the Office of Science of the US Department
of Energy under Contract No DE-AC02-05CH11231.
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PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
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JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083027
DI 10.1088/0029-5515/53/8/083027
PG 11
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000029
ER
PT J
AU Hollmann, EM
Austin, ME
Boedo, JA
Brooks, NH
Commaux, N
Eidietis, NW
Humphreys, DA
Izzo, VA
James, AN
Jernigan, TC
Loarte, A
Martin-Solis, J
Moyer, RA
Munoz-Burgos, JM
Parks, PB
Rudakov, DL
Strait, EJ
Tsui, C
Van Zeeland, MA
Wesley, JC
Yu, JH
AF Hollmann, E. M.
Austin, M. E.
Boedo, J. A.
Brooks, N. H.
Commaux, N.
Eidietis, N. W.
Humphreys, D. A.
Izzo, V. A.
James, A. N.
Jernigan, T. C.
Loarte, A.
Martin-Solis, J.
Moyer, R. A.
Munoz-Burgos, J. M.
Parks, P. B.
Rudakov, D. L.
Strait, E. J.
Tsui, C.
Van Zeeland, M. A.
Wesley, J. C.
Yu, J. H.
TI Control and dissipation of runaway electron beams created during rapid
shutdown experiments in DIII-D
SO NUCLEAR FUSION
LA English
DT Article
ID TOKAMAK; AVALANCHE; SPECTRA
AB DIII-D experiments on rapid shutdown runaway electron (RE) beams have improved the understanding of the processes involved in RE beam control and dissipation. Improvements in RE beam feedback control have enabled stable confinement of RE beams out to the volt-second limit of the ohmic coil, as well as enabling a ramp down to zero current. Spectroscopic studies of the RE beam have shown that neutrals tend to be excluded from the RE beam centre. Measurements of the RE energy distribution function indicate a broad distribution with mean energy of order several MeV and peak energies of order 30-40 MeV. The distribution function appears more skewed towards low energies than expected from avalanche theory. The RE pitch angle appears fairly directed (theta similar to 0.2) at high energies and more isotropic at lower energies (epsilon < 100 keV). Collisional dissipation of RE beam current has been studied by massive gas injection of different impurities into RE beams; the equilibrium assimilation of these injected impurities appears to be reasonably well described by radial pressure balance between neutrals and ions. RE current dissipation following massive impurity injection is shown to be more rapid than expected from avalanche theory-this anomalous dissipation may be linked to enhanced radial diffusion caused by the significant quantity of high-Z impurities (typically argon) in the plasma. The final loss of RE beams to the wall has been studied: it was found that conversion of magnetic to kinetic energy is small for RE loss times smaller than the background plasma ohmic decay time of order 1-2 ms.
C1 [Hollmann, E. M.; Boedo, J. A.; Izzo, V. A.; Rudakov, D. L.; Yu, J. H.] Univ Calif San Diego, La Jolla, CA 92093 USA.
[Austin, M. E.] Univ Texas Austin, Inst Fus Studies, Austin, TX 78712 USA.
[Brooks, N. H.; Eidietis, N. W.; Humphreys, D. A.; Parks, P. B.; Strait, E. J.; Van Zeeland, M. A.; Wesley, J. C.] Gen Atom, San Diego, CA 92186 USA.
[Commaux, N.; Jernigan, T. C.] Oak Ridge Natl Lab, Oak Ridge, TX 37831 USA.
[James, A. N.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Loarte, A.] ITER Org, F-13115 St Paul Les Durance, France.
[Martin-Solis, J.] Univ Carlos III Madrid, Madrid, Spain.
[Munoz-Burgos, J. M.] Oak Ridge Associated Univ, Oak Ridge, TN 37830 USA.
[Tsui, C.] Univ Toronto, Inst Aerosp Studies, Toronto M3H 5T6, ON, Canada.
RP Hollmann, EM (reprint author), Univ Calif San Diego, 9500 Gilman Dr, La Jolla, CA 92093 USA.
FU US Department of Energy [DE-FG02-07ER54917, DE-FG03-97ER54415,
DE-FC02-04ER54698, DE-AC05-00OR22725, DE-AC52-07NS27344,
DE-AC05-06OR23100]
FX This work was supported in part by the US Department of Energy under
DE-FG02-07ER54917, DE-FG03-97ER54415, DE-FC02-04ER54698,
DE-AC05-00OR22725, DE-AC52-07NS27344 and DE-AC05-06OR23100. Suggestions
from R. Goldston are acknowledged.
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PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083004
DI 10.1088/0029-5515/53/8/083004
PG 15
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000006
ER
PT J
AU Jaworski, MA
Abrams, T
Allain, JP
Bell, MG
Bell, RE
Diallo, A
Gray, TK
Gerhardt, SP
Kaita, R
Kugel, HW
LeBlanc, BP
Maingi, R
McLean, AG
Menard, J
Nygren, R
Ono, M
Podesta, M
Roquemore, AL
Sabbagh, SA
Scotti, F
Skinner, CH
Soukhanovskii, VA
Stotler, DP
AF Jaworski, M. A.
Abrams, T.
Allain, J. P.
Bell, M. G.
Bell, R. E.
Diallo, A.
Gray, T. K.
Gerhardt, S. P.
Kaita, R.
Kugel, H. W.
LeBlanc, B. P.
Maingi, R.
McLean, A. G.
Menard, J.
Nygren, R.
Ono, M.
Podesta, M.
Roquemore, A. L.
Sabbagh, S. A.
Scotti, F.
Skinner, C. H.
Soukhanovskii, V. A.
Stotler, D. P.
CA NSTX Team
TI Liquid lithium divertor characteristics and plasma-material interactions
in NSTX high-performance plasmas
SO NUCLEAR FUSION
LA English
DT Article
ID OPERATION; LIMITER; SURFACE
AB Liquid metal plasma-facing components (PFCs) have been proposed as a means of solving several problems facing the creation of economically viable fusion power reactors. To date, few demonstrations exist of this approach in a diverted tokamak and we here provide an overview of such work on the National Spherical Torus Experiment (NSTX). The Liquid Lithium Divertor (LLD) was installed and operated for the 2010 run campaign using evaporated coatings as the filling method. The LLD consisted of a copper-backed structure with a porous molybdenum front face. Nominal Li filling levels by the end of the run campaign exceeded the porosity void fraction by 150%. Despite a nominal liquid level exceeding the capillary structure and peak current densities into the PFCs exceeding 100 kA m(-2), no macroscopic ejection events were observed. In addition, no substrate line emission was observed after achieving lithium-melt temperatures indicating the lithium wicks and provides a protective coating on the molybdenum porous layer. Impurity emission from the divertor suggests that the plasma is interacting with oxygen-contaminated lithium whether diverted on the LLD or not. A database of LLD discharges is analysed to consider whether there is a net effect on the discharges over the range of total deposited lithium in the machine. Examination of H-97L indicates that performance was constant throughout the run, consistent with the hypothesis that it is the quality of the surface layers of the lithium that impact performance. The accumulation of impurities suggests a fully flowing liquid lithium system to obtain a steady-state PFC on timescales relevant to NSTX.
C1 [Jaworski, M. A.; Abrams, T.; Bell, M. G.; Bell, R. E.; Diallo, A.; Gerhardt, S. P.; Kaita, R.; Kugel, H. W.; LeBlanc, B. P.; Menard, J.; Ono, M.; Podesta, M.; Roquemore, A. L.; Scotti, F.; Skinner, C. H.; Stotler, D. P.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Allain, J. P.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA.
[Gray, T. K.; Maingi, R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[McLean, A. G.; Soukhanovskii, V. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
[Nygren, R.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Sabbagh, S. A.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA.
RP Jaworski, MA (reprint author), Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
EM mjaworsk@pppl.gov
RI Stotler, Daren/J-9494-2015;
OI Stotler, Daren/0000-0001-5521-8718; Menard,
Jonathan/0000-0003-1292-3286; Allain, Jean Paul/0000-0003-1348-262X
FU USDOE [DE-AC02-09CH11466, DE-AC05-00OR22725, DE-AC52-07NA27344,
DE-FG02-99ER54524, DE-FG02-08ER54990, DE-AC04-94AL85000]
FX M.A.J. would like to thank R. Axford (U-Illinois) for useful discussions
on the Raleigh-Taylor analysis presented in this work. This work
supported by USDOE contracts DE-AC02-09CH11466, DE-AC05-00OR22725,
DE-AC52-07NA27344, DE-FG02-99ER54524, DE-FG02-08ER54990 and
DE-AC04-94AL85000.
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PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083032
DI 10.1088/0029-5515/53/8/083032
PG 9
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000034
ER
PT J
AU Kolesnikov, RA
Bulmer, RH
LoDestro, L
Casper, TA
Pitts, RA
AF Kolesnikov, R. A.
Bulmer, R. H.
LoDestro, L.
Casper, T. A.
Pitts, R. A.
TI Equilibrium and vertical-instability considerations for vertical
strike-point shifts on the ITER divertor targets
SO NUCLEAR FUSION
LA English
DT Article
AB The study of operation with raised strike points on the first ITER divertor target plates is motivated by the need to gain experience with operation with strike points on tungsten (W) surfaces during the non-active phases (in the case of an initial carbon fibre composite (CFC)/W divertor); or (if ITER begins with a full-W divertor), to gain experience with plasma control and transients while operating with raised strike points to avoid damaging the baseline strike regions in preparation for the nuclear phase, and to provide a means for operation should damage occur in the baseline strike zone. For operation with raised strike points, we use the Corsica code to investigate the range of possible H- and L-mode equilibria, with emphasis on the maximum plasma current, achievable shapes, etc. With raised strike points the maximum achievable plasma current is close to 14 MA. The operating space (beta(p) - l(i)) for raised strike points has been studied. The size of the beta(p) - l(i) operating space shrinks (compared to using standard strike-point positions) at 14 MA. For 12 MA, however, the operating space is not affected when using raised strike points. For equilibria with elevated strike points (at roughly the CFC/W transitions, following the 2007 ITER Design Review) the vertical-instability growth-rates at high plasma current (14 MA) are somewhat high but are within the 20s(-1) which studies indicate are controllable in ITER. At lower currents (12 MA) in H-mode, the vertical-instability growth rates stay below 10.0s(-1) for most of beta(p) - l(i) space. At 12 MA in H-mode, multiple equilibria which meet our constraints have been found in overlapping regions of the beta(p) - l(i) operating space.
C1 [Kolesnikov, R. A.; Bulmer, R. H.; LoDestro, L.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Casper, T. A.; Pitts, R. A.] ITER Org, Cadarache, France.
RP Kolesnikov, RA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA USA.
FU US Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]
FX This work was performed under the auspices of the US Department of
Energy by Lawrence Livermore National Laboratory under Contract
DE-AC52-07NA27344.
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SN 0029-5515
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JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083021
DI 10.1088/0029-5515/53/8/083021
PG 11
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000023
ER
PT J
AU Lanctot, MJ
Buttery, RJ
de Grassie, JS
Evans, TE
Ferraro, NM
Hanson, JM
Haskey, SR
Moyer, RA
Nazikian, R
Osborne, TH
Orlov, DM
Snyder, PB
Wade, MR
AF Lanctot, M. J.
Buttery, R. J.
de Grassie, J. S.
Evans, T. E.
Ferraro, N. M.
Hanson, J. M.
Haskey, S. R.
Moyer, R. A.
Nazikian, R.
Osborne, T. H.
Orlov, D. M.
Snyder, P. B.
Wade, M. R.
CA DIII-D Team
TI Sustained suppression of type-I edge-localized modes with dominantly n=2
magnetic fields in DIII-D
SO NUCLEAR FUSION
LA English
DT Article
ID FEEDBACK STABILIZATION; COLLISIONALITY REGIME; D TOKAMAK; TRANSPORT;
STABILITY; ITER
AB Type-I edge-localized modes (ELMs) have been suppressed in DIII-D (Luxon et al 2003 Nucl. Fusion 43 1813) H-mode discharges with a H-98Y2 confinement factor near 1.0 using magnetic perturbations (MPs) with dominant toroidal mode number n = 2. This expands access to the ELM-suppressed regime, which was previously attainable in DIII-D only with n = 3 fields. ELM suppression is obtained with two rows of internal coils for 1.8 s with normalized beta of 1.9 and average triangularity of 0.53, corresponding to a scaled version of ITER scenario 2 at an ITER relevant electron collisionality of 0.2. The applied field reduces the pedestal pressure and edge current via the density without degrading the edge thermal transport barrier. ELITE calculations find that the resulting profiles are stable to intermediate-n peeling-ballooning modes. ELM suppression is found within different ranges of q(95) depending on the coil configuration used to generate the MP. The edge safety factors associated with suppression do not correspond to those that maximize the pitch-resonant components of the applied vacuum field. Instead, ELM suppression is correlated with an increase in the amplification of kink-resonant components of the calculated ideal MHD plasma response field.
C1 [Lanctot, M. J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Lanctot, M. J.; Buttery, R. J.; de Grassie, J. S.; Evans, T. E.; Ferraro, N. M.; Osborne, T. H.; Snyder, P. B.; Wade, M. R.] Gen Atom Co, San Diego, CA 92186 USA.
[Hanson, J. M.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA.
[Haskey, S. R.] Australian Natl Univ, Res Sch Phys Sci & Engn, Plasma Res Lab, Canberra, ACT 0200, Australia.
[Moyer, R. A.; Orlov, D. M.] Univ Calif San Diego, Energy Res Ctr, La Jolla, CA 92093 USA.
[Nazikian, R.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Lanctot, MJ (reprint author), Gen Atom Co, POB 85608, San Diego, CA 92186 USA.
RI Haskey, Shaun/M-1469-2015; Orlov, Dmitriy/D-2406-2016; Lanctot, Matthew
J/O-4979-2016;
OI Haskey, Shaun/0000-0002-9978-6597; Orlov, Dmitriy/0000-0002-2230-457X;
Lanctot, Matthew J/0000-0002-7396-3372; Ferraro,
Nathaniel/0000-0002-6348-7827
FU US Department of Energy [DE-AC52-07NA27344, DE-FC02-04ER54698,
DE-FG02-04ER54761, DE-FG02-07ER54917]; AINSE; ANSTO
FX This work was supported by the US Department of Energy under
DE-AC52-07NA27344, DE-FC02-04ER54698, DE-FG02-04ER54761, and
DE-FG02-07ER54917. S.H. was supported by AINSE and ANSTO. The authors
acknowledge valuable comments and suggestions from E.J. Strait, I.
Joseph, F.L. Waelbroeck and J.D. Callen.
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JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083019
DI 10.1088/0029-5515/53/8/083019
PG 9
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000021
ER
PT J
AU Litaudon, X
Bernard, JM
Colas, L
Dumont, R
Argouarch, A
Bottollier-Curtet, H
Bremond, S
Champeaux, S
Corre, Y
Dumortier, P
Firdaouss, M
Guilhem, D
Gunn, JP
Gouard, P
Hoang, GT
Jacquot, J
Klepper, CC
Kubic, M
Kyrytsya, V
Lombard, G
Milanesio, D
Messiaen, A
Mollard, P
Meyer, O
Zarzoso, D
AF Litaudon, X.
Bernard, J. M.
Colas, L.
Dumont, R.
Argouarch, A.
Bottollier-Curtet, H.
Bremond, S.
Champeaux, S.
Corre, Y.
Dumortier, P.
Firdaouss, M.
Guilhem, D.
Gunn, J. P.
Gouard, Ph.
Hoang, G. T.
Jacquot, J.
Klepper, C. C.
Kubic, M.
Kyrytsya, V.
Lombard, G.
Milanesio, D.
Messiaen, A.
Mollard, P.
Meyer, O.
Zarzoso, D.
TI Physics and technology in the ion-cyclotron range of frequency on Tore
Supra and TITAN test facility: implication for ITER
SO NUCLEAR FUSION
LA English
DT Article
ID WAVE CURRENT DRIVE; FARADAY SHIELD; ICRF ANTENNAS; DIII-D; JET;
PERFORMANCE; SHEATHS; TOKAMAK; SIMULATION; PLASMAS
AB To support the design of an ITER ion-cyclotron range of frequency heating (ICRH) system and to mitigate risks of operation in ITER, CEA has initiated an ambitious Research & Development program accompanied by experiments on Tore Supra or test-bed facility together with a significant modelling effort. The paper summarizes the recent results in the following areas:
Comprehensive characterization (experiments and modelling) of a new Faraday screen concept tested on the Tore Supra antenna. A new model is developed for calculating the ICRH sheath rectification at the antenna vicinity. The model is applied to calculate the local heat flux on Tore Supra and ITER ICRH antennas.
Full-wave modelling of ITER ICRH heating and current drive scenarios with the EVE code. With 20 MW of power, a current of +/- 400 kA could be driven on axis in the DT scenario. Comparison between DT and DT(He-3) scenario is given for heating and current drive efficiencies.
First operation of CW test-bed facility, TITAN, designed for ITER ICRH components testing and could host up to a quarter of an ITER antenna.
R&D of high permittivity materials to improve load of test facilities to better simulate ITER plasma antenna loading conditions.
C1 [Litaudon, X.; Bernard, J. M.; Colas, L.; Dumont, R.; Argouarch, A.; Bottollier-Curtet, H.; Bremond, S.; Corre, Y.; Firdaouss, M.; Guilhem, D.; Gunn, J. P.; Hoang, G. T.; Jacquot, J.; Kubic, M.; Lombard, G.; Mollard, P.; Meyer, O.; Zarzoso, D.] CEA, IRFM, F-13108 St Paul Les Durance, France.
[Champeaux, S.] CEA, DAM, DIF, F-91297 Arpajon, France.
[Dumortier, P.; Kyrytsya, V.; Messiaen, A.] Royal Mil Acad, TEC, Assoc EURATOM Belgian State, Brussels, Belgium.
[Klepper, C. C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Milanesio, D.] Politecn Torino, Dept Elect, Turin, Italy.
RP Litaudon, X (reprint author), CEA, IRFM, F-13108 St Paul Les Durance, France.
EM xavier.litaudon@cea.fr
FU European Communities; French government
FX Part of this work, supported by the European Communities under the
contract of Association between EURATOM and CEA, was carried out within
the framework of the European Fusion Development Agreement. The views
and opinions expressed herein do not necessarily reflect those of the
European Commission. The new test stand facility, TITAN, was supported
within the framework of the French government stimulus plan 2010.
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PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083012
DI 10.1088/0029-5515/53/8/083012
PG 11
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000014
ER
PT J
AU Park, YS
Sabbagh, SA
Bialek, JM
Berkery, JW
Lee, SG
Ko, WH
Bak, JG
Jeon, YM
Park, JK
Kim, J
Hahn, SH
Ahn, JW
Yoon, SW
Lee, KD
Choi, MJ
Yun, GS
Park, HK
You, KI
Bae, YS
Oh, YK
Kim, WC
Kwak, JG
AF Park, Y. S.
Sabbagh, S. A.
Bialek, J. M.
Berkery, J. W.
Lee, S. G.
Ko, W. H.
Bak, J. G.
Jeon, Y. M.
Park, J. K.
Kim, J.
Hahn, S. H.
Ahn, J. -W.
Yoon, S. W.
Lee, K. D.
Choi, M. J.
Yun, G. S.
Park, H. K.
You, K. -I.
Bae, Y. S.
Oh, Y. K.
Kim, W. -C.
Kwak, J. G.
TI Investigation of MHD instabilities and control in KSTAR preparing for
high beta operation
SO NUCLEAR FUSION
LA English
DT Article
ID TOROIDAL-MOMENTUM DISSIPATION; DIII-D; TOKAMAK; PLASMAS; NSTX
AB Initial H-mode operation of the Korea Superconducting Tokamak Advanced Research (KSTAR) is expanded to higher normalized beta and lower plasma internal inductance moving towards design target operation. As a key supporting device for ITER, an important goal for KSTAR is to produce physics understanding of MHD instabilities at long pulse with steady-state profiles, at high normalized beta, and over a wide range of plasma rotation profiles. An advance from initial plasma operation is a significant increase in plasma stored energy and normalized beta, with W-tot = 340 kJ, beta(N) = 1.9, which is 75% of the level required to reach the computed ideal n = 1 no-wall stability limit. The internal inductance was lowered to 0.9 at sustained H-mode duration up to 5 s. In ohmically heated plasmas, the plasma current reached 1 MA with prolonged pulse length up to 12 s. Rotating MHD modes are observed in the device with perturbations having tearing rather than ideal parity. Modes with m/n = 3/2 are triggered during the H-mode phase but are relatively weak and do not substantially reduce W-tot. In contrast, 2/1 modes to date only appear when the plasma rotation profiles are lowered after H-L back-transition. Subsequent 2/1 mode locking creates a repetitive collapse of beta(N) by more than 50%. Onset behaviour suggests the 3/2 mode is close to being neoclassically unstable. A correlation between the 2/1 mode amplitude and local rotation shear from an x-ray imaging crystal spectrometer suggests that the rotation shear at the mode rational surface is stabilizing. As a method to access the ITER-relevant low plasma rotation regime, plasma rotation alteration by n = 1, 2 applied fields and associated neoclassical toroidal viscosity (NTV) induced torque is presently investigated. The net rotation profile change measured by a charge exchange recombination diagnostic with proper compensation of plasma boundary movement shows initial evidence of non-resonant rotation damping by the n = 1, 2 applied field configurations. The result addresses perspective on access to low rotation regimes for MHD instability studies applicable to ITER. Computation of active RWM control using the VALEN-3D code examines control performance using midplane locked mode detection sensors. The LM sensors are found to be strongly affected by mode and control coil-induced vessel current, and consequently lead to limited control performance theoretically.
C1 [Park, Y. S.; Sabbagh, S. A.; Bialek, J. M.; Berkery, J. W.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA.
[Lee, S. G.; Ko, W. H.; Bak, J. G.; Jeon, Y. M.; Kim, J.; Hahn, S. H.; Yoon, S. W.; Lee, K. D.; You, K. -I.; Bae, Y. S.; Oh, Y. K.; Kim, W. -C.; Kwak, J. G.] Natl Fus Res Inst, Taejon, South Korea.
[Park, J. K.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Ahn, J. -W.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Choi, M. J.; Yun, G. S.; Park, H. K.] Pohang Univ Sci & Technol, Pohang, South Korea.
RP Park, YS (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA.
EM ypark@pppl.gov
FU US Department of Energy [DE-FG02-99ER54524]
FX This research was supported by the US Department of Energy under
contract DE-FG02-99ER54524.
NR 29
TC 7
Z9 7
U1 2
U2 14
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083029
DI 10.1088/0029-5515/53/8/083029
PG 10
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000031
ER
PT J
AU Perkins, RJ
Ahn, JW
Bell, RE
Diallo, A
Gerhardt, S
Gray, TK
Green, DL
Jaeger, EF
Hosea, JC
Jaworski, MA
LeBlanc, BP
Kramer, GJ
McLean, A
Maingi, R
Phillips, CK
Podesta, M
Roquemore, L
Ryan, PM
Sabbagh, S
Scotti, F
Taylor, G
Wilson, JR
AF Perkins, R. J.
Ahn, J. -W.
Bell, R. E.
Diallo, A.
Gerhardt, S.
Gray, T. K.
Green, D. L.
Jaeger, E. F.
Hosea, J. C.
Jaworski, M. A.
LeBlanc, B. P.
Kramer, G. J.
McLean, A.
Maingi, R.
Phillips, C. K.
Podesta, M.
Roquemore, L.
Ryan, P. M.
Sabbagh, S.
Scotti, F.
Taylor, G.
Wilson, J. R.
TI Fast-wave power flow along SOL field lines in NSTX and the associated
power deposition profile across the SOL in front of the antenna
SO NUCLEAR FUSION
LA English
DT Article
ID HARMONIC FAST WAVES; SPHERICAL-TORUS-EXPERIMENT; ALCATOR C-MOD; PLASMAS;
PERFORMANCE; DIVERTOR; TOKAMAK; ARRAY; HHFW; FLUX
AB Fast-wave heating and current drive efficiencies can be reduced by a number of processes in the vicinity of the antenna and in the scrape-off layer (SOL). On NSTX from around 25% to more than 60% of the high-harmonic fast-wave power can be lost to the SOL regions, and a large part of this lost power flows along SOL magnetic field lines and is deposited in bright spirals on the divertor floor and ceiling. We show that field-line mapping matches the location of heat deposition on the lower divertor, albeit with a portion of the heat outside of the predictions. The field-line mapping can then be used to partially reconstruct the profile of lost fast-wave power at the midplane in front of the antenna, and the losses peak close to the last closed flux surface as well as the antenna. This profile suggests a radial standing-wave pattern formed by fast-wave propagation in the SOL, and this hypothesis will be tested on NSTX-U. RF codes must reproduce these results so that such codes can be used to understand this edge loss and to minimize RF heat deposition and erosion in the divertor region on ITER.
C1 [Perkins, R. J.; Bell, R. E.; Diallo, A.; Gerhardt, S.; Hosea, J. C.; Jaworski, M. A.; LeBlanc, B. P.; Kramer, G. J.; Maingi, R.; Phillips, C. K.; Podesta, M.; Roquemore, L.; Scotti, F.; Taylor, G.; Wilson, J. R.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Ahn, J. -W.; Gray, T. K.; Green, D. L.; McLean, A.; Ryan, P. M.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Jaeger, E. F.] XCEL Engn Inc, Oak Ridge, TN USA.
[Sabbagh, S.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY USA.
RP Perkins, RJ (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM rperkins@pppl.gov
OI Perkins, Rory/0000-0002-7216-0201
FU USDOE [DE-AC02-09CH11466]
FX This work is supported by USDOE Contract No DE-AC02-09CH11466.
NR 28
TC 12
Z9 12
U1 3
U2 15
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083025
DI 10.1088/0029-5515/53/8/083025
PG 8
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000027
ER
PT J
AU Ren, Y
Guttenfelder, W
Kaye, SM
Mazzucato, E
Bell, RE
Diallo, A
Domier, CW
LeBlanc, BP
Lee, KC
Podesta, M
Smith, DR
Yuh, H
AF Ren, Y.
Guttenfelder, W.
Kaye, S. M.
Mazzucato, E.
Bell, R. E.
Diallo, A.
Domier, C. W.
LeBlanc, B. P.
Lee, K. C.
Podesta, M.
Smith, D. R.
Yuh, H.
TI Electron-scale turbulence spectra and plasma thermal transport
responding to continuous E x B shear ramp-up in a spherical tokamak
SO NUCLEAR FUSION
LA English
DT Article
ID MAGNETIC SHEAR; CONFINEMENT; NSTX
AB Microturbulence is considered to be a major candidate in driving anomalous transport in fusion plasmas, and the equilibrium E x B shear generated by externally driven flow can be a powerful tool to control microturbulence in future fusion devices such as FNSF and ITER. Here we present the first observation of the change in electron-scale turbulence wavenumber spectrum (measured by a high-k scattering system) and thermal transport responding to continuous E x B shear ramp-up in an NSTX centre-stack limited and neutral beam injection-heated L-mode plasma. It is found that while linear stability analysis shows that the maximum electron temperature gradient mode linear growth rate far exceeds the observed E x B shearing rate in the measurement region of the high-k scattering system, the unstable ion temperature gradient (ITG) modes are susceptible to E x B shear stabilization. We observed that as the E x B shearing rate is continuously ramped up in the high-k measurement region, the ratio between the E x B shearing rate and maximum ITG mode growth rate continuously increases (from about 0.2 to 0.7) and the maximum power of the measured electron-scale turbulence wavenumber spectra decreases. Meanwhile, electron and ion thermal transport is also reduced in the outer half of the plasmas as long as magnetohydrodynamic activities are not important and the L-mode plasmas eventually reach H-mode-like confinement. Linear and nonlinear gyrokinetic simulations are presented to address the experimental observations.
C1 [Ren, Y.; Guttenfelder, W.; Kaye, S. M.; Mazzucato, E.; Diallo, A.; LeBlanc, B. P.; Podesta, M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Domier, C. W.; Lee, K. C.] Univ Calif Davis, Dept Elect & Comp Engn, Davis, CA 95616 USA.
[Smith, D. R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA.
[Yuh, H.] Nova Photon Inc, Princeton, NJ 08540 USA.
RP Ren, Y (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
FU US Department of Energy [DE-AC02-09CH11466, DE-FG03-95ER54295,
DE-FG03-99ER54518]
FX The author would like to thank the NSTX Team for the excellent technical
support for this work. This work was supported by the US Department of
Energy contracts No DE-AC02-09CH11466, No DE-FG03-95ER54295 and No
DE-FG03-99ER54518.
NR 21
TC 13
Z9 13
U1 0
U2 16
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083007
DI 10.1088/0029-5515/53/8/083007
PG 12
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000009
ER
PT J
AU Schmitt, JC
Talmadge, JN
Anderson, DT
AF Schmitt, J. C.
Talmadge, J. N.
Anderson, D. T.
TI Measurement of a helical Pfirsch-Schluter current with reduced magnitude
in HSX
SO NUCLEAR FUSION
LA English
DT Article
ID MAGNETIC-FIELD; STELLARATORS; PLASMAS; MOMENT
AB Measurements of the helical rotation and the reduction of the magnitude of the Pfirsch-Schluter current compared to an equivalent tokamak are reported in a device that has quasihelical symmetry. The Pfirsch-Schluter current is helical due to the lack of toroidal curvature, and is reduced in magnitude by the high effective transform. A 3D equilibrium reconstruction based on magnetic diagnostics agrees well with the profiles measured with Thomson scattering and diamagnetic flux loop measurements.
C1 [Schmitt, J. C.; Talmadge, J. N.; Anderson, D. T.] Univ Wisconsin, Dept Elect & Comp Engn, Madison, WI 53706 USA.
RP Schmitt, JC (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM jschmitt@pppl.gov
FU DOE [DE-FG02-93ER54222]
FX The authors would like to thank J.D. Hanson and S.P. Knowlton of Auburn
University for their assistance in using V3FIT. This work was supported
by DOE grant DE-FG02-93ER54222.
NR 17
TC 6
Z9 6
U1 0
U2 6
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 082001
DI 10.1088/0029-5515/53/8/082001
PG 5
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000001
ER
PT J
AU Scotti, F
Soukhanovskii, VA
Bell, RE
Gerhardt, S
Guttenfelder, W
Kaye, S
Andre, R
Diallo, A
Kaita, R
LeBlanc, BP
Podesta, M
AF Scotti, F.
Soukhanovskii, V. A.
Bell, R. E.
Gerhardt, S.
Guttenfelder, W.
Kaye, S.
Andre, R.
Diallo, A.
Kaita, R.
LeBlanc, B. P.
Podesta, M.
CA NSTX Team
TI Core transport of lithium and carbon in ELM-free discharges with lithium
wall conditioning in NSTX
SO NUCLEAR FUSION
LA English
DT Article
ID ROTATING TOKAMAK PLASMA; IMPURITY TRANSPORT; NEOCLASSICAL TRANSPORT;
ASDEX UPGRADE; Z DEPENDENCE; JET
AB Core transport of intrinsic carbon and lithium impurities is analysed in H-mode discharges in NSTX. The application of lithium coatings on graphite plasma-facing components led to high-performance H-mode discharges with edge localized mode (ELM) suppression and resulted in core carbon accumulation. Lithium ions did not accumulate and had densities less than 1% of carbon densities. Core transport codes NCLASS, NEO and MIST are used to assess the impact of lithium evaporative coatings on impurity transport. The disappearance of ELMs, due to changes in the electron pressure profiles, together with modifications in neoclassical transport, due to changes in main ion temperature and density profiles, explains the core carbon accumulation in discharges with lithium coatings. Residual anomalous transport in the pedestal region is needed to explain the experimental carbon density profile shape and evolution. The enhancement in neoclassical lithium particle diffusivities due to the high carbon concentration is partially responsible for the low lithium core concentration.
C1 [Scotti, F.; Bell, R. E.; Gerhardt, S.; Guttenfelder, W.; Kaye, S.; Andre, R.; Diallo, A.; Kaita, R.; LeBlanc, B. P.; Podesta, M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Soukhanovskii, V. A.] Lawrence Livermore Natl Lab, Livermore, CA USA.
RP Scotti, F (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM fscotti@pppl.gov
FU US DOE [DE-AC02-09CH11466, DE-AC52-07NA27344]
FX Work supported by the US DOE Contract DE-AC02-09CH11466 and
DE-AC52-07NA27344. The authors would like to thank Dr Steve Sabbagh for
EFIT calculations, Dr Rajesh Maingi, Dr Eric Meier and Dr Alessandro
Bortolon for useful discussions, Dr Emily Belli and Dr Jeff Candy for
the availability of the NEO code and useful discussions.
NR 30
TC 17
Z9 17
U1 7
U2 19
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083001
DI 10.1088/0029-5515/53/8/083001
PG 12
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000003
ER
PT J
AU Sung, C
White, AE
Howard, NT
Oi, CY
Rice, JE
Gao, C
Ennever, P
Porkolab, M
Parra, F
Mikkelsen, D
Ernst, D
Walk, J
Hughes, JW
Irby, J
Kasten, C
Hubbard, AE
Greenwald, MJ
AF Sung, C.
White, A. E.
Howard, N. T.
Oi, C. Y.
Rice, J. E.
Gao, C.
Ennever, P.
Porkolab, M.
Parra, F.
Mikkelsen, D.
Ernst, D.
Walk, J.
Hughes, J. W.
Irby, J.
Kasten, C.
Hubbard, A. E.
Greenwald, M. J.
CA Alcator C-Mod Team
TI Changes in core electron temperature fluctuations across the ohmic
energy confinement transition in Alcator C-Mod plasmas
SO NUCLEAR FUSION
LA English
DT Article
ID TOKAMAK PLASMA; TRANSPORT; TURBULENCE; DISCHARGES
AB The first measurements of long wavelength (k(y)rho(s) < 0.3) electron temperature fluctuations in Alcator C-Mod made with a new correlation electron cyclotron emission diagnostic support a long-standing hypothesis regarding the confinement transition from linear ohmic confinement (LOC) to saturated ohmic confinement (SOC). Electron temperature fluctuations decrease significantly (similar to 40%) crossing from LOC to SOC, consistent with a change from trapped electron mode (TEM) turbulence domination to ion temperature gradient (ITG) turbulence as the density is increased. Linear stability analysis performed with the GYRO code (Candy and Waltz 2003 J. Comput. Phys. 186 545) shows that TEMs are dominant for long wavelength turbulence in the LOC regime and ITG modes are dominant in the SOC regime at the radial location (rho similar to 0.8) where the changes in electron temperature fluctuations are measured. In contrast, deeper in the core (rho < 0.8), linear stability analysis indicates that ITG modes remain dominant across the LOC/SOC transition. This radial variation suggests that the robust global changes in confinement of energy and momentum occurring across the LOC/SOC transition are correlated to local changes in the dominant turbulent mode near the edge.
C1 [Sung, C.; White, A. E.; Howard, N. T.; Oi, C. Y.; Rice, J. E.; Gao, C.; Ennever, P.; Porkolab, M.; Parra, F.; Ernst, D.; Walk, J.; Hughes, J. W.; Irby, J.; Kasten, C.; Hubbard, A. E.; Greenwald, M. J.; Alcator C-Mod Team] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA.
[Mikkelsen, D.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Sung, C (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA.
RI Parra, Felix I./C-1442-2012; Ernst, Darin/A-1487-2010;
OI Parra, Felix I./0000-0001-9621-7404; Ernst, Darin/0000-0002-9577-2809;
Greenwald, Martin/0000-0002-4438-729X
FU US Department of Energy [DE-SC0006419, DE-FC02-99ER54512]
FX The authors thank S. Wolfe for EFIT analysis in C-Mod, and thank J.
Wright and T. Baker for maintaining the LOKI computer cluster, used to
perform the GYRO simulations. The authors are also very grateful to M.
L. Reinke for rotation profile and ion temperature profile analysis and
for extensive discussions of error analysis. This work is supported by
the US Department of Energy under Grant Nos DE-SC0006419 and
DE-FC02-99ER54512.
NR 36
TC 14
Z9 14
U1 1
U2 13
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0029-5515
J9 NUCL FUSION
JI Nucl. Fusion
PD AUG
PY 2013
VL 53
IS 8
AR 083010
DI 10.1088/0029-5515/53/8/083010
PG 13
WC Physics, Fluids & Plasmas
SC Physics
GA 196RS
UT WOS:000322794000012
ER
PT J
AU Cho, S
Cha, W
Park, HJ
Lee, JM
Kim, EB
Rhee, HW
Jiang, Z
Strzalka, J
Kim, H
AF Cho, Sanghyeok
Cha, Wonsuk
Park, Hyun-jun
Lee, Jung-Min
Kim, Eun-Bee
Rhee, Hee-Woo
Jiang, Zhang
Strzalka, Joseph
Kim, Hyunjung
TI Effects of siloxane nanoparticles on glass transition temperature and
crystallization in PEO-LiPF6 polymer electrolytes
SO SYNTHETIC METALS
LA English
DT Article
DE Polymer electrolyte; Polyethylene oxide; LiPF6; Siloxane nanoparticle;
X-ray diffraction
ID LITHIUM BATTERIES; ION-TRANSPORT; CONDUCTIVITY
AB We study the glass transition temperature and the crystallization in PEO-based polymer electrolytes with addition of siloxane nanoparticles of <3 nm. The PEO nanocomposite electrolytes with 39 wt% of siloxane nanoparticles show maximum conductivity enhanced by 400 times to that of pure PEO when siloxane nanoparticles were added to pure PEO with 22 wt% of LiPF6, the molar ratio for maximum conductivity. Differential scanning calorimetry and wide angle X-ray scattering results show that siloxane nanoparticles reduce the crystallization of PEO by increasing the amount of complexes of ethylene oxide (EO) and Li ions in PEO-LiPF6. In contrast to other additives, the glass transition temperature of the electrolyte is lowered with increasing concentration of siloxane nanoparticles. Enhancement of the conductivity with siloxane nanoparticles is due to the increased ion mobility and amorphous area in electrolytes. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Cho, Sanghyeok; Cha, Wonsuk; Park, Hyun-jun; Kim, Hyunjung] Sogang Univ, Dept Phys, Seoul 121742, South Korea.
[Lee, Jung-Min; Kim, Eun-Bee; Rhee, Hee-Woo] Sogang Univ, Dept Chem & Biomol Engn, Seoul 121742, South Korea.
[Jiang, Zhang; Strzalka, Joseph] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA.
RP Kim, H (reprint author), Sogang Univ, Dept Phys, Seoul 121742, South Korea.
EM hkim@sogang.ac.kr
RI Jiang, Zhang/A-3297-2012
OI Jiang, Zhang/0000-0003-3503-8909
FU National Research Foundation of Korea (NRF); Korea government (MOE)
[2011-0012251]; Korea government (MSIP) [R15-2008-006-01001-0]; Sogang
University; Fundamental R&D program for Core Technology of Materials;
MKE; US Department of Energy, Office of Basic Energy Science
[DE-AC02-06CH11357]; Pohang Accelerator Laboratory through the abroad
beamtime program of Synchrotron Radiation Facility Project under MEST
FX This work was supported by National Research Foundation of Korea (NRF)
grant funded by the Korea government (MOE, 2011-0012251 and MSIP,
R15-2008-006-01001-0), Sogang University Research Grant (2012), and
Fundamental R&D program for Core Technology of Materials funded by MKE.
Use of the Advanced Photon Source was supported by the US Department of
Energy, Office of Basic Energy Science, under Contract No.
DE-AC02-06CH11357. We also thank the support by Pohang Accelerator
Laboratory through the abroad beamtime program of Synchrotron Radiation
Facility Project under MEST.
NR 17
TC 3
Z9 3
U1 2
U2 26
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0379-6779
J9 SYNTHETIC MET
JI Synth. Met.
PD AUG 1
PY 2013
VL 177
BP 110
EP 113
DI 10.1016/j.synthmet.2013.06.020
PG 4
WC Materials Science, Multidisciplinary; Physics, Condensed Matter; Polymer
Science
SC Materials Science; Physics; Polymer Science
GA 207IR
UT WOS:000323592600013
ER
PT J
AU Piepel, GF
AF Piepel, Greg F.
TI Comment: Spurious Correlation and Other Observations on Experimental
Design for Engineering Dimensional Analysis
SO TECHNOMETRICS
LA English
DT Editorial Material
C1 Pacific NW Natl Lab, Richland, WA 99354 USA.
RP Piepel, GF (reprint author), Pacific NW Natl Lab, Richland, WA 99354 USA.
EM greg.piepel@pnnl.gov
NR 9
TC 1
Z9 1
U1 1
U2 6
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
J9 TECHNOMETRICS
JI Technometrics
PD AUG
PY 2013
VL 55
IS 3
BP 286
EP 289
DI 10.1080/00401706.2013.778792
PG 4
WC Statistics & Probability
SC Mathematics
GA 206TZ
UT WOS:000323547200006
ER
PT J
AU Burr, T
Hamada, MS
AF Burr, Tom
Hamada, Michael S.
TI Moving Neutron Source Detection in Radiation Portal Monitoring
SO TECHNOMETRICS
LA English
DT Article
DE Cumulative count; CUSUM; EWMA; Matched filter; Maximum count; Poisson;
Power; Profile monitoring
ID OCCURRING RADIOACTIVE MATERIALS; QUALITY PROFILES; CONTROL CHARTS;
PRODUCT; BORDERS
AB Radiation detection systems are deployed at U.S. borders to guard against entry of illicit radioactive material. This article uses realistic simulated data under different vehicle and illicit material scenarios to compare the performance of six detection methods for analyzing neutron count data collected as a vehicle passes through a radiation portal monitor, that is, a neutron count vehicle profile. The six methods are based on the cumulative count, the maximum count, sequential cumulative sum, sequential exponentially weighted moving average, comparison against a matched filter (MF) library, and a new estimated MF that estimates the shape of a neutron count vehicle profile.
C1 [Burr, Tom; Hamada, Michael S.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA.
RP Burr, T (reprint author), Los Alamos Natl Lab, Stat Sci Grp, POB 1663,MS F600, Los Alamos, NM 87545 USA.
EM tburr@lanl.gov; hamada@lanl.gov
FU U.S. Department of Homeland Security under DOE [DE-AC52-06NA25396]
FX We acknowledge the U.S. Department of Homeland Security for funding this
work under DOE Contract Number DE-AC52-06NA25396 for the management and
operation of Los Alamos National Laboratory. We thank Bill Woodall and
Megahed Fadel for insightful comments on an earlier version. We also
thank the editor, associate editor, and three referees for their
extensive comments that improved our article.
NR 21
TC 0
Z9 0
U1 1
U2 3
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
J9 TECHNOMETRICS
JI Technometrics
PD AUG
PY 2013
VL 55
IS 3
BP 296
EP 308
DI 10.1080/00401706.2013.775909
PG 13
WC Statistics & Probability
SC Mathematics
GA 206TZ
UT WOS:000323547200009
ER
PT J
AU Zhu, X
Do-Thanh, CL
Murdock, CR
Nelson, KM
Tian, CC
Brown, S
Mahurin, SM
Jenkins, DM
Hu, J
Zhao, B
Liu, HL
Dai, S
AF Zhu, Xiang
Chi-Linh Do-Thanh
Murdock, Christopher R.
Nelson, Kimberly M.
Tian, Chengcheng
Brown, Suree
Mahurin, Shannon M.
Jenkins, David M.
Hu, Jun
Zhao, Bin
Liu, Honglai
Dai, Sheng
TI Efficient CO2 Capture by a 3D Porous Polymer Derived from Troger's Base
SO ACS MACRO LETTERS
LA English
DT Article
ID CARBON-DIOXIDE CAPTURE; BENZIMIDAZOLE-LINKED POLYMERS; COVALENT ORGANIC
POLYMERS; TRIAZINE FRAMEWORKS; ENERGY APPLICATIONS; IONIC LIQUIDS;
SURFACE-AREA; GAS-STORAGE; SELECTIVITY; SEPARATION
AB A 3D Troger's-base-derived microporous organic polymer with a high surface area and good thermal stability was facilely synthesized from a one-pot metal-free polymerization reaction between dimethoxymethane and triaminotriptycene. The obtained material displays excellent CO2 uptake abilities as well as good adsorption selectivity for CO2 over N-2. The CO2 storage can reach up to 4.05 mmol g(-1) (17.8 wt %) and 2.57 mmol g(-1) (11.3 wt %) at 273 K and 298 K, respectively. Moreover, the high selectivity of the polymer toward CO2 over N-2 (50.6, 298 K) makes it a promising material for potential application in CO2 separation from flue gas.
C1 [Zhu, Xiang; Tian, Chengcheng; Hu, Jun; Liu, Honglai] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China.
[Zhu, Xiang; Tian, Chengcheng; Hu, Jun; Liu, Honglai] E China Univ Sci & Technol, Dept Chem, Shanghai 200237, Peoples R China.
[Zhu, Xiang; Tian, Chengcheng; Mahurin, Shannon M.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
[Chi-Linh Do-Thanh; Murdock, Christopher R.; Nelson, Kimberly M.; Brown, Suree; Jenkins, David M.; Zhao, Bin; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
RP Liu, HL (reprint author), E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China.
EM hlliu@ecust.edu.cn; dais@ornl.gov
RI Zhu, Xiang/P-6867-2014; Dai, Sheng/K-8411-2015;
OI Zhu, Xiang/0000-0002-3973-4998; Dai, Sheng/0000-0002-8046-3931;
Do-Thanh, Chi-Linh/0000-0003-2263-8331
FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of
Basic Energy Sciences, U.S. Department of Energy; National Basic
Research Program of China [2013CB733501]; National Natural Science
Foundation of China [20990224, 21176066]; 111 Project of China [B08021];
Fundamental Research Funds for the Central Universities of China
FX We are grateful to the financial support from the Division of Chemical
Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences,
U.S. Department of Energy. X.Z., C.C.T., J.H., and H.L.L. thank the
National Basic Research Program of China (2013CB733501), the National
Natural Science Foundation of China (No. 20990224, 21176066), the 111
Project of China (No. B08021), and the Fundamental Research Funds for
the Central Universities of China.
NR 39
TC 57
Z9 60
U1 9
U2 199
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 2161-1653
J9 ACS MACRO LETT
JI ACS Macro Lett.
PD AUG
PY 2013
VL 2
IS 8
BP 660
EP 663
DI 10.1021/mz4003485
PG 4
WC Polymer Science
SC Polymer Science
GA 205VE
UT WOS:000323472100006
ER
PT J
AU Maskey, S
Osti, NC
Perahia, D
Grest, GS
AF Maskey, Sabina
Osti, Naresh C.
Perahia, Dvora
Grest, Gary S.
TI Internal Correlations and Stability of Polydots, Soft Conjugated
Polymeric Nanoparticles
SO ACS MACRO LETTERS
LA English
DT Article
ID MOLECULAR-DYNAMICS; CROSS-LINKING; SCATTERING; DOTS
AB Conjugated polymers collapsed into long-lived highly luminescent nanoparticles, or polydots, have opened a new paradigm of tunable organic particles with an immense potential enhancing intracellular imaging and drug delivery. Albeit the chains are not in their equilibrium conformation and are not confined by cross-links, they remain stable over astounding long times. Using fully atomistic molecular dynamics simulations with an innovative method to controllably collapse an inherently rigid polymer, we determined for the first time the internal structure and stability of polydots made of dialkyl-para-phenylene ethynylene, immersed in water, a biological relevant medium. In contrast to natural aggregates, the aromatic rings within the polydots are uncorrelated, with little to no water in its interior. This lack of correlation explains the differences of luminescence characteristics between spontaneously aggregated conjugated polymers and polydots. Resolving the conformation and stability of these particles will enable transforming an idea to a new effective tool.
C1 [Maskey, Sabina; Osti, Naresh C.; Perahia, Dvora] Clemson Univ, Dept Chem, Clemson, SC 29634 USA.
[Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Perahia, D (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA.
EM dperahi@clemson.edu
RI Osti, Naresh/B-3413-2016
OI Osti, Naresh/0000-0002-0213-2299
FU DOE [DE-FG02-12ER46843]; U.S. Department of Energy's National Nuclear
Security Administration [DE-AC04-94AL85000]
FX The authors gratefully acknowledge financial support from DOE Grant No.
DE-FG02-12ER46843. This work was made possible by advanced computational
resources deployed and maintained by Clemson Computing and Information
Technology. This work was performed, in part, at the Center for
Integrated Nanotechnology, a U.S. Department of Energy and Office of
Basic Energy Sciences user facility. Sandia National Laboratories is a
multi-program laboratory managed and operated by Sandia Corporation, a
wholly owned subsidiary of Lockheed Martin Corporation, for the U.S.
Department of Energy's National Nuclear Security Administration under
Contract No. DE-AC04-94AL85000. We thank S. J. Plimpton, F. Pierce, and
J. McNeill for helpful discussions.
NR 21
TC 6
Z9 6
U1 1
U2 30
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 2161-1653
J9 ACS MACRO LETT
JI ACS Macro Lett.
PD AUG
PY 2013
VL 2
IS 8
BP 700
EP 704
DI 10.1021/mz400225d
PG 5
WC Polymer Science
SC Polymer Science
GA 205VE
UT WOS:000323472100013
ER
PT J
AU Ahn, SK
Pickel, DL
Kochemba, WM
Chen, JH
Uhrig, D
Hinestrosa, JP
Carrillo, JM
Shao, M
Do, C
Messman, JM
Brown, WM
Sumpter, BG
Kilbey, SM
AF Ahn, Suk-kyun
Pickel, Deanna L.
Kochemba, W. Michael
Chen, Jihua
Uhrig, David
Hinestrosa, Juan Pablo
Carrillo, Jan-Michael
Shao, Ming
Do, Changwoo
Messman, Jamie M.
Brown, W. Michael
Sumpter, Bobby G.
Kilbey, S. Michael, II
TI Poly(3-hexylthiophene) Molecular Bottlebrushes via Ring-Opening
Metathesis Polymerization: Macromolecular Architecture Enhanced
Aggregation
SO ACS MACRO LETTERS
LA English
DT Article
ID REGIOREGULAR POLY(3-HEXYLTHIOPHENE); SOLAR-CELLS; CONJUGATED POLYMERS;
GRAFT-COPOLYMERS; SIDE-CHAINS; CATALYST; BRUSHES; FUNCTIONALIZATION;
MACROMONOMERS; MORPHOLOGY
AB We report a facile synthetic strategy based on a grafting through approach to prepare well-defined molecular bottlebrushes composed of regioregular poly(3-hexylthiophene) (rr-P3HT) as the conjugated polymeric side chain. To this end, the exo-norbornenyl-functionalized P3HT macromonomer was synthesized by Kumada catalyst transfer polycondensation (KCTP) followed by postpolymerization modifications, and the resulting conjugated macromonomer was successfully polymerized by ring-opening metathesis polymerization (ROMP) in a controlled manner. The P3HT molecular bottlebrushes display an unprecedented strong physical aggregation upon drying during recovery, as verified by several analyses of the solution and solid states. This remarkably strong aggregation behavior is attributed to a significant enhancement in the number of pi-pi interactions between grafted P3HT side chains, brought about due to the bottlebrush architecture. This behavior is qualitatively supported by coarse-grained molecular dynamics simulations.
C1 [Ahn, Suk-kyun; Pickel, Deanna L.; Chen, Jihua; Uhrig, David; Hinestrosa, Juan Pablo; Shao, Ming; Messman, Jamie M.; Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Carrillo, Jan-Michael; Brown, W. Michael] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA.
[Do, Changwoo] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.
[Sumpter, Bobby G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.
[Kochemba, W. Michael; Kilbey, S. Michael, II] Univ Tennessee, Dept Chem & Chem & Biomol Engn, Knoxville, TN 37996 USA.
RP Pickel, DL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM deannapickel@gmail.com; mkilbey@utk.edu
RI Chen, Jihua/F-1417-2011; Carrillo, Jan-Michael/K-7170-2013; Sumpter,
Bobby/C-9459-2013; Uhrig, David/A-7458-2016; Do, Changwoo/A-9670-2011
OI Chen, Jihua/0000-0001-6879-5936; Carrillo,
Jan-Michael/0000-0001-8774-697X; Sumpter, Bobby/0000-0001-6341-0355;
Uhrig, David/0000-0001-8447-6708; Do, Changwoo/0000-0001-8358-8417
FU Division of Scientific User Facilities, U.S. Department of Energy;
TN-SCORE; NSF EPSCOR [EPS-1004083]
FX This research was conducted at the Center for Nanophase Materials
Sciences (CNMS) and the Leadership Computing Facility (OLCF), which are
sponsored at Oak Ridge National Laboratory (ORNL) by the Division of
Scientific User Facilities, U.S. Department of Energy, managed by
UT-Battelle, LLC. S.-K.A. acknowledges fruitful discussions with Prof.
B. Boudouris and Prof. J. Mays, Drs. K. Hong, B. Lokitz, R Kumar, and J.
Keum. W.M.K. and S.M.K. acknowledge support from TN-SCORE which is
sponsored by NSF EPSCOR (EPS-1004083).
NR 34
TC 15
Z9 15
U1 2
U2 76
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 2161-1653
J9 ACS MACRO LETT
JI ACS Macro Lett.
PD AUG
PY 2013
VL 2
IS 8
BP 761
EP 765
DI 10.1021/mz4003563
PG 5
WC Polymer Science
SC Polymer Science
GA 205VE
UT WOS:000323472100026
ER
PT J
AU Huh, JH
Kittleson, JT
Arkin, AP
Anderson, JC
AF Huh, Jin H.
Kittleson, Josh T.
Arkin, Adam P.
Anderson, J. Christopher
TI Modular Design of a Synthetic Payload Delivery Device
SO ACS SYNTHETIC BIOLOGY
LA English
DT Article
DE synthetic biology; system level engineering modular design; payload
delivery; tumor-killing bacterium
ID LISTERIA-MONOCYTOGENES; ESCHERICHIA-COLI; INTRACELLULAR BACTERIA;
EPITHELIAL-CELLS; MAMMALIAN-CELLS; GENE-TRANSFER; BIOLOGY; THERAPY;
PROTEIN; SEQUENCE
AB Predictable engineering of complex biological behaviors using characterized molecular functions remains a key challenge in synthetic biology. To explore the process of engineering biological behaviors, we applied a modular design strategy to the development of E. coli that deliver macromolecules to the cytoplasm of cancer cells in vitro. First, we specified five abstract, qualitative behaviors that would act in concert to achieve payload delivery. Drawing from disparate sources of previously described genetic components, we then designed, constructed, and tested individual genetic circuits to implement each module. Subsequent coupling of the modules and system optimization, aided by quantitative predictions, generated a system that delivers proteins to 80% of targeted cancer cells. Development of an effective delivery system provides strong evidence that advanced cellular behaviors, not just transcriptional circuits, can be rationally decomposed into a series of functional genetic modules and then constructed to achieve the target activity with the existing synthetic biology toolkit.
C1 [Huh, Jin H.; Kittleson, Josh T.; Arkin, Adam P.; Anderson, J. Christopher] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.
[Arkin, Adam P.; Anderson, J. Christopher] Univ Calif Berkeley, Calif Inst Quantitat Biol Res QB3, Berkeley, CA 94720 USA.
[Huh, Jin H.; Kittleson, Josh T.; Arkin, Adam P.; Anderson, J. Christopher] Synthet Biol Engn Res Ctr SynBERC, Berkeley, CA 94720 USA.
[Arkin, Adam P.; Anderson, J. Christopher] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys Sci, Berkeley, CA 94720 USA.
RP Anderson, JC (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.
EM jcanderson@berkeley.edu
RI Arkin, Adam/A-6751-2008
OI Arkin, Adam/0000-0002-4999-2931
FU National Science Foundation Synthetic Biology Engineering Research
Center (SynBERC); National Science Foundation; Siebel Scholar award
FX We thank the CNR Biological Imaging Facility (University of California,
Berkeley) for assistance in microscopy. We also thank Lon Chubiz for
providing a CRLM helper plasmid for integrating DNA into the attP21 site
of the E. coil genome. This work was supported by the National Science
Foundation Synthetic Biology Engineering Research Center (SynBERC).
J.T.K. received support from a National Science Foundation Graduate
Research Fellowship and a Siebel Scholar award.
NR 40
TC 7
Z9 7
U1 2
U2 17
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 2161-5063
J9 ACS SYNTH BIOL
JI ACS Synth. Biol.
PD AUG
PY 2013
VL 2
IS 8
BP 418
EP 424
DI 10.1021/sb300107h
PG 7
WC Biochemical Research Methods
SC Biochemistry & Molecular Biology
GA 204JX
UT WOS:000323362700002
PM 23654275
ER
PT J
AU Straneo, F
Heimbach, P
Sergienko, O
Hamilton, G
Catania, G
Griffies, S
Hallberg, R
Jenkins, A
Joughin, I
Motyka, R
Pfeffer, WT
Price, SF
Rignot, E
Scambos, T
Truffer, M
Vieli, A
AF Straneo, Fiammetta
Heimbach, Patrick
Sergienko, Olga
Hamilton, Gordon
Catania, Ginny
Griffies, Stephen
Hallberg, Robert
Jenkins, Adrian
Joughin, Ian
Motyka, Roman
Pfeffer, W. Tad
Price, Stephen F.
Rignot, Eric
Scambos, Ted
Truffer, Martin
Vieli, Andreas
TI Challenges to Understanding the Dynamic Response of Greenland's Marine
Terminating Glaciers to Oceanic and Atmospheric Forcing
SO BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY
LA English
DT Article
ID SEA-LEVEL RISE; FULL STOKES MODEL; ICE-SHEET; JAKOBSHAVN ISBRAE; WEST
GREENLAND; OUTLET GLACIERS; EAST GREENLAND; THERMOHALINE CIRCULATION;
TIDEWATER GLACIERS; NORTH-ATLANTIC
AB The recent retreat and speedup of outlet glaciers, as well as enhanced surface melting around the ice sheet margin, have increased Greenland's contribution to sea level rise to 0.6 +/- 0.1 mm yr(-1) and its discharge of freshwater into the North Atlantic. The widespread, near-synchronous glacier retreat, and its coincidence with a period of oceanic and atmospheric warming, suggests a common climate driver. Evidence points to the marine margins of these glaciers as the region from which changes propagated inland. Yet, the forcings and mechanisms behind these dynamic responses are poorly understood and are either missing or crudely parameterized in climate and ice sheet models. Resulting projected sea level rise contributions from Greenland by 2100 remain highly uncertain. This paper summarizes the current state of knowledge and highlights key physical aspects of Greenland's coupled ice sheet-ocean-atmosphere system. Three research thrusts are identified to yield fundamental insights into ice sheet, ocean, sea ice, and atmosphere interactions, their role in Earth's climate system, and probable trajectories of future changes: 1) focused process studies addressing critical glacier, ocean, atmosphere, and coupled dynamics; 2) sustained observations at key sites; and 3) inclusion of relevant dynamics in Earth system models. Understanding the dynamic response of Greenland's glaciers to climate forcing constitutes both a scientific and technological frontier, given the challenges of obtaining the appropriate measurements from the glaciers' marine termini and the complexity of the dynamics involved, including the coupling of the ocean, atmosphere, glacier, and sea ice systems. Interdisciplinary and international cooperation are crucial to making progress on this novel and complex problem.
C1 [Straneo, Fiammetta] Woods Hole Oceanog Inst, Woods Hole, MA 02543 USA.
[Heimbach, Patrick] MIT, Cambridge, MA 02139 USA.
[Sergienko, Olga] Princeton Univ, Princeton, NJ 08544 USA.
[Sergienko, Olga; Griffies, Stephen; Hallberg, Robert] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA.
[Hamilton, Gordon] Univ Maine, Orono, ME USA.
[Catania, Ginny] Univ Texas Austin, Austin, TX 78712 USA.
[Jenkins, Adrian] British Antarctic Survey, Cambridge CB3 0ET, England.
[Joughin, Ian] Univ Washington, Seattle, WA 98195 USA.
[Motyka, Roman; Truffer, Martin] Univ Alaska Fairbanks, Fairbanks, AK USA.
[Pfeffer, W. Tad] Univ Colorado, Boulder, CO 80309 USA.
[Price, Stephen F.] Los Alamos Natl Lab, Los Alamos, NM USA.
[Rignot, Eric] Univ Calif Irvine, Irvine, CA USA.
[Rignot, Eric] CALTECH, Jet Prop Lab, Pasadena, CA USA.
[Scambos, Ted] Univ Colorado, Natl Snow & Ice Data Ctr, Boulder, CO 80309 USA.
[Vieli, Andreas] Univ Durham, Durham, England.
RP Straneo, F (reprint author), Woods Hole Oceanog Inst, Mail Stop 21,266 Woods Hole Rd, Woods Hole, MA 02543 USA.
EM fstraneo@whoi.edu
RI Catania, Ginny/B-9787-2008; Heimbach, Patrick/K-3530-2013; Joughin,
Ian/A-2998-2008; Price, Stephen /E-1568-2013; Rignot, Eric/A-4560-2014;
OI Heimbach, Patrick/0000-0003-3925-6161; Joughin, Ian/0000-0001-6229-679X;
Price, Stephen /0000-0001-6878-2553; Rignot, Eric/0000-0002-3366-0481;
Vieli, Andreas/0000-0002-2870-5921; Straneo,
Fiammetta/0000-0002-1735-2366
FU Norwegian Centre for International Cooperation in Education (SiU)
FX This is a contribution to the activity of the U.S. CLIVAR Working Group
on Greenland Ice Sheet-Ocean Interactions (GRISO). Mike Patterson is
thanked for his engagement and guidance. The idea for establishment of
such a working group originated during the Advanced Climate Dynamics
Course (ACDC) 2010 on Ice Sheet-Ocean Interactions at the MIT-Fablab in
Lyngen, Norway (see
http://onlinelibrary.wiley.com/doi/10.1029/2010EO450006/abstract), with
the Norwegian Centre for International Cooperation in Education (SiU) as
its main sponsor. We thank three anonymous reviewers for their comments.
NR 97
TC 51
Z9 51
U1 0
U2 80
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0003-0007
EI 1520-0477
J9 B AM METEOROL SOC
JI Bull. Amer. Meteorol. Soc.
PD AUG
PY 2013
VL 94
IS 8
BP 1131
EP 1144
DI 10.1175/BAMS-D-12-00100.1
PG 14
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 205YZ
UT WOS:000323482200005
ER
PT J
AU Appel, AM
Bercaw, JE
Bocarsly, AB
Dobbek, H
DuBois, DL
Dupuis, M
Ferry, JG
Fujita, E
Hille, R
Kenis, PJA
Kerfeld, CA
Morris, RH
Peden, CHF
Portis, AR
Ragsdale, SW
Rauchfuss, TB
Reek, JNH
Seefeldt, LC
Thauer, RK
Waldrop, GL
AF Appel, Aaron M.
Bercaw, John E.
Bocarsly, Andrew B.
Dobbek, Holger
DuBois, Daniel L.
Dupuis, Michel
Ferry, James G.
Fujita, Etsuko
Hille, Russ
Kenis, Paul J. A.
Kerfeld, Cheal A.
Morris, Robert H.
Peden, Charles H. F.
Portis, Archie R.
Ragsdale, Stephen W.
Rauchfuss, Thomas B.
Reek, Joost N. H.
Seefeldt, Lance C.
Thauer, Rudolf K.
Waldrop, Grover L.
TI Frontiers, Opportunities, and Challenges in Biochemical and Chemical
Catalysis of CO2 Fixation
SO CHEMICAL REVIEWS
LA English
DT Review
ID CARBON-MONOXIDE DEHYDROGENASE; ASYMMETRIC TRANSFER HYDROGENATION;
COENZYME-A SYNTHASE; FISCHER-TROPSCH SYNTHESIS; CONTAINING FORMATE
DEHYDROGENASE; TRANSITION-METAL CATALYSTS; COUPLED ELECTRON-TRANSFER;
WOOD-LJUNGDAHL PATHWAY; FRUSTRATED LEWIS PAIRS; ELECTROCHEMICAL
REDUCTION
C1 [Appel, Aaron M.; DuBois, Daniel L.; Dupuis, Michel; Peden, Charles H. F.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.
[Bercaw, John E.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA.
[Bocarsly, Andrew B.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA.
[Dobbek, Holger] Humboldt Univ, Inst Biol Strukturbiol Biochem, D-10099 Berlin, Germany.
[Ferry, James G.] Penn State Univ, Dept Biochem & Mol Biol, University Pk, PA 16801 USA.
[Fujita, Etsuko] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Hille, Russ] Univ Calif Riverside, Dept Biochem, Riverside, CA 92521 USA.
[Kenis, Paul J. A.] Univ Illinois, Dept Chem & Biochem Engn, Urbana, IL 61801 USA.
[Portis, Archie R.] Univ Illinois, Dept Crop Sci, Urbana, IL 61801 USA.
[Portis, Archie R.] Univ Illinois, Dept Plant Biol, Urbana, IL 61801 USA.
[Rauchfuss, Thomas B.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA.
[Kerfeld, Cheal A.] DOE Joint Genome Inst, Walnut Creek, CA 94598 USA.
[Kerfeld, Cheal A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.
[Morris, Robert H.] Univ Toronto, Dept Chem, Toronto, ON M5S 3H6, Canada.
[Ragsdale, Stephen W.] Univ Michigan, Dept Biol Chem, Ann Arbor, MI 48109 USA.
[Reek, Joost N. H.] Univ Amsterdam, vant Hoff Inst Mol Sci, NL-1098 XH Amsterdam, Netherlands.
[Seefeldt, Lance C.] Utah State Univ, Dept Chem & Biochem, Logan, UT 84322 USA.
[Thauer, Rudolf K.] Max Planck Inst Terr Microbiol, D-35043 Marburg, Germany.
[Waldrop, Grover L.] Louisiana State Univ, Dept Biol Sci, Baton Rouge, LA 70803 USA.
RP DuBois, DL (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA.
EM daniel.dubois@pnnl.gov; sragsdal@umich.edu; rauchfuz@illinois.edu
RI Morris, Robert/R-8760-2016; Kenis, Paul/S-7229-2016;
OI Morris, Robert/0000-0002-7574-9388; Kenis, Paul/0000-0001-7348-0381;
Peden, Charles/0000-0001-6754-9928; Appel, Aaron/0000-0002-5604-1253
FU Council on Chemical and Biochemical Sciences of the U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences
FX This article evolved from presentations and discussion at the workshop
"Frontiers, Opportunities, and Challenges in the Biochemical and
Chemical Catalysis of CO2" held in October 2011, in
Annapolis, Maryland, sponsored by the Council on Chemical and
Biochemical Sciences of the U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences. The authors thank the members
of the Council for their encouragement and assistance in developing this
workshop. In addition, the authors are indebted to the agencies
responsible for funding of their individual research efforts, without
which this work would not have been possible.
NR 389
TC 379
Z9 385
U1 105
U2 950
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0009-2665
EI 1520-6890
J9 CHEM REV
JI Chem. Rev.
PD AUG
PY 2013
VL 113
IS 8
BP 6621
EP 6658
DI 10.1021/cr300463y
PG 38
WC Chemistry, Multidisciplinary
SC Chemistry
GA 203NZ
UT WOS:000323301200017
PM 23767781
ER
PT J
AU Budworth, H
McMurray, CT
AF Budworth, Helen
McMurray, Cynthia T.
TI Bidirectional transcription of trinucleotide repeats: Roles for excision
repair
SO DNA REPAIR
LA English
DT Article
DE Bidirectional transcription; Trinucleotide; Excision repair;
Neurodegenerative; Coding; RNA transcript
ID THYMINE-DNA GLYCOSYLASE; FRAGILE-X-SYNDROME; RNA-BINDING PROTEIN;
GROUP-B PROTEIN; MYOTONIC-DYSTROPHY; HUNTINGTONS-DISEASE; HUMAN-CELLS;
FMR1 GENE; CHROMATIN-STRUCTURE; TET PROTEINS
AB Genomic instability at repetitive DNA regions in cells of the nervous system leads to a number of neurodegenerative and neuromuscular diseases, including those with an expanded trinucleotide repeat (TNR) tract at or nearby an expressed gene. Expansion causes disease when a particular base sequence is repeated beyond the normal range, interfering with the expression or properties of a gene product. Disease severity and onset depend on the number of repeats. As the length of the repeat tract grows, so does the size of the successive expansions and the likelihood of another unstable event. In fragile X syndrome, for example, CGG repeat instability and pathogenesis are not typically observed below tracts of roughly 50 repeats, but occur frequently at or above 55 repeats, and are virtually certain above 100-300 repeats.
Recent evidence points to bidirectional transcription as a new aspect of TNR instability and pathophysiology. Bidirectional transcription of TNR genes produces novel proteins and/or regulatory RNAs that influence both toxicity and epigenetic changes in TNR promoters. Bidirectional transcription of the TNR tract appears to influence aspects of its stability, gene processing, splicing, gene silencing, and chemical modification of DNAs. Paradoxically, however, some of the same effects are observed on both the expanded TNR gene and on its normal gene counterpart. In this review, we discuss the possible normal and abnormal effects of bidirectional transcription on trinucleotide repeat instability, the role of DNA repair in causing, preventing, or maintaining methylation, and chromatin environment of TNR genes. Published by Elsevier B.V.
C1 [Budworth, Helen; McMurray, Cynthia T.] Univ Calif Berkeley, Div Life Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP McMurray, CT (reprint author), Univ Calif Berkeley, Div Life Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM ctmcmurray@lbl.gov
FU National Institutes of Health [NS40738, GM066359, NS062384, NS060115,
CA092584]
FX This work was supported by the National Institutes of Health grants
NS40738 (CTM), GM066359 (CTM), NS062384 (to CTM), and NS060115 (to CTM),
and CA092584 (CTM).
NR 158
TC 8
Z9 8
U1 1
U2 18
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1568-7864
J9 DNA REPAIR
JI DNA Repair
PD AUG
PY 2013
VL 12
IS 8
SI SI
BP 672
EP 684
DI 10.1016/j.dnarep.2013.04.019
PG 13
WC Genetics & Heredity; Toxicology
SC Genetics & Heredity; Toxicology
GA 200QS
UT WOS:000323084600014
PM 23669397
ER
PT J
AU Zinkle, SJ
AF Zinkle, Steven J.
TI CHALLENGES IN DEVELOPING MATERIALS FOR FUSION TECHNOLOGY-PAST, PRESENT
AND FUTURE
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID RESEARCH-AND-DEVELOPMENT; PLASMA-FACING MATERIALS; HIGH-HEAT-FLUX;
AUSTENITIC STAINLESS-STEELS; REACTOR MATERIALS RESEARCH; CASCADE DAMAGE
CONDITIONS; LOW-ACTIVATION MATERIALS; REDUCED-ACTIVATION;
MECHANICAL-PROPERTIES; MARTENSITIC STEELS
AB A brief historical review of the evolution in structural materials options for fusion energy systems is presented, along with the author's perspective on emerging trends in advanced manufacturing techniques and new high-performance materials.
C1 [Zinkle, Steven J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Zinkle, SJ (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA.
EM zinklesj@ornl.gov
OI Zinkle, Steven/0000-0003-2890-6915
NR 152
TC 9
Z9 9
U1 0
U2 27
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
EI 1943-7641
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 65
EP 75
PG 11
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200002
ER
PT J
AU Pitcher, CS
Barnsley, R
Bertalot, L
Encheva, A
Feder, R
Friconneau, JP
Hu, Q
Levesy, B
Loesser, GD
Lyublin, B
Macklin, B
Martins, JP
Padasalagi, S
Pak, S
Reichle, R
Sato, K
Serikov, A
Seyvet, F
Suarez, A
Udintsev, V
Vayakis, G
Veshchev, E
Walker, C
Walsh, M
Watts, C
Zhai, Y
AF Pitcher, C. S.
Barnsley, R.
Bertalot, L.
Encheva, A.
Feder, R.
Friconneau, J. P.
Hu, Q.
Levesy, B.
Loesser, G. D.
Lyublin, B.
Macklin, B.
Martins, J. P.
Padasalagi, S.
Pak, S.
Reichle, R.
Sato, K.
Serikov, A.
Seyvet, F.
Suarez, A.
Udintsev, V.
Vayakis, G.
Veshchev, E.
Walker, C.
Walsh, M.
Watts, C.
Zhai, Y.
TI PORT-BASED PLASMA DIAGNOSTIC INFRASTRUCTURE ON ITER
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB The port-based plasma diagnostic infrastructure on ITER is described, including the port plugs, the interspace support structure and port cell structure. These systems are modular in nature with standardized dimensions. The design of the equatorial and upper port plugs and their modules is discussed, as well as the dominant loading mechanisms. The port infrastructure design has now matured to the point that port plugs are now being populated with multiple diagnostics supplied by a number of ITER partners - two port plug examples are given.
C1 [Pitcher, C. S.; Barnsley, R.; Bertalot, L.; Encheva, A.; Friconneau, J. P.; Levesy, B.; Macklin, B.; Martins, J. P.; Reichle, R.; Udintsev, V.; Vayakis, G.; Veshchev, E.; Walker, C.; Walsh, M.; Watts, C.] ITER Org, F-13115 St Paul Les Durance, France.
[Feder, R.; Loesser, G. D.; Zhai, Y.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Hu, Q.] Chinese Acad Sci, Inst Plasma Phys, Beijing 100864, Peoples R China.
[Lyublin, B.] Efremov, St Petersburg, Russia.
[Padasalagi, S.] Inst Plasma Res, Gandhinagar, Gujarat, India.
[Pak, S.] Natl Fus Res Inst, Taejon, South Korea.
[Sato, K.] Japan Atom Energy Agcy, Naka, Ibaraki, Japan.
[Serikov, A.] KIT, Eggenstein Leopoldshafen, Germany.
[Seyvet, F.] F4E, Barcelona, Spain.
[Suarez, A.] CIEMAT, E-28040 Madrid, Spain.
RP Pitcher, CS (reprint author), ITER Org, Route Vinon Verdon, F-13115 St Paul Les Durance, France.
NR 8
TC 1
Z9 1
U1 0
U2 5
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 118
EP 125
PG 8
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200008
ER
PT J
AU Titus, PH
Kalish, M
Hause, CM
Heitzenroeder, P
Hsiao, J
Pillsbury, R
Daly, E
AF Titus, Peter H.
Kalish, Michael
Hause, Christopher M.
Heitzenroeder, Philip
Hsiao, Jushin
Pillsbury, Robert
Daly, Edward
TI DESIGN AND ANALYSIS OF THE ITER VERTICAL STABILITY (VS) COILS
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB The ITER vertical stability (VS) coils have been developed through the preliminary design phase by Princeton Plasma Physics Laboratory (PPPL). Final design, prototyping and construction will be carried out by the Chinese Participant Team contributing lab, Institute of Plasma Physics, Chinese Academy of Sciences (ASIPP). The VS coils are a part of the in-vessel coil systems which include edge localized mode (ELM) coils as well as the VS coils.
The VS design employs four turns of stainless steel jacketed mineral insulated copper (SSMIC) conductors The mineral insulation is Magnesium Oxide (MgO). Joule and nuclear heat are removed by water flowing through the hollow copper conductor. The slightly elevated temperatures in the conductor and its support spine during operation impose compressive stresses that mitigate fatigue damage. Away from joints, and break-outs, conductor thermal stresses are low because of the axisymmetry of the winding (there are no corner bends as in the ELM coils). The joints, and break-out or terminal regions are designed with similar but imperfect constraint compared with the ring coil portion of the VS. The support for the break-out region is made from a high strength copper alloy, CuCrZr. This is needed to conduct nuclear heat to the actively cooled conductor and to the vessel wall. The support "spine" for the ring coil portion of the VS is 316 stainless steel, held to the vessel with preloaded Inconel 718 bolts. Lorentz loads resulting from normal operating loads, disruption loads and loads from disruption currents in the support spine shared with vessel, are applied to the VS coil. Stresses in the coil, joints, and break-outs are presented. These are compared with static and fatigue allowables. Design for fatigue is much less demanding than for the ELM coils. A total of 30,000 cycles is required for VS design.
C1 [Titus, Peter H.; Kalish, Michael; Hause, Christopher M.; Heitzenroeder, Philip] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Pillsbury, Robert] Sherbrooke Consulting Inc, Sherbrooke, PQ, Canada.
[Daly, Edward] ITER Org, Cadarache, France.
RP Titus, PH (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM ptitus@pppl.gov
NR 15
TC 1
Z9 1
U1 0
U2 5
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 136
EP 145
PG 10
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200011
ER
PT J
AU Kotulski, JD
Coats, RS
Ulrickson, M
AF Kotulski, J. D.
Coats, R. S.
Ulrickson, M.
TI TRANSIENT ELECTROMAGNETIC ANALYSIS OF BLANKET MODULE 1 OF THE ITER
BLANKET SYSTEM DUE TO PLASMA DISRUPTION
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB The prediction of electromagnetic loads on blanket module I of the ITER device during a plasma disruption event is considered This analysis is performed for a number of design variations (of the blanket module) and different disruption events.
The key features of the analysis procedure will be presented including the geometric description of the blanket module composed of a first wall, shield block, and vacuum vessel. The modeling of the plasma current will also be described.
The electromagnetic analyses are performed using the Opera-3d software. The transient eddy currents are first calculated, from which the electromagnetic loads are determined Once these loads have been calculated they can also be exported for additional post-processing to assess the mechanical loading effects.
C1 [Kotulski, J. D.; Coats, R. S.; Ulrickson, M.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Kotulski, JD (reprint author), Sandia Natl Labs, POB 5800,MS 1152, Albuquerque, NM 87185 USA.
EM jdkotul@sandia.gov
NR 6
TC 0
Z9 0
U1 0
U2 3
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 146
EP 150
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200012
ER
PT J
AU Loesser, GD
Pitcher, CS
Feder, R
Johnson, D
Pak, S
Walsh, M
Zhai, Y
AF Loesser, G. D.
Pitcher, C. S.
Feder, R.
Johnson, D.
Pak, S.
Walsh, M.
Zhai, Y.
TI ITER DIAGNOSTIC FIRST WALL
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB The ITER Diagnostic Division is responsible for designing and procuring the First Wall Blankets that are mounted on the vacuum vessel port plugs at both the upper and equatorial levels. This paper will discuss the effects of the diagnostic aperture shape and configuration on the coolant circuit design. The Diagnostic First Wall (DFW) design is driven in large part by the need to conform the coolant arrangement to a wide variety of diagnostic apertures combined with the more severe heating conditions at the surface facing the plasma, the First Wall (FW). At the FW, a radiant heat flux of 35W/cm(2) combines with approximate peak volumetric heating rates of 8W/cm(3) (equatorial ports) and 5W/cm3 (upper ports). Here at the FW, a fast thermal response is desirable and leads to a thin element between the heat flux and coolant. This requirement conflicts with the desire to have a thicker FW element to accommodate surface erosion and other off-normal plasma events.
C1 [Loesser, G. D.; Feder, R.; Johnson, D.; Zhai, Y.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Pitcher, C. S.; Walsh, M.] ITER Org, F-13115 St Paul Les Durance, France.
[Pak, S.] Natl Fus Res Inst, Taejon, South Korea.
RP Loesser, GD (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM dloesser@pppl.gov
NR 4
TC 0
Z9 0
U1 0
U2 1
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 156
EP 160
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200014
ER
PT J
AU Myatt, RL
Martovetsky, NN
Barbier, C
Freudenberg, KD
AF Myatt, R. Leonard
Martovetsky, Nicolai N.
Barbier, Charlotte
Freudenberg, Kevin D.
TI ITER CS CONDUCTOR HELIUM INLET DESIGN OPTIMIZATION AND EVALUATION
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB The ITER central solenoid (CS) is wound from cable-in-conduit-conductor (CICC) and cooled by supercritical Helium (He) delivered to similar to 120 inner diameter (ID) turns through integrally welded "inlets." The flow to each inlet splits and passes through two pancakes, exiting at outlets. While both the He supply and return points (outlets) require penetrating the conduit wag the inlets reside in the highest stress field, and thus become the more critical structural element.
The CS Conceptual Design Review (CRD) reference He inlet design has a long, narrow slot in the inside diameter (ID) turn wall with pencil-tip shaped ends. This shape is optimized in order to minimize the hoop stress concentration. The slot length is chosen to expose each of the six superconducting (SC) sub-cables to the He cooling supply. Implementing this design at 120 inlet sites requires substantial machining and welding operations where even virgin conduit has minimal structural margin.
A design space exploration produces numerous inlet options. One configuration emerges as the new reference configuration: the oblong, heavy-wall boss. It addresses all of the critical issues: bi-axial stress field, pressure drop and sub-cable flow uniformity, manufacturing costs (complexities and risks) and in-service robustness (least invasive, greatest margin).
Finite element (FE) simulations are presented which highlight the results of the optimization and evaluation process.
C1 [Myatt, R. Leonard] Myatt Consulting Inc, Norfolk, MA 02056 USA.
[Martovetsky, Nicolai N.] ORNL, LLNL, Oak Ridge, TN 37831 USA.
[Barbier, Charlotte; Freudenberg, Kevin D.] ORNL, Oak Ridge, TN 37831 USA.
RP Myatt, RL (reprint author), Myatt Consulting Inc, 8 Eric Rd, Norfolk, MA 02056 USA.
EM leonard.myatt@myattconsulting.com
NR 4
TC 0
Z9 0
U1 0
U2 3
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 161
EP 167
PG 7
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200015
ER
PT J
AU Daly, EF
Ioki, K
Loarte, A
Martin, A
Brooks, A
Heitzenroeder, P
Kalish, M
Neumeyer, C
Titus, P
Zhai, Y
Wu, Y
Jin, H
Long, F
Song, Y
Wang, Z
Pillsbury, R
Feng, J
Bohm, T
Sawan, M
Preble, J
AF Daly, E. F.
Ioki, K.
Loarte, A.
Martin, A.
Brooks, A.
Heitzenroeder, P.
Kalish, M.
Neumeyer, C.
Titus, P.
Zhai, Y.
Wu, Y.
Jin, H.
Long, F.
Song, Y.
Wang, Z.
Pillsbury, R.
Feng, J.
Bohm, T.
Sawan, M.
Preble, J.
TI UPDATE ON DESIGN OF THE ITER IN-VESSEL COILS
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB The ITER project baseline now includes two sets of in-vessel coils, one to mitigate the effects of Edge Localized Modes (ELMs) and another to provide vertical stabilization (VS). The in-vessel location presents special challenges in terms of nuclear radiation and temperature, and requires the use of mineral-insulated conductors. An update to the preliminary design based on this conductor technology is presented for both coil designs. Results from an on-going R&D program consisting of conductor development, welding and brazing process development, electrical testing and mechanical testing in order to demonstrate manufacturability of this style of conductor are presented. Plans for two prototype coils, one of each type, are presented.
C1 [Daly, E. F.; Ioki, K.; Loarte, A.; Martin, A.] ITER Org, F-13115 St Paul Les Durance, France.
[Brooks, A.; Heitzenroeder, P.; Kalish, M.; Neumeyer, C.; Titus, P.; Zhai, Y.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Wu, Y.; Jin, H.; Long, F.; Song, Y.; Wang, Z.] Chinese Acad Sci, Inst Plasma Phys, Beijing 100864, Anhui, Peoples R China.
[Pillsbury, R.] Sherbrooke Consulting, Arlington, VA USA.
[Feng, J.] MIT Plasma Sci & Fus Ctr, Cambridge, MA USA.
[Bohm, T.; Sawan, M.] Univ Wisconsin, Fus Technol Inst, Madison, WI USA.
[Preble, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA USA.
RP Daly, EF (reprint author), ITER Org, Route Vinon, F-13115 St Paul Les Durance, France.
EM Edward.Daly@iter.org
NR 6
TC 11
Z9 11
U1 0
U2 6
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 168
EP 175
PG 8
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200016
ER
PT J
AU Reyes, S
Anklam, T
Babineau, D
Becnel, J
Davis, R
Dunne, M
Farmer, J
Flowers, D
Kramer, K
Martinez-Frias, J
Miles, R
Taylor, C
AF Reyes, S.
Anklam, T.
Babineau, D.
Becnel, J.
Davis, R.
Dunne, M.
Farmer, J.
Flowers, D.
Kramer, K.
Martinez-Frias, J.
Miles, R.
Taylor, C.
TI LIFE TRITIUM PROCESSING: A SUSTAINABLE SOLUTION FOR CLOSING THE FUSION
FUEL CYCLE
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID HYDROGEN ISOTOPE-SEPARATION; ENERGY
AB The Laser Inertial Fusion Energy (LIFE) power plant is being designed to deliver a transformative source of safe, secure, sustainable electricity, in a time scale that is consistent with the global energy market needs. The LIFE market entry plant will demonstrate the feasibility of a closed fusion fuel cycle, including tritium breeding, extraction, processing, re-fueling, accountability and safety, in a steady-state power-producing device. While many fusion plant designs require large quantities of tritium for startup and operations, a range of design choices made for the LIFE fuel cycle act to reduce the in-process tritium inventory. The high fractional burn-up (similar to 30%) in an Inertial Fusion Energy (IFE) capsule relaxes the tritium breeding requirements, while the use of only milligram quantities of fuel per shot and choice of a pure lithium heat transfer fluid substantially reduce the amount of material entrained in the facility. Additionally, the high solubility of tritium in the lithium breeder is expected to mitigate the need for development of permeation barriers in the engine systems, normally required to control routine releases within the allowable regulatory limits.
The present paper offers an overview of the design of the LIFE fuel cycle, including a summary of the technology development plan consistent with the delivery schedule of the LIFE market entry plant.
C1 [Reyes, S.; Anklam, T.; Dunne, M.; Farmer, J.; Flowers, D.; Kramer, K.; Martinez-Frias, J.; Miles, R.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Babineau, D.; Becnel, J.] Savannah River Natl Lab, Aiken, SC USA.
[Taylor, C.] Los Alamos Natl Lab, Los Alamos, NM USA.
RP Reyes, S (reprint author), Lawrence Livermore Natl Lab, Livermore, CA USA.
EM reyes20@llnl.gov
RI Dunne, Mike/B-4318-2014; Johnson, Marilyn/E-7209-2011
OI Dunne, Mike/0000-0001-8740-3870;
NR 12
TC 3
Z9 3
U1 0
U2 6
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 187
EP 193
PG 7
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200018
ER
PT J
AU Rapp, J
Biewer, TM
Canik, J
Caughman, JBO
Goulding, RH
Hillis, DL
Lore, JD
Owen, LW
AF Rapp, J.
Biewer, T. M.
Canik, J.
Caughman, J. B. O.
Goulding, R. H.
Hillis, D. L.
Lore, J. D.
Owen, L. W.
TI THE DEVELOPMENT OF PLASMA-MATERIAL INTERACTION FACILITIES FOR THE FUTURE
OF FUSION TECHNOLOGY
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID NEUTRON-IRRADIATION; SURFACE INTERACTION; TUNGSTEN; EROSION; DEVICES;
ITER
AB A new era of fusion research has started with ITER being constructed and DEMO for power demonstration on the horizon. However, the fusion nuclear science needs to be developed before DEMO can be designed One of the most crucial and most complex outstanding science issues to be solved is the plasma surface interaction (PSI) in the hostile environment of a nuclear fusion reactor. Not only are materials exposed to unprecedented steady-state and transient power fluxes, but they are also exposed to unprecedented neutron fluxes. Both the ion fluxes and the neutron fluxes will change the micro-structure of the plasma facing materials significantly even to the extent that their structural integrity is compromised. New devices have to be developed to address the challenges ahead Linear plasma-material interaction facilities can play a crucial role in advancing the plasma-material interaction science and the development of plasma facing components for future fusion reactors.
C1 [Rapp, J.; Biewer, T. M.; Canik, J.; Caughman, J. B. O.; Goulding, R. H.; Hillis, D. L.; Lore, J. D.; Owen, L. W.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Rapp, J (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
EM rappj@ornl.gov
RI Goulding, Richard/C-5982-2016; Caughman, John/R-4889-2016;
OI Goulding, Richard/0000-0002-1776-7983; Caughman,
John/0000-0002-0609-1164; Canik, John/0000-0001-6934-6681; Rapp,
Juergen/0000-0003-2785-9280; Lore, Jeremy/0000-0002-9192-465X
NR 27
TC 8
Z9 8
U1 1
U2 11
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 237
EP 244
PG 8
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200026
ER
PT J
AU Zhang, H
Titus, PH
Ellis, R
Harrison, S
Vieira, R
AF Zhang, Han
Titus, Peter H.
Ellis, Robert
Harrison, Soren
Vieira, Rui
TI THERMAL ANALYSIS TO CALCULATE THE VESSEL TEMPERATURE AND STRESS IN
ALCATOR C-MOD DUE TO THE DIVERTOR UPGRADE
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB Alcator C-Mod is planning an upgrade to its outer divertor. The upgrade is intended to correct the existing outer divertor alignment with the plasma, and to operate at elevated temperatures. Higher temperature operation will allow study of edge physics behavior at reactor relevant temperatures. The outer divertor and tiles will be capable of operating at 600 degrees C. Longer pulse length, together with the plasma and RF heat of 9 MW, and the inclusion of heater elements within the outer divertor produces radiative energy which makes the sustained operation much more difficult than before. An ANSYS model was built for the global thermal analysis of C-Mod. It models the radiative surfaces inside the vessel and between the components, and also includes plasma energy deposition. Different geometries have been simulated and compared Results show that steady state operation with the divertor at 600 degrees C is possible with no damage to major vessel internal components. The differential temperature between inner divertor structure, or "girdle" and inner vessel wall is 70 degrees C. This differential temperature is limited by the capacity of the studs that hold the inner divertor backing plates to the vessel wall. At a 70 degrees C temperature differential the stress on the studs is within allowable limits. The thermal model was then used for a stress pass to quantify vessel shell stresses where thermal gradients are significant.
C1 [Zhang, Han; Titus, Peter H.; Ellis, Robert; Harrison, Soren] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Harrison, Soren; Vieira, Rui] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA.
RP Zhang, H (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM hzhang@pppl.gov
NR 5
TC 2
Z9 2
U1 0
U2 1
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 250
EP 254
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200028
ER
PT J
AU Zhai, YH
Titus, P
Brooks, A
Hatcher, R
AF Zhai, Yuhu
Titus, Peter
Brooks, Art
Hatcher, Ronald
TI DISRUPTION ANALYSIS AND RESPONSE IMPLICATION OF PASSIVE PLATES FOR THE
NSTX UPGRADE
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB The National Spherical Torus eXperiment (NSTX) upgrade project requires analysis qualifications of existing vacuum vessel and passive stabilizing plates for increased plasma performance. Vertical stability is critically dependent on the passive conducting structure that surrounds the plasma. In this paper, the passive plate is analyzed for the upgrade condition during plasma disruption to ensure the level of stress in the plate and the fastener is within its design limits. The counter-bore of the passive plate for bolting is evaluated in detail and counter-bore bushing is redesigned to prevent shear failure during disruptions as a result of high pulling and pushing forces, particularly for support at corner bolts.
C1 [Zhai, Yuhu; Titus, Peter; Brooks, Art; Hatcher, Ronald] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Zhai, YH (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM yzhai@pppl.gov
NR 6
TC 0
Z9 0
U1 0
U2 2
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 255
EP 259
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200029
ER
PT J
AU Youchison, DL
Ulrickson, MA
AF Youchison, Dennis L.
Ulrickson, Michael A.
TI PLASMA FACING COMPONENT DESIGN THROUGH MULTIPHYSICS SIMULATION
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID COMPUTATIONAL FLUID-DYNAMICS; ITER 1ST WALL
AB Continual technology development for fusion has come to rely on the principle of "design by analysis" where advanced finite element analysis (FEA) or finite volume analysis provides insight on the performance of engineered systems. Extensive three-dimensional (3D) computations in fluid dynamics, heat transfer, neutronics, magneto-hydrodynamics and electro-magnetics are involved in an iterative design process for magnets, vacuum vessels and in-vessel components. Many difficulties arose in the integration of computer-assisted design (CAD) packages and the numeric models and results from different FEA codes. Over the last decade, engineers developed a vast array of specialized translators and interpolation programs to deal with geometry, mesh and load transfers between single-discipline codes, often with mixed outcomes. Now, several multiphysics codes that allow calculations on the same mesh and easy transfer of loads and other boundary conditions are emerging in the commercial market. These codes often have a robust library of physics models and solvers that address both steady state and transient phenomena and provide simultaneous solutions to heat transfer, fluid flow and structural mechanics problems. This article reviews three existing design tools, provides some examples of how the multiphysics codes are impacting practical engineering design, and identifies some important gaps that still exist today.
C1 [Youchison, Dennis L.; Ulrickson, Michael A.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Youchison, DL (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM dlyouch@sandia.gov
OI Youchison, Dennis/0000-0002-7366-1710
NR 18
TC 0
Z9 0
U1 0
U2 7
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 269
EP 276
PG 8
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200031
ER
PT J
AU Harrison, S
Vieira, R
Lipschultz, B
Ellis, R
Karnes, D
Titus, P
Zhou, LH
Zhang, H
Beck, W
AF Harrison, Soren
Vieira, Rui
Lipschultz, Bruce
Ellis, Robert
Karnes, Dan
Titus, Peter
Zhou, Lihua
Zhang, Han
Beck, William
TI DESIGN AND R&D FOR THE C-MOD OUTER DIVERTOR UPGRADE
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB Operational requirements and research considerations make a high-temperature, toroidally continuous outer divertor an important upgrade to the Alcator C-Mod tokamak. Leading edge melting of tiles, non-uniform heat loads, large electromagnetic forces, and localized impurity sources limit the performance of bulk plasmas. These issues can be addressed by the installation of a well-aligned, toroidally continuous outer divertor. Additionally, future long pulse operation will cause the temperature of the outer divertor to reach bulk temperatures as high as 500 - 600 degrees C. This future operational requirement combined with the strong temperature dependence of plasma surface interactions (especially fuel retention), makes a controllable, high-temperature outer divertor desirable and necessary. The motivation, criteria, design, and R&D for the upgrade are discussed below.
C1 [Harrison, Soren; Ellis, Robert; Karnes, Dan; Titus, Peter; Zhou, Lihua; Zhang, Han] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA.
[Harrison, Soren; Vieira, Rui; Lipschultz, Bruce; Karnes, Dan; Beck, William] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA.
RP Harrison, S (reprint author), Princeton Plasma Phys Lab, 100 Stellarator Rd, Princeton, NJ 08540 USA.
EM harrison1@psfc.mit.edu
RI Lipschultz, Bruce/J-7726-2012
OI Lipschultz, Bruce/0000-0001-5968-3684
NR 3
TC 1
Z9 1
U1 0
U2 2
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 277
EP 281
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200032
ER
PT J
AU Zhou, LH
Vieira, R
Harrison, S
Karnes, D
Lipschultz, B
AF Zhou, Lihua
Vieira, Rui
Harrison, Soren
Karnes, Dan
Lipschultz, Bruce
TI HEAT TRANSFER SIMULATION OF A-FRAME ASSEMBLY TO SUPPORT ALCATOR C-MOD
OUTER DIVERTOR UPGRADE
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB To design the Alcator C-Mod outer divertor to operate at 600 degrees C and determine its effect on the surrounding vessel and diagnostics, heat transfer analysis must be performed. This paper describes the analysis and the results of heat transfer simulations of the outer divertor tiles, tile-mounting plate, support structure, and current shunt. Using Comsol, commercial FEA software package, a 3D wedge model that exploits the cyclic symmetry of the divertor, is created By adjusting the power level of each of the 7 heaters used to elevate and control the divertor temperature, a uniform poloidal temperature distribution is achieved and the power requirements for the heaters are determined The temperature of each component in the assembly is calculated, and results are used for further design changes. Additionally, radiation simulation on thermal shields are presented, which is used as ambient temperature for the heat transfer of the A-frame assembly. Furthermore, a full model of the entire outer divertor ring is presented with its toroidal temperature distribution. Finally, thermal stress of the plate is analyzed besides an analytical calculation of the maximum allowable temperature difference.
C1 [Zhou, Lihua; Vieira, Rui; Harrison, Soren; Karnes, Dan; Lipschultz, Bruce] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA.
[Harrison, Soren; Karnes, Dan] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Zhou, LH (reprint author), MIT, Plasma Sci & Fus Ctr, 190 Albany St, Cambridge, MA 02139 USA.
EM lihua@psfc.mit.edu
RI Lipschultz, Bruce/J-7726-2012
OI Lipschultz, Bruce/0000-0001-5968-3684
NR 2
TC 2
Z9 2
U1 0
U2 3
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 293
EP 297
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200035
ER
PT J
AU Berlinger, B
Brooks, A
Feder, H
Gumbas, J
Franckowiak, T
Cohen, SA
AF Berlinger, B.
Brooks, A.
Feder, H.
Gumbas, J.
Franckowiak, T.
Cohen, S. A.
TI USE OF POLYCARBONATE VACUUM VESSELS IN HIGH-TEMPERATURE FUSION-PLASMA
RESEARCH
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID FIELD-REVERSED CONFIGURATIONS
AB Magnetic fusion energy (MFE) research requires ultrahigh-vacuum conditions, primarily to reduce plasma contamination by impurities. For radiofrequency (RF)-heated plasmas, a great benefit may accrue from a non-conducting vacuum vessel, allowing external RF antennas to avoid the complications and cost of internal antennas and high-voltage high-current feedthroughs. In this paper we describe these and other criteria, e.g., safety, design flexibility, structural integrity, access, outgassing, transparency, and fabrication techniques that led to the selection and use of 25.4-cm OD, 1.6-cm wall polycarbonate pipe as the main vacuum vessel for an MFE research device whose plasmas are expected to reach keV energies for durations exceeding 0.1 s.
C1 [Berlinger, B.; Brooks, A.; Feder, H.; Gumbas, J.; Franckowiak, T.; Cohen, S. A.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Berlinger, B (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM BBerling@Princeton.edu
NR 11
TC 0
Z9 0
U1 0
U2 2
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 298
EP 302
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200036
ER
PT J
AU Ying, A
Zhang, HJ
Garde, JM
Ulrickson, M
AF Ying, Alice
Zhang, Hongjie
Garde, Joseph Mauricio
Ulrickson, Mike
TI STRUCTURAL ANALYSIS FOR EHF HYPERVAPOTRON TWIN FINGERS AND BERYLLIUM
TILE SIZE STUDY
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID 1ST WALL
AB The impact of Be tile size on the stress exerted on the CuCrZr heat sink for the ITER EHF finger was examined. The study especially focused on the areas beneath the tiles that are exposed to the high convective heat flux. For reference, in a Be tile size of 50x50x8 mm(3), the calculated equivalent strain range using elastic analysis for the path of interest through the side wall of the CuCrZr heat sink resulted in a peak value at the inner wall of similar to 0.492%. The corresponding fatigue lifetime of the heat sink locally is unacceptably low, 1400 cyclic operations. By using smaller tiles, lower stress amplitudes are observed due to a smaller deformation. In this paper, the total strain range under ITER projected pulsed operating conditions is analyzed for a range of Be tile sizes. The analysis model uses a complete pair of twin fingers as opposed to a sub-model of two tiles. The paper documents the calculated cyclic lifetime of the ITER EHF CuCrZr heat sink with respect to Be tile size and peak heat loads by evaluating the total strain range both from elastic and time independent elasto-plastic analyses for repeated cycle.
C1 [Ying, Alice; Zhang, Hongjie] Univ Calif Los Angeles, Dept Mech & Aerosp Engn, Los Angeles, CA 90095 USA.
[Garde, Joseph Mauricio; Ulrickson, Mike] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Ying, A (reprint author), Univ Calif Los Angeles, Dept Mech & Aerosp Engn, Los Angeles, CA 90095 USA.
EM ying@fusion.ucla.edu
NR 9
TC 1
Z9 1
U1 0
U2 1
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 309
EP 314
PG 6
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200038
ER
PT J
AU Doody, J
Granetz, R
Lipschultz, B
Zhang, H
Titus, P
Vieira, R
AF Doody, Jeffrey
Granetz, Robert
Lipschultz, Bruce
Zhang, Han
Titus, Peter
Vieira, Rui
TI ANSYS MODEL TO PREDICT MAGNETIC FIELDS AND LOADS IN ALCATOR C-MOD'S NEW
OUTER DIVERTOR DURING A DISRUPTION
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
AB A new outer divertor is being designed for installation on Alcator C-Mod. This divertor will be toroidally continuous such that the currents during a disruption will be driven in the toroidal direction and not cross Alcator's large toroidal field and it eliminates leading edges. However, currents will still cross the poloidal fields, and so it is important to properly predict the poloidal fields in the area of the divertor so that we can properly predict the loads on the divertor during a disruption. To that end, an ANSYS model has been built which can predict the fields and field transients in C-Mod given two inputs, the currents for the toroidal and poloidal field coils which come from measured data taken during a discharge, and the current in the plasma, which comes from another model that solves Maxwell's equations to reconstruct the plasma as 24 current carrying filaments. The advantage of using this method to predict fields is that it provides the ability to create a model based on actual measured data and to model whichever type of disruption, whether a midplane disruption or a vertical displacement event, is deemed necessary for the design. The ANSYS model then is able to predict the fields, including the shielding effects of the structures in the vessel, and the currents induced in the vessel and these structures. These results can then be mapped to a sub-model of the divertor to predict loading and stress during the disruption.
C1 [Doody, Jeffrey; Granetz, Robert; Lipschultz, Bruce; Vieira, Rui] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA.
[Zhang, Han; Titus, Peter] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Doody, J (reprint author), MIT, Plasma Sci & Fus Ctr, 190 Albany St, Cambridge, MA 02139 USA.
EM doody@psfc.mit.edu
RI Lipschultz, Bruce/J-7726-2012
OI Lipschultz, Bruce/0000-0001-5968-3684
NR 5
TC 1
Z9 1
U1 0
U2 2
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 320
EP 324
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200040
ER
PT J
AU Humrickhouse, PW
Merrill, BJ
AF Humrickhouse, Paul W.
Merrill, Brad J.
TI MELCOR ACCIDENT ANALYSIS FOR ARIES-ACT
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID DESIGN
AB We model a loss of flow accident (LOFA) in the ARIES-ACT1 tokamak design. ARIES-ACT1 features an advanced SiC blanket with LiPb as coolant and breeder, a helium cooled steel structural ring and tungsten divertors, a thin-walled, helium cooled vacuum vessel, and a room temperature water-cooled shield outside the vacuum vessel. The water heat transfer system is designed to remove heat by natural circulation during a LOFA. The MELCOR model uses time-dependent decay heats for each component determined by 1-D modeling. The MELCOR model shows that, despite periodic boiling of the water coolant, that structures are kept adequately cool by the passive safety system.
C1 [Humrickhouse, Paul W.; Merrill, Brad J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
RP Humrickhouse, PW (reprint author), Idaho Natl Lab, POB 1625 MS 3840, Idaho Falls, ID 83415 USA.
EM paul.humrickhouse@inl.gov
NR 11
TC 3
Z9 3
U1 0
U2 4
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 340
EP 344
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200043
ER
PT J
AU Cadwallader, L
Pinna, T
AF Cadwallader, L.
Pinna, T.
TI RELIABILITY ESTIMATION FOR DOUBLE CONTAINMENT PIPING
SO FUSION SCIENCE AND TECHNOLOGY
LA English
DT Article; Proceedings Paper
CT 20th American-Nuclear-Society (ANS) Topical Meeting on the Technology of
Fusion Energy (TOFE)
CY AUG 27-31, 2012
CL Nashville, TN
SP Amer Nucl Soc (ANS), Oak Ridge Natl Lab, US ITER, Lawrence Livermore Natl Lab, Princeton Plasma Phys Lab, Naval Res Lab, Atom Energy Soc Japan, Canadian Nucl Soc, Inst Elect & Elect Engineers
ID STORAGE TANKS; SYSTEMS; PIPE
AB Double walled or double containment piping is considered for use in the ITER international project and other next-generation fusion device designs to provide an extra barrier for tritium gas and other radioactive materials. The extra barrier improves confinement of these materials and enhances safety of the facility. This paper describes some of the design challenges in designing double containment piping systems. There is also a brief review of a few operating experiences of double walled piping used with hazardous chemicals in different industries. The authors recommend approaches for the reliability analyst to use to quantify leakage from a double containment piping system in conceptual and more advanced designs. The paper also cites quantitative data that can be used to support such reliability analyses.
C1 [Cadwallader, L.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Pinna, T.] ENEA, I-00044 Frascati, Rome, Italy.
RP Cadwallader, L (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA.
EM lee.cadwallader@inl.gov
RI Cadwallader, Lee/F-6933-2014
NR 26
TC 2
Z9 2
U1 0
U2 1
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 1536-1055
J9 FUSION SCI TECHNOL
JI Fusion Sci. Technol.
PD AUG
PY 2013
VL 64
IS 2
BP 351
EP 356
PG 6
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 198RE
UT WOS:000322939200045
ER
PT J
AU Humble, TS
AF Humble, Travis S.
TI Quantum Security for the Physical Layer
SO IEEE COMMUNICATIONS MAGAZINE
LA English
DT Article
AB The physical layer describes how communication signals are encoded and transmitted across a channel. Physical security often requires either restricting access to the channel or performing periodic manual inspections. In this tutorial, we describe how the field of quantum communication offers new techniques for securing the physical layer. We describe the use of quantum seals as a unique way to test the integrity and authenticity of a communication channel and to provide security for the physical layer. We present the theoretical and physical underpinnings of quantum seals including the quantum optical encoding used at the transmitter and the test for non-locality used at the receiver. We describe how the envisioned quantum physical sublayer senses tampering and how coordination with higher protocol layers allows quantum seals to influence secure routing or tailor data management methods. We conclude by discussing challenges in the development of quantum seals, the overlap with existing quantum key distribution cryptographic services, and the relevance of a quantum physical sublayer to the future of communication security.
C1 Oak Ridge Natl Lab, Oak Ridge, TN USA.
RP Humble, TS (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN USA.
EM humblets@ornl.gov
FU Defense Threat Reduction Agency; U.S. Department of Energy
[DE-AC05-00OR22725]
FX This work was supported by the Defense Threat Reduction Agency. This
manuscript has been authored by UT-Battelle, LLC, under Contract No.
DE-AC05-00OR22725 with the U.S. Department of Energy. Accordingly, the
U.S. Government retains a non-exclusive, royalty-free license to publish
or reproduce the published form of this contribution, or allow others to
do so, for U.S. Government purposes.
NR 11
TC 5
Z9 5
U1 0
U2 11
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0163-6804
J9 IEEE COMMUN MAG
JI IEEE Commun. Mag.
PD AUG
PY 2013
VL 51
IS 8
BP 56
EP 62
PG 7
WC Engineering, Electrical & Electronic; Telecommunications
SC Engineering; Telecommunications
GA 206AT
UT WOS:000323488500007
ER
PT J
AU Bolotnikov, AE
Butcher, J
Camarda, GS
Cui, YG
De Geronimo, G
Fried, J
Fochuk, PM
Hossain, A
Kim, KH
Kopach, OV
Mahler, G
Marshall, M
McCall, B
Petryk, M
Vernon, E
Yang, G
James, RB
AF Bolotnikov, Aleksey E.
Butcher, Jamie
Camarda, Giuseppe S.
Cui, Yonggang
De Geronimo, Gianluigi
Fried, Jack
Fochuk, P. M.
Hossain, Anwar
Kim, Kihyun H.
Kopach, O. V.
Mahler, G.
Marshall, Matthew
McCall, B.
Petryk, Matthew
Vernon, Emerson
Yang, Ge.
James, Ralph B.
TI Design Considerations and Testing of Virtual Frisch-Grid CdZnTe Detector
Arrays Using the H3D ASIC
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE CdZnTe; charge-loss correction; crystal defects; virtual Frisch grid
detectors
ID CHARGE-COLLECTION EVENTS; READOUT; PERFORMANCE; DEFECTS
AB We discussed the design implementation and results from testing 2 x 2-, 3 x 3-, and 2 x 4-arrays of 6 x 6 x 15 mm(3) CdZnTe virtual Frisch-grid detectors. In these measurements we employed a data acquisition system based on the H3D ASIC developed by BNL's Instrumentation Division in collaboration with the University of Michigan for 3D position-sensitive detectors. We used CZT crystals with a range of performance attributes to evaluate practical array configurations and detector-assembling procedures. The detector ratings were assigned based on the pulse-height spectra and correlated with data from X-ray diffraction topography measurements and X-ray response mapping obtained at BNL's National Synchrotron Light Source. The results helped us to better understand the performance limits of these detectors, and to identify future improvements in the array's design and requirements for the new readout ASIC.
C1 [Bolotnikov, Aleksey E.; Camarda, Giuseppe S.; Cui, Yonggang; De Geronimo, Gianluigi; Fried, Jack; Hossain, Anwar; Kim, Kihyun H.; Mahler, G.; Petryk, Matthew; Vernon, Emerson; Yang, Ge.; James, Ralph B.] Brookhaven Natl Lab, Upton, NY 11793 USA.
[Butcher, Jamie] SUNY Coll Geneseo, Geneseo, NY 14454 USA.
[Fochuk, P. M.; Kopach, O. V.] Chernivtsi Natl Univ, UA-58000 Chernovtsy, Ukraine.
[Marshall, Matthew] Univ New Mexico, Albuquerque, NM 87131 USA.
[McCall, B.] Alabama A&M Univ, Huntsville, AL 35810 USA.
RP Bolotnikov, AE (reprint author), Brookhaven Natl Lab, Upton, NY 11793 USA.
EM bolotnik@bnl.gov
RI Fochuk, Petro/D-9409-2016; Kopach, Oleh/C-3993-2017;
OI Fochuk, Petro/0000-0002-4149-4882; Kopach, Oleh/0000-0002-1513-5261;
Marshall, Matthew/0000-0002-6440-8713
FU U.S. Department of Energy, Office of Nonproliferation and Verification
Research Development [NA-22]; U.S. Defense Threat Reduction Agency
(DTRA); BNL's Technology Maturation Award; U.S. Department of Energy
[DE-AC02-98CH1-886]
FX This work was supported by U.S. Department of Energy, Office of
Nonproliferation and Verification Research & Development, NA-22, U.S.
Defense Threat Reduction Agency (DTRA) and BNL's Technology Maturation
Award. The manuscript has been authored by Brookhaven Science
Associates, LLC under Contract DE-AC02-98CH1-886 with the U.S.
Department of Energy.
NR 16
TC 3
Z9 3
U1 1
U2 14
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2875
EP 2882
DI 10.1109/TNS.2013.2274054
PN 2
PG 8
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800008
ER
PT J
AU Mandal, KC
Muzykov, PG
Chaudhuri, SK
Terry, JR
AF Mandal, Krishna C.
Muzykov, Peter G.
Chaudhuri, Sandeep K.
Terry, J. Russell
TI Low Energy X-Ray and gamma-Ray Detectors Fabricated on n-Type 4H-SiC
Epitaxial Layer
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Defect delineating etching; epitaxial layer; Schottky barrier detector;
thermally stimulated current (TSC) spectroscopy; x/gamma ray detection
and XRD rocking curve; 4H-SiC
ID SILICON-CARBIDE; SCHOTTKY DIODES; RADIATION DETECTORS
AB Schottky barrier diode (SBD) radiation detectors have been fabricated on n-type 4H-SiC epitaxial layers and evaluated for low energy x- and gamma-rays detection. The detectors were found to be highly sensitive to soft x-rays in the 50 eV to few keV range and showed 2.1 % energy resolution for 59.6 keV gamma rays. The response to soft x-rays for these detectors was significantly higher than that of commercial off-the-shelf (COTS) SiC UV photodiodes. The devices have been characterized by current-voltage (I-V) measurements in the 94-700 K range, thermally stimulated current (TSC) spectroscopy, x-ray diffraction (XRD) rocking curve measurements, and defect delineating chemical etching. I-V characteristics of the detectors at 500 K showed low leakage current (<2 nA at 200 V) revealing a possibility of high temperature operation. The XRD rocking curve measurements revealed high quality of the epitaxial layer exhibiting a full width at half maximum (FWHM) of the rocking curve similar to 3.6 arc sec. TSC studies in a wide range of temperature (94-550 K) revealed presence of relatively shallow levels (similar to 0.25 eV) in the epi bulk with a density similar to 7 x 10(13) cm(-3) related to Al and B impurities and deeper levels located near the metal-semiconductor interface.
C1 [Mandal, Krishna C.; Muzykov, Peter G.; Chaudhuri, Sandeep K.] Univ S Carolina, Dept Elect Engn, Columbia, SC 29208 USA.
[Terry, J. Russell] Los Alamos Natl Lab, Space Sci & Applicat Grp, Intelligence & Space Res Div ISR 1, Los Alamos, NM 87545 USA.
RP Mandal, KC (reprint author), Univ S Carolina, Dept Elect Engn, Columbia, SC 29208 USA.
EM mandalk@cec.sc.edu
FU Los Alamos National Laboratory/DOE [143479]; Advanced Support Program
for Innovative Research Excellence-I (ASPIRE-I) of the University of
South Carolina, Columbia [15530-A401]
FX This work was supported in part by Los Alamos National Laboratory/DOE
(Grant 143479) and the Advanced Support Program for Innovative Research
Excellence-I (ASPIRE-I) of the University of South Carolina, Columbia,
Grant 15530-A401.
NR 25
TC 23
Z9 23
U1 4
U2 21
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2888
EP 2893
DI 10.1109/TNS.2013.2273673
PN 2
PG 6
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800010
ER
PT J
AU Hauf, S
Kuster, M
Batic, M
Bell, ZW
Hoffmann, DHH
Lang, PM
Neff, S
Pia, MG
Weidenspointner, G
Zoglauer, A
AF Hauf, Steffen
Kuster, Markus
Batic, Matej
Bell, Zane W.
Hoffmann, Dieter H. H.
Lang, Philipp M.
Neff, Stephan
Pia, Maria Grazia
Weidenspointner, Georg
Zoglauer, Andreas
TI Radioactive Decays in Geant4
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE ENSDF; Geant4; Monte-Carlo Simulation; radioactive decay; validation
ID ALGEBRAIC APPROACH; EQUATIONS; VALIDATION; SYSTEM
AB The simulation of radioactive decays is a common task in Monte-Carlo systems such as Geant4. Usually, a system either uses an approach focusing on the simulations of every individual decay or an approach which simulates a large number of decays with a focus on correct overall statistics. The radioactive decay package presented in this work permits, for the first time, the use of both methods within the same simulation framework-Geant4. The accuracy of the statistical approach in our new package, RDM-extended, and that of the existing Geant4 per-decay implementation ( original RDM), which has also been refactored, are verified against the ENSDF database. The new verified package is beneficial for a wide range of experimental scenarios, as it enables researchers to choose the most appropriate approach for their Geant4-based application.
C1 [Hauf, Steffen] European XFEL GmbH, Hamburg, Germany.
[Hoffmann, Dieter H. H.; Lang, Philipp M.; Neff, Stephan] Tech Univ Darmstadt, Inst Nucl Sci, Darmstadt, Germany.
[Batic, Matej; Pia, Maria Grazia] Ist Nazl Fis Nucl, I-16146 Genoa, Italy.
[Bell, Zane W.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Weidenspointner, Georg] Max Planck Halbleiter Labor, Munich, Germany.
[Weidenspointner, Georg] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany.
[Zoglauer, Andreas] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA.
RP Hauf, S (reprint author), European XFEL GmbH, Hamburg, Germany.
EM steffen.hauf@xfel.eu
RI Kuster, Markus/C-5742-2014; Pia, Maria Grazia/C-7034-2012;
OI Pia, Maria Grazia/0000-0002-3579-9639; Bell, Zane/0000-0003-1115-8674
FU Deutsches Zentrum fur Luft- und Raumfahrt e.V. (DLR) [50 QR 0902, 50 QR
1102]; Deutsche Zentrum fuer Luft- und Raumfahrt (DLR) [50QR902,
50Q1102]
FX This work has been supported by Deutsches Zentrum fur Luft- und
Raumfahrt e.V. (DLR) under grants 50 QR 0902 and 50 QR 1102.; This work
was supported by the Deutsche Zentrum fuer Luft- und Raumfahrt (DLR)
under Grant number 50QR902 and 50Q1102.
NR 42
TC 7
Z9 7
U1 0
U2 6
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2966
EP 2983
DI 10.1109/TNS.2013.2270894
PN 2
PG 18
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800019
ER
PT J
AU Hauf, S
Kuster, M
Batic, M
Bell, ZW
Hoffmann, DHH
Lang, PM
Neff, S
Pia, MG
Weidenspointner, G
Zoglauer, A
AF Hauf, Steffen
Kuster, Markus
Batic, Matej
Bell, Zane W.
Hoffmann, Dieter H. H.
Lang, Philipp M.
Neff, Stephan
Pia, Maria Grazia
Weidenspointner, Georg
Zoglauer, Andreas
TI Validation of Geant4-Based Radioactive Decay Simulation
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Geant4; high purity germanium detector; radioactive decay; simulation;
validation
ID EFFICIENCY CALIBRATION; ATOMIC RELAXATION; DETECTOR; CODE
AB Radioactive decays are of concern in a wide variety of applications using Monte-Carlo simulations. In order to properly estimate the quality of such simulations, knowledge of the accuracy of the decay simulation is required. We present a validation of the original Geant4 Radioactive Decay Module, which uses a per-decay sampling approach, and of an extended package for Geant4-based simulation of radioactive decays, which, in addition to being able to use a refactored per-decay sampling, is capable of using a statistical sampling approach. The validation is based on measurements of calibration isotope sources using a high purity Germanium (HPGe) detector; no calibration of the simulation is performed. For the considered validation experiment equivalent simulation accuracy can be achieved with per-decay and statistical sampling.
C1 [Hauf, Steffen; Kuster, Markus] European XFEL GmbH, Hamburg, Germany.
[Batic, Matej; Pia, Maria Grazia] Ist Nazl Fis Nucl, I-16146 Genoa, Italy.
[Bell, Zane W.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Hoffmann, Dieter H. H.; Lang, Philipp M.; Neff, Stephan] Tech Univ Darmstadt, Inst Nucl Sci, Darmstadt, Germany.
[Weidenspointner, Georg] Max Planck Halbleiter Labor, Munich, Germany.
[Weidenspointner, Georg] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany.
[Zoglauer, Andreas] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA.
RP Hauf, S (reprint author), European XFEL GmbH, Hamburg, Germany.
EM steffen.hauf@xfel.eu
RI Kuster, Markus/C-5742-2014; Pia, Maria Grazia/C-7034-2012;
OI Pia, Maria Grazia/0000-0002-3579-9639; Bell, Zane/0000-0003-1115-8674
FU Deutsches Zentrum fur Luft- und Raumfahrt e.V. (DLR) [50 QR 0902, 50 QR
1102]
FX This work has been supported by Deutsches Zentrum fur Luft- und
Raumfahrt e.V. (DLR) under grants 50 QR 0902 and 50 QR 1102.
NR 19
TC 6
Z9 6
U1 0
U2 5
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 2984
EP 2997
DI 10.1109/TNS.2013.2271047
PN 2
PG 14
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800020
ER
PT J
AU Alamaniotis, M
Heifetz, A
Raptis, AC
Tsoukalas, LH
AF Alamaniotis, Miltiadis
Heifetz, Alexander
Raptis, Apostolos C.
Tsoukalas, Lefteri H.
TI Fuzzy-Logic Radioisotope Identifier for Gamma Spectroscopy in Source
Search
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Fuzzy logic; maximum likelihood fitting; nuclear detection; radioisotope
identifier; source search
ID RAY SPECTRA; NEURAL-NETWORKS; ISOTOPE IDENTIFICATION; DETECTORS
AB Detection and identification of radioactive nuclear materials in urban searches can be fully performed with a portable gamma ray detector-spectrometer. Due to limited acquisition time and, as a consequence, low signal to noise ratio (SNR), development of fast and accurate real-time radioisotope identifier (RIID) algorithms is essential for automated source detection. In this paper, we evaluate the performance of fuzzy logic real-time radioisotope identification (FL-RIID) in several urban search scenarios. FL-RIID performance is tested on a database of searches consisting of injections of synthetic sources into experimental nuclear background spectra, acquired in one-second time intervals with a moving sodium iodide (NaI) gamma radiation detector-spectrometer. Performance of FL-RIID is benchmarked against that of maximum-likelihood (ML) fitting method. Demonstrated advantages of FL-RIID over ML in search applications include lower false alarm rate and faster execution time.
C1 [Alamaniotis, Miltiadis] Purdue Univ, Sch Nucl Engn, Appl Intelligent Syst Lab, W Lafayette, IN 47907 USA.
[Heifetz, Alexander; Raptis, Apostolos C.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA.
[Tsoukalas, Lefteri H.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA.
RP Alamaniotis, M (reprint author), Univ Utah, Utah Nucl Engn Program, Salt Lake City, UT 84112 USA.
EM miltos.alamaniotis@utah.edu; aheifetz@anl.gov; raptis@anl.gov;
tsoukala@ecn.purdue.edu
FU National Nuclear Security Administration, Office of Non-Proliferation
and Verification, Research and Development [DR-PS52-09NA29330, NA-22]
FX This work was supported in part by the National Nuclear Security
Administration, Office of Non-Proliferation and Verification, Research
and Development (NA-22), under Contract DR-PS52-09NA29330.
NR 27
TC 8
Z9 8
U1 0
U2 5
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 3014
EP 3024
DI 10.1109/TNS.2013.2265307
PN 2
PG 11
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800023
ER
PT J
AU Li, SR
De Geronimo, G
Chen, W
D'Anadragora, A
Fried, J
Li, Z
Pinelli, DA
Smith, GC
Gaskin, JA
Ramsey, BD
AF Li, Shaorui
De Geronimo, Gianluigi
Chen, Wei
D'Anadragora, Alessio
Fried, Jack
Li, Zheng
Pinelli, Donald A.
Smith, Graham C.
Gaskin, Jessica A.
Ramsey, Brian D.
TI A Low-Power, Radiation-Resistant ASIC for SDD-Based X-Ray Spectrometers
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE ASIC; radiation-resistant; SDD; x-ray spectrometer.
ID COMMERCIAL CMOS TECHNOLOGIES; ISOLATION OXIDES; DEGRADATION
AB We present an Application Specific Integrated Circuit (ASIC) for high resolution X-ray spectrometers (XRS) in radiation harsh environment (such as Jovian system). The ASIC was designed to read out signals from low resistivity pixelated Silicon-Drift-Detectors (SDD) to ensure radiation hardness. The readout is done by wire-bonding the anodes to the inputs of the ASIC. The ASIC dissipates 32 mW and provides 16 channels of low-noise charge amplification, high-order shaping with baseline stabilization, discrimination, pile-up rejection, and peak detection with analog memory. The readout is sparse and based on a custom low-power tri-stable low-voltage differential signaling digital interface. A unit of 64 SDD pixels, read out by four ASICs, covers an area of 12.8 cm(2), and dissipates less than 20 mW/cm(2). The ASICs were powered on and irradiated using a beam line with 203 MeV protons, to total doses ranging from 0.25 Mrad to 12 Mrad. Performance degradation due to radiation-induced leakage current was observed to peak around 2 Mrad dose. Critical contributors to the degradation were identified through simulation and measurements, and corresponding circuitry was thus modified to address the issues. Measurements on the radiation-resistant design have shown excellent radiation resistance at total doses ranging from 1 to 8 Mrad.
C1 [Li, Shaorui; De Geronimo, Gianluigi; Chen, Wei; D'Anadragora, Alessio; Fried, Jack; Li, Zheng; Pinelli, Donald A.; Smith, Graham C.] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Gaskin, Jessica A.; Ramsey, Brian D.] NASA, George C Marshall Space Flight Ctr, Huntsville, AL 35812 USA.
RP Li, SR (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA.
EM shaoruili@bnl.gov
FU U.S. Department of Energy [DE-AC02-98CH10886]; NASA Research
Opportunities in Space and Earth Science, Planetary Instrument
Definition and Development Program
FX This work was supported in part by the U.S. Department of Energy under
Contract DE-AC02-98CH10886, and in part by the NASA Research
Opportunities in Space and Earth Science, Planetary Instrument
Definition and Development Program.
NR 13
TC 0
Z9 0
U1 0
U2 7
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 3057
EP 3062
DI 10.1109/TNS.2013.2268980
PN 2
PG 6
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800028
ER
PT J
AU Cates, JW
Hayward, JP
Zhang, X
AF Cates, J. W.
Hayward, J. P.
Zhang, X.
TI Measurement of Achievable Timing Resolution With ZnO:Ga Films
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Achievable timing with scintillators; associated particle imaging; D-T
neutron generator; timing resolution
ID MATERIALS IDENTIFICATION SYSTEM; ALPHA-PARTICLE DETECTORS; NEUTRON
GENERATOR; PHOTOMULTIPLIER SYSTEMS; SCINTILLATORS; PBI2; CDS
AB ZnO:Ga films are attractive phosphors for a number of high energy physics and security applications because of their extremely fast temporal response (typically less than 1 ns). Significant efforts have been undertaken to study the dependence of luminescence properties of ZnO:Ga on dopant constituency and temperature. However, most of these studies simply report the decay time of the phosphor, and there is a lack of published values for measured timing resolution with ZnO:Ga. This work aims to present achievable timing resolution with ZnO:Ga through predictive models and experimentally measured values. Careful characterization of a ZnO:Ga sample's temporal distribution and photosensor response provided inputs for an analytical timing model to predict the timing performance of ZnO:Ga. Additionally, the statistical limit on timing performance is calculated via the Cramer-Rao statistic. The timing performance of a thin-film reference detector is quantified for alpha particle irradiation, and the timing resolution of a ZnO:Ga film is measured against the reference detector. A consistent and precise timestamp from the onset of the rising edge of the ZnO:Ga sample yielded a timing resolution of 52.5 +/- 10.0 ps FWHM was measured for the case of 50 detected photons. Good agreement is shown between measured and predicted timing performance, and the relation to the statistical limit is presented. The reported timing performance for a scintillator with an extremely fast decay but poor light yield has meaningful impact in many areas of study where a fast scintillator is required, including its use in the associated particle detector of a neutron generator to enable multimodal, time-of-flight (TOF) based imaging and TOF Positron Emission Tomography Imaging.
C1 [Cates, J. W.; Hayward, J. P.; Zhang, X.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA.
[Hayward, J. P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Cates, JW (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA.
EM jcates7@utk.edu
FU U.S. Department of Homeland Security, Domestic Nuclear Detection Office
[2010-DN-077-ARI044-02]
FX This work was supported by the U.S. Department of Homeland Security,
Domestic Nuclear Detection Office, under competitively awarded Grant
Award 2010-DN-077-ARI044-02. This support does not constitute an express
or implied endorsement on the part of the Government.
NR 24
TC 1
Z9 1
U1 0
U2 23
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 3127
EP 3133
DI 10.1109/TNS.2013.2272883
PN 2
PG 7
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800036
ER
PT J
AU Feng, PL
Foster, ME
AF Feng, Patrick L.
Foster, Michael E.
TI Pulse-Shape Discrimination in High-Symmetry Organic Scintillators
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Crystals; neutron detection; organic scintillator; pulse-shape
discrimination
ID EXCITATION-ENERGY TRANSFER; FAST-NEUTRON SPECTROMETRY; FLUORESCENCE;
CRYSTALS; SYSTEMS
AB In this work, we report the targeted structural modification of luminescent organic molecules to impart changes to the corresponding molecular and crystallographic symmetries. Fast neutron/gamma pulse-shape discrimination (PSD) has been characterized in high-symmetry organic crystals composed of chromophores that do not intrinsically exhibit PSD. These findings are rationalized in the context of second-rank tensor properties, which are symmetry-dependent factors that control key quantities such as the transport mobility, light yield anisotropy, refractive index, strain, and thermal expansion coefficient. Density-functional theory calculations confirm the role of crystallographic packing and symmetry upon the magnitude of exchange interactions between triplet excited states, as relevant to triplet-triplet annihilation and PSD.
C1 [Feng, Patrick L.; Foster, Michael E.] Sandia Natl Labs, Livermore, CA 94550 USA.
RP Feng, PL (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA.
EM plfeng@sandia.gov
FU office of NA-22, NNSA, U.S. Department of Energy; National Nuclear
Security Administration [DE-AC04-94AL85000]
FX This work was supported by the office of NA-22, NNSA, U.S. Department of
Energy. Sandia National Laboratories is a multi-program laboratory
managed and operated by Sandia Corporation, a wholly owned subsidiary of
Lockheed Martin Corporation, for the National Nuclear Security
Administration under Contract DE-AC04-94AL85000.
NR 26
TC 1
Z9 1
U1 0
U2 11
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2013
VL 60
IS 4
BP 3142
EP 3149
DI 10.1109/TNS.2013.2272893
PN 2
PG 8
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA 205NT
UT WOS:000323451800038
ER
PT J
AU Franz, R
Polcik, P
Anders, A
AF Franz, Robert
Polcik, Peter
Anders, Andre
TI Ion Charge State Distributions of Al and Cr in Cathodic Arc Plasmas from
Composite Cathodes in Vacuum, Argon, Nitrogen, and Oxygen
SO IEEE TRANSACTIONS ON PLASMA SCIENCE
LA English
DT Article
DE AlCr; cathodic arc; composite cathode; ionization; process gas
ID MAGNETIC-FIELD; TEMPORAL DEVELOPMENT; ALLOY CATHODES; GAS-PRESSURE;
EVAPORATION; COATINGS; FLUCTUATIONS; ENVIRONMENT; MECHANISM; TARGETS
AB Multielement cathodes are increasingly used for advanced coatings, yet most cathodic arc plasma measurements have been reported for pure element cathodes. In this contribution, we measure the charge state distributions of aluminum and chromium ions from Al-Cr composite cathodes of different Al to Cr ratios. The arc discharges are pulsed, with pulse duration of around 300 mu s and currents of 175 A, operated at high vacuum and in gases with a pressure of up to 1.3 Pa of Ar, N-2, and O-2. For comparison with literature data, the measurements also included the plasma compositions of discharges using pure Al and Cr cathodes. As expected, the charge distributions are found to be affected by the cathode conditions, the type of gas, and the pressure of the gas into which the arc spot plasma is expanding. Generally, large effects of gas are observed when the pressure exceeded 0.1 Pa, which can be mainly associated with the ions' mean-free path with respect to charge exchange collisions. Differences between ions can be attributed to the energy-and species-dependent charge-exchange cross sections. Considering different cathode compositions, we found that Cr ions tend to have lower charge states from the composite cathodes compared with the pure element cathode, whereas Al ions are relatively unaffected by the cathode composition. Despite the wealth of detailed experimental results, it is difficult to discern trends and rules that could be generalized because measured data involve a convolution of cathode phenomena and gas collisional effects.
C1 [Franz, Robert; Anders, Andre] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Polcik, Peter] PLANSEE Composite Mat GmbH, D-86983 Lechbruck, Germany.
RP Franz, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM rfranz@lbl.gov; peter.polcik@plansee.com; aanders@lbl.gov
RI Franz, Robert/G-5263-2010; Anders, Andre/B-8580-2009
OI Franz, Robert/0000-0003-4842-7276; Anders, Andre/0000-0002-5313-6505
FU E. Schrodinger Program of the Austrian Science Fund (FWF) [J3168-N20]
FX The authors would like to thank the E. Schrodinger Program under Project
J3168-N20 of the Austrian Science Fund (FWF) for their financial
support.
NR 40
TC 7
Z9 7
U1 0
U2 7
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0093-3813
EI 1939-9375
J9 IEEE T PLASMA SCI
JI IEEE Trans. Plasma Sci.
PD AUG
PY 2013
VL 41
IS 8
SI SI
BP 1929
EP 1937
DI 10.1109/TPS.2013.2254135
PN 2
PG 9
WC Physics, Fluids & Plasmas
SC Physics
GA 202JQ
UT WOS:000323211500008
ER
PT J
AU Jiang, RW
Wang, JH
Zhang, MH
Guan, YP
AF Jiang, Ruiwei
Wang, Jianhui
Zhang, Muhong
Guan, Yongpei
TI Two-Stage Minimax Regret Robust Unit Commitment
SO IEEE TRANSACTIONS ON POWER SYSTEMS
LA English
DT Article
DE Benders' decomposition; minimax regret; uncertainty; unit commitment
ID STOCHASTIC SECURITY; WIND POWER; DISCRETE OPTIMIZATION;
LAGRANGIAN-RELAXATION; RISK ANALYSIS; MIN-MAX; SYSTEM; TRANSMISSION;
UNCERTAINTY; GENERATION
AB In addition to long-existing load uncertainty on power systems, continuously increasing renewable energy injections (such as wind and solar) have further made the power grid more volatile and uncertain. Stochastic and recently introduced robust optimization approaches have been studied to provide the day-ahead unit commitment decision with the consideration of real-time load and supply uncertainties. In this paper, we introduce an innovative minimax regret unit commitment model aiming to minimize the maximum regret of the day-ahead decision from the actual realization of the uncertain real-time wind power generation. Our approach will ensure the robustness of the unit commitment decision considering the inherent uncertainty in wind generation. Meanwhile, our approach will provide a system operator a clear picture in terms of the maximum regret value among all possible scenarios. A Benders' decomposition algorithm is developed to solve the problem. Finally, our extensive case studies compare the performances of three different approaches (robust optimization, minimax regret, and stochastic optimization) and verify the effectiveness of our proposed algorithm.
C1 [Jiang, Ruiwei; Guan, Yongpei] Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
[Wang, Jianhui] Argonne Natl Lab, Lemont, IL 60439 USA.
[Zhang, Muhong] Arizona State Univ, Sch Comp Informat & Decis Syst Engn, Tempe, AZ 85281 USA.
RP Jiang, RW (reprint author), Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
EM rwjiang@ufl.edu; jianhui.wang@anl.gov; Muhong.Zhang@asu.edu;
guan@ise.ufl.edu
FU University of Chicago Argonne, LLC, Operator of Argonne National
Laboratory ("Argonne"); Argonne, a U.S. Department of Energy Office of
Science laboratory [DE-AC02-06CH11357]; U.S. National Science Foundation
[ECCS-1202264]
FX This work was supported in part by University of Chicago Argonne, LLC,
Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S.
Department of Energy Office of Science laboratory, is operated under
Contract No. DE-AC02-06CH11357. This work was also supported in part by
the U.S. National Science Foundation under Award ECCS-1202264. Paper no.
TPWRS-00089-2012.
NR 49
TC 52
Z9 54
U1 0
U2 22
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-8950
J9 IEEE T POWER SYST
JI IEEE Trans. Power Syst.
PD AUG
PY 2013
VL 28
IS 3
BP 2271
EP 2282
DI 10.1109/TPWRS.2013.2250530
PG 12
WC Engineering, Electrical & Electronic
SC Engineering
GA 199JD
UT WOS:000322989900023
ER
PT J
AU Wang, QF
Watson, JP
Guan, YP
AF Wang, Qianfan
Watson, Jean-Paul
Guan, Yongpei
TI Two-Stage Robust Optimization for N -k Contingency-Constrained Unit
Commitment
SO IEEE TRANSACTIONS ON POWER SYSTEMS
LA English
DT Article
DE Contingency analysis; N -k security criterion; robust optimization; unit
commitment
ID POWER-SYSTEM
AB This paper proposes a two-stage robust optimization approach to solve the N -k contingency-constrained unit commitment (CCUC) problem. In our approach, both generator and transmission line contingencies are considered. Compared to the traditional approach using a given set of components as candidates for possible failures, our approach considers all possible component failure scenarios. We consider the objectives of minimizing the total generation cost under the worst-case contingency scenario and/or the total pre-contingency cost. We formulate CCUC as a two-stage robust optimization problem and develop a decomposition framework to enable tractable computation. In our framework, the master problem makes unit commitment decisions and the subproblem discovers the worst-case contingency scenarios. By using linearization techniques and duality theory, we transform the subproblem into a mixed-integer linear program (MILP). The most violated inequalities generated from the subproblem are fed back into the master problem during each iteration. Our approach guarantees a globally optimal solution in a finite number of iterations. In reported computational experiments, we test both primal and dual decomposition approaches. Our computational results verify the effectiveness of our proposed approach.
C1 [Wang, Qianfan; Guan, Yongpei] Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
[Watson, Jean-Paul] Sandia Natl Labs, Discrete Math & Complex Syst Dept, Albuquerque, NM 87185 USA.
RP Wang, QF (reprint author), Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
EM jwatson@sandia.gov; guan@ise.ufl.edu
FU Office of Advanced Scientific Computing Research within the Department
of Energy's Office of Science as part of the Complex Interconnected
Distributed Systems program; U.S. Department of Energy's National
Nuclear Security Administration [DE-AC04-94AL85000]
FX This work was supported in part by the Office of Advanced Scientific
Computing Research within the Department of Energy's Office of Science
as part of the Complex Interconnected Distributed Systems program.
Sandia National Laboratories is a multiprogram laboratory managed and
operated by Sandia Corporation, a wholly owned subsidiary of Lockheed
Martin Corporation, for the U.S. Department of Energy's National Nuclear
Security Administration under contract DE-AC04-94AL85000. Paper no.
TPWRS-00207-2012.
NR 24
TC 27
Z9 30
U1 0
U2 12
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-8950
EI 1558-0679
J9 IEEE T POWER SYST
JI IEEE Trans. Power Syst.
PD AUG
PY 2013
VL 28
IS 3
BP 2366
EP 2375
DI 10.1109/TPWRS.2013.2244619
PG 10
WC Engineering, Electrical & Electronic
SC Engineering
GA 199JD
UT WOS:000322989900032
ER
PT J
AU Zhao, CY
Wang, JH
Watson, JP
Guan, YP
AF Zhao, Chaoyue
Wang, Jianhui
Watson, Jean-Paul
Guan, Yongpei
TI Multi-Stage Robust Unit Commitment Considering Wind and Demand Response
Uncertainties
SO IEEE TRANSACTIONS ON POWER SYSTEMS
LA English
DT Article
DE Benders' decomposition; demand response uncertainty; robust
optimization; wind power uncertainty
ID POWER-GENERATION; SECURITY
AB With the increasing penetration of wind power into the power grid, maintaining system reliability has been a challenging issue for ISOs/RTOs, due to the intermittent nature of wind power. In addition to the traditional reserves provided by thermal, hydro, and gas generators, demand response (DR) programs have gained much attention recently as another reserve resource to mitigate wind power output uncertainty. However, the price-elastic demand curve is not exactly known in advance, which provides another dimension of uncertainty. To accommodate the combined uncertainties from wind power and DR, we allow the wind power output to vary within a given interval with the price-elastic demand curve also varying in this paper. We develop a robust optimization approach to derive an optimal unit commitment decision for the reliability unit commitment runs by ISOs/RTOs, with the objective of maximizing total social welfare under the joint worst-case wind power output and demand response scenario. The problem is formulated as a multi-stage robust mixed-integer programming problem. An exact solution approach leveraging Benders' decomposition is developed to obtain the optimal robust unit commitment schedule for the problem. Additional variables are introduced to parameterize the conservatism of our model and avoid over-protection. Finally, we test the performance of the proposed approach using a case study based on the IEEE 118-bus system. The results verify that our proposed approach can accommodate both wind power and demand response uncertainties, and demand response can help accommodate wind power output uncertainty by lowering the unit load cost.
C1 [Zhao, Chaoyue; Guan, Yongpei] Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
[Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Lemont, IL 60439 USA.
[Watson, Jean-Paul; Guan, Yongpei] Sandia Natl Labs, Discrete Math & Complex Syst Dept, Albuquerque, NM 87185 USA.
RP Zhao, CY (reprint author), Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
FU University of Chicago Argonne, LLC, Operator of Argonne National
Laboratory ("Argonne"); U.S. Department of Energy Office of Science
laboratory [DE-AC02-06CH11357]; Office of Advanced Scientific Computing
Research within the Department of Energy's Office of Science; Sandia
National Laboratories; U.S. Department of Energy's National Nuclear
Security Administration [DE-AC04-94AL85000]
FX This work was supported in part by University of Chicago Argonne, LLC,
Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S.
Department of Energy Office of Science laboratory, is operated under
Contract No. DE-AC02-06CH11357. This work was also supported in part by
the Office of Advanced Scientific Computing Research within the
Department of Energy's Office of Science and Sandia National
Laboratories, a multiprogram laboratory managed and operated by Sandia
Corporation, a wholly owned subsidiary of Lockheed Martin Corporation,
for the U.S. Department of Energy's National Nuclear Security
Administration under contract DE-AC04-94AL85000. The preliminary study
of this research is published at the Proceedings of ISERC 2012 with the
title "Two-stage robust optimization for power grid with uncertain
demand response". Paper no. TPWRS-00522-2012.
NR 29
TC 99
Z9 114
U1 3
U2 38
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-8950
J9 IEEE T POWER SYST
JI IEEE Trans. Power Syst.
PD AUG
PY 2013
VL 28
IS 3
BP 2708
EP 2717
DI 10.1109/TPWRS.2013.2244231
PG 10
WC Engineering, Electrical & Electronic
SC Engineering
GA 199JD
UT WOS:000322989900067
ER
PT J
AU Wang, QF
Wang, JH
Guan, YP
AF Wang, Qianfan
Wang, Jianhui
Guan, Yongpei
TI Price-Based Unit Commitment With Wind Power Utilization Constraints
SO IEEE TRANSACTIONS ON POWER SYSTEMS
LA English
DT Article
DE Chance constrains; mixed integer programming; price based unit
commitment; sample average approximation; stochastic programming; wind
power
ID AVERAGE APPROXIMATION METHOD; GENERATION; OPTIMIZATION; MARKETS
AB This paper proposes an optimal bidding strategy for independent power producers (IPPs) in the deregulated electricity market. The IPPs are assumed to be price takers, whose objectives are to maximize their profits considering price and wind power output uncertainties, while ensuring high wind power utilization. The problem is formulated as a two-stage stochastic price-based unit commitment problem with chance constraints to ensure wind power utilization. In our model, the first stage decision includes unit commitment and quantity of electricity submitted to the day-ahead market. The second stage decision includes generation dispatch, actual usage of wind power, and amount of energy imbalance between the day-ahead and real-time markets. The chance constraint is applied to ensure a certain percentage of wind power utilization so as to comply with renewable energy utilization regulations. Finally, a sample average approximation (SAA) approach is applied to solve the problem, and the computational results are reported for the proposed SAA algorithm showing the sensitivity of the total profit as the requirement of wind power utilization changes.
C1 [Wang, Qianfan; Guan, Yongpei] Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
[Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Lemont, IL 60439 USA.
RP Wang, QF (reprint author), Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.
EM qfwang@ufl.edu; jianhui.wang@anl.gov; guan@ise.ufl.edu
FU University of Chicago Argonne, LLC, Operator of Argonne National
Laboratory ("Argonne"); U.S. Department of Energy Office of Science
laboratory [DE-AC02-06CH11357]
FX This work was supported in part by University of Chicago Argonne, LLC,
Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S.
Department of Energy Office of Science laboratory, is operated under
Contract No. DE-AC02-06CH11357. The preliminary two-page abstract of
this paper, entitled "Wind Power Bidding Based on Chance-constrained
Optimization," appears as the summary of an invited panel session
presentation for the IEEE PES General Meeting 2011. Paper no.
TPWRS-00523-2012.
NR 29
TC 25
Z9 26
U1 1
U2 14
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-8950
J9 IEEE T POWER SYST
JI IEEE Trans. Power Syst.
PD AUG
PY 2013
VL 28
IS 3
BP 2718
EP 2726
DI 10.1109/TPWRS.2012.2231968
PG 9
WC Engineering, Electrical & Electronic
SC Engineering
GA 199JD
UT WOS:000322989900068
ER
PT J
AU Marinovici, LD
Lian, JM
Kalsi, K
Du, PW
Elizondo, M
AF Marinovici, Laurentiu Dan
Lian, Jianming
Kalsi, Karanjit
Du, Pengwei
Elizondo, Marcelo
TI Distributed Hierarchical Control Architecture for Transient Dynamics
Improvement in Power Systems
SO IEEE TRANSACTIONS ON POWER SYSTEMS
LA English
DT Article
DE Automatic Generation Control; decentralized robust control; distributed
hierarchical control; frequency restoration
ID AUTOMATIC-GENERATION CONTROL; ROBUST DECENTRALIZED CONTROL; EXCITATION
CONTROL; FEEDBACK; OSCILLATIONS; PERFORMANCE; DESIGN
AB In this paper, a novel distributed hierarchical control architecture is proposed for large-scale power systems. The newly proposed architecture facilitates faster and more accurate frequency restoration during primary frequency control, by providing decentralized robust control to several selected pilot generators in each area. At the local level, these decentralized robust controllers are designed to quickly damp oscillations and restore frequency after large faults and disturbances in the system. Incorporating this supplementary governor control helps the system reach the nominal frequency without necessarily requiring secondary frequency control. Thus, at the area level, automatic generation control (AGC) actions are alleviated in terms of conducting frequency restoration. Moreover, at the area level, AGC coordinates with the decentralized robust controllers to successfully perform tie-line power balancing, while efficiently damping low-frequency inter-area oscillations. The interaction of local and area controllers is validated through detailed simulations.
C1 [Marinovici, Laurentiu Dan; Lian, Jianming; Kalsi, Karanjit; Du, Pengwei] Pacific NW Natl Lab, Richland, WA 99354 USA.
[Elizondo, Marcelo] Pacific NW Natl Lab, Seattle, WA 98109 USA.
RP Marinovici, LD (reprint author), Pacific NW Natl Lab, Richland, WA 99354 USA.
EM Laurentiu.Marinovici@pnnl.gov; Jianming.Lian@pnnl.gov;
Karanjit.Kalsi@pnnl.gov; Pengwei.Du@pnnl.gov; Marcelo.Elizondo@pnnl.gov
FU Future Power Grid Initiative at Pacific Northwest National Laboratory;
U.S. Department of Energy [DE-AC05-76RL01830]
FX This work was supported by the Future Power Grid Initiative at Pacific
Northwest National Laboratory. Pacific Northwest National Laboratory is
operated for the U.S. Department of Energy by Battelle Memorial
Institute under Contract DE-AC05-76RL01830. Paper no. TPWRS-00767-2012.
NR 27
TC 11
Z9 12
U1 1
U2 9
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-8950
J9 IEEE T POWER SYST
JI IEEE Trans. Power Syst.
PD AUG
PY 2013
VL 28
IS 3
BP 3065
EP 3074
DI 10.1109/TPWRS.2012.2236655
PG 10
WC Engineering, Electrical & Electronic
SC Engineering
GA 199JD
UT WOS:000322989900104
ER
PT J
AU Hua, BW
Bie, ZH
Liu, C
Li, GF
Wang, XF
AF Hua, Bowen
Bie, Zhaohong
Liu, Cong
Li, Gengfeng
Wang, Xifan
TI Eliminating Redundant Line Flow Constraints in Composite System
Reliability Evaluation
SO IEEE TRANSACTIONS ON POWER SYSTEMS
LA English
DT Article
DE Composite system reliability; linear programming; optimal power flow;
redundant constraints
ID MONTE-CARLO SIMULATION; POWER-SYSTEMS
AB Reliability evaluation of composite systems involves extensive calculations. Current solutions to this computational burden have mainly focused on extracting failure states from the state space. Instead, the evaluation of failure states is accelerated by methods presented in this paper. The scale of optimizations required for generation redispatching and/or load shedding in failure states is reduced by eliminating redundant line flow constraints.
First, a sufficient and necessary condition for a line flow constraint to be redundant is established in the form of a linear programming problem, based on the concept of steady-state security region (SSR). Then, two redundancy elimination methods are proposed-a conservative one based on a heuristic, and a radical one based on an analytical condition. Numerical tests are conducted on IEEE-RTS79 and a real-life system. More than half of the line flow constraints are eliminated by the conservative method and nearly 90% by the radical method. The proposed methods can be used in conjunction with most of the existing acceleration techniques to further improve efficiency.
C1 [Hua, Bowen; Bie, Zhaohong; Li, Gengfeng; Wang, Xifan] Xi An Jiao Tong Univ, State Key Lab Elect Insulat & Power Equipment, Dept Elect Engn, Xian 710049, Peoples R China.
[Liu, Cong] Argonne Natl Lab, Lemont, IL 60439 USA.
RP Hua, BW (reprint author), Xi An Jiao Tong Univ, State Key Lab Elect Insulat & Power Equipment, Dept Elect Engn, Xian 710049, Peoples R China.
EM zhbie@mail.xjtu.edu.cn
RI Li, Gengfeng/P-7068-2015;
OI Li, Gengfeng/0000-0001-6488-4683; Bie, Zhaohong/0000-0002-8458-0887
FU National High Technology Research and Development Program of China (863
Program) [2012AA050201]
FX Manuscript received October 20, 2012; revised January 13, 2013; accepted
February 15, 2013. Date of publication March 18, 2013; date of current
version July 18, 2013. This work was supported by the National High
Technology Research and Development Program of China (863 Program) under
Grant 2012AA050201. Paper no. TPWRS-01174-2012.
NR 24
TC 2
Z9 4
U1 1
U2 24
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-8950
J9 IEEE T POWER SYST
JI IEEE Trans. Power Syst.
PD AUG
PY 2013
VL 28
IS 3
BP 3490
EP 3498
DI 10.1109/TPWRS.2013.2248762
PG 9
WC Engineering, Electrical & Electronic
SC Engineering
GA 199JD
UT WOS:000322989900148
ER
PT J
AU Hansen, K
Montavon, G
Biegler, F
Fazli, S
Rupp, M
Scheffler, M
von Lilienfeld, OA
Tkatchenko, A
Muller, KR
AF Hansen, Katja
Montavon, Gregoire
Biegler, Franziska
Fazli, Siamac
Rupp, Matthias
Scheffler, Matthias
von Lilienfeld, O. Anatole
Tkatchenko, Alexandre
Mueller, Klaus-Robert
TI Assessment and Validation of Machine Learning Methods for Predicting
Molecular Atomization Energies
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID MIXED-EFFECTS MODELS; NEURAL-NETWORKS; SURFACES; DEEP; RECOGNITION;
REGRESSION; SELECTION; NETS; BIAS
AB The accurate and reliable prediction of properties of molecules typically requires computationally intensive quantum-chemical calculations. Recently, machine learning techniques applied to ab initio calculations have been proposed as an efficient approach for describing the energies of molecules in their given ground-state structure throughout chemical compound space (Rupp et al. Phys. Rev. Lett. 2012, 108, 058301). In this paper we outline a number of established machine learning techniques and investigate the influence of the molecular representation on the methods performance. The best methods achieve prediction errors of 3 kcal/mol for the atomization energies of a wide variety of molecules. Rationales for this performance improvement are given together with pitfalls and challenges when applying machine learning approaches to the prediction of quantum-mechanical observables.
C1 [Hansen, Katja; Scheffler, Matthias; Tkatchenko, Alexandre] Max Planck Gesell, Fritz Haber Inst, Berlin, Germany.
[Montavon, Gregoire; Biegler, Franziska; Fazli, Siamac; Mueller, Klaus-Robert] TU Berlin, Machine Learning Grp, Berlin, Germany.
[Rupp, Matthias] Swiss Fed Inst Technol, Inst Pharmaceut Sci, Zurich, Switzerland.
[von Lilienfeld, O. Anatole] Argonne Natl Lab, Argonne Leadership Comp Facil, Lemont, IL USA.
[Mueller, Klaus-Robert] Korea Univ, Dept Brain & Cognit Engn, Seoul, South Korea.
RP Hansen, K (reprint author), Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, Berlin, Germany.
EM hansen@fhi-berlin.mpg.de; klaus-robert.mueller@tu-berlin.de
RI von Lilienfeld, O. Anatole/D-8529-2011; Scheffler, Matthias/O-4649-2016;
Rupp, Matthias/P-8680-2016; Montavon, Gregoire/Q-1836-2016
OI Rupp, Matthias/0000-0002-2934-2958;
FU European Research Council (ERC); World Class University Program through
the National Research Foundation of Korea; Ministry of Education,
Science, and Technology [R31-10008]; Einstein Foundation; U.S.
Department of Energy, Basic Energy Sciences, Office of Science
[DE-AC02-06CH11357]; Natural Sciences and Engineering Research Council
of Canada; DFG [MU 987/17-1]; FP7 programme of the European Community
[Marie Curie IEF 273039]
FX This work is supported by the European Research Council (ERC Starting
Grant VDW-CMAT), by the World Class University Program through the
National Research Foundation of Korea funded by the Ministry of
Education, Science, and Technology, under Grant R31-10008, the Einstein
Foundation, and by the U.S. Department of Energy, Basic Energy Sciences,
Office of Science, under contract # DE-AC02-06CH11357. The work of
Franziska Biegler is funded, in part, by the Natural Sciences and
Engineering Research Council of Canada. The authors also acknowledge
partial support by DFG (MU 987/17-1). Matthias Rupp acknowledges support
by FP7 programme of the European Community (Marie Curie IEF 273039).
NR 78
TC 57
Z9 57
U1 7
U2 64
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
EI 1549-9626
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD AUG
PY 2013
VL 9
IS 8
BP 3404
EP 3419
DI 10.1021/ct400195d
PG 16
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 202DK
UT WOS:000323193500015
PM 26584096
ER
PT J
AU Ho, MH
Raugei, S
Rousseau, R
Dupuis, M
Bullock, RM
AF Ho, Ming-Hsun
Raugei, Simone
Rousseau, Roger
Dupuis, Michel
Bullock, R. Morris
TI Evaluation of the Role of Water in the H-2 Bond Formation by
Ni(II)-Based Electrocatalysts
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID COUPLED ELECTRON-TRANSFER; DENSITY-FUNCTIONAL THEORY; FREE HYDROGEN
ACTIVATION; FRUSTRATED LEWIS PAIRS; AQUEOUS-SOLUTION; PENDANT AMINES;
SN2 REACTION; ACTIVE-SITE; MOLECULAR CATALYSTS; TRANSITION-METALS
AB We investigate the role of water in the H-H bond formation by a family of nickel molecular catalysts that exhibit high rates for H-2 production in acetonitrile solvent. A key feature leading to the high reactivity is the Lewis acidity of the Ni(II) center and pendant amines in the diphosphine ligand that function as Lewis bases, facilitating H-H bond formation or cleavage. Significant increases in the rate of H-2 production have been reported in the presence of added water. Our calculations show that molecular water can displace an acetonitrile solvent molecule in the first solvation shell of the metal. One or two water molecules can also participate in shuttling a proton that can combine with a metal hydride to form the H-H bond. However the participation of the water molecules does not lower the barrier to H-H bond formation. Thus these calculations suggest that the rate increase due to water in these electrocatalysts is not associated with the elementary step of H-H bond formation or cleavage but rather with the proton delivery steps. We attribute the higher barrier in the H-H bond formation in the presence of water to a decrease in direct interaction between the protic and hydridic hydrogen atoms forced by the water molecules.
C1 [Ho, Ming-Hsun; Raugei, Simone; Rousseau, Roger; Dupuis, Michel; Bullock, R. Morris] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Richland, WA 99352 USA.
RP Raugei, S (reprint author), Pacific NW Natl Lab, Ctr Mol Electrocatalysis, POB 999,K1-83, Richland, WA 99352 USA.
EM simone.raugei@pnnl.gov; michel.dupuis@pnnl.gov
RI Rousseau, Roger/C-3703-2014; Bullock, R. Morris/L-6802-2016
OI Bullock, R. Morris/0000-0001-6306-4851
FU Center for Molecular Electrocatalysis, an Energy Frontier Research
Center; US Department of Energy, Office of Science, Office of Basic
Energy Sciences
FX This research was supported as part of the Center for Molecular
Electrocatalysis, an Energy Frontier Research Center funded by the US
Department of Energy, Office of Science, Office of Basic Energy
Sciences. Computational resources were provided at W. R. Wiley
Environmental Molecular Science Laboratory-Pacific Northwest National
Laboratory, the National Energy Research Scientific Computing Center
(NERSC) at Lawrence Berkeley National Laboratory, and the Jaguar
supercomputer at Oak Ridge National Laboratory.
NR 79
TC 6
Z9 6
U1 1
U2 30
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
EI 1549-9626
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD AUG
PY 2013
VL 9
IS 8
BP 3505
EP 3514
DI 10.1021/ct400396s
PG 10
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 202DK
UT WOS:000323193500026
PM 26584107
ER
PT J
AU Huang, L
Roux, B
AF Huang, Lei
Roux, Benoit
TI Automated Force Field Parameterization for Nonpolarizable and
Polarizable Atomic Models Based on Ab Initio Target Data
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID MOLECULAR-DYNAMICS SIMULATIONS; CLASSICAL DRUDE OSCILLATOR; PARTICLE
MESH EWALD; POTENTIAL FUNCTIONS; VOLTAGE-SENSOR; NUCLEIC-ACIDS;
FREE-ENERGIES; RESP MODEL; WATER; ALGORITHM
AB Classical molecular dynamics (MD) simulations based on atomistic models are increasingly used to study a wide range of biological systems. A prerequisite for meaningful results from such simulations is an accurate molecular mechanical force field. Most biomolecular simulations are currently based on the widely used AMBER and CHARMM force fields, which were parametrized and optimized to cover a small set of basic compounds corresponding to the natural amino acids and nucleic acid bases. Atomic models of additional compounds are commonly generated by analogy to the parameter set of a given force field. While this procedure yields models that are internally consistent, the accuracy of the resulting models can be limited. In this work, we propose a method, general automated atomic model parameterization (GAAMP), for generating automatically the parameters of atomic models of small molecules using the results from ab initio quantum mechanical (QM) calculations as target data. Force fields that were previously developed for a wide range of model compounds serve as initial guesses, although any of the final parameter can be optimized. The electrostatic parameters (partial charges, polarizabilities, and shielding) are optimized on the basis of QM electrostatic potential (ESP) and, if applicable, the interaction energies between the compound and water molecules. The soft dihedrals are automatically identified and parametrized by targeting QM dihedral scans as well as the energies of stable conformers. To validate the approach, the solvation free energy is calculated for more than 200 small molecules and MD simulations of three different proteins are carried out.
C1 [Huang, Lei; Roux, Benoit] Univ Chicago, Dept Biochem & Mol Biol, Chicago, IL 60637 USA.
[Roux, Benoit] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA.
RP Roux, B (reprint author), Univ Chicago, Dept Biochem & Mol Biol, 929 East 57th St, Chicago, IL 60637 USA.
EM roux@uchicago.edu
FU NIH/NIGMS [U54-GM087519]; Argonne National Laboratory through NIH [S10
RR029030-0]
FX We thank Drs. Alexander D. MacKerell Jr., Christopher N. Rowley,
Janamejaya Chowdhary, James Gumbart, Haibo Yu, Yen-tin Lin, and Yilin
Meng for valuable discussions. We thank Allen Zhu for preparing the
molecule structures for 17 UAAs. We are grateful to two referees for
their insightful comments and suggestions. This work was supported by
NIH/NIGMS through grant U54-GM087519 and was carried out in the context
of the Membrane Protein Structural Dynamics Consortium. The computations
were made possible by the resources provided by the Computation
Institute and the Biological Sciences Division of the University of
Chicago and Argonne National Laboratory through NIH Grant S10
RR029030-0.
NR 65
TC 51
Z9 51
U1 2
U2 43
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD AUG
PY 2013
VL 9
IS 8
BP 3543
EP 3556
DI 10.1021/ct4003477
PG 14
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 202DK
UT WOS:000323193500030
ER
PT J
AU Bea, SA
Wainwright, H
Spycher, N
Faybishenko, B
Hubbard, SS
Denham, ME
AF Bea, Sergio A.
Wainwright, Haruko
Spycher, Nicolas
Faybishenko, Boris
Hubbard, Susan S.
Denham, Miles E.
TI Identifying key controls on the behavior of an acidic-U(VI) plume in the
Savannah River Site using reactive transport modeling
SO JOURNAL OF CONTAMINANT HYDROLOGY
LA English
DT Article
DE Reactive transport modeling; Acidic plume; Vadose zone; Richards
equation; Uranium; Surface complexation modeling; Reactive facies;
Uncertainty quantification; ASCEM
ID VARIABLE CHEMICAL CONDITIONS; SURFACE COMPLEXATION; URANIUM(VI)
ADSORPTION; CONTAMINATED GROUNDWATER; FACILITATED TRANSPORT;
POROUS-MEDIA; WATER; AQUIFER; MIGRATION; KINETICS
AB Acidic low-level waste radioactive waste solutions were discharged to three unlined seepage basins at the F-Area of the Department of Energy (DOE) Savannah River Site (SRS), South Carolina, USA, from 1955 through 1989. Despite many years of active remediation, the groundwater remains acidic and contaminated with significant levels of U(VI) and other radionuclides. Monitored Natural Attenuation (MNA) is a desired closure strategy for the site, based on the premise that regional flow of dean background groundwater will eventually neutralize the groundwater acidity, immobilizing U(VI) through adsorption. An in situ treatment system is currently in place to accelerate this in the downgradient portion of the plume and similar measures could be taken upgradient if necessary. Understanding the long-term pH and U(VI) adsorption behavior at the site is critical to assess feasibility of MNA along with the in-situ remediation treatments. This paper presents a reactive transport (RT) model and uncertainty quantification (UQ) analyses to explore key controls on the U(VI)-plume evolution and long-term mobility at this site. Two-dimensional numerical RT simulations are run including the saturated and unsaturated (vadose) zones, U(VI) and H+ adsorption (surface complexation) onto sediments, dissolution and precipitation of Al and Fe minerals, and key hydrodynamic processes are considered. UQ techniques are applied using a new open-source tool that is part of the developing ASCEM reactive transport modeling and analysis framework to: (1) identify the complex physical and geochemical processes that control the U(VI) plume migration in the pH range where the plume is highly mobile, (2) evaluate those physical and geochemical parameters that are most controlling, and (3) predict the future plume evolution constrained by historical, chemical and hydrological data. The RT simulation results show a good agreement with the observed historical pH and concentrations of U(VI), nitrates and Al concentrations at multiple locations. Mineral dissolution and precipitation combined with adsorption reactions on goethite and kaolinite (the main minerals present with quartz) could buffer pH at the site for long periods of time. UQ analysis using the Morris one-at-a-time (OAT) method indicates that the model/parameter is most sensitive to the pH of the waste solution, discharge rates, and the reactive surface area available for adsorption. However, as a key finding, UQ analysis also indicates that this model (and parameters) sensitivity evolves in space and time, and its understanding could be crucial to assess the temporal efficiency of a remediation strategy in contaminated sites. Results also indicate that residual U(VI) and H+ adsorbed in the vadose zone, as well as aquifer permeability, could have a significant impact on the acidic plume long-term mobility. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Bea, Sergio A.; Wainwright, Haruko; Spycher, Nicolas; Faybishenko, Boris; Hubbard, Susan S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Denham, Miles E.] Savannah River Natl Lab, Aiken, SC 29808 USA.
RP Bea, SA (reprint author), CONICET IHLLA, Republ Italia 730, RA-7300 Azul, BA, Argentina.
EM SABea@lbl.gov; HMWainwright@lbl.gov; NSpycher@lbl.gov;
BFaybishenko@lbl.gov; SSHubbard@lbl.gov; MILES.Denham@srnl.doe.gov
RI Bea, Sergio /A-9056-2012; Wainwright, Haruko/A-5670-2015; Hubbard,
Susan/E-9508-2010; Spycher, Nicolas/E-6899-2010; Faybishenko,
Boris/G-3363-2015
OI Bea, Sergio /0000-0001-9237-4103; Wainwright,
Haruko/0000-0002-2140-6072; Faybishenko, Boris/0000-0003-0085-8499
FU Subsurface Science Scientific Focus Area (SFA); U.S. Department of
Energy, Office of Science, Office of Biological and Environmental
Research [DE-AC02-05CH11231]; U.S. Department of Energy Environmental
Management [DE-AC02-05CH11231]
FX This study was supported as part of the Subsurface Science Scientific
Focus Area (SFA) funded by the U.S. Department of Energy, Office of
Science, Office of Biological and Environmental Research to the
Sustainable Systems SFA and by the ASCEM project, which is supported by
U.S. Department of Energy Environmental Management both under award
number DE-AC02-05CH11231 to the LBNL. We sincerely thank Greg Flach
(Savannah River National Laboratory) for the support in developing the
site conceptual model and for providing the concentration data used in
this study.
NR 80
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0169-7722
J9 J CONTAM HYDROL
JI J. Contam. Hydrol.
PD AUG
PY 2013
VL 151
BP 34
EP 54
DI 10.1016/j.jconhyd.2013.04.005
PG 21
WC Environmental Sciences; Geosciences, Multidisciplinary; Water Resources
SC Environmental Sciences & Ecology; Geology; Water Resources
GA 204XF
UT WOS:000323403900003
PM 23707874
ER
PT J
AU Chen, MJ
Abriola, LM
Amos, BK
Suchomel, EJ
Pennell, KD
Loeffler, FE
Christ, JA
AF Chen, Mingjie
Abriola, Linda M.
Amos, Benjamin K.
Suchomel, Eric J.
Pennell, Kurt D.
Loeffler, Frank E.
Christ, John A.
TI Microbially enhanced dissolution and reductive dechlorination of PCE by
a mixed culture: Model validation and sensitivity analysis
SO JOURNAL OF CONTAMINANT HYDROLOGY
LA English
DT Article
DE PCE; NAPL; Enhanced dissolution; Modeling; Model verification; Reductive
dechlorination
ID NONAQUEOUS PHASE LIQUID; SATURATED SUBSURFACE SYSTEMS; MASS-TRANSFER
RATES; IN-SOURCE ZONES; TETRACHLOROETHENE DNAPL; FIELD-EVALUATION;
COMPETITION; KINETICS; BIOAUGMENTATION; BIODEGRADATION
AB Reductive dechlorination catalyzed by organohalide-respiring bacteria is often considered for remediation of non-aqueous phase liquid (NAPL) source zones due to cost savings, ease of implementation, regulatory acceptance, and sustainability. Despite knowledge of the key dechlorinators, an understanding of the processes and factors that control NAPL dissolution rates and detoxification (i.e., ethene formation) is lacking. A recent column study demonstrated a 5-fold cumulative enhancement in tetrachloroethene (PCE) dissolution and ethene formation (Amos et al., 2009). Spatial and temporal monitoring of key geochemical and microbial (i.e., Geobacter lovleyi and Dehalococcoides mccartyi strains) parameters in the column generated a data set used herein as the basis for refinement and testing of a multiphase, compositional transport model. The refined model is capable of simulating the reactive transport of multiple chemical constituents produced and consumed by organohalide-respiring bacteria and accounts for substrate limitations and competitive inhibition. Parameter estimation techniques were used to optimize the values of sensitive microbial kinetic parameters, including maximum utilization rates, biomass yield coefficients, and endogenous decay rates. Comparison and calibration of model simulations with the experimental data demonstrate that the model is able to accurately reproduce measured effluent concentrations, while delineating trends in dechlorinator growth and reductive dechlorination kinetics along the column. Sensitivity analyses performed on the optimized model parameters indicate that the rates of PCE and cis-1,2-dichloroethene (cis-DCE) transformation and Dehalococcoides growth govern bioenhanced dissolution, as long as electron donor (i.e., hydrogen flux) is not limiting. Dissolution enhancements were shown to be independent of cis-DCE accumulation; however, accumulation of cis-DCE, as well as column length and flow rate (i.e., column residence time), strongly influenced the extent of reductive dechlorination. When cis-DCE inhibition was neglected, the model over-predicted ethene production ten-fold, while reductions in residence time (i.e., a two-fold decrease in column length or two-fold increase in flow rate) resulted in a more than 70% decline in ethene production. These results suggest that spatial and temporal variations in microbial community composition and activity must be understood to model, predict, and manage bioenhanced NAPL dissolution. Published by Elsevier B.V.
C1 [Chen, Mingjie] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA.
[Abriola, Linda M.; Pennell, Kurt D.] Tufts Univ, Dept Civil & Environm Engn, Medford, MA 02155 USA.
[Amos, Benjamin K.] Geosyntec Consultants, Kennesaw, GA 30144 USA.
[Suchomel, Eric J.] Geosyntec Consultants, San Francisco, CA 94105 USA.
[Loeffler, Frank E.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA.
[Loeffler, Frank E.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA.
[Loeffler, Frank E.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA.
[Christ, John A.] US Air Force Acad, Dept Civil & Environm Engn, Colorado Springs, CO 80840 USA.
RP Christ, JA (reprint author), USAF Acad, Dept Civil & Environm Engn, 2354 Fairchild Dr,Suite 6J-159, Colorado Springs, CO 80840 USA.
EM john.christ@usafa.edu
RI Loeffler, Frank/M-8216-2013; Pennell, Kurt/F-6862-2010
OI Pennell, Kurt/0000-0002-5788-6397
FU Strategic Environmental Research and Development Program (SERDP)
[W912HQ-04-0006, ER-1293, W91HQ-08-C-0003, ER-1612, W912HQ-13-C-0011,
ER-2311]
FX This research was supported by the Strategic Environmental Research and
Development Program (SERDP) under contract W912HQ-04-0006 (Project
ER-1293), contract W91HQ-08-C-0003 (Project ER-1612), and contract
W912HQ-13-C-0011 (Project ER-2311). This content of this manuscript has
not been subject to agency review and does not necessarily represent the
view of the agency sponsor.
NR 61
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0169-7722
J9 J CONTAM HYDROL
JI J. Contam. Hydrol.
PD AUG
PY 2013
VL 151
BP 117
EP 130
DI 10.1016/j.jconhyd.2013.05.005
PG 14
WC Environmental Sciences; Geosciences, Multidisciplinary; Water Resources
SC Environmental Sciences & Ecology; Geology; Water Resources
GA 204XF
UT WOS:000323403900009
PM 23774611
ER
PT J
AU Szecsody, JE
Truex, MJ
Qafoku, NP
Wellman, DM
Resch, T
Zhong, LR
AF Szecsody, Jim E.
Truex, Mike J.
Qafoku, Nikolla P.
Wellman, Dawn M.
Resch, Tom
Zhong, Lirong
TI Influence of acidic and alkaline waste solution properties on uranium
migration in subsurface sediments
SO JOURNAL OF CONTAMINANT HYDROLOGY
LA English
DT Article
DE Uranium; Subsurface contamination; Acidic waste; Alkaline waste; Uranium
dissolution/precipitation; Uranium adsorption
ID HANFORD TANK WASTE; VADOSE ZONE; CONTAMINATED SEDIMENTS; CANCRINITE;
DISSOLUTION; EXTRACTION; SODALITE; PRECIPITATION; NITRATE; SOILS
AB This study shows that acidic and alkaline wastes co-disposed with uranium into subsurface sediments have significant impact on changes in uranium retardation, concentration, and mass during downward migration. For uranium co-disposal with acidic wastes, significant rapid (i.e., hours) carbonate and slow (i.e., 100 s of hours) clay dissolution resulted, releasing significant sediment-associated uranium, but the extent of uranium release and mobility change was controlled by the acid mass added relative to the sediment proton adsorption capacity. Mineral dissolution in acidic solutions (pH 2) resulted in a rapid (<10 h) increase in aqueous carbonate (with Ca2+, Mg2+) and phosphate and a slow (100 s of hours) increase in silica, Al3+, and K+, likely from 2:1 clay dissolution. Infiltration of uranium with a strong acid resulted in significant shallow uranium mineral dissolution and deeper uranium precipitation (likely as phosphates and carbonates) with downward uranium migration of three times greater mass at a faster velocity relative to uranium infiltration in pH neutral groundwater. In contrast, mineral dissolution in an alkaline environment (pH 13) resulted in a rapid (<10 h) increase in carbonate, followed by a slow (10 s to 100 s of hours) increase in silica concentration, likely from montmorillonite, muscovite, and kaolinite dissolution. Infiltration of uranium with a strong base resulted in not only uranium-silicate precipitation (presumed Na-boltwoodite) but also desorption of natural uranium on the sediment due to the high ionic strength solution, or 60% greater mass with greater retardation compared with groundwater. Overall, these results show that acidic or alkaline co-contaminant disposal with uranium can result in complex depth- and time-dependent changes in uranium dissolution/precipitation reactions and uranium sorption, which alter the uranium migration mass, concentration, and velocity. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Szecsody, Jim E.; Truex, Mike J.; Qafoku, Nikolla P.; Wellman, Dawn M.; Resch, Tom; Zhong, Lirong] Pacific NW Natl Lab, Richland, WA 99354 USA.
RP Szecsody, JE (reprint author), Pacific NW Natl Lab, POB 999,MSIN K3-61, Richland, WA 99354 USA.
EM jim.szecsody@pnnl.gov; mj.truex@pnnl.gov; Nik.Qafoku@pnnl.gov;
Dawn.Wellman@pnnl.gov; Tom.Resch@pnnl.gov; Lirong.Zhong@pnnl.gov
OI Qafoku, Nikolla P./0000-0002-3258-5379
FU U.S. Department of Energy Office of Environmental Management; Richland
Operations Office; Department of Energy (DOE) [DE-AC05-76RL01830]
FX Funding for this work was provided by the U.S. Department of Energy
Office of Environmental Management and Richland Operations Office. The
Pacific Northwest National Laboratory is operated by Battelle Memorial
Institute for the Department of Energy (DOE) under Contract
DE-AC05-76RL01830.
NR 47
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U1 1
U2 40
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0169-7722
J9 J CONTAM HYDROL
JI J. Contam. Hydrol.
PD AUG
PY 2013
VL 151
BP 155
EP 175
DI 10.1016/j.jconhyd.2013.05.009
PG 21
WC Environmental Sciences; Geosciences, Multidisciplinary; Water Resources
SC Environmental Sciences & Ecology; Geology; Water Resources
GA 204XF
UT WOS:000323403900012
PM 23851265
ER
PT J
AU Rau, P
Steinheimer, J
Schramm, S
Stocker, H
AF Rau, P.
Steinheimer, J.
Schramm, S.
Stoecker, H.
TI Chiral hadronic mean field model including quark degrees of freedom
SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS
LA English
DT Article
ID HEAVY-ION COLLISIONS; EQUATION-OF-STATE; PHASE-TRANSITION; GLUON PLASMA;
NUCLEAR-MATTER; FINITE-TEMPERATURE; LATTICE QCD; ELLIPTIC FLOW;
THERMODYNAMICS; COLLABORATION
AB In an approach inspired by Polyakov loop extended Nambu-Jona-Lasinio models, we present a nonlinear hadronic SU(3) sigma-omega mean field model augmented by quark degrees of freedom. By introducing the effective Polyakov loop related scalar field Phi and an associated effective potential, the model includes all known hadronic degrees of freedom at low temperatures and densities as well as a quark phase at high temperatures and densities. Hadrons in the model exhibit a finite volume in order to suppress baryons at high T and mu. This ensures that the right asymptotic degrees of freedom are attained for the description of strongly interacting matter and allows one to study the QCD phase diagram in a wide range of temperatures and chemical potentials. Therefore, with this model it is possible to study the phase transition of chiral restoration and deconfinement. In this paper, the impact of quarks on the resulting phase diagram is shown. The results from the chiral model are compared with recent data from lattice QCD.
C1 [Rau, P.; Schramm, S.; Stoecker, H.] Goethe Univ Frankfurt, Inst Theoret Phys, D-60438 Frankfurt, Germany.
[Rau, P.; Schramm, S.] FIAS, D-60438 Frankfurt, Germany.
[Steinheimer, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Stoecker, H.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany.
RP Rau, P (reprint author), Goethe Univ Frankfurt, Inst Theoret Phys, Max von Laue Str 1, D-60438 Frankfurt, Germany.
EM rau@th.physik.uni-frankfurt.de
RI Stoecker, Horst/D-6173-2013; Stoecker, Horst/F-8382-2012
OI Stoecker, Horst/0000-0002-3282-3664; Stoecker, Horst/0000-0002-3282-3664
FU BMBF; GSI; Hessian excellence initiative LOEWE (Landesoffensive zur
Entwicklung Wissenschaftlich-okonomischer Exzellenz) through the
Helmholtz International Center for FAIR (HIC for FAIR); Helmholtz
Graduate School for Hadron and Ion Research (HGS-HIRe); Feodor Lynen
fellowship of the Alexander von Humboldt foundation
FX This work was supported by BMBF, GSI, and by the Hessian excellence
initiative LOEWE (Landesoffensive zur Entwicklung
Wissenschaftlich-okonomischer Exzellenz) through the Helmholtz
International Center for FAIR (HIC for FAIR), and the Helmholtz Graduate
School for Hadron and Ion Research (HGS-HIRe). Computational resources
were provided by the Center for the Scientific Computing (CSC) of the
Goethe University Frankfurt. JS acknowledges a Feodor Lynen fellowship
of the Alexander von Humboldt foundation. The authors thank M Bleicher
for fruitful discussion.
NR 95
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U1 0
U2 4
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0954-3899
EI 1361-6471
J9 J PHYS G NUCL PARTIC
JI J. Phys. G-Nucl. Part. Phys.
PD AUG
PY 2013
VL 40
IS 8
AR 085001
DI 10.1088/0954-3899/40/8/085001
PG 22
WC Physics, Nuclear; Physics, Particles & Fields
SC Physics
GA 200JE
UT WOS:000323063900002
ER
PT J
AU Wandkowsky, N
Drexlin, G
Frankle, FM
Gluck, F
Groh, S
Mertens, S
AF Wandkowsky, N.
Drexlin, G.
Fraenkle, F. M.
Glueck, F.
Groh, S.
Mertens, S.
TI Validation of a model for radon-induced background processes in
electrostatic spectrometers
SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS
LA English
DT Article
ID RUNGE-KUTTA METHODS; DOUBLE-BETA DECAY; CROSS-SECTIONS; ALPHA-DECAY;
IMPACT IONIZATION; NEUTRINO MASS; ELECTRONS; KATRIN; SCATTERING;
MOLECULES
AB The Karlsruhe Tritium Neutrino (KATRIN) experiment investigating tritium beta-decay close to the endpoint with unprecedented precision has stringent requirements on the background level of less than 10(-2) counts per second. Electron emission during the alpha-decay of Rn-219,Rn-220 atoms in the electrostatic spectrometers of KATRIN is a serious source of background exceeding this limit. In this paper we compare extensive simulations of Rn-induced background to specific measurements with the KATRIN pre-spectrometer to fully characterize the observed Rn-background rates and signatures and determine generic Rn emanation rates from the pre-spectrometer bulk material and its vacuum components.
C1 [Wandkowsky, N.; Drexlin, G.; Fraenkle, F. M.; Glueck, F.; Groh, S.; Mertens, S.] Karlsruhe Inst Technol, KCETA, D-76131 Karlsruhe, Germany.
[Fraenkle, F. M.] Univ N Carolina, Dept Phys, Chapel Hill, NC USA.
[Glueck, F.] Res Inst Nucl & Particle Phys, Theory Dep, Budapest, Hungary.
[Mertens, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Inst Nucl & Particle Astrophys, Berkeley, CA 94720 USA.
RP Wandkowsky, N (reprint author), Karlsruhe Inst Technol, KCETA, D-76131 Karlsruhe, Germany.
EM nancy.wandkowsky@kit.edu
FU Bundesministerium fur Bildung und Forschung (BMBF) [05A08VK2]; Deutsche
Forschungsgemeinschaft (DFG) [Transregio 27]; Karlsruhe House of Young
Scientists (KHYS) of KIT
FX This work has been supported by the Bundesministerium fur Bildung und
Forschung (BMBF) with project number 05A08VK2 and the Deutsche
Forschungsgemeinschaft (DFG) via Transregio 27 'Neutrinos and beyond'.
We also would like to thank the Karlsruhe House of Young Scientists
(KHYS) of KIT for their support (SG, SM, NW).
NR 57
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U1 0
U2 1
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0954-3899
J9 J PHYS G NUCL PARTIC
JI J. Phys. G-Nucl. Part. Phys.
PD AUG
PY 2013
VL 40
IS 8
AR 085102
DI 10.1088/0954-3899/40/8/085102
PG 18
WC Physics, Nuclear; Physics, Particles & Fields
SC Physics
GA 200JE
UT WOS:000323063900008
ER
PT J
AU Olson, IC
Metzler, RA
Tamura, N
Kunz, M
Killian, CE
Gilbert, PUPA
AF Olson, Ian C.
Metzler, Rebecca A.
Tamura, Nobumichi
Kunz, Martin
Killian, Christopher E.
Gilbert, Pupa U. P. A.
TI Crystal lattice tilting in prismatic calcite
SO JOURNAL OF STRUCTURAL BIOLOGY
LA English
DT Article
DE Biomineral; Mollusca; PIC-mapping; PEEM; Mesocrystal; Nanocrystal;
Hardness
ID RAY-ABSORPTION SPECTROSCOPY; MOLLUSK SHELL NACRE;
PINCTADA-MARGARITIFERA; ATRINA-RIGIDA; ORIENTED ATTACHMENT;
PINNA-NOBILIS; RED ABALONE; X-PEEM; CARBONATE; ORIENTATION
AB We analyzed the calcitic prismatic layers in Atrina rigida (Ar), Haliotis iris (Hi), Haliotis laevigata (HL), Haliotis rufescens (Hrf), Mytilus californianus (Mc), Pinctada fucata (Pf), Pinctada margaritifera (Pm) shells, and the aragonitic prismatic layer in the Nautilus pompilius (Np) shell. Dramatic structural differences were observed across species, with 100-mu m wide single-crystalline prisms in Hi, HL and Hrf, 1-mu m wide needle-shaped calcite prisms in Mc, 1-mu m wide spherulitic aragonite prisms in Np, 20-mu m wide single-crystalline calcite prisms in Ar, and 20-mu m wide polycrystalline calcite prisms in Pf and Pm. The calcite prisms in Pf and Pm are subdivided into sub-prismatic domains of orientations, and within each of these domains the calcite crystal lattice tilts gradually over long distances, on the order of 100 mu m, with an angle spread of crystal orientation of 10-20 degrees. Furthermore, prisms in Pf and Pm are harder than in any other calcite prisms analyzed, their nanoparticles are smaller, and the angle spread is strongly correlated with hardness in all shells that form calcitic prismatic layers. One can hypothesize a causal relationship of these correlated parameters: greater angle spread may confer greater hardness and resistance to wear, thus providing Pf and Pm with a structural advantage in their environment. This is the first structure-property relationship thus far hypothesized in mollusk shell prisms. (c) 2013 Elsevier Inc. All rights reserved.
C1 [Olson, Ian C.; Killian, Christopher E.; Gilbert, Pupa U. P. A.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA.
[Metzler, Rebecca A.] Colgate Univ, Dept Phys & Astron, Hamilton, NY 13346 USA.
[Tamura, Nobumichi; Kunz, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Gilbert, Pupa U. P. A.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA.
RP Gilbert, PUPA (reprint author), Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53706 USA.
EM pupa@physics.wisc.edu
FU NSF [DMR-1105167, EAR-103979]; DOE [DE-FG02-07ER15899,
DE-AC02-05CH11231]
FX We are grateful to an anonymous reviewer for requiring the Hall-Petch
plot in Fig. 7B. We thank Robert O. Ritchie for discussions. We thank
ALS beamline scientists Andreas Scholl and Anthony Young for their
technical support during the PEEM-3 experiments, and Richard Celestre
for help during shell sample preparation. This work was supported by NSF
award DMR-1105167, and DOE Award DE-FG02-07ER15899 to PUPAG, and by NSF
award EAR-103979 to RAM. The experiments were performed at the Berkeley
Advanced Light Source, supported by DOE under contract
DE-AC02-05CH11231.
NR 94
TC 21
Z9 21
U1 5
U2 71
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 1047-8477
J9 J STRUCT BIOL
JI J. Struct. Biol.
PD AUG
PY 2013
VL 183
IS 2
BP 180
EP 190
DI 10.1016/j.jsb.2013.06.006
PG 11
WC Biochemistry & Molecular Biology; Biophysics; Cell Biology
SC Biochemistry & Molecular Biology; Biophysics; Cell Biology
GA 204XU
UT WOS:000323405400009
PM 23806677
ER
PT J
AU Strelcov, E
Kim, Y
Jesse, S
Cao, Y
Ivanov, IN
Kravchenko, II
Wang, CH
Teng, YC
Chen, LQ
Chu, YH
Kalinin, SV
AF Strelcov, Evgheni
Kim, Yunseok
Jesse, Stephen
Cao, Ye
Ivanov, Ilia N.
Kravchenko, Ivan I.
Wang, Chih-Hung
Teng, Yung-Chun
Chen, Long-Qing
Chu, Ying Hao
Kalinin, Sergei V.
TI Probing Local Ionic Dynamics in Functional Oxides at the Nanoscale
SO NANO LETTERS
LA English
DT Article
DE SPM; ionic dynamics; Ca-BFO; voltage spectroscopy; oxygen vacancy;
FORC-IV
ID PIEZORESPONSE FORCE MICROSCOPY; ACTIVATION-ENERGY; TRANSPORT; DIFFUSION;
FERROELECTRICS; POLARIZATION; SPECTROSCOPY; CHALLENGES; PROSPECTS;
PHYSICS
AB A scanning probe microscopy technique for probing local ionic dynamics in electrochemically active materials based on the first-order reversal curve current-voltage (FORC-IV) method is presented. FORC-IV imaging mode is applied to a Ca-substituted bismuth ferrite (Ca-BFO) system to separate the electronic and ionic phenomena in this material and visualize the spatial variability of these behaviors. The variable-temperature measurements further demonstrate the interplay between the thermally and electric-field-driven resistance changes in Ca-BFO. The FORC-IV is shown to be a simple, powerful, and flexible method for studying electrochemical activity of materials at the nanoscale and, in conjunction with the electrochemical strain microscopy, it can be used for differentiating ferroelectric and ionic behaviors.
C1 [Strelcov, Evgheni; Kim, Yunseok; Jesse, Stephen; Ivanov, Ilia N.; Kravchenko, Ivan I.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Wang, Chih-Hung; Teng, Yung-Chun; Chu, Ying Hao] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan.
[Cao, Ye; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA.
[Kim, Yunseok] Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, Suwon 440746, Gyeonggi Do, South Korea.
RP Strelcov, E (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM strelcove@ornl.gov; sergei2@ornl.gov
RI Ying-Hao, Chu/A-4204-2008; Strelcov, Evgheni/H-1654-2013; Chen,
LongQing/I-7536-2012; ivanov, ilia/D-3402-2015; Kravchenko,
Ivan/K-3022-2015; Kalinin, Sergei/I-9096-2012; Jesse,
Stephen/D-3975-2016; Cao, Ye/L-1271-2016
OI Ying-Hao, Chu/0000-0002-3435-9084; Chen, LongQing/0000-0003-3359-3781;
ivanov, ilia/0000-0002-6726-2502; Kravchenko, Ivan/0000-0003-4999-5822;
Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483;
Cao, Ye/0000-0002-7365-7447
FU Scientific User Facilities Division, Office of Basic Energy Sciences,
U.S. Department of Energy; National Science Council of Republic of China
[NSC-101-2119-M-009-003-MY2]; Ministry of Education [MOE-ATU 101W961];
Center for Interdisciplinary Science at National Chiao Tung University
FX A part of this research was conducted at the Center for Nanophase
Materials Sciences, which is sponsored at Oak Ridge National Laboratory
by the Scientific User Facilities Division, Office of Basic Energy
Sciences, U.S. Department of Energy. The work in National Chiao Tung
University was supported by the National Science Council of Republic of
China (under contract No. NSC-101-2119-M-009-003-MY2), Ministry of
Education (Grant MOE-ATU 101W961), and Center for Interdisciplinary
Science at National Chiao Tung University.
NR 54
TC 25
Z9 25
U1 4
U2 128
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3455
EP 3462
DI 10.1021/nl400780d
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000002
PM 23865960
ER
PT J
AU Berciaud, S
Li, XL
Htoon, H
Brus, LE
Doorn, SK
Heinz, TF
AF Berciaud, Stephane
Li, Xianglong
Htoon, Han
Brus, Louis E.
Doorn, Stephen K.
Heinz, Tony F.
TI Intrinsic Line Shape of the Raman 2D-Mode in Freestanding Graphene
Monolayers
SO NANO LETTERS
LA English
DT Article
DE Graphene; Raman spectroscopy; 2D-mode; multiphonon resonant Raman
scattering; electrostatic doping; freestanding graphene
ID SPECTROSCOPY; SCATTERING; GRAPHITE; LAYER
AB We report a comprehensive study of the two-phonon intervalley (2D) Raman mode in graphene monolayers, motivated by recent reports of asymmetric 2D-mode line shapes in freestanding graphene. For photon energies in the range 1.53-2.71 eV, the 2D-mode Raman response of freestanding samples appears as bimodal, in stark contrast with the Lorentzian approximation that is commonly used for supported monolayers. The transition between the freestanding and supported cases is mimicked by electrostatically doping freestanding graphene at carrier densities above 2 x 10(11) cm(-2). This result quantitatively demonstrates that low levels of charging can obscure the intrinsically bimodal 2D-mode line shape of monolayer graphene. In pristine freestanding graphene, we observe a broadening of the 2D-mode feature with decreasing photon energy that cannot be rationalized using a simple one-dimensional model based on resonant inner and outer processes. This indicates that phonon wavevectors away from the high-symmetry lines of the Brillouin zone must contribute to the 2D-mode, so that a full two-dimensional calculation is required to properly describe multiphonon-resonant Raman processes.
C1 [Berciaud, Stephane] Univ Strasbourg, Inst Phys & Chim Mat Strasbourg, F-67034 Strasbourg 2, France.
[Berciaud, Stephane] Univ Strasbourg, NIE, UMR 7504, F-67034 Strasbourg 2, France.
[Berciaud, Stephane] CNRS, F-67034 Strasbourg 2, France.
[Li, Xianglong; Htoon, Han; Doorn, Stephen K.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.
[Brus, Louis E.] Columbia Univ, Dept Chem, New York, NY 10027 USA.
[Heinz, Tony F.] Columbia Univ, Dept Phys, New York, NY 10027 USA.
[Heinz, Tony F.] Columbia Univ, Dept Elect Engn, New York, NY 10027 USA.
RP Berciaud, S (reprint author), Univ Strasbourg, Inst Phys & Chim Mat Strasbourg, 23 Rue Loess,BP43, F-67034 Strasbourg 2, France.
EM stephane.berciaud@ipcms.unistra.fr
RI Li, Xianglong/A-9010-2010; BERCIAUD, Stephane/B-5257-2015; Heinz,
Tony/K-7797-2015;
OI Li, Xianglong/0000-0002-6200-1178; BERCIAUD,
Stephane/0000-0002-5753-3671; Heinz, Tony/0000-0003-1365-9464; Htoon,
Han/0000-0003-3696-2896
FU MURI program AFOSR [FA9550-09-1-0705]; DOE [DE-FG02-11ER16224];
Universite de Strasbourg; CNRS; C'Nano GE; LANL LDRD program
FX We are grateful to J. Maultzsch, F. Mauri, and R. Narula for inspiring
discussions and to M.Y. Han and M. Romeo for experimental help. We
acknowledge support from the MURI program AFOSR through grant
FA9550-09-1-0705 for Raman measurements at shorter wavelengths and from
the DOE through grant DE-FG02-11ER16224 for data analysis at Columbia
University, from the Universite de Strasbourg, the CNRS, and C'Nano GE
for research carried out in France, and from the LANL LDRD program. The
Raman spectra at longer wavelengths were measured at the Center for
Integrated Nanotechnologies, a U.S. Department of Energy, Office of
Basic Energy Sciences user facility.
NR 31
TC 35
Z9 35
U1 6
U2 66
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3517
EP 3523
DI 10.1021/nl400917e
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000011
PM 23799800
ER
PT J
AU Conley, HJ
Wang, B
Ziegler, JI
Haglund, RF
Pantelides, ST
Bolotin, KI
AF Conley, Hiram J.
Wang, Bin
Ziegler, Jed I.
Haglund, Richard F., Jr.
Pantelides, Sokrates T.
Bolotin, Kirill I.
TI Bandgap Engineering of Strained Monolayer and Bilayer MoS2
SO NANO LETTERS
LA English
DT Article
DE MoS2; strain; bandgap engineering; photoluminescence; Gruneisen
parameter
ID SINGLE-LAYER MOS2; VALLEY POLARIZATION; ELECTRICAL CONTROL
AB We report the influence of uniaxial tensile mechanical strain in the range 0-2.2% on the phonon spectra and bandstructures of monolayer and bilayer molybdenum disulfide (MoS2) two-dimensional crystals. First, we employ Raman spectroscopy to observe phonon softening with increased strain, breaking the degeneracy in the E' Raman mode of MoS2, and extract a Gruneisen parameter of similar to 1.06. Second, using photoluminescence spectroscopy we measure a decrease in the optical band gap of MoS2 that is approximately linear with strain, similar to 45 meV/% strain for monolayer MoS2 and similar to 120 meV/% strain for bilayer MoS2. Third, we observe a pronounced strain-induced decrease in the photoluminescence intensity of monolayer MoS2 that is indicative of the direct-to-indirect transition of the character of the optical band gap of this material at applied strain of similar to 1%. These observations constitute a demonstration of strain engineering the band structure in the emergent class of two-dimensional crystals, transition-metal dichalcogenides.
C1 [Conley, Hiram J.; Wang, Bin; Ziegler, Jed I.; Haglund, Richard F., Jr.; Pantelides, Sokrates T.; Bolotin, Kirill I.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA.
[Pantelides, Sokrates T.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RP Bolotin, KI (reprint author), Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA.
EM kirill.bolotin@vanderbilt.edu
RI Wang, Bin/E-8301-2011; Bolotin, Kirill/O-5101-2016
OI Wang, Bin/0000-0001-8246-1422;
FU NSF [DMR-1056859, EPS-1004083]; ONR [N000141310299]; DTRA
[HDTRA1-1-10-1-0047]
FX This research was supported by NSF DMR-1056859, NSF EPS-1004083, and ONR
N000141310299. B.W. and J.I.Z. were supported by DTRA
HDTRA1-1-10-1-0047. We thank John Fellenstein for help in designing the
four point bending apparatus, Branton Campbell for teaching us about
phonon naming conventions, and Ashwin Ramasubramaniam for discussions
about the first-principles calculations.
NR 32
TC 411
Z9 414
U1 86
U2 699
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3626
EP 3630
DI 10.1021/nl4014748
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000028
PM 23819588
ER
PT J
AU Iancu, V
Zhang, XG
Kim, TH
Menard, LD
Kent, PRC
Woodson, ME
Ramsey, JM
Li, AP
Weitering, HH
AF Iancu, Violeta
Zhang, X. -G.
Kim, Tae-Hwan
Menard, Laurent D.
Kent, P. R. C.
Woodson, Michael E.
Ramsey, J. Michael
Li, An-Ping
Weitering, Hanno H.
TI Polaronic Transport and Current Blockades in Epitaxial Silicide
Nanowires and Nanowire Arrays
SO NANO LETTERS
LA English
DT Article
DE suicide nanowires; one-dimensional conductance; self-assembly; scanning
tunneling microscopy; polarons
ID TEMPERATURE-DEPENDENCE; SI(001); SURFACE; ELECTRON; STATE; WIRES
AB Crystalline micrometer-long YSi2 nanowires with cross sections as small as 1 x 0.5 nm can be grown on the Si(001) surface. Their extreme aspect ratios make electron conduction within these nanowires almost ideally one-dimensional, while their compatibility with the silicon platform suggests application as metallic interconnect in Si-based nanoelectronic devices. Here we combine bottom-up epitaxial wire synthesis in ultrahigh vacuum with top-down miniaturization of the electrical measurement probes to elucidate the electronic conduction mechanism of both individual wires and arrays of nanowires. Temperature-dependent transport through individual nanowires is indicative of thermally assisted tunneling of small polarons between atomic-scale defect centers. In-depth analysis of complex wire networks emphasize significant electronic crosstalk between the nanowires due to the long-range Coulomb fields associated with polaronic charge fluctuations. This work establishes a semiquantitative correlation between the density and distributions of atomic-scale defects and resulting current-voltage characteristics of nanoscale network devices.
C1 [Iancu, Violeta; Weitering, Hanno H.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA.
[Zhang, X. -G.; Kim, Tae-Hwan; Kent, P. R. C.; Li, An-Ping] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Menard, Laurent D.; Woodson, Michael E.; Ramsey, J. Michael] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA.
[Zhang, X. -G.; Kent, P. R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.
[Weitering, Hanno H.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RP Weitering, HH (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA.
EM hanno@utk.edu
RI Kent, Paul/A-6756-2008; Li, An-Ping/B-3191-2012; Kim,
Tae-Hwan/A-5636-2010; Iancu, Violeta/B-7657-2008
OI Kent, Paul/0000-0001-5539-4017; Li, An-Ping/0000-0003-4400-7493; Kim,
Tae-Hwan/0000-0001-5328-0913; Iancu, Violeta/0000-0003-1146-2959
FU NIH [R01HG002647]; NSF [DMR-1005488]; Scientific User Facilities
Division, Office of Basic Energy Sciences, U.S. Department of Energy
FX We thank Stephen Jesse for his help with the MM measurements. The
experimental research was sponsored by NIH Grant R01HG002647 and NSF
Grant DMR-1005488. A portion of this research was conducted at the
Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge
National Laboratory by the Scientific User Facilities Division, Office
of Basic Energy Sciences, U.S. Department of Energy (X.G.Z., T.H.K,
P.R.C.K, and A.P.L.).
NR 23
TC 3
Z9 3
U1 2
U2 50
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3684
EP 3689
DI 10.1021/nl401574c
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000038
PM 23902411
ER
PT J
AU Quan, ZW
Luo, ZP
Wang, YX
Xu, HW
Wang, CY
Wang, ZW
Fang, JY
AF Quan, Zewei
Luo, Zhiping
Wang, Yuxuan
Xu, Hongwu
Wang, Chenyu
Wang, Zhongwu
Fang, Jiye
TI Pressure-Induced Switching between Amorphization and Crystallization in
PbTe Nanoparticles
SO NANO LETTERS
LA English
DT Article
DE Amorphization; crystallization; high pressure; PbTe nanoparticle; phase
transformation; synchrotron XRD
ID INDUCED STRUCTURAL TRANSFORMATIONS; PHASE-TRANSITION; NANOCRYSTALS;
STABILITY; SURFACE; MEMORY
AB Combining in situ high-pressure X-ray scattering with transmission electron microscopy, we investigated the pressure-induced structural switches between the rock salt and amorphous phases as well as the associated mechanisms of their crystallization and growth in 6 nm PbTe nanocrystal. It was observed that rock salt PbTe nanocrystal started to become amorphous above 10 GPa and then underwent a low-to-high density amorphous phase transformation at pressures over 15 GPa. The low-density amorphous phase exhibited a structural memory of the rock salt phase, as manifested by a backward transformation to the rock salt phase via single nucleation inside each nanoparticle upon the release of pressure. In contrast, the high-density amorphous phase remained stable and could be preserved at ambient conditions. In addition, electron beam-induced heating could drive a recrystallization of the rock salt phase on the recovered amorphous nanoparticles. These studies provide significant insights into structural mechanisms for pressure-induced switching between amorphous and crystalline phases as well as their associated growth processes.
C1 [Quan, Zewei; Wang, Chenyu; Fang, Jiye] SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA.
[Wang, Yuxuan; Fang, Jiye] SUNY Binghamton, Mat Sci & Engn Program, Binghamton, NY 13902 USA.
[Quan, Zewei; Xu, Hongwu] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA.
[Luo, Zhiping] Texas A&M Univ, Microscopy & Imaging Ctr, College Stn, TX 77843 USA.
[Luo, Zhiping] Fayetteville State Univ, Dept Chem & Phys, Fayetteville, NC 28301 USA.
[Wang, Zhongwu] Cornell Univ, Wilson Lab, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA.
RP Fang, JY (reprint author), SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA.
EM jfang@binghamton.edu
RI Fang, Jiye/H-8266-2013; Luo, Zhiping/C-4435-2014; Quan,
Zewei/G-4759-2011; Wang, Yuxuan/P-4470-2014;
OI Luo, Zhiping/0000-0002-8264-6424; Xu, Hongwu/0000-0002-0793-6923
FU S3IP at Binghamton University; DOE STTR program; laboratory-directed
research and development (LDRD) program of Los Alamos National
Laboratory; DOE [DE-AC52-06NA25396]; NSF [DMR-0936384]
FX This work was partially supported by S3IP at Binghamton
University and DOE STTR program. Z.Q. acknowledges the J. Robert
Oppenheimer (JRO) fellowship supported by the laboratory-directed
research and development (LDRD) program of Los Alamos National
Laboratory, which is operated by Los Alamos National Security LLC under
DOE Contract No. DE-AC52-06NA25396. Z.L. thanks Dr. Masahiro Kawasaki
from JEOL USA Inc., for assistance in the electron dose calculations.
CHESS is supported by the NSF award DMR-0936384.
NR 24
TC 15
Z9 15
U1 5
U2 80
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3729
EP 3735
DI 10.1021/nl4016705
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000045
PM 23805798
ER
PT J
AU Guo, HW
Noh, JH
Dong, S
Rack, PD
Gai, Z
Xu, XS
Dagotto, E
Shen, J
Ward, TZ
AF Guo, Hangwen
Noh, Joo H.
Dong, Shuai
Rack, Philip D.
Gai, Zheng
Xu, Xiaoshan
Dagotto, Elbio
Shen, Jian
Ward, T. Zac
TI Electrophoretic-like Gating Used To Control Metal-Insulator Transitions
in Electronically Phase Separated Manganite Wires
SO NANO LETTERS
LA English
DT Article
DE Nanoconfined oxides; magnetotransport; electronic phase separation;
electrophoretic switching transition metal oxides
ID MIXED-VALENT MANGANITES; RESISTIVITY; PERCOLATION; PROSPECTS
AB Electronically phase separated manganite wires are found to exhibit controllable metal insulator transitions under local electric fields. The switching characteristics are shown to be fully reversible, polarity independent, and highly resistant to thermal breakdown caused by repeated cycling. It is further demonstrated that multiple discrete resistive states can be accessed in a single wire. The results conform to a phenomenological model in which the inherent nanoscale insulating and metallic domains are rearranged through electrophoretic-like processes to open and close percolation channels.
C1 [Guo, Hangwen; Dong, Shuai; Xu, Xiaoshan; Dagotto, Elbio; Ward, T. Zac] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
[Guo, Hangwen; Dong, Shuai; Dagotto, Elbio; Shen, Jian] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
[Noh, Joo H.; Rack, Philip D.] Univ Tennessee, Knoxville, TN 37996 USA.
[Noh, Joo H.; Rack, Philip D.; Gai, Zheng; Xu, Xiaoshan] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Dong, Shuai] SE Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China.
[Shen, Jian] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China.
RP Shen, J (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
EM shenj5494@fudan.edu.cn; 5zw@ornl.gov
RI Gai, Zheng/B-5327-2012; Dong (董), Shuai (帅)/A-5513-2008; Xu,
Xiaoshan/B-1255-2009; Ward, Thomas/I-6636-2016;
OI Gai, Zheng/0000-0002-6099-4559; Dong (董), Shuai (帅)/0000-0002-6910-6319;
Xu, Xiaoshan/0000-0002-4363-392X; Ward, Thomas/0000-0002-1027-9186;
Rack, Philip/0000-0002-9964-3254
FU US DOE, Office of Basic Energy Sciences, Materials Sciences and
Engineering Division; US DOE [DE-SC0002136]; Scientific User Facilities
Division, Office of Basic Energy Sciences, U.S. Department of Energy;
Joint Institute of Advanced Materials; National Science Foundation of
China [11274060]; National Basic Research Program of China (973 Program)
[2011CB921801]
FX This effort was supported by the US DOE, Office of Basic Energy
Sciences, Materials Sciences and Engineering Division (T.Z.W., E.D., and
X.X.) and under US DOE grant DE-SC0002136 (H.W.G.). Nanofabrication
(P.D.R, J.H.N.) and magnetization measurements (Z.G.) were conducted at
the Center for Nanophase Materials Sciences, which is sponsored at Oak
Ridge National Laboratory by the Scientific User Facilities Division,
Office of Basic Energy Sciences, U.S. Department of Energy. J.H.N. also
acknowledges support from the Joint Institute of Advanced Materials
Partial support was also supplied from the National Science Foundation
of China no. 11274060 (S.D.) and the National Basic Research Program of
China (973 Program) under grant no. 2011CB921801 (J.S.).
NR 38
TC 22
Z9 22
U1 7
U2 89
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3749
EP 3754
DI 10.1021/nl4016842
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000048
PM 23899098
ER
PT J
AU Zheng, JM
Gu, M
Xiao, J
Zuo, PJ
Wang, CM
Zhang, JG
AF Zheng, Jianming
Gu, Meng
Xiao, Jie
Zuo, Pengjian
Wang, Chongmin
Zhang, Ji-Guang
TI Corrosion/Fragmentation of Layered Composite Cathode and Related
Capacity/Voltage Fading during Cycling Process
SO NANO LETTERS
LA English
DT Article
DE Voltage fading; fragmentation; etched surface; Mn2+ formation; layered
cathode; lithium ion battery
ID LITHIUM-ION BATTERIES; ELECTROCHEMICAL PERFORMANCE; ANOMALOUS CAPACITY;
CO ELECTRODES; NICKEL; OXIDES; MN; NI; LI1.2NI0.2MN0.6O2; LI2MNO3
AB The Li-rich, Mn-rich (LMR) layered structure materials exhibit very high discharge capacities exceeding 250 mAh g(-1) and are very promising cathodes to be used in lithium ion batteries. However, significant barriers, such as voltage fade and low rate capability, still need to be overcome before the practical applications of these materials. A detailed study of the voltage/capacity fading mechanism will be beneficial for further tailoring the electrode structure and thus improving the electrochemical performances of these layered cathodes. Here, we report detailed studies of structural changes of LMR layered cathode Li[Li0.2Ni0.2Mn0.6]O-2 after long-term cycling by aberration-corrected scanning transmission electron microscopy (STEM) and electron energy loss spectroscopy (EELS). The fundamental findings provide new insights into capacity/voltage fading mechanism of Li[Li0.2Ni0.2Mn0.6]O-2. Sponge-like structure and fragmented pieces were found on the surface of cathode after extended cycling. Formation of Mn2+ species and reduced Li content in the fragments leads to the significant capacity loss during cycling. These results also imply the functional mechanism of surface coatings, for example, AlF3, which can protect the electrode from etching by acidic species in the electrolyte, suppress cathode corrosion/fragmentation, and thus improve long-term cycling stability.
C1 [Zheng, Jianming; Xiao, Jie; Zuo, Pengjian; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA.
[Gu, Meng; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
RP Wang, CM (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
EM chongmin.wang@pnnl.gov; jiguang.zhang@pnnl.gov
RI Gu, Meng/B-8258-2013; Zheng, Jianming/F-2517-2014
OI Zheng, Jianming/0000-0002-4928-8194
FU Office of Vehicle Technologies of the U.S. Department of Energy
[DE-AC02-05CH11231, 18769]; DOE's Office of Biological and Environmental
Research; DOE [DE-AC05-76RLO1830]
FX This work is supported by the Assistant Secretary for Energy Efficiency
and Renewable Energy, Office of Vehicle Technologies of the U.S.
Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract
No. 18769, under the Batteries for Advanced Transportation Technologies
program. The microscopic study described in this paper is part of the
Chemical Imaging Initiative at Pacific Northwest National Laboratory
(PNNL). It was conducted under the Laboratory Directed Research and
Development Program at PNNL, a multiprogram national laboratory operated
by Battelle for the U.S. Department of Energy (DOE). The work was
conducted in the William R Wiley Environmental Molecular Sciences
Laboratory (EMSL), a national scientific user facility sponsored by
DOE's Office of Biological and Environmental Research and located at
PNNL. PNNL is operated by Battelle for the DOE under Contract
DE-AC05-76RLO1830.
NR 31
TC 123
Z9 125
U1 29
U2 304
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3824
EP 3830
DI 10.1021/nl401849t
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000060
PM 23802657
ER
PT J
AU Lau, PH
Takei, K
Wang, C
Ju, Y
Kim, J
Yu, ZB
Takahashi, T
Cho, G
Javey, A
AF Lau, Pak Heng
Takei, Kuniharu
Wang, Chuan
Ju, Yeonkyeong
Kim, Junseok
Yu, Zhibin
Takahashi, Toshitake
Cho, Gyoujin
Javey, Ali
TI Fully Printed, High Performance Carbon Nanotube Thin-Film Transistors on
Flexible Substrates
SO NANO LETTERS
LA English
DT Article
DE Flexible electronics; thin-film transistors; semiconducting nanotube
networks; printable electronics
ID INTEGRATED-CIRCUITS; ELECTRONICS; SENSORS; INKS
AB Fully printed transistors are a key component of ubiquitous flexible electronics. In this work, the advantages of an inverse gravure printing technique and the solution processing of semiconductor-enriched single-walled carbon nanotubes (SWNTs) are combined to fabricate fully printed thin-film transistors on mechanically flexible substrates. The fully printed transistors are configured in a top-gate device geometry and utilize silver metal electrodes and an inorganic/organic high-kappa (similar to 17) gate dielectric. The devices exhibit excellent performance for a fully printed process, with mobility and on/off current ratio of up to similar to 9 cm(2)/(V s) and 10(5), respectively. Extreme bendability is observed, without measurable change in the electrical performance down to a small radius of curvature of 1 mm. Given the high performance of the transistors, our high-throughput printing process serves as an enabling nanomanufacturing scheme for a wide range of large-area electronic applications based on carbon nanotube networks.
C1 [Lau, Pak Heng; Takei, Kuniharu; Wang, Chuan; Yu, Zhibin; Takahashi, Toshitake; Javey, Ali] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Lau, Pak Heng; Takei, Kuniharu; Wang, Chuan; Yu, Zhibin; Takahashi, Toshitake; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA.
[Takei, Kuniharu; Wang, Chuan; Yu, Zhibin; Takahashi, Toshitake; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Ju, Yeonkyeong; Kim, Junseok; Cho, Gyoujin] Sunchon Natl Univ, World Class Univ Program, Sunchon 540742, Jeonnam, South Korea.
RP Javey, A (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA.
EM ajavey@eecs.berkeley.edu
RI Wang, Chuan/B-3649-2011; Javey, Ali/B-4818-2013
FU NSF NASCENT Center; World Class University program at Sunchon National
University
FX This work was supported by NSF NASCENT Center. A.J. and G.C. acknowledge
support from the World Class University program at Sunchon National
University
NR 20
TC 140
Z9 140
U1 25
U2 215
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3864
EP 3869
DI 10.1021/nl401934a
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000066
PM 23899052
ER
PT J
AU Shao, YY
Xiao, J
Wang, W
Engelhard, M
Chen, XL
Nie, ZM
Gu, M
Saraf, LV
Exarhos, G
Zhang, JG
Liu, J
AF Shao, Yuyan
Xiao, Jie
Wang, Wei
Engelhard, Mark
Chen, Xilin
Nie, Zimin
Gu, Meng
Saraf, Laxmikant V.
Exarhos, Gregory
Zhang, Ji-Guang
Liu, Jun
TI Surface-Driven Sodium Ion Energy Storage in Nanocellular Carbon Foams
SO NANO LETTERS
LA English
DT Article
DE Energy storage; sodium battery; surface driven reaction; oxygen
functional group; nanocellular carbon foams
ID LONG CYCLE LIFE; LITHIUM BATTERIES; ELECTRODE MATERIALS; LOW-COST;
ELECTROCHEMICAL INTERCALATION; POSITIVE ELECTRODE; FUNCTIONAL-GROUPS;
CATHODE MATERIAL; ANODE MATERIAL; METAL OXIDE
AB Sodium ion (Na+) batteries have attracted increased attention for energy storage due to the natural abundance of sodium, but their development is hindered by poor intercalation property of Na+ in electrodes. This paper reports a detailed study of high capacity, high rate sodium ion energy storage in functionalized high-surface-area nanocellular carbon foams (NCCF). The energy storage mechanism is surface-driven reactions between Na+ and oxygen-containing functional groups on the surface of NCCF. The surface reaction, rather than a Na+ bulk intercalation reaction, leads to high rate performance and cycling stability due to the enhanced reaction kinetics and the absence of electrode structure change. The NCCF makes more surface area and surface functional groups available for the Na+ reaction. It delivers 152 mAh/g capacity at the rate of 0.1 A/g and a capacity retention of 90% for over 1600 cycles.
C1 [Shao, Yuyan; Xiao, Jie; Wang, Wei; Engelhard, Mark; Chen, Xilin; Nie, Zimin; Gu, Meng; Saraf, Laxmikant V.; Exarhos, Gregory; Zhang, Ji-Guang; Liu, Jun] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Shao, YY (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM yuyan.shao@pnnl.gov; jun.liu@pnnl.gov
RI Shao, Yuyan/A-9911-2008; Chen, Xilin/A-1409-2012; Wang, Wei/F-4196-2010;
Gu, Meng/B-8258-2013;
OI Shao, Yuyan/0000-0001-5735-2670; Wang, Wei/0000-0002-5453-4695;
Engelhard, Mark/0000-0002-5543-0812
FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of
Materials Sciences and Engineering; Office of Electricity Delivery and
Energy Reliability of the U.S. Department of Energy (DOE); Department of
Energy's Office of Biological and Environmental Research
FX This work was primarily supported by the U.S. Department of Energy,
Office of Basic Energy Sciences, Division of Materials Sciences and
Engineering. We are grateful for the financial support from the Office
of Electricity Delivery and Energy Reliability of the U.S. Department of
Energy (DOE) for developing the Na-ion storage battery technology. The
XPS, TEM, and SEM work was performed using EMSL, a national scientific
user facility sponsored by the Department of Energy's Office of
Biological and Environmental Research and located at Pacific Northwest
National Laboratory (PNNL). PNNL is a multiprogram national laboratory
operated for DOE by Battelle.
NR 56
TC 64
Z9 64
U1 12
U2 158
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3909
EP 3914
DI 10.1021/nl401995a
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000073
PM 23879207
ER
PT J
AU Raja, SN
Olson, ACK
Thorkelsson, K
Luong, AJ
Hsueh, L
Chang, GQ
Gludovatz, B
Lin, LW
Xu, T
Ritchie, RO
Alivisatos, AP
AF Raja, Shilpa N.
Olson, Andrew C. K.
Thorkelsson, Kari
Luong, Andrew J.
Hsueh, Lillian
Chang, Guoqing
Gludovatz, Bernd
Lin, Liwei
Xu, Ting
Ritchie, Robert O.
Alivisatos, A. Paul
TI Tetrapod Nanocrystals as Fluorescent Stress Probes of Electrospun
Nanocomposites
SO NANO LETTERS
LA English
DT Article
DE Nanocomposite; polymer; nanocrystal; electrospinning; mechanical; sensor
ID NANOTUBE-POLYMER COMPOSITES; ATOMIC-FORCE MICROSCOPE;
MECHANICAL-PROPERTIES; VISCOELASTIC PROPERTIES; GREEN COMPOSITES; EPOXY
COMPOSITES; SEEDED GROWTH; FIBER LENGTH; NANOFIBERS; NANOPARTICLES
AB A nanoscale, visible-light, self-sensing stress probe would be highly desirable in a variety of biological, imaging, and materials engineering applications, especially a device that does not alter the mechanical properties of the material it seeks to probe. Here we present the CdSe-CdS tetrapod quantum dot, incorporated into polymer matrices via electrospinning, as an in situ luminescent stress probe for the mechanical properties of polymer fibers. The mechanooptical sensing performance is enhanced with increasing nanocrystal concentration while causing minimal change in the mechanical properties even up to 20 wt % incorporation. The tetrapod nanoprobe is elastic and recoverable and undergoes no permanent change in sensing ability even upon many cycles of loading to failure. Direct comparisons to side-by-side traditional mechanical tests further validate the tetrapod as a luminescent stress probe. The tetrapod fluorescence stress-strain curve shape matches well with uniaxial stress-strain curves measured mechanically at all filler concentrations reported.
C1 [Raja, Shilpa N.; Olson, Andrew C. K.; Thorkelsson, Kari; Gludovatz, Bernd; Xu, Ting; Ritchie, Robert O.; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Raja, Shilpa N.; Thorkelsson, Kari; Luong, Andrew J.; Hsueh, Lillian; Xu, Ting; Ritchie, Robert O.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Olson, Andrew C. K.; Xu, Ting; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Luong, Andrew J.; Hsueh, Lillian] Univ Calif Berkeley, Dept Chem Engn, Berkeley, CA 94720 USA.
[Chang, Guoqing; Lin, Liwei; Ritchie, Robert O.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA.
RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM alivis@berkeley.edu
RI Ritchie, Robert/A-8066-2008; Alivisatos , Paul /N-8863-2015;
OI Ritchie, Robert/0000-0002-0501-6998; Alivisatos , Paul
/0000-0001-6895-9048; Gludovatz, Bernd/0000-0002-2420-3879
FU Office of Science, Office of Basic Energy Sciences, Division of
Materials Science and Engineering, of the U.S. Department of Energy
[DE-AC02-05CH11231]; NSF [ECCS-0901864]; China Scholarship Council
[2011619026]
FX Work on tetrapod nanocrystal-polymer nanocomposite electrospinning and
optical, mechanical, and structural characterization was supported by
the Director, Office of Science, Office of Basic Energy Sciences,
Division of Materials Science and Engineering, of the U.S. Department of
Energy under contract DE-AC02-05CH11231, specifically on the
Inorganic/Organic Nanocomposites NSET Program (to S.N.R, K.T., T.X., and
A.P.A). Support for mechanical characterization was provided by the
Director, Office of Science, Office of Basic Energy Sciences, Division
of Materials Science and Engineering, of the U.S. Department of Energy
under Contract No. DE-AC02-05CH11231 (to B.G. and R.O.R). K.T. further
acknowledges an NSF Graduate Fellowship. Electrospinning work was
supported by the China Scholarship Council (2011619026) (to G.C), and
NSF Grant ECCS-0901864 (to L.L.).
NR 58
TC 24
Z9 24
U1 7
U2 131
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3915
EP 3922
DI 10.1021/nl401999t
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000074
PM 23815586
ER
PT J
AU Sun, YG
Foley, JJ
Peng, S
Li, Z
Gray, SK
AF Sun, Yugang
Foley, Jonathan J.
Peng, Sheng
Li, Zheng
Gray, Stephen K.
TI Interfaced Metal Heterodimers in the Quantum Size Regime
SO NANO LETTERS
LA English
DT Article
DE Metal nanoparticle dimers; surface plasmon resonance; plasmomics;
quantum-size effects; epitaxial overgrowth; discrete dipole
approximation
ID DISCRETE-DIPOLE APPROXIMATION; PLASMON RESONANCES; NANOPARTICLES;
NANOSTRUCTURES; PARTICLES; OXIDATION; NANORODS
AB Synthesis of nanoparticle dimers made of asymmetric compositions is very challenging because of the difficulty in manipulating the nanoparticles' surface chemistries in order to control the assembly and/or growth of different nanoparticles. In this Letter, we report a seed-mediated, surface-confined epitaxial overgrowth strategy that enables the synthesis of high-quality interfaced Au-Ag heterodimers in the quantum size regime (diameters <10 nm). Au and Ag share a common face-centered cubic lattice and have nearly identical lattice constants, which facilitates epitaxial overgrowth and allows direct contact between the Au and Ag domains. Quantum size effects, formation of the Au/Ag interfaces, and chemical interactions with surfactant molecules strongly influence the optical properties of the dimers and lead to the observation of unique surface plasmon resonances. In particular, we find an unusual enhancement of the characteristic Au surface plasmon resonance and the emergence of a charge transfer plasmon across the Au/Ag domains, which together lead to broad-band absorption spanning visible to near-infrared wavelengths. A model that captures the changes in optical behavior due to chemical interactions and quantum size effects is used to calculate the absorption spectra of the interfaced heterodimers, resulting in good agreement with experimental measurements.
C1 [Sun, Yugang; Foley, Jonathan J.; Peng, Sheng; Li, Zheng; Gray, Stephen K.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
RP Sun, YG (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM ygsun@anl.gov; gray@anl.gov
RI Sun, Yugang /A-3683-2010; Li, Zheng/L-1355-2016
OI Sun, Yugang /0000-0001-6351-6977; Li, Zheng/0000-0001-5281-8101
FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences User Facility
[DE-AC02-06CH11357]; Electron Microscopy Center at Argonne National
Laboratory, a U.S. Department of Energy Office of Science Laboratory
[DE-AC02-06CH11357]
FX This work was performed at the Center for Nanoscale Materials, a U.S.
Department of Energy, Office of Science, Office of Basic Energy Sciences
User Facility under Contract No. DE-AC02-06CH11357. The electron
microscopy was partially accomplished at the Electron Microscopy Center
at Argonne National Laboratory, a U.S. Department of Energy Office of
Science Laboratory under contract No. DE-AC02-06CH11357 by UChicago
Argonne, LLC. Help from Dr. Yuzi Liu on electron microscopy is
appreciated. J.J.F. gratefully acknowledges Dr. Piotr Flatau for helpful
discussion regarding convergence of the DDA method.
NR 29
TC 15
Z9 15
U1 1
U2 75
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2013
VL 13
IS 8
BP 3958
EP 3964
DI 10.1021/nl402361b
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 202SX
UT WOS:000323241000081
PM 23879377
ER
PT J
AU Dera, P
Finkelstein, GJ
Duffy, TS
Downs, RT
Meng, Y
Prakapenka, V
Tkachev, S
AF Dera, Przemyslaw
Finkelstein, Gregory J.
Duffy, Thomas S.
Downs, Robert T.
Meng, Yue
Prakapenka, Vitali
Tkachev, Sergey
TI Metastable high-pressure transformations of orthoferrosilite Fs(82)
SO PHYSICS OF THE EARTH AND PLANETARY INTERIORS
LA English
DT Article
DE Ferrosilite; Enstatite; Pyroxenes; High-pressure phase transition; Upper
mantle; Synchrotron single-crystal X-ray diffraction
ID LATTICE-PREFERRED ORIENTATIONS; PHASE-TRANSITION; ORTHOENSTATITE MGSIO3;
CRYSTAL-CHEMISTRY; ROOM-TEMPERATURE; ELECTRON-DENSITY; RICH PYROXENES;
ORDER-DISORDER; FERROSILITE; MANTLE
AB High-pressure single-crystal X-ray diffraction experiments with natural ferrosilite Fs(82) (Fe0.822+Mg0.16-Al0.01Ca0.01)(Si0.09Al0.01)O-3 orthopyroxene (opx) reveal that at ambient temperature the sample does not transform to the clinopyroxene (cpx) structure, as reported earlier for a synthetic Fs(100) end-member (Hugh-Jones et al., 1996), but instead undergoes a series of two polymorphic transitions, first above 10.1(1) GPa, to the monoclinic P2(1)/c phase beta-opx (distinctly different from both P2(1)/c and C2/c cpx), also observed in natural enstatite (Zhang et al., 2012), and then, above 12.3(1) GPa to a high-pressure ortho-rhombic Pbca phase gamma-opx, predicted for MgSiO3 by atomistic simulations (Jahn, 2008). The structures of phases alpha, beta and gamma have been determined from the single-crystal data at pressures of 2.3(1), 11.1(1), and 14.6(1) GPa, respectively. The two new high-pressure transitions, very similar in their character to the P2(1)/c-C2/c transformation of cpx, make opx approximately as dense as cpx above 12.3(1) GPa and significantly change the elastic anisotropy of the crystal, with the [100] direction becoming almost twice as stiff as in the ambient alpha-opx phase. Both transformations involve mainly tetrahedral rotation, are reversible and are not expected to leave microstructural evidence that could be used as a geobarometric proxy. The high Fe2+ content in Fs(82) shifts the alpha-beta transition to slightly lower pressure, compared to MgSiO3, and has a very dramatic effect on reducing the (meta) stability range of the beta-phase. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Dera, Przemyslaw; Prakapenka, Vitali; Tkachev, Sergey] Univ Chicago, Argonne Natl Lab, Ctr Adv Radiat Sources, Argonne, IL 60439 USA.
[Finkelstein, Gregory J.; Duffy, Thomas S.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA.
[Downs, Robert T.] Univ Arizona, Dept Geol, Tucson, AZ 85721 USA.
[Meng, Yue] Carnegie Inst Sci, High Pressure Collaborat Access Team, Washington, DC USA.
[Dera, Przemyslaw] Univ Hawaii Manoa, Hawaii Inst Geophys & Planetol, Sch Ocean & Earth Sci & Technol, Honolulu, HI 96822 USA.
RP Dera, P (reprint author), Univ Hawaii Manoa, Hawaii Inst Geophys & Planetol, Sch Ocean & Earth Sci & Technol, 1680 East West Rd,POST Bldg,Off 819 EHonolulu, Honolulu, HI 96822 USA.
EM dera@cars.uchicago.edu
RI Duffy, Thomas/C-9140-2017
OI Duffy, Thomas/0000-0002-5357-1259
FU DOE-NNSA; DOE-BES; NSF; National Science Foundation - Earth Sciences
[EAR-1128799]; Department of Energy - Geosciences [DE-FG02-94ER14466];
U. S. Department of Energy, Office of Science, Office of Basic Energy
Sciences [DE-AC02-06CH11357]
FX This work was performed at HPCAT (Sector 16) and GeoSoilEnviroCARS
(Sector 13), Advanced Photon Source (APS), Argonne National Laboratory.
HPCAT operations are supported by CIW, CDAC, UNLV and LANL through
funding from DOE-NNSA and DOE-BES, with partial instrumentation funding
by NSF. GeoSoilEnviroCARS is supported by the National Science
Foundation - Earth Sciences (EAR-1128799) and Department of Energy -
Geosciences (DE-FG02-94ER14466). Use of the Advanced Photon Source was
supported by the U. S. Department of Energy, Office of Science, Office
of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357.
NR 58
TC 13
Z9 13
U1 2
U2 14
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0031-9201
J9 PHYS EARTH PLANET IN
JI Phys. Earth Planet. Inter.
PD AUG
PY 2013
VL 221
BP 15
EP 21
DI 10.1016/j.pepi.2013.06.006
PG 7
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 204YS
UT WOS:000323407800002
ER
PT J
AU Jing, DW
Shi, JW
Shen, SH
Guo, LJ
AF Jing, Dengwei
Shi, Jinwen
Shen, Shaohua
Guo, Liejin
TI Efficient Photocatalytic Hydrogen Evolution Under Visible Light Over a
Mesoporous Titania Crystallized by Thermal Treatment in Hydrogen
SO SCIENCE OF ADVANCED MATERIALS
LA English
DT Article
DE Hydrogenation; Visible Light; Crystal Structure; Hydrogen Production
ID NANOPARTICLES; TIO2
AB TiO2 was prepared by a sot gel method with TiCl4 as precursor and calcined under N-2, Ar, air, and H-2, respectively. The samples are subjected to various physiochemical characterizations. Our results showed that the reducing hydrogen gas atmosphere significantly affected the growth of TiO2 crystallite, leading to formation of mesoporous TiO2 with crystalline framework and high surface area. It also shows high photocatalytic activity for hydrogen production under visible light. Our report shows that the mesoporous TiO2 exhibiting high photocatalytic activity under visible light can be obtained by thermal treatment in certain atmosphere, needless of additional ionic doping which is often employed in traditional strategies. Our finding is believed to be useful for the batch production of TiO2 with high activity and especially with visible light response for the utilization of Solar hydrogen fuel production.
C1 [Jing, Dengwei; Shi, Jinwen; Shen, Shaohua; Guo, Liejin] Xi An Jiao Tong Univ, State Key Lab Multiphase Flow Power Engn, Int Res Ctr Renewable Energy, Xian 710049, Peoples R China.
[Shen, Shaohua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
RP Jing, DW (reprint author), Xi An Jiao Tong Univ, State Key Lab Multiphase Flow Power Engn, Int Res Ctr Renewable Energy, Xian 710049, Peoples R China.
EM dwjing@mail.xjtu.edu.cn; lj-guo@mail.xjtu.edu.cn
RI Shi, Jinwen/D-3054-2011; Shen, Shaohua/E-9507-2011; Jing,
Dengwei/J-2819-2012
OI Shi, Jinwen/0000-0001-7291-2840;
FU National Natural Science Foundation of China [50821064, 21276206];
National Basic Research Program of China [2009CB220000]
FX The authors gratefully acknowledge the financial supports of the
National Natural Science Foundation of China (Nos. 50821064, 21276206)
and National Basic Research Program of China (Nos. 2009CB220000).
NR 20
TC 7
Z9 7
U1 1
U2 26
PU AMER SCIENTIFIC PUBLISHERS
PI VALENCIA
PA 26650 THE OLD RD, STE 208, VALENCIA, CA 91381-0751 USA
SN 1947-2935
J9 SCI ADV MATER
JI Sci. Adv. Mater.
PD AUG
PY 2013
VL 5
IS 8
BP 982
EP 986
DI 10.1166/sam.2013.1546
PG 5
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA 204HK
UT WOS:000323356000009
ER
PT J
AU Forni, O
Maurice, S
Gasnault, O
Wiens, RC
Cousin, A
Clegg, SM
Sirven, JB
Lasue, J
AF Forni, Olivier
Maurice, Sylvestre
Gasnault, Olivier
Wiens, Roger C.
Cousin, Agnes
Clegg, Samuel M.
Sirven, Jean-Baptiste
Lasue, Jeremie
TI Independent component analysis classification of laser induced breakdown
spectroscopy spectra
SO SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY
LA English
DT Article
DE Laser induced breakdown spectroscopy; Chemometrics/statistics; ChemCam;
Mars
ID SOURCE SEPARATION; INSTRUMENT
AB The ChemCam instrument on board Mars Science Laboratory (MSL) rover uses the laser-induced breakdown spectroscopy (LIBS) technique to remotely analyze Martian rocks. It retrieves spectra up to a distance of seven meters to quantify and to quantitatively analyze the sampled rocks. Like any field application, on-site measurements by LIBS are altered by diverse matrix effects which induce signal variations that are specific to the nature of the sample. Qualitative aspects remain to be studied, particularly LIBS sample identification to determine which samples are of interest for further analysis by ChemCam and other rover instruments. This can be performed with the help of different chemometric methods that model the spectra variance in order to identify a the rock from its spectrum. In this paper we test independent components analysis (ICA) rock classification by remote LIBS. We show that using measures of distance in ICA space, namely the Manhattan and the Mahalanobis distance, we can efficiently classify spectra of an unknown rock. The Mahalanobis distance gives overall better performances and is easier to manage than the Manhattan distance for which the determination of the cut-off distance is not easy. However these two techniques are complementary and their analytical performances will improve with time during MSL operations as the quantity of available Martian spectra will grow. The analysis accuracy and performances will benefit from a combination of the two approaches. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Forni, Olivier; Maurice, Sylvestre; Gasnault, Olivier; Cousin, Agnes; Lasue, Jeremie] Univ Toulouse, Inst Rech Astrophys & Planetol, UPS OMP, Toulouse, France.
[Forni, Olivier; Maurice, Sylvestre; Gasnault, Olivier; Cousin, Agnes; Lasue, Jeremie] CNRS, IRAP, F-31028 Toulouse 4, France.
[Wiens, Roger C.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA.
[Cousin, Agnes; Clegg, Samuel M.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87544 USA.
[Sirven, Jean-Baptiste] CEA Saclay, DEN, DPC, SCP, F-91191 Gif Sur Yvette, France.
RP Forni, O (reprint author), CNRS, IRAP, 9 Av Colonel Roche,BP 44346, F-31028 Toulouse 4, France.
EM olivier.forni@irap.omp.eu; sylvestre.maurice@irap.omp.eu;
olivier.gasnault@irap.omp.eu; rwiens@lanl.gov; acousin@lanl.gov;
sclegg@lanl.gov; jean-baptiste.sirven@cea.f; jeremie.lasue@irap.omp.eu
RI Sirven, Jean-Baptiste/H-5782-2013; Gasnault, Olivier/F-4327-2010;
OI Sirven, Jean-Baptiste/0000-0002-5523-6809; Gasnault,
Olivier/0000-0002-6979-9012; Forni, Olivier/0000-0001-6772-9689; Clegg,
Sam/0000-0002-0338-0948
FU ChemCam Project through CNES, France; NASA, US; LANL Lab-Directed
Research and Development (LDRD)
FX This work was supported by the ChemCam Project through CNES funding in
France and NASA funding in the US. Additional support to RCW was
provided by LANL Lab-Directed Research and Development (LDRD) funding.
We thank an anonymous reviewer for her/his helpful comments.
NR 23
TC 29
Z9 29
U1 4
U2 49
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0584-8547
J9 SPECTROCHIM ACTA B
JI Spectroc. Acta Pt. B-Atom. Spectr.
PD AUG 1
PY 2013
VL 86
BP 31
EP 41
DI 10.1016/j.sab.2013.05.003
PG 11
WC Spectroscopy
SC Spectroscopy
GA 203MX
UT WOS:000323298400004
ER
PT J
AU Cheng, CL
Perfect, E
Mills, RT
AF Cheng, C. -L.
Perfect, E.
Mills, R. T.
TI Forward Prediction of Height-Averaged Capillary Pressure-Saturation
Parameters Using the BC-vG Upscaler
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID HETEROGENEOUS POROUS-MEDIA; HYDRAULIC FUNCTIONS; 2-PHASE FLOW;
BROOKS-COREY; SOILS
AB There is ongoing interest in approaches for upscaling point (e.g., pixel or voxel scale) measurements of soil hydraulic properties to predict column-scale behavior in the laboratory, or even field-scale processes. We have developed the BC-vG Upscaler for estimating the height-averaged capillary pressure-saturation relationship, (theta) over bar((h) over bar), for a given porous medium based on equations used in the TrueCell program. Whereas TrueCell inversely estimates point Brooks and Corey (BC) equation parameters from (theta) over bar((h) over bar) data, the BC-vG Upscaler uses point BC parameters as inputs for the forward prediction of height-averaged van Genuchten (vG) parameters. The BC-vG Upscaler was verified using previously published, independent point and height-averaged capillary pressure-saturation data sets for silica sand. The capability of the BC-vG Upscaler was demonstrated in three separate applications. The first showed how the program can be used to predict height-averaged vG equation parameters using three different relationships between n and m. The second explored the effects of varying column height on the predicted vG parameters for a hypothetical porous medium. The third used the BC-vG Upscaler to predict height-averaged vG parameters for a 50-cm-tall column based on previously published point BC parameters for a wide range of porous media. The BC-vG Upscaler is available free upon request. It should prove useful for converting point BC parameters into height-averaged vG parameters suitable for inclusion in numerical models for simulating variably saturated flow. The program could also be used to develop new scale-dependent relationships between the parameters of the BC and vG equations.
C1 [Cheng, C. -L.; Perfect, E.] Univ Tennessee, Dep Earth & Planetary Sci, Knoxville, TN 37996 USA.
[Mills, R. T.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA.
RP Perfect, E (reprint author), Univ Tennessee, Dep Earth & Planetary Sci, Knoxville, TN 37996 USA.
EM eperfect@utk.edu
RI Cheng, Chu-Lin/G-3471-2013
OI Cheng, Chu-Lin/0000-0002-1900-463X
FU Joint Directed Research and Development (JDRD) program of the UT-ORNL
Science Alliance at the University of Tennessee-Knoxville; Laboratory
Directed Research and Development (LDRD) program of Oak Ridge National
Laboratory (ORNL); U.S. Department of Energy [DE-AC05-00OR22725]
FX Funding for C.-L. Cheng was provided by the Joint Directed Research and
Development (JDRD) program of the UT-ORNL Science Alliance at the
University of Tennessee-Knoxville and the Laboratory Directed Research
and Development (LDRD) program of Oak Ridge National Laboratory (ORNL).
Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the
U.S. Department of Energy under Contract No. DE-AC05-00OR22725. We thank
Dr. Toshihiro Sakaki for providing the data from Sakaki and
Illangasekare (2007) in spreadsheet format.
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PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD AUG
PY 2013
VL 12
IS 3
DI 10.2136/vzj2012.0174
PG 9
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA 201RV
UT WOS:000323161600003
ER
PT J
AU Kang, M
Perfect, E
Cheng, CL
Bilheux, HZ
Gragg, M
Wright, DM
Lamanna, JM
Horita, J
Warren, JM
AF Kang, M.
Perfect, E.
Cheng, C. L.
Bilheux, H. Z.
Gragg, M.
Wright, D. M.
Lamanna, J. M.
Horita, J.
Warren, J. M.
TI Diffusivity and Sorptivity of Berea Sandstone Determined using Neutron
Radiography
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID POROUS BUILDING-MATERIALS; SOIL-WATER DIFFUSIVITY; HORIZONTAL
INFILTRATION; SPONTANEOUS IMBIBITION; ROCK SAMPLES; MEDIA; ABSORPTION;
FLOW; CAPILLARITY; TOMOGRAPHY
AB Neutron radiography is increasingly being used to study the dynamics of water movement in variably saturated porous media. It has been applied to visualize water imbibition in both natural and engineered materials, including soil, rock, brick, concrete, and glass. The sorptivity, S, and unsaturated diffusivity, D(theta), are important parameters for describing water movement under partially saturated conditions. Estimates of S and D(theta) have been obtained using a variety of techniques, including neutron imaging. However, we could find no previous reports of such measurements for the Berea sandstone, regardless of the method employed. Berea sandstone is a widespread, medium-to fine-grained terrestrial sandstone of Mississippian age that is used extensively as a standard porous medium in the geology and petroleum engineering fields. We used the CG-1D neutron imaging facility at the High Flux Isotope Reactor of Oak Ridge National Laboratory to estimate S and D(theta) from radiographs acquired every 26 s. A 25 mu m thick LiF/ZnS scintillator was employed in conjunction with a DW936 IkonL ANDOR charge coupled device (CCD) camera system, giving a spatial imaging resolution of similar to 75 mu m. Four replicate cores were investigated. The positions of the observed wetting fronts were linearly regressed against the square root of time. Sorptivity values calculated from the slopes of these relations ranged from 0.89 to 1.46 mm s(-1/2). Further analysis yielded D(theta) functions. These functions were very reproducible and showed good agreement with independent D(theta) values calculated from relative permeability and capillary pressure-saturation data for Berea sandstone. To the best of our knowledge, these are the first published estimates of S and D(theta) for Berea sandstone. Our results clearly demonstrate the effectiveness of neutron imaging in providing high quality, quantitative data for the computation of unsaturated flow parameters.
C1 [Kang, M.; Perfect, E.; Cheng, C. L.; Gragg, M.; Wright, D. M.] Univ Tennessee, Dep Earth & Planetary Sci, Knoxville, TN 37996 USA.
[Kang, M.; Bilheux, H. Z.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA.
[Lamanna, J. M.] Univ Tennessee, Dep Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA.
[Horita, J.] Texas Tech Univ, Dept Geosci, Lubbock, TX 79409 USA.
[Warren, J. M.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN USA.
RP Perfect, E (reprint author), Univ Tennessee, Dep Earth & Planetary Sci, Knoxville, TN 37996 USA.
EM eperfect@utk.edu
RI Cheng, Chu-Lin/G-3471-2013; Warren, Jeffrey/B-9375-2012; Bilheux,
Hassina/H-4289-2012
OI Cheng, Chu-Lin/0000-0002-1900-463X; Warren, Jeffrey/0000-0002-0680-4697;
Bilheux, Hassina/0000-0001-8574-2449
FU Scientific User Facilities Division, Office of Basic Energy Sciences,
United States Department of Energy; Laboratory Directed Research and
Development Program of ORNL; Joint Directed Research and Development
Program of the UT-ORNL Science Alliance at UTK
FX This paper is based in part on assignments prepared by graduate students
participating in a seminar course on imaging water in porous media (GEOL
685) taught by E. Perfect at the University of Tennessee-Knoxville (UTK)
in the spring semester of 2012. The neutron imaging at Oak Ridge
National Laboratory's (ORNL) High Flux Isotope Reactor (HFIR) was
sponsored by the Scientific User Facilities Division, Office of Basic
Energy Sciences, United States Department of Energy, which is managed by
UT-Battelle, LLC. Lakeisha Walker provided excellent technical support
at HFIR. Portions of the MATLAB code used for the quantitative image
analyses were developed by Keely Willis and Sophie Voisin at ORNL.
Funding was provided by the Laboratory Directed Research and Development
Program of ORNL and the Joint Directed Research and Development Program
of the UT-ORNL Science Alliance at UTK.
NR 60
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PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD AUG
PY 2013
VL 12
IS 3
DI 10.2136/vzj2012.0135
PG 8
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA 201RV
UT WOS:000323161600021
ER
PT J
AU Andrade, GA
Pistner, AJ
Yap, GPA
Lutterman, DA
Rosenthal, J
AF Andrade, Gabriel A.
Pistner, Allen J.
Yap, Glenn P. A.
Lutterman, Daniel A.
Rosenthal, Joel
TI Photocatalytic Conversion of CO2 to CO Using Rhenium Bipyridine
Platforms Containing Ancillary Phenyl or BODIPY Moieties
SO ACS CATALYSIS
LA English
DT Article
DE BODIPY; carbon dioxide; catalysis; electrochemistry; photochemistry;
rhenium bipyridine derivatives
ID PORPHYRIN-CATALYZED REDUCTION; ELECTROGENERATED CHEMILUMINESCENCE;
ELECTRON-TRANSFER; CARBON-DIOXIDE; ELECTROCATALYTIC REDUCTION;
ELECTROCHEMISTRY; PHOTOPHYSICS; COMPLEXES; COBALT; PHOTOCHEMISTRY
AB Harnessing of solar energy to drive the reduction of carbon dioxide to fuels requires the development of efficient catalysts that absorb sunlight. In this work, we detail the synthesis, electrochemistry, and photophysical properties of a set of homologous fac-Re-1(CO)(3) complexes containing either an ancillary phenyl (8) or BODIPY (12) substituent. These studies demonstrate that both the electronic properties of the rhenium center and BODIPY chromophore are maintained for these complexes. Photolysis studies demonstrate that both assemblies 8 and 12 are competent catalysts for the photochemical reduction of CO2 to CO in dimethylformamide (DMF) using triethanolamine (TEOA) as a sacrificial reductant. Both compounds 8 and 12 display turnover frequencies (TOFs) for photocatalytic CO production upon irradiation with light (lambda(ex) >= 400 nm) of similar to 5 h(-1). with turnover number (TON) values of approximately 20. Although structural and photophysical measurements demonstrate that electronic coupling between the BODIPY and fac-Re-1(CO)(3) units is limited for complex 12, this work dearly shows that the photoactive BODIPY moiety is tolerated during catalysis and does not interfere with the observed photochemistry. When taken together, these results provide a clear roadmap for the development of advanced rhenium bipyridine complexes bearing ancillary BODIPY groups for the efficient photocatalytic reduction of CO2 using visible light.
C1 [Andrade, Gabriel A.; Pistner, Allen J.; Yap, Glenn P. A.; Rosenthal, Joel] Univ Delaware, Dept Chem & Biochem, Newark, DE 19716 USA.
[Lutterman, Daniel A.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
RP Lutterman, DA (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
EM luttermanda@ornl.gov; joelr@udel.edu
RI Lutterman, Daniel/C-9704-2016
OI Lutterman, Daniel/0000-0002-4875-6056
FU Institutional Development Award (IDeA) from the National Institute of
General Medical Sciences of the National Institutes of Health
[P20GM103541]; NSF; American Chemical Society's Petroleum Research Fund;
Laboratory Directed Research and Development Program of Oak Ridge
National Laboratory
FX Research reported in this publication was supported by an Institutional
Development Award (IDeA) from the National Institute of General Medical
Sciences of the National Institutes of Health under Grant P20GM103541.
G.A.A. and J.R. were supported through an NSF sponsored LSAMP, "bridge
to the doctorate fellowship" and a DuPont Young Professor award,
respectively. J.R. also thanks the University of Delaware Research
Foundation and the donors of the American Chemical Society's Petroleum
Research Fund for financial support. D.A.L. was sponsored by the
Laboratory Directed Research and Development Program of Oak Ridge
National Laboratory, managed by UT-Battelle, LLC, for the U.S.
Department of Energy. NMR and other data were acquired at UD using
instrumentation obtained with assistance from the NSF and NIH (NSF-MRI
0421224, NSF-CRIF CHE-0840401 and CHE-1048367, NIH P20 RR017716).
NR 53
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 2155-5435
J9 ACS CATAL
JI ACS Catal.
PD AUG
PY 2013
VL 3
IS 8
BP 1685
EP 1692
DI 10.1021/cs400332y
PG 8
WC Chemistry, Physical
SC Chemistry
GA 197LO
UT WOS:000322852900001
PM 24015374
ER
PT J
AU Martin, SL
He, LL
Meilleur, F
Guenther, RH
Sit, TL
Lommel, SA
Heller, WT
AF Martin, Stanton L.
He, Lilin
Meilleur, Flora
Guenther, Richard H.
Sit, Tim L.
Lommel, Steven A.
Heller, William T.
TI New insight into the structure of RNA in red clover necrotic mosaic
virus and the role of divalent cations revealed by small-angle neutron
scattering
SO ARCHIVES OF VIROLOGY
LA English
DT Article
ID CUCUMBER-NECROSIS-VIRUS; BUSHY STUNT VIRUS; BIOLOGICAL STRUCTURES;
PROTEIN COMPLEXES; BIPARTITE GENOME; ORGANIZATION; DIFFRACTION;
RESOLUTION; SEQUENCE; PARTICLE
AB Red clover necrotic mosaic virus (RCNMV) is a 36-nm-diameter, T = 3 icosahedral plant virus with a genome that is split between two single-stranded RNA molecules of approximately 3.9 kb and 1.5 kb, as well as a 400-nucleotide degradation product. The structure of the virus capsid and its response to removing Ca2+ and Mg2+ was previously studied by cryo-electron microscopy (cryo-EM) (Sherman et al. J Virol 80:10395-10406, 2006) but the structure of the RNA was only partially resolved in that study. To better understand the organization of the RNA and conformational changes resulting from the removal of divalent cations, small-angle neutron scattering with contrast variation experiments were performed. The results expand upon the cryo-EM results by clearly showing that virtually all of the RNA is contained in a thin shell that is in contact with the interior domains of the viral capsid protein, and they provide new insight into changes in the RNA packing that result from removal of divalent cations.
C1 [Martin, Stanton L.; Guenther, Richard H.; Sit, Tim L.; Lommel, Steven A.] N Carolina State Univ, Dept Plant Pathol, Raleigh, NC 27695 USA.
[He, Lilin; Heller, William T.] Oak Ridge Natl Lab, Ctr Struct Mol Biol, Oak Ridge, TN 37831 USA.
[He, Lilin; Heller, William T.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
[He, Lilin; Meilleur, Flora; Heller, William T.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.
[Meilleur, Flora] N Carolina State Univ, Dept Mol & Struct Biochem, Raleigh, NC 27695 USA.
RP Heller, WT (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.
EM hellerwt@ornl.gov
OI He, Lilin/0000-0002-9560-8101
FU Laboratory Directed Research and Development Program of Oak Ridge
National Laboratory (ORNL); U.S. Department of Energy's Office of
Biological and Environmental Research [FWP ERKP291]; Scientific User
Facilities Division, Office of Basic Energy Sciences, U.S. Department of
Energy; U.S. Department of Energy [DO-AC05-00OR22725, DE-AC05-00OR22725]
FX This research was supported by the Laboratory Directed Research and
Development Program of Oak Ridge National Laboratory (ORNL). The
research at ORNL's Center for Structural Molecular Biology (FWP ERKP291)
was supported by the U.S. Department of Energy's Office of Biological
and Environmental Research. Work at HFIR was sponsored by the Scientific
User Facilities Division, Office of Basic Energy Sciences, U.S.
Department of Energy. Oak Ridge National Laboratory is managed by
UT-Battelle, LLC for the U.S. Department of Energy under contract No.
DO-AC05-00OR22725. This manuscript has been authored by UT-Battelle,
LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of
Energy. The United States Government retains, and the publisher, by
accepting the article for publication, acknowledges that the United
States Government retains a nonexclusive, paid-up, irrevocable,
world-wide license to publish or reproduce the published form of this
manuscript, or allow others to do so, for United States Government
purposes.
NR 35
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U1 0
U2 11
PU SPRINGER WIEN
PI WIEN
PA SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA
SN 0304-8608
J9 ARCH VIROL
JI Arch. Virol.
PD AUG
PY 2013
VL 158
IS 8
BP 1661
EP 1669
DI 10.1007/s00705-013-1650-6
PG 9
WC Virology
SC Virology
GA 191BF
UT WOS:000322386900004
PM 23483344
ER
PT J
AU Bahnfleth, WP
Fisk, WJ
Burroughs, HEB
Persily, A
Martin, SB
Stanke, D
Li, YG
AF Bahnfleth, William P.
Fisk, William J.
Burroughs, H. E. Barney
Persily, Andrew
Martin, Stephen B.
Stanke, Dennis
Li, Yuguo
TI Shaping the Next Indoor Air Quality
SO ASHRAE JOURNAL
LA English
DT Article
C1 [Fisk, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Indoor Environm Grp, Berkeley, CA 94720 USA.
[Persily, Andrew] NIST, Div Energy & Environm, Indoor Air Qual & Ventilat Grp, Gaithersburg, MD USA.
[Martin, Stephen B.] NIOSH, Ctr Dis Control & Prevent, Div Resp Dis Studies, Field Studies Branch, Washington, DC USA.
[Li, Yuguo] Univ Hong Kong, Dept Mech Engn, Hong Kong, Hong Kong, Peoples R China.
NR 3
TC 0
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U1 1
U2 7
PU AMER SOC HEATING REFRIGERATING AIR-CONDITIONING ENG, INC,
PI ATLANTA
PA 1791 TULLIE CIRCLE NE, ATLANTA, GA 30329 USA
SN 0001-2491
J9 ASHRAE J
JI ASHRAE J.
PD AUG
PY 2013
VL 55
IS 8
BP 50
EP +
PG 7
WC Thermodynamics; Construction & Building Technology; Engineering,
Mechanical
SC Thermodynamics; Construction & Building Technology; Engineering
GA 202DH
UT WOS:000323193200015
ER
PT J
AU Rutberg, M
Hastbacka, M
Bouza, A
AF Rutberg, Michael
Hastbacka, Mildred
Bouza, Antonio
TI TES for Residential Settings
SO ASHRAE JOURNAL
LA English
DT Editorial Material
C1 [Rutberg, Michael] Mech Syst Grp, Lexington, MA USA.
[Hastbacka, Mildred] TIAX LLC, Lexington, MA USA.
[Bouza, Antonio] US DOE, Washington, DC USA.
RP Rutberg, M (reprint author), Mech Syst Grp, Lexington, MA USA.
NR 11
TC 1
Z9 1
U1 0
U2 1
PU AMER SOC HEATING REFRIGERATING AIR-CONDITIONING ENG, INC,
PI ATLANTA
PA 1791 TULLIE CIRCLE NE, ATLANTA, GA 30329 USA
SN 0001-2491
J9 ASHRAE J
JI ASHRAE J.
PD AUG
PY 2013
VL 55
IS 8
BP 92
EP 94
PG 3
WC Thermodynamics; Construction & Building Technology; Engineering,
Mechanical
SC Thermodynamics; Construction & Building Technology; Engineering
GA 202DH
UT WOS:000323193200020
ER
PT J
AU Guo, YC
Ferguson, HC
Giavalisco, M
Barro, G
Willner, SP
Ashby, MLN
Dahlen, T
Donley, JL
Faber, SM
Fontana, A
Galametz, A
Grazian, A
Huang, KH
Kocevski, DD
Koekemoer, AM
Koo, DC
McGrath, EJ
Peth, M
Salvato, M
Wuyts, S
Castellano, M
Cooray, AR
Dickinson, ME
Dunlop, JS
Fazio, GG
Gardner, JP
Gawiser, E
Grogin, NA
Hathi, NP
Hsu, LT
Lee, KS
Lucas, RA
Mobasher, B
Nandra, K
Newman, JA
van der Wel, A
AF Guo, Yicheng
Ferguson, Henry C.
Giavalisco, Mauro
Barro, Guillermo
Willner, S. P.
Ashby, Matthew L. N.
Dahlen, Tomas
Donley, Jennifer L.
Faber, Sandra M.
Fontana, Adriano
Galametz, Audrey
Grazian, Andrea
Huang, Kuang-Han
Kocevski, Dale D.
Koekemoer, Anton M.
Koo, David C.
McGrath, Elizabeth J.
Peth, Michael
Salvato, Mara
Wuyts, Stijn
Castellano, Marco
Cooray, Asantha R.
Dickinson, Mark E.
Dunlop, James S.
Fazio, G. G.
Gardner, Jonathan P.
Gawiser, Eric
Grogin, Norman A.
Hathi, Nimish P.
Hsu, Li-Ting
Lee, Kyoung-Soo
Lucas, Ray A.
Mobasher, Bahram
Nandra, Kirpal
Newman, Jeffery A.
van der Wel, Arjen
TI CANDELS MULTI-WAVELENGTH CATALOGS: SOURCE DETECTION AND PHOTOMETRY IN
THE GOODS-SOUTH FIELD
SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES
LA English
DT Article
DE catalogs; galaxies: high-redshift; galaxies: photometry; methods: data
analysis; techniques: image processing
ID ORIGINS DEEP SURVEY; SPECTRAL ENERGY-DISTRIBUTIONS; STAR-FORMATION
HISTORY; SIMILAR-TO 2; GMASS ULTRADEEP SPECTROSCOPY; EXTRAGALACTIC
LEGACY SURVEY; REST-FRAME ULTRAVIOLET; UV LUMINOSITY FUNCTION;
HIGH-REDSHIFT GALAXIES; SPACE-TELESCOPE
AB We present a UV to mid-infrared multi-wavelength catalog in the CANDELS/GOODS-S field, combining the newly obtained CANDELS HST/WFC3 F105W, F125W, and F160W data with existing public data. The catalog is based on source detection in the WFC3 F160W band. The F160W mosaic includes the data from CANDELS deep and wide observations as well as previous ERS and HUDF09 programs. The mosaic reaches a 5 sigma limiting depth (within an aperture of radius 0 ''.17) of 27.4, 28.2, and 29.7 AB for CANDELS wide, deep, and HUDF regions, respectively. The catalog contains 34,930 sources with the representative 50% completeness reaching 25.9, 26.6, and 28.1 AB in the F160W band for the three regions. In addition to WFC3 bands, the catalog also includes data from UV (U band from both CTIO/MOSAIC and VLT/VIMOS), optical (HST/ACS F435W, F606W, F775W, F814W, and F850LP), and infrared (HST/WFC3 F098M, VLT/ISAAC K s, VLT/HAWK-I K s, and Spitzer/IRAC 3.6, 4.5, 5.8, 8.0 mu m) observations. The catalog is validated via stellar colors, comparison with other published catalogs, zero-point offsets determined from the best-fit templates of the spectral energy distribution of spectroscopically observed objects, and the accuracy of photometric redshifts. The catalog is able to detect unreddened star-forming (passive) galaxies with stellar mass of 10(10) M-circle dot at a 50% completeness level to z similar to 3.4 (2.8), 4.6 (3.2), and 7.0 (4.2) in the three regions. As an example of application, the catalog is used to select both star-forming and passive galaxies at z similar to 2-4 via the Balmer break. It is also used to study the color-magnitude diagram of galaxies at 0 < z < 4.
C1 [Guo, Yicheng; Barro, Guillermo; Faber, Sandra M.; Koo, David C.] Univ Calif Santa Cruz, Lick Observ, Dept Astron & Astrophys, UCO, Santa Cruz, CA 95064 USA.
[Guo, Yicheng; Giavalisco, Mauro] Univ Massachusetts, Dept Astron, Amherst, MA 01003 USA.
[Ferguson, Henry C.; Dahlen, Tomas; Huang, Kuang-Han; Koekemoer, Anton M.; Lucas, Ray A.] Space Telescope Sci Inst, Baltimore, MD 21218 USA.
[Willner, S. P.; Ashby, Matthew L. N.; Fazio, G. G.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA.
[Donley, Jennifer L.] Los Alamos Natl Lab, Los Alamos, NM USA.
[Fontana, Adriano; Galametz, Audrey; Grazian, Andrea; Castellano, Marco] INAF, Osservatorio Astron, I-00040 Monte Porzio Catone, Italy.
[Huang, Kuang-Han; Peth, Michael] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA.
[Kocevski, Dale D.] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA.
[McGrath, Elizabeth J.] Colby Coll, Dept Phys & Astron, Waterville, ME 04901 USA.
[Salvato, Mara; Wuyts, Stijn; Hsu, Li-Ting; Nandra, Kirpal] Max Planck Inst Extraterr Phys, D-85741 Garching, Germany.
[Salvato, Mara] Excellence Cluster, D-85748 Garching, Germany.
[Cooray, Asantha R.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA.
[Dickinson, Mark E.] Natl Opt Astron Observ, Tucson, AZ 85726 USA.
[Dunlop, James S.] Univ Edinburgh, Royal Observ, Inst Astron, Edinburgh EH9 3HJ, Midlothian, Scotland.
[Gardner, Jonathan P.] NASAs Goddard Space Flight Ctr, Astrophys Sci Div, Observat Cosmol Lab, Greenbelt, MD USA.
[Gawiser, Eric] Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA.
[Hathi, Nimish P.] Carnegie Observ, Pasadena, CA USA.
[Lee, Kyoung-Soo] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA.
[Mobasher, Bahram] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA.
[Newman, Jeffery A.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA.
[van der Wel, Arjen] Max Planck Inst Astron, D-69117 Heidelberg, Germany.
RP Guo, YC (reprint author), Univ Calif Santa Cruz, Lick Observ, Dept Astron & Astrophys, UCO, Santa Cruz, CA 95064 USA.
EM ycguo@ucolick.org
RI Hathi, Nimish/J-7092-2014;
OI Hathi, Nimish/0000-0001-6145-5090; Koekemoer, Anton/0000-0002-6610-2048;
Castellano, Marco/0000-0001-9875-8263; fontana,
adriano/0000-0003-3820-2823
FU NASA through a grant from the Space Telescope Science Institute
[HST-GO-12060]; NASA [NAS5-26555]; NASA HST [GO-12060.10-A]; NSF
[AST-0808133]; European Research Council; Royal Society
FX We thank the anonymous referee for constructive comments that improve
this article. Support for program number HST-GO-12060 was provided by
NASA through a grant from the Space Telescope Science Institute, which
is operated by the Association of Universities for Research in
Astronomy, Incorporated, under NASA contract NAS5-26555. Y.G. and the
authors from UCSC acknowledge support from NASA HST grant GO-12060.10-A
and NSF grant AST-0808133. J.S.D. acknowledges the support of the
European Research Council via the award of an Advanced Grant and the
support of the Royal Society via a Wolfson Research Merit Award. This
work is based in part on observations made with the Spitzer Space
Telescope, which is operated by the Jet Propulsion Laboratory,
California Institute of Technology, under a contract with NASA. Support
for this work was provided by NASA through an award issued by
JPL/Caltech.
NR 84
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U1 0
U2 6
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0067-0049
EI 1538-4365
J9 ASTROPHYS J SUPPL S
JI Astrophys. J. Suppl. Ser.
PD AUG
PY 2013
VL 207
IS 2
AR UNSP 24
DI 10.1088/0067-0049/207/2/24
PG 23
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 195NO
UT WOS:000322710000006
ER
PT J
AU Pal'shin, VD
Hurley, K
Svinkin, DS
Aptekar, RL
Golenetskii, SV
Frederiks, DD
Mazets, EP
Oleynik, PP
Ulanov, MV
Cline, T
Mitrofanov, IG
Golovin, DV
Kozyrev, AS
Litvak, ML
Sanin, AB
Boynton, W
Fellows, C
Harshman, K
Trombka, J
McClanahan, T
Starr, R
Goldsten, J
Gold, R
Rau, A
von Kienlin, A
Savchenko, V
Smith, DM
Hajdas, W
Barthelmy, SD
Cummings, J
Gehrels, N
Krimm, H
Palmer, D
Yamaoka, K
Ohno, M
Fukazawa, Y
Hanabata, Y
Takahashi, T
Tashiro, M
Terada, Y
Murakami, T
Makishima, K
Briggs, MS
Kippen, RM
Kouveliotou, C
Meegan, C
Fishman, G
Connaughton, V
Boer, M
Guidorzi, C
Frontera, F
Montanari, E
Rossi, F
Feroci, M
Amati, L
Nicastro, L
Orlandini, M
DelMonte, E
Costa, E
Donnarumma, I
Evangelista, Y
Lapshov, I
Lazzarotto, F
Pacciani, L
Rapisarda, M
Soffitta, P
Di Cocco, G
Fuschino, F
Galli, M
Labanti, C
Marisaldi, M
Atteia, JL
Vanderspek, R
Ricker, G
AF Pal'shin, V. D.
Hurley, K.
Svinkin, D. S.
Aptekar, R. L.
Golenetskii, S. V.
Frederiks, D. D.
Mazets, E. P.
Oleynik, P. P.
Ulanov, M. V.
Cline, T.
Mitrofanov, I. G.
Golovin, D. V.
Kozyrev, A. S.
Litvak, M. L.
Sanin, A. B.
Boynton, W.
Fellows, C.
Harshman, K.
Trombka, J.
McClanahan, T.
Starr, R.
Goldsten, J.
Gold, R.
Rau, A.
von Kienlin, A.
Savchenko, V.
Smith, D. M.
Hajdas, W.
Barthelmy, S. D.
Cummings, J.
Gehrels, N.
Krimm, H.
Palmer, D.
Yamaoka, K.
Ohno, M.
Fukazawa, Y.
Hanabata, Y.
Takahashi, T.
Tashiro, M.
Terada, Y.
Murakami, T.
Makishima, K.
Briggs, M. S.
Kippen, R. M.
Kouveliotou, C.
Meegan, C.
Fishman, G.
Connaughton, V.
Boer, M.
Guidorzi, C.
Frontera, F.
Montanari, E.
Rossi, F.
Feroci, M.
Amati, L.
Nicastro, L.
Orlandini, M.
DelMonte, E.
Costa, E.
Donnarumma, I.
Evangelista, Y.
Lapshov, I.
Lazzarotto, F.
Pacciani, L.
Rapisarda, M.
Soffitta, P.
Di Cocco, G.
Fuschino, F.
Galli, M.
Labanti, C.
Marisaldi, M.
Atteia, J. -L.
Vanderspek, R.
Ricker, G.
TI INTERPLANETARY NETWORK LOCALIZATIONS OF KONUS SHORT GAMMA-RAY BURSTS
SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES
LA English
DT Article
DE catalogs; gamma-ray burst: general; techniques: miscellaneous
ID ARRIVAL-TIME LOCALIZATIONS; PIONEER-VENUS-ORBITER; ULYSSES SUPPLEMENT;
GIANT FLARE; LIGO OBSERVATIONS; GRB 051103; CATALOG; MISSION; BATSE;
SPECTROMETER
AB Between the launch of the Global Geospace Science Wind spacecraft in 1994 November and the end of 2010, the Konus-Wind experiment detected 296 short-duration gamma-ray bursts (including 23 bursts which can be classified as short bursts with extended emission). During this period, the Interplanetary Network (IPN) consisted of up to 11 spacecraft, and using triangulation, the localizations of 271 bursts were obtained. We present the most comprehensive IPN localization data on these events. The short burst detection rate, similar to 18 yr(-1), exceeds that of many individual experiments.
C1 [Pal'shin, V. D.; Svinkin, D. S.; Aptekar, R. L.; Golenetskii, S. V.; Frederiks, D. D.; Mazets, E. P.; Oleynik, P. P.; Ulanov, M. V.] AF Ioffe Phys Tech Inst, St Petersburg 194021, Russia.
[Hurley, K.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA.
[Cline, T.; Trombka, J.; McClanahan, T.; Starr, R.; Barthelmy, S. D.; Gehrels, N.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA.
[Mitrofanov, I. G.; Golovin, D. V.; Kozyrev, A. S.; Litvak, M. L.; Sanin, A. B.] Space Res Inst, Moscow 117997, Russia.
[Boynton, W.; Fellows, C.; Harshman, K.] Univ Arizona, Dept Planetary Sci, Tucson, AZ 85721 USA.
[Goldsten, J.; Gold, R.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA.
[Rau, A.; von Kienlin, A.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany.
[Savchenko, V.] Univ Paris Diderot, Observ Paris, Francois Arago Ctr, APC,CNRS,CEA,Irfu,IN2P3, F-75205 Paris 13, France.
[Smith, D. M.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA.
[Smith, D. M.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA.
[Hajdas, W.] Paul Scherrer Inst, CH-5232 Villigen, Switzerland.
[Cummings, J.; Krimm, H.] NASA, UMBC, CRESST, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA.
[Cummings, J.] UMBC Phys Dept, Baltimore, MD 21250 USA.
[Krimm, H.] Univ Space Res Assoc, Columbia, MD 20144 USA.
[Palmer, D.; Kippen, R. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Yamaoka, K.; Takahashi, T.] Inst Space & Astronaut Sci ISAS JAXA, Chuo Ku, Sagamihara, Kanagawa 2525210, Japan.
[Ohno, M.; Fukazawa, Y.; Hanabata, Y.] Hiroshima Univ, Dept Phys, Hiroshima 7398526, Japan.
[Tashiro, M.; Terada, Y.] Saitama Univ, Dept Phys, Sakura Ku, Saitama 3388570, Japan.
[Murakami, T.] Kanazawa Univ, Dept Phys, Kanazawa, Ishikawa 9201192, Japan.
[Makishima, K.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan.
[Briggs, M. S.; Connaughton, V.] Univ Alabama, CSPAR, Huntsville, AL 35899 USA.
[Briggs, M. S.; Connaughton, V.] Univ Alabama, Dept Phys, Huntsville, AL 35899 USA.
[Kouveliotou, C.; Fishman, G.] NASA, Space Sci Off, Marshall Space Flight Ctr, Huntsville, AL 35812 USA.
[Meegan, C.] Univ Space Res Assoc, Huntsville, AL 35805 USA.
[Boer, M.] Observ Haute Provence CNRS, F-04870 St Michel lObservatoire, France.
[Guidorzi, C.; Frontera, F.; Montanari, E.; Rossi, F.] Univ Ferrara, Dept Phys, I-44100 Ferrara, Italy.
[Frontera, F.; Amati, L.; Nicastro, L.; Orlandini, M.; Di Cocco, G.; Fuschino, F.; Labanti, C.; Marisaldi, M.] INAF, Ist Astrofis Spaziale & Fis Cosm Bologna, I-40129 Bologna, Italy.
[Montanari, E.] Ist IS Calvi, I-41034 Finale Emilia, MO, Italy.
[Feroci, M.; DelMonte, E.; Costa, E.; Donnarumma, I.; Evangelista, Y.; Lapshov, I.; Lazzarotto, F.; Pacciani, L.; Rapisarda, M.; Soffitta, P.] INAF, Ist Astrofis Spaziale & Fis Cosm, I-00133 Rome, Italy.
[Galli, M.] ENEA Bologna, I-40129 Bologna, Italy.
[Atteia, J. -L.] Univ Toulouse, F-31400 Toulouse, France.
[Atteia, J. -L.] UPS OMP, F-31400 Toulouse, France.
[Atteia, J. -L.] CNRS, F-31400 Toulouse, France.
[Atteia, J. -L.] IRAP, F-31400 Toulouse, France.
[Vanderspek, R.; Ricker, G.] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA.
RP Pal'shin, VD (reprint author), AF Ioffe Phys Tech Inst, Politekhnicheskaya 26, St Petersburg 194021, Russia.
EM val@mail.ioffe.ru
RI Oleynik, Philipp/C-1104-2014; Svinkin, Dmitry/C-1934-2014; Frederiks,
Dmitry/C-7612-2014; Amati, Lorenzo/N-5586-2015; Pal'shin,
Valentin/F-3973-2014; Orlandini, Mauro/H-3114-2014; Ulanov,
Mikhail/B-3467-2015; Aptekar, Raphail/B-3456-2015; Golenetskii,
Sergey/B-3818-2015; Terada, Yukikatsu/A-5879-2013; Nicastro,
Luciano/F-5866-2015
OI Costa, Enrico/0000-0003-4925-8523; Donnarumma,
Immacolata/0000-0002-4700-4549; Marisaldi, Martino/0000-0002-4000-3789;
Labanti, Claudio/0000-0002-5086-3619; galli,
marcello/0000-0002-9135-3228; Pacciani, Luigi/0000-0001-6897-5996;
Frederiks, Dmitry/0000-0002-1153-6340; Feroci,
Marco/0000-0002-7617-3421; Soffitta, Paolo/0000-0002-7781-4104;
Fuschino, Fabio/0000-0003-2139-3299; Lazzarotto,
Francesco/0000-0003-4871-4072; Amati, Lorenzo/0000-0001-5355-7388;
Orlandini, Mauro/0000-0003-0946-3151; Ulanov,
Mikhail/0000-0002-0076-5228; Terada, Yukikatsu/0000-0002-2359-1857;
Nicastro, Luciano/0000-0001-8534-6788
FU Russian Space Agency; RFBR [12-02-00032a, 13-02-12017-ofi-m]; IPN under
NASA; IPN under JPL; IPN under MIT; JPL [958056, 1268385, 1282043];
[NNX07AH52G]; [NNX12AE41G]; [NAG5-12614]; [NNG04GM50G];
[NNG06GE69G]; [NNX07AQ22G]; [NNX08AC90G]; [NNX08AX95G];
[NNX09AR28G]; [NNG05GTF72G]; [NNG06GI89G]; [NNX07AJ65G];
[NNX08AN23G]; [NNX09AO97G]; [NNX10AI23G]; [NNX12AD68G]; [NAG5-3500];
[NAG5-9503]; [MIT-SC-R-293291]; [NAG5-11451]; [NNX06AI36G];
[NNX08AB84G]; [NNX08AZ85G]; [NNX09AV61G]; [NNX10AR12G];
[NNX09AU03G]; [NNX10AU34G]; [NNX11AP96G]; [NNX07AR71G]; [NAG5-7766];
[NAG5-9126]; [NAG5-10710]
FX The Konus-Wind experiment is supported by a Russian Space Agency
contract and RFBR grants 12-02-00032a and 13-02-12017-ofi-m. K. H. is
grateful for IPN support under the following NASA, JPL, and MIT grants
and contracts. JPL 958056 and 1268385 (Ulysses); NNX07AH52G and
NNX12AE41G (ADA and ADAP); NAG5-12614, NNG04GM50G, NNG06GE69G,
NNX07AQ22G, NNX08AC90G, NNX08AX95G and NNX09AR28G (INTEGRAL);
NNG05GTF72G, NNG06GI89G, NNX07AJ65G, NNX08AN23G, NNX09AO97G, NNX10AI23G,
and NNX12AD68G (Swift); NAG5-3500 and NAG5-9503 (NEAR); MIT-SC-R-293291
and NAG5-11451 (HETE-2); JPL 1282043 (Odyssey); NNX06AI36G, NNX08AB84G,
NNX08AZ85G, NNX09AV61G, NNX10AR12G (Suzaku); NNX09AU03G, NNX10AU34G, and
NNX11AP96G (Fermi); NNX07AR71G (MESSENGER); NAG5-7766, NAG5-9126, and
NAG5-10710 (BeppoSAX).
NR 65
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U1 1
U2 13
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0067-0049
EI 1538-4365
J9 ASTROPHYS J SUPPL S
JI Astrophys. J. Suppl. Ser.
PD AUG
PY 2013
VL 207
IS 2
AR UNSP 38
DI 10.1088/0067-0049/207/2/38
PG 14
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 195NO
UT WOS:000322710000020
ER
PT J
AU Trajano, HL
Engle, NL
Foston, M
Ragauskas, AJ
Tschaplinski, TJ
Wyman, CE
AF Trajano, Heather L.
Engle, Nancy L.
Foston, Marcus
Ragauskas, Arthur J.
Tschaplinski, Timothy J.
Wyman, Charles E.
TI The fate of lignin during hydrothermal pretreatment
SO BIOTECHNOLOGY FOR BIOFUELS
LA English
DT Article
DE Condensation; Depolymerization; Flowthrough pretreatment; Hydrothermal
pretreatment; Lignin-carbohydrate complex; Phase transition
ID EXTRACTED AUTOHYDROLYSIS LIGNIN; POPULUS-TREMULOIDES LIGNINS; MILLED
WOOD LIGNIN; TOTAL MASS REMOVAL; CORN STOVER; ENZYMATIC-HYDROLYSIS;
STRUCTURAL-CHANGES; MODEL COMPOUNDS; ASPEN WOOD; FLOW-RATE
AB Background: Effective enzymatic hydrolysis of lignocellulosic biomass benefits from lignin removal, relocation, and/or modification during hydrothermal pretreatment. Phase transition, depolymerization/repolymerization, and solubility effects may all influence these lignin changes. To better understand how lignin is altered, Populus trichocarpa x P. deltoides wood samples and cellulolytic enzyme lignin (CEL) isolated from P. trichocarpa x P. deltoides were subjected to batch and flowthrough pretreatments. The residual solids and liquid hydrolysate were characterized by gel permeation chromatography, heteronuclear single quantum coherence NMR, compositional analysis, and gas chromatography-mass spectrometry.
Results: Changes in the structure of the solids recovered after the pretreatment of CEL and the production of aromatic monomers point strongly to depolymerization and condensation being primary mechanisms for lignin extraction and redeposition. The differences in lignin removal and phenolic compound production from native P. trichocarpa x P. deltoides and CEL suggested that lignin-carbohydrate interactions increased lignin extraction and the extractability of syringyl groups relative to guaiacyl groups.
Conclusions: These insights into delignification during hydrothermal pretreatment point to desirable pretreatment strategies and plant modifications. Because depolymerization followed by repolymerization appears to be the dominant mode of lignin modification, limiting the residence time of depolymerized lignin moieties in the bulk liquid phase should reduce lignin content in pretreated biomass. In addition, the increase in lignin removal in the presence of polysaccharides suggests that increasing lignin-carbohydrate cross-links in biomass would increase delignification during pretreatment.
C1 [Trajano, Heather L.; Wyman, Charles E.] Univ Calif Riverside, Dept Environm Chem & Engn, Riverside, CA 92507 USA.
[Trajano, Heather L.; Wyman, Charles E.] Univ Calif Riverside, Ctr Environm Res & Technol, Bourns Coll Engn, Riverside, CA 92507 USA.
[Engle, Nancy L.; Tschaplinski, Timothy J.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA.
[Foston, Marcus; Ragauskas, Arthur J.] Georgia Inst Technol, Sch Chem & Biochem, Inst Paper Sci & Technol, Atlanta, GA 30332 USA.
[Foston, Marcus] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA.
[Trajano, Heather L.; Engle, Nancy L.; Foston, Marcus; Ragauskas, Arthur J.; Tschaplinski, Timothy J.; Wyman, Charles E.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA.
RP Wyman, CE (reprint author), Univ British Columbia, Dept Chem & Biol Engn, 2360 East Mall, Vancouver, BC V6T 1Z3, Canada.
EM cewyman@engr.ucr.edu
OI Tschaplinski, Timothy/0000-0002-9540-6622; Engle,
Nancy/0000-0003-0290-7987
FU Office of Biological and Environmental Research in the DOE Office of
Science through the BioEnergy Science Center (BESC); Office of
Biological and Environmental Research in the DOE Office of Science; U.S.
Government [DE-AC05-00OR22725]
FX We thank the Office of Biological and Environmental Research in the DOE
Office of Science for supporting this work through the BioEnergy Science
Center (BESC). BESC is a U.S. Department of Energy Bioenergy Reseach
Center supported by the Office of Biological and Environmental Research
in the DOE Office of Science. This manuscript has been co-authored by a
contractor of the U.S. Government under contract DE-AC05-00OR22725. We
also wish to thank Dr. Shilin Cao, previously at the School of Chemistry
and Biochemistry, Institute of Paper Science and Technology, Georgia
Institute of Technology and now at the College of Material Engineering
at Fujian Agriculture and Forestry University, for preparing the
cellulolytic enzyme lignin for this study. We acknowledge support by the
Ford Motor Company for the Chair in Environmental Engineering at the
University of California Riverside (UCR) that augments our ability to
perform such research.
NR 48
TC 48
Z9 48
U1 7
U2 132
PU BIOMED CENTRAL LTD
PI LONDON
PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND
SN 1754-6834
J9 BIOTECHNOL BIOFUELS
JI Biotechnol. Biofuels
PD AUG 1
PY 2013
VL 6
AR 110
DI 10.1186/1754-6834-6-110
PG 16
WC Biotechnology & Applied Microbiology; Energy & Fuels
SC Biotechnology & Applied Microbiology; Energy & Fuels
GA 201TN
UT WOS:000323166000001
PM 23902789
ER
PT J
AU Fiaux, P
Sun, MY
Bradel, L
North, C
Ramakrishnan, N
Endert, A
AF Fiaux, Patrick
Sun, Maoyuan
Bradel, Lauren
North, Chris
Ramakrishnan, Naren
Endert, Alex
TI Bixplorer: Visual Analytics with Biclusters
SO COMPUTER
LA English
DT Editorial Material
AB A prototype visual analytics tool uses data mining algorithms to find patterns in textual datasets and then supports exploration of these patterns in the form of biclusters on a high-resolution display.
C1 [Fiaux, Patrick; Sun, Maoyuan; Bradel, Lauren; North, Chris] Virginia Tech, Dept Comp Sci, Blacksburg, VA USA.
[North, Chris] Virginia Tech, InfoVis Lab, Nashville, TN USA.
[Endert, Alex] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Fiaux, P (reprint author), Virginia Tech, Dept Comp Sci, Blacksburg, VA USA.
EM pfiaux@cs.vt.edu; smaoyuan@cs.vt.edu; lbradel1@vt.edu; north@vt.edu;
naren@cs.vt.edu; alex.endert@pnnl.gov
NR 0
TC 3
Z9 3
U1 0
U2 1
PU IEEE COMPUTER SOC
PI LOS ALAMITOS
PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA
SN 0018-9162
J9 COMPUTER
JI Computer
PD AUG
PY 2013
VL 46
IS 8
BP 90
EP 94
PG 5
WC Computer Science, Hardware & Architecture; Computer Science, Software
Engineering
SC Computer Science
GA 201LL
UT WOS:000323143000021
ER
PT J
AU Shekhawat, D
Srivastava, RD
Ciferno, J
Litynski, J
Morreale, BD
AF Shekhawat, Dushyant
Srivastava, Rameshwar D.
Ciferno, Jared
Litynski, John
Morreale, Bryan D.
TI Accelerating Technology Development through Integrated Computation and
Experimentation
SO ENERGY & FUELS
LA English
DT Editorial Material
C1 [Shekhawat, Dushyant; Ciferno, Jared; Litynski, John; Morreale, Bryan D.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
[Srivastava, Rameshwar D.] US DOE, Natl Energy Technol Lab, KeyLog Syst Inc, Pittsburgh, PA 15236 USA.
RP Shekhawat, D (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA.
NR 0
TC 0
Z9 0
U1 0
U2 36
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4085
EP 4086
DI 10.1021/ef400975r
PG 2
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300001
ER
PT J
AU Miller, DD
Siriwardane, R
AF Miller, Duane D.
Siriwardane, Ranjani
TI Mechanism of Methane Chemical Looping Combustion with Hematite Promoted
with CeO2
SO ENERGY & FUELS
LA English
DT Article
ID OXYGEN STORAGE CAPACITY; 3-WAY CATALYSTS; IRON-OXIDE; CERIA; CARRIERS;
REACTIVITY; SYSTEM; MOBILITY; HYDROGEN; BEHAVIOR
AB Chemical looping combustion (CLC) is a promising technology for fossil fuel combustion that produces sequestration-ready CO2 stream, reducing the energy penalty of CO2 separation from flue gases. An effective oxygen carrier for CLC will readily react with the fuel gas and will be reoxidized upon contact with oxygen. This study investigated the development of a CeO2-promoted Fe2O3-hematite oxygen carrier suitable for the methane CLC process. Composition of CeO2 is between S and 25 wt % and is lower than what is generally used for supports in Fe2O3 carrier preparations. The incorporation of CeO2 to the natural ore hematite strongly modifies the reduction behavior in comparison to that of CeO2 and hematite alone. Temperature-programmed reaction studies revealed that the addition of even 5 wt % CeO2 enhances the reaction capacity of the Fe2O3 oxygen carrier by promoting the decomposition and partial oxidation of methane. Fixed-bed reactor data showed that the 5 wt % cerium oxides with 95 wt % iron oxide produce 2 tithes as much carbon dioxide in comparison to the sum of carbon dioxide produced when the oxides were tested separately. This effect is likely due to the reaction of CeO2 with methane forming intermediates, which are reactive for extracting oxygen from Fe2O3 at a considerably faster rate than the rate of the direct reaction of Fe2O3 with methane. These studies reveal that 5 wt % CeO2/Fe2O3 gives stable conversions over 15 reduction/oxidation cycles. Lab-scale reactor studies (pulsed Mode) suggest the methane reacts initially with CeO2 lattice oxygen to form partial oxidation products (CO + H-2), which continue to react with oxygen from neighboring Fe2O3, leading to its complete oxidation to form CO2. The reduced cerium oxide promotes the methane decomposition reaction to form C + H-2, which continue to react with Fe2O3/Fe3O4 to form CO/CO2 and H2O. This mechanism is supported by the characterization studies, which also suggest that the formation of carbonaceous intermediates may affect the reaction rate and selectivity of the oxygen carrier.
C1 [Miller, Duane D.; Siriwardane, Ranjani] US DOE, NETL, Morgantown, WV 26507 USA.
[Miller, Duane D.] URS Corp, Morgantown, WV 26507 USA.
RP Miller, DD (reprint author), US DOE, NETL, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA.
EM duane.miller@netl.doe.gov
FU NETL's ongoing research on CO2 capture in the Separations and
Fuels Processing Division [DE-FE0004000]
FX We thank Esmail Monazam for his help with the Gibbs energy calculations.
This technical work was performed in support of NETL's ongoing research
on CO2 capture in the Separations and Fuels Processing
Division (Project DE-FE0004000).
NR 40
TC 12
Z9 13
U1 6
U2 88
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4087
EP 4096
DI 10.1021/ef302132e
PG 10
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300002
ER
PT J
AU Tian, HJ
Siriwardane, R
Simonyi, T
Poston, J
AF Tian, Hanjing
Siriwardane, Ranjani
Simonyi, Thomas
Poston, James
TI Natural Ores as Oxygen Carriers in Chemical Looping Combustion
SO ENERGY & FUELS
LA English
DT Article
ID SOLID FUELS; COAL; HYDROGEN; NIO; ILMENITE; KINETICS; MN3O4; FE2O3
AB Chemical looping combustion (CLC) is a combustion technology that utilizes from oxygen carriers (OC), such as metal oxides, instead of air to combust fuels. The use of natural minerals as oxygen carriers has advantages, such as lower cost and availability. Eight materials, based on copper or iron oxides, were selected for screening tests of CLC processes using coal and methane as fuels. Thermogravimetric experiments and bench-scale fixed-bed reactor tests were conducted to investigate the oxygen transfer capacity, reaction kinetics, and stability during cyclic reduction/oxidation reaction. Most natural minerals showed lower combustion capacity than pure CuO/Fe2O3 due to low-concentration of active oxide species in minerals. In coal CLC, chryscolla (Cu-based), magenetite, and limonite (Fe-based) demonstrated better reaction performance than other materials. The addition of steam improved the coal CLC performance when using natural ores because of the steam gasification of coal and the subsequent reaction of gaseous fuels with active oxide species in the natural ores. In methane CLC, chryscolla, hematite, and limonite demonstrated excellent reactivity and stability in 50-cycle thermogravimetric analysis tests. Fe2O3-based ores process greater oxygen utilization but require an activation period before achieving full performance in methane CLC. Particle agglomeration issues associated with the application of natural ores in CLC process were also studied by scanning electron microscopy (SEM).
C1 [Tian, Hanjing; Siriwardane, Ranjani; Simonyi, Thomas; Poston, James] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
[Tian, Hanjing; Simonyi, Thomas] URS, Morgantown, WV 26507 USA.
RP Siriwardane, R (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA.
EM ranjani.siriwardane@netl.doe.gov
NR 26
TC 16
Z9 16
U1 6
U2 81
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4108
EP 4118
DI 10.1021/ef301486n
PG 11
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300004
ER
PT J
AU Godec, ML
Kuuskraa, VA
Dipietro, P
AF Godec, Michael L.
Kuuskraa, Vello A.
Dipietro, Phil
TI Opportunities for Using Anthropogenic CO2 for Enhanced Oil Recovery and
CO2 Storage
SO ENERGY & FUELS
LA English
DT Article
AB CO2-enhanced Oil recovery (CO2=EOR) has emerged as a Major option for productively using CO2 emissions. captured from electric power and other industrial facilities as part of carbon capture and storage (CCS) operations. Not only can depleting oil fields provide secure, well-characterized sites for storing CO2, such fields can also provide a source of revenues to offset the costs of capturing CO2 by producing incremental oil. This paper draws significantly on work by Advanced Resources International, Inc. (ARI), sponsored by the United States Department of Energy's National Energy Technology Laboratory (U.S. DOE/NETL) [Advanced Resources International, Inc. (ARI). Improving Domestic Energy Security and Lowering CO2 Emissions with "Next Generation" CO2-Enhanced Oil Recovery; ARI: Arlington, VA; 2011; http://www.netl.doe.gov/energy-analyses/pubs/storing%20co2%20w%eor_final.pdf] and the International Energy Agency Greenhouse Gas Research and Development Programme (IEAGHG) [Advanced Resources International, Inc: (ARI). CO2 Storage in Depleted,Oilfields Global Application Criteria for Carbon. Dioxide Enhanced Oil Recovery; ARI: Arlington, VA, Dec 2009; IEAGHG Programme Technical Report Number 2009-12], that demonstrates that CO2-EOR Offers large CO2 storage capacity potential and could accommodate a major portion of the CO2 captured from industrial facilities for the next 30 years. This work also demonstrates that CO2 can be effectively and permanently stored when deployed in association with CO2-EOR, with the amount stored depending upon the, priority placed on maximizing storage. In addition to showing that CCS benefits from CO2-EOR by providing the revenues from sale of CO2, overcoming other barriers, while producing oil with a lower CO2 emissions "footprint", the report demonstrates that, CO2-EOR needs CCS, because large-scale future implementation of CO2-EOR will be dependent upon CO2 supplies from industrial sources.
C1 [Godec, Michael L.; Kuuskraa, Vello A.] Adv Resources Int Inc ARI, Arlington, VA 22203 USA.
[Dipietro, Phil] US DOE, NETL, Pittsburgh, PA 15236 USA.
RP Godec, ML (reprint author), Adv Resources Int Inc ARI, 4501 Fairfax Dr,Suite 910, Arlington, VA 22203 USA.
EM mgodec@adv-res.com
FU U.S. DOE/NETL; IEAGHG; U.K. Department of Energy and Climate Change
FX The results presented in this paper were sponsored by the U.S. DOE/NETL,
the IEAGHG, and the U.K. Department of Energy and Climate Change.
NR 9
TC 20
Z9 22
U1 3
U2 38
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4183
EP 4189
DI 10.1021/ef302040u
PG 7
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300012
ER
PT J
AU Brunet, JPL
Li, L
Karpyn, ZT
Kutchko, BG
Strazisar, B
Bromhal, G
AF Brunet, Jean-Patrick Leopold
Li, Li
Karpyn, Zuleima T.
Kutchko, Barbara G.
Strazisar, Brian
Bromhal, Grant
TI Dynamic Evolution of Cement Composition and Transport Properties under
Conditions Relevant to Geological Carbon Sequestration
SO ENERGY & FUELS
LA English
DT Article
ID H WELL CEMENT; PERMEABILITY-POROSITY RELATIONSHIPS; CO2
STORAGE-CONDITIONS; AQUEOUS NACL SOLUTIONS; REACTIVE SURFACE-AREA;
LIMESTONE DISSOLUTION; HYDROTHERMAL SYSTEMS; CHEMICAL-REACTIONS;
PORE-SCALE; LEAKAGE
AB Assessing the possibility of CO2 leakage is one of the challenges for geological carbon sequestration. Injected CO2 can react with wellbore cement, which can potentially change cement composition and transport properties. In this work, we develop a reactive transport model based on experimental observations understand and predict the property evolution of Cement in direct contact with CO2-saturated brine under, diffusion controlled conditions. The model reproduced the observed zones, of portlandite depletion and calcite formation. Cement alteration is initially fast and slows down at later times This work also quantified the role of initial cement properties, in particular the ratio of the initial portlandite content to porosity (defined here as phi), in determining the evolution of cement properties. Portlandite-rich cement with large phi values results in a, localized "sharp" reactive diffusive front characterized by calcite precipitation, leading to significant porosity reduction, which eventually clogs the pore space and prevents further acid penetration. Severe degradation occurs at the cement-brine interface with large phi values. This alteration increases effective permeability by orders of magnitude for fluids that preferentially flow through the degraded zone. The significant porosity decrease in the calcite zone also leads to orders of magnitude decrease in effective permeability, where fluids flow through the low-permeability calcite zone also leads to orders of magnitude decrease in provides a valuable tool to link cement-CO2 reactions with the evolution of porosity and permeability. It can be used to quantify and predict long-term wellbore cement behavior and can facilitate the risk assessment associated with geological CO2 sequestration.
C1 [Brunet, Jean-Patrick Leopold; Li, Li; Karpyn, Zuleima T.] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA.
[Brunet, Jean-Patrick Leopold; Li, Li; Karpyn, Zuleima T.] Penn State Univ, Earth & Mineral Sci EMS Energy Inst, University Pk, PA 16802 USA.
[Li, Li] Penn State Univ, Earth & Environm Syst Inst, University Pk, PA 16802 USA.
[Kutchko, Barbara G.; Strazisar, Brian] US DOE, NETL, Pittsburgh, PA 15236 USA.
[Bromhal, Grant] US DOE, NETL, Morgantown, WV 26507 USA.
RP Li, L (reprint author), Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA.
EM lili@eme.psu.edu
RI Li, Li/A-6077-2008
OI Li, Li/0000-0002-1641-3710
FU National Energy Technology Laboratory (NETL), U.S. Department of Energy,
an agency of the United States Government [RES1000026]; URS Energy and
Construction, Inc.
FX This project was funded by the National Energy Technology Laboratory
(NETL), U.S. Department of Energy, an agency of the United States
Government, through a support contract through Project RES1000026 with
URS Energy and Construction, Inc.
NR 73
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U2 32
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4208
EP 4220
DI 10.1021/ef302023v
PG 13
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300015
ER
PT J
AU Deng, H
Ellis, BR
Peters, CA
Fitts, JP
Crandall, D
Bromhal, GS
AF Deng, Hang
Ellis, Brian R.
Peters, Catherine A.
Fitts, Jeffrey P.
Crandall, Dustin
Bromhal, Grant S.
TI Modifications of Carbonate Fracture Hydrodynamic Properties by
CO2-Acidified Brine Flow
SO ENERGY & FUELS
LA English
DT Article
ID ROUGH-WALLED FRACTURES; FLUID-FLOW; APERTURE FIELDS; SINGLE FRACTURE;
ROCK FRACTURES; CO2 STORAGE; PERMEABILITY; TRANSPORT; DISSOLUTION;
SYSTEMS
AB Acidic reactive flow in fractures is relevant in subsurface activities, such as CO2 geological storage and hydraulic fracturing. Understanding reaction-induced changes in fracture hydrodynmic properties is essential for predicting subsurface flows, such as leakage, injectability, and fluid production. In this study, X-ray computed tomography scans of a fractured carbonate caprock were used. to create three-dimensional (3D) reconstructions of the fracture before and after reaction with CO2-acidified brine (Ellis; B; Peters, C.; Fitts, J.; Bromhal, G.; McIntyre, D.; Warzinski, R.; Rosenbaum, E. Deterioration of a fractured carbonate caprock exposed to CO2-acidified brine flow. Greenhouse Gases: Sci. Technol. 2011, 1, 248-260). As expected, mechanical apertures were found to increase substantially, doubling and even tripling in some places. However, the surface geometry evolved in complex ways, including "comb-tooth" structures created from preferential dissolution of calcite in transverse sedimentary, bands and the creation of degraded zones, i.e., porous calcite-depleted areas in reacted fracture surfaces. These geometric alterations resulted in increased fracture roughness, as measured by surface Z(2) parameters and fractal dimensions D-f. Computational fluid dynamics (CFD) simulations were conducted to quantify the changes in hydraulic apertaure, fracture transmissivity, and permeability. The result shows that the effective hydraulic aperatures are smaller than the mechanical aperatures and the changes in hydraulic aperatures are nonlinear. Overestimation of the flow rate by a factor of 2 or more would be introduced if fracture hydrodynamic properties were based on mechanical aperatures or if hydraulic aperture is assumed to change proportionally with mechanical aperture The difference can be attributed, in part, to the increase in roughness after reaction and is likely affected by contiguous transverse sedimentary features. Hydraulic apertures estimated by the one-dimensional (1D) statistical model and two-dimensional (2D) local cubic law (LCL) model are consistently larger than those calculated from the CFD simulations. In addition, a novel ternary segmentation method was devised to handle the degraded zones, allowing for a bounding analysis of the effects on hydraulic properties. We found that the degraded zones account for less than 15% of the fracture volume but cover 70-80% of the fracture surface. When the degraded zones are treated as part of the the fracture transmissivities are 2-4 times larger because the fracture, surfaces after reaction are not as rough as they would be if one considers the degraded zone as part of the rock. Therefore, while degraded zones created during geochemical reactions may not significantly, increase mechanical aperture, this type of feature cannot he ignored and should be treated with prudence when predicting fracture hydrodynamic properties.
C1 [Deng, Hang; Ellis, Brian R.; Peters, Catherine A.; Fitts, Jeffrey P.] Princeton Univ, Princeton, NJ 08544 USA.
[Crandall, Dustin; Bromhal, Grant S.] Natl Energy Technol Lab, Morgantown, WV 26507 USA.
[Crandall, Dustin] URS Corp, Morgantown, WV 26507 USA.
RP Peters, CA (reprint author), Princeton Univ, Princeton, NJ 08544 USA.
EM cap@princeton.edu
RI Fitts, Jeffrey/J-3633-2012; Peters, Catherine/B-5381-2013; Deng,
Hang/E-5302-2015
OI Peters, Catherine/0000-0003-2418-795X; Deng, Hang/0000-0001-5784-996X
FU Department of Energy (DOE) [DE-FE0000749, DE-FG02-09ER64748]; National
Science Foundation (NSF) [CBET-1134397]; National Energy Technology
Laboratory under the RES [DE-FE0004000]
FX This work is funded by Department of Energy (DOE) awards DE-FE0000749
and DE-FG02-09ER64748, as well as by National Science Foundation (NSF)
Grant CBET-1134397. Additional support came from the National Energy
Technology Laboratory's ongoing research under the RES contract
DE-FE0004000. We also thank the anonymous reviewers for their insightful
comments, which led to valuable improvements in the manuscript.
NR 52
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Z9 25
U1 9
U2 67
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
EI 1520-5029
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4221
EP 4231
DI 10.1021/ef302041s
PG 11
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300016
ER
PT J
AU Siriwardane, HJ
Gondle, RK
Bromhal, GS
AF Siriwardane, Hema J.
Gondle, Raj K.
Bromhal, Grant S.
TI Coupled Flow and Deformation Modeling of Carbon Dioxide Migration in the
Presence of a Caprock Fracture during Injection
SO ENERGY & FUELS
LA English
DT Article
ID RESERVOIR-GEOMECHANICAL ANALYSIS; DEEP SALINE AQUIFERS; NORTHERN
NORTH-SEA; CO2 STORAGE SITE; FLUID-FLOW; GEOLOGICAL STORAGE; PLUME
BEHAVIOR; GAS-RESERVOIRS; SEQUESTRATION; PRESSURE
AB Understanding the transport of carbon dioxide (CO2) during long-term CO2 injection into a typical geologic reservoir, such as a saline aquifer, could be complicated because of changes in geochemical, hydrogeological, and hydromechanical behaviour. While the caprock layer overlying the target aquifer is intended to provide a tight, impermeable seal in securing injected CO2, the presence of geologic uncertainties, such as a caprock fracture or fault, may provide a channel for CO2 leakage. There could also be a possibility of the activation of a new or existing dormant fault or fracture, which could act as a leakage pathway. Such a leakage event during CO2 injection may lead to a different pressure and ground response over a period of time. In the present study, multiphase fluid flow simulations in porous media coupled with geomechanics were used to investigate the overburden geologic response and plume behavior during CO2 injection in the presence of a hypothetical permeable fractured zone in a caprock, existing or activated. Both single-phase and multiphase fluid flow simulations were performed. The CO2 migration through an existing fractured zone leads to changes in the fluid pressure in the overburden geologic layers and could have a significant impact on ground deformation behavior. Results of the study show that pressure signature and displacement patterns are significantly different in the presence of a fractured zone in the caprock layer. The variation in pressure and displacement signatures because of the presence of a fractured zone in the caprock at different locations may be useful in identifying the presence of a fault/fractured zone in the caprock. The pressure signatures can also serve as a mechanism to identify the activation of leakage pathways through the caprock during CO2 injection. Pressure response and ground deformation behaviour from sequestration modeling could be useful in the development of smart technologies to monitor safe CO2 storage and understand CO2 transport, with limited field instrumentation.
C1 [Siriwardane, Hema J.; Gondle, Raj K.] W Virginia Univ, NETL RUA, Morgantown, WV 26506 USA.
[Siriwardane, Hema J.; Gondle, Raj K.] W Virginia Univ, Dept Civil & Environm Engn, Morgantown, WV 26506 USA.
[Bromhal, Grant S.] US DOE, NETL, Morgantown, WV 26507 USA.
RP Siriwardane, HJ (reprint author), W Virginia Univ, NETL RUA, Morgantown, WV 26506 USA.
EM hema.siriwardane@mail.wvu.edu
FU URS Energy & Construction, Inc. under RES [RES1000023]
FX The work presented in this paper was performed with the funding provided
by URS Energy & Construction, Inc. under RES Contract RES1000023 to
support National Energy Technology Laboratory's ongoing research in
CO2 sequestration. Also, the authors greatly acknowledge the
Computer Modeling Group (CMG) for their technical support.
NR 64
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Z9 8
U1 2
U2 50
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4232
EP 4243
DI 10.1021/ef400194n
PG 12
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300017
ER
PT J
AU Lister, TE
Dufek, EJ
AF Lister, Tedd E.
Dufek, Eric J.
TI Chlor-syngas: Coupling of Electrochemical Technologies for Production of
Commodity Chemicals
SO ENERGY & FUELS
LA English
DT Article
ID CARBON-DIOXIDE; METAL-ELECTRODES; LOW-TEMPERATURE; AG ELECTRODES; CO2
REDUCTION; REACTOR; CELL; OPERATION; METHANE; FUTURE
AB This paper describes a novel electrolysis process called chlor-syngas, where synthesis gas is produced at the cathode and chlorine gas is produced at the anode. The work presented is an extension of previous electrolysis system development, where syngas was cathodically generated from water, CO2, and electricity. The process described here uses chloride-based electrolytes. Using HCl as the anolyte provides a low-cost source of Cl-, and leakage of excess protons lowers the catholyte pH, preventing carbonate buildup in the catholyte. Initial electrolysis data are presented here to demonstrate the feasibility of the process in KCl/KCl and KCl/HCl electrolytes. Using the electrolysis data, an estimation of the energetic and environmental benefits is presented. The process could be a path to a more sustainable chemical industry, where the starting materials are low-value or wastes from other related processes.
C1 [Lister, Tedd E.; Dufek, Eric J.] INL, Idaho Falls, ID 83404 USA.
RP Lister, TE (reprint author), INL, POB 1625, Idaho Falls, ID 83404 USA.
EM tedd.lister@inl.gov
RI Dufek, Eric/B-8847-2017
OI Dufek, Eric/0000-0003-4802-1997
FU INL Laboratory Directed Research and Development (LDRD) Program under
DOE Idaho Operations Office; U.S. Department of Energy
[DE-AC07-05ID14517]
FX We acknowledge Dr. Lenny Scott of Olin Chemical (Augusta, GA) for
providing helpful discussion in the development of this concept. We also
acknowledge Simon Stone at Giner, Inc. for helpful discussions about
this work. Work was supported through the INL Laboratory Directed
Research and Development (LDRD) Program under DOE Idaho Operations
Office. This manuscript has been authored by Battelle Energy Alliance,
LLC under Contract DE-AC07-05ID14517 with the U.S. Department of Energy.
NR 31
TC 3
Z9 3
U1 2
U2 32
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
EI 1520-5029
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4244
EP 4249
DI 10.1021/ef302033j
PG 6
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300018
ER
PT J
AU Siefert, NS
Shekhawat, D
Litster, S
Berry, DA
AF Siefert, Nicholas S.
Shekhawat, Dushyant
Litster, Shawn
Berry, David A.
TI Steam-Coal Gasification Using CaO and KOH for in Situ Carbon and Sulfur
Capture
SO ENERGY & FUELS
LA English
DT Article
ID CALCIUM-OXIDE SORBENTS; CO2 CAPTURE; HYDROGEN-PRODUCTION; CATALYTIC
GASIFICATION; DIOXIDE CAPTURE; SOLID FUELS; SEQUESTRATION; CALCINATION;
PERFORMANCE; TECHNOLOGY
AB We present experimental results of coal gasification with and without the addition of calcium oxide and potassium hydroxide as dual-functioning catalyst capture agents. using different coal types and temperatures 700 and 900 degrees C, we studied the effect of these catalyst-capture agents on (1) the syngas composition, (2) CO2 and H2S capture, and (3) the stem-coal gasification kinetic rate. The syngas composition from the gasifier was roughly 20% methane, 70% hydrogen, and 10% other species when a CaO/C molar ratio of 0.5 was added. We demonstrated significantly enhanced steam-coal gasification kinetic rate when adding small amounts of potassium hydroxide to coal when operating a CaO-CaCO3 chemical looping gasification reactor. For example, the steam-coal, gasification kinetic rate increased 250% when dry mixing calcium oxide at a Ca/C molar ratio of 0.5 with a sub-bituminous coal, and the kinetic rate increased 1000% when aqueously mixing calcium oxide at a Ca/C molar ratio of 0.5 along with potassium-hydroxide at a K/C molar, ratio of 0.06. In addition, we conducted multi-cycle studies in which CaCO3 was calcined by heating to 900 degrees C regenerate the CaO, which was then reused repeated CaO-CaCO3 cycles. The increased steam-coal gasification kinetics rates for both CaO and CaO + KOH persisted even when the material was reused in six cycles of gasification and calcination. The ability of CaO to capture carbon dioxide decreased roughly 2-4% per CaO-CaCO3 cycle. We also discuss an important application of this combined gasifier-calciner to electricity generation and selling the purge stream as a precalcined feedstock to a cement kiln. In this scenario, the amount of purge stream required is fixed not by the degradation in the capture ability but rather by the requirements cement at the cement kiln on the amount of CaSO4 and ash in the precalcined feedstock.
C1 [Siefert, Nicholas S.] US DOE, NETL, Pittsburgh, PA 15236 USA.
[Siefert, Nicholas S.; Litster, Shawn] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA.
[Shekhawat, Dushyant; Berry, David A.] US DOE, NETL, Morgantown, WV 26507 USA.
RP Siefert, NS (reprint author), US DOE, NETL, Pittsburgh, PA 15236 USA.
EM nicholas.siefert@netl.doe.gov
FU NETL Strategic Center for Coal
FX We thank the NETL Strategic Center for Coal for their support of this
research. In particular, we thank Tristan McQuain, Jack Ferrel, Richard
Bergen, David Ruehl, and William Grimes for their expertise during the
operation of the gasifier.
NR 41
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U1 3
U2 70
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4278
EP 4289
DI 10.1021/ef302192p
PG 12
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300022
ER
PT J
AU Smith, MW
Shekhawa, D
Berry, DA
Haynes, DJ
Floyd, DL
Spivey, JJ
Zondlo, JW
AF Smith, Mark W.
Shekhawa, Dushyant
Berry, David A.
Haynes, Daniel J.
Floyd, Donald L.
Spivey, James J.
Zondlo, John W.
TI Effect of the Catalyst Bed Configuration on the Partial Oxidation of
Liquid Hydrocarbons
SO ENERGY & FUELS
LA English
DT Article
ID SYNTHESIS GAS-FORMATION; N-TETRADECANE; HIGH YIELDS; METHANE; SYNGAS;
METAL; PYROCHLORES; SULFUR; RH; COMBUSTION
AB Rh-substituted pyrochlores have been shown to be excellent diesel reforming catalysts. However, it is desirable to reduce the amount of this expensive material while maintaining acceptable level of hydrogen production. This study demonstrates that a segmented catalyst bed approach can be used to achieve this objective. Two strategies were examined: (1) promotion of the indirect reforming mechanism with a combustion catalyst in the reactor inlet, followed by a reforming catalyst, and (2) placement of catalysts in regions of the reactor that have conditions in which they are less likely to deactivate. The first approach demonstrated that a Ni-substituted barium hexaaluminate catalyst can be used in the reactor inlet to promote combustion with a Rh-substituted pyrochlore in the reactor outlet, but the combustion catalyst should fill less than 50% of the reactor. The second approach showed a benefit in the use of a sulfur-tolerant noble metal catalyst in the reactor outlet and that a significant portion of the carbon formed on the Ni-substituted pyrochlore is located of e catalyst bed.
C1 [Smith, Mark W.; Shekhawa, Dushyant; Berry, David A.; Haynes, Daniel J.; Floyd, Donald L.; Spivey, James J.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
[Smith, Mark W.; Floyd, Donald L.] URS Corp, Morgantown, WV 26507 USA.
[Smith, Mark W.; Zondlo, John W.] W Virginia Univ, Morgantown, WV 26506 USA.
[Spivey, James J.] Louisiana State Univ, Baton Rouge, LA 70803 USA.
RP Smith, MW (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA.
EM mark.smith@contr.netl.doe.gov
FU National Energy Technology Laboratory (NETL), U.S. Department of Energy,
Morgantown, WV, under the SECA program; NETL [FE-000004000,
3.610.248.003]
FX This work was supported by the National Energy Technology Laboratory
(NETL), U.S. Department of Energy, Morgantown, WV, under the SECA
program, and was performed in support of NETL's ongoing research in fuel
processing under Contract FE-000004000 Subtask 3.610.248.003.
NR 41
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U1 1
U2 26
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4363
EP 4370
DI 10.1021/ef3021975
PG 8
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300027
ER
PT J
AU Pomerantz, AE
Seifert, DJ
Bake, KD
Craddock, PR
Mullins, OC
Kodalen, BG
Mitra-Kirtley, S
Bolin, TB
AF Pomerantz, Andrew E.
Seifert, Douglas J.
Bake, Kyle D.
Craddock, Paul R.
Mullins, Oliver C.
Kodalen, Brian G.
Mitra-Kirtley, Sudipa
Bolin, Trudy B.
TI Sulfur Chemistry of Asphaltenes from a Highly Compositionally Graded Oil
Column
SO ENERGY & FUELS
LA English
DT Article
ID RAY-ABSORPTION-SPECTROSCOPY; NEAR-EDGE STRUCTURE;
NUCLEAR-MAGNETIC-RESONANCE; LASER MASS-SPECTROMETRY; X-RAY; PETROLEUM
ASPHALTENES; XANES SPECTROSCOPY; ORGANIC SULFUR; SPECIATION; MODEL
AB Hydrocarbons in subsurface reservoirs are generally found to be compositionally graded, with fluids deeper in connected and equilibrated reservoirs being relatively enriched in asphaltenes. These gradients result from effects such as gravity, entropy, and solubility. However, it is unclear if those same effects lead to gradients in the detailed molecular composition of asphaltenes. Here, we investigate the sulfur chemistry of asphaltenes from a reservoir with a large gradient in asphaltene content. Measurements of the sulfur content from combustion as well as measurements of sulfur speciation from K-edge X-ray absorption near edge structure (XANES) spectroscopy find no significant difference in the composition of the asphaltenes. Thus, different locations within this reservoir contain oils with different asphaltene concentrations, but the asphaltenes from throughout the reservoir all have the same sulfur chemistry. This result suggests that gradients in asphaltene content can be successfully modeled with the simplifying assumption that the asphaltene molecular composition is not graded in connected and equilibrated reservoirs.
C1 [Pomerantz, Andrew E.; Bake, Kyle D.; Craddock, Paul R.; Mullins, Oliver C.] Schlumberger Doll Res Ctr, Cambridge, MA 02139 USA.
[Seifert, Douglas J.] Saudi Aramco, Dhahran 31311, Saudi Arabia.
[Kodalen, Brian G.; Mitra-Kirtley, Sudipa] Rose Hulman Inst Technol, Terre Haute, IN 47803 USA.
[Bolin, Trudy B.] Argonne Natl Lab, Argonne, IL 60439 USA.
RP Pomerantz, AE (reprint author), Schlumberger Doll Res Ctr, Cambridge, MA 02139 USA.
EM apomerantz@slb.com
OI Craddock, Paul/0000-0003-4702-0204
FU U.S. DOE [DE-AC02-06CH11357]
FX Use of the Advanced Photon Source, an Office of Science User Facility
operated for the United States Department of Energy (U.S. DOE) Office of
Science by Argonne National Laboratory, was supported by the U.S. DOE
under Contract DE-AC02-06CH11357.
NR 45
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U1 0
U2 35
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
J9 ENERG FUEL
JI Energy Fuels
PD AUG
PY 2013
VL 27
IS 8
BP 4604
EP 4608
DI 10.1021/ef400773f
PG 5
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 203OA
UT WOS:000323301300051
ER
PT J
AU Allured, R
Fernandez-Perea, M
Soufli, R
Alameda, JB
Pivovaroff, MJ
Gullikson, EM
Kaaret, P
AF Allured, Ryan
Fernandez-Perea, Monica
Soufli, Regina
Alameda, Jennifer B.
Pivovaroff, Michael J.
Gullikson, Eric M.
Kaaret, Philip
TI A soft X-ray beam-splitting multilayer optic for the NASA GEMS Bragg
Reflection Polarimeter
SO EXPERIMENTAL ASTRONOMY
LA English
DT Article
DE Multilayers; X-ray polarimetry; Beamsplitters; Thin films
ID TELESCOPE
AB A soft X-ray, beam-splitting, multilayer optic has been developed for the Bragg Reflection Polarimeter (BRP) on the NASA Gravity and Extreme Magnetism Small Explorer Mission (GEMS). The optic is designed to reflect 0.5 keV X-rays through a angle to the BRP detector, and transmit 2-10 keV X-rays to the primary polarimeter. The transmission requirement prevents the use of a thick substrate, so a 2 mu m thick polyimide membrane was used. Atomic force microscopy has shown the membrane to possess high spatial frequency roughness less than 0.2 nm rms, permitting adequate X-ray reflectance. A multilayer thin film was especially developed and deposited via magnetron sputtering with reflectance and transmission properties that satisfy the BRP requirements and with near-zero stress. Reflectance and transmission measurements of BRP prototype elements closely match theoretical predictions, both before and after rigorous environmental testing.
C1 [Allured, Ryan; Kaaret, Philip] Univ Iowa, Iowa City, IA 52242 USA.
[Fernandez-Perea, Monica; Soufli, Regina; Alameda, Jennifer B.; Pivovaroff, Michael J.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Gullikson, Eric M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Allured, R (reprint author), Univ Iowa, Iowa City, IA 52242 USA.
EM rallured@gmail.com
RI Pivovaroff, Michael/M-7998-2014
OI Pivovaroff, Michael/0000-0001-6780-6816
FU U.S. Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]; University of California Lawrence Berkeley National
Laboratory [DE-AC03-76F00098]; Office of Science, Office of Basic Energy
Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; NASA
[NNX08AY58G]
FX The authors would like to thank Bruce Lairson of Luxel Corp. for
providing helpful advice, many polyimide samples for analysis, and
confocal microscope data. We also thank Steve McBride for use of his
thermal cycling chamber, and John Tomsick for making the arrangements.
Ryan Allured and Philip Kaaret are grateful to Takashi Okajima and Yang
Soong at GSFC for guidance during the early stages of reflector
development. We acknowledge that nearly all of our multilayer modeling
was made possible with David Windt's IMD software. This work was
performed under the auspices of the U.S. Department of Energy by
Lawrence Livermore National Laboratory under Contract No.
DE-AC52-07NA27344 and by the University of California Lawrence Berkeley
National Laboratory under Contract No. DE-AC03-76F00098. The Advanced
Light Source is supported by the Director, Office of Science, Office of
Basic Energy Sciences of the U.S. Department of Energy under Contract
No. DE-AC02-05CH11231. Ryan Allured and Philip Kaaret acknowledge
partial support from NASA grant NNX08AY58G.
NR 17
TC 1
Z9 1
U1 1
U2 6
PU SPRINGER
PI DORDRECHT
PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS
SN 0922-6435
J9 EXP ASTRON
JI Exp. Astron.
PD AUG
PY 2013
VL 36
IS 1-2
BP 371
EP 388
DI 10.1007/s10686-013-9337-2
PG 18
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 198HV
UT WOS:000322914200013
ER
PT J
AU Jacob, RE
Colby, SM
Kabilan, S
Einstein, DR
Carson, JP
AF Jacob, Richard E.
Colby, Sean M.
Kabilan, Senthil
Einstein, Daniel R.
Carson, James P.
TI In situ casting and imaging of the rat airway tree for accurate 3D
reconstruction
SO EXPERIMENTAL LUNG RESEARCH
LA English
DT Article
DE airways; bronchial cast; CT; pulmonary; warping
ID RESPIRATORY AIRWAYS; AEROSOL DEPOSITION; PULMONARY AIRWAYS; HUMAN LUNGS;
MODELS; FLOW; SIMULATIONS; REPAIR; VOLUME
AB The use of anatomically accurate, animal-specific airway geometries is important for understanding and modeling the physiology of the respiratory system. One approach for acquiring detailed airway architecture is to create a bronchial cast of the conducting airways. However, typical casting procedures either do not faithfully preserve the in vivo branching angles or produce rigid casts that when removed for imaging are fragile and thus easily damaged. We address these problems by creating an in situ bronchial cast of the conducting airways in rats that can be subsequently imaged in situ using three-dimensional micro-CT imaging. We also demonstrate that deformations in airway branch angles resulting from the casting procedure are small, and that these angle deformations can be reversed through an interactive adjustment of the segmented cast geometry. Animal work was approved by the Institutional Animal Care and Use Committee of Pacific Northwest National Laboratory.
C1 [Jacob, Richard E.; Colby, Sean M.; Kabilan, Senthil; Einstein, Daniel R.; Carson, James P.] Pacific NW Natl Lab, Dept Syst Toxicol, Richland, WA 99352 USA.
RP Jacob, RE (reprint author), Pacific NW Natl Lab, Dept Syst Toxicol, 902 Battelle Blvd, Richland, WA 99352 USA.
EM richard.jacob@pnnl.gov
FU National Heart, Lung, and Blood Institute [R01HL073598]; PNNL through
internal Laboratory Directed Research and Development LDR
[DE-AC05-76RL01830]
FX We thank Tao Ju of Washington University in St. Louis for his helpful
discussions, and T. Curry of PNNL for assistance with animal handling.
This work was supported by award number R01HL073598 from the National
Heart, Lung, and Blood Institute, and by PNNL through internal
Laboratory Directed Research and Development LDRD DE-AC05-76RL01830.
NR 33
TC 5
Z9 5
U1 1
U2 15
PU INFORMA HEALTHCARE
PI LONDON
PA TELEPHONE HOUSE, 69-77 PAUL STREET, LONDON EC2A 4LQ, ENGLAND
SN 0190-2148
J9 EXP LUNG RES
JI Exp. Lung Res.
PD AUG
PY 2013
VL 39
IS 6
BP 249
EP 257
DI 10.3109/01902148.2013.801535
PG 9
WC Respiratory System
SC Respiratory System
GA 198MZ
UT WOS:000322928300004
PM 23786464
ER
PT J
AU Luu, T
AF Luu, Thomas
TI Multi-Baryon Systems from Lattice QCD
SO FEW-BODY SYSTEMS
LA English
DT Article; Proceedings Paper
CT 20th International IUPAP Conference on Few-Body Problems in Physics (FB)
CY AUG 20-25, 2012
CL Fukuoka, JAPAN
SP IUPAP
ID DIBARYON; STATES
AB I provide a short overview of the current status of nuclear physics calculations using lattice quantum chromodynamics (LQCD). I give an heuristic description of how LQCD calculations are performed and how nuclear scattering data are extracted from these calculations, emphasizing the overlap between traditional nuclear many-body theory and LQCD calculations. I look at the Omega (-) Omega (-) system as a concrete example, and in so doing demonstrate the predictive nature of LQCD calculations as applied to nuclear physics.
C1 Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
RP Luu, T (reprint author), Lawrence Livermore Natl Lab, POB 808,L-059, Livermore, CA 94551 USA.
EM tluu@llnl.gov
NR 21
TC 0
Z9 0
U1 1
U2 1
PU SPRINGER WIEN
PI WIEN
PA SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA
SN 0177-7963
J9 FEW-BODY SYST
JI Few-Body Syst.
PD AUG
PY 2013
VL 54
IS 7-10
BP 835
EP 841
DI 10.1007/s00601-013-0695-0
PG 7
WC Physics, Multidisciplinary
SC Physics
GA 192MV
UT WOS:000322489800009
ER
PT J
AU Quaglioni, S
Navratil, P
Hupin, G
Langhammer, J
Romero-Redondo, C
Roth, R
AF Quaglioni, Sofia
Navratil, Petr
Hupin, Guillaume
Langhammer, Joachim
Romero-Redondo, Carolina
Roth, Robert
TI No-Core Shell Model Analysis of Light Nuclei
SO FEW-BODY SYSTEMS
LA English
DT Article; Proceedings Paper
CT 20th International IUPAP Conference on Few-Body Problems in Physics (FB)
CY AUG 20-25, 2012
CL Fukuoka, JAPAN
SP IUPAP
AB The fundamental description of both structural properties and reactions of light nuclei in terms of constituent protons and neutrons interacting through nucleon-nucleon and three-nucleon forces is a long-sought goal of nuclear theory. I will briefly present a promising technique, built upon the ab initio no-core shell model, which emerged recently as a candidate to reach such a goal: the no-core shell model/resonating-group method. This approach, capable of describing simultaneously both bound and scattering states in light nuclei, complements a microscopic cluster technique with the use of two-nucleon realistic interactions, and a microscopic and consistent description of the nucleon clusters. I will discuss applications to light nuclei binary scattering processes and fusion reactions that power stars and Earth based fusion facilities, such as the deuterium-He-3 fusion, and outline the progress toward the inclusion of the three-nucleon force into the formalism and the treatment of three-body clusters.
C1 [Quaglioni, Sofia; Navratil, Petr; Hupin, Guillaume] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
[Navratil, Petr; Romero-Redondo, Carolina] TRIUMF, Vancouver, BC V6T 2A3, Canada.
[Langhammer, Joachim; Roth, Robert] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany.
RP Quaglioni, S (reprint author), Lawrence Livermore Natl Lab, POB 808,L-414, Livermore, CA 94551 USA.
EM quaglioni1@llnl.gov
RI Romero-Redondo, Carolina/D-2381-2014
NR 19
TC 4
Z9 4
U1 0
U2 7
PU SPRINGER WIEN
PI WIEN
PA SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA
SN 0177-7963
EI 1432-5411
J9 FEW-BODY SYST
JI Few-Body Syst.
PD AUG
PY 2013
VL 54
IS 7-10
BP 877
EP 884
DI 10.1007/s00601-012-0505-0
PG 8
WC Physics, Multidisciplinary
SC Physics
GA 192MV
UT WOS:000322489800015
ER
PT J
AU Bacher, AD
Casey, DT
Frenje, JA
Johnson, MJG
Manuel, M
Sinenian, N
Zylstra, AB
Seguin, FH
Li, CK
Petrasso, RD
Glebov, VY
Radha, PB
Meyerhofer, DD
Sangster, TC
McNabb, DP
Amendt, PA
Boyd, RN
Caggiano, JA
Hatchett, SP
Pino, JE
Quaglioni, S
Rygg, JR
Thompson, IJ
Herrmann, HW
Kim, YH
AF Bacher, A. D.
Casey, D. T.
Frenje, J. A.
Johnson, M. J. Gatu
Manuel, M.
Sinenian, N.
Zylstra, A. B.
Seguin, F. H.
Li, C. K.
Petrasso, R. D.
Glebov, V. Yu
Radha, P. B.
Meyerhofer, D. D.
Sangster, T. C.
McNabb, D. P.
Amendt, P. A.
Boyd, R. N.
Caggiano, J. A.
Hatchett, S. P.
Pino, J. E.
Quaglioni, S.
Rygg, J. R.
Thompson, I. J.
Herrmann, H. W.
Kim, Y. H.
TI T-T Neutron Spectrum from Inertial Confinement Implosions
SO FEW-BODY SYSTEMS
LA English
DT Article; Proceedings Paper
CT 20th International IUPAP Conference on Few-Body Problems in Physics (FB)
CY AUG 20-25, 2012
CL Fukuoka, JAPAN
SP IUPAP
AB A new technique that uses inertial confinement implosions for measuring low-energy nuclear reactions important to nuclear astrophysics is described. Simultaneous measurements of n-D and n-T elastic scattering at 14.1 MeV using deuterium-tritium gas-filled capsules provide a proof of principle for this technique. Measurements have been made of D(d,p)T (dd) and T(t,2n)He-4 (tt) reaction yields relative to the D(t,n)He-4 (dt) reaction yield for deuterium-tritium mixtures with f (T) /f (D) between 0.62 and 0.75 and for a wide range of ion temperatures to test our understanding of the implosion processes. Measurements of the shape of the neutron spectrum from the T(t,2n)He-4 reaction have been made for each of these target configurations.
C1 [Bacher, A. D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA.
[Casey, D. T.; Frenje, J. A.; Johnson, M. J. Gatu; Manuel, M.; Sinenian, N.; Zylstra, A. B.; Seguin, F. H.; Li, C. K.; Petrasso, R. D.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA.
[Glebov, V. Yu; Radha, P. B.; Meyerhofer, D. D.; Sangster, T. C.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA.
[McNabb, D. P.; Amendt, P. A.; Boyd, R. N.; Caggiano, J. A.; Hatchett, S. P.; Pino, J. E.; Quaglioni, S.; Rygg, J. R.; Thompson, I. J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Herrmann, H. W.; Kim, Y. H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Bacher, AD (reprint author), Indiana Univ, Dept Phys, Bloomington, IN 47405 USA.
EM bacher@indiana.edu
RI Pino, Jesse/C-9183-2014; Manuel, Mario/L-3213-2015
OI Manuel, Mario/0000-0002-5834-1161
NR 10
TC 1
Z9 1
U1 1
U2 10
PU SPRINGER WIEN
PI WIEN
PA SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA
SN 0177-7963
J9 FEW-BODY SYST
JI Few-Body Syst.
PD AUG
PY 2013
VL 54
IS 7-10
BP 1599
EP 1602
DI 10.1007/s00601-012-0524-x
PG 4
WC Physics, Multidisciplinary
SC Physics
GA 192MV
UT WOS:000322489800169
ER
PT J
AU Gibson, BF
Afnan, IR
AF Gibson, B. F.
Afnan, I. R.
TI The Triton from the Reid93 Potential in the UPA
SO FEW-BODY SYSTEMS
LA English
DT Article; Proceedings Paper
CT 20th International IUPAP Conference on Few-Body Problems in Physics (FB)
CY AUG 20-25, 2012
CL Fukuoka, JAPAN
SP IUPAP
ID 3-NUCLEON SYSTEM
AB The unitary pole approximation (UPA) provides an effective means to construct a rank one separable potential for calculations in which one requires a simple representation of the deuteron and/or triton ground-state wave function. By construction the deuteron wave function and the S-1(0) anti-bound state wave function of the original potential are reproduced. We report results for the corresponding triton ground state. We choose to utilize the realistic Reid93 potential for this purpose. The Reid93 potential, generated by the Nijmegen group, is a Reid-like, partial-wave local potential that produces a chi(2) representation of the nucleon-nucleon (NN) scattering data that is as precise as an NN partial-wave analysis. Results for properties of H-2 and H-3 from the UPA are compared with those for the original potential. To further illustrate the precision of the method, results for properties of the deuteron and triton from the UPA are also compared with those for the original Reid68 potential.
C1 [Gibson, B. F.] Los Alamos Natl Lab, Div Theoret, Astrophys & Cosmol Grp, Los Alamos, NM 87545 USA.
[Afnan, I. R.] Flinders Univ S Australia, Sch Chem & Phys Sci, Adelaide, SA 5001, Australia.
RP Gibson, BF (reprint author), Los Alamos Natl Lab, Div Theoret, Astrophys & Cosmol Grp, Los Alamos, NM 87545 USA.
EM bfgibson@lanl.gov; iraj@chariot.net.au
NR 10
TC 0
Z9 0
U1 0
U2 1
PU SPRINGER WIEN
PI WIEN
PA SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA
SN 0177-7963
J9 FEW-BODY SYST
JI Few-Body Syst.
PD AUG
PY 2013
VL 54
IS 7-10
BP 1641
EP 1643
DI 10.1007/s00601-012-0515-y
PG 3
WC Physics, Multidisciplinary
SC Physics
GA 192MV
UT WOS:000322489800179
ER
PT J
AU Patel, GP
Anderson, DE
Peplov, VV
Saethre, RB
Solley, DJ
Wezensky, MW
AF Patel, Gunjan P.
Anderson, David E.
Peplov, Vladimir V.
Saethre, Robert B.
Solley, Dennis J.
Wezensky, Mark W.
TI Experimental Results from Droop Compensation for the High Voltage
Converter Modulators
SO IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION
LA English
DT Article
DE Accelerators; resonant power conversion; insulated gate bipolar
transistors; pulse width modulation; losses; reliability
AB The High Voltage Convertor Modulators are used to power the RF klystrons used throughout the linear accelerator at the Spallation Neutron Source. The output voltage of the modulator has significant voltage droop and ripple which, combined with low level RF system limitations, affect performance and stability of the accelerator cavities. In conjunction with the progress in the development of the new controller, different modulation techniques were implemented and studied on the test modulator rated at 75 kV, 125 A. This paper presents experimental results from implementation of frequency sweep, phase sweep and combined phase and frequency sweep modulation on the modulator output voltage pulse. Thermal measurements were carried out to determine the effect of these modulations schemes on long term reliability of the modulator. Future plans are also discussed.
C1 [Patel, Gunjan P.; Anderson, David E.; Peplov, Vladimir V.; Saethre, Robert B.; Solley, Dennis J.; Wezensky, Mark W.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA.
RP Patel, GP (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA.
OI Saethre, Robert/0000-0002-7907-3960
FU U.S. Department of Energy [DE-AC05-00OR22725]
FX This work is performed at Oak Ridge National Laboratory, which is
managed by UT-Battelle, LLC for the U.S. Department of Energy under
contract DE-AC05-00OR22725.
NR 16
TC 0
Z9 0
U1 0
U2 3
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 1070-9878
J9 IEEE T DIELECT EL IN
JI IEEE Trns. Dielectr. Electr. Insul.
PD AUG
PY 2013
VL 20
IS 4
BP 1093
EP 1100
PG 8
WC Engineering, Electrical & Electronic; Physics, Applied
SC Engineering; Physics
GA 197EO
UT WOS:000322832600013
ER
PT J
AU Vanderburg, A
Stefani, F
Motes, D
Surls, D
Crawford, M
AF Vanderburg, Andrew
Stefani, Francis
Motes, Doyle
Surls, Dwayne
Crawford, Mark
TI Measurements of Electrical Specific Action to Melt for Brass and
Aluminum Alloys
SO IEEE TRANSACTIONS ON PLASMA SCIENCE
LA English
DT Article
DE Al 2024; Al 6061; aluminum alloy; brass; C27400; electrical action to
melt; exploding wire experiment; specific action to melt
AB This paper describes a novel method for determining the specific action to melt the metals, and reports the values for action to melt that measure for several elements and three alloys: aluminum 2024, aluminum 6061, and C27400 brass. We electrically heat small diameter wires (127 mu m) to the point of vaporization using a slow regime exploding wire experiment. Using high-resolution voltage and current data, we compute the derivative of electrical resistivity with respect to specific electrical action. Features in the plot of this derivative clearly show the onset of melting for many of the materials we tested. We compare our results for copper, silver, aluminum, molybdenum, and titanium to those published by Tucker and Toth in the 1970s. Our data agree with their published values for silver and molybdenum, but not with those for copper, aluminum, and titanium. This paper presents our results and discusses possible reasons for the discrepancies between some of our measurements and those of Tucker and Toth.
C1 [Vanderburg, Andrew] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Stefani, Francis] Univ Texas Austin, Inst Adv Technol, Austin, TX 78759 USA.
[Motes, Doyle] Texas Res Int, Austin, TX 78733 USA.
[Surls, Dwayne] Univ Texas Austin, Austin, TX 78759 USA.
[Crawford, Mark] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Vanderburg, A (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
EM andrew.vanderburg@berkeley.edu; stefani@iat.utexas.edu;
dmotes@tri-austin.com; dwayne_surls@iat.utexas.edu; mtc@lanl.gov
FU U.S. Army [W911QX-07-D-0002]
FX This work was supported by the U.S. Army under Contract
W911QX-07-D-0002.
NR 8
TC 1
Z9 1
U1 0
U2 5
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0093-3813
J9 IEEE T PLASMA SCI
JI IEEE Trans. Plasma Sci.
PD AUG
PY 2013
VL 41
IS 8
BP 2427
EP 2433
DI 10.1109/TPS.2013.2266900
PN 3
PG 7
WC Physics, Fluids & Plasmas
SC Physics
GA 202JX
UT WOS:000323212400027
ER
PT J
AU Smilowitz, HM
Slatkin, DN
Micca, PL
Miura, M
AF Smilowitz, Henry M.
Slatkin, Daniel N.
Micca, Peggy L.
Miura, Michiko
TI Microlocalization of lipophilic porphyrins: Non-toxic enhancers of boron
neutron-capture therapy
SO INTERNATIONAL JOURNAL OF RADIATION BIOLOGY
LA English
DT Article
DE Porphyrins; carborane; confocal microscopy; BNCT
ID TUMOR-BEARING MICE; GLIOBLASTOMA-MULTIFORME; COPPER
OCTABROMOTETRACARBORANYLPHENYLPORPHYRIN; SUBCELLULAR-LOCALIZATION;
BRAIN-TUMORS; PHASE-II; BIODISTRIBUTION; TOXICITY; CELLS;
BORONOPHENYLALANINE
AB Purpose : To compare the macroscopic and microscopic distributions of the novel non-toxic lipophilic porphyrins copper (II) 5,10,15,20-tetrakis-(3-[1,2 dicarba-closo -dodecaboranyl]methoxyphenyl)- porphyrin (CuTCPH), potentially useful for boron neutron-capture therapy (BNCT), with those of its zinc fluorescent congener zinc (II) 5,10,15,20-tetrakis-(3-[1,2 dicarba-closo-dodecaboranyl] methoxyphenyl)-porphyrin (ZnTCPH) in tissues of tumor-bearing mice.
Materials and methods : ZnTCPH and CuTCPH were synthesized, then injected intraperitoneally (ip) into tumor-bearing mice. Macroscopic biodistribution was assessed by determining average boron concentrations in tumor, blood, brain, skin, and liver using atomic-emission spectrometry. The euthanized mice and their vital organs were photographed first under an ultraviolet lamp and then under a bright fluorescent lamp. Thin sections of liver and tumor were analyzed by confocal fluorescence microscopy (CFM).
Results : ZnTCPH-injected, but not CuTCPH-injected mice bearing subcutaneous tumors showed fluorescence from liver, spleen and tumors. Macrodistributions of boron in various tissues were similar in mice whether injected with ZnTCPH or CuTCPH. CFM of unfixed liver sections showed cytoplasmic fluorescence from Kupffer cells in a periportal lobular distribution evenly throughout the liver. In the tumors studied, such fluorescence was also cytoplasmic but unlike liver fluorescence, was macroscopically heterogeneous.
Conclusion : ZnTCPH serves as a useful fluorescent experimental surrogate for CuTCPH to delineate its macroscopic and microscopic distributions in organs and tumors.
C1 [Smilowitz, Henry M.] Univ Connecticut, Ctr Hlth, Dept Cell Biol, Farmington, CT 06030 USA.
[Slatkin, Daniel N.; Micca, Peggy L.; Miura, Michiko] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA.
RP Smilowitz, HM (reprint author), Univ Connecticut, Ctr Hlth, Dept Cell Biol, 263 Farmington Ave, Farmington, CT 06030 USA.
EM Smilowitz@nso1.uchc.edu
FU Office of Biological and Environmental Research of the U.S. Department
of Energy [DE-AC02-98CH10986]
FX This work was supported by the Office of Biological and Environmental
Research of the U.S. Department of Energy under Contract
DE-AC02-98CH10986.
NR 35
TC 1
Z9 1
U1 2
U2 13
PU INFORMA HEALTHCARE
PI LONDON
PA TELEPHONE HOUSE, 69-77 PAUL STREET, LONDON EC2A 4LQ, ENGLAND
SN 0955-3002
J9 INT J RADIAT BIOL
JI Int. J. Radiat. Biol.
PD AUG
PY 2013
VL 89
IS 8
BP 611
EP 617
DI 10.3109/09553002.2013.782446
PG 7
WC Biology; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
SC Life Sciences & Biomedicine - Other Topics; Nuclear Science &
Technology; Radiology, Nuclear Medicine & Medical Imaging
GA 193VG
UT WOS:000322589000003
PM 23484623
ER
PT J
AU Cunningham, P
Linn, RR
Koo, E
Wilson, CJ
AF Cunningham, Philip
Linn, Rodman R.
Koo, Eunmo
Wilson, Cathy J.
TI Large-Eddy Simulations of Air Flow and Turbulence within and around
Low-Aspect-Ratio Cylindrical Open-Top Chambers
SO JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY
LA English
DT Article
DE Airflow; Mixing; Turbulence; Vegetation-atmosphere interactions; Large
eddy simulations; Biosphere-atmosphere interaction
ID OIL STORAGE TANKS; CIRCULAR-CYLINDER; INFRARED HEATER; WIND-TUNNEL;
FLAT-PLATE; FIELD; MODEL; RESPONSES; BEHAVIOR; SURFACE
AB The flow around cylindrical open-top chambers (OTCs) with aspect ratios (i.e., height-to-diameter ratios) much less than unity is investigated using a large-eddy simulation (LES) model. The solid structures are represented using the immersed boundary method, and the ambient flow in which the OTCs are embedded is representative of a turbulent atmospheric boundary layer. Results from the LES model show that the flow inside OTCs depends strongly on the height of the chamber wall. In particular, as chamber height increases the flow impinging on the upstream wall is deflected more in the vertical direction, a stronger recirculation flow develops inside the chamber, turbulence intensities are greater, and there is stronger vertical transport and mixing within the OTC, even at or near the ground. For low wall heights (i.e., very low aspect ratios), however, the flow impinging on the OTC is only diverted weakly in the vertical direction; aside from a small recirculation zone inside the OTC near the upstream wall and a small region near the downstream wall as the flow separates from the ground, there is minimal vertical mixing and the turbulence intensities are small. The results of these simulations, while general in nature, are particularly relevant to design considerations for manipulative field experiments in highly heterogeneous, low-stature ecosystems such as Arctic shrubs and grasses.
C1 [Cunningham, Philip; Linn, Rodman R.; Koo, Eunmo; Wilson, Cathy J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Cunningham, P (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, EES 16, Los Alamos, NM 87545 USA.
EM pcunning@lanl.gov
OI Koo, Eunmo/0000-0001-9943-9694
FU Regional Climate Impacts project; Next Generation Ecosystem Experiments
(NGEE Arctic) project; U.S. Department of Energy Office of Science,
Biological and Environmental Research Program
FX This research was supported by the Regional Climate Impacts and Next
Generation Ecosystem Experiments (NGEE Arctic) projects, both sponsored
by the U.S. Department of Energy Office of Science, Biological and
Environmental Research Program. Computational resources for the
numerical simulations were provided by Los Alamos National Laboratory
Institutional Computing. The authors thank Stan Wullschleger, Nathan
McDowell, and Jon Reisner for insightful comments and suggestions
throughout the course of this work.
NR 44
TC 1
Z9 1
U1 0
U2 13
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 1558-8424
J9 J APPL METEOROL CLIM
JI J. Appl. Meteorol. Climatol.
PD AUG
PY 2013
VL 52
IS 8
BP 1716
EP 1737
DI 10.1175/JAMC-D-12-041.1
PG 22
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 200BP
UT WOS:000323041800004
ER
PT J
AU Yang, Q
Berg, LK
Pekour, M
Fast, JD
Newsom, RK
Stoelinga, M
Finley, C
AF Yang, Qing
Berg, Larry K.
Pekour, Mikhail
Fast, Jerome D.
Newsom, Rob K.
Stoelinga, Mark
Finley, Catherine
TI Evaluation of WRF-Predicted Near-Hub-Height Winds and Ramp Events over a
Pacific Northwest Site with Complex Terrain
SO JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY
LA English
DT Article
DE Model evaluation; performance; Renewable energy
ID PART I; MODEL; IMPLEMENTATION; SENSITIVITY; CONVECTION
AB One challenge with wind-power forecasts is the accurate prediction of rapid changes in wind speed (ramps). To evaluate the Weather Research and Forecasting (WRF) model's ability to predict such events, model simulations, conducted over an area of complex terrain in May 2011, are used. The sensitivity of the model's performance to the choice among three planetary boundary layer (PBL) schemes [Mellor-Yamada-Janji (MYJ), University of Washington (UW), and Yonsei University (YSU)] is investigated. The simulated near-hub-height winds (62 m), vertical wind speed profiles, and ramps are evaluated against measurements obtained from tower-mounted anemometers, a Doppler sodar, and a radar wind profiler deployed during the Columbia Basin Wind Energy Study (CBWES). The predicted winds at near-hub height have nonnegligible biases in monthly mean under stable conditions. Under stable conditions, the simulation with the UW scheme better predicts upward ramps and the MYJ scheme is the most successful in simulating downward ramps. Under unstable conditions, simulations using the YSU and UW schemes show good performance in predicting upward ramps and downward ramps, with the YSU scheme being slightly better at predicting ramps with durations longer than 1 h. The largest differences in mean wind speed profiles among simulations using the three PBL schemes occur during upward ramps under stable conditions, which were frequently associated with low-level jets. The UW scheme has the best overall performance in ramp prediction over the CBWES site when evaluated using prediction accuracy and capture-rate statistics, but no single PBL parameterization is clearly superior to the others when all atmospheric conditions are considered.
C1 [Yang, Qing; Berg, Larry K.; Pekour, Mikhail; Fast, Jerome D.; Newsom, Rob K.] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Stoelinga, Mark] 3TIER Inc, Seattle, WA USA.
[Finley, Catherine] WindLogics Inc, Grand Rapids, MI USA.
RP Yang, Q (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA.
EM qing.yang@pnnl.gov
RI Yang, Qing/H-3275-2011; Berg, Larry/A-7468-2016
OI Yang, Qing/0000-0003-2067-5999; Berg, Larry/0000-0002-3362-9492
FU U.S. Department of Energy (DOE), Office of Energy Efficiency and
Renewable Energy; DOE [DE-AC06-76RL01830]
FX We thank Julia Flaherty of Pacific Northwest National Laboratory (PNNL)
for providing Fig. 1. We also thank Prof. Songyou Hong for the helpful
discussion and two anonymous reviewers for their helpful comments and
suggestions. This work was supported by the U.S. Department of Energy
(DOE), Office of Energy Efficiency and Renewable Energy. The RWP was
provided by the DOE's Atmospheric Radiation Measurement Program Climate
Research Facility, and the tower anemometer data were provided by the
Bonneville Power Administration. A portion of the research was performed
using PNNL Institutional Computing. PNNL is operated by Battelle for the
DOE under Contract DE-AC06-76RL01830.
NR 25
TC 13
Z9 14
U1 1
U2 27
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 1558-8424
J9 J APPL METEOROL CLIM
JI J. Appl. Meteorol. Climatol.
PD AUG
PY 2013
VL 52
IS 8
BP 1753
EP 1763
DI 10.1175/JAMC-D-12-0267.1
PG 11
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 200BP
UT WOS:000323041800006
ER
PT J
AU Collis, S
Protat, A
May, PT
Williams, C
AF Collis, Scott
Protat, Alain
May, Peter T.
Williams, Christopher
TI Statistics of Storm Updraft Velocities from TWP-ICE Including
Verification with Profiling Measurements
SO JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY
LA English
DT Article
DE Tropics; Dynamics; Vertical motion; Monsoons; Profilers; atmospheric;
Radars; Radar observations
ID VERTICAL VELOCITY; MICROPHYSICAL EVOLUTION; FLORIDA CUMULONIMBUS; RADAR
NETWORK; WIND PROFILER; DOPPLER; MOTION; PRECIPITATION; BAND
AB Comparisons between direct measurements and modeled values of vertical air motions in precipitating systems are complicated by differences in temporal and spatial scales. On one hand, vertically profiling radars more directly measure the vertical air motion but do not adequately capture full storm dynamics. On the other hand, vertical air motions retrieved from two or more scanning Doppler radars capture the full storm dynamics but require model constraints that may not capture all updraft features because of inadequate sampling, resolution, numerical constraints, and the fact that the storm is evolving as it is scanned by the radars. To investigate the veracity of radar-based retrievals, which can be used to verify numerically modeled vertical air motions, this article presents several case studies from storm events around Darwin, Northern Territory, Australia, in which measurements from a dual-frequency radar profiler system and volumetric radar-based wind retrievals are compared. While a direct comparison was not possible because of instrumentation location, an indirect comparison shows promising results, with volume retrievals comparing well to those obtained from the profiling system. This prompted a statistical analysis of an extended period of an active monsoon period during the Tropical Warm Pool International Cloud Experiment (TWP-ICE). Results show less vigorous deep convective cores with maximum updraft velocities occurring at lower heights than some cloud-resolving modeling studies suggest.
C1 [Collis, Scott] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA.
[Protat, Alain; May, Peter T.] Australian Bur Meteorol, Ctr Australian Weather & Climate Res, Melbourne, Vic, Australia.
[Williams, Christopher] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA.
[Williams, Christopher] NOAA, Earth Syst Res Lab, Boulder, CO USA.
RP Collis, S (reprint author), Argonne Natl Lab, Div Environm Sci, Bldg 240,9700 South Cass Ave, Argonne, IL 60439 USA.
EM scollis@anl.gov
RI Williams, Christopher/A-2723-2015
OI Williams, Christopher/0000-0001-9394-8850
FU U.S. Department of Energy, Office of Science, Office of Biological and
Environmental Research [DE-AC02-06CH11357]; Office of Biological and
Environmental Research (OBER) of the U.S. Department of Energy (DOE) as
part of the ARM Program; DOE Atmospheric Sciences Research (ASR) program
[DE-SC0007080]
FX Argonne National Laboratory's work was supported by the U.S. Department
of Energy, Office of Science, Office of Biological and Environmental
Research, under Contract DE-AC02-06CH11357. This work has been supported
by the Office of Biological and Environmental Research (OBER) of the
U.S. Department of Energy (DOE) as part of the ARM Program. Author CRW
was supported by DOE Atmospheric Sciences Research (ASR) program Grant
DE-SC0007080. We thank all involved in the TWP-ICE field program for
their work in collecting a world-class dataset. Special thanks are given
to Brad Atkinson and Dennis Klau for the continual upkeep of the CPOL
radar. Thanks are also given to Kao-Shen Chung and Isztar Zawadzki for
providing the original McGill multi-Doppler code. The bulk of the code
has been written using the open-source NumPy and SciPy projects, and the
authors are grateful to the authors of these projects. This manuscript
has benefited greatly from reviews from Susan Rennie and Edwin Campos
and the two anonymous reviewers.
NR 31
TC 22
Z9 22
U1 0
U2 17
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 1558-8424
J9 J APPL METEOROL CLIM
JI J. Appl. Meteorol. Climatol.
PD AUG
PY 2013
VL 52
IS 8
BP 1909
EP 1922
DI 10.1175/JAMC-D-12-0230.1
PG 14
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 200BP
UT WOS:000323041800016
ER
PT J
AU Lovejoy, KS
Davis, LE
McClellan, LM
Lillo, AM
Welsh, JD
Schmidt, EN
Sanders, CK
Lou, AJ
Fox, DT
Koppisch, AT
Del Sesto, RE
AF Lovejoy, Katherine S.
Davis, Lauren E.
McClellan, Lisa M.
Lillo, Antonietta M.
Welsh, John D.
Schmidt, Emily N.
Sanders, Claire K.
Lou, Alexander J.
Fox, David T.
Koppisch, Andrew T.
Del Sesto, Rico E.
TI Evaluation of ionic liquids on phototrophic microbes and their use in
biofuel extraction and isolation
SO JOURNAL OF APPLIED PHYCOLOGY
LA English
DT Article
DE Botryococcenes; Milking; Ionic liquids; Biofuels
ID MICROALGA BOTRYOCOCCUS-BRAUNII; WHOLE-CELL BIOCATALYSIS;
DUNALIELLA-SALINA; HYDROCARBONS; SOLVENTS; CAROTENOIDS; RECOVERY;
SYSTEMS; WATER; ACID
AB Multiple ionic liquids (ILs) were assessed for their ability to extract branched, unsaturated hydrocarbons from an aqueous medium. In addition, IL cytotoxicity studies were performed on two phototrophic microbes, Synechocystis sp. PCC6803 and Botryococcus braunii var Showa. The optimum IL for use in an isoprenoid hydrocarbon extraction may vary based on the biological source of the isoprenoids. Our results suggest that ionic liquids have the potential to serve as novel biocompatible milking agents for extracting high-value chemicals from the microbes, with toxicity to both species minimized by considerations of ionic liquid structure and hydrophobicity.
C1 [Lovejoy, Katherine S.; Davis, Lauren E.; Lou, Alexander J.; Del Sesto, Rico E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[McClellan, Lisa M.; Lillo, Antonietta M.; Welsh, John D.; Schmidt, Emily N.; Sanders, Claire K.; Fox, David T.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA.
[Koppisch, Andrew T.] No Arizona Univ, Dept Chem & Biochem, Flagstaff, AZ 86011 USA.
RP Del Sesto, RE (reprint author), Los Alamos Natl Lab, POB 1663,MS J514, Los Alamos, NM 87545 USA.
EM dfox@lanl.gov; andy.koppisch@nau.edu; ricod@lanl.gov
OI Lovejoy, Katherine/0000-0002-9606-9453
FU US Department of Energy LANL LDRD Program; National Alliance for
Advanced Biofuels and Bioproducts; Los Alamos National Flow Cytometry
Resource; National Center for Research Resources of NIH [P41-RR01315];
National Nuclear Security Administration of the US Department of Energy
[DE-AC52-06NA25396]
FX This work was supported by the US Department of Energy LANL LDRD
Program, National Alliance for Advanced Biofuels and Bioproducts, and
the Los Alamos National Flow Cytometry Resource funded by the National
Center for Research Resources of NIH (grant P41-RR01315). The authors
are grateful to Cytec Canada for supplying the [R3R'P]Cl
starting material and to Taylor Weiss and Dr. Tim Devarenne (Texas A&M
University) for supplying an authentic sample of isolated
botryococcenes. We also thank Dr. Taraka Dale (LANL) for the critical
analysis of the flow cytometry data. Los Alamos National Laboratory is
operated by Los Alamos National Security, LLC, for the National Nuclear
Security Administration of the US Department of Energy under contract
DE-AC52-06NA25396.
NR 37
TC 10
Z9 10
U1 2
U2 34
PU SPRINGER
PI DORDRECHT
PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS
SN 0921-8971
J9 J APPL PHYCOL
JI J. Appl. Phycol.
PD AUG
PY 2013
VL 25
IS 4
BP 973
EP 981
DI 10.1007/s10811-012-9907-0
PG 9
WC Biotechnology & Applied Microbiology; Marine & Freshwater Biology
SC Biotechnology & Applied Microbiology; Marine & Freshwater Biology
GA 180JA
UT WOS:000321588800006
ER
PT J
AU Knoshaug, EP
Shi, B
Shannon, TG
Mleziva, MM
Pienkos, PT
AF Knoshaug, Eric P.
Shi, Bo
Shannon, Tom G.
Mleziva, Mark M.
Pienkos, Philip T.
TI The potential of photosynthetic aquatic species as sources of useful
cellulose fibers-a review
SO JOURNAL OF APPLIED PHYCOLOGY
LA English
DT Review
DE Cellulose; Papermaking; Macroalgae; Microalgae; Aquatic plants
ID HYACINTH EICHHORNIA-CRASSIPES; WATER-HYACINTH; CELL-WALLS; RED ALGAE;
CLADOPHORA CELLULOSE; CHEMICAL-COMPOSITION; NATIVE CELLULOSE;
PAPER-PRODUCTION; CODIUM-FRAGILE; WASTE-WATER
AB Photosynthetic aquatic species, i.e., micro- and macroalgae and fresh or salt water plants, contain cellulose or other fibrous materials potentially suitable for paper making. Photosynthetic aquatic species having cellulosic or fibrous characteristics necessary for paper production were reviewed. These characteristics include overall fiber content, fiber size and morphology, and fiber composition. Several species of algae and aquatic plants are reported to possess cellulose in quantities greater than 10 % of total dry weight, and in general, the cellulose content in aquatic species is lower than that of most wood species. Commercial application of these aquatic algal or plant materials has been limited to simple milling, and no commercial applications utilizing processes to isolate the cellulosic fibers from these materials have yet been found.
C1 [Knoshaug, Eric P.; Pienkos, Philip T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA.
[Shi, Bo; Mleziva, Mark M.] Kimberly Clark Inc, Corp Res & Engn, Neenah, WI 54956 USA.
[Shannon, Tom G.] Kimberly Clark Inc, Family Care Res & Dev, North Atlantic Consumer Prod, Neenah, WI 54956 USA.
RP Knoshaug, EP (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA.
EM Eric.Knoshaug@nrel.gov
FU Kimberly-Clark Corporation, Neenah, WI
FX We would like to thank David Johnson and Ashutosh Mittal for technical
input. The funding for this project was provided by Kimberly-Clark
Corporation, Neenah, WI.
NR 80
TC 6
Z9 6
U1 2
U2 55
PU SPRINGER
PI DORDRECHT
PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS
SN 0921-8971
EI 1573-5176
J9 J APPL PHYCOL
JI J. Appl. Phycol.
PD AUG
PY 2013
VL 25
IS 4
BP 1123
EP 1134
DI 10.1007/s10811-012-9958-2
PG 12
WC Biotechnology & Applied Microbiology; Marine & Freshwater Biology
SC Biotechnology & Applied Microbiology; Marine & Freshwater Biology
GA 180JA
UT WOS:000321588800022
ER
PT J
AU Kim, HC
Fthenakis, V
AF Kim, Hyung Chul
Fthenakis, Vasilis
TI Life Cycle Energy and Climate Change Implications of Nanotechnologies A
Critical Review
SO JOURNAL OF INDUSTRIAL ECOLOGY
LA English
DT Article
DE climate change; energy consumption; industrial ecology; nanocoatings;
nanocomposites; nanomaterials
ID NANOPARTICLE PRODUCTION; ENVIRONMENTAL-IMPACT; CARBON; CONSUMPTION;
COMPOSITES; COST
AB The potential environmental and health impacts of nanotechnologies triggered a recent surge of life cycle assessment (LCA) studies on nanotechnologies. Focusing on the energy use and greenhouse gas emissions impacts, we reviewed 22 LCA-based studies on nanomaterials, coatings, photovoltaic devices, and fabrication technologies that were published until 2011. The reviewed LCA studies indicate that nanomaterials have higher cradle-to-gate energy demand per functional unit, and thus higher global warming impact, than their conventional counterparts. Depending on the synthesis method, carbon-based nanoparticles (i.e., carbon nanofibers, carbon nanotubes, and fullerenes) require 1 to 900 gigajoules per kilogram (GJ/kg) of primary energy to produce, compared with similar to 200 megajoules per kilogram (MJ/kg) for aluminum. This is mainly attributed to the fact that nanomaterials involve an energy-intensive synthesis process or an additional mechanical process to reduce particle size. Most reviewed studies ascertain, however, that the cradle-to-grave energy demand and global warming impact from nanotechnologies at a device level are lower than from conventional technologies because nanomaterials are typically used in a small amount to improve functionality and the upgraded functionality offers more energy-efficient operation of the device. Because of the immature status of most nanotechnologies, the studies reviewed here often rely on inventory data estimated from literature values and parametric analyses based on laboratory or prototype production, warranting future analyses to confirm the current findings.
C1 [Kim, Hyung Chul; Fthenakis, Vasilis] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Fthenakis, Vasilis] Columbia Univ, Earth & Environm Engn Dept, New York, NY USA.
RP Kim, HC (reprint author), Ford Res & Innovat Ctr, 2101 Village Rd, Dearborn, MI 48124 USA.
EM hkim41@ford.com
OI Kim, Hyung Chul/0000-0002-0992-4547
NR 28
TC 21
Z9 21
U1 6
U2 43
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1088-1980
J9 J IND ECOL
JI J. Ind. Ecol.
PD AUG
PY 2013
VL 17
IS 4
BP 528
EP 541
DI 10.1111/j.1530-9290.2012.00538.x
PG 14
WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Environmental;
Environmental Sciences
SC Science & Technology - Other Topics; Engineering; Environmental Sciences
& Ecology
GA 195QS
UT WOS:000322719300006
ER
PT J
AU Abraham, P
Adams, RM
Tuskan, GA
Hettich, RL
AF Abraham, Paul
Adams, Rachel M.
Tuskan, Gerald A.
Hettich, Robert L.
TI Moving Away from the Reference Genome: Evaluating a Peptide Sequencing
Tagging Approach for Single Amino Acid Polymorphism Identifications in
the Genus Populus
SO JOURNAL OF PROTEOME RESEARCH
LA English
DT Article
DE plant proteomics; Populus; single amino acid polymorphisms; mass
spectrometry; peptide sequence tagging; high energy collisional
dissociation
ID TANDEM MASS-SPECTRA; SITE LOCALIZATION; POSTTRANSLATIONAL MODIFICATIONS;
PROTEIN MODIFICATIONS; SHOTGUN PROTEOMICS; MS/MS; FRAGMENTATION;
TRICHOCARPA; ACCURATE; SEARCH
AB The genetic diversity across natural populations of the model organism, Populus, is extensive, containing a single nucleotide polymorphism roughly every 200 base pairs. When deviations from the reference genome occur in coding regions, they can impact protein sequences. Rather than relying on a static reference database to profile protein expression, we employed a peptide sequence tagging (PST) approach capable of decoding the plasticity of the Populus proteome. Using shotgun proteomics data from two genotypes of P. trichocarpa, a tag-based approach enabled the detection of 6653 unexpected sequence variants. Through manual validation, our study investigated how the most abundant chemical modification (methionine oxidation) could masquerade as a sequence variant (Ala-->Ser) when few site-determining ions existed. In fact, precise localization of an oxidation site for peptides with more than one potential placement was indeterminate for 70% of the MS/MS spectra. We demonstrate that additional fragment ions made available by high energy collisional dissociation enhances the robustness of the peptide sequence tagging approach (81% of oxidation events could be exclusively localized to a methionine). We are confident that augmenting fragmentation processes for a PST approach will further improve the identification of single amino acid polymorphism in Populus and potentially other species as well.
C1 [Abraham, Paul; Adams, Rachel M.] Univ Tennessee, Grad Sch Genome Sci & Technol, Knoxville, TN 37830 USA.
[Abraham, Paul; Adams, Rachel M.; Hettich, Robert L.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
[Tuskan, Gerald A.] Oak Ridge Natl Lab, Biol Sci Div, Oak Ridge, TN 37831 USA.
RP Hettich, RL (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
EM hettichrl@ornl.gov
RI Abraham, Paul/K-5599-2015; Hettich, Robert/N-1458-2016; Tuskan,
Gerald/A-6225-2011
OI Hettich, Robert/0000-0001-7708-786X; Tuskan, Gerald/0000-0003-0106-1289
FU U.S. Department of Energy, Office of Biological and Environmental
Research, Genome Sciences Program; Genome Science and Technology
Graduate Program at the University of Tennessee
FX This study was conducted as part of the BioEnergy Science Center through
funding from the U.S. Department of Energy, Office of Biological and
Environmental Research, Genome Sciences Program. P.A. and R.A. would
like to acknowledge financial support from the Genome Science and
Technology Graduate Program at the University of Tennessee. Oak Ridge
National Laboratory is managed for the U.S. Department of Energy by the
University of Tennessee - Battelle, L.L.C.
NR 35
TC 5
Z9 6
U1 0
U2 15
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1535-3893
J9 J PROTEOME RES
JI J. Proteome Res.
PD AUG
PY 2013
VL 12
IS 8
BP 3642
EP 3651
DI 10.1021/pr400192r
PG 10
WC Biochemical Research Methods
SC Biochemistry & Molecular Biology
GA 197LN
UT WOS:000322852800009
PM 23795892
ER
PT J
AU Saparov, B
Sefat, AS
AF Saparov, Bayrammurad
Sefat, Athena S.
TI Crystals, magnetic and electronic properties of a new ThCr2Si2-type
BaMn2Bi2 and K-doped compositions
SO JOURNAL OF SOLID STATE CHEMISTRY
LA English
DT Article
DE Superconductivity; ThCr2Si2 structure; Hole doping; Transition-metal
pnictide; BaMn2Bi2; Correlated electron materials
ID SINGLE-CRYSTALS; SUPERCONDUCTIVITY; BAMN2SB2; METAL; BREAKING; SYSTEM;
BA
AB This is a report on the new 122 ternary transition-metal pnictide of BaMn2Bi2, which is crystallized from bismuth flux. BaMn2Bi2 adopts ThCr2Si2-type structure (I4/mmm) with 0=4.4902(3) angstrom and c=14.687(1) angstrom; it is antiferromagnetic with anisotropic magnetic susceptibility and semiconducting with a band gap of E-g=6 meV. Heat capacity result confirms the insulating ground state in BaMn2Bi2 with the electronic residual Sommerfeld coefficient of gamma=0. The high temperature magnetization results show that magnetic ordering temperature is T-N similar to 400 K. Hole-doping in BaMn2Bi2 via potassium in Ba1-xKxMn2Bi2 results in metallic behavior for x=0.10(1), 032(1) and 036(1). With K-doping, more magnetically anisotropic behavior is observed. Although there is a downturn in electrical resistivity and low-field magnetization data below 4 K in > 30%-doped crystals, there is no sign of zero resistance or diamagnetism. Published by Elsevier Inc.
C1 [Saparov, Bayrammurad; Sefat, Athena S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
RP Saparov, B (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, POB 2008,Bldg 4100,1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.
EM saparovbi@ornl.gov
RI Sefat, Athena/R-5457-2016
OI Sefat, Athena/0000-0002-5596-3504
FU Department of Energy, Basic Energy Sciences, Materials Sciences and
Engineering Division
FX This work was supported by the Department of Energy, Basic Energy
Sciences, Materials Sciences and Engineering Division. We thank R.
Custelcean for his assistance with the single crystal X-ray diffraction
experiments.
NR 42
TC 12
Z9 12
U1 2
U2 63
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0022-4596
EI 1095-726X
J9 J SOLID STATE CHEM
JI J. Solid State Chem.
PD AUG
PY 2013
VL 204
BP 32
EP 39
DI 10.1016/j.jssc.2013.05.010
PG 8
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical
SC Chemistry
GA 198OQ
UT WOS:000322932600006
ER
PT J
AU Silverstein, HJ
Sharma, AZ
Cruz-Kan, K
Zhou, HD
Huq, A
Flacau, R
Wiebe, CR
AF Silverstein, H. J.
Sharma, A. Z.
Cruz-Kan, K.
Zhou, H. D.
Huq, A.
Flacau, R.
Wiebe, C. R.
TI Complex long-range magnetic ordering in the Mn-bearing dugganite
Pb3TeMn3P2O14
SO JOURNAL OF SOLID STATE CHEMISTRY
LA English
DT Article
DE Langasite; Dugganite; Neutron scattering; Antiferromagnetic;
Ba3NbFe3S12O14; Pb3TeMn3P2O14
ID CA3GA2GE4O14 STRUCTURE; POWDER DIFFRACTION; LANGASITE FAMILY; CRYSTALS;
DISTORTIONS; GROWTH; STATE
AB Spin liquids, multiferroics, and doubly-chiral helical structures are just some of the exotic magnetic states found in the langasite compounds. A subclass of the langasite group, the Te6+-containing dugganites, has also shown exotic magnetism including magnetoelectric coupling, coexisting complex long-ranged ordered structures, and low-field induced magnetic transitions. Here, we present the first detailed structural study of Pb3TeMn3P2O14 as well as the first neutron scattering measurements. This material undergoes long-range magnetic ordering, similar to the multiferroic Ba3NbFe3Si2O14, at T-N=6.6 K, which is consistent with previous magnetization measurements. However unlike any other langasite or dugganite studied to date, we present evidence of a large, pseudohexagonal incommensurate supercell that alters the nuclear and magnetic structures away from the langasite ideal. (C) 2013 Elsevier Inc. All rights reserved.
C1 [Silverstein, H. J.; Wiebe, C. R.] Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada.
[Sharma, A. Z.; Cruz-Kan, K.; Wiebe, C. R.] Univ Winnipeg, Dept Chem, Winnipeg, MB R3B 2E9, Canada.
[Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
[Huq, A.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA.
[Flacau, R.] CNR, Chalk River Labs, Chalk River, ON K0J 1J0, Canada.
RP Silverstein, HJ (reprint author), Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada.
EM harlyn.silverstein@gmail.com
RI Huq, Ashfia/J-8772-2013; Zhou, Haidong/O-4373-2016;
OI Huq, Ashfia/0000-0002-8445-9649; Silverstein, Harlyn/0000-0002-7743-9842
FU NSERC; CFI; ACS Petroleum Fund; Vanier CGS; MGS; University of Manitoba;
NSERC USRA Program; Canada Research Chair Program (Tier II); Scientific
User Facilities Division, Office of Basic Energy Sciences, US Department
of Energy (APS) [DE-AC02-06CH11357]
FX The authors would like to thank NSERC, CFI and the ACS Petroleum Fund
for funding. HJS gratefully acknowledges funding from the Vanier CGS,
MGS, and University of Manitoba. KC-K would like to thank the NSERC USRA
Program for funding. CRW would like to thank the Canada Research Chair
Program (Tier II) for funding. Portions of this research at the Oak
Ridge National Laboratory's SNS and Argonne National Laboratory's APS
were sponsored by the Scientific User Facilities Division, Office of
Basic Energy Sciences, US Department of Energy (APS under Contract no.
DE-AC02-06CH11357). Additionally, we would like to thank the amazing
support staff at the CNBC, the SNS, and the APS, and useful discussions
with P. Whitfield and M. Bieringer.
NR 38
TC 3
Z9 3
U1 0
U2 30
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0022-4596
J9 J SOLID STATE CHEM
JI J. Solid State Chem.
PD AUG
PY 2013
VL 204
BP 102
EP 107
DI 10.1016/j.jssc.2013.05.019
PG 6
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical
SC Chemistry
GA 198OQ
UT WOS:000322932600017
ER
PT J
AU Xiong, YX
AF Xiong, Yongliang
TI An Aqueous Thermodynamic Model for the Solubility of Potassium Ferrate
in Alkaline Solutions to High Ionic Strengths from 283.15 to 333.15 K
SO JOURNAL OF SOLUTION CHEMISTRY
LA English
DT Article
DE K2FeO4(cr); Solubility product; Aqueous solubility; Standard
thermodynamic properties
ID SUPER-IRON BATTERY; RESEARCH PROGRESS; REMEDIATION; OXIDATION;
CHEMISTRY; OXIDANT
AB Potassium ferrate, K2FeO4(cr), has numerous promising environmental applications. An aqueous thermodynamic model applicable to high ionic strengths is essential for guiding its applications. In this study, a thermodynamic model is developed for the solubility of K2FeO4(cr) in aqueous alkali metal hydroxide solutions, from 283.15 to 333.15 K to high ionic strengths, up to saturation of KOH and NaOH, based on the Pitzer activity coefficient model for aqueous species. The solubility products for K2FeO4(cr) at infinite dilution in the temperature range from 283.15 to 333.15 K were obtained. Based on the thermodynamic solubility product of K2FeO4(cr) at 298.15 and its temperature dependence, in combination with thermodynamic properties for and K+ from the literature, standard thermodynamic properties of K2FeO4(cr) at 298.15 K and 0.1 MPa (1 bar) are derived for the first time as follows: Delta(f) G (0) = -(896 +/- A 8) kJ center dot mol(-1), Delta(f) H (0) = -(1026 +/- A 4) kJ center dot mol(-1), and S (0) = (130 +/- A 17) J center dot mol(-1)center dot K-1. Using the above thermodynamic properties for K2FeO4(cr), the potential presence or preservation of K2FeO4(cr) in the Martian soils under the conditions relevant to Mars were quantitatively evaluated. Thermodynamic calculations pertaining to the Martian conditions indicate that the presence or preservation of K2FeO4(cr) as a strong oxidant in the Martian soils can be supported.
C1 [Xiong, Yongliang] Univ Idaho, Dept Geol Sci, Moscow, ID 83844 USA.
RP Xiong, YX (reprint author), Sandia Natl Labs, Carlsbad Programs Grp, 4100 Natl Pk Highway, Carlsbad, NM 88220 USA.
EM yxiong@sandia.gov
NR 29
TC 0
Z9 0
U1 1
U2 23
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 0095-9782
J9 J SOLUTION CHEM
JI J. Solut. Chem.
PD AUG
PY 2013
VL 42
IS 7
BP 1393
EP 1403
DI 10.1007/s10953-013-0038-2
PG 11
WC Chemistry, Physical
SC Chemistry
GA 202WC
UT WOS:000323250200003
ER
PT J
AU Rai, D
Yui, M
Kitamura, A
Yoshikawa, H
Felmy, AR
AF Rai, Dhanpat
Yui, Mikazu
Kitamura, Akira
Yoshikawa, Hideki
Felmy, A. R.
TI Thermodynamic Model for the Solubility of NdF3(cr) in the Na+-NH
(+)(4)-Nd3+-F--H2O System at 25 degrees C
SO JOURNAL OF SOLUTION CHEMISTRY
LA English
DT Article
DE Solubility; Neodymium; Fluoride complexes of Nd; Solubility product;
Thermodynamic data; NdF2+; NdF2+; NdF3(cr); Nd(OH)(3)(aq)
ID RARE-EARTH-ELEMENTS; FLUORO COMPLEXES; AQUEOUS-SOLUTION;
EQUILIBRIUM-CONSTANTS; STABILITY-CONSTANTS; GEOCHEMICAL SYSTEMS; AM3+-F
INTERACTION; IONIC-STRENGTH; TRACE-ELEMENTS; MIXED SYSTEM
AB The major objective of this study, based on critical review and experimental studies, was to develop a reliable thermodynamic model for the Nd-F system at 25 A degrees C. The SIT model was used to convert concentration constants reported in the literature to constants at zero ionic strengths for cross comparison and selection of reliable values. The critically evaluated thermodynamic constants for the formation of NdF2+ and NdF (2) (+) were then used to interpret the extensive NdF3(cr) solubility data in NaF and NH4F solutions, ranging in concentrations from extremely low values to as high as 1.0 mol center dot kg(-1), equilibrated for different periods ranging up to as long as 72 days. These efforts have resulted in for the reaction [Nd3+ + nF(-) a double dagger OE NdF (n) (3-n) ] of (3.81 +/- A 0.10), (5.89 +/- A 0.77), and < 12.48 for n values of 1-3, respectively. The for the solubility of NdF3(cr) (NdF3(cr) a double dagger OE Nd3+ + 3F(-)) was determined to be (-20.49 +/- A 0.37). Because (1) Nd is an excellent analog for trivalent actinides-An(III) (i.e., Pu(III), Am(III), and Cm(III)), and (2) the available data for the An(III)-F system, especially the solubility products of AnF(3)(cr), are of extremely poor quality, the critical literature review in combination with the experimental Nd-F system data have been used to assign thermodynamic constants for the An(III)-F reactions until good quality specific data for them becomes available.
C1 [Rai, Dhanpat] Rai Enviro Chem LLC, Yachats, OR 97498 USA.
[Yui, Mikazu; Kitamura, Akira; Yoshikawa, Hideki] Japan Atom Energy Agcy, Tokai, Ibaraki, Japan.
[Felmy, A. R.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Rai, D (reprint author), Rai Enviro Chem LLC, 1000 Hanley Dr,POB 784, Yachats, OR 97498 USA.
EM dhan.rai@raienvirochem.com
FU Japan Atomic Energy Agency (JAEA) [PNC ZA0865 92-001]
FX This research was supported by Japan Atomic Energy Agency (JAEA) Tokai
Works, under a collaborative agreement between JAEA and Rai
Enviro-Chem., LLC. The experimental data were developed at Battelle
Northwest Division under funding from and reported in JAEA internal
report (PNC ZA0865 92-001). We thank Marv Mason and Bob Fulton for
technical support. The senior author gratefully acknowledges the
financial support for this research provided by JAEA.
NR 38
TC 3
Z9 3
U1 0
U2 8
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 0095-9782
J9 J SOLUTION CHEM
JI J. Solut. Chem.
PD AUG
PY 2013
VL 42
IS 7
BP 1500
EP 1517
DI 10.1007/s10953-013-0049-z
PG 18
WC Chemistry, Physical
SC Chemistry
GA 202WC
UT WOS:000323250200010
ER
PT J
AU Halvorsen, MB
Zeddies, DG
Chicoine, D
Popper, AN
AF Halvorsen, Michele B.
Zeddies, David G.
Chicoine, David
Popper, Arthur N.
TI Effects of low-frequency naval sonar exposure on three species of fish
SO JOURNAL OF THE ACOUSTICAL SOCIETY OF AMERICA
LA English
DT Article
ID HIGH-INTENSITY; RAINBOW-TROUT; ACTIVE SONAR; HEARING; NOISE
AB To address growing concern over the impact of anthropogenic sound on fishes, a series of experiments was conducted that exposed several fish species to high-intensity low-frequency naval sonar. This study extends auditory findings by adding largemouth bass, yellow perch, and channel catfish. No effects on hearing were found in largemouth bass and yellow perch and only small effects in channel catfish (a fish with morphological adaptations for enhanced pressure reception). Together with prior findings, these results suggest limited impact on hearing from high-intensity sonar. Susceptibility may be due to genetic stock, developmental conditions, seasonal variation, and/or buoyancy during exposure. (C) 2013 Acoustical Society of America
C1 [Halvorsen, Michele B.; Zeddies, David G.; Popper, Arthur N.] Univ Maryland, Dept Biol, College Pk, MD 20742 USA.
[Halvorsen, Michele B.; Zeddies, David G.; Popper, Arthur N.] Univ Maryland, Ctr Comparat & Evolutionary Biol Hearing, College Pk, MD 20742 USA.
[Chicoine, David] New York State Chiropract Coll, Seneca Falls, NY 13148 USA.
RP Halvorsen, MB (reprint author), Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA.
EM Mhalvy@gmail.com; david.zeddies@jasco.com; drchicoine@gmail.com;
apopper@umd.edu
NR 11
TC 5
Z9 5
U1 1
U2 31
PU ACOUSTICAL SOC AMER AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 0001-4966
J9 J ACOUST SOC AM
JI J. Acoust. Soc. Am.
PD AUG
PY 2013
VL 134
IS 2
BP EL205
EP EL210
DI 10.1121/1.4812818
PN 1
PG 6
WC Acoustics; Audiology & Speech-Language Pathology
SC Acoustics; Audiology & Speech-Language Pathology
GA 195YE
UT WOS:000322738900013
PM 23927226
ER
PT J
AU Rossol, MN
Shaw, JH
Bale, H
Ritchie, RO
Marshall, DB
Zok, FW
AF Rossol, Michael N.
Shaw, John H.
Bale, Hrishikesh
Ritchie, Robert O.
Marshall, David B.
Zok, Frank W.
TI Characterizing Weave Geometry in Textile Ceramic Composites Using
Digital Image Correlation
SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY
LA English
DT Article
ID MICRO-COMPUTED-TOMOGRAPHY
AB Techniques for characterizing tow architectures and defects in woven ceramic composites are required for generating high-fidelity geometric models and subsequently probing effects of defects on composite performance. Although X-ray computed tomography (CT) has been shown to provide the requisite information with potentially sub-m resolution, the technique is inherently limited to probing only small volumes: on the order of a few unit cells of typical weaves. Here, we present an assessment of the efficacy of a complementary 2D technique, based on surface topography mapping via 3-D (three-dimensional) digital image correlation (DIC), with potential for ascertaining long-range features in weaves and defects that cannot be gleaned from CT imaging alone. Upon comparing surfaces reconstructed from CT and DIC data, we find that DIC is capable of resolving surface heights with a root mean square(RMS) error of similar to 10m (about twice the CT voxel size, 4.4m) and a spatial resolution of similar to 20m over areas of several cm(2). Achieving this level of resolution requires use of sufficiently small speckles (similar to 50m) and small subset size (similar to 300m) relative to the characteristic tow dimensions (similar to 1mm). The error is somewhat higher (about 20m) in areas where surface discontinuities or rapid changes in topography exist (e.g., at tow boundaries).
C1 [Rossol, Michael N.; Shaw, John H.; Zok, Frank W.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA.
[Bale, Hrishikesh; Ritchie, Robert O.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Bale, Hrishikesh; Ritchie, Robert O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Marshall, David B.] Teledyne Sci Co, Thousand Oaks, CA 91360 USA.
RP Zok, FW (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA.
EM zok@engineering.ucsb.edu
RI Ritchie, Robert/A-8066-2008
OI Ritchie, Robert/0000-0002-0501-6998
FU US AFOSR [FA9550-09-1-0477, B9U538772]; NASA under the National
Hypersonics Science Center for Materials and Structures; Office of
Science of the U.S. Department of Energy [DE-AC02-05CH11231]
FX This work was supported by the US AFOSR (Ali Sayir) and NASA (Anthony
Calomino) under the National Hypersonics Science Center for Materials
and Structures (AFOSR Prime Contract No. FA9550-09-1-0477 to Teledyne
Scientific and Subcontract No. B9U538772 to UCSB and to UCB). The use of
the X-ray microtomography beam line (8.3.2) at the Advanced Light
Source.; (Lawrence Berkeley National Laboratory) was supported by the
Office of Science of the U.S. Department of Energy under contract no.
DE-AC02-05CH11231. The authors also gratefully acknowledge fruitful
discussions with Varun Rajan (UCSB).
NR 10
TC 8
Z9 9
U1 0
U2 31
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0002-7820
J9 J AM CERAM SOC
JI J. Am. Ceram. Soc.
PD AUG
PY 2013
VL 96
IS 8
BP 2362
EP 2365
DI 10.1111/jace.12468
PG 4
WC Materials Science, Ceramics
SC Materials Science
GA 199AE
UT WOS:000322965300003
ER
PT J
AU Dai, SX
AF Dai, Steve X.
TI Localized Temperature Stability in Low-Temperature Cofired Ceramics
SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY
LA English
DT Article
ID COEFFICIENT; RESONATORS; CRYSTALLIZATION; DENSIFICATION; FREQUENCY;
FILTERS
AB Low-temperature cofired ceramic (LTCC) is a multilayer 3D packaging, interconnection, and integration technology. For LTCC modules targeting radio and microwave frequency (RF and MW) applications, a low or near 0ppm/degrees C temperature coefficient of resonant frequency ((f)) ensures temperature stability of embedded resonator and filter functions. The base dielectrics of most commercial LTCC systems have a (f) in the range -50 to -80ppm/degrees C. This study explored a method to achieve a zero (f) on stripline (SL) resonators by locally cofiring, in a multilayer LTCC structure, compensating dielectrics (CD) with an opposite (f) to that of the host dielectric. The formulation, synthesis, dielectric properties, and microstructure of SrTiO3 (STO)-based low-fire (f) CD are presented. Chemical interactions and physical compatibility between the compensating and the host LTCC dielectrics are investigated for cofireability. The dependence of (f) compensation on the wt% of STO, the printed thickness, and the location of the CD in multilayer LTCC are discussed. The most effective (f) compensation is achieved by integrating CD next to the resonator lines, and can be explained by the concentration of electromagnetic energy via total internal reflection of electromagnetic waves inside the CD layer.
C1 Sandia Natl Labs, Mat Sci & Engn Ctr, Albuquerque, NM 87185 USA.
RP Dai, SX (reprint author), Sandia Natl Labs, Mat Sci & Engn Ctr, POB 5800, Albuquerque, NM 87185 USA.
EM sxdai@sandia.gov
FU Laboratory Directed Research and Development program at Sandia National
Laboratories; U.S. Department of Energy's National Nuclear Security
Administration [DE-AC04-94AL85000]
FX The author would like to thank Dr Lung-Hwa Hsieh for the design of SL
resonators, Dr Mark Rodriguez for XRD analysis, Bonnie Mckenzie for SEM
characterization, Tom Chavez for synthesis of STO-based compensating
dielectrics, and Shelley Williams for LTCC panel fabrication. The author
also thanks Dr Robert Grubbs for his critical review of the manuscript.
This work was supported by the Laboratory Directed Research and
Development program at Sandia National Laboratories, a multiprogram
laboratory managed and operated by Sandia Corporation, a wholly owned
subsidiary of Lockheed Martin Corporation, for the U.S. Department of
Energy's National Nuclear Security Administration under contract
DE-AC04-94AL85000.
NR 22
TC 1
Z9 1
U1 3
U2 28
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0002-7820
J9 J AM CERAM SOC
JI J. Am. Ceram. Soc.
PD AUG
PY 2013
VL 96
IS 8
BP 2499
EP 2505
DI 10.1111/jace.12347
PG 7
WC Materials Science, Ceramics
SC Materials Science
GA 199AE
UT WOS:000322965300024
ER
PT J
AU Jackson, MD
Moon, J
Gotti, E
Taylor, R
Chae, SR
Kunz, M
Emwas, AH
Meral, C
Guttmann, P
Levitz, P
Wenk, HR
Monteiro, PJM
AF Jackson, Marie D.
Moon, Juhyuk
Gotti, Emanuele
Taylor, Rae
Chae, Sejung R.
Kunz, Martin
Emwas, Abdul-Hamid
Meral, Cagla
Guttmann, Peter
Levitz, Pierre
Wenk, Hans-Rudolf
Monteiro, Paulo J. M.
TI Material and Elastic Properties of Al-Tobermorite in Ancient Roman
Seawater Concrete
SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY
LA English
DT Article
ID C-S-H; HYDROUS CALCIUM SILICATES; ADVANCED-LIGHT-SOURCE; SUBSTITUTED
TOBERMORITES; AUTOCLAVING PROCESS; CRYSTAL-CHEMISTRY; NMR-SPECTROSCOPY;
AERATED CONCRETE; CATION-EXCHANGE; MINERALS
AB The material characteristics and elastic properties of aluminum-substituted 11 angstrom tobermorite in the relict lime clasts of 2000-year-old Roman seawater harbor concrete are described with TG-DSC and Si-29 MAS NMR studies, along with nanoscale tomography, X-ray microdiffraction, and high-pressure X-ray diffraction synchrotron radiation applications. The crystals have aluminum substitution for silicon in tetrahedral bridging and branching sites and 11.49(3)angstrom interlayer (002) spacing. With prolonged heating to 350 degrees C, the crystals exhibit normal behavior. The experimentally measured isothermal bulk modulus at zero pressure, K-0, 55 +/- 5GPa, is less than ab initio and molecular dynamics models for ideal tobermorite with a double-silicate chain structure. Even so, K-0, is substantially higher than calcium-aluminum-silicate-hydrate binder (C-A-S-H) in slag concrete. Based on nanoscale tomographic study, the crystal clusters form a well connected solid, despite having about 52% porosity. In the pumiceous cementitious matrix, Al-tobermorite with 11.27 angstrom interlayer spacing is locally associated with phillipsite, similar to geologic occurrences in basaltic tephra. The ancient concretes provide a sustainable prototype for producing Al-tobermorite in high-performance concretes with natural volcanic pozzolans.
C1 [Jackson, Marie D.; Moon, Juhyuk; Taylor, Rae; Chae, Sejung R.; Meral, Cagla; Monteiro, Paulo J. M.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA.
[Moon, Juhyuk] SUNY Stony Brook, Dept Mech Engn, Civil Engn Program, Stony Brook, NY 11794 USA.
[Gotti, Emanuele] CTG Italcementi SpA, I-24126 Bergamo, Italy.
[Kunz, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Emwas, Abdul-Hamid] King Abdullah Univ Sci & Technol, Thuwal 239556900, Saudi Arabia.
[Meral, Cagla] Middle E Tech Univ, TR-06800 Ankara, Turkey.
[Guttmann, Peter] Helmholtz Zentrum Mat & Energie GmbH, Inst Soft Matter & Funct Mat, D-12489 Berlin, Germany.
[Levitz, Pierre] Univ Paris 06, CNRS, Lab PECSA, F-75005 Paris, France.
[Wenk, Hans-Rudolf] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.
RP Monteiro, PJM (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA.
EM monteiro@ce.berkeley.edu
RI Meral, Cagla/K-8590-2013; Guttmann, Peter/H-9869-2015;
OI Meral, Cagla/0000-0001-8720-1216; Guttmann, Peter/0000-0002-0534-238X;
Jackson, Marie D./0000-0002-5180-3060; Moon, Juhyuk/0000-0002-7049-892X
FU King Abdullah University of Science and Technology (KAUST)
[KUS-l1-004021]; Office of Science, Department of Energy
[DE-AC02-05CH11231]; Advanced Nanofabrication Imaging and
Characterization Laboratories at King Abdullah University of Science and
Technology; ROMACONS drilling program
FX This research was supported by Award No. KUS-l1-004021, from King
Abdullah University of Science and Technology (KAUST). Data were
acquired at beamlines 12.2.2 and 12.3.2 at the Advanced Light Source at
the Lawrence Berkeley Laboratories, supported by the Director of the
Office of Science, Department of Energy, under Contract No.
DE-AC02-05CH11231, and the Advanced Nanofabrication Imaging and
Characterization Laboratories at King Abdullah University of Science and
Technology. We thank CTG Italcementi researchers and staff, especially
B. Zanga, in Bergamo, Italy; G. Vola at Cimprogetti S.p.A., Dalmine,
Italy; S. Clark at the 12.2.2 beamline; and N. Tamura at the 12.3.2
beamline; and the ROMACONS drilling program: J. P. Oleson, C. Brandon,
R. Hohlfelder. T. Teague, D. Hernandez, C. Hargis, I. A. Delaney, and B.
Black provided research support. We thank J. G. Moore, M. Sintubin, G.
Sposito, P.-A. Itty, and J. Kirz for critical discussions, and three
anonymous reviewers whose comments improved the manuscript.
NR 72
TC 21
Z9 21
U1 4
U2 49
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0002-7820
J9 J AM CERAM SOC
JI J. Am. Ceram. Soc.
PD AUG
PY 2013
VL 96
IS 8
BP 2598
EP 2606
DI 10.1111/jace.12407
PG 9
WC Materials Science, Ceramics
SC Materials Science
GA 199AE
UT WOS:000322965300040
ER
PT J
AU Joshi, BN
Yoon, H
van Hest, MFAM
Yoon, SS
AF Joshi, Bhavana N.
Yoon, Hyun
van Hest, Maikel F. A. M.
Yoon, Sam S.
TI Niobium-Doped Titania Photocatalyst Film Prepared via a Nonaqueous
Sol-Gel Method
SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY
LA English
DT Article
ID TIO2 THIN-FILMS; POLYCRYSTALLINE FILMS; ANATASE TIO2; NANOPARTICLES;
DEPOSITION
AB Niobium-doped Titanium dioxide (Nb:TiO2) transparent films were successfully deposited on glass substrates using a non-aqueous sol-gel spin coating technique. The effect of Nb concentration on the structural and photocatalytic properties of Nb:TiO2 films was studied using X-ray diffraction (XRD), scanning electron microscopy (SEM), atomic force microscopy (AFM), and UV visible spectroscopy. The films with 12at.% (atomic percent) Nb doped TiO2 showed excellent photocatalytic activity through 97.3% degradation of methylene blue (MB) after 2h of UV irradiation.
C1 [Joshi, Bhavana N.; Yoon, Hyun; Yoon, Sam S.] Korea Univ Anamdong, Sch Mech Eng, Seoul 136713, South Korea.
[van Hest, Maikel F. A. M.] Natl Renewable Energy Lab, Golden, CO 80407 USA.
RP Yoon, SS (reprint author), Korea Univ Anamdong, Sch Mech Eng, Seoul 136713, South Korea.
EM skyoon@korea.ac.kr
FU cooperative RD Program [B551179-08-03-00]; Korea Research Council
Industrial Science and Technology, Republic of Korea; Converging
Research Center Program through the Ministry of Education, Science and
Technology [2010K000969]; [NRF-2012029433]; [NRF-2012-0001169];
[NRF-2012K1A3A1A09054910]
FX This study was supported by a grant from the cooperative R&D Program
(B551179-08-03-00) funded by Korea Research Council Industrial Science
and Technology, Republic of Korea. This research was also supported by
Converging Research Center Program through the Ministry of Education,
Science and Technology (2010K000969), and NRF-2012029433,
NRF-2012-0001169, and NRF-2012K1A3A1A09054910.
NR 18
TC 5
Z9 5
U1 5
U2 59
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0002-7820
J9 J AM CERAM SOC
JI J. Am. Ceram. Soc.
PD AUG
PY 2013
VL 96
IS 8
BP 2623
EP 2627
DI 10.1111/jace.12336
PG 5
WC Materials Science, Ceramics
SC Materials Science
GA 199AE
UT WOS:000322965300043
ER
PT J
AU Petrick, N
Sahiner, B
Armato, SG
Bert, A
Correale, L
Delsanto, S
Freedman, MT
Fryd, D
Gur, D
Hadjiiski, L
Huo, ZM
Jiang, YL
Morra, L
Paquerault, S
Raykar, V
Samuelson, F
Summers, RM
Tourassi, G
Yoshida, H
Zheng, B
Zhou, C
Chan, HP
AF Petrick, Nicholas
Sahiner, Berkman
Armato, Samuel G., III
Bert, Alberto
Correale, Loredana
Delsanto, Silvia
Freedman, Matthew T.
Fryd, David
Gur, David
Hadjiiski, Lubomir
Huo, Zhimin
Jiang, Yulei
Morra, Lia
Paquerault, Sophie
Raykar, Vikas
Samuelson, Frank
Summers, Ronald M.
Tourassi, Georgia
Yoshida, Hiroyuki
Zheng, Bin
Zhou, Chuan
Chan, Heang-Ping
TI Evaluation of computer-aided detection and diagnosis systems
SO MEDICAL PHYSICS
LA English
DT Article
DE computer-aided detection and diagnosis (CAD); computer-aided detection
(CADe); computer-aided diagnosis (CADx); performance assessment;
standalone performance; reader performance; clinical performance
ID OPERATING CHARACTERISTIC ANALYSIS; BREAST-CANCER DETECTION;
MAXIMUM-LIKELIHOOD-ESTIMATION; IMAGE DATABASE CONSORTIUM; SMALL
PULMONARY NODULES; MEMORIAL FUND LECTURE; CT COLONOGRAPHY; LUNG NODULES;
SCREENING MAMMOGRAPHY; OBSERVER-PERFORMANCE
AB Computer-aided detection and diagnosis (CAD) systems are increasingly being used as an aid by clinicians for detection and interpretation of diseases. Computer-aided detection systems mark regions of an image that may reveal specific abnormalities and are used to alert clinicians to these regions during image interpretation. Computer-aided diagnosis systems provide an assessment of a disease using image-based information alone or in combination with other relevant diagnostic data and are used by clinicians as a decision support in developing their diagnoses. While CAD systems are commercially available, standardized approaches for evaluating and reporting their performance have not yet been fully formalized in the literature or in a standardization effort. This deficiency has led to difficulty in the comparison of CAD devices and in understanding how the reported performance might translate into clinical practice. To address these important issues, the American Association of Physicists in Medicine (AAPM) formed the Computer Aided Detection in Diagnostic Imaging Subcommittee (CADSC), in part, to develop recommendations on approaches for assessing CAD system performance. The purpose of this paper is to convey the opinions of the AAPM CADSC members and to stimulate the development of consensus approaches and "best practices" for evaluating CAD systems. Both the assessment of a standalone CAD system and the evaluation of the impact of CAD on end-users are discussed. It is hoped that awareness of these important evaluation elements and the CADSC recommendations will lead to further development of structured guidelines for CAD performance assessment. Proper assessment of CAD system performance is expected to increase the understanding of a CAD system's effectiveness and limitations, which is expected to stimulate further research and development efforts on CAD technologies, reduce problems due to improper use, and eventually improve the utility and efficacy of CAD in clinical practice. (C) 2013 American Association of Physicists in Medicine.
C1 [Petrick, Nicholas; Sahiner, Berkman; Samuelson, Frank] US FDA, Ctr Devices & Radiol Hlth, Silver Spring, MD 20993 USA.
[Armato, Samuel G., III; Jiang, Yulei] Univ Chicago, Dept Radiol, Chicago, IL 60637 USA.
[Bert, Alberto; Correale, Loredana; Delsanto, Silvia; Morra, Lia] im3D SpA, I-10153 Turin, Italy.
[Freedman, Matthew T.] Georgetown Univ, Lombardi Comprehens Canc Ctr, Washington, DC 20057 USA.
[Fryd, David] Riverain Med, Miamisburg, OH 45342 USA.
[Gur, David] Univ Pittsburgh, Dept Radiol, Pittsburgh, PA 15213 USA.
[Hadjiiski, Lubomir; Zhou, Chuan; Chan, Heang-Ping] Univ Michigan, Dept Radiol, Ann Arbor, MI 48109 USA.
[Huo, Zhimin] Carestream Hlth Inc, Rochester, NY 14615 USA.
[Raykar, Vikas] IBM Res, Nagawara Bangalore 560045, India.
[Summers, Ronald M.] NIH, Ctr Clin, Bethesda, MD 20892 USA.
[Tourassi, Georgia] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA.
[Yoshida, Hiroyuki] Massachusetts Gen Hosp, Dept Radiol, Boston, MA 02114 USA.
[Yoshida, Hiroyuki] Harvard Univ, Sch Med, Boston, MA 02114 USA.
[Zheng, Bin] Univ Oklahoma, Sch Elect & Comp Engn, Norman, OK 73019 USA.
RP Chan, HP (reprint author), Univ Michigan, Dept Radiol, 1500 East Med Ctr Dr,MIB C479, Ann Arbor, MI 48109 USA.
EM chanhp@umich.edu
OI Bert, Alberto/0000-0001-8391-7508; Tourassi,
Georgia/0000-0002-9418-9638; Zheng, Bin/0000-0002-7682-6648
FU Intramural Research Program of the National Institutes of Health,
Clinical Center; University of Chicago; iCAD; Riverain Technologies
through Georgetown University Medical Center
FX The authors are grateful to the members and participants of the CADSC
who have contributed to the stimulating discussions during many meetings
and teleconferences. R. M. S. is supported in part by the Intramural
Research Program of the National Institutes of Health, Clinical Center;
the views expressed in this paper are the opinions of the authors and do
not necessarily represent the views of the National Institutes of Health
or the Department of Health and Human Services. S. G. A. and H.Y.
receive royalties and licensing fees through the University of Chicago
related to CAD. R. M. S. receives patent royalties and research support
related to CAD from iCAD. M. T. F. receives funding from Riverain
Technologies through Georgetown University Medical Center.
NR 139
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U1 4
U2 34
PU AMER ASSOC PHYSICISTS MEDICINE AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 0094-2405
J9 MED PHYS
JI Med. Phys.
PD AUG
PY 2013
VL 40
IS 8
AR 087001
DI 10.1118/1.4816310
PG 17
WC Radiology, Nuclear Medicine & Medical Imaging
SC Radiology, Nuclear Medicine & Medical Imaging
GA 195XC
UT WOS:000322735900073
PM 23927365
ER
PT J
AU Salmeron, M
AF Salmeron, Miquel
TI Physics and chemistry of material surfaces under ambient conditions of
gases and liquids: What's new?
SO MRS BULLETIN
LA English
DT Article
ID PHOTOELECTRON-SPECTROSCOPY; IN-SITU; CO; OXIDATION; ICE
AB The atoms at the surfaces of materials represent the frontier separating the bulk from the surrounding medium. Over the last decades, scientists have intensely studied the structure and properties of surfaces with the goal of understanding and improving the electronic and chemical properties of materials. The surface-medium interaction determines wetting, friction, chemical, biological, and electronic properties. The activity of catalysts, phenomena occurring in water droplets and particles in the atmosphere, and the electronic properties of semiconductor devices are direct consequences of surface-environment interactions. While the need to pursue studies in the normal environment that surrounds a material has always been recognized, the techniques used in the past have only partially fulfilled this need, as most of them work best under high vacuum conditions. My research over the last 10 years has focused on discovering the structure of a surface and its dynamics in real life-in everyday environments. This required the development of new techniques and methods. I present some of the new tools developed in my laboratory and new properties that were discovered by their application in the areas of environmental science, surface chemistry, and catalysis.
C1 Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA.
RP Salmeron, M (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA.
EM mbsalmeron@lbl.gov
FU Department of Energy, Office of Basic Energy Sciences, Division of
Materials Sciences and Engineering of the United States
[DE-AC02-05CH11231]
FX This is the work of a large number of students and postdoctoral
researchers in my group and of collaborations with many colleagues in
various fields, which would be long and difficult to mention here. Their
names appear in the many publications that have resulted from it and are
cited here. I am fortunate to have enjoyed the support of the Laboratory
Director and of the Advanced Light Source, the Berkeley Synchrotron,
during the development and commissioning stages of the APPES project. I
also want to thank the Department of Energy, Office of Basic Energy
Sciences, Division of Materials Sciences and Engineering of the United
States, currently under Contract No. DE-AC02-05CH11231, for its support
of my research for more than 30 years.
NR 19
TC 6
Z9 6
U1 2
U2 40
PU CAMBRIDGE UNIV PRESS
PI NEW YORK
PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA
SN 0883-7694
J9 MRS BULL
JI MRS Bull.
PD AUG
PY 2013
VL 38
IS 8
BP 650
EP 657
DI 10.1557/mrs.2013.162
PG 8
WC Materials Science, Multidisciplinary; Physics, Applied
SC Materials Science; Physics
GA 198JF
UT WOS:000322918100017
ER
PT J
AU Ruan, LJ
AF Ruan, Lijuan
CA STAR Collaboration
TI The di-lepton physics program at STAR
SO NUCLEAR PHYSICS A
LA English
DT Article
DE di-electron continuum; cocktail simulation; low-mass enhancement; QGP
thermal radiation; mu-e correlation
ID PARTICLE IDENTIFICATION; AU COLLISIONS; RESTORATION; TPC
AB The recent results on di-electron production in p + p and Au+Au collisions at root s(NN) = 200 GeV are presented. The cocktail simulations of di-electrons from light and heavy flavor hadron decays are reported and compared with data. The perspectives for di-lepton measurements in lower energy Au+Au collisions and with future detector upgrades are discussed.
C1 [Ruan, Lijuan; STAR Collaboration] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
RP Ruan, LJ (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
EM ruanlj@rcf.rhic.bnl.gov
NR 39
TC 0
Z9 0
U1 2
U2 8
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 171
EP 178
DI 10.1016/j.nuclphysa.2012.12.084
PG 8
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900023
ER
PT J
AU Vogt, R
Nelson, RE
Frawley, AD
AF Vogt, R.
Nelson, R. E.
Frawley, A. D.
TI Improving the J/psi Production Baseline at RHIC and the LHC
SO NUCLEAR PHYSICS A
LA English
DT Article
DE quarkonium; cold nuclear matter
ID COLLISIONS
AB We assess the theoretical uncertainties on the inclusive J/psi production cross section in the Color Evaporation Model (CEM) using values for the charm quark mass, renormalization and factorization scales obtained from a fit to the charm production data. We use our new results to provide improved baseline comparison calculations at RHIC and the LHC. We also study cold matter effects on J/psi production at leading relative to next-to-leading order in the CEM within this approach.
C1 [Vogt, R.; Nelson, R. E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Vogt, R.; Nelson, R. E.] Univ Calif Davis, Davis, CA 95616 USA.
[Frawley, A. D.] Florida State Univ, Tallahassee, FL 32301 USA.
RP Vogt, R (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
EM vogt2@11n1.gov
FU U.S. Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]; JET Collaboration; National Science Foundation
[PHY-07-54674]
FX We thank M. Cheng, L. Linden Levy, P. Petreczky, R. Soltz and P. Vranas
for discussions. The work of R. V. and R. E. N. was performed under the
auspices of the U.S. Department of Energy by Lawrence Livermore National
Laboratory under Contract DE-AC52-07NA27344 and was also supported in
part by the JET Collaboration. The work of A. D. F. was supported by the
National Science Foundation grant PHY-07-54674.
NR 14
TC 0
Z9 0
U1 3
U2 6
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 231
EP 234
DI 10.1016/j.nuclphysa.2012.12.106
PG 4
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900035
ER
PT J
AU Zhang, BW
He, YC
Neufeld, RB
Vitev, I
Wang, EK
AF Zhang, Ben-Wei
He, Yuncun
Neufeld, R. B.
Vitev, Ivan
Wang, Enke
TI Probing nuclear matter with jets
SO NUCLEAR PHYSICS A
LA English
DT Article
DE Quark-gluon plasma (QGP); jet production; parton energy loss;
perturbative QCD
ID HEAVY-ION REACTIONS; ORDER ALPHA-S(3); COLLISIONS; GLUONS
AB Jet physics in relativistic heavy ion collisions, which combines perturbative QCD jet production with quark and gluon energy loss and in-medium parton shower modification, has emerged as a powerful tool to probe the properties of strongly-interacting matter formed in high-energy nuclear reactions. We present selected results for the modification of jet cross sections and related observables in the ambiance of hot and/or dense nuclear medium. We focus on the inclusive jet spectrum and dijets [O(alpha(3)(s))], and Z(0)/y* tagged jets [O(G(F)alpha(2)(s))] in the framework of perturbative QCD.
C1 [Zhang, Ben-Wei; He, Yuncun; Wang, Enke] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China.
[Zhang, Ben-Wei; He, Yuncun; Wang, Enke] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.
[Neufeld, R. B.; Vitev, Ivan] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
RP Zhang, BW (reprint author), Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China.
EM bwzhang@iopp.ccnu.edu.cn
FU US Department of Energy, Office of Science; MOE of China [NCET-09-0411];
NSF of China [11075062, 11221504]; NSF of Hubei [2010CDA075]; CCNU
FX This research is supported by the US Department of Energy, Office of
Science, and by the MOE of China with the Program NCET-09-0411, by NSF
of China with Project Nos. 11075062 and 11221504, and NSF of Hubei with
Project No. 2010CDA075, and in party by CCNU self-determined fundings.
NR 18
TC 0
Z9 0
U1 0
U2 1
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 256
EP 259
DI 10.1016/j.nuclphysa.2012.12.113
PG 4
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900041
ER
PT J
AU Jia, JY
AF Jia, Jiangyong
CA ATLAS Collaboration
TI Measurement of Event Plane Correlations in Pb-Pb Collisions at root
s(NN)=2.76 TeV with the ATLAS Detector
SO NUCLEAR PHYSICS A
LA English
DT Article
AB A measurement of correlations between event-plane angles Phi(n) is presented as a function of centrality for Pb-Pb collisions at root s(NN) = 2.76 TeV. These correlations are estimated from observed event-plane angles Psi(n) obtained from charged particle or transverse energy flow measured over a large pseudorapidity range vertical bar eta vertical bar < 4.8, followed by a resolution correction that accounts for the dispersion of Psi(n) relative to Phi(n). Various correlators involving two or three event planes with acceptable resolution are measured. Significant positive correlations are observed for 4(Phi(2) - Phi(4)), 6(Phi(2) - Phi(6)), 6(Phi(3) - Phi(6)), 2 Phi(2) + 3 Phi(3) - 5 Phi(5), 2 Phi(2) + 4 Phi(4) - 6 Phi(6) and 10 Phi(2) + 4 Phi(4) + 6 Phi(6). However, the measured correlations for 2 Phi(2) - 6 Phi(3) + 4 Phi(4) are negative. These results may shed light on the patterns of the fluctuation of the created matter in the initial state as well as the subsequent hydrodynamic evolution.
C1 [Jia, Jiangyong] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
Brookhaven Natl Lab, Dept Phys, Brookhaven, NY 11796 USA.
RP Jia, JY (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
EM jjia@bnl.gov
RI Pacheco Pages, Andres/C-5353-2011
OI Pacheco Pages, Andres/0000-0001-8210-1734
FU NSF [PHY-1019387]
FX This work is in part supported by NSF under award number PHY-1019387.
NR 12
TC 19
Z9 19
U1 0
U2 2
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 276
EP 280
DI 10.1016/j.nuclphysa.2012.12.043
PG 5
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900046
ER
PT J
AU de Barros, GOV
Fenton-Olsen, B
Jacobs, P
Ploskon, M
AF de Barros, G. O. V.
Fenton-Olsen, Bo
Jacobs, Peter
Ploskon, Mateusz
TI Data-driven analysis methods for the measurement of reconstructed jets
in heavy ion collisions at RHIC and LHC
SO NUCLEAR PHYSICS A
LA English
DT Article
DE Jet Reconstruction; Heavy Ion Collisions; Iterative Bayesian Unfolding
AB We present data-driven methods for the full reconstruction of jets in heavy ion collisions, for inclusive and coincidence jet measurements at both RHIC and LHC. The complex structure of heavy ion events generates a large background of combinatorial jets, and smears the measured energy of the true hard jet signal. Techniques to correct for these background effects can induce biases in the reported jet distributions, which must be well controlled for accurate measurement of jet quenching. Using model studies, we evaluate the proposed methods for measuring jet distributions accurately while minimizing the fragmentation bias of the measured population.
C1 [de Barros, G. O. V.] Univ Sao Paulo, Inst Fis, BR-05508090 Sao Paulo, Brazil.
[Fenton-Olsen, Bo; Jacobs, Peter; Ploskon, Mateusz] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Jacobs, Peter] CERN, CH-1211 Geneva 23, Switzerland.
RP de Barros, GOV (reprint author), Univ Sao Paulo, Inst Fis, Rua Matao Travessa R 187, BR-05508090 Sao Paulo, Brazil.
EM gbarros@dfn.if.usp.br
NR 13
TC 3
Z9 3
U1 0
U2 4
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 314
EP 318
DI 10.1016/j.nuclphysa.2012.12.019
PG 5
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900055
ER
PT J
AU Read, KF
AF Read, K. F.
CA PHENIX Collaboration
TI Open Heavy Flavor Production at Forward Angles in PHENIX
SO NUCLEAR PHYSICS A
LA English
DT Article
DE PHENIX; heavy ions; heavy flavor
AB The measurement of the nuclear modification factor (R-AA) for heavy-flavor production in heavy-ion collisions tests predictions for cold- and hot-nuclear-matter effects. Heavy-flavor production in p+p collisions tests pQCD calculations and serves as a reference for understanding heavy-flavor production in heavy-ion collisions. Using the PHENIX muon-arm spectrometers, the transverse momentum spectra of inclusive muon candidates are measured for p+p and Cu + Cu collisions at root s(NN) = 200 GeV. After subtracting backgrounds, we obtain the measured invariant yields of negative muons from the decay of heavy flavor mesons. For p+p collisions, we measure the charm-production cross section integrated over p(T) and in the rapidity range 1.4 < y < 1.9 to be d sigma(cc)/dy = 0.139 +/- 0.029 (stat)(-0.058)(+0.051) (syst) mb. This result is compared to a recent FONLL calculation and to a PHENIX measurement at mid-rapidity. For Cu + Cu collisions, we measure the R-AA for heavy-flavor muons in three centrality bins for 1 < p(T) < 4 GeV/c, with suppression observed for central collisions. We compare our measurement for central collisions to a recent theoretical prediction.
C1 [Read, K. F.; PHENIX Collaboration] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Read, KF (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
EM readkf@ornl.gov
OI Read, Kenneth/0000-0002-3358-7667
FU Office of Nuclear Physics, U.S. Department of Energy
FX Research sponsored by the Office of Nuclear Physics, U.S. Department of
Energy
NR 8
TC 0
Z9 0
U1 0
U2 2
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 359
EP 362
DI 10.1016/j.nuclphysa.2012.12.080
PG 4
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900066
ER
PT J
AU Steinberg, P
AF Steinberg, Peter
TI Measurement of high p(T) isolated prompt photons in lead-lead collisions
at root s(NN)=2.76 TeV with the ATLAS detector at the LHC
SO NUCLEAR PHYSICS A
LA English
DT Article
DE Large Hadron Collider; ultrarelativistic heavy ion collisions; prompt
photons
ID PP
AB Prompt photons are a powerful tool to study heavy ion collisions. Their production rates provide access to the initial state parton distribution functions and also provide a means to calibrate the expected energy of the recoil jet. The ATLAS detector measures photons with its hermetic, longitudinally segmented calorimeter, which gives excellent spatial and energy resolutions, and detailed information about the shower shape of each measured photon. This provides significant rejection against the expected background from the decays of neutral pions in jets. Rejection against jet fragmentation products is further enhanced by requiring candidate photons to be isolated. First results on the spectra of isolated prompt photons from a dataset with an integrated luminosity of approximately 0.13 nb(-1) of lead-lead collisions at root s(NN) = 2.76 TeV are shown as a function of transverse momentum and centrality. The measured spectra are compared to expectations from perturbative QCD calculations.
C1 Brookhaven Natl Lab, Upton, NY 11973 USA.
RP Steinberg, P (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA.
EM peter.steinberg@bnl.gov
NR 16
TC 0
Z9 0
U1 0
U2 0
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
EI 1873-1554
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 371
EP 375
DI 10.1016/j.nuclphysa.2012.12.090
PG 5
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900069
ER
PT J
AU Zhao, J
AF Zhao, Jie
CA STAR Collaboration
TI Dielectron production from root sNN=200 GeV Au + Au collisions at STAR
SO NUCLEAR PHYSICS A
LA English
DT Article
DE Dielectron; Quark-Gluon Plasma
ID COLLISIONS; STAR
AB We present the first STAR dielectron measurement in 200 GeV Au + Au collisions. Results are compared to hadron decay cocktail to search for in-medium modification of vector mesons in low mass region and thermal radiation in the intermediate mass region. The transverse mass slope parameters in the intermediate mass region are also discussed.
C1 [Zhao, Jie] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
[Zhao, Jie; STAR Collaboration] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Zhao, J (reprint author), Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
EM zhaojie@sinap.ac.cn
FU National Natural Science Foundation of China [11035009, 10905085,
11275250]; Chinese Academy of Sciences [KJCX2-EW-N01]
FX This work was supported in part by the National Natural Science
Foundation of China under contract No. 11035009, 10905085, 11275250 and
the Knowledge Innovation Project of the Chinese Academy of Sciences
under Grant No. KJCX2-EW-N01.
NR 13
TC 0
Z9 0
U1 0
U2 3
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 383
EP 386
DI 10.1016/j.nuclphysa.2012.12.114
PG 4
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900072
ER
PT J
AU Dusling, K
Epelbaum, T
Gelis, F
Venugopalan, R
AF Dusling, K.
Epelbaum, T.
Gelis, F.
Venugopalan, R.
TI Initial state and thermalization
SO NUCLEAR PHYSICS A
LA English
DT Article
DE Heavy ion collisions; Color Glass Condensate; Thermalization;
Bose-Einstein condensation
ID COLOR GLASS CONDENSATE; FLUCTUATIONS
AB We report recent results on the role of instabilities in the isotropization and thermalization of a longitudinally expanding system of quantum fields.
C1 [Dusling, K.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA.
[Epelbaum, T.; Gelis, F.] CEA, Inst Phys Theor, F-91191 Gif Sur Yvette, France.
[Venugopalan, R.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
RP Dusling, K (reprint author), N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA.
EM francois.gelis@cea.fr
OI Dusling, Kevin/0000-0001-9598-0416
FU Agence Nationale de la Recherche [11-BS04-015-01]; US Department of
Energy under DOE Contract [DE-AC02-98CH10886]; LORD grant from
Brookhaven Science Associates
FX F.G. and T.E. are supported by the Agence Nationale de la Recherche
project # 11-BS04-015-01. R.V.'s work is supported by the US Department
of Energy under DOE Contract No.DE-AC02-98CH10886 and by an LORD grant
from Brookhaven Science Associates.
NR 13
TC 1
Z9 1
U1 0
U2 3
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 437
EP 441
DI 10.1016/j.nuclphysa.2012.12.035
PG 5
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900085
ER
PT J
AU Xing, HX
Guo, Y
Wang, EK
Wang, XN
AF Xing, Hongxi
Guo, Yun
Wang, Enke
Wang, Xin-Nian
TI Parton energy loss in cold nuclei
SO NUCLEAR PHYSICS A
LA English
DT Article
DE Multiple scattering; high twist; perturbative QCD; parton energy loss
ID SCATTERING; COLLISIONS
AB Within the generalized high-twist factorization formalism, we express the contribution from multiple parton scattering and induced gluon radiation to the DY dilepton spectra in terms of nuclear modified effective beam quark distribution function. We show that beam quark energy loss is characterized by jet transport parameter (q) over cap, which is related to the local gluon density of the medium. Using the value of (q) over cap determined from the deeply inelastic scattering (DIS) data, we evaluate the nuclear modification factor in the Drell-Yan process in p+A collisions. Effects of parton energy loss in the DY spectra are found negligible in the Fermilab experimental data at E-lab = 800 GeV relative to parton shadowing while the predicted suppression of the DY spectra are significant at E-lab, = 120 GeV.
C1 [Xing, Hongxi; Wang, Enke; Wang, Xin-Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.
[Wang, Xin-Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA.
[Guo, Yun] Guangxi Normal Univ, Dept Phys, Guilin 541004, Peoples R China.
RP Xing, HX (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.
EM xnwang@lbl.gov
OI Wang, Xin-Nian/0000-0002-9734-9967
FU NSFC of China [10825523, 11205035]; Office of Energy Research, Office of
High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the
U.S. Department of Energy [DE-AC02-05CH11231]
FX This work is supported by the NSFC of China under Projects Nos.
10825523, 11205035 and by the Director, Office of Energy Research,
Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics,
of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231
and within the framework of the JET Collaboration.
NR 14
TC 2
Z9 2
U1 0
U2 2
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 442
EP 445
DI 10.1016/j.nuclphysa.2012.12.107
PG 4
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900086
ER
PT J
AU Young, C
Schenke, B
Icon, S
Gale, C
AF Young, Clint
Schenke, Bjoern
Icon, Sangyong
Gale, Charles
TI Realistic modelling of jets in heavy-ion collisions
SO NUCLEAR PHYSICS A
LA English
DT Article
AB The reconstruction of jets in heavy-ion collisions provides insight into the dynamics of hard partons in media. Unlike the spectrum of single hadrons, the spectrum of jets is highly sensitive to (q) over cap (perpendicular to), as well as being sensitive to partonic energy loss and radiative processes. We use MARTINI, an event generator, to study how finite-temperature processes at leading order affect dijets.
C1 [Young, Clint; Icon, Sangyong; Gale, Charles] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada.
[Schenke, Bjoern] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
RP Young, C (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada.
EM clinty@physics.mcgill.ca
NR 12
TC 1
Z9 1
U1 0
U2 0
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 494
EP 497
DI 10.1016/j.nuclphysa.2012.12.112
PG 4
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900099
ER
PT J
AU Xu, R
Deng, WT
Wang, XN
AF Xu, Rong
Deng, Wei-Tian
Wang, Xin-Nian
TI Suppression of high p(T) hadron spectra in p plus A collisions
SO NUCLEAR PHYSICS A
LA English
DT Article
DE Cronin effect; HIJING; valence quark number conservation
AB Multiple hard and semi-hard parton scatterings in high-energy p + A collisions involve multi-parton correlation inside the projectile in both momentum and flavor which will lead to modification of the final hadron spectra relative to that in p + p collisions. Such modification of the final hadron transverse momentum spectra in p + A collisions is studied within HIJING 2.1 Monte Carlo model which includes nuclear shadowing of the initial parton distributions and transverse momentum broadening. Multi-parton flavor and momentum correlation inside the projectile are incorporated through flavor and momentum conservation which are shown to modify the flavor content and momentum spectra of final partons and most importantly lead to suppression of large PT hadron spectra in p + A collisions at both RHIC and LHC energies.
C1 [Xu, Rong; Wang, Xin-Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.
[Deng, Wei-Tian] KEK, IPNS, Ctr Theory, Tsukuba, Ibaraki 3050801, Japan.
[Deng, Wei-Tian] FIAS, D-60438 Frankfurt, Germany.
[Wang, Xin-Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA.
RP Xu, R (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.
EM deng@post.kek.jp
FU NSFC [10825523]; CCNU from the colleges basic research and operation of
MOE; Helmholtz International Center for FAIR within the framework of the
LOEWE program; State of Hesse, US Depart of Energy [DE-AC02-05CH11231];
Ministry of Education, Culture, Sports, Science and Technology (MEXT) of
Japan [22340064]
FX This work was supported in part by the NSFC under the project No.
10825523, by self-determined research funds of CCNU from the colleges
basic research and operation of MOE, Helmholtz International Center for
FAIR within the framework of the LOEWE program launched by the State of
Hesse, US Depart of Energy under Contract No. DE-AC02-05CH11231 and
within the framework of the JET Collaboration, and Grant-in Aid for
Scientific Research (No. 22340064) from the Ministry of Education,
Culture, Sports, Science and Technology (MEXT) of Japan.
NR 12
TC 0
Z9 0
U1 0
U2 2
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0375-9474
J9 NUCL PHYS A
JI Nucl. Phys. A
PD AUG
PY 2013
VL 910
BP 514
EP 517
DI 10.1016/j.nuclphysa.2012.12.025
PG 4
WC Physics, Nuclear
SC Physics
GA 198NZ
UT WOS:000322930900104
ER
PT J
AU Aharmim, B
Ahmed, SN
Anthony, AE
Barros, N
Beier, EW
Bellerive, A
Beltran, B
Bergevin, M
Biller, SD
Boudjemline, K
Boulay, MG
Cai, B
Chan, YD
Chauhan, D
Chen, M
Cleveland, BT
Cox, GA
Dai, X
Deng, H
Detwiler, JA
DiMarco, M
Doe, PJ
Doucas, G
Drouin, PL
Duncan, FA
Dunford, M
Earle, ED
Elliott, SR
Evans, HC
Ewan, GT
Farine, J
Fergani, H
Fleurot, F
Ford, RJ
Formaggio, JA
Gagnon, N
Goon, JTM
Graham, K
Guillian, E
Habib, S
Hahn, RL
Hallin, AL
Hallman, ED
Harvey, PJ
Hazama, R
Heintzelman, WJ
Heise, J
Helmer, RL
Hime, A
Howard, C
Huang, M
Jagam, P
Jamieson, B
Jelley, NA
Jerkins, M
Keeter, KJ
Klein, JR
Kormos, LL
Kos, M
Kraus, C
Krauss, CB
Kruger, A
Kutter, T
Kyba, CCM
Lange, R
Law, J
Lawson, IT
Lesko, KT
Leslie, JR
Loach, JC
MacLellan, R
Majerus, S
Mak, HB
Maneira, J
Martin, R
McCauley, N
McDonald, AB
McGee, SR
Miller, ML
Monreal, B
Monroe, J
Nickel, BG
Noble, AJ
O'Keeffe, HM
Oblath, NS
Ollerhead, RW
Gann, GDO
Oser, SM
Ott, RA
Peeters, SJM
Poon, AWP
Prior, G
Reitzner, SD
Rielage, K
Robertson, BC
Robertson, RGH
Rosten, RC
Schwendener, MH
Secrest, JA
Seibert, SR
Simard, O
Simpson, JJ
Skensved, P
Sonley, TJ
Stonehill, LC
Tesic, G
Tolich, N
Tsui, T
Van Berg, R
VanDevender, BA
Virtue, CJ
Tseung, HWC
Wark, DL
Watson, PJS
Wendland, J
West, N
Wilkerson, JF
Wilson, JR
Wouters, JM
Wright, A
Yeh, M
Zhang, F
Zuber, K
AF Aharmim, B.
Ahmed, S. N.
Anthony, A. E.
Barros, N.
Beier, E. W.
Bellerive, A.
Beltran, B.
Bergevin, M.
Biller, S. D.
Boudjemline, K.
Boulay, M. G.
Cai, B.
Chan, Y. D.
Chauhan, D.
Chen, M.
Cleveland, B. T.
Cox, G. A.
Dai, X.
Deng, H.
Detwiler, J. A.
DiMarco, M.
Doe, P. J.
Doucas, G.
Drouin, P. -L.
Duncan, F. A.
Dunford, M.
Earle, E. D.
Elliott, S. R.
Evans, H. C.
Ewan, G. T.
Farine, J.
Fergani, H.
Fleurot, F.
Ford, R. J.
Formaggio, J. A.
Gagnon, N.
Goon, J. T. M.
Graham, K.
Guillian, E.
Habib, S.
Hahn, R. L.
Hallin, A. L.
Hallman, E. D.
Harvey, P. J.
Hazama, R.
Heintzelman, W. J.
Heise, J.
Helmer, R. L.
Hime, A.
Howard, C.
Huang, M.
Jagam, P.
Jamieson, B.
Jelley, N. A.
Jerkins, M.
Keeter, K. J.
Klein, J. R.
Kormos, L. L.
Kos, M.
Kraus, C.
Krauss, C. B.
Kruger, A.
Kutter, T.
Kyba, C. C. M.
Lange, R.
Law, J.
Lawson, I. T.
Lesko, K. T.
Leslie, J. R.
Loach, J. C.
MacLellan, R.
Majerus, S.
Mak, H. B.
Maneira, J.
Martin, R.
McCauley, N.
McDonald, A. B.
McGee, S. R.
Miller, M. L.
Monreal, B.
Monroe, J.
Nickel, B. G.
Noble, A. J.
O'Keeffe, H. M.
Oblath, N. S.
Ollerhead, R. W.
Gann, G. D. Orebi
Oser, S. M.
Ott, R. A.
Peeters, S. J. M.
Poon, A. W. P.
Prior, G.
Reitzner, S. D.
Rielage, K.
Robertson, B. C.
Robertson, R. G. H.
Rosten, R. C.
Schwendener, M. H.
Secrest, J. A.
Seibert, S. R.
Simard, O.
Simpson, J. J.
Skensved, P.
Sonley, T. J.
Stonehill, L. C.
Tesic, G.
Tolich, N.
Tsui, T.
Van Berg, R.
VanDevender, B. A.
Virtue, C. J.
Tseung, H. Wan Chan
Wark, D. L.
Watson, P. J. S.
Wendland, J.
West, N.
Wilkerson, J. F.
Wilson, J. R.
Wouters, J. M.
Wright, A.
Yeh, M.
Zhang, F.
Zuber, K.
CA SNO Collaboration
TI Combined analysis of all three phases of solar neutrino data from the
Sudbury Neutrino Observatory
SO PHYSICAL REVIEW C
LA English
DT Article
ID CALIBRATION SOURCE; OSCILLATIONS; MATTER; MODEL
AB We report results from a combined analysis of solar neutrino data from all phases of the Sudbury Neutrino Observatory (SNO). By exploiting particle identification information obtained from the proportional counters installed during the third phase, this analysis improved background rejection in that phase of the experiment. The combined analysis of the SNO data resulted in a total flux of active neutrino flavors from B-8 decays in the Sun of (5.25 +/- 0.16(stat.)(-0.13)(+0.11)(syst.)) x 10(6) cm(-2)s(-1), while a two-flavor neutrino oscillation analysis yielded Delta m(21)(2) = (5.6(-1.4)(+1.9)) x 10(-5) eV(2) and tan(2) theta(12) = 0.427(-0.029)(+0.033). A three-flavor neutrino oscillation analysis combining the SNO result with results of all other solar neutrino experiments and reactor neutrino experiments yielded Delta m(21)(2) = (7.46(-0.19)(+0.20)) x 10(-5) eV(2), tan(2) theta(12) = 0.443(-0.025)(+0.030), and sin(2) theta(13) = (2.49(-0.32)(+0.20)) x 10(-2).
C1 [Beltran, B.; Habib, S.; Hallin, A. L.; Howard, C.; Krauss, C. B.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2R3, Canada.
[Heise, J.; Jamieson, B.; Oser, S. M.; Tsui, T.; Wendland, J.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada.
[Hahn, R. L.; Lange, R.; Yeh, M.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Bellerive, A.; Boudjemline, K.; Dai, X.; Drouin, P. -L.; Farine, J.; Graham, K.; Noble, A. J.; Simard, O.; Tesic, G.; Watson, P. J. S.; Zhang, F.] Carleton Univ, Dept Phys, Ottawa Carleton Inst Phys, Ottawa, ON K1S 5B6, Canada.
[Bergevin, M.; Jagam, P.; Law, J.; Lawson, I. T.; Nickel, B. G.; Ollerhead, R. W.; Reitzner, S. D.; Simpson, J. J.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada.
[Aharmim, B.; Chauhan, D.; Farine, J.; Fleurot, F.; Hallman, E. D.; Huang, M.; Kraus, C.; Kruger, A.; Schwendener, M. H.; Virtue, C. J.] Laurentian Univ, Dept Phys & Astron, Sudbury, ON P3E 2C6, Canada.
[Bergevin, M.; Chan, Y. D.; Detwiler, J. A.; Gagnon, N.; Lesko, K. T.; Loach, J. C.; Martin, R.; Poon, A. W. P.; Prior, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Inst Nucl & Particle Astrophys, Berkeley, CA 94720 USA.
[Bergevin, M.; Chan, Y. D.; Detwiler, J. A.; Gagnon, N.; Lesko, K. T.; Loach, J. C.; Martin, R.; Poon, A. W. P.; Prior, G.] Univ Calif Berkeley, Div Nucl Sci, Berkeley, CA 94720 USA.
[Barros, N.; Maneira, J.] Lab Instrumentacao & Fis Expt Particulas, P-1000149 Lisbon, Portugal.
[Elliott, S. R.; Gagnon, N.; Heise, J.; Hime, A.; Rielage, K.; Seibert, S. R.; Stonehill, L. C.; Wouters, J. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Goon, J. T. M.; Kutter, T.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA.
[Formaggio, J. A.; Miller, M. L.; Monreal, B.; Monroe, J.; Oblath, N. S.; Ott, R. A.; Sonley, T. J.] MIT, Nucl Sci Lab, Cambridge, MA 02139 USA.
[Biller, S. D.; Cleveland, B. T.; Dai, X.; Doucas, G.; Fergani, H.; Gagnon, N.; Jelley, N. A.; Loach, J. C.; Majerus, S.; McCauley, N.; O'Keeffe, H. M.; Gann, G. D. Orebi; Peeters, S. J. M.; Tseung, H. Wan Chan; West, N.; Wilson, J. R.; Zuber, K.] Univ Oxford, Dept Phys, Oxford OX1 3RH, England.
[Beier, E. W.; Deng, H.; Dunford, M.; Heintzelman, W. J.; Klein, J. R.; Kyba, C. C. M.; McCauley, N.; Gann, G. D. Orebi; Secrest, J. A.; Seibert, S. R.; Van Berg, R.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA.
[Ahmed, S. N.; Boudjemline, K.; Boulay, M. G.; Cai, B.; Chen, M.; Dai, X.; DiMarco, M.; Duncan, F. A.; Earle, E. D.; Evans, H. C.; Ewan, G. T.; Ford, R. J.; Graham, K.; Guillian, E.; Harvey, P. J.; Heise, J.; Keeter, K. J.; Kormos, L. L.; Kos, M.; Kraus, C.; Leslie, J. R.; MacLellan, R.; Mak, H. B.; Martin, R.; McDonald, A. B.; Noble, A. J.; Robertson, B. C.; Skensved, P.; Wright, A.] Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada.
[Wark, D. L.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England.
[Duncan, F. A.; Ford, R. J.; Lawson, I. T.] SNOLAB, Sudbury, ON P3Y 1M3, Canada.
[Anthony, A. E.; Huang, M.; Jerkins, M.; Klein, J. R.; Seibert, S. R.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA.
[Helmer, R. L.] TRIUMF, Vancouver, BC V6T 2A3, Canada.
[Cox, G. A.; Doe, P. J.; Elliott, S. R.; Formaggio, J. A.; Gagnon, N.; Hazama, R.; McGee, S. R.; Oblath, N. S.; Rielage, K.; Robertson, R. G. H.; Rosten, R. C.; Stonehill, L. C.; Tolich, N.; VanDevender, B. A.; Tseung, H. Wan Chan; Wilkerson, J. F.] Univ Washington, Ctr Expt Nucl Phys & Astrophys, Seattle, WA 98195 USA.
[Cox, G. A.; Doe, P. J.; Elliott, S. R.; Formaggio, J. A.; Gagnon, N.; Hazama, R.; McGee, S. R.; Oblath, N. S.; Rielage, K.; Robertson, R. G. H.; Rosten, R. C.; Stonehill, L. C.; Tolich, N.; VanDevender, B. A.; Tseung, H. Wan Chan; Wilkerson, J. F.] Univ Washington, Dept Phys, Seattle, WA 98195 USA.
RP Aharmim, B (reprint author), Laurentian Univ, Dept Phys & Astron, Sudbury, ON P3E 2C6, Canada.
RI Prior, Gersende/I-8191-2013; Maneira, Jose/D-8486-2011; Barros,
Nuno/O-1921-2016;
OI Maneira, Jose/0000-0002-3222-2738; Barros, Nuno/0000-0002-1192-0705;
Prior, Gersende/0000-0002-6058-1420; Rielage, Keith/0000-0002-7392-7152
FU Natural Sciences and Engineering Research Council, Canada; Industry
Canada, Canada; National Research Council, Canada; Atomic Energy of
Canada, Ltd., Canada; Ontario Power Generation, Canada; High Performance
Computing Virtual Laboratory, Canada; Canada Foundation for Innovation,
Canada; Canada Research Chairs, Canada; Department of Energy, US;
National Energy Research Scientific Computing Center, US; Alfred P.
Sloan Foundation, US; Science and Technology Facilities Council, UK;
Fundacao para a Ciencia e a Tecnologia, Portugal; Northern Ontario
Heritage Fund, Canada
FX This research was supported by Canada: Natural Sciences and Engineering
Research Council, Industry Canada, National Research Council, Northern
Ontario Heritage Fund, Atomic Energy of Canada, Ltd., Ontario Power
Generation, High Performance Computing Virtual Laboratory, Canada
Foundation for Innovation, Canada Research Chairs; US: Department of
Energy, National Energy Research Scientific Computing Center, Alfred P.
Sloan Foundation; UK: Science and Technology Facilities Council;
Portugal: Fundacao para a Ciencia e a Tecnologia. We thank the SNO
technical staff for their strong contributions. We thank Vale (formerly
Inco, Ltd.) for hosting this project.
NR 55
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PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0556-2813
J9 PHYS REV C
JI Phys. Rev. C
PD AUG 1
PY 2013
VL 88
IS 2
AR 025501
DI 10.1103/PhysRevC.88.025501
PG 27
WC Physics, Nuclear
SC Physics
GA 195SM
UT WOS:000322723900002
ER
PT J
AU Soderstrom, PA
Lorusso, G
Watanabe, H
Nishimura, S
Doornenbal, P
Thiamova, G
Browne, F
Gey, G
Jung, HS
Sumikama, T
Taprogge, J
Vajta, Z
Wu, J
Xu, ZY
Baba, H
Benzoni, G
Chae, KY
Crespi, FCL
Fukuda, N
Gernhauser, R
Inabe, N
Isobe, T
Jungclaus, A
Kameda, D
Kim, GD
Kim, YK
Kojouharov, I
Kondev, FG
Kubo, T
Kurz, N
Kwon, YK
Lane, GJ
Li, Z
Montaner-Piza, A
Moschner, K
Naqvi, F
Niikura, M
Nishibata, H
Odahara, A
Orlandi, R
Patel, Z
Podolyak, Z
Sakurai, H
Schaffner, H
Simpson, GS
Steiger, K
Suzuki, H
Takeda, H
Wendt, A
Yagi, A
Yoshinaga, K
AF Soederstoerm, P. -A.
Lorusso, G.
Watanabe, H.
Nishimura, S.
Doornenbal, P.
Thiamova, G.
Browne, F.
Gey, G.
Jung, H. S.
Sumikama, T.
Taprogge, J.
Vajta, Zs.
Wu, J.
Xu, Z. Y.
Baba, H.
Benzoni, G.
Chae, K. Y.
Crespi, F. C. L.
Fukuda, N.
Gernhaeuser, R.
Inabe, N.
Isobe, T.
Jungclaus, A.
Kameda, D.
Kim, G. D.
Kim, Y. -K.
Kojouharov, I.
Kondev, F. G.
Kubo, T.
Kurz, N.
Kwon, Y. K.
Lane, G. J.
Li, Z.
Montaner-Piza, A.
Moschner, K.
Naqvi, F.
Niikura, M.
Nishibata, H.
Odahara, A.
Orlandi, R.
Patel, Z.
Podolyak, Zs.
Sakurai, H.
Schaffner, H.
Simpson, G. S.
Steiger, K.
Suzuki, H.
Takeda, H.
Wendt, A.
Yagi, A.
Yoshinaga, K.
TI Shape evolution in Ru-116,Ru-118: Triaxiality and transition between the
O(6) and U(5) dynamical symmetries
SO PHYSICAL REVIEW C
LA English
DT Article
ID INTERACTING BOSON MODEL; RU ISOTOPES; NEUTRON; FISSION; NUCLEI; PROTON;
STATES; ASYMMETRY; EUROBALL; DETECTOR
AB Ru-116 and Ru-118 have been studied via beta-delayed gamma-ray spectroscopy of nuclei produced in fragmentation reactions at the Radioactive Ion-Beam Factory (RIBF) facility. Level schemes with positive-parity states up to spin J = 6 have been constructed. The results have been discussed in terms of the interacting boson model, the algebraic collective model, and total Routhian surfaces. We conclude that the very neutron-rich nuclei still show many features associated with triaxial gamma-soft nuclei, represented by the O(6) symmetry, but are approaching a spherical structure, the U(5) symmetry, with increasing neutron number towards the N = 82 shell closure. In Ru-118, hints of a shape transition in the ground state have been observed.
C1 [Soederstoerm, P. -A.; Lorusso, G.; Watanabe, H.; Nishimura, S.; Doornenbal, P.; Browne, F.; Gey, G.; Taprogge, J.; Vajta, Zs.; Wu, J.; Baba, H.; Fukuda, N.; Inabe, N.; Isobe, T.; Kameda, D.; Kubo, T.; Sakurai, H.; Suzuki, H.; Takeda, H.] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan.
[Watanabe, H.] Beihang Univ, Dept Phys, Beijing 100191, Peoples R China.
[Thiamova, G.; Gey, G.; Simpson, G. S.] Univ Grenoble 1, Inst Natl Polytech Grenoble, CNRS, LPSC,IN2P3, F-38026 Grenoble, France.
[Browne, F.] Univ Brighton, Sch Comp Engn & Math, Brighton BN2 4JG, E Sussex, England.
[Jung, H. S.] Chung Ang Univ, Dept Phys, Seoul 156756, South Korea.
[Sumikama, T.] Tohoku Univ, Dept Phys, Aoba Ku, Sendai, Miyagi 9808578, Japan.
[Taprogge, J.] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain.
[Taprogge, J.; Jungclaus, A.] CSIC, Inst Estruct Mat, E-28006 Madrid, Spain.
[Vajta, Zs.] Hungarian Acad Sci, Inst Nucl Res, H-4001 Debrecen, Hungary.
[Wu, J.] Peking Univ, Dept Phys, Beijing 100871, Peoples R China.
[Xu, Z. Y.; Niikura, M.; Sakurai, H.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan.
[Benzoni, G.; Crespi, F. C. L.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy.
[Chae, K. Y.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea.
[Crespi, F. C. L.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy.
[Gernhaeuser, R.; Steiger, K.] Tech Univ Munich, Phys Dept E12, D-85748 Garching, Germany.
[Kim, G. D.; Kim, Y. -K.; Kwon, Y. K.] Inst for Basic Sci Korea, Rare Isotope Sci Project, Taejon 305811, South Korea.
[Kim, Y. -K.] Hanyang Univ, Dept Nucl Engn, Seoul 133791, South Korea.
[Kojouharov, I.; Kurz, N.; Schaffner, H.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany.
[Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA.
[Lane, G. J.] Australian Natl Univ, RSPE, Dept Nucl Phys, Canberra, ACT 0200, Australia.
[Li, Z.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China.
[Montaner-Piza, A.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46980 Paterna, Spain.
[Moschner, K.; Wendt, A.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany.
[Naqvi, F.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06520 USA.
[Nishibata, H.; Odahara, A.; Yagi, A.] Osaka Univ, Dept Phys, Toyonaka, Osaka 5600043, Japan.
[Orlandi, R.] Univ Louvain, KU Leuven, Inst Kern Stralingsfys, B-3001 Louvain, Belgium.
[Patel, Z.; Podolyak, Zs.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England.
[Yoshinaga, K.] Tokyo Univ Sci, Dept Phys, Noda, Chiba 2788510, Japan.
RP Soderstrom, PA (reprint author), RIKEN, Nishina Ctr, 2-1 Hirosawa, Wako, Saitama 3510198, Japan.
EM pasoder@ribf.riken.jp
RI Lane, Gregory/A-7570-2011; SAKURAI, HIROYOSHI/G-5085-2014;
OI Lane, Gregory/0000-0003-2244-182X; Soderstrom,
Par-Anders/0000-0002-9504-2814
FU Rare Isotope Science Project; Ministry of Science, ICT & Future Planning
(MSIP); National Research Foundation (NRF) of Korea; Japan Society for
the Promotion of Science (JSPS) Kakenhi [23.01752]; US Department of
Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; OTKA [K100835];
Spanish Ministerio de Ciencia e Innovacion [FPA2009-13377-C02,
FPA2011-29854-C04]; Priority Centers Research Program in Korea
[2009-0093817]; National Research Foundation of Korea
[NRF-2012R1A1A1041763]; U.S. DOE [DE-FG02-91ER-40609]
FX We would like to thank Dr. V. Werner for valuable discussions about the
IBM calculations. This work was carried out at the RIBF operated by the
RIKEN Nishina Center, RIKEN and CNS, University of Tokyo. We acknowledge
the EUROBALL Owners Committee for the loan of germanium detectors and
the PreSpec Collaboration for the readout electronics of the cluster
detectors. Part of the WAS3ABi was supported by the Rare Isotope Science
Project which is funded by the Ministry of Science, ICT & Future
Planning (MSIP) and the National Research Foundation (NRF) of Korea.
P.A.S. was financed by the Japan Society for the Promotion of Science
(JSPS) Kakenhi Grant No. 23.01752. F.G.K. was supported by the US
Department of Energy, Office of Nuclear Physics, under Contract No.
DE-AC02-06CH11357. Zs.V. was supported by OTKA Contract No. K100835. We
acknowledge financial support from the Spanish Ministerio de Ciencia e
Innovacion under Contracts No. FPA2009-13377-C02 and No.
FPA2011-29854-C04. H.S.J. was supported by the Priority Centers Research
Program in Korea (2009-0093817). K.Y.C. was supported by National
Research Foundation of Korea Grant No. NRF-2012R1A1A1041763. F.N. was
supported by U.S. DOE Grant No. DE-FG02-91ER-40609.
NR 44
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PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0556-2813
EI 1089-490X
J9 PHYS REV C
JI Phys. Rev. C
PD AUG 1
PY 2013
VL 88
IS 2
AR 024301
DI 10.1103/PhysRevC.88.024301
PG 10
WC Physics, Nuclear
SC Physics
GA 195SM
UT WOS:000322723900001
ER
PT J
AU Barnes, M
Parra, FI
Lee, JP
Belli, EA
Nave, MFF
White, AE
AF Barnes, M.
Parra, F. I.
Lee, J. P.
Belli, E. A.
Nave, M. F. F.
White, A. E.
TI Intrinsic Rotation Driven by Non-Maxwellian Equilibria in Tokamak
Plasmas
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID TOROIDAL ROTATION; TRANSPORT; TURBULENCE; MODE
AB The effect of small deviations from a Maxwellian equilibrium on turbulent momentum transport in tokamak plasmas is considered. These non-Maxwellian features, arising from diamagnetic effects, introduce a strong dependence of the radial flux of cocurrent toroidal angular momentum on collisionality: As the plasma goes from nearly collisionless to weakly collisional, the flux reverses direction from radially inward to outward. This indicates a collisionality-dependent transition from peaked to hollow rotation profiles, consistent with experimental observations of intrinsic rotation.
C1 [Barnes, M.; Parra, F. I.; Lee, J. P.; White, A. E.] MIT, Plasma Sci & Fusion Ctr, Cambridge, MA 02138 USA.
[Barnes, M.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA.
[Belli, E. A.] Gen Atom, San Diego, CA 92168 USA.
[Nave, M. F. F.] Inst Plasmas & Fusao Nucl, Assoc EURATOM IST, P-1049001 Lisbon, Portugal.
RP Barnes, M (reprint author), MIT, Plasma Sci & Fusion Ctr, Cambridge, MA 02138 USA.
EM mabarnes@mit.edu
RI Parra, Felix I./C-1442-2012; Nave, Maria/A-5581-2013
OI Parra, Felix I./0000-0001-9621-7404; Nave, Maria/0000-0003-2078-6584
FU U.S. DoE FES Postdoctoral Fellowship program; U.S. DoE [DE-SC008435];
Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]
FX We thank J. Candy and P. J. Catto for useful discussions. M. B. was
supported by a U.S. DoE FES Postdoctoral Fellowship program, F.I.P. was
supported by U.S. DoE Grant No. DE-SC008435, and computing time was
provided by the National Energy Scientific Computing Center, supported
by the Office of Science of the U.S. Department of Energy under Contract
No. DE-AC02-05CH11231.
NR 34
TC 27
Z9 27
U1 0
U2 16
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 1
PY 2013
VL 111
IS 5
AR 055005
DI 10.1103/PhysRevLett.111.055005
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196LQ
UT WOS:000322777400007
PM 23952414
ER
PT J
AU Qi, J
Durakiewicz, T
Trugman, SA
Zhu, JX
Riseborough, PS
Baumbach, R
Bauer, ED
Gofryk, K
Meng, JQ
Joyce, JJ
Taylor, AJ
Prasankumar, RP
AF Qi, J.
Durakiewicz, T.
Trugman, S. A.
Zhu, J. -X.
Riseborough, P. S.
Baumbach, R.
Bauer, E. D.
Gofryk, K.
Meng, J. -Q.
Joyce, J. J.
Taylor, A. J.
Prasankumar, R. P.
TI Measurement of Two Low-Temperature Energy Gaps in the Electronic
Structure of Antiferromagnetic USb2 Using Ultrafast Optical Spectroscopy
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID CYLINDRICAL FERMI SURFACES; COHERENT PHONONS; CRYSTAL-GROWTH;
THIN-FILMS; SUPERCONDUCTIVITY; YBA2CU3O7-DELTA; SCATTERING; DYNAMICS;
RELAXATION; SILICON
AB Ultrafast optical spectroscopy is used to study the antiferromagnetic f-electron system USb2. We observe the opening of two charge gaps at low temperatures (less than or similar to 45 K), arising from renormalization of the electronic structure. Analysis of our data indicates that one gap is due to hybridization between localized f-electron and conduction electron bands, while band renormalization involving magnons leads to the emergence of the second gap. These experiments thus enable us to shed light on the complex electronic structure emerging at the Fermi surface in f-electron systems.
C1 [Qi, J.; Durakiewicz, T.; Trugman, S. A.; Zhu, J. -X.; Baumbach, R.; Bauer, E. D.; Gofryk, K.; Meng, J. -Q.; Joyce, J. J.; Taylor, A. J.; Prasankumar, R. P.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Qi, J.] Peac Inst Multiscale Sci, Chengdu 610225, Sichuan, Peoples R China.
[Qi, J.] Sichuan Univ, Chengdu 610225, Sichuan, Peoples R China.
[Riseborough, P. S.] Temple Univ, Philadelphia, PA 19121 USA.
RP Prasankumar, RP (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM rpprasan@lanl.gov
RI Meng, Jianqiao/D-2667-2013; Riseborough, Peter/D-4689-2011; Gofryk,
Krzysztof/F-8755-2014;
OI Meng, Jianqiao/0000-0003-3168-9819; Gofryk,
Krzysztof/0000-0002-8681-6857; Trugman, Stuart/0000-0002-6688-7228;
Bauer, Eric/0000-0003-0017-1937; Zhu, Jianxin/0000-0001-7991-3918
FU Department of Energy, Office of Basic Energy Sciences, Division of
Material Sciences; National Nuclear Security administration of the U.S.
Department of Energy [DE-AC52-06NA25396]
FX This work was performed under the auspices of the Department of Energy,
Office of Basic Energy Sciences, Division of Material Sciences. Los
Alamos National Laboratory, is operated by Los Alamos National Security,
LLC, for the National Nuclear Security administration of the U.S.
Department of Energy under Contract No. DE-AC52-06NA25396.
NR 40
TC 13
Z9 13
U1 4
U2 45
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 1
PY 2013
VL 111
IS 5
AR 057402
DI 10.1103/PhysRevLett.111.057402
PG 5
WC Physics, Multidisciplinary
SC Physics
GA 196LQ
UT WOS:000322777400012
PM 23952443
ER
PT J
AU Saul, L
Wurz, P
Vorburger, A
Rodriguez, DF
Fuselier, SA
McComas, DJ
Mobius, E
Barabash, S
Funsten, H
Janzen, P
AF Saul, L.
Wurz, P.
Vorburger, A.
Rodriguez M, D. F.
Fuselier, S. A.
McComas, D. J.
Moebius, E.
Barabash, S.
Funsten, Herb
Janzen, Paul
TI Solar wind reflection from the lunar surface: The view from far and near
SO PLANETARY AND SPACE SCIENCE
LA English
DT Article
DE Moon; ENAs; IBEX
ID CHANDRAYAAN-1 MISSION; MOON; INSTRUMENT
AB The Moon appears bright in the sky as a source of energetic neutral atoms (ENAs). These ENAs have recently been imaged over a broad energy range both from near the lunar surface, by India's Chandrayaan-1 mission (CH-1), and from a much more distant Earth orbit by NASA's Interstellar Boundary Explorer (IBEX) satellite. Both sets of observations have indicated that a relatively large fraction of the solar wind is reflected from the Moon as energetic neutral hydrogen. CH-l's angular resolution over different viewing angles of the lunar surface has enabled measurement of the emission as a function of angle. IBEX in contrast views not just a swath but a whole quadrant of the Moon as effectively a single pixel, as it subtends even at the closest approach no more than a few degrees on the sky. Here we use the scattering function measured by CH-1 to model global lunar ENA emission and combine these with IBEX observations. The deduced global reflection is modestly larger (by a factor of 1.25) when the angular scattering function is included. This provides a slightly updated IBEX estimate of A(H) = 0.11 +/- 0.06 for the global neutralized albedo, which is similar to 25% larger than the previous values of 0.09 +/- 0.05, based on an assumed uniform scattering distribution. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Saul, L.; Wurz, P.; Vorburger, A.; Rodriguez M, D. F.] Univ Bern, Inst Phys, CH-3012 Bern, Switzerland.
[Fuselier, S. A.; McComas, D. J.] SW Res Inst, San Antonio, TX 78228 USA.
[Moebius, E.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA.
[Moebius, E.] Univ New Hampshire, Dept Phys, Durham, NH 03824 USA.
[Barabash, S.] Swedish Inst Space Phys, SE-98128 Kiruna, Sweden.
[Funsten, Herb] Los Alamos Natl Lab, Los Alamos, NM USA.
[Janzen, Paul] Univ Montana, Dept Phys & Astron, Missoula, MT 59812 USA.
[McComas, D. J.] Univ Texas San Antonio, San Antonio, TX 78249 USA.
RP Saul, L (reprint author), Univ Bern, Inst Phys, Sidlerstr 5, CH-3012 Bern, Switzerland.
EM saul@space.unibe.ch
RI Funsten, Herbert/A-5702-2015;
OI Funsten, Herbert/0000-0002-6817-1039; Vorburger,
Audrey/0000-0002-7400-9142; Moebius, Eberhard/0000-0002-2745-6978
NR 17
TC 3
Z9 3
U1 0
U2 10
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0032-0633
J9 PLANET SPACE SCI
JI Planet Space Sci.
PD AUG
PY 2013
VL 84
BP 1
EP 4
DI 10.1016/j.pss.2013.02.004
PG 4
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 196VI
UT WOS:000322805100001
ER
PT J
AU Kvasnytsya, V
Wirth, R
Dobrzhinetskaya, L
Matzel, J
Jacobsen, B
Hutcheon, I
Tappero, R
Kovalyukh, M
AF Kvasnytsya, Victor
Wirth, Richard
Dobrzhinetskaya, Larissa
Matzel, Jennifer
Jacobsen, Benjamin
Hutcheon, Ian
Tappero, Ryan
Kovalyukh, Mykola
TI New evidence of meteoritic origin of the Tunguska cosmic body
SO PLANETARY AND SPACE SCIENCE
LA English
DT Article
DE Diamond; Lonsdaleite; Graphite; Troilite; Taenite; gamma-iron;
Schreibersite; Intergrowths; Meteorite; Tunguska area
ID NOVO UREI METEORITES; ION-BEAM FIB; EXPLOSION SITE; CANYON DIABLO;
IRON-METEORITES; IMPACT CRATER; DIAMONDS; CARBON; PEAT; ANOMALIES
AB Diamond-lonsdaleite-graphite micro-samples collected from peat after the 1908 catastrophic blast in the Tunguska area were studied with scanning (SEM) and transmission electron (TEM) microscopy, NanoSecondary Ion Mass Spectrometry (NanoSIMS) and X-ray synchrotron technique. The high-pressure carbon allotropes in the Tunguska samples are being described for the first time and contain inclusions of FeS (troilite), Fe-Ni (taenite), gamma-Fe and (FeNi)(3)P (schreibersite). The samples are nodule-like in shape and consist of 99.5% carbon minerals, e.g. diamond > lonsdaleite > graphite. Micro- and nanoinclusions of troilite (up to 0.5 vol%), taenite, gamma-iron and schreibersite fill cracks, cleavages and pores in the carbon matrix. Carbon isotope studies from the two analyses of the Tunguska foil showed delta C-13=-16.0 +/- 1.9 parts per thousand and delta C-13=-15.2 +/- 2.1 parts per thousand, suggesting delta C-13=-15.6 +/- 2 parts per thousand as an average characteristic of the carbon reservoir. That value is close to delta C-13 of some extraterrestrial samples. A negligible concentration of Ir and Os in the carbonaceous matrix promotes some controversial interpretation of the origin of the studied materials. Attributing this fact to the primary inhomogeneity, and considering the micro-structural features such as cracks, deformation of the crystal lattices, etc. coupled with high-pressure carbon allotropes association with metals, sulfides and phosphides, and the high ratio of Fe:Ni=22:1 suggest that the studied samples are meteorite micro-remnants. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Kvasnytsya, Victor] Natl Acad Sci Ukraine, Inst Geochem Mineral & Ore Format, UA-03680 Kiev 142, Ukraine.
[Wirth, Richard] GFZ, German Res Ctr Geosci, Helmholtz Ctr Potsdam, D-14473 Potsdam, Germany.
[Dobrzhinetskaya, Larissa] Univ Calif Riverside, Dept Earth Sci, Riverside, CA 92521 USA.
[Matzel, Jennifer; Jacobsen, Benjamin; Hutcheon, Ian] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Tappero, Ryan] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Kovalyukh, Mykola] Natl Acad Sci Ukraine, Inst Environm Geochem, UA-03680 Kiev 142, Ukraine.
RP Kvasnytsya, V (reprint author), Natl Acad Sci Ukraine, Inst Geochem Mineral & Ore Format, Palladin Ave 34, UA-03680 Kiev 142, Ukraine.
EM vmkvas@hotmail.com
FU German Science Foundation (DFG), Bonn-Bad Godesberg; LAB-FEE Research
Grant; US Department of Energy-Geosciences [DE-FG02-92ER14244]; US
Department of Energy, Office of Science, Office of Basic Energy Sciences
[DE-AC02-98CH10886]
FX VK thanks the German Science Foundation (DFG), Bonn-Bad Godesberg for a
travel grant. Part of this research conducted in the Lawrence Livermore
National Laboratory was supported by LAB-FEE Research Grant
(LD-JM-BJ-IH). The work performed at Beamline X27A, National Synchrotron
Light Source (NSLS) of the Brookhaven National Laboratory. It was
supported in part by the US Department of Energy-Geosciences
(DE-FG02-92ER14244 to The University of Chicago-CARS). Use of the NSLS
was supported by the US Department of Energy, Office of Science, Office
of Basic Energy Sciences, under Contract no. DE-AC02-98CH10886. A.
Schreiber (GFZ Potsdam) is thanked for the TEM sample preparation with
FIB. Thanks to M. M. Taran for useful advices and discussion. We also
thank anonymous reviewers and Felix Kaminsky for helpful criticism that
significantly improved the manuscript.
NR 58
TC 7
Z9 7
U1 3
U2 41
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0032-0633
J9 PLANET SPACE SCI
JI Planet Space Sci.
PD AUG
PY 2013
VL 84
BP 131
EP 140
DI 10.1016/j.pss.2013.05.003
PG 10
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 196VI
UT WOS:000322805100013
ER
PT J
AU Chatterjee, S
Bryan, SA
Seliskar, CJ
Heineman, WR
AF Chatterjee, Sayandev
Bryan, Samuel A.
Seliskar, Carl J.
Heineman, William R.
TI Three-component spectroelectrochemical sensor module for the detection
of pertechnetate (TcO4-)
SO REVIEWS IN ANALYTICAL CHEMISTRY
LA English
DT Article
DE pertechnetate; technetium; three-component sensor
ID DMPE = 1,2-BIS(DIMETHYLPHOSPHINO)ETHANE; ELECTRON-TRANSFER REACTIONS;
OPTICALLY TRANSPARENT ELECTRODES; SINGLE DEVICE; RHENIUM COMPLEXES;
SELECTIVITY; TECHNETIUM; BEHAVIOR; SORPTION; FILMS
AB This rewview looks at the advancements in the development of a sensor for technetium (Tc) that is applicable to characterizing and monitoring the vadose zone and associated subsurface water. Subsurface contamination by Tc is of particular concern for two reasons: the long lifetime of its most common isotope Tc-99 (half-life = 2 x 10(5) years) and the fast migration in soils of pertechnetate (TcO4-), which is considered to be the dominant 99 Tc species in ground water. TcO4- does not have a characteristic spectral signature which prevents its rapid, sensitive, and economic in situ detection. To address this problem, a novel spectroelectrochemical sensor has been designed, that combines three modes of selectivity (electrochemistry, spectroscopy, and selective partitioning) into a single sensor to substantially improve specificity, which is critical in the specific detection of an analyte in the presence of potential interfering species. The sensor consists of a basic spectroelectrochemical configuration: a waveguide with an optically transparent electrode (OTE) that is coated with a thin chemically-selective film that preconcentrates the analyte. The key to adapting this generic sensor to detect TcO4- and Tc complexes lies in the development of chemically-selective films that preconcentrate the analyte and, when necessary, chemically convert it into a complex with electrochemical and spectroscopic properties appropriate for sensing. The chemically selective films can be combined with ligands which are capable of reacting with TcO4- to form coordination complexes, the spectral properties of which can be used to enhance the sensitivity of detection. The first half of this review describes the general concept of the sensor and the rationale for the selection of its specific components, and the development and characterization of the sensor for the different detection modules. The second half summarizes the synthesis and characterization of complexes relevant for the detection of technetium, and the progress in the utilization of the sensor module for the effective detection of these complexes.
C1 [Chatterjee, Sayandev; Bryan, Samuel A.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA.
[Seliskar, Carl J.; Heineman, William R.] Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA.
RP Chatterjee, S (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA.
EM sayandev.chatterjee@pnnl.gov; sam.bryan@pnnl.gov;
carl.j.seliskar@uc.edu; william.heineman@uc.edu
RI Bryan, Samuel/D-5457-2015;
OI Bryan, Samuel/0000-0001-5664-3249; Chatterjee,
Sayandev/0000-0003-2218-5635
NR 51
TC 2
Z9 2
U1 1
U2 13
PU WALTER DE GRUYTER GMBH
PI BERLIN
PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY
SN 0793-0135
EI 2191-0189
J9 REV ANAL CHEM
JI Rev. Anal. Chem.
PD AUG
PY 2013
VL 32
IS 3
BP 209
EP 224
DI 10.1515/revac-2013-0001
PG 16
WC Chemistry, Analytical
SC Chemistry
GA 200AV
UT WOS:000323039000004
ER
PT J
AU Zhu, GD
AF Zhu, Guangdong
TI Development of an analytical optical method for linear Fresnel
collectors
SO SOLAR ENERGY
LA English
DT Article
DE Concentrating solar power; Linear Fresnel collector; Solar thermal;
Non-imaging optics; Intercept factor; Incidence angle modifier
ID SOLAR CONCENTRATORS; GEOMETRIC ANALYSIS
AB An analytical optical approach-First-principle OPTical Intercept Calculation (FirstOPTIC)-is developed for the optical performance evaluation of linear Fresnel collectors. Instead of treating all optical error sources as probability distributions and convolving them with the sun shape into an overall beam spread function, FirstOPTIC treats mirror slope error, receiver position error, and collector tracking error as geometric modifications to the collector, as interpreted in laboratory measurements. Calculation of intercept factors is analytically derived through a rigorous mathematical model. It is shown through test cases that FirstOPTIC can provide accurate and fast calculation of collector intercept factors as a function of incidence angle. Finally, FirstOPTIC is used to conduct analysis on the incidence angle modifier (JAM) and indicates that the factorized IAM representation with respect to independent transversal and longitudinal components can be a good approximation but in general underestimates the optical performance of a linear Fresnel collector. (C) 2013 Elsevier Ltd. All rights reserved.
C1 Natl Renewable Energy Lab, Concentrating Solar Power Program, Golden, CO USA.
RP Zhu, GD (reprint author), Natl Renewable Energy Lab, Concentrating Solar Power Program, 15013 Denver West Pkwy, Golden, CO USA.
EM Guangdong.Zhu@nrel.gov
FU U.S. Department of Energy under National Renewable Energy Laboratory
(NREL) [DE-AC36-08GO28308]
FX This work was supported by the U.S. Department of Energy under Contract
No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory
(NREL).
NR 28
TC 15
Z9 15
U1 1
U2 17
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0038-092X
J9 SOL ENERGY
JI Sol. Energy
PD AUG
PY 2013
VL 94
BP 240
EP 252
DI 10.1016/j.solener.2013.05.003
PG 13
WC Energy & Fuels
SC Energy & Fuels
GA 198RX
UT WOS:000322941100021
ER
PT J
AU Idriss, H
Bagus, PS
Ilton, ES
AF Idriss, Hicham
Bagus, Paul S.
Ilton, Eugene S.
TI Progress in Electronic and Vibrational Spectroscopy of Catalytic
Materials and Catalytic Reactions: Theoretical and Experimental Studies
SO TOPICS IN CATALYSIS
LA English
DT Editorial Material
C1 [Idriss, Hicham] Univ Aberdeen, Dept Chem, Aberdeen, Scotland.
[Idriss, Hicham] SABIC T&I, Riyadh, Saudi Arabia.
[Idriss, Hicham] KAUST, CRI, Thuwal, Saudi Arabia.
[Bagus, Paul S.] Univ N Texas, Dept Chem, Denton, TX 76203 USA.
[Ilton, Eugene S.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Idriss, H (reprint author), SABIC T&I, Riyadh, Saudi Arabia.
EM h.idriss@abdn.ac.uk; bagus@unt.edu; Ilton@pnnl.gov
RI Bagus, Paul/M-1273-2015
NR 0
TC 0
Z9 0
U1 0
U2 10
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1022-5528
J9 TOP CATAL
JI Top. Catal.
PD AUG
PY 2013
VL 56
IS 12
BP 1047
EP 1048
DI 10.1007/s11244-013-0081-7
PG 2
WC Chemistry, Applied; Chemistry, Physical
SC Chemistry
GA 200WF
UT WOS:000323100900001
ER
PT J
AU Gross, E
Somorjai, GA
AF Gross, Elad
Somorjai, Gabor A.
TI The Impact of Electronic Charge on Catalytic Reactivity and Selectivity
of Metal-Oxide Supported Metallic Nanoparticles
SO TOPICS IN CATALYSIS
LA English
DT Article
DE Heterogeneous catalysis; Selectivity; Charge transfer; CO oxidation;
Metal-oxide; Metal-support interactions
ID GENERATION VIBRATIONAL SPECTROSCOPY; CO OXIDATION; HETEROGENEOUS
CATALYST; NANOCRYSTALLINE CEO2; CARBON-MONOXIDE; TITANIUM-OXIDE; LEWIS
ACIDITY; SYNTHESIS GAS; GOLD; HYDROGENATION
AB The catalytic reactivity and selectivity of metallic nanoclusters supported on a metal-oxide can be tuned by electronic charge. In this review, different approaches for controlling the electronic properties of metallic nanoclusters and its impact on catalytic reactions are discussed. Electronic charge can transfer from the metal-oxide support to the metallic catalyst and change the metal-reactants interaction and as a consequence modify as-well the catalytic reactivity and selectivity. In other cases, the electronic properties of the metal-oxide have an active role in the catalytic process and the metal oxide can be used as a co-catalyst. Another approach is to directly change the electronic properties of the metallic catalyst. It is demonstrated that dendrimer-encapsulated metallic nanoparticles can be directly oxidized by the addition of an inorganic oxidizer to the solution phase. In this case, even while supported on inert oxides, novel catalytic reactivity and selectivity can be gained by the formation of highly oxidized metal ions.
C1 [Gross, Elad; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
[Gross, Elad; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
EM somorjai@berkeley.edu
FU Office of Science, Office of Basic Energy Sciences of the US Department
of Energy [DE-AC02-05CH11231]
FX This work was supported by the Director, Office of Science, Office of
Basic Energy Sciences of the US Department of Energy under Contract No.
DE-AC02-05CH11231.
NR 47
TC 12
Z9 12
U1 3
U2 83
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1022-5528
EI 1572-9028
J9 TOP CATAL
JI Top. Catal.
PD AUG
PY 2013
VL 56
IS 12
BP 1049
EP 1058
DI 10.1007/s11244-013-0069-3
PG 10
WC Chemistry, Applied; Chemistry, Physical
SC Chemistry
GA 200WF
UT WOS:000323100900002
ER
PT J
AU Choi, YM
Kuttiyiel, KA
Labis, JP
Sasaki, K
Park, GG
Yang, TH
Adzic, RR
AF Choi, YongMan
Kuttiyiel, Kurian A.
Labis, Joselito P.
Sasaki, Kotaro
Park, Gu-Gon
Yang, Tae-Hyun
Adzic, Radoslav R.
TI Enhanced Oxygen Reduction Activity of IrCu Core Platinum Monolayer Shell
Nano-electrocatalysts
SO TOPICS IN CATALYSIS
LA English
DT Article
DE Fuel cells; Electrocatalysis; Core-shell catalyst; Pt monolayer; Cu
underpotential deposition; Oxygen reduction
ID CATALYTIC-ACTIVITY; NANOPARTICLES; STABILITY
AB Designing novel cathode materials for a proton exchange membrane fuel cell with high activity for the oxygen reduction reaction, low Pt loading, and enhanced long-term stability is imperative for its sustainability. To date, Pt monolayer based electrocatalysts deposited on a metallic core substrate have shown promising possibilities. In this study, we synthesized bimetallic IrCu nanoparticles and used them as a core for Pt monolayer electrocatalysts. It was found that the de-alloyed IrCu nanoparticle surfaces increased both the mass and specific activities of the resulting Pt monolayer catalyst. In addition, we demonstrated that Pt monolayer electrocatalysts with a de-alloyed IrCu core have a better stability than those using a non-dealloyed core based on a 5,000 potential cycling test. These data describe a new simple synthesis of a high-performance catalyst suitable for practical applications.
C1 [Choi, YongMan] SABIC Technol Ctr, Riyadh 11551, Saudi Arabia.
[Choi, YongMan; Kuttiyiel, Kurian A.; Sasaki, Kotaro; Adzic, Radoslav R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Labis, Joselito P.] King Saud Univ, King Abdullah Inst Nanotechnol, Riyadh 11451, Saudi Arabia.
[Park, Gu-Gon; Yang, Tae-Hyun] Korea Inst Energy Res, Fuel Cell Res Ctr, Taejon 305343, South Korea.
RP Choi, YM (reprint author), SABIC Technol Ctr, Riyadh 11551, Saudi Arabia.
EM choiy@sabic.com; adzic@bnl.gov
RI Choi, YongMan/N-3559-2014; Park, Gu-Gon/A-6175-2013
OI Choi, YongMan/0000-0003-4276-1599; Park, Gu-Gon/0000-0002-4606-0661
FU Brookhaven National laboratory [DE-AC02-98CH10886]; Korea Institute of
Energy Research (KIER) [B3-2415]
FX This research was performed at Brookhaven National laboratory under
contract DE-AC02-98CH10886 with the US Department of Energy, Division of
Chemical Sciences, Geosciences and Biosciences Division. This work was
conducted under the framework of Research and Development Program of the
Korea Institute of Energy Research (KIER) (B3-2415). Y.C. truly
acknowledges the kind support by Drs. Hicham Idriss and Essam H. Jamea
to carry out this project in Brookhaven National Laboratory. Also, Y.C.
thanks Dr. Toseef N. Ahmed and Hugh Issacs and Wei-Fu Chen for SEM/EDX
measurements and fruitful discussion on electrochemistry, respectively.
NR 25
TC 11
Z9 11
U1 6
U2 94
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1022-5528
EI 1572-9028
J9 TOP CATAL
JI Top. Catal.
PD AUG
PY 2013
VL 56
IS 12
BP 1059
EP 1064
DI 10.1007/s11244-013-0070-x
PG 6
WC Chemistry, Applied; Chemistry, Physical
SC Chemistry
GA 200WF
UT WOS:000323100900003
ER
PT J
AU Tobin, JG
Yu, SW
Chung, BW
AF Tobin, J. G.
Yu, S. -W.
Chung, B. W.
TI Splittings, Satellites and Fine Structure in the Soft X-ray Spectroscopy
of the Actinides
SO TOPICS IN CATALYSIS
LA English
DT Article
DE XAS U d levels; XAS Ce d levels; Lanthanides satellites fine structure;
U 5f DOS; XPS U 4d; EELS Ce 3d; UO2 Bremstrahlung isochromat
spectroscopy (BIS); UO2 resonant inverse photoelectron spectroscopy
(RIPES)
ID UNOCCUPIED ELECTRONIC-STRUCTURE; RESONANT INVERSE-PHOTOEMISSION;
URANIUM-DIOXIDE; PHOTOELECTRON; THORIUM; SYSTEMS; ENERGY; STATES; 5F
AB Perhaps the most demanding and powerful actinide spectroscopy is that using soft X-ray and VUV photons. Because of the relatively low energy and fairly small sampling depths of these photons and the corresponding electrons, it is necessary to use un-encapsulated samples with highly cleaned and well-prepared surfaces. This causes a myriad of sample containment problems for these radioactive materials. Despite these hindrances and difficulties, the soft-X-ray and ultra-violet spectroscopy of the actinides can provide an amazing level of detailed information, particularly having to do with 5f electronic structure. In this paper, the splittings, satellites and fine structure of the following actinide soft X-ray spectroscopies will be discussed: X-ray photoelectron spectroscopy; X-ray absorption spectroscopy; and inverse photoelectron spectroscopy, including Bremstrahlung isochromat spectroscopy and resonant inverse photoelectron spectroscopy.
C1 [Tobin, J. G.; Yu, S. -W.; Chung, B. W.] Lawrence Livermore Natl Lab, Livermore, CA USA.
RP Tobin, JG (reprint author), Lawrence Livermore Natl Lab, Livermore, CA USA.
EM Tobin1@LLNL.Gov
RI Tobin, James/O-6953-2015; Chung, Brandon/G-2929-2012
FU U.S. Department of Energy, National Nuclear Security Administration
[DE-AC52-07NA27344]; DOE Office of Science, Office of Basic Energy
Science, Division of Materials Science and Engineering
FX Lawrence Livermore National Laboratory is operated by Lawrence Livermore
National Security, LLC, for the U.S. Department of Energy, National
Nuclear Security Administration under Contract DE-AC52-07NA27344. This
work was supported by the DOE Office of Science, Office of Basic Energy
Science, Division of Materials Science and Engineering.
NR 34
TC 2
Z9 2
U1 0
U2 36
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1022-5528
J9 TOP CATAL
JI Top. Catal.
PD AUG
PY 2013
VL 56
IS 12
BP 1104
EP 1111
DI 10.1007/s11244-013-0076-4
PG 8
WC Chemistry, Applied; Chemistry, Physical
SC Chemistry
GA 200WF
UT WOS:000323100900009
ER
PT J
AU Bagus, P
Ilton, E
AF Bagus, Paul S.
Ilton, Eugene S.
TI Theory for the XPS of Actinides
SO TOPICS IN CATALYSIS
LA English
DT Article
DE XPS; Actinides; Covalent bonding; Electronic structure; Wavefunctions;
Intermediate coupling
ID RAY PHOTOEMISSION SPECTRA; TRANSITION-METALS; IONIC-CRYSTALS; FIELD;
SPECTROSCOPY; SATELLITES; STATES; UO2
AB Two aspects of the electronic structure of actinide oxides that significantly affect the X-ray photoelectron spectroscopy (XPS) spectra are described; these aspects are also important for the materials properties of the oxides. The two aspects considered are: (1) The spin-orbit coupling of the open 5f shell electrons in actinide cations and how this coupling affects the electronic structure. And, (2) the covalent character of the metal oxygen interaction in actinide compounds. Because of this covalent character, there are strong departures from the nominal oxidation states that are significantly larger in core-hole states than in the ground state. The consequences of this covalent character for the XPS are examined. A proper understanding of the way in which they influence the XPS makes it possible to use the XPS to correctly characterize the electronic structure of the oxides.
C1 [Bagus, Paul S.] Univ N Texas, Dept Chem, Denton, TX 76203 USA.
[Ilton, Eugene S.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Bagus, PS (reprint author), Univ N Texas, Dept Chem, Denton, TX 76203 USA.
EM bagus@unt.edu
RI Bagus, Paul/M-1273-2015
FU Geosciences Research Program, Office of Basic Energy Sciences, U.S. DOE
FX We acknowledge support by the Geosciences Research Program, Office of
Basic Energy Sciences, U.S. DOE.
NR 35
TC 5
Z9 5
U1 2
U2 21
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1022-5528
EI 1572-9028
J9 TOP CATAL
JI Top. Catal.
PD AUG
PY 2013
VL 56
IS 12
BP 1121
EP 1128
DI 10.1007/s11244-013-0078-2
PG 8
WC Chemistry, Applied; Chemistry, Physical
SC Chemistry
GA 200WF
UT WOS:000323100900011
ER
PT J
AU Liebschner, D
Dauter, M
Brzuszkiewicz, A
Dauter, Z
AF Liebschner, Dorothee
Dauter, Miroslawa
Brzuszkiewicz, Anna
Dauter, Zbigniew
TI On the reproducibility of protein crystal structures: five atomic
resolution structures of trypsin
SO ACTA CRYSTALLOGRAPHICA SECTION D-BIOLOGICAL CRYSTALLOGRAPHY
LA English
DT Article
ID INDEPENDENTLY REFINED MODELS; X-RAY CRYSTALLOGRAPHY; RADIATION-DAMAGE;
ACCURACY; DIFFRACTION; HYDRATION; GEOMETRY; DATABASE
AB Structural studies of proteins usually rely on a model obtained from one crystal. By investigating the details of this model, crystallographers seek to obtain insight into the function of the macromolecule. It is therefore important to know which details of a protein structure are reproducible or to what extent they might differ. To address this question, the high-resolution structures of five crystals of bovine trypsin obtained under analogous conditions were compared. Global parameters and structural details were investigated. All of the models were of similar quality and the pairwise merged intensities had large correlation coefficients. The C-alpha and backbone atoms of the structures superposed very well. The occupancy of ligands in regions of low thermal motion was reproducible, whereas solvent molecules containing heavier atoms (such as sulfur) or those located on the surface could differ significantly. The coordination lengths of the calcium ion were conserved. A large proportion of the multiple conformations refined to similar occupancies and the residues adopted similar orientations. More than three quarters of the water-molecule sites were conserved within 0.5 angstrom and more than one third were conserved within 0.1 angstrom. An investigation of the protonation states of histidine residues and carboxylate moieties was consistent for all of the models. Radiation-damage effects to disulfide bridges were observed for the same residues and to similar extents. Main-chain bond lengths and angles averaged to similar values and were in agreement with the Engh and Huber targets. Other features, such as peptide flips and the double conformation of the inhibitor molecule, were also reproducible in all of the trypsin structures. Therefore, many details are similar in models obtained from different crystals. However, several features of residues or ligands located in flexible parts of the macromolecule may vary significantly, such as side-chain orientations and the occupancies of certain fragments.
C1 [Liebschner, Dorothee; Brzuszkiewicz, Anna; Dauter, Zbigniew] NCI, Argonne Natl Lab, MCL, Synchrotron Radiat Res Sect, Argonne, IL 60439 USA.
[Dauter, Miroslawa] Argonne Natl Lab, Basic Res Program, SAIC Frederick Inc, Argonne, IL 60439 USA.
[Brzuszkiewicz, Anna] Univ Wroclaw, Fac Chem, PL-50383 Wroclaw, Poland.
RP Dauter, Z (reprint author), NCI, Argonne Natl Lab, MCL, Synchrotron Radiat Res Sect, Argonne, IL 60439 USA.
EM dauter@anl.gov
FU National Cancer Institute, National Institutes of Health [NO1-CO-12400];
NIH, National Cancer Institute, Center for Cancer Research; US
Department of Energy, Office of Science, Office of Basic Energy Sciences
[W-31-109-Eng-38]
FX This work was supported in part with Federal funds from the National
Cancer Institute, National Institutes of Health contract No.
NO1-CO-12400 and the Intramural Research Program of the NIH, National
Cancer Institute, Center for Cancer Research. The content of this
publication does not necessarily reflect the views or policies of the
Department of Health and Human Services, nor does the mention of trade
names, commercial products or organizations imply endorsement by the US
Government. Diffraction data were collected on the NE-CAT beamline 24-ID
at the Advanced Photon Source, Argonne National Laboratory. Use of the
Advanced Photon Source was supported by the US Department of Energy,
Office of Science, Office of Basic Energy Sciences, under Contract No.
W-31-109-Eng-38.
NR 41
TC 23
Z9 24
U1 2
U2 23
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0907-4449
J9 ACTA CRYSTALLOGR D
JI Acta Crystallogr. Sect. D-Biol. Crystallogr.
PD AUG
PY 2013
VL 69
BP 1447
EP 1462
DI 10.1107/S0907444913009050
PN 8
PG 16
WC Biochemical Research Methods; Biochemistry & Molecular Biology;
Biophysics; Crystallography
SC Biochemistry & Molecular Biology; Biophysics; Crystallography
GA 191WJ
UT WOS:000322445100012
PM 23897468
ER
PT J
AU Finfrock, YZ
Stern, EA
Alkire, RW
Kas, JJ
Evans-Lutterodt, K
Stein, A
Duke, N
Lazarski, K
Joachimiak, A
AF Finfrock, Y. Zou
Stern, Edward A.
Alkire, R. W.
Kas, Joshua J.
Evans-Lutterodt, Kenneth
Stein, Aaron
Duke, Norma
Lazarski, Krzysztof
Joachimiak, Andrzej
TI Mitigation of X-ray damage in macromolecular crystallography by
submicrometre line focusing
SO ACTA CRYSTALLOGRAPHICA SECTION D-BIOLOGICAL CRYSTALLOGRAPHY
LA English
DT Article
ID RADIATION-DAMAGE; PROTEIN CRYSTALS; CRYOGENIC TEMPERATURES; DIFFRACTION;
DEPENDENCE; ELECTRON; BEAM; RESOLUTION; SULFUR; CASINO
AB Reported here are measurements of the penetration depth and spatial distribution of photoelectron (PE) damage excited by 18.6 keV X-ray photons in a lysozyme crystal with a vertical submicrometre line-focus beam of 0.7 mm full-width half-maximum (FWHM). The experimental results determined that the penetration depth of PEs is 5 +/- 0.5 mu m with a monotonically decreasing spatial distribution shape, resulting in mitigation of diffraction signal damage. This does not agree with previous theoretical predication that the mitigation of damage requires a peak of damage outside the focus. A new improved calculation provides some qualitative agreement with the experimental results, but significant errors still remain. The mitigation of radiation damage by line focusing was measured experimentally by comparing the damage in the X-ray-irradiated regions of the submicrometre focus with the large-beam case under conditions of equal exposure and equal volumes of the protein crystal, and a mitigation factor of 4.4 +/- 0.4 was determined. The mitigation of radiation damage is caused by spatial separation of the dominant PE radiation-damage component from the crystal region of the line-focus beam that contributes the diffraction signal. The diffraction signal is generated by coherent scattering of incident X-rays (which introduces no damage), while the overwhelming proportion of damage is caused by PE emission as X-ray photons are absorbed.
C1 [Finfrock, Y. Zou; Stern, Edward A.; Kas, Joshua J.] Univ Washington, Dept Phys, Seattle, WA 98195 USA.
[Alkire, R. W.; Duke, Norma; Lazarski, Krzysztof] Argonne Natl Lab, Struct Biol Ctr, Argonne, IL 60439 USA.
[Evans-Lutterodt, Kenneth; Stein, Aaron] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA.
[Joachimiak, Andrzej] Argonne Natl Lab, Ctr Mechanist Biol & Biotechnol, Argonne, IL 60439 USA.
RP Stern, EA (reprint author), Univ Washington, Dept Phys, Seattle, WA 98195 USA.
EM stern@phys.washington.edu
OI Stein, Aaron/0000-0003-4424-5416
FU National Science Foundation (NSF) [0650547]; US Department of Energy
(DOE), Office of Biological and Environmental Research
[DE-AC02-06CH11357]; US DOE, Office of Basic Energy Sciences
[DE-AC02-98CH10886]
FX The authors wish to thank the members of the Structural Biology Center
at Argonne National Laboratory for their help with data collection on
the 19-ID beamline, Kenneth Thompson and Jim Greenwell at the University
of Washington Physics Shop for helping with the design and construction
of the apparatus and Yizhak Yacoby from Hebrew University for valuable
discussions. This work was supported by the National Science Foundation
(NSF) under Grant No. 0650547 and by the US Department of Energy (DOE),
Office of Biological and Environmental Research under contract
DE-AC02-06CH11357. The lenses were fabricated in part at the Brookhaven
National Laboratory CFN supported by the US DOE, Office of Basic Energy
Sciences under Contract No. DE-AC02-98CH10886 and in part at the Cornell
CNF, a member of the NNIN, supported by the NSF.
NR 34
TC 4
Z9 4
U1 3
U2 15
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0907-4449
J9 ACTA CRYSTALLOGR D
JI Acta Crystallogr. Sect. D-Biol. Crystallogr.
PD AUG
PY 2013
VL 69
BP 1463
EP 1469
DI 10.1107/S0907444913009335
PN 8
PG 7
WC Biochemical Research Methods; Biochemistry & Molecular Biology;
Biophysics; Crystallography
SC Biochemistry & Molecular Biology; Biophysics; Crystallography
GA 191WJ
UT WOS:000322445100013
PM 23897469
ER
PT J
AU Saleh, AA
Pereloma, EV
Clausen, B
Brown, DW
Tome, CN
Gazder, AA
AF Saleh, Ahmed A.
Pereloma, Elena V.
Clausen, Bjorn
Brown, Donald W.
Tome, Carlos N.
Gazder, Azdiar A.
TI On the evolution and modelling of lattice strains during the cyclic
loading of TWIP steel
SO ACTA MATERIALIA
LA English
DT Article
DE TWIP steel; Neutron diffraction; Lattice strain; Bauschinger effect;
EPSC
ID INDUCED PLASTICITY STEELS; STACKING-FAULT ENERGY; STAINLESS-STEEL;
SINGLE-CRYSTALS; INTERGRANULAR STRAINS; STRESS-RELAXATION;
ELASTIC-CONSTANTS; INTERNAL-STRESSES; AUSTENITIC STEEL; METAL CRYSTALS
AB The evolution of lattice strains in fully annealed Fe-24Mn-3Al-2Si-1Ni-0.06C twinning-induced plasticity (TWIP) steel is investigated via in situ neutron diffraction during cyclic (tension compression) loading between strain limits of +/- 1%. The pronounced Bauschinger effect observed upon load reversal is accounted for by a combination of the intergranular residual stresses and the intragranular sources of back stress, such as dislocation pile-ups at the intersection of stacking faults. The recently modified elasto-plastic self-consistent (EPSC) model which empirically accounts for both intergranular and intragranular back stresses has been successfully used to simulate the macroscopic stress-strain response and the evolution of the lattice strains. The EPSC model captures the experimentally observed tension-compression asymmetry as it accounts for the directionality of twinning as well as Schmid factor considerations. For the strain limits used in this study, the EPSC model also predicts that the lower flow stress on reverse shear loading reported in earlier Bauschinger-type experiments on TWIP steel is a geometrical or loading path effect. (C) 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
C1 [Saleh, Ahmed A.; Pereloma, Elena V.; Gazder, Azdiar A.] Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2522, Australia.
[Pereloma, Elena V.; Gazder, Azdiar A.] Univ Wollongong, Electron Microscopy Ctr, Wollongong, NSW 2519, Australia.
[Clausen, Bjorn] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA.
[Brown, Donald W.; Tome, Carlos N.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
RP Saleh, AA (reprint author), Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2522, Australia.
EM asaleh@uow.edu.au
RI Clausen, Bjorn/B-3618-2015; Tome, Carlos/D-5058-2013;
OI Clausen, Bjorn/0000-0003-3906-846X; Saleh, Ahmed/0000-0002-0807-6718
FU Commonwealth of Australia under the International Science Linkages
program; US Department of Energy, Office of Basic Energy Sciences,
Division of Materials Sciences and Engineering [FWP 06SCPE401,
W-7405-ENG-36]; Office of Basic Energy Sciences (DOE), USA; Engineering
Materials Institute, UOW, Australia; Los Alamos National Security LLC
under US DOE [DE AC52 06NA25396]
FX The authors are grateful to Prof. D.B. Santos of the Federal University
of Minas Gerais, Brazil for providing the source material. The access to
major research facilities program (AMRFP) is supported by the
Commonwealth of Australia under the International Science Linkages
program. Dr. Carlos Tome was fully supported by the US Department of
Energy, Office of Basic Energy Sciences, Division of Materials Sciences
and Engineering, Project FWP 06SCPE401 under US DOE Contract No.
W-7405-ENG-36. This work has benefited from the use of the Lu-jan
Neutron Scattering Center at LANSCE, which is funded by the Office of
Basic Energy Sciences (DOE), USA and from the partial funding from the
Engineering Materials Institute, UOW, Australia. The Los Alamos National
Laboratory is operated by Los Alamos National Security LLC under US DOE
Contract DE AC52 06NA25396.
NR 60
TC 13
Z9 13
U1 2
U2 39
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-6454
J9 ACTA MATER
JI Acta Mater.
PD AUG
PY 2013
VL 61
IS 14
BP 5247
EP 5262
DI 10.1016/j.actamat.2013.05.017
PG 16
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering
SC Materials Science; Metallurgy & Metallurgical Engineering
GA 196CK
UT WOS:000322750800013
ER
PT J
AU Porta, M
Lookman, T
AF Porta, Marcel
Lookman, Turab
TI Heterogeneity and phase transformation in materials: Energy
minimization, iterative methods and geometric nonlinearity
SO ACTA MATERIALIA
LA English
DT Article
DE Strain compatibility; Finite deformation; Ferroelastics; Spectral
methods; Dynamics
ID MARTENSITIC-TRANSFORMATION; COMPOSITES; COMPATIBILITY; STRAINS;
FERROELASTICS; DISLOCATIONS; MECHANICS; CONTRAST; KINETICS; ALLOYS
AB We consider the relationship between methods used to solve problems involving heterogeneities with a focus on phase transformations. We compare methods that solve for mechanical equilibrium based on iterative spectral techniques with those evolving a free energy using inertial and relaxational dynamics in terms of microstructure, convergence and efficiency for the two-dimensional versions of the cubic-to-tetragonal and hexagonal-to-orthorhombic transformations. We generalize the strain-based approach using kinematic compatibility, in conjunction with a Landau-based nonconvex energy functional, to the geometrically nonlinear case for computation using the iterative spectral as well energy-minimizing methods. Our approach uses the strain compatibility equations for geometrically nonlinear elasticity in two dimensions, the geometrically linear strain compatibility equations being recovered in the small strain limit. We show how for the two-dimensional version of the hexagonal-to-orthorhombic transformation with three variant distortions in the microstructure, the linear compatibility equations capture relatively large rotations with small to moderate stains. We propose a reconstruction that uses the mapping between displacement gradients and Lagrange strains to approximate the geometrically nonlinear result within the scope of the linear strain theory if the linear strains are substituted for the Lagrange strains. We illustrate this by evaluating the disclination angle associated with the unique microstructure for this transformation, which otherwise requires geometric nonlinear theory to correctly capture. (C) 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
C1 [Porta, Marcel; Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
RP Porta, M (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
EM mportatena@gmail.com
OI Porta Tena, Marcel/0000-0001-7582-9671
FU US DOE [DE-AC52-06NA25396]; NSERC of Canada
FX We thank A. Acharya, K. Barros, K. Dayal, R. Groger, R.A. Lebensohn and
S.R. Shenoy for stimulating discussions on aspects of this work. Support
from the US DOE under Contract No. DE-AC52-06NA25396 and NSERC of Canada
is gratefully acknowledged.
NR 44
TC 4
Z9 4
U1 2
U2 18
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-6454
J9 ACTA MATER
JI Acta Mater.
PD AUG
PY 2013
VL 61
IS 14
BP 5311
EP 5340
DI 10.1016/j.actamat.2013.05.022
PG 30
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering
SC Materials Science; Metallurgy & Metallurgical Engineering
GA 196CK
UT WOS:000322750800018
ER
PT J
AU Tracey, B
Wolpert, D
Alonso, JJ
AF Tracey, Brendan
Wolpert, David
Alonso, Juan J.
TI Using Supervised Learning to Improve Monte Carlo Integral Estimation
SO AIAA JOURNAL
LA English
DT Article
ID POLYNOMIAL CHAOS
AB Monte Carlo techniques are used to estimate the integrals of a function using randomly generated samples. The interest in uncertainty quantification and robust design makes calculating the expected values of such functions (e.g., performance measures) important. Recent developments in scramjets, aircraft technology forecasting, structural reliability, and robust low-boom aircraft designs use Monte Carlo techniques to ensure the appropriate quantification of uncertainties. Because of high variance and slow convergence, Monte Carlo techniques require a large number of function evaluations, limiting the fidelity of the tools that can be used to predict performance. Stacked Monte Carlo is presented, which is a new method for postprocessing an existing set of Monte Carlo samples to improve integral estimation. Stacked Monte Carlo is based on combining fitting functions with cross-validation and should reduce the variance of any type of Monte Carlo integral estimate (importance sampling, quasi-Monte Carlo, etc.) without adding bias. An extensive set of experiments is reported, confirming that the stacked Monte Carlo estimate is more accurate than both the unprocessed Monte Carlo estimate and the estimate from a functional fit. Stacked Monte Carlo is applied to estimate the fuel-burn metrics of future commercial aircraft and sonic boom loudness measures, and the efficiency of Monte Carlo is compared with that of more standard methods. It is shown that for negligible, additional, computational cost, significant increases in accuracy are gained.
C1 [Tracey, Brendan; Alonso, Juan J.] Stanford Univ, Dept Aeronaut & Astronaut, Stanford, CA 94305 USA.
[Wolpert, David] Los Alamos Natl Lab, Informat Sci Grp, Santa Fe Inst, Los Alamos, NM 87545 USA.
RP Tracey, B (reprint author), Stanford Univ, Dept Aeronaut & Astronaut, Durand Bldg 496 Lomita Mall, Stanford, CA 94305 USA.
NR 23
TC 4
Z9 4
U1 0
U2 8
PU AMER INST AERONAUTICS ASTRONAUTICS
PI RESTON
PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA
SN 0001-1452
J9 AIAA J
JI AIAA J.
PD AUG
PY 2013
VL 51
IS 8
BP 2015
EP 2023
DI 10.2514/1.J051655
PG 9
WC Engineering, Aerospace
SC Engineering
GA 193JZ
UT WOS:000322557400019
ER
PT J
AU Swisher, JA
Lin, LC
Kim, J
Smit, B
AF Swisher, Joseph A.
Lin, Li-Chiang
Kim, Jihan
Smit, Berend
TI Evaluating mixture adsorption models using molecular simulation
SO AICHE JOURNAL
LA English
DT Article
DE adsorption; gas; simulation; molecular; computer simulations (MC and
MD); thermodynamics; classical; zeolites
ID METAL-ORGANIC FRAMEWORKS; ADSORBED SOLUTION THEORY; CARBON-DIOXIDE
ADSORPTION; MONTE-CARLO SIMULATIONS; MIXED-GAS ADSORPTION; ACTIVATED
CARBON; BINARY-MIXTURES; HETEROGENEOUS SURFACES; NANOPOROUS MATERIALS;
NONIDEAL MIXTURES
AB The design of adsorption-based separation processes using novel adsorbents requires reliable data for the adsorption of fluid mixtures on candidate adsorbents. Due to the difficulty of generating sufficient data across possible operating conditions, process designs generally rely on interpolation of pure-component data using a model, most commonly ideal adsorbed solution theory (IAST), and related theories. There are many cases where IAST fails to provide an adequate description of mixture adsorption, usually due to the fact that practical adsorbents do not have uniform surfaces. We have evaluated the use of a segregated version of IAST, where competition is assumed to occur at isolated adsorption sites. This simple modification can provide the correct description of adsorption across a large range of pressures using ideal isotherm models. We also demonstrate the importance of identifying multiple sites even for weakly adsorbing components to provide the correct behavior at high pressure. (c) 2013 American Institute of Chemical Engineers AIChE J, 59: 3054-3064, 2013
C1 [Swisher, Joseph A.; Lin, Li-Chiang; Kim, Jihan] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.
[Swisher, Joseph A.; Lin, Li-Chiang; Kim, Jihan; Smit, Berend] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
RP Smit, B (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
EM berend-smit@berkeley.edu
RI Smit, Berend/B-7580-2009; EFRC, CGS/I-6680-2012; Kim, Jihan/H-8002-2013;
Lin, Li-Chiang/J-8120-2014; Stangl, Kristin/D-1502-2015;
OI Smit, Berend/0000-0003-4653-8562; Lin, Li-Chiang/0000-0002-2821-9501
FU Advanced Research Projects Agency-Energy (ARPA-E), U.S. Department of
Energy; Deutsche Forschungsgemeinschaft (DFG) [SPP 1570]; U.S.
Department of Energy through the Carbon Capture Simulation Initiative
(CCSI) [DE-AC02-05CH11231]; Center for Gas Separations Relevant to Clean
Energy Technologies, an Energy Frontier Research Center; U.S. Department
of Energy, Office of Science, Office of Basic Energy Sciences
[DE-SC0001015]; NIH; Theoretical and Computational Biophysics group at
the Beckman Institute, University of Illinois at Urbana-Champaign
FX J.A.S. was supported by funding from the Advanced Research Projects
Agency-Energy (ARPA-E), U.S. Department of Energy. L.-C. L. was
supported by the Deutsche Forschungsgemeinschaft (DFG, priority program
SPP 1570). J.K. was supported by the U.S. Department of Energy under
contract DE-AC02-05CH11231 through the Carbon Capture Simulation
Initiative (CCSI). B. S. was supported as part of the Center for Gas
Separations Relevant to Clean Energy Technologies, an Energy Frontier
Research Center funded by the U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences under Award Number
DE-SC0001015. Figures 3, 5, and 7 were made with VMD software support.
VMD is developed with NIH support by the Theoretical and Computational
Biophysics group at the Beckman Institute, University of Illinois at
Urbana-Champaign.
NR 41
TC 9
Z9 9
U1 2
U2 48
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0001-1541
J9 AICHE J
JI AICHE J.
PD AUG
PY 2013
VL 59
IS 8
BP 3054
EP 3064
DI 10.1002/aic.14058
PG 11
WC Engineering, Chemical
SC Engineering
GA 185IG
UT WOS:000321960400029
ER
PT J
AU Spagnolo, V
Patimisco, P
Borri, S
Scamarcio, G
Bernacki, BE
Kriesel, J
AF Spagnolo, Vincenzo
Patimisco, Pietro
Borri, Simone
Scamarcio, Gaetano
Bernacki, Bruce E.
Kriesel, Jason
TI Mid-infrared fiber-coupled QCL-QEPAS sensor
SO APPLIED PHYSICS B-LASERS AND OPTICS
LA English
DT Article
ID QUANTUM CASCADE LASER; ENHANCED PHOTOACOUSTIC-SPECTROSCOPY
AB An innovative spectroscopic system based on an external cavity quantum cascade laser (EC-QCL) coupled with a mid-infrared (mid-IR) fiber and quartz enhanced photoacoustic spectroscopy (QEPAS) is described. SF6 has been selected as a target gas in demonstration of the system for trace gas sensing. Single mode laser delivery through the prongs of the quartz tuning fork has been obtained employing a hollow waveguide fiber with inner silver-silver iodine (Ag-AgI) coatings and internal core diameter of 300 mu m. A detailed design and realization of the QCL fiber coupling and output collimator system allowed almost practically all (99.4 %) of the laser beam to be transmitted through the spectrophone module. The achieved sensitivity of the system is 50 parts per trillion in 1 s, corresponding to a record for QEPAS normalized noise-equivalent absorption of 2.7 x 10(-10) W cm(-1) Hz(-1/2).
C1 [Spagnolo, Vincenzo; Patimisco, Pietro; Borri, Simone; Scamarcio, Gaetano] Univ Bari, Dipartimento Interateneo Fis, Bari, Italy.
[Spagnolo, Vincenzo; Patimisco, Pietro; Borri, Simone; Scamarcio, Gaetano] Politecn Bari, CNR IFN UOS BARI, Bari, Italy.
[Bernacki, Bruce E.] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Kriesel, Jason] Optoknowledge Syst Inc, Torrance, CA USA.
RP Spagnolo, V (reprint author), Univ Bari, Dipartimento Interateneo Fis, Via Amendola 173, Bari, Italy.
EM spagnolo@fisica.uniba.it
RI Scamarcio, Gaetano/I-7674-2014;
OI Scamarcio, Gaetano/0000-0003-0808-4336; Borri,
Simone/0000-0001-8471-2803; Spagnolo, Vincenzo/0000-0002-4867-8166
FU [PON01_02238]; [PON02_00675]
FX The authors acknowledge financial support from the Italian research
projects: PON01_02238 and PON02_00675.
NR 26
TC 35
Z9 36
U1 6
U2 55
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 0946-2171
J9 APPL PHYS B-LASERS O
JI Appl. Phys. B-Lasers Opt.
PD AUG
PY 2013
VL 112
IS 1
BP 25
EP 33
DI 10.1007/s00340-013-5388-3
PG 9
WC Optics; Physics, Applied
SC Optics; Physics
GA 194ZP
UT WOS:000322671500003
ER
PT J
AU Kuncarayakti, H
Doi, M
Aldering, G
Arimoto, N
Maeda, K
Morokuma, T
Pereira, R
Usuda, T
Hashiba, Y
AF Kuncarayakti, Hanindyo
Doi, Mamoru
Aldering, Greg
Arimoto, Nobuo
Maeda, Keiichi
Morokuma, Tomoki
Pereira, Rui
Usuda, Tomonori
Hashiba, Yasuhito
TI INTEGRAL FIELD SPECTROSCOPY OF SUPERNOVA EXPLOSION SITES: CONSTRAINING
THE MASS AND METALLICITY OF THE PROGENITORS. II. TYPE II-P AND II-L
SUPERNOVAE
SO ASTRONOMICAL JOURNAL
LA English
DT Article
DE stars: massive; supernovae: general
ID CORE-COLLAPSE SUPERNOVAE; RED SUPERGIANT PROGENITOR; STAR-CLUSTERS;
SPIRAL GALAXIES; EVOLUTIONARY SEQUENCES; RADIATIVE OPACITIES; STELLAR
MODELS; HOST GALAXIES; SN 2002HH; REGIONS
AB Thirteen explosion sites of Type II-P and II-L supernovae (SNe) in nearby galaxies have been observed using integral field spectroscopy, enabling both spatial and spectral study of the explosion sites. We used the properties of the parent stellar population of the coeval SN progenitor star to derive its metallicity and initial mass. The spectrum of the parent stellar population yields estimates of metallicity via the strong-line method and age via a comparison with simple stellar population models. These metallicity and age parameters are adopted for the progenitor star. Age, or lifetime of the star, was used to derive the initial (zero-age main sequence) mass of the star using comparisons with stellar evolution models. With this technique, we were able to determine the metallicities and initial masses of the SN progenitors in our sample. Our results indicate that some Type II SN progenitors may have been stars with masses comparable to those of SN Ib/c progenitors.
C1 [Kuncarayakti, Hanindyo; Maeda, Keiichi] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan.
[Kuncarayakti, Hanindyo; Doi, Mamoru; Morokuma, Tomoki; Hashiba, Yasuhito] Univ Tokyo, Grad Sch Sci, Inst Astron, Mitaka, Tokyo 1810015, Japan.
[Kuncarayakti, Hanindyo; Hashiba, Yasuhito] Univ Tokyo, Grad Sch Sci, Dept Astron, Bunkyo Ku, Tokyo 1130033, Japan.
[Doi, Mamoru] Univ Tokyo, Res Ctr Early Universe, Bunkyo Ku, Tokyo 1130033, Japan.
[Aldering, Greg] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA.
[Arimoto, Nobuo] Natl Astron Observ Japan, Mitaka, Tokyo 1810015, Japan.
[Arimoto, Nobuo; Usuda, Tomonori] Natl Astron Observ Japan, Subaru Telescope, Hilo, HI 96720 USA.
[Pereira, Rui] Inst Phys Nucl, CNRS, IN2P3, F-69622 Villeurbanne, France.
RP Kuncarayakti, H (reprint author), Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, 5-1-5 Kashiwanoha, Kashiwa, Chiba 2778583, Japan.
EM hanindyo.kuncarayakti@ipmu.jp
FU JSPS core-to-core program "International Research Network for Dark
Energy"; JSPS; National Astronomical Observatory of Japan; World Premier
International Research Center Initiative (WPI Initiative), MEXT, Japan;
Office of Science, Office of High Energy Physics, of the U.S. Department
of Energy [DE-AC02-05CH11231]; National Aeronautics and Space
Administration; [23740141]
FX We acknowledge the anonymous referee for helpful comments and
suggestions. H.K. acknowledges generous support from the Japanese
government MEXT (Monbukagakusho) scholarship. Useful help from R. Pain,
S. Rodney, and P. Weilbacher on working with data cubes is appreciated.
We thank G. Leloudas for carefully reading the draft and providing
important comments. We also thank J. Sollerman and F. Taddia for helpful
comments on the draft of the manuscript. This work was supported in part
by a JSPS core-to-core program "International Research Network for Dark
Energy" and by JSPS research grants. This work is based on the data from
the University of Hawaii 88 inch Telescope (UH88); the telescope time
was afforded from funding from the National Astronomical Observatory of
Japan. The work of K.M. is supported by the World Premier International
Research Center Initiative (WPI Initiative), MEXT, Japan, and
Grant-in-aid for Scientific Research (23740141). G.A. was supported by
the Director, Office of Science, Office of High Energy Physics, of the
U.S. Department of Energy under Contract No. DE-AC02-05CH11231. SNIFS on
the UH 2.2 m telescope is part of the Nearby Supernova Factory II
project, a scientific collaboration among the Centre de Recherche
Astronomique de Lyon, Institut de Physique Nucleaire de Lyon,
Laboratoire de Physique Nucleaire et des Hautes Energies, Lawrence
Berkeley National Laboratory, Yale University, University of Bonn, Max
Planck Institute for Astrophysics, Tsinghua Center for Astrophysics, and
the Centre de Physique des Particules de Marseille. This research has
made use of the SIMBAD database and ALADIN, operated at CDS, Strasbourg,
France. This research has made use of the NASA/IPAC Extragalactic
Database (NED), which is operated by the Jet Propulsion Laboratory,
California Institute of Technology, under contract with the National
Aeronautics and Space Administration. The authors recognize and
acknowledge the very significant cultural role and reverence that the
summit of Mauna Kea has always had within the indigenous Hawaiian
community. We are most fortunate to have the opportunity to conduct
observations from this mountain.
NR 66
TC 18
Z9 18
U1 0
U2 3
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-6256
EI 1538-3881
J9 ASTRON J
JI Astron. J.
PD AUG
PY 2013
VL 146
IS 2
AR 31
DI 10.1088/0004-6256/146/2/31
PG 14
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 183TW
UT WOS:000321841100013
ER
PT J
AU Kuncarayakti, H
Doi, M
Aldering, G
Arimoto, N
Maeda, K
Morokuma, T
Pereira, R
Usuda, T
Hashiba, Y
AF Kuncarayakti, Hanindyo
Doi, Mamoru
Aldering, Greg
Arimoto, Nobuo
Maeda, Keiichi
Morokuma, Tomoki
Pereira, Rui
Usuda, Tomonori
Hashiba, Yasuhito
TI INTEGRAL FIELD SPECTROSCOPY OF SUPERNOVA EXPLOSION SITES: CONSTRAINING
THE MASS AND METALLICITY OF THE PROGENITORS. I. TYPE Ib AND Ic
SUPERNOVAE
SO ASTRONOMICAL JOURNAL
LA English
DT Article
DE stars: massive; supernovae: general
ID CORE-COLLAPSE SUPERNOVAE; STAR-FORMATION; OBSERVATIONAL CONSTRAINTS;
MULTIOBJECT SPECTROGRAPH; EVOLUTIONARY SEQUENCES; SUPERGIANT PROGENITOR;
RELATIVE FREQUENCIES; RADIATIVE OPACITIES; STELLAR POPULATIONS;
SYNTHESIS MODELS
AB Integral field spectroscopy of 11 Type Ib/Ic supernova (SN Ib/Ic) explosion sites in nearby galaxies has been obtained using UH88/SNIFS and Gemini-N/GMOS. The use of integral field spectroscopy enables us to obtain both spatial and spectral information about the explosion site, enabling the identification of the parent stellar population of the SN progenitor star. The spectrum of the parent population provides metallicity determination via strong-line method and age estimation obtained via comparison with simple stellar population models. We adopt this information as the metallicity and age of the SN progenitor, under the assumption that it was coeval with the parent stellar population. The age of the star corresponds to its lifetime, which in turn gives the estimate of its initial mass. With this method we were able to determine both the metallicity and initial (zero-age main sequence) mass of the progenitor stars of SNe Ib and Ic. We found that on average SN Ic explosion sites are more metal-rich and younger than SN Ib sites. The initial mass of the progenitors derived from parent stellar population age suggests that SN Ic has more massive progenitors than SN Ib. In addition, we also found indication that some of our SN progenitors are less massive than similar to 25M(circle dot), indicating that they may have been stars in a close binary system that have lost their outer envelope via binary interactions to produce SNe Ib/Ic, instead of single Wolf-Rayet stars. These findings support the current suggestions that both binary and single progenitor channels are in effect in producing SNe Ib/Ic. This work also demonstrates the power of integral field spectroscopy in investigating SN environments and active star-forming regions.
C1 [Kuncarayakti, Hanindyo; Maeda, Keiichi] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan.
[Kuncarayakti, Hanindyo; Doi, Mamoru; Morokuma, Tomoki; Hashiba, Yasuhito] Univ Tokyo, Grad Sch Sci, Inst Astron, Mitaka, Tokyo 1810015, Japan.
[Kuncarayakti, Hanindyo; Hashiba, Yasuhito] Univ Tokyo, Grad Sch Sci, Dept Astron, Bunkyo Ku, Tokyo 1130033, Japan.
[Doi, Mamoru] Univ Tokyo, Res Ctr Early Universe, Bunkyo Ku, Tokyo 1130033, Japan.
[Aldering, Greg] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA.
[Arimoto, Nobuo] Natl Astron Observ Japan, Mitaka, Tokyo 1810015, Japan.
[Arimoto, Nobuo; Usuda, Tomonori] Natl Astron Observ Japan, Subaru Telescope, Hilo, HI 96720 USA.
[Pereira, Rui] Inst Phys Nucl, CNRS, IN2P3, F-69622 Villeurbanne, France.
RP Kuncarayakti, H (reprint author), Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, 5-1-5 Kashiwanoha, Kashiwa, Chiba 2778583, Japan.
EM hanindyo.kuncarayakti@ipmu.jp
FU National Astronomical Observatory of Japan; JSPS core-to core program
"International Research Network for Dark Energy"; JSPS; World Premier
International Research Center Initiative (WPI Initiative), MEXT, Japan;
Office of Science, Office of High Energy Physics, of the U.S. Department
of Energy [DE-AC02-05CH11231]; National Aeronautics and Space
Administration; [23740141]
FX We acknowledge the anonymous referee for helpful comments and
suggestions. H.K. acknowledges generous support from the Japanese
government MEXT (Monbukagakusho) scholarship. Useful help from R. Pain,
S. Rodney, and P. Weilbacher on working with data cubes is appreciated.
We thank G. Leloudas for carefully reading the draft and providing
important comments. We also thank J. Sollerman and F. Taddia for helpful
comments on the draft of the manuscript. We acknowledge excellent
support from Gemini Observatory staff for our observation. This work is
based on data collected using the Gemini Telescope, the opportunity for
which was made available by making use of the inter-observatory
time-exchange framework between Gemini and Subaru Observatories. This
work is based on data using the University of Hawaii 88 inch Telescope
(UH88), for which the telescope time was afforded by funding from the
National Astronomical Observatory of Japan. This work was supported in
part by a JSPS core-to core program "International Research Network for
Dark Energy" and by JSPS research grants. The work of K.M. is supported
by a World Premier International Research Center Initiative (WPI
Initiative), MEXT, Japan, and a Grant-in-aid for Scientific Research
(23740141). G.A. was supported by the Director, Office of Science,
Office of High Energy Physics, of the U.S. Department of Energy under
Contract No. DE-AC02-05CH11231. SNIFS on the UH 2.2 m telescope is part
of the Nearby Supernova Factory II project, a scientific collaboration
among the Centre de Recherche Astronomique de Lyon, Institut de Physique
Nucleaire de Lyon, Laboratoire de Physique Nucleaire et des Hautes
Energies, Lawrence Berkeley National Laboratory, Yale University,
University of Bonn, Max Planck Institute for Astrophysics, Tsinghua
Center for Astrophysics, and the Centre de Physique des Particules de
Marseille. This research has made use of the SIMBAD database and ALADIN,
operated at CDS, Strasbourg, France. This research has made use of the
NASA/IPAC Extragalactic Database (NED) which is operated by the Jet
Propulsion Laboratory, California Institute of Technology, under
contract with the National Aeronautics and Space Administration. This
research is based on observations obtained at the Gemini Observatory,
which is operated by the Association of Universities for Research in
Astronomy, Inc., under a cooperative agreement with the NSF on behalf of
the Gemini partnership: the National Science Foundation (United States),
the Science and Technology Facilities Council (United Kingdom), the
National Research Council (Canada), CONICYT (Chile), the Australian
Research Council (Australia), Ministerio da Ciencia, Tecnologia e
Inovacao (Brazil), and Ministerio de Ciencia, Tecnologia e Innovacion
Productiva (Argentina). The authors recognize and acknowledge the very
significant cultural role and reverence that the summit of Mauna Kea has
always had within the indigenous Hawaiian community. We are most
fortunate to have the opportunity to conduct observations from this
mountain.
NR 90
TC 20
Z9 20
U1 0
U2 4
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-6256
EI 1538-3881
J9 ASTRON J
JI Astron. J.
PD AUG
PY 2013
VL 146
IS 2
AR 30
DI 10.1088/0004-6256/146/2/30
PG 14
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 183TW
UT WOS:000321841100012
ER
PT J
AU Sesar, B
Ivezic, Z
Stuart, JS
Morgan, DM
Becker, AC
Sharma, S
Palaversa, L
Juric, M
Wozniak, P
Oluseyi, H
AF Sesar, Branimir
Ivezic, Zeljko
Stuart, J. Scott
Morgan, Dylan M.
Becker, Andrew C.
Sharma, Sanjib
Palaversa, Lovro
Juric, Mario
Wozniak, Przemyslaw
Oluseyi, Hakeem
TI EXPLORING THE VARIABLE SKY WITH LINEAR. II. HALO STRUCTURE AND
SUBSTRUCTURE TRACED BY RR LYRAE STARS TO 30 kpc
SO ASTRONOMICAL JOURNAL
LA English
DT Article
DE Galaxy: halo; Galaxy: stellar content; Galaxy: structure; stars:
variables: RR Lyrae
ID HORIZONTAL-BRANCH STARS; WAY STELLAR HALO; SURVEY STRIPE 82; MILKY-WAY;
GALACTIC HALO; GLOBULAR-CLUSTERS; PHOTOMETRIC SURVEY; GALAXY FORMATION;
VELOCITY GROUPS; PROPER MOTIONS
AB We present a sample of similar to 5000 RR Lyrae stars selected from the recalibrated LINEAR data set and detected at heliocentric distances between 5 kpc and 30 kpc over similar to 8000 deg(2) of sky. The coordinates and light curve properties, such as period and Oosterhoff type, are made publicly available. We analyze in detail the light curve properties and Galactic distribution of the subset of similar to 4000 type ab RR Lyrae (RRab) stars, including a search for new halo substructures and the number density distribution as a function of Oosterhoff type. We find evidence for the Oosterhoff dichotomy among field RR Lyrae stars, with the ratio of the type II and I subsamples of about 1:4, but with a weaker separation than for globular cluster stars. The wide sky coverage and depth of this sample allow unique constraints for the number density distribution of halo RRab stars as a function of galactocentric distance: it can be described as an oblate ellipsoid with an axis ratio q = 0.63 and with either a single or a double power law with a power-law index in the range -2 to -3. Consistent with previous studies, we find that the Oosterhoff type II subsample has a steeper number density profile than the Oosterhoff type I subsample. Using the group-finding algorithm EnLink, we detected seven candidate halo groups, only one of which is statistically spurious. Three of these groups are near globular clusters (M53/NGC 5053, M3, M13), and one is near a known halo substructure (Virgo Stellar Stream); the remaining three groups do not seem to be near any known halo substructures or globular clusters and seem to have a higher ratio of Oosterhoff type II to Oosterhoff type I RRab stars than what is found in the halo. The extended morphology and the position (outside the tidal radius) of some of the groups near globular clusters are suggestive of tidal streams possibly originating from globular clusters. Spectroscopic follow-up of detected halo groups is encouraged.
C1 [Sesar, Branimir] CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA.
[Ivezic, Zeljko; Morgan, Dylan M.; Becker, Andrew C.] Univ Washington, Dept Astron, Seattle, WA 98195 USA.
[Stuart, J. Scott] MIT, Lincoln Lab, Lexington, MA 02420 USA.
[Sharma, Sanjib] Univ Sydney, Sch Phys, Sydney Inst Astron, Sydney, NSW 2006, Australia.
[Palaversa, Lovro] Univ Geneva, Astron Observ, CH-1290 Sauverny, Switzerland.
[Juric, Mario] Univ Arizona, Steward Observ, Tucson, AZ 85121 USA.
[Juric, Mario] LSST Corp, Tucson, AZ 85721 USA.
[Wozniak, Przemyslaw] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Oluseyi, Hakeem] Florida Inst Technol, Melbourne, FL 32901 USA.
RP Sesar, B (reprint author), CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA.
OI Wozniak, Przemyslaw/0000-0002-9919-3310; Sharma,
Sanjib/0000-0002-0920-809X
FU NSF grant [AST-0908139, AST-0707901, AST-1008784, AST-0551161]; Croatian
National Science Foundation [O-1548-2009]; NASA ADP grant [NNX09AC77G];
National Aeronautics and Space Administration at MIT Lincoln Laboratory
under Air Force Contract [FA8721-05-C-0002]
FX B.S. is grateful for NSF grant AST-0908139 to Judith G. Cohen for
partial support. Z.I. acknowledges support by NSF grants AST-0707901 and
AST-1008784 to the University of Washington, by NSF grant AST-0551161 to
LSST for design and development activity, and by the Croatian National
Science Foundation grant O-1548-2009. A.C.B. acknowledges support from
NASA ADP grant NNX09AC77G. The LINEAR program is funded by the National
Aeronautics and Space Administration at MIT Lincoln Laboratory under Air
Force Contract FA8721-05-C-0002. Opinions, interpretations, conclusions,
and recommendations are those of the authors and are not necessarily
endorsed by the United States Government.
NR 67
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U1 0
U2 2
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-6256
J9 ASTRON J
JI Astron. J.
PD AUG
PY 2013
VL 146
IS 2
AR 21
DI 10.1088/0004-6256/146/2/21
PG 17
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 183TW
UT WOS:000321841100003
ER
PT J
AU Smee, SA
Gunn, JE
Uomoto, A
Roe, N
Schlegel, D
Rockosi, CM
Carr, MA
Leger, F
Dawson, KS
Olmstead, MD
Brinkmann, J
Owen, R
Barkhouser, RH
Honscheid, K
Harding, P
Long, D
Lupton, RH
Loomis, C
Anderson, L
Annis, J
Bernardi, M
Bhardwaj, V
Bizyaev, D
Bolton, AS
Brewington, H
Briggs, JW
Burles, S
Burns, JG
Castander, FJ
Connolly, A
Davenport, JRA
Ebelke, G
Epps, H
Feldman, PD
Friedman, SD
Frieman, J
Heckman, T
Hull, CL
Knapp, GR
Lawrence, DM
Loveday, J
Mannery, EJ
Malanushenko, E
Malanushenko, V
Merrelli, AJ
Muna, D
Newman, PR
Nichol, RC
Oravetz, D
Pan, K
Pope, AC
Ricketts, PG
Shelden, A
Sandford, D
Siegmund, W
Simmons, A
Smith, DS
Snedden, S
Schneider, DP
SubbaRao, M
Tremonti, C
Waddell, P
York, DG
AF Smee, Stephen A.
Gunn, James E.
Uomoto, Alan
Roe, Natalie
Schlegel, David
Rockosi, Constance M.
Carr, Michael A.
Leger, French
Dawson, Kyle S.
Olmstead, Matthew D.
Brinkmann, Jon
Owen, Russell
Barkhouser, Robert H.
Honscheid, Klaus
Harding, Paul
Long, Dan
Lupton, Robert H.
Loomis, Craig
Anderson, Lauren
Annis, James
Bernardi, Mariangela
Bhardwaj, Vaishali
Bizyaev, Dmitry
Bolton, Adam S.
Brewington, Howard
Briggs, John W.
Burles, Scott
Burns, James G.
Javier Castander, Francisco
Connolly, Andrew
Davenport, James R. A.
Ebelke, Garrett
Epps, Harland
Feldman, Paul D.
Friedman, Scott D.
Frieman, Joshua
Heckman, Timothy
Hull, Charles L.
Knapp, Gillian R.
Lawrence, David M.
Loveday, Jon
Mannery, Edward J.
Malanushenko, Elena
Malanushenko, Viktor
Merrelli, Aronne James
Muna, Demitri
Newman, Peter R.
Nichol, Robert C.
Oravetz, Daniel
Pan, Kaike
Pope, Adrian C.
Ricketts, Paul G.
Shelden, Alaina
Sandford, Dale
Siegmund, Walter
Simmons, Audrey
Smith, D. Shane
Snedden, Stephanie
Schneider, Donald P.
SubbaRao, Mark
Tremonti, Christy
Waddell, Patrick
York, Donald G.
TI THE MULTI-OBJECT, FIBER-FED SPECTROGRAPHS FOR THE SLOAN DIGITAL SKY
SURVEY AND THE BARYON OSCILLATION SPECTROSCOPIC SURVEY
SO ASTRONOMICAL JOURNAL
LA English
DT Article
DE cosmology: observations; instrumentation: spectrographs; surveys
ID 9TH DATA RELEASE; SDSS-III; ACOUSTIC-OSCILLATIONS; TARGET SELECTION;
GALAXY SAMPLE; TELESCOPE; CALIBRATION; SYSTEM; STARS; CCDS
AB We present the design and performance of the multi-object fiber spectrographs for the Sloan Digital Sky Survey (SDSS) and their upgrade for the Baryon Oscillation Spectroscopic Survey (BOSS). Originally commissioned in Fall 1999 on the 2.5 m aperture Sloan Telescope at Apache Point Observatory, the spectrographs produced more than 1.5 million spectra for the SDSS and SDSS-II surveys, enabling a wide variety of Galactic and extra-galactic science including the first observation of baryon acoustic oscillations in 2005. The spectrographs were upgraded in 2009 and are currently in use for BOSS, the flagship survey of the third-generation SDSS-III project. BOSS will measure redshifts of 1.35 million massive galaxies to redshift 0.7 and Ly alpha absorption of 160,000 high redshift quasars over 10,000 deg(2) of sky, making percent level measurements of the absolute cosmic distance scale of the universe and placing tight constraints on the equation of state of dark energy. The twin multi-object fiber spectrographs utilize a simple optical layout with reflective collimators, gratings, all-refractive cameras, and state-of-the-art CCD detectors to produce hundreds of spectra simultaneously in two channels over a bandpass covering the near-ultraviolet to the near-infrared, with a resolving power R = lambda/FWHM similar to 2000. Building on proven heritage, the spectrographs were upgraded for BOSS with volume-phase holographic gratings and modern CCD detectors, improving the peak throughput by nearly a factor of two, extending the bandpass to cover 360 nm < lambda < 1000 nm, and increasing the number of fibers from 640 to 1000 per exposure. In this paper we describe the original SDSS spectrograph design and the upgrades implemented for BOSS, and document the predicted and measured performances.
C1 [Smee, Stephen A.; Barkhouser, Robert H.; Feldman, Paul D.; Heckman, Timothy] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA.
[Gunn, James E.; Carr, Michael A.; Lupton, Robert H.; Loomis, Craig; Knapp, Gillian R.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA.
[Uomoto, Alan; Hull, Charles L.] Observ Carnegie Inst Washington, Pasadena, CA 91101 USA.
[Roe, Natalie; Schlegel, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA.
[Rockosi, Constance M.; Epps, Harland; Sandford, Dale] Univ Calif Santa Cruz, UC Observ, Santa Cruz, CA 95064 USA.
[Rockosi, Constance M.; Epps, Harland; Sandford, Dale] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA.
[Leger, French; Owen, Russell; Anderson, Lauren; Bhardwaj, Vaishali; Connolly, Andrew; Davenport, James R. A.; Mannery, Edward J.; Siegmund, Walter] Univ Washington, Dept Astron, Seattle, WA 09195 USA.
[Dawson, Kyle S.; Olmstead, Matthew D.; Bolton, Adam S.; Lawrence, David M.; Ricketts, Paul G.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA.
[Brinkmann, Jon; Long, Dan; Bizyaev, Dmitry; Brewington, Howard; Ebelke, Garrett; Malanushenko, Elena; Malanushenko, Viktor; Newman, Peter R.; Oravetz, Daniel; Pan, Kaike; Shelden, Alaina; Simmons, Audrey; Snedden, Stephanie] Apache Point Observ, Sunspot, NM 88349 USA.
[Honscheid, Klaus; Burns, James G.; Smith, D. Shane] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA.
[Honscheid, Klaus; Burns, James G.; Smith, D. Shane] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA.
[Harding, Paul] Case Western Reserve Univ, Dept Astron, Cleveland, OH 44106 USA.
[Annis, James; Frieman, Joshua] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Bernardi, Mariangela; SubbaRao, Mark] Univ Penn, Dept Astron & Astrophys, Philadelphia, PA 19104 USA.
[Briggs, John W.] Mittelman Family Fdn, HUT Observ, Eagle, CO 81631 USA.
[Burles, Scott] MIT, Dept Phys, Cambridge, MA 02139 USA.
[Javier Castander, Francisco] Inst Ciencies Espai IEEC CSIC, E-08193 Barcelona, Spain.
[Javier Castander, Francisco; Friedman, Scott D.] Space Telescope Sci Inst, Baltimore, MD 21218 USA.
[Loveday, Jon] Univ Sussex, Ctr Astron, Brighton BN1 9QJ, E Sussex, England.
[Merrelli, Aronne James] CALTECH, Dept Astron, Pasadena, CA 91125 USA.
[Muna, Demitri] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA.
[Nichol, Robert C.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England.
[Pope, Adrian C.] Argonne Natl Lab, Div High Energy Phys, Lemont, IL 60439 USA.
[Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA.
[Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA.
[Tremonti, Christy] Univ Wisconsin, Dept Astron, Madison, WI 53703 USA.
[Waddell, Patrick] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA.
[York, Donald G.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA.
[York, Donald G.] Univ Chicago, Fermi Inst, Chicago, IL 60637 USA.
RP Smee, SA (reprint author), Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA.
EM smee@pha.jhu.edu
OI Davenport, James/0000-0002-0637-835X
FU Alfred P. Sloan Foundation; National Science Foundation; U.S. Department
of Energy Office of Science
FX Funding for SDSS-III has been provided by the Alfred P. Sloan
Foundation, the Participating Institutions, the National Science
Foundation, and the U.S. Department of Energy Office of Science. The
SDSS-III Web site is http://www.sdss3.org/.; SDSS-III is managed by the
Astrophysical Research Consortium for the Participating Institutions of
the SDSS-III Collaboration including the University of Arizona, the
Brazilian Participation Group, Brookhaven National Laboratory,
University of Cambridge, Carnegie Mellon University, University of
Florida, the French Participation Group, the German Participation Group,
Harvard University, the Instituto de Astrofisica de Canarias, the
Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins
University, Lawrence Berkeley National Laboratory, Max Planck Institute
for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New
Mexico State University, New York University, Ohio State University,
Pennsylvania State University, University of Portsmouth, Princeton
University, the Spanish Participation Group, University of Tokyo,
University of Utah, Vanderbilt University, University of Virginia,
University of Washington, and Yale University.
NR 49
TC 223
Z9 223
U1 1
U2 17
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-6256
J9 ASTRON J
JI Astron. J.
PD AUG
PY 2013
VL 146
IS 2
AR 32
DI 10.1088/0004-6256/146/2/32
PG 40
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 183TW
UT WOS:000321841100014
ER
PT J
AU Engel, K
Sasaki, T
Wang, Q
Kuriyan, J
AF Engel, Kate
Sasaki, Tomoaki
Wang, Qi
Kuriyan, John
TI A highly efficient peptide substrate for EGFR activates the kinase by
inducing aggregation
SO BIOCHEMICAL JOURNAL
LA English
DT Article
DE activation; aggregation; dimer; epidermal growth factor receptor (EGFR);
fibril; kinetics
ID GROWTH-FACTOR RECEPTOR; PROTEIN-TYROSINE KINASE; KINETIC-PROPERTIES;
BINDING AFFINITY; MECHANISM; DIMERIZATION; INHIBITOR; DOMAIN;
AUTOPHOSPHORYLATION; PHOSPHORYLATION
AB Formation of an asymmetric dimer by the EGFR (epidermal growth factor receptor) kinase domains results in allosteric activation. Since this dimer does not readily form in solution, the EGFR kinase domain phosphorylates most peptide substrates with a relatively low catalytic efficiency. Peptide C is a synthetic peptide substrate of EGFR developed by others that is phosphorylated with a significantly higher catalytic efficiency, and we sought to understand the basis for this. Peptide C was found to increase EGFR kinase activity by promoting formation of the EGFR kinase domain asymmetric dimer. Activation of the kinase domain by Peptide C also enhances phosphorylation of other substrates. Aggregation of the EGFR kinase domain by Peptide C probably underlies activation, and Peptide C precipitates several other proteins. Peptide C was found to form fibrils independent of the presence of EGFR, and these fibrils may facilitate aggregation and activation of the kinase domain. These results establish that a peptide substrate of EGFR may increase catalytic activity by promoting kinase domain dimerization by an aggregation-mediated mechanism.
C1 [Engel, Kate; Sasaki, Tomoaki; Wang, Qi; Kuriyan, John] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA.
[Engel, Kate; Sasaki, Tomoaki; Wang, Qi; Kuriyan, John] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA.
[Kuriyan, John] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Kuriyan, John] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.
[Kuriyan, John] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
RP Kuriyan, J (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.
EM kuriyan@berkeley.edu
FU Howard Hughes Medical Institute; National Cancer Institute
[2-R01-CA096504-06]; Susan G. Komen for the Cure [KG081684]
FX This work was funded by institutional funds from the Howard Hughes
Medical Institute, the National Cancer Institute [grant number
2-R01-CA096504-06] and Susan G. Komen for the Cure [grant number
KG081684].
NR 28
TC 2
Z9 2
U1 0
U2 8
PU PORTLAND PRESS LTD
PI LONDON
PA THIRD FLOOR, EAGLE HOUSE, 16 PROCTER STREET, LONDON WC1V 6 NX, ENGLAND
SN 0264-6021
EI 1470-8728
J9 BIOCHEM J
JI Biochem. J.
PD AUG 1
PY 2013
VL 453
BP 337
EP 344
DI 10.1042/BJ20130537
PN 3
PG 8
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 190RU
UT WOS:000322358700003
PM 23734957
ER
PT J
AU Muckerman, JT
Skone, JH
Ning, M
Wasada-Tsutsui, Y
AF Muckerman, James T.
Skone, Jonathan H.
Ning, Ming
Wasada-Tsutsui, Yuko
TI Toward the accurate calculation of pK(a) values in water and
acetonitrile
SO BIOCHIMICA ET BIOPHYSICA ACTA-BIOENERGETICS
LA English
DT Article
DE pK(a) value; Solvation model; Acidity
ID GAS-PHASE ACIDITIES; DENSITY-FUNCTIONAL THEORY; SOLVATION FREE-ENERGIES;
PRINCIPLES-BASED METHOD; AB-INITIO CALCULATIONS; PROTON AFFINITIES;
ORGANIC-ACIDS; DISSOCIATION-CONSTANTS; DIMETHYL-SULFOXIDE;
CARBOXYLIC-ACIDS
AB We present a simple approach for the calculation of accurate pK(a) values in water and acetonitrile based on the straightforward calculation of the gas-phase absolute free energies of the acid and conjugate base with use of only a continuum solvation model to obtain the corresponding solution-phase free energies. Most of the error in such an approach arises from inaccurate differential solvation free energies of the acid and conjugate base which is removed in our approach using a correction based on the realization that the gas-phase acidities have only a small systematic error relative to the dominant systematic error in the differential solvation. The methodology is outlined in the context of the calculation of a set of neutral acids with water as the solvent for a reasonably accurate electronic structure level of theory (DFT), basis set, and implicit solvation model. It is then applied to the comparison of results for three different hybrid density functionals to illustrate the insensitivity to the functional. Finally, the approach is applied to the comparison of results for sets of neutral acids and protonated amine cationic acids in both aqueous (water) and nonaqueous (acetonitrile) solvents. The methodology is shown to generally predict the pK(a) values for all the cases investigated to within I pH unit so long as the differential solvation error is larger than the systematic error in the gas-phase acidity calculations. Such an approach is rather general and does not have additional complications that would arise in a cluster-continuum method, thus giving it strength as a simple high-throughput means to calculate absolute pK(a) values. This article is part of a Special Issue entitled: Metals in Bioenergetics and Biomimetics Systems. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Muckerman, James T.; Skone, Jonathan H.; Ning, Ming] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Wasada-Tsutsui, Yuko] Nagoya Inst Technol, Grad Sch Engn, Showa Ku, Nagoya, Aichi 4668555, Japan.
RP Muckerman, JT (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM muckerma@bnl.gov
NR 68
TC 18
Z9 18
U1 2
U2 63
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0005-2728
J9 BBA-BIOENERGETICS
JI Biochim. Biophys. Acta-Bioenerg.
PD AUG-SEP
PY 2013
VL 1827
IS 8-9
SI SI
BP 882
EP 891
DI 10.1016/j.bbabio.2013.03.011
PG 10
WC Biochemistry & Molecular Biology; Biophysics
SC Biochemistry & Molecular Biology; Biophysics
GA 191LK
UT WOS:000322414300003
PM 23567870
ER
PT J
AU King, PW
AF King, Paul W.
TI Designing interfaces of hydrogenase-nanomaterial hybrids for efficient
solar conversion
SO BIOCHIMICA ET BIOPHYSICA ACTA-BIOENERGETICS
LA English
DT Review
DE Interface; Electron-transfer; Nanoparticle; Photocatalysis; Enzyme
biohybrid; Solar conversion
ID DIRECT ELECTRON-TRANSFER; PHOTOELECTROCHEMICAL BIOFUEL CELL;
SEMICONDUCTOR QUANTUM DOTS; WALL CARBON NANOTUBES; PHOTOSYSTEM-I;
CLOSTRIDIUM-PASTEURIANUM; CHARGE-TRANSFER; H-2 PRODUCTION;
CHLAMYDOMONAS-REINHARDTII; PHOTOSYNTHETIC ORGANISMS
AB The direct conversion of sunlight into biofuels is an intriguing alternative to a continued reliance on fossil fuels. Natural photosynthesis has long been investigated both as a potential solution, and as a model for utilizing solar energy to drive a water-to-fuel cycle. The molecules and organizational structure provide a template to inspire the design of efficient molecular systems for photocatalysis. A clear design strategy is the coordination of molecular interactions that match kinetic rates and energetic levels to control the direction and flow of energy from light harvesting to catalysis. Energy transduction and electron-transfer reactions occur through interfaces formed between complexes of donor-acceptor molecules. Although the structures of several of the key biological complexes have been solved, detailed descriptions of many electron-transfer complexes are lacking, which presents a challenge to designing and engineering biomolecular systems for solar conversion. Alternatively, it is possible to couple the catalytic power of biological enzymes to light harvesting by semiconductor nanomaterials. In these molecules, surface chemistry and structure can be designed using ligands. The passivation effect of the ligand can also dramatically affect the photophysical properties of the semiconductor, and energetics of external charge-transfer. The length, degree of bond saturation (aromaticity), and solvent exposed functional groups of ligands can be manipulated to further tune the interface to control molecular assembly, and complex stability in photocatalytic hybrids. The results of this research show how ligand selection is critical to designing molecular interfaces that promote efficient self-assembly, charge-transfer and photocatalysis. This article is part of a Special Issue entitled: Metals in Bioenergetics and Biomimetics Systems. (C) 2013 Elsevier B.V. All rights reserved.
C1 Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA.
RP King, PW (reprint author), Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA.
EM paul.king@nrel.gov
RI King, Paul/D-9979-2011
OI King, Paul/0000-0001-5039-654X
FU U.S. Department of Energy, Division of Chemical Sciences, Geosciences,
and Biosciences, Office of Basic Energy Sciences; U.S. Department of
Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory
FX I would like to thank Dr. Katherine A. Brown (NREL), Prof. Gordana
Dukovic (CU-Boulder), Dr. Maria L Ghirardi (NREL), Dr. David W. Mulder
(NREL), Michael W. Ratzloff (NREL) and Dr. Qing Song (IBM) for insights
and helpful discussions in preparation of this manuscript, and to Drs.
Brown and Song for the use of preliminary data shown in Fig. 5.1 am
grateful for funding support from the U.S. Department of Energy,
Division of Chemical Sciences, Geosciences, and Biosciences, Office of
Basic Energy Sciences; and for support by the U.S. Department of Energy
under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy
Laboratory.
NR 115
TC 30
Z9 30
U1 10
U2 176
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0005-2728
J9 BBA-BIOENERGETICS
JI Biochim. Biophys. Acta-Bioenerg.
PD AUG-SEP
PY 2013
VL 1827
IS 8-9
SI SI
BP 949
EP 957
DI 10.1016/j.bbabio.2013.03.006
PG 9
WC Biochemistry & Molecular Biology; Biophysics
SC Biochemistry & Molecular Biology; Biophysics
GA 191LK
UT WOS:000322414300008
PM 23541891
ER
PT J
AU Fujita, E
Muckerman, JT
Himeda, Y
AF Fujita, Etsuko
Muckerman, James T.
Himeda, Yuichiro
TI Interconversion of CO2 and formic acid by bio-inspired Ir complexes with
pendent bases
SO BIOCHIMICA ET BIOPHYSICA ACTA-BIOENERGETICS
LA English
DT Review
DE CO2 hydrogenation; Formic acid; Dehydrogenation; Ir complexes; H-2
storage; Bio-inspired catalysts
ID SUPERCRITICAL CARBON-DIOXIDE; AQUEOUS HYDROGEN CARBONATE; HALF-SANDWICH
COMPLEXES; FE-ONLY HYDROGENASE; HOMOGENEOUS HYDROGENATION;
CATALYTIC-HYDROGENATION; MILD CONDITIONS; RUTHENIUM CATALYSTS;
AMBIENT-TEMPERATURE; WATER SOLUBILITY
AB Recent investigations of the interconversion of CO2 and formic acid using Ru, Ir and Fe complexes are summarized in this review. During the past several years, both the reaction rates and catalyst stabilities have been significantly improved. Remarkably, the interconversion (i.e., reversibility) has also been achieved under mild conditions in environmentally benign water solvent by slightly changing the pH of the aqueous solution. Only a few catalysts seem to reflect a bin-inspired design such as the use of proton responsive ligands, ligands with pendent bases or acids for a second-coordination-sphere interaction, electroresponsive ligands, and/or ligands having a hydrogen bonding function with a solvent molecule or an added reagent. The most successful of these is an iridium dinuclear complex catalyst that at least has the first three of these characteristics associated with its bridging ligand. By utilizing an acid/base equilibrium for proton removal, the ligand becomes a strong electron donor, resulting in Ir(I) character with a vacant coordination site at each metal center in slightly basic solution. Complemented by DFT calculations, kinetic studies of the rates of formate production using a related family of Ir complexes with and without such functions on the ligand reveal that the rate-determining step for the CO2 hydrogenation is likely to be H-2 addition through heterolytic cleavage involving a "proton relay" through the pendent base. The dehydrogenation of formic acid, owing to the proton responsive ligands changing character under slightly acidic pH conditions, is likely to occur by a mechanism with a different rate-determining step. This article is part of a Special Issue entitled: Metals in Bioenergetics and Biomimetics Systems. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Fujita, Etsuko; Muckerman, James T.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Himeda, Yuichiro] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058565, Japan.
RP Fujita, E (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM fujita@bnl.gov
RI Himeda, Yuichiro/E-8613-2014
FU U.S. Department of Energy [DE-AC02-98CH10886]; Division of Chemical
Sciences, Geosciences, & Biosciences, Office of Basic Energy Sciences;
Japanese Ministry of Economy, Trade, and Industry
FX The work at BNL was carried out under contract DE-AC02-98CH10886 with
the U.S. Department of Energy and supported by its Division of Chemical
Sciences, Geosciences, & Biosciences, Office of Basic Energy Sciences.
YH thanks the Japanese Ministry of Economy, Trade, and Industry for
financial support.
NR 62
TC 45
Z9 46
U1 6
U2 157
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0005-2728
J9 BBA-BIOENERGETICS
JI Biochim. Biophys. Acta-Bioenerg.
PD AUG-SEP
PY 2013
VL 1827
IS 8-9
SI SI
BP 1031
EP 1038
DI 10.1016/j.bbabio.2012.11.004
PG 8
WC Biochemistry & Molecular Biology; Biophysics
SC Biochemistry & Molecular Biology; Biophysics
GA 191LK
UT WOS:000322414300014
PM 23174332
ER
PT J
AU Shaw, WJ
Helm, ML
DuBois, DL
AF Shaw, Wendy J.
Helm, Monte L.
DuBois, Daniel L.
TI A modular, energy-based approach to the development of nickel containing
molecular electrocatalysts for hydrogen production and oxidation
SO BIOCHIMICA ET BIOPHYSICA ACTA-BIOENERGETICS
LA English
DT Review
DE Hydrogen; Electrochemistry; Hydrogenase mimic; Homogeneous catalysis;
Proton transport
ID OUTER-COORDINATION SPHERE; FE-ONLY HYDROGENASE; H-2 PRODUCTION;
ACTIVE-SITE; IRON HYDROGENASE; PROTON RELAYS;
DESULFOVIBRIO-DESULFURICANS; LOW OVERPOTENTIALS; OXYGEN REDUCTION;
PENDANT AMINES
AB This review discusses the development of molecular electrocatalysts for H-2 production and oxidation based on nickel. A modular approach is used in which the structure of the catalyst is divided into first, second, and outer coordination spheres. The first coordination sphere consists of the ligands bound directly to the metal center, and this coordination sphere can be used to control such factors as the presence or absence of vacant coordination sites, redox potentials, hydride donor abilities and other important thermodynamic parameters. The second coordination sphere includes functional groups such as pendent acids or bases that can interact with bound substrates such as H-2 molecules and hydride ligands, but that do not form strong bonds with the metal center. These functional groups can play diverse roles such as assisting the heterolytic cleavage of H-2, controlling intra-and intermolecular proton transfer reactions, and providing a physical pathway for coupling proton and electron transfer reactions. By controlling both the hydride donor ability of the catalysts using the first coordination sphere and the proton donor abilities of the functional groups in the second coordination sphere, catalysts can be designed that are biased toward H-2 production, oxidation, or bidirectional (catalyzing both H-2 oxidation and production). The outer coordination sphere is defined as that portion of the catalytic system that is beyond the second coordination sphere. This coordination sphere can assist in the delivery of protons and electrons to and from the catalytically active site, thereby adding another important avenue for controlling catalytic activity. Many features of these simple catalytic systems are good models for enzymes, and these simple systems provide insights into enzyme function and reactivity that may be difficult to probe in enzymes. This article is part of a Special Issue entitled: Metals in Bioenergetics and Biomimetics Systems. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Shaw, Wendy J.; Helm, Monte L.; DuBois, Daniel L.] Pacific NW Natl Lab, Div Phys Sci, POB 999,K2-57, Richland, WA 99352 USA.
RP Helm, ML (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,K2-57, Richland, WA 99352 USA.
EM monte.helm@pnnl.gov
FU Center for Molecular Electrocatalysis, an Energy Frontier Research
Center; US Department of Energy, Office of Science, Office of Basic
Energy Sciences.; DOE Office of Science Early Career Research Program
through the Office of Basic Energy Sciences
FX MLH and DLD acknowledge the support of the Center for Molecular
Electrocatalysis, an Energy Frontier Research Center funded by the US
Department of Energy, Office of Science, Office of Basic Energy
Sciences. WJS acknowledges the support of the DOE Office of Science
Early Career Research Program through the Office of Basic Energy
Sciences. Pacific Northwest National Laboratory is operated by Battelle
for the U.S. Department of Energy.
NR 71
TC 48
Z9 48
U1 3
U2 62
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0005-2728
EI 0006-3002
J9 BBA-BIOENERGETICS
JI Biochim. Biophys. Acta-Bioenerg.
PD AUG-SEP
PY 2013
VL 1827
IS 8-9
SI SI
BP 1123
EP 1139
DI 10.1016/j.bbabio.2013.01.003
PG 17
WC Biochemistry & Molecular Biology; Biophysics
SC Biochemistry & Molecular Biology; Biophysics
GA 191LK
UT WOS:000322414300020
PM 23313415
ER
PT J
AU Kwon, HY
Mueller, S
Dunn, JB
Wander, MM
AF Kwon, Ho-Young
Mueller, Steffen
Dunn, Jennifer B.
Wander, Michelle M.
TI Modeling state-level soil carbon emission factors under various
scenarios for direct land use change associated with United States
biofuel feedstock production
SO BIOMASS & BIOENERGY
LA English
DT Article
DE Soil C emissions factors; Direct land use change; United States biofuel
feedstock production; Process-based modeling; Surrogate CENTURY soil
organic C model
ID MISCANTHUS X GIGANTEUS; ORGANIC-MATTER; LONG-TERM; CHEMICAL-COMPOSITION;
GREAT-PLAINS; CROP; NITROGEN; BIOMASS; DYNAMICS; TILLAGE
AB Current estimates of life cycle greenhouse gas emissions of biofuels produced in the US can be improved by refining soil C emission factors (EF; C emissions per land area per year) for direct land use change associated with different biofuel feedstock scenarios. We developed a modeling framework to estimate these EFs at the state-level by utilizing remote sensing data, national statistics databases, and a surrogate model for CENTURY's soil organic C dynamics submodel (SCSOC). We estimated the forward change in soil C concentration within the 0-30 cm depth and computed the associated EFs for the 2011 to 2040 period for croplands, grasslands or pasture/hay, croplands/conservation reserve, and forests that were suited to produce any of four possible biofuel feedstock systems [corn (Zea Mays L)-corn, corn-corn with stover harvest, switchgrass (Panicum virgatum L), and miscanthus (Miscanthus x giganteus Greef et Deuter)]. Our results predict smaller losses or even modest gains in sequestration for corn based systems, particularly on existing croplands, than previous efforts and support assertions that production of perennial grasses will lead to negative emissions in most situations and that conversion of forest or established grasslands to biofuel production would likely produce net emissions. The proposed framework and use of the SCSOC provide transparency and relative simplicity that permit users to easily modify model inputs to inform biofuel feedstock production targets set forth by policy. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Kwon, Ho-Young; Wander, Michelle M.] Univ Illinois, Dept Nat Resources & Environm Sci, Urbana, IL 61801 USA.
[Mueller, Steffen] Univ Illinois, Energy Resources Ctr, Chicago, IL 60607 USA.
[Dunn, Jennifer B.] Argonne Natl Lab, Ctr Transportat Res, Argonne, IL 60439 USA.
RP Kwon, HY (reprint author), Univ Illinois, Dept Nat Resources & Environm Sci, W-503 Turner Hall,MC 047,1102 South Goodwin Ave, Urbana, IL 61801 USA.
EM hkwon2@illinois.edu; muellers@uic.edu; jdunn@anl.gov;
mwander@illinois.edu
FU Biomass Program of the Office of Energy Efficiency and Renewable Energy
of the United States Department of Energy [DE-AC02-06CH11357]
FX This work was supported by the Biomass Program of the Office of Energy
Efficiency and Renewable Energy of the United States Department of
Energy, under contract DE-AC02-06CH11357. The authors are very grateful
to Dr. Michael Q. Wang of Argonne National Laboratory for helpful
discussions.
NR 63
TC 18
Z9 18
U1 1
U2 55
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0961-9534
J9 BIOMASS BIOENERG
JI Biomass Bioenerg.
PD AUG
PY 2013
VL 55
BP 299
EP 310
DI 10.1016/j.biombioe.2013.02.021
PG 12
WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy &
Fuels
SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels
GA 180LE
UT WOS:000321595900032
ER
PT J
AU Shao, QJ
Cheng, C
Ong, RG
Zhu, L
Zhao, C
AF Shao, Qianjun
Cheng, Cheng
Ong, Rebecca G.
Zhu, Li
Zhao, Chao
TI Hydrogen peroxide presoaking of bamboo prior to AFEX pretreatment and
impact on enzymatic conversion to fermentable sugars
SO BIORESOURCE TECHNOLOGY
LA English
DT Article
DE Bamboo; Pretreatment; Enzymatic hydrolysis; Hydrogen peroxide; AFEX
ID FIBER EXPANSION AFEX; DEGRADATION-PRODUCTS; CORN STOVER; BIOMASS;
AMMONIA; HYDROLYSIS; OPTIMIZATION; SWITCHGRASS; CELLULOSE; BIOFUELS
AB Bamboo is a fast growing plant found worldwide that has high potential as an energy crop. This project evaluated the effectiveness of AFEX pretreatment for converting moso bamboo (Phyllostachys heterocycla var. pubescens) to fermentable sugars, both with and without pre-soaking in hydrogen peroxide. Pretreatment conditions including temperature, water loading, residence time, ammonia loading, and hydrogen peroxide loadings were varied to maximize hydrolysis yields. The optimal conditions for AFEX were 150 degrees C, 0.8 or 2.0 (w/w) water loading, 10-30 min residence time, and 2.0-5.0 (w/w) ammonia loading. The optimal conditions for H-AFEX were same AFEX conditions with 0.7-1.9 (w/w) 30% (wt) hydrogen peroxide solutions loading. Using 15 FPU/g glucan cellulase and under optimal conditions, AFEX pretreatment achieved a theoretical sugars yield of 64.8-72.7% and addition of hydrogen peroxide presoaking increased the yield to 83.4-92.1%. It is about 5-fold and 7-fold increase in sugars yield for AFEX-treated and H-AFEX-treated bamboo respectively. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Shao, Qianjun; Cheng, Cheng; Zhu, Li; Zhao, Chao] Zhejiang A&F Univ, Sch Engn, Linan 311300, Zhejiang, Peoples R China.
[Shao, Qianjun] Georgia Inst Technol, Sch Chem & Biochem, Inst Paper Sci & Technol, BioEnergy Sci Ctr, Atlanta, GA 30332 USA.
[Ong, Rebecca G.] Michigan State Univ, Dept Chem Engn & Mat Sci, Biomass Convers Res Lab, Lansing, MI 48910 USA.
[Ong, Rebecca G.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA.
RP Shao, QJ (reprint author), Zhejiang A&F Univ, Sch Engn, Linan 311300, Zhejiang, Peoples R China.
EM shawqj@gmail.com
OI Shao, Qianjun/0000-0002-7101-6654; Ong, Rebecca/0000-0001-5020-646X
FU National Natural Science Foundation of China [30871991]; Innovative
Research Team of Zhejiang Province [2009R50012]; Research Foundation of
Education Bureau of Zhejiang Province [Z201017451]
FX This research was supported by funds from National Natural Science
Foundation of China (No. 30871991), Innovative Research Team of Zhejiang
Province (No. 2009R50012), and Research Foundation of Education Bureau
of Zhejiang Province (No. Z201017451).
NR 34
TC 12
Z9 16
U1 2
U2 50
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0960-8524
J9 BIORESOURCE TECHNOL
JI Bioresour. Technol.
PD AUG
PY 2013
VL 142
BP 26
EP 31
DI 10.1016/j.biortech.2013.05.011
PG 6
WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy &
Fuels
SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels
GA 189UC
UT WOS:000322292800004
PM 23732919
ER
PT J
AU Merkulov, IA
Yoon, M
Geohegan, DB
AF Merkulov, I. A.
Yoon, Mina
Geohegan, David B.
TI How the shape of catalyst nanoparticles determines their
crystallographic orientation during carbon nanofiber growth
SO CARBON
LA English
DT Article
ID FCC METALS
AB A theoretical model is presented that explains spontaneous changes in the crystalline orientation of nanoparticles. The spontaneous changes in crystalline orientation are attributed to the crystal anisotropy of the surface energy of nanocrystalline particles. We consider an important specific case of the chemical vapor deposition growth of carbon nanofibers, where previous studies have shown that both the catalyst nanoparticle shape and the nanofiber growth rate change with changes in the chemical potential of diluted carbon. Energetic considerations of the nanoparticle's free surface and its interfacial energy with the nanofiber during these shape changes are shown to force a reorientation of the nanoparticle crystallographic axes at a critical growth rate. The model therefore reveals the mechanism by which the shape and crystallographic orientation of the catalyst nanoparticle are linked to the nanofiber growth rate. The model suggests a new way, based upon measurable geometry of nanoparticles during in situ growth experiments, to estimate the role of chemisorption in the attraction of the graphene film to the curved catalyst surface and the anisotropy energy of this interface. Published by Elsevier Ltd.
C1 [Merkulov, I. A.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.
[Merkulov, I. A.; Yoon, Mina; Geohegan, David B.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Merkulov, I. A.] RAS, AF Ioffe Physicotech Inst, St Petersburg 19021, Russia.
RP Yoon, M (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM myoon@ornl.gov
RI Yoon, Mina/A-1965-2016; Geohegan, David/D-3599-2013
OI Yoon, Mina/0000-0002-1317-3301; Geohegan, David/0000-0003-0273-3139
FU Materials Sciences and Engineering Division, Office of Basic Energy
Sciences, U.S. Department of Energy; Scientific User Facilities
Division, Office of Basic Energy Sciences, U.S. Department of Energy;
theme research at the Center for Nanophase Materials Sciences
FX We would like to thank A.V. Melechko for fruitful discussions. Synthesis
science (M.Y., D.G.) supported by the Materials Sciences and Engineering
Division, Office of Basic Energy Sciences, U.S. Department of Energy.
General theory of nanoparticle energetics (I.M., M.Y.) supported by
theme research at the Center for Nanophase Materials Sciences, which is
sponsored at Oak Ridge National Laboratory by the Scientific User
Facilities Division, Office of Basic Energy Sciences, U.S. Department of
Energy.
NR 19
TC 5
Z9 5
U1 0
U2 22
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD AUG
PY 2013
VL 60
BP 41
EP 45
DI 10.1016/j.carbon.2013.03.054
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 180MB
UT WOS:000321598200005
ER
PT J
AU Sharma, P
Mayes, MA
Tang, GP
AF Sharma, Prasesh
Mayes, Melanie A.
Tang, Guoping
TI Role of soil organic carbon and colloids in sorption and transport of
TNT, RDX and HMX in training range soils
SO CHEMOSPHERE
LA English
DT Article
DE Explosives; Colloids; Organic carbon; Operational training range; Column
experiments
ID ADSORPTION; 2,4,6-TRINITROTOLUENE; EXPLOSIVES; BINDING; MATTER; WATER;
CLAY; DEGRADATION; METABOLITES; SUBSURFACE
AB Contamination of soils and groundwater by munitions compounds (MCs) is of significant concern at many U.S. Department of Defense sites. Soils were collected from operational training ranges in Maryland (APG), Massachusetts (MMR-B and MMR-E) and Washington (JBLM) and sorption and transport studies were conducted to investigate the effects of soil organic carbon (OC) and textural clay content on fate of dissolved MCs (TNT, RDX, HMX). Sorption experiments showed higher distribution coefficients [TNT:42-68 L kg(-1), RDX:6.9-8.7 L kg(-1) and HMX:2.6-3.1 L kg(-1)] in OC rich soils (JBLM, MMR-E) compared to clay rich soils (MMR-B and APG) [TNT:19-21 L kg(-1), RDX:2.5-3.4 L kg(-1), HMX:0.9-1.2 L kg(-1)]. In column experiments, breakthrough of MCs was faster in MMR-B and APG compared to MMR-E and JBLM soils. Among TNT, RDX and HMX, breakthrough was fastest for RDX followed by HMX and TNT for all columns. Defining the colloidal fraction as the difference between unfiltered samples and samples filtered with a 3 kDa filter, similar to 36%, similar to 15% and similar to 9% of TNT, RDX and HMX were found in the colloidal fraction in the solutions from sorption experiments, and around 20% of TNT in the effluent from the transport experiments. Results demonstrate that OC rich soils may enhance sorption and delay transport of TNT, RDX and HMX compared to clay-rich soils. Further, transport of TNT may be associated with soil colloid mobilization. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Sharma, Prasesh; Mayes, Melanie A.; Tang, Guoping] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA.
RP Tang, GP (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Bethel Valley Rd,MS-6038, Oak Ridge, TN 37831 USA.
EM mayesma@ornal.org
RI Tang, Guoping/A-5141-2010
OI Tang, Guoping/0000-0003-1090-3564
FU Strategic Environmental Research and Development Program (SERDP)
[ER-1690]; University of Tennessee-Battelle, LLC [DE-AC05-00OR22725];
U.S. DOE
FX This work was supported by the Strategic Environmental Research and
Development Program (SERDP) Project ER-1690 to MAM. We would like to
thank Wei Wang, Balaji Rao, Jana Phillips, Tonia Melhorn, Sindhu
Jagadamma from ORNL, Matthew Jones (University of Tennessee and ORNL)
for their help with analysis and/or suggestions for improving the
manuscript. Oak Ridge National Laboratory is managed by the University
of Tennessee-Battelle, LLC, under Contract DE-AC05-00OR22725 with the
U.S. DOE.
NR 42
TC 4
Z9 5
U1 6
U2 51
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0045-6535
J9 CHEMOSPHERE
JI Chemosphere
PD AUG
PY 2013
VL 92
IS 8
BP 993
EP 1000
DI 10.1016/j.chemosphere.2013.03.028
PG 8
WC Environmental Sciences
SC Environmental Sciences & Ecology
GA 191QU
UT WOS:000322428500017
PM 23602657
ER
PT J
AU Chen, MJ
Sun, YW
Fu, PC
Carrigan, CR
Lu, ZM
Tong, CH
Buscheck, TA
AF Chen, Mingjie
Sun, Yunwei
Fu, Pengcheng
Carrigan, Charles R.
Lu, Zhiming
Tong, Charles H.
Buscheck, Thomas A.
TI Surrogate-based optimization of hydraulic fracturing in pre-existing
fracture networks
SO COMPUTERS & GEOSCIENCES
LA English
DT Article
DE Hydraulic fracturing; Fractal dimension; Surrogate model; Optimization;
Global sensitivity
ID REGRESSION; SYSTEMS; DESIGN; CONNECTIVITY; ENSEMBLE
AB Hydraulic fracturing has been used widely to stimulate production of oil, natural gas, and geothermal energy in formations with low natural permeability. Numerical optimization of fracture stimulation often requires a large number of evaluations of objective functions and constraints from forward hydraulic fracturing models, which are computationally expensive and even prohibitive in some situations. Moreover, there are a variety of uncertainties associated with the pre-existing fracture distributions and rock mechanical properties, which affect the optimized decisions for hydraulic fracturing. In this study, a surrogate-based approach is developed for efficient optimization of hydraulic fracturing well design in the presence of natural-system uncertainties. The fractal dimension is derived from the simulated fracturing network as the objective for maximizing energy recovery sweep efficiency. The surrogate model, which is constructed using training data from high-fidelity fracturing models for mapping the relationship between uncertain input parameters and the fractal dimension, provides fast approximation of the objective functions and constraints. A suite of surrogate models constructed using different fitting methods is evaluated and validated for fast predictions. Global sensitivity analysis is conducted to gain insights into the impact of the input variables on the output of interest, and further used for parameter screening. The high efficiency of the surrogate-based approach is demonstrated for three optimization scenarios with different and uncertain ambient conditions. Our results suggest the critical importance of considering uncertain pre-existing fracture networks in optimization studies of hydraulic fracturing. (c) 2013 Elsevier Ltd. All rights reserved.
C1 [Chen, Mingjie; Sun, Yunwei; Fu, Pengcheng; Carrigan, Charles R.; Buscheck, Thomas A.] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94551 USA.
[Lu, Zhiming] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA.
[Tong, Charles H.] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA.
RP Chen, MJ (reprint author), Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, POB 808,L-223, Livermore, CA 94551 USA.
EM cmj1014@yahoo.com
RI Sun, Yunwei/C-9751-2010; Fu, Pengcheng/D-7483-2012;
OI Fu, Pengcheng/0000-0002-7408-3350; Lu, Zhiming/0000-0001-5800-3368
FU U.S. Department of Energy by Lawrence Livermore National Laboratory
(LLNL) [DE-AC52-07NA27344]; LDRD-SI program of Lawrence Livermore
National Laboratory
FX This work was performed under the auspices of the U.S. Department of
Energy by Lawrence Livermore National Laboratory (LLNL) under contract
DE-AC52-07NA27344. This work was supported by LDRD-SI program of
Lawrence Livermore National Laboratory. We wish to thank Andrew Tompson
at LLNL and two anonymous reviewers for their comments that improved the
paper.
NR 43
TC 5
Z9 5
U1 3
U2 48
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0098-3004
EI 1873-7803
J9 COMPUT GEOSCI-UK
JI Comput. Geosci.
PD AUG
PY 2013
VL 58
BP 69
EP 79
DI 10.1016/j.cageo.2013.05.006
PG 11
WC Computer Science, Interdisciplinary Applications; Geosciences,
Multidisciplinary
SC Computer Science; Geology
GA 190PT
UT WOS:000322353400009
ER
PT J
AU Moridis, GJ
Reagan, MT
Kuzma, HA
Blasingame, TA
Huang, YW
Santos, R
Boyle, KL
Freeman, CM
Ilk, D
Cossio, M
Bhattacharya, S
Nikolaou, M
AF Moridis, George J.
Reagan, Matthew T.
Kuzma, Heidi Anderson
Blasingame, Thomas A.
Huang, Y. Wayne
Santos, Ralph
Boyle, Katie L.
Freeman, Craig M.
Ilk, Dilhan
Cossio, Manuel
Bhattacharya, Srimoyee
Nikolaou, Michael
TI SeTES: A self-teaching expert system for the analysis, design, and
prediction of gas production from unconventional gas resources
SO COMPUTERS & GEOSCIENCES
LA English
DT Article
DE Machine learning; Expert system; Bayesian networks; Simulation;
Optimization; Unconventional gas
AB SeTES is a self-teaching expert system that (a) can incorporate evolving databases involving any type and amount of relevant data (geological, geophysical, geomechanical, stimulation, petrophysical, reservoir, production, etc.) originating from unconventional gas reservoirs, i.e., tight sands, shale or coalbeds, (b) can continuously update its built-in public database and refine the its underlying decision-making metrics and process, (c) can make recommendations about well stimulation, well location, orientation, design, and operation, (d) offers predictions of the performance of proposed wells (and quantitative estimates of the corresponding uncertainty), and (e) permits the analysis of data from installed wells for parameter estimation and continuous expansion of its database. Thus, SeTES integrates and processes information from multiple and diverse sources to make recommendations and support decision making at multiple time-scales, while expanding its internal database and explicitly addressing uncertainty. It receives and manages data in three forms: public data, that have been made available by various contributors, semi-public data, which conceal some identifying aspects but are available to compute important statistics, and a user's private data, which can be protected and used for more targeted design and decision making. It is the first implementation of a novel architecture that allows previously independent analysis methods and tools to share data, integrate results, and intelligently and iteratively extract the most value from the dataset. SeTES also presents a new paradigm for communicating research and technology to the public and distributing scientific tools and methods. It is expected to result in a significant improvement in reserve estimates, and increases in production by increasing efficiency and reducing uncertainty. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Moridis, George J.; Reagan, Matthew T.; Santos, Ralph; Boyle, Katie L.; Freeman, Craig M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Blasingame, Thomas A.; Freeman, Craig M.; Ilk, Dilhan; Cossio, Manuel] Texas A&M Univ, Dept Petr Engn, College Stn, TX 77843 USA.
[Huang, Y. Wayne] Linear Time Informat LLC, Kansas City, MO USA.
[Bhattacharya, Srimoyee; Nikolaou, Michael] Univ Houston, Dept Chem Engn, Houston, TX 77204 USA.
RP Moridis, GJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd,MS 84R0171, Berkeley, CA 94720 USA.
EM GJMoridis@lbl.gov
RI Reagan, Matthew/D-1129-2015
OI Reagan, Matthew/0000-0001-6225-4928
FU Research Partnership to Secure Energy for America (RPSEA) through the
Ultra-Deepwater and Unconventional Natural Gas and Other Petroleum
Resources Research [07122-23]
FX This work was funded by the Research Partnership to Secure Energy for
America (RPSEA-Contract No. 07122-23) through the Ultra-Deepwater and
Unconventional Natural Gas and Other Petroleum Resources Research and
Development Program as authorized by the US Energy Policy Act (EPAct) of
2005.
NR 25
TC 1
Z9 1
U1 6
U2 35
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0098-3004
J9 COMPUT GEOSCI-UK
JI Comput. Geosci.
PD AUG
PY 2013
VL 58
BP 100
EP 115
DI 10.1016/j.cageo.2013.04.001
PG 16
WC Computer Science, Interdisciplinary Applications; Geosciences,
Multidisciplinary
SC Computer Science; Geology
GA 190PT
UT WOS:000322353400012
ER
PT J
AU Kim, TN
Underwood, N
Inouye, BD
AF Kim, Tania N.
Underwood, Nora
Inouye, Brian D.
TI Insect herbivores change the outcome of plant competition through both
inter- and intraspecific processes
SO ECOLOGY
LA English
DT Article
DE biocontrol; coexistence; competition; density dependence; insect
herbivory; intrinsic rate of increase; model selection; old-field
communities; plant-insect interactions; response surface; Solanum
carolinense; Solidago altissima
ID SOLANUM-CAROLINENSE; INTERSPECIFIC COMPETITION; 2-SPECIES COMPETITION;
SPECIES COEXISTENCE; SOLIDAGO-CANADENSIS; COMMUNITIES; FIELD;
CONSEQUENCES; SUCCESSION; GOLDENROD
AB Insect herbivores can affect plant abundance and community composition, and theory suggests that herbivores influence plant communities by altering interspecific interactions among plants. Because the outcome of interspecific interactions is influenced by the per capita competitive ability of plants, density dependence, and intrinsic rates of increase, measuring herbivore effects on all these processes is necessary to understand the mechanisms by which herbivores influence plant communities. We fit alternative competition models to data from a response surface experiment conducted over four years to examine how herbivores affected the outcome of competition between two perennial plants, Solidago altissima and Solanum carolinense. Within a growing season, herbivores reduced S. carolinense plant size but did not affect the size of S. altissima, which exhibited compensatory growth. Across seasons, herbivores did not affect S. carolinense density or biomass but reduced both the density and population growth of S. altissima. The best-fit models indicated that the effects of herbivores varied with year. In some years, herbivores increased the per capita competitive effect of S. altissima on S. carolinense; in other years, herbivores influenced the intrinsic rate of increase of S. altissima. We examined possible herbivore effects on the longer-term outcome of competition (over the time scale of a typical old-field habitat), using simulations based on the best-fit models. In the absence of herbivores, plant coexistence was observed. In the presence of herbivores, S. carolinense was excluded by S. altissima in 72.3% of the simulations. We demonstrate that herbivores can influence the outcome of competition through changes in both per capita competitive effects and intrinsic rates of increase. We discuss the implications of these results for ecological succession and biocontrol.
C1 [Kim, Tania N.; Underwood, Nora; Inouye, Brian D.] Florida State Univ, Dept Biol Sci, Tallahassee, FL 32306 USA.
RP Kim, TN (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA.
EM tkim@glbrc.wisc.edu
FU Robert K. Godfrey award in Botany; NSF [DEB-0717221]
FX We thank B. J. Spiesman, T. E. Miller, A. A. Winn, members of the
Underwood and Inouye labs, and two anonymous reviewers for helpful
comments on earlier drafts of the manuscript. We also thank the staff at
the Mission Road Research Facilities at Florida State University for
logistical support. This research was supported by the Robert K. Godfrey
award in Botany to T. Kim and NSF DEB-0717221 to N. Underwood.
NR 42
TC 11
Z9 12
U1 8
U2 182
PU ECOLOGICAL SOC AMER
PI WASHINGTON
PA 1990 M STREET NW, STE 700, WASHINGTON, DC 20036 USA
SN 0012-9658
J9 ECOLOGY
JI Ecology
PD AUG
PY 2013
VL 94
IS 8
BP 1753
EP 1763
DI 10.1890/12-1261.1
PG 11
WC Ecology
SC Environmental Sciences & Ecology
GA 190JU
UT WOS:000322336600010
PM 24015519
ER
PT J
AU Lee, PKH
Cheng, D
West, KA
Alvarez-Cohen, L
He, JZ
AF Lee, Patrick K. H.
Cheng, Dan
West, Kimberlee A.
Alvarez-Cohen, Lisa
He, Jianzhong
TI Isolation of two new Dehalococcoides mccartyi strains with dissimilar
dechlorination functions and their characterization by comparative
genomics via microarray analysis
SO ENVIRONMENTAL MICROBIOLOGY
LA English
DT Article
ID REDUCTIVE DEHALOGENASE GENES; VINYL-CHLORIDE REDUCTASE; 16S
RIBOSOMAL-RNA; CONTAMINATED GROUNDWATER; TRANS-DICHLOROETHENE; ANAEROBIC
BACTERIUM; ELECTRON-ACCEPTORS; CIS-DICHLOROETHENE; QUANTITATIVE PCR;
TETRACHLOROETHENE
AB Microbial reductive dechlorination of trichloroethene (TCE) in groundwater often results in the accumulation of dichloroethenes (DCEs). Dehalococcoides mccartyi (Dhc) are the only known bacteria capable of dechlorination beyond DCE to non-toxic ethene. In this study, two newly isolated Dhc strains (11a and 11a5) with dissimilar functional abilities are described. Strain 11a reductively dechlorinates TCE, 1,1-DCE, cis-DCE, trans-DCE, and vinyl chloride (VC) to ethene, while strain 11a5 dechlorinates TCE and all three DCE isomers only to VC. Each of these dechlorination reactions are coupled to growth by these strains. The VC dechlorination rate of strain 11a occurs at a rate of 258 nmol per min per mg of protein, about two times faster than previously reported stains. Strain 11a possesses the vcrA gene while strain 11a5 contains the tceA gene. Strains 11a and 11a5 share 100% 16S rRNA gene sequence identity with previously sequenced Dhc strains BAV1 and CBDB1, placing it within the Pinellas subgroup, and 85.4% and 89.5% of all genes present in the CBDB1 and BAV1 genomes were detected in strains 11a and 11a5, respectively, using a custom-designed microarray targeting four sequenced Dhc strains. Genes that were not detected in strains 11a and 11a5 are mostly within the high plasticity regions or integrated elements of the sequenced strains. This study reports the functional description and comparative genomics of two additional Dhc isolates and provides evidence that the observed functional incongruence between the activity and core genome phylogenies of Dhc strains is likely driven by the horizontal transfer of key reductive dehalogenase-encoding genes.
C1 [Lee, Patrick K. H.; West, Kimberlee A.; Alvarez-Cohen, Lisa] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA.
[Lee, Patrick K. H.] City Univ Hong Kong, Sch Energy & Environm, Hong Kong, Hong Kong, Peoples R China.
[Cheng, Dan; He, Jianzhong] Natl Univ Singapore, Dept Civil & Environm Engn, Singapore 117576, Singapore.
[Alvarez-Cohen, Lisa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
RP Alvarez-Cohen, L (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA.
EM alvarez@ce.berkeley.edu; jianzhong.he@nus.edu.sg
RI Lee, Patrick K H/L-1844-2016
OI Lee, Patrick K H/0000-0003-0911-5317
FU Strategic Environmental Research and Development Program [ER-1587];
NIEHS Superfund Basic Research Project [ES04705-19]; Singapore National
Research Foundation [NRF - CRP 5-2009-05]; Singapore Agency for Science,
Technology and Research (A*STAR) of the Science and Engineering Research
Council [102 101 0025]
FX This research was supported by the Strategic Environmental Research and
Development Program through Grant ER-1587, the NIEHS Superfund Basic
Research Project ES04705-19, the Competitive Research Programme from
Singapore National Research Foundation under Project No.: NRF - CRP
5-2009-05, and the Singapore Agency for Science, Technology and Research
(A*STAR) of the Science and Engineering Research Council under Project
No. 102 101 0025. We would like to thank Beiping Zhang from the Huazhong
University of Science and Technology (Wuhan, Hubei, China) for providing
sediments for this study.
NR 50
TC 7
Z9 7
U1 0
U2 53
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1462-2912
J9 ENVIRON MICROBIOL
JI Environ. Microbiol.
PD AUG
PY 2013
VL 15
IS 8
BP 2293
EP 2305
DI 10.1111/1462-2920.12099
PG 13
WC Microbiology
SC Microbiology
GA 194IP
UT WOS:000322625500013
PM 23480482
ER
PT J
AU Honnicke, MG
Huang, XR
Cusatis, C
Koditwuakku, CN
Cai, YQ
AF Hoennicke, Marcelo Goncalves
Huang, Xianrong
Cusatis, Cesar
Koditwuakku, Chaminda Nalaka
Cai, Yong Q.
TI High-quality quartz single crystals for high-energy-resolution inelastic
X-ray scattering analyzers
SO JOURNAL OF APPLIED CRYSTALLOGRAPHY
LA English
DT Article
ID GRADED MULTILAYER MIRROR; SYNTHETIC QUARTZ; SPECTROMETER;
BACKSCATTERING; SPECTROSCOPY; REFLECTIONS; TOPOGRAPHY; INTENSITY
AB Spherical analyzers are well known instruments for inelastic X-ray scattering (IXS) experiments. High-resolution IXS experiments almost always use Si single crystals as monochromators and spherical analyzers. At higher energies (>20 keV) Si shows a high energy resolution (<10 meV), at an exact symmetric back-diffraction condition, since the energy resolution is given by the real part of the susceptibility or polarizability. However, at low energies (<10 keV), high energy resolution is difficult to achieve with Si. alpha-SiO2 (quartz) can be an option, since it offers high energy resolution at low energies. In this work, the characterization of high-quality alpha-SiO2 is presented. Such characterization is made by high-resolution rocking curve, topography and lattice parameter mapping in different samples from a single block. X-ray optics with alpha-SiO2 for IXS at lower energies (from 2.5 to 12.6 keV) with medium to high energy resolution (from 90 to 11 meV) are proposed and theoretically exploited.
C1 [Hoennicke, Marcelo Goncalves] Univ Fed Integracao Latinoamer, BR-85867970 Foz Do Iguacu, Parana, Brazil.
[Huang, Xianrong] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Cusatis, Cesar] Univ Fed Parana, Dept Fis, BR-81531990 Curitiba, Parana, Brazil.
[Koditwuakku, Chaminda Nalaka; Cai, Yong Q.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA.
RP Honnicke, MG (reprint author), Univ Fed Integracao Latinoamer, Caixa Postal 2044, BR-85867970 Foz Do Iguacu, Parana, Brazil.
EM marcelo.honnicke@unila.edu.br
RI Cusatis, Cesar/N-7559-2014; Cai, Yong/C-5036-2008; Honnicke,
Marcelo/I-8624-2012
OI Cusatis, Cesar/0000-0002-1621-3727; Cai, Yong/0000-0002-9957-6426;
FU CNPq/PQ [305034/2010-3, 311570/2009-7]; US Department of Energy, Office
of Science, Office of Basic Energy Sciences [DE-AC-02-06CH11357,
DE-AC-02-98CH10886]
FX MGH is grateful to CNPq/PQ (305034/2010-3) for his research fellowship.
CC acknowledges CNPq/PQ (311570/2009-7) for support. This work was also
supported by the US Department of Energy, Office of Science, Office of
Basic Energy Sciences, under contract numbers DE-AC-02-06CH11357 and
DE-AC-02-98CH10886.
NR 28
TC 5
Z9 5
U1 2
U2 14
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0021-8898
J9 J APPL CRYSTALLOGR
JI J. Appl. Crystallogr.
PD AUG
PY 2013
VL 46
BP 939
EP 944
DI 10.1107/S0021889813004731
PN 4
PG 6
WC Chemistry, Multidisciplinary; Crystallography
SC Chemistry; Crystallography
GA 186HI
UT WOS:000322032300018
ER
PT J
AU Toby, BH
Madden, TJ
Suchomel, MR
Baldwin, JD
Von Dreele, RB
AF Toby, B. H.
Madden, T. J.
Suchomel, M. R.
Baldwin, J. D.
Von Dreele, R. B.
TI A scanning CCD detector for powder diffraction measurements
SO JOURNAL OF APPLIED CRYSTALLOGRAPHY
LA English
DT Article
ID POSITION-SENSITIVE DETECTOR; SWISS LIGHT-SOURCE; CRYSTALLOGRAPHY;
ACQUISITION; ASYMMETRY; BEAMLINE
AB Several different approaches have traditionally been used for detection of X-ray powder diffraction patterns, including area detectors, point detectors and position-sensitive detectors. Each has advantages. This paper discusses use of a low-cost CCD detector attached to a diffractometer arm, where line-by-line readout of the CCD is coupled to continuous motion of the arm. When this type of detector is used and where X-ray optics are employed to focus the source image onto the detector plane both high-resolution and rapid measurements can be performed, with data collection over a complete 2 theta range. This is particularly advantageous for synchrotron applications but valuable also for Guinier diffractometer laboratory instruments. Peak resolutions are shown to be moderately better than what can be obtained with a position-sensitive detector and significantly better than with an area detector. Many samples have intrinsically broadened peak shapes for which little improvement in data quality could be obtained with an analyzer-crystal detector. With comparable numbers of modules, these CCD data collection speeds can be close to those with position-sensitive detectors, but without the low-angle asymmetry seen in the latter.
C1 [Toby, B. H.; Madden, T. J.; Suchomel, M. R.; Baldwin, J. D.; Von Dreele, R. B.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Von Dreele, RB (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA.
EM vondreele@anl.gov
RI Toby, Brian/F-3176-2013; Suchomel, Matthew/C-5491-2015;
OI Toby, Brian/0000-0001-8793-8285; SUCHOMEL, Matthew/0000-0002-9500-5079
FU US DOE [DE-AC02-06CH11357]
FX Use of the Advanced Photon Source, an Office of Science user facility
operated for the US Department of Energy (DOE) Office of Science by
Argonne National Laboratory, was supported by the US DOE under contract
No. DE-AC02-06CH11357. We thank Lynn Ribaud for his great assistance
with data collection at APS beamline 11-BM. The jadrarite sample was
kindly provided by Dr Pamela Whitfield of the National Research Council
Canada.
NR 33
TC 0
Z9 0
U1 0
U2 13
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0021-8898
J9 J APPL CRYSTALLOGR
JI J. Appl. Crystallogr.
PD AUG
PY 2013
VL 46
BP 1058
EP 1063
DI 10.1107/S0021889813013824
PN 4
PG 6
WC Chemistry, Multidisciplinary; Crystallography
SC Chemistry; Crystallography
GA 186HI
UT WOS:000322032300032
ER
PT J
AU Borziak, K
Fleetwood, AD
Zhulin, IB
AF Borziak, Kirill
Fleetwood, Aaron D.
Zhulin, Igor B.
TI Chemoreceptor Gene Loss and Acquisition via Horizontal Gene Transfer in
Escherichia coli
SO JOURNAL OF BACTERIOLOGY
LA English
DT Article
ID SIGNAL TRANSDUCER; VIRULENCE FACTORS; CHEMOTAXIS; STRAINS; SEQUENCE;
SHIGELLA; AER; ADAPTATION; EVOLUTION; TAP
AB Chemotaxis allows bacteria to more efficiently colonize optimal microhabitats within their larger environment. Chemotaxis in Escherichia coli is the best-studied model system, and a large number of E. coli strains have been sequenced. The Escherichia/Shigella genus encompasses a great variety of commensal and pathogenic strains, but the role of chemotaxis in their association with the host remains poorly understood. Here we show that the core chemotaxis genes are lost in many, but not all, nonmotile strains but are well preserved in all motile strains. The genes encoding the Tar, Tsr, and Aer chemoreceptors, which mediate chemotaxis to a broad spectrum of chemical and physical cues, are also nearly uniformly conserved in motile strains. In contrast, the clade of extraintestinal pathogenic E. coli strains apparently underwent an ancestral loss of Trg and Tap chemoreceptors, which sense sugars, dipeptides, and pyrimidines. The broad range of time estimated for the loss of these genes (1 to 3 million years ago) corresponds to the appearance of the genus Homo.
C1 [Borziak, Kirill; Fleetwood, Aaron D.; Zhulin, Igor B.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA.
[Zhulin, Igor B.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN USA.
RP Borziak, K (reprint author), Syracuse Univ, Dept Biol, Syracuse, NY 13244 USA.
EM ijouline@utk.edu
RI Zhulin, Igor/A-2308-2012
OI Zhulin, Igor/0000-0002-6708-5323
FU National Institutes of Health [GM072295]; Graduate Program in Genome
Science and Technology, University of Tennessee-Oak Ridge National
Laboratory
FX This work was supported by National Institutes of Health grant GM072295
(to I.B.Z.). K.B. and A.D.F. received support from the Graduate Program
in Genome Science and Technology, University of Tennessee-Oak Ridge
National Laboratory.
NR 60
TC 4
Z9 4
U1 2
U2 14
PU AMER SOC MICROBIOLOGY
PI WASHINGTON
PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA
SN 0021-9193
J9 J BACTERIOL
JI J. Bacteriol.
PD AUG
PY 2013
VL 195
IS 16
BP 3596
EP 3602
DI 10.1128/JB.00421-13
PG 7
WC Microbiology
SC Microbiology
GA 188VX
UT WOS:000322226100011
PM 23749975
ER
PT J
AU Xie, SC
Liu, XH
Zhao, CF
Zhang, YY
AF Xie, Shaocheng
Liu, Xiaohong
Zhao, Chuanfeng
Zhang, Yuying
TI Sensitivity of CAM5-Simulated Arctic Clouds and Radiation to Ice
Nucleation Parameterization
SO JOURNAL OF CLIMATE
LA English
DT Article
DE Aerosols; Cloud microphysics; Ice crystals; Climate models; Cloud
parameterizations; Model evaluation; performance
ID COMMUNITY ATMOSPHERE MODEL; INSTRUMENT SIMULATORS; CLIMATE SIMULATIONS;
REMOTE SENSORS; VERSION-3 CAM3; GLOBAL-MODELS; PART I; NUCLEI;
MICROPHYSICS; SHEBA
AB Sensitivity of Arctic clouds and radiation in the Community Atmospheric Model, version 5, to the ice nucleation process is examined by testing a new physically based ice nucleation scheme that links the variation of ice nuclei (IN) number concentration to aerosol properties. The default scheme parameterizes the IN concentration simply as a function of ice supersaturation. The new scheme leads to a significant reduction in simulated IN concentration at all latitudes while changes in cloud amounts and properties are mainly seen at high- and midlatitude storm tracks. In the Arctic, there is a considerable increase in midlevel clouds and a decrease in low-level clouds, which result from the complex interaction among the cloud macrophysics, microphysics, and large-scale environment. The smaller IN concentrations result in an increase in liquid water path and a decrease in ice water path caused by the slowdown of the Bergeron-Findeisen process in mixed-phase clouds. Overall, there is an increase in the optical depth of Arctic clouds, which leads to a stronger cloud radiative forcing (net cooling) at the top of the atmosphere. The comparison with satellite data shows that the new scheme slightly improves low-level cloud simulations over most of the Arctic but produces too many midlevel clouds. Considerable improvements are seen in the simulated low-level clouds and their properties when compared with Arctic ground-based measurements. Issues with the observations and the model-observation comparison in the Arctic region are discussed.
C1 [Xie, Shaocheng; Zhao, Chuanfeng; Zhang, Yuying] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Liu, Xiaohong] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Xie, SC (reprint author), Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div L103, POB 808, Livermore, CA 94550 USA.
EM xie2@llnl.gov
RI Liu, Xiaohong/E-9304-2011; Zhang, Yuying/H-5011-2012; Zhao,
Chuanfeng/G-8546-2013; Xie, Shaocheng/D-2207-2013
OI Liu, Xiaohong/0000-0002-3994-5955; Xie, Shaocheng/0000-0001-8931-5145
FU Earth System Modeling Program of the Office of Science at the U.S.
Department of Energy (DOE); Atmospheric Radiation Measurement Program of
the Office of Science at the U.S. Department of Energy (DOE); DOE Office
of Science Atmospheric System Research (ASR) Program; DOE Office of
Science Earth System Modeling Program; DOE, Office of Science, Office of
Biological and Environmental Research by Lawrence Livermore National
Laboratory [DE-AC52-07NA27344]; Battelle Memorial Institute
[DE-AC06-76RLO 1830]
FX S. Xie, C. Zhao, and Y. Zhang are supported by the Earth System Modeling
Program and Atmospheric Radiation Measurement Program of the Office of
Science at the U.S. Department of Energy (DOE). Support for X. Liu was
provided by the DOE Office of Science Atmospheric System Research (ASR)
Program and Earth System Modeling Program. Work at LLNL was performed
under the auspices of the DOE, Office of Science, Office of Biological
and Environmental Research by Lawrence Livermore National Laboratory
under Contract DE-AC52-07NA27344. The Pacific Northwest National
Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute
under Contract DE-AC06-76RLO 1830. Discussions with Neil Barton, Stephen
Klein, James Boyle, and Yunyan Zhang of Lawrence Livermore National
Laboratory were helpful. We also thank the anonymous reviewers, whose
valuable comments helped to clarify and improve the paper.
NR 66
TC 22
Z9 23
U1 4
U2 35
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0894-8755
J9 J CLIMATE
JI J. Clim.
PD AUG
PY 2013
VL 26
IS 16
BP 5981
EP 5999
DI 10.1175/JCLI-D-12-00517.1
PG 19
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 196FU
UT WOS:000322759700016
ER
PT J
AU Kamarchik, E
Jasper, AW
AF Kamarchik, Eugene
Jasper, Ahren W.
TI Anharmonic Vibrational Properties from Intrinsic n-Mode State Densities
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID ENERGY-LEVEL SUMS; PARTITION-FUNCTION; HINDERED ROTORS; LARGE MOLECULES;
OF-STATES; QUANTUM; NUMBERS; APPROXIMATION; ACCURATE; SYSTEMS
AB A method for calculating fully anharmonic vibrational state counts, state densities, and partition functions for molecules is presented. The method makes use of a new quantity, the intrinsic density of states, which is associated with the states that uniquely arise from a given mode, mode pairing, or higher-order mode coupling. By using only low-order intrinsic densities, the fully coupled anharmonic vibrational result can be constructed, as shown by our application of the method to methane, CH4, and cyclopropene, C3H4. Truncation of the intrinsic expansion at the coupling of pairs of modes yields greatly improved scaling over direct evaluation of the full-dimensional result and recovers a large fraction of the total anharmonicity. We also discuss the relation of the new quantities to the structure of the potential energy surface.
C1 [Kamarchik, Eugene; Jasper, Ahren W.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA.
RP Kamarchik, E (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA.
EM ekamarc@sandia.gov; ajasper@sandia.gov
RI Jasper, Ahren/A-5292-2011
FU United States Department of Energy [DE-AC04-94-AL85000]
FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a
Lockheed Martin Company, for the United States Department of Energy
under contract DE-AC04-94-AL85000.
NR 40
TC 6
Z9 6
U1 0
U2 15
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 1
PY 2013
VL 4
IS 15
BP 2430
EP 2435
DI 10.1021/jz401181q
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 196WH
UT WOS:000322807600006
ER
PT J
AU Hong, WT
Gadre, M
Lee, YL
Biegalski, MD
Christen, HM
Morgan, D
Shao-Horn, Y
AF Hong, Wesley T.
Gadre, Milind
Lee, Yueh-Lin
Biegalski, Michael D.
Christen, Hans M.
Morgan, Dane
Shao-Horn, Yang
TI Tuning the Spin State in LaCoO3 Thin Films for Enhanced High-Temperature
Oxygen Electrocatalysis
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID OXIDE FUEL-CELLS; SURFACE EXCHANGE KINETICS; REDUCTION KINETICS; TRACER
DIFFUSION; CATHODES; ION; LA0.6SR0.4COO3-DELTA; CONDUCTIVITY;
PEROVSKITES; COEFFICIENT
AB The slow kinetics of oxygen surface exchange hinders the efficiency of high-temperature oxygen electrocatalytic devices such as solid oxide fuel cells and oxygen separation membranes. Systematic investigations of material properties that link to catalytic activity can aid in the rational design of highly active cathode materials. Here, we explore LaCoO3 thin films as a model system for tuning catalytic activity through strain-induced changes in the Co spin state. We demonstrate that Raman spectroscopy can be used to probe the Co-O bond strength at different temperatures to determine the relative spin occupancies of LaCoO3. We find that strain can be used to reduce the spin transition temperature and promote the occupation of higher spin states that weaken the Co-O bond. The decrease in Co-O bond strength and increased spin moment of the thin films result in significant enhancements of the oxygen surface exchange kinetics by up to 2 orders of magnitude.
C1 [Hong, Wesley T.; Shao-Horn, Yang] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA.
[Hong, Wesley T.; Gadre, Milind; Lee, Yueh-Lin; Shao-Horn, Yang] MIT, Electrochem Energy Lab, Cambridge, MA 02139 USA.
[Shao-Horn, Yang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA.
[Gadre, Milind; Morgan, Dane] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA.
[Biegalski, Michael D.; Christen, Hans M.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
RP Shao-Horn, Y (reprint author), MIT, Dept Mat Sci & Engn, 31-056,77 Massachusetts Ave, Cambridge, MA 02139 USA.
EM shaohorn@mit.edu
RI Hong, Wesley/H-1102-2014; Albe, Karsten/F-1139-2011; Christen,
Hans/H-6551-2013; LEE, YUEH-LIN/F-6274-2011
OI Christen, Hans/0000-0001-8187-7469; LEE, YUEH-LIN/0000-0003-2477-6412
FU U.S. Department of Energy [SISGR DE-SC0002633]; Oak Ridge National
Laboratory; Scientific User Facilities Division, Office of Basic Energy
Sciences, U.S. Department of Energy; National Science Foundation
[DMR-08-19762]
FX This work was supported in part by the U.S. Department of Energy (SISGR
DE-SC0002633). Pulsed laser deposition was performed at the Center for
Nanophase Materials Sciences, which is sponsored at Oak Ridge National
Laboratory by the Scientific User Facilities Division, Office of Basic
Energy Sciences, U.S. Department of Energy. This work made use of the
MRSEC Shared Experimental Facilities at MIT, supported by the National
Science Foundation under Award Number DMR-08-19762. We thank Dongkyu Lee
and Zhenxing Feng for their help with sample preparation for this study
and Justin Breucop for his help with developing the Raman measurement
protocol.
NR 47
TC 21
Z9 21
U1 1
U2 98
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 1
PY 2013
VL 4
IS 15
BP 2493
EP 2499
DI 10.1021/jz401271m
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 196WH
UT WOS:000322807600015
ER
PT J
AU Liu, SD
Wang, XP
Li, EY
Douglas, CJ
Chen, JG
Wang, SC
AF Liu, Shanda
Wang, Xiaoping
Li, Eryang
Douglas, Carl J.
Chen, Jin-Gui
Wang, Shucai
TI R2R3 MYB transcription factor PtrMYB192 regulates flowering time in
Arabidopsis by activating FLOWERING LOCUS C
SO JOURNAL OF PLANT BIOLOGY
LA English
DT Article
DE Arabidopsis; Flowering time; MYB transcription factors; Populus
trichocarpa
ID EXPRESSION ANALYSIS; EPIGENETIC REGULATION; POPULUS-TRICHOCARPA; WALL
BIOSYNTHESIS; GENE FAMILY; THALIANA; VERNALIZATION; CONSTANS; PATHWAY;
PROTEIN
AB R2R3 MYB transcription factors regulate multiple aspects of plant growth and development. Here we report the identification of PtrMYB192, a Populus R2R3 MYB transcription factor, as a negative regulator of flowering time. By using quantitative RT-PCR, we found that PtrMYB192, but not its closely homologous gene PtrMYB028, is highly expressed in mature leaves in Populus. Heterologously expression of PtrMYB192 under control of 35S promoter in Arabidopsis resulted in late flowering phenotypes under both long and short day conditions, indicating that PtrMYB192 controls flowering time independent of the photoperiod pathway. Domain swapping experiment showed that neither PtrMYB028DB-192AD nor PtrMYB192DB-028AD affected flowering time when heterologously expressed in Arabidopsis. However, when recruit to the promoter of a GAL4-GUS reporter gene by a GAL4 DNA binding domain in Arabidopsis protoplasts, both of PtrMYB028DB-192AD and PtrMYB192DB-028AD activated the reporter gene. Quantitative RT-PCR results showed an elevated expression of the floral repressor gene FLOWERING LOCUS C (FLC), but not the flowering-promoting gene CONSTANS (CO) in PtrMYB192 transgenic plants. Taken together, these results suggest that PtrMYB192 is a transcription activator that negatively regulating flowering time in Arabidopsis by activating FLC and possible other genes, and that both R2R3 DNA binding domain and activation domain maybe required for its full function.
C1 [Liu, Shanda; Wang, Xiaoping; Wang, Shucai] NE Normal Univ, Key Lab Mol Epigenet MOE, Changchun 130024, Peoples R China.
[Liu, Shanda; Wang, Xiaoping; Wang, Shucai] NE Normal Univ, Inst Genet & Cytol, Changchun 130024, Peoples R China.
[Li, Eryang; Douglas, Carl J.] Univ British Columbia, Dept Bot, Vancouver, BC V6T 1Z4, Canada.
[Chen, Jin-Gui] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA.
RP Wang, SC (reprint author), NE Normal Univ, Key Lab Mol Epigenet MOE, Changchun 130024, Peoples R China.
EM wangsc550@nenu.edu.cn
RI Chen, Jin-Gui/A-4773-2011
OI Chen, Jin-Gui/0000-0002-1752-4201
FU Northeast Normal University; Programme for Introducing Talents to
Universities [B07017]; Laboratory Directed Research and Development
Program of Oak Ridge National Laboratory; U.S. Department of Energy
[DE-AC05-00OR22725]
FX We thank Drs. Tom Guilfoyle and Gretchen Hagen (University of
Missouri-Columbia) for providing vectors for Arabidopsis protoplast
transfection assays. This work was supported by a startup fund from
Northeast Normal University [to S. W.], the Programme for Introducing
Talents to Universities (B07017) and the Laboratory Directed Research
and Development Program of Oak Ridge National Laboratory [to J.-G.C].
Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the
U.S. Department of Energy under contract DE-AC05-00OR22725.
NR 43
TC 6
Z9 6
U1 2
U2 43
PU SPRINGER HEIDELBERG
PI HEIDELBERG
PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY
SN 1226-9239
J9 J PLANT BIOL
JI J. Plant Biol.
PD AUG
PY 2013
VL 56
IS 4
BP 243
EP 250
DI 10.1007/s12374-013-0135-1
PG 8
WC Plant Sciences
SC Plant Sciences
GA 195WE
UT WOS:000322733500006
ER
PT J
AU Fortino, G
North, MJ
AF Fortino, G.
North, M. J.
TI Simulation-based development and validation of multi-agent systems: AOSE
and ABMS approaches
SO JOURNAL OF SIMULATION
LA English
DT Article
DE agent-based modelling; agent-oriented software engineering; multi-agent
systems
ID AGENT; METHODOLOGY; DESIGN
AB This paper briefly surveys an emerging research area: the integration of agent-oriented software engineering (AOSE) and agent-based modelling and simulation (ABMS). Both AOSE and ABMS are well-established research areas in the agent-based computing domain. Specifically, this paper provides an overview of the main simulation-based methodologies for developing multi-agent systems (MASs) that describe interesting ABMS application domains where the integration of AOSE and ABMS can benefit MAS development.
C1 [Fortino, G.] Univ Calabria, DIMES, DEIS, I-87036 Arcavacata Di Rende, CS, Italy.
[North, M. J.] Argonne Natl Lab, Argonne, IL 60439 USA.
RP North, MJ (reprint author), Argonne Natl Lab, Decis & Informat Sci Div, 9700 S Cass Ave,Bldg 221, Argonne, IL 60439 USA.
EM north@anl.gov
OI Fortino, Giancarlo/0000-0002-4039-891X
NR 40
TC 2
Z9 2
U1 2
U2 9
PU PALGRAVE MACMILLAN LTD
PI BASINGSTOKE
PA BRUNEL RD BLDG, HOUNDMILLS, BASINGSTOKE RG21 6XS, HANTS, ENGLAND
SN 1747-7778
J9 J SIMUL
JI J. Simul.
PD AUG
PY 2013
VL 7
IS 3
SI SI
BP 137
EP 143
DI 10.1057/jos.2013.12
PG 7
WC Computer Science, Interdisciplinary Applications; Operations Research &
Management Science
SC Computer Science; Operations Research & Management Science
GA 196CC
UT WOS:000322750000001
ER
PT J
AU Hagos, S
Feng, Z
McFarlane, S
Leung, LR
AF Hagos, Samson
Feng, Zhe
McFarlane, Sally
Leung, L. Ruby
TI Environment and the Lifetime of Tropical Deep Convection in a
Cloud-Permitting Regional Model Simulation
SO JOURNAL OF THE ATMOSPHERIC SCIENCES
LA English
DT Article
DE Cloud resolving models; Clouds; Cumulus clouds; Model evaluation;
performance; Regional models
ID LIVED SQUALL LINES; PACIFIC WARM POOL; WESTERN PACIFIC; STRATIFORM
PRECIPITATION; TOGA COARE; SYSTEMS; RESOLUTION
AB By applying a cloud-tracking algorithm to tropical convective systems in a regional high-resolution model simulation, this study documents the environmental conditions before and after convective systems are initiated over ocean and land by following them during their lifetime. The comparative roles of various mechanisms of convection-environment interaction on the longevity of convective systems are quantified. The statistics of lifetime, maximum area, and propagation speed of the simulated deep convection agree well with geostationary satellite observations.Among the environmental variables considered, lifetime of convective systems is found to be most related to midtropospheric moisture before as well as after the initiation of convection. Over ocean, convective systems enhance surface fluxes through the associated cooling and drying of the boundary layer as well as increased wind gusts. This process appears to play a minor positive role in the longevity of systems. For systems of equal lifetime, those over land tend to be more intense than those over ocean especially during the early stages of their life cycle. Both over ocean and land, convection is found to transport momentum vertically to increase low-level shear and decrease upper-level shear, but no discernible effect of shear on the lifetime of the convective systems is found.
C1 [Hagos, Samson; Feng, Zhe; McFarlane, Sally; Leung, L. Ruby] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Hagos, S (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA.
EM samson.hagos@pnnl.gov
RI Feng, Zhe/D-9531-2013; Feng, Zhe/E-1877-2015
OI Feng, Zhe/0000-0002-7540-9017
FU U.S. Department of Energy under the Atmospheric System Research Program;
U.S. Department of Energy under the Regional and Global Climate Modeling
Program; U.S. Department of Energy [AC06-76RLO1830]
FX The authors thank Dr. Jin-Ho Yoon for his comments and suggestions. This
work is supported by the U.S. Department of Energy under the Atmospheric
System Research Program and the Regional and Global Climate Modeling
Program. Computing resources for the simulations are provided by the
National Center for Computational Sciences (NCCS) through the INCITE
Climate End Station project and National Energy Research Scientific
Computing Center (NERSC). Pacific Northwest National Laboratory is
operated by Battelle for the U.S. Department of Energy under Contract
DE-AC06-76RLO1830.
NR 27
TC 9
Z9 9
U1 2
U2 9
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0022-4928
J9 J ATMOS SCI
JI J. Atmos. Sci.
PD AUG
PY 2013
VL 70
IS 8
BP 2409
EP 2425
DI 10.1175/JAS-D-12-0260.1
PG 17
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 195RK
UT WOS:000322721100005
ER
PT J
AU Li, ACY
Nozick, L
Davidson, R
Brown, N
Jones, DA
Wolshon, B
AF Li, Anna C. Y.
Nozick, Linda
Davidson, Rachel
Brown, Nathanael
Jones, Dean A.
Wolshon, Brian
TI Approximate Solution Procedure for Dynamic Traffic Assignment
SO JOURNAL OF TRANSPORTATION ENGINEERING
LA English
DT Article
DE Hurricane evacuation; Dynamic traffic assignment; User equilibrium
ID VARIATIONAL INEQUALITY FORMULATION; ROUTE CHOICE PROBLEM; KINEMATIC
WAVES; ROAD NETWORKS; MODEL; EVACUATION; ALGORITHM; FLOWS
AB This paper proposes an approximate dynamic traffic assignment algorithm for the analysis of traffic conditions in large-scale road networks over several days. The time-dependent origin-destination trips are assumed to be known. A case study for evacuation of the New Orleans metropolitan area prior to the landfall of Hurricane Katrina is presented to test the efficiency and effectiveness of the proposed procedure. The model results are compared to the traffic counts collected during the evacuation and then further tested by the mesoscopic simulation-based model, DynusT. The study shows that the traffic pattern produced by the proposed procedure is a good approximation to traffic count data and that the algorithm provides a good approximation to the computations performed by DynusT. (C) 2013 American Society of Civil Engineers.
C1 [Li, Anna C. Y.; Nozick, Linda] Cornell Univ, Sch Civil & Environm Engn, Ithaca, NY 14853 USA.
[Davidson, Rachel] Univ Delaware, Dept Civil & Environm Engn, Newark, DE 19716 USA.
[Brown, Nathanael; Jones, Dean A.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Wolshon, Brian] Louisiana State Univ, Dept Civil & Environm Engn, Gulf Coast Res Ctr Evacuat & Transportat Resilien, Baton Rouge, LA 70803 USA.
RP Nozick, L (reprint author), Cornell Univ, Sch Civil & Environm Engn, Ithaca, NY 14853 USA.
EM lkn3@cornell.edu
FU National Science Foundation [SES-0826832]
FX This work has been funded by the National Science Foundation under grant
No. SES-0826832. The authors gratefully acknowledge the continuing
support and data provided by the Louisiana Department of Transportation
and Development.
NR 49
TC 2
Z9 2
U1 2
U2 26
PU ASCE-AMER SOC CIVIL ENGINEERS
PI RESTON
PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA
SN 0733-947X
J9 J TRANSP ENG
JI J. Transp. Eng.
PD AUG 1
PY 2013
VL 139
IS 8
BP 822
EP 832
DI 10.1061/(ASCE)TE.1943-5436.0000518
PG 11
WC Engineering, Civil; Transportation Science & Technology
SC Engineering; Transportation
GA 195RH
UT WOS:000322720800006
ER
PT J
AU Matsuda, K
Brown, CR
Foley, B
Goeken, R
Whitted, S
Dang, Q
Wu, F
Plishka, R
Buckler-White, A
Hirscha, VM
AF Matsuda, Kenta
Brown, Charles R.
Foley, Brian
Goeken, Robert
Whitted, Sonya
Dang, Que
Wu, Fan
Plishka, Ronald
Buckler-White, Alicia
Hirscha, Vanessa M.
TI Laser Capture Microdissection Assessment of Virus Compartmentalization
in the Central Nervous Systems of Macaques Infected with Neurovirulent
Simian Immunodeficiency Virus
SO JOURNAL OF VIROLOGY
LA English
DT Article
ID CNS PENETRATION-EFFECTIVENESS; ANTIRETROVIRAL THERAPY; CHOROID-PLEXUS;
PROGRESSOR MACAQUES; CEREBROSPINAL-FLUID; HIV-INFECTION; BRAIN-REGIONS;
TYPE-1; SEQUENCES; ENCEPHALITIS
AB Nonhuman primate-simian immunodeficiency virus (SIV) models are powerful tools for studying the pathogenesis of human immunodeficiency virus type 1 (HIV-1) in the brain. Our laboratory recently isolated a neuropathogenic viral swarm, SIVsmH804E, a derivative of SIVsmE543-3, which was the result of sequential intravenous passages of viruses isolated from the brains of rhesus macaques with SIV encephalitis. Animals infected with SIVsmH804E or its precursor (SIVsmH783Br) developed SIV meningitis and/or encephalitis at high frequencies. Since we observed macaques with a combination of meningitis and encephalitis, as well as animals in which meningitis or encephalitis was the dominant component, we hypothesized that distinct mechanisms could be driving the two pathological states. Therefore, we assessed viral populations in the meninges and the brain parenchyma by laser capture microdissection. Viral RNAs were isolated from representative areas of the meninges, brain parenchyma, terminal plasma, and cerebrospinal fluid (CSF) and from the inoculum, and the SIV envelope fragment was amplified by PCR. Phylogenetic analysis of envelope sequences from the conventional progressors revealed compartmentalization of viral populations between the meninges and the parenchyma. In one of these animals, viral populations in meninges were closely related to those from CSF and shared signature truncations in the cytoplasmic domain of gp41, consistent with a common origin. Apart from magnetic resonance imaging (MRI) and positron-emission tomography (PET) imaging, CSF is the most accessible assess to the central nervous system for HIV-1-infected patients. However, our results suggest that the virus in the CSF may not always be representative of viral populations in the brain and that caution should be applied in extrapolating between the properties of viruses in these two compartments.
C1 [Matsuda, Kenta; Brown, Charles R.; Goeken, Robert; Whitted, Sonya; Dang, Que; Wu, Fan; Plishka, Ronald; Buckler-White, Alicia; Hirscha, Vanessa M.] NIAID, Mol Microbiol Lab, NIH, Bethesda, MD 20892 USA.
[Foley, Brian] Los Alamos Natl Lab, Grp T 6, Los Alamos, NM USA.
RP Hirscha, VM (reprint author), NIAID, Mol Microbiol Lab, NIH, Bethesda, MD 20892 USA.
EM vhirsch@niaid.nih.gov
OI Foley, Brian/0000-0002-1086-0296
FU NIAID, NIH; JSPS Research Fellowship for Japanese Biomedical and
Behavioral Researchers at NIH
FX This work was supported by the intramural research program of NIAID,
NIH, and by a JSPS Research Fellowship for Japanese Biomedical and
Behavioral Researchers at NIH.
NR 47
TC 11
Z9 11
U1 3
U2 8
PU AMER SOC MICROBIOLOGY
PI WASHINGTON
PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA
SN 0022-538X
J9 J VIROL
JI J. Virol.
PD AUG
PY 2013
VL 87
IS 16
BP 8896
EP 8908
DI 10.1128/JVI.00874-13
PG 13
WC Virology
SC Virology
GA 193CS
UT WOS:000322535600008
PM 23720733
ER
PT J
AU Payne, SJ
McCaffrey, R
Kattenhorn, SA
AF Payne, S. J.
McCaffrey, R.
Kattenhorn, S. A.
TI Extension-driven right-lateral shear in the Centennial shear zone
adjacent to the eastern Snake River Plain, Idaho
SO LITHOSPHERE
LA English
DT Article
ID LIMA RESERVOIR FAULT; SEISMIC REFRACTION; SOUTHWESTERN MONTANA; CRUSTAL
STRUCTURE; RANGE PROVINCE; STRAIN RATES; BORAH PEAK; BASIN; DEFORMATION;
EARTHQUAKE
AB We evaluate global positioning system (GPS) surface velocities and gravitational potential energy (GPE) variations to assess the causes of right-lateral shear in the Centennial shear zone, a NE-trending accommodation zone between the extensional Centennial tectonic belt (Montana-Idaho) and volcanic terrain of the eastern Snake River Plain (Idaho). We test the hypothesized "bookshelf" faulting model and find that the normal faults in the Centennial tectonic belt do not accommodate distributed dextral shear. Instead, GPS data reveal that rapid extension in the Centennial tectonic belt adjacent to the much more slowly deforming region of the Snake River Plain drives right-lateral shear between them at rates of 0.3-1.5 mm yr(-1). GPE variations support gravitational collapse at a higher rate in the Centennial tectonic belt due to higher topography than in eastern Snake River Plain, which has lower GPE variations due to its low-relief, flat topography and a denser crustal composition. Surface velocity gradients observed in GPS data across the 40-45-km-wide Centennial shear zone reveal distributed deformation due to strike-slip faulting, distributed simple shear, regional-scale rotation, or some combination thereof. In the Centennial shear zone, the fastest lateral shearing is closest to the Yellowstone Plateau, where fault plane solutions with components of right-lateral strike slip are documented within a NE-trending zone of seismicity. Here, two Basin and Range normal faults have Holocene and late Pleistocene slip along their segments that suggest they each may have linked under right-lateral shear. We also propose that right-lateral strike-slip motion may be accommodated on existing NE-trending faults.
C1 [Payne, S. J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[McCaffrey, R.] Portland State Univ, Dept Geol, Portland, OR 97207 USA.
[Kattenhorn, S. A.] Univ Idaho, Dept Geol Sci, Moscow, ID 83844 USA.
RP Payne, SJ (reprint author), Idaho Natl Lab, POB 1625,MS 2203, Idaho Falls, ID 83415 USA.
FU Idaho National Laboratory through the U.S. Department of Energy Idaho
Operations Office [DE-AC07-05ID14517]; National Earthquake Hazards
Research Program (NEHRP) [2010-0006]; National Science Foundation (NSF)
[EAR-1062251]
FX We very much appreciate the reviews by David Anastasio, Eric Kirby, and
an anonymous reviewer, which helped improve the manuscript. We thank Bob
King for his support and processing of the global positioning system
data used in the study. We also thank Mike Stickney for providing us
with fault plane solutions from the unpublished Montana Bureau of Mines
and Geology catalog. Payne appreciates the helpful discussions and
reviews by Seth Carpenter. The research was funded in part by the Idaho
National Laboratory through the U.S. Department of Energy Idaho
Operations Office contract DE-AC07-05ID14517. The research was supported
by the National Earthquake Hazards Research Program (NEHRP) grant
2010-0006 and National Science Foundation (NSF) grant EAR-1062251 to
McCaffrey.
NR 61
TC 3
Z9 3
U1 0
U2 6
PU GEOLOGICAL SOC AMER, INC
PI BOULDER
PA PO BOX 9140, BOULDER, CO 80301-9140 USA
SN 1941-8264
J9 LITHOSPHERE-US
JI Lithosphere
PD AUG
PY 2013
VL 5
IS 4
BP 407
EP 419
DI 10.1130/L200.1
PG 13
WC Geochemistry & Geophysics; Geology
SC Geochemistry & Geophysics; Geology
GA 193GW
UT WOS:000322548100006
ER
PT J
AU Baidoo, EEK
Keasling, JD
AF Baidoo, Edward E. K.
Keasling, Jay D.
TI Microbial metabolomics: welcome to the real world!
SO METABOLOMICS
LA English
DT Editorial Material
C1 [Baidoo, Edward E. K.; Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Bioenergy Inst, Phys Biosci Div, Berkeley, CA 94720 USA.
[Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.
[Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.
RP Keasling, JD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Bioenergy Inst, Phys Biosci Div, Berkeley, CA 94720 USA.
EM eebaidoo@lbl.gov; jdkeasling@lbl.gov
RI Keasling, Jay/J-9162-2012
OI Keasling, Jay/0000-0003-4170-6088
NR 0
TC 1
Z9 1
U1 0
U2 43
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1573-3882
J9 METABOLOMICS
JI Metabolomics
PD AUG
PY 2013
VL 9
IS 4
BP 755
EP 756
DI 10.1007/s11306-013-0562-5
PG 2
WC Endocrinology & Metabolism
SC Endocrinology & Metabolism
GA 186CJ
UT WOS:000322019100001
ER
PT J
AU Ganeshalingam, M
Li, WD
Filippenko, AV
AF Ganeshalingam, Mohan
Li, Weidong
Filippenko, Alexei V.
TI Constraints on dark energy with the LOSS SN Ia sample
SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY
LA English
DT Article
DE supernovae: general; cosmological parameters; cosmology: observations;
distance scale
ID OBSERVATORY SUPERNOVA SEARCH; HUBBLE-SPACE-TELESCOPE; DIGITAL SKY
SURVEY; PHOTOMETRIC STANDARD STARS; BVRI LIGHT CURVES; 2-PARAMETER
LUMINOSITY CORRECTION; AUTOMATIC IMAGING TELESCOPE; LEGACY SURVEY;
LOW-REDSHIFT; DATA RELEASE
AB We present a cosmological analysis of the Lick Observatory Supernova Search (LOSS) Type Ia supernova (SN Ia) photometry sample introduced by Ganeshalingam et al. These supernovae (SNe) provide an effective anchor point to estimate cosmological parameters when combined with data sets at higher redshift. The data presented by Ganeshalingam et al. have been rereduced in the natural system of the Katzman Automatic Imaging Telescope (KAIT) and Nickel telescopes to minimize systematic uncertainties. We have run the light-curve-fitting software salt2 on our natural-system light curves to measure light-curve parameters for LOSS light curves and available SN Ia data sets in the literature. We present a Hubble diagram of 586 SNe in the redshift range z = 0.01-1.4 with a residual scatter of 0.176 mag. Of the 226 low-z SNe Ia in our sample, 91 objects are from LOSS, including 45 without previously published distances. Assuming a flat Universe, we find that the best fit for the dark energy equation-of-state parameter w = -0.86(-0.16)(+0.13) +/- 0.11 (sys) from SNe alone, consistent with a cosmological constant. Our data prefer a Universe with an accelerating rate of expansion with 99.999 per cent confidence. When looking at Hubble residuals as a function of host-galaxy morphology, we do not see evidence for a significant trend, although we find a somewhat reduced scatter in Hubble residuals from SNe residing within a projected distance < 10 kpc of the host-galaxy nucleus (Sigma = 0.156 mag). Similar to the results of Blondin, Mandel and Kirshner and Silverman et al., we find that Hubble residuals do not correlate with the expansion velocity of Si ii lambda 6355 measured in optical spectra near maximum light. Our data are consistent with no presence of a local 'Hubble bubble.' Improvements in cosmological analyses within low-z samples can be achieved by better constraining calibration uncertainties in the zero-points of photometric systems.
C1 [Ganeshalingam, Mohan; Li, Weidong; Filippenko, Alexei V.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA.
[Ganeshalingam, Mohan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Ganeshalingam, M (reprint author), Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA.
EM mganeshalingam@lbl.gov
FU US National Science Foundation (NSF) [AST-0908886, AST-1211916]; TABASGO
Foundation; Christopher R. Redlich Fund; US Department of Energy SciDAC
grant [DE-FC02-06ER41453]; US Department of Energy [DE-FG02-08ER41563];
NASA
FX The work of AVF's supernova group at UC Berkeley has been generously
supported by the US National Science Foundation (NSF; most recently
through grants AST-0908886 and AST-1211916), the TABASGO Foundation, the
Christopher R. Redlich Fund, US Department of Energy SciDAC grant
DE-FC02-06ER41453 and US Department of Energy grant DE-FG02-08ER41563.
KAIT and its ongoing operation were made possible by donations from Sun
Microsystems, Inc., the Hewlett-Packard Company, AutoScope Corporation,
Lick Observatory, the NSF, the University of California, the Sylvia and
Jim Katzman Foundation, the Christopher R. Redlich Fund, the Richard and
Rhoda Goldman Fund, and the TABASGO Foundation. We give particular
thanks to Russell M. Genet, who made KAIT possible with his initial
special gift to AVF; Joseph S. Miller, who allowed KAIT to be placed at
Lick Observatory and provided staff support; Jack Borde, who provided
invaluable advice regarding the KAIT optics; Richard R. Treffers, KAIT's
chief engineer; and the TABASGO Foundation, without which this work
would not have been completed. We made use of the NASA/IPAC
Extragalactic Database (NED), which is operated by the Jet Propulsion
Laboratory, California Institute of Technology, under contract with
NASA.
NR 124
TC 19
Z9 19
U1 0
U2 6
PU OXFORD UNIV PRESS
PI OXFORD
PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND
SN 0035-8711
J9 MON NOT R ASTRON SOC
JI Mon. Not. Roy. Astron. Soc.
PD AUG
PY 2013
VL 433
IS 3
BP 2240
EP 2258
DI 10.1093/mnras/stt893
PG 19
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 191HK
UT WOS:000322403800040
ER
PT J
AU Schneider, MD
Cole, S
Frenk, CS
Kelvin, L
Mandelbaum, R
Norberg, P
Bland-Hawthorn, J
Brough, S
Driver, S
Hopkins, A
Liske, J
Loveday, J
Robotham, A
AF Schneider, Michael D.
Cole, Shaun
Frenk, Carlos S.
Kelvin, Lee
Mandelbaum, Rachel
Norberg, Peder
Bland-Hawthorn, Joss
Brough, Sarah
Driver, Simon
Hopkins, Andrew
Liske, Jochen
Loveday, Jon
Robotham, Aaron
TI Galaxy And Mass Assembly (GAMA): galaxy radial alignments in GAMA groups
SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY
LA English
DT Article
DE galaxies: clusters: general; galaxies: formation; galaxies: statistics
ID DIGITAL SKY SURVEY; DARK-MATTER SUBHALOES; WEAK-LENSING SURVEYS;
INTRINSIC ALIGNMENTS; SATELLITE GALAXIES; CLUSTER GALAXIES; COMA
CLUSTER; ORIENTATIONS; SIMULATIONS; CATALOG
AB We constrain the distributions of projected radial alignment angles of satellite galaxy shapes within the Galaxy And Mass Assembly survey group catalogue. We identify the galaxy groups using spectroscopic redshifts and measure galaxy projected ellipticities from Sloan Digital Sky Survey imaging. With a sample of 3850 groups with 13 655 satellite galaxies with high quality shape measurements, we find a less than 2 Sigma signal of radial alignments in the mean projected ellipticity components and the projected position angle when using galaxy shape estimates optimized for weak lensing measurements. Our radial alignment measurement increases to greater than 3 Sigma significance relative to the expectation for no alignments if we use 2D Sersic model fits to define galaxy orientations. Our weak measurement of radial alignments is in conflict with predictions from dark-matter N-body simulations, which we interpret as evidence for large misalignments of baryons and dark matter in group and cluster satellites. Within our uncertainties, that are dominated by our small sample size, we find only weak and marginally significant trends of the radial alignment angle distributions on projected distance from the group centre, host halo mass, and redshift that could be consistent with a tidal torquing mechanism for radial alignments. Using our lensing optimized shape estimators, we estimate that intrinsic alignments of galaxy group members may contribute a systematic error to the mean differential projected surface mass density of groups inferred from weak lensing observations by -1 +/- 20 per cent at scales around 300 h(-1) kpc from the group centre assuming a photometric redshift rms error of 10 per cent, and given our group sample with median redshift of 0.17 and median virial masses similar to 10(13) h(-1) M-circle dot.
C1 [Schneider, Michael D.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA.
[Schneider, Michael D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
[Cole, Shaun; Frenk, Carlos S.; Norberg, Peder] Univ Durham, Dept Phys, Inst Computat Cosmol, Durham DH1 3LE, England.
[Kelvin, Lee; Driver, Simon; Robotham, Aaron] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland.
[Kelvin, Lee; Driver, Simon; Robotham, Aaron] Univ Western Australia, Int Ctr Radio Astron Res, Perth, WA 6009, Australia.
[Mandelbaum, Rachel] Princeton Univ Observ, Princeton, NJ 08544 USA.
[Mandelbaum, Rachel] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA.
[Bland-Hawthorn, Joss] Univ Sydney, Sydney Inst Astron, Sydney, NSW 2006, Australia.
[Brough, Sarah; Hopkins, Andrew] Australian Astron Observ, Epping, NSW 1710, Australia.
[Liske, Jochen] European So Observ, D-85748 Garching, Germany.
[Loveday, Jon] Univ Sussex, Ctr Astron, Brighton BN1 9QH, E Sussex, England.
RP Schneider, MD (reprint author), Univ Calif Davis, Dept Phys, 1 Shields Ave, Davis, CA 95616 USA.
EM schneider@ucdavis.edu
RI Robotham, Aaron/H-5733-2014; Mandelbaum, Rachel/N-8955-2014; Driver,
Simon/H-9115-2014
OI Liske, Jochen/0000-0001-7542-2927; Robotham, Aaron/0000-0003-0429-3579;
Mandelbaum, Rachel/0000-0003-2271-1527; Driver,
Simon/0000-0001-9491-7327
FU ERC StG grant [DEGAS-259586]; US Department of Energy by Lawrence
Livermore National Laboratory [DE-AC52-07NA27344]; STFC (UK);
Astrophysical Research Consortium (ARC; Australia); AAO; Alfred P. Sloan
Foundation; National Science Foundation; U.S. Department of Energy;
National Aeronautics and Space Administration; Japanese Monbukagakusho;
Max Planck Society; Higher Education Funding Council for England;
American Museum of Natural History; Astrophysical Institute Potsdam;
University of Basel; University of Cambridge; Case Western Reserve
University; University of Chicago; Drexel University; Fermilab;
Institute for Advanced Study; Johns Hopkins University; Joint Institute
for Nuclear Astrophysics; Kavli Institute for Particle Astrophysics and
Cosmology; Chinese Academy of Sciences (LAMOST); Los Alamos National
Laboratory; Max-Planck-Institute for Astronomy (MPIA);
Max-Planck-Institute for Astrophysics (MPA); New Mexico State
University; Ohio State University; University of Pittsburgh; University
of Portsmouth; Princeton University; United States Naval Observatory;
University of Washington
FX We thank Jonathan Blazek for helpful feedback on an early version of
this paper and an anonymous referee for many helpful improvements
including the suggestion to measure alignments for different galaxy
morphologies. PN acknowledges a Royal Society URF and ERC StG grant
(DEGAS-259586). Part of this work performed under the auspices of the US
Department of Energy by Lawrence Livermore National Laboratory under
Contract DE-AC52-07NA27344. GAMA is a joint European-Australasian
project based around a spectroscopic campaign using the Anglo-Australian
Telescope. The GAMA input catalogue is based on data taken from the
Sloan Digital Sky Survey and the UKIRT Infrared Deep Sky Survey.
Complementary imaging of the GAMA regions is being obtained by a number
of independent survey programs including GALEX MIS, VST KIDS, VISTA
VIKING, WISE, Herschel-ATLAS, GMRT and ASKAP providing UV to radio
coverage. GAMA is funded by the STFC (UK), the Astrophysical Research
Consortium (ARC; Australia), the AAO and the participating institutions.
The GAMA website is http://www.gama-survey.org/.; Funding for the SDSS
and SDSS-II has been provided by the Alfred P. Sloan Foundation, the
Participating Institutions, the National Science Foundation, the U.S.
Department of Energy, the National Aeronautics and Space Administration,
the Japanese Monbukagakusho, the Max Planck Society, and the Higher
Education Funding Council for England. The SDSS Web Site is
http://www.sdss.org/.; The SDSS is managed by the ARC for the
Participating Institutions. The Participating Institutions are the
American Museum of Natural History, Astrophysical Institute Potsdam,
University of Basel, University of Cambridge, Case Western Reserve
University, University of Chicago, Drexel University, Fermilab, the
Institute for Advanced Study, the Japan Participation Group, Johns
Hopkins University, the Joint Institute for Nuclear Astrophysics, the
Kavli Institute for Particle Astrophysics and Cosmology, the Korean
Scientist Group, the Chinese Academy of Sciences (LAMOST), Los Alamos
National Laboratory, the Max-Planck-Institute for Astronomy (MPIA), the
Max-Planck-Institute for Astrophysics (MPA), New Mexico State
University, Ohio State University, University of Pittsburgh, University
of Portsmouth, Princeton University, the United States Naval
Observatory, and the University of Washington.
NR 43
TC 18
Z9 18
U1 0
U2 3
PU OXFORD UNIV PRESS
PI OXFORD
PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND
SN 0035-8711
J9 MON NOT R ASTRON SOC
JI Mon. Not. Roy. Astron. Soc.
PD AUG
PY 2013
VL 433
IS 4
BP 2727
EP 2738
DI 10.1093/mnras/stt855
PG 12
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 191IF
UT WOS:000322405900003
ER
PT J
AU Chuang, CH
Prada, F
Cuesta, AJ
Eisenstein, DJ
Kazin, E
Padmanabhan, N
Sanchez, AG
Xu, XY
Beutler, F
Manera, M
Schlegel, DJ
Schneider, DP
Weinberg, DH
Brinkmann, J
Brownstein, JR
Thomas, D
AF Chuang, Chia-Hsun
Prada, Francisco
Cuesta, Antonio J.
Eisenstein, Daniel J.
Kazin, Eyal
Padmanabhan, Nikhil
Sanchez, Ariel G.
Xu, Xiaoying
Beutler, Florian
Manera, Marc
Schlegel, David J.
Schneider, Donald P.
Weinberg, David H.
Brinkmann, Jon
Brownstein, Joel R.
Thomas, Daniel
TI The clustering of galaxies in the SDSS-III Baryon Oscillation
Spectroscopic Survey: single-probe measurements and the strong power of
f(z)Sigma(8)(z) on constraining dark energy
SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY
LA English
DT Article
DE cosmological parameters; cosmology: observations; distance scale;
large-scale structure of Universe
ID DIGITAL SKY SURVEY; LUMINOUS RED GALAXIES; 2-POINT CORRELATION-FUNCTION;
REDSHIFT-SPACE DISTORTIONS; DATA RELEASE; ACOUSTIC-OSCILLATIONS;
COSMOLOGICAL IMPLICATIONS; TO 0.5; SCALE; SAMPLE
AB We present measurements of the anisotropic galaxy clustering from the Data Release 9 (DR9) CMASS sample of the Sloan Digital Sky Survey (SDSS)-III Baryon Oscillation Spectroscopic Survey (BOSS). We analyse the broad-range shape of the monopole and quadrupole correlation functions to obtain constraints, at the effective redshift z = 0.57 of the sample, on the Hubble expansion rate H(z), the angular-diameter distance D-A(z), the normalized growth rate f (z)Sigma(8)(z), the physical matter density (m)h(2), and the biased amplitude of matter fluctuation b Sigma(8)(z). We obtain H(0.57), D-A(0.57), f (0.57)Sigma(8)(0.57), (m)h(2), b Sigma(8)(0.57) = 87.6_-6.8 boolean AND+6.7 kms(-1) Mpc(-1), 1396 +/- 73 Mpc, 0.428 +/- 0.066,0.126_-0.010+0.008, 1.19 +/- 0.14} and their covariance matrix as well. The parameters which are not well constrained by our galaxy clustering analysis are marginalized over with wide flat priors. Since no priors from other data sets [i.e. cosmic microwave background (CMB)] are adopted and no dark energy models are assumed, our results from BOSS CMASS galaxy clustering alone may be combined with other data sets, i.e. CMB, SNe, lensing or other galaxy clustering data to constrain the parameters of a given cosmological model. We show that the major power on constraining dark energy from the anisotropic galaxy clustering signal, as compared to the angular-averaged one (monopole), arises from including the normalized growth rate f (z)Sigma(8)(z). In the case of the cosmological model assuming a constant dark energy equation of state and a flat universe (wCDM), our single-probe CMASS constraints, combined with CMB (WMAP9+SPT), yield a value for the dark energy equation-of-state parameter of w = -0.90 +/- 0.11. Therefore, it is important to include f (z)Sigma(8)(z) while investigating the nature of dark energy with current and upcoming large-scale galaxy surveys.
C1 [Chuang, Chia-Hsun; Prada, Francisco] Univ Autonoma Madrid, CSIC, Inst Fis Teor, E-28049 Madrid, Spain.
[Prada, Francisco] Univ Autonoma Madrid, CSIC, E-28049 Madrid, Spain.
[Prada, Francisco] CSIC, Inst Astrofis Andalucia, E-18080 Granada, Spain.
[Cuesta, Antonio J.; Padmanabhan, Nikhil] Yale Univ, Dept Phys, New Haven, CT 06520 USA.
[Eisenstein, Daniel J.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA.
[Kazin, Eyal] Swinburne Univ Technol, Ctr Astrophys & Supercomp, Hawthorn, Vic 3122, Australia.
[Sanchez, Ariel G.] Max Planck Inst Extraterr Phys, D-85741 Garching, Germany.
[Xu, Xiaoying] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA.
[Beutler, Florian; Schlegel, David J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Manera, Marc; Thomas, Daniel] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England.
[Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA.
[Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA.
[Weinberg, David H.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA.
[Weinberg, David H.] Ohio State Univ, CCAPP, Columbus, OH 43210 USA.
[Brinkmann, Jon] Apache Point Observ, Sunspot, NM 88349 USA.
[Brownstein, Joel R.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA.
RP Chuang, CH (reprint author), Univ Autonoma Madrid, CSIC, Inst Fis Teor, E-28049 Madrid, Spain.
EM chuang@nhn.ou.edu
FU Spanish MICINN [MultiDarkCSD2009-00064, AYA201021231- C02-01]; Comunidad
de Madrid [HEPHACOS S2009/ESP-1473]; NASA Office of Space Science; ICG;
SEPNet; University of Portsmouth; Alfred P. Sloan Foundation; National
Science Foundation; U.S. Department of Energy Office of Science;
University of Arizona; Brookhaven National Laboratory; University of
Cambridge; Carnegie Mellon University; University of Florida; Harvard
University; Instituto de Astrofisica de Canarias; Johns Hopkins
University; Lawrence Berkeley National Laboratory; Max Planck Institute
for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New
Mexico State University; New York University; Ohio State University;
Pennsylvania State University; Princeton University; University of
Tokyo; University of Utah; Vanderbilt University; University of
Virginia; University of Washington; Yale University
FX We would like to thank Graeme Addison, Chris Blake, Ryan Keisler, Savvas
Nesseris, Christian Reichardt, Beth Reid, Lado Samushia and Kyle Story
for useful discussions. CC and FP acknowledge support from the Spanish
MICINN Consolider-Ingenio 2010 Programme under grant
MultiDarkCSD2009-00064 andAYA201021231- C02-01 grant. CC and FP were
also supported by the Comunidad de Madrid under grant HEPHACOS
S2009/ESP-1473.; We acknowledge the use of the Legacy Archive for
Microwave Background Data Analysis (LAMBDA). Support for LAMBDA is
provided by the NASA Office of Space Science. The mock catalogues used
were produced in SCIAMA High Performance Supercomputer (HPC) cluster,
supported by the ICG, SEPNet and the University of Portsmouth.; Funding
for SDSS-III has been provided by the Alfred P. Sloan Foundation, the
Participating Institutions, the National Science Foundation and the U.S.
Department of Energy Office of Science. The SDSS-III web site is
http://www.sdss3.org/.; SDSS-III is managed by the Astrophysical
Research Consortium for the Participating Institutions of the SDSS-III
Collaboration including the University of Arizona, the Brazilian
Participation Group, Brookhaven National Laboratory, University of
Cambridge, Carnegie Mellon University, University of Florida, the French
Participation Group, the German Participation Group, Harvard University,
the Instituto de Astrofisica de Canarias, the Michigan State/Notre
Dame/JINA Participation Group, Johns Hopkins University, Lawrence
Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max
Planck Institute for Extraterrestrial Physics, New Mexico State
University, New York University, Ohio State University, Pennsylvania
State University, University of Portsmouth, Princeton University, the
Spanish Participation Group, University of Tokyo, University of Utah,
Vanderbilt University, University of Virginia, University of Washington
and Yale University.
NR 83
TC 34
Z9 34
U1 0
U2 7
PU OXFORD UNIV PRESS
PI OXFORD
PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND
SN 0035-8711
EI 1365-2966
J9 MON NOT R ASTRON SOC
JI Mon. Not. Roy. Astron. Soc.
PD AUG
PY 2013
VL 433
IS 4
BP 3559
EP 3571
DI 10.1093/mnras/stt988
PG 13
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 191IF
UT WOS:000322405900063
ER
PT J
AU Allan, MP
Massee, F
Morr, DK
Van Dyke, J
Rost, AW
Mackenzie, AP
Petrovic, C
Davis, JC
AF Allan, M. P.
Massee, F.
Morr, D. K.
Van Dyke, J.
Rost, A. W.
Mackenzie, A. P.
Petrovic, C.
Davis, J. C.
TI Imaging Cooper pairing of heavy fermions in CeCoIn5
SO NATURE PHYSICS
LA English
DT Article
ID QUASI-PARTICLE INTERFERENCE; SUPERCONDUCTIVITY; CEIRIN5; LATTICE; ORDER
AB The Cooper pairing mechanism of heavy fermion superconductors(1-4), long thought to be due to spin fluctuations(5-7), has not yet been determined. It is the momentum space (k-space) structure of the superconducting energy gap Delta(k) that encodes specifics of this pairing mechanism. However, because the energy scales are so low, it has not been possible to directly measure Delta(k) for any heavy fermion superconductor. Bogoliubov quasiparticle interference imaging(8), a proven technique for measuring the energy gaps of superconductors with high critical temperatures(9-11), has recently been proposed(12) as a new method to measure Delta(k) in heavy fermion superconductors, specifically CeCoIn5 (ref. 13). By implementing this method, we detect a superconducting energy gap whose nodes are oriented along k parallel to (+/- 1; +/- 1)pi/a(0) directions(14-17). Moreover, for the first time in any heavy fermion superconductor, we determine the detailed structure of its multiband energy gaps Delta(i)(k). For CeCoIn5, this information includes: the complex band structure and Fermi surface of the hybridized heavy bands, the fact that largest magnitude Delta(k) opens on a high-k band so that the primary gap nodes occur at unforeseen k-space locations, and that the Bogoliubov quasiparticle interference patterns are most consistent with d(x2-y2) gap symmetry. Such quantitative knowledge of both the heavy band-structure and superconducting gap-structure will be critical in identifying the microscopic pairing mechanism of heavy fermion superconductivity.
C1 [Allan, M. P.; Massee, F.; Petrovic, C.; Davis, J. C.] Brookhaven Natl Lab, CMPMS Dept, Upton, NY 11973 USA.
[Allan, M. P.; Massee, F.; Rost, A. W.; Davis, J. C.] Cornell Univ, Dept Phys, LASSP, Ithaca, NY 14853 USA.
[Allan, M. P.; Rost, A. W.; Mackenzie, A. P.; Davis, J. C.] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland.
[Allan, M. P.] ETH, Dept Phys, CH-8093 Zurich, Switzerland.
[Morr, D. K.; Van Dyke, J.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA.
[Mackenzie, A. P.] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany.
[Davis, J. C.] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA.
RP Morr, DK (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA.
EM dkmorr@uic.edu; jcseamusdavis@gmail.com
RI Allan, Milan/D-7763-2012; Rost, Andreas/F-3004-2011; Petrovic,
Cedomir/A-8789-2009; Mackenzie, Andrew/K-6742-2015; Massee,
Freek/N-2617-2015
OI Allan, Milan/0000-0002-5437-1945; Petrovic, Cedomir/0000-0001-6063-1881;
FU US DOE [DEAC02-98CH10886, DE-FG02-05ER46225]; UK EPSRC; ETH Fellowship
program; Royal Society-Wolfson Award
FX We are particularly grateful to I. Eremin, J. E. Hoffman, D-H. Lee and
A. R. Schmidt for advice and discussions. We acknowledge and thank A.
Akbari, M. Aprili, M. H. Fischer, M. Hamidian, E-A. Kim, S. A. Kivelson,
M. Norman, J. P. Reid, D-H. Lee, D. J. Scalapino and K. Shen for helpful
discussions, advice and communications. Supported by US DOE under
contract number DEAC02-98CH10886 (J.C.D. and C.P.) and under Award No.
DE-FG02-05ER46225 (D. K. M., J. v. D.); by the UK EPSRC under programme
grant 'Topological Protection and Non-equilibrium States in Correlated
Electron Systems' (A.R., A.P.M.); M.P.A. acknowledges support through
the ETH Fellowship program; A.P.M. acknowledges support of a Royal
Society-Wolfson Award.
NR 34
TC 71
Z9 72
U1 10
U2 75
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 1745-2473
J9 NAT PHYS
JI Nat. Phys.
PD AUG
PY 2013
VL 9
IS 8
BP 468
EP 473
DI 10.1038/NPHYS2671
PG 6
WC Physics, Multidisciplinary
SC Physics
GA 193WK
UT WOS:000322592000014
ER
PT J
AU Zhou, BB
Misra, S
Neto, EHD
Aynajian, P
Baumbach, RE
Thompson, JD
Bauer, ED
Yazdani, A
AF Zhou, Brian B.
Misra, Shashank
da Silva Neto, Eduardo H.
Aynajian, Pegor
Baumbach, Ryan E.
Thompson, J. D.
Bauer, Eric D.
Yazdani, Ali
TI Visualizing nodal heavy fermion superconductivity in CeCoIn5
SO NATURE PHYSICS
LA English
DT Article
ID UNCONVENTIONAL SUPERCONDUCTORS; STATES; BI2SR2CACU2O8+DELTA; PSEUDOGAP;
PRECURSOR; MAGNETISM; SYSTEMS
AB Understanding the origin of superconductivity in strongly correlated electron systems continues to be at the forefront of the unsolved problems of physics(1). Among the heavy f-electron systems, CeCoIn5 is one of the most fascinating, as it shares many of the characteristics of correlated d-electron high-T-c cuprate and pnictide superconductors(2-4), including competition between antiferromagnetism and superconductivity(5). Although there has been evidence for unconventional pairing in this compound(6-11), high-resolution spectroscopic measurements of the superconducting state have been lacking. Previously, we have used high-resolution scanning tunnelling microscopy (STM) techniques to visualize the emergence of heavy fermion excitations in CeCoIn5 and demonstrate the composite nature of these excitations well above T-c (ref. 12). Here we extend these techniques to much lower temperatures to investigate how superconductivity develops within a strongly correlated band of composite excitations. We find the spectrum of heavy excitations to be strongly modified just before the onset of superconductivity by a suppression of the spectral weight near the Fermi energy (E-F), reminiscent of the pseudogap state(13,14) in the cuprates. By measuring the response of superconductivity to various perturbations, through both quasiparticle interference (QPI) and local pair-breaking experiments, we demonstrate the nodal d-wave character of superconducting pairing in CeCoIn5.
C1 [Zhou, Brian B.; Misra, Shashank; da Silva Neto, Eduardo H.; Aynajian, Pegor; Yazdani, Ali] Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA.
[Zhou, Brian B.; Misra, Shashank; da Silva Neto, Eduardo H.; Aynajian, Pegor; Yazdani, Ali] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA.
[Baumbach, Ryan E.; Thompson, J. D.; Bauer, Eric D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Yazdani, A (reprint author), Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA.
EM yazdani@princeton.edu
OI Bauer, Eric/0000-0003-0017-1937
FU DOE-BES; Princeton Nanoscale Microscopy Laboratory [NSF-DMR1104612];
NSF-MRSEC program through Princeton Center for Complex Materials
[DMR-0819860]; Linda and Eric Schmidt Transformative Fund; W. M. Keck
Foundation; US Department of Energy, Office of Basic Energy Sciences,
Division of Materials Science and Engineering
FX We thank K. D. Eaton for helpful discussions. The work at Princeton was
primarily supported by a grant from DOE-BES. The instrumentation and
infrastructure at the Princeton Nanoscale Microscopy Laboratory used for
this work were also supported by grants from NSF-DMR1104612, the
NSF-MRSEC program through Princeton Center for Complex Materials
(DMR-0819860), the Linda and Eric Schmidt Transformative Fund, and the
W. M. Keck Foundation. Work at Los Alamos was performed under the
auspices of the US Department of Energy, Office of Basic Energy
Sciences, Division of Materials Science and Engineering.
NR 35
TC 74
Z9 75
U1 8
U2 70
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 1745-2473
EI 1745-2481
J9 NAT PHYS
JI Nat. Phys.
PD AUG
PY 2013
VL 9
IS 8
BP 474
EP 479
DI 10.1038/NPHYS2672
PG 6
WC Physics, Multidisciplinary
SC Physics
GA 193WK
UT WOS:000322592000015
ER
PT J
AU Cao, Y
Waugh, JA
Zhang, XW
Luo, JW
Wang, Q
Reber, TJ
Mo, SK
Xu, Z
Yang, A
Schneeloch, J
Gu, GD
Brahlek, M
Bansal, N
Oh, S
Zunger, A
Dessau, DS
AF Cao, Yue
Waugh, J. A.
Zhang, X-W.
Luo, J-W.
Wang, Q.
Reber, T. J.
Mo, S. K.
Xu, Z.
Yang, A.
Schneeloch, J.
Gu, G. D.
Brahlek, M.
Bansal, N.
Oh, S.
Zunger, A.
Dessau, D. S.
TI Mapping the orbital wavefunction of the surface states in
three-dimensional topological insulators
SO NATURE PHYSICS
LA English
DT Article
ID SINGLE DIRAC CONE; SUPERCONDUCTORS
AB Understanding the structure of the wavefunction is essential for depicting the surface states of a topological insulator. Owing to the inherent strong spin-orbit coupling, the conventional hand-waving picture of the Dirac surface state with a single chiral spin texture is incomplete, as this ignores the orbital components of the Dirac wavefunction and their coupling to the spin textures. Here, by combining orbital-selective angle-resolved photoemission experiments and first-principles calculations, we deconvolve the in-plane and out-of-plane p-orbital components of the Dirac wavefunction. The in-plane orbital wavefunction is asymmetric relative to the Dirac point. It is predominantly tangential (radial) to the k-space constant energy surfaces above (below) the Dirac point. This orbital texture switch occurs exactly at the Dirac point, and therefore should be intrinsic to the topological physics. Our results imply that the Dirac wavefunction has a spin-orbital texture-a superposition of orbital wavefunctions coupled with the corresponding spin textures.
C1 [Cao, Yue; Waugh, J. A.; Wang, Q.; Reber, T. J.; Dessau, D. S.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA.
[Zhang, X-W.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA.
[Zhang, X-W.; Luo, J-W.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Mo, S. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Xu, Z.; Yang, A.; Schneeloch, J.; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
[Brahlek, M.; Bansal, N.; Oh, S.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA.
[Zunger, A.] Univ Colorado, Boulder, CO 80309 USA.
RP Cao, Y (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA.
EM ycao@colorado.edu; Dessau@colorado.edu
RI ZHANG, XIUWEN/K-7383-2012; xu, zhijun/A-3264-2013; Mo,
Sung-Kwan/F-3489-2013; LUO, JUNWEI/B-6545-2013;
OI xu, zhijun/0000-0001-7486-2015; Mo, Sung-Kwan/0000-0003-0711-8514;
Schneeloch, John/0000-0002-3577-9574; Cao, Yue/0000-0002-3989-158X
FU DOE Office of Basic Science [DE-FG02-03ER46066]; NSF [DMR-1007014];
Center for Inverse Design, an Energy Frontier Research Center; US
Department of Energy, Office of Science, Office of Basic Energy Sciences
[DEAC 36-08GO28308]; REMRSEC under NSF [DMR-0820518]; Colorado School of
Mines, Golden, Colorado; IAMDN of Rutgers University, National Science
Foundation [NSF DMR-0845464]; Office of Naval Research [ONR
N000140910749]; DOE [DE-AC03-76SF00098]
FX We acknowledge helpful discussions with S-C. Zhang, S-R. Park, M.
Hermele, A. Essin and G. Chen. The ARPES work was carried out at the
Advanced Light Source, LBL, and was supported by the DOE Office of Basic
Science by grant DE-FG02-03ER46066 and by the NSF under DMR-1007014.
A.Z., X-W.Z. and J-W.L. were supported as part of the Center for Inverse
Design, an Energy Frontier Research Center funded by the US Department
of Energy, Office of Science, Office of Basic Energy Sciences, under
award number DEAC 36-08GO28308. X-W.Z. also acknowledges the
administrative support of REMRSEC under NSF grant number DMR-0820518,
Colorado School of Mines, Golden, Colorado. The Rutgers work was
supported by IAMDN of Rutgers University, National Science Foundation
(NSF DMR-0845464) and Office of Naval Research (ONR N000140910749), and
the Brookhaven work was supported by the DOE under contract number
DE-AC03-76SF00098. Both LBL and BNL are supported by the DOE, Office of
Basic Energy Sciences.
NR 27
TC 42
Z9 42
U1 6
U2 104
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 1745-2473
J9 NAT PHYS
JI Nat. Phys.
PD AUG
PY 2013
VL 9
IS 8
BP 499
EP 504
DI 10.1038/NPHYS2685
PG 6
WC Physics, Multidisciplinary
SC Physics
GA 193WK
UT WOS:000322592000020
ER
PT J
AU Sun, JC
Evrin, C
Samel, SA
Fernandez-Cid, A
Riera, A
Kawakami, H
Stillman, B
Speck, C
Li, HL
AF Sun, Jingchuan
Evrin, Cecile
Samel, Stefan A.
Fernandez-Cid, Alejandra
Riera, Alberto
Kawakami, Hironori
Stillman, Bruce
Speck, Christian
Li, Huilin
TI Cryo-EM structure of a helicase loading intermediate containing
ORC-Cdc6-Cdt1-MCM2-7 bound to DNA
SO NATURE STRUCTURAL & MOLECULAR BIOLOGY
LA English
DT Article
ID REPLICATION ORIGIN RECOGNITION; SACCHAROMYCES-CEREVISIAE; MCM2-7
HELICASE; ATPASE ACTIVITY; CONFORMATIONAL-CHANGES; ELECTRON-MICROSCOPY;
EUKARYOTIC CELLS; PROTEIN COMPLEX; CMG COMPLEX; IN-VITRO
AB In eukaryotes, the Cdt1-bound replicative helicase core MCM2-7 is loaded onto DNA by the ORC-Cdc6 ATPase to form a prereplicative complex (pre-RC) with an MCM2-7 double hexamer encircling DNA. Using purified components in the presence of ATP-gamma S, we have captured in vitro an intermediate in pre-RC assembly that contains a complex between the ORC-Cdc6 and Cdt1-MCM2-7 heteroheptamers called the OCCM. Cryo-EM studies of this 14-subunit complex reveal that the two separate heptameric complexes are engaged extensively, with the ORC-Cdc6 N-terminal AAA+ domains latching onto the C-terminal AAA+ motor domains of the MCM2-7 hexamer. The conformation of ORC-Cdc6 undergoes a concerted change into a right-handed spiral with helical symmetry that is identical to that of the DNA double helix. The resulting ORC-Cdc6 helicase loader shows a notable structural similarity to the replication factor C clamp loader, suggesting a conserved mechanism of action.
C1 [Sun, Jingchuan; Li, Huilin] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA.
[Evrin, Cecile; Samel, Stefan A.; Fernandez-Cid, Alejandra; Riera, Alberto; Speck, Christian] Univ London Imperial Coll Sci Technol & Med, DNA Replicat Grp, MRC, Clin Sci Ctr,Fac Med, London, England.
[Kawakami, Hironori; Stillman, Bruce] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA.
[Li, Huilin] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA.
RP Stillman, B (reprint author), Cold Spring Harbor Lab, POB 100, Cold Spring Harbor, NY 11724 USA.
EM stillman@cshl.edu; chris.speck@csc.mrc.ac.uk; hli@bnl.gov
RI Speck, Christian/G-2882-2011;
OI Speck, Christian/0000-0001-6646-1692; Stillman,
Bruce/0000-0002-9453-4091; Fernandez-Cid, Alejandra/0000-0002-6746-6791
FU US National Institutes of Health [GM45436, GM74985]; United Kingdom
Medical Research Council; Japan Society for the Promotion of Science;
Uehara Memorial Foundation
FX We thank M. Smulczeski and S. Zhang for helping to manually select a
large number of particles from raw cryo-EM micrographs and E. Gardenal
and C. Winkler for the MCM2-7-Cdc6 interaction analysis. This work was
supported by US National Institutes of Health grants GM45436 (to B. S.)
and GM74985 (to H. L.) and the United Kingdom Medical Research Council
(to C. S.). H. K. was supported by Postdoctoral Fellowships for Research
Abroad from the Japan Society for the Promotion of Science and the
Uehara Memorial Foundation.
NR 60
TC 51
Z9 51
U1 0
U2 25
PU NATURE PUBLISHING GROUP
PI NEW YORK
PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA
SN 1545-9993
J9 NAT STRUCT MOL BIOL
JI Nat. Struct. Mol. Biol.
PD AUG
PY 2013
VL 20
IS 8
BP 944
EP +
DI 10.1038/nsmb.2629
PG 10
WC Biochemistry & Molecular Biology; Biophysics; Cell Biology
SC Biochemistry & Molecular Biology; Biophysics; Cell Biology
GA 195PH
UT WOS:000322715300007
PM 23851460
ER
PT J
AU Zhu, XF
Feng, L
Zhang, P
Yin, XB
Zhang, X
AF Zhu, Xuefeng
Feng, Liang
Zhang, Peng
Yin, Xiaobo
Zhang, Xiang
TI One-way invisible cloak using parity-time symmetric transformation
optics
SO OPTICS LETTERS
LA English
DT Article
ID METAMATERIALS; LIGHT
AB We propose a one-way invisible cloak using transformation optics of parity-time (PT) symmetric optical materials. At the spontaneous PT-symmetry breaking point, light is scattered only for incidence along one direction since the phase-matching condition is unidirectionally satisfied, making the cloak one-way invisible. Moreover, optical scattering from the one-way cloak can be further engineered to realize more interesting effects, for example, creating a unidirectional optical illusion of the concealed object. (C) 2013 Optical Society of America
C1 [Zhu, Xuefeng; Feng, Liang; Zhang, Peng; Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA.
[Zhu, Xuefeng] Huazhong Univ Sci & Technol, Wuhan 430074, Hubei, Peoples R China.
[Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, 3112 Etcheverry Hall, Berkeley, CA 94720 USA.
EM xiang@berkeley.edu
RI Zhang, Peng/D-9624-2011; Yin, Xiaobo/A-4142-2011; Feng,
Liang/H-7367-2014; Zhang, Xiang/F-6905-2011
FU US ARO MURI program [W911NF-09-1-0539]; Bird Nest Plan of HUST
FX This work was supported by the US ARO MURI program (W911NF-09-1-0539).
X. F. Zhu acknowledges the financial support from the Bird Nest Plan of
HUST.
NR 24
TC 41
Z9 41
U1 2
U2 52
PU OPTICAL SOC AMER
PI WASHINGTON
PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA
SN 0146-9592
J9 OPT LETT
JI Opt. Lett.
PD AUG 1
PY 2013
VL 38
IS 15
BP 2821
EP 2824
DI 10.1364/OL.38.002821
PG 4
WC Optics
SC Optics
GA 193QM
UT WOS:000322576200057
PM 23903152
ER
PT J
AU Schwaller, P
Tait, TMP
Vega-Morales, R
AF Schwaller, Pedro
Tait, Tim M. P.
Vega-Morales, Roberto
TI Dark matter and vectorlike leptons from gauged lepton number
SO PHYSICAL REVIEW D
LA English
DT Article
ID STANDARD MODEL; BOSON; SYMMETRY; PARTICLE; SEARCH; BARYON; MASS; LHC
AB We investigate a simple model where lepton number is promoted to a local U(1)(L) gauge symmetry which is then spontaneously broken, leading to a viable thermal dark matter (DM) candidate and vectorlike leptons as a byproduct. The dark matter arises as part of the exotic lepton sector required by the need to satisfy anomaly cancellation and is a Dirac electroweak (mostly) singlet neutrino. It is stabilized by an accidental global symmetry of the renormalizable Lagrangian which is preserved even after the gauged lepton number is spontaneously broken and can annihilate efficiently to give the correct thermal relic abundance. We examine the ability of this model to give a viable DM candidate and discuss both direct and indirect detection implications. We also examine some of the LHC phenomenology of the associated exotic lepton sector and in particular its effects on Higgs decays.
C1 [Schwaller, Pedro] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA.
[Schwaller, Pedro] Univ Illinois, Dept Phys, Chicago, IL 60607 USA.
[Tait, Tim M. P.] Univ Calif Irvine, Dept Phys, Irvine, CA 92697 USA.
[Vega-Morales, Roberto] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Vega-Morales, Roberto] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA.
RP Schwaller, P (reprint author), Argonne Natl Lab, HEP Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
FU NSF [PHY-0970171]; University of California, Irvine; Fermilab Graduate
Student Fellowship program; Fermi Research Alliance, LLC
[De-AC02-07CH11359]; U.S. Department of Energy; U.S. Department of
Energy, Division of High Energy Physics [DE-AC02-06CH11357,
DE-FG02-12ER41811]
FX The authors thank Andre de Gouvea, Bogdan Dobrescu, Patrick Fox, Roni
Harnik, Carlos Wagner, and Felix Yu for useful conversations. The
research of T. M. P. T. is supported in part by NSF Grant No.
PHY-0970171 and by the University of California, Irvine through a
Chancellor's fellowship. R. V.-M. is supported by the Fermilab Graduate
Student Fellowship program. This research is also partially supported by
Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with
the U.S. Department of Energy. The work of P. S. is supported in part by
the U.S. Department of Energy, Division of High Energy Physics, under
Grants No. DE-AC02-06CH11357 and No. DE-FG02-12ER41811.
NR 57
TC 13
Z9 13
U1 0
U2 4
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 2470-0010
EI 2470-0029
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 1
PY 2013
VL 88
IS 3
AR 035001
DI 10.1103/PhysRevD.88.035001
PG 15
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 195TF
UT WOS:000322725800001
ER
PT J
AU Lazerson, SA
Chapman, IT
AF Lazerson, S. A.
Chapman, I. T.
TI STELLOPT modeling of the 3D diagnostic response in ITER
SO PLASMA PHYSICS AND CONTROLLED FUSION
LA English
DT Article; Proceedings Paper
CT 17th Annual Workshop on Magnetohydrodynamic (MHD) Stability Control -
Addressing the Disruption Challenge for ITER
CY NOV 05-07, 2012
CL Columbia Univ, New York, NY
HO Columbia Univ
ID EQUILIBRIUM
AB The ITER three-dimensional (3D) diagnostic response to an n = 3 resonant magnetic perturbation (RMP) is modeled using the STELLOPT code. The in-vessel coils apply a RMP field which generates a 4 cm edge displacement from axisymmetry as modeled by the VMEC 3D equilibrium code. Forward modeling of flux loop and magnetic probe response with the DIAGNO code indicates up to 20% changes in measured plasma signals. Simulated LIDAR measurements of electron temperature indicate 2 cm shifts on the low-field side of the plasma. This suggests that the ITER diagnostic will be able to diagnose the 3D structure of the equilibria.
C1 [Lazerson, S. A.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Chapman, I. T.] EURATOM CCFE Fus Assoc Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England.
RP Lazerson, SA (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM lazerson@pppl.gov
RI Lazerson, Samuel/E-4816-2014
OI Lazerson, Samuel/0000-0001-8002-0121
NR 19
TC 10
Z9 10
U1 0
U2 7
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0741-3335
J9 PLASMA PHYS CONTR F
JI Plasma Phys. Control. Fusion
PD AUG
PY 2013
VL 55
IS 8
AR 084004
DI 10.1088/0741-3335/55/8/084004
PG 7
WC Physics, Fluids & Plasmas
SC Physics
GA 195LB
UT WOS:000322702700005
ER
PT J
AU Sassenberg, K
Richardson, AS
Brennan, DP
Finn, JM
AF Sassenberg, K.
Richardson, A. S.
Brennan, D. P.
Finn, J. M.
TI Control of magnetohydrodynamic modes in reversed field pinches with
normal and tangential magnetic field sensing and two resistive walls
SO PLASMA PHYSICS AND CONTROLLED FUSION
LA English
DT Article; Proceedings Paper
CT 17th Annual Workshop on Magnetohydrodynamic (MHD) Stability Control -
Addressing the Disruption Challenge for ITER
CY NOV 05-07, 2012
CL Columbia Univ, New York, NY
HO Columbia Univ
ID POLOIDAL CURRENT DRIVE; ACTIVE MHD CONTROL; FEEDBACK-CONTROL; HELICITY
STATES; EXTRAP T2R; RFX-MOD; SINGLE; PARADIGM; PLASMAS; TORUS
AB Numerical results are presented on control of magnetohydrodynamic (MHD) modes in reversed field pinches (RFPs) for a geometry with two resistive walls. We use measurements of the normal component of the magnetic field and introduce the use of both tangential components. In Richardson et al (2010 Phys. Plasmas 17 112511), RFP control studies were performed sensing the radial (normal) component of the magnetic field and a single tangential component just inside the wall, showing that it is possible to stabilize the MHD modes in an RFP for current up to the ideal plasma-ideal wall limit in that configuration. Here, we extend our modeling by including two resistive walls, in a configuration relevant to experiments such as RFX-mod, and measuring all three magnetic field components, i.e. including a second tangential component, as an exploratory effort. We present our study incrementally, starting with a single resistive wall, and conclude that with the first tangential sensor located inside the wall, the plasma can be stabilized up to the ideal plasma-ideal wall limit, as in Richardson et al. With the first tangential sensor outside the wall, stabilization is possible only up to the ideal wall-resistive plasma (tearing) limit. We then show that for experimentally relevant parameters the thin-wall approximation is indeed valid for the MHD modes of interest but invalid for the high-frequency magnetosonic mode (Richardson et al) driven by the (first) tangential component feedback. In fact, when a thick-wall formulation with realistic parameters is considered, the high-frequency magnetosonic mode is found to be destabilized only for a very high gain parameter, and we conclude that this mode can be ignored for an experimentally relevant analysis. Consequently, the plasma can be stabilized in a much larger region of feedback gain parameter space than found in Richardson et al. In the presence of two walls, with the first tangential component measured just outside the inner wall and with RFX-mod relevant time constants, we show that feedback control can stabilize the plasma at currents much larger than the ideal wall-resistive plasma limit. The current limit is still less, however, than the ideal plasma-ideal wall limit. Use of the second tangential component appears in all cases to lead to significantly different but not necessarily improved feedback stabilization. These results may lead to better understanding and improved stability properties in current-day RFP experiments through robust access to quasi-single-helicity states.
C1 [Sassenberg, K.; Brennan, D. P.] Univ Tulsa, Dept Phys, Tulsa, OK 74104 USA.
[Richardson, A. S.] Naval Res Lab, Washington, DC 20375 USA.
[Finn, J. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Sassenberg, K (reprint author), Univ Tulsa, Dept Phys, Tulsa, OK 74104 USA.
EM dylan-brennan@utulsa.edu
OI Richardson, Andrew/0000-0002-3056-6334
NR 31
TC 2
Z9 2
U1 0
U2 2
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0741-3335
J9 PLASMA PHYS CONTR F
JI Plasma Phys. Control. Fusion
PD AUG
PY 2013
VL 55
IS 8
AR 084002
DI 10.1088/0741-3335/55/8/084002
PG 19
WC Physics, Fluids & Plasmas
SC Physics
GA 195LB
UT WOS:000322702700003
ER
PT J
AU Green, MA
Emery, K
Hishikawa, Y
Warta, W
Dunlop, ED
AF Green, Martin A.
Emery, Keith
Hishikawa, Yoshihiro
Warta, Wilhelm
Dunlop, Ewan D.
TI Solar cell efficiency tables (version 42)
SO PROGRESS IN PHOTOVOLTAICS
LA English
DT Article
DE solar cell efficiency; photovoltaic efficiency; energy conversion
efficiency
ID MULTICRYSTALLINE; CONCENTRATOR; STABILITY; MODULE
AB Consolidated tables showing an extensive listing of the highest independently confirmed efficiencies for solar cells and modules are presented. Guidelines for inclusion of results into these tables are outlined, and new entries since January 2013 are reviewed. Copyright (c) 2013 John Wiley & Sons, Ltd.
C1 [Green, Martin A.] Univ New S Wales, Australian Ctr Adv Photovolta, Sydney, NSW 2052, Australia.
[Emery, Keith] Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Hishikawa, Yoshihiro] Natl Inst Adv Ind Sci & Technol, Res Ctr Photovolta RCPV, Tsukuba, Ibaraki 3058568, Japan.
[Warta, Wilhelm] Fraunhofer Inst Solar Energy Syst, Solar Cells Mat & Technol Dept, D-79110 Freiburg, Germany.
[Dunlop, Ewan D.] European Commiss Joint Res Ctr, Renewable Energy Unit, Inst Energy, IT-21027 Ispra, Italy.
RP Green, MA (reprint author), Univ New S Wales, Australian Ctr Adv Photovolta, Sydney, NSW 2052, Australia.
EM m.green@unsw.edu.au
FU Australian Renewable Energy Agency
FX The Australian Centre for Advanced Photovoltaics commenced operation in
2013 with support from the Australian Renewable Energy Agency.
NR 45
TC 318
Z9 319
U1 9
U2 269
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1062-7995
J9 PROG PHOTOVOLTAICS
JI Prog. Photovoltaics
PD AUG
PY 2013
VL 21
IS 5
BP 827
EP 837
DI 10.1002/pip.2404
PG 11
WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied
SC Energy & Fuels; Materials Science; Physics
GA 186AF
UT WOS:000322012700002
ER
PT J
AU Peshek, TJ
Zhang, L
Singh, RK
Tang, ZZ
Vahidi, M
To, B
Coutts, TJ
Gessert, TA
Newman, N
van Schilfgaarde, M
AF Peshek, Timothy J.
Zhang, Lei
Singh, Rakesh K.
Tang, ZhiZhong
Vahidi, Mahmoud
To, Bobby
Coutts, Timothy J.
Gessert, Timothy A.
Newman, Nathan
van Schilfgaarde, Mark
TI Criteria for improving the properties of ZnGeAs2 solar cells
SO PROGRESS IN PHOTOVOLTAICS
LA English
DT Article
DE ZnGeAs2; chalcopyrites; earth-abundant; photovoltaics; pulsed laser
deposition; solar cell
ID GROWTH
AB We explore the potential utility of the II-IV-V semiconductor ZnGeAs2 as the absorber material in solar cells. As-deposited ZnGeAs2 films prepared by pulsed laser deposition are amorphous because of the limited substrate temperature that can be used without the rapid loss of volatile Zn and As. Thermal processing above 450 degrees C results in crystallization and improved electrical properties with hole mobilities as high as 58cm(2)/Vs. The annealed films were used to fabricate p-type ZnGeAs2: n-type CdS cells on SnO2-buffered borosilicate glass substrates in the so-called superstrate geometry. Light-induced currents of up to similar to 2mA/cm(2) and open-circuit voltages of up to 470mV were observed using backside illumination, indicating that these nascent devices hold potential for realizing high performance solar cells from earth-abundant elements. The performance of the devices fabricated to-date is degraded by conduction through shorts resulting from the presence of micron-sized pinholes in the absorber layer. Copyright (c) 2012 John Wiley & Sons, Ltd.
C1 [Peshek, Timothy J.; Zhang, Lei; Singh, Rakesh K.; Tang, ZhiZhong; Vahidi, Mahmoud; Newman, Nathan; van Schilfgaarde, Mark] Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA.
[Peshek, Timothy J.; To, Bobby; Coutts, Timothy J.; Gessert, Timothy A.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Peshek, Timothy J.] LLC, eQED, Mayfield Village, OH 44143 USA.
RP Peshek, TJ (reprint author), LLC, eQED, Mayfield Village, OH 44143 USA.
EM tpeshek@asu.edu
RI Newman, Nathan/E-1466-2011
OI Newman, Nathan/0000-0003-2819-9616
FU DOE-EERE [DE-FG36-08GO18002]
FX The authors would like to recognize the LeRoy Eyring Center for Solid
State Science at Arizona State University and the National Center for
Photovoltaics at the National Renewable Energy Laboratory for facilities
to make this work possible. This project was supported by DOE-EERE grant
DE-FG36-08GO18002.
NR 21
TC 6
Z9 6
U1 0
U2 16
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1062-7995
J9 PROG PHOTOVOLTAICS
JI Prog. Photovoltaics
PD AUG
PY 2013
VL 21
IS 5
BP 906
EP 917
DI 10.1002/pip.2177
PG 12
WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied
SC Energy & Fuels; Materials Science; Physics
GA 186AF
UT WOS:000322012700010
ER
PT J
AU Cruz-Campa, JL
Nielson, GN
Resnick, PJ
Okandan, M
Young, R
Zubia, D
Gupta, V
AF Cruz-Campa, Jose L.
Nielson, Gregory N.
Resnick, Paul J.
Okandan, Murat
Young, Ralph
Zubia, David
Gupta, Vipin
TI Ultrathin and micro-sized solar cell performance optimization via
simulations
SO PROGRESS IN PHOTOVOLTAICS
LA English
DT Article
DE solar cell simulation; ultrathin solar cell; microsystems-enabled
photovoltaics; miniature solar cells; optimization solar cells
AB Back-contacted, ultrathin (<10 mu m), and submillimeter-sized solar cells made with microsystem tools are a new type of cell that has not been optimized for performance. The literature reports efficiencies up to 15% using thicknesses of 14 mu m and cell sizes of 250 mu m. In this paper, we present the design, conditions, and fabrication parameters necessary to optimize these devices. The optimization was performed using commercial simulation tools from the microsystems arena. A systematic variation of the different parameters that influence the performance of the cell was accomplished. The researched parameters were resistance, Shockley-Read-Hall (SRH) lifetime, contact separation, implant characteristics (size, dosage, energy, and ratio between the species), contact size, substrate thickness, surface recombination, and light concentration. The performance of the cell was measured with efficiency, open-circuit voltage, and short-circuit current. Among all the parameters investigated, surface recombination and SRH lifetime proved to be the most important. Through completing the simulations, an optimized concept solar cell design was introduced for two scenarios: high and low quality materials/passivation. Simulated efficiencies up to 23.4% (1sun) and 26.7% (100suns) were attained for 20-mu m-thick devices. Copyright (c) 2012 John Wiley & Sons, Ltd.
C1 [Cruz-Campa, Jose L.; Nielson, Gregory N.; Resnick, Paul J.; Okandan, Murat] Sandia Natl Labs, MEMS Technol, Albuquerque, NM 87185 USA.
[Young, Ralph] Sandia Natl Labs, Rad Hard CMOS Technol, Albuquerque, NM 87185 USA.
[Zubia, David] Univ Texas El Paso, El Paso, TX 79968 USA.
[Cruz-Campa, Jose L.; Gupta, Vipin] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Cruz-Campa, JL (reprint author), Sandia Natl Labs, POB 5800,MS 1080, Albuquerque, NM 87185 USA.
EM jlcruzc@sandia.gov
FU US Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]; DOE Solar Energy Technology Program Seed Fund
FX Sandia National Laboratories is a multi-program laboratory managed and
operated by Sandia Corporation, a wholly owned subsidiary of Lockheed
Martin Corporation, for the US Department of Energy's National Nuclear
Security Administration under contract DE-AC04-94AL85000. This work was
sponsored by the DOE Solar Energy Technology Program Seed Fund.
NR 15
TC 3
Z9 3
U1 1
U2 19
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1062-7995
J9 PROG PHOTOVOLTAICS
JI Prog. Photovoltaics
PD AUG
PY 2013
VL 21
IS 5
BP 1114
EP 1126
DI 10.1002/pip.2214
PG 13
WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied
SC Energy & Fuels; Materials Science; Physics
GA 186AF
UT WOS:000322012700030
ER
PT J
AU Gray, MF
Zalupski, P
Nilsson, M
AF Gray, Michael F.
Zalupski, Peter
Nilsson, Mikael
TI Determination of Activity Coefficients of di-(2-ethylhexyl) Phosphoric
Acid Dimer in Select Organic Solvents Using Vapor Phase Osmometry
SO SOLVENT EXTRACTION AND ION EXCHANGE
LA English
DT Article
DE di-(2-ethylhexyl) phosphoric acid; vapor pressure osmometry; activity
coefficients; solubility parameters
ID PRESSURE OSMOMETRY; REFERENCE SOLUTES; SELF-ASSOCIATION; EXTRACTANTS;
OCTYLAMINE; BENZENE; SYSTEMS
AB Effective models for solvent extraction require accurate characterization of the nonideality effects for each component, including the extractants. In this study, the nonideal behavior of the industrial extractant di(2-ethylhexyl) phosphoric acid has been investigated using vapor pressure osmometry (VPO). From the osmometry data, activity coefficients for the HDEHP dimer were obtained based on a formulation of the regular solution theory of Scatchard and Hildebrand, and the Margules two- and three-suffix equations. The results show similarity with a slope-analysis based relation from previous literature, although important differences are highlighted. The work points towards VPO as a useful technique for this type of study, but care must be taken with the choice of standard and method of analysis.
C1 [Gray, Michael F.; Nilsson, Mikael] Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92697 USA.
[Zalupski, Peter] Idaho Natl Lab, Dept Aqueous Separat & Radiochem, Idaho Falls, ID 83415 USA.
RP Nilsson, M (reprint author), Univ Calif Irvine, Dept Chem Engn & Mat Sci, 916 Engn Tower, Irvine, CA 92697 USA.
EM nilssonm@uci.edu
FU Idaho National Laboratory, Fuel Cycle Research and Development program
(FCR&D), U.S. DOE, Office of Nuclear Energy; [107827]
FX Work was supported under subcontract number 107827 with the Idaho
National Laboratory, Fuel Cycle Research and Development program
(FCR&D), U.S. DOE, Office of Nuclear Energy.
NR 23
TC 0
Z9 0
U1 2
U2 17
PU TAYLOR & FRANCIS INC
PI PHILADELPHIA
PA 325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA
SN 0736-6299
J9 SOLVENT EXTR ION EXC
JI Solvent Extr. Ion Exch.
PD AUG 1
PY 2013
VL 31
IS 5
BP 550
EP 563
DI 10.1080/07366299.2013.785870
PG 14
WC Chemistry, Multidisciplinary
SC Chemistry
GA 194FC
UT WOS:000322615400006
ER
PT J
AU Genc, A
Kovarik, L
Gu, M
Cheng, HK
Plachinda, P
Pullan, L
Freitag, B
Wang, CM
AF Genc, Arda
Kovarik, Libor
Gu, Meng
Cheng, Huikai
Plachinda, Paul
Pullan, Lee
Freitag, Bert
Wang, Chongmin
TI XEDS STEM tomography for 3D chemical characterization of nanoscale
particles
SO ULTRAMICROSCOPY
LA English
DT Article
DE Tomography; XEDS; STEM; Silicon drift detector; Li ion battery; 3D
chemical mapping; Li1.2Ni0.2Mn0.6O2
ID SPECTROSCOPIC TOMOGRAPHY; RUTHERFORD SCATTERING; ELECTRON TOMOGRAPHY;
EFTEM TOMOGRAPHY; Z-CONTRAST; FIB
AB We present a tomography technique which couples scanning transmission electron microscopy (STEM) and X-ray energy dispersive spectrometry (XEDS) to resolve 3D distribution of elements in nanoscale materials. STEM imaging when combined with XEDS mapping using a symmetrically arranged XEDS detector design around the specimen overcomes many of the obstacles in 3D chemical imaging of nanoscale materials and successfully elucidates the 3D chemical information in a large field of view of the transmission electron microscopy (TEM) sample. We employed this technique to investigate 3D distribution of Nickel (Ni), Manganese (Mn) and Oxygen (0) in a Li1.2Ni0.2Mn0.6O2 (LNMO) nanoparticle used as a cathode material in Lithium (Li) ion batteries. For this purpose, 2D elemental maps were acquired for a range of tilt angles and reconstructed to obtain 3D elemental distribution in an isolated LNMO nanoparticle. The results highlight the strength of this technique in 3D chemical analysis of nanoscale materials by successfully resolving Ni, Mn and 0 elemental distributions in 3D and discovering the new phenomenon of Ni surface segregation in this material. Furthermore, the comparison of simultaneously acquired high angle annular dark field (HAADF) STEM and XEDS STEM tomography results shows that XEDS STEM tomography provides additional 3D chemical information of the material especially when there is low atomic number (Z) contrast in the material of interest. (C) 2013 Elsevier BY. All rights reserved.
C1 [Genc, Arda; Cheng, Huikai; Plachinda, Paul; Pullan, Lee] FEI Co, Hillsboro, OR 97124 USA.
[Kovarik, Libor; Gu, Meng; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
[Freitag, Bert] FEI Co, NL-5600 KA Eindhoven, Netherlands.
RP Genc, A (reprint author), FEI Co, 5350 NE Dawson Creek Dr, Hillsboro, OR 97124 USA.
EM arda.genc@fei.com
RI Gu, Meng/B-8258-2013; Kovarik, Libor/L-7139-2016;
OI Kovarik, Libor/0000-0002-2418-6925
FU DOE's Office of Biological and Environmental Research; DOE
[DE-AC05-76RLO1830]
FX The authors would like to thank Dr. Dapeng Wang, Bias Belharouak and
Khalil Amine at Argonne National Laboratory for the sample synthesis.
Research described in this paper is part of the Chemical Imaging
Initiative at Pacific Northwest National Laboratory. It was conducted
under the Laboratory Directed Research and Development Program at PNNL,
a multiprogram national laboratory operated by Battelle for the U.S.
Department of Energy. Part of the work was conducted in the William R.
Wiley Environmental Molecular Sciences Laboratory (EMSL), a national
scientific user facility sponsored by DOE's Office of Biological and
Environmental Research and located at PNNL. PNNL is operated by Battelle
for the DOE under Contract DE-AC05-76RLO1830.
NR 23
TC 33
Z9 34
U1 3
U2 96
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0304-3991
J9 ULTRAMICROSCOPY
JI Ultramicroscopy
PD AUG
PY 2013
VL 131
BP 24
EP 32
DI 10.1016/j.ultramic.2013.03.023
PG 9
WC Microscopy
SC Microscopy
GA 194KG
UT WOS:000322631200003
PM 23676452
ER
PT J
AU Passian, A
Tetard, L
Thundat, T
AF Passian, Ali
Tetard, Laurene
Thundat, Thomas
TI Comments on the paper "A comprehensive modeling and vibration analysis
of AFM microcantilevers subjected to nonlinear tip-sample interaction
forces" by Sohrab Eslami and Nader Jalili
SO ULTRAMICROSCOPY
LA English
DT Editorial Material
DE Microscopy; AFM; MSAFM; Imaging; Nonlinear dynamics; Nanomechanical
forces
ID MICROSCOPY; HOLOGRAPHY
AB This comment on the paper "A comprehensive modeling and vibration analysis of AFM microcantilevers subjected to nonlinear tip-sample interaction forces" by Sohrab Eslami and Jalili (2012)[1] aims to: (1) discuss and elucidate the concept of "virtual resonance" and thus (2) avert a misinterpretation of the experimental results and findings reported in the Tetard et al. Physical Review Letters 106, 180801 (2011) [2]. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Passian, Ali; Tetard, Laurene] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA.
[Passian, Ali] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA.
[Passian, Ali] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA.
[Thundat, Thomas] Univ Alberta, Dept Chem & Mat Engn, Edmonton, AB T6G 2V4, Canada.
RP Passian, A (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA.
EM passianan@ornl.gov
NR 15
TC 0
Z9 0
U1 2
U2 21
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0304-3991
J9 ULTRAMICROSCOPY
JI Ultramicroscopy
PD AUG
PY 2013
VL 131
BP 92
EP 93
DI 10.1016/j.ultramic.2013.03.016
PG 2
WC Microscopy
SC Microscopy
GA 194KG
UT WOS:000322631200010
PM 23735319
ER
PT J
AU Tu, QC
He, ZL
Deng, Y
Zhou, JH
AF Tu, Qichao
He, Zhili
Deng, Ye
Zhou, Jizhong
TI Strain/Species-Specific Probe Design for Microbial Identification
Microarrays
SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY
LA English
DT Article
ID FUNCTIONAL GENE MICROARRAYS; OLIGONUCLEOTIDE DESIGN; COMMUNITY
COMPOSITION; CRITERIA
AB Specific identification of microorganisms in the environment is important but challenging, especially at the species/strain level. Here, we have developed a novel k-mer-based approach to select strain/species-specific probes for microbial identification with diagnostic microarrays. Application of this approach to human microbiome genomes showed that multiple (>= 10 probes per strain) strain-specific 50-mer oligonucleotide probes could be designed for 2,012 of 3,421 bacterial strains of the human microbiome, and species-specific probes could be designed for most of the other strains. The method can also be used to select strain/species-specific probes for sequenced genomes in any environments, such as soil and water.
C1 [Tu, Qichao; He, Zhili; Deng, Ye; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA.
[Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China.
RP Zhou, JH (reprint author), Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA.
EM zhili.he@ou.edu; jzhou@ou.edu
OI ?, ?/0000-0002-7584-0632
FU Ecosystems and Networks Integrated with Genes and Molecular Assemblies
(ENIGMA) [DE-AC02-05CH11231]; Oklahoma Center for the Advancement of
Science and Technology (OCAST) through Oklahoma Applied Research Support
(OARS) project [AR11-035]
FX This work was supported by Ecosystems and Networks Integrated with Genes
and Molecular Assemblies (ENIGMA) under contract no. DE-AC02-05CH11231
and by the Oklahoma Center for the Advancement of Science and Technology
(OCAST) through Oklahoma Applied Research Support (OARS) project
AR11-035.
NR 18
TC 5
Z9 5
U1 2
U2 20
PU AMER SOC MICROBIOLOGY
PI WASHINGTON
PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA
SN 0099-2240
J9 APPL ENVIRON MICROB
JI Appl. Environ. Microbiol.
PD AUG
PY 2013
VL 79
IS 16
BP 5085
EP 5088
DI 10.1128/AEM.01124-13
PG 4
WC Biotechnology & Applied Microbiology; Microbiology
SC Biotechnology & Applied Microbiology; Microbiology
GA 187ZV
UT WOS:000322161700037
PM 23747703
ER
PT J
AU Lee, JC
Xu, Y
Huber, GW
AF Lee, Jechan
Xu, Ye
Huber, George W.
TI High-throughput screening of monometallic catalysts for aqueous-phase
hydrogenation of biomass-derived oxygenates
SO APPLIED CATALYSIS B-ENVIRONMENTAL
LA English
DT Article
DE Aqueous-phase hydrogenation; Aqueous-phase hydrogenolysis; Binding
energy; Biomass conversion; Heterogeneous catalysts; High-throughput
ID SUPPORTED METAL-CATALYSTS; ETHYLENE-GLYCOL; HETEROGENEOUS CATALYSIS;
RUTHENIUM CATALYST; LIQUID ALKANES; PD; HYDROCARBONS; KINETICS; XYLOSE;
CO
AB The initial reaction rates on a per site basis for aqueous-phase hydrogenation (APH) of different oxygenated compounds: including acetaldehyde, propanal, acetone, xylose, furfural, and furfuryl alcohol and aqueous-phase hydrogenolysis of tetrahydrofurfuryl alcohol (THFA) and xylitol were measured over various alumina-supported monometallic catalysts (Pd, Pt, Ru, Rh, Ni, and Co) in a high-throughput reactor. These oxygenated compounds have the same functionality that is found in aqueous solutions derived from biomass including pyrolysis oils and aqueous hydrolysis solutions. The initial rate of APH of the different carbonyls groups was dependent on the functionality of the feed molecule and catalyst used. Ru was the most active metal for APH of acetaldehyde, propanal, acetone, and xylose. Pd was the most active metal for APH of furfural and furfuryl alcohol. Only Pt and Ni catalysts were able to produce 1,2-pentanediol and 1,5-pentanediol from aqueous-phase hydrogenolysis of THFA. Ru was active for conversion of THFA but only made coke. The initial activity for aqueous-phase hydrogenolysis of xylitol decreased in the order of Ru > Co > Pt > Ni >= Pd. The initial rates of APH of carbonyl groups (C=O bond) measured in this study decreased in the order: hydrogenation of acetone > hydrogenation of acetaldehyde and propanal > hydrogenation of xylose > hydrogenation of furfural. The initial rates of aqueous-phase hydrogenolysis of THFA and xylitol were much lower than the initial rate for APH of C=O and C=C bonds. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Lee, Jechan; Huber, George W.] Univ Massachusetts, Dept Chem Engn, Amherst, MA 01003 USA.
[Xu, Ye] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
RP Huber, GW (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, 1415 Engn Dr, Madison, WI 53706 USA.
EM huber@engr.wisc.edu
RI Xu, Ye/B-5447-2009; Lee, Jechan/J-1229-2016
OI Xu, Ye/0000-0002-6406-7832; Lee, Jechan/0000-0002-9759-361X
FU Catalysis Center for Energy Innovation, an Energy Frontier Research
Center; U.S. Department of Energy, Office of Science, Office of Basic
Energy Sciences [DE-SC0001004]; Scientific User Facilities Division,
Office of Basic Energy Sciences, U.S. Department of Energy; US-DOE
Office of Science [DE-AC02-05CH11231]
FX This work was supported as part of the Catalysis Center for Energy
Innovation, an Energy Frontier Research Center funded by the U.S.
Department of Energy, Office of Science, Office of Basic Energy Sciences
under Award Number DE-SC0001004. Theoretical work was performed at the
Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge
National Laboratory by the Scientific User Facilities Division, Office
of Basic Energy Sciences, U.S. Department of Energy, and used computing
resources of the National Energy Research Scientific Computing Center,
which is supported by US-DOE Office of Science under Contract
DE-AC02-05CH11231.
NR 86
TC 44
Z9 44
U1 22
U2 226
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0926-3373
J9 APPL CATAL B-ENVIRON
JI Appl. Catal. B-Environ.
PD AUG-SEP
PY 2013
VL 140
BP 98
EP 107
DI 10.1016/j.apcatb.2013.03.031
PG 10
WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical
SC Chemistry; Engineering
GA 185ST
UT WOS:000321991300012
ER
PT J
AU Ji, YY
Toops, TJ
Crocker, M
AF Ji, Yaying
Toops, Todd. J.
Crocker, Mark
TI Isocyanate formation and reactivity on a Ba-based LNT catalyst studied
by DRIFTS
SO APPLIED CATALYSIS B-ENVIRONMENTAL
LA English
DT Article
DE NOx reduction; Isocyanate; Ba nitrate; Carbon monoxide; Hydrolysis;
Isotopic labeling
ID NOX TRAP CATALYSTS; STORED NOX; REDUCTION CATALYST; NITROGEN-OXIDES;
REDUCING AGENT; NH3 FORMATION; STORAGE; H-2; REGENERATION; CO
AB Diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) and mass spectrometry (MS), coupled with the use of isotopically-labeled reactants ((NO)-N-15-O-18 and (CO)-C-13), were employed to study the formation of isocyanate species during NOx reduction with CO, as well as isocyanate reactivity toward typical exhaust gas components. DRIFTS demonstrated that both Ba-NCO and Al-NCO were simultaneously formed during NOx reduction by CO under dry lean-rich cycling conditions. The Ba-NCO band was more intense than that of Al-NCO, and became comparatively stronger at high temperatures. During rich purging at 300 and 400 degrees C, a near linear relationship was found between the increase in Ba-NCO band intensity and the decrease in Ba-NO3 band intensity, suggesting that Ba-NCO is directly derived from the reaction of Ba nitrate with CO. Both temperature-programmed surface reaction (TPSR) and isothermal reaction modes (ISR) were utilized to study the reactivity of isocyanate species under lean conditions. Simultaneous DRIFTS and mass spectrometric measurements during TPSR indicated that isocyanate reaction with H2O, O-2, NO and NO/O-2 took place almost immediately the temperature was raised above 100 degrees C, and that all NCO species were removed below 300 degrees C. The evolution of the NCO IR bands during ISR at 350 degrees C demonstrated that the kinetics of NCO hydrolysis are fast, although a delay in N-2 formation indicated that N-2 is not the initial product of the reaction. In contrast, immediate N-2 evolution was observed during NCO reaction with O-2 and with NO + O-2. Overall, it can be inferred that under dry cycling conditions with CO as the sole reductant, N-2 is mainly generated via NCO reaction with NO/O-2 after the switch to lean conditions, rather than being evolved during the rich phase. However, in the presence of water, isocyanate undergoes rapid hydrolysis in the rich phase, N-2 generation proceeding via NH3. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Ji, Yaying; Crocker, Mark] Univ Kentucky, Ctr Appl Energy Res, Lexington, KY 40511 USA.
[Toops, Todd. J.] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Knoxville, TN 37932 USA.
RP Crocker, M (reprint author), Univ Kentucky, Ctr Appl Energy Res, 3572 Iron Works Pike, Lexington, KY 40511 USA.
EM mark.crocker@uky.edu
FU U.S. Department of Energy (DOE) [DE-EE0000205, DE-AC05-00OR22725]
FX This project was funded by the U.S. Department of Energy (DOE) under
award number DE-EE0000205. Oak Ridge National Laboratory is managed by
UT-Battelle, LLC, for the U.S. Department of Energy under contract
number DE-AC05-00OR22725.
NR 33
TC 8
Z9 8
U1 2
U2 23
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0926-3373
J9 APPL CATAL B-ENVIRON
JI Appl. Catal. B-Environ.
PD AUG-SEP
PY 2013
VL 140
BP 265
EP 275
DI 10.1016/j.apcatb.2013.04.017
PG 11
WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical
SC Chemistry; Engineering
GA 185ST
UT WOS:000321991300031
ER
PT J
AU Jung, HB
Um, W
AF Jung, Hun Bok
Um, Wooyong
TI Experimental study of potential wellbore cement carbonation by various
phases of carbon dioxide during geologic carbon sequestration
SO APPLIED GEOCHEMISTRY
LA English
DT Article
ID WET SUPERCRITICAL CO2; DEGRADATION; FORSTERITE; AQUIFERS; IMPACTS
AB Hydrated Portland cement was reacted with CO2 in supercritical, gaseous and aqueous phases to understand the potential cement alteration processes along the length of a wellbore, extending from a deep CO2 storage reservoir to the shallow subsurface during geologic carbon sequestration. The 3-D X-ray microtomography (XMT) images showed that the cement alteration was significantly more extensive with CO2-saturated synthetic groundwater than dry or wet supercritical CO2 at high P (10 MPa)-T (50 degrees C) conditions. Scanning electron microscopy with energy dispersive spectroscopy (SEM-EDS) analysis also exhibited a systematic Ca depletion and C enrichment in cement matrix exposed to CO2-saturated groundwater. Integrated XMT, XRD and SEM-EDS analyses identified the formation of an extensive carbonated zone filled with CaCO3(s), as well as a porous degradation front and an outermost silica-rich zone in cement after exposure to CO2-saturated groundwater. Cement alteration by CO2-saturated groundwater for 2-8 months overall decreased the porosity from 31% to 22% and the permeability by an order of magnitude. Cement alteration by dry or wet supercritical CO2 was slow and minor compared to CO2-saturated groundwater. A thin single carbonation zone was formed in cement after exposure to wet supercritical CO2 for 8 months or dry supercritical CO2 for 15 months. An extensive calcite coating was formed on the outside surface of a cement sample after exposure to wet gaseous CO2 for 1-3 months. The chemical-physical characterization of hydrated Portland cement after exposure to various phases of CO2 indicates that the extent of cement carbonation can be significantly heterogeneous depending on the CO2 phase present in the wellbore environment. Both experimental and geochemical modeling results suggest that wellbore cement exposure to supercritical, gaseous and aqueous phases of CO2 during geologic C sequestration is unlikely to damage the wellbore integrity because cement alteration by all phases of CO2 is dominated by carbonation reactions. This is consistent with previous field studies of wellbore cement with extensive carbonation after exposure to CO2 for three decades. However, XMT imaging indicates that preferential cement alteration by supercritical CO2 or CO2-saturated groundwater can occur along the cement-steel or cement-rock interfaces. This highlights the importance of further investigation of cement degradation along the interfaces of wellbore materials to ensure permanent geologic carbon storage. Published by Elsevier Ltd.
C1 [Jung, Hun Bok; Um, Wooyong] Pacific NW Natl Lab, Richland, WA 99354 USA.
RP Um, W (reprint author), Pacific NW Natl Lab, POB 999,P7-54,902 Battelle Blvd, Richland, WA 99354 USA.
EM wooyong.um@pnnl.gov
FU National Risk Assessment Partnership (NRAP) in the US Department of
Energy Office of Fossil Energy's Carbon Sequestration Program; US DOE
[DE-AC06-76RLO 1830]
FX The authors are grateful to Toni Owen, Tamas Varga and Danielle Jansik
for XMT data collection and analyses, as well as Paul Martin for
experimental setup. The authors would like to thank Mark Bowden for
micro-XRD analysis and Laxmikant Saraf for SEM-EDS analysis in EMSL
(Environmental Molecular Sciences Laboratory), a DOE national scientific
user facility at Pacific Northwest National Laboratory (PNNL). Funding
for this research was provided by the National Risk Assessment
Partnership (NRAP) in the US Department of Energy Office of Fossil
Energy's Carbon Sequestration Program. PNNL is operated by Battelle for
the US DOE under Contract DE-AC06-76RLO 1830.
NR 37
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U1 2
U2 38
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0883-2927
J9 APPL GEOCHEM
JI Appl. Geochem.
PD AUG
PY 2013
VL 35
BP 161
EP 172
DI 10.1016/j.apgeochem.2013.04.007
PG 12
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 186SR
UT WOS:000322065800017
ER
PT J
AU Smith, SD
Solomon, DK
Gardner, WP
AF Smith, Stanley D.
Solomon, D. Kip
Gardner, W. Payton
TI Testing helium equilibrium between quartz and pore water as a method to
determine pore water helium concentrations
SO APPLIED GEOCHEMISTRY
LA English
DT Article
ID NOBLE-GASES; COSMOGENIC HE-3; DIFFUSION; GROUNDWATER; TRANSPORT;
MINERALS; AQUITARD; CRUSTAL; ROCKS; CLAY
AB The effectiveness of carbon capture and geologic storage depends on many factors, including and especially the permeability of the reservoir's caprock. While caprock integrity is generally assumed if petroleum has been preserved, it is poorly constrained in reservoirs containing only saline waters, and CO2 leakage poses a potential risk to shallow aquifers. Naturally-occurring He accumulates in pore waters over time with the concentration being strongly dependent on the long term flux of fluid through the caprock. Furthermore, a small fraction of pore-water He diffuses into quartz and this may be used as a proxy for He concentrations in pore water, where dissolved gas samples are difficult to obtain, such as in deep sedimentary basins. In this paper He contained in quartz grains is measured and compared to previously measured pore water concentrations. Quartz was purified from core samples from the San Juan Basin, New Mexico and the Great Artesian Basin, South Australia. Quartz separates were heated at 290 degrees C to release He from the quartz. The quartz from the San Juan Basin and high purity quartz from the Spruce Pine Intrusion, North Carolina was repeatedly impregnated at varying pressures using pure He, heated and analyzed to build He sorption isotherms. The isotherms appear linear but vary between samples, possibly due to fluid inclusions within the quartz grains as high purity quartz samples partition only 1.5% of He that partitions into San Juan Basin samples. Concentrations of He in the pore water were calculated using the He-accessible volume of the quartz and the air-water He solubility. The mean San Juan Basin He pore water concentration was 2 x 10(-5) cc STP He/g water, similar to 400 times greater than atmospheric solubility. Great Artesian Basin samples contain a mean He concentration of 3 x 10(-6) cc STP He/g water or 65 times greater than atmospheric solubility. However, pore water He concentrations in both the San Juan and Great Artesian Basins differ by up to an order of magnitude compared to samples collected with an alternate method. The reason for the offset is attributable to either partial saturation of the pore volume or a lack of He equilibrium between quartz and pore water. Coating of clay or other mineral phases on quartz grains, which tends to reduce the effective diffusion coefficient, may cause the latter. This technique of assessing permeability is promising due to the abundance of existing core samples from numerous basins where carbon sequestration may ultimately occur. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Smith, Stanley D.; Solomon, D. Kip] Univ Utah, Dept Geol & Geophys, Salt Lake City, UT 84112 USA.
[Gardner, W. Payton] CSIRO, Land & Water, Glen Osmond, SA 5064, Australia.
[Gardner, W. Payton] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Smith, SD (reprint author), Univ Utah, Dept Geol & Geophys, 115 S 1460 E, Salt Lake City, UT 84112 USA.
EM stan.smith@csiro.au
RI Smith, Stanley/E-2351-2013; Solomon, Douglas/C-7951-2016
OI Solomon, Douglas/0000-0001-6370-7124
FU EPA STAR Program [RD-83438601]
FX The authors would like to thank V. Heilweil and an anonymous reviewer
for their contributions towards a better article. This work was
supported by the EPA STAR Program Award RD-83438601. High purity quartz
from the Spruce Pine Pluton was provided by Unimin Inc. Core samples
from the Kirtland Formation were provided by Jason Heath.
NR 35
TC 2
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U1 1
U2 17
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0883-2927
J9 APPL GEOCHEM
JI Appl. Geochem.
PD AUG
PY 2013
VL 35
BP 187
EP 195
DI 10.1016/j.apgeochem.2013.04.010
PG 9
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 186SR
UT WOS:000322065800019
ER
PT J
AU Chatellier, X
Grybos, M
Abdelmoula, M
Kemner, KM
Leppard, GG
Mustin, C
West, MM
Paktunc, D
AF Chatellier, Xavier
Grybos, Malgorzata
Abdelmoula, Mustapha
Kemner, Kenneth M.
Leppard, Gary G.
Mustin, Christian
West, M. Marcia
Paktunc, Dogan
TI Immobilization of P by oxidation of Fe(II) ions leading to nanoparticle
formation and aggregation
SO APPLIED GEOCHEMISTRY
LA English
DT Article
ID RAY-ABSORPTION-SPECTROSCOPY; K-EDGE EXAFS; BACTERIAL SURFACES; GROWTH
MECHANISMS; MOSSBAUER-SPECTRA; AQUEOUS-SOLUTIONS; FE OXYHYDROXIDE;
FERROUS-IONS; GREEN RUST; PO4 IONS
AB Ferrous iron was oxidized at pH 6.0 in the presence of dissolved oxygen and increasing concentrations of phosphate. The resulting precipitates were characterized by TEM, SEM, XRD, IR spectroscopy, Mossbauer spectroscopy, EXAFS spectroscopy, and chemical analyses. The kinetics and the stoichiometry of oxidation were also determined. Chemical analyses revealed that all the P introduced was immobilized up to an introduced P/Fe molar ratio of 0.6-0.7. In the presence of excess phosphate, the maximum P/Fe ratio of the precipitates was found to be equal to about 0.86. Incorporation of phosphate hindered the sorption of dissolved carbonates, but favored the immobilization of monovalent cations such as Na or K. The number of OH ions per Fe atom introduced during the reaction decreased from 2 in the absence of P to about 1.5 +/- 0.1 in the presence of excess phosphate. In all cases, no residual Fe(II) could be detected. In the absence of phosphate, the samples were composed of poorly crystallized ferrihydrite, lepidocrocite and goethite nanoparticles. Even just a small amount of phosphate (P/Fe = 0.02) was sufficient to effectively restrict the formation of goethite. In contrast, the formation of lepidocrocite was detected by XRD for P/Fe ratios as high as 0.1. At higher P/Fe ratios, only non-crystalline particles were detected. For 0.1 < P/Fe < 0.5, the characteristic size of all particles was smaller than 10 nm. For P/Fe > 0.5, a new category of particles with characteristic length scales larger than 10 nm appeared and became prominent as P/Fe increased. The transition was accompanied by a change in color of the suspension, from dark red to light yellow. For an introduced P/Fe ratio larger than 1, only the larger particles remained. As the introduced P/Fe ratio increased further, the incorporated P/Fe ratio increased only slightly. In contrast the size of the particles increased significantly, reaching a size larger than 50 nm in the presence of a large excess of PO43-. The kinetics of oxidation and hydrolysis were shown to obey a typical autocatalytic process in the presence as well as in the absence of PO43-. Published by Elsevier Ltd.
C1 [Chatellier, Xavier] Univ Rennes 1, CNRS, F-35042 Rennes, France.
[Grybos, Malgorzata] Univ Limoges FST, GRESE, F-87060 Limoges, France.
[Abdelmoula, Mustapha] Univ Lorraine, CNRS, UMR 7564, Lab Chim Phys & Microbiol Environnement, F-54600 Villers Les Nancy, France.
[Kemner, Kenneth M.] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA.
[Leppard, Gary G.] Natl Water Res Inst Branch, Aquat Ecosyst Management Res Div, Burlington, ON L7R 4A6, Canada.
[Mustin, Christian] Univ Lorraine, CNRS, LIMOS, F-54506 Vandoeuvre Les Nancy, France.
[West, M. Marcia] McMaster Univ, Fac Hlth Sci, Hamilton, ON L8N 3Z5, Canada.
[Paktunc, Dogan] CANMET Min & Mineral Sci Labs, Ottawa, ON K1A 0G1, Canada.
RP Chatellier, X (reprint author), Burgemeester Patijnlaan 90, NL-2585 BL The Hague, Netherlands.
EM xavier.chatellier@univ-rennes1.fr
RI ID, MRCAT/G-7586-2011
FU Argonne Subsurface Science Focus Area is part of the United States
Department of Energy (US DOE), Office of Science (OS), Office of
Biological and Environmental Research Subsurface Biogeochemical Research
Program; US DOE OS Office of Basic Energy Science (BES); MRCAT/EnviroCAT
member institutions; US DOE OS BES [DE-AC02-06CH11357]
FX We thank Bruce Ravel, Martine Bouhnik-Le Coz, Beatrice Trinkler, and
Joseph Le Lannic for contributing to the EXAFS spectroscopy, ICP-MS, CN
and SEM measurements, respectively. We thank Patrice Petitjean for
performing AAS measurements (not shown here), which confirmed the ICP-MS
results. We thank Odile Henin for some valuable help in the laboratory.
This work was supported in part by the Argonne Subsurface Science Focus
Area, which is part of the United States Department of Energy (US DOE),
Office of Science (OS), Office of Biological and Environmental Research
Subsurface Biogeochemical Research Program. Use of the MRCAT/EnviroCAT
at the Advanced Photon Source (APS) was supported by the US DOE OS
Office of Basic Energy Science (BES) and the MRCAT/EnviroCAT member
institutions. Use of the APS was supported by the US DOE OS BES under
contract DE-AC02-06CH11357.
NR 66
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U1 4
U2 53
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0883-2927
J9 APPL GEOCHEM
JI Appl. Geochem.
PD AUG
PY 2013
VL 35
BP 325
EP 339
DI 10.1016/j.apgeochem.2013.04.019
PG 15
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 186SR
UT WOS:000322065800031
ER
PT J
AU Huh, SS
Gunter, D
Chivers, D
Mihailescu, L
Vetter, K
AF Huh, Sam S.
Gunter, Donald
Chivers, Daniel
Mihailescu, Lucian
Vetter, Kai
TI Unbiased and biased estimators in coded aperture imaging for far field
standoff detection at low count rates
SO APPLIED OPTICS
LA English
DT Article
ID UNIFORMLY REDUNDANT ARRAYS
AB In general, the reconstructed image in coded aperture imaging is affected by the source configuration. Fenimore's balanced convolution method in conjunction with the uniformly redundant array can remove the interference due to the source configuration. As an extensiono of Fenimore's balanced convolution method, we present general conditions for designing an unbiased mean estimator for a far-field coded aperture imaging system with a random binary mask. As part of the general conditions, we propose decoding arrays whose elements are variable with respect to source directions. We also show that the unbiased mean estimator from Fenimore's balanced convolution method is a special case of the general conditions. We also present a practical example of designing restoring arrays for a coded aperture system with a random mask. (C) 2013 Optical Society of America
C1 [Huh, Sam S.; Gunter, Donald; Chivers, Daniel; Mihailescu, Lucian; Vetter, Kai] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Appl Nucl Phys Program, Berkeley, CA 94720 USA.
[Vetter, Kai] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA.
RP Huh, SS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Appl Nucl Phys Program, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM sshuh@lbl.gov
NR 6
TC 0
Z9 0
U1 0
U2 3
PU OPTICAL SOC AMER
PI WASHINGTON
PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA
SN 1559-128X
J9 APPL OPTICS
JI Appl. Optics
PD AUG 1
PY 2013
VL 52
IS 22
BP 5478
EP 5492
DI 10.1364/AO.52.005478
PG 15
WC Optics
SC Optics
GA 193OP
UT WOS:000322569800035
PM 23913069
ER
PT J
AU Maroni, VA
Johnson, CS
Rood, SCM
Kropf, AJ
Bass, DA
AF Maroni, Victor A.
Johnson, Christopher S.
Rood, Shawn C. M.
Kropf, A. Jeremy
Bass, Dean A.
TI Characterization of Novel Lithium Battery Cathode Materials by
Spectroscopic Methods: The Li5+xFeO4 System
SO APPLIED SPECTROSCOPY
LA English
DT Article
DE Raman; X-ray absorption; X-ray diffraction; Lithium battery; Cathode
material; Li5FeO4 (LFO)
ID ION BATTERIES; SECONDARY BATTERIES; METAL-OXIDES; LI5FEO4; CELLS; FE
AB The novel, lithium-rich oxide-phase Li5FeO4 (LFO) could, in theory, deliver a specific capacity >900 mAh/g when deployed as a cathode or cathode precursor in a battery with a lithium-based anode. However, research results to date on LFO indicate that less than one of the five Li+ cations can be reversibly de-intercalated/re-intercalated during repetitive charging and discharging cycles. In the present research, the system Li5+xFeO4 with x values in the range of 0.0-2.0 was investigated by a combination of Raman and X-ray absorption spectroscopic methods supported by X-ray diffraction (XRD) analysis in order to determine if the Li5FeO4 lattice would accommodate additional Li+ ions, with concomitant lowering of the valence on the Fe-III cations. Both the Raman phonon spectra and the XRD patterns were invariant for all values of x, strongly indicating that additional Li+ did not enter the Li5FeO4 lattice. Also, Raman spectral results and high-resolution synchrotron XRD data revealed the presence of second-phase Li2O in all samples with x greater than 0.0. Synchrotron X-ray absorption spectroscopy at the Fe k alpha edge performed on the sample with a Li-Fe ratio of 7.0 (i.e., x = 2.0) showed no evidence for the presence of Fe-II. This resistance to accepting more lithium into the Li5FeO4 structure is attributed to the exceedingly stable nature of high-spin Fe-III in tetrahedral "(FeO4)-O-III" structural units of Li5FeO4. Partial substitution of the Fern with other cations could provide a path toward increasing the reversible Li+ content of Li5xFeO4-type phases.
C1 [Maroni, Victor A.; Johnson, Christopher S.; Rood, Shawn C. M.; Kropf, A. Jeremy; Bass, Dean A.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
RP Maroni, VA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM Maroni@anl.gov
RI Rood, Shawn/O-9843-2015
OI Rood, Shawn/0000-0002-5416-9894
FU U.S. Department of Energy (USDOE) [DE-FG02-09ER85385]; University of
Chicago Argonne, L.L.C. [DE-AC02-06CH11357]; USDOE [DE-AC02-06CH11357]
FX The research described in this paper was sponsored by the U.S.
Department of Energy (USDOE) as part of a Phase H Small Business
Innovative Research Project (no. DE-FG02-09ER85385) between Farasis
Energy, Inc., and ANL. The support and encouragement of Dr. Keith Kepler
at Farasis Energy, Inc., and the assistance of Dr. David Gosztola with
the use of the Raman instrumentation is gratefully acknowledged. Use of
instrumentation at Argonne's Center for Nanoscale Materials and Advanced
Photon Source was supported by the USDOE, Office of Science, Office of
Basic Energy Sciences. The work carried out at the ANL was performed
under contract DE-AC02-06CH11357 between University of Chicago Argonne,
L.L.C., and the USDOE.
NR 26
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U1 5
U2 51
PU SOC APPLIED SPECTROSCOPY
PI FREDERICK
PA 5320 SPECTRUM DRIVE SUITE C, FREDERICK, MD 21703 USA
SN 0003-7028
J9 APPL SPECTROSC
JI Appl. Spectrosc.
PD AUG
PY 2013
VL 67
IS 8
BP 903
EP 912
DI 10.1366/12-06893
PG 10
WC Instruments & Instrumentation; Spectroscopy
SC Instruments & Instrumentation; Spectroscopy
GA 193KW
UT WOS:000322559700011
PM 23876729
ER
PT J
AU Jones, S
Hirschi, R
Nomoto, K
Fischer, T
Timmes, FX
Herwig, F
Paxton, B
Toki, H
Suzuki, T
Martinez-Pinedo, G
Lam, YH
Bertolli, MG
AF Jones, S.
Hirschi, R.
Nomoto, K.
Fischer, T.
Timmes, F. X.
Herwig, F.
Paxton, B.
Toki, H.
Suzuki, T.
Martinez-Pinedo, G.
Lam, Y. H.
Bertolli, M. G.
TI ADVANCED BURNING STAGES AND FATE OF 8-10 M-circle dot STARS
SO ASTROPHYSICAL JOURNAL
LA English
DT Article
DE nuclear reactions, nucleosynthesis, abundances; stars: AGB and post-AGB;
stars: evolution; stars: neutron; supernovae: general
ID ELECTRON-CAPTURE SUPERNOVAE; MASSIVE AGB STARS; CORE-COLLAPSE
SUPERNOVAE; WEAK INTERACTION RATES; GIANT BRANCH STARS; DEGENERATE
CORES; MODEL STAR; CONDUCTIVE PROPAGATION; STELLAR EVOLUTION; NUCLEAR
FLAMES
AB The stellar mass range 8 less than or similar to M/M-circle dot less than or similar to 12 corresponds to the most massive asymptotic giant branch (AGB) stars and the most numerous massive stars. It is host to a variety of supernova (SN) progenitors and is therefore very important for galactic chemical evolution and stellar population studies. In this paper, we study the transition from super-AGB (SAGB) star to massive star and find that a propagating neon-oxygen-burning shell is common to both the most massive electron capture supernova (EC-SN) progenitors and the lowest mass iron-core-collapse supernova (FeCCSN) progenitors. Of the models that ignite neon-burning off-center, the 9.5 M-circle dot star would evolve to an FeCCSN after the neon-burning shell propagates to the center, as in previous studies. The neon-burning shell in the 8.8 M-circle dot model, however, fails to reach the center as the URCA process and an extended (0.6 M-circle dot) region of low Y-e (0.48) in the outer part of the core begin to dominate the late evolution; the model evolves to an EC-SN. This is the first study to follow the most massive EC-SN progenitors to collapse, representing an evolutionary path to EC-SN in addition to that from SAGB stars undergoing thermal pulses (TPs). We also present models of an 8.75 M-circle dot SAGB star through its entire TP phase until electron captures on Ne-20 begin at its center and of a 12 M-circle dot star up to the iron core collapse. We discuss key uncertainties and how the different pathways to collapse affect the pre-SN structure. Finally, we compare our results to the observed neutron star mass distribution.
C1 [Jones, S.; Hirschi, R.] Keele Univ, Astrophys Grp, Keele ST5 5BG, Staffs, England.
[Hirschi, R.; Nomoto, K.] Univ Tokyo, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan.
[Fischer, T.; Martinez-Pinedo, G.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany.
[Fischer, T.; Martinez-Pinedo, G.; Lam, Y. H.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany.
[Timmes, F. X.] Univ Arizona, Sch Earth & Space Explorat, Tempe, AZ 85287 USA.
[Timmes, F. X.; Herwig, F.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA.
[Herwig, F.] Univ Victoria, Dept Phys & Astron, Victoria, BC V8W 3P6, Canada.
[Paxton, B.] Univ Calif Santa Barbara, KITP, Santa Barbara, CA 93106 USA.
[Paxton, B.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA.
[Toki, H.] Osaka Univ, Res Ctr Nucl Phys RCNP, Osaka 5670047, Japan.
[Suzuki, T.] Nihon Univ, Coll Human & Sci, Dept Phys, Setagaya Ku, Tokyo 1568550, Japan.
[Suzuki, T.] Natl Astron Observ Japan, Mitaka, Tokyo 1818588, Japan.
[Bertolli, M. G.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
RP Jones, S (reprint author), Keele Univ, Astrophys Grp, Lennard Jones Bldg, Keele ST5 5BG, Staffs, England.
EM s.w.jones@keele.ac.uk
RI Martinez-Pinedo, Gabriel/A-1915-2013
OI Martinez-Pinedo, Gabriel/0000-0002-3825-0131
FU European Research Council under the European Union's Seventh Framework
Programme/ERC [306901]; NSF [PHY 02-16783, PHY 0922648]; Eurocore
project Eurogenesis; World Premier International Research Center
Initiative (WPI Initiative), MEXT, Japan; Swiss National Science
Foundation [PBBSP2-133378]; National Science Foundation [PHY 11-25915,
AST 11-09174]; National Nuclear Security Administration of the U.S.
Department of Energy at Los Alamos National Laboratory
[DE-AC52-06NA25396]
FX The research leading to these results has received funding from the
European Research Council under the European Union's Seventh Framework
Programme (FP/2007-2013)/ERC Grant Agreement No. 306901. NuGrid
acknowledges significant support from NSF grants PHY 02-16783 and PHY
0922648 (Joint Institute for Nuclear Astrophysics, JINA). R.H. thanks
the Eurocore project Eurogenesis for support. K.N., R.H., and S.J.
acknowledge support from the World Premier International Research Center
Initiative (WPI Initiative), MEXT, Japan. T.F. acknowledges support from
the Swiss National Science Foundation under project no. PBBSP2-133378
and HIC for FAIR. B.P.'s research has been supported by the National
Science Foundation under grants PHY 11-25915 and AST 11-09174. M.G.B.'s
research was carried out under the auspices of the National Nuclear
Security Administration of the U.S. Department of Energy at Los Alamos
National Laboratory under contract No. DE-AC52-06NA25396.
NR 56
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U1 0
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PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-637X
J9 ASTROPHYS J
JI Astrophys. J.
PD AUG 1
PY 2013
VL 772
IS 2
AR 150
DI 10.1088/0004-637X/772/2/150
PG 14
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 186EL
UT WOS:000322024700072
ER
PT J
AU Luo, B
Brandt, WN
Alexander, DM
Harrison, FA
Stern, D
Bauer, FE
Boggs, SE
Christensen, FE
Comastri, A
Craig, WW
Fabian, AC
Farrah, D
Fiore, F
Fuerst, F
Grefenstette, BW
Hailey, CJ
Hickox, R
Madsen, KK
Matt, G
Ogle, P
Risaliti, G
Saez, C
Teng, SH
Walton, DJ
Zhang, WW
AF Luo, B.
Brandt, W. N.
Alexander, D. M.
Harrison, F. A.
Stern, D.
Bauer, F. E.
Boggs, S. E.
Christensen, F. E.
Comastri, A.
Craig, W. W.
Fabian, A. C.
Farrah, D.
Fiore, F.
Fuerst, F.
Grefenstette, B. W.
Hailey, C. J.
Hickox, R.
Madsen, K. K.
Matt, G.
Ogle, P.
Risaliti, G.
Saez, C.
Teng, S. H.
Walton, D. J.
Zhang, W. W.
TI WEAK HARD X-RAY EMISSION FROM TWO BROAD ABSORPTION LINE QUASARS OBSERVED
WITH NuSTAR: COMPTON-THICK ABSORPTION OR INTRINSIC X-RAY WEAKNESS?
SO ASTROPHYSICAL JOURNAL
LA English
DT Article
DE accretion, accretion disks; galaxies: active; galaxies: nuclei; quasars:
absorption lines; quasars: emission lines; X-rays: general
ID ACTIVE GALACTIC NUCLEI; DIGITAL SKY SURVEY; SPECTRAL
ENERGY-DISTRIBUTIONS; OPTICALLY SELECTED QUASARS; XMM-NEWTON
SPECTROSCOPY; HUBBLE-SPACE-TELESCOPE; ACCRETION DISK WINDS; RADIO-LOUD
QUASARS; SEYFERT 1 GALAXIES; 7TH DATA RELEASE
AB We present Nuclear Spectroscopic Telescope Array (NuSTAR) hard X-ray observations of two X-ray weak broad absorption line (BAL) quasars, PG 1004+130 (radio loud) and PG 1700+518 (radio quiet). Many BAL quasars appear X-ray weak, probably due to absorption by the shielding gas between the nucleus and the accretion-disk wind. The two targets are among the optically brightest BAL quasars, yet they are known to be significantly X-ray weak at rest-frame 2-10 keV (16-120 times fainter than typical quasars). We would expect to obtain approximate to 400-600 hard X-ray (greater than or similar to 10 keV) photons with NuSTAR, provided that these photons are not significantly absorbed (N-H less than or similar to 10(24) cm(-2)). However, both BAL quasars are only detected in the softer NuSTAR bands (e.g., 4-20 keV) but not in its harder bands (e.g., 20-30 keV), suggesting that either the shielding gas is highly Compton-thick or the two targets are intrinsically X-ray weak. We constrain the column densities for both to be N-H approximate to 7 x 10(24) cm(-2) if the weak hard X-ray emission is caused by obscuration from the shielding gas. We discuss a few possibilities for how PG 1004+130 could have Compton-thick shielding gas without strong Fe K alpha line emission; dilution from jet-linked X-ray emission is one likely explanation. We also discuss the intrinsic X-ray weakness scenario based on a coronal-quenching model relevant to the shielding gas and disk wind of BAL quasars. Motivated by our NuSTAR results, we perform a Chandra stacking analysis with the Large Bright Quasar Survey BAL quasar sample and place statistical constraints upon the fraction of intrinsically X-ray weak BAL quasars; this fraction is likely 17%-40%.
C1 [Luo, B.; Brandt, W. N.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA.
[Luo, B.; Brandt, W. N.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA.
[Alexander, D. M.; Hickox, R.] Univ Durham, Dept Phys, Durham DH1 3LE, England.
[Harrison, F. A.; Fuerst, F.; Grefenstette, B. W.; Madsen, K. K.; Walton, D. J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA.
[Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA.
[Bauer, F. E.; Saez, C.] Pontificia Univ Catolica Chile, Dept Astron & Astrofis, Santiago 22, Chile.
[Bauer, F. E.] Space Sci Inst, Boulder, CO 80301 USA.
[Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA.
[Christensen, F. E.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark.
[Comastri, A.] INAF, Osservatorio Astron Bologna, I-40127 Bologna, Italy.
[Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Fabian, A. C.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England.
[Farrah, D.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA.
[Fiore, F.] Osserv Astron Roma, I-00040 Monte Porzio Catone, Italy.
[Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA.
[Hickox, R.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA.
[Matt, G.] Univ Roma Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy.
[Ogle, P.] CALTECH, IPAC, Pasadena, CA 91125 USA.
[Risaliti, G.] INAF, Osservatorio Astrofis Arcetri, I-50125 Florence, Italy.
[Risaliti, G.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA.
[Teng, S. H.] NASA, Goddard Space Flight Ctr, Observat Cosmol Lab, Greenbelt, MD 20771 USA.
[Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA.
RP Luo, B (reprint author), Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA.
RI Boggs, Steven/E-4170-2015; Brandt, William/N-2844-2015; Comastri,
Andrea/O-9543-2015;
OI Boggs, Steven/0000-0001-9567-4224; Brandt, William/0000-0002-0167-2453;
Comastri, Andrea/0000-0003-3451-9970; Alexander,
David/0000-0002-5896-6313; Fiore, Fabrizio/0000-0002-4031-4157;
Risaliti, Guido/0000-0002-3556-977X
FU California Institute of Technology (Caltech) NuSTAR [44A-1092750]; NASA
ADP Grant [NNX10AC99G]; Leverhulme trust; Science Technology and
Facilities Council; Basal-CATA [PFB-06/2007]; CONICYT-Chile [FONDECYT
1101024, Anillo ACT1101, FONDECYT 3120198]; NASA [NNG08FD60C]; National
Aeronautics and Space Administration
FX We acknowledge support from the California Institute of Technology
(Caltech) NuSTAR subcontract 44A-1092750 (B.L. and W.N.B.), NASA ADP
Grant NNX10AC99G (B.L. and W.N.B.), the Leverhulme trust and the Science
Technology and Facilities Council (D.M.A.), Basal-CATA Grant PFB-06/2007
and CONICYT-Chile Grants FONDECYT 1101024 and Anillo ACT1101 (F.E.B.),
and CONICYT-Chile Grant FONDECYT 3120198 (C.S.). We thank M. Young for
help with the planning of this project and K. Forster for help with the
NuSTAR data access, and we thank M. Balokovic, K. Boydstun, T. N. Lu, B.
P. Miller, Jianfeng Wu, and T. Yaqoob for helpful discussions. We thank
the referee, S. C. Gallagher, for carefully reviewing the manuscript and
providing helpful comments.; This work was supported under NASA contract
No. NNG08FD60C, and made use of data from the NuSTAR mission, a project
led by Caltech, managed by the Jet Propulsion Laboratory, and funded by
the National Aeronautics and Space Administration. We thank the NuSTAR
Operations, Software and Calibration teams for support with the
execution and analysis of these observations. This research has made use
of NuSTAR-DAS jointly developed by the ASI Science Data Center (ASDC,
Italy) and Caltech (USA).
NR 146
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PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-637X
J9 ASTROPHYS J
JI Astrophys. J.
PD AUG 1
PY 2013
VL 772
IS 2
AR 153
DI 10.1088/0004-637X/772/2/153
PG 17
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 186EL
UT WOS:000322024700075
ER
PT J
AU Muratov, AL
Gnedin, OY
Gnedin, NY
Zemp, M
AF Muratov, Alexander L.
Gnedin, Oleg Y.
Gnedin, Nickolay Y.
Zemp, Marcel
TI REVISITING THE FIRST GALAXIES: THE EFFECTS OF POPULATION III STARS ON
THEIR HOST GALAXIES
SO ASTROPHYSICAL JOURNAL
LA English
DT Article
DE cosmology: theory; galaxies: evolution; galaxies: formation; methods:
numerical; stars: formation
ID HIGH-REDSHIFT GALAXIES; KENNICUTT-SCHMIDT RELATION; INITIAL MASS
FUNCTION; LAMBDA-CDM UNIVERSE; COSMOLOGICAL SIMULATIONS; RADIATIVE
FEEDBACK; DWARF GALAXIES; PRIMORDIAL GAS; PROTOSTELLAR FEEDBACK; STELLAR
POPULATIONS
AB We revisit the formation and evolution of the first galaxies using new hydrodynamic cosmological simulations with the adaptive refinement tree code. Our simulations feature a recently developed model for H-2 formation and dissociation, and a star formation recipe that is based on molecular rather than atomic gas. Here, we develop and implement a recipe for the formation of metal-free Population III (Pop III) stars in galaxy-scale simulations that resolve primordial clouds with sufficiently high density. We base our recipe on the results of prior zoom-in simulations that resolved the protostellar collapse in pre-galactic objects. We find the epoch during which Pop III stars dominated the energy and metal budget of the first galaxies to be short-lived. Galaxies that host Pop III stars do not retain dynamical signatures of their thermal and radiative feedback for more than 10(8) years after the lives of the stars end in pair-instability supernovae, even when we consider the maximum reasonable efficiency of the feedback. Though metals ejected by the supernovae can travel well beyond the virial radius of the host galaxy, they typically begin to fall back quickly, and do not enrich a large fraction of the intergalactic medium. Galaxies with a total mass in excess of 3 x 10(6) M-circle dot re-accrete most of their baryons and transition to metal-enriched Pop II star formation.
C1 [Muratov, Alexander L.; Gnedin, Oleg Y.; Zemp, Marcel] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA.
[Gnedin, Nickolay Y.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA.
[Gnedin, Nickolay Y.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA.
[Gnedin, Nickolay Y.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA.
[Gnedin, Nickolay Y.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA.
[Zemp, Marcel] Peking Univ, Kavli Inst Astron & Astrophys, Beijing 100871, Peoples R China.
RP Muratov, AL (reprint author), Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA.
EM muratov@umich.edu
OI Zemp, Marcel/0000-0002-0498-3812; Gnedin, Oleg/0000-0001-9852-9954
FU Rackham pre-Doctoral Fellowship; University of Michigan; NSF
[AST-0708087, AST-0708154]; NASA [NNX12AG44G]; DOE at Fermilab; Peking
University
FX A.L.M. acknowledges the support of the Rackham pre-Doctoral Fellowship
awarded by The University of Michigan. O.Y.G. was supported in part by
NSF grant AST-0708087 and NASA grant NNX12AG44G. This work was supported
in part by the DOE at Fermilab and by NSF grant AST-0708154. M.Z. is in
part supported by a 985 grant from Peking University. We thank the
anonymous referee for a thorough and insightful report. We also thank
Alexander Heger for discussion of the evolution of a 100 Mcircle
dot star, and John Wise, Andrey Kravtsov, Milos Milosavljevic,
Michael Anderson, Wen-Hsin Hsu, and Doug Rudd for various constructive
suggestions.
NR 70
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PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-637X
J9 ASTROPHYS J
JI Astrophys. J.
PD AUG 1
PY 2013
VL 772
IS 2
AR 106
DI 10.1088/0004-637X/772/2/106
PG 13
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 186EL
UT WOS:000322024700028
ER
PT J
AU Silverman, JM
Nugent, PE
Gal-Yam, A
Sullivan, M
Howell, DA
Filippenko, AV
Pan, YC
Cenko, SB
Hook, IM
AF Silverman, Jeffrey M.
Nugent, Peter E.
Gal-Yam, Avishay
Sullivan, Mark
Howell, D. Andrew
Filippenko, Alexei V.
Pan, Yen-Chen
Cenko, S. Bradley
Hook, Isobel M.
TI LATE-TIME SPECTRAL OBSERVATIONS OF THE STRONGLY INTERACTING TYPE Ia
SUPERNOVA PTF11kx
SO ASTROPHYSICAL JOURNAL
LA English
DT Article
DE circumstellar matter; supernovae: general; supernovae: individual
(PTF11kx)
ID DARK-ENERGY CONSTRAINTS; WHITE-DWARF STAR; IIN SUPERNOVA; CIRCUMSTELLAR
INTERACTION; SODIUM-ABSORPTION; LEGACY SURVEY; SN 2011FE; PROGENITOR;
2009DC; 2010JL
AB PTF11kx was a Type Ia supernova (SN Ia) that showed time-variable absorption features, including saturated Ca II H and K lines that weakened and eventually went into emission. The strength of the emission component of H alpha gradually increased, implying that the SN was undergoing significant interaction with its circumstellar medium (CSM). These features, and many others, were blueshifted slightly and showed a P-Cygni profile, likely indicating that the CSM was directly related to, and probably previously ejected by, the progenitor system itself. These and other observations led Dilday et al. to conclude that PTF11kx came from a symbiotic nova progenitor like RS Oph. In this work we extend the spectral coverage of PTF11kx to 124-680 rest-frame days past maximum brightness. The late-time spectra of PTF11kx are dominated by Ha emission (with widths of full width at half-maximum intensity approximate to 2000 km s(-1)), strong Ca II emission features (similar to 10,000 km s(-1) wide), and a blue "quasi-continuum" due to many overlapping narrow lines of Fe II. Emission from oxygen, He I, and Balmer lines higher than Ha is weak or completely absent at all epochs, leading to large observed H alpha/H beta intensity ratios. The H alpha emission appears to increase in strength with time for similar to 1 yr, but it subsequently decreases significantly along with the Ca II emission. Our latest spectrum also indicates the possibility of newly formed dust in the system as evidenced by a slight decrease in the red wing of H alpha. During the same epochs, multiple narrow emission features from the CSM temporally vary in strength. The weakening of the H alpha and Ca II emission at late times is possible evidence that the SN ejecta have overtaken the majority of the CSM and agrees with models of other strongly interacting SNe Ia. The varying narrow emission features, on the other hand, may indicate that the CSM is clumpy or consists of multiple thin shells.
C1 [Silverman, Jeffrey M.] Univ Texas Austin, Dept Astron, Austin, TX 78712 USA.
[Silverman, Jeffrey M.; Nugent, Peter E.; Filippenko, Alexei V.; Cenko, S. Bradley] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA.
[Nugent, Peter E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Gal-Yam, Avishay] Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel.
[Sullivan, Mark] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England.
[Howell, D. Andrew] Las Cumbres Observ, Global Telescope Network, Goleta, CA 93117 USA.
[Howell, D. Andrew] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA.
[Pan, Yen-Chen; Hook, Isobel M.] Univ Oxford, Dept Phys Astrophys, Oxford OX1 3RH, England.
[Hook, Isobel M.] Osserv Astron Roma, INAF, I-00040 Monte Porzio Catone, RM, Italy.
RP Silverman, JM (reprint author), Univ Texas Austin, Dept Astron, RLM 15308, Austin, TX 78712 USA.
EM jsilverman@astro.as.utexas.edu
OI Sullivan, Mark/0000-0001-9053-4820; Hook, Isobel/0000-0002-2960-978X
FU W. M. Keck Foundation; NASA; Alfred P. Sloan Foundation; National
Science Foundation (NSF); U.S. Department of Energy Office of Science;
Richard and Rhoda Goldman Fund; Christopher R. Redlich Fund; TABASGO
Foundation; NSF [AST-0908886, AST-1211916]; ISF; BSF; GIF; Minerva, an
FP7/ERC grant; Helen and Martin Kimmel Award for Innovative
Investigation; Royal Society
FX We thank J. S. Bloom, K. Clubb, A. A. Miller, and A. Morgan for their
assistance with some of the observations, B. Dilday, O. Fox, and L. Wang
for helpful discussions, and the anonymous referee for providing
comments and suggestions that improved the manuscript. We are grateful
to the staffs at the WHT and the Keck Observatory for their support. The
WHT is operated on the island of La Palma by the Isaac Newton Group in
the Spanish Observatorio del Roque de los Muchachos of the Instituto de
Astrofisica de Canarias. Some of the data presented herein were obtained
at the W. M. Keck Observatory, which is operated as a scientific
partnership among the California Institute of Technology, the University
of California, and the National Aeronautics and Space Administration
(NASA); the observatory was made possible by the generous financial
support of the W. M. Keck Foundation. The authors wish to recognize and
acknowledge the very significant cultural role and reverence that the
summit of Mauna Kea has always had within the indigenous Hawaiian
community; we are most fortunate to have the opportunity to conduct
observations from this mountain. This research has made use of the
NASA/IPAC Extragalactic Database (NED) which is operated by the Jet
Propulsion Laboratory, California Institute of Technology, under
contract with NASA. Funding for SDSS-III has been provided by the Alfred
P. Sloan Foundation, the Participating Institutions, the National
Science Foundation (NSF), and the U.S. Department of Energy Office of
Science. The SDSS-III Web site is http://www.sdss3.org/. Supernova
research by A.V.F.'s group at U.C. Berkeley is supported by Gary and
Cynthia Bengier, the Richard and Rhoda Goldman Fund, the Christopher R.
Redlich Fund, the TABASGO Foundation, and NSF Grants AST-0908886 and
AST-1211916. Work by A.G.-Y. and his group is supported by grants from
the ISF, BSF, GIF, and Minerva, an FP7/ERC grant, and the Helen and
Martin Kimmel Award for Innovative Investigation. M. S. acknowledges
support from the Royal Society.
NR 55
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PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-637X
J9 ASTROPHYS J
JI Astrophys. J.
PD AUG 1
PY 2013
VL 772
IS 2
AR 125
DI 10.1088/0004-637X/772/2/125
PG 7
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 186EL
UT WOS:000322024700047
ER
PT J
AU Van Dyk, SD
Zheng, WK
Clubb, KI
Filippenko, AV
Cenko, SB
Smith, N
Fox, OD
Kelly, PL
Shivvers, I
Ganeshalingam, M
AF Van Dyk, Schuyler D.
Zheng, WeiKang
Clubb, Kelsey I.
Filippenko, Alexei V.
Cenko, S. Bradley
Smith, Nathan
Fox, Ori D.
Kelly, Patrick L.
Shivvers, Isaac
Ganeshalingam, Mohan
TI THE PROGENITOR OF SUPERNOVA 2011dh HAS VANISHED
SO ASTROPHYSICAL JOURNAL LETTERS
LA English
DT Article
DE galaxies: individual (NGC 5194); stars: evolution; supernovae: general;
supernovae: individual (SN 2011dh)
ID RED SUPERGIANT PROGENITOR; SN 2011DH; IIB SUPERNOVA; EVOLUTION; 1993J;
STAR; M51; SPECTRA; COMPACT; SEARCH
AB We conducted Hubble Space Telescope (HST) Snapshot observations of the Type IIb supernova (SN) 2011dh in M51 at an age of similar to 641 days with the Wide Field Camera 3. We find that the yellow supergiant star, clearly detected in pre-SN HST images, has disappeared, implying that this star was almost certainly the progenitor of the SN. Interpretation of the early time SN data which led to the inference of a compact nature for the progenitor, and to the expected survival of this yellow supergiant, is now clearly incorrect. We also present ground-based UBVRI light curves obtained with the Katzman Automatic Imaging Telescope at Lick Observatory up to SN age similar to 70 days. From the light-curve shape including the very late time HST data, and from recent interacting binary models for SN 2011dh, we estimate that a putative surviving companion star to the now deceased yellow supergiant could be detectable by late 2013, especially in the ultraviolet. No obvious light echoes are detectable yet in the SN environment.
C1 [Van Dyk, Schuyler D.] CALTECH, Spitzer Sci Ctr, Pasadena, CA 91125 USA.
[Zheng, WeiKang; Clubb, Kelsey I.; Filippenko, Alexei V.; Cenko, S. Bradley; Fox, Ori D.; Kelly, Patrick L.; Shivvers, Isaac] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA.
[Cenko, S. Bradley] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA.
[Smith, Nathan] Univ Arizona, Steward Observ, Tucson, AZ 85720 USA.
[Ganeshalingam, Mohan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Van Dyk, SD (reprint author), CALTECH, Spitzer Sci Ctr, Mailcode 220-6, Pasadena, CA 91125 USA.
EM vandyk@ipac.caltech.edu
OI Shivvers, Isaac/0000-0003-3373-8047; Van Dyk,
Schuyler/0000-0001-9038-9950
FU NASA [NAS 05-26555]; NASA from STScI [AR-12623, GO-13029]; Richard and
Rhoda Goldman Fund; Christopher R. Redlich Fund; TABASGO Foundation; NSF
[AST-1211916]
FX This work is based in part on observations made with the NASA/ESA Hubble
Space Telescope, obtained from the Data Archive at the Space Telescope
Science Institute (STScI), which is operated by the Association of
Universities for Research in Astronomy (AURA), Inc., under NASA contract
NAS 05-26555. KAIT and its ongoing research were made possible by
donations from Sun Microsystems, Inc., the Hewlett-Packard Company,
AutoScope Corporation, Lick Observatory, the NSF, the University of
California, the Sylvia & Jim Katzman Foundation, and the TABASGO
Foundation. Support for this research was provided by NASA through
grants AR-12623 and GO-13029 from STScI. A.V.F. and his group at UC
Berkeley also wish to acknowledge generous support from Gary and Cynthia
Bengier, the Richard and Rhoda Goldman Fund, the Christopher R. Redlich
Fund, the TABASGO Foundation, and NSF grant AST-1211916.
NR 43
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PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 2041-8205
J9 ASTROPHYS J LETT
JI Astrophys. J. Lett.
PD AUG 1
PY 2013
VL 772
IS 2
AR L32
DI 10.1088/2041-8205/772/2/L32
PG 5
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA 186CR
UT WOS:000322020000019
ER
PT J
AU Fosso-Tande, J
Harrison, RJ
AF Fosso-Tande, Jacob
Harrison, Robert J.
TI Confinement effects of solvation on a molecule physisorbed on a
polarizable continuum particle
SO COMPUTATIONAL AND THEORETICAL CHEMISTRY
LA English
DT Article
DE Multiresolution; Multiwavelet; Physisorption; Confinement;
Electrostatic; Enhancement; Poisson's equation
ID SURFACE-ENHANCED RAMAN; SINGLE MOLECULES; 2ND HYPERPOLARIZABILITY;
SCATTERING SERS; SILVER; NANOPARTICLES; SPECTRA; ELECTRODE; MODELS
AB We investigate the effects of solvation on the static properties of a molecule physisorbed on a spherical polarizable continuum particle, with a static dielectric constant. The effective polarizability of the physisorbed molecule is enhanced by a factor of 10(5) in vacuo and by only 10(2) when solvated. The electrostatic interaction between molecules and the polarizable continuum particle (PCP) results in a magnified reflected electric field with a magnitude that depends on the PCP-molecule separation. A similar and greater magnification effect in reflected field also results from the PCP-field (external electric field) interaction. The variation of the polarizability of the molecules with respect to the changes in their environment illustrates the importance of electrostatic interaction in the enhancement of the effective polarizability. In the course of the investigation, the solute and the continuous body are represented with the same adaptive multi-wavelet basis functions, thereby, within the user specified precision, eliminating basis set error. Published by Elsevier B.V.
C1 [Fosso-Tande, Jacob; Harrison, Robert J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
[Harrison, Robert J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Fosso-Tande, J (reprint author), Univ Tennessee, Dept Chem, 552 Buehler Hall,142 Circle Dr, Knoxville, TN 37996 USA.
EM jtande@utk.edu
FU National Science Foundation [OCI-0904972]; Department of Energy
[DE-AC05-00OR22725]
FX This work was supported by the National Science Foundation under Grant
OCI-0904972 (Computational Chemistry and Physics Beyond the Petascale).
Simulations were performed at the National Center for Computational
Sciences at Oak Ridge National Laboratory under contract
DE-AC05-00OR22725 from the Department of Energy.
NR 27
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U1 0
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2210-271X
J9 COMPUT THEOR CHEM
JI Comput. Theor. Chem.
PD AUG 1
PY 2013
VL 1017
BP 22
EP 30
DI 10.1016/j.comptc.2013.05.006
PG 9
WC Chemistry, Physical
SC Chemistry
GA 189VV
UT WOS:000322297300004
ER
PT J
AU Zhai, P
Haussener, S
Ager, J
Sathre, R
Walczak, K
Greenblatt, J
McKone, T
AF Zhai, Pei
Haussener, Sophia
Ager, Joel
Sathre, Roger
Walczak, Karl
Greenblatt, Jeffery
McKone, Thomas
TI Net primary energy balance of a solar-driven photoelectrochemical
water-splitting device
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID LIFE-CYCLE ASSESSMENT; HYDROGEN-PRODUCTION; CHALLENGES; FUTURE;
ELECTROCATALYSTS; ELECTRODES; SYSTEMS
AB A fundamental requirement for a renewable energy generation technology is that it should produce more energy during its lifetime than is required to manufacture it. In this study we evaluate the primary energy requirements of a prospective renewable energy technology, solar-driven photoelectrochemical (PEC) production of hydrogen from water. Using a life cycle assessment (LCA) methodology, we evaluate the primary energy requirements for upstream raw material preparation and fabrication under a range of assumptions of processes and materials. As the technology is at a very early stage of research and development, the analysis has considerable uncertainties. We consider and analyze three cases that we believe span a relevant range of primary energy requirements: 1550 MJ m(-2) (lower case), 2110 MJ m(-2) (medium case), and 3440 MJ m(-2) (higher case). We then use the medium case primary energy requirement to estimate the net primary energy balance (energy produced minus energy requirement) of the PEC device, which depends on device performance, e. g. longevity and solar-to-hydrogen (STH) efficiency. We consider STH efficiency ranging from 3% to 10% and longevity ranging from 5 to 30 years to assist in setting targets for research, development and future commercialization. For example, if STH efficiency is 3%, the longevity must be at least 8 years to yield a positive net energy. A sensitivity analysis shows that the net energy varies significantly with different assumptions of STH efficiency, longevity and thermo-efficiency of fabrication. Material choices for photoelectrodes or catalysts do not have a large influence on primary energy requirements, though less abundant materials like platinum may be unsuitable for large scale-up.
C1 [Zhai, Pei; Haussener, Sophia; Sathre, Roger; Greenblatt, Jeffery; McKone, Thomas] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
[Haussener, Sophia; Ager, Joel; Walczak, Karl] Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA USA.
[Haussener, Sophia] Ecole Polytech Fed Lausanne, Inst Engn Mech, CH-1015 Lausanne, Switzerland.
[Ager, Joel] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA.
RP Zhai, P (reprint author), Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM clarezhai@gmail.com
OI Ager, Joel/0000-0001-9334-9751
FU Lawrence Berkeley National Laboratory (LBNL); US Department of Energy
[DE-AC02-05CH11231]; Joint Center for Artificial Photosynthesis (JCAP),
a DOE Energy Innovation Hub; Office of Science of the US Department of
Energy [DE-SC0004993]
FX This research was supported by Laboratory Directed Research and
Development funding at the Lawrence Berkeley National Laboratory (LBNL),
which is operated for US Department of Energy under Contract Grant no.
DE-AC02-05CH11231 (Zhai, Ager, Sathre, Greenblatt and McKone). The work
was also supported in part by the Joint Center for Artificial
Photosynthesis (JCAP), a DOE Energy Innovation Hub, supported through
the Office of Science of the US Department of Energy under Award no.
DE-SC0004993 (Haussener and Walczak).
NR 49
TC 25
Z9 25
U1 4
U2 71
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD AUG
PY 2013
VL 6
IS 8
BP 2380
EP 2389
DI 10.1039/c3ee40880a
PG 10
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 185QB
UT WOS:000321983800010
ER
PT J
AU McDaniel, AH
Miller, EC
Arifin, D
Ambrosini, A
Coker, EN
O'Hayre, R
Chueh, WC
Tong, JH
AF McDaniel, Anthony H.
Miller, Elizabeth C.
Arifin, Darwin
Ambrosini, Andrea
Coker, Eric N.
O'Hayre, Ryan
Chueh, William C.
Tong, Jianhua
TI Sr- and Mn-doped LaAlO3-delta for solar thermochemical H-2 and CO
production
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID HYDROGEN-PRODUCTION; CYCLES; OXIDE; CERIA; FERRITES
AB The increasing global appetite for energy within the transportation sector will inevitably result in the combustion of more fossil fuel. A renewable-derived approach to carbon-neutral synthetic fuels is therefore needed to offset the negative impacts of this trend, which include climate change. In this communication we report the use of nonstoichiometric perovskite oxides in two-step, solar-thermochemical water or carbon dioxide splitting cycles. We find that LaAlO3 doped with Mn and Sr will efficiently split both gases. Moreover the H-2 yields are 9x greater, and the CO yields 6x greater, than those produced by the current state-of-the-art material, ceria, when reduced at 1350 degrees C and re-oxidized at 1000 degrees C. The temperature at which O-2 begins to evolve from the perovskite is fully 300 degrees C below that of ceria. The materials are also very robust, maintaining their redox activity over at least 80 CO2 splitting cycles. This discovery has profound implications for the development of concentrated solar fuel technologies.
C1 [McDaniel, Anthony H.; Miller, Elizabeth C.; Arifin, Darwin; Chueh, William C.] Sandia Natl Labs, Livermore, CA 94551 USA.
[Miller, Elizabeth C.; Ambrosini, Andrea; Coker, Eric N.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[O'Hayre, Ryan; Tong, Jianhua] Colorado Sch Mines, Golden, CO 80401 USA.
RP McDaniel, AH (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA.
EM amcdani@sandia.gov; jhtongm@gmail.com
RI Tong, Jianhua/C-8324-2016
OI Tong, Jianhua/0000-0002-0684-1658
FU DOE NNSA [DE-FC52-08NA28752]; Sandia National Laboratories Truman
Fellowship in National Security Science and Engineering; National
Science Foundation MRSEC program [DMR-0820518]; DOE Fuel Cell
Technologies Office as part of the Production technology development
area; Laboratory Directed Research and Development at Sandia National
Laboratories; United States Department of Energy's National Nuclear
Security Administration [DE-AC04-94AL85000]
FX E.C.M. was supported by a DOE NNSA Stewardship Science Graduate
Fellowship, grant number DE-FC52-08NA28752. W. C. C. was supported by an
appointment to the Sandia National Laboratories Truman Fellowship in
National Security Science and Engineering. Work conducted at Colorado
School of Mines was supported by the National Science Foundation MRSEC
program under grant no. DMR-0820518. Work at Sandia was supported by the
DOE Fuel Cell Technologies Office as part of the Production technology
development area, and by Laboratory Directed Research and Development at
Sandia National Laboratories. Sandia is a multi-program laboratory
operated by Sandia Corporation, a Lockheed Martin Company, for the
United States Department of Energy's National Nuclear Security
Administration under Contract DE-AC04-94AL85000.
NR 25
TC 72
Z9 73
U1 12
U2 130
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD AUG
PY 2013
VL 6
IS 8
BP 2424
EP 2428
DI 10.1039/c3ee41372a
PG 5
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 185QB
UT WOS:000321983800013
ER
PT J
AU Shirpour, M
Cabana, J
Doeff, M
AF Shirpour, Mona
Cabana, Jordi
Doeff, Marca
TI New materials based on a layered sodium titanate for dual
electrochemical Na and Li intercalation systems
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID SOLID-ELECTROLYTE INTERPHASE; LITHIUM-ION BATTERIES; ENERGY-STORAGE;
RECHARGEABLE BATTERIES; CRYSTAL-STRUCTURE; ANODE; INSERTION; TIO2;
STABILITY; NA2TI3O7
AB The electrochemical properties of materials derived from NaTi3O6(OH)center dot 2H(2)O have been investigated for the first time. The parent compound has a corrugated layered structure consisting of {Ti6O14}(4-) units with hydrated sodium cations and protons in the interlayer spaces. Upon heating to 600 degrees C, water is removed irreversibly, the interlayer distances become smaller, and connecting bonds between the octahedral layers form. It was found that this material can reversibly intercalate both lithium and sodium. The initial specific discharge capacities, as measured in half-cells, varied with the state of hydration and the nature of the counter electrode (Na or Li). The electrochemical potential showed a non-linear sloping dependence with degree of intercalation, indicative of a solid-solution mechanism of intercalation. The process was centered at a low average potential of about 0.3 V vs. Na or Li, the lowest ever reported for titanate-based Li hosts. The higher density and potential for higher rate capability of this compound, in comparison to carbonaceous materials with similar voltage and reversible capacities, make a compelling case for its development as an anode material, for both lithium and sodium ion batteries.
C1 [Shirpour, Mona; Cabana, Jordi; Doeff, Marca] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
RP Shirpour, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM MShirpour@lbl.gov
RI Cabana, Jordi/G-6548-2012;
OI Cabana, Jordi/0000-0002-2353-5986; Doeff, Marca/0000-0002-2148-8047
FU Laboratory Directed Research and Development Program of Lawrence
Berkeley National Laboratory under U.S. Department of Energy
[DE-AC02-05CH11231]
FX This work was supported by the Laboratory Directed Research and
Development Program of Lawrence Berkeley National Laboratory under U.S.
Department of Energy Contract DE-AC02-05CH11231.
NR 56
TC 74
Z9 74
U1 20
U2 293
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD AUG
PY 2013
VL 6
IS 8
BP 2538
EP 2547
DI 10.1039/c3ee41037d
PG 10
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 185QB
UT WOS:000321983800027
ER
PT J
AU Kelkar, S
Srinivasan, G
Robinson, BA
Roback, R
Viswanathan, H
Rehfeldt, K
Tucci, P
AF Kelkar, S.
Srinivasan, G.
Robinson, B. A.
Roback, R.
Viswanathan, H.
Rehfeldt, K.
Tucci, P.
TI Breakthrough of contaminant plumes in saturated volcanic rock:
implications from the Yucca Mountain site
SO GEOFLUIDS
LA English
DT Review
DE contaminant transport; fractured rock; plumes; saturated zone;
transverse dispersion
ID RIVER PLAIN AQUIFER; FRACTURED POROUS-MEDIA; SOLUTE TRANSPORT;
STOCHASTIC-ANALYSIS; RADIONUCLIDE MIGRATION; TRANSVERSE DISPERSION;
ZONE; MODEL; FLOW; SORPTION
AB This manuscript addresses the topic of transverse dispersion and its impact on the behavior of the saturated zone below Yucca Mountain, a site that had been proposed for a US nuclear waste repository. Guided by a review of relevant observations of dispersion in similar formations, this study evaluates the importance of uncertainty in dispersion, particularly dispersion transverse to the mean transport direction, on metrics of interest to the Yucca Mountain risk assessment. Although as expected, larger values of transverse dispersivity lead to greater spreading of the plume in directions orthogonal to the mean flow direction, a corresponding sensitivity is not observed to the travel time statistics of the breakthrough curve at the compliance boundary. Thus, when a risk assessment is based on contaminant mass flux at compliance well or 'fence line' downstream from the source, as in the Yucca Mountain case, transverse dispersion may be of secondary importance to other parameters that more directly impact travel times. This result is in contrast to systems in which reactive transport processes are important to the attenuation of the plume, in which case transverse dispersion and mixing may be expected to play a dominant role in controlling the reaction rates and contaminant concentrations in the plume.
C1 [Kelkar, S.; Srinivasan, G.; Robinson, B. A.; Roback, R.; Viswanathan, H.; Rehfeldt, K.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Tucci, P.] US Geol Survey, Denver, CO 80225 USA.
RP Kelkar, S (reprint author), Los Alamos Natl Lab, MS T003,EES 16, Los Alamos, NM 87545 USA.
EM kelkar@lanl.gov
OI Roback, Robert/0000-0003-2748-1580
FU US Department of Energy [DE-AC04-94AL85000, DE-AI28-02RW12167]
FX This manuscript has been authored by Los Alamos National Laboratory,
under contract to Sandia National Laboratories under Contract
DE-AC04-94AL85000 with the US Department of Energy, and the United
States Geological Survey, under interagency agreement number
DE-AI28-02RW12167 with the US Department of Energy. The statements
expressed in this article are those of the authors and do not
necessarily reflect the views or policies of the United States
Department of Energy, Sandia National Laboratories, and Los Alamos
National Laboratory. Additionally, Gary LeCain of the US Geological
Survey participated in this study by reviewing the literature and
summarizing the results for several of the sites included in the study,
and Bill Arnold of Sandia National Laboratories provided the authors
with insights on the performance assessment studies for Yucca Mountain.
The authors would also like to acknowledge the efforts of the anonymous
reviewers, whose editorial and substantive comments greatly improve the
quality of the manuscript.
NR 48
TC 0
Z9 1
U1 1
U2 18
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1468-8115
J9 GEOFLUIDS
JI Geofluids
PD AUG
PY 2013
VL 13
IS 3
BP 273
EP 282
DI 10.1111/gfl.12035
PG 10
WC Geochemistry & Geophysics; Geology
SC Geochemistry & Geophysics; Geology
GA 187ZI
UT WOS:000322160100001
ER
PT J
AU Han, WS
Lu, M
McPherson, BJ
Keating, EH
Moore, J
Park, E
Watson, ZT
Jung, NH
AF Han, W. S.
Lu, M.
McPherson, B. J.
Keating, E. H.
Moore, J.
Park, E.
Watson, Z. T.
Jung, N. -H.
TI Characteristics of CO2-driven cold-water geyser, Crystal Geyser in Utah:
experimental observation and mechanism analyses
SO GEOFLUIDS
LA English
DT Article
DE CO2; geologic CO2 sequestration; geyser; Navajo Sandstone; seismicity
ID CO2 GEOLOGICAL STORAGE; YELLOWSTONE-NATIONAL-PARK; EARTH TIDAL FORCES;
CARBON-DIOXIDE; BAROMETRIC-PRESSURE; INDUSTRIAL ANALOGS; TECTONIC
STRESSES; MAMMOTH MOUNTAIN; GAS-RESERVOIRS; LEAKAGE
AB Geologic carbon capture and storage (CCS) is an option for reducing CO2 emissions, but leakage to the surface is a risk factor. Natural CO2 reservoirs that erupt from abandoned oil and gas holes leak to the surface as spectacular cold geysers in the Colorado Plateau, United States. A better understanding of the mechanisms of CO2-driven cold-water geysers will provide valuable insight about the potential modes of leakage from engineered CCS sites. A notable example of a CO2-driven cold-water geyser is Crystal Geyser in central Utah. We investigated the fluid mechanics of this regularly erupting geyser by instrumenting its conduit with sensors and measuring pressure and temperature every 20 sec over a period of 17 days. Analyses of these measurements suggest that the timescale of a single-eruption cycle is composed of four successive eruption types with two recharge periods ranging from 30 to 40 h. Current eruption patterns exhibit a bimodal distribution, but these patterns evolved during past 80 years. The field observation suggests that the geyser's eruptions are regular and predictable and reflect pressure and temperature changes resulting from Joule-Thomson cooling and endothermic CO2 exsolution. The eruption interval between multiple small-scale eruptions is a direct indicator of the subsequent large-scale eruption.
C1 [Han, W. S.; Watson, Z. T.; Jung, N. -H.] Univ Wisconsin, Dept Geosci, Milwaukee, WI 53201 USA.
[Lu, M.] CSIRO, Div Earth Sci & Resource Engn, Clayton North, Vic, Australia.
[McPherson, B. J.] Univ Utah, Dept Civil & Environm Engn, Salt Lake City, UT USA.
[Keating, E. H.] Los Alamos Natl Lab, Dept Computat Geosci, Los Alamos, NM USA.
[Moore, J.] Univ Utah, Energy & Geosci Inst, Salt Lake City, UT USA.
[Park, E.] Kyungpook Natl Univ, Dept Geol, Taegu, South Korea.
RP Han, WS (reprint author), Univ Wisconsin, Dept Geosci, POB 413,Lapham Hall 366, Milwaukee, WI 53201 USA.
EM hanw@uwm.edu
FU National Science Foundation [EAR-1246404]; Korea National Oil
Corporation; Korea Institute of Energy Technology Evaluation and
Planning [2011T100100331]
FX The authors would like to thank an anonymous reviewer and Jim Evans for
their technical review and Amir Mijatovic and Rich Esser for assisting
field work. All financial support for this research was provided by both
National Science Foundation (EAR-1246404) and Korea National Oil
Corporation funded by the Korea Institute of Energy Technology
Evaluation and Planning (2011T100100331).
NR 88
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Z9 15
U1 1
U2 34
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1468-8115
J9 GEOFLUIDS
JI Geofluids
PD AUG
PY 2013
VL 13
IS 3
BP 283
EP 297
DI 10.1111/gfl.12018
PG 15
WC Geochemistry & Geophysics; Geology
SC Geochemistry & Geophysics; Geology
GA 187ZI
UT WOS:000322160100002
ER
PT J
AU DasGupta, S
Kaplar, RJ
Atcitty, S
Marinella, MJ
AF DasGupta, Sandeepan
Kaplar, Robert J.
Atcitty, Stanley
Marinella, Matthew J.
TI Photocapacitance Decay Technique for Interface Trap Characterization
Near Inversion Band in Wide Bandgap MOS Capacitors
SO IEEE TRANSACTIONS ON ELECTRON DEVICES
LA English
DT Article
DE Metal-oxide-semiconductor (MOS); photocapacitance; wide bandgap
ID FIELD-EFFECT TRANSISTORS; SILICON-CARBIDE; 4H-SIC MOSFETS; NITRIC-OXIDE;
DENSITIES; MOBILITY; DEVICES; STATES; 4H
AB A technique to characterize interface traps near the minority carrier band for wide bandgap metal-oxide-semiconductor (MOS) capacitors at room temperature is presented. The method uses photogeneration of minority carriers and transient analysis of the subsequent photocapacitance decay to evaluate trap response times. The technique is demonstrated using n-type substrate 6H-SiC/SiO2 MOS capacitors to extract interface trap density (D-it) ranging in energy from 0.2 to 0.8 eV above the valence band edge (E-nu) and trap cross sections from 0.4 to 0.7 eV above E-nu. For the given material system, traps near Ev exhibit significant differences between n- and p-type substrate MOS capacitors.
C1 [DasGupta, Sandeepan; Kaplar, Robert J.; Atcitty, Stanley; Marinella, Matthew J.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP DasGupta, S (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM sdasgup@sandia.gov; rjkapla@sandia.gov; satcitt@sandia.gov;
mmarine@sandia.gov
FU Sandia National Laboratories, a multiprogram laboratory managed by the
Sandia Corporation, a wholly owned subsidiary of Lockheed Martin
Corporation, the U.S. Department of Energy's National Nuclear Security
Administration [DE-AC0494AL85000]; DOE Energy Storage Program
FX This work was supported in part by the Sandia National Laboratories, a
multiprogram laboratory managed by the Sandia Corporation, a wholly
owned subsidiary of Lockheed Martin Corporation, the U.S. Department of
Energy's National Nuclear Security Administration under Contract
DE-AC0494AL85000, and the DOE Energy Storage Program managed by Dr. Imre
Gyuk of the DOE Office of Electricity. The review of this paper was
arranged by Editor Z. Celik-Butler.
NR 33
TC 0
Z9 0
U1 2
U2 21
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9383
EI 1557-9646
J9 IEEE T ELECTRON DEV
JI IEEE Trans. Electron Devices
PD AUG
PY 2013
VL 60
IS 8
BP 2619
EP 2625
DI 10.1109/TED.2013.2270287
PG 7
WC Engineering, Electrical & Electronic; Physics, Applied
SC Engineering; Physics
GA 187MV
UT WOS:000322124100029
ER
PT J
AU Nerva, JG
Genzale, CL
Kook, S
Garcia-Oliver, JM
Pickett, LM
AF Nerva, Jean-Guillaume
Genzale, Caroline L.
Kook, Sanghoon
Garcia-Oliver, Jose M.
Pickett, Lyle M.
TI Fundamental spray and combustion measurements of soy methyl-ester
biodiesel
SO INTERNATIONAL JOURNAL OF ENGINE RESEARCH
LA English
DT Article
DE Biodiesel; soy methyl-ester; liquid length; spray penetration; ignition;
lift-off length; soot volume fraction; spray combustion modelling;
diesel engine
ID LIQUID-PHASE PENETRATION; HSDI DIESEL-ENGINE; SOOT FORMATION; FUEL;
PRESSURE; STABILIZATION; TEMPERATURE; EMISSIONS; IGNITION; FLAME
AB Although biodiesel has begun to penetrate the fuel market, its effect on injection processes, combustion and emission formation under diesel engine conditions remains somewhat unclear. Typical exhaust measurements from engines running biodiesel indicate that particulate matter, carbon monoxide and unburnt hydrocarbons are decreased, whereas nitrogen oxide emissions tend to be increased. However, these observations are the result of complex interactions between physical and chemical processes occurring in the combustion chamber, for which understanding is still needed. To characterize and decouple the physical and chemical influences of biodiesel on spray mixing, ignition, combustion and soot formation, a soy methyl-ester (SME) biodiesel is injected into a constant-volume combustion facility under diesel-like operating conditions. A range of optical diagnostics is performed, comparing biodiesel to a conventional #2 diesel at the same injection and ambient conditions. Schlieren high-speed imaging shows virtually the same vapour-phase penetration for the two fuels, while simultaneous Mie-scatter imaging shows that the maximum liquid-phase penetration of biodiesel is higher than diesel. Differences in the liquid-phase penetration are expected because of the different boiling-point temperatures of the two fuels. However, the different liquid-phase penetration does not affect overall mixing rate and downstream vapour-phase penetration because each fuel spray has similar momentum and spreading angle. For the biodiesel and diesel samples used in this study, the ignition delay and lift-off length are only slightly less for biodiesel compared to diesel, consistent with the fuel cetane number (51 for biodiesel, 46 for diesel). Because of the similarity in lift-off length, the differences in equivalence ratio distribution at the lift-off length are mainly affected by the oxygen content of the fuels. For biodiesel, the equivalence ratio is reduced, which, along with the fuel molecular structure and oxygen content, significantly affects soot formation downstream. Spatially resolved soot volume fraction measurements obtained by combining line-of-sight laser extinction measurements with planar laser-induced incandescence imaging show that the soot concentration can be reduced by an order of magnitude for biodiesel. These integrated measurements of spray mixing, combustion and quantitative soot concentration provide new validation data for the development of computational fluid dynamics spray, combustion and soot formation models suitable for the latest biofuels.
C1 [Nerva, Jean-Guillaume; Garcia-Oliver, Jose M.] Univ Politecn Valencia, CMT Motores Term, Valencia 46022, Spain.
[Genzale, Caroline L.] Georgia Inst Technol, GW Woodruff Sch Mech Engn, Atlanta, GA 30332 USA.
[Kook, Sanghoon] Univ New S Wales, Sch Mech & Mfg Engn, Sydney, NSW 2052, Australia.
[Pickett, Lyle M.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA.
RP Nerva, JG (reprint author), Univ Politecn Valencia, CMT Motores Term, Edificio 6D,Camino Vera S-N, Valencia 46022, Spain.
EM jeaner1@mot.upv.es
RI Garcia-Oliver, Jose/L-6517-2014; Kook, Sanghoon/C-5372-2009
OI Garcia-Oliver, Jose/0000-0002-2676-9681; Kook,
Sanghoon/0000-0002-7620-9789
FU Spanish Ministry of Science and Innovation through the OPTICOMB project
[TRA2007-67961-C03-01]
FX This work was supported by the Spanish Ministry of Science and
Innovation for Jean-Guillaume Nerva's visiting research, through the
OPTICOMB project [TRA2007-67961-C03-01].
NR 66
TC 19
Z9 20
U1 3
U2 33
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1468-0874
J9 INT J ENGINE RES
JI Int. J. Engine Res.
PD AUG
PY 2013
VL 14
IS 4
BP 373
EP 390
DI 10.1177/1468087412456688
PG 18
WC Thermodynamics; Engineering, Mechanical; Transportation Science &
Technology
SC Thermodynamics; Engineering; Transportation
GA 188NB
UT WOS:000322198600006
ER
PT J
AU Shade, A
Caporaso, JG
Handelsman, J
Knight, R
Fierer, N
AF Shade, Ashley
Caporaso, J. Gregory
Handelsman, Jo
Knight, Rob
Fierer, Noah
TI A meta-analysis of changes in bacterial and archaeal communities with
time
SO ISME JOURNAL
LA English
DT Article
DE similarity-decay; species-time relationship; beta diversity; 16S rRNA;
turnover; high-throughput sequencing
ID MICROBIAL COMMUNITIES; ECOLOGICAL COMMUNITIES; DISTANCE-DECAY; TEMPORAL
VARIABILITY; SPECIES RICHNESS; GLOBAL PATTERNS; RARE BIOSPHERE;
EUTROPHIC LAKE; DIVERSITY; DYNAMICS
AB Ecologists have long studied the temporal dynamics of plant and animal communities with much less attention paid to the temporal dynamics exhibited by microbial communities. As a result, we do not know if overarching temporal trends exist for microbial communities or if changes in microbial communities are generally predictable with time. Using microbial time series assessed via high-throughput sequencing, we conducted a meta-analysis of temporal dynamics in microbial communities, including 76 sites representing air, aquatic, soil, brewery wastewater treatment, human- and plant-associated microbial biomes. We found that temporal variability in both within- and between-community diversity was consistent among microbial communities from similar environments. Community structure changed systematically with time in less than half of the cases, and the highest rates of change were observed within ranges of 1 day to 1 month for all communities examined. Microbial communities exhibited species-time relationships (STRs), which describe the accumulation of new taxa to a community, similar to those observed previously for plant and animal communities, suggesting that STRs are remarkably consistent across a broad range of taxa. These results highlight that a continued integration of microbial ecology into the broader field of ecology will provide new insight into the temporal patterns of microbial and 'macro'-bial communities alike.
C1 [Shade, Ashley; Handelsman, Jo] Yale Univ, Dept Mol Cellular & Dev Biol, New Haven, CT USA.
[Caporaso, J. Gregory] No Arizona Univ, Dept Comp Sci, Flagstaff, AZ 86011 USA.
[Caporaso, J. Gregory] Argonne Natl Lab, Argonne, IL 60439 USA.
[Knight, Rob] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA.
[Knight, Rob] Univ Colorado, Biofrontiers Inst, Boulder, CO 80309 USA.
[Knight, Rob] Univ Colorado, Howard Hughes Med Inst, Boulder, CO 80309 USA.
[Fierer, Noah] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA.
[Fierer, Noah] Univ Colorado, Dept Ecol & Evolut Biol, Boulder, CO 80309 USA.
RP Fierer, N (reprint author), Univ Colorado, Cooperat Inst Res Environm Sci, 216 UCB, Boulder, CO 80309 USA.
EM noah.fierer@colorado.edu
RI Knight, Rob/D-1299-2010;
OI Shade, Ashley/0000-0002-7189-3067
FU National Science Foundation; US Department of Agriculture; Howard Hughes
Medical Institute; National Institutes of Health
FX This work would not have been possible without the generosity and
collaborative spirit of the many primary authors of the data sets
included in the meta-analysis. AS is a Gordon and Betty Moore Foundation
Fellow of the Life Sciences Research Foundation. We thank Petr Keil for
insightful discussions. We thank Jack Gilbert for the Western English
Channel dataset, and Jack Gilbert and Trina McMahon for the lakes
dataset. NF was supported by funding from the National Science
Foundation and the US Department of Agriculture. RK was supported, in
part, by the Howard Hughes Medical Institute and the National Institutes
of Health.
NR 98
TC 80
Z9 84
U1 23
U2 293
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 1751-7362
EI 1751-7370
J9 ISME J
JI ISME J.
PD AUG
PY 2013
VL 7
IS 8
BP 1493
EP 1506
DI 10.1038/ismej.2013.54
PG 14
WC Ecology; Microbiology
SC Environmental Sciences & Ecology; Microbiology
GA 187LF
UT WOS:000322119600004
PM 23575374
ER
PT J
AU Pint, BA
AF Pint, B. A.
TI High-Temperature Corrosion in Fossil Fuel Power Generation: Present and
Future
SO JOM
LA English
DT Article
ID COAL-FIRED BOILERS; NI-CR ALLOYS; OXIDATION BEHAVIOR; WATER-VAPOR;
GAS-TURBINES; MATERIALS TECHNOLOGY; STEAM OXIDATION; PLANTS; COATINGS;
COMBUSTION
AB Fossil fuels have historically represented two-thirds of all electricity generation in the United States and are projected to continue to play a similar role despite historically low projected growth rates in electricity demand and the recent dramatic shift from coal to more natural gas usage. Economic and environmental drivers will require more reliable and efficient fossil fuel generation systems in the future, likely with new system designs, higher operating temperatures, and more aggressive environments. Some of the current corrosion issues in power plants are reviewed along with research on materials solutions for systems envisioned for the near future, such as coal gasification and oxy-fired coal boilers.
C1 Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RP Pint, BA (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
EM pintba@ornl.gov
RI Pint, Bruce/A-8435-2008
OI Pint, Bruce/0000-0002-9165-3335
FU Electric Power Research Institute (EPRI); U.S. Department of Energy,
Office of Fossil Energy, Advanced Research Materials Program; Office of
Coal and Power RD
FX The research shown was sponsored by the Electric Power Research
Institute (EPRI) and the U.S. Department of Energy, Office of Fossil
Energy, Advanced Research Materials Program and the Office of Coal and
Power R&D. The author is grateful from insights gained from discussions
with I.G. Wright, R. Klueh, and P.J. Maziasz at ORNL; V. Cedro, R.
Dennis, and B. White at NETL; J. Shingledecker at EPRI; B. Nagaraj at
General Electric; A. Kulkarni at Siemens; and S. Sampath at Stonybrook
University. The author is thankful also for the assistance of S.
Dryepondt, J. Thomson, G. Garner, T. Lowe, H. Longmire, and T. Jordan
with the experimental work at ORNL. P. F. Tortorelli and M. P. Brady at
ORNL provided helpful comments on the manuscript.
NR 54
TC 15
Z9 15
U1 5
U2 45
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1047-4838
J9 JOM-US
JI JOM
PD AUG
PY 2013
VL 65
IS 8
BP 1024
EP 1032
DI 10.1007/s11837-013-0642-z
PG 9
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering; Mineralogy; Mining & Mineral Processing
SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy;
Mining & Mineral Processing
GA 187RN
UT WOS:000322136400018
ER
PT J
AU Caro, M
Woloshun, K
Rubio, F
Maloy, SA
Hosemann, P
AF Caro, M.
Woloshun, K.
Rubio, F.
Maloy, S. A.
Hosemann, P.
TI Heavy Liquid Metal Corrosion of Structural Materials in Advanced Nuclear
Systems
SO JOM
LA English
DT Article
ID COOLED FAST-REACTOR; BISMUTH EUTECTIC SYSTEMS; FLOWING LEAD-BISMUTH; 450
DEGREES-C; PB-BI; MOLTEN LEAD; STAINLESS-STEEL; EROSION TEST;
FUEL-CYCLE; DESIGN
AB Interest in advanced nuclear concepts using liquid metal coolant has increased in the past few years. Liquid metal coolants have been proposed for the next generation of small-sized nuclear reactors, which offer exceptional safety and reliability, sustainability, nonproliferation, and economic competitiveness. Heavy liquid metal coolants are investigated for advanced fast reactors that operate at high temperatures, reaching high efficiencies. Lead and lead-bismuth eutectic (LBE) coolants are also proposed as coolants and targets of accelerator driven systems. High temperature, corrosive environment, high fast neutron flux, high fluence, and radiation damage, among other physical phenomena, challenge the integrity of materials in these advanced systems. Excellent compatibility with the liquid coolant is recognized as a key factor in the selection of structural materials for advanced concepts. In this article, we review materials requirements for heavy metal cooled systems with emphasis on lead and LBE materials corrosion properties. We describe experimental corrosion tests currently ongoing at the Los Alamos National Laboratory (LANL) Development of Lead Alloy Technical Applications (DELTA) loop. DELTA is a facility designed to study the long-term corrosive effects of LBE on structural materials under relevant conditions of chemistry, flow, and temperature. The research studies will provide data of corrosion rates and corrosion mechanisms in selected steel exposed to high velocity (above 2 m/s) in flowing LBE at 500A degrees C. Fundamental research studies will help support conceptual design efforts and further the development of heavy liquid metals technology.
C1 [Caro, M.; Woloshun, K.; Rubio, F.; Maloy, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Hosemann, P.] Univ Calif Berkeley, Berkeley, CA 94720 USA.
RP Caro, M (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM magda@lanl.gov
RI Maloy, Stuart/A-8672-2009;
OI Maloy, Stuart/0000-0001-8037-1319; Hosemann, Peter/0000-0003-2281-2213
FU NRC faculty development grant [NRC-38-09-948]; Department of Energy
[DE-EE0005941]
FX The work described here summarizes the contribution of the effort of
several people and institutions in the United States and abroad. The
test matrix selection is the result of numerous fruitful discussions.
The authors want to thank the NRC faculty development grant number
NRC-38-09-948. This material is also partially based on work supported
by the Department of Energy under Award Number DE-EE0005941.
NR 83
TC 5
Z9 5
U1 4
U2 53
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1047-4838
J9 JOM-US
JI JOM
PD AUG
PY 2013
VL 65
IS 8
BP 1057
EP 1066
DI 10.1007/s11837-013-0663-7
PG 10
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering; Mineralogy; Mining & Mineral Processing
SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy;
Mining & Mineral Processing
GA 187RN
UT WOS:000322136400021
ER
PT J
AU Lin, YL
Zhao, M
Ming, Y
Golaz, JC
Donner, LJ
Klein, SA
Ramaswamy, V
Xie, SC
AF Lin, Yanluan
Zhao, Ming
Ming, Yi
Golaz, Jean-Christophe
Donner, Leo J.
Klein, Stephen A.
Ramaswamy, V.
Xie, Shaocheng
TI Precipitation Partitioning, Tropical Clouds, and Intraseasonal
Variability in GFDL AM2
SO JOURNAL OF CLIMATE
LA English
DT Article
DE Climate models; Convective parameterization; Intraseasonal variability
ID MADDEN-JULIAN OSCILLATION; GENERAL-CIRCULATION MODELS; STATIC ENERGY
BUDGET; LARGE-SCALE MODELS; CONVECTIVE PARAMETERIZATION;
ARAKAWA-SCHUBERT; ECMWF MODEL; ATMOSPHERE; FREQUENCY; WAVES
AB A set of Geophysical Fluid Dynamics Laboratory (GFDL) Atmospheric Model version 2 (AM2) sensitivity simulations by varying an entrainment threshold rate to control deep convection occurrence are used to investigate how cumulus parameterization impacts tropical cloud and precipitation characteristics. In the tropics, model convective precipitation (CP) is frequent and light, while large-scale precipitation (LSP) is intermittent and strong. With deep convection inhibited, CP decreases significantly over land and LSP increases prominently over ocean. This results in an overall redistribution of precipitation from land to ocean. A composite analysis reveals that cloud fraction (low and middle) and cloud condensate associated with LSP are substantially larger than those associated with CP. With about the same total precipitation and precipitation frequency distribution over the tropics, simulations having greater LSP fraction tend to have larger cloud condensate and low and middle cloud fraction.Simulations having a greater LSP fraction tend to be drier and colder in the upper troposphere. The induced unstable stratification supports strong transient wind perturbations and LSP. Greater LSP also contributes to greater intraseasonal (20-100 days) precipitation variability. Model LSP has a close connection to the low-level convergence via the resolved grid-scale dynamics and, thus, a close coupling with the surface heat flux. Such wind-evaporation feedback is essential to the development and maintenance of LSP and enhances model precipitation variability. LSP has stronger dependence and sensitivity on column moisture than CP. The moisture-convection feedback, critical to tropical intraseasonal variability, is enhanced in simulations with large LSP. Strong precipitation variability accompanied by a worse mean state implies that an optimal precipitation partitioning is critical to model tropical climate simulation.
C1 [Lin, Yanluan; Zhao, Ming] Univ Corp Atmospheric Res, Boulder, CO USA.
[Lin, Yanluan; Zhao, Ming; Ming, Yi; Golaz, Jean-Christophe; Donner, Leo J.; Ramaswamy, V.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA.
[Klein, Stephen A.; Xie, Shaocheng] Lawrence Livermore Natl Lab, Livermore, CA USA.
RP Lin, YL (reprint author), Princeton Univ, NOAA, Geophys Fluid Dynam Lab, Forrestal Campus,POB 308, Princeton, NJ 08540 USA.
EM yanluan.lin@noaa.gov
RI Ming, Yi/F-3023-2012; Golaz, Jean-Christophe/D-5007-2014; lin,
yanluan/A-6333-2015; Xie, Shaocheng/D-2207-2013; Zhao, Ming/C-6928-2014;
Klein, Stephen/H-4337-2016
OI Golaz, Jean-Christophe/0000-0003-1616-5435; Xie,
Shaocheng/0000-0001-8931-5145; Klein, Stephen/0000-0002-5476-858X
FU Office of Science (BER), U.S. Department of Energy; Office of Science at
the U.S. Department of Energy; U.S. Department of Energy by the Lawrence
Livermore National Laboratory [DE-AC52-07NA27344]
FX This research is supported by the Office of Science (BER), U.S.
Department of Energy (Lin). Support for S. A. Klein and S. Xie was
provided by the Atmospheric System Research and Regional and Global
Climate Modeling Programs of the Office of Science at the U.S.
Department of Energy. Their contribution to this work was performed
under the auspices of the U.S. Department of Energy by the Lawrence
Livermore National Laboratory under contract DE-AC52-07NA27344. We are
grateful to Dr. Waliser for providing us with the ice retrievals from
CloudSat. We thank Hiram Levy II and Huan Guo for their comments on the
manuscript. We also acknowledge the three anonymous reviewers for their
constructive comments, which significantly improved the organization and
clarity of the paper.
NR 53
TC 5
Z9 5
U1 2
U2 10
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0894-8755
EI 1520-0442
J9 J CLIMATE
JI J. Clim.
PD AUG
PY 2013
VL 26
IS 15
BP 5453
EP 5466
DI 10.1175/JCLI-D-12-00442.1
PG 14
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 190GP
UT WOS:000322327700009
ER
PT J
AU Song, H
Lin, WY
Lin, YL
Wolf, AB
Neggers, R
Donner, LJ
Del Genio, AD
Liu, YG
AF Song, Hua
Lin, Wuyin
Lin, Yanluan
Wolf, Audrey B.
Neggers, Roel
Donner, Leo J.
Del Genio, Anthony D.
Liu, Yangang
TI Evaluation of Precipitation Simulated by Seven SCMs against the ARM
Observations at the SGP Site
SO JOURNAL OF CLIMATE
LA English
DT Article
DE Model comparison; Model evaluation; performance; Single column models
ID SINGLE-COLUMN MODEL; GENERAL-CIRCULATION MODELS; LARGE-SCALE MODELS;
COMMUNITY ATMOSPHERE MODEL; DIURNAL CYCLE; CUMULUS PARAMETERIZATION;
CONVECTIVE PRECIPITATION; CLIMATE SIMULATIONS; MOIST CONVECTION;
GREAT-PLAINS
AB This study evaluates the performances of seven single-column models (SCMs) by comparing simulated surface precipitation with observations at the Atmospheric Radiation Measurement Program Southern Great Plains (SGP) site from January 1999 to December 2001. Results show that although most SCMs can reproduce the observed precipitation reasonably well, there are significant and interesting differences in their details. In the cold season, the model-observation differences in the frequency and mean intensity of rain events tend to compensate each other for most SCMs. In the warm season, most SCMs produce more rain events in daytime than in nighttime, whereas the observations have more rain events in nighttime. The mean intensities of rain events in these SCMs are much stronger in daytime, but weaker in nighttime, than the observations. The higher frequency of rain events during warm-season daytime in most SCMs is related to the fact that most SCMs produce a spurious precipitation peak around the regime of weak vertical motions but rich in moisture content. The models also show distinct biases between nighttime and daytime in simulating significant rain events. In nighttime, all the SCMs have a lower frequency of moderate-to-strong rain events than the observations for both seasons. In daytime, most SCMs have a higher frequency of moderate-to-strong rain events than the observations, especially in the warm season. Further analysis reveals distinct meteorological backgrounds for large underestimation and overestimation events. The former occur in the strong ascending regimes with negative low-level horizontal heat and moisture advection, whereas the latter occur in the weak or moderate ascending regimes with positive low-level horizontal heat and moisture advection.
C1 [Song, Hua; Lin, Wuyin; Lin, Yanluan; Liu, Yangang] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Lin, Yanluan; Donner, Leo J.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA.
[Wolf, Audrey B.] Columbia Univ, New York, NY USA.
[Neggers, Roel] Royal Netherlands Meteorol Inst, NL-3730 AE De Bilt, Netherlands.
[Del Genio, Anthony D.] NASA Goddard Inst Space Studies, New York, NY USA.
RP Song, H (reprint author), Brookhaven Natl Lab, Div Atmospher Sci, 75 Rutherford Dr,Bldg 815E, Upton, NY 11973 USA.
EM hsong@bnl.gov
RI Liu, Yangang/H-6154-2011; lin, yanluan/A-6333-2015
FU U.S. Department of Energy Earth System Modeling (ESM) program
FX This work is part of the FASTER project (http://www.bnl.gov/faster/)
supported by the U.S. Department of Energy Earth System Modeling (ESM)
program. The authors thank the two anonymous reviewers for their
constructive comments. The first author also would like to express her
sincere gratitude to her former advisor Dr. Minghua Zhang for his
incessant support and encouragement throughout her research.
NR 60
TC 12
Z9 12
U1 0
U2 16
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0894-8755
J9 J CLIMATE
JI J. Clim.
PD AUG
PY 2013
VL 26
IS 15
BP 5467
EP 5492
DI 10.1175/JCLI-D-12-00263.1
PG 26
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 190GP
UT WOS:000322327700010
ER
PT J
AU Xin, HLL
Dwyer, C
Muller, DA
Zheng, HM
Ercius, P
AF Xin, Huolin L.
Dwyer, Christian
Muller, David A.
Zheng, Haimei
Ercius, Peter
TI Scanning Confocal Electron Energy-Loss Microscopy Using Valence-Loss
Signals
SO MICROSCOPY AND MICROANALYSIS
LA English
DT Article; Proceedings Paper
CT 10th EMAS Regional Workshop
CY JUN 17-20, 2012
CL Padua, ITALY
DE scanning confocal electron energy-loss microscopy; inelastic confocal;
aberration-corrected electron microscopy; chromatic aberration
correction
ID INELASTICALLY SCATTERED ELECTRONS; SPATIAL-FREQUENCY CUTOFFS;
IMAGE-FORMATION; BRIGHT-FIELD; ATOMIC-SCALE; RESOLUTION; 3D; TOMOGRAPHY;
STEM; PROSPECTS
AB Finding a faster alternative to tilt-series electron tomography is critical for rapidly evolving fields such as the semiconductor industry, where failure analysis could greatly benefit from higher throughput. We present a theoretical and experimental evaluation of scanning confocal electron energy-loss microscopy (SCEELM) using valence-loss signals, which is a promising technique for the reliable reconstruction of materials with sub-10-nm resolution. Such a confocal geometry transfers information from the focused portion of the electron beam and enables rapid three-dimensional (3D) reconstruction by depth sectioning. SCEELM can minimize or eliminate the missing-information cone and the elongation problem that are associated with other depth-sectioning image techniques in a transmission electron microscope. Valence-loss SCEELM data acquisition is an order of magnitude faster and requires little postprocessing compared with tilt-series electron tomography. With postspecimen chromatic aberration (C-c) correction, SCEELM signals can be acquired in parallel in the direction of energy dispersion with the aid of a physical pinhole. This increases the efficiency by 10X-100X, and can provide 3D resolved chemical information for multiple core-loss signals simultaneously.
C1 [Xin, Huolin L.; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Dwyer, Christian] Monash Univ, Monash Ctr Electron Microscopy, ARC Ctr Excellence Design Light Met, Dept Mat Engn, Clayton, Vic 3800, Australia.
[Muller, David A.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14850 USA.
[Muller, David A.] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14850 USA.
[Ercius, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA.
RP Xin, HLL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM hxin@lbl.gov; percius@lbl.gov
RI Xin, Huolin/E-2747-2010; Muller, David/A-7745-2010
OI Xin, Huolin/0000-0002-6521-868X; Muller, David/0000-0003-4129-0473
FU Materials Sciences Division, Lawrence Berkeley National Laboratory; U.S.
Department of Energy (DOE) [DE-AC02-05CH11231]
FX Research was support by Materials Sciences Division, Lawrence Berkeley
National Laboratory. Electron microscopy facilities in National Center
for Electron Microscopy at Lawrence Berkeley National Laboratory was
supported by the U.S. Department of Energy (DOE) under Contract
#DE-AC02-05CH11231.
NR 48
TC 4
Z9 4
U1 1
U2 30
PU CAMBRIDGE UNIV PRESS
PI NEW YORK
PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA
SN 1431-9276
EI 1435-8115
J9 MICROSC MICROANAL
JI Microsc. microanal.
PD AUG
PY 2013
VL 19
IS 4
BP 1036
EP 1049
DI 10.1017/S1431927613001438
PG 14
WC Materials Science, Multidisciplinary; Microscopy
SC Materials Science; Microscopy
GA 182SP
UT WOS:000321764700031
PM 23692691
ER
PT J
AU Van Weverberg, K
AF Van Weverberg, Kwinten
TI Impact of Environmental Instability on Convective Precipitation
Uncertainty Associated with the Nature of the Rimed Ice Species in a
Bulk Microphysics Scheme
SO MONTHLY WEATHER REVIEW
LA English
DT Article
DE Cloud microphysics; Convective storms; Cloud parameterizations; Cloud
resolving models; Numerical weather prediction; forecasting;
Parameterization
ID SIMULATED SQUALL LINE; VERTICAL WIND SHEAR; PARAMETERIZATION; STORMS;
SIZE
AB Despite a number of studies dedicated to the sensitivity of deep convection simulations to the properties of the rimed ice species in microphysics schemes, no consensus has been achieved on the nature of the impact. Considering the need for improved quantitative precipitation forecasts, it is crucial that the cloud modeling community better understands the reasons for these differing conclusions and knows the relevance of these sensitivities for the numerical weather prediction. This study examines the role of environmental conditions and storm type on the sensitivity of precipitation simulations to the nature of the rimed ice species (graupel or hail). Idealized 3D simulations of supercells/multicells and squall lines have been performed in varying thermodynamic environments. It has been shown that for simulation periods of sufficient length (>2 h), graupel-containing and hail-containing storms produce domain-averaged surface precipitation that is more similar than many earlier studies suggest. While graupel is lofted to higher altitudes and has a longer residence time aloft than hail, these simulations suggest that most of this graupel eventually reaches the surface and the surface precipitation rates of hail- and graupel-containing storms converge. However, environmental conditions play an important role in the magnitude of this sensitivity. Storms in large-CAPE environments (typical of storms in the U.S. Midwest) are more sensitive than their low-CAPE counterparts (typical of storms in Europe) to the nature of the rimed ice species in terms of domain-average surface precipitation. Supercells/multicells are more sensitive than squall lines to the nature of the rimed ice species in terms of spatial precipitation distribution and peak precipitation, disregarding of the amount of CAPE.
C1 [Van Weverberg, Kwinten] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Van Weverberg, Kwinten] Catholic Univ Louvain, B-1348 Louvain, Belgium.
RP Van Weverberg, K (reprint author), Catholic Univ Louvain, Georges Lemaitre Ctr Earth & Climate Res, SC10-L4-03-08 Mercator,Pl Louis Pasteur 3, B-1348 Louvain, Belgium.
EM kwinten.vanweverberg@uclouvain.be
FU U.S. Department of Energy's Atmospheric System Research (ASR), an Office
of Science Program; Earth System Modeling Program via the Fast-Physics
System Testbed and Research (FASTER) project
FX This research was supported by the U.S. Department of Energy's
Atmospheric System Research (ASR), an Office of Science Program, and by
the Earth System Modeling Program via the Fast-Physics System Testbed
and Research (FASTER) project (www.bnl.gov/esm). The author is grateful
to Andy M. Vogelmann for stimulating discussions and to H. Morrison for
assistance with the cold pool initiation of the squall-line simulations.
NR 16
TC 7
Z9 7
U1 0
U2 9
PU AMER METEOROLOGICAL SOC
PI BOSTON
PA 45 BEACON ST, BOSTON, MA 02108-3693 USA
SN 0027-0644
J9 MON WEATHER REV
JI Mon. Weather Rev.
PD AUG
PY 2013
VL 141
IS 8
BP 2841
EP 2849
DI 10.1175/MWR-D-13-00036.1
PG 9
WC Meteorology & Atmospheric Sciences
SC Meteorology & Atmospheric Sciences
GA 188VR
UT WOS:000322225200015
ER
PT J
AU Haudry, A
Platts, AE
Vello, E
Hoen, DR
Leclercq, M
Williamson, RJ
Forczek, E
Joly-Lopez, Z
Steffen, JG
Hazzouri, KM
Dewar, K
Stinchcombe, JR
Schoen, DJ
Wang, XW
Schmutz, J
Town, CD
Edger, PP
Pires, JC
Schumaker, KS
Jarvis, DE
Mandakova, T
Lysak, MA
van den Bergh, E
Schranz, ME
Harrison, PM
Moses, AM
Bureau, TE
Wright, SI
Blanchette, M
AF Haudry, Annabelle
Platts, Adrian E.
Vello, Emilio
Hoen, Douglas R.
Leclercq, Mickael
Williamson, Robert J.
Forczek, Ewa
Joly-Lopez, Zoe
Steffen, Joshua G.
Hazzouri, Khaled M.
Dewar, Ken
Stinchcombe, John R.
Schoen, Daniel J.
Wang, Xiaowu
Schmutz, Jeremy
Town, Christopher D.
Edger, Patrick P.
Pires, J. Chris
Schumaker, Karen S.
Jarvis, David E.
Mandakova, Terezie
Lysak, Martin A.
van den Bergh, Erik
Schranz, M. Eric
Harrison, Paul M.
Moses, Alan M.
Bureau, Thomas E.
Wright, Stephen I.
Blanchette, Mathieu
TI An atlas of over 90,000 conserved noncoding sequences provides insight
into crucifer regulatory regions
SO NATURE GENETICS
LA English
DT Article
ID ARABIDOPSIS-THALIANA; HUMAN GENOME; DNA ELEMENTS; ULTRACONSERVED
ELEMENTS; BRASSICA-OLERACEA; GENE-EXPRESSION; EVOLUTION; DROSOPHILA;
SIZE; ANNOTATION
AB Despite the central importance of noncoding DNA to gene regulation and evolution, understanding of the extent of selection on plant noncoding DNA remains limited compared to that of other organisms. Here we report sequencing of genomes from three Brassicaceae species (Leavenworthia alabamica, Sisymbrium irio and Aethionema arabicum) and their joint analysis with six previously sequenced crucifer genomes. Conservation across orthologous bases suggests that at least 17% of the Arabidopsis thaliana genome is under selection, with nearly one-quarter of the sequence under selection lying outside of coding regions. Much of this sequence can be localized to approximately 90,000 conserved noncoding sequences (CNSs) that show evidence of transcriptional and post-transcriptional regulation. Population genomics analyses of two crucifer species, A. thaliana and Capsella grandiflora, confirm that most of the identified CNSs are evolving under medium to strong purifying selection. Overall, these CNSs highlight both similarities and several key differences between the regulatory DNA of plants and other species.
C1 [Haudry, Annabelle; Williamson, Robert J.; Hazzouri, Khaled M.; Stinchcombe, John R.; Moses, Alan M.; Wright, Stephen I.] Univ Toronto, Dept Ecol & Evolutionary Biol, Toronto, ON, Canada.
[Haudry, Annabelle] Univ Lyon 1, CNRS, UMR 5558, Lab Biometrie & Biol Evolut, F-69622 Villeurbanne, France.
[Platts, Adrian E.; Vello, Emilio; Leclercq, Mickael; Blanchette, Mathieu] McGill Univ, Sch Comp Sci, Montreal, PQ, Canada.
[Platts, Adrian E.; Vello, Emilio; Leclercq, Mickael; Blanchette, Mathieu] McGill Univ, McGill Ctr Bioinformat, Montreal, PQ, Canada.
[Hoen, Douglas R.; Forczek, Ewa; Joly-Lopez, Zoe; Schoen, Daniel J.; Harrison, Paul M.; Bureau, Thomas E.] McGill Univ, Dept Biol, Montreal, PQ H3A 1B1, Canada.
[Steffen, Joshua G.] Colby Sawyer Coll, Nat Sci Dept, New London, NH USA.
[Dewar, Ken] McGill Univ, Dept Human Genet, Montreal, PQ, Canada.
[Wang, Xiaowu] Chinese Acad Agr Sci, Inst Vegetables & Flowers, Beijing 100193, Peoples R China.
[Schmutz, Jeremy] US DOE, Joint Genome Inst, Walnut Creek, CA USA.
[Schmutz, Jeremy] HudsonAlpha Inst Biotechnol, Huntsville, AL USA.
[Town, Christopher D.] J Craig Venter Inst, Rockville, MD USA.
[Edger, Patrick P.; Pires, J. Chris] Univ Missouri, Div Biol Sci, Columbia, MO 65211 USA.
[Schumaker, Karen S.; Jarvis, David E.] Univ Arizona, Sch Plant Sci, Tucson, AZ USA.
[Mandakova, Terezie; Lysak, Martin A.] Masaryk Univ, Cent European Inst Technol CEITEC, Brno, Czech Republic.
[van den Bergh, Erik; Schranz, M. Eric] Wageningen Univ, Biosystemat Grp, NL-6700 AP Wageningen, Netherlands.
[Wright, Stephen I.] Univ Toronto, Ctr Anal Genome Evolut & Funct, Toronto, ON, Canada.
RP Blanchette, M (reprint author), McGill Univ, Sch Comp Sci, Montreal, PQ, Canada.
EM alan.moses@utoronto.ca; thomas.bureau@mcgill.ca;
stephen.wright@utoronto.ca; blanchem@cs.mcgill.ca
RI Lysak, Martin/D-2439-2014; Wright, Stephen/C-3113-2008; Haudry,
Annabelle/A-1887-2013; Mandakova, Terezie/E-1365-2012; Schranz,
Michael/D-7155-2017; Stinchcombe, John/A-2941-2008; Platts,
Adrian/H-5633-2013; Schmutz, Jeremy/N-3173-2013;
OI Lysak, Martin/0000-0003-0318-4194; Wright, Stephen/0000-0001-9973-9697;
Schranz, Michael/0000-0001-6777-6565; Stinchcombe,
John/0000-0003-3349-2964; Platts, Adrian/0000-0001-9238-9647; Schmutz,
Jeremy/0000-0001-8062-9172; van den Bergh, Erik/0000-0001-9865-574X;
Pires, J Chris/0000-0001-9682-2639; Williamson,
Robert/0000-0001-9732-0964
FU Genome Canada/Genome Quebec; European Regional Development Fund
[CZ.1.05/1.1.00/02.0068]; Czech Science Foundation [P501/12/G090];
National Science Foundation (NSF) [0929262]; Netherlands Organisation
for Scientific Research
FX We would like to thank the US Department of Energy Joint Genome
Institute (for the C. rubella genome sequence, produced under a
Community Sequencing Program (CSP) proposal submitted by D. Weigel and
colleagues, and the E. salsugineum genome sequence, produced under a CSP
proposal submitted by K. Schumaker, R. Wing and T. Mitchell-Olds) and R.
Clark (for A. lyrata mRNA sequencing). We also thank S.-C. Chantha for
assistance with genome sequencing in L. alabamica, S. Joly for
suggestions on the genomic DNA isolation protocol and D. Scofield for
helpful discussions about intron-exon structure. We thank M. Freeling,
D. Weigel, E. Harmsen and I. Lacroix for comments on the manuscript.
This project was funded by a Genome Canada/Genome Quebec grant to T. E.
B., S. I. W., M. B., J.S., A. M. M., D.J.S. and P. M. H. In addition, T.
M. and M. A. L. were supported by the European Regional Development Fund
(CZ.1.05/1.1.00/02.0068) and by the Czech Science Foundation (excellence
cluster P501/12/G090). J.G.S. was supported by National Science
Foundation (NSF) award 0929262. M. E. S. and E.v.d.B. were supported by
a Vidi grant from the Netherlands Organisation for Scientific Research.
NR 95
TC 94
Z9 95
U1 2
U2 84
PU NATURE PUBLISHING GROUP
PI NEW YORK
PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA
SN 1061-4036
J9 NAT GENET
JI Nature Genet.
PD AUG
PY 2013
VL 45
IS 8
BP 891
EP U228
DI 10.1038/ng.2684
PG 10
WC Genetics & Heredity
SC Genetics & Heredity
GA 190WW
UT WOS:000322374900011
PM 23817568
ER
PT J
AU Soukoulis, CM
AF Soukoulis, Costas M.
TI Greece in crisis
SO NATURE MATERIALS
LA English
DT Editorial Material
C1 [Soukoulis, Costas M.] Iowa State Univ, Dept Phys, Ames, IA 50011 USA.
[Soukoulis, Costas M.] Ames Lab, Ames, IA 50011 USA.
[Soukoulis, Costas M.] Univ Crete, Dept Mat Sci & Engn, Iraklion, Greece.
RP Soukoulis, CM (reprint author), Iowa State Univ, Dept Phys, Ames, IA 50011 USA.
EM soukouli@iastate.edu
NR 4
TC 1
Z9 1
U1 0
U2 14
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 1476-1122
J9 NAT MATER
JI Nat. Mater.
PD AUG
PY 2013
VL 12
IS 8
BP 683
EP 685
DI 10.1038/nmat3727
PG 3
WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics,
Applied; Physics, Condensed Matter
SC Chemistry; Materials Science; Physics
GA 187LB
UT WOS:000322119100002
PM 23877387
ER
PT J
AU Wang, YM
Sansoz, F
LaGrange, T
Ott, RT
Marian, J
Barbee, TW
Hamza, AV
AF Wang, Y. Morris
Sansoz, Frederic
LaGrange, Thomas
Ott, Ryan T.
Marian, Jaime
Barbee, Troy W., Jr.
Hamza, Alex V.
TI Defective twin boundaries in nanotwinned metals
SO NATURE MATERIALS
LA English
DT Article
ID DEFORMATION MECHANISMS; PLASTIC-DEFORMATION; MAXIMUM STRENGTH; COPPER;
ORIENTATION; ANISOTROPY; NANOSCALE
AB Coherent twin boundaries (CTBs) are widely described, both theoretically and experimentally, as perfect interfaces that play a significant role in a variety of materials. Although the ability of CTBs in strengthening, maintaining the ductility and minimizing the electron scattering is well documented(1-3), most of our understanding of the origin of these properties relies on perfect-interface assumptions. Here we report experiments and simulations demonstrating that as-grown CTBs in nanotwinned copper are inherently defective with kink-like steps and curvature, and that these imperfections consist of incoherent segments and partial dislocations. We further show that these defects play a crucial role in the deformation mechanisms and mechanical behaviour of nanotwinned copper. Our findings offer a view of the structure of CTBs that is largely different from that in the literature(2,4,5), and underscore the significance of imperfections in nanotwin-strengthened materials.
C1 [Wang, Y. Morris; LaGrange, Thomas; Marian, Jaime; Barbee, Troy W., Jr.; Hamza, Alex V.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
[Sansoz, Frederic] Univ Vermont, Sch Engn, Burlington, VT 05405 USA.
[Ott, Ryan T.] Ames Lab USDOE, Div Engn & Mat Sci, Ames, IA 50011 USA.
RP Wang, YM (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
EM ymwang@llnl.gov
RI Wang, Yinmin (Morris)/F-2249-2010
OI Wang, Yinmin (Morris)/0000-0002-7161-2034
FU US Department of Energy (DOE) by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]; Ames Laboratory (Office of Basic Energy Sciences)
[DE-AC02-07CH11358]; US DOE [DE-AC02-06CH11357]; NSF CAREER program
[DMR-0747658]; Vermont Advanced Computing Centre (NASA) [NNX06AC88G]; US
DOE Early Career Research Program
FX The authors thank V. Bulatov and A. Stukowski for helpful discussions,
and M. Besser, J. Almer, N. Teslich and R. Gross for experimental
assistance. This work was performed under the auspices of the US
Department of Energy (DOE) by Lawrence Livermore National Laboratory
under Contract No. DE-AC52-07NA27344, and Ames Laboratory (Office of
Basic Energy Sciences) under Contract No. DE-AC02-07CH11358. The use of
APS was supported by the US DOE under Contract No. DE-AC02-06CH11357.
F.S. is grateful for support from the NSF CAREER program (grant
DMR-0747658) and the computational resources provided by the Vermont
Advanced Computing Centre (NASA grant NNX06AC88G). T.L. and IPFOM
measurements are supported by US DOE, Office of Basic Energy Sciences.
J.M. acknowledges financial support from the US DOE Early Career
Research Program.
NR 31
TC 81
Z9 82
U1 18
U2 221
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 1476-1122
J9 NAT MATER
JI Nat. Mater.
PD AUG
PY 2013
VL 12
IS 8
BP 697
EP 702
DI 10.1038/NMAT3646
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics,
Applied; Physics, Condensed Matter
SC Chemistry; Materials Science; Physics
GA 187LB
UT WOS:000322119100013
PM 23685864
ER
EF