FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Hlushak, SP Cummings, PT McCabe, C AF Hlushak, S. P. Cummings, P. T. McCabe, C. TI Comparison of several classical density functional theories for the adsorption of flexible chain molecules into cylindrical nanopores SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MEAN SPHERICAL MODEL; NONUNIFORM POLYATOMIC SYSTEMS; FUNDAMENTAL-MEASURE-THEORY; CHARGED HARD-SPHERES; WHITE BEAR VERSION; PERTURBATION-THEORY; INHOMOGENEOUS FLUIDS; SQUARE-WELL; MIXTURES; APPROXIMATION AB Adsorption of flexible oligomers into narrow cylindrical pores has been studied by means of several versions of classical density functional theory (CDFT) and Monte Carlo simulation. The adsorption process is interesting to study due to the competition between the entropic depletion of oligomers from the pores and the wall-oligomer attraction. It is also challenging to describe using current CDFTs, which tend to overestimate the amount of the adsorbed fluid. From a comparison of several different CDFT approaches, we find that this is due to the assumption of ideal or freely jointed chain conformations. Moreover, it is demonstrated that it is impossible to obtain a reasonable description of the adsorption isotherms without taking into account accurate contact values in the distribution functions describing the structure of the reference monomer fluid. At low densities, more accurate result are obtained in comparison with Monte Carlo simulation data when accurate contact values are incorporated into the theory rather than the more commonly used hard-sphere contact value. However, even the CDFT with accurate contact values still overestimates the amount of the adsorbed fluid due to the ideal or freely jointed chain approximation, used for the description of chain conformations in most CDFT approaches. We find that significant improvement can achieved by employing self-consistent field theory, which samples self-avoiding chain conformations and decreases the number of possible chain conformations, and, consequently, the amount of the adsorbed fluid. (C) 2013 AIP Publishing LLC. C1 [Hlushak, S. P.; Cummings, P. T.; McCabe, C.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. [Hlushak, S. P.] Inst Condensed Matter Phys, UA-79011 Lvov, Ukraine. [Cummings, P. T.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [McCabe, C.] Vanderbilt Univ, Dept Chem, Nashville, TN 37235 USA. RP Hlushak, SP (reprint author), Vanderbilt Univ, Dept Chem & Biomol Engn, 221 Kirkland Hall, Nashville, TN 37235 USA. EM stepan.hlushak@gmail.com RI McCabe, Clare/I-8017-2012 OI McCabe, Clare/0000-0002-8552-9135 FU Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy FX The authors acknowledge support from the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. NR 60 TC 1 Z9 1 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD DEC 21 PY 2013 VL 139 IS 23 AR 234902 DI 10.1063/1.4843655 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 282RV UT WOS:000329191300043 PM 24359388 ER PT J AU Edwards, TG Hung, I Gan, Z Kalkan, B Raoux, S Sen, S AF Edwards, T. G. Hung, I. Gan, Z. Kalkan, B. Raoux, S. Sen, S. TI Structural transformations in amorphous <-> crystalline phase change of Ga-Sb alloys SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ADIABATIC PULSES; CHANGE MEMORY; DATA-STORAGE; NMR; SENSITIVITY; ACQUISITION; PRESSURE; EXAFS AB Ga-Sb alloys with compositions ranging between similar to 12 and 50 at. % Ga are promising materials for phase change random access memory applications. The short-range structures of two such alloys with compositions Ga14Sb86 and Ga46Sb54 are investigated, in their amorphous and crystalline states, using Ga-71 and Sb-121 nuclear magnetic resonance spectroscopy and synchrotron x-ray diffraction. The Ga and Sb atoms are fourfold coordinated in the as-deposited amorphous Ga46Sb54 with nearly 40% of the constituent atoms being involved in Ga-Ga and Sb-Sb homopolar bonding. This necessitates extensive bond switching and elimination of homopolar bonds during crystallization. On the other hand, Ga and Sb atoms are all threefold coordinated in the as-deposited amorphous Ga14Sb86. Crystallization of this material involves phase separation of GaSb domains in Sb matrix and a concomitant increase in the Ga coordination number from 3 to 4. Results from crystallization kinetics experiments suggest that the melt-quenching results in the elimination of structural "defects" such as the homopolar bonds and threefold coordinated Ga atoms in the amorphous phases of these alloys, thereby rendering them structurally more similar to the corresponding crystalline states compared to the as-deposited amorphous phases. (C) 2013 AIP Publishing LLC. C1 [Edwards, T. G.; Sen, S.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Hung, I.; Gan, Z.] Natl High Magnet Field Lab, Ctr Interdisciplinary Magnet Resonance, Tallahassee, FL 32310 USA. [Kalkan, B.] Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 20015 USA. [Raoux, S.] IBM Corp, TJ Watson Res Ctr, Yorktown Hts, NY 10598 USA. RP Edwards, TG (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. RI Gan, Zhehong/C-2400-2011; Raoux, Simone/G-3920-2016 FU National Science Foundation [NSF GOALI 1104869, DMR-0084173]; State of Florida; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DEAC02-05CH11231] FX This work was funded by a grant from the National Science Foundation (NSF GOALI 1104869). The National High Magnetic Field Laboratory is supported through the National Science Foundation Cooperative Agreement (DMR-0084173) and by the State of Florida. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) under Contract No. DEAC02-05CH11231. NR 34 TC 2 Z9 2 U1 4 U2 32 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 21 PY 2013 VL 114 IS 23 AR 233512 DI 10.1063/1.4854575 PG 7 WC Physics, Applied SC Physics GA 280UR UT WOS:000329056800022 ER PT J AU Mastandrea, JP Sherburne, MP Boswell-Koller, CN Sawyer, CA Guzman, J Bustillo, KC Ager, JW Haller, EE Chrzan, DC AF Mastandrea, J. P. Sherburne, M. P. Boswell-Koller, C. N. Sawyer, C. A. Guzman, J. Bustillo, K. C. Ager, J. W., III Haller, E. E. Chrzan, D. C. TI Self-consistent mean-field theory of size distribution narrowing during ramped temperature ion beam synthesis SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NANOCRYSTALS; IMPLANTATION; GROWTH AB A simple mathematical argument explains a recently identified route for the ion beam synthesis of nanoclusters with a narrowed size distribution. The key idea is that growth conditions for which the average nanocluster size is increasing rapidly can lead to narrowed size distributions. Modeling candidate processes using a self-consistent, mean-field theory shows that normalized nanocluster size distributions with full-width at half-maximum of 17% of the average can be attained. (C) 2013 AIP Publishing LLC. C1 [Mastandrea, J. P.; Sherburne, M. P.; Boswell-Koller, C. N.; Sawyer, C. A.; Guzman, J.; Bustillo, K. C.; Haller, E. E.; Chrzan, D. C.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Mastandrea, J. P.; Sherburne, M. P.; Boswell-Koller, C. N.; Sawyer, C. A.; Guzman, J.; Bustillo, K. C.; Ager, J. W., III; Haller, E. E.; Chrzan, D. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Mastandrea, JP (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. OI Ager, Joel/0000-0001-9334-9751 FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-A02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-A02-05CH11231. NR 18 TC 1 Z9 1 U1 0 U2 18 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 21 PY 2013 VL 114 IS 23 AR 234301 DI 10.1063/1.4846737 PG 7 WC Physics, Applied SC Physics GA 280UR UT WOS:000329056800046 ER PT J AU Peyronel, F Ilavsky, J Mazzanti, G Marangoni, AG Pink, DA AF Peyronel, Fernanda Ilavsky, Jan Mazzanti, Gianfranco Marangoni, Alejandro G. Pink, David A. TI Edible oil structures at low and intermediate concentrations. II. Ultra-small angle X-ray scattering of in situ tristearin solids in triolein SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ADVANCED PHOTON SOURCE; FAT CRYSTAL NETWORKS; FRACTAL NATURE; MECHANICAL-PROPERTIES; SCALING BEHAVIOR; MILK-FAT; NANOSCALE; RHEOLOGY; MODEL; MICROSTRUCTURE AB Ultra-small angle X-ray scattering has been used for the first time to elucidate, in situ, the aggregation structure of a model edible oil system. The three-dimensional nano-to micro-structure of tristearin solid particles in triolein solvent was investigated using 5, 10, 15, and 20% solids. Three different sample preparation procedures were investigated: two slow cooling rates of 0.5 degrees/min, case 1 (22 days of storage at room temperature) and case 2 (no storage), and one fast cooling of 30 degrees/min, case 3 (no storage). The length scale investigated, by using the Bonse-Hart camera at beamline ID-15D at the Advanced Photon Source, Argonne National Laboratory, covered the range from 300 angstrom to 10 mu m. The unified fit and the Guinier-Porod models in the Irena software were used to fit the data. The former was used to fit 3 structural levels. Level 1 structures showed that the primary scatterers were essentially 2-dimensional objects for the three cases. The scatterers possessed lateral dimensions between 1000 and 4300 angstrom. This is consistent with the sizes of crystalline nanoplatelets present which were observed using cryo-TEM. Level 2 structures were aggregates possessing radii of gyration, R-g2 between 1800 angstrom and 12000 angstrom and fractal dimensions of either D-2 = 1 for case 3 or 1.8 <= D-2 <= 2.1 for case 1 and case 2. D-2 = 1 is consistent with unaggregated 1-dimensional objects. 1.8 <= D-2 <= 2.1 is consistent with these 1-dimensional objects (below) forming structures characteristic of diffusion or reaction limited cluster-cluster aggregation. Level 3 structures showed that the spatial distribution of the level 2 structures was uniform, on the average, for case 1, with fractal dimension D-3 approximate to 3 while for case 2 and case 3 the fractal dimension was D-3 approximate to 2.2, which suggested that the large-scale distribution had not come to equilibrium. The Guinier-Porod model showed that the structures giving rise to the aggregates with a fractal dimension given by D-2 in the unified fit level 2 model were cylinders described by the parameter s approximate to 1 in the Guinier-Porod model. The size of the base of these cylinders was in agreement with the cryo-TEM observations as well as with the results of the level 1 unified fit model. By estimating the size of the nanoplatelets and understanding the structures formed via their aggregation, it will be possible to engineer novel lipids systems that embody desired functional characteristics. VC 2013 AIP Publishing LLC. C1 [Peyronel, Fernanda; Marangoni, Alejandro G.; Pink, David A.] Univ Guelph, Dept Food Sci, Guelph, ON N1G 2W1, Canada. [Ilavsky, Jan] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Mazzanti, Gianfranco] Dalhousie Univ, Dept Proc Engn & Appl Sci, Halifax, NS B3H 4R2, Canada. [Pink, David A.] St Francis Xavier Univ, Dept Phys, Antigonish, NS B2G 2W5, Canada. RP Peyronel, F (reprint author), Univ Guelph, Dept Food Sci, Guelph, ON N1G 2W1, Canada. RI USAXS, APS/D-4198-2013 FU NSERC; National Science Foundation/Department of Energy [NSF/CHE-0822838]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX It is a pleasure for D. A. P. to thank Ms. Bonnie Quinn (St. Francis Xavier University) and Dr. Shajahan Razul (ACEnet and St. FXU) for their collaborations. Thanks also to NSERC for grants and to ACEnet for ample computing time and technical advice. ChemMatCARS Sector 15 is principally supported by the National Science Foundation/Department of Energy under Grant No. NSF/CHE-0822838. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 42 TC 17 Z9 17 U1 2 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 21 PY 2013 VL 114 IS 23 AR 234902 DI 10.1063/1.4847997 PG 9 WC Physics, Applied SC Physics GA 280UR UT WOS:000329056800062 ER PT J AU Tringe, JW Letant, SE Dugan, LC Levie, HW Kuhl, AL Murphy, GA Alves, SW Vandersall, KS Pantoya, ML AF Tringe, J. W. Letant, S. E. Dugan, L. C. Levie, H. W. Kuhl, A. L. Murphy, G. A. Alves, S. W. Vandersall, K. S. Pantoya, M. L. TI Comparison of Bacillus atrophaeus spore viability following exposure to detonation of C4 and to deflagration of halogen-containing thermites SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INACTIVATION; ANTHRACIS; COMBUSTION; DECONTAMINATION; CALORIMETERS; DESTRUCTION; BACTERIA; WASTE AB Energetic materials are being considered for the neutralization of spore-forming bacteria. In this study, the neutralization effects of a monomolecular explosive were compared to the effects of halogen-containing thermites. Bacillus atrophaeus spores were exposed to the post-detonation environment of a 100 g charge of the military explosive C-4 at a range of 50 cm. These tests were performed in the thermodynamically closed environment of a 506-l barometric calorimeter. Associated temperatures were calculated using a thermodynamic model informed by calculations with the Cheetah thermochemical code. Temperatures in the range of 2300-2800 K were calculated to persist for nearly the full 4 ms pressure observation time. After the detonation event, spores were characterized using optical microscopy and the number of viable spores was assessed. Results showed live spore survival rates in the range of 0.01%-1%. For the thermite tests, a similar, smaller-scale configuration was employed that examined the spore neutralization effects of two thermites: aluminum with iodine pentoxide and aluminum with potassium chlorate. Only the former mixture resulted in spore neutralization. These results indicate that the detonation environment produced by an explosive with no chemical biocides may provide effective spore neutralization similar to a deflagrating thermite containing iodine. (C) 2013 AIP Publishing LLC. C1 [Tringe, J. W.; Letant, S. E.; Dugan, L. C.; Levie, H. W.; Kuhl, A. L.; Murphy, G. A.; Alves, S. W.; Vandersall, K. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Pantoya, M. L.] Texas Tech Univ, Dept Mech Engn, Lubbock, TX 79409 USA. RP Tringe, JW (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Department of Homeland Security Science and Technology Directorate [HSHQPM-10-X-00070]; Defense Threat Reduction Agency (DTRA) FX We gratefully acknowledge Dr. John Densmore for helpful discussions on temperature and pressure calculations relevant to post-detonation conditions in the barometric calorimeter, as well as Ron Chambers and Dan Greenwood for help in execution of the calorimeter experiments. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Some parts of this work were funded by the Department of Homeland Security Science and Technology Directorate under the Contract No. HSHQPM-10-X-00070. M. Pantoya gratefully acknowledges support from the Defense Threat Reduction Agency (DTRA) and encouragement from our program manager, Dr. Suhithi Peiris. NR 26 TC 2 Z9 2 U1 1 U2 11 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 21 PY 2013 VL 114 IS 23 AR 234903 DI 10.1063/1.4849835 PG 6 WC Physics, Applied SC Physics GA 280UR UT WOS:000329056800063 ER PT J AU Bubna, M Alagoz, E Cervantes, M Krzywda, A Arndt, K Obertino, M Solano, A Dalla Betta, GF Menace, D Moroni, L Uplegger, L Rivera, R Osipenkov, I Andresen, J Bolla, G Bortoletto, D Boscardin, M Brom, JM Brosius, R Chramowicz, J Cumalat, J Dinardo, M Dini, P Jensen, F Kumar, A Kwan, S Lei, CM Povoli, M Prosser, A Ngadiuba, J Perera, L Shipsey, I Tan, P Tentindo, S Terzo, S Tran, N Wagner, SR AF Bubna, Mayur Alagoz, Enver Cervantes, Mayra Krzywda, Alex Arndt, Kirk Obertino, Margherita Solano, Ada Dalla Betta, Gian-Franco Menace, Dario Moroni, Luigi Uplegger, Lorenzo Rivera, Ryan Osipenkov, Ilya Andresen, Jeff Bolla, Gino Bortoletto, Daniela Boscardin, Maurizio Brom, Jean Marie Brosius, Richard Chramowicz, John Cumalat, John Dinardo, Mauro Dini, Paolo Jensen, Frank Kumar, Ashish Kwan, Simon Lei, C. M. Povoli, Marco Prosser, Alan Ngadiuba, Jennifer Perera, Lalith Shipsey, Ian Tan, Ping Tentindo, Silvia Terzo, Stefano Nhan Tran Wagner, Stephen R. TI Testbeam and laboratory test results of irradiated 3D CMS pixel detectors SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE CMS pixel detector; LHC upgrade; 3D technology; Radiation hardness ID DESIGN AB The CMS silicon pixel detector is the tracking device closest to the LHC p-p collisions, which precisely reconstructs the charged particle trajectories. The planar technology used in the current innermost layer of the pixel detector will reach the design limit for radiation hardness at the end of Phase I upgrade and will need to be replaced before the Phase II upgrade in 2020. Due to its unprecedented performance in harsh radiation environments, 3D silicon technology is under consideration as a possible replacement of planar technology for the High Luminosity-LHC or HL-LHC. 3D silicon detectors are fabricated by the Deep Reactive-Ion-Etching (DRIE) technique which allows p- and n-type electrodes to be processed through the silicon substrate as opposed to being implanted through the silicon surface. The 3D CMS pixel devices presented in this paper were processed at FBK. They were bump bonded to the current CMS pixel readout chip, tested in the laboratory, and testbeams carried out at FNAL with the proton beam of 120 GeV/c. In this paper we present the laboratory and beam test results for the irradiated 3D CMS pixel devices. (C) 2013 CERN. Published by Elsevier B.V. All rights reserved. C1 [Bubna, Mayur; Alagoz, Enver; Cervantes, Mayra; Krzywda, Alex; Arndt, Kirk; Bolla, Gino; Bortoletto, Daniela; Shipsey, Ian] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Obertino, Margherita; Solano, Ada] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Menace, Dario; Moroni, Luigi; Dinardo, Mauro; Dini, Paolo; Ngadiuba, Jennifer; Terzo, Stefano] Ist Nazl Fis Nucl, Sez Milano Bicocca, Milan, Italy. [Menace, Dario; Moroni, Luigi; Dinardo, Mauro; Dini, Paolo; Ngadiuba, Jennifer] Univ Milano Bicocca, I-20126 Milan, Italy. [Uplegger, Lorenzo; Rivera, Ryan; Andresen, Jeff; Chramowicz, John; Kwan, Simon; Lei, C. M.; Prosser, Alan; Tan, Ping; Nhan Tran] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Cumalat, John; Jensen, Frank; Wagner, Stephen R.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Brosius, Richard; Kumar, Ashish] SUNY Buffalo, Dept Phys, Buffalo, NY 14260 USA. [Osipenkov, Ilya] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Perera, Lalith] Univ Mississippi, Dept Phys & Astron, University, MS 38677 USA. [Povoli, Marco] INFN Padova, Grp Coll Trento, Padua, Italy. [Dalla Betta, Gian-Franco] Univ Trento, Dipartimento Ingn & Sci Informaz, I-38123 Povo, TN, Italy. [Boscardin, Maurizio] FBK, Ctr Mat & Microsistemi, I-38123 Povo, TN, Italy. [Bubna, Mayur] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Brom, Jean Marie] Strasbourg IPHC, Inst Pluriedisciplinaire Hubert Curien, F-67037 Strasbourg, France. [Tentindo, Silvia] Florida State Univ, Tallahassee, FL 32306 USA. RP Alagoz, E (reprint author), Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. EM enver.alagoz@cern.ch RI Dalla Betta, Gian-Franco/I-1783-2012; Boscardin, Maurizio/A-4420-2014; OI Dalla Betta, Gian-Franco/0000-0001-5516-9282; Arndt, Kirk/0000-0002-6826-8340; Terzo, Stefano/0000-0003-3388-3906 NR 16 TC 1 Z9 1 U1 0 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 52 EP 56 DI 10.1016/j.nima.2013.07.042 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400011 ER PT J AU Giubilato, P Bisello, D Chalmet, P Denes, P Kloukinas, K Mattiazzo, S Marchioro, A Mugnier, H Pantano, D Potenza, A Rivetti, A Rousset, J Snoeys, W Tindall, C AF Giubilato, P. Bisello, D. Chalmet, P. Denes, P. Kloukinas, K. Mattiazzo, S. Marchioro, A. Mugnier, H. Pantano, D. Potenza, A. Rivetti, A. Rousset, J. Snoeys, W. Tindall, C. TI LePix-A high resistivity, fully depleted monolithic pixel detector SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE CMOS; Monolithic; Pixels; Detector; X-ray ID BEAM AB The LePix project explores monolithic pixel sensors fabricated in a 90 nm CMOS technology built over a lightly doped substrate. This approach keeps the advantages usually offered by Monolithic Active Pixel Sensors (MAPS), like a low input capacitance, having a single piece detector and using a standard CMOS production line, and adds the benefit of charge collection by drift from a depleted region several tens of microns deep into the substrate, therefore providing an excellent signal to noise ratio and a radiation tolerance superior to conventional un-depleted MAPS. Such sensors are expected to offer significant cost savings and reduction of power consumption for the same performance, leading to the use of much less material in the detector (less cooling and less copper), addressing one of the main limitations of present day particle tracking systems. The latest evolution of the project uses detectors thinned down to 50 mu m to obtain back illuminated sensors operated in full depletion mode. By back processing the chip and collecting the charge from the full substrate it is hence possible to efficiently detect soft X-rays up to 10 keV. Test results from first successfully processed detectors will be presented and discussed. (C) 2013 Elsevier B.V. All rights reserved. C1 [Giubilato, P.; Bisello, D.; Mattiazzo, S.; Pantano, D.; Potenza, A.; Rivetti, A.] INFN Padova, Padua, Italy. [Giubilato, P.; Bisello, D.; Mattiazzo, S.; Pantano, D.] Univ Padua, Dipartimento Fis, I-35131 Padua, Italy. [Potenza, A.] Univ Turin, Dipartimento Fis, Turin, Italy. [Kloukinas, K.; Marchioro, A.; Snoeys, W.] CERN, Geneva, Switzerland. [Chalmet, P.; Mugnier, H.; Rousset, J.] MIND Micro Technol, Bat Archamps, France. [Denes, P.; Tindall, C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Giubilato, P (reprint author), Univ Padua, Dipartimento Fis, Via Marzolo 8, I-35131 Padua, Italy. EM piero.giubilato@gmail.com RI Snoeys, Walter/K-8259-2015; OI Snoeys, Walter/0000-0003-3541-9066; Giubilato, Piero/0000-0003-4358-5355 NR 8 TC 1 Z9 1 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 91 EP 94 DI 10.1016/j.nima.2013.05.189 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400020 ER PT J AU Antonioli, MA Boiarinov, S Bonneau, P Elouadrhiri, L Eng, B Gotra, Y Kurbatov, E Leffel, M Mandal, S McMullen, M Merkin, M Raydo, B Teachey, W Tucker, R Ungaro, M Yegneswaran, A Ziegler, V AF Antonioli, M. A. Boiarinov, S. Bonneau, P. Elouadrhiri, L. Eng, B. Gotra, Y. Kurbatov, E. Leffel, M. Mandal, S. McMullen, M. Merkin, M. Raydo, B. Teachey, W. Tucker, R. Ungaro, M. Yegneswaran, A. Ziegler, V. TI Performance of the CLAS12 Silicon Vertex Tracker modules SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE Tracking and position-sensitive detectors; Solid-state detectors; Hybrid integrated circuits AB For the 12 GeV upgrade, the CLAS12 experiment has designed a Silicon Vertex Tracker (SVT) using single sided microstrip sensors fabricated by Hamamatsu. The sensors have graded angle design to minimize dead areas and a readout pitch of 156 mu m, with intermediate strip. Double sided SVT module hosts three daisy-chained sensors On each side with a full strip length of 33 cm. There are 512 channels per module read out by four Fermilab Silicon Strip Readout (FSSR2) chips featuring data driven architecture, mounted on a rigid-flex hybrid. Modules are assembled on the barrel using unique cantilevered geometry to minimize the amount of material in the tracking volume. Design and performance of the SVT modules are presented, focusing on results of electrical measurements. (C) 2013 Elsevier B.V. All rights reserved. C1 [Antonioli, M. A.; Boiarinov, S.; Bonneau, P.; Elouadrhiri, L.; Eng, B.; Gotra, Y.; Leffel, M.; Mandal, S.; McMullen, M.; Raydo, B.; Teachey, W.; Ungaro, M.; Yegneswaran, A.; Ziegler, V.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA USA. [Kurbatov, E.; Merkin, M.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Tucker, R.] Arizona State Univ, Tempe, AZ USA. RP Gotra, Y (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA USA. EM gotra@jlab.org RI Merkin, Mikhail/D-6809-2012 NR 6 TC 1 Z9 1 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 99 EP 102 DI 10.1016/j.nima.2013.06.077 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400022 ER PT J AU Hartman, N Silber, J Anderssen, E Garcia-Sciveres, M Gilchriese, M Johnson, T Cepeda, M AF Hartman, Neal Silber, Joseph Anderssen, Eric Garcia-Sciveres, Maurice Gilchriese, Murdock Johnson, Thomas Cepeda, Mario TI Novel fabrication techniques for low-mass composite structures in silicon particle detectors SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE ATLAS; Carbon fiber composite; Detector; I-beam; Pixel; Stave AB The structural design of silicon-based particle detectors is governed by competing demands of reducing mass while maximizing stability and accuracy. These demands can only be met by fiber reinforced composite laminates (CFRP). As defecting sensors and electronics become lower mass, the motivation to reduce structure as a proportion of overall mass pushes modern detector structures to the lower limits of composite ply thickness, while demanding maximum stiffness. However, classical approaches to composite laminate design require symmetric laminates and Hat structures, in order to minimize warping during fabrication. This constraint asymmetry in laminate design, and a "flat plate" approach to fabrication, results in more massive structures. This study presents an approach to fabricating stable and accurate, geometrically complex composite structures by bonding warped, asymmetric, but ultra thin component laminates together in an accurate tool, achieving final overall precision normally associated with planar structures. This technique has been used to fabricate a prototype "I-beam" that supports two layers of detecting elements, while being up to 20 limes stiffer and up to 30% lower mass than comparable, independent planar structures (typically known as "slaves"). (C) 2013 Elsevier B.V. All rights reserved. C1 [Hartman, Neal; Silber, Joseph; Anderssen, Eric; Garcia-Sciveres, Maurice; Gilchriese, Murdock; Johnson, Thomas; Cepeda, Mario] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Hartman, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM neal.hartman@cern.ch NR 4 TC 3 Z9 3 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 103 EP 108 DI 10.1016/j.nima.2013.07.005 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400023 ER PT J AU Amole, C Andresen, GB Ashkezari, MD Baquero-Ruiz, M Bertsche, W Burrows, C Butler, E Capra, A Cesar, CL Chapman, S Charlton, M Deller, A Eriksson, S Fajans, J Friesen, T Fujiwara, MC Gill, DR Gutierrez, A Hangst, JS Hardy, WN Hayden, ME Humphries, AJ Isaac, CA Jonsell, S Kurchaninov, L Little, A Madsen, N McKenna, JTK Menary, S Napoli, SC Nolan, P Olchanski, K Olin, A Povilus, A Pusa, P Rasmussen, CO Robicheaux, F Sacramento, RL Stracka, S Sampson, JA Sarid, E Seddon, D Silveira, DM So, C Thompson, RI Tharp, T Thornhill, J Tooley, MP van der Werf, DP Wells, D AF Amole, C. Andresen, G. B. Ashkezari, M. D. Baquero-Ruiz, M. Bertsche, W. Burrows, C. Butler, E. Capra, A. Cesar, C. L. Chapman, S. Charlton, M. Deller, A. Eriksson, S. Fajans, J. Friesen, T. Fujiwara, M. C. Gill, D. R. Gutierrez, A. Hangst, J. S. Hardy, W. N. Hayden, M. E. Humphries, A. J. Isaac, C. A. Jonsell, S. Kurchaninov, L. Little, A. Madsen, N. McKenna, J. T. K. Menary, S. Napoli, S. C. Nolan, P. Olchanski, K. Olin, A. Povilus, A. Pusa, P. Rasmussen, C. O. Robicheaux, F. Sacramento, R. L. Stracka, S. Sampson, J. A. Sarid, E. Seddon, D. Silveira, D. M. So, C. Thompson, R. I. Tharp, T. Thornhill, J. . Tooley, M. P. van der Werf, D. P. Wells, D. TI Silicon vertex detector upgrade in the ALPHA experiment SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE Silicon Vertex Detector; Antihydrogen; Antimatter; Event reconstruction; Cosmic ray background suppression ID TRAPPED ANTIHYDROGEN AB The Silicon Vertex Detector (SVD) is the main diagnostic tool in the ALPHA-experiment. It provides precise spatial and timing information of antiproton (antihydrogen) annihilation events (vertices), and most importantly, the SVD is capable of directly identifying and analysing single annihilation events, thereby forming the basis of ALPHA's analysis. This paper describes the ALPHA SVD and its upgrade, installed in the ALPHA's new neutral atom trap. (C) 2013 CERN. Published by Elsevier B.V. All rights reserved. C1 [Amole, C.; Capra, A.; Menary, S.] York Univ, Dept Phys & Astron, N York, ON M3J 1P3, Canada. [Andresen, G. B.; Rasmussen, C. O.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Ashkezari, M. D.; Hayden, M. E.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Baquero-Ruiz, M.; Chapman, S.; Fajans, J.; Little, A.; Povilus, A.; So, C.; Tharp, T.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bertsche, W.; Tooley, M. P.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Bertsche, W.; Tooley, M. P.] Cockcroft Inst, Daresbuty Lab, Warrington WA4 4AD, Cheshire, England. [Burrows, C.; Charlton, M.; Deller, A.; Eriksson, S.; Humphries, A. J.; Isaac, C. A.; Madsen, N.; van der Werf, D. P.] Swansea Univ, Dept Phys, Coll Sci, Swansea SA2 8PP, W Glam, Wales. [Butler, E.] CERN, Dept Phys, CH-1211 Geneva, Switzerland. [Cesar, C. L.; Sacramento, R. L.; Silveira, D. M.] Univ Fed Rio de Janeiro, Inst Fis, BR-21941972 Rio De Janeiro, Brazil. [Fajans, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Friesen, T.; Fujiwara, M. C.; Thompson, R. I.] Univ Calgary, Dept Phys & Astron, Calgary, AB T2N 1N4, Canada. [Fujiwara, M. C.; Gill, D. R.; Kurchaninov, L.; Olchanski, K.; Olin, A.; Stracka, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Gutierrez, A.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Hardy, W. N.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. [Jonsell, S.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [McKenna, J. T. K.; Napoli, S. C.; Nolan, P.; Pusa, P.; Sampson, J. A.; Seddon, D.; Thornhill, J. .; Wells, D.] Univ Liverpool, Dept Phys, Liverpool L69 7ZE, Merseyside, England. [Robicheaux, F.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Sarid, E.] Nucl Res Ctr Negev, Dept Phys, IL-84190 Beer Sheva, Israel. RP McKenna, JTK (reprint author), Univ Liverpool, Dept Phys, Liverpool L69 7ZE, Merseyside, England. EM jtkm@ns.ph.liv.ac.uk RI Bertsche, William/A-3678-2012; Stracka, Simone/M-3931-2015; Jonsell, Svante/J-2251-2016; Fajans, Joel/J-6597-2016; Robicheaux, Francis/F-4343-2014 OI Andresen, Gorm Bruun/0000-0002-4820-020X; Bertsche, William/0000-0002-6565-9282; Stracka, Simone/0000-0003-0013-4714; Isaac, Aled/0000-0002-7813-1903; Jonsell, Svante/0000-0003-4969-1714; Fajans, Joel/0000-0002-4403-6027; van der Werf, Dirk/0000-0001-5436-5214; Robicheaux, Francis/0000-0002-8054-6040 NR 10 TC 2 Z9 2 U1 0 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 134 EP 136 DI 10.1016/j.nima.2013.05.188 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400030 ER PT J AU Canonica, L Biassoni, M Brofferio, C Bucci, C Calvano, S Di Vacri, ML Goett, J Gorla, P Pavan, M Yeh, M AF Canonica, L. Biassoni, M. Brofferio, C. Bucci, C. Calvano, S. Di Vacri, M. L. Goett, J. Gorla, P. Pavan, M. Yeh, M. TI Rejection of surface background in thermal detectors: The ABSuRD project SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE Thermal detectors; Rare events searches; Scintillation; Surface background ID PLASTIC SCINTILLATOR; LIGHT; SEARCH AB Thermal detectors have recently achieved a leading role in the fields of Neutrinoless Double Beta Decay and Dark Matter searches thanks to their excellent energy resolution and to the wide choice of absorber materials. In these fields the background coming from surface contaminations is frequently dominant. ABSuRD (A Background Surface Rejection Detector) is a scintillation-based approach for tagging this type of background. We discuss the innovative application of this technique in non-scintillating bolometric detectors which will allow for a more favorable signal to background ratio. (C) 2013 Elsevier B.V. All rights reserved. C1 [Canonica, L.; Bucci, C.; Calvano, S.; Di Vacri, M. L.; Gorla, P.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. [Biassoni, M.; Brofferio, C.; Pavan, M.] Univ Milano Bicocca, Milan, Italy. [Biassoni, M.; Brofferio, C.; Pavan, M.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Goett, J.] Los Alamos Natl Lab, Los Alamos, NM USA. [Yeh, M.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Canonica, L (reprint author), Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. EM lucia.canonica@lngs.infn.it RI Gorla, Paolo/B-5243-2014; OI Canonica, Lucia/0000-0001-8734-206X; Goett, Johnny/0000-0002-3685-2227; pavan, maura/0000-0002-9723-7834 NR 10 TC 3 Z9 3 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 286 EP 289 DI 10.1016/j.nima.2013.05.114 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400065 ER PT J AU Adams, B Elagin, A Frisch, H Obaid, R Oberla, E Vostrikov, A Wagner, R Wetstein, M AF Adams, Bernhard Elagin, Andrey Frisch, Henry Obaid, Razib Oberla, Eric Vostrikov, Alexander Wagner, Robert Wetstein, Matthew TI Measurements of the gain, time resolution, and spatial resolution of a 20 x 20 cm(2) MCP-based picosecond photo-detector SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE Microchannel plates; Photodetector s; Large-area detectors; Time-of-flight ID PMT AB Microchannel plates (MCPs) allow for micron-level spatial imaging and picosecond-level time resolution, making them a good choice for the next generation of photo-detectors aiming for precision time-of-flight measurements. The Large-Area Picosecond Photo-Detector Collaboration (LAPPD) is currently developing a 20 x 20 cm(2), thin, planar, glass-body detector with two MCPs in chevron geometry with 8 degrees bias angle. The modular design of the strip-line anode allows covering large areas while keeping the number of electronics channels low. We have built a complete detector system approximating the final detector design. We have measured a gain of up to 2 x 10(7), time-of-Bight resolution of up to 35 ps, differential time resolution of similar to 6 ps, and spatial resolution of better than 1 mm. (C) 2013 Elsevier BY. All rights reserved. C1 [Adams, Bernhard; Wagner, Robert] Argonne Natl Lab, Argonne, IL 60439 USA. [Elagin, Andrey; Frisch, Henry; Obaid, Razib; Oberla, Eric; Vostrikov, Alexander; Wetstein, Matthew] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Elagin, A (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM elagin@hep.uchicago.edu NR 11 TC 12 Z9 12 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 392 EP 396 DI 10.1016/j.nima.2013.07.091 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400089 ER PT J AU Repond, J AF Repond, Jose CA CALICE Collaboration TI Imaging hadron calorimetry for future Lepton Colliders SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE Calorimetry; Particle Flow Algorithms; Jet energy resolution AB To fully exploit the physics potential of a future Lepton Collider requires detectors with unprecedented jet energy and dijet-mass resolution. To meet these challenges, detectors optimized for the application of Particle Flow Algorithms (PFAs) are being designed and developed. The application of PFAs, in turn, requires calorimeters with very fine segmentation of the readout, so-called imaging calorimeters. This talk reviews progress in imaging hadron calorimetry as it is being developed for implementation in a detector at a future Lepton Collider. Recent results from the large prototypes built by the CALICE Collaboration, such as the Scintillator Analog Hadron Calorimeter (AHCAL) and the Digital Hadron Calorimeters (DHCAL and SDHCAL) are being presented. In addition, various R&D efforts beyond the present prototypes are being discussed. (C) 2013 Elsevier B.V. All rights reserved. C1 [Repond, Jose] Argonne Natl Lab, Argonne, IL 60439 USA. RP Repond, J (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM repond@hep.anl.gov NR 7 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 466 EP 469 DI 10.1016/j.nima.2013.05.036 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400104 ER PT J AU Metcalfe, J Geronimo, G Fried, J Li, S Nambiar, N Polychronakos, V Vernon, E AF Metcalfe, Jessica De Geronimo, Gianluigi Fried, Jack Li, Shaorui Nambiar, Neena Polychronakos, Venetios Vernon, Emerson TI Design and characterization of the VMM1 ASIC for micropattern gas detectors SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 13th Vienna Conference on Instrumentation CY FEB 11-15, 2013 CL Tech Univ Vienna, Vienna, AUSTRIA SP Austrian Fed Minist Sci & Res, Int Atom Energy Agcy, European Phys Soc, Vienna Convent Bur HO Tech Univ Vienna DE ASIC; Micromegas; TGC AB Measurements of the first prototype VMM1 ASIC designed at Brookhaven National Laboratory in 130 nm CMOS and fabricated in spring 2012 are presented. The 64-channel AMC features a novel design for use with several types of micropattern gas detectors. The data driven system measures peak amplitude and timing information in tracking mode including sub-threshold neighbors and first channel hit address in trigger mode. Several programmable gain and integration times allows the flexibility to work with Micromegas, Thin Gap Chambers (TGCs), and Gas Electron Multiplier (GEM) detectors. The IC design and features are presented along with measurements characterizing the performance of the VMM1 such as noise, linearity of the response, time walk, and calibration range. Published by Elsevier B.V. C1 [Metcalfe, Jessica; De Geronimo, Gianluigi; Fried, Jack; Li, Shaorui; Nambiar, Neena; Polychronakos, Venetios; Vernon, Emerson] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Metcalfe, J (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM Jessica.Metcalfe@cern.ch NR 6 TC 2 Z9 2 U1 1 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 21 PY 2013 VL 732 BP 526 EP 529 DI 10.1016/j.nima.2013.07.092 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258WW UT WOS:000327490400118 ER PT J AU Fryer, CL AF Fryer, Chris L. TI Compact object formation and the supernova explosion engine SO CLASSICAL AND QUANTUM GRAVITY LA English DT Article ID CORE-COLLAPSE SUPERNOVAE; SUPERMASSIVE BLACK-HOLES; GAMMA-RAY BURSTS; NEUTRON-STAR; CONVECTIVE ENGINE; MASS-DISTRIBUTION; ACCRETION SHOCK; ROTATING STARS; RADIO PULSARS; MECHANISM AB When a massive star ends its life, its core collapses, forming a neutron star or black hole and producing some of the most energetic explosions in the universe. Core-collapse supernovae and long-duration gamma-ray bursts are the violent signatures of compact remnant formation. As such, both fields are intertwined and, coupled with theory, observations of transients can help us better understand compact remnants just as neutron star and black hole observations can constrain the supernova and gamma-ray burst engine. We review these ties in this paper. C1 Los Alamos Natl Lab, CCS 2, MS D409, Los Alamos, NM 87544 USA. RP Fryer, CL (reprint author), Los Alamos Natl Lab, CCS 2, MS D409, POB 1663, Los Alamos, NM 87544 USA. EM fryer@lanl.gov NR 82 TC 5 Z9 5 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0264-9381 EI 1361-6382 J9 CLASSICAL QUANT GRAV JI Class. Quantum Gravity PD DEC 21 PY 2013 VL 30 IS 24 AR 244002 DI 10.1088/0264-9381/30/24/244002 PG 17 WC Astronomy & Astrophysics; Physics, Multidisciplinary; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 259RG UT WOS:000327543400003 ER PT J AU Adare, A Afanasiev, S Aidala, C Ajitanand, NN Akiba, Y Al-Bataineh, H Alexander, J Aoki, K Aramaki, Y Atomssa, ET Averbeck, R Awes, TC Azmoun, B Babintsev, V Bai, M Baksay, G Baksay, L Barish, KN Bassalleck, B Basye, AT Bathe, S Baublis, V Baumann, C Bazilevsky, A Belikov, S Belmont, R Bennett, R Berdnikov, A Berdnikov, Y Bickley, AA Bok, JS Boyle, K Brooks, ML Buesching, H Bumazhnov, V Bunce, G Butsyk, S Camacho, CM Campbell, S Chen, CH Chi, CY Chiu, M Choi, IJ Choudhury, RK Christiansen, P Chujo, T Chung, P Chvala, O Cianciolo, V Citron, Z Cole, BA Connors, M Constantin, P Csanad, M Csorgo, T Dahms, T Dairaku, S Danchev, I Das, K Datta, A David, G Denisov, A Deshpande, A Desmond, EJ Dietzsch, O Dion, A Donadelli, M Drapier, O Drees, A Drees, KA Durham, JM Durum, A Dutta, D Edwards, S Efremenko, YV Ellinghaus, F Engelmore, T Enokizono, A En'yo, H Esumi, S Fadem, B Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Fraenkel, Z Frantz, JE Franz, A Frawley, AD Fujiwara, K Fukao, Y Fusayasu, T Garishvili, I Glenn, A Gong, H Gonin, M Goto, Y de Cassagnac, RG Grau, N Greene, SV Perdekamp, MG Gunji, T Gustafsson, HA Haggerty, JS Hahn, KI Hamagaki, H Hamblen, J Han, R Hanks, J Hartouni, EP Haslum, E Hayano, R He, X Heffner, M Hemmick, TK Hester, T Hill, JC Hohlmann, M Holzmann, W Homma, K Hong, B Horaguchi, T Hornback, D Huang, S Ichihara, T Ichimiya, R Ide, J Ikeda, Y Imai, K Inaba, M Isenhower, D Ishihara, M Isobe, T Issah, M Isupov, A Ivanischev, D Jacak, BV Jia, J Jin, J Johnson, BM Joo, KS Jouan, D Jumper, DS Kajihara, F Kametani, S Kamihara, N Kamin, J Kang, JH Kapustinsky, J Karatsu, K Kawall, D Kawashima, M Kazantsev, AV Kempel, T Khanzadeev, A Kijima, KM Kim, BI Kim, DH Kim, DJ Kim, E Kim, EJ Kim, SH Kim, YJ Kinney, E Kiriluk, K Kiss, A Kistenev, E Kochenda, L Komkov, B Konno, M Koster, J Kotchetkov, D Kozlov, A Kral, A Kravitz, A Kunde, GJ Kurita, K Kurosawa, M Kwon, Y Kyle, GS Lacey, R Lai, YS Lajoie, JG Lebedev, A Lee, DM Lee, J Lee, K Lee, KB Lee, KS Leitch, MJ Leite, MAL Leitner, E Lenzi, B Li, X Liebing, P Levy, LAL Liska, T Litvinenko, A Liu, H Liu, MX Love, B Luechtenborg, R Lynch, D Maguire, CF Makdisi, YI Malakhov, A Malik, MD Manko, VI Mannel, E Mao, Y Masui, H Matathias, F McCumber, M McGaughey, PL Means, N Meredith, B Miake, Y Mignerey, AC Mikes, P Miki, K Milov, A Mishra, M Mitchell, JT Mohanty, AK Morino, Y Morreale, A Morrison, DP Moukhanova, TV Murata, J Nagamiya, S Nagle, JL Naglis, M Nagy, MI Nakagawa, I Nakamiya, Y Nakamura, T Nakano, K Newby, J Nguyen, M Nouicer, R Nyanin, AS O'Brien, E Oda, SX Ogilvic, CA Oka, M Okada, K Onuki, Y Oskarsson, A Ouchida, M Ozawa, K Pak, R Pantuev, V Papavassiliou, V Park, IH Park, J Park, SK Park, WJ Pate, SF Pei, H Peng, JC Pereira, H Peresedov, V Peressounko, DY Pinkenburg, C Pisani, RP Proissl, M Purschke, ML Purwar, AK Qu, H Rak, J Rakotozafindrabe, A Ravinovich, I Read, KF Reygers, K Riabov, V Riabov, Y Richardson, E Roach, D Roche, G Rolnick, SD Rosati, M Rosen, CA Rosendahl, SSE Rosnet, P Rukoyatkin, P Ruzicka, P Sahlmueller, B Saito, N Sakaguchi, T Sakashita, K Samsonov, V Sano, S Sato, T Sawada, S Sedgwick, K Seele, J Seidl, R Semenov, AY Seto, R Sharma, D Shein, I Shibata, TA Shigaki, K Shimomura, M Shoji, K Shukla, P Sickles, A Silva, CL Silvermyr, D Silvestre, C Sim, KS Singh, BK Singh, CP Singh, V Slunecka, M Soltz, RA Sondheim, WE Sorensen, SP Sourikova, IV Sparks, NA Stankus, PW Stenlund, E Stoll, SP Sugitate, T Sukhanov, A Sziklai, J Takagui, EM Taketani, A Tanabe, R Tanaka, Y Tanida, K Tannenbaum, MJ Tarafdar, S Taranenko, A Tarjan, P Themann, H Thomas, TL Togawa, M Toia, A Tomasek, L Torii, H Towell, RS Tserruya, I Tsuchimoto, Y Vale, C Valle, H Van Hecke, HW Vazquez-Zambrano, E Veicht, A Velkovska, J Vertesi, R Vinogradov, AA Virius, M Vrba, V Vznuzdaev, E Wang, XR Watanabe, D Watanabe, K Watanabe, Y Wei, F Wei, R Wessels, J White, SN Winter, D Wood, JP Woody, CL Wright, RM Wysocki, M Xie, W Yamaguchi, YL Yamaura, K Yang, R Yanovich, A Ying, J Yokkaichi, S You, Z Young, GR Younus, I Yushmanov, IE Zajc, WA Zhang, C Zhou, S Zolin, L AF Adare, A. Afanasiev, S. Aidala, C. Ajitanand, N. N. Akiba, Y. Al-Bataineh, H. Alexander, J. Aoki, K. Aramaki, Y. Atomssa, E. T. Averbeck, R. Awes, T. C. Azmoun, B. Babintsev, V. Bai, M. Baksay, G. Baksay, L. Barish, K. N. Bassalleck, B. Basye, A. T. Bathe, S. Baublis, V. Baumann, C. Bazilevsky, A. Belikov, S. Belmont, R. Bennett, R. Berdnikov, A. Berdnikov, Y. Bickley, A. A. Bok, J. S. Boyle, K. Brooks, M. L. Buesching, H. Bumazhnov, V. Bunce, G. Butsyk, S. Camacho, C. M. Campbell, S. Chen, C. -H. Chi, C. Y. Chiu, M. Choi, I. J. Choudhury, R. K. Christiansen, P. Chujo, T. Chung, P. Chvala, O. Cianciolo, V. Citron, Z. Cole, B. A. Connors, M. Constantin, P. Csanad, M. Csoergo, T. Dahms, T. Dairaku, S. Danchev, I. Das, K. Datta, A. David, G. Denisov, A. Deshpande, A. Desmond, E. J. Dietzsch, O. Dion, A. Donadelli, M. Drapier, O. Drees, A. Drees, K. A. Durham, J. M. Durum, A. Dutta, D. Edwards, S. Efremenko, Y. V. Ellinghaus, F. Engelmore, T. Enokizono, A. En'yo, H. Esumi, S. Fadem, B. Fields, D. E. Finger, M. Finger, M., Jr. Fleuret, F. Fokin, S. L. Fraenkel, Z. Frantz, J. E. Franz, A. Frawley, A. D. Fujiwara, K. Fukao, Y. Fusayasu, T. Garishvili, I. Glenn, A. Gong, H. Gonin, M. Goto, Y. de Cassagnac, R. Granier Grau, N. Greene, S. V. Perdekamp, M. Grosse Gunji, T. Gustafsson, H. -A. Haggerty, J. S. Hahn, K. I. Hamagaki, H. Hamblen, J. Han, R. Hanks, J. Hartouni, E. P. Haslum, E. Hayano, R. He, X. Heffner, M. Hemmick, T. K. Hester, T. Hill, J. C. Hohlmann, M. Holzmann, W. Homma, K. Hong, B. Horaguchi, T. Hornback, D. Huang, S. Ichihara, T. Ichimiya, R. Ide, J. Ikeda, Y. Imai, K. Inaba, M. Isenhower, D. Ishihara, M. Isobe, T. Issah, M. Isupov, A. Ivanischev, D. Jacak, B. V. Jia, J. Jin, J. Johnson, B. M. Joo, K. S. Jouan, D. Jumper, D. S. Kajihara, F. Kametani, S. Kamihara, N. Kamin, J. Kang, J. H. Kapustinsky, J. Karatsu, K. Kawall, D. Kawashima, M. Kazantsev, A. V. Kempel, T. Khanzadeev, A. Kijima, K. M. Kim, B. I. Kim, D. H. Kim, D. J. Kim, E. Kim, E. -J. Kim, S. H. Kim, Y. -J. Kinney, E. Kiriluk, K. Kiss, A. Kistenev, E. Kochenda, L. Komkov, B. Konno, M. Koster, J. Kotchetkov, D. Kozlov, A. Kral, A. Kravitz, A. Kunde, G. J. Kurita, K. Kurosawa, M. Kwon, Y. Kyle, G. S. Lacey, R. Lai, Y. S. Lajoie, J. G. Lebedev, A. Lee, D. M. Lee, J. Lee, K. Lee, K. B. Lee, K. S. Leitch, M. J. Leite, M. A. L. Leitner, E. Lenzi, B. Li, X. Liebing, P. Levy, L. A. Linden Liska, T. Litvinenko, A. Liu, H. Liu, M. X. Love, B. Luechtenborg, R. Lynch, D. Maguire, C. F. Makdisi, Y. I. Malakhov, A. Malik, M. D. Manko, V. I. Mannel, E. Mao, Y. Masui, H. Matathias, F. McCumber, M. McGaughey, P. L. Means, N. Meredith, B. Miake, Y. Mignerey, A. C. Mikes, P. Miki, K. Milov, A. Mishra, M. Mitchell, J. T. Mohanty, A. K. Morino, Y. Morreale, A. Morrison, D. P. Moukhanova, T. V. Murata, J. Nagamiya, S. Nagle, J. L. Naglis, M. Nagy, M. I. Nakagawa, I. Nakamiya, Y. Nakamura, T. Nakano, K. Newby, J. Nguyen, M. Nouicer, R. Nyanin, A. S. O'Brien, E. Oda, S. X. Ogilvic, C. A. Oka, M. Okada, K. Onuki, Y. Oskarsson, A. Ouchida, M. Ozawa, K. Pak, R. Pantuev, V. Papavassiliou, V. Park, I. H. Park, J. Park, S. K. Park, W. J. Pate, S. F. Pei, H. Peng, J. -C. Pereira, H. Peresedov, V. Peressounko, D. Yu. Pinkenburg, C. Pisani, R. P. Proissl, M. Purschke, M. L. Purwar, A. K. Qu, H. Rak, J. Rakotozafindrabe, A. Ravinovich, I. Read, K. F. Reygers, K. Riabov, V. Riabov, Y. Richardson, E. Roach, D. Roche, G. Rolnick, S. D. Rosati, M. Rosen, C. A. Rosendahl, S. S. E. Rosnet, P. Rukoyatkin, P. Ruzicka, P. Sahlmueller, B. Saito, N. Sakaguchi, T. Sakashita, K. Samsonov, V. Sano, S. Sato, T. Sawada, S. Sedgwick, K. Seele, J. Seidl, R. Semenov, A. Yu. Seto, R. Sharma, D. Shein, I. Shibata, T. -A. Shigaki, K. Shimomura, M. Shoji, K. Shukla, P. Sickles, A. Silva, C. L. Silvermyr, D. Silvestre, C. Sim, K. S. Singh, B. K. Singh, C. P. Singh, V. Slunecka, M. Soltz, R. A. Sondheim, W. E. Sorensen, S. P. Sourikova, I. V. Sparks, N. A. Stankus, P. W. Stenlund, E. Stoll, S. P. Sugitate, T. Sukhanov, A. Sziklai, J. Takagui, E. M. Taketani, A. Tanabe, R. Tanaka, Y. Tanida, K. Tannenbaum, M. J. Tarafdar, S. Taranenko, A. Tarjan, P. Themann, H. Thomas, T. L. Togawa, M. Toia, A. Tomasek, L. Torii, H. Towell, R. S. Tserruya, I. Tsuchimoto, Y. Vale, C. Valle, H. Van Hecke, H. W. Vazquez-Zambrano, E. Veicht, A. Velkovska, J. Vertesi, R. Vinogradov, A. A. Virius, M. Vrba, V. Vznuzdaev, E. Wang, X. R. Watanabe, D. Watanabe, K. Watanabe, Y. Wei, F. Wei, R. Wessels, J. White, S. N. Winter, D. Wood, J. P. Woody, C. L. Wright, R. M. Wysocki, M. Xie, W. Yamaguchi, Y. L. Yamaura, K. Yang, R. Yanovich, A. Ying, J. Yokkaichi, S. You, Z. Young, G. R. Younus, I. Yushmanov, I. E. Zajc, W. A. Zhang, C. Zhou, S. Zolin, L. CA PHENIX Collaboration TI Azimuthal anisotropy of pi(0) and eta mesons in Au plus Au collisions at root s(NN)=200 GeV SO PHYSICAL REVIEW C LA English DT Article ID QUARK-GLUON PLASMA; PB COLLISIONS; FLOW; COLLABORATION; PERSPECTIVE; MOMENTUM AB The azimuthal anisotropy coefficients v2 and v4 of p 0 and. mesons are measured in Au + Au collisions at root s(NN) = 200 GeV as a function of transverse momentum p(T) (1-14 GeV/c) and centrality. The extracted v(2) coefficients are found to be consistent between the two meson species over the measured p(T) range. The ratio of v(4)/v(2)(2) for pi(0) mesons is found to be independent of p(T) for 1- 9 GeV/c, implying a lack of sensitivity of the ratio to the change of underlying physics with p(T). Furthermore, the ratio of v(4)/v(2)(2) is systematically larger in central collisions, which may reflect the combined effects of fluctuations in the initial collision geometry and finite viscosity in the evolving medium. C1 [Basye, A. 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[Aidala, C.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Baumann, C.; Luechtenborg, R.; Reygers, K.; Sahlmueller, B.; Wessels, J.] Univ Munster, Inst Kernphys, D-48149 Munster, Germany. [Fadem, B.; Ide, J.] Muhlenberg Coll, Allentown, PA 18104 USA. [Joo, K. S.; Kim, D. H.] Myongji Univ, Yongin 449728, Kyonggido, South Korea. [Fusayasu, T.; Tanaka, Y.] Nagasaki Inst Appl Sci, Nagasaki 8510193, Japan. [Bassalleck, B.; Fields, D. E.; Kotchetkov, D.; Liu, H.; Malik, M. D.; Thomas, T. L.; Younus, I.] Univ New Mexico, Albuquerque, NM 87131 USA. [Al-Bataineh, H.; Kyle, G. S.; Papavassiliou, V.; Pate, S. F.; Wang, X. R.] New Mexico State Univ, Las Cruces, NM 88003 USA. [Frantz, J. E.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Awes, T. C.; Cianciolo, V.; Efremenko, Y. V.; Read, K. F.; Silvermyr, D.; Stankus, P. W.; Young, G. R.; Zhang, C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jouan, D.] Univ Paris 11, IPN Orsay, CNRS IN2P3, F-91406 Orsay, France. [Han, R.; Mao, Y.; You, Z.] Peking Univ, Beijing 100871, Peoples R China. [Baublis, V.; Ivanischev, D.; Khanzadeev, A.; Kochenda, L.; Komkov, B.; Riabov, V.; Riabov, Y.; Samsonov, V.; Vznuzdaev, E.] PNPI, Gatchina 188300, Leningrad Regio, Russia. [Akiba, Y.; Dairaku, S.; En'yo, H.; Fujiwara, K.; Fukao, Y.; Goto, Y.; Ichihara, T.; Ichimiya, R.; Imai, K.; Ishihara, M.; Isobe, T.; Kametani, S.; Karatsu, K.; Kawashima, M.; Kurita, K.; Kurosawa, M.; Mao, Y.; Miki, K.; Murata, J.; Nakagawa, I.; Nakano, K.; Onuki, Y.; Ouchida, M.; Sakashita, K.; Shibata, T. -A.; Shoji, K.; Taketani, A.; Tanida, K.; Togawa, M.; Watanabe, Y.; Yokkaichi, S.] RIKEN Nishina Ctr Accelerator Based Sci, Wako, Saitama 3510198, Japan. [Akiba, Y.; Bunce, G.; Deshpande, A.; En'yo, H.; Goto, Y.; Perdekamp, M. Grosse; Ichihara, T.; Kamihara, N.; Kawall, D.; Liebing, P.; Nakagawa, I.; Okada, K.; Taketani, A.; Tanida, K.; Watanabe, Y.; Xie, W.; Yokkaichi, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Kawashima, M.; Kurita, K.; Murata, J.] Rikkyo Univ, Dept Phys, Toshima, Tokyo 1718501, Japan. [Berdnikov, A.; Berdnikov, Y.] St Petersburg State Polytech Univ, St Petersburg 195251, Russia. [Dietzsch, O.; Donadelli, M.; Leite, M. A. L.; Lenzi, B.; Silva, C. L.; Takagui, E. M.] Univ Sao Paulo, Inst Fis, BR-CEP05315 Sao Paulo, Brazil. [Kim, E.; Lee, K.; Park, J.] Seoul Natl Univ, Seoul, South Korea. [Ajitanand, N. N.; Alexander, J.; Chung, P.; Jia, J.; Lacey, R.; Taranenko, A.; Wei, R.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Averbeck, R.; Bennett, R.; Boyle, K.; Campbell, S.; Chen, C. -H.; Citron, Z.; Connors, M.; Dahms, T.; Deshpande, A.; Dion, A.; Drees, A.; Durham, J. M.; Frantz, J. E.; Gong, H.; Hemmick, T. K.; Jacak, B. V.; Kamin, J.; Kozlov, A.; McCumber, M.; Means, N.; Nguyen, M.; Pantuev, V.; Proissl, M.; Sahlmueller, B.; Themann, H.; Toia, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Garishvili, I.; Hamblen, J.; Hornback, D.; Read, K. F.; Sorensen, S. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Nakano, K.; Sakashita, K.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Chujo, T.; Esumi, S.; Ikeda, Y.; Inaba, M.; Konno, M.; Masui, H.; Miake, Y.; Miki, K.; Oka, M.; Sato, T.; Shimomura, M.; Tanabe, R.; Watanabe, K.] Univ Tsukuba, Inst Phys, Tsukuba, Ibaraki 305, Japan. [Belmont, R.; Danchev, I.; Greene, S. V.; Huang, S.; Issah, M.; Leitner, E.; Love, B.; Maguire, C. F.; Roach, D.; Valle, H.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Sano, S.] Waseda Univ, Adv Res Inst Sci & Engn, Tokyo 1620044, Japan. [Fraenkel, Z.; Kozlov, A.; Naglis, M.; Ravinovich, I.; Sharma, D.; Tserruya, I.] Weizmann Inst Sci, IL-76100 Rehovot, Israel. [Csoergo, T.; Sziklai, J.; Vertesi, R.] Hungarian Acad Sci Wigner RCP, RMKI, Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Bok, J. S.; Choi, I. J.; Kang, J. H.; Kim, S. H.; Kwon, Y.] Yonsei Univ, IPAP, Seoul 120749, South Korea. RP Adare, A (reprint author), Abilene Christian Univ, Abilene, TX 79699 USA. RI Tomasek, Lukas/G-6370-2014; Dahms, Torsten/A-8453-2015; En'yo, Hideto/B-2440-2015; Hayano, Ryugo/F-7889-2012; HAMAGAKI, HIDEKI/G-4899-2014; Durum, Artur/C-3027-2014; Sorensen, Soren /K-1195-2016; Yokkaichi, Satoshi/C-6215-2017; Taketani, Atsushi/E-1803-2017 OI Tomasek, Lukas/0000-0002-5224-1936; Dahms, Torsten/0000-0003-4274-5476; Hayano, Ryugo/0000-0002-1214-7806; Sorensen, Soren /0000-0002-5595-5643; Taketani, Atsushi/0000-0002-4776-2315 FU Office of Nuclear Physics in the Office of Science of the Department of Energy; National Science Foundation; Abilene Christian University Research Council; Research Foundation of SUNY; Dean of the College of Arts and Sciences; Vanderbilt University (USA); Ministry of Education, Culture, Sports, Science, and Technology; Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (P. R. China); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique; Commissariat a l'Energie Atomique; Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung; Deutscher Akademischer Austausch Dienst; Alexander von Humboldt Stiftung (Germany); Hungarian National Science Fund; OTKA (Hungary); Department of Atomic Energy (India); Israel Science Foundation (Israel); National Research Foundation and WCU program of the Ministry Education Science and Technology (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science; VR and Wallenberg Foundation (Sweden); US Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; US-Hungarian Fulbright Foundation for Educational Exchange; US-Israel Binational Science Foundation; Russian Academy of Sciences; Federal Agency of Atomic Energy (Russia); Department of Science and Technology (India) FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (USA); Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan), Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (P. R. China); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch Dienst, and Alexander von Humboldt Stiftung (Germany); Hungarian National Science Fund, OTKA (Hungary); Department of Atomic Energy and Department of Science and Technology (India); Israel Science Foundation (Israel); National Research Foundation and WCU program of the Ministry Education Science and Technology (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia); VR and Wallenberg Foundation (Sweden); the US Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the US-Hungarian Fulbright Foundation for Educational Exchange, and the US-Israel Binational Science Foundation. NR 41 TC 5 Z9 5 U1 6 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD DEC 20 PY 2013 VL 88 IS 6 AR 064910 DI 10.1103/PhysRevC.88.064910 PG 10 WC Physics, Nuclear SC Physics GA 276DZ UT WOS:000328729600002 ER PT J AU Buttazzo, D Degrassi, G Giardino, PP Giudice, GF Sala, F Salvio, A Strumia, A AF Buttazzo, Dario Degrassi, Giuseppe Giardino, Pier Paolo Giudice, Gian F. Sala, Filippo Salvio, Alberto Strumia, Alessandro TI Investigating the near-criticality of the Higgs boson SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; Standard Model; Renormalization Group ID RENORMALIZATION-GROUP EQUATIONS; QUANTUM-FIELD THEORY; 2-LOOP PROPAGATOR INTEGRALS; ABELIAN GAUGE THEORIES; QCD BETA-FUNCTION; STANDARD-MODEL; ELECTROWEAK VACUUM; RADIATIVE-CORRECTIONS; TOP-QUARK; ANOMALOUS DIMENSIONS AB We extract from data the parameters of the Higgs potential, the top Yukawa coupling and the electroweak gauge couplings with full 2-loop NNLO precision, and we extrapolate the SM parameters up to large energies with full 3-loop NNLO RGE precision. Then we study the phase diagram of the Standard Model in terms of high-energy parameters, finding that the measured Higgs mass roughly corresponds to the minimum values of the Higgs quartic and top Yukawa and the maximum value of the gauge couplings allowed by vacuum metastability. We discuss various theoretical interpretations of the near-criticality of the Higgs mass. C1 [Buttazzo, Dario; Giardino, Pier Paolo; Giudice, Gian F.] CERN, Div Theory, CH-1211 Geneva 23, Switzerland. [Buttazzo, Dario; Sala, Filippo; Salvio, Alberto] Scuola Normale Super Pisa, Pisa, Italy. [Buttazzo, Dario; Sala, Filippo; Salvio, Alberto] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Degrassi, Giuseppe] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Degrassi, Giuseppe] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Giardino, Pier Paolo; Strumia, Alessandro] Univ Pisa, Dipartimento Fis, Pisa, Italy. [Giardino, Pier Paolo; Strumia, Alessandro] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Sala, Filippo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Salvio, Alberto] Univ Autonoma Madrid, Dept Fis Teor, Madrid, Spain. [Salvio, Alberto] CSIC, UAM, IFT, Madrid, Spain. RP Buttazzo, D (reprint author), CERN, Div Theory, CH-1211 Geneva 23, Switzerland. EM dario.buttazzo@sns.it; degrassi@fis.uniroma3.it; pierpaolo.giardino@pi.infn.it; Gian.Giudice@cern.ch; filippo.sala@sns.it; alberto.salvio@uam.es; astrumia@cern.ch OI Giardino, Pier Paolo/0000-0002-3379-5917; Salvio, Alberto/0000-0002-1780-9944; Sala, Filippo/0000-0001-6565-0862 FU Research Executive Agency (REA) of the European Union [SF0690030s09, PITN-GA-2010-264564]; EU ITN "Unification in the LHC Era" [PITN-GA-2009-237920]; MIUR [2006022501]; Spanish Ministry of Economy and Competitiveness [FPA2012-32828, CSD2007-00042]; "Centro de Excelencia Severo Ochoa" Programme [SEV-2012-0249]; C.A. de Madrid [HEPHACOS-S2009/ESP1473] FX This work was supported by the SF0690030s09 project, by the Research Executive Agency (REA) of the European Union under the Grant Agreement number PITN-GA-2010-264564 (LHCPhenoNet); by the EU ITN "Unification in the LHC Era", contract PITN-GA-2009-237920 (UNILHC) and by MIUR under contract 2006022501; by the Spanish Ministry of Economy and Competitiveness under grant FPA2012-32828, Consolider-CPAN (CSD2007-00042), the grant SEV-2012-0249 of the "Centro de Excelencia Severo Ochoa" Programme and the grant HEPHACOS-S2009/ESP1473 from the C.A. de Madrid. We thank Simone Alioli, Claudio Bonati, Lawrence Hall, Luis E. Ibanez, Gino Isidori, and Riccardo Rattazzi for useful discussions. The work of P. P. G. has been partially funded by the "Fondazione A. Della Riccia". NR 146 TC 214 Z9 214 U1 2 U2 17 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD DEC 20 PY 2013 IS 12 AR 089 DI 10.1007/JHEP12(2013)089 PG 49 WC Physics, Particles & Fields SC Physics GA 278NV UT WOS:000328897900003 ER PT J AU Rice, DW Alverson, AJ Richardson, AO Young, GJ Sanchez-Puerta, MV Munzinger, J Barry, K Boore, JL Zhang, Y dePamphilis, CW Knox, EB Palmer, JD AF Rice, Danny W. Alverson, Andrew J. Richardson, Aaron O. Young, Gregory J. Virginia Sanchez-Puerta, M. Munzinger, Jerome Barry, Kerrie Boore, Jeffrey L. Zhang, Yan dePamphilis, Claude W. Knox, Eric B. Palmer, Jeffrey D. TI Horizontal Transfer of Entire Genomes via Mitochondrial Fusion in the Angiosperm Amborella SO SCIENCE LA English DT Article ID FLOWERING PLANTS; GENE-TRANSFER; ORIGINS; EVOLUTION; SUGGESTS; FISSION AB We report the complete mitochondrial genome sequence of the flowering plant Amborella trichopoda. This enormous, 3.9-megabase genome contains six genome equivalents of foreign mitochondrial DNA, acquired from green algae, mosses, and other angiosperms. Many of these horizontal transfers were large, including acquisition of entire mitochondrial genomes from three green algae and one moss. We propose a fusion-compatibility model to explain these findings, with Amborella capturing whole mitochondria from diverse eukaryotes, followed by mitochondrial fusion (limited mechanistically to green plant mitochondria) and then genome recombination. Amborella's epiphyte load, propensity to produce suckers from wounds, and low rate of mitochondrial DNA loss probably all contribute to the high level of foreign DNA in its mitochondrial genome. C1 [Rice, Danny W.; Alverson, Andrew J.; Richardson, Aaron O.; Young, Gregory J.; Virginia Sanchez-Puerta, M.; Knox, Eric B.; Palmer, Jeffrey D.] Indiana Univ, Dept Biol, Bloomington, IN 47405 USA. [Munzinger, Jerome] IRD, Lab Bot & Ecol Vegetale Appl, UMR Bot & Bioinformat Architecture Plantes AMAP, Noumea, New Caledonia. [Barry, Kerrie; Boore, Jeffrey L.] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. [Zhang, Yan; dePamphilis, Claude W.] Penn State Univ, Dept Biol, University Pk, PA 16802 USA. RP Palmer, JD (reprint author), Indiana Univ, Dept Biol, Bloomington, IN 47405 USA. EM jpalmer@indiana.edu RI Palmer, Jeffrey/P-6747-2014; dePamphilis, Claude/P-6652-2016; OI Palmer, Jeffrey/0000-0002-4626-2220; Sanchez-Puerta, Maria Virginia/0000-0003-2511-5093; Alverson, Andrew/0000-0003-1241-2654 FU U.S. Department of Energy-Joint Genome Institute Community Sequencing Program [DE-AC02-05CH11231, NSF-GRF-112955, NSF-DBI-0638595]; METACyt Initiative of Indiana University; Lilly Endowment; [NIH-RO1-GM-76012] FX We thank E. Dalin, J. Gummow, and P. Lowry for assistance; R. Wing and the Arizona Genomics Institute for Amborella bacterial artificial chromosome sequences; the North and South Environmental Services of New Caledonia for collecting permits; M. Moore, P. Soltis, and D. Soltis for two unpublished plastid-genome sequences; and those individuals (see table S11) who supplied the photographs for figures. This work was supported by NIH-RO1-GM-76012 (J.D.P. and E. B. K), the U.S. Department of Energy-Joint Genome Institute Community Sequencing Program under contract DE-AC02-05CH11231 (J.D.P, E. B. K, and J.L.B), NSF-GRF-112955 (A.O.R.), NSF-DBI-0638595 (C. W. D), and the METACyt Initiative of Indiana University, funded by the Lilly Endowment. The data reported in this paper are deposited in GenBank under accessions KF754799-KF754803 and KF798319-KF798355. NR 31 TC 74 Z9 78 U1 14 U2 82 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD DEC 20 PY 2013 VL 342 IS 6165 BP 1468 EP 1473 DI 10.1126/science.1246275 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 274ZI UT WOS:000328644300048 PM 24357311 ER PT J AU Elkins, MH Williams, HL Shreve, AT Neumark, DM AF Elkins, Madeline H. Williams, Holly L. Shreve, Alexander T. Neumark, Daniel M. TI Relaxation Mechanism of the Hydrated Electron SO SCIENCE LA English DT Article ID RESOLVED PHOTOELECTRON-SPECTROSCOPY; WATER CLUSTER ANIONS; LOW KINETIC-ENERGY; SOLVATED ELECTRONS; AQUEOUS-SOLUTIONS; EXCESS ELECTRONS; LIQUID WATER; DYNAMICS; BULK; SPECTRA AB The relaxation dynamics of the photoexcited hydrated electron have been subject to conflicting interpretations. Here, we report time-resolved photoelectron spectra of hydrated electrons in a liquid microjet with the aim of clarifying ambiguities from previous experiments. A sequence of three ultrashort laser pulses (similar to 100 femtosecond duration) successively created hydrated electrons by charge-transfer-to-solvent excitation of dissolved anions, electronically excited these electrons via the s -> p transition, and then ejected them into vacuum. Two distinct transient signals were observed. One was assigned to the initially excited p-state with a lifetime of similar to 75 femtoseconds, and the other, with a lifetime of similar to 400 femtoseconds, was attributed to s-state electrons just after internal conversion in a nonequilibrated solvent environment. These assignments support the nonadiabatic relaxation model. C1 [Elkins, Madeline H.; Williams, Holly L.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shreve, Alexander T.] Intel Corp, Hillsboro, OR 97124 USA. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU National Science Foundation (NSF) [CHE-1011819] FX This research is supported by the National Science Foundation (NSF) under grant CHE-1011819. The data presented in this paper are available upon request sent to dneumark@berkeley.edu. NR 39 TC 31 Z9 31 U1 12 U2 117 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD DEC 20 PY 2013 VL 342 IS 6165 BP 1496 EP 1499 DI 10.1126/science.1246291 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 274ZI UT WOS:000328644300054 PM 24357314 ER PT J AU Brunecky, R Alahuhta, M Xu, Q Donohoe, BS Crowley, MF Kataeva, IA Yang, SJ Resch, MG Adams, MWW Lunin, VV Himmel, ME Bomble, YJ AF Brunecky, Roman Alahuhta, Markus Xu, Qi Donohoe, Bryon S. Crowley, Michael F. Kataeva, Irina A. Yang, Sung-Jae Resch, Michael G. Adams, Michael W. W. Lunin, Vladimir V. Himmel, Michael E. Bomble, Yannick J. TI Revealing Nature's Cellulase Diversity: The Digestion Mechanism of Caldicellulosiruptor bescii CelA SO SCIENCE LA English DT Article ID THERMOPHILUM DSM 6725; ANAEROCELLUM-THERMOPHILUM; CELLOBIOHYDROLASE-I; BETA-GLUCOSIDASE; PRETREATMENT; CELLULOSOMES; DEGRADATION; EXPLOSION; MIXTURES; SEQUENCE AB Most fungi and bacteria degrade plant cell walls by secreting free, complementary enzymes that hydrolyze cellulose; however, some bacteria use large enzymatic assemblies called cellulosomes, which recruit complementary enzymes to protein scaffolds. The thermophilic bacterium Caldicellulosiruptor bescii uses an intermediate strategy, secreting many free cellulases that contain multiple catalytic domains. One of these, CelA, comprises a glycoside hydrolase family 9 and a family 48 catalytic domain, as well as three type III cellulose-binding modules. In the saccharification of a common cellulose standard, Avicel, CelA outperforms mixtures of commercially relevant exo- and endoglucanases. From transmission electron microscopy studies of cellulose after incubation with CelA, we report morphological features that suggest that CelA not only exploits the common surface ablation mechanism driven by general cellulase processivity, but also excavates extensive cavities into the surface of the substrate. These results suggest that nature's repertoire of cellulose digestion paradigms remain only partially discovered and understood. C1 [Brunecky, Roman; Alahuhta, Markus; Xu, Qi; Donohoe, Bryon S.; Crowley, Michael F.; Resch, Michael G.; Lunin, Vladimir V.; Himmel, Michael E.; Bomble, Yannick J.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Kataeva, Irina A.; Yang, Sung-Jae; Adams, Michael W. W.] Univ Georgia, Dept Biochem & Mol Biol, Athens, GA 30602 USA. RP Bomble, YJ (reprint author), Natl Renewable Energy Lab, Biosci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM yannick.bomble@nrel.gov FU BioEnergy Science Center (BESC); Office of Biological and Environmental Research in the U.S. DOE Office of Science FX This work was supported by the BioEnergy Science Center (BESC). BESC is a U.S. Department of Energy (DOE) Bioenergy Research Center supported by the Office of Biological and Environmental Research in the U.S. DOE Office of Science. We acknowledge colleagues at the Biomass Conversion Research Laboratory at Michigan State University for providing the AFEX-pretreated materials. Structures have been deposited in the Protein Data Bank with PDB codes 4DOD (GH9), 4DOE (GH9-CB), and 4EL8 (GH48). NR 24 TC 74 Z9 75 U1 13 U2 115 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD DEC 20 PY 2013 VL 342 IS 6165 BP 1513 EP 1516 DI 10.1126/science.1244273 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 274ZI UT WOS:000328644300059 PM 24357319 ER PT J AU Moro, EA Briggs, ME Hull, LM AF Moro, Erik A. Briggs, Matthew E. Hull, Lawrence M. TI Defining parametric dependencies for the correct interpretation of speckle dynamics in photon Doppler velocimetry SO APPLIED OPTICS LA English DT Article AB Laser speckle dynamics manifest themselves in photon Doppler velocimetry (PDV) data as low-frequency amplitude fluctuations, and analysis of these fluctuations provides insight into the transverse speed of the surface under observation. We previously demonstrated that a single measurement probe is capable of simultaneously measuring (1) axial motion, through frequency analysis of Doppler shifts, and (2) transverse speed, through analysis of the speckle's coherence time. However, the performance of this technique hinges on a correct understanding of the speckle pattern's response to surface motion. In this paper, we model the origination of the speckle pattern, and we describe a methodology for calculating the speckle's coherence time from the autocorrelation of a noisy signal. We then test a suite of optical probes over a range of standoff distances, demonstrating a significant reduction in the speckle's coherence time, which correlates to the increase in speckle boiling when the target surface is located near a probe's focal length. We show that spatial regions of decreased coherence time may be predicted a priori by a probe's parameters, since they stem from boiling dominance. We analyze this result as a function of probe parameters for a surface-scattering target and a volume-scattering target. Although the coherence time's behavior in the focal plane makes velocity extraction difficult, far from the probe's focal lengths, we are able to measure rigid body transverse speeds exceeding 20 m/s with an absolute accuracy of +/- 15% using the speckle dynamics measured by a PDV setup. (C) 2013 Optical Society of America C1 [Moro, Erik A.; Briggs, Matthew E.; Hull, Lawrence M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Moro, EA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM moro@lanl.gov NR 19 TC 2 Z9 2 U1 0 U2 6 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD DEC 20 PY 2013 VL 52 IS 36 BP 8661 EP 8669 DI 10.1364/AO.52.008661 PG 9 WC Optics SC Optics GA 279GL UT WOS:000328948300005 PM 24513931 ER PT J AU Bazhirov, T Coh, S Louie, SG Cohen, ML AF Bazhirov, Timur Coh, Sinisa Louie, Steven G. Cohen, Marvin L. TI Importance of oxygen octahedra tilts for the electron-phonon coupling in K-doped BaBiO3 SO PHYSICAL REVIEW B LA English DT Article ID STRUCTURAL PHASE-DIAGRAM; BAPB1-XBIXO3 SYSTEM; WANNIER FUNCTIONS; CRYSTAL-STRUCTURE; BA1-XKXBIO3; SUPERCONDUCTIVITY; ENERGY; TEMPERATURE; DYNAMICS; MODES AB Despite considerable research efforts, a clear understanding of superconductivity in Ba0.5K0.5BiO3 has been elusive. Recent studies showed that although electron-correlation effects in this compound can significantly increase the electron-phonon coupling, they do not reproduce the measured Eliashberg spectral function (alpha F-2). We show that the oxygen octahedra tilts in Ba0.5K0.5BiO3 increase alpha F-2 in the range of frequencies near 30 meV, even on the level of the generalized gradient approximation. This increase in alpha F-2 changes its shape to provide better agreement with experiment and results in a 50-60% increase of the average electron-phonon coupling strength lambda. We use the Wannier interpolation technique to determine the electron-phonon coupling with high precision. C1 [Bazhirov, Timur] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Bazhirov, T (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. FU NSF [DMR10-1006184]; Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231]; Simons Foundation FX Structural study and the work on the ground-state properties were supported by NSF Grant No. DMR10-1006184. The electron-phonon properties calculations were supported by the Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, US Department of Energy, under Contract No. DE-AC02-05CH11231. S. G. L. acknowledges support of a Simons Foundation Fellowship in Theoretical Physics. Computational resources were provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy. NR 36 TC 4 Z9 4 U1 2 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 20 PY 2013 VL 88 IS 22 AR 224509 DI 10.1103/PhysRevB.88.224509 PG 6 WC Physics, Condensed Matter SC Physics GA 275PA UT WOS:000328688100005 ER PT J AU Joshua, CJ Perez, LD Keasling, JD AF Joshua, Chijioke J. Perez, Luis D. Keasling, Jay D. TI Functional Characterization of the Origin of Replication of pRN1 from Sulfolobus islandicus REN1H1 SO PLOS ONE LA English DT Article ID ROLLING-CIRCLE REPLICATION; PLASMID PRN1; HYPERTHERMOPHILIC ARCHAEON; BACTERIAL PLASMIDS; GENUS SULFOLOBUS; MODEL ORGANISMS; SOLFATARICUS; DNA; ACIDOCALDARIUS; SEQUENCE AB Plasmid pRN1 from Sulfolc)bus islandicus REN1H1 is believed to replicate by a rolling circle mechanism but its origin and mechanism of replication are not well understood. We sought to create minimal expression vectors based on pRN1 that would be useful for heterologous gene expression in S. acidocaidarius, and n the process improve our understanding of the mechanism of replication. We constructed and transformed shuttle vectors that harbored different contiguous stretches of DNA from pFZNI1 into S. aciclocaidarius E4-39, a uracil ataxotropli. A 232-bp region of orf904 was found to be critical for pRN1 replication and is therefore proposed to be the putative origin of replication. This 232-bp region contains a 100-bp stem-loop structure believed to be the double-strand origin of replication. The loop of the 100-bp structure contains a GTG tri-nucleotide motif, a feature that was previously reported to be important for the primase activity of 0rf904. This putative origin and the associated orf56 and orf904 ere identified as the minimal replicon of pRN1 because transforrnants of plasmids lacking any of these three eatures were not recovered. Plasmids lacking orf904 and or156 but harboring the putative origin were transformable hen orf904 and orf56 were provided in-trans; a 75-bp region 5' of the 011904 start codon was found to be essential or this complementation. Detailed knowledge of he pRN1 origin of replication will broaden the application of the plasmid as a genetic tool for Suffo/obtis species. C1 [Joshua, Chijioke J.; Keasling, Jay D.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Perez, Luis D.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Joshua, Chijioke J.; Perez, Luis D.; Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Joshua, Chijioke J.; Perez, Luis D.; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP Keasling, JD (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM Keasling@berkeley.edu RI Keasling, Jay/J-9162-2012 OI Keasling, Jay/0000-0003-4170-6088 FU United States Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-ACO2-05CH11231] FX This work was part of the Department of Energy Joint BioEnergy Institute (http://vvww.jbei.org) supported by the United States Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-ACO2-05CH11231 between Lawrence Berkeley National Laboratory and the United States Department of Energy. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 43 TC 3 Z9 3 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 20 PY 2013 VL 8 IS 12 AR e84664 DI 10.1371/journal.pone.0084664 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 276IX UT WOS:000328745100181 PM 24376833 ER PT J AU Aartsen, MG Abbasi, R Abdou, Y Ackermann, M Adams, J Aguilar, JA Ahlers, M Altmann, D Auffenberg, J Bai, X Baker, M Barwick, SW Baum, V Bay, R Beatty, JJ Bechet, S Tjus, JB Becker, KH Benabderrahmane, ML BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohaichuk, S Bohm, C Bose, D Boser, S Botner, O Brayeur, L Bretz, HP Brown, AM Bruijn, R Brunner, J Carson, M Casey, J Casier, M Chirkin, D Christov, A Christy, B Clark, K Clevermann, F Coenders, S Cohen, S Cowen, DF Silva, AHC Danninger, M Daughhetee, J Davis, JC Day, M De Clercq, C De Ridder, S Desiati, P de Vries, KD de With, M DeYoung, T Diaz-Velez, JC Dunkman, M Eagan, R Eberhardt, B Eisch, J Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feintzeig, J Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Flis, S Franckowiak, A Frantzen, K Fuchs, T Gaisser, TK Gallagher, J Gerhardt, L Gladstone, L Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grandmont, DT Grant, D Gross, A Ha, C Ismail, AH Hallen, P Hallgren, A Halzen, F Hanson, K Heereman, D Heinen, D Helbing, K Hellauer, R Hickford, S Hill, GC Hoffman, KD Hoffmann, R Homeier, A Hoshina, K Huelsnitz, W Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobi, E Jacobsen, J Jagielski, K Japaridze, GS Jero, K Jlelati, O Kaminsky, B Kappes, A Karg, T Karle, A Kelley, JL Kiryluk, J Klas, J Klein, SR Kohne, JH Kohnen, G Kolanoski, H Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krasberg, M Krings, K Kroll, G Kunnen, J Kurahashi, N Kuwabara, T Labare, M Landsman, H Larson, MJ Lesiak-Bzdak, M Leuermann, M Leute, J Lunemann, J Macias, O Madsen, J Maggi, G Maruyama, R Mase, K Matis, HS McNally, F Meagher, K Merck, M Meures, T Miarecki, S Middell, E Milke, N Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Odrowski, S Olivas, A Omairat, A O'Murchadha, A Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Radel, L Rameez, M Rawlins, K Redl, P Reimann, R Resconi, E Rhode, W Ribordy, M Richman, M Riedel, B Rodrigues, JP Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Salameh, T Sander, HG Santander, M Sarkar, S Schatto, K Scheriau, F Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schukraft, A Schulte, L Schulz, O Seckel, D Sestayo, Y Seunarine, S Shanidze, R Sheremata, C Smith, MWE Soldin, D Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Sullivan, GW Taavola, H Taboada, I Tamburro, A Tepe, A Ter-Antonyan, S Tesic, G Tilav, S Toale, PA Toscano, S Unger, E Usner, M Vallecorsa, S van Eijndhoven, N Van Overloop, A van Santen, J Vehring, M Voge, M Vraeghe, M Walck, C Waldenmaier, T Wallraff, M Weaver, C Wellons, M Wendt, C Westerhoff, S Whitehorn, N Wiebe, K Wiebusch, CH Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Ziemann, J Zierke, S Zoll, M AF Aartsen, M. G. Abbasi, R. Abdou, Y. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Altmann, D. Auffenberg, J. Bai, X. Baker, M. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Bechet, S. Tjus, J. Becker Becker, K. -H. Benabderrahmane, M. L. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohaichuk, S. Bohm, C. Bose, D. Boeser, S. Botner, O. Brayeur, L. Bretz, H. -P. Brown, A. M. Bruijn, R. Brunner, J. Carson, M. Casey, J. Casier, M. Chirkin, D. Christov, A. Christy, B. Clark, K. Clevermann, F. Coenders, S. Cohen, S. Cowen, D. F. Silva, A. H. Cruz Danninger, M. Daughhetee, J. Davis, J. C. Day, M. De Clercq, C. De Ridder, S. Desiati, P. de Vries, K. D. de With, M. DeYoung, T. Diaz-Velez, J. C. Dunkman, M. Eagan, R. Eberhardt, B. Eisch, J. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feintzeig, J. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Franckowiak, A. Frantzen, K. Fuchs, T. Gaisser, T. K. Gallagher, J. Gerhardt, L. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grandmont, D. T. Grant, D. Gross, A. Ha, C. Ismail, A. Haj Hallen, P. Hallgren, A. Halzen, F. Hanson, K. Heereman, D. Heinen, D. Helbing, K. Hellauer, R. Hickford, S. Hill, G. C. Hoffman, K. D. Hoffmann, R. Homeier, A. Hoshina, K. Huelsnitz, W. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobi, E. Jacobsen, J. Jagielski, K. Japaridze, G. S. Jero, K. Jlelati, O. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kelley, J. L. Kiryluk, J. Klaes, J. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krasberg, M. Krings, K. Kroll, G. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Landsman, H. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leute, J. Luenemann, J. Macias, O. Madsen, J. Maggi, G. Maruyama, R. Mase, K. Matis, H. S. McNally, F. Meagher, K. Merck, M. Meures, T. Miarecki, S. Middell, E. Milke, N. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Odrowski, S. Olivas, A. Omairat, A. O'Murchadha, A. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Reimann, R. Resconi, E. Rhode, W. Ribordy, M. Richman, M. Riedel, B. Rodrigues, J. P. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Salameh, T. Sander, H. -G. Santander, M. Sarkar, S. Schatto, K. Scheriau, F. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Schulz, O. Seckel, D. Sestayo, Y. Seunarine, S. Shanidze, R. Sheremata, C. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Strom, R. Sullivan, G. W. Taavola, H. Taboada, I. Tamburro, A. Tepe, A. Ter-Antonyan, S. Tesic, G. Tilav, S. Toale, P. A. Toscano, S. Unger, E. Usner, M. Vallecorsa, S. van Eijndhoven, N. Van Overloop, A. van Santen, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Waldenmaier, T. Wallraff, M. Weaver, Ch Wellons, M. Wendt, C. Westerhoff, S. Whitehorn, N. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Ziemann, J. Zierke, S. Zoll, M. TI SEARCH FOR TIME-INDEPENDENT NEUTRINO EMISSION FROM ASTROPHYSICAL SOURCES WITH 3 yr OF IceCube DATA SO ASTROPHYSICAL JOURNAL LA English DT Article DE astroparticle physics; cosmic rays; neutrinos; telescopes ID GAMMA-RAY EMISSION; HIGH-ENERGY NEUTRINOS; BRIGHT GALAXY SAMPLE; FERMI-LAT DISCOVERY; SUPERNOVA-REMNANTS; COSMIC-RAYS; CRAB-NEBULA; STARBURST GALAXIES; MOLECULAR CLOUDS; GALACTIC SOURCES AB We present the results of a search for neutrino point sources using the IceCube data collected between 2008 April and 2011 May with three partially completed configurations of the detector: the 40-, 59-, and 79-string configurations. The live-time of this data set is 1040 days. An unbinned maximum likelihood ratio test was used to search for an excess of neutrinos above the atmospheric background at any given direction in the sky. By adding two more years of data with improved event selection and reconstruction techniques, the sensitivity was improved by a factor of 3.5 or more with respect to the previously published results obtained with the 40-string configuration of IceCube. We performed an all-sky survey and a dedicated search using a catalog of a priori selected objects observed by other telescopes. In both searches, the data are compatible with the background-only hypothesis. In the absence of evidence for a signal, we set upper limits on the flux of muon neutrinos. For an E-2 neutrino spectrum, the observed limits are (0.9-5) x 10(-12) TeV-1 cm(-2) s(-1) for energies between 1 TeV and 1 PeV in the northern sky and (0.9-23.2) x 10(-12) TeV-1 cm(-2) s(-1) for energies between 10(2) TeV and 10(2) PeV in the southern sky. We also report upper limits for neutrino emission from groups of sources that were selected according to theoretical models or observational parameters and analyzed with a stacking approach. Some of the limits presented already reach the level necessary to quantitatively test current models of neutrino emission. C1 [Aartsen, M. G.; Hill, G. C.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Abbasi, R.; Ahlers, M.; Auffenberg, J.; Baker, M.; BenZvi, S.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kelley, J. L.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Abbasi, R.; Ahlers, M.; Auffenberg, J.; Baker, M.; BenZvi, S.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kelley, J. L.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Abdou, Y.; Carson, M.; De Ridder, S.; Feusels, T.; Ismail, A. Haj; Jlelati, O.; Labare, M.; Ryckbosch, D.; Van Overloop, A.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Ackermann, M.; Benabderrahmane, M. L.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Brunner, J.; Silva, A. H. Cruz; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Kaminsky, B.; Karg, T.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Stoessl, A.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. [Adams, J.; Brown, A. M.; Hickford, S.; Macias, O.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Aguilar, J. A.; Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [Altmann, D.; de With, M.; Kappes, A.; Kolanoski, H.; Waldenmaier, T.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Barwick, S. W.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Baum, V.; Eberhardt, B.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Bay, R.; Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Bechet, S.; Hanson, K.; Heereman, D.; Meures, T.; O'Murchadha, A.; Pinat, E.] Univ Libre Brussels, Sci Fac CP230, B-1050 Brussels, Belgium. [Tjus, J. Becker; Fedynitch, A.; Saba, S. M.; Schoeneberg, S.; Unger, E.] Ruhr Univ Bochum, Fac Phys & Astron, D-44780 Bochum, Germany. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D.; Tepe, A.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Berley, D.; Blaufuss, E.; Christy, B.; Goodman, J. A.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Meagher, K.; Olivas, A.; Redl, P.; Richman, M.; Schmidt, T.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Bernhard, A.; Gross, A.; Leute, J.; Odrowski, S.; Resconi, E.; Schulz, O.; Sestayo, Y.] Tech Univ Munich, D-85748 Garching, Germany. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bissok, M.; Blumenthal, J.; Coenders, S.; Euler, S.; Hallen, P.; Heinen, D.; Jagielski, K.; Krings, K.; Leuermann, M.; Paul, L.; Raedel, L.; Reimann, R.; Schoenen, S.; Schukraft, A.; Vehring, M.; Wallraff, M.; Wiebusch, C. H.; Zierke, S.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Boersma, D. J.; Botner, O.; Hallgren, A.; de los Heros, C. Perez; Strom, R.; Taavola, H.] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Bohaichuk, S.; Grandmont, D. T.; Grant, D.; Nowicki, S. C.; Sheremata, C.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Bose, D.; Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; Golup, G.; Kunnen, J.; Maggi, G.; Miller, J.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Boeser, S.; Franckowiak, A.; Homeier, A.; Kowalski, M.; Schulte, L.; Stasik, A.; Usner, M.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Bruijn, R.; Cohen, S.; Ribordy, M.] Ecole Polytech Fed Lausanne, High Energy Phys Lab, CH-1015 Lausanne, Switzerland. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Clark, K.; Cowen, D. F.; DeYoung, T.; Dunkman, M.; Eagan, R.; Koskinen, D. J.; Salameh, T.; Smith, M. W. E.; Tesic, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Clevermann, F.; Frantzen, K.; Fuchs, T.; Koehne, J. -H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.; Scheriau, F.; Schmitz, M.; Ziemann, J.] TU Dortmund Univ, Dept Phys, Dortmund, Germany. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Ishihara, A.; Mase, K.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Larson, M. J.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Bai, X.] South Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Huelsnitz, W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Montaruli, T.] Sezione Ist Nazl Fis Nucl, Dipartimento Fis, I-70126 Bari, Italy. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Aartsen, MG (reprint author), Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. RI Taavola, Henric/B-4497-2011; Tjus, Julia/G-8145-2012; Wiebusch, Christopher/G-6490-2012; Auffenberg, Jan/D-3954-2014; Koskinen, David/G-3236-2014; Brunner, Juergen/G-3540-2015; Aguilar Sanchez, Juan Antonio/H-4467-2015; Maruyama, Reina/A-1064-2013; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011 OI Taavola, Henric/0000-0002-2604-2810; Carson, Michael/0000-0003-0400-7819; Perez de los Heros, Carlos/0000-0002-2084-5866; Benabderrahmane, Mohamed Lotfi/0000-0003-4410-5886; Rott, Carsten/0000-0002-6958-6033; Ter-Antonyan, Samvel/0000-0002-5788-1369; Schukraft, Anne/0000-0002-9112-5479; Wiebusch, Christopher/0000-0002-6418-3008; Auffenberg, Jan/0000-0002-1185-9094; Koskinen, David/0000-0002-0514-5917; Brunner, Juergen/0000-0002-5052-7236; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Maruyama, Reina/0000-0003-2794-512X; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952 FU US National Science Foundation's Office of Polar Programs; US National Science Foundation's Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison; Open Science Grid (OSG) grid infrastructure; US Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada; West-Grid; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus program; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF) FX We acknowledge support from the following agencies: US National Science Foundation's Office of Polar Programs, US National Science Foundation's Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; US Department of Energy and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, West-Grid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus program, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; and National Research Foundation of Korea (NRF). NR 88 TC 43 Z9 43 U1 0 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR 132 DI 10.1088/0004-637X/779/2/132 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200042 ER PT J AU Aliu, E Archambault, S Arlen, T Aune, T Beilicke, M Benbow, W Bird, R Bouvier, A Buckley, JH Bugaev, V Cesarini, A Ciupik, L Connolly, MP Cui, W Dumm, J Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fortin, P Fortson, L Furniss, A Galante, N Gerard, L Gillanders, GH Griffin, S Grube, J Gyuk, G Hanna, D Holder, J Hughes, G Humensky, TB Kaaret, P Kertzman, M Khassen, Y Kieda, D Krawczynski, H Krennrich, F Lang, MJ Madhavan, AS Maier, G Majumdar, P McArthur, S McCann, A Moriarty, P Mukherjee, R Nieto, D De Bhroithe, AO Ong, RA Orr, M Otte, AN Park, N Perkins, JS Pohl, M Popkow, A Prokoph, H Quinn, J Ragan, K Reyes, LC Reynolds, PT Richards, GT Roache, E Saxon, DB Sembroski, GH Skole, C Smith, AW Soares-Furtado, M Staszak, D Telezhinsky, I Tesic, G Theiling, M Varlotta, A Vassiliev, VV Vincent, S Wakely, SP Weekes, TC Weinstein, A Welsing, R Williams, DA Zitzer, B Bottcher, M Fumagalli, M Jadhav, J AF Aliu, E. Archambault, S. Arlen, T. Aune, T. Beilicke, M. Benbow, W. Bird, R. Bouvier, A. Buckley, J. H. Bugaev, V. Cesarini, A. Ciupik, L. Connolly, M. P. Cui, W. Dumm, J. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortin, P. Fortson, L. Furniss, A. Galante, N. Gerard, L. Gillanders, G. H. Griffin, S. Grube, J. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krawczynski, H. Krennrich, F. Lang, M. J. Madhavan, A. S. Maier, G. Majumdar, P. McArthur, S. McCann, A. Moriarty, P. Mukherjee, R. Nieto, D. De Bhroithe, A. O'Faolain Ong, R. A. Orr, M. Otte, A. N. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Prokoph, H. Quinn, J. Ragan, K. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Saxon, D. B. Sembroski, G. H. Skole, C. Smith, A. W. Soares-Furtado, M. Staszak, D. Telezhinsky, I. Tesic, G. Theiling, M. Varlotta, A. Vassiliev, V. V. Vincent, S. Wakely, S. P. Weekes, T. C. Weinstein, A. Welsing, R. Williams, D. A. Zitzer, B. Bottcher, M. Fumagalli, M. Jadhav, J. CA VERITAS Collaboration TI LONG TERM OBSERVATIONS OF B2 1215+30 WITH VERITAS SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: general; BL Lacertae objects: individual (B2 1215+30, VER J1217+301) ID BL LACERTAE OBJECTS; LARGE-AREA TELESCOPE; SIMULTANEOUS MULTIWAVELENGTH OBSERVATIONS; SWIFT ULTRAVIOLET/OPTICAL TELESCOPE; SPECTRAL ENERGY-DISTRIBUTIONS; ACTIVE GALACTIC NUCLEI; GAMMA-RAY ASTRONOMY; BACKGROUND-RADIATION; LAC OBJECTS; W-COMAE AB We report on VERITAS observations of the BL Lac object B2 1215+30 between 2008 and 2012. During this period, the source was detected at very high energies (VHEs; E > 100 GeV) by VERITAS with a significance of 8.9s and showed clear variability on timescales larger than months. In 2011, the source was found to be in a relatively bright state and a power-law fit to the differential photon spectrum yields a spectral index of 3.6 +/- 0.4(stat) +/- 0.3(syst) with an integral flux above 200 GeV of (8.0 +/- 0.9(stat) +/- 3.2(syst)) x 10(-12) cm(-2) s(-1). No short term variability could be detected during the bright state in 2011. Multi-wavelength data were obtained contemporaneously with the VERITAS observations in 2011 and cover optical (Super-LOTIS, MDM, Swift/UVOT), X-ray (Swift/XRT), and gamma-ray (Fermi-LAT) frequencies. These were used to construct the spectral energy distribution (SED) of B2 1215+30. A one-zone leptonic model is used to model the blazar emission and the results are compared to those of MAGIC from early 2011 and other VERITAS-detected blazars. The SED can be reproduced well with model parameters typical for VHE-detected BL Lac objects. C1 [Aliu, E.; Errando, M.; Mukherjee, R.] Columbia Univ Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Archambault, S.; Griffin, S.; Hanna, D.; Ragan, K.; Staszak, D.; Tesic, G.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Arlen, T.; Aune, T.; Majumdar, P.; Ong, R. A.; Popkow, A.; Vassiliev, V. V.] Calif State Univ Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Beilicke, M.; Buckley, J. H.; Bugaev, V.; Krawczynski, H.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Fortin, P.; Galante, N.; Roache, E.; Weekes, T. C.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Bird, R.; Khassen, Y.; De Bhroithe, A. O'Faolain; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Bouvier, A.; Furniss, A.; Soares-Furtado, M.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Bouvier, A.; Furniss, A.; Soares-Furtado, M.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Cesarini, A.; Connolly, M. P.; Gillanders, G. H.; Lang, M. J.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Cui, W.; Feng, Q.; Finley, J. P.; Sembroski, G. H.; Theiling, M.; Varlotta, A.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Dumm, J.; Fortson, L.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Federici, S.; Gerard, L.; Hughes, G.; Maier, G.; Pohl, M.; Prokoph, H.; Skole, C.; Telezhinsky, I.; Vincent, S.; Welsing, R.] DESY, D-15738 Zeuthen, Germany. [Federici, S.; Pohl, M.; Telezhinsky, I.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Fortin, P.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Holder, J.; Saxon, D. B.] Univ Delaware, Dept Phys, Newark, DE 19716 USA. [Holder, J.; Saxon, D. B.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Humensky, T. B.; Nieto, D.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Kieda, D.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Krennrich, F.; Madhavan, A. S.; Orr, M.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Majumdar, P.] Saha Inst Nucl Phys, Kolkata 700064, India. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Galway, Ireland. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Perkins, J. S.] CRESST, Greenbelt, MD 20771 USA. [Perkins, J. S.] Astroparticle Phys Lab NASA GSFC, Greenbelt, MD 20771 USA. [Perkins, J. S.] Univ Maryland Baltimore Cty, Baltimore, MD 21250 USA. [Reyes, L. C.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 94307 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. [Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Bottcher, M.; Jadhav, J.] North West Univ, Ctr Space Res, ZA-2520 Potchefstroom, South Africa. [Bottcher, M.] Ohio Univ, Inst Astrophys, Dept Phys & Astron, Athens, OH 45701 USA. [Fumagalli, M.] Carnegie Observ, Pasadena, CA 91101 USA. [Fumagalli, M.] Princeton Univ, Dept Astrophys, Princeton, NJ 08544 USA. RP Aliu, E (reprint author), Columbia Univ Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. EM heike.prokoph@desy.de RI Khassen, Yerbol/I-3806-2015; Nieto, Daniel/J-7250-2015; Fumagalli, Michele/K-9510-2015; OI Cui, Wei/0000-0002-6324-5772; Khassen, Yerbol/0000-0002-7296-3100; Nieto, Daniel/0000-0003-3343-0755; Fumagalli, Michele/0000-0001-6676-3842; Cesarini, Andrea/0000-0002-8611-8610; Errando, Manel/0000-0002-1853-863X; Lang, Mark/0000-0003-4641-4201; Bird, Ralph/0000-0002-4596-8563 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the U.K.; NASA Swift Guest Investigator program [NNX12AJ12G]; Helmholtz Association; South African Research Chairs Initiative of the Department of Science and Technology; National Research Foundation of South Africa; NASA through Hubble Fellowship grant [HF-51305.01-A]; Space Telescope Science Institute; NASA [NAS 5-26555] FX This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748) and by STFC in the U.K., as well as award NNX12AJ12G from the NASA Swift Guest Investigator program. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. We are also grateful to Grant Williams and Daniel Kiminki for their dedication to the operation and support of the Super-LOTIS telescope. H.P. acknowledges support through the Young Investigators Program of the Helmholtz Association. M.B. acknowledges support by the South African Research Chairs Initiative of the Department of Science and Technology and the National Research Foundation of South Africa. Support for M.F. was provided by NASA through Hubble Fellowship grant HF-51305.01-A awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555. NR 59 TC 7 Z9 7 U1 0 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR 92 DI 10.1088/0004-637X/779/2/92 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200002 ER PT J AU An, HJ Hascoet, R Kaspi, VM Beloborodov, AM Dufour, F Gotthelf, EV Archibald, R Bachetti, M Boggs, SE Christensen, FE Craig, WW Greffenstette, BW Hailey, CJ Harrison, FA Kitaguchi, T Kouveliotou, C Madsen, KK Markwardt, CB Stern, D Vogel, JK Zhang, WW AF An, Hongjun Hascoet, Romain Kaspi, Victoria M. Beloborodov, Andrei M. Dufour, Francois Gotthelf, Eric V. Archibald, Robert Bachetti, Matteo Boggs, Steven E. Christensen, Finn E. Craig, William W. Greffenstette, Brian W. Hailey, Charles J. Harrison, Fiona A. Kitaguchi, Takao Kouveliotou, Chryssa Madsen, Kristin K. Markwardt, Craig B. Stern, Daniel Vogel, Julia K. Zhang, William W. TI NuSTAR OBSERVATIONS OF MAGNETAR 1E 1841-045 SO ASTROPHYSICAL JOURNAL LA English DT Article DE pulsars: individual (1E 1841-045); stars: magnetars; stars: neutron ID X-RAY PULSAR; SOFT GAMMA-REPEATERS; HIGH-ENERGY CHARACTERISTICS; SWIFT J1822.3-1606; NEUTRON-STARS; XMM-NEWTON; 4U 0142+61; SPIN-DOWN; KES 73; EMISSION AB We report new spectral and temporal observations of the magnetar 1E 1841-045 in the Kes 73 supernova remnant obtained with the Nuclear Spectroscopic Telescope Array. Combined with new Swift and archival XMM-Newton and Chandra observations, the phase-averaged spectrum is well characterized by a blackbody plus double power law, in agreement with previous multimission X-ray results. However, we are unable to reproduce the spectral results reported based on Suzaku observations. The pulsed fraction of the source is found to increase with photon energy. The measured rms pulsed fractions are similar to 12% and similar to 17% at similar to 20 and similar to 50 keV, respectively. We detect a new feature in the 24-35 keV band pulse profile that is uniquely double peaked. This feature may be associated with a possible absorption or emission feature in the phase-resolved spectrum. We fit the X-ray data using the recently developed electron-positron outflow model by Beloborodov for the hard X-ray emission from magnetars. This produces a satisfactory fit, allowing a constraint on the angle between the rotation and magnetic axes of the neutron star of similar to 20 degrees and on the angle between the rotation axis and line of sight of similar to 50 degrees. In this model, the soft X-ray component is inconsistent with a single blackbody; adding a second blackbody or a power-law component fits the data. The two-blackbody interpretation suggests a hot spot of temperature kT approximate to 0.9 keV occupying similar to 1% of the stellar surface. C1 [An, Hongjun; Kaspi, Victoria M.; Dufour, Francois; Archibald, Robert] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Hascoet, Romain; Beloborodov, Andrei M.; Gotthelf, Eric V.; Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Bachetti, Matteo] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Bachetti, Matteo] Inst Rech Astrophys & Planetol, CNRS, F-31028 Toulouse 4, France. [Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, Finn E.] Tech Univ Denmark, DTU Space, Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, William W.; Vogel, Julia K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Greffenstette, Brian W.; Harrison, Fiona A.; Madsen, Kristin K.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Kitaguchi, Takao] RIKEN, Wako, Saitama 3510198, Japan. [Kouveliotou, Chryssa] NASA, George C Marshall Space Flight Ctr, Space Sci Off, Huntsville, AL 35812 USA. [Markwardt, Craig B.; Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP An, HJ (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337; Madsen, Kristin/0000-0003-1252-4891 FU NASA [NNG08FD60C, NNX10AI72G, NNX13AI34G]; NSERC Discovery Grant; FQRNT Centre de Recherche Astrophysique du Quebec; R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Research (CIFAR); Canada Research Chairs Program; Lorne Trottier Chair in Astrophysics and Cosmology; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported under NASA contract NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration Teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS), jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (US). V. M. K. acknowledges support from an NSERC Discovery Grant, the FQRNT Centre de Recherche Astrophysique du Quebec, an R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Research (CIFAR), the Canada Research Chairs Program, and the Lorne Trottier Chair in Astrophysics and Cosmology. A. M. B. acknowledges the support by NASA grants NNX10AI72G and NNX13AI34G. Part of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 45 TC 12 Z9 12 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR 163 DI 10.1088/0004-637X/779/2/163 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200072 ER PT J AU Archambault, S Beilicke, M Benbow, W Berger, K Bird, R Bouvier, A Buckley, JH Bugaev, V Byrum, K Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Duke, C Dumm, J Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fortson, L Furniss, A Galante, N Gillanders, GH Griffin, S Griffiths, ST Grube, J Gyuk, G Hanna, D Holder, J Hughes, G Humensky, TB Kaaret, P Kertzman, M Khassen, Y Kieda, D Krawczynski, H Lang, MJ Madhavan, AS Maier, G Majumdar, P McArthur, S McCann, A Moriarty, P Mukherjee, R Nieto, D de Bhroithe, AO Ong, RA Otte, AN Pandel, D Park, N Perkins, JS Pohl, M Popkow, A Prokoph, H Quinn, J Ragan, K Rajotte, J Reyes, LC Reynolds, PT Richards, GT Roache, E Sembroski, GH Sheidaei, F Smith, AW Staszak, D Telezhinsky, I Theiling, M Tucci, JV Tyler, J Varlotta, A Vincent, S Wakely, SP Weekes, TC Weinstein, A Williams, DA Zitzer, B McCollough, ML AF Archambault, S. Beilicke, M. Benbow, W. Berger, K. Bird, R. Bouvier, A. Buckley, J. H. Bugaev, V. Byrum, K. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Duke, C. Dumm, J. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortson, L. Furniss, A. Galante, N. Gillanders, G. H. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krawczynski, H. Lang, M. J. Madhavan, A. S. Maier, G. Majumdar, P. McArthur, S. McCann, A. Moriarty, P. Mukherjee, R. Nieto, D. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Pandel, D. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Prokoph, H. Quinn, J. Ragan, K. Rajotte, J. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Sembroski, G. H. Sheidaei, F. Smith, A. W. Staszak, D. Telezhinsky, I. Theiling, M. Tucci, J. V. Tyler, J. Varlotta, A. Vincent, S. Wakely, S. P. Weekes, T. C. Weinstein, A. Williams, D. A. Zitzer, B. McCollough, M. L. CA VERITAS Collaboration Smithsonian Astrophys Observ TI VERITAS OBSERVATIONS OF THE MICROQUASAR CYGNUS X-3 SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; binaries: close; gamma rays: stars; X-rays: individual (Cygnus X-3) ID GAMMA-RAY EMISSION; LARGE-AREA TELESCOPE; X-RAY; CYG X-3; CHERENKOV TELESCOPES; RELATIVISTIC JET; SCATTERING HALO; CONSTRAINTS; MISSION; SEARCH AB We report results from TeV gamma-ray observations of the microquasar Cygnus X-3. The observations were made with the Very Energetic Radiation Imaging Telescope Array System (VERITAS) over a time period from 2007 June 11 to 2011 November 28. VERITAS is most sensitive to gamma rays at energies between 85 GeV and 30 TeV. The effective exposure time amounts to a total of about 44 hr, with the observations covering six distinct radio/X-ray states of the object. No significant TeV gamma-ray emission was detected in any of the states, nor with all observations combined. The lack of a positive signal, especially in the states where GeV gamma rays were detected, places constraints on TeV gamma-ray production in Cygnus X-3. We discuss the implications of the results. C1 [Archambault, S.; Griffin, S.; Hanna, D.; Ragan, K.; Rajotte, J.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Beilicke, M.; Buckley, J. H.; Bugaev, V.; Krawczynski, H.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Cerruti, M.; Galante, N.; Roache, E.; Weekes, T. C.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Berger, K.; Holder, J.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Berger, K.; Holder, J.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bird, R.; Khassen, Y.; de Bhroithe, A. O'Faolain; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Byrum, K.; Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Chen, X.; Federici, S.; Pohl, M.; Telezhinsky, I.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Chen, X.; Federici, S.; Hughes, G.; Maier, G.; Pohl, M.; Prokoph, H.; Telezhinsky, I.; Vincent, S.] DESY, D-15738 Zeuthen, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Gillanders, G. H.; Lang, M. J.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Cui, W.; Feng, Q.; Finley, J. P.; Sembroski, G. H.; Theiling, M.; Tucci, J. V.; Varlotta, A.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Duke, C.] Grinnell Coll, Dept Phys, Grinnell, IA 50112 USA. [Dumm, J.; Fortson, L.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Errando, M.; Mukherjee, R.] Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Griffiths, S. T.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Humensky, T. B.; Nieto, D.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Kieda, D.; Sheidaei, F.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Madhavan, A. S.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Majumdar, P.; Ong, R. A.; Popkow, A.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Majumdar, P.] Saha Inst Nucl Phys, Kolkata 700064, India. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Galway, Ireland. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Pandel, D.] Grand Valley State Univ, Dept Phys, Allendale, MI 49401 USA. [Perkins, J. S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Reyes, L. C.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 94307 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. [McCollough, M. L.] Smithsonian Astrophys Observ, Cambridge, MA 02138 USA. RP Cui, W (reprint author), Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. EM cui@purdue.edu; avarlott@purdue.edu RI Khassen, Yerbol/I-3806-2015; Nieto, Daniel/J-7250-2015; OI Khassen, Yerbol/0000-0002-7296-3100; Nieto, Daniel/0000-0003-3343-0755; Cui, Wei/0000-0002-6324-5772; Pandel, Dirk/0000-0003-2085-5586; Lang, Mark/0000-0003-4641-4201; Bird, Ralph/0000-0002-4596-8563 FU NASA through a Fermi GI grant [NNX11AP90G]; Purdue University; U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the U.K. FX This work has made use of high-level data products provided by the ASM/RXTE, MAXI, and BAT/Swift teams. The AMI-LA radio results were obtained from a public archive maintained by Guy Pooley. Paul Ray is thanked for making available the ephemeris for PSR J2032+4127. A. V. and W. C. gratefully acknowledge financial support from NASA through a Fermi GI grant (NNX11AP90G) and from Purdue University. The VERI-TAS operation is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748), and by STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. NR 48 TC 2 Z9 2 U1 0 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR UNSP 150 DI 10.1088/0004-637X/779/2/150 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200059 ER PT J AU Howell, DA Kasen, D Lidman, C Sullivan, M Conley, A Astier, P Balland, C Carlberg, RG Fouchez, D Guy, J Hardin, D Pain, R Palanque-Delabrouille, N Perrett, K Pritchet, CJ Regnault, N Rich, J Ruhlmann-Kleider, V AF Howell, D. A. Kasen, D. Lidman, C. Sullivan, M. Conley, A. Astier, P. Balland, C. Carlberg, R. G. Fouchez, D. Guy, J. Hardin, D. Pain, R. Palanque-Delabrouille, N. Perrett, K. Pritchet, C. J. Regnault, N. Rich, J. Ruhlmann-Kleider, V. TI TWO SUPERLUMINOUS SUPERNOVAE FROM THE EARLY UNIVERSE DISCOVERED BY THE SUPERNOVA LEGACY SURVEY SO ASTROPHYSICAL JOURNAL LA English DT Article DE supernovae: general ID CORE-COLLAPSE SUPERNOVAE; PAIR-INSTABILITY; LIGHT CURVES; MEASURED METALLICITIES; IC SUPERNOVAE; IA SUPERNOVAE; EXPLOSION; GALAXIES; TRANSIENT; SPECTROSCOPY AB We present spectra and light curves of SNLS 06D4eu and SNLS 07D2bv, two hydrogen-free superluminous supernovae (SNe) discovered by the Supernova Legacy Survey. At z = 1.588, SNLS 06D4eu is the highest redshift superluminous SN with a spectrum, at M-U = -22.7 it is one of the most luminous SNe ever observed, and it gives a rare glimpse into the rest-frame ultraviolet where these SNe put out their peak energy. SNLS 07D2bv does not have a host galaxy redshift, but on the basis of the SN spectrum, we estimate it to be at z similar to 1.5. Both SNe have similar observer-frame griz light curves, which map to rest-frame light curves in the U band and UV, rising in similar to 20 rest-frame days or longer and declining over a similar timescale. The light curves peak in the shortest wavelengths first, consistent with an expanding blackbody starting near 15,000 K and steadily declining in temperature. We compare the spectra with theoretical models, and we identify lines of C II, C III, Fe III, and Mg II in the spectra of SNLS 06D4eu and SCP 06F6 and find that they are consistent with an expanding explosion of only a few solar masses of carbon, oxygen, and other trace metals. Thus, the progenitors appear to be related to those suspected for SNe Ic. A high kinetic energy, 10(52) erg, is also favored. Normal mechanisms of powering core-collapse or thermonuclear SNe do not seem to work for these SNe. We consider models powered by Ni-56 decay and interaction with circumstellar material, but we find that the creation and spin-down of a magnetar with a period of 2 ms, a magnetic field of 2 x 10(14) G, and a 3 M-circle dot progenitor provides the best fit to the data. C1 [Howell, D. A.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. [Howell, D. A.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Kasen, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kasen, D.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Kasen, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Lidman, C.] Australian Astron Observ, N Ryde, NSW 1670, Australia. [Sullivan, M.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Conley, A.] Univ Colorado, Ctr Astrophys & Space Astron, Boulder, CO 80309 USA. [Astier, P.; Balland, C.; Guy, J.; Hardin, D.; Pain, R.; Regnault, N.] CNRS, IN2P3, LPNHE, F-75005 Paris, France. [Astier, P.; Balland, C.; Guy, J.; Hardin, D.; Pain, R.; Regnault, N.] Univ Paris VI & VII, F-75005 Paris, France. [Balland, C.] Univ Paris 11, F-91405 Orsay, France. [Carlberg, R. G.] Univ Toronto, Dept Astron & Astrophys, Toronto, ON M5S 3H8, Canada. [Fouchez, D.] CNRS, IN2P3, CPPM, F-13288 Marseille 9, France. [Fouchez, D.] Univ Aix Marseille 2, F-13288 Marseille 9, France. [Palanque-Delabrouille, N.; Rich, J.; Ruhlmann-Kleider, V.] CEA Saclay, DSM, IRFU, SPP, F-91191 Gif Sur Yvette, France. [Perrett, K.] DRDC Ottawa, Ottawa, ON K1A 0Z4, Canada. [Pritchet, C. J.] Univ Victoria, Dept Phys & Astron, Victoria, BC V8W 3P6, Canada. RP Howell, DA (reprint author), Las Cumbres Observ Global Telescope Network, 6740 Cortona Dr,Suite 102, Goleta, CA 93117 USA. OI Sullivan, Mark/0000-0001-9053-4820 FU LCOGT; Oskar Klein Center at the University of Stockholm; ESO programs [176.A-0589, 384.D-0222]; Natural Sciences and Engineering Research Council of Canada; French state funds; ANR within the Investissements d'Avenir program [ANR-1-IDEX-0005-02] FX D.A.H. acknowledges support from LCOGT. C. Lidman acknowledges the support provided by the Oskar Klein Center at the University of Stockholm. Based on observations obtained with MegaPrime/MegaCam, a joint project of CFHT and CEA/DAPNIA, at the Canada-France-Hawaii Telescope (CFHT), which is operated by the National Research Council (NRC) of Canada, the Institut National des Science de l'Univers of the Centre National de la Recherche Scientifique (CNRS) of France, and the University of Hawaii. Based in part on observations taken at the ESO Paranal Observatory (ESO programs 176.A-0589 and 384.D-0222). C.P. and R.C. acknowledge financial support from the Natural Sciences and Engineering Research Council of Canada. This work was supported in part by French state funds managed by the ANR within the Investissements d'Avenir program under reference ANR-1-IDEX-0005-02. NR 41 TC 28 Z9 29 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR UNSP 98 DI 10.1088/0004-637X/779/2/98 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200008 ER PT J AU Klein, SR Mikkelsen, RE Tjus, JB AF Klein, Spencer R. Mikkelsen, Rune E. Tjus, Julia Becker TI MUON ACCELERATION IN COSMIC-RAY SOURCES SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; astroparticle physics; magnetic fields; neutrinos; relativistic processes ID HIGH-ENERGY NEUTRINOS; SHOCK FRONTS; COLD MEDIA; BURSTS; MAGNETARS; TRANSPORT; ORIGIN; FLUX AB Many models of ultra-high energy cosmic-ray production involve acceleration in linear accelerators located in gamma-ray bursts, magnetars, or other sources. These transient sources have short lifetimes, which necessitate very high accelerating gradients, up to 1013 keV cm(-1). At gradients above 1.6 keV cm-1, muons produced by hadronic interactions undergo significant acceleration before they decay. This muon acceleration hardens the neutrino energy spectrum and greatly increases the high-energy neutrino flux. Using the IceCube high-energy diffuse neutrino flux limits, we set two-dimensional limits on the source opacity and matter density, as a function of accelerating gradient. These limits put strong constraints on different models of particle acceleration, particularly those based on plasma wake-field acceleration, and limit models for sources like gamma-ray bursts and magnetars. C1 [Klein, Spencer R.; Mikkelsen, Rune E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Klein, Spencer R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mikkelsen, Rune E.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Tjus, Julia Becker] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. RP Klein, SR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RI Tjus, Julia/G-8145-2012 FU U.S. National Science Foundation [0653266]; U.S. Department of Energy [DE-AC02-05CH11231] FX We thank R. Schlickeiser and W. Winter for comments. This work was funded in part by the U.S. National Science Foundation under grant No. 0653266 and the U.S. Department of Energy under contract number DE-AC02-05CH11231. NR 41 TC 12 Z9 12 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR 106 DI 10.1088/0004-637X/779/2/106 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200016 ER PT J AU Walton, DJ Fuerst, F Harrison, F Stern, D Bachetti, M Barret, D Bauer, F Boggs, SE Christensen, FE Craig, WW Fabian, AC Grefenstette, BW Hailey, CJ Madsen, KK Miller, JM Ptak, A Rana, V Webb, NA Zhang, WW AF Walton, D. J. Fuerst, F. Harrison, F. Stern, D. Bachetti, M. Barret, D. Bauer, F. Boggs, S. E. Christensen, F. E. Craig, W. W. Fabian, A. C. Grefenstette, B. W. Hailey, C. J. Madsen, K. K. Miller, J. M. Ptak, A. Rana, V. Webb, N. A. Zhang, W. W. TI AN EXTREMELY LUMINOUS AND VARIABLE ULTRALUMINOUS X-RAY SOURCE IN THE OUTSKIRTS OF CIRCINUS OBSERVED WITH NuSTAR SO ASTROPHYSICAL JOURNAL LA English DT Article DE black hole physics; X-rays: binaries; X-rays: individual (Circinus ULX5) ID MASS BLACK-HOLES; ACTIVE GALACTIC NUCLEI; HOLMBERG IX X-1; SPECTRAL STATE TRANSITIONS; SPITZER-SPACE-TELESCOPE; PHOTON IMAGING CAMERA; COOL ACCRETION DISKS; NGC 1313 X-1; XMM-NEWTON; ESO 243-49 AB Following a serendipitous detection with the Nuclear Spectroscopic Telescope Array (NuSTAR), we present a multi-epoch spectral and temporal analysis of an extreme ultraluminous X-ray source (ULX) located in the outskirts of the Circinus galaxy, hereafter Circinus ULX5, including coordinated XMM-Newton+NuSTAR follow-up observations. The NuSTAR data presented here represent one of the first instances of a ULX reliably detected at hard (E > 10 keV) X-rays. Circinus ULX5 is variable on long time scales by at least a factor of similar to 5 in flux, and was caught in a historically bright state during our 2013 observations (0.3-30.0 keV luminosity of 1.6 x 10(40) erg s(-1)). During this epoch, the source displayed a curved 3-10 keV spectrum, broadly similar to other bright ULXs. Although pure thermal models result in a high energy excess in the NuSTAR data, this excess is too weak to be modeled with the disk reflection interpretation previously proposed to explain the 3-10 keV curvature in other ULXs. In addition to flux variability, clear spectral variability is also observed. While in many cases the interpretation of spectral components in ULXs is uncertain, the spectral and temporal properties of all the high quality data sets currently available strongly support a simple disk-corona model reminiscent of that invoked for Galactic binaries, with the accretion disk becoming more prominent as the luminosity increases. However, although the disk temperature and luminosity are well correlated across all time scales currently probed, the observed luminosity follows L proportional to T1.70+/-0.17, flatter than expected for simple blackbody radiation. The spectral variability displayed here is highly reminiscent of that observed from known Galactic black hole binaries (BHBs) at high luminosities. This comparison implies a black hole mass of similar to 90 M-circle dot for Circinus ULX5. However, given the diverse behavior observed from Galactic BHB accretion disks, this mass estimate is still uncertain. Finally, the limits placed on any undetected iron absorption features with the 2013 data set imply that we are not viewing the central regions of Circinus ULX5 through any extreme super-Eddington outflow. C1 [Walton, D. J.; Fuerst, F.; Harrison, F.; Stern, D.; Grefenstette, B. W.; Madsen, K. K.; Rana, V.] CALTECH, Space Radiat Lab, Pasadena, CA 91125 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Bachetti, M.; Barret, D.; Webb, N. A.] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Bachetti, M.; Barret, D.; Webb, N. A.] IRAP, CNRS, F-31028 Toulouse 4, France. [Bauer, F.] Pontificia Univ Catolica Chile, Fac Fis, Inst Astrofis, Santiago 22, Chile. [Bauer, F.] Space Sci Inst, Boulder, CO 80301 USA. [Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Fabian, A. C.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Miller, J. M.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Ptak, A.; Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Walton, DJ (reprint author), CALTECH, Space Radiat Lab, Pasadena, CA 91125 USA. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337; Rana, Vikram/0000-0003-1703-8796 FU NASA; XMM-Newton; ESA Member States; Suzaku observatory; Basal-CATA [PFB-06/2007]; CONICYT-Chile [FONDECYT 1101024, Anillo ACT1101]; Centre National DEtudes Spatiales (CNES) FX The authors thank Koji Mukai for useful discussion regarding Galactic CVs, and Rubens Reis for discussion regarding Galactic BHBs. This research has made use of data obtained with the NuSTAR mission, a project led by the California Institute of Technology (Caltech), managed by the Jet Propulsion Laboratory (JPL) and funded by NASA, XMM-Newton, an ESA science mission with instruments and contributions directly funded by ESA Member States and NASA, and the Suzaku observatory, a collaborative mission between the space agencies of Japan (JAXA) and the USA (NASA). In addition, this research has also made use of data obtained from NASA's Swift, Chandra, and Spitzer satellites. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NUSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and Caltech (USA). We also made use of the NASA/IPAC Extragalactic Database (NED), which is operated by JPL, Caltech, under contract with NASA. Some of the figures included in this work have been produced with the Veusz plotting package: http://home.gna.org/veusz, written and maintained by Jeremy Sanders. F. E. B. acknowledges support from Basal-CATA (PFB-06/2007) and CONICYT-Chile (under grants FONDECYT 1101024 and Anillo ACT1101). M. B. wishes to acknowledge the support from the Centre National DEtudes Spatiales (CNES). NR 126 TC 37 Z9 37 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR 148 DI 10.1088/0004-637X/779/2/148 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200057 ER PT J AU Wozniakiewicz, PJ Bradley, JP Ishii, HA Price, MC Brownlee, DE AF Wozniakiewicz, P. J. Bradley, J. P. Ishii, H. A. Price, M. C. Brownlee, D. E. TI PRE-ACCRETIONAL SORTING OF GRAINS IN THE OUTER SOLAR NEBULA SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; comets: general; Kuiper belt: general; protoplanetary disks ID INTERPLANETARY DUST PARTICLES; IRON-NICKEL SULFIDES; ORDINARY CHONDRITES; SIZE DISTRIBUTION; INTERSTELLAR GRAINS; CHONDRULES; METAL; GEMS; IDENTIFICATION; DISTRIBUTIONS AB Despite their micrometer-scale dimensions and nanogram masses, chondritic porous interplanetary dust particles (CP IDPs) are an important class of extraterrestrial material since their properties are consistent with a cometary origin and they show no evidence of significant post-accretional parent body alteration. Consequently, they can provide information about grain accretion in the comet-forming region of the outer solar nebula. We have previously reported our comparative study of the sizes and size distributions of crystalline silicate and sulfide grains in CP IDPs, in which we found these components exhibit a size-density relationship consistent with having been sorted together prior to accretion. Here we extend our data set and include GEMS (glass with embedded metal and sulfide), the most abundant amorphous silicate phase observed in CP IDPs. We find that while the silicate and sulfide sorting trend previously observed is maintained, the GEMS size data do not exhibit any clear relationship to these crystalline components. Therefore, GEMS do not appear to have been sorted with the silicate and sulfide crystals. The disparate sorting trends observed in GEMS and the crystalline grains in CP IDPs present an interesting challenge for modeling early transport and accretion processes. They may indicate that several sorting mechanisms operated on these CP IDP components, or alternatively, they may simply be a reflection of different source environments. C1 [Wozniakiewicz, P. J.] Nat Hist Museum, Dept Earth Sci, Mineral & Planetary Sci Div, London SW7 5BD, England. [Wozniakiewicz, P. J.; Price, M. C.] Univ Kent, Sch Phys Sci, Canterbury CT2 7NH, Kent, England. [Bradley, J. P.; Ishii, H. A.] Lawrence Livermore Natl Lab, Inst Geophys & Planetary Phys, Livermore, CA 94550 USA. [Brownlee, D. E.] Univ Washington, Dept Astron, Seattle, WA 98195 USA. RP Wozniakiewicz, PJ (reprint author), Nat Hist Museum, Dept Earth Sci, Mineral & Planetary Sci Div, Cromwell Rd, London SW7 5BD, England. EM p.wozniakiewicz@nhm.ac.uk FU NASA's Cosmochemistry program; LDRD [09-ERI-004]; NASA's Laboratory Analysis of Returned Samples program; U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX This work was funded in part by a grant from NASA's Cosmochemistry program (J.P.B.) and LDRD grant 09-ERI-004 (J.P.B.). H. A. Ishii was supported by NASA's Laboratory Analysis of Returned Samples program. Portions of this work were performed under the auspices of the U.S. Department of Energy by LLNL under contract DE-AC52-07NA27344. NR 46 TC 3 Z9 3 U1 0 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR 164 DI 10.1088/0004-637X/779/2/164 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200073 ER PT J AU Zeimann, GR Stanford, SA Brodwin, M Gonzalez, AH Mancone, C Snyder, GF Stern, D Eisenhardt, P Dey, A Moustakas, J AF Zeimann, Gregory R. Stanford, S. A. Brodwin, Mark Gonzalez, Anthony H. Mancone, Conor Snyder, Gregory F. Stern, Daniel Eisenhardt, Peter Dey, Arjun Moustakas, John TI H alpha STAR FORMATION RATES OF z > 1 GALAXY CLUSTERS IN THE IRAC SHALLOW CLUSTER SURVEY SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: clusters: general; galaxies: evolution; galaxies: high-redshift ID FUNDAMENTAL METALLICITY RELATION; HUBBLE-SPACE-TELESCOPE; WIDE-FIELD SURVEY; X-RAY SURVEY; FORMING GALAXIES; RED SEQUENCE; STELLAR MASS; DENSITY RELATION; DUST EXTINCTION; LENSED GALAXIES AB We present Hubble Space Telescope near-IR spectroscopy for 18 galaxy clusters at 1.0 < z < 1.5 in the IRAC Shallow Cluster Survey. We use Wide Field Camera 3 grism data to spectroscopically identify H alpha emitters in both the cores of galaxy clusters as well as in field galaxies. We find a large cluster-to-cluster scatter in the star formation rates within a projected radius of 500 kpc, and many of our clusters (similar to 60%) have significant levels of star formation within a projected radius of 200 kpc. A stacking analysis reveals that dust reddening in these star-forming galaxies is positively correlated with stellar mass and may be higher in the field than the cluster at a fixed stellar mass. This may indicate a lower amount of gas in star-forming cluster galaxies than in the field population. Also, H alpha equivalent widths of star-forming galaxies in the cluster environment are still suppressed below the level of the field. This suppression is most significant for lower mass galaxies (log M-* < 10.0 M-circle dot). We therefore conclude that environmental effects are still important at 1.0 < z < 1.5 for star-forming galaxies in galaxy clusters with log M-* less than or similar to 10.0 M-circle dot. C1 [Zeimann, Gregory R.; Stanford, S. A.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Zeimann, Gregory R.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Stanford, S. A.] Lawrence Livermore Natl Lab, Inst Geophys & Planetary Phys, Livermore, CA 94550 USA. [Brodwin, Mark] Univ Missouri, Kansas City, MO 64110 USA. [Gonzalez, Anthony H.; Mancone, Conor] Univ Florida, Dept Astron, Gainesville, FL 32611 USA. [Snyder, Gregory F.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Stern, Daniel; Eisenhardt, Peter] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Dey, Arjun] Natl Opt Astron Observ, Tucson, AZ 85719 USA. [Moustakas, John] Siena Coll, Dept Phys & Astron, Loudonville, NY 12211 USA. RP Zeimann, GR (reprint author), Univ Calif Davis, Dept Phys, 1 Shields Ave, Davis, CA 95616 USA. FU National Science Foundation [AST-0708490]; NASA [NAS 5-26555]; JPL/Caltech; NASA through Space Telescope Science Institute [10496, 11002, 11597, 11663]; U.S. Department of Energy [W-7405-ENG-48] FX A.H.G. acknowledges support from the National Science Foundation through grant AST-0708490. This work is based in part on observations made with the Spitzer Space Telescope, which is operated by the Jet Propulsion Laboratory, California Institute of Technology under a contract with NASA. Support for this work was provided by NASA through an award issued by JPL/Caltech. Support for HST programs 10496, 11002, 11597, and 11663 were provided by NASA through a grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., under NASA contract NAS 5-26555. This work makes use of image data from the NOAO Deep Wide-Field Survey (NDWFS) as distributed by the NOAO Science Archive. NOAO is operated by the Association of Universities for Research in Astronomy (AURA), Inc., under a cooperative agreement with the National Science Foundation.; We thank Matt Ashby for creating the IRAC catalogs for SDWFS, Buell Jannuzi for his work on the NDWFS, Michael Brown for combining the NDWFS with SDWFS catalogs, and Steve Murray and the XBootes team for obtaining the Chandra data in the Bootes field. This paper would not have been possible without the efforts of the support staffs of the Spitzer Space Telescope, Hubble Space Telescope, and Chandra X-ray Observatory. The work by S. A. S. at LLNL was performed under the auspices of the U.S. Department of Energy under Contract No. W-7405-ENG-48. NR 66 TC 20 Z9 20 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 20 PY 2013 VL 779 IS 2 AR 137 DI 10.1088/0004-637X/779/2/137 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268RC UT WOS:000328187200046 ER PT J AU Agapov, RL Srijanto, B Fowler, C Briggs, D Lavrik, NV Sepaniak, MJ AF Agapov, Rebecca L. Srijanto, Bernadeta Fowler, Chris Briggs, Dayrl Lavrik, Nickolay V. Sepaniak, Michael J. TI Lithography-free approach to highly efficient, scalable SERS substrates based on disordered clusters of disc-on-pillar structures SO NANOTECHNOLOGY LA English DT Article ID ENHANCED RAMAN-SCATTERING; LARGE-AREA; METAL NANOPARTICLES; SURFACE; ARRAYS; SPECTROSCOPY; FABRICATION; NANOSTRUCTURES; NANOANTENNA; NANOPILLARS AB We present a lithography-free technological strategy that enables fabrication of large area substrates for surface-enhanced Raman spectroscopy (SERS) with excellent performance in the red to NIR spectral range. Our approach takes advantage of metal dewetting as a facile means to create stochastic arrays of circular patterns suitable for subsequent fabrication of plasmonic disc-on-pillar (DOP) structures using a combination of anisotropic reactive ion etching (RIE) and thin film deposition. Consistent with our previous studies of individual DOP structures, pillar height which, in turn, is defined by the RIE processing time, has a dramatic effect on the SERS performance of stochastic arrays of DOP structures. Our computational analysis of model DOP systems confirms the strong effect of the pillar height and also explains the broadband sensitivity of the implemented SERS substrates. Our Raman mapping data combined with SEM structural analysis of the substrates exposed to benzenethiol solutions indicates that clustering of shorter DOP structures and bundling of taller ones is a likely mechanism contributing to higher SERS activity. Nonetheless, bundled DOP structures appeared to be consistently less SERS-active than vertically aligned clusters of DOPs with optimized parameters. The latter are characterized by average SERS enhancement factors above 10(7). C1 [Agapov, Rebecca L.; Srijanto, Bernadeta; Fowler, Chris; Briggs, Dayrl; Lavrik, Nickolay V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Srijanto, Bernadeta] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Sepaniak, Michael J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Agapov, RL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM lavriknv@ornl.gov RI Lavrik, Nickolay/B-5268-2011; Srijanto, Bernadeta/D-4213-2016 OI Lavrik, Nickolay/0000-0002-9543-5634; Srijanto, Bernadeta/0000-0002-1188-1267 FU Division of Scientific User Facilities, US Department of Energy FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, US Department of Energy. NR 46 TC 8 Z9 8 U1 8 U2 52 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD DEC 20 PY 2013 VL 24 IS 50 AR 505302 DI 10.1088/0957-4484/24/50/505302 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 272RU UT WOS:000328478900004 PM 24285471 ER PT J AU Harrison, N Moll, PJW Sebastian, SE Balicas, L Altarawneh, MM Zhu, JX Tobash, PH Ronning, F Bauer, ED Batlogg, B AF Harrison, N. Moll, P. J. W. Sebastian, S. E. Balicas, L. Altarawneh, M. M. Zhu, J. -X. Tobash, P. H. Ronning, F. Bauer, E. D. Batlogg, B. TI Magnetic field-tuned localization of the 5f-electrons in URu2Si2 SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM PHASE-TRANSITIONS; FERMI-SURFACE; METAMAGNETIC TRANSITION; HIDDEN ORDER; CRITICAL PRESSURE; SUPERCONDUCTIVITY; CERHIN5; LATTICE AB We report Shubnikov-de Haas oscillation measurements within the high magnetic field (mu H-0 > 39 T) magnetically polarized regime of URu2Si2, made possible using mesoscopic samples prepared by means of focused ion beam lithography. A significant change in the Fermi surface topology relative to the "hidden-order" phase is observed, signaling a transformation into a high magnetic field regime in which 5f-electrons are removed from the Fermi surface. URu2Si2 is therefore a rare example of an actinide compound in which a transformation of 5f-electrons can be directly observed at low temperatures, setting the stage for the unconventional ordering and high magnetic field quantum criticality in this material. C1 [Harrison, N.; Zhu, J. -X.; Tobash, P. H.; Ronning, F.; Bauer, E. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Moll, P. J. W.; Batlogg, B.] ETH, Solid State Phys Lab, CH-8093 Zurich, Switzerland. [Sebastian, S. E.] Univ Cambridge, Cavendish Lab, Cambridge CB3 OHE, England. [Balicas, L.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Altarawneh, M. M.] Mutah Univ, Dept Phys, Mutah 61710, Karak, Jordan. RP Harrison, N (reprint author), Los Alamos Natl Lab, MS E536, Los Alamos, NM 87545 USA. OI Ronning, Filip/0000-0002-2679-7957; Harrison, Neil/0000-0001-5456-7756; Bauer, Eric/0000-0003-0017-1937; Zhu, Jianxin/0000-0001-7991-3918 FU US Department of Energy (DOE), Office of Basic Energy Sciences (BES); DOE-BES [DE-SC0002613]; US DOE, Office of BES, MSE Division; LANL LDRD program; US DOE; National Science Foundation; State of Florida FX N.H. and M.M.A.s acknowledge the provision of the US Department of Energy (DOE), Office of Basic Energy Sciences (BES) funding for the "Science of 100 Tesla." M. M. A. further acknowledges a Seaborg fellowship. L. B. is supported by DOE-BES through award DE-SC0002613. Work by P. H. T., F. R., and E. D. B. is supported by the US DOE, Office of BES, MSE Division and by the LANL LDRD program. S. E. S. acknowledges the Royal Society. Experiments were performed at the NHMFL, which is supported by the US DOE, the National Science Foundation and the State of Florida. N.H. thanks P. Oppeneer for providing cross-sections of the calculated Fermi surface. Electron microscopy and FIB work was performed at the Electron Microscopy group ETH Zurich (EMEZ). NR 33 TC 3 Z9 3 U1 5 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 20 PY 2013 VL 88 IS 24 AR 241108 DI 10.1103/PhysRevB.88.241108 PG 4 WC Physics, Condensed Matter SC Physics GA 275PF UT WOS:000328688600001 ER PT J AU Lazar, EA Mason, JK MacPherson, RD Srolovitz, DJ AF Lazar, Emanuel A. Mason, Jeremy K. MacPherson, Robert D. Srolovitz, David J. TI Statistical topology of three-dimensional Poisson-Voronoi cells and cell boundary networks SO PHYSICAL REVIEW E LA English DT Article ID SIZE DISTRIBUTION; GRAIN-GROWTH; MONTE-CARLO; PLANAR; TESSELATION; PARTITION; ALGORITHM; DIVISION; GEOMETRY; SPACE AB Voronoi tessellations of Poisson point processes are widely used for modeling many types of physical and biological systems. In this paper, we analyze simulated Poisson-Voronoi structures containing a total of 250 000 000 cells to provide topological and geometrical statistics of this important class of networks. We also report correlations between some of these topological and geometrical measures. Using these results, we are able to corroborate several conjectures regarding the properties of three-dimensional Poisson-Voronoi networks and refute others. In many cases, we provide accurate fits to these data to aid further analysis. We also demonstrate that topological measures represent powerful tools for describing cellular networks and for distinguishing among different types of networks. C1 [Lazar, Emanuel A.] Columbia Univ, New York, NY 10027 USA. [Mason, Jeremy K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Mason, Jeremy K.] Bogazici Univ, TR-34342 Istanbul, Turkey. [MacPherson, Robert D.] Inst Adv Study, Sch Math, Princeton, NJ 08540 USA. [Lazar, Emanuel A.; Srolovitz, David J.] Univ Penn, Philadelphia, PA 19104 USA. RP Lazar, EA (reprint author), Columbia Univ, New York, NY 10027 USA. RI Mason, Jeremy/P-8188-2014; Mason, Jeremy/P-9567-2015 OI Mason, Jeremy/0000-0002-0425-9816; Mason, Jeremy/0000-0002-0425-9816 NR 72 TC 11 Z9 11 U1 5 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD DEC 20 PY 2013 VL 88 IS 6 AR 063309 DI 10.1103/PhysRevE.88.063309 PG 14 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 275SQ UT WOS:000328698200004 PM 24483586 ER PT J AU Huang, XJ Yan, HF Nazaretski, E Conley, R Bouet, N Zhou, J Lauer, K Li, L Eom, D Legnini, D Harder, R Robinson, IK Chu, YS AF Huang, Xiaojing Yan, Hanfei Nazaretski, Evgeny Conley, Raymond Bouet, Nathalie Zhou, Juan Lauer, Kenneth Li, Li Eom, Daejin Legnini, Daniel Harder, Ross Robinson, Ian K. Chu, Yong S. TI 11 nm hard X-ray focus from a large-aperture multilayer Laue lens SO SCIENTIFIC REPORTS LA English DT Article ID K-B MIRRORS; ZONE-PLATE; MICROSCOPY; RETRIEVAL; BEAM AB The focusing performance of a multilayer Laue lens (MLL) with 43.4 mm aperture, 4 mu m finest zone width and 4.2 mm focal length at 12 keV was characterized with X-rays using ptychography method. The reconstructed probe shows a full-width-at-half-maximum (FWHM) peak size of 11.2 nm. The obtained X-ray wavefront shows excellent agreement with the dynamical calculations, exhibiting aberrations less than 0.3 wave period, which ensures the MLL capable of producing a diffraction-limited focus while offering a sufficient working distance. This achievement opens up opportunities of incorporating a variety of in-situ experiments into ultra high-resolution X-ray microscopy studies. C1 [Huang, Xiaojing; Yan, Hanfei; Nazaretski, Evgeny; Conley, Raymond; Bouet, Nathalie; Zhou, Juan; Lauer, Kenneth; Li, Li; Eom, Daejin; Chu, Yong S.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Conley, Raymond; Legnini, Daniel; Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Robinson, Ian K.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Robinson, Ian K.] Res Complex Harwell, Didcot OX11 0DE, Oxon, England. RP Chu, YS (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM ychu@bnl.gov RI Huang, Xiaojing/K-3075-2012; Yan, Hanfei/F-7993-2011; OI Huang, Xiaojing/0000-0001-6034-5893; Yan, Hanfei/0000-0001-6824-0367; Bouet, Nathalie/0000-0002-5816-9429 FU Department of Energy, Office of Basic Energy Sciences [DE-AC-02-98CH10886]; ERC [227711]; US National Science Foundation [DMR-9724294]; US Department of Energy, Office of Basic Energy Sciences [DE-AC0206CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors acknowledge B. Mullany (BNL) for help with 3D modeling of the microscope and D. Kuhne (BNL) for machining/assembling of mechanical parts. We thank C. Kewish for fruitful discussion at the early stage of this project. Work at Brookhaven was supported by the Department of Energy, Office of Basic Energy Sciences under contract DE-AC-02-98CH10886. I.K.R. is supported by the ERC "nanosculpture'' advanced grant 227711. The measurements were carried out at APS beamline 34-ID-C, built with US National Science Foundation grant DMR-9724294 and operated by the US Department of Energy, Office of Basic Energy Sciences, under contract no. DE-AC0206CH11357. The MLL post-growth processing was performed in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 29 TC 32 Z9 32 U1 3 U2 31 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD DEC 20 PY 2013 VL 3 AR 3562 DI 10.1038/srep03562 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 275SH UT WOS:000328697300003 PM 24356395 ER PT J AU McLaughlin, BM Ballance, CP Bowen, KP Gardenghi, DJ Stolte, WC AF McLaughlin, B. M. Ballance, C. P. Bowen, K. P. Gardenghi, D. J. Stolte, W. C. TI HIGH PRECISION K-SHELL PHOTOABSORPTION CROSS SECTIONS FOR ATOMIC OXYGEN: EXPERIMENT AND THEORY (vol 771 pg L8, 2013) SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Correction C1 [McLaughlin, B. M.] Queens Univ Belfast, Sch Math & Phys, CTAMOP, Belfast BT7 1NN, Antrim, North Ireland. [McLaughlin, B. M.] Harvard Smithsonian Ctr Astrophys, ITAMP, Cambridge, MA 02138 USA. [Ballance, C. P.] Auburn Univ, Allison Lab 206, Dept Phys, Auburn, AL 36849 USA. [Bowen, K. P.; Gardenghi, D. J.; Stolte, W. C.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Stolte, W. C.] Univ Nevada, Harry Reid Ctr Environm Studies, Las Vegas, NV 89154 USA. [Stolte, W. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP McLaughlin, BM (reprint author), Queens Univ Belfast, Sch Math & Phys, CTAMOP, Belfast BT7 1NN, Antrim, North Ireland. EM b.mclaughlin@qub.ac.uk; ballance@physics.auburn.edu; bowenk4@gmail.com; dgardenghi@gmail.com; wcstolte@lbl.gov NR 4 TC 3 Z9 3 U1 0 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD DEC 20 PY 2013 VL 779 IS 2 AR L31 DI 10.1088/2041-8205/779/2/L31 PG 3 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 269RZ UT WOS:000328260900017 ER PT J AU Gussev, MN Busby, JT Byun, TS Parish, CM AF Gussev, M. N. Busby, J. T. Byun, T. S. Parish, C. M. TI Twinning and martensitic transformations in nickel-enriched 304 austenitic steel during tensile and indentation deformations SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Austenitic metastable steel; Twinning; Martensitic transformation; Grain orientation influence; EBSD ID STAINLESS-STEELS; VARIANT SELECTION; STRAIN-RATE; PLASTIC-DEFORMATION; GRAIN-ORIENTATION; 304-STAINLESS-STEEL; MICROSTRUCTURE; DEPENDENCE; NITROGEN; BEHAVIOR AB Twinning and martensitic transformation have been investigated in nickel-enriched AISI 304 stainless steel subjected to tensile and indentation deformation. Using electron backscatter diffraction (EBSD), the morphology of alpha- and epsilon-martensite and the effect of grain orientation to load axis on phase and structure transformations were analyzed in detail. It was found that the twinning occurred less frequently under indentation than under tension; also, twinning was not observed in [001] and [101] grains. In tensile tests, the martensite particles preferably formed at the deformation twins, intersections between twins, or at the twin-grain boundary intersections. Conversely, martensite formation in the indentation tests was not closely associated with twinning; instead, the majority of martensite was concentrated in the dense colonies near grain boundaries. Martensitic transformation seemed to be obstructed in the [001] grains in both tensile and indentation test cases. Under a tensile stress of 800 MPa, both alpha- and epsilon-martensites were found in the microstructure, but at 1100 MPa only alpha-martensite presented in the specimen. Under indentation, alpha- and epsilon-martensite were observed in the material regardless of the stress level. (C) 2013 Elsevier B.V. All rights reserved. C1 [Gussev, M. N.; Busby, J. T.; Byun, T. S.; Parish, C. M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Gussev, MN (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd,POB 2008,MS-6151, Oak Ridge, TN 37831 USA. EM gussevmn@ornl.gov RI Parish, Chad/J-8381-2013 FU U.S. Department of Energy, Office of Nuclear Energy; Scientific User Facilities Division, Office of Basic Energy Sciences; U.S. Department of Energy FX This research was sponsored by the U.S. Department of Energy, Office of Nuclear Energy, for the Light Water Reactor Sustainability Research and Development Effort, and the SHaRE User Facility, sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, and the U.S. Department of Energy. Authors also would like to thank Dr. L Tan (Oak Ridge National Laboratory) for the fruitful discussion of the EBSD results. NR 40 TC 9 Z9 9 U1 3 U2 50 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD DEC 20 PY 2013 VL 588 BP 299 EP 307 DI 10.1016/j.msea.2013.08.072 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 268NF UT WOS:000328176900038 ER PT J AU Blaizot, JP Liao, JF McLerran, L AF Blaizot, Jean-Paul Liao, Jinfeng McLerran, Larry TI Gluon transport equation in the small angle approximation and the onset of Bose-Einstein condensation SO NUCLEAR PHYSICS A LA English DT Article DE Quark-gluon plasma; Glasma; Thermalization; Bose-Einstein condensation ID THERMALIZATION AB In this paper, we study the evolution of a dense system of gluons, such as those produced in the early stages of ultra-relativistic heavy ion collisions. We describe the approach to thermal equilibrium using the small angle approximation for gluon scattering in a Boltzmann equation that includes the effects of Bose statistics. In the present study we ignore the effect of the longitudinal expansion, i.e., we restrict ourselves to spatially uniform systems, with spherically symmetric momentum distributions. Furthermore we take into account only elastic scattering, i.e., we neglect inelastic, number changing, processes. We solve the transport equation for various initial conditions that correspond to small or large initial gluon phase-space densities. For a small initial phase-space density, the system evolves towards thermal equilibrium, as expected. For a large enough initial phase-space density the equilibrium state contains a Bose condensate. We present numerical evidence that such over-populated systems reach the onset of Bose-Einstein condensation in a finite time. The approach to condensation is characterized by a scaling behavior that we briefly analyze. (C) 2013 Elsevier B.V. All rights reserved. C1 [Blaizot, Jean-Paul] CEA Saclay, Inst Phys Theor, CNRS, URA 2306, F-91191 Gif Sur Yvette, France. [Liao, Jinfeng] Indiana Univ, Dept Phys, Bloomington, IN 47408 USA. [Liao, Jinfeng] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47408 USA. [Liao, Jinfeng; McLerran, Larry] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [McLerran, Larry] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [McLerran, Larry] Cent China Normal Univ, Dept Phys, Wuhan, Peoples R China. RP Liao, JF (reprint author), Indiana Univ, Dept Phys, 2401 N Milo B Sampson Lane, Bloomington, IN 47408 USA. FU DOE [DE-AC02-98CH10886]; RIKEN BNL Research Center; European Research Council under the Advanced Investigator Grant [ERC-AD-267258] FX The research of L.M. and J.L. is supported under DOE Contract No. DE-AC02-98CH10886. J.L. is also grateful to the RIKEN BNL Research Center for partial support. The research of J.P.B. is supported by the European Research Council under the Advanced Investigator Grant ERC-AD-267258. NR 15 TC 38 Z9 38 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9474 EI 1873-1554 J9 NUCL PHYS A JI Nucl. Phys. A PD DEC 20 PY 2013 VL 920 BP 58 EP 77 DI 10.1016/j.nuclphysa.2013.10.010 PG 20 WC Physics, Nuclear SC Physics GA 266DN UT WOS:000328002900005 ER PT J AU Kendall, B Brennecka, GA Weyer, S Anbar, AD AF Kendall, Brian Brennecka, Gregory A. Weyer, Stefan Anbar, Ariel D. TI Uranium isotope fractionation suggests oxidative uranium mobilization at 2.50 Ga SO CHEMICAL GEOLOGY LA English DT Article DE Mt. McRae Shale; Hamersley basin; Uranium isotopes; Uranium geochemical cycle; Earth surface oxygenation; Archean ID BLACK-SEA SEDIMENTS; BILLION YEARS AGO; WESTERN-AUSTRALIA; CONTINENTAL-CRUST; NITROGEN-CYCLE; OXIDE MINERALS; ARCHEAN OCEAN; REACTIVE IRON; OXYGENATION; EVENT AB Geochemical data from late Archean sedimentary rocks point to photosynthetic O-2 production and at least intermittent occurrences of locally mild oxidative weathering and surface ocean oxygenation ("oxygen oases") prior to the early Paleoproterozoic Great Oxidation Event. For example, distinctive authigenic enrichments of Mo and Re in euxinic (anoxic and sulfidic) black shales are best explained by the oxidative mobilization of these metals from crustal sulfide minerals and their accumulation as oxyanions in seawater. In contrast, it is not clear if low U enrichments in the same shales reflect negligible oxidation of U from the upper crust or a very small oceanic U inventory that was derived from oxidative U mobilization. Here, we report U isotope data for the 2.50 Ga Mt. McRae Shale (Hamersley basin, Western Australia), which provides a more sensitive test for the presence or absence of authigenic U compared to U concentrations and enrichment factors normalized to average shale or upper crustal compositions (that may not be representative of the local detrital composition). We find instances where the U isotope composition in the upper Mt. McRae Shale (delta U-238 = -0.2 to 0.0 parts per thousand relative to standard SRM950a) is isotopically heavier than average upper crust (delta U-238 = -0.31 +/- 0.14 [2SD] based on granitoids and basalts). The high delta U-238 values point to U isotope fractionation in the late Archean marine environment and hence indicate the presence of a small amount of dissolved U in seawater and authigenic U in the Mt. McRae Shale. Volume-dependent equilibrium isotope fractionation during the reduction of dissolved UVI to insoluble U-IV, like that observed in the modern Black Sea, may explain the high delta U-238 signatures if U removal from bottom waters was not quantitative. Alternatively, quantitative U removal would require that late Archean seawater had high delta U-238, which could have arisen from the preferential sequestration of U-235 to Fe (oxyhydr) oxide minerals elsewhere in the Hamersley basin. The supracrustal delta U-238 signatures are associated with some of the highest Mo and Re enrichments in the Mt. McRae Shale as well as distinctive Mo, S and N isotope signatures that are indicative of mild environmental oxygenation. Hence, our findings suggest that small amounts of U were oxidatively mobilized from the upper crust at 2.50 Ga. Unlike Mo and Re, however, U oxidation may not have occurred on land. Instead, we hypothesize that oxidative U mobilization occurred by submarine weathering in an oxygen oasis. (C) 2013 Elsevier B. V. All rights reserved. C1 [Kendall, Brian] Univ Waterloo, Dept Earth & Environm Sci, Waterloo, ON N2L 3G1, Canada. [Kendall, Brian; Brennecka, Gregory A.; Anbar, Ariel D.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Brennecka, Gregory A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Weyer, Stefan] Leibniz Univ Hannover, Inst Mineral, D-30167 Hannover, Germany. [Anbar, Ariel D.] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. RP Kendall, B (reprint author), Univ Waterloo, Dept Earth & Environm Sci, 200 Univ Ave West, Waterloo, ON N2L 3G1, Canada. EM bkendall@uwaterloo.ca FU National Science Foundation; Agouron Institute; NASA Astrobiology Institute FX This research was financially supported by the National Science Foundation, the Agouron Institute, and the NASA Astrobiology Institute. Dr. Gwyneth Gordon, Carina Arrua, and Christy Meza are thanked for analytical support and sample preparation. Constructive comments and suggestions from three anonymous reviewers improved the manuscript. NR 70 TC 28 Z9 28 U1 5 U2 44 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD DEC 20 PY 2013 VL 362 SI SI BP 105 EP 114 DI 10.1016/j.chemgeo.2013.08.010 PG 10 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 262UV UT WOS:000327764300012 ER PT J AU Moradi, CP Morrison, AM Klippenstein, SJ Goldsmith, CF Douberly, GE AF Moradi, Christopher P. Morrison, Alexander M. Klippenstein, Stephen J. Goldsmith, C. Franklin Douberly, Gary E. TI Propargyl + O-2 Reaction in Helium Droplets: Entrance Channel Barrier or Not? SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID AROMATIC-HYDROCARBON FORMATION; RESONANCE-STABILIZED RADICALS; SUPERFLUID-HELIUM DROPLETS; 193 NM PHOTOLYSIS; LIQUID-HELIUM; INFRARED-SPECTROSCOPY; HE-4 CLUSTERS; PERTURBATION-THEORY; SELF-REACTION; NANODROPLETS AB A combination of liquid He droplet experiments and multi-reference electronic structure calculations is used to probe the potential energy surface for the reaction between the propargyl radical and O-2. Infrared laser spectroscopy is used to probe the outcome of the low temperature, liquid Hemediated reaction; Bands in the spectrum are assigned to the acetylenic CH stretch (nu(1)), the symmetric CH2 stretch (nu(1)), and the antisymmetric CH2 stretch (nu(13)) of the trans-acetylenic propargyl peroxy radical ((OO)-O-center dot-CH2-C CH). The observed band origins are in excellent agreement with previously reported anharmonic frequency computations for this species [Jochnowitz, E. B.; Zhang, X.; Nimlos, M. R.; Flowers, B. A.; Stanton, J. F.; Ellison, G. B. J. Phys. Chem. A 2010, 114, 1498]. The Stark spectrum of the ut band provides further evidence that the reaction leads only to the trans-acetylenic species. There are no other bands in the CH2 stretching region that can be attributed to any of the other three propargyl peroxy isomers/conformers that are predicted to be minimum energy structures (gauche-acetylenic, cis-allenic, and trans-allenic). There is also no evidence for the kinetic stabilization of a van der Waals complex between propargyl and O-2. A combination of multireference and coupled-cluster electronic structure calculations is used to probe the potential energy surface in the neighborhood of the transition state connecting reactants with the acetylenic adduct. The multireference based evaluation of the doublet-quartet splitting added to the coupled-cluster calculated quartet state energies yields what are likely the most accurate predictions for the doublet potential curve. This calculation suggests that there is no saddle point for the addition process, in agreement with the experimental observations. Other calculations suggest the possible presence of a small submerged barrier. C1 [Moradi, Christopher P.; Morrison, Alexander M.; Douberly, Gary E.] Univ Georgia, Dept Chem, Athens, GA 30602 USA. [Klippenstein, Stephen J.; Goldsmith, C. Franklin] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Douberly, GE (reprint author), Univ Georgia, Dept Chem, Athens, GA 30602 USA. EM douberly@uga.edu OI Klippenstein, Stephen/0000-0001-6297-9187 FU Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy (DOE) [DE-FG02-12ER16298]; American Chemical Society Petroleum Research Fund [50223-DNI6]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357]; Argonne Director's Postdoctoral Fellowship FX G.E.D. acknowledges support from the Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy (DOE) under Contract No. DE-FG02-12ER16298. G.E.D. acknowledges partial support from the donors of the American Chemical Society Petroleum Research Fund (50223-DNI6). The work at Argonne was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Contract No. DE-AC02-06CH11357. C.F.G. acknowledges support from the Argonne Director's Postdoctoral Fellowship. NR 60 TC 9 Z9 9 U1 3 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD DEC 19 PY 2013 VL 117 IS 50 BP 13626 EP 13635 DI 10.1021/jp407652f PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 278WI UT WOS:000328920200047 PM 24015722 ER PT J AU Cich, MJ Forthomme, D McRaven, CP Lopez, GV Hall, GE Sears, TJ Mantz, AW AF Cich, Matthew J. Forthomme, Damien McRaven, Christopher P. Lopez, Gary V. Hall, Gregory E. Sears, Trevor J. Mantz, Arlan. W. TI Temperature-Dependent, Nitrogen-Perturbed Line Shape Measurements in the nu(1) + nu(3) Band of Acetylene Using a Diode Laser Referenced to a Frequency Comb SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID 1.5 MU-M; LINESHAPE MODELS; SPECTRAL-LINES; ACETYLENE TRANSITIONS; SHIFT COEFFICIENTS; FREQUENCY ATLAS; 1550 NM; BAND; AR; REGION AB The P(11) line of the nu(1) + nu(3) combination band of C2H2 was studied using an extended cavity diode laser locked to a frequency comb. Line shapes were measured for acetylene and nitrogen gas mixtures at a series of temperatures between 125 and 296 K and total pressures up to 1 atm. The data were fit to two speed-dependent line shape models and the results were compared. Line shape parameters were determined by simultaneously fitting data for all temperatures and pressures in a single multispectrum analysis. Earlier pure acetylene measurements [Cich et al. Appl. Phys. B 2012, 109, 373-38] were incorporated to account for self-perturbation. The resulting parameters reproduce the observed line shapes for the acetylene-nitrogen system over the range of temperatures and pressures studied with average root-mean-square observed-calculated errors of individual line measurement fits of approximately 0.01% of maximum transmission, close to the experimental signal-to-noise ratios. Errors in the pressure measurements constitute the major systematic errors in these measurements, and a statistical method is developed to quantify their effects on the line shape parameters for the present system. C1 [Cich, Matthew J.; Lopez, Gary V.; Sears, Trevor J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Forthomme, Damien; McRaven, Christopher P.; Hall, Gregory E.; Sears, Trevor J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Mantz, Arlan. W.] Connecticut Coll, Dept Phys Astron & Geophys, New London, CT 06320 USA. RP Sears, TJ (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM Sears@bnl.gov RI Sears, Trevor/B-5990-2013; Hall, Gregory/D-4883-2013 OI Sears, Trevor/0000-0002-5559-0154; Hall, Gregory/0000-0002-8534-9783 FU American Chemical Society; Brookhaven National Laboratory; NASA EPSCoR [PS 4990]; U.S. Department of Energy, Office of Science [DE-AC02-98CH10886]; Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences FX Acknowledgement is made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this research. We are grateful for Program Development Funding awarded to T.J.S. by Brookhaven National Laboratory, which provided funds for some of the equipment used in this work. A.W.M. gratefully acknowledges support by NASA EPSCoR Grant No. PS 4990 for supporting the development of low temperature cells. Work at Brookhaven National Laboratory was carried out under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences. NR 63 TC 5 Z9 5 U1 1 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD DEC 19 PY 2013 VL 117 IS 50 BP 13908 EP 13918 DI 10.1021/jp408960e PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 278WI UT WOS:000328920200077 PM 24125088 ER PT J AU Kim, H Sakaki, K Ogawa, H Nakamura, Y Nakamura, J Akiba, E Machida, A Watanuki, T Proffen, T AF Kim, Hyunjeong Sakaki, Kouji Ogawa, Hiroshi Nakamura, Yumiko Nakamura, Jin Akiba, Etsuo Machida, Akihiko Watanuki, Tetsu Proffen, Thomas TI Origin of Degradation in the Reversible Hydrogen Storage Capacity of V1-xTix Alloys from the Atomic Pair Distribution Function Analysis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY-DIFFRACTION; POWDER DIFFRACTION; MG50CO50; METALS; LANI5 AB Reduction in reversible hydrogen storage capacity with increasing hydrogenation and dehydrogenation cycle number is observed in numerous hydrogen storage materials, but the mechanism behind this unfavorable change has not been elucidated yet. In this study, we have investigated the development of structural defects or disorders in V1-xTixH2, x = 0, 0.2, and 0.5, during the first 15 hydrogen absorption and desorption cycles using the atomic pair distribution function (PDF) analysis of synchrotron X-ray total scattering data to find out the possible structural origin of the poor cyclic stability of V1-xTix alloys. While pure vanadium shows no significant change in the PDF, alloy samples subject to several hydrogenation and dehydrogenation cycles display fast decaying of the PDF profile due to a progressive increase in the PDF peak width with increasing r. This r-dependent PDF peak broadening effect becomes stronger with cycle number. Molecular dynamics (MD) simulations demonstrated that dislocation defects explain characteristic features in our experimental PDFs very well and suggested that a large number of dislocations are formed during hydrogen cycling. We found there is a close relation between the reduced amount of the reversible hydrogen content of V0.8Ti0.2 and the amount of generated dislocations. On the basis of the PDF analysis results, a possible mechanism behind degradation in the reversible hydrogen storage capacity of V1-xTix is discussed. C1 [Kim, Hyunjeong; Sakaki, Kouji; Ogawa, Hiroshi; Nakamura, Yumiko] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058565, Japan. [Nakamura, Jin] Japan Met & Chem Co Ltd, Yamagata 9991351, Japan. [Akiba, Etsuo] Kyushu Univ, Int Inst Carbon Neutral Energy Res, Nishi Ku, Fukuoka 8190395, Japan. [Machida, Akihiko; Watanuki, Tetsu] Japan Atom Energy Agcy, Sayo, Hyogo 6795148, Japan. [Proffen, Thomas] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Kim, H (reprint author), Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058565, Japan. EM hj.kim@aist.go.jp RI Proffen, Thomas/B-3585-2009; U-ID, Kyushu/C-5291-2016 OI Proffen, Thomas/0000-0002-1408-6031; FU New Energy and Industrial Technology Development Organization (NEDO) under the Advanced Fundamental Research Project on Hydrogen Storage Materials (HYDRO-STAR) FX H.K. thanks Nobuhiko Takeichi and Itoko Matsumoto for help with experiments. This work was partly supported by the New Energy and Industrial Technology Development Organization (NEDO) under the Advanced Fundamental Research Project on Hydrogen Storage Materials (HYDRO-STAR). The synchrotron X-ray experiments were performed under the Shared Use Program of JAEA Facilities (Proposal No.2011B-E09) at JAEA beamline BL22XU in SPring-8 (Proposal No.2011A3703 and 2011B3784). NR 28 TC 8 Z9 8 U1 5 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26543 EP 26550 DI 10.1021/jp408766r PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500016 ER PT J AU Yu, TH Hofmann, T Sha, Y Merinov, BV Myers, DJ Heske, C Goddard, WA AF Yu, Ted H. Hofmann, Timo Sha, Yao Merinov, Boris V. Myers, Deborah J. Heske, Clemens Goddard, William A., III TI Finding Correlations of the Oxygen Reduction Reaction Activity of Transition Metal Catalysts with Parameters Obtained from Quantum Mechanics SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PLATINUM-MONOLAYER ELECTROCATALYSTS; SURFACE ELECTRONIC-STRUCTURE; FUEL-CELL CATHODE; ALLOY SURFACES; NOBLE-METALS; TRENDS; APPROXIMATION; SPECTROSCOPY; ADSORPTION; STABILITY AB To facilitate a less empirical approach to developing improved catalysts, it is important to correlate catalytic performance to surrogate properties that can be measured or predicted accurately and quickly, allowing experimental synthesis and testing of catalysts to focus on the most promising cases. Particularly hopeful is correlating catalysis performance to the electronic density of states (DOS). Indeed, there has been success in using just the center of the d-electron density, which in some cases correlates linearly with oxygen atom chemisorption energy, leading to a volcano plot for catalytic performance versus "d-band center". To test such concepts we calculated the barriers and binding energies for the various reactions and intermediates involved in the oxygen reduction reaction (ORR) for all 12 transition metals in groups 8-11 (Fe-Cu columns). Our results show that the oxygen binding energy can serve as a useful parameter in describing the catalytic activity for pure metals, but it does not necessarily correlate with the d-band center. In addition, we find that the d-band center depends substantially on the calculation method or the experimental setup, making it a much less reliable indicator for ORR activity than the oxygen binding energy. We further examine several surfaces of the same pure metals to evaluate how the d-band center and oxygen binding energy depend on the surface. C1 [Yu, Ted H.; Sha, Yao; Merinov, Boris V.; Goddard, William A., III] CALTECH, Mat & Proc Simulat Ctr, Pasadena, CA 91125 USA. [Yu, Ted H.] Calif State Univ Long Beach, Dept Chem Engn, Long Beach, CA 90840 USA. [Hofmann, Timo; Heske, Clemens] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Hofmann, Timo] Bundeswehr Res Inst Mat Fuels & Lubricants, D-85435 Erding, Germany. [Myers, Deborah J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Heske, Clemens] Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat IPS, D-76344 Eggenstein Leopoldshafen, Germany. [Heske, Clemens] Karlsruhe Inst Technol, ANKA Synchrotron Radiat Facil, D-76344 Eggenstein Leopoldshafen, Germany. [Heske, Clemens] Karlsruhe Inst Technol, Inst Chem Technol & Polymer Chem, D-76128 Karlsruhe, Germany. RP Merinov, BV (reprint author), CALTECH, Mat & Proc Simulat Ctr, M-C 139-74,1200 East Calif Blvd, Pasadena, CA 91125 USA. EM merinov@wag.caltech.edu; wag@wag.caltech.edu FU U.S. Department of Energy [DE-AC02-06CH11357]; ANL [7F-01041, 7F-01321]; National Science Foundation [CBET-1067848]; DURIP-ONR; DURIP-ARO; NSF-CSEM FX We gratefully acknowledge funding by the U.S. Department of Energy, Prime Contract No. DE-AC02-06CH11357 (ANL) and ANL Subcontract Nos. 7F-01041 (UNLV) and 7F-01321 (Caltech), and National Science Foundation (Grant CBET-1067848, Caltech). The facilities of the Materials and Process Simulation Center used in this study were established with grants from DURIP-ONR, DURIP-ARO, and NSF-CSEM. NR 43 TC 32 Z9 32 U1 4 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26598 EP 26607 DI 10.1021/jp4071554 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500022 ER PT J AU Alayoglu, S An, KJ Melaet, G Chen, SY Bernardi, F Wang, LW Lindeman, AE Musselwhite, N Guo, JH Liu, Z Marcus, MA Somorjai, GA AF Alayoglu, Selim An, Kwangjin Melaet, Gerome Chen, Shiyou Bernardi, Fabiano Wang, Lin Wang Lindeman, Avery E. Musselwhite, Nathan Guo, Jinghua Liu, Zhi Marcus, Matthew A. Somorjai, Gabor A. TI Pt-Mediated Reversible Reduction and Expansion of CeO2 in Pt Nanoparticle/Mesoporous CeO2 Catalyst: In Situ X-ray Spectroscopy and Diffraction Studies under Redox (H-2 and O-2) Atmospheres SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID WATER-GAS-SHIFT; OXIDE ELECTROCHEMICAL-CELLS; CERIA-SUPPORTED CATALYSTS; PREFERENTIAL CO OXIDATION; HYDROGEN PROX; PHOTOELECTRON-SPECTROSCOPY; REACTION-MECHANISM; MESOPOROUS SILICA; DOPED CERIA; FUEL-CELLS AB Here, we report the Pt nanoparticle mediated reduction (oxidation) and lattice expansion (contraction) of mesoporous CeO2 under H-2 (O-2) atmospheres and in the temperature range of 50-350 degrees C. We found that CeO2 in the Pt/CeO2 catalyst was partially reduced in H-2 (and fully oxidized back in O-2) as demonstrated by several in situ techniques: APXPS spectra (4d core levels) for the topmost surface, NEXAFS total electron yield spectra (at the M-5,M-4 edges) in the near surface regions, and (N)EXAFS fluorescence spectra (at the L-3 edge) in the bulk. Moreover, XRD and EXAFS showed the reversible expansion and contraction of the CeO2 unit cell in H-2 and O-2 environments, respectively. The expansion of the CeO2 cell was mainly associated with the formation of oxygen vacancies as a result of the Pt-mediated reduction of Ce4+ to Ce3+. We also found that pure mesoporous CeO2 can not be reduced in H-2 under identical conditions but can be partially reduced at above 450 degrees C as revealed by APXPS. The-role of Pt in H-2 was identified as a catalytic one that reduces the activation barrier for the reduction of CeO2 via hydrogen spillover. C1 [Alayoglu, Selim; An, Kwangjin; Melaet, Gerome; Lindeman, Avery E.; Musselwhite, Nathan; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94704 USA. [Alayoglu, Selim; An, Kwangjin; Melaet, Gerome; Lindeman, Avery E.; Musselwhite, Nathan; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Chen, Shiyou; Wang, Lin Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Guo, Jinghua; Liu, Zhi; Marcus, Matthew A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Bernardi, Fabiano] Univ Fed Rio Grande do Sul, Inst Fis, Dept Fis, BR-90040060 Porto Alegre, RS, Brazil. RP Alayoglu, S (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94704 USA. RI Bernardi, Fabiano/G-2450-2012; Liu, Zhi/B-3642-2009; Melaet, Gerome/N-4879-2015; Foundry, Molecular/G-9968-2014 OI Liu, Zhi/0000-0002-8973-6561; Melaet, Gerome/0000-0003-1414-1683; FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Energy Research, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; JCAP, a DOE Energy Innovation Hub [DE-SC0004993]; CNPq-Brazil FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The user projects in the Advanced Light Source and Molecular Foundry at the Lawrence Berkeley National Laboratory were supported by the Director, Office of Energy Research, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract DE-AC02-05CH11231. The work (theoretical calculation) is supported by JCAP, a DOE Energy Innovation Hub, under Award No. DE-SC0004993. F.B. received a research grant from CNPq-Brazil. The authors would like to thank Doctors Simon Clark, Jason Knight, Bora Kalkan, and Alastair Macdowell at beamline 12.2.2 in the Advanced Light Source for technical support, Dr. Fan Zheng for the design of EXAFS cell, and Eric Granlund for the construction of EXAFS and XRD cells. NR 42 TC 20 Z9 20 U1 8 U2 91 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26608 EP 26616 DI 10.1021/jp407280e PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500023 ER PT J AU Mebane, DS Kress, JD Storlie, CB Fauth, DJ Gray, ML Li, KJ AF Mebane, David S. Kress, Joel D. Storlie, Curtis B. Fauth, Daniel J. Gray, McMahan L. Li, Kuijun TI Transport, Zwitterions, and the Role of Water for CO2 Adsorption in Mesoporous Silica-Supported Amine Sorbents SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CARBON-DIOXIDE CAPTURE; SENSITIVITY-ANALYSIS; CARBAMATE FORMATION; MOLECULAR-SIEVE; HIGH-CAPACITY; AB-INITIO; SOL-GEL; KINETICS; MODEL; ALKANOLAMINES AB The uptake of CO2 in highly loaded, silica-supported, polyethylenimine (PEI)-impregnated sorbents was investigated in a reaction-diffusion model of the CO2 adsorption process. The model successfully replicated the pseudoequilibrium behavior experimentally observed in thermogravimetry (TGA) experiments. A parametric study and sensitivity analysis of the model revealed that the stability and mobility of diffusive intermediates-assumed in the model to be zwitterions-effectively control the observable capacity of the sorbent. A subsequent quantum chemical study called into question the stability of zwitterions in PEI but suggested that physically bonded moieties involving water, amines, and CO2 may be better candidates for diffusive intermediates. The implications are a strong dependence of the observable CO2 capacity of the sorbent on the presence of water in the gas stream, which was found to be consistent with TGA results. C1 [Mebane, David S.; Fauth, Daniel J.; Gray, McMahan L.] Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Mebane, David S.; Fauth, Daniel J.; Gray, McMahan L.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Mebane, David S.; Li, Kuijun] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [Kress, Joel D.; Storlie, Curtis B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Mebane, DS (reprint author), Natl Energy Technol Lab, Morgantown, WV 26507 USA. EM david.mebane@mail.wvu.edu FU ORISE postdoctoral fellowship; Department of Energy through the Carbon Capture Simulation Initiative; agency of the United States Government FX Help and support from David C. Miller and Leslie M. Moore is gratefully acknowledged. Partial support for David Mebane was provided by an ORISE postdoctoral fellowship. Funding for this work was provided by the Department of Energy through the Carbon Capture Simulation Initiative.; This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 59 TC 21 Z9 21 U1 4 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26617 EP 26627 DI 10.1021/jp4076417 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500024 ER PT J AU Borodko, Y Ercius, P Zherebetskyy, D Wang, YH Sun, YT Somorjai, G AF Borodko, Yuri Ercius, Peter Zherebetskyy, Danylo Wang, Yihai Sun, Yintao Somorjai, Gabor TI From Single Atoms to Nanocrystals: Photoreduction of [PtCl6](2-) in Aqueous and Tetrahydrofuran Solutions of PVP SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SPECTRA; PHOTOCHEMISTRY; NANOPARTICLES; RAMAN AB Structured platinum nanoclusters Pt-n (n = 5-30) capped by poly(N-vinylpyrrolidone) (PVP) have unique and highly attractive properties as potential selective catalysts. We show that the assembly of Pt mononuclear compounds in aqueous and tetrahydrofuran (THF) solutions under UV irradiation proceed via several steps: formation of linear Pt clusters (n = 2- 8), coalescence into mesocrystals, and transformation into Pt nanocrystals. The "quantum" size range of Pt-n (n = 5-100) clusters is intermediate between those clusters with molecular properties and those with metallic properties. The PVP "cage" acts as a nano reactor and can hinder diffusion of photoexcited Pt atoms. The diffusion of the Pt from the polymer cage is strongly affected by the hydrophobic or hydrophilic property of the solution. An aqueous solution of [PtCl6](2-) + PVP transforms into noncrystalline aggregates of molecules of less than 1.5-2 nm in diameter, whereas in THF solution Pt nanocrystals increase proportional to the UV irradiation time up to 10 nm in diameter. Dynamic imaging by high-resolution microscopy and low-frequency UV Raman spectra show the initial stages of Pt atoms assembled into Pt-n clusters. The assignment of the Raman bands is supported by density functional theory calculations. The proposed scheme of photoinduced reactions suggests the coupling of coordinatively unsaturated Pt ions inside the amidate-rich polymeric stabilizer. C1 [Borodko, Yuri; Zherebetskyy, Danylo; Somorjai, Gabor] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Wang, Yihai; Sun, Yintao; Somorjai, Gabor] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ercius, Peter] Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Somorjai, G (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu RI Zherebetskyy, Danylo/B-3404-2015; Foundry, Molecular/G-9968-2014 FU Office of Science, Office of Basic Energy Sciences, Material and Engineering Divisions of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy; National Natural Science Foundation of China; Chinese University of Hong Kong FX This work is supported by the Director, Office of Science, Office of Basic Energy Sciences, Material and Engineering Divisions of the U.S. Department of Energy under Contract DE-AC02-05CH11231. The National Center for Electron Microscopy at Lawrence Berkeley National Laboratory is supported by the U.S. Department of Energy under Contract DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center (NERSC) supported by the Office of Science of the U.S. Department of Energy. Y.W. appreciates support from the Basic Research Program of Young Scientists by the National Natural Science Foundation of China and Chinese University of Hong Kong. NR 23 TC 10 Z9 10 U1 12 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26667 EP 26674 DI 10.1021/jp409960p PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500030 ER PT J AU Robinson, AM Montemore, MM Tenney, SA Sutter, P Medlin, JW AF Robinson, Allison M. Montemore, Matthew M. Tenney, Samuel A. Sutter, Peter Medlin, J. Will TI Interactions of Hydrogen, CO, Oxygen, and Water with Molybdenum-Modified Pt(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DENSITY-FUNCTIONAL THEORY; AUGMENTED-WAVE METHOD; RHENIUM CATALYSTS; ETHYLENE-GLYCOL; SURFACE ALLOYS; OXIDATION; SPECTROSCOPY; GLYCEROL; H-2; CHEMISORPTION AB Modification of Pt group catalysts by molybdenum is known to improve catalyst performance in a number of important chemical reactions. To investigate fundamental mechanisms responsible for the promoting effect of Mo, temperature-programmed desorption (TPD) and low energy electron diffraction (LEED) experiments were performed to examine the adsorption of O-2, D-2, CO, and water on Pt(111) modified with submonolayer quantities of molybdenum. Auger electron spectroscopy (AES) was used to detect and quantify the Mo coverage and X-ray photoelectron spectroscopy (XPS) was employed in conjunction with density functional theory (DFT) calculations to identify Mo species present following various surface treatments. The state of Mo on the surface was found to vary depending on prior surface treatment. Treatment with oxygen resulted in a surface molybdenum oxide, whereas treatment with hydrogen resulted in a reduced bimetallic surface. XPS results indicate that high pressures of oxygen create a higher valent oxide than what is created under ultrahigh vacuum. Oxidized Mo appeared to block Pt surface sites without significantly altering the behavior of species adsorbed on Pt. Reduced surfaces, on the other hand, were shown to decrease yield and desorption temperature for both D-2 and CO. Isotopic TPD studies provided evidence of water dissociation on the reduced Mo modified surface, with a maximum extent of water dissociation occurring at intermediate Mo coverages. C1 [Robinson, Allison M.; Medlin, J. Will] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80309 USA. [Montemore, Matthew M.] Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA. [Tenney, Samuel A.; Sutter, Peter] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Medlin, JW (reprint author), Univ Colorado, Dept Chem & Biol Engn, UCB 596, Boulder, CO 80309 USA. EM will.medlin@colorado.edu OI Montemore, Matthew/0000-0002-4157-1745 FU National Science Foundation [CHE-1149752]; Department of Education Graduate Assistantships in Areas of National Need (GAANN); National Renewable Energy Laboratory; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-AC02-06CH11357] FX The authors acknowledge support from the National Science Foundation for funding this research (Award CHE-1149752). A.M.R. also acknowledges partial support from the Department of Education Graduate Assistantships in Areas of National Need (GAANN) and from the National Renewable Energy Laboratory. Research carried out in part at the Center for Functional Nanomaterials and National Synchrotron Light Source, Brookhaven National Laboratory, which are supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We acknowledge supercomputing time at the Center for Nanoscale Materials at Argonne National Laboratory, supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 47 TC 6 Z9 6 U1 4 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26716 EP 26724 DI 10.1021/jp410563s PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500036 ER PT J AU Wagner, P Ewels, CP Adjizian, JJ Magaud, L Pochet, P Roche, S Lopez-Bezanilla, A Ivanovskaya, VV Yaya, A Rayson, M Briddon, P Humbert, B AF Wagner, Philipp Ewels, Christopher P. Adjizian, Jean-Joseph Magaud, Laurence Pochet, Pascal Roche, Stephan Lopez-Bezanilla, Alejandro Ivanovskaya, Viktoria V. Yaya, Abu Rayson, Mark Briddon, Patrick Humbert, Bernard TI Band Gap Engineering via Edge-Functionalization of Graphene Nanoribbons SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID BORON-NITRIDE NANORIBBONS; DER-WAALS RADII; ELECTRONIC-PROPERTIES; SPECTROSCOPY; RIBBONS AB Density functional calculations are used to perform a systematic study of the effect of edge-functionalization on the structure and electronic properties of graphene nanoribbons (GNRs). -H, -F, -Cl, -Br, -S, -SH, and -OH edge-functionalization of armchair, zigzag, and reconstructed Klein-type GNRs was considered. The most energetically favorable edge structure varies depending on the choice of functional group. It is shown, for the first time, that reconstructed Klein-type GNRs are important stable configurations for several edge-functional groups. Band gaps using three different exchange-correlation functionals are calculated. The band gap for armchair GNRs can be tuned over a range of similar to 1.2 eV by varying the edge-functional groups. In contrast, the band gaps of zigzag and reconstructed Klein edge GNRs are largely insensitive to the choice of edge-functional group, and ribbon width is instead the defining factor. Alternatively, the armchair GNR band gap can be controlled by varying the number of functional groups per opposing edge, altering the GNR "effective" width. Edge-functionalization design is an appropriate mechanism to tune the band gap of armchair GNRs. C1 [Wagner, Philipp; Ewels, Christopher P.; Adjizian, Jean-Joseph; Briddon, Patrick; Humbert, Bernard] Univ Nantes, CNRS UMR 6502, Inst Mat Jean Rouxel IMN, F-44322 Nantes, France. [Magaud, Laurence] CNRS UJF, Inst Neel, F-38042 Grenoble, France. [Pochet, Pascal] CEA UJF, INAC, SP2M, Lab Simulat Atomist L Sim, F-38054 Grenoble, France. [Roche, Stephan] ICN2, Barcelona 08193, Spain. [Roche, Stephan] ICREA, Barcelona 08010, Spain. [Lopez-Bezanilla, Alejandro] Argonne Natl Lab, Argonne, IL 60439 USA. [Ivanovskaya, Viktoria V.] CNRS Thales, Unite Mixte Phys, F-91767 Palaiseau, France. [Ivanovskaya, Viktoria V.] Univ Paris 11, F-91405 Orsay, France. [Yaya, Abu] Univ Ghana, Dept Mat Sci & Engn, Legon, Accra, Ghana. [Rayson, Mark] Univ Surrey, Dept Chem, Guildford GU2 7XH, Surrey, England. [Briddon, Patrick] Newcastle Univ, Sch Elect Elect & Comp Engn, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. RP Ewels, CP (reprint author), Univ Nantes, CNRS UMR 6502, Inst Mat Jean Rouxel IMN, F-44322 Nantes, France. EM chris.ewels@cnrs-imn.fr RI Pochet, Pascal/B-2380-2009; Roche, Stephan/B-1116-2012; Ivanovskaya, Viktoria/A-1073-2015; Lopez-Bezanilla, Alejandro/B-9125-2015; humbert, bernard/K-4696-2015; Ewels, Chris/A-1543-2012 OI Adjizian, Jean-Joseph/0000-0002-7899-4565; Pochet, Pascal/0000-0002-1521-973X; Roche, Stephan/0000-0003-0323-4665; Lopez-Bezanilla, Alejandro/0000-0002-4142-2360; Ewels, Chris/0000-0001-5530-9601 FU NANOSIM-GRAPHENE [ANR-09-NANO-016-01]; French National Research Agency (ANR) [P3N2009]; SPRINT [ANR-10-BLAN-0819]; Spanish Ministry of Economy and Competitiveness [MAT2012-33911]; GENCI [2013-097015]; COST [MP0901] FX P.W., C.P.E., L.M., P.P., S.R, and V.V.I. thank the NANOSIM-GRAPHENE project no. ANR-09-NANO-016-01 funded by the French National Research Agency (ANR) in the frame of its 2009 programme in Nanosciences, Nanotechnologies & Nanosystems (P3N2009). P.W., C.P.E., J.-JA., and B.H. thank the SPRINT project ANR-10-BLAN-0819. S.R. acknowledges funding support from the Spanish Ministry of Economy and Competitiveness (MAT2012-33911). We thank the CCIPL, CLUSTUS (IMN), and GENCI (Grant 2013-097015) for computing time. We thank COST project MP0901 NanoTP for support. NR 60 TC 24 Z9 24 U1 7 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26790 EP 26796 DI 10.1021/jp408695c PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500045 ER PT J AU Wheeler, DA Ling, YC Dillon, RJ Fitzmorris, RC Dudzik, CG Zavodivker, L Rajh, T Dimitrijevic, NM Millhauser, G Bardeen, C Li, Y Zhang, JZ AF Wheeler, Damon A. Ling, Yichuan Dillon, Robert J. Fitzmorris, Robert C. Dudzik, Christopher G. Zavodivker, Liat Rajh, Tijana Dimitrijevic, Nada M. Millhauser, Glenn Bardeen, Christopher Li, Yat Zhang, Jin Z. TI Probing the Nature of Bandgap States in Hydrogen-Treated TiO2 Nanowires SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID QUANTUM-DOT SENSITIZATION; TITANIUM-DIOXIDE; RUTILE TIO2; SOLAR-CELLS; PHOTOCATALYTIC ACTIVITY; VISIBLE-LIGHT; SURFACE; ENHANCEMENT; PRINCIPLES; ARRAYS AB Hydrogen treatment of TiO2 has been demonstrated to significantly alter its optical properties, including substantially enhanced visible light absorption that has important implications for various applications. The chemical nature of the bandgap states responsible for the increased visible absorption is not yet well understood. This work reports a detailed study of the structural, optical, electronic, and ultrafast properties of hydrogen-treated TiO2 (H:TiO2) nanowires (NWs) using a combination of experimental techniques including high-resolution transmission electron microscopy (HRTEM), electron spin resonance spectroscopy (ESR), time-resolved fluorescence (TRF), and femto-second transient absorption (TA) spectroscopy in order to explain the origin of the strong visible absorption. The combined TEM, ESR, TRF, and TA data suggest that the presence of a localized mid-bandgap oxygen vacancy (V-O) occupied by a lone electron in an antibonding orbital situated at a surface site is likely responsible for the visible absorption of the material. The data further indicate that while untreated TiO2 NWs are fluorescent, the hydrogen treatment leads to quenching of the fluorescence and highly efficient charge carrier recombination from the V-O state following excitation with visible light. With UV excitation, however, the charge carrier recombination of the H:TiO2 NWs exhibits a larger component of a slow decay compared to that of untreated TiO2, which is correlated with enhanced photoelectrochernical performance. Both the treated and untreated samples exhibit a fast decay that dominates the TA signals, which is likely caused by a high density of surface trap states. A simple model is proposed to explain all the key optical and dynamic features observed. The results have provided deeper insight into the chemical nature and photophysical properties of bandgap states in chemically modified TiO2 nanomaterials. C1 [Wheeler, Damon A.; Ling, Yichuan; Fitzmorris, Robert C.; Dudzik, Christopher G.; Zavodivker, Liat; Millhauser, Glenn; Li, Yat; Zhang, Jin Z.] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. [Dillon, Robert J.; Bardeen, Christopher] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. [Rajh, Tijana; Dimitrijevic, Nada M.] Argonne Natl Lab, Ctr Nanoscale Mat, NanoBio Interface Grp, Argonne, IL 60439 USA. RP Li, Y (reprint author), Univ Calif Santa Cruz, Dept Chem & Biochem, 1156 High St, Santa Cruz, CA 95064 USA. EM yatli@ucsc.edu; zhang@ucsc.edu RI Ling, Yichuan/I-9567-2016 FU BES Division of the U.S. DOE [DE-FG02-ER46232]; U.S. NSF [DMR-0847786]; UCSC; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX J.Z.Z. acknowledges the BES Division of the U.S. DOE (DE-FG02-ER46232) for financial support. Y.L. acknowledges the support of this work partially by U.S. NSF (DMR-0847786) and UCSC faculty startup funds. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 49 TC 21 Z9 21 U1 5 U2 99 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 19 PY 2013 VL 117 IS 50 BP 26821 EP 26830 DI 10.1021/jp409857j PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 278WL UT WOS:000328920500049 ER PT J AU Sheps, L AF Sheps, Leonid TI Absolute Ultraviolet Absorption Spectrum of a Criegee Intermediate CH2OO SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID GAS-PHASE OZONOLYSIS; RATE CONSTANTS; O-2; SPECTROSCOPY; RADICALS; OZONE; PHOTOLYSIS; KINETICS; HUGGINS; BANDS AB We present the time-resolved UV absorption spectrum of the (B) over tilde ((1)A') <- (X) over tilde ((1)A') electronic transition of formaldehyde oxide, CH2OO, produced by the reaction of CH2I radicals with O-2. In contrast to its UV photodissociation action spectrum, the absorption spectrum of formaldehyde oxide extends to longer wavelengths and exhibits resolved vibrational structure on its low-energy side. Chemical kinetics measurements of its reactivity establish the identity of the absorbing species as CH2OO. Separate measurements of the initial CH2I radical concentration allow a determination of the absolute absorption cross section of CH2OO, with the value at the peak of the absorption band, 355 nm, of sigma(abs) = (3.6 +/- 0.9) x 10(-17) cm(2). The difference between the absorption and action spectra likely arises from excitation to long-lived B ((1)A') vibrational states that relax to lower electronic states by fluorescence or nonradiative processes, rather than by photodissociation. C1 Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Sheps, L (reprint author), Sandia Natl Labs, Combust Res Facil, Mail Stop 9055, Livermore, CA 94551 USA. EM lsheps@sandia.gov FU National Nuclear Security Administration [DE-AC04-94-AL85000]; Sandia National Laboratories under the Laboratory-Directed Research and Development (LDRD) program FX We would like to thank Dr. David W. Chandler for his mentorship in the development of this experimental technique. We thank Prof. Marsha I. Lester for providing the action spectrum of CH2OO. We are also grateful to Dr. Craig A. Taatjes and Dr. David L. Osborn for useful discussions during the preparation of this manuscript. This work was supported by Sandia National Laboratories under the Laboratory-Directed Research and Development (LDRD) program. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under Contract DE-AC04-94-AL85000. NR 27 TC 52 Z9 52 U1 3 U2 70 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD DEC 19 PY 2013 VL 4 IS 24 BP 4201 EP 4205 DI 10.1021/jz402191w PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 278WN UT WOS:000328920700002 PM 26296165 ER PT J AU Gilbert, JA Krajmalnik-Brown, R Porazinska, DL Weiss, SJ Knight, R AF Gilbert, Jack A. Krajmalnik-Brown, Rosa Porazinska, Dorota L. Weiss, Sophie J. Knight, Rob TI Toward Effective Probiotics for Autism and Other Neurodevelopmental Disorders SO CELL LA English DT Editorial Material ID GUT MICROBIOTA AB Hsaio and colleagues link gut microbes to autism spectrum disorders (ASD) in a mouse model. They show that ASD symptoms are triggered by compositional and structural shifts of microbes and associated metabolites, but symptoms are relieved by a Bacteroides fragilis probiotic. Thus probiotics may provide therapeutic strategies for neurodevelopmental disorders. C1 [Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Krajmalnik-Brown, Rosa] Arizona State Univ, Swette Ctr Environm Biotechnol, Biodesign Inst, Tempe, AZ 85287 USA. [Krajmalnik-Brown, Rosa] Arizona State Univ, Sch Sustainable Engn & Built Environm, Tempe, AZ 85287 USA. [Porazinska, Dorota L.; Weiss, Sophie J.; Knight, Rob] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Porazinska, Dorota L.; Weiss, Sophie J.; Knight, Rob] Univ Colorado, BioFrontiers Inst, Boulder, CO 80309 USA. [Knight, Rob] Univ Colorado, Howard Hughes Med Inst, Boulder, CO 80309 USA. RP Knight, R (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. EM rob.knight@colorado.edu RI Knight, Rob/D-1299-2010 FU Howard Hughes Medical Institute; NIDDK NIH HHS [P30 DK042086] NR 11 TC 25 Z9 29 U1 5 U2 59 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD DEC 19 PY 2013 VL 155 IS 7 BP 1446 EP 1448 DI 10.1016/j.cell.2013.11.035 PG 3 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 275QW UT WOS:000328693300002 PM 24360269 ER PT J AU Tsai, CL Tainer, JA AF Tsai, Chi-Lin Tainer, John A. TI Probing DNA by 2-OG-Dependent Dioxygenase SO CELL LA English DT Editorial Material ID REPAIR; PROTEIN; DEMETHYLATION; ENZYMES; DAMAGE; TET2 AB TET-mediated 5-methyl cytosine (5mC) oxidation acts in epigenetic regulation, stem cell development, and cancer. Hu et al. now determine the crystal structure of the TET2 catalytic domain bound to DNA, shedding light on 5mC-DNA substrate recognition and the catalytic mechanism of 5mC oxidation. C1 [Tsai, Chi-Lin; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Tainer, John A.] Scripps Res Inst, Skaggs Inst Chem Biol, Dept Mol Biol, La Jolla, CA 92037 USA. RP Tainer, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM jat@scripps.edu OI Tsai, Chi-Lin/0000-0002-0365-2405 FU NCI NIH HHS [P01 CA092584, R01 CA097209]; NIGMS NIH HHS [R01 GM046312] NR 9 TC 0 Z9 0 U1 2 U2 20 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD DEC 19 PY 2013 VL 155 IS 7 BP 1448 EP 1450 DI 10.1016/j.cell.2013.12.002 PG 4 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 275QW UT WOS:000328693300003 PM 24360270 ER PT J AU Kieffer-Kwon, KR Tang, ZH Mathe, E Qian, JS Sung, MH Li, GL Resch, W Baek, S Pruett, N Grontved, L Vian, L Nelson, S Zare, H Hakim, O Reyon, D Yamane, A Nakahashi, H Kovalchuk, AL Zou, JZ Joung, JK Sartorelli, V Wei, CL Ruan, XA Hager, GL Ruan, YJ Casellas, R AF Kieffer-Kwon, Kyong-Rim Tang, Zhonghui Mathe, Ewy Qian, Jason Sung, Myong-Hee Li, Guoliang Resch, Wolfgang Baek, Songjoon Pruett, Nathanael Grontved, Lars Vian, Laura Nelson, Steevenson Zare, Hossein Hakim, Ofir Reyon, Deepak Yamane, Arito Nakahashi, Hirotaka Kovalchuk, Alexander L. Zou, Jizhong Joung, J. Keith Sartorelli, Vittorio Wei, Chia-Lin Ruan, Xiaoan Hager, Gordon L. Ruan, Yijun Casellas, Rafael TI Interactome Maps of Mouse Gene Regulatory Domains Reveal Basic Principles of Transcriptional Regulation SO CELL LA English DT Article ID ACTIVATION-INDUCED DEAMINASE; EMBRYONIC STEM-CELLS; LONG NONCODING RNAS; HUMAN GENOME; CHROMATIN INTERACTIONS; AID EXPRESSION; ENHANCERS; LYMPHOCYTES; ELEMENTS; RECOMBINATION AB A key finding of the ENCODE project is that the enhancer landscape of mammalian cells undergoes marked alterations during ontogeny. However, the nature and extent of these changes are unclear. As part of the NIH Mouse Regulome Project, we here combined DNaseI hypersensitivity, ChIP-seq, and ChIA-PET technologies to map the promoter-enhancer interactomes of pluripotent ES cells and differentiated B lymphocytes. We confirm that enhancer usage varies widely across tissues. Unexpectedly, we find that this feature extends to broadly transcribed genes, including Myc and Pim1 cell-cycle regulators, which associate with an entirely different set of enhancers in ES and B cells. By means of high-resolution CpG methylomes, genome editing, and digital footprinting, we show that these enhancers recruit lineage-determining factors. Furthermore, we demonstrate that the turning on and off of enhancers during development correlates with promoter activity. We propose that organisms rely on a dynamic enhancer landscape to control basic cellular functions in a tissue-specific manner. C1 [Kieffer-Kwon, Kyong-Rim; Mathe, Ewy; Qian, Jason; Resch, Wolfgang; Pruett, Nathanael; Vian, Laura; Nelson, Steevenson; Yamane, Arito; Nakahashi, Hirotaka; Casellas, Rafael] NIAMS, NIH, Bethesda, MD 20892 USA. [Tang, Zhonghui; Li, Guoliang; Ruan, Xiaoan; Ruan, Yijun] Univ Connecticut, Jackson Lab Genom Med, Farmington, CT 06030 USA. [Tang, Zhonghui; Li, Guoliang; Ruan, Xiaoan; Ruan, Yijun] Univ Connecticut, Dept Genet & Dev Biol, Farmington, CT 06030 USA. [Sung, Myong-Hee; Baek, Songjoon; Grontved, Lars; Hager, Gordon L.] NCI, Lab Receptor Biol & Gene Express, NIH, Bethesda, MD 20892 USA. [Zare, Hossein; Sartorelli, Vittorio] NIAMS, Lab Muscle Stem Cells & Gene Regulat, NIH, Bethesda, MD 20892 USA. [Hakim, Ofir] Bar Ilan Univ, IL-5290002 Ramat Gan, Israel. [Reyon, Deepak; Joung, J. Keith] Massachusetts Gen Hosp, Ctr Computat & Integrat Biol, Mol Pathol Unit, Charlestown, MA 02129 USA. [Reyon, Deepak; Joung, J. Keith] Massachusetts Gen Hosp, Ctr Canc Res, Charlestown, MA 02129 USA. [Reyon, Deepak; Joung, J. Keith] Harvard Univ, Sch Med, Dept Pathol, Boston, MA 02115 USA. [Kovalchuk, Alexander L.] NIAID, Immunogenet Lab, NIH, Rockville, MD 20852 USA. [Zou, Jizhong] NIAMS, Lab Stem Cell Biol, NIH, Bethesda, MD 20892 USA. [Wei, Chia-Lin] DOE Joint Genome Inst, Walnut Creek, CA 94598 USA. [Casellas, Rafael] NCI, Ctr Canc Res, NIH, Bethesda, MD 20892 USA. RP Casellas, R (reprint author), NIAMS, NIH, Bethesda, MD 20892 USA. EM rafael.casellas@nih.gov RI Li, Guoliang/I-1494-2015; OI Li, Guoliang/0000-0003-1601-6640; Grontved, Lars/0000-0002-6735-8483 FU Intramural Research Program of NIAMS; NCI; internal Jackson Laboratory fund [JAX19020120]; NIH [DP1 GM105378, P50 HG005550]; Defense Advanced Research Projects Agency [W911NF-11-2-0056]; Jim and Ann Orr Massachusetts General Hospital Research Scholar Award; NIH UGSP program FX We thank Kefei Yu for CH12 cells and protocols; J. Simone and J. Lay for cell sorting; G. Gutierrez for technical assistance with Illumina analyzer. This work was supported by the Intramural Research Program of NIAMS and NCI, and internal Jackson Laboratory fund JAX19020120 to Y.R. J.K.J. was supported by NIH grants DP1 GM105378 and P50 HG005550, the Defense Advanced Research Projects Agency grant W911NF-11-2-0056 and The Jim and Ann Orr Massachusetts General Hospital Research Scholar Award. J. Q. was supported by the NIH UGSP program. All animal experiments were performed according to NIH guidelines. High-performance computation was performed using NIH Helix Systems (http://helix.nih.gov). J. K. J. has a financial interest in Transposagen Biopharmaceuticals. J.K.J.'s interests were reviewed and are managed by Massachusetts General Hospital and Partners HealthCare in accordance with their conflict of interest policies. NR 49 TC 116 Z9 120 U1 3 U2 44 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD DEC 19 PY 2013 VL 155 IS 7 BP 1507 EP 1520 DI 10.1016/j.cell.2013.11.039 PG 14 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 275QW UT WOS:000328693300008 PM 24360274 ER PT J AU Nord, AS Blow, MJ Attanasio, C Akiyama, JA Holt, A Hosseini, R Phouanenavong, S Plajzer-Frick, I Shoukry, M Afzal, V Rubenstein, JLR Rubin, EM Pennacchio, LA Visel, A AF Nord, Alex S. Blow, Matthew J. Attanasio, Catia Akiyama, Jennifer A. Holt, Amy Hosseini, Roya Phouanenavong, Sengthavy Plajzer-Frick, Ingrid Shoukry, Malak Afzal, Veena Rubenstein, John L. R. Rubin, Edward M. Pennacchio, Len A. Visel, Axel TI Rapid and Pervasive Changes in Genome-wide Enhancer Usage during Mammalian Development SO CELL LA English DT Article ID GENE-EXPRESSION; EMBRYONIC-DEVELOPMENT; TRANSCRIPTION FACTORS; REGULATORY SEQUENCES; NEURONAL DEVELOPMENT; CARDIAC DEVELOPMENT; IN-VIVO; HEART; STATE; MICE AB Enhancers are distal regulatory elements that can activate tissue-specific gene expression and are abundant throughout mammalian genomes. Although substantial progress has been made toward genome-wide annotation of mammalian enhancers, their temporal activity patterns and global contributions in the context of developmental in vivo processes remain poorly explored. Here we used epigenomic profiling for H3K27ac, a mark of active enhancers, coupled to transgenic mouse assays to examine the genome-wide utilization of enhancers in three different mouse tissues across seven developmental stages. The majority of the similar to 90,000 enhancers identified exhibited tightly temporally restricted predicted activity windows and were associated with stage-specific biological functions and regulatory pathways in individual tissues. Comparative genomic analysis revealed that evolutionary conservation of enhancers decreases following midgestation across all tissues examined. The dynamic enhancer activities uncovered in this study illuminate rapid and pervasive temporal in vivo changes in enhancer usage that underlie processes central to development and disease. C1 [Nord, Alex S.; Blow, Matthew J.; Attanasio, Catia; Akiyama, Jennifer A.; Holt, Amy; Hosseini, Roya; Phouanenavong, Sengthavy; Plajzer-Frick, Ingrid; Shoukry, Malak; Afzal, Veena; Rubin, Edward M.; Pennacchio, Len A.; Visel, Axel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Blow, Matthew J.; Rubin, Edward M.; Pennacchio, Len A.; Visel, Axel] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Rubenstein, John L. R.] Univ Calif San Francisco, Dept Psychiat, San Francisco, CA 94158 USA. [Visel, Axel] Univ Calif, Sch Nat Sci, Merced, CA 95343 USA. RP Pennacchio, LA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, MS 84-171, Berkeley, CA 94720 USA. EM lapennacchio@lbl.gov; avisel@lbl.gov RI Visel, Axel/A-9398-2009; Blow, Matthew/G-6369-2012; attanasio, catia/D-5042-2017 OI Visel, Axel/0000-0002-4130-7784; Blow, Matthew/0000-0002-8844-9149; FU NIH/NIGMS NRSA [GM105202]; SNSF advanced researchers fellowship; NIH [R01NS062859A, R01HG003988, U01DE020060]; NIMH [R37MH049428]; Department of Energy, University of California [DE-AC02-05CH11231] FX sThe authors thank Chia-lin Wei and Cindy Choi for help with chromatin immunoprecipitation from embryonic mouse tissue and Diane Dickel and Han Wu for guidance and advice regarding enhancer activity analysis. A.S.N. was supported by NIH/NIGMS NRSA F32 fellowship GM105202. C. A. was supported by a SNSF advanced researchers fellowship. A. V. and L. A. P. were supported by NIH grants R01NS062859A, R01HG003988, and U01DE020060. J.L.R.R. was supported by NIMH grant R37MH049428. Research was conducted at the E.O. Lawrence Berkeley National Laboratory and performed under Department of Energy Contract DE-AC02-05CH11231, University of California. NR 66 TC 86 Z9 86 U1 2 U2 18 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD DEC 19 PY 2013 VL 155 IS 7 BP 1521 EP 1531 DI 10.1016/j.cell.2013.11.033 PG 11 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 275QW UT WOS:000328693300009 PM 24360275 ER PT J AU Eliseev, EA Kalinin, SV Gu, YJ Glinchuk, MD Khist, V Borisevich, A Gopalan, V Chen, LQ Morozovska, AN AF Eliseev, Eugene A. Kalinin, Sergei V. Gu, Yijia Glinchuk, Maya D. Khist, Victoria Borisevich, Albina Gopalan, Venkatraman Chen, Long-Qing Morozovska, Anna N. TI Universal emergence of spatially modulated structures induced by flexoantiferrodistortive coupling in multiferroics SO PHYSICAL REVIEW B LA English DT Article ID SIMILAR MAGNETIC-ALLOYS; THIN-FILMS; EXTRINSIC MAGNETOSTRICTION; HETEROGENEOUS MODEL; PHASE-TRANSITIONS; ELECTRIC-FIELD; DOMAIN-WALLS; FE-GA; FERROELECTRICS; CRYSTALS AB We proved the existence of a universal flexoantiferrodistortive coupling as a necessary complement to the well-known flexoelectric coupling. The coupling is universal for all antiferrodistortive systems and can lead to the formation of incommensurate, spatially modulated phases in multiferroics. Our analysis can provide a self-consistent mesoscopic explanation for a broad range of modulated domain structures observed experimentally in multiferroics. C1 [Eliseev, Eugene A.; Glinchuk, Maya D.; Khist, Victoria] Natl Acad Sci Ukraine, Inst Problems Mat Sci, UA-03142 Kiev, Ukraine. [Kalinin, Sergei V.; Borisevich, Albina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Gu, Yijia; Gopalan, Venkatraman; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Morozovska, Anna N.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. RP Eliseev, EA (reprint author), Natl Acad Sci Ukraine, Inst Problems Mat Sci, 3 Krjijanovskogo, UA-03142 Kiev, Ukraine. EM sergei2@ornl.gov; morozo@i.com.ua RI Borisevich, Albina/B-1624-2009; Gu, Yijia/A-6418-2013; Chen, LongQing/I-7536-2012; Kalinin, Sergei/I-9096-2012 OI Borisevich, Albina/0000-0002-3953-8460; Gu, Yijia/0000-0001-8036-6309; Chen, LongQing/0000-0003-3359-3781; Kalinin, Sergei/0000-0001-5354-6152 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; National Science Foundation [DMR-1210588, DMR-0820404]; State Fund of Fundamental State Fund of Fundamental Research of Ukraine, SFFR-NSF [UU48/002] FX The work was supported in part (S. V. K., A. B.) by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, the National Science Foundation Grants No. DMR-1210588 and No. DMR-0820404 (V. G., L. Q. C., and Y.G.). A.N.M. and E. A. E. acknowledge Prof. Yulian M. Vysochanskii for fruitful discussion as well as the State Fund of Fundamental State Fund of Fundamental Research of Ukraine, SFFR-NSF Project No. UU48/002 (NSF Grant No. DMR-1210588). NR 72 TC 12 Z9 12 U1 3 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD DEC 19 PY 2013 VL 88 IS 22 AR 224105 DI 10.1103/PhysRevB.88.224105 PG 9 WC Physics, Condensed Matter SC Physics GA 275OS UT WOS:000328687300003 ER PT J AU Kogan, VG Prozorov, R Mishra, V AF Kogan, V. G. Prozorov, R. Mishra, V. TI London penetration depth and pair breaking SO PHYSICAL REVIEW B LA English DT Article ID SUPERFLUID DENSITY TENSOR; D-WAVE SUPERCONDUCTORS; UNCONVENTIONAL SUPERCONDUCTORS; PARAMAGNETIC IMPURITIES; SCATTERING; ALLOYS AB The London penetration depth is evaluated for isotropic materials for any transport and pair-breaking Born scattering rates. Besides known results, a number of features are found. The slope vertical bar d rho/d theta vertical bar of the normalized superfluid density rho = lambda(2)(0)/lambda(2)(theta) at the transition theta = T/T-c = 1 has a minimum near the value of the pair-breaking parameter separating gapped and gapless states. The low-T exponentially flat part of rho for the s-wave materials is suppressed by increasing pair breaking. For strong T-c suppression by magnetic impurities the "Homes scaling" lambda(-2)(0) proportional to sigma T-c with sigma being the normal conductivity gives way to lambda(-2)(0) proportional to sigma T-c(2). For the d-wave order parameter, the transport and spin-flip Born scattering rates enter the theory only as a sum; in particular, they affect the T-c depression in the same manner. We confirm that the linear low-temperature behavior of rho in a broad range of the combined scattering parameter turns to the T-2 behavior only when the critical temperature is suppressed at least by a factor of 3 relative to the clean limit T-c0. Moreover, in this range, rho(theta) is only weakly dependent on the scattering parameter, i.e., it is nearly universal. C1 [Kogan, V. G.; Prozorov, R.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Kogan, V. G.; Prozorov, R.] Iowa State Univ, Dept Phys, Ames, IA 50011 USA. [Mishra, V.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Kogan, VG (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; Center for Emergent Superconductivity, an Energy Frontier Research Center; U.S. DOE, Office of Science [DE-AC0298CH1088] FX We are grateful to P. Hirschfeld, J. Clem, and M. Tanatar for illuminating discussions. The work at Ames Lab was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. V. M. acknowledges support from the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the U.S. DOE, Office of Science, under Award No. DE-AC0298CH1088. NR 26 TC 4 Z9 4 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 19 PY 2013 VL 88 IS 22 AR 224508 DI 10.1103/PhysRevB.88.224508 PG 9 WC Physics, Condensed Matter SC Physics GA 275OS UT WOS:000328687300006 ER PT J AU Wang, SY Wang, WH Tan, LZ Li, XG Shi, ZL Kuang, GW Liu, PNA Louie, SG Lin, NA AF Wang, Shiyong Wang, Weihua Tan, Liang Z. Li, Xing Guang Shi, Zilang Kuang, Guowen Liu, Pei Nian Louie, Steven G. Lin, Nian TI Tuning two-dimensional band structure of Cu(111) surface-state electrons that interplay with artificial supramolecular architectures SO PHYSICAL REVIEW B LA English DT Article ID DIRAC FERMIONS; CONFINEMENT; INTERFERENCE; GRAPHENE; GAS AB We report on the modulation of two-dimensional (2D) bands of Cu(111) surface-state electrons by three isostructural supramolecular honeycomb architectures with different periodicity or constituent molecules. Using Fourier-transformed scanning tunneling spectroscopy and model calculations, we resolved the 2D band structures and found that the intrinsic surface-state band is split into discrete bands. The band characteristics including band gap, band bottom, and bandwidth are controlled by the network unit cell size and the nature of the molecule-surface interaction. In particular, Dirac cones emerge where the second and third bands meet at the K points of the Brillouin zone of the supramolecular lattice. C1 [Wang, Shiyong; Wang, Weihua; Shi, Zilang; Kuang, Guowen; Lin, Nian] Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Tan, Liang Z.; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Tan, Liang Z.; Louie, Steven G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Li, Xing Guang; Liu, Pei Nian] E China Univ Sci & Technol, Shanghai Key Lab Funct Mat Chem, Shanghai 200237, Peoples R China. [Li, Xing Guang; Liu, Pei Nian] E China Univ Sci & Technol, Inst Fine Chem, Shanghai 200237, Peoples R China. [Louie, Steven G.] Hong Kong Univ Sci & Technol, Inst Adv Study, Hong Kong, Hong Kong, Peoples R China. RP Lin, NA (reprint author), Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China. EM phnlin@ust.hk RI Wang, Weihua/K-1297-2012; OI Wang, Weihua/0000-0002-2269-1952; Tan, Liang Z/0000-0003-4724-6369 FU Hong Kong RGC [D-HK008/11T]; U.S. National Science Foundation [DMR1-1006184]; Simons Foundation Fellowship in Theoretical Physics FX This work is supported in part by the Hong Kong RGC (D-HK008/11T) and the U.S. National Science Foundation Grant No. DMR1-1006184. S. G. L. acknowledges support of a Simons Foundation Fellowship in Theoretical Physics. We acknowledge the assistance of the XSEDE computational cluster resource provided by NICS (kraken), supported by the National Science Foundation NR 32 TC 13 Z9 13 U1 6 U2 46 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 19 PY 2013 VL 88 IS 24 AR 245430 DI 10.1103/PhysRevB.88.245430 PG 6 WC Physics, Condensed Matter SC Physics GA 275OW UT WOS:000328687700002 ER PT J AU Ghosh, D AF Ghosh, Diptimoy TI Boosted dibosons from mixed heavy top squarks SO PHYSICAL REVIEW D LA English DT Article ID COLLIDERS; PROGRAM; HADRON; HIGGS AB The lighter mass eigenstate ((t) over tilde (1)) of the two top squarks, the scalar superpartners of the top quark, is extremely difficult to discover if it is almost degenerate with the lightest neutralino ((chi) over tilde (0)(1)), the lightest stable supersymmetric particle in the R-parity conserving supersymmetry. The current experimental bound on (t) over tilde (1) mass in this scenario stands only around 200 GeV. For such a light (t) over tilde (1), the heavier top squark ((t) over tilde (2)) can also be around the TeV scale. Moreover, the high value of the Higgs (h) mass prefers the left-and right-handed top squarks to be highly mixed, allowing the possibility of a considerable branching ratio for (t) over tilde (2) -> -> (t) over tilde (1)h and (t) over tilde (2) -> (t) over tilde (1)Z. In this paper, we explore the above possibility together with the pair production of (t) over tilde (2) -> (t) over tilde (2), giving rise to the spectacular diboson + missing transverse energy final state. For an approximately 1 TeV (t) over tilde (2) and a few hundred GeV (t) over tilde (1) the final state particles can be moderately boosted, which encourages us to propose a novel search strategy employing the jet substructure technique to tag the boosted h and Z. The reconstruction of the h and Z momenta also allows us to construct the stransverse mass M-T2, providing an additional efficient handle to fight the backgrounds. We show that a 4-5 sigma signal can be observed at the 14 TeV LHC for similar to 1 TeV (t) over tilde (2) with 100 fb(-1) integrated luminosity. C1 [Ghosh, Diptimoy] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Ghosh, Diptimoy] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Ghosh, D (reprint author), Ist Nazl Fis Nucl, Sez Roma, Piazzale A Moro 2, I-00185 Rome, Italy. EM diptimoy.ghosh@roma1.infn.it FU European Research Council under the European Union's Seventh Framework Programme [279972] FX We thank JoAnne Hewett and Tom Rizzo for the hospitality at the SLAC Theory Group where this work was started. We also thank Prateek Agrawal, Wolfgang Altmannshofer, Martin Bauer, Patrick Fox, Raoul Rontsch, and Felix Yu for useful discussions. The research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework Programme (FP/2007-2013)/ERC Grant No. 279972. NR 39 TC 12 Z9 12 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD DEC 19 PY 2013 VL 88 IS 11 AR 115013 DI 10.1103/PhysRevD.88.115013 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 275RA UT WOS:000328693800001 ER PT J AU Reichhardt, C Reichhardt, CJO AF Reichhardt, C. Reichhardt, C. J. Olson TI Active matter ratchets with an external drift SO PHYSICAL REVIEW E LA English DT Article ID BROWNIAN MOTORS; PARTICLE SEPARATION; SURFACE SCATTERING; SWIMMING BACTERIA; MICROSWIMMERS; TRANSPORT; MOTION; MACROMOLECULES; SWIMMERS; CELL AB When active matter particles such as swimming bacteria are placed in an asymmetric array of funnels, it has been shown that a ratchet effect can occur even in the absence of an external drive. Here we examine active ratchets for two-dimensional arrays of funnels or L shapes where there is also an externally applied dc drive or drift. We show that for certain conditions the ratchet effect can be strongly enhanced and it is possible to have conditions under which run-and-tumble particles with one run length move in the opposite direction from particles with a different run length. For the arrays of L shapes, we find that the application of a drift force can enhance a transverse rectification in the direction perpendicular to the drift. When particle-particle steric interactions are included, we find that the ratchet effects can be either enhanced or suppressed depending on barrier geometry, particle run length, and particle density. C1 [Reichhardt, C.; Reichhardt, C. J. Olson] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reichhardt, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Reichhardt, Cynthia/0000-0002-3487-5089 FU NNSA of the U.S. DOE at LANL [DE-AC52-06NA25396] FX This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396. NR 93 TC 13 Z9 13 U1 0 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD DEC 19 PY 2013 VL 88 IS 6 AR 062310 DI 10.1103/PhysRevE.88.062310 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 275SN UT WOS:000328697900001 PM 24483447 ER PT J AU Lockyer, N AF Lockyer, Nigel TI Together to the next frontier SO NATURE LA English DT Editorial Material C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Lockyer, N (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM lockyer@fnal.gov NR 0 TC 2 Z9 2 U1 1 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD DEC 19 PY 2013 VL 504 IS 7480 BP 367 EP 368 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 273ZR UT WOS:000328575300028 PM 24358507 ER PT J AU Thorne, RM Li, W Ni, B Ma, Q Bortnik, J Chen, L Baker, DN Spence, HE Reeves, GD Henderson, MG Kletzing, CA Kurth, WS Hospodarsky, GB Blake, JB Fennell, JF Claudepierre, SG Kanekal, SG AF Thorne, R. M. Li, W. Ni, B. Ma, Q. Bortnik, J. Chen, L. Baker, D. N. Spence, H. E. Reeves, G. D. Henderson, M. G. Kletzing, C. A. Kurth, W. S. Hospodarsky, G. B. Blake, J. B. Fennell, J. F. Claudepierre, S. G. Kanekal, S. G. TI Rapid local acceleration of relativistic radiation-belt electrons by magnetospheric chorus SO NATURE LA English DT Article ID PC5 WAVES; ENERGIZATION; SCATTERING; DIFFUSION; STORMS; MODEL AB Recent analysis of satellite data obtained during the 9 October 2012 geomagnetic storm identified the development of peaks in electron phase space density(1), which are compelling evidence for local electron acceleration in the heart of the outer radiation belt(2,3), but are inconsistent with acceleration by inward radial diffusive transport(4,5). However, the precise physical mechanism responsible for the acceleration on 9 October was not identified. Previous modelling has indicated that a magnetospheric electromagnetic emission known as chorus could be a potential candidate for local electron acceleration(6-10), but a definitive resolution of the importance of chorus for radiation-belt acceleration was not possible because of limitations in the energy range and resolution of previous electron observations and the lack of a dynamic global wave model. Here we report high-resolution electron observations(11) obtained during the 9 October storm and demonstrate, using a two-dimensional simulation performed with a recently developed time-varying data-driven model(12), that chorus scattering explains the temporal evolution of both the energy and angular distribution of the observed relativistic electron flux increase. Our detailed modelling demonstrates the remarkable efficiency of wave acceleration in the Earth's outer radiation belt, and the results presented have potential application to Jupiter, Saturn and other magnetized astrophysical objects. C1 [Thorne, R. M.; Li, W.; Ni, B.; Ma, Q.; Bortnik, J.; Chen, L.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. [Baker, D. N.] Univ Colorado, Lab Atmospher & Space Res, Boulder, CO 80303 USA. [Spence, H. E.] Univ New Hampshire, Each Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Reeves, G. D.; Henderson, M. G.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM 87544 USA. [Kletzing, C. A.; Kurth, W. S.; Hospodarsky, G. B.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Blake, J. B.; Fennell, J. F.; Claudepierre, S. G.] Aerosp Corp, Los Angeles, CA 90245 USA. [Kanekal, S. G.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Thorne, RM (reprint author), Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. EM rmt@atmos.ucla.edu RI Li, Wen/F-3722-2011; Henderson, Michael/A-3948-2011; OI Henderson, Michael/0000-0003-4975-9029; Kletzing, Craig/0000-0002-4136-3348; Spence, Harlan/0000-0002-2526-2205; Kurth, William/0000-0002-5471-6202; Reeves, Geoffrey/0000-0002-7985-8098; Hospodarsky, George/0000-0001-9200-9878 FU JHU/APL under NASA [967399, 921647, NAS5-01072]; EMFISIS [1001057397:01]; ECT [13-041] FX This work was supported by JHU/APL contracts 967399 and 921647 under NASA's prime contract NAS5-01072. The analysis at UCLA was supported by the EMFISIS sub-award 1001057397:01 and by the ECT sub-award 13-041. We thank OMNIweb for providing geomagnetic indices and solar wind parameters used in this study and the NOAA POES team for providing POES electron data. NR 30 TC 162 Z9 163 U1 5 U2 35 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD DEC 19 PY 2013 VL 504 IS 7480 BP 411 EP + DI 10.1038/nature12889 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 273ZR UT WOS:000328575300046 PM 24352287 ER PT J AU Yee, BT Weatherford, BR Barnat, EV Foster, JE AF Yee, B. T. Weatherford, B. R. Barnat, E. V. Foster, J. E. TI Dynamics of a helium repetitively pulsed nanosecond discharge SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article ID PRESSURE GLOW-DISCHARGE; EXCITATION-TRANSFER; METASTABLE HELIUM; ELECTRIC-FIELDS; FLOW-CONTROL; AIR FLOWS; PLASMA; IGNITION; TEMPERATURE; IONIZATION AB Empirical study of repetitively pulsed nanosecond discharges (RPNDs) on time scales relevant to their formation is notably difficult. Here, we present measurements of the metastable dynamics in a helium RPND with a time resolution of 5 ns at 1.0, 4.0 and 8.0 Torr. A detailed global model is developed in which the applied electric field is chosen to match the measured metastable densities. This approach results in predictions of the local electric fields and the evolution of the electron densities and temperatures. The estimated electric fields in the bulk of plasma range from 150-350 Td, and the peak electron temperatures range from 11-75 eV. The large temperatures necessary for the simulations to match the observed metastable densities may indicate a distribution function far from equilibrium. Experimental and simulation results indicate a delay between the applied field and the peak excitation and ionization rates, likely a consequence of the finite rate coefficients. Finally, evidence is provided to suggest that that optimization of electron production is mutually exclusive with that of the metastables. C1 [Yee, B. T.; Foster, J. E.] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Weatherford, B. R.; Barnat, E. V.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Yee, BT (reprint author), Univ Michigan, Dept Nucl Engn & Radiol Sci, 2355 Bonisteel Blvd, Ann Arbor, MI 48109 USA. EM btyee@umich.edu OI Yee, Benjamin/0000-0002-8808-3546 FU Department of Energy Office of Fusion Energy Science [DE-SC0001939] FX This work was supported by the Department of Energy Office of Fusion Energy Science Contract DE-SC0001939. NR 47 TC 3 Z9 3 U1 6 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD DEC 18 PY 2013 VL 46 IS 50 AR 505204 DI 10.1088/0022-3727/46/50/505204 PG 10 WC Physics, Applied SC Physics GA AA5MN UT WOS:000331143600013 ER PT J AU Laurens, LML Wolfrum, EJ AF Laurens, L. M. L. Wolfrum, E. J. TI High-Throughput Quantitative Biochemical Characterization of Algal Biomass by NIR Spectroscopy; Multiple Linear Regression and Multivariate Linear Regression Analysis SO JOURNAL OF AGRICULTURAL AND FOOD CHEMISTRY LA English DT Article DE microalgae; biomass; lipids; infrared spectroscopy; multivariate calibration; chemometrics ID MICROALGAE AB One of the challenges associated with microalgal biomass characterization and the comparison of microalgal strains and conversion processes is the rapid determination of the composition of algae. We have developed and applied a high-throughput screening technology based on near-infrared (NIR) spectroscopy for the rapid and accurate determination of algal biomass composition. We show that NIR spectroscopy can accurately predict the full composition using multivariate linear regression analysis of varying lipid, protein, and carbohydrate content of algal biomass samples from three strains. We also demonstrate a high quality of predictions of an independent validation set. A high-throughput 96-well configuration for spectroscopy gives equally good prediction relative to a ring-cup configuration, and thus, spectra can be obtained from as little as 10-20 mg of material. We found that lipids exhibit a dominant, distinct, and unique fingerprint in the NIR spectrum that allows for the use of single and multiple linear regression of respective wavelengths for the prediction of the biomass lipid content. This is not the case for carbohydrate and protein content, and thus, the use of multivariate statistical modeling approaches remains necessary. C1 [Laurens, L. M. L.; Wolfrum, E. J.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Laurens, LML (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Lieve.Laurens@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy jointly as part of the BioEnergy Technology Office (BETO) [9.6.1.8]; Sustainable Algal Biofuels Consortium project; DOE [DE-EE0003372] FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy jointly as part of the BioEnergy Technology Office (BETO), under task 9.6.1.8 and the Sustainable Algal Biofuels Consortium project, funded under DOE Award No. DE-EE0003372. NR 18 TC 4 Z9 4 U1 9 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0021-8561 EI 1520-5118 J9 J AGR FOOD CHEM JI J. Agric. Food Chem. PD DEC 18 PY 2013 VL 61 IS 50 BP 12307 EP 12314 DI 10.1021/jf403086f PG 8 WC Agriculture, Multidisciplinary; Chemistry, Applied; Food Science & Technology SC Agriculture; Chemistry; Food Science & Technology GA 278CI UT WOS:000328865200017 PM 24229385 ER PT J AU Chien, MP Carlini, AS Hu, DH Barback, CV Rush, AM Hall, DJ Orr, G Gianneschi, NC AF Chien, Miao-Ping Carlini, Andrea S. Hu, Dehong Barback, Christopher V. Rush, Anthony M. Hall, David J. Orr, Galya Gianneschi, Nathan C. TI Enzyme-Directed Assembly of Nanoparticles in Tumors Monitored by in Vivo Whole Animal Imaging and ex Vivo Super-Resolution Fluorescence Imaging SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OPTICAL RECONSTRUCTION MICROSCOPY; CELL-PENETRATING PEPTIDES; MATRIX METALLOPROTEINASES; MICELLAR NANOPARTICLES; PROBES; POLYMERIZATION; CONTRAST; LIMIT; ROMP AB Matrix metalloproteinase enzymes, overexpressed in HT-1080 human fibrocarcinoma tumors, were used to guide the accumulation and retention of an enzyme-responsive nanoparticle in a xenograft mouse model. The nanoparticles were prepared as micelles from amphiphilic block copolymers bearing a simple hydrophobic block and a hydrophilic peptide brush. The polymers were end-labeled with Alexa Fluor 647 dyes leading to the formation of labeled micelles upon dialysis of the polymers from DMSO/DMF to aqueous buffer. This dye-labeling strategy allowed the presence of the retained material to be visualized via whole animal imaging in vivo and in ex vivo organ analysis following intratumoral injection into HT-1080 xenograft tumors. We propose that the material is retained by virtue of an enzyme-induced accumulation process whereby particles change morphology from 20 nm spherical micelles to micrometer-scale aggregates, kinetically trapping them within the tumor. This hypothesis is tested here via an unprecedented super-resolution fluorescence analysis of ex vivo tissue slices confirming a particle size increase occurs concomitantly with extended retention of responsive particles compared to unresponsive controls. C1 [Chien, Miao-Ping; Carlini, Andrea S.; Rush, Anthony M.; Gianneschi, Nathan C.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Barback, Christopher V.; Hall, David J.] Univ Calif San Diego, Dept Radiol, La Jolla, CA 92093 USA. [Hu, Dehong; Orr, Galya] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. RP Gianneschi, NC (reprint author), Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. EM ngianneschi@ucsd.edu RI Hu, Dehong/B-4650-2010 OI Hu, Dehong/0000-0002-3974-2963 FU NIH [NIBIB - 1R01EB011633, 1DP2OD008724]; Henry & Camille Dreyfus Foundation; Alfred P. Sloan Foundation; Department of Energy's Office of Biological and Environmental Research FX The authors acknowledge support for this work from NIH (NIBIB - 1R01EB011633). Furthermore, we thank NIH via a Director's New Innovator Award (1DP2OD008724). N.C.G. acknowledges the Henry & Camille Dreyfus Foundation for a New Faculty Award and the Alfred P. Sloan Foundation for a fellowship. Part of this research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 29 TC 31 Z9 31 U1 14 U2 135 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 18 PY 2013 VL 135 IS 50 BP 18710 EP 18713 DI 10.1021/ja408182p PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 278CH UT WOS:000328865100002 PM 24308273 ER PT J AU Zhao, C Sun, QF Hart-Cooper, WM Dipasquale, AG Toste, FD Bergman, RG Raymond, KN AF Zhao, Chen Sun, Qing-Fu Hart-Cooper, William M. Dipasquale, Antonio G. Toste, F. Dean Bergman, Robert G. Raymond, Kenneth N. TI Chiral Amide Directed Assembly of a Diastereo- and Enantiopure Supramolecular Host and its Application to Enantioselective Catalysis of Neutral Substrates SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CARBONYL-ENE CYCLIZATION; TITANIUM PERCHLORATE; ASYMMETRIC CATALYSIS; WATER; ENCAPSULATION; STABILIZATION; RECOGNITION; CHEMISTRY; CLUSTER; CAGE AB The synthesis of a novel supramolecular tetrahedral assembly of K12Ga4L6 stoichiometry is reported. The newly designed chiral ligand exhibits high diastereoselective control during cluster formation, leading exclusively to a single diastereomer of the desired host. This new assembly also exhibits high stability toward oxidation or a low pH environment and is a more robust and efficient catalyst for asymmetric organic transformations of neutral substrates. C1 [Toste, F. Dean] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Toste, FD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM fdtoste@berkeley.edu; rbergman@berkeley.edu; raymond@socrates.berkeley.edu RI Sun, Qing-Fu/C-9406-2011; OI Toste, F. Dean/0000-0001-8018-2198 FU Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX This research was supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL (DE-AC02-05CH11231. The authors thank Amela Drljevic, Kristen Burford, and Rebecca Triano for helpful discussions. NR 34 TC 66 Z9 66 U1 13 U2 120 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 18 PY 2013 VL 135 IS 50 BP 18802 EP 18805 DI 10.1021/ja411631v PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 278CH UT WOS:000328865100025 PM 24283463 ER PT J AU Payne, CM Jiang, W Shirts, MR Himmel, ME Crowley, MF Beckham, GT AF Payne, Christina M. Jiang, Wei Shirts, Michael R. Himmel, Michael E. Crowley, Michael F. Beckham, Gregg T. TI Glycoside Hydrolase Processivity Is Directly Related to Oligosaccharide Binding Free Energy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRICHODERMA-REESEI CELLOBIOHYDROLASE; AROMATIC-CARBOHYDRATE INTERACTIONS; PHANEROCHAETE-CHRYSOSPORIUM CEL7D; FAMILY 7 CELLOBIOHYDROLASE; SERRATIA-MARCESCENS; CELLULOSE HYDROLYSIS; ANGSTROM RESOLUTION; MOLECULAR-DYNAMICS; SUBSTRATE-BINDING; CRYSTAL-STRUCTURE AB Many glycoside hydrolase (GH) enzymes act via a processive mechanism whereby an individual carbohydrate polymer chain is decrystallized and hydrolyzed along the chain without substrate dissociation. Despite considerable structural and biochemical studies, a molecular-level theory of processivity that relates directly to structural features of GH enzymes does not exist. Here, we hypothesize that the degree of processivity is directly linked to the ability of an enzyme to decrystallize a polymer chain from a crystal, quantified by the binding free energy of the enzyme to the cello-oligosaccharide. We develop a simple mathematical relationship formalizing this hypothesis to quantitatively relate the binding free energy to experimentally measurable kinetic parameters. We then calculate the absolute ligand binding free energy of cellulose chains to the biologically and industrially important GH Family 7 processive cellulases with free energy perturbation/replica-exchange molecular dynamics. Taken with previous observations, our results suggest that degree of processivity is directly correlated to the binding free energy of cello-oligosaccharide ligands to GH7s. The observed binding free energies also suggest candidate polymer morphologies susceptible to enzyme action when compared to the work required to decrystallize cellulose chains. We posit that the ligand binding free energy is a key parameter in comparing the activity and function of GHs and may offer a molecular-level basis toward a general theory of carbohydrate processivity in GHs and other enzymes able to process linear carbohydrate polymers, such as cellulose and chitin synthases. C1 [Payne, Christina M.] Univ Kentucky, Dept Chem & Mat Engn, Lexington, KY 40506 USA. [Payne, Christina M.] Univ Kentucky, Ctr Computat Sci, Lexington, KY 40506 USA. [Jiang, Wei] Argonne Natl Lab, Argonne Leadership Comp Facil, Lemont, IL 60439 USA. [Shirts, Michael R.] Univ Virginia, Dept Chem Engn, Charlottesville, VA 22904 USA. [Himmel, Michael E.; Crowley, Michael F.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Payne, CM (reprint author), Univ Kentucky, Dept Chem & Mat Engn, Lexington, KY 40506 USA. EM Christy.Payne@ulcy.edu; wjiang@alclanl.gov; Gregg.Beckham@nrel.gov RI Payne, Christina/C-7338-2011 OI Payne, Christina/0000-0001-5264-0964 FU Department of Energy (DOE) BioEnergy Technologies Office; DOE Office of Science [DE-AC02-06CH11357]; National Institute for Computational Sciences Kraken cluster under the National Science Foundation Extreme Science and Engineering Discovery Environment (XSEDE) Grant [MCB090159]; DOE Office of Energy Efficiency and Renewable Energy [DE-AC36-08GO28308] FX This work was supported by the Department of Energy (DOE) BioEnergy Technologies Office (to C.M.P., M.E.H., M.F.C., and G.T.B.). Computational resources were provided by the Argonne Leadership Computing Facility at Argonne National Laboratory supported by the DOE Office of Science under contract DE-AC02-06CH11357, the National Institute for Computational Sciences Kraken cluster under the National Science Foundation Extreme Science and Engineering Discovery Environment (XSEDE) Grant MCB090159, and the National Renewable Energy Laboratory Computational Sciences Center supported by the DOE Office of Energy Efficiency and Renewable Energy under contract DE-AC36-08GO28308. The HjeCel7A free energy calculations and method development were performed under an INCITE allocation. PchCel7D, HirCel7A, MalCel7B, and ThaCel7A free energy calculations were performed with the XSEDE allocation. NR 96 TC 33 Z9 33 U1 3 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 18 PY 2013 VL 135 IS 50 BP 18831 EP 18839 DI 10.1021/ja407287f PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 278CH UT WOS:000328865100029 PM 24279927 ER PT J AU Robinson, JR Gordon, Z Booth, CH Carroll, PJ Walsh, PJ Schelter, EJ AF Robinson, Jerome R. Gordon, Zachary Booth, Corwin H. Carroll, Patrick J. Walsh, Patrick J. Schelter, Eric J. TI Tuning Reactivity and Electronic Properties through Ligand Reorganization within a Cerium Heterobimetallic Framework SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID 2,2-DISUBSTITUTED TERMINAL EPOXIDES; WATER-OXIDATION CATALYSTS; INNER-SPHERE MECHANISMS; RAY CRYSTAL-STRUCTURES; GAS-SHIFT REACTION; OUTER-SPHERE; TETRAVALENT CERIUM; METAL-COMPLEXES; LEWIS ACIDITY; SOLID-STATE AB Cerium compounds have played vital roles in organic, inorganic, and materials chemistry due to their reversible redox chemistry between trivalent and tetravalent oxidation states. However, attempts to rationally access molecular cerium complexes in both oxidation states have been frustrated by unpredictable reactivity in cerium(III) oxidation chemistry. Such oxidation reactions are limited by steric saturation at the metal ion, which can result in high energy activation barriers for electron transfer. An alternative approach has been realized using a rare earth/alkali metal/1,1'-BINOLate (REMB) heterobimetallic framework, which uses redox-inactive metals within the secondary coordination sphere to control ligand reorganization. The rational syntheses of functionalized cerium(IV) products and a mechanistic examination of the role of ligand reorganization in cerium(III) oxidation are presented. C1 [Robinson, Jerome R.; Gordon, Zachary; Carroll, Patrick J.; Walsh, Patrick J.; Schelter, Eric J.] Univ Penn, Dept Chem, P Roy & Diana T Vagelos Labs, Philadelphia, PA 19104 USA. [Booth, Corwin H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Walsh, PJ (reprint author), Univ Penn, Dept Chem, P Roy & Diana T Vagelos Labs, Philadelphia, PA 19104 USA. EM pwalsh@sas.upenn.edu; schelter@sas.upenn.edu FU Penn University Research Foundation; Office of Science (OS), Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX E.J.S. and P.J.W. acknowledge the University of Pennsylvania and the NSF (CHE-1026553 and CHE-0840438 for an X-ray diffractometer). The Penn University Research Foundation is acknowledged for support of the PerkinElmer 950 UV-vis-NIR spectrophotometer. Portions of this work were supported by the Director, Office of Science (OS), Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231, and were carried out at SSRL, a Directorate of SLAC National Accelerator Laboratory and an OS User Facility operated for the DOE OS by Stanford University. NR 140 TC 25 Z9 26 U1 5 U2 105 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 18 PY 2013 VL 135 IS 50 BP 19016 EP 19024 DI 10.1021/ja410688w PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 278CH UT WOS:000328865100049 PM 24274665 ER PT J AU Matveev, KA Furusaki, A AF Matveev, K. A. Furusaki, A. TI Decay of Fermionic Quasiparticles in One-Dimensional Quantum Liquids SO PHYSICAL REVIEW LETTERS LA English DT Article ID LUTTINGER-LIQUID AB The low-energy properties of one-dimensional quantum liquids are commonly described in terms of the Tomonaga-Luttinger liquid theory, in which the elementary excitations are free bosons. To this approximation, the theory can be alternatively recast in terms of free fermions. In both approaches, small perturbations give rise to finite lifetimes of excitations. We evaluate the decay rate of fermionic excitations and show that it scales as the eighth power of energy, in contrast to the much faster decay of bosonic excitations. Our results can be tested experimentally by measuring the broadening of power-law features in the density structure factor or spectral functions. C1 [Matveev, K. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Furusaki, A.] RIKEN, Condensed Matter Theory Lab, Wako, Saitama 3510198, Japan. [Furusaki, A.] RIKEN, CEMS, Wako, Saitama 3510198, Japan. RP Matveev, KA (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Furusaki, Akira/B-3204-2008 OI Furusaki, Akira/0000-0001-8394-0003 FU UChicago Argonne, LLC [DE-AC02-06CH11357]; JSPS KAKENHI [24540338]; RIKEN iTHES Project; National Science Foundation [PHYS-1066293] FX The authors are grateful to L. I. Glazman, M. Pustilnik, and Z. Ristivojevic for helpful discussions. This work was supported by UChicago Argonne, LLC, under Contract No. DE-AC02-06CH11357, by JSPS KAKENHI Grant No. 24540338, and by the RIKEN iTHES Project. Additionally, this work was supported in part by the National Science Foundation under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. NR 21 TC 10 Z9 10 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 18 PY 2013 VL 111 IS 25 AR 256401 DI 10.1103/PhysRevLett.111.256401 PG 4 WC Physics, Multidisciplinary SC Physics GA 278IU UT WOS:000328884000011 PM 24483750 ER PT J AU Oh, J Le, MD Jeong, J Lee, JH Woo, H Song, WY Perring, TG Buyers, WJL Cheong, SW Park, JG AF Oh, Joosung Le, Manh Duc Jeong, Jaehong Lee, Jung-hyun Woo, Hyungje Song, Wan-Young Perring, T. G. Buyers, W. J. L. Cheong, S. -W. Park, Je-Geun TI Magnon Breakdown in a Two Dimensional Triangular Lattice Heisenberg Antiferromagnet of Multiferroic LuMnO3 SO PHYSICAL REVIEW LETTERS LA English DT Article ID QUANTUM SPIN LIQUID; SUPERCONDUCTORS; TRANSITION AB The breakdown of magnons, the quasiparticles of magnetic systems, has rarely been seen. By using an inelastic neutron scattering technique, we report the observation of spontaneous magnon decay in multiferroic LuMnO3, a simple two dimensional Heisenberg triangular lattice antiferromagnet, with large spin S = 2. The origin of this rare phenomenon lies in the nonvanishing cubic interaction between magnons in the spin Hamiltonian arising from the noncollinear 120 degrees spin structure. We observed all three key features of the nonlinear effects as theoretically predicted: a rotonlike minimum, a flat mode, and a linewidth broadening, in our inelastic neutron scattering measurements of single crystal LuMnO3. Our results show that quasiparticles in a system hitherto thought of as "classical" can indeed break down. C1 [Oh, Joosung; Le, Manh Duc; Jeong, Jaehong; Park, Je-Geun] IBS, Ctr Correlated Electron Syst, Seoul 151747, South Korea. [Oh, Joosung; Le, Manh Duc; Jeong, Jaehong; Park, Je-Geun] Seoul Natl Univ, Dept Phys & Astron, Seoul 151747, South Korea. [Lee, Jung-hyun; Song, Wan-Young; Park, Je-Geun] Seoul Natl Univ, Ctr Strongly Correlated Mat Res, Seoul 151747, South Korea. [Lee, Jung-hyun; Song, Wan-Young] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Woo, Hyungje; Perring, T. G.] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Woo, Hyungje] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Buyers, W. J. L.] CNR, Chalk River Labs, Chalk River, ON K0J 1J0, Canada. [Cheong, S. -W.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Cheong, S. -W.] Rutgers State Univ, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA. RP Oh, J (reprint author), IBS, Ctr Correlated Electron Syst, Seoul 151747, South Korea. EM jgpark10@snu.ac.kr RI Park, Je Geun/K-8571-2013; Le, Manh Duc/D-9901-2011 OI Le, Manh Duc/0000-0003-3012-6053 FU Institute for Basic Science (IBS) in Korea; National Research Foundation of Korea [KRF-2008-220-C00012, R17-2008-033-01000-0]; DOE [DE-FG02-07ER46382] FX We thank A. L. Chernyshev, M. E. Zhitomirsky, R. Coldea, T. J. Sato, Y. K. Bang, D. Khomskii, D. C. Peets, H. Jin, and M. Mostovoy for helpful discussions. This work was supported by the Institute for Basic Science (IBS) in Korea. Work at the CSCMR and SKKU was partly supported by the National Research Foundation of Korea (Grants No. KRF-2008-220-C00012 and No. R17-2008-033-01000-0). The work at Rutgers University was supported by the DOE under Grant No. DE-FG02-07ER46382. NR 34 TC 20 Z9 20 U1 1 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 18 PY 2013 VL 111 IS 25 AR 257202 DI 10.1103/PhysRevLett.111.257202 PG 5 WC Physics, Multidisciplinary SC Physics GA 278IU UT WOS:000328884000013 PM 24483753 ER PT J AU Dugger, M Ritchie, BG Collins, P Pasyuk, E Briscoe, WJ Strakovsky, II Workman, RL Azimov, Y Adhikari, KP Adikaram, D Aghasyan, M Amaryan, MJ Anderson, MD Pereira, SA Avakian, H Ball, J Baltzell, NA Battaglieri, M Batourine, V Bedlinskiy, I Biselli, AS Boiarinov, S Burkert, VD Carman, DS Celentano, A Chandavar, S Cole, PL Contalbrigo, M Cortes, O Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Doughty, D Dupre, R Egiyan, H El Alaoui, A El Fassi, L Eugenio, P Fedotov, G Fegan, S Fleming, JA Gevorgyan, N Gilfoyle, GP Giovanetti, KL Girod, FX Goetz, JT Gohn, W Golovatch, E Gothe, RW Griffioen, KA Guidal, M Guo, L Hafidi, K Hakobyan, H Hanretty, C Harrison, N Heddle, D Hicks, K Ho, D Holtrop, M Ilieva, Y Ireland, DG Ishkhanov, BS Isupov, EL Jo, HS Joo, K Keller, D Khandaker, M Kim, W Klein, A Klein, FJ Koirala, S Kubarovsky, A Kubarovsky, V Kuleshov, SV Lewis, S Livingston, K Lu, HY MacGregor, IJD Martinez, D Mayer, M McKinnon, B Mineeva, T Mirazita, M Mokeev, V Montgomery, RA Moutarde, H Munevar, E Camacho, CM Nadel-Turonski, P Nepali, CS Niccolai, S Niculescu, G Niculescu, I Osipenko, M Ostrovidov, AI Pappalardo, LL Paremuzyan, R Park, K Park, S Phelps, E Phillips, JJ Pisano, S Pogorelko, O Pozdniakov, S Price, JW Procureur, S Prok, Y Protopopescu, D Raue, BA Rimal, D Ripani, M Rosner, G Rossi, P Sabatie, F Saini, MS Salgado, C Schott, D Schumacher, RA Seder, E Seraydaryan, H Sharabian, YG Smith, GD Sober, DI Sokhan, D Stepanyan, SS Stoler, P Strauch, S Taiuti, M Tang, W Tian, Y Tkachenko, S Torayev, B Voskanyan, H Voutier, E Walford, NK Watts, DP Weygand, DP Zachariou, N Zana, L Zhang, J Zhao, ZW Zonta, I AF Dugger, M. Ritchie, B. G. Collins, P. Pasyuk, E. Briscoe, W. J. Strakovsky, I. I. Workman, R. L. Azimov, Y. Adhikari, K. P. Adikaram, D. Aghasyan, M. Amaryan, M. J. Anderson, M. D. Pereira, S. Anefalos Avakian, H. Ball, J. Baltzell, N. A. Battaglieri, M. Batourine, V. Bedlinskiy, I. Biselli, A. S. Boiarinov, S. Burkert, V. D. Carman, D. S. Celentano, A. Chandavar, S. Cole, P. L. Contalbrigo, M. Cortes, O. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Doughty, D. Dupre, R. Egiyan, H. El Alaoui, A. El Fassi, L. Eugenio, P. Fedotov, G. Fegan, S. Fleming, J. A. Gevorgyan, N. Gilfoyle, G. P. Giovanetti, K. L. Girod, F. X. Goetz, J. T. Gohn, W. Golovatch, E. Gothe, R. W. Griffioen, K. A. Guidal, M. Guo, L. Hafidi, K. Hakobyan, H. Hanretty, C. Harrison, N. Heddle, D. Hicks, K. Ho, D. Holtrop, M. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Isupov, E. L. Jo, H. S. Joo, K. Keller, D. Khandaker, M. Kim, W. Klein, A. Klein, F. J. Koirala, S. Kubarovsky, A. Kubarovsky, V. Kuleshov, S. V. Lewis, S. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Martinez, D. Mayer, M. McKinnon, B. Mineeva, T. Mirazita, M. Mokeev, V. Montgomery, R. A. Moutarde, H. Munevar, E. Camacho, C. Munoz Nadel-Turonski, P. Nepali, C. S. Niccolai, S. Niculescu, G. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Pappalardo, L. L. Paremuzyan, R. Park, K. Park, S. Phelps, E. Phillips, J. J. Pisano, S. Pogorelko, O. Pozdniakov, S. Price, J. W. Procureur, S. Prok, Y. Protopopescu, D. Raue, B. A. Rimal, D. Ripani, M. Rosner, G. Rossi, P. Sabatie, F. Saini, M. S. Salgado, C. Schott, D. Schumacher, R. A. Seder, E. Seraydaryan, H. Sharabian, Y. G. Smith, G. D. Sober, D. I. Sokhan, D. Stepanyan, S. S. Stoler, P. Strauch, S. Taiuti, M. Tang, W. Tian, Ye Tkachenko, S. Torayev, B. Voskanyan, H. Voutier, E. Walford, N. K. Watts, D. P. Weygand, D. P. Zachariou, N. Zana, L. Zhang, J. Zhao, Z. W. Zonta, I. CA CLAS Collaboration TI Beam asymmetry Sigma for pi(+) and pi(0) photoproduction on the proton for photon energies from 1.102 to 1.862 GeV SO PHYSICAL REVIEW C LA English DT Article ID POSITIVE PION-PHOTOPRODUCTION; RESONANCE REGION; POLARIZED PHOTONS; CROSS-SECTION; PI-0 MESONS; CLAS; PARAMETERS; SYSTEM; PI0 AB Beam asymmetries for the reactions gamma p -> p pi(0) and gamma p -> n pi(+) have been measured with the CEBAF Large Acceptance Spectrometer (CLAS) and a tagged, linearly polarized photon beam with energies from 1.102-1.862 GeV. A Fourier moment technique for extracting beam asymmetries from experimental data is described. The results reported here possess greater precision and finer energy resolution than previous measurements. Our data for both pion reactions appear to favor the SAID and Bonn-Gatchina scattering analyses over the older Mainz MAID predictions. After incorporating the present set of beam asymmetries into the world database, exploratory fits made with the SAID analysis indicate that the largest changes from previous fits are for properties of the Delta(1700)3/2(-) and Delta(1905) 5/2(+) states. C1 [Baltzell, N. A.; El Alaoui, A.; El Fassi, L.; Hafidi, K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Dugger, M.; Ritchie, B. G.; Collins, P.; Pasyuk, E.] Arizona State Univ, Tempe, AZ 85287 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Biselli, A. S.; Ho, D.; Schumacher, R. A.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Klein, F. J.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Ball, J.; Girod, F. X.; Moutarde, H.; Procureur, S.; Sabatie, F.] CEA, Ctr Saclay, Irfu Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Doughty, D.; Heddle, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Gohn, W.; Harrison, N.; Joo, K.; Kubarovsky, A.; Mineeva, T.; Seder, E.] Univ Connecticut, Storrs, CT 06269 USA. [Fleming, J. A.; Watts, D. P.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. Fairfield Univ, Fairfield, CT 06824 USA. [Guo, L.; Raue, B. A.; Rimal, D.] Florida Int Univ, Miami, FL 33199 USA. [Crede, V.; Eugenio, P.; Ostrovidov, A. I.; Park, S.; Saini, M. S.] Florida State Univ, Tallahassee, FL 32306 USA. [Taiuti, M.] Univ Genoa, I-16146 Genoa, Italy. [Briscoe, W. J.; Strakovsky, I. I.; Workman, R. L.; Ilieva, Y.; Nadel-Turonski, P.; Schott, D.; Strauch, S.] George Washington Univ, Washington, DC 20052 USA. [Cole, P. L.; Cortes, O.; Martinez, D.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Pappalardo, L. L.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Aghasyan, M.; Pereira, S. Anefalos; De Sanctis, E.; Mirazita, M.; Pisano, S.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [D'Angelo, A.; Zonta, I.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Dupre, R.; Guidal, M.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.] Inst Phys Nucl ORSAY, Orsay, France. [Bedlinskiy, I.; Kuleshov, S. V.; Pogorelko, O.; Pozdniakov, S.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Giovanetti, K. L.; Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Batourine, V.; Kim, W.; Park, K.; Stepanyan, S. S.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Voutier, E.] Univ Grenoble 1, LPSC, CNRS, IN2P3,INPG, Grenoble, France. [Egiyan, H.; Holtrop, M.; Zana, L.] Univ New Hampshire, Durham, NH 03824 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Chandavar, S.; Goetz, J. T.; Hicks, K.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Adhikari, K. P.; Adikaram, D.; Amaryan, M. J.; Klein, A.; Koirala, S.; Mayer, M.; Nepali, C. S.; Prok, Y.; Seraydaryan, H.; Tkachenko, S.; Torayev, B.; Zhang, J.] Old Dominion Univ, Norfolk, VA 23529 USA. [Azimov, Y.] Petersburg Nucl Phys Inst, Gatchina 188300, Russia. [Kubarovsky, V.; Stoler, P.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Gilfoyle, G. P.] Univ Richmond, Richmond, VA 23173 USA. [D'Angelo, A.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Fedotov, G.; Golovatch, E.; Ishkhanov, B. S.; Isupov, E. L.; Kubarovsky, A.; Mokeev, V.] Skobeltsyn Nucl Phys Inst, Moscow 119899, Russia. [Baltzell, N. A.; Djalali, C.; Fedotov, G.; Gothe, R. W.; Ilieva, Y.; Lu, H. Y.; Phelps, E.; Strauch, S.; Tian, Ye; Zachariou, N.] Univ S Carolina, Columbia, SC 29208 USA. [Avakian, H.; Batourine, V.; Boiarinov, S.; Burkert, V. D.; Carman, D. S.; Deur, A.; Doughty, D.; Egiyan, H.; Girod, F. X.; Guo, L.; Heddle, D.; Kubarovsky, V.; Mokeev, V.; Munevar, E.; Nadel-Turonski, P.; Park, K.; Prok, Y.; Raue, B. A.; Rossi, P.; Sharabian, Y. G.; Weygand, D. P.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Hakobyan, H.; Kuleshov, S. V.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Anderson, M. D.; Ireland, D. G.; Lewis, S.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Montgomery, R. A.; Phillips, J. J.; Protopopescu, D.; Ripani, M.; Rosner, G.; Smith, G. D.; Sokhan, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Hanretty, C.; Keller, D.; Prok, Y.; Tkachenko, S.; Zhao, Z. W.] Univ Virginia, Charlottesville, VA 22901 USA. [Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Dashyan, N.; Gevorgyan, N.; Hakobyan, H.; Paremuzyan, R.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Dugger, M (reprint author), Arizona State Univ, Tempe, AZ 85287 USA. RI Osipenko, Mikhail/N-8292-2015; Zhang, Jixie/A-1461-2016; Adikaram, Dasuni/D-1539-2016; Adikaram, D/H-7128-2016; Celentano, Andrea/J-6190-2012; Schumacher, Reinhard/K-6455-2013; MacGregor, Ian/D-4072-2011; D'Angelo, Annalisa/A-2439-2012; Lu, Haiyun/B-4083-2012; Ireland, David/E-8618-2010; El Alaoui, Ahmed/B-4638-2015; Sabatie, Franck/K-9066-2015 OI Osipenko, Mikhail/0000-0001-9618-3013; Celentano, Andrea/0000-0002-7104-2983; Schumacher, Reinhard/0000-0002-3860-1827; D'Angelo, Annalisa/0000-0003-3050-4907; Ireland, David/0000-0001-7713-7011; Sabatie, Franck/0000-0001-7031-3975 FU National Science Foundation; U.S. Department of Energy (DOE); French Centre National de la Recherche Scientifique; Commissariat a l'Energie Atomique; Italian Istituto Nazionale di Fisica Nucleare; United Kingdom's Science and Technology Facilities Council (STFC); National Research Foundation of Korea; Southeastern Universities Research Association (SURA) operated Jefferson Lab for DOE [DE-AC05-84ER40150] FX The authors gratefully acknowledge the work of the Jefferson Lab Accelerator Division staff. This work was supported by the National Science Foundation, the U.S. Department of Energy (DOE), the French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique, the Italian Istituto Nazionale di Fisica Nucleare, the United Kingdom's Science and Technology Facilities Council (STFC), and the National Research Foundation of Korea. The Southeastern Universities Research Association (SURA) operated Jefferson Lab for DOE under Contract No. DE-AC05-84ER40150 during this work. NR 35 TC 17 Z9 17 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD DEC 18 PY 2013 VL 88 IS 6 AR 065203 DI 10.1103/PhysRevC.88.065203 PG 23 WC Physics, Nuclear SC Physics GA 275PY UT WOS:000328690500003 ER PT J AU Mazzocchi, C Surman, R Grzywacz, R Batchelder, JC Bingham, CR Fong, D Hamilton, JH Hwang, JK Karny, M Krolas, W Liddick, SN Mantica, PF Morton, AC Mueller, WF Rykaczewski, KP Steiner, M Stolz, A Winger, JA Borzov, IN AF Mazzocchi, C. Surman, R. Grzywacz, R. Batchelder, J. C. Bingham, C. R. Fong, D. Hamilton, J. H. Hwang, J. K. Karny, M. Krolas, W. Liddick, S. N. Mantica, P. F. Morton, A. C. Mueller, W. F. Rykaczewski, K. P. Steiner, M. Stolz, A. Winger, J. A. Borzov, I. N. TI New half-lives of very neutron-rich iron isotopes SO PHYSICAL REVIEW C LA English DT Article ID R-PROCESS; NUCLEOSYNTHESIS; NUCLEI AB The beta decay of the most neutron-rich iron isotopes was investigated, leading to the first determination of the Fe-72 half-life and new measurements of the half-lives of Fe69-71. The experimental results are compared with theoretical predictions and presented in the context of the weak astrophysical rapid neutron capture process. C1 [Mazzocchi, C.; Karny, M.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. [Mazzocchi, C.; Grzywacz, R.; Bingham, C. R.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Surman, R.] Union Coll, Dept Phys, Schenectady, NY 12308 USA. [Grzywacz, R.; Bingham, C. R.; Rykaczewski, K. P.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Batchelder, J. C.] UNIRIB Oak Ridge Assoc Univ, Oak Ridge, TN 37831 USA. [Fong, D.; Hamilton, J. H.; Hwang, J. K.] Vanderbilt Univ, Dept Phys, Nashville, TN 37235 USA. [Krolas, W.; Borzov, I. N.] Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. [Krolas, W.] Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland. [Liddick, S. N.; Mantica, P. F.; Morton, A. C.; Mueller, W. F.; Steiner, M.; Stolz, A.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Liddick, S. N.; Mantica, P. F.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Morton, A. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Winger, J. A.] Mississippi State Univ, Dept Phys, Mississippi State, MS 39762 USA. [Borzov, I. N.] Joint Inst Nucl Res, Bogoliubov Lab Theoret Phys, Dubna 141980, Russia. RP Mazzocchi, C (reprint author), Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. EM chiara.mazzocchi@fuw.edu.pl RI Morton, Colin/K-1561-2015; OI Morton, Colin/0000-0003-0214-7551; Hwang, Jae-Kwang/0000-0002-4100-3473 FU Office of Nuclear Physics, US Department of Energy; US DOE [DE-FG02-96ER40983, DE-FG02-05ER41398, DE-AC05-00OR22725, DE-AC05-06OR23100, DE-FG05-88ER40407]; National Nuclear Security Administration [DEFC03-03NA00143]; National Science Foundation [PHY-01-10253, PHY-11-02511]; National Science Center of the Polish Ministry of Science and Higher Education [2011/01/B/ST2/02476]; Helmholtz Alliance EMMI; [IN2P3-RFBR]; [110291054] FX This research is sponsored by the Office of Nuclear Physics, US Department of Energy, and supported under US DOE grants DE-FG02-96ER40983, DE-FG02-05ER41398, DE-AC05-00OR22725, DE-AC05-06OR23100, and DE-FG05-88ER40407; National Nuclear Security Administration Grant No. DEFC03-03NA00143; National Science Foundation Grants PHY-01-10253 and PHY-11-02511; and the National Science Center of the Polish Ministry of Science and Higher Education, Grant No. 2011/01/B/ST2/02476. I. B. is partially supported by the Helmholtz Alliance EMMI and a grant by IN2P3-RFBR under Agreement No. 110291054. NR 17 TC 8 Z9 8 U1 0 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD DEC 18 PY 2013 VL 88 IS 6 AR 064320 DI 10.1103/PhysRevC.88.064320 PG 4 WC Physics, Nuclear SC Physics GA 275PY UT WOS:000328690500001 ER PT J AU Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, Z Masoodi, AA Ahmad, N Ahmed, I Ahn, SA Ahn, SU Aimo, I Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alexandre, D Alici, A Alkin, A Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Andrei, C Andronic, A Anguelov, V Anielski, J Anson, C Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Arend, A Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Asryan, A Augustinus, A Averbeck, R Awes, TC Auml;ysto, J Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, R Baumann, C Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bergognon, AAE Bertens, RA Berzano, D Betev, L Bhasin, A Bhati, AK Bhom, J Bianchi, N Bianchi, L Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Bjelogrlic, S Blanco, F Blanco, F Blau, D Blume, C Boccioli, M Bock, F Bottger, S Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bossu, F Botje, M Botta, E Braidot, E Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brun, R Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Caffarri, D Cai, X Caines, H Caliva, A Villar, EC Camerini, P Roman, VC Romeo, GC Carena, F Carena, W Carlin, NC Carminati, E Diaz, AC Castellanos, JC Hernandez, JFC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JL Chattopadhyay, S Chattopadhyay, S Cherney, M Cheshkov, C Cheynis, B Barroso, VC 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CA ALICE Collaboration TI Multiplicity dependence of the average transverse momentum in pp, p-Pb, and Pb-Pb collisions at the LHC SO PHYSICS LETTERS B LA English DT Article ID PROTON-PROTON COLLISIONS; CHARGED-PARTICLES; 7 TEV; ANGULAR-CORRELATIONS; LONG-RANGE; ROOT-S=0.9; MODEL; SPECTRA; PIONS; KAONS AB The average transverse momentum (p(T)) versus the charged-particle multiplicity N-ch was measured in p-Pb collisions at a collision energy per nucleon-nucleon root S-NN = 5.02 TeV and in pp collisions at collision energies of root s = 0.9, 2.76, and 7 TeV in the kinematic range 0.15 < p(T) < 10.0 GeV/c and vertical bar eta vertical bar < 0.3 with the ALICE apparatus at the LHC. These data are compared to results in Pb-Pb collisions at root S-NN = 2.76 TeV at similar charged-particle multiplicities. In pp and p-Pb collisions, a strong increase of (p(T)) with N-ch is observed, which is much stronger than that measured in Pb-Pb collisions. For pp collisions, this could be attributed, within a model of hadronizing strings, to multiple-parton interactions and to a final-state color reconnection mechanism. The data in p-Pb and Pb-Pb collisions cannot be described by an incoherent superposition of nucleon-nucleon collisions and pose a challenge to most of the event generators. (C) 2013 CERN. Published by Elsevier B.V. All rights reserved. C1 ASRT, Cairo, Egypt. [Grigoryan, A.; Gulkanyan, H.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Cahuantzi, M. Rodriguez; Munoz, G. Tejeda; Vargas, A.; Vergara, S.] Benemerita Univ Autanoma Puebla, Puebla, Mexico. [Alkin, A.; Grinyov, B.; Ivanytskyi, O.; Martynov, Y.; Trubnikov, V.; Zinovjev, G.; Zynovyev, M.] Bogolyubov Inst Theoret Phys, Kiev, Ukraine. [Das, S.] Bose Inst, Dept Phys, Kolkata, India. [Das, S.] CAPSS, Kolkata, India. 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Martinez; Mas, A.; Massacrier, L.; Pillot, R.; Schutz, Y.; Shabetai, A.; Stocco, D.] Univ Nantes, SUBATECH, CNRS, Ecole Mines Nantes,IN2P3, Nantes, France. Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ, Split FESB, Split, Croatia. [Ketzer, B.] Tech Univ Munich, D-80290 Munich, Germany. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Gomez, R.; Kowalski, M.; Matyja, A.; Mayer, C.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Knospe, A. G.; Markert, C.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Carlin Filho, N.; de Barros, G. O. V.; Deppman, A.; Feldkamp, L.; Figueredo, M. A. S.; Jahnke, C.; Fernandes, C. Lagana; Moreira De Godoy, D. A.; Munhoz, M. G.; Oliveira Da Silva, A. C.; De Oliveira Filho, E. Pereira; Suaide, A. A. P.; de Toledo, A. Szanto] Univ Sao Paulo, Sao Paulo, Brazil. [Dash, A.; Takahashi, J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Guilbaud, M.; Tieulent, R.; Uras, A.; Zoccarato, Y.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Bellwied, R.; Blanco, F.; Chinellato, D. D.; Jayarathna, P. H. S. Y.; Madagodahettige-Don, D. M.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.; Weber, M.] Univ Houston, Houston, TX USA. Univ Technol, Vienna, Austria. Austrian Acad Sci, A-1010 Vienna, Austria. [Martashvili, I.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.] Univ Tennessee, Knoxville, TN USA. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Hori, Y.; Ozawa, K.; Torii, H.; Tsuji, T.; Yamaguchi, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Chujo, T.; Esumi, S.; Inaba, M.; Miake, Y.; Sakata, D.; Sano, M.; Watanabe, K.; Watanabe, D.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Hess, B. A.; Schmidt, H. R.; Wiechula, J.] Univ Tubingen, Tubingen, Germany. [Ahammed, Z.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; De, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Langoy, R.; Lien, J.] Vestfold Univ Coll, Tonsberg, Norway. [Altsybeev, I.; Asryan, A.; Feofilov, G.; Ivanov, A.; Kolojvari, A.; Kompaniets, M.; Kondratiev, V.; Kovalenko, V.; Ochirov, A.; Vechernin, V.; Vinogradov, L.; Vorobyev, I.; Zarochentsev, A.; Zadvada, P.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Ostrowski, P.; Pawlak, T.; Peryt, W.; Pluta, J.; Szymanski, M.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Borissov, A.; Cormier, T. M.; Dobrin, A.; Jha, D. M.; Loggins, V. R.; Mlynarz, J.; Pavlinov, A.; Prasad, S. K.; Pruneau, C. A.; Putschke, J.; Verweij, M.; Voloshin, S.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Agocs, A. G.; Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Denes, E.; Hamar, G.; Levai, R.; Molnar, L.; Pochybova, S.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Adare, A. M.; Aronsson, T.; Caines, H.; Connors, M. E.; Harris, J. W.; Hicks, B.; Ma, R.; Oh, S.; Reed, R. J.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. Yildiz Tech Univ, Istanbul, Turkey. [Chang, B.; Kang, J. H.; Kim, B.; Kim, T.; Kim, M.; Kwon, Y.; Moon, T.; Song, M.; Yoon, J.] Yonsei Univ, Seoul, South Korea. [Keidel, R.] Zentrum Technologietransfer & Telekommun ZIT, Fachhsch Worms, Worms, Germany. [Malinina, L.; Zetina, L. Montano] Moscow MV Lomonosov State Univ, DN Skobeltsyn Inst Nucl Phys, Moscow, Russia. RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Ahmed, Ijaz/E-9144-2015; Usai, Gianluca/E-9604-2015; Kovalenko, Vladimir/C-5709-2013; Takahashi, Jun/B-2946-2012; Castillo Castellanos, Javier/G-8915-2013; Bregant, Marco/I-7663-2012; Wagner, Vladimir/G-5650-2014; Sevcenco, Adrian/C-1832-2012; Kucera, Vit/G-8459-2014; Vajzer, Michal/G-8469-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Adamova, Dagmar/G-9789-2014; Barnby, Lee/G-2135-2010; Rui, Rinaldo/L-1926-2015; Nielsen, Borge S/C-3719-2015; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Janik, Malgorzata/O-7520-2015; Graczykowski, Lukasz/O-7522-2015; feofilov, grigory/A-2549-2013; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Salgado, Carlos A./G-2168-2015; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Kompaniets, Mikhail/F-5025-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Zarochentsev, Andrey/J-6253-2013 OI van Leeuwen, Marco/0000-0002-5222-4888; Murray, Sean/0000-0003-0548-588X; Masera, Massimo/0000-0003-1880-5467; Gaardhoje, Jens-Jorgen/0000-0001-6122-4698; Fernandez Tellez, Arturo/0000-0001-5092-9748; Zhou, You/0000-0002-7868-6706; Fiore, Enrichetta Maria/0000-0002-3548-2690; Di Bari, Domenico/0000-0002-5559-8906; Feliciello, Alessandro/0000-0001-5823-9733; Martynov, Yevgen/0000-0003-0753-2205; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; Usai, Gianluca/0000-0002-8659-8378; Kovalenko, Vladimir/0000-0001-6012-6615; Takahashi, Jun/0000-0002-4091-1779; Castillo Castellanos, Javier/0000-0002-5187-2779; Sevcenco, Adrian/0000-0002-4151-1056; Barnby, Lee/0000-0001-7357-9904; Monteno, Marco/0000-0002-3521-6333; Bhasin, Anju/0000-0002-3687-8179; SANTORO, ROMUALDO/0000-0002-4360-4600; Scarlassara, Fernando/0000-0002-4663-8216; Turrisi, Rosario/0000-0002-5272-337X; Beole', Stefania/0000-0003-4673-8038; Scomparin, Enrico/0000-0001-9015-9610; Gago Medina, Alberto Martin/0000-0002-0019-9692; Riggi, Francesco/0000-0002-0030-8377; Dainese, Andrea/0000-0002-2166-1874; Paticchio, Vincenzo/0000-0002-2916-1671; Christiansen, Peter/0000-0001-7066-3473; Lemmon, Roy/0000-0002-1259-979X; Rui, Rinaldo/0000-0002-6993-0332; Virgili, Tiziano/0000-0003-0471-7052; Guerzoni, Barbara/0000-0003-3187-7051; Nielsen, Borge S/0000-0002-0091-1934; Read, Kenneth/0000-0002-3358-7667; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Janik, Malgorzata/0000-0002-3356-3438; feofilov, grigory/0000-0003-3700-8623; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Salgado, Carlos A./0000-0003-4586-2758; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Kompaniets, Mikhail/0000-0001-8831-0553; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Zarochentsev, Andrey/0000-0002-3502-8084 FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP; National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French [CNRS-IN2P3]; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology; Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science and Technology of the Government of Indi; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research - NASR; Autoritatea Nationala pentru Cercetare Stiintifica - ANCS; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN; Cubaenergia; Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio FX The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector:; State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia;; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP);; National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC);; Ministry of Education and Youth of the Czech Republic;; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation;; The European Research Council under the European Community's Seventh Framework Programme;; Helsinki Institute of Physics and the Academy of Finland;; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne and CEA, France;; German BMBF and the Helmholtz Association;; General Secretariat for Research and Technology, Ministry of Development, Greece;; Hungarian OTKA and National Office for Research and Technology (NKTH);; Department of Atomic Energy and Department of Science and Technology of the Government of India;; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy;; MEXT Grant-in-Aid for Specially Promoted Research, Japan;; Joint Institute for Nuclear Research, Dubna;; National Research Foundation of Korea (NRF);; CONACYT, DGAPA, Mexico, ALFA-EC and the EPLANET Program (European Particle Physics Latin American Network);; Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands;; Research Council of Norway (NFR);; Polish Ministry of Science and Higher Education;; National Authority for Scientific Research - NASR (Autoritatea Nationala pentru Cercetare Stiintifica - ANCS);; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and the Russian Foundation for Basic Research;; Ministry of Education of Slovakia;; Department of Science and Technology, South Africa;; CIEMAT, EELA, Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency);; Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW);; Ukraine Ministry of Education and Science;; United Kingdom Science and Technology Facilities Council (STFC);; The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 56 TC 63 Z9 63 U1 3 U2 94 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD DEC 18 PY 2013 VL 727 IS 4-5 BP 371 EP 380 DI 10.1016/j.physletb.2013.10.054 PG 10 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 276BG UT WOS:000328722500005 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruehwirth, R Ghete, VM Hormann, N Hrubec, J Jeitlerl, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, R Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, R Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, R Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, R Lemaitre, V Liao, J Militaru, . Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Aida, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Laydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, X Wang, Z Xiao, H Asawatangtrakuldee, C Ban, Y Guo, Y Li, W Liu, S Mao, Y Qian, SJ Teng, H Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Awad, AMK Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M Baffloni, S Beaudette, F Benhabib, L Bluj, M Busson, R Chariot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, R Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C 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Swanson, J. CA CMS Collaboration TI Measurement of the prompt J/psi and psi(2S) polarizations in pp collisions at root s=7 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; Quarkonium production; Quarkonium polarization ID HEAVY-QUARKONIUM AB The polarizations of prompt J/psi and psi(2S) mesons are measured in proton-proton collisions at root s = 7 TeV, using a dimuon data sample collected by the CMS experiment at the LHC, corresponding to an integrated luminosity of 4.9 fb(-1). The prompt J/psi and psi(2S) polarization parameters lambda, lambda, and lambda, as well as the frame-invariant quantity (lambda) over bar. are measured from the dimuon decay angular distributions in three different polarization frames. The J/psi results are obtained in the transverse momentum range 14 < P-T < 70 GeV, in the rapidity intervals |y| < 0.6 and 0.6 < |y| < 1.2. The corresponding psi(2S) results cover 14 < PT < 50 GeV and include a third rapidity bin, 1.2 < |y| < 1.5. 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[Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, Ks.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Moreno, S. Carrillo; Valencia, F. Vazquez] Univ lberoamericana, Mexico City, DF, Mexico. [Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Linares, E. Casimiro; Pineda, A. Morelos; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, R.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Almeida, N.; Bargassa, R.; Beirao, C.; Silva, Da Cruz E.; Faccioli, R.; Parracho, P. G. Ferreira; Gallinaro, M.; Nguyen, R.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Laney, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, S.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, E.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, R.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, R. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tiuscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, R.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Liyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. k.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Canner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, R.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; One, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, R.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, R.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Loveless, R.; Mohapatra, A.; Mozer, M. U.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. 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M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. 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RI Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Leonidov, Andrey/P-3197-2014; 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Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Dahms, Torsten/0000-0003-4274-5476; Montanari, Alessandro/0000-0003-2748-6373; Moon, Chang-Seong/0000-0001-8229-7829; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Novaes, Sergio/0000-0003-0471-8549; Codispoti, Giuseppe/0000-0003-0217-7021; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland; MEC; HIP (Finland); CEA; CNRS/IN2P3 (France); BMBF; DFG; HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea; WCU (Republic of Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU; Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain);.Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 28 TC 50 Z9 50 U1 4 U2 142 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD DEC 18 PY 2013 VL 727 IS 4-5 BP 381 EP 402 DI 10.1016/j.physletb.2013.10.055 PG 22 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 276BG UT WOS:000328722500006 ER PT J AU Zhu, RL Sun, P Yuan, F AF Zhu, Ruilin Sun, Peng Yuan, Feng TI Low transverse momentum heavy quark pair production to probe gluon tomography SO PHYSICS LETTERS B LA English DT Article ID QCD; SCATTERING; ELECTROPRODUCTION; PHOTOPRODUCTION AB We derive the transverse momentum dependent (TMD) factorization for heavy quark pair production in deep inelastic scattering, where the total transverse momentum is much smaller than the invariant mass of the pair. The factorization is demonstrated at one-loop order, in both Ji-Ma-Yuan and Collins-11 schemes for the TMD definitions, and the hard factors are calculated accordingly. Our result provides a solid theoretical foundation for the phenomenological investigations of the gluon TMDs in this process, and can be extended to other similar hard processes, including di-jet (di-hadron) production in DIS. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zhu, Ruilin] Univ Chinese Acad Sci, Sch Phys, Beijing, Peoples R China. [Zhu, Ruilin; Sun, Peng; Yuan, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Zhu, RL (reprint author), Univ Chinese Acad Sci, Sch Phys, Beijing, Peoples R China. RI Yuan, Feng/N-4175-2013; Zhu, Rui-Lin/L-6440-2016 OI Zhu, Rui-Lin/0000-0001-6733-859X FU China Scholarship Council; U.S. Department of Energy [DE-AC02-05CH11231] FX We thank L Yang for discussions concerning the results in Ref. [17]. R.Z. particularly thanks Prof. C.F. Qiao for discussions, and he is partially supported by China Scholarship Council. This work was partially supported by the U.S. Department of Energy via grant DE-AC02-05CH11231. NR 23 TC 11 Z9 11 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD DEC 18 PY 2013 VL 727 IS 4-5 BP 474 EP 479 DI 10.1016/j.physletb.2013.11.002 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 276BG UT WOS:000328722500019 ER PT J AU Barbagallo, M Guerrero, C Tsinganis, A Tarrio, D Altstadt, S Andriamonje, S Andrzejewski, J Audouin, L Becares, V Becvar, F Belloni, F Berthoumieux, E Billowes, J Boccone, V Bosnar, D Brugger, M Calviani, M Calvino, F Cano-Ott, D Carrapico, C Cerutti, F Chiaveri, E Chin, M Colonna, N Cortes, G Cortes-Giraldo, MA Diakaki, M Domingo-Pardo, C Duran, I Dressler, R Dzysiuk, N Eleftheriadis, C Ferrari, A Fraval, K Ganesan, S Garcia, AR Giubrone, G Gobel, K Gomez-Hornillos, MB Goncalves, IF Gonzalez-Romero, E Griesmayer, E Gunsing, F Gurusamy, P Hernandez-Prieto, A Jenkins, DG Jericha, E Kadi, Y Kappeler, F Karadimos, D Kivel, N Koehler, P Kokkoris, M Krticka, M Kroll, J Lampoudis, C Langer, C Leal-Cidoncha, E Lederer, C Leeb, H Leong, LS Losito, R Manousos, A Marganiec, J Martinez, T Massimi, C Mastinu, PF Mastromarco, M Meaze, M Mendoza, E Mengoni, A Milazzo, PM Mingrone, F Mirea, M Mondalaers, W Papaevangelou, T Paradela, C Pavlik, A Perkowski, J Plompen, A Praena, J Quesada, JM Rauscher, T Reifarth, R Riego, A Roman, F Rubbia, C Sabate-Gilarte, M Sarmento, R Saxena, A Schillebeeckx, P Schmidt, S Schumann, D Steinegger, P Tagliente, G Tain, JL Tassan-Got, L Valenta, S Vannini, G Variale, V Vaz, P Ventura, A Versaci, R Vermeulen, MJ Vlachoudis, V Vlastou, R Wallner, A Ware, T Weigand, M Weiss, C Wright, T Zugec, P AF Barbagallo, M. Guerrero, C. Tsinganis, A. Tarrio, D. Altstadt, S. Andriamonje, S. Andrzejewski, J. Audouin, L. Becares, V. Becvar, F. Belloni, F. Berthoumieux, E. Billowes, J. Boccone, V. Bosnar, D. Brugger, M. Calviani, M. Calvino, F. Cano-Ott, D. Carrapico, C. Cerutti, F. Chiaveri, E. Chin, M. Colonna, N. Cortes, G. Cortes-Giraldo, M. A. Diakaki, M. Domingo-Pardo, C. Duran, I. Dressler, R. Dzysiuk, N. Eleftheriadis, C. Ferrari, A. Fraval, K. Ganesan, S. Garcia, A. R. Giubrone, G. Goebel, K. Gomez-Hornillos, M. B. Goncalves, I. F. Gonzalez-Romero, E. Griesmayer, E. Gunsing, F. Gurusamy, P. Hernandez-Prieto, A. Jenkins, D. G. Jericha, E. Kadi, Y. Kaeppeler, F. Karadimos, D. Kivel, N. Koehler, P. Kokkoris, M. Krticka, M. Kroll, J. Lampoudis, C. Langer, C. Leal-Cidoncha, E. Lederer, C. Leeb, H. Leong, L. S. Losito, R. Manousos, A. Marganiec, J. Martinez, T. Massimi, C. Mastinu, P. F. Mastromarco, M. Meaze, M. Mendoza, E. Mengoni, A. Milazzo, P. M. Mingrone, F. Mirea, M. Mondalaers, W. Papaevangelou, T. Paradela, C. Pavlik, A. Perkowski, J. Plompen, A. Praena, J. Quesada, J. M. Rauscher, T. Reifarth, R. Riego, A. Roman, F. Rubbia, C. Sabate-Gilarte, M. Sarmento, R. Saxena, A. Schillebeeckx, P. Schmidt, S. Schumann, D. Steinegger, P. Tagliente, G. Tain, J. L. Tassan-Got, L. Valenta, S. Vannini, G. Variale, V. Vaz, P. Ventura, A. Versaci, R. Vermeulen, M. J. Vlachoudis, V. Vlastou, R. Wallner, A. Ware, T. Weigand, M. Weiss, C. Wright, T. Zugec, P. TI High-accuracy determination of the neutron flux at n_TOF SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID FACILITY; CERN; STANDARDS; SCIENCE; BEAM AB The neutron flux of the n_TOF facility at CERN was measured, after installation of the new spallation target, with four different systems based on three neutron-converting reactions, which represent accepted cross sections standards in different energy regions. A careful comparison and combination of the different measurements allowed us to reach an unprecedented accuracy on the energy dependence of the neutron flux in the very wide range (thermal to 1 GeV) that characterizes the n_TOF neutron beam. This is a pre-requisite for the high accuracy of cross section measurements at n_TOF. An unexpected anomaly in the neutron-induced fission cross section of U-235 is observed in the energy region between 10 and 30keV, hinting at a possible overestimation of this important cross section, well above currently assigned uncertainties. C1 [Barbagallo, M.; Colonna, N.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, I-70125 Bari, Italy. [Guerrero, C.; Tsinganis, A.; Andriamonje, S.; Berthoumieux, E.; Boccone, V.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Ferrari, A.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Manousos, A.; Roman, F.; Rubbia, C.; Versaci, R.; Vlachoudis, V.; Weiss, C.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Tsinganis, A.; Diakaki, M.; Karadimos, D.; Kokkoris, M.; Vlastou, R.] Natl Tech Univ Athens, GR-10682 Athens, Greece. [Tarrio, D.; Duran, I.; Leal-Cidoncha, E.; Paradela, C.] Univ Santiago de Compostela, Santiago De Compostela, Spain. [Altstadt, S.; Goebel, K.; Langer, C.; Lederer, C.; Reifarth, R.; Schmidt, S.; Weigand, M.; Weiss, C.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Andrzejewski, J.; Marganiec, J.; Perkowski, J.] Uniwersytet Lodzki, Lodz, Poland. [Audouin, L.; Leong, L. S.; Tassan-Got, L.] CNRS, IN2P3, IPN, F-91405 Orsay, France. [Becares, V.; Cano-Ott, D.; Garcia, A. R.; Gonzalez-Romero, E.; Martinez, T.; Mendoza, E.] CIEMAT, E-28040 Madrid, Spain. [Becvar, F.; Krticka, M.; Kroll, J.; Valenta, S.] Charles Univ Prague, Prague, Czech Republic. [Belloni, F.; Berthoumieux, E.; Chiaveri, E.; Fraval, K.; Gunsing, F.; Lampoudis, C.; Papaevangelou, T.] CEA Saclay, F-91191 Gif Sur Yvette, France. [Billowes, J.; Ware, T.; Wright, T.] Univ Manchester, Manchester, Lancs, England. [Bosnar, D.; Zugec, P.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia. [Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Hernandez-Prieto, A.; Riego, A.] Univ Politecn Cataluna, Barcelona, Spain. [Carrapico, C.; Goncalves, I. F.; Sarmento, R.; Vaz, P.] Univ Tecn Lisboa, Inst Super Tecn, Inst Tecnol & Nucl, P-1096 Lisbon, Portugal. [Cortes-Giraldo, M. A.; Praena, J.; Quesada, J. M.; Sabate-Gilarte, M.] Univ Seville, Seville, Spain. [Domingo-Pardo, C.; Giubrone, G.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46003 Valencia, Spain. [Dressler, R.; Kivel, N.; Schumann, D.; Steinegger, P.] Paul Scherrer Inst, Villigen, Switzerland. [Dzysiuk, N.; Mastinu, P. F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Eleftheriadis, C.; Manousos, A.] Aristotle Univ Thessaloniki, GR-54006 Thessaloniki, Greece. [Ganesan, S.; Gurusamy, P.; Saxena, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Griesmayer, E.; Jericha, E.; Leeb, H.] Vienna Univ Technol, Atominst, Vienna, Austria. [Jenkins, D. G.; Vermeulen, M. J.] Univ York, York YO10 5DD, N Yorkshire, England. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Lederer, C.; Pavlik, A.; Wallner, A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Lederer, C.; Pavlik, A.; Wallner, A.] Univ Vienna, Fac Phys, A-1010 Vienna, Austria. [Massimi, C.; Mingrone, F.; Vannini, G.] Univ Bologna, Dipartimento Fis, I-40126 Bologna, Italy. [Massimi, C.; Mingrone, F.; Vannini, G.] Ist Nazl Fis Nucl, Sez Bologna, Milan, Italy. [Mengoni, A.; Ventura, A.] Agenzia Nazl Nuove tecnol Energia & Sviluppo Econ, Bologna, Italy. [Milazzo, P. M.] Ist Nazl Fis Nucl, Sez Trieste, Milan, Italy. [Mirea, M.; Roman, F.] Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HH, Bucharest, Romania. [Mondalaers, W.; Plompen, A.; Schillebeeckx, P.] European Commiss JRC, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rubbia, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. RP Barbagallo, M (reprint author), Ist Nazl Fis Nucl, Sez Bari, V Orabona 4, I-70125 Bari, Italy. EM massimo.barbagallo@ba.infn.it RI Guerrero, Carlos/L-3251-2014; Gonzalez Romero, Enrique/L-7561-2014; Martinez, Trinitario/K-6785-2014; Massimi, Cristian/B-2401-2015; Duran, Ignacio/H-7254-2015; Massimi, Cristian/K-2008-2015; Paradela, Carlos/J-1492-2012; Wallner, Anton/G-1480-2011; Papaevangelou, Thomas/G-2482-2016; Gobel, Kathrin/B-8531-2016; Langer, Christoph/L-3422-2016; Calvino, Francisco/K-5743-2014; Quesada Molina, Jose Manuel/K-5267-2014; Mendoza Cembranos, Emilio/K-5789-2014; Cortes-Giraldo, Miguel Antonio/K-6031-2014; Mirea, Mihail/C-2297-2011; Rauscher, Thomas/D-2086-2009; Vaz, Pedro/K-2464-2013; Langer, Christoph/D-5490-2014; Chin, Mary Pik Wai/B-6644-2012; Steinegger, Patrick/M-5531-2013; Versaci, Roberto/G-8577-2014; Tain, Jose L./K-2492-2014; Becares, Vicente/K-4514-2014; Cano Ott, Daniel/K-4945-2014; Mengoni, Alberto/I-1497-2012; Jericha, Erwin/A-4094-2011; OI Guerrero, Carlos/0000-0002-2111-546X; Gonzalez Romero, Enrique/0000-0003-2376-8920; Martinez, Trinitario/0000-0002-0683-5506; Massimi, Cristian/0000-0001-9792-3722; Massimi, Cristian/0000-0003-2499-5586; Wallner, Anton/0000-0003-2804-3670; Papaevangelou, Thomas/0000-0003-2829-9158; Gobel, Kathrin/0000-0003-2832-8465; Calvino, Francisco/0000-0002-7198-4639; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mendoza Cembranos, Emilio/0000-0002-2843-1801; Cortes-Giraldo, Miguel Antonio/0000-0002-3646-1015; Mirea, Mihail/0000-0002-9333-6595; Rauscher, Thomas/0000-0002-1266-0642; Vaz, Pedro/0000-0002-7186-2359; Chin, Mary Pik Wai/0000-0001-5176-9723; Steinegger, Patrick/0000-0002-5054-0924; Becares, Vicente/0000-0003-3434-9086; Cano Ott, Daniel/0000-0002-9568-7508; Koehler, Paul/0000-0002-6717-0771; Domingo-Pardo, Cesar/0000-0002-2915-5466; Tarrio, Diego/0000-0002-9858-3341; Mengoni, Alberto/0000-0002-2537-0038; Sarmento, Raul/0000-0002-5018-5467; Jericha, Erwin/0000-0002-8663-0526; Pavlik, Andreas/0000-0001-7526-3372; Paradela Dobarro, Carlos/0000-0003-0175-8334; Garcia Rios, Aczel Regino/0000-0002-7955-1475 FU European Commission [FP7-249671] FX The authors are indebted to the national and international funding agencies that have supported the n_TOF Collaboration. This work is also supported by the European Commission with the FP7 project ANDES (FP7-249671). Furthermore, the measurements with the PTB detector would not have been possible without the support from the Physikalisch-Technische Bundesanstalt Institute, particularly from Ralf Nolte and Marita Mosconi who helped in installing and using the detector at n_TOF. NR 26 TC 17 Z9 18 U1 3 U2 43 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD DEC 18 PY 2013 VL 49 IS 12 BP 1 EP 11 AR UNSP 156 DI 10.1140/epja/i2013-13156-x PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 270WW UT WOS:000328351000001 ER PT J AU Sarkar, A Sun, X Sundaresan, S AF Sarkar, Avik Sun, Xin Sundaresan, Sankaran TI Sub-grid drag models for horizontal cylinder arrays immersed in gas-particle multiphase flows SO CHEMICAL ENGINEERING SCIENCE LA English DT Article DE Computational fluid dynamics (CFD); Cylinders; Filtered models; Fluidization; Multiphase flow; Multiscale ID FILTERED 2-FLUID MODELS; SOLID FLUIDIZED-BEDS; GRANULAR FLOW; KINETIC-THEORY; TUBE BUNDLE; SIMULATIONS AB Immersed cylindrical tube arrays often are used as heat exchangers in gas-particle fluidized beds. In multiphase computational fluid dynamics (CFD) simulations of large fluidized beds, explicit resolution of small cylinders is computationally infeasible. Instead, the cylinder array may be viewed as an effective porous medium in coarse-grid simulations. The cylinders' influence on the suspension as a whole, manifested as an effective drag force, and on the relative motion between gas and particles, manifested as a correction to the gas-particle drag, must be modeled via suitable sub-grid constitutive relationships. In this work, highly-resolved unit-cell simulations of flow around an array of horizontal cylinders, arranged in a staggered configuration, are filtered to construct sub-grid, or 'filtered', drag models, which can be implemented in coarse-grid simulations. The force on the suspension exerted by the cylinders is composed of, as expected, a buoyancy contribution, and a kinetic component analogous to fluid drag on a single cylinder. Furthermore, the introduction of tubes also is found to enhance segregation at the scale of the cylinder size, which, in turn, leads to a reduction in the filtered gas-particle drag. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Sarkar, Avik; Sun, Xin] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Sundaresan, Sankaran] Princeton Univ, Dept Chem & Biol Engn, Princeton, NJ 08544 USA. RP Sarkar, A (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, POB 999,MSIN K7-90, Richland, WA 99352 USA. EM avik.sarkar@pnnl.gov FU U.S. Department of Energy, Office of Fossil Energy's Carbon Capture Simulation Initiative (CCSI) through the National Energy Technology Laboratory FX This work was funded by the U.S. Department of Energy, Office of Fossil Energy's Carbon Capture Simulation Initiative (CCSI) through the National Energy Technology Laboratory. NR 29 TC 10 Z9 10 U1 3 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0009-2509 EI 1873-4405 J9 CHEM ENG SCI JI Chem. Eng. Sci. PD DEC 18 PY 2013 VL 104 BP 399 EP 412 DI 10.1016/j.ces.2013.08.050 PG 14 WC Engineering, Chemical SC Engineering GA 262LE UT WOS:000327735900037 ER PT J AU Xing, R Rao, YX TeGrotenhuis, W Canfield, N Zheng, F Winiarski, DW Liu, W AF Xing, Rong Rao, Yuxiang TeGrotenhuis, Ward Canfield, Nathan Zheng, Feng Winiarski, David W. Liu, Wei TI Advanced thin zeolite/metal flat sheet membrane for energy efficient air dehumidification and conditioning SO CHEMICAL ENGINEERING SCIENCE LA English DT Article DE Zeolite membrane; Metal sheet; Dehumidification; Gas drying; Air conditioning; Energy efficiency ID WATER TRANSPORT-PROPERTIES; NAFION MEMBRANES; GAS SEPARATION; PERVAPORATION; SYSTEM; MODULE; PERMEATION; CONTACTOR; MIXTURES; SURFACE AB Air conditioning consumes a very large amount of electricity globally. Energy efficiency of the conventional vapor compression cooling is low in warm and humid climates due to water condensation. Membrane separation is viewed as one efficient process for air dehumidification. In this paper, we report the development of a novel thin flat sheet zeolite membrane for the air dehumidification application. The membrane is prepared by deposition of an ultra-thin H2O-selective zeolite membrane film (similar to 3 mu m) on a thin (similar to 50 mu m) porous metal sheet support. Under separation temperature of 32 degrees C and feed air relative humidity (RH) of 90%, a quality membrane shows water permeance as high as 6.8 x 10(-6) mol m(-2) Pa-1 s(-1), which is about 1 to 3 orders of magnitude higher than the previously reported in the literature, and a water vapor/air separation factor over 300. In addition, this zeolite/metal thin-sheet membrane exhibits excellent stability as no apparent decline of separation performances is observed during 8-day continuous testing with humid in-house air. To simulate various climate conditions, the membrane is tested over a range of separation conditions which include temperature, feed air RH, and permeate pressure, It is estimated that 50% or higher energy efficiency gain over the conventional vapor compression system can be obtained when the membrane separation factor is above 200. The results suggest the possibility to develop an on-line, compact membrane dehumidifier for significant enhancement of air conditioning energy efficiency. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Xing, Rong; Rao, Yuxiang; TeGrotenhuis, Ward; Canfield, Nathan; Zheng, Feng; Winiarski, David W.; Liu, Wei] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. RP Liu, W (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99354 USA. EM Wei.Liu@pnnl.gov RI Zheng, Feng/C-7678-2009 OI Zheng, Feng/0000-0002-5427-1303 FU Advanced Research Project Association-Energy (ARPA-E) [DE-AR0000138] FX This work has been financially supported by the Advanced Research Project Association-Energy (ARPA-E) under the Grant DE-AR0000138. We would like to thank our industrial partner, ADMA Products, Inc, and collaborator, Energy Science Laboratory of Texas AM University, for their contribution to this project. We also thank our colleague at PNNL, Dr. Cheng Huang, for his help with initial setup of membrane characterization testing apparatus. NR 44 TC 10 Z9 10 U1 4 U2 47 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0009-2509 EI 1873-4405 J9 CHEM ENG SCI JI Chem. Eng. Sci. PD DEC 18 PY 2013 VL 104 BP 596 EP 609 DI 10.1016/j.ces.2013.08.061 PG 14 WC Engineering, Chemical SC Engineering GA 262LE UT WOS:000327735900053 ER PT J AU Dervishi, E Hategekimana, F Boyer, L Watanabe, F Mustafa, T Biswas, A Biris, AR Biris, AS AF Dervishi, Enkeleda Hategekimana, Festus Boyer, Laurent Watanabe, Fumiya Mustafa, Thikra Biswas, Abhijit Biris, Alexandru R. Biris, Alexandru S. TI The effect of carbon nanotubes and graphene on the mechanical properties of multi-component polymeric composites SO CHEMICAL PHYSICS LETTERS LA English DT Article ID ELASTIC PROPERTIES; STRENGTH; SYSTEM; SPECTROSCOPY; NANOSHEETS; GROWTH; CELLS AB Two types of nano-materials (nanotubes and graphene) were incorporated at different concentrations into a bio-compatible polymer matrix, and the mechanical properties of the composite films were studied. Although both nanomaterials improved the mechanical attributes of the polymer, it was found that the composites containing the nanotube-graphene mixture exhibited significantly superior elasto-plastic properties. This work presents a facile technique of fabricating nano-composites that could be scaled up and applied to various types of polymers. These multi-component films have the potential to be used in a wide range of applications including bio-medicine and photovoltaics, as well as the military and automotive industry. (C) 2013 Elsevier B. V. All rights reserved. C1 [Dervishi, Enkeleda; Hategekimana, Festus; Watanabe, Fumiya; Mustafa, Thikra; Biris, Alexandru S.] Univ Arkansas, Ctr Integrat Nanotechnol Sci, Little Rock, AR 72204 USA. [Boyer, Laurent] Sch Engn, Ctr Ind Higher Educ, F-62000 Arras, France. [Biswas, Abhijit] Univ Notre Dame, Dept Elect Engn, Ctr Nanosci & Technol NDnano, Notre Dame, IN 46556 USA. [Biris, Alexandru R.] Natl Inst Res & Dev Isotop & Mol Technol, Cluj Napoca, Romania. RP Dervishi, E (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87544 USA. EM exdervishi@gmail.com; Abhijit.Biswas.5@nd.edu; alexandru.biris@itimcj.ro; asbiris@ualr.edu FU Arkansas Science & Technology Authority [08-CAT-03]; Department of Energy [DE-FG36-06GO86072]; National Science Foundation [NSF/EPS-1003970] FX Financial support from the Arkansas Science & Technology Authority (Grant # 08-CAT-03), and the Department of Energy (DE-FG36-06GO86072) and National Science Foundation (NSF/EPS-1003970) is greatly appreciated. The editorial assistance of Dr. Marinelle Ringer is also acknowledged. NR 34 TC 6 Z9 6 U1 2 U2 46 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD DEC 18 PY 2013 VL 590 BP 126 EP 130 DI 10.1016/j.cplett.2013.10.060 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262FZ UT WOS:000327721000023 ER PT J AU Nelson, T Fernandez-Alberti, S Roitberg, AE Tretiak, S AF Nelson, Tammie Fernandez-Alberti, Sebastian Roitberg, Adrian E. Tretiak, Sergei TI Artifacts due to trivial unavoided crossings in the modeling of photoinduced energy transfer dynamics in extended conjugated molecules SO CHEMICAL PHYSICS LETTERS LA English DT Article ID OPTICAL-EXCITATIONS; VITREOUS SILICA; LOCALIZATION; SPECTROSCOPY; SIMULATIONS; TEMPERATURE; DENDRIMERS; VIBRATIONS; COHERENCE AB A previously developed algorithm to identify potential energy surface crossings involving interacting or noninteracting states during nonadiabatic excited-state molecular dynamics simulations, allows the diabatic pathway to be followed through the crossing region so that there is no experienced change in the states identity. In this Letter, we investigate the transition from interacting/delocalized states to noninteracting/localized states in oligomers of poly-phenylene vinylene separated by varying distances. We demonstrate that the appearance of trivial unavoided crossings during nonadiabatic dynamics leads to artifacts in the state population analysis. Consequently, changes in the localization of the electronic transition density must be followed instead. (C) 2013 Elsevier B. V. All rights reserved. C1 [Nelson, Tammie; Tretiak, Sergei] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies CNLS, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. [Fernandez-Alberti, Sebastian] Univ Nacl Quilmes, Bernal, Argentina. [Roitberg, Adrian E.] Univ Florida, Dept Phys, Quantum Theory Project, Gainesville, FL 32611 USA. [Roitberg, Adrian E.] Univ Florida, Dept Chem, Quantum Theory Project, Gainesville, FL 32611 USA. RP Tretiak, S (reprint author), Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies CNLS, Ctr Integrated Nanotechnol CINT, POB 1663, Los Alamos, NM 87545 USA. EM serg@lanl.gov RI Tretiak, Sergei/B-5556-2009; Roitberg, Adrian/A-2378-2009 OI Tretiak, Sergei/0000-0001-5547-3647; FU Directed Research and Development Fund at Los Alamos National Laboratory (LANL); CONICET; UNQ; ANPCIT [PICT-2010-2375]; NSF [CHE-0239120, CHE-0808910]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; Center for Integrated Nanotechnology (CINT); Center for Nonlinear Studies (CNLS) FX T. N. and S. T. acknowledge support of Directed Research and Development Fund at Los Alamos National Laboratory (LANL). A. E. R and S. F.-A. acknowledge supported from CONICET, UNQ, ANPCIT (PICT-2010-2375), NSF Grants CHE-0239120 and CHE-0808910. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. We acknowledge support of Center for Integrated Nanotechnology (CINT) and Center for Nonlinear Studies (CNLS). NR 36 TC 14 Z9 14 U1 0 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD DEC 18 PY 2013 VL 590 BP 208 EP 213 DI 10.1016/j.cplett.2013.10.052 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262FZ UT WOS:000327721000039 ER PT J AU Smith, ME Knauss, KG Higgins, SR AF Smith, Michael E. Knauss, Kevin G. Higgins, Steven R. TI Effects of crystal orientation on the dissolution of calcite by chemical and microscopic analysis SO CHEMICAL GEOLOGY LA English DT Article DE Calcite; Surface chemistry; Surface morphology; Dissolution; Atomic force microscopy; Vertical scanning interferometry ID ATOMIC-FORCE-MICROSCOPY; MINERAL DISSOLUTION; SURFACE-MORPHOLOGY; CO2 SEQUESTRATION; SATURATION STATE; RATE LAWS; KINETICS; GROWTH; RATES; CARBONATE AB The purpose of this work was to examine the effects of polished crystal-surface orientation and degree of solution under saturation on the dissolution kinetics of calcite. Crystallographic surface orientations utilized in this study included natural calcite specimens polished approximately parallel to the (104) plane, giving rise to surfaces with flat terraces with few steps, as well as fully kinked surfaces created by sectioning approximately parallel to the (001) plane. Results from inductively coupled plasma optical emission spectroscopy (ICP-OES) and vertical scanning interferometry (VSI) investigations revealed how crystallographic orientations of calcite with initially higher energy surface morphologies were associated with greater extent of reaction, greater surface retreat, and therefore, greater initial transient dissolution rates than those with lower energy initial surface morphologies. However, both the ICP-OES and atomic force microscopy(AFM) results confirm that the effects of crystal orientation become minimal under long-term conditions because (1) variously oriented calcite surfaces exhibited similar "long-term" rates and (2) orientations with high initial reactive site densities developed lower energy morphologies. Estimating a step rate coefficient from the experimental data from a miscut sample suggest that these coefficients may be highly morphology dependent. Results from this study are significant for predicting long term calcite dissolution rates because they suggest that the "long-term" dissolution rate of calcite will be governed by the rates of the rhombohedral faces and microfacets and the time-scale for approaching such conditions is of the order of days at room temperature and slightly alkaline solution conditions. (C) 2013 Elsevier B. V. All rights reserved. C1 [Smith, Michael E.; Higgins, Steven R.] Wright State Univ, Dept Chem, Dayton, OH 45435 USA. [Knauss, Kevin G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Higgins, SR (reprint author), Wright State Univ, Dept Chem, 3640 Colonel Glenn Highway, Dayton, OH 45435 USA. EM steven.higgins@wright.edu FU United States Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division; Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was funded by the United States Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division. The LBL work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors wish to acknowledge Weifu Fang for his generous assistance with deriving the sample tilt parameters for the c-plane samples, and David A. Dolson and Ioana E. Sizemore for their editorial help during the writing of this manuscript. The ICP-OES technical support of Garrett VanNess is also gratefully acknowledged. NR 48 TC 9 Z9 9 U1 5 U2 54 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD DEC 18 PY 2013 VL 360 BP 10 EP 21 DI 10.1016/j.chemgeo.2013.09.015 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 259MX UT WOS:000327532100002 ER PT J AU Lu, ZF Streets, DG de Foy, B Krotkov, NA AF Lu, Zifeng Streets, David G. de Foy, Benjamin Krotkov, Nickolay A. TI Ozone Monitoring Instrument Observations of Interannual Increases in SO2 Emissions from Indian Coal-Fired Power Plants during 2005-2012 SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SULFUR-DIOXIDE EMISSIONS; NOX EMISSIONS; CHINA; RETRIEVALS; INVENTORY; AEROSOLS; TRENDS; ASIA; OMI AB Due to the rapid growth of electricity demand and the absence of regulations, sulfur dioxide (SO2) emissions from coal-fired power plants in India have increased notably in the past decade. In this study, we present the first interannual comparison of SO2 emissions and the satellite SO2 observations from the Ozone Monitoring Instrument (OMI) for Indian coal-fired power plants during the OMI era of 2005-2012. A detailed unit-based inventory is developed for the Indian coal-fired power sector, and results show that its SO2 emissions increased dramatically by 71% during 2005-2012. Using the oversampling technique, yearly high-resolution OMI maps for the whole domain of India are created, and they reveal a continuous increase in SO2 columns over India. Power plant regions with annual SO2 emissions greater than 50 Gg year(-1) produce statistically significant OMI signals, and a high correlation (R = 0.93) is found between SO2 emissions and OMI-observed SO2 burdens. Contrary to the decreasing trend of national mean SO2 concentrations reported by the Indian Government, both the total OMI-observed SO2 and annual average SO2 concentrations in coal-fired power plant regions increased by >60% during 2005-2012, implying the air quality monitoring network needs to be optimized to reflect the true SO2 situation in India. C1 [Lu, Zifeng; Streets, David G.] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. [de Foy, Benjamin] St Louis Univ, Dept Earth & Atmospher Sci, St Louis, MO 63108 USA. [Krotkov, Nickolay A.] NASA, Goddard Space Flight Ctr, Atmospher Chem & Dynam Lab, Maryland, MD 20771 USA. RP Lu, ZF (reprint author), Argonne Natl Lab, Decis & Informat Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zlu@anl.gov RI Lu, Zifeng/F-3266-2012; de Foy, Benjamin/A-9902-2010; Krotkov, Nickolay/E-1541-2012; OI de Foy, Benjamin/0000-0003-4150-9922; Krotkov, Nickolay/0000-0001-6170-6750; Streets, David/0000-0002-0223-1350 FU National Aeronautics and Space Administration (NASA) as part of the Air Quality Applied Sciences Team (AQAST) program; Ganges Valley Aerosol Experiment (GVAX) by the Office of Biological and Environmental Research in the U.S. Department of Energy, Office of Science. Argonne National Laboratory; U.S. Department of Energy [DE-AC02-06CH11357] FX This work was sponsored by the National Aeronautics and Space Administration (NASA) as part of the Air Quality Applied Sciences Team (AQAST) program. The India emission inventory was partially funded in support of the Ganges Valley Aerosol Experiment (GVAX) by the Office of Biological and Environmental Research in the U.S. Department of Energy, Office of Science. Argonne National Laboratory is operated by UChicago Argonne, LLC, under Contract No. DE-AC02-06CH11357 with the U.S. Department of Energy. NR 42 TC 17 Z9 19 U1 0 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD DEC 17 PY 2013 VL 47 IS 24 BP 13993 EP 14000 DI 10.1021/es4039648 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 277CT UT WOS:000328796900013 PM 24274462 ER PT J AU Muehe, EM Obst, M Hitchcock, A Tyliszczak, T Behrens, S Schroder, C Byrne, JM Michel, FM Kramer, U Kapplert, A AF Muehe, E. Marie Obst, Martin Hitchcock, Adam Tyliszczak, Tolek Behrens, Sebastian Schroeder, Christian Byrne, James M. Michel, F. Marc Kraemer, Ute Kapplert, Andreas TI Fate of Cd during Microbial Fe(III) Mineral Reduction by a Novel and Cd-Tolerant Geobacter Species SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID METAL-REDUCING BACTERIA; URANIUM-CONTAMINATED AQUIFER; HEAVY-METALS; SURFACE COMPLEXATION; AGRICULTURAL SOILS; ARSENIC RETENTION; TRACE-METALS; SP-NOV; IRON; SEDIMENTS AB Fe(III) (oxyhydr)oxides affect the mobility of contaminants in the environment by providing reactive surfaces for sorption. This includes the toxic metal cadmium (Cd), which prevails in agricultural soils and is taken up by crops. Fe(III)-reducing bacteria can mobilize such contaminants by Fe(III) mineral dissolution or immobilize them by sorption to or coprecipitation with secondary Fe minerals. To date, not much is known about the fate of Fe(III) mineral-associated Cd during microbial Fe(III) reduction. Here, we describe the isolation of a new Geobacter sp. strain Cd1 from a Cd-contaminated field site, where the strain accounts for 10(4) cells g(-1) dry soil. Strain Cd1 reduces the poorly crystalline Fe(III) oxyhydroxide ferrihydrite in the presence of at least up to 112 mg Cd L-1. During initial microbial reduction of Cd-loaded ferrihydrite, sorbed Cd was mobilized. However, during continuous microbial Fe(III) reduction, Cd was immobilized by sorption to and/or coprecipitation within newly formed secondary minerals that contained Ca, Fe, and carbonate, implying the formation of an otavite-siderite-calcite (CdCO3-FeCO3-CaCO3) mixed mineral phase. Our data shows that microbially mediated turnover of Fe minerals affects the mobility of Cd in soils, potentially altering the dynamics of Cd uptake into food or phyto-remediating plants. C1 [Muehe, E. Marie; Behrens, Sebastian; Schroeder, Christian; Byrne, James M.; Kapplert, Andreas] Univ Tubingen, Ctr Appl Geosci, D-72076 Tubingen, Germany. [Obst, Martin] Univ Tubingen, Ctr Appl Geosci, D-72074 Tubingen, Germany. [Hitchcock, Adam] McMaster Univ, Dept Chem & Chem Biol, Hamilton, ON L8S 4M1, Canada. [Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Michel, F. Marc] Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. [Kraemer, Ute] Ruhr Univ Bochum, Dept Plant Physiol, D-44801 Bochum, Germany. RP Kapplert, A (reprint author), Univ Tubingen, Ctr Appl Geosci, D-72076 Tubingen, Germany. EM andreas.kappler@uni-tuebingen.de RI Schroder, Christian/B-3870-2009; Kraemer, Ute/C-5025-2008; Kappler, Andreas/G-7221-2016; Byrne, James/L-4860-2016 OI Schroder, Christian/0000-0002-7935-6039; Kraemer, Ute/0000-0001-7870-4508; Byrne, James/0000-0002-4399-7336 FU German Federal Environmental Foundation; Emmy-Noether program of the DFG [OB 362/1-1]; Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank C. Herth, B. Ruediger, and K. Stoegerer for assistance in the lab, T. Losekann-Behrens for primer design and sequence data analysis, S. Flaiz and P. Kuehn for Cd analysis, W. Kilmer, H. Schulz, M. Stuh,r and E. Adaktylou for SEM-support, F. Zeitvogel for providing the ImageJ plugin for visualizing the 2D-scatterplots for correlative SEM-EDX map analysis, and N. Hageman for the SEM image in Figure if. This work was supported by the scholarship program of the German Federal Environmental Foundation to EMM and by the Emmy-Noether program of the DFG to MO (OB 362/1-1). STXM analysis was supported by NSERC (Canada), Canada Foundation for Innovation and the Canada Research Chair program. The Advanced Light Source is supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences Division of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 73 TC 17 Z9 17 U1 10 U2 82 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD DEC 17 PY 2013 VL 47 IS 24 BP 14099 EP 14109 DI 10.1021/es403365w PG 11 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 277CT UT WOS:000328796900025 PM 24274146 ER PT J AU Schmidt, M Lee, SS Wilson, RE Knope, KE Bellucci, F Eng, PJ Stubbs, JE Soderholm, L Fenter, P AF Schmidt, Moritz Lee, Sang Soo Wilson, Richard E. Knope, Karah E. Bellucci, Francesco Eng, Peter J. Stubbs, Joanne E. Soderholm, L. Fenter, P. TI Surface-Mediated Formation of Pu(IV) Nanoparticles at the Muscovite-Electrolyte Interface SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID X-RAY REFLECTIVITY; PLUTONIUM OXIDE NANOPARTICLES; ACID; SOLUBILITY; TRANSPORT; SPECTRA; WATER; IONS; HYDROLYSIS; ADSORPTION AB The formation of Pu(IV)-oxo-nanoparticles from Pu(III) solutions by a surface-enhanced redox/polymerization reaction at the muscovite (001) basal plane is reported, with a continuous increase in plutonium coverage observed in situ over several hours. The sorbed Pu extends >70 angstrom from the surface with a maximum concentration at 10.5 angstrom and a total coverage of >9 Pu atoms per unit cell area of muscovite (0.77 mu g Pu/cm(2)) (determined independently by in situ resonant anomalous X-ray reflectivity and by ex-situ alpha-spectrometry). The presence of discrete nanoparticles is confirmed by high resolution atomic force microscopy. We propose that the formation of these Pu(IV) nanoparticles from an otherwise stable Pu(III) solution can be explained by the combination of a highly concentrated interfacial Pu-ion species, the Pu(III) Pu(IV) redox equilibrium, and the strong proclivity of tetravalent Pu to hydrolyze and form polymeric species. These results are the first direct observation of such behavior of plutonium on a naturally occurring mineral, providing insights into understanding the environmental transport of plutonium and other contaminants capable of similar redox/polymerization reactions. C1 [Schmidt, Moritz; Lee, Sang Soo; Wilson, Richard E.; Knope, Karah E.; Bellucci, Francesco; Soderholm, L.; Fenter, P.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Eng, Peter J.; Stubbs, Joanne E.] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60637 USA. RP Fenter, P (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM fenter@anl.gov RI Schmidt, Moritz/C-2610-2011; Wilson, Richard/H-1763-2011; Stubbs, Joanne/F-9710-2013 OI Schmidt, Moritz/0000-0002-8419-0811; Wilson, Richard/0000-0001-8618-5680; Stubbs, Joanne/0000-0002-8509-2009 FU United States Department of Energy Office of Science [DE-AC02-06CH11357]; BER; NSF; EPA; DOE/BES Geoscience; DOE/BES Chemical Sciences; National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-Geosciences [DE-FG02-94ER14466] FX This work, conducted at Argonne National Laboratory, operated by UChicago Argonne, LLC for the United States Department of Energy under contract number DE-AC02-06CH11357, is jointly supported by the United States Department of Energy Office of Science, BER, NSF, and the EPA (MS), and by the DOE/BES Geoscience (S.S.L., F.B., and P.F.) and Chemical Sciences (K.E.K., R.E.W., and L.S.) research programs. The X-ray data were collected at the GeoSoilEnviroCARS beamline 13-ID-C and the X-ray Operations and Research beamline 6-ID-B at the Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (EAR-1128799) and Department of Energy-Geosciences (DE-FG02-94ER14466). NR 42 TC 5 Z9 5 U1 1 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD DEC 17 PY 2013 VL 47 IS 24 BP 14178 EP 14184 DI 10.1021/es4037258 PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 277CT UT WOS:000328796900034 PM 24266655 ER PT J AU Betts, AR Chen, N Hamilton, JG Peak, D AF Betts, Aaron R. Chen, Ning Hamilton, Jordan G. Peak, Derek TI Rates and Mechanisms of Zn2+ Adsorption on a Meat and Bonemeal Biochar SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; SMELTER-CONTAMINATED SOIL; EXAFS SPECTROSCOPY; MINERAL APATITE; METAL SORPTION; ZN(II) IONS; HYDROXYAPATITE; ZINC; REMEDIATION; REMOVAL AB Biochars produced from meat and bonemeal (MBM) waste materials contain large amounts of calcium phosphate and are potentially useful sorbents for the remediation of metals. Because the reactivity of biochars depends strongly upon the conditions used in their production, the objective of this study was to evaluate the rates and mechanisms of Zn sorption onto a commercially supplied MBM biochar prior to its application in a field-scale revegetation project. Sorption experiments varying pH, time, and Zn concentration found that, above pH 6.1, Zn adsorbed to MBM biochar quickly (within 5 h) with a maximum adsorption capacity of 0.65 mmol Zn g(-1). Synchrotron-based Zn K-edge extended X-ray absorption fine structure spectroscopy was consistent with a tetrahedral Zn bound to phosphate groups in a monodentate inner-sphere surface complex for all conditions tested. With an acidification pretreatment and at more acidic pH, MBM biochar causes precipitation of a ZnPO4 phase. On the basis of these results, this MBM biochar has a high capacity to rapidly adsorb Zn in adsorption experiments and can be considered a promising sorbent for Zn remediation of contaminated soils. C1 [Betts, Aaron R.] US EPA, Oak Ridge Inst Sci & Educ, Cincinnati, OH 45268 USA. [Chen, Ning] Canadian Light Source Inc, Saskatoon, SK S7N 2V3, Canada. [Hamilton, Jordan G.; Peak, Derek] Univ Saskatchewan, Dept Soil Sci, Saskatoon, SK S7N 5A8, Canada. RP Peak, D (reprint author), Univ Saskatchewan, Dept Soil Sci, Saskatoon, SK S7N 5A8, Canada. EM derek.peak@usask.ca FU Natural Science and Engineering Research Council (NSERC); HudBay Minerals Inc.; Saskatchewan Ministry of Agriculture Strategic Research Program-Soils and Environment; Natural Sciences and Engineering Research Council of Canada; National Research Council Canada; Canadian Institutes of Health Research; Province of Saskatchewan; Western Economic Diversification Canada; University of Saskatchewan FX This research was supported by a Natural Science and Engineering Research Council (NSERC) Collaborative Research and Development (CRD) grant with HudBay Minerals Inc. (formerly Hudson Bay Mining and Smelting Co., Limited). Additional support was provided through the Saskatchewan Ministry of Agriculture Strategic Research Program-Soils and Environment. We would also like to thank the HXMA beamline personnel at CLS who assisted in beamline optimization. Research described in this paper was performed at the Canadian Light Source, which is supported by the Natural Sciences and Engineering Research Council of Canada, the National Research Council Canada, the Canadian Institutes of Health Research, the Province of Saskatchewan, Western Economic Diversification Canada, and the University of Saskatchewan. NR 37 TC 9 Z9 10 U1 8 U2 102 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD DEC 17 PY 2013 VL 47 IS 24 BP 14350 EP 14357 DI 10.1021/es4032198 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 277CT UT WOS:000328796900054 PM 24228903 ER PT J AU Kirchner, TB Hatab, NA Lavrik, NV Sepaniak, MJ AF Kirchner, Teresa B. Hatab, Nahla A. Lavrik, Nickolay V. Sepaniak, Michael J. TI Highly Ordered Silicon Pillar Arrays As Platforms for Planar Chromatography SO ANALYTICAL CHEMISTRY LA English DT Article ID THIN-LAYER-CHROMATOGRAPHY; LIQUID-CHROMATOGRAPHY; MASS-SPECTROMETRY; POROUS SILICON; COLUMNS; SEPARATIONS; PLATES; PHASE; PERFORMANCES; SURFACES AB Unlike HPLC, there has been sparse advancement in the stationary phases used for planar chromatography. Nevertheless, modernization of planar chromatography platforms can further highlight the technique's ability to separate multiple samples simultaneously, utilize orthogonal separation formats, image (detect) separations without rigorous temporal demands, and its overall simplicity. This paper describes the fabrication and evaluation of ordered pillar arrays that are chemically modified for planar chromatography and inspected by fluorescence microscopy to detect solvent development and analyte bands (spots). Photolithography, in combination with anisotropic deep reactive ion etching, is used to produce uniform high aspect ratio silicon pillars. The pillar heights, diameters, and pitch variations are approximately 15-20 mu m, 1-3 mu m, and 2-6 mu m, respectively, with the total pillar array size typically 1 cm x 3 cm. The arrays are imaged using scanning electron microscopy in order to measure the pillar diameter and pitch as well as analyze the pillar sidewalls after etching and stationary phase functionalization. These fluidic arrays will enable exploration of the impact on mass transport and chromatographic efficiency caused by altering the pillar array morphology. A C18 reverse stationary phase (RP), common RP solvents that are transported by traditional but uniquely rapid capillary flow, and Rhodamine 6G (R6G) as the preliminary analyte are used for this initial evaluation. The research presented in this article is aimed at understanding and overcoming the unique challenges in developing and utilizing ordered pillar arrays as a new platform for planar chromatography: focusing on fabrication of expansive arrays, studies of solvent transport, methods to create compatible sample spots, and an initial evaluation of band dispersion. C1 [Kirchner, Teresa B.; Hatab, Nahla A.; Sepaniak, Michael J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Lavrik, Nickolay V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Sepaniak, MJ (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM msepaniak@utk.edu RI Kirchner, Teresa/O-4771-2014; Lavrik, Nickolay/B-5268-2011 OI Kirchner, Teresa/0000-0003-3984-0624; Lavrik, Nickolay/0000-0002-9543-5634 FU National Science Foundation [1144947]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy at Oak Ridge National Laboratory FX This material is based upon work supported by the National Science Foundation under Grant No. 1144947. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 39 TC 11 Z9 11 U1 2 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD DEC 17 PY 2013 VL 85 IS 24 BP 11802 EP 11808 DI 10.1021/ac402261p PG 7 WC Chemistry, Analytical SC Chemistry GA 277CV UT WOS:000328797200021 PM 24228860 ER PT J AU Arnault, P Clerouin, J Robert, G Ticknor, C Kress, JD Collins, LA AF Arnault, Philippe Clerouin, Jean Robert, Gregory Ticknor, Christopher Kress, Joel D. Collins, Lee A. TI Thomas-Fermi Z-scaling laws and coupling stabilization for plasmas SO PHYSICAL REVIEW E LA English DT Article ID ONE-COMPONENT PLASMA; DENSE IONIZED MATTER; EQUATION-OF-STATE; MOLECULAR-DYNAMICS; STATISTICAL-MECHANICS; PRESSURE IONIZATION; ELEMENTS; MODELS AB Extending the well-known Thomas-Fermi Z-scaling laws to the Coulomb coupling parameter, we investigate the stabilization of the ionic coupling in isochoric heating [Clerouin et al., Phys. Rev. E 87, 061101 (2013)]. This stabilization is restricted to a domain in atomic number Z, temperature, and density, including strong limitations on high couplings, that can only be obtained for high-Z elements. Contact is made with recent isochoric heating experiments. The consequences for corresponding states with respect to ionic coupling are also quantified via orbital free molecular dynamics simulations. This opens avenues for future isochoric heating experiments. C1 [Arnault, Philippe; Clerouin, Jean; Robert, Gregory] CEA, DAM, DIF, F-91297 Arpajon, France. [Ticknor, Christopher; Kress, Joel D.; Collins, Lee A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Arnault, P (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. EM philippe.arnault@cea.fr RI Ticknor, Christopher/B-8651-2014; Clerouin, jean/D-8528-2015; OI Clerouin, jean/0000-0003-2144-2759; Ticknor, Christopher/0000-0001-9972-4524 FU U.S. Department of Energy [DE-AC52-06NA25396] FX This work was done under the NNSA/DAM collaborative agreement P184. We especially thank Flavien Lambert for providing his OFMD code and L. Colombet for his assistance. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 44 TC 10 Z9 10 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD DEC 17 PY 2013 VL 88 IS 6 AR 063106 DI 10.1103/PhysRevE.88.063106 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 275SE UT WOS:000328697000006 PM 24483576 ER PT J AU Madrid, EA Rose, DV Welch, DR Clark, RE Mostrom, CB Stygar, WA Cuneo, ME Gomez, MR Hughes, TP Pointon, TD Seidel, DB AF Madrid, E. A. Rose, D. V. Welch, D. R. Clark, R. E. Mostrom, C. B. Stygar, W. A. Cuneo, M. E. Gomez, M. R. Hughes, T. P. Pointon, T. D. Seidel, D. B. TI Steady-state modeling of current loss in a post-hole convolute driven by high power magnetically insulated transmission lines SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID ELECTRON FLOW; ION DIODES; PLASMA AB Quasiequilibrium power flow in two radial magnetically insulated transmission lines (MITLs) coupled to a vacuum post-hole convolute is studied at 50 TW-200 TW using three-dimensional particle-in-cell simulations. The key physical dimensions in the model are based on the ZR accelerator [D. H. McDaniel, et al., Proceedings of 5th International Conference on Dense Z-Pinches, edited by J. Davis (AIP, New York, 2002), p. 23]. The voltages assumed for this study result in electron emission from all cathode surfaces. Electrons emitted from the MITL cathodes upstream of the convolute cause a portion of the MITL current to be carried by an electron sheath. Under the simplifying assumptions made by the simulations, it is found that the transition from the two MITLs to the convolute results in the loss of most of the sheath current to anode structures. The loss is quantified as a function of radius and correlated with Poynting vector stream lines which would be followed by individual electrons. For a fixed MITL-convolute geometry, the current loss, defined to be the difference between the total (i.e. anode) current in the system upstream of the convolute and the current delivered to the load, increases with both operating voltage and load impedance. It is also found that in the absence of ion emission, the convolute is efficient when the load impedance is much less than the impedance of the two parallel MITLs. The effects of space-charge-limited (SCL) ion emission from anode surfaces are considered for several specific cases. Ion emission from anode surfaces in the convolute is found to increase the current loss by a factor of 2-3. When SCL ion emission is allowed from anode surfaces in the MITLs upstream of the convolute, substantially higher current losses are obtained. Note that the results reported here are valid given the spatial resolution used for the simulations. C1 [Madrid, E. A.; Rose, D. V.; Welch, D. R.; Clark, R. E.; Mostrom, C. B.] Voss Sci LLC, Albuquerque, NM 87108 USA. [Stygar, W. A.; Cuneo, M. E.; Gomez, M. R.; Hughes, T. P.; Pointon, T. D.; Seidel, D. B.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Madrid, EA (reprint author), Voss Sci LLC, Albuquerque, NM 87108 USA. EM elizabethm@vosssci.com FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would very much like to thank J. L. Porter, M. K. Matzen, G. R. McKee, and L. X. Schneider at Sandia National Laboratories for invaluable contributions. Numerical simulation results presented here were carried on computer facilities at Sandia and Voss Scientific. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 53 TC 5 Z9 7 U1 0 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD DEC 17 PY 2013 VL 16 IS 12 AR 120401 DI 10.1103/PhysRevSTAB.16.120401 PG 16 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 275UA UT WOS:000328701900001 ER PT J AU Singh, DJ Parker, D AF Singh, David J. Parker, David TI Itinerant magnetism in doped semiconducting beta-FeSi2 and CrSi2 SO SCIENTIFIC REPORTS LA English DT Article ID HALF-METALLIC FERROMAGNETS; ELECTRONIC-STRUCTURE; FILMS; TEMPERATURE; DISILICIDE; EMISSION; SILICON; GROWTH; LAYERS; CRO2 AB Novel or unusual magnetism is a subject of considerable interest, particularly in metals and degenerate semiconductors. In such materials the interplay of magnetism, transport and other Fermi liquid properties can lead to fascinating physical behavior. One example is in magnetic semiconductors, where spin polarized currents may be controlled and used. We report density functional calculations predicting magnetism in doped semiconducting beta-FeSi2 and CrSi2 at relatively low doping levels particularly for n-type. In this case, there is a rapid cross-over to a half-metallic state as a function of doping level. The results are discussed in relation to the electronic structure and other properties of these compounds. C1 [Singh, David J.; Parker, David] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Singh, DJ (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM singhdj@ornl.gov FU Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX Work at ORNL was supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 45 TC 2 Z9 2 U1 1 U2 39 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD DEC 17 PY 2013 VL 3 AR 3517 DI 10.1038/srep03517 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 273YC UT WOS:000328571200005 PM 24343332 ER PT J AU Tang, CS Xia, B Zou, XQ Chen, S Ou, HW Wang, L Rusydi, A Zhu, JX Chia, EEM AF Tang, Chi Sin Xia, Bin Zou, Xingquan Chen, Shi Ou, Hong-Wei Wang, Lan Rusydi, A. Zhu, Jian-Xin Chia, Elbert E. M. TI Terahertz conductivity of topological surface states in Bi1.5Sb0.5Te1.8Se1.2 SO SCIENTIFIC REPORTS LA English DT Article ID INSULATOR BI2SE3; PHASE; RAMAN AB Topological insulators are electronic materials with an insulating bulk and conducting surface. However, due to free carriers in the bulk, the properties of the metallic surface are difficult to detect and characterize in most topological insulator materials. Recently, a new topological insulator Bi1.5Sb0.5Te1.7Se1.3 (BSTS) was found, showing high bulk resistivities of 1-10 Omega.cm and greater contrast between the bulk and surface resistivities compared to other Bi-based topological insulators. Using Terahertz Time-Domain Spectroscopy (THz-TDS), we present complex conductivity of BSTS single crystals, disentangling the surface and bulk contributions. We find that the Drude spectral weight is 1-2 orders of magnitude smaller than in other Bi-based topological insulators, and similar to that of Bi2Se3 thin films, suggesting a significant contribution of the topological surface states to the conductivity of the BSTS sample. Moreover, an impurity band is present about 30 meV below the Fermi level, and the surface and bulk carrier densities agree with those obtained from transport data. Furthermore, from the surface Drude contribution, we obtain a similar to 98% transmission through one surface layer - this is consistent with the transmission through single-layer or bilayer graphene, which shares a common Dirac-cone feature in the band structure. C1 [Tang, Chi Sin; Xia, Bin; Zou, Xingquan; Chen, Shi; Wang, Lan; Chia, Elbert E. M.] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore. [Ou, Hong-Wei; Rusydi, A.] Natl Univ Singapore, Dept Phys, NUSNNI NanoCore, Singapore 117542, Singapore. [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Wang, L (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore. EM wanglan@ntu.edu.sg; phyandri@nus.edu.sg; elbertchia@ntu.edu.sg RI Chia, Elbert/B-6996-2011; Wang, Lan/B-6990-2011; Rusydi, Andrivo/I-1849-2016; OI Chia, Elbert/0000-0003-2066-0834; Wang, Lan/0000-0001-7124-2718; Zhu, Jianxin/0000-0001-7991-3918 FU Singapore National Research Foundation [RCA-08/018]; Singapore Ministry of Education AcRF [MOE2010-T2-2-059, RG13/12, ARC 23/08]; National Research Foundation Competitive Research Programme [NRF-CRP4-2008-04]; National Nuclear Security Administration of the U.S. DOE at LANL [DE-AC52-06NA25396]; US. DOE Office of Basic Energy Sciences; Center for Integrated Nanotechnologies, a U.S. DOE Office of Basic Energy Sciences FX We thank A. Castro Neto, D. Talbayev, V. Venkatesan, P. Di Pietro and S. Lupi for discussions. L.W. acknowledges funding from Singapore National Research Foundation RCA-08/018 and Singapore Ministry of Education AcRF Tier 2 (MOE2010-T2-2-059). E.E.M.C. acknowledges support from Singapore Ministry of Education AcRF Tier 1 (RG13/12), Tier 2 (ARC 23/08), as well as the National Research Foundation Competitive Research Programme (NRF-CRP4-2008-04). J.-X.Z. is supported by the National Nuclear Security Administration of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396, the US. DOE Office of Basic Energy Sciences, and in part by the Center for Integrated Nanotechnologies, a U.S. DOE Office of Basic Energy Sciences user facility. NR 32 TC 24 Z9 24 U1 6 U2 52 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD DEC 17 PY 2013 VL 3 AR 3513 DI 10.1038/srep03513 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 273YC UT WOS:000328571200001 PM 24343202 ER PT J AU Zeldin, OB Brockhauser, S Bremridge, J Holton, JM Garman, EF AF Zeldin, Oliver B. Brockhauser, Sandor Bremridge, John Holton, James M. Garman, Elspeth F. TI Predicting the X-ray lifetime of protein crystals SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID MACROMOLECULAR CRYSTALLOGRAPHY; RADIATION-DAMAGE; CRYOGENIC TEMPERATURES; RADDOSE; SAMPLES AB Radiation damage is a major cause of failure in macromolecular crystallography experiments. Although it is always best to evenly illuminate the entire volume of a homogeneously diffracting crystal, limitations of the available equipment and imperfections in the sample often require a more sophisticated targeting strategy, involving microbeams smaller than the crystal, and translations of the crystal during data collection. This leads to a highly inhomogeneous distribution of absorbed X-rays (i.e., dose). Under these common experimental conditions, the relationship between dose and time is nonlinear, making it difficult to design an experimental strategy that optimizes the radiation damage lifetime of the crystal, or to assign appropriate dose values to an experiment. We present, and experimentally validate, a predictive metric diffraction-weighted dose for modeling the rate of decay of total diffracted intensity from protein crystals in macromolecular crystallography, and hence we can now assign appropriate "dose" values to modern experimental setups. Further, by taking the ratio of total elastic scattering to diffraction-weighted dose, we show that it is possible to directly compare potential data-collection strategies to optimize the diffraction for a given level of damage under specific experimental conditions. As an example of the applicability of this method, we demonstrate that by offsetting the rotation axis from the beam axis by 1.25 times the full-width half maximum of the beam, it is possible to significantly extend the dose lifetime of the crystal, leading to a higher number of diffracted photons, better statistics, and lower overall radiation damage. C1 [Zeldin, Oliver B.; Bremridge, John; Garman, Elspeth F.] Univ Oxford, Dept Biochem, Oxford OX1 3QU, England. [Brockhauser, Sandor] Univ Grenoble, Alpes European Mol Biol Lab, CNRS, European Mol Biol Lab,Grenoble Outstn, F-38042 Grenoble, France. [Brockhauser, Sandor] Univ Grenoble, Alpes European Mol Biol Lab, CNRS, Unit Virus Host Cell Interact, F-38042 Grenoble, France. [Holton, James M.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. [Holton, James M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Garman, EF (reprint author), Univ Oxford, Dept Biochem, Oxford OX1 3QU, England. EM elspeth.garman@bioch.ox.ac.uk FU University of Oxford Engineering and Physical Sciences Research Council Life Science Interface Doctoral Training Centre; National Institutes of Health [GM073210, GM082250, GM094625]; Department of Energy:Integrated Diffraction Analysis Technologies [DE-AC02-05CH11231]; Lawrence Berkeley National Laboratory FX The authors thank Markus Gerstel for his great assistance in the development of the program RADDOSE-3D, and Arwen Pearson for valuable discussions during the development of this work. O.B.Z. was funded by a studentship through the University of Oxford Engineering and Physical Sciences Research Council Life Science Interface Doctoral Training Centre. J.M.H. is funded by the National Institutes of Health (GM073210, GM082250, and GM094625) and the Department of Energy:Integrated Diffraction Analysis Technologies Contract DE-AC02-05CH11231 with Lawrence Berkeley National Laboratory. Beamtime at ESRF ID14-4 was provided through the Radiation Damage Block Allocation Group. NR 28 TC 21 Z9 21 U1 0 U2 15 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD DEC 17 PY 2013 VL 110 IS 51 BP 20551 EP 20556 DI 10.1073/pnas.1315879110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 273PR UT WOS:000328548600052 PM 24297937 ER PT J AU Benzine, J Shelobolina, E Xiong, MY Kennedy, DW McKinley, JP Lin, XJ Roden, EE AF Benzine, Jason Shelobolina, Evgenya Xiong, Mai Yia Kennedy, David W. McKinley, James P. Lin, Xueju Roden, Eric E. TI Fe-phyllosilicate redox cycling organisms from a redox transition zone in Hanford 300 Area sediments SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE subsurface; sediment; microbial; phyllosilicate; iron; redox; enrichment; isolation ID IRON-REDUCING BACTERIA; SOLID-WATER INTERFACE; MICROBIAL REDUCTION; BRADYRHIZOBIUM-JAPONICUM; BIOGENIC FE(II); CLAY-MINERALS; FERRIC-IRON; SP NOV.; SITE; RESPIRATION AB Microorganisms capable of reducing or oxidizing structural iron (Fe) in Fe-bearing phyllosilicate minerals were enriched and isolated from a subsurface redox transition zone at the Hanford 300 Area site in eastern Washington, USA. Both conventional and in situ "i-chip" enrichment strategies were employed. One Fe(III)-reducing Geobacter (G. bremensis strain R1, Deltaproteobacteria) and six Fe(II) phyllosilicate-oxidizing isolates from the Alphaproteobacteria (Bradyrhizobium japonicum strains 22, is5, and in8p8), Betaproteobacteria (Cupriavidus necator strain A5-1, Dechloromonas agitata strain is5), and Actinobacteria (Nocardioides sp. strain in31) were recovered. The G. bremensis isolate grew by oxidizing acetate with the oxidized form of NAu-2 smectite as the electron acceptor. The Fe(ll)-oxidizers grew by oxidation of chemically reduced smectite as the energy source with nitrate as the electron acceptor. The Bradyrhizobium isolates could also carry out aerobic oxidation of biotite. This is the first report of the recovery of a Fe(ll)-oxidizing Nocardioides, and to date only one other Fe(ll)-oxidizing Bradyrhizobium is known. The 16S rRNA gene sequences of the isolates were similar to ones found in clone libraries from Hanford 300 sediments and groundwater, suggesting that such organisms may be present and active in situ. Whole genome sequencing of the isolates is underway, the results of which will enable comparative genomic analysis of mechanisms of extracellular phyllosilicate Fe redox metabolism, and facilitate development of techniques to detect the presence and expression of genes associated with microbial phyllosilicate Fe redox cycling in sediments. C1 [Benzine, Jason; Shelobolina, Evgenya; Xiong, Mai Yia; Roden, Eric E.] Univ Wisconsin, Dept Geosci, Madison, WI 53706 USA. [Kennedy, David W.; McKinley, James P.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Lin, Xueju] Georgia Inst Technol, Sch Biol, Atlanta, GA 30332 USA. RP Shelobolina, E (reprint author), Univ Wisconsin, Dept Geosci, 1215 W Dayton St, Madison, WI 53706 USA. EM shelobolina@wisc.edu; eroden@geology.wisc.edu OI Kennedy, David/0000-0003-0763-501X FU U.S. Department of Energy, Office of Biological and Environmental Research, Subsurface Biogeochemical Research Program through the SBR Scientific Focus Area at the Pacific Northwest National Laboratory FX This work was supported by the U.S. Department of Energy, Office of Biological and Environmental Research, Subsurface Biogeochemical Research Program through the SBR Scientific Focus Area at the Pacific Northwest National Laboratory. NR 56 TC 9 Z9 9 U1 5 U2 46 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD DEC 16 PY 2013 VL 4 AR 388 DI 10.3389/fmicb.2013.00388 PG 13 WC Microbiology SC Microbiology GA AB1KZ UT WOS:000331551900001 PM 24379809 ER PT J AU Carroll, AW Joshi, HJ Heazlewood, JL AF Carroll, Andrew W. Joshi, Hiren J. Heazlewood, Joshua L. TI Managing the green proteomes for the next decade of plant research SO FRONTIERS IN PLANT SCIENCE LA English DT Editorial Material DE proteomics; informatics; database; phosphorylation; proteogenomic; subcellular ID DATABASE; ARABIDOPSIS; PROTEINS C1 [Carroll, Andrew W.; Heazlewood, Joshua L.] Univ Copenhagen, Dept Cellular & Mol Biol, Copenhagen Ctr Glyc, Copenhagen, Denmark. [Joshi, Hiren J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Joshi, Hiren J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. RP Heazlewood, JL (reprint author), Univ Copenhagen, Dept Cellular & Mol Biol, Copenhagen Ctr Glyc, Copenhagen, Denmark. EM jlheazlewood@lbl.gov RI Heazlewood, Joshua/A-2554-2008 OI Heazlewood, Joshua/0000-0002-2080-3826 NR 22 TC 1 Z9 2 U1 0 U2 4 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD DEC 16 PY 2013 VL 4 AR 501 DI 10.3389/fpls.2013.00501 PG 2 WC Plant Sciences SC Plant Sciences GA AB1AQ UT WOS:000331524000001 PM 24379820 ER PT J AU Kravitz, B Rasch, PJ Forster, PM Andrews, T Cole, JNS Irvine, PJ Ji, DY Kristjansson, JE Moore, JC Muri, H Niemeier, U Robock, A Singh, B Tilmes, S Watanabe, S Yoon, JH AF Kravitz, Ben Rasch, Philip J. Forster, Piers M. Andrews, Timothy Cole, Jason N. S. Irvine, Peter J. Ji, Duoying Kristjansson, Jon Egill Moore, John C. Muri, Helene Niemeier, Ulrike Robock, Alan Singh, Balwinder Tilmes, Simone Watanabe, Shingo Yoon, Jin-Ho TI An energetic perspective on hydrological cycle changes in the Geoengineering Model Intercomparison Project SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE geoengineering; model intercomparison; energetic perspective; hydrologic cycle ID SOLAR-RADIATION MANAGEMENT; CLIMATE-CHANGE; HADLEY CIRCULATION; WARMING CONTRAST; CARBON-DIOXIDE; CO2; PRECIPITATION; RESPONSES; SIMULATIONS; ADJUSTMENT AB Analysis of surface and atmospheric energy budget responses to CO2 and solar forcings can be used to reveal mechanisms of change in the hydrological cycle. We apply this energetic perspective to output from 11 fully coupled atmosphere-ocean general circulation models simulating experiment G1 of the Geoengineering Model Intercomparison Project (GeoMIP), which achieves top-of-atmosphere energy balance between an abrupt quadrupling of CO2 from preindustrial levels (abrupt4xCO2) and uniform solar irradiance reduction. We divide the climate system response into a rapid adjustment, in which climate response is due to adjustment of the atmosphere and land surface on short time scales, and a feedback response, in which the climate response is predominantly due to feedback related to global mean temperature changes. Global mean temperature change is small in G1, so the feedback response is also small. G1 shows a smaller magnitude of land sensible heat flux rapid adjustment than in abrupt4xCO2 and a larger magnitude of latent heat flux adjustment, indicating a greater reduction of evaporation and less land temperature increase than abrupt4xCO2. The sum of surface flux changes in G1 is small, indicating little ocean heat uptake. Using an energetic perspective to assess precipitation changes, abrupt4xCO2 shows decreased mean evaporative moisture flux and increased moisture convergence, particularly over land. However, most changes in precipitation in G1 are in mean evaporative flux, suggesting that changes in mean circulation are small. C1 [Kravitz, Ben; Rasch, Philip J.; Singh, Balwinder; Yoon, Jin-Ho] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Forster, Piers M.] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England. [Andrews, Timothy] Met Off Hadley Ctr, Exeter, Devon, England. [Cole, Jason N. S.] Environm Canada, Canadian Ctr Climate Modelling & Anal, Toronto, ON, Canada. [Irvine, Peter J.] Inst Adv Sustainabil Studies, Potsdam, Germany. [Ji, Duoying; Moore, John C.] Beijing Normal Univ, Coll Global Change & Earth Syst Sci, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China. [Kristjansson, Jon Egill; Muri, Helene] Univ Oslo, Dept Geosci, Oslo, Norway. [Niemeier, Ulrike] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Robock, Alan] Rutgers State Univ, Dept Environm Sci, New Brunswick, NJ 08903 USA. [Tilmes, Simone] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Watanabe, Shingo] Japan Agcy Marine Earth Sci & Technol, Yokohama, Kanagawa, Japan. RP Kravitz, B (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, 902 Battelle Blvd,POB 999,MSIN K9-24, Richland, WA 99352 USA. EM ben.kravitz@pnnl.gov RI Andrews, Timothy/C-5912-2014; Moore, John/B-2868-2013; YOON, JIN-HO/A-1672-2009; Kravitz, Ben/P-7925-2014; Muri, Helene/D-4845-2015; Robock, Alan/B-6385-2016; Forster, Piers/F-9829-2010; Watanabe, Shingo/L-9689-2014; OI Andrews, Timothy/0000-0002-8248-8753; Moore, John/0000-0001-8271-5787; YOON, JIN-HO/0000-0002-4939-8078; Kravitz, Ben/0000-0001-6318-1150; Muri, Helene/0000-0003-4738-493X; Forster, Piers/0000-0002-6078-0171; Watanabe, Shingo/0000-0002-2228-0088; Cole, Jason/0000-0003-0450-2748 FU Fund for Innovative Climate and Energy Research (FICER); U.S. Department of Energy by Battelle Memorial Institute [DE-AC05-76RL01830]; NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center; Joint DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; NSF [AGS-1157525, CBET-1240507]; EuTRACE project, the European Union 7th Framework Programme [306395]; European Union [226567-IMPLICC]; Norwegian Research Council; HPC resources of [CCT/TGCC/CINES/IDRIS] under GENCI (Grand Equipement National de Calcul Intensif) [2012-t2012012201]; National Science Foundation; Innovative Program of Climate Change Projection for the 21st century, MEXT, Japan; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank three anonymous reviewers for their helpful comments in improving the manuscript. We also thank all participants of the Geoengineering Model Intercomparison Project and their model development teams, CLIVAR/WCRP Working Group on Coupled Modeling for endorsing GeoMIP, and the scientists managing the Earth System Grid data nodes who have assisted with making GeoMIP output available. We acknowledge the World Climate Research Programme's Working Group on Coupled Modelling, which is responsible for CMIP, and we thank the climate modeling groups for producing and making available their model output. For CMIP, the U.S. Department of Energy's Program for Climate Model Diagnosis and Intercomparison provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals. Ben Kravitz is supported by the Fund for Innovative Climate and Energy Research (FICER). The Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RL01830. Simulations performed by Ben Kravitz were supported by the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center. Timothy Andrews was supported by the Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). Duoying Ji and John C. Moore thank all members of the BNU-ESM model group, as well as the Center of Information and Network Technology at Beijing Normal University for assistance in publishing the GeoMIP data set. Alan Robock is supported by NSF grants AGS-1157525 and CBET-1240507. Helene Muri was supported by the EuTRACE project, the European Union 7th Framework Programme grant 306395. Jon Egill Kristjansson, Ulrike Niemeier, and Michael Schulz received funding from the European Union's Seventh Framework Programme (FP7/2007-2013) under grant agreement 226567-IMPLICC. Jon Egill Kristjansson received support from the Norwegian Research Council's Programme for Supercomputing (NOTUR) through a grant of computing time. Simulations with the IPSL-CM5 model were supported through HPC resources of [CCT/TGCC/CINES/IDRIS] under the allocation 2012-t2012012201 made by GENCI (Grand Equipement National de Calcul Intensif). Duoying Ji and John C. Moore thank all members of the BNU-ESM model group, as well as the Center of Information and Network Technology at Beijing Normal University for assistance in publishing the GeoMIP data set. The National Center for Atmospheric Research is funded by the National Science Foundation. Shingo Watanabe was supported by the Innovative Program of Climate Change Projection for the 21st century, MEXT, Japan. Computer resources for Philip J. Rasch, Balwinder Singh, and Jin-Ho Yoon were provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 58 TC 24 Z9 24 U1 2 U2 24 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD DEC 16 PY 2013 VL 118 IS 23 BP 13087 EP 13102 DI 10.1002/2013JD020502 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PD UT WOS:000330266500024 ER PT J AU Kravitz, B Robock, A Forster, PM Haywood, JM Lawrence, MG Schmidt, H AF Kravitz, Ben Robock, Alan Forster, Piers M. Haywood, James M. Lawrence, Mark G. Schmidt, Hauke TI An overview of the Geoengineering Model Intercomparison Project (GeoMIP) SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE Geoengineering; Model Intercomparison ID CLIMATE; RADIATION; RESPONSES; AEROSOLS; IMPACT; CMIP5; LAND AB The Geoengineering Model Intercomparison Project (GeoMIP) was designed to determine robust climate system model responses to solar geoengineering. GeoMIP currently consists of four standardized simulations involving reduction of insolation or increased amounts of stratospheric sulfate aerosols. Three more experiments involving marine cloud brightening are planned. This project has improved confidence in the expected climate effects of geoengineering in several key areas, such as the effects of geoengineering on spatial patterns of temperature and the spatial distribution of precipitation, especially extreme precipitation events. However, GeoMIP has also highlighted several important research gaps, such as the effects on terrestrial net primary productivity and the importance of the CO2 physiological effect in determining the hydrologic cycle response to geoengineering. Future efforts will endeavor to address these gaps, as well as encourage cooperation with the chemistry modeling communities, the impact assessment communities, and other groups interested in model output. C1 [Kravitz, Ben] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Robock, Alan] Rutgers State Univ, Dept Environm Sci, New Brunswick, NJ 08903 USA. [Forster, Piers M.] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England. [Haywood, James M.] Met Off Hadley Ctr, Exeter, Devon, England. [Haywood, James M.] Univ Exeter, Coll Engn Math & Phys Sci, Exeter, Devon, England. [Lawrence, Mark G.] Inst Adv Sustainabil Studies, Potsdam, Germany. [Schmidt, Hauke] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. RP Kravitz, B (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, POB 999,MSIN K9-24, Richland, WA 99352 USA. EM ben.kravitz@pnnl.gov RI Kravitz, Ben/P-7925-2014; Robock, Alan/B-6385-2016; Forster, Piers/F-9829-2010 OI Kravitz, Ben/0000-0001-6318-1150; Forster, Piers/0000-0002-6078-0171 FU Battelle Memorial Institute [DE-AC05-76RL01830]; NSF [AGS-1157525, CBET-1240507]; DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; European Union [306395] FX We thank all participants of the Geoengineering Model Intercomparison Project and their model development teams, the CLIVAR/WCRP Working Group on Coupled Modeling for endorsing GeoMIP, and the scientists managing the Earth System Grid data nodes who have assisted in making the GeoMIP output available. Ben Kravitz is supported by the Fund for Innovative Climate and Energy Research (FICER). The Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RL01830. Alan Robock is supported by NSF grants AGS-1157525 and CBET-1240507. Jim Haywood was supported by the joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101) and funding from the European Union Seventh Framework Programme through the EuTRACE project (306395). NR 28 TC 13 Z9 13 U1 2 U2 37 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD DEC 16 PY 2013 VL 118 IS 23 BP 13103 EP 13107 DI 10.1002/2013JD020569 PG 5 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PD UT WOS:000330266500029 ER PT J AU Bennett, PB Pedramrazi, Z Madani, A Chen, YC de Oteyza, DG Chen, C Fischer, FR Crommie, MF Bokor, J AF Bennett, Patrick B. Pedramrazi, Zahra Madani, Ali Chen, Yen-Chia de Oteyza, Dimas G. Chen, Chen Fischer, Felix R. Crommie, Michael F. Bokor, Jeffrey TI Bottom-up graphene nanoribbon field-effect transistors SO APPLIED PHYSICS LETTERS LA English DT Article ID CARBON NANOTUBE TRANSISTORS; RESISTANCE; DEVICE AB Recently developed processes have enabled bottom-up chemical synthesis of graphene nanoribbons (GNRs) with precise atomic structure. These GNRs are ideal candidates for electronic devices because of their uniformity, extremely narrow width below 1 nm, atomically perfect edge structure, and desirable electronic properties. Here, we demonstrate nano-scale chemically synthesized GNR field-effect transistors, made possible by development of a reliable layer transfer process. We observe strong environmental sensitivity and unique transport behavior characteristic of sub-1 nm width GNRs. (C) 2013 AIP Publishing LLC. C1 [Bennett, Patrick B.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Bennett, Patrick B.; Madani, Ali; Bokor, Jeffrey] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Pedramrazi, Zahra; Chen, Yen-Chia; de Oteyza, Dimas G.; Crommie, Michael F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Chen, Yen-Chia; Fischer, Felix R.; Crommie, Michael F.; Bokor, Jeffrey] Lawrence Berkeley Natl Labs, Div Mat Sci, Berkeley, CA 94720 USA. [de Oteyza, Dimas G.] Univ Basque Country, CSIC, Ctr Phys Mat, E-20018 San Sebastian, Spain. [Chen, Chen; Fischer, Felix R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Bokor, J (reprint author), 253 Cory Hall MC 1770, Berkeley, CA 94720 USA. EM jbokor@eecs.berkeley.edu RI de Oteyza, Dimas/H-5955-2013; Foundry, Molecular/G-9968-2014; CSIC-UPV/EHU, CFM/F-4867-2012 OI de Oteyza, Dimas/0000-0001-8060-6819; FU Office of Naval Research BRC Program; Helios Solar Energy Research Center; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR-1206512]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Research was supported by the Office of Naval Research BRC Program, by the Helios Solar Energy Research Center, which is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and by National Science Foundation award DMR-1206512. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. All devices were fabricated in the UC Berkeley Nanolab. We would like to thank Professor M. Lundstrom, Professor Sumon Datta, Dr. D. Haberer, and Professor S. J. Choi for useful discussions. NR 30 TC 50 Z9 50 U1 11 U2 130 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 16 PY 2013 VL 103 IS 25 AR 253114 DI 10.1063/1.4855116 PG 4 WC Physics, Applied SC Physics GA 293LU UT WOS:000329973800078 ER PT J AU Hurtado, A Xu, H Wright, JB Liu, S Li, Q Wang, GT Luk, TS Figiel, JJ Cross, K Balakrishnan, G Lester, LF Brener, I AF Hurtado, A. Xu, H. Wright, J. B. Liu, Sheng Li, Q. Wang, G. T. Luk, T. S. Figiel, J. J. Cross, K. Balakrishnan, G. Lester, L. F. Brener, I. TI Polarization switching in GaN nanowire lasers SO APPLIED PHYSICS LETTERS LA English DT Article ID FLIP-FLOP OPERATION; EMISSION AB The polarization properties of a GaN nanowire laser are studied experimentally by direct analysis of the nanowire's end-facet emission. Linear and elliptical light polarizations are measured at different pumping strengths. Switching between these two polarization states is also observed as the optical excitation is increased. We attribute this polarization switching to a change in the transverse modes due to their different cavity losses. (C) 2013 AIP Publishing LLC. C1 [Hurtado, A.; Xu, H.; Wright, J. B.; Balakrishnan, G.; Lester, L. F.] Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87106 USA. [Hurtado, A.] Univ Essex, Sch Comp Sci & Elect Engn, Colchester CO4 3SQ, Essex, England. [Wright, J. B.; Liu, Sheng; Li, Q.; Wang, G. T.; Luk, T. S.; Figiel, J. J.; Cross, K.; Brener, I.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Liu, Sheng; Luk, T. S.; Brener, I.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Hurtado, A (reprint author), Univ New Mexico, Ctr High Technol Mat, 1313 Goddard St SE, Albuquerque, NM 87106 USA. EM ahurta01@unm.edu RI Wright, Jeremy/G-7149-2011; OI Wright, Jeremy/0000-0001-6861-930X; Hurtado, Antonio/0000-0002-4448-9034 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; European Union [PIOF-GA-2010-273822]; Sandia's Solid-State-Lighting Science Energy Frontier Research Center; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences FX This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U. S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. A. Hurtado was funded by the European Union Seventh Framework Programme (FP7/2007-2013) under Grant Agreement No. PIOF-GA-2010-273822. The other authors were supported by Sandia's Solid-State-Lighting Science Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences. NR 24 TC 8 Z9 8 U1 2 U2 31 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 16 PY 2013 VL 103 IS 25 AR 251107 DI 10.1063/1.4835115 PG 4 WC Physics, Applied SC Physics GA 293LU UT WOS:000329973800007 ER PT J AU Meng, XQ Chen, ZH Chen, Z Wu, FM Li, SS Li, JB Wu, JQ Wei, SH AF Meng, Xiuqing Chen, Zhanghui Chen, Zhuo Wu, Fengmin Li, Shu-Shen Li, Jingbo Wu, Junqiao Wei, Su-Huai TI Enhancing structural transition by carrier and quantum confinement: Stabilization of cubic InN quantum dots by Mn incorporation SO APPLIED PHYSICS LETTERS LA English DT Article ID INDIUM NITRIDE; NANOCRYSTALS; TEMPERATURE; WAVELENGTH; LASERS; FILMS AB We demonstrate in this work controllable synthesis of cubic InN nanocrystals' through Mn doping. We show that the pristine nanocrystal has the wurtzite structure, but can be converted into the zinc-blende (ZB) structure when it is doped with Mn. Our first-principles calculations show that the phase transition is caused by the stronger p-d coupling between the host p valence state and the impurity d level in the ZB structure, which makes the hole generation in the ZB structure easier. Quantum confinement in the nanocrystals further enhanced this effect. This observation lays an important foundation for defects control of crystal phases. (C) 2013 AIP Publishing LLC. C1 [Meng, Xiuqing; Wu, Fengmin; Li, Jingbo] Zhejiang Normal Univ, Jinhua 321004, Zhejiang, Peoples R China. [Chen, Zhanghui; Li, Shu-Shen; Li, Jingbo] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China. [Chen, Zhuo] Beijing Inst Technol, Dept Phys, Beijing 100081, Peoples R China. [Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Li, JB (reprint author), Zhejiang Normal Univ, Jinhua 321004, Zhejiang, Peoples R China. EM jbli@semi.ac.cn; swei@nrel.gov RI Wu, Junqiao/G-7840-2011; chen, zhuo/A-6430-2013 OI Wu, Junqiao/0000-0002-1498-0148; chen, zhuo/0000-0002-0671-4974 FU National Science Fund for Distinguished Young Scholar [60925016, 91233120]; National Natural Science Foundation of China [11104250, 50902125]; National Science Foundation [CMMI-1000176]; DOE [DE-AC36-08GO28308] FX J. Li gratefully acknowledges financial support from the National Science Fund for Distinguished Young Scholar (Grant Nos. 60925016 and 91233120). This work was supported by the National Natural Science Foundation of China (Grant Nos. 11104250 and 50902125). The work at UC Berkeley was supported by the National Science Foundation under Grant No. CMMI-1000176. The work at NREL was funded by DOE under Grant No. DE-AC36-08GO28308. NR 31 TC 0 Z9 0 U1 2 U2 26 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 16 PY 2013 VL 103 IS 25 AR 253102 DI 10.1063/1.4850755 PG 4 WC Physics, Applied SC Physics GA 293LU UT WOS:000329973800066 ER PT J AU Zawadzki, P Baranowski, LL Peng, HW Toberer, ES Ginley, DS Tumas, W Zakutayev, A Lany, S AF Zawadzki, Pawel Baranowski, Lauryn L. Peng, Haowei Toberer, Eric S. Ginley, David S. Tumas, W. Zakutayev, Andriy Lany, Stephan TI Evaluation of photovoltaic materials within the Cu-Sn-S family SO APPLIED PHYSICS LETTERS LA English DT Article ID SEMICONDUCTOR THIN-FILMS; SOLAR-CELLS; CRYSTAL-STRUCTURE; OPTICAL-PROPERTIES; EFFICIENCY; CU4SN7S16; SULFIDES; CU2SNS3 AB Next-generation thin film solar cell technologies require earth abundant photovoltaic absorber materials. Here we demonstrate an alternative approach to design of such materials, evaluating candidates grouped by constituent elements rather than underlying crystal structures. As an example, we evaluate thermodynamic stability, electrical transport, electronic structure, optical and defect properties of Cu-Sn-S candidates using complementary theory and experiment. We conclude that Cu2SnS3 avoids many issues associated with the properties of Cu4SnS4, Cu4Sn7S16, and other Cu-Sn-S materials. This example demonstrates how this element-specific approach quickly identifies potential problems with less promising candidates and helps focusing on the more promising solar cell absorbers. (C) 2013 AIP Publishing LLC. C1 [Zawadzki, Pawel; Baranowski, Lauryn L.; Peng, Haowei; Toberer, Eric S.; Ginley, David S.; Tumas, W.; Zakutayev, Andriy; Lany, Stephan] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Baranowski, Lauryn L.; Toberer, Eric S.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. RP Zakutayev, A (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM andriy.zakutayev@nrel.gov; stephan.lany@nrel.gov RI Peng, Haowei/K-4654-2012; OI Peng, Haowei/0000-0002-6502-8288; Zakutayev, Andriy/0000-0002-3054-5525; Lany, Stephan/0000-0002-8127-8885 FU U.S. Department of Energy, office of Energy Efficiency and Renewable Energy; NSF MRSEC program through the REMRSEC Center; Department of Defense (DoD) through National Defense Science and Engineering Graduate Fellowship (NDSEG) Program FX This work was funded by the U.S. Department of Energy, office of Energy Efficiency and Renewable Energy, as a part of the "Rapid Development of Earth-abundant thin film solar cells" agreement. E. S. T. acknowledges support of the NSF MRSEC program through the REMRSEC Center. L. L. B. acknowledges support of the Department of Defense (DoD) through National Defense Science and Engineering Graduate Fellowship (NDSEG) Program. NR 53 TC 47 Z9 48 U1 5 U2 73 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 16 PY 2013 VL 103 IS 25 AR 253902 DI 10.1063/1.4851896 PG 5 WC Physics, Applied SC Physics GA 293LU UT WOS:000329973800102 ER PT J AU Jain, PK Manthiram, K Engel, JH White, SL Faucheaux, JA Alivisatos, AP AF Jain, Prashant K. Manthiram, Karthish Engel, Jesse H. White, Sarah L. Faucheaux, Jacob A. Alivisatos, A. Paul TI Doped Nanocrystals as Plasmonic Probes of Redox Chemistry SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE copper sulfide; doping; ion exchange; nanocrystals; semiconductor plasmons ID CU2-XSE NANOCRYSTALS; QUANTUM DOTS; SENSITIVITY; RESONANCE; NANOSHELLS; SULFIDES; COLLOIDS; PBSE C1 [Jain, Prashant K.; White, Sarah L.; Faucheaux, Jacob A.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Jain, Prashant K.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Jain, Prashant K.] Univ Illinois, Mat Res Lab, Urbana, IL 61801 USA. [Manthiram, Karthish; Engel, Jesse H.; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Manthiram, Karthish] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Engel, Jesse H.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Mat Sci, Berkeley, CA 94720 USA. RP Jain, PK (reprint author), Univ Illinois, Dept Chem, 600 S Mathews Ave, Urbana, IL 61801 USA. EM jain@illinois.edu; apalivisatos@lbl.gov RI Jain, Prashant/A-4779-2009; Alivisatos , Paul /N-8863-2015 OI Jain, Prashant/0000-0002-7306-3972; Alivisatos , Paul /0000-0001-6895-9048 FU Dupont Young Professor Award; National Science Foundation Graduate Research Fellowship [DGE-1144245]; IACAT fellowship; Physical Chemistry of Inorganic Nanostructures Program [KC3103]; Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DE-AC02-05CH11231]; Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF); ORISE-ORAU [DE-AC05-06OR23100]; Self-Assembly of Organic/Inorganic Nanocomposite Materials [DE-AC02-05CH11231] FX Work by P.K.J. and S. L. W. on oxidation/reduction chemistry of nanocrystals and their plasmonic/structural characterization was supported by the Dupont Young Professor Award (P.K.J.). Simulations were supported by a National Science Foundation Graduate Research Fellowship awarded to J.F. under Grant No. DGE-1144245 and an IACAT fellowship to P.K.J. Work on methods of nanocrystal doping was supported by the Physical Chemistry of Inorganic Nanostructures Program, KC3103, Director, Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under contract DE-AC02-05CH11231 and a graduate fellowship awarded to K. M. from the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under contract no. DE-AC05-06OR23100. Electrical characterization by J.H.E. was supported by Self-Assembly of Organic/Inorganic Nanocomposite Materials (Grant DE-AC02-05CH11231 to A. P. A.). We thank Jessy Rivest for CdS nanorod samples. NR 28 TC 42 Z9 42 U1 7 U2 97 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD DEC 16 PY 2013 VL 52 IS 51 BP 13671 EP 13675 DI 10.1002/anie.201303707 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 272CF UT WOS:000328437200035 PM 24155083 ER PT J AU O'Neill, BJ Jackson, DHK Crisci, AJ Farberow, CA Shi, FY Alba-Rubio, AC Lu, JL Dietrich, PJ Gu, XK Marshall, CL Stair, PC Elam, JW Miller, JT Ribeiro, FH Voyles, PM Greeley, J Mavrikakis, M Scott, SL Kuech, TF Dumesic, JA AF O'Neill, Brandon J. Jackson, David H. K. Crisci, Anthony J. Farberow, Carrie A. Shi, Fengyuan Alba-Rubio, Ana C. Lu, Junling Dietrich, Paul J. Gu, Xiangkui Marshall, Christopher L. Stair, Peter C. Elam, Jeffrey W. Miller, Jeffrey T. Ribeiro, Fabio H. Voyles, Paul M. Greeley, Jeffrey Mavrikakis, Manos Scott, Susannah L. Kuech, Thomas F. Dumesic, James A. TI Stabilization of Copper Catalysts for Liquid-Phase Reactions by Atomic Layer Deposition SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE atomic layer deposition; biomass; catalyst stability; copper; hydrogenation ID METAL-CATALYSTS; CO ADSORPTION; DEACTIVATION AB Atomic layer deposition (ALD) of an alumina overcoat can stabilize a base metal catalyst (e.g., copper) for liquid-phase catalytic reactions (e.g., hydrogenation of biomass-derived furfural in alcoholic solvents or water), thereby eliminating the deactivation of conventional catalysts by sintering and leaching. This method of catalyst stabilization alleviates the need to employ precious metals (e.g., platinum) in liquid-phase catalytic processing. The alumina overcoat initially covers the catalyst surface completely. By using solid state NMR spectroscopy, X-ray diffraction, and electron microscopy, it was shown that high temperature treatment opens porosity in the overcoat by forming crystallites of -Al2O3. Infrared spectroscopic measurements and scanning tunneling microscopy studies of trimethylaluminum ALD on copper show that the remarkable stability imparted to the nanoparticles arises from selective armoring of under-coordinated copper atoms on the nanoparticle surface. C1 [O'Neill, Brandon J.; Crisci, Anthony J.; Farberow, Carrie A.; Alba-Rubio, Ana C.; Mavrikakis, Manos; Kuech, Thomas F.; Dumesic, James A.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Jackson, David H. K.; Shi, Fengyuan; Voyles, Paul M.; Kuech, Thomas F.] Univ Wisconsin, Mat Sci Program, Madison, WI 53706 USA. [Crisci, Anthony J.; Scott, Susannah L.] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Lu, Junling] Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Peoples R China. [Dietrich, Paul J.; Gu, Xiangkui; Ribeiro, Fabio H.; Greeley, Jeffrey] Purdue Univ, Dept Chem Engn, W Lafayette, IN 47907 USA. [Marshall, Christopher L.; Stair, Peter C.; Miller, Jeffrey T.] Argonne Natl Lab, Argonne, IL 60439 USA. [Stair, Peter C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Dumesic, JA (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. EM dumesic@engr.wisc.edu RI Mavrikakis, Manos/D-5702-2012; Lu, Junling/F-3791-2010; Gu, Xiangkui/H-3706-2014; ID, MRCAT/G-7586-2011; Shi, Fengyuan/Q-2584-2015; Marshall, Christopher/D-1493-2015 OI Mavrikakis, Manos/0000-0002-5293-5356; Lu, Junling/0000-0002-7371-8414; Shi, Fengyuan/0000-0001-9769-3824; Marshall, Christopher/0000-0002-1285-7648 FU Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy (DOE), Office of Basic Energy Sciences [DE-FG02-99ER45777, DE-FG02-84ER13183]; National Science Foundation (NSF) under Center for Enabling New Technologies through Catalysis (CENTC); MRSEC Program of the NSF [DMR05-20415]; U.S. DOE [DE-AC02-06CH11357]; DOE; MRCAT member institutions FX This material is based upon work supported as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Electron microscopy was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences (DE-FG02-99ER45777). Chemisorption/kinetics were supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences (DE-FG02-84ER13183). NMR was supported by the National Science Foundation (NSF) under the Center for Enabling New Technologies through Catalysis (CENTC) and used the Materials Research Laboratory, supported by the MRSEC Program of the NSF (DMR05-20415). Use of the Advanced Photon Source was supported by the U.S. DOE (DE-AC02-06CH11357). MRCAT operations are supported by DOE and the MRCAT member institutions. Some computational work was performed using resources from the Pacific Northwest National Laboratory and the National Energy Research Scientific Computing Center. NR 22 TC 50 Z9 50 U1 15 U2 211 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD DEC 16 PY 2013 VL 52 IS 51 BP 13808 EP 13812 DI 10.1002/anie.201308245 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 272CF UT WOS:000328437200064 PM 24282166 ER PT J AU Seisenbaeva, GA Nedelec, JM Daniel, G Tiseanu, C Parvulescu, V Pol, VG Abrego, L Kessler, VG AF Seisenbaeva, Gulaim A. Nedelec, Jean-Marie Daniel, Geoffrey Tiseanu, Carmen Parvulescu, Vasile Pol, Vilas G. Abrego, Luis Kessler, Vadim G. TI Mesoporous Anatase TiO2 Nanorods as Thermally Robust Anode Materials for Li-Ion Batteries: Detailed Insight into the Formation Mechanism SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE anatase; Li-ion battery performance; mesoporous materials; thermal stability; titania ID ELECTROCHEMICAL ENERGY-STORAGE; ELECTRODE PERFORMANCE; TITANIA NANOTUBES; LITHIUM; NANOSTRUCTURES; INTERCALATION; NANOPARTICLES; PHASE; MICROSPHERES; NANOFIBERS AB Uniformly mesoporous and thermally robust anatase nanorods were produced with quantitative yield by a simple and efficient one-step approach. The mechanism of this process was revealed by insertion of Eu3+ cations from the reaction medium as luminescent probes. The obtained structure displays an unusually high porosity, an active surface area of about 300m(2)g(-1) and a specific capacity of 167mAhg(-1) at a C/3 rate, making it attractive as an anode electrode for Li-ion batteries. An additional attractive feature is its remarkable thermal stability; heating to 400 degrees C results in a decrease in the active surface area to a still relatively high value of 110m(2)g(-1) with conservation of open mesoporosity. Thermal treatment at 800 degrees C or higher, however, causes transformation into a non-porous rutile monolith, as commonly observed with nanoscale titania. C1 [Seisenbaeva, Gulaim A.; Kessler, Vadim G.] Swedish Univ Agr Sci, Dept Chem, Bioctr, S-75007 Uppsala, Sweden. [Nedelec, Jean-Marie] Clermont Univ, ENSCCF, Inst Chim Clermont Ferrand, CNRS UMR 6296, F-63177 Clermont Ferrand, France. [Daniel, Geoffrey] Swedish Univ Agr Sci, Dept Forest Prod Wood Sci, S-75007 Uppsala, Sweden. [Tiseanu, Carmen] Natl Inst Laser Plasma & Radiat Phys, RO-76900 Bucharest, Romania. [Parvulescu, Vasile] Univ Bucuresti, Dept Chem, Bucharest 030018, Romania. [Pol, Vilas G.; Abrego, Luis] Argonne Natl Lab, Electrochem Energy Storage Dept, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Seisenbaeva, GA (reprint author), Swedish Univ Agr Sci, Dept Chem, Bioctr, Box 7015, S-75007 Uppsala, Sweden. EM gulaim.seisenbaeva@slu.se; vadim.kessler@slu.se RI NEDELEC, jean-marie/A-6920-2008; Parvulescu, Vasile/A-9117-2011; OI NEDELEC, jean-marie/0000-0002-8243-6849; Seisenbaeva, Gulaim/0000-0003-0072-6082; Kessler, Vadim/0000-0001-7570-2814; Daniel, Geoffrey/0000-0002-8886-1942 FU Swedish Research Council (Vetenskapsradet); Center for Electrical Energy Storage: Tailored Interfaces, an Energy Frontier Research Center; US Department of Energy, Office of Science, Office of Basic Energy Sciences; Romanian National Authority for Scientific Research (CNCS-UEFISCDI) [PN-II-ID-PCE-2011-3-0534] FX The authors express their gratitude to the Swedish Research Council (Vetenskapsradet) for the Support to the grant "Molecular Precursors and Molecular Models of Nanoporous Materials". V. G. P. and L. A. were supported by the Center for Electrical Energy Storage: Tailored Interfaces, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. C. T. acknowledges the support from the Romanian National Authority for Scientific Research (CNCS-UEFISCDI) (project number PN-II-ID-PCE-2011-3-0534). NR 46 TC 6 Z9 7 U1 2 U2 81 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD DEC 16 PY 2013 VL 19 IS 51 BP 17439 EP 17444 DI 10.1002/chem.201303283 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA 264OY UT WOS:000327889800025 PM 24243542 ER PT J AU Peri, D Ciston, J Gandara, F Zhao, YB Yaghi, OM AF Peri, Dani Ciston, Jim Gandara, Felipe Zhao, Yingbo Yaghi, Omar M. TI Crystalline Fibers of Metal-Peptide Double Ladders SO INORGANIC CHEMISTRY LA English DT Article ID ORGANIC FRAMEWORKS; POROUS MATERIAL AB Despite remarkable progress in the field of MOFs, structures based on long-flexible organic linkers are scarce and the majority of such materials rely on rigid linkers. In this work, crystals of a new metal-organic double ladder (MODL) are obtained by linking a pentapeptide (NH2-Glu-pCO(2)Phe-pCO(2)Phe-Ala-Gly-OH) with cadmium acetate to produce a Cd(2-pyrrolidone-pCO(2)Phe-pCO(2)Phe-Ala-Gly)(H2O)(3) framework. SEM and TEM analyses show the fibrous nature of the crystals and show that the infinite cadmium oxide rod secondary building units (SBUs) are aligned with the longitudinal axis of the nanofibers. C1 [Peri, Dani; Gandara, Felipe; Zhao, Yingbo; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Peri, Dani; Gandara, Felipe; Zhao, Yingbo; Yaghi, Omar M.] Univ Calif Berkeley, Kavli Energy Nano Sci Inst, Berkeley, CA 94720 USA. [Peri, Dani; Gandara, Felipe; Zhao, Yingbo; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ciston, Jim] Univ Calif Berkeley, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM yaghi@berkeley.edu RI EFRC, CGS/I-6680-2012; Gandara, Felipe/B-9198-2013; Stangl, Kristin/D-1502-2015; Foundry, Molecular/G-9968-2014; OI Gandara, Felipe/0000-0002-1671-6260; Yaghi, Omar/0000-0002-5611-3325 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported as part of the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0001015. The TEM portion of this work was carried out at NCEM, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 12 TC 3 Z9 3 U1 3 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 16 PY 2013 VL 52 IS 24 BP 13818 EP 13820 DI 10.1021/ic402435z PG 3 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 275IB UT WOS:000328668400006 PM 24256366 ER PT J AU Schnaars, DD Wilson, RE AF Schnaars, David D. Wilson, Richard E. TI Structural and Vibrational Properties of U(VI)O2Cl42- and Pu(VI)O2Cl42- Complexes SO INORGANIC CHEMISTRY LA English DT Article ID URANYL TETRACHLORIDE COMPLEXES; NORMAL COORDINATE ANALYSIS; ELECTRONIC-STRUCTURE; CRYSTAL-STRUCTURE; FORCE-CONSTANTS; ACTINYL IONS; INTERNUCLEAR DISTANCES; SOLUTION CHEMISTRY; INFRARED-SPECTRA; RAMAN-SPECTRA AB In actinide chemistry, it has been shown that equatorial ligands bound to the metal centers of actinyl ions have a strong influence on the chemistry and therefore the electronic structure of the O=An=O moiety. While this influence has received a significant amount of attention, considerably less research has been done to investigate how the identity of the actinide metal itself (U, Np, Pu, Am) affects the actinyl stretching frequencies. Herein, we present the structural and spectroscopic characterization of six actinyl tetrachloride compounds (M(2)AnO(2)Cl(4): M = Rb, Cs, Me4N; An = U, Pu) as well as the stretching and interactive force constants of the actinyl moiety in each species. Our results show a decrease in the stretching force constant and a weakening of the An=O bond when traversing the actinides from uranyl to plutonyl, which is interesting because the solid state molecular structures show a slight contraction of the An=O bond length when uranium is replaced with plutonium. Additionally, the interaction force constants for both the uranyl and plutonyl compounds were found to be negative, which corresponds to a reduction of the force constant for the symmetric stretching mode. C1 [Schnaars, David D.; Wilson, Richard E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Wilson, RE (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rewilson@anl.gov RI Wilson, Richard/H-1763-2011 OI Wilson, Richard/0000-0001-8618-5680 FU United States Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was performed at Argonne National Laboratory, operated for the United States Department of Energy, Office of Science, Office of Basic Energy Sciences, by UChicagoArgonne LLC under Contract DE-AC02-06CH11357. NR 103 TC 14 Z9 14 U1 7 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 16 PY 2013 VL 52 IS 24 BP 14138 EP 14147 DI 10.1021/ic401991n PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 275IB UT WOS:000328668400042 PM 24256199 ER PT J AU Musfeldt, JL Brinzari, TV Schlueter, JA Manson, JL Litvinchuk, AP Liu, Z AF Musfeldt, J. L. Brinzari, T. V. Schlueter, J. A. Manson, J. L. Litvinchuk, A. P. Liu, Z. TI Pressure-Induced Local Lattice Distortions in alpha-Co[N(CN)(2)](2) SO INORGANIC CHEMISTRY LA English DT Article ID MOLECULE-BASED MAGNET; EXCHANGE INTERACTIONS; TRANSITION; SEMICONDUCTORS; ELECTRONS; CYANIDE; SERIES; NI; CO AB This work brings together diamond anvil cell techniques, vibrational spectroscopies, and complementary lattice dynamics calculations to investigate pressure-induced local lattice distortions in alpha-Co[N(CN)(2)](2). Analysis of mode behavior and displacement patterns reveals a series of pressure-driven transitions that modify the CoN6 counter-rotations, distort the octahedra, and flatten the C-N-ax-C linkages. These local lattice distortions may be responsible for the low temperature magnetic crossover. We also discuss prospects for negative thermal expansion and show that there is not a straightforward low pressure pathway between the pink alpha and blue beta ambient pressure phases of Co[N(CN)(2)](2). C1 [Musfeldt, J. L.; Brinzari, T. V.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Schlueter, J. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Manson, J. L.] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. [Litvinchuk, A. P.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Litvinchuk, A. P.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Liu, Z.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. RP Musfeldt, JL (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RI Litvinchuk, Alexander/K-6991-2012 OI Litvinchuk, Alexander/0000-0002-5128-5232 FU PRF [52053-ND 10]; NSF [DMR-1063880, DMR-1005825]; DoE; COMPRES under NSF [EAR 06-49658] FX This research was supported by the PRF (52053-ND 10, UT), NSF (DMR-1063880, UT and DMR-1005825, EWU), and the DoE (BNL, ANL). The U2A Beam line is supported by COMPRES under NSF Cooperative Agreement EAR 06-49658. We thank Y. Song for useful discussions and P. Chen for technical assistance. NR 66 TC 4 Z9 4 U1 2 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 16 PY 2013 VL 52 IS 24 BP 14148 EP 14154 DI 10.1021/ic402010h PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 275IB UT WOS:000328668400043 PM 24299233 ER PT J AU Pereira, CCL Michelini, MD Marcalo, J Gong, Y Gibson, JK AF Pereira, Claudia C. L. Michelini, Maria del Carmen Marcalo, Joaquim Gong, Yu Gibson, John K. TI Synthesis and Properties of Uranium Sulfide Cations. An Evaluation of the Stability of Thiouranyl, {S=U=S}(2+) SO INORGANIC CHEMISTRY LA English DT Article ID GAS-PHASE CHEMISTRY; URANYL-ION; INFRARED-SPECTRA; IMIDO ANALOGS; BASIS-SETS; THERMOCHEMISTRY; COMPLEXES; BONDS; METAL; TE AB Atomic uranium cations, U+ and U2+, reacted with the facile sulfur-atom donor OCS to produce several monopositive and dipositive uranium sulfide species containing up to four sulfur atoms. Sequential abstraction of two sulfur atoms by U2+ resulted in US22+; density functional theory computations indicate that the ground-state structure for this species is side-on eta(2)-S-2 triangular US22+, with the linear thiouranyl isomer, {S= U-VI=S}(2+), some 171 kJ mol(-1) higher in energy. The result that the linear thiouranyl structure is a local minimum at a moderate energy suggests that it should be feasible to stabilize this moiety in molecular compounds. C1 [Pereira, Claudia C. L.; Marcalo, Joaquim] Univ Lisbon, Inst Super Tecn, Ctr Ciencias & Tecnol Nucl, P-2695066 Bobadela Lrs, Portugal. [Michelini, Maria del Carmen] Univ Calabria, Dipartimento Chim, I-87030 Arcavacata Di Rende, Italy. [Gong, Yu; Gibson, John K.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Michelini, MD (reprint author), Univ Calabria, Dipartimento Chim, I-87030 Arcavacata Di Rende, Italy. EM mc.michelini@unical.it; jmarcalo@ctn.ist.utl.pt RI PTMS, RNEM/C-1589-2014; Marcalo, Joaquim/J-5476-2013; OI Marcalo, Joaquim/0000-0001-7580-057X; Pereira, Claudia/0000-0003-3421-8676 FU Fundacao para a Ciencia e a Tecnologia; Universita della Calabria; U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by Fundacao para a Ciencia e a Tecnologia under the Ciencia 2007 Programme, by Universita della Calabria, and by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL under Contract DE-AC02-05CH11231 (Y.G. and J.K.G.). The OCS was a generous gift from Dr. Joao M. A. Frazao at ISEL, Lisbon, Portugal. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 57 TC 1 Z9 1 U1 2 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 16 PY 2013 VL 52 IS 24 BP 14162 EP 14167 DI 10.1021/ic4020493 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 275IB UT WOS:000328668400045 PM 24256167 ER PT J AU Johnstone, EV Poineau, F Starkey, J Hartmann, T Forster, PM Ma, LZ Hilgar, J Rodriguez, EE Farmand, R Czerwinski, KR Sattelberger, AP AF Johnstone, Erik V. Poineau, Frederic Starkey, Jenna Hartmann, Thomas Forster, Paul M. Ma, Longzhou Hilgar, Jeremy Rodriguez, Efrain E. Farmand, Romina Czerwinski, Kenneth R. Sattelberger, Alfred P. TI Synthetic and Coordination Chemistry of the Heavier Trivalent Technetium Binary Halides: Uncovering Technetium Triiodide SO INORGANIC CHEMISTRY LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; RHENIUM(III) IODIDE; METAL CARBOXYLATES; CHLORIDE; TRICHLORIDE; TRIHALIDES; BROMIDE; CRYSTAL; CLUSTER; SYSTEM AB Technetium tribromide and triiodide were obtained from the reaction of the quadruply Tc-Tc-bonded dimer Tc-2(O2CCH3)(4)Cl-2 with flowing HX(g) (X = Br, I) at elevated temperatures. At 150 and 300 degrees C, the reaction with HBr(g) yields TcBr3 crystallizing with the TiI3 structure type. The analogous reactions with flowing HI(g) yield TcI3, the first technetium binary iodide to be reported. Powder X-ray diffraction (PXRD) measurements show the compound to be amorphous at 150 degrees C and semicrystalline at 300 degrees C. X-ray absorption fine structure spectroscopy indicates TcI3 to consist of face-sharing TcI6 octahedra. Reactions of technetium metal with elemental iodine in a sealed Pyrex ampules in the temperature range 250-400 degrees C were performed. At 250 degrees C, no reaction occurred, while the reaction at 400 degrees C yielded a product whose PXRD pattern matches the one of TcI3 obtained from the reaction of Tc-2(O2CCH3)(4)Cl-2 and flowing HI(g). The thermal stability of TcBr3 and TcI3 was investigated in Pyrex and/or quartz ampules at 450 degrees C under vacuum. Technetium tribromide decomposes to Na{[TC6Br12](2)Br} in a Pyrex ampule and to technetium metal in a quartz ampule; technetium triiodide decomposes to technetium metal in a Pyrex ampule. C1 [Johnstone, Erik V.; Poineau, Frederic; Forster, Paul M.; Hilgar, Jeremy; Farmand, Romina; Czerwinski, Kenneth R.; Sattelberger, Alfred P.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Starkey, Jenna] Virginia Wesleyan Coll, Dept Chem, Norfolk, VA 23502 USA. [Hartmann, Thomas; Ma, Longzhou] Harry Reid Ctr Environm Studies, Las Vegas, NV 89154 USA. [Rodriguez, Efrain E.] Univ Maryland, Dept Chem, College Pk, MD 20742 USA. [Sattelberger, Alfred P.] Argonne Natl Lab, Energy Engn & Syst Anal Directorate, Argonne, IL 60439 USA. RP Johnstone, EV (reprint author), Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. EM erikvjohnstone@gmail.com FU NEUP from the U.S. Department of Energy, Office of Nuclear Energy, through INL/BEA, LLC [89445]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Funding for this research was provided by NEUP grant "Development of Alternative Technetium Waste Forms" from the U.S. Department of Energy, Office of Nuclear Energy, through INL/BEA, LLC (Grant 89445). Use of the Advanced Photon Source (APS) at Argonne was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. The authors thank Trevor Low and Julie Bertoia for exceptional health physics support, Dr. Minghua Ren for significant support with SEM and EDX, and Dr. Sungsik Lee at the APS for outstanding support during EXAFS experiments. NR 57 TC 2 Z9 2 U1 0 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 16 PY 2013 VL 52 IS 24 BP 14309 EP 14316 DI 10.1021/ic402278c PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 275IB UT WOS:000328668400063 PM 24295331 ER PT J AU Dong, YK Wang, H Nolas, GS AF Dong, Yongkwan Wang, Hsin Nolas, George S. TI Synthesis, Crystal Structure, and High Temperature Transport Properties of p-Type Cu2Zn1-xFexSnSe4 SO INORGANIC CHEMISTRY LA English DT Article ID THERMOELECTRIC PROPERTIES; STANNITE; CU; SEMICONDUCTOR; NANOCRYSTALS; OXYSELENIDES; CU2CDSNSE4; BICUSEO; SERIES AB Iron substituted Cu2Zn1-xFexSnSe4 stannites were synthesized by reaction of the constituent elements and subsequent annealing, followed by densification by hot-pressing. The compositions for each specimen were confirmed with a combination of Rietveld refinement and elemental analysis. Refinement results indicated that only the 2a site was occupied by Zn and Fe. High temperature transport properties were measured from 300 to 800 K. The electrical resistivity and thermal conductivity decrease with increasing Fe content. For the lower Fe content specimens with x = 0.2 and 0.4, the electrical properties are strongly temperature dependent, unlike that of the higher Fe content specimens (x = 0.6 and 0.8). A maximum ZT value of 0.46 was obtained at 800 K for Cu(2)Zn(0.4)Fe(0.6)Sn(5)e(4). C1 [Dong, Yongkwan; Nolas, George S.] Univ S Florida, Dept Phys, Tampa, FL 33620 USA. [Wang, Hsin] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Nolas, GS (reprint author), Univ S Florida, Dept Phys, Tampa, FL 33620 USA. EM gnolas@usf.edu RI Wang, Hsin/A-1942-2013 OI Wang, Hsin/0000-0003-2426-9867 FU National Science Foundation; Department of Energy Partnership on Thermoelectric Devices for Vehicle Applications [1048796]; Oak Ridge National Laboratory [DE-AC05000OR22725] FX Y.D. and G.S.N. gratefully acknowledge financial support from the National Science Foundation and Department of Energy Partnership on Thermoelectric Devices for Vehicle Applications (Grant No. 1048796). H.W. would like to thank the support of the assistant secretary for Energy Efficiency and Renewable Energy of the Department of Energy and the Propulsion Materials program under the Vehicle Technologies program. Oak Ridge National Laboratory is managed by UT-Battelle LLC under contract DE-AC05000OR22725. NR 29 TC 10 Z9 10 U1 2 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 16 PY 2013 VL 52 IS 24 BP 14364 EP 14367 DI 10.1021/ic402455x PG 4 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 275IB UT WOS:000328668400069 PM 24283617 ER PT J AU Wiedner, ES Appel, AM DuBois, DL Bullock, RM AF Wiedner, Eric S. Appel, Aaron M. DuBois, Daniel L. Bullock, R. Morris TI Thermochemical and Mechanistic Studies of Electrocatalytic Hydrogen Production by Cobalt Complexes Containing Pendant Amines SO INORGANIC CHEMISTRY LA English DT Article ID CYCLIC DIPHOSPHINE LIGANDS; TRANS-DIHYDRIDE COMPLEX; H-2 PRODUCTION; HYDRIDE DONOR; H BOND; COBALOXIME CATALYSTS; ELECTRODE-POTENTIALS; DITHIOLENE COMPLEXES; DIHYDROGEN COMPLEXES; FUNCTIONAL MODELS AB Two cobalt(tetraphosphine) complexes [Co-((p(2)(nC-Pph2)N(2)(ph))(CH3CN)RBF4)(2) with a tetradentate phosphine ligand (p(2)(nC-Pph2)N(2)(ph) = 1,5-diphenyl-3,7-bis((diphenylphosphino)alkyl)-1,5-diaza-3,7-diphosphacyclooctane; alkyl = (CH2)(2), n = 2 (L2); (CH2)(3), n = 3 (L3)) have been studied for electrocatalytic hydrogen production using 1:1 [(DMF)H](+):DMF. A turnover frequency (TOF) of 980 s(-1) with an overpotential at E-cat/2 of 1210 mV was measured for [Co-II(L2)(CH3CN)](2+), and a TOF of 980 s(-1) with an overpotential at E-cat/2 of 930 mV was measured for [Co-II(L3)(CH3CN)](2+). Addition of water increases the TOF of [Co-II(L2)(CH3CN)(2+) to 18,000 s(-1). The catalytic wave for each of these complexes occurs at the reduction potential of the corresponding HCoIII complex. Comprehensive thermochemical studies of [Co-II(L2)(CH3CN)](2+) and [Coll(L3)(CH3CN)](2+) and species derived from them by addition/removal of protons/electrons were carried out using values measured experimentally and calculated using density functional theory (DFT). Notably, HCoI(L2) and HCoI(L3) were found to be remarkably strong hydride donors, with HCoI(L2) being a better hydride donor than BE4-. Mechanistic studies of these catalysts reveal that H-2 formation can occur by protonation of a HCoII intermediate, and that the pendant amines of these complexes facilitate proton delivery to the cobalt center. The rate-limiting step for catalysis is a net intramolecular isomerization of the protonated pendant amine from the nonproductive exoisomer to the productive endo isomer. C1 [Wiedner, Eric S.; Appel, Aaron M.; DuBois, Daniel L.; Bullock, R. Morris] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Div Phys Sci, Richland, WA 99352 USA. RP Wiedner, ES (reprint author), Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Div Phys Sci, POB 999,K2-57, Richland, WA 99352 USA. EM eric.wiedner@pnnl.gov; morris.bullock@pnnl.gov RI Bullock, R. Morris/L-6802-2016; OI Bullock, R. Morris/0000-0001-6306-4851; Wiedner, Eric/0000-0002-7202-9676; Appel, Aaron/0000-0002-5604-1253 FU Center for Molecular Electrocatalysis, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX We thank Dr. Shentan Chen for many helpful discussions. This research was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Computational resources were provided at the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy. NR 104 TC 30 Z9 30 U1 7 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 16 PY 2013 VL 52 IS 24 BP 14391 EP 14403 DI 10.1021/ic4025475 PG 13 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 275IB UT WOS:000328668400073 PM 24261463 ER PT J AU Batell, B Jung, S Wagner, CEM AF Batell, Brian Jung, Sunghoon Wagner, Carlos E. M. TI Very light charginos and Higgs decays SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; LEP HERA and SLC Physics; Supersymmetric Standard Model ID OF-MASS ENERGIES; PARITY VIOLATING DECAYS; SUSY BREAKING TOPOLOGIES; PROTON-PROTON COLLISIONS; EXPLICIT CP VIOLATION; E(+)E(-) COLLISIONS; MISSING ENERGY; SUPERSYMMETRIC PARTICLES; ATLAS DETECTOR; ROOT-S AB We explore modifications to the loop-induced Higgs couplings h gamma gamma and h gamma Z from light charginos in the Minimal Supersymmetric Standard Model. When the lightest chargino mass is above the kinematic LEP bound of order 100 GeV the effects are modest, with deviations in the decay branching ratios typically less than 15% from the Standard Model predictions. However, if the charginos are lighter than 100 GeV, more dramatic alterations to these couplings are possible as a consequence of the rise of the one loop form factor. For example, the diphoton signal strength can be enhanced by as much as 70% compared to the Standard Model value. We scrutinize in detail the existing LEP, Tevatron, and LHC searches and present a scenario in which a very light chargino with a mass as light as half the Higgs mass is allowed by all direct collider searches and electroweak precision tests. The scenario has a sneutrino LSP that decays through an R-parity violating coupling and has a macroscopic decay length of order 10-100 cm. The characteristic signature is a displaced e mu resonance arising when a sneutrino decays in the inner detector. We outline potential search strategies to test this scenario at the LHC. C1 [Batell, Brian; Jung, Sunghoon; Wagner, Carlos E. M.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Batell, Brian; Jung, Sunghoon; Wagner, Carlos E. M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Jung, Sunghoon] Korea Inst Adv Study, Seoul 130722, South Korea. [Wagner, Carlos E. M.] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. [Wagner, Carlos E. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Batell, B (reprint author), Univ Chicago, Dept Phys, 5720 S Ellis Ave, Chicago, IL 60637 USA. EM batell@uchicago.edu; nejsh21@kias.re.kr; cwagner@hep.anl.gov FU U.S. Department of Energy [DE-AC02-06CH11357]; NSF [PHY-0756966]; DOE [DE-SC0003930]; Los Alamos National Laboratory FX We thank Y. Gershtein, P. Ko, H.M. Lee, S. Martin, T. Roy, P. Saraswat, and L.T. Wang for helpful discussions. Work at ANL is supported in part by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. B.B. is supported by the NSF under grant PHY-0756966 and the DOE Early Career Award under grant DE-SC0003930. S.J. thanks KIAS Center for Advanced Computation for providing computing resources. B.B. and C.W. thank the Aspen Center for Physics and the KITP, Santa Barbara, where part of the work has been done. B.B. also thanks KIAS and the 2013 Santa Fe workshop INFO, sponsored by Los Alamos National Laboratory, where part of this work was completed. NR 124 TC 15 Z9 15 U1 0 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD DEC 16 PY 2013 IS 12 AR 075 DI 10.1007/JHEP12(2013)075 PG 30 WC Physics, Particles & Fields SC Physics GA 278NN UT WOS:000328897100001 ER PT J AU Craig, IM Taubman, MS Lea, AS Phillips, MC Josberger, EE Raschke, MB AF Craig, Ian M. Taubman, Matthew S. Lea, A. Scott Phillips, Mark C. Josberger, Erik E. Raschke, Markus B. TI Infrared near-field spectroscopy of trace explosives using an external cavity quantum cascade laser SO OPTICS EXPRESS LA English DT Article ID ELASTIC LIGHT-SCATTERING; LOCK-IN DETECTION; OPTICAL MICROSCOPY; SPATIAL-RESOLUTION; ANALYTICAL-MODEL; TIP; ABSORPTION; NANOSCOPY; RDX AB Utilizing a broadly-tunable external cavity quantum cascade laser for scattering-type scanning near-field optical microscopy (s-SNOM), we measure infrared spectra of particles of explosives by probing characteristic nitro-group resonances in the 7.1-7.9 mu m wavelength range. Measurements are presented with spectral resolution of 0.25 cm(-1), spatial resolution of 25 nm, sensitivity better than 100 attomoles, and at a rapid acquisition time of 90 s per spectrum. We demonstrate high reproducibility of the acquired s-SNOM spectra with very high signal-to-noise ratios and relative noise of <0.02 in self-homodyne detection. (C) 2013 Optical Society of America C1 [Craig, Ian M.; Lea, A. Scott] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Craig, Ian M.; Taubman, Matthew S.; Phillips, Mark C.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Josberger, Erik E.; Raschke, Markus B.] Univ Colorado, Dept Chem, Dept Phys, Boulder, CO 80303 USA. [Josberger, Erik E.; Raschke, Markus B.] Univ Colorado, JILA, Boulder, CO 80303 USA. RP Phillips, MC (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. EM mark.phillips@pnnl.gov RI Craig, Ian/C-3799-2009; Raschke, Markus/F-8023-2013; OI Craig, Ian/0000-0003-4481-3700; Lea, Alan/0000-0002-4232-1553 FU U.S. Department of Energy [DE-AC05-76RL01830]; Department of Energy's Office of Biological and Environmental Research FX The research is part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multi-program national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. The work was performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. A portion of this research was made possible through the "Development of capability for Scanning-Probe Infrared-Spectroscopic Imaging with Nanometer Spatial Resolution" Scientific Partner Proposal at EMSL. NR 50 TC 16 Z9 16 U1 2 U2 48 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD DEC 16 PY 2013 VL 21 IS 25 BP 30401 EP 30414 DI 10.1364/OE.21.030401 PG 14 WC Optics SC Optics GA 273ZV UT WOS:000328575700027 PM 24514618 ER PT J AU Poplawsky, JD Nishikawa, A Fujiwara, Y Dierolf, V AF Poplawsky, Jonathan D. Nishikawa, Atsushi Fujiwara, Yasufumi Dierolf, Volkmar TI Defect roles in the excitation of Eu ions in Eu:GaN SO OPTICS EXPRESS LA English DT Article ID ELECTRON AB Eu ions in situ doped in GaN with V/III ratios varying from 3200 to 9600 have been investigated using resonant site-selective photoluminescence (PL), power dependent cathodoluminescence (CL), and a unique electron beam power dependent dual excitation experiment combining the techniques of PL and CL. The results of these experiments reveal the role of defects in the electronic excitation of Eu ions and the link between the GaN host and Eu ion dopants. The relative number of beneficial defects present in each sample for a majority Eu site (Eu1) and a specific secondary site (Eu2) are revealed. Also, a room temperature activated non-radiative recombination pathway linked to a specific, sample dependent Eu2 excitation pathway is identified. Unlike conventional GaN LEDs, Eu: GaN device performance does not rely completely on crystalline quality, but on the presence of specific excitation enhancing defects and the absence of non-radiative de-excitation channels. (C) 2013 Optical Society of America C1 [Poplawsky, Jonathan D.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Poplawsky, Jonathan D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Nishikawa, Atsushi; Fujiwara, Yasufumi] Osaka Univ, Div Mat & Mfg Sci, Osaka, Japan. [Poplawsky, Jonathan D.; Dierolf, Volkmar] Lehigh Univ, Dept Phys, Bethlehem, PA 18015 USA. RP Poplawsky, JD (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM poplawskyjd@ornl.gov RI Fujiwara, Yasufumi/D-9052-2012; Poplawsky, Jonathan/Q-2456-2015 OI Poplawsky, Jonathan/0000-0002-4272-7043 FU Japan Society for the Promotion of Science [19GS1209, 24226009]; Global Centre of Excellence Program "Advanced Structural and Functional Materials Design" from the Ministry of Education, Culture, Sports, Science and Technology of Japan; NSF [ECCS-1140038] FX This work was partly supported by a Grant-in-Aid for Creative Scientific Research (Grant No. 19GS1209) and a Grant-in-Aid for Scientific Research (S) (Grant No. 24226009) from the Japan Society for the Promotion of Science, and partly by the Global Centre of Excellence Program "Advanced Structural and Functional Materials Design" from the Ministry of Education, Culture, Sports, Science and Technology of Japan. All experimental work was preformed at Lehigh University supported by NSF grant ECCS-1140038. NR 14 TC 4 Z9 4 U1 1 U2 18 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD DEC 16 PY 2013 VL 21 IS 25 BP 30633 EP 30641 DI 10.1364/OE.21.030633 PG 9 WC Optics SC Optics GA 273ZV UT WOS:000328575700048 PM 24514639 ER PT J AU Stoupin, S Shvyd'ko, YV Shu, D Blank, VD Terentyev, SA Polyakov, SN Kuznetsov, MS Lemesh, I Mundboth, K Collins, SP Sutter, JP Tolkiehn, M AF Stoupin, S. Shvyd'ko, Y. V. Shu, D. Blank, V. D. Terentyev, S. A. Polyakov, S. N. Kuznetsov, M. S. Lemesh, I. Mundboth, K. Collins, S. P. Sutter, J. P. Tolkiehn, M. TI Hybrid diamond-silicon angular-dispersive x-ray monochromator with 0.25-meV energy bandwidth and high spectral efficiency SO OPTICS EXPRESS LA English DT Article ID SYNCHROTRON-RADIATION; OPTICAL-ELEMENTS; RESOLUTION; SCATTERING; SPECTROSCOPY; CRYSTALS AB We report on the design, implementation, and performance of an x-ray monochromator with ultra-high energy resolution (Delta E/E similar or equal to 2.7 x 10(-8)) and high spectral efficiency using x rays with photon energies E similar or equal to 9.13 keV. The operating principle of the monochromator is based on the phenomenon of angular dispersion in Bragg back-diffraction. The optical scheme of the monochromator is a modification of a scheme reported earlier [Shvyd'ko et al., Phys. Rev. A 84, 053823 (2011)], where a collimator/wavelength selector Si crystal was replaced with a 100-m m-thick type IIa diamond crystal. This modification provides a very-small-energy bandwidth Delta E similar or equal to 0.25 meV, a 3-fold increase in the aperture of the accepted beam, a reduction in the cumulative angular dispersion rate of x rays emanating from the monochromator for better focusing on a sample, a sufficient angular acceptance matching the angular divergence of an undulator source (approximate to 10 mu rad), and an improved throughput due to low x-ray absorption in the thin diamond crystal. The measured spectral efficiency of the monochromator was approximate to 65% with an aperture of 0.3 x 1 mm(2). The performance parameters of the monochromator are suitable for inelastic x-ray spectroscopy with an absolute energy resolution Delta E < 1 meV. (C) 2013 Optical Society of America C1 [Stoupin, S.; Shvyd'ko, Y. V.; Shu, D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Blank, V. D.; Terentyev, S. A.; Polyakov, S. N.; Kuznetsov, M. S.; Lemesh, I.] Technol Inst Superhard & Novel Carbon Mat, Moscow, Russia. [Polyakov, S. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Mundboth, K.; Collins, S. P.; Sutter, J. P.] Diamond Light Source, Oxford, England. [Tolkiehn, M.] DESY, Hamburg, Germany. RP Stoupin, S (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM sstoupin@aps.anl.gov RI Blank, Vladimir/A-5577-2014 FU Russian Ministry of Education and Science [16.552.11.7014]; U.S. DOE [DE-AC02-06CH11357] FX We are grateful to L. Young for support of this project at the Advanced Photon Source. We thank T. Roberts, K. Goetze, J. Kirchman, R. Krakora, W. Jansma, and S. Ross for help with instrumentation and controls. J. Kim, M. Upton, and Y. Ding are acknowledged for technical support of the experiment. The present work was supported through a research grant from the Russian Ministry of Education and Science (Contract Nos.16.552.11.7014). Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 38 TC 14 Z9 14 U1 0 U2 7 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD DEC 16 PY 2013 VL 21 IS 25 BP 30932 EP 30946 DI 10.1364/OE.21.030932 PG 15 WC Optics SC Optics GA 273ZV UT WOS:000328575700075 PM 24514666 ER PT J AU Laporte, GPJ Conkey, DB Vasdekis, A Piestun, R Psaltis, D AF Laporte, G. P. J. Conkey, D. B. Vasdekis, A. Piestun, R. Psaltis, D. TI Double-helix enhanced axial localization in STED nanoscopy SO OPTICS EXPRESS LA English DT Article ID POINT-SPREAD FUNCTIONS; FLUORESCENCE MICROSCOPY; 3-DIMENSIONAL TRACKING; RESOLUTION; INCREASE; LIGHT AB Stimulated Emission Depletion (STED) microscopy enables subdiffraction resolution in the imaging plane. However, STED's lateral improvement in resolution is generally better than the enhancement in the axial direction. Here, we combine conventional STED superresolution imaging with Double Helix Point Spread Function (PSF) modulation for axial localization with a precision better than the classical Rayleigh limit. To demonstrate the capability of the method we resolve in a STED microscope sub-diffraction fluorescent bead assemblies, and localize them axially with better than 25nm precision. We also show that the same setup allows straightforward implementation of wide field phase contrast by imaging larger beads with spiral and dark field phase filtering. (C) 2013 Optical Society of America C1 [Laporte, G. P. J.; Psaltis, D.] Ecole Polytech Fed Lausanne, Sch Engn, Lab Opt, Stn 17, CH-1015 Lausanne, Switzerland. [Conkey, D. B.; Piestun, R.] Univ Colorado, Dept Elect Comp & Energy Engn, Boulder, CO 80309 USA. [Vasdekis, A.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Laporte, GPJ (reprint author), Ecole Polytech Fed Lausanne, Sch Engn, Lab Opt, Stn 17, CH-1015 Lausanne, Switzerland. EM gregoire.laporte@epfl.ch OI Vasdekis, Andreas/0000-0003-4315-1047 FU Swiss SystemX.ch [2010/072] FX We would like to thank Prof. Bart Deplancke for helpful discussions and Dr. Marcel Leutenegger for his advices about the STED microscope implementation. We thankfully acknowledge support from Swiss SystemX.ch through grant No2010/072. NR 26 TC 2 Z9 2 U1 2 U2 24 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD DEC 16 PY 2013 VL 21 IS 25 BP 30984 EP 30992 DI 10.1364/OE.21.030984 PG 9 WC Optics SC Optics GA 273ZV UT WOS:000328575700080 PM 24514671 ER PT J AU Liu, B Braiman, Y AF Liu, B. Braiman, Y. TI Coherent beam combining of high power broad-area laser diode array with near diffraction limited beam quality and high power conversion efficiency SO OPTICS EXPRESS LA English DT Article ID EXTERNAL TALBOT CAVITY; PHASE-LOCKED ARRAYS; SINGLE-LOBED BEAM; SEMICONDUCTOR-LASER; FEEDBACK; BAR; EMISSION; LOCKING; OUTPUT; NM AB We explored a path of achieving high quality phase-locking of broad-area laser diode (BALD) array that operates at high electrical to optical power conversion efficiency (PCE). We found that (a) improving single transverse mode control for each individual BALD, (b) employing global Talbot optical coupling among diodes, and (c) enhancing strength of optical coupling among diodes are key factors in achieving high quality phase-locking of high power BALD array. Subsequently, we redesigned and improved a V-shaped external Talbot cavity and employed low reflectivity anti-reflection (AR) coated, low-"smile" BALD array to meet these three important requirements. We demonstrated near-diffraction limit far-field coherent pattern with 19% PCE and 95% visibility. The far-field angle (full-width at half-maximum (FWHM)) of center lobe was measured as 1.5 diffraction angular limited with visibility of 99% for 5A injection current and 1.6 diffraction angular limited with visibility of 95% for 14A injection current. Power scaling of diode array is discussed. (C) 2013 Optical Society of America C1 [Liu, B.; Braiman, Y.] Oak Ridge Natl Lab, Ctr Engn Syst Adv Res, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Liu, B.; Braiman, Y.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. RP Liu, B (reprint author), Oak Ridge Natl Lab, Ctr Engn Syst Adv Res, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. EM liub@ornl.gov FU Office of Naval Research; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725]; NSF [1024660] FX This research was supported in part by the Office of Naval Research and by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory. Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725. Y. B would like to acknowledge NSF support under grant EFRI#1024660. NR 53 TC 8 Z9 8 U1 4 U2 45 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD DEC 16 PY 2013 VL 21 IS 25 BP 31218 EP 31228 DI 10.1364/OE.21.031218 PG 11 WC Optics SC Optics GA 273ZV UT WOS:000328575700105 PM 24514696 ER PT J AU Aartsen, MG Abbasi, R Ackermann, M Adams, J Aguilar, JA Ahlers, M Altmann, D Arguelles, C Auffenberg, J Bai, X Baker, M Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Bose, D Boser, S Botner, O Brayeur, L Bretz, HP Brown, AM Bruijn, R Casey, J Casier, M Chirkin, D Christov, A Christy, B Clark, K Clevermann, F Coenders, S Cohen, S Cowen, DF Silva, AHC Danninger, M Daughhetee, J Davis, JC Day, M De Clercq, C De Ridder, S Desiati, P de Vries, KD de With, M DeYoung, T Diaz-Velez, JC Dunkman, M Eagan, R Eberhardt, B Eisch, J Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feintzeig, J Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Flis, S Franckowiak, A Frantzen, K Fuchs, T Gaisser, TK Gallagher, J Gerhardt, L Gladstone, L Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grandmont, DT Grant, D Gretskov, P Groh, JC Gross, A Ha, C Ismail, AH Hallen, P Hallgren, A Halzen, F Hanson, K Heereman, D Heinen, D Helbing, K Hellauer, R Hickford, S Hill, GC Hoffman, KD Hoffmann, R Homeier, A Hoshina, K Huelsnitz, W Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobi, E Jacobsen, J Jagielski, K Japaridze, GS Jero, K Jlelati, O Kaminsky, B Kappes, A Karg, T Karle, A Kauer, M Kelley, JL Kiryluk, J Klas, J Klein, SR Kohne, JH Kohnen, G Kolanoski, H Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krasberg, M Kriesten, A Krings, K Kroll, G Kunnen, J Kurahashi, N Kuwabara, T Labare, M Landsman, H Larson, MJ Lesiak-Bzdak, M Leuermann, M Leute, J Lunemann, J Macias, O Madsen, J Maggi, G Maruyama, R Mase, K Matis, HS McNally, F Meagher, K Merck, M Meures, T Miarecki, S Middell, E Milke, N Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Odrowski, S Olivas, A Omairat, A O'Murchadha, A Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Radel, L Rameez, M Rawlins, K Redl, P Reimann, R Resconi, E Rhode, W Ribordy, M Richman, M Riedel, B Rodrigues, JP Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Sander, HG Santander, M Sarkar, S Schatto, K Scheriau, F Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schukraft, A Schulte, L Schulz, O Seckel, D Sestayo, Y Seunarine, S Shanidze, R Sheremata, C Smith, MWE Soldin, D Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stanisha, NA Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Sullivan, GW Taavola, H Taboada, I Tamburro, A Tepe, A Ter-Antonyan, S Tesic, G Tilav, S Toale, PA Tobin, MN Toscano, S Unger, E Usner, M Vallecorsa, S van Eijndhoven, N van Overloop, A van Santen, J Vehring, M Voge, M Vraeghe, M Walck, C Waldenmaier, T Wallraff, M Weaver, C Wellons, M Wendt, C Westerhoff, S Whitehorn, N Wiebe, K Wiebusch, CH Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Ziemann, J Zierke, S Zoll, M AF Aartsen, M. G. Abbasi, R. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Altmann, D. Arguelles, C. Auffenberg, J. Bai, X. Baker, M. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Bose, D. Boeser, S. Botner, O. Brayeur, L. Bretz, H. -P. Brown, A. M. Bruijn, R. Casey, J. Casier, M. Chirkin, D. Christov, A. Christy, B. Clark, K. Clevermann, F. Coenders, S. Cohen, S. Cowen, D. F. Silva, A. H. Cruz Danninger, M. Daughhetee, J. Davis, J. C. Day, M. De Clercq, C. De Ridder, S. Desiati, P. de Vries, K. D. de With, M. DeYoung, T. Diaz-Velez, J. C. Dunkman, M. Eagan, R. Eberhardt, B. Eisch, J. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feintzeig, J. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Franckowiak, A. Frantzen, K. Fuchs, T. Gaisser, T. K. Gallagher, J. Gerhardt, L. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grandmont, D. T. Grant, D. Gretskov, P. Groh, J. C. Gross, A. Ha, C. Ismail, A. Haj Hallen, P. Hallgren, A. Halzen, F. Hanson, K. Heereman, D. Heinen, D. Helbing, K. Hellauer, R. Hickford, S. Hill, G. C. Hoffman, K. D. Hoffmann, R. Homeier, A. Hoshina, K. Huelsnitz, W. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobi, E. Jacobsen, J. Jagielski, K. Japaridze, G. S. Jero, K. Jlelati, O. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kauer, M. Kelley, J. L. Kiryluk, J. Klaes, J. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krasberg, M. Kriesten, A. Krings, K. Kroll, G. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Landsman, H. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leute, J. Luenemann, J. Macias, O. Madsen, J. Maggi, G. Maruyama, R. Mase, K. Matis, H. S. McNally, F. Meagher, K. Merck, M. Meures, T. Miarecki, S. Middell, E. Milke, N. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Odrowski, S. Olivas, A. Omairat, A. O'Murchadha, A. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Reimann, R. Resconi, E. Rhode, W. Ribordy, M. Richman, M. Riedel, B. Rodrigues, J. P. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Sander, H. -G. Santander, M. Sarkar, S. Schatto, K. Scheriau, F. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Schulz, O. Seckel, D. Sestayo, Y. Seunarine, S. Shanidze, R. Sheremata, C. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stanisha, N. A. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Strom, R. Sullivan, G. W. Taavola, H. Taboada, I. Tamburro, A. Tepe, A. Ter-Antonyan, S. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Toscano, S. Unger, E. Usner, M. Vallecorsa, S. van Eijndhoven, N. van Overloop, A. van Santen, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Waldenmaier, T. Wallraff, M. Weaver, Ch. Wellons, M. Wendt, C. Westerhoff, S. Whitehorn, N. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Ziemann, J. Zierke, S. Zoll, M. CA IceCube Collaboration TI Probing the origin of cosmic rays with extremely high energy neutrinos using the IceCube Observatory SO PHYSICAL REVIEW D LA English DT Article ID COSMOGENIC NEUTRINOS; FERMI-LAT; SPECTRUM; LIMIT; PERFORMANCE; COMPONENT; SELECTION; SYSTEM; MODEL; FLUX AB We have searched for extremely high energy neutrinos using data taken with the IceCube detector between May 2010 and May 2012. Two neutrino-induced particle shower events with energies around 1 PeV were observed, as reported previously. In this work, we investigate whether these events could originate from cosmogenic neutrinos produced in the interactions of ultrahigh energy cosmic rays with ambient photons while propagating through intergalactic space. Exploiting IceCube's large exposure for extremely high energy neutrinos and the lack of observed events above 100 PeV, we can rule out the corresponding models at more than 90% confidence level. The model-independent quasidifferential 90% C. L. upper limit, which amounts to E-2 phi(nu e)+(nu mu)+(nu tau) = 1.2 x 10(-7) GeV cm(-2) s(-1) sr(-1) at 1 EeV, provides the most stringent constraint in the energy range from 10 PeV to 10 EeV. Our observation disfavors strong cosmological evolution of the highest energy cosmic-ray sources such as the Fanaroff-Riley type II class of radio galaxies. C1 [Bissok, M.; Blumenthal, J.; Coenders, S.; Euler, S.; Gretskov, P.; Hallen, P.; Heinen, D.; Jagielski, K.; Kriesten, A.; Krings, K.; Leuermann, M.; Paul, L.; Raedel, L.; Reimann, R.; Schoenen, S.; Schukraft, A.; Vehring, M.; Wallraff, M.; Wiebusch, C. H.; Zierke, S.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Aartsen, M. G.; Hill, G. C.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Bay, R.; Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [de With, M.; Kolanoski, H.; Waldenmaier, T.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Tjus, J. Becker; Fedynitch, A.; Saba, S. M.; Schoeneberg, S.; Unger, E.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Boeser, S.; Franckowiak, A.; Homeier, A.; Kowalski, M.; Schulte, L.; Stasik, A.; Usner, M.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Hanson, K.; Heereman, D.; Meures, T.; O'Murchadha, A.; Pinat, E.] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium. [Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; Golup, G.; Kunnen, J.; Maggi, G.; Miller, J.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Ishihara, A.; Mase, K.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Adams, J.; Brown, A. M.; Hickford, S.; Macias, O.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Berley, D.; Blaufuss, E.; Christy, B.; Goodman, J. A.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Meagher, K.; Olivas, A.; Redl, P.; Richman, M.; Schmidt, T.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Koskinen, D. J.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Clevermann, F.; Frantzen, K.; Fuchs, T.; Koehne, J. -H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.; Scheriau, F.; Schmitz, M.; Ziemann, J.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Grandmont, D. T.; Grant, D.; Nowicki, S. C.; Odrowski, S.; Sheremata, C.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Altmann, D.; Gora, D.; Kappes, A.] Univ Erlangen Nurnberg, Erlangen Ctr Astroparticle Phys, D-91058 Erlangen, Germany. [Aguilar, J. A.; Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [De Ridder, S.; Feusels, T.; Ismail, A. Haj; Jlelati, O.; Labare, M.; Ryckbosch, D.; van Overloop, A.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Barwick, S. W.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Bruijn, R.; Cohen, S.; Ribordy, M.] Ecole Polytech Fed Lausanne, High Energy Phys Lab, CH-1015 Lausanne, Switzerland. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Abbasi, R.; Ahlers, M.; Arguelles, C.; Auffenberg, J.; Baker, M.; BenZvi, S.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Tobin, M. N.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Abbasi, R.; Ahlers, M.; Arguelles, C.; Auffenberg, J.; Baker, M.; BenZvi, S.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Tobin, M. N.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Baum, V.; Eberhardt, B.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Bernhard, A.; Gross, A.; Leute, J.; Resconi, E.; Schulz, O.; Sestayo, Y.] Tech Univ Munich, D-85748 Garching, Germany. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DC 19716 USA. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DC 19716 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bose, D.; Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Clark, K.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Larson, M. J.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Cowen, D. F.; DeYoung, T.; Dunkman, M.; Eagan, R.; Groh, J. C.; Smith, M. W. E.; Stanisha, N. A.; Tesic, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Boersma, D. J.; Botner, O.; Hallgren, A.; de los Heros, C. Perez; Strom, R.; Taavola, H.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D.; Tepe, A.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Silva, A. H. Cruz; Gluesenkamp, T.; Jacobi, E.; Kaminsky, B.; Karg, T.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Stoessl, A.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. [Bai, X.] South Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Montaruli, T.] Dipartimento Fis, Sez INFN, I-70126 Bari, Italy. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Ishihara, A (reprint author), Chiba Univ, Dept Phys, Chiba 2638522, Japan. EM aya@hepburn.s.chiba-u.ac.jp; mase@hepburn.s.chiba-u.ac.jp; syoshida@hepburn.s.chiba-u.ac.jp RI Taavola, Henric/B-4497-2011; Tjus, Julia/G-8145-2012; Wiebusch, Christopher/G-6490-2012; Auffenberg, Jan/D-3954-2014; Koskinen, David/G-3236-2014; Aguilar Sanchez, Juan Antonio/H-4467-2015; Maruyama, Reina/A-1064-2013; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; OI Groh, John/0000-0001-9880-3634; Taavola, Henric/0000-0002-2604-2810; Perez de los Heros, Carlos/0000-0002-2084-5866; Arguelles Delgado, Carlos/0000-0003-4186-4182; Ter-Antonyan, Samvel/0000-0002-5788-1369; Schukraft, Anne/0000-0002-9112-5479; Wiebusch, Christopher/0000-0002-6418-3008; Auffenberg, Jan/0000-0002-1185-9094; Koskinen, David/0000-0002-0514-5917; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Maruyama, Reina/0000-0003-2794-512X; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Rott, Carsten/0000-0002-6958-6033 FU U.S. National Science Foundation - Office of Polar Programs; U.S. National Science Foundation - Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI); Natural Sciences and Engineering Research Council of Canada; WestGrid and Compute/Calcul Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus Programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF) FX We acknowledge the support from the following agencies: U.S. National Science Foundation - Office of Polar Programs, U.S. National Science Foundation - Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus Programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF). NR 63 TC 40 Z9 41 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD DEC 16 PY 2013 VL 88 IS 11 AR 112008 DI 10.1103/PhysRevD.88.112008 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 275QS UT WOS:000328692900001 ER PT J AU Agnese, R Ahmed, Z Anderson, AJ Arrenberg, S Balakishiyeva, D Thakur, RB Bauer, DA Billard, J Borgland, A Brandt, D Brink, PL Bruch, T Bunker, R Cabrera, B Caldwell, DO Cerdeno, DG Chagani, H Cooley, J Cornell, B Crewdson, CH Cushman, P Daal, M Dejongh, F Silva, EDE Doughty, T Esteban, L Fallows, S Figueroa-Feliciano, E Filippini, J Fox, J Fritts, M Godfrey, GL Golwala, SR Hall, J Harris, RH Hertel, SA Hofer, T Holmgren, D Hsu, L Huber, ME Jastram, A Kamaev, O Kara, B Kelsey, MH Kennedy, A Kim, P Kiveni, M Koch, K Kos, M Leman, SW Loer, B Asamar, EL Mahapatra, R Mandic, V Martinez, C McCarthy, KA Mirabolfathi, N Moffatt, RA Moore, DC Nadeau, P Nelson, RH Page, K Partridge, R Pepin, M Phipps, A Prasad, K Pyle, M Qiu, H Rau, W Redl, P Reisetter, A Ricci, Y Saab, T Sadoulet, B Sander, J Schneck, K Schnee, RW Scorza, S Serfass, B Shank, B Speller, D Sundqvist, KM Villano, AN Welliver, B Wright, DH Yellin, S Yen, JJ Yoo, J Young, BA Zhang, J AF Agnese, R. Ahmed, Z. Anderson, A. J. Arrenberg, S. Balakishiyeva, D. Thakur, R. Basu Bauer, D. A. Billard, J. Borgland, A. Brandt, D. Brink, P. L. Bruch, T. Bunker, R. Cabrera, B. Caldwell, D. O. Cerdeno, D. G. Chagani, H. Cooley, J. Cornell, B. Crewdson, C. H. Cushman, P. Daal, M. Dejongh, F. do Couto e Silva, E. Doughty, T. Esteban, L. Fallows, S. Figueroa-Feliciano, E. Filippini, J. Fox, J. Fritts, M. Godfrey, G. L. Golwala, S. R. Hall, J. Harris, R. H. Hertel, S. A. Hofer, T. Holmgren, D. Hsu, L. Huber, M. E. Jastram, A. Kamaev, O. Kara, B. Kelsey, M. H. Kennedy, A. Kim, P. Kiveni, M. Koch, K. Kos, M. Leman, S. W. Loer, B. Asamar, E. Lopez Mahapatra, R. Mandic, V. Martinez, C. McCarthy, K. A. Mirabolfathi, N. Moffatt, R. A. Moore, D. C. Nadeau, P. Nelson, R. H. Page, K. Partridge, R. Pepin, M. Phipps, A. Prasad, K. Pyle, M. Qiu, H. Rau, W. Redl, P. Reisetter, A. Ricci, Y. Saab, T. Sadoulet, B. Sander, J. Schneck, K. Schnee, R. W. Scorza, S. Serfass, B. Shank, B. Speller, D. Sundqvist, K. M. Villano, A. N. Welliver, B. Wright, D. H. Yellin, S. Yen, J. J. Yoo, J. Young, B. A. Zhang, J. CA CDMS Collaboration TI Silicon Detector Dark Matter Results from the Final Exposure of CDMS II SO PHYSICAL REVIEW LETTERS LA English DT Article ID CONSTRAINTS; CANDIDATES; SEARCH AB We report results of a search for weakly interacting massive particles (WIMPS) with the silicon detectors of the CDMS II experiment. This blind analysis of 140.2 kg day of data taken between July 2007 and September 2008 revealed three WIMP-candidate events with a surface-event background estimate of 0.41(-0.08)(+0.20)(stat)(-0.24)(+0.28)(syst). Other known backgrounds from neutrons and Pb-206 are limited to <0.13 and <0.08 events at the 90% confidence level, respectively. The exposure of this analysis is equivalent to 23.4 kg day for a recoil energy range of 7-100 keV for a WIMP of mass 10 GeV/c(2). The probability that the known backgrounds would produce three or more events in the signal region is 5.4%. A profile likelihood ratio test of the three events that includes the measured recoil energies gives a 0.19% probability for the known-background-only hypothesis when tested against the alternative WIMP + background hypothesis. The highest likelihood occurs for a WIMP mass of 8.6 GeV/c(2) and WIMP-nucleon cross section of 1.9 x 10(-41) cm(2). C1 [Ahmed, Z.; Cornell, B.; Filippini, J.; Golwala, S. R.; Moore, D. C.; Nelson, R. H.] CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA. [Thakur, R. Basu; Bauer, D. A.; Dejongh, F.; Holmgren, D.; Hsu, L.; Loer, B.; Yoo, J.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Sadoulet, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Anderson, A. J.; Figueroa-Feliciano, E.; Hertel, S. A.; Leman, S. W.; McCarthy, K. A.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Hall, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Crewdson, C. H.; Fox, J.; Kamaev, O.; Martinez, C.; Nadeau, P.; Page, K.; Rau, W.; Ricci, Y.] Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada. [Young, B. A.] Santa Clara Univ, Dept Phys, Santa Clara, CA 95053 USA. [Borgland, A.; Brandt, D.; Brink, P. L.; do Couto e Silva, E.; Godfrey, G. L.; Kelsey, M. H.; Kim, P.; Partridge, R.; Schneck, K.; Wright, D. H.] Kavli Inst Particle Astrophys & Cosmol, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Cooley, J.; Kara, B.; Qiu, H.; Scorza, S.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Cabrera, B.; Moffatt, R. A.; Redl, P.; Shank, B.; Yellin, S.; Yen, J. J.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Bunker, R.; Kiveni, M.; Kos, M.; Schnee, R. W.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Harris, R. H.; Jastram, A.; Mahapatra, R.; Prasad, K.; Sander, J.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Cerdeno, D. G.; Esteban, L.; Asamar, E. Lopez] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Cerdeno, D. G.; Esteban, L.; Asamar, E. Lopez] Univ Autonoma Madrid, Inst Fis Teor UAM CSIC, E-28049 Madrid, Spain. [Billard, J.; Daal, M.; Doughty, T.; Mirabolfathi, N.; Phipps, A.; Pyle, M.; Sadoulet, B.; Serfass, B.; Speller, D.; Sundqvist, K. M.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Caldwell, D. O.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Huber, M. E.] Univ Colorado, Dept Phys, Denver, CO 80217 USA. [Reisetter, A.] Univ Evansville, Dept Phys, Evansville, IN 47722 USA. [Agnese, R.; Balakishiyeva, D.; Saab, T.; Welliver, B.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Chagani, H.; Cushman, P.; Fallows, S.; Fritts, M.; Hofer, T.; Kennedy, A.; Koch, K.; Mandic, V.; Pepin, M.; Villano, A. N.; Zhang, J.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Arrenberg, S.; Bruch, T.] Univ Zurich, Inst Phys, CH-8057 Zurich, Switzerland. RP Figueroa-Feliciano, E (reprint author), MIT, Dept Phys, Cambridge, MA 02139 USA. EM enectali@mit.edu RI Pyle, Matt/E-7348-2015; Hall, Jeter/E-9294-2015; Yoo, Jonghee/K-8394-2016; OI Pyle, Matt/0000-0002-3490-6754; Holmgren, Donald/0000-0001-6701-7737; Cerdeno, David G./0000-0002-7649-1956 FU National Science Foundation [AST-9978911, NSF-0847342, NSF-1151869, PHY-0542066, PHY-0503729, PHY-0503629, PHY-0503641, PHY-0504224, PHY-0705052, PHY-0801708, PHY-0801712, PHY-0802575, PHY-0847342, PHY-0855299, PHY-0855525, PHY-1102795, PHY-1205898]; Department of Energy [DE-AC03-76SF00098, DE-FG02-92ER40701, DE-FG02-94ER40823, DE-FG03-90ER40569, DE-FG03-91ER40618, DE-SC0004022]; Swiss National Foundation (SNF) [20-118119]; NSERC Canada [SAPIN 341314, SAPPJ 386399]; MULTIDARK Grants [CSD2009-00064, FPA2012-34694]; Fermi Research Alliance, LLC [De-AC02-07CH11359]; United States Department of Energy [DE-AC02-76SF00515] FX The CDMS Collaboration gratefully acknowledges the contributions of numerous engineers and technicians; we would like to especially thank Dennis Seitz, Jim Beaty, Bruce Hines, Larry Novak, Richard Schmitt, and Astrid Tomada. In addition, we gratefully acknowledge assistance from the staff of the Soudan Underground Laboratory and the Minnesota Department of Natural Resources. This work is supported in part by the National Science Foundation (Grants No. AST-9978911, No. NSF-0847342, No. NSF-1151869, No. PHY-0542066, No. PHY-0503729, No. PHY-0503629, No. PHY-0503641, No. PHY-0504224, No. PHY-0705052, No. PHY-0801708, No. PHY-0801712, No. PHY-0802575, No. PHY-0847342, No. PHY-0855299, No. PHY-0855525, No. PHY-1102795, and No. PHY-1205898), by the Department of Energy (Contracts No. DE-AC03-76SF00098, No. DE-FG02-92ER40701, No. DE-FG02-94ER40823, No. DE-FG03-90ER40569, No. DE-FG03-91ER40618, and No. DE-SC0004022), by the Swiss National Foundation (SNF Grant No. 20-118119), by NSERC Canada (Grants No. SAPIN 341314 and No. SAPPJ 386399), and by MULTIDARK Grants No. CSD2009-00064 and No. FPA2012-34694. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. De-AC02-07CH11359, while SLAC is operated under Contract No. DE-AC02-76SF00515 with the United States Department of Energy. NR 36 TC 266 Z9 271 U1 16 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 16 PY 2013 VL 111 IS 25 AR 251301 DI 10.1103/PhysRevLett.111.251301 PG 6 WC Physics, Multidisciplinary SC Physics GA 278IN UT WOS:000328883000001 PM 24483735 ER PT J AU Rubio, EJ Martinez, G Noor-A-Alam, M Stafford, SW Shutthanandan, V Ramana, CV AF Rubio, E. J. Martinez, G. Noor-A-Alam, M. Stafford, S. W. Shutthanandan, V. Ramana, C. V. TI Microstructure and thermal oxidation behavior of yttria-stabilized hafnia nanostructured coatings deposited on alumina SO SURFACE & COATINGS TECHNOLOGY LA English DT Article DE Yttria-stabilized hafnia; Thermal barrier coatings; Nanostructure; Phase evolution; Microstructure; Thermal oxidation ID BARRIER COATINGS; THIN-FILMS; CERAMIC COATINGS; GRAIN-SIZE; ZIRCONIA; CONDUCTIVITY; GROWTH AB Nanostructured yttria-stabilized hafnia (YSH) coatings were grown on alpha-Al2O3 substrates with variable coating thickness in a wide range of similar to 50 nm to 1 mu m. Microstructure and thermal oxidation behavior of the grown YSH coatings were studied employing X-ray diffraction (XRD), Rutherford backscattering spectrometry (RBS), scanning electron microscopy (SEM) and isothermal furnace oxidation testing. The effect of coating thickness on the crystal structure, surface/interface morphology and thermal oxidation was investigated. X-ray diffraction analyses revealed the formation of monoclinic phase for relatively thin coatings (<100 nm) indicating that the interfacial phenomena play a dominant role in phase stabilization. The evolution towards stabilized cubic phase with increasing coating thickness is observed. The SEM results indicate the dense, columnar structure of YSH coatings as a function of thickness. Thermal oxidation measurements indicate the enhanced high-temperature oxidation resistance of cubic YSH coatings. (C) 2013 Elsevier B.V. All rights reserved. C1 [Rubio, E. J.; Martinez, G.; Noor-A-Alam, M.; Ramana, C. V.] Univ Texas El Paso, Dept Mech Engn, El Paso, TX 79968 USA. [Stafford, S. W.] Univ Texas El Paso, Dept Met & Mat Engn, El Paso, TX 79968 USA. [Shutthanandan, V.] PNNL, EMSL, Richland, WA 99352 USA. RP Ramana, CV (reprint author), Univ Texas El Paso, Dept Mech Engn, El Paso, TX 79968 USA. EM rychintalapalle@utep.edu FU Department of Energy [DE-FE0000765]; National Science Foundation [NSF-DMR-0521650]; Department of Energy's Office of Biological and Environmental Research FX This material is based upon work supported by the Department of Energy under Award Number DE-FE0000765. The Hitachi 4800 SEM used for the morphology and X-ray chemical analysis of the samples in this work was acquired through the support from the National Science Foundation (NSF-DMR-0521650). A portion of the research (RBS measurements) was performed using the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 34 TC 1 Z9 1 U1 2 U2 10 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0257-8972 J9 SURF COAT TECH JI Surf. Coat. Technol. PD DEC 15 PY 2013 VL 236 BP 142 EP 148 DI 10.1016/j.surfcoat.2013.09.004 PG 7 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA 292EF UT WOS:000329884300021 ER PT J AU Salam, S Hou, PY Zhang, YD Zhang, XH Wang, HF Zhang, C Yang, ZG AF Salam, S. Hou, P. Y. Zhang, Y. -D. Zhang, X. -H. Wang, H. -F. Zhang, C. Yang, Z. -G. TI Microstructural modelling solution for complex Co based alloys and coatings SO SURFACE & COATINGS TECHNOLOGY LA English DT Article DE Thermo-Calc; MCrAlY; Bond coat; Microstructure; Hardness ID CYCLIC-OXIDATION; GAMMA' EQUILIBRIUM; PHASE-EQUILIBRIA; BOND COAT; SYSTEM; SUPERALLOY; RE; RESISTANCE AB Microstructural changes following oxidation at high temperatures of a complex coating or alloy can significantly influence its properties. This paper investigates possible solutions that can accurately model alloy microstructures that result from such a process in a cobalt-rich CoNiCrAIReY bond coat alloy system. Four different alloys with varying aluminum content were studied after heat treatments at 1000 degrees C or 1150 degrees C. SEM, EPMA and XRD were used to characterize the alloy microstructure, and hardness testing was performed to determine the role of microstructure on mechanical properties. Experimental microstructures were modeled using two databases of Thermo-Calc, namely TTNI8 and SSOL5. Effects of Al content on phase changes and materials properties were quantitatively investigated. Data showed that a 1 wt. % increase of Al in the alloy caused an 8% increase in the beta phase, and a Cr and Re rich sigma phase precipitated preferentially at high Al concentrations. In addition, alloy hardness was found to increase by 4 and 81%, respectively, with a 10% increase in the beta and sigma phases. Modeled results using the TTNI8 database showed excellent agreement with experimental observations, but the SSOL5 database produced erroneous information. (C) 2013 Elsevier B.V. All rights reserved. C1 [Salam, S.; Zhang, Y. -D.; Zhang, X. -H.; Wang, H. -F.; Zhang, C.; Yang, Z. -G.] Tsinghua Univ, Sch Mat Sci & Engn, Key Lab Adv Mat, Minist Educ, Beijing 100084, Peoples R China. [Hou, P. Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Yang, ZG (reprint author), Tsinghua Univ, Sch Mat Sci & Engn, Key Lab Adv Mat, Minist Educ, Beijing 100084, Peoples R China. EM zgyang@tsinghua.edu.cn OI Salam, Shahzad/0000-0002-6710-2947 FU National Basic Research Program of China [2010CB731600]; National Natural Science Foundation of China (NSFC) [51101091] FX The authors are grateful for the financial support by both the National Basic Research Program of China (2010CB731600) and the National Natural Science Foundation of China (NSFC No. 51101091). NR 28 TC 3 Z9 3 U1 2 U2 13 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0257-8972 J9 SURF COAT TECH JI Surf. Coat. Technol. PD DEC 15 PY 2013 VL 236 BP 510 EP 517 DI 10.1016/j.surfcoat.2013.10.059 PG 8 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA 292EF UT WOS:000329884300069 ER PT J AU Xiong, R Sun, FC He, HW Nguyen, TD AF Xiong, Rui Sun, Fengchun He, Hongwen Trong Duy Nguyen TI A data-driven adaptive state of charge and power capability joint estimator of lithium-ion polymer battery used in electric vehicles SO ENERGY LA English DT Article DE Electric vehicles; Lithium-ion polymer battery; Data-driven; Adaptive extended Kalman filter; State of charge (SoC); State of power capability (SOP) ID EXTENDED KALMAN FILTER; ONLINE ESTIMATION; PERFORMANCE; MANAGEMENT; SERIES; CELLS; MODEL AB An accurate SoC (state of charge) and SoP (state of power capability) joint estimator is the most significant techniques for electric vehicles. This paper makes two contributions to the existing literature. (1) A data-driven parameter identification method has been proposed for accurately capturing the real-time characteristic of the battery through the recursive least square algorithm, where the parameter of the battery model is updated with the real-time measurements of battery current and voltage at each sampling interval. (2) An adaptive extended Kalman filter algorithm based multi-state joint estimator has been developed in accordance with the relationship of the battery SoC and its power capability. Note that the SoC and SoP can be predicted accurately against the degradation and various operating environments of the battery through the data-driven parameter identification method. The robustness of the proposed data-driven joint estimator has been verified by different degradation states of lithium-ion polymer battery cells. The result indicates that the estimation errors of voltage and SoC are less than 1% even if given a large erroneous initial state of joint estimator, which makes the SoP estimate more accurate and reliable for the electric vehicles application. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Xiong, Rui; Sun, Fengchun; He, Hongwen] Beijing Inst Technol, Natl Engn Lab Elect Vehicles, Sch Mech Engn, Beijing 100081, Peoples R China. [Xiong, Rui; Trong Duy Nguyen] Univ Michigan, Dept Elect & Comp Engn, DOE GATE Ctr Elect Drive Transportat, Dearborn, MI 48128 USA. RP Xiong, R (reprint author), Beijing Inst Technol, Natl Engn Lab Elect Vehicles, Sch Mech Engn, 5 South Zhongguancun St, Beijing 100081, Peoples R China. EM rxiong6@gmail.com; hwhebit@bit.edu.cn RI 熊, 瑞/B-6545-2015 OI 熊, 瑞/0000-0003-4608-7597 FU National Natural Science Foundation of China [51276022]; Higher school discipline innovation intelligence plan ("111"plan) of China; National High Technology Research and Development Program of China [2012AA111603, 2011AA11A228, 2011AA1290] FX This work was supported by the National Natural Science Foundation of China (51276022) and the Higher school discipline innovation intelligence plan ("111"plan) of China in part, the National High Technology Research and Development Program of China (2012AA111603, 2011AA11A228, 2011AA1290) in part. The authors would also like to express deep gratitude to Kathy McNamara for English editing. NR 22 TC 48 Z9 49 U1 11 U2 63 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-5442 EI 1873-6785 J9 ENERGY JI Energy PD DEC 15 PY 2013 VL 63 BP 295 EP 308 DI 10.1016/j.energy.2013.10.027 PG 14 WC Thermodynamics; Energy & Fuels SC Thermodynamics; Energy & Fuels GA 287OQ UT WOS:000329552500031 ER PT J AU Portillo, M Amthor, AM Chouhan, S Cooper, K Gehring, A Hausmann, M Hitchcock, S Kwarsick, J Manikonda, S Sumithrarachchi, C AF Portillo, M. Amthor, A. M. Chouhan, S. Cooper, K. Gehring, A. Hausmann, M. Hitchcock, S. Kwarsick, J. Manikonda, S. Sumithrarachchi, C. TI Quadrupole magnet field mapping for FRIB SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE Fragment mass separator; Fringing field; Mapping AB Extensive magnetic field map measurements have been done on a newly built superconducting quadrupole triplet with sextupole and octupole coils nested within every quadrupole. The magnetic field multipole composition and fringe field distributions have been analyzed and an improved parameterization of the field has been developed within the beam transport simulation framework. Parameter fits yielding standard deviations as low as 0.3% between measured and modeled values are reported here. (C) 2013 Elsevier B.V. All rights reserved. C1 [Portillo, M.; Amthor, A. M.; Chouhan, S.; Hausmann, M.] Michigan State Univ, Facil Rare Isotope Beams, E Lansing, MI 48824 USA. [Cooper, K.; Gehring, A.; Hitchcock, S.; Kwarsick, J.; Sumithrarachchi, C.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Manikonda, S.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Portillo, M (reprint author), Michigan State Univ, Facil Rare Isotope Beams, E Lansing, MI 48824 USA. EM portillo@frib.msu.edu NR 8 TC 3 Z9 3 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 271 EP 273 DI 10.1016/j.nimb.2013.07.036 PN B PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400019 ER PT J AU Seweryniak, D AF Seweryniak, D. CA FMA & AGFA Collaboration TI Status and plans for recoil separators for experiments with intense stable beams from ATLAS SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE Electromagnetic separator; Gas-filled separator; Digital acquisition system AB The Argonne fragment mass analyzer (FMA) has been a very important component of the experimental program at the ATLAS facility for many years and is expected to be a viable instrument for experiments with more intense beams which will become available when the ATLAS intensity upgrade is completed. Several upgrades of FMA itself and of the FMA detector suite in preparation for high-intensity beams will be presented. To accommodate experiments with extremely low cross sections, such as studies of super-heavy nuclei, construction of the Argonne gas-filled analyzer (AGFA), which will be complementary to FMA, was proposed. The design considerations for AGFA will be discussed. (C) 2013 Elsevier B.V. All rights reserved. C1 [Seweryniak, D.; FMA & AGFA Collaboration] Argonne Natl Lab, Argonne, IL 60439 USA. RP Seweryniak, D (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM seweryniak@anl.gov NR 7 TC 1 Z9 1 U1 1 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 274 EP 276 DI 10.1016/j.nimb.2013.07.027 PN B PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400020 ER PT J AU Kurtukian-Nieto, T Baartman, R Blank, B Chiron, T Davids, C Delalee, F Duval, M El Abbeir, S Fournier, A Lunney, D Meot, F Serani, L Stodel, MH Varenne, F Weick, H AF Kurtukian-Nieto, T. Baartman, R. Blank, B. Chiron, T. Davids, C. Delalee, F. Duval, M. El Abbeir, S. Fournier, A. Lunney, D. Meot, F. Serani, L. Stodel, M. -H. Varenne, F. Weick, H. TI SPIRAL2/DESIR high resolution mass separator SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE High-resolution isobar separator; Charged-particle spectrometers; Particle beam transport AB DESIR is the low-energy part of the SPIRAL2 ISOL facility under construction at GANIL. DESIR includes a high-resolution mass separator (HRS) with a designed resolving power m/Delta m of 31,000 for a 1 Pi-mm-mrad beam emittance, obtained using a high-intensity beam cooling device. The proposed design consists of two 90-degree magnetic dipoles, complemented by electrostatic quadrupoles, sextupoles, and a multipole, arranged in a symmetric configuration to minimize aberrations. A detailed description of the design and results of extensive simulations are given. (C) 2013 Elsevier B.V. All rights reserved. C1 [Kurtukian-Nieto, T.; Blank, B.; Chiron, T.; Delalee, F.; El Abbeir, S.; Fournier, A.; Serani, L.] Univ Bordeaux 1, CNRS, IN2P3, Ctr Etud Nucl Bordeaux Gradignan, F-33175 Gradignan, France. [Baartman, R.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Davids, C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Duval, M.; Stodel, M. -H.; Varenne, F.] CEA DSM CNRS IN2P3, GANIL, F-14076 Caen 5, France. [Lunney, D.] Univ Paris 11, CSNSM CNRS IN2P3, F-91405 Orsay, France. [Meot, F.] BNL, Long Isl City, NY USA. [Weick, H.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. RP Kurtukian-Nieto, T (reprint author), Univ Bordeaux 1, CNRS, IN2P3, Ctr Etud Nucl Bordeaux Gradignan, BP 120, F-33175 Gradignan, France. EM kurtukia@cenbg.in2p3.fr RI Kurtukian-Nieto, Teresa/J-1707-2014 OI Kurtukian-Nieto, Teresa/0000-0002-0028-0220 NR 16 TC 4 Z9 4 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 284 EP 289 DI 10.1016/j.nimb.2013.07.066 PN B PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400022 ER PT J AU Yun, CC Kim, MJ Kim, DG Song, JS Kim, MJ Kim, JW Kim, JR Wan, W AF Yun, C. C. Kim, Mi-Jung Kim, D. G. Song, J. S. Kim, Myeong-Jin Kim, J. W. Kim, J. R. Wan, W. TI Beam optical design of in-flight fragment separator for high-power heavy ion beam SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE In-flight fragment separator; Rare isotope beam; Beam optics; Non-linear optics ID BIGRIPS SEPARATOR; RIKEN; ISOTOPES; CODE AB An in-flight fragment separator has been designed for the rare isotope science project CRISP) in Korea. A beam used for the design is U-238 in the energy of 200 MeV/u with the maximum beam power of 400 kW. The use of high-power beam requires careful removal of the primary beam by pre-separator, for which its configuration was revised to employ four dipole magnets instead of two. Different configurations of the separator have been tested in search of optimal design in non-linear optics, which was complicated by the space needed for the target, beam dump and radiation shielding. Non-linear optical calculations have been carried out using GICOSY and COSY Infinity including the fringe fields of large-aperture quadrupole magnets. Correction of non-linear terms is made with multipole coils located inside the superconducting quadrupole magnets and by external multipole magnets. Beam simulations using LISE++ and MOCADI have been performed to consider the effects of multiple charge states of the primary and isotope beams produced at the target. Layout of the separator is being finalized, and detailed optics simulation will continue to refine its design. (C) 2013 Elsevier B.V. All rights reserved. C1 [Yun, C. C.; Kim, Mi-Jung; Kim, D. G.; Song, J. S.; Kim, Myeong-Jin; Kim, J. W.] Inst for Basic Sci Korea, Rare Isotope Sci Project, Taejon 305811, South Korea. [Kim, J. R.] Chung Ang Univ, Dept Phys, Seoul 156756, South Korea. [Wan, W.] Lawrence Berkeley Lab, Accelerator Div, Berkeley, CA 94720 USA. RP Kim, JW (reprint author), Inst for Basic Sci Korea, Rare Isotope Sci Project, Taejon 305811, South Korea. EM jwkim@ibs.re.kr NR 22 TC 9 Z9 9 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 342 EP 348 DI 10.1016/j.nimb.2013.08.015 PN B PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400032 ER PT J AU Hausmann, M Aaron, AM Amthor, AM Avilov, M Bandura, L Bennett, R Bollen, G Borden, T Burgess, TW Chouhan, SS Graves, VB Mittig, W Morrissey, DJ Pellemoine, F Portillo, M Ronningen, RM Schein, M Sherrill, BM Zeller, A AF Hausmann, M. Aaron, A. M. Amthor, A. M. Avilov, M. Bandura, L. Bennett, R. Bollen, G. Borden, T. Burgess, T. W. Chouhan, S. S. Graves, V. B. Mittig, W. Morrissey, D. J. Pellemoine, F. Portillo, M. Ronningen, R. M. Schein, M. Sherrill, B. M. Zeller, A. TI Design of the Advanced Rare Isotope Separator ARIS at FRIB SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE Rare isotope production and separation; Fragment separator; Beam Physics ID A1900 FRAGMENT SEPARATOR; RELATIVISTIC HEAVY-IONS; MOMENTUM DISTRIBUTIONS; FISSION; SYSTEMATICS; INTENSITY; MATTER; NSCL AB The Facility for Rare Isotopes Beams (FRIB) at Michigan State University will use projectile fragmentation and induced in-flight fission of heavy-ion primary beams at energies of 200 MeV/u and higher and at a beam power of 400 kW to generate rare isotope beams for experiments in nuclear physics, nuclear astrophysics, and fundamental symmetries, as well as for societal needs. The Advanced Rare Isotope Separator (ARIS) has been designed as a three-stage fragment separator for the efficient collection and purification of the rare isotope beams of interest. A vertically bending preseparator (first stage) with production target and beam dump is fully integrated into a production target facility hot cell with remote handling. The new separator compresses the accepted momentum width of up to +/-5% of the beam by a factor of three in the standard operational mode. Provisions for alternate operational modes for specific cases are included in the design. This preseparator is followed by two, horizontally-bending separator stages (second and third stages) utilizing the magnets from the existing A1900 fragment separator at the National Superconducting Cyclotron Laboratory (NSCL). These stages can alternatively be coupled to a single high-resolution separator stage, resulting in the flexibility to optimize the operation for different experiments, including momentum tagging and in-flight particle identification of rare isotope beams. The design of ARIS will be presented with an emphasis on beam physics characteristics, and anticipated operational modes will be described. (C) 2013 Elsevier B.V. All rights reserved. C1 [Hausmann, M.; Avilov, M.; Bandura, L.; Bennett, R.; Bollen, G.; Borden, T.; Chouhan, S. S.; Mittig, W.; Pellemoine, F.; Portillo, M.; Ronningen, R. M.; Schein, M.; Sherrill, B. M.; Zeller, A.] Michigan State Univ, Facil Rare Isotope Beams, E Lansing, MI 48824 USA. [Aaron, A. M.; Burgess, T. W.; Graves, V. B.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Amthor, A. M.] Bucknell Univ, Dept Phys & Astron, Lewisburg, PA 17837 USA. [Mittig, W.; Morrissey, D. J.; Sherrill, B. M.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. RP Hausmann, M (reprint author), Michigan State Univ, Facil Rare Isotope Beams, E Lansing, MI 48824 USA. EM hausmann@frib.msu.edu RI Sherrill, Bradley/B-3378-2011 NR 27 TC 13 Z9 13 U1 1 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 349 EP 353 DI 10.1016/j.nimb.2013.06.042 PN B PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400033 ER PT J AU Shornikov, A Pikin, A Scrivens, R Wenander, F AF Shornikov, A. Pikin, A. Scrivens, R. Wenander, F. TI Design study of an upgraded charge breeder for ISOLDE SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE Charge breeding; EBIS; Radioactive ion beams AB In this work we present our progress in the design study of a new Electron Beam Ion Source (EBIS) to be installed as a charge breeder for reacceleration of rare ions at ISOLDE. The work is triggered by the HIE-ISOLDE upgrade [1] and the planned TSR@ISOLDE project [2]. To fulfill the requests of the user community the new EBIS should reach an electron beam density of 10(4) A/cm(2) at electron energies up to 150 key and, provide UHV environment and ion cooling in the breeding region to ensure confinement of the ions long enough to reach the requested charge states. We report on the established design parameters and first prototyping steps towards production and testing of suitable equipment. (C) 2013 Elsevier B.V. All rights reserved. C1 [Shornikov, A.; Scrivens, R.; Wenander, F.] CERN, Dept AB, CH-1211 Geneva 23, Switzerland. [Pikin, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Shornikov, A (reprint author), CERN, Dept AB, CH-1211 Geneva 23, Switzerland. EM andrey.shornikov@cern.ch NR 19 TC 6 Z9 6 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 395 EP 398 DI 10.1016/j.nimb.2013.06.030 PN B PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400043 ER PT J AU Litvinov, YA Bishop, S Blaum, K Bosch, F Brandau, C Chen, LX Dillmann, I Egelhof, P Geissel, H Grisenti, RE Hagmann, S Heil, M Heinz, A Kalantar-Nayestanaki, N Knobel, R Kozhuharov, C Lestinsky, M Ma, XW Nilsson, T Nolden, F Ozawa, A Raabe, R Reed, MW Reifarth, R Sanjari, MS Schneider, D Simon, H Steck, M Stohlker, T Sun, BH Tu, XL Uesaka, T Walker, PM Wakasugi, M Weick, H Winckler, N Woods, PJ Xu, HS Yamaguchi, T Yamaguchi, Y Zhang, YH AF Litvinov, Yu. A. Bishop, S. Blaum, K. Bosch, F. Brandau, C. Chen, L. X. Dillmann, I. Egelhof, P. Geissel, H. Grisenti, R. E. Hagmann, S. Heil, M. Heinz, A. Kalantar-Nayestanaki, N. Knoebel, R. Kozhuharov, C. Lestinsky, M. Ma, X. W. Nilsson, T. Nolden, F. Ozawa, A. Raabe, R. Reed, M. W. Reifarth, R. Sanjari, M. S. Schneider, D. Simon, H. Steck, M. Stoehlker, T. Sun, B. H. Tu, X. L. Uesaka, T. Walker, P. M. Wakasugi, M. Weick, H. Winckler, N. Woods, P. J. Xu, H. S. Yamaguchi, T. Yamaguchi, Y. Zhang, Y. H. TI Nuclear physics experiments with ion storage rings SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE Ion storage rings; Exotic nuclei; Nuclear structure; Nuclear astrophysics ID FRS-ESR FACILITY; STORED EXOTIC NUCLEI; ISOCHRONOUS MASS-SPECTROMETRY; ORBITAL ELECTRON-CAPTURE; HALF-LIFE MEASUREMENTS; RELATIVISTIC ENERGIES; PRECISION EXPERIMENTS; PROJECTILE FRAGMENTS; RADIOACTIVE BEAMS; LASER-RADIATION AB In the last two decades a number of nuclear structure and astrophysics experiments were performed at heavy-ion storage rings employing unique experimental conditions offered by such machines. Furthermore, building on the experience gained at the two facilities presently in operation, several new storage ring projects were launched worldwide. This contribution is intended to provide a brief review of the fast growing field of nuclear structure and astrophysics research at storage rings. (C) 2013 Elsevier B.V. All rights reserved. C1 [Litvinov, Yu. A.; Bosch, F.; Dillmann, I.; Egelhof, P.; Geissel, H.; Grisenti, R. E.; Hagmann, S.; Heil, M.; Knoebel, R.; Kozhuharov, C.; Lestinsky, M.; Nolden, F.; Sanjari, M. S.; Simon, H.; Steck, M.; Stoehlker, T.; Tu, X. L.; Weick, H.; Winckler, N.] GSI Helmholtzzentrum Schwerionenforsch GSI, D-64291 Darmstadt, Germany. [Litvinov, Yu. A.] Heidelberg Univ, D-69120 Heidelberg, Germany. [Bishop, S.] Tech Univ Munich, D-85748 Garching, Germany. [Blaum, K.; Winckler, N.] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Brandau, C.; Sanjari, M. S.] ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Brandau, C.; Dillmann, I.; Geissel, H.; Knoebel, R.] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA. [Chen, L. X.] Univ Giessen, D-35392 Giessen, Germany. [Grisenti, R. E.; Hagmann, S.; Reifarth, R.] Goethe Univ Frankfurt, D-60438 Frankfurt, Germany. [Heinz, A.; Nilsson, T.] Chalmers, SE-41296 Gothenburg, Sweden. [Kalantar-Nayestanaki, N.] Univ Groningen, Kernfys Versneller Inst, NL-9747 AA Groningen, Netherlands. [Ma, X. W.; Tu, X. L.; Xu, H. S.; Zhang, Y. H.] Chinese Acad Sci IMP, Inst Modern Phys, Lanzhou 730000, Peoples R China. [Ozawa, A.] Univ Tsukuba, Inst Phys, Ibaraki 3058571, Japan. [Raabe, R.] Katholieke Univ Leuven, Inst Kern Stralingsfys, B-3001 Louvain, Belgium. [Reed, M. W.] Australian Natl Univ, Canberra, ACT 0200, Australia. [Schneider, D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Stoehlker, T.] Helmholtz Inst Jena, D-07743 Jena, Germany. [Stoehlker, T.] Univ Jena, D-07737 Jena, Germany. [Sun, B. H.] Beihang Univ, Sch Phys & Nucl Energy Engn, Beijing 100191, Peoples R China. [Uesaka, T.; Wakasugi, M.; Yamaguchi, Y.] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan. [Walker, P. M.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Woods, P. J.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland. [Yamaguchi, T.] Saitama Univ, Dept Phys, Saitama 3388570, Japan. RP Litvinov, YA (reprint author), GSI Helmholtzzentrum Schwerionenforsch GSI, D-64291 Darmstadt, Germany. EM y.litvinov@gsi.de RI Nilsson, Thomas/B-7705-2009; Heinz, Andreas/E-3191-2014; Uesaka, Tomohiro/C-1943-2015; Kalantar-Nayestanaki, Nasser/A-3582-2016; Sun, Baohua/C-6823-2009 OI Nilsson, Thomas/0000-0002-6990-947X; Kalantar-Nayestanaki, Nasser/0000-0002-1033-7200; Sun, Baohua/0000-0001-9868-5711 NR 162 TC 21 Z9 22 U1 1 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 603 EP 616 DI 10.1016/j.nimb.2013.07.025 PN B PG 14 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400084 ER PT J AU Lee, IY AF Lee, I-Yang TI Large gamma-ray detector arrays and electromagnetic separators SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE Gamma-ray detectors; Electromagnetic separators; Gamma-ray energy tracking array ID GRETA AB The use of large gamma-ray detector arrays with electromagnetic separators is a powerful combination. Various types of gamma-ray detectors have been used; some provide high detector efficiency such as scintillation detector array, others use Ge detectors for good energy resolution, and recently developed Ge energy tracking arrays gives both high peak-to-background ratio and position resolution. Similarly, different types of separators were used to optimize the performance under different experimental requirements and conditions. For example, gas-filled separators were used in heavy element studies for their large efficiency and beam rejection factor. Vacuum separators with good isotope resolution were used in transfer and fragmentation reactions for the study of nuclei far from stability. This paper presents results from recent experiments using gamma-ray detector arrays in combination with electromagnetic separators, and discusses the physics opportunities provided by these instruments. In particular, we review the performance of the instruments currently in use, and discuss the requirements of instruments for future radioactive beam accelerator facilities. (C) 2013 Elsevier B.V. All rights reserved. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Lee, IY (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM iyanglee1@gmail.com NR 15 TC 0 Z9 0 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 644 EP 648 DI 10.1016/j.nimb.2013.08.012 PN B PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400090 ER PT J AU Takeda, H Kubo, T Kusaka, K Suzuki, H Inabe, N Nolen, JA AF Takeda, Hiroyuki Kubo, Toshiyuki Kusaka, Kensuke Suzuki, Hiroshi Inabe, Naohito Nolen, Jerry A. TI Extraction of 3D field maps of magnetic multipoles from 2D surface measurements with applications to the optics calculations of the large-acceptance superconducting fragment separator BigRIPS SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 16th International Conference on ElectroMagnetic Isotope Separators and Techniques Related to their Applications (EMIS) CY DEC 02-07, 2012 CL RIKEN Nishina Ctr Accelerator Based Sci, Matsue, JAPAN SP High Energy Accelerator Res Org, Chinese Acad Sci, Inst Modern Phys, Fuji Daimond Int Co Ltd, Hamamatsu Photon K K, IDX Co Ltd, NEC Tokin Corp, REPIC Corp, Shimadzu Corp, Tecno Elect Ind Co Ltd, Thamway Co Ltd HO RIKEN Nishina Ctr Accelerator Based Sci DE Ion-optical calculations; Large-aperture short-length superconducting quadrupole magnet; 3D field map; Fringing field; In-flight fragment separator ID QUADRUPOLE LENSES; PROJECTILE-FISSION; RIKEN; COMPONENTS; TRIPLET AB The fringing fields of magnets with large apertures and short lengths greatly affect ion-optical calculations. In particular, for a high magnetic field where the iron core becomes saturated, the effective lengths and shapes of the field distribution must be considered because they change with the excitation current. Precise measurement of the three-dimensional magnetic fields and the correct application of parameters in the ion-optical calculations are necessary. First we present a practical numerical method of extracting full 3D magnetic field maps of magnetic multipoles from 2D field measurements of the surface of a cylinder. Using this novel method, we extracted the distributions along the beam axis for the coefficient of the first-order quadrupole component, which is the leading term of the quadrupole components in the multipole expansion of magnetic fields and proportional to the distance from the axis. Higher order components of the 3D magnetic field can be extracted from the leading term via recursion relations. The measurements were done for many excitation current values for the large-aperture superconducting triplet quadrupole magnets (STQs) in the BigRIPS fragment separator at the RIKEN Nishina Center RI Beam Factory. These distributions were parameterized using the Enge functions to fit the fringe field shapes at all excitation current values, so that unmeasured values are interpolated. The extracted distributions depend only on the position along the beam axis, and thus the measured three-dimensional field can easily be parameterized for ion-optical calculations. We implemented these parameters in the ion-optical calculation code COSY INFINITY and realized a first-order calculation that incorporates the effect of large and varying fringe fields more accurately. We applied the calculation to determine the excitation current settings of the STQs to realize various optics modes of BigRIPS and the effectiveness of this approach has been demonstrated. (C) 2013 Elsevier B.V. All rights reserved. C1 [Takeda, Hiroyuki; Kubo, Toshiyuki; Kusaka, Kensuke; Suzuki, Hiroshi; Inabe, Naohito] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan. [Nolen, Jerry A.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Takeda, H (reprint author), RIKEN, Nishina Ctr, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. EM takeda@ribf.riken.jp NR 34 TC 5 Z9 5 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 798 EP 809 DI 10.1016/j.nimb.2013.08.052 PN B PG 12 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 287GQ UT WOS:000329530400121 ER PT J AU Uberuaga, BP Vernon, LJ AF Uberuaga, Blas Pedro Vernon, Louis J. TI Interstitial and vacancy mediated transport mechanisms in perovskites: A comparison of chemistry and potentials SO SOLID STATE IONICS LA English DT Article DE Perovskite; Accelerated molecular dynamics; Adaptive kinetic Monte Carlo; Defect migration ID OXYGEN-ION MIGRATION; OXIDES; CONDUCTIVITY; IRRADIATION; SIMULATION; DIFFUSION; DEFECT; AMORPHIZATION; ELECTROLYTES; CONDUCTORS AB Perovskites are important materials for fast-ion conduction applications and have been used extensively as model systems for irradiation studies, two situations where understanding defect mobility is critical for predicting performance. Using long-time scale simulation methods, we examine point defect mobility in perovskites as a function of the chemistry of the perovskite and the empirical potential used. We find that, while the basic mechanisms are the same regardless of these factors, the energies associated with the mechanisms vary significantly. We identify diffusion pathways for each type of interstitial, finding relatively complex behavior for A cation interstitials, which can diffuse one-dimensionally, and oxygen interstitials, which exhibit a two-dimensional diffusion mechanism. We further find that several cation defects are immobile with a preference to transform into antisite complexes rather than migrate. These results provide new insight into the migration behavior of point defects in perovskites and complex oxides more generally. (C) 2013 Elsevier B.V. All rights reserved. C1 [Uberuaga, Blas Pedro; Vernon, Louis J.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Uberuaga, BP (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. EM blas@lanl.gov RI Vernon, Louis/K-9729-2016 OI Vernon, Louis/0000-0001-5379-7488 FU Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [2008LANL1026]; U.S. DOE [DE-AC52-06NA25396] FX This work was supported as part of the Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research. Center funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences under Award Number 2008LANL1026. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under contract DE-AC52-06NA25396. NR 55 TC 11 Z9 11 U1 3 U2 36 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD DEC 15 PY 2013 VL 253 BP 18 EP 26 DI 10.1016/j.ssi.2013.08.022 PG 9 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA 286OK UT WOS:000329478400003 ER PT J AU Tomkiewicz, AC Tamimi, MA Huq, A McIntosh, S AF Tomkiewicz, Alex C. Tamimi, Mazin A. Huq, Ashfia McIntosh, Steven TI Evidence for the low oxygen stoichiometry of cubic Ba0.5Sr0.5Co0.5Fe0.5O3-delta from in-situ neutron diffraction SO SOLID STATE IONICS LA English DT Article DE In-Situ neutron diffraction; Solid oxide fuel cell (SOFC); Barium Strontium Cobalt Iron Oxide (BSCF); Oxygen stoichiometry; Crystal structure ID INTERMEDIATE TEMPERATURES; ELECTRON-MICROSCOPY; PEROVSKITE; BA0.5SR0.5CO0.8FE0.2O3-DELTA; STABILITY; DECOMPOSITION; TRANSPORT; PHASE; (BA,SR)(CO,FE)O3-DELTA; NONSTOICHIOMETRY AB The structure and oxygen stoichiometry of Ba0.5Sr0.5Co0.5Fe0.5O3-delta (BSCF) between 793 K and 1100 K at an oxygen partial pressure of 0.1 atm were determined by in-situ neutron diffraction. Additional analysis at room temperature was conducted by synchrotron X-ray diffraction. BSCF has the cubic perovskite structure, space group Pm (3) over barn, for all investigated temperatures. The oxygen stoichiometry ranged from 226 (2) at 1100 K to 2.36 (2) at 793 K. The formation of secondary phases during long equilibration periods is suggested to be responsible for the discrepancy between oxygen stoichiometry values determined by neutron diffraction and those determined by thermogravimetry for this class of materials. (C) 2013 Elsevier B.V. All rights reserved. C1 [Tomkiewicz, Alex C.; Tamimi, Mazin A.; McIntosh, Steven] Lehigh Univ, Dept Chem Engn, Bethlehem, PA 18015 USA. [Huq, Ashfia] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. RP McIntosh, S (reprint author), Lehigh Univ, Dept Chem Engn, Bethlehem, PA 18015 USA. EM mcintosh@lehigh.edu RI Huq, Ashfia/J-8772-2013 OI Huq, Ashfia/0000-0002-8445-9649 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation under contract of the Faculty Early Career Development Program (CAREER) [CBET-1101814]; Saudi Aramco Oil Company; Lehigh University; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Research carried out at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This work was partially funded by the National Science Foundation under contract of the Faculty Early Career Development Program (CAREER) grant CBET-1101814. Mazin Tamimi is a sponsored student supported by the Saudi Aramco Oil Company. Additional support was provided by Lehigh University.; Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank Dr. Matthew Suchomel for his assistance with these synchrotron measurements. NR 29 TC 12 Z9 12 U1 2 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD DEC 15 PY 2013 VL 253 BP 27 EP 31 DI 10.1016/j.ssi.2013.08.026 PG 5 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA 286OK UT WOS:000329478400004 ER PT J AU Kim, JH Kim, YN Bi, ZH Manthiram, A Paranthaman, MP Huq, A AF Kim, Jung-Hyun Kim, Young Nam Bi, Zhonghe Manthiram, Arumugam Paranthaman, M. Parans Huq, Ashfia TI Overcoming phase instability of RBaCo2O5+delta (R = Y and Ho) by Sr substitution for application as cathodes in solid oxide fuel cells SO SOLID STATE IONICS LA English DT Article DE Solid oxide fuel cells; Layered perovskite cathode; Phase decomposition; YBaCo2O5+delta; HOBaCo2O5+delta ID COMPOSITE CATHODES; EXCHANGE KINETICS; OXYGEN REDUCTION; THIN-FILM; PEROVSKITES; LNBACO(2)O(5+DELTA); YBACO2O5+X; CHEMISTRY; DIFFUSION; SOFC AB Phase instabilities of the RBaCo2O5+delta (R = Y and Ho) layered-perovskites and their decompositions into RCoO3 and BaCoO3-z at 800 degrees in air were investigated. The phase instability will restrict their high temperature applications such as cathodes in solid oxide fuel cells (SOFC). However, appropriate amount of Sr substitution (>= 60% for R = Y and >= 70% for R = Ho) for Ba successfully stabilized the R(Ba1-xSrx)Co2O5+delta phase at elevated temperatures. This can be explained to be due to the decrease in oxygen vacancies in the R-O layer, decrease in R-O bond length, and consequent improvement in structural integrity. In addition, the Sr substitution (x = 0.6-1.0) for Ba provided added benefit with respect to the chemical stability against Ce0.8Gd0.2O1.9 (GDC) electrolyte, which is a critical requirement for the cathodes in SOFC. Among the various compositions investigated, the Y(Ba0.3Sr0.7)Co2O5+delta + GDC composite cathode delivered the optimum electrochemical performances with a stable phase, demonstrating the potential as a cathode in SOFC. (C) 2013 Elsevier B.V. All rights reserved. C1 [Kim, Jung-Hyun; Huq, Ashfia] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Kim, Young Nam; Manthiram, Arumugam] Univ Texas Austin, Electrochem Energy Lab, Austin, TX 78712 USA. [Kim, Young Nam; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Bi, Zhonghe; Paranthaman, M. Parans] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Huq, A (reprint author), Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. EM huqa@ornl.gov RI Kim, Jung-Hyun/I-5273-2013; Albe, Karsten/F-1139-2011; Huq, Ashfia/J-8772-2013; Paranthaman, Mariappan/N-3866-2015 OI Kim, Jung-Hyun/0000-0002-4598-4686; Huq, Ashfia/0000-0002-8445-9649; Paranthaman, Mariappan/0000-0003-3009-8531 FU Laboratory Directed Research and Development (LDRD) Program of Oak Ridge National Laboratory (ORNL); ORISE; Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC; Welch Foundation [F-1254] FX This work was sponsored by the Laboratory Directed Research and Development (LDRD) Program of Oak Ridge National Laboratory (ORNL). Jung-Hyun Kim and Zhonghe Bi acknowledge the support of the ORISE postdoctoral fellowship. Support (MPP) for electrochemical measurements was provided by Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy. The authors would also like to thank Andrew E. Payzant of Neutron Scattering Science Division in ORNL for supporting XRD measurements. Financial and technical supports by Spallation Neutron Source, ORNL SHaRE user facility, and Center for Nanophase Materials Sciences which are sponsored by the Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy, under contract DE-AC05-00OR22725 with UT-Battelle, LLC, are gratefully acknowledged. Financial support by the Welch Foundation grant F-1254 for the work carried out at the University of Texas at Austin is gratefully acknowledged by Young Nam Kim and Arumugam Manthiram. NR 33 TC 7 Z9 7 U1 1 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD DEC 15 PY 2013 VL 253 BP 81 EP 87 DI 10.1016/j.ssi.2013.09.001 PG 7 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA 286OK UT WOS:000329478400013 ER PT J AU Deiterding, R Wood, S AF Deiterding, R. Wood, S. TI Parallel adaptive fluid-structure interaction simulation of explosions impacting on building structures SO COMPUTERS & FLUIDS LA English DT Article DE Fluid-structure interaction; Adaptive mesh refinement; Cartesian embedded boundary method; Building structures; Parallelization ID BOUNDARY METHODS; MESH METHOD; SHOCK; ALGORITHM AB We pursue a level set approach to couple an Eulerian shock-capturing fluid solver with space-time refinement to an explicit solid dynamics solver for large deformations and fracture. The coupling algorithms considering recursively finer fluid time steps as well as overlapping solver updates are discussed. Our ideas are implemented in the AMROC adaptive fluid solver framework and are used for effective fluid-structure coupling to the general purpose solid dynamics code DYNA3D. Beside simulations verifying the coupled fluid-structure solver and assessing its parallel scalability, the detailed structural analysis of a reinforced concrete column under blast loading and the simulation of a prototypical blast explosion in a realistic multistory building are presented. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Deiterding, R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Wood, S.] Univ Tennessee, Bredesen Ctr, Knoxville, TN 37996 USA. RP Deiterding, R (reprint author), Oak Ridge Natl Lab, POB 2008,MS-6367, Oak Ridge, TN 37831 USA. EM deiterdingr@ornl.gov; swood@utk.edu RI Deiterding, Ralf/A-3394-2009 OI Deiterding, Ralf/0000-0003-4776-8183 FU [DE-AC05-00OR22725] FX This material is based in part on work performed by S. Wood while being a RAMS intern and 1 TN_SCORE Energy Scholar. All computations were carried out at the Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725. NR 36 TC 2 Z9 3 U1 2 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD DEC 15 PY 2013 VL 88 BP 719 EP 729 DI 10.1016/j.compfluid.2013.05.009 PG 11 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 283QR UT WOS:000329262600062 ER PT J AU Kim, D Hong, S Hong, J Choi, YY Kim, J Park, M Sung, TH No, K AF Kim, Dongjin Hong, Seungbum Hong, Jongin Choi, Yoon-Young Kim, Jiyoon Park, Moonkyu Sung, Tae-hyun No, Kwangsoo TI Fabrication of Vertically Aligned Ferroelectric Polyvinylidene Fluoride Mesoscale Rod Arrays SO JOURNAL OF APPLIED POLYMER SCIENCE LA English DT Article DE polyvinylidene (PVDF); piezoelectrics; mesoscale rods arrays; anodized alumina oxide (AAO) ID POLY(VINYLIDENE FLUORIDE); CRYSTALLINE PHASES; THIN-FILMS; POLYMER; MEMORY; NANOSTRUCTURES; TRANSDUCERS; NANOTUBES; DESIGN; ENERGY AB We have fabricated vertically aligned ferroelectric PVDF mesoscale rod arrays comprising and phases using a 200 nm diameter anodized aluminum oxide (AAO) as the porous template. We could synthesize the ferroelectric phase in mesoscale rod forms by combining the well-established recipe for crystallizing the phase using dimethyl sulfoxide (DMSO) at low temperature and template-guided infiltration processing for the rods using AAO. We measured the dimensions of the PVDF rods by scanning electron microscopy and identified the polymorph phases by X-ray diffraction and Fourier transform infrared spectroscopy. The length of the rods varied from 3.82 m to 1.09 m and the diameter from 232 nm to 287 nm when the volume ratio between DMSO and acetone changed from 5 : 5 to 10 : 0. We obtained well-defined piezoresponse hysteresis loops for all rods with remnant piezoresponse ranging from 2.12 pm/V to 5.04 pm/V and coercive voltage ranging from 2.29 V to 2.71 V using piezoresponse force microscopy. Our results serve as a processing platform for flexible electronic devices that need high capacitance and piezoelectric functionalities such as flexible memory devices or body energy harvesting devices for intelligent systems. (c) 2013 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 130: 3842-3848, 2013 C1 [Kim, Dongjin; Hong, Seungbum; Choi, Yoon-Young; Kim, Jiyoon; Park, Moonkyu; No, Kwangsoo] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. [Kim, Dongjin; Hong, Seungbum] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Hong, Seungbum; Choi, Yoon-Young] Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA. [Hong, Jongin] Chung Ang Univ, Dept Chem, Seoul 156756, South Korea. [Sung, Tae-hyun] Hanyang Univ, Dept Elect Engn, Seoul 133791, South Korea. RP Hong, S (reprint author), Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. EM hong@anl.gov; ksno@kaist.ac.kr RI Hong, Seungbum/B-7708-2009; No, Kwangsoo/C-1983-2011; Hong, Jongin/B-4504-2009 OI Hong, Seungbum/0000-0002-2667-1983; Hong, Jongin/0000-0002-2891-5785 FU National Research Foundation of Korea (NRF) [2010-0015063, 2011K000674]; Ministry of Education, Science and Technology (MEST); New and Renewable Energy of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) [20103020060010]; Ministry of Knowledge Economy, Korea; UChicago Argonne, a US DOE Office of Science Laboratory [DE-AC02-06CH11357]; Chung-Ang University FX This research was supported by the Mid-career Researcher Program (No. 2010-0015063) and the Conversion Research Center Program (No. 2011K000674) through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (MEST) and by a New and Renewable Energy of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant (No. 20103020060010) funded by the Ministry of Knowledge Economy, Korea. Work at Argonne National Laboratory (S.H., D.K. and Y.C., data analysis and writing of manuscript) was supported by UChicago Argonne, a US DOE Office of Science Laboratory, operated under Contract No. DE-AC02-06CH11357. J.H. acknowledges Chung-Ang University Research Grants in 2011. NR 45 TC 6 Z9 6 U1 4 U2 57 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0021-8995 EI 1097-4628 J9 J APPL POLYM SCI JI J. Appl. Polym. Sci. PD DEC 15 PY 2013 VL 130 IS 6 BP 3842 EP 3848 DI 10.1002/app.39415 PG 7 WC Polymer Science SC Polymer Science GA 282EO UT WOS:000329153300002 ER PT J AU Moffet, ML La Saponara, V AF Moffet, Mitchell L. La Saponara, Valeria TI Rheological Properties of Neat Epoxy Exposed to In-Service Aerospace Contaminants SO JOURNAL OF APPLIED POLYMER SCIENCE LA English DT Article DE composites; rheology; thermosets; viscosity and viscoelasticity ID COMPOSITE-MATERIALS; WATER-ABSORPTION; CARBON/EPOXY COMPOSITE; CHEMICAL DEGRADATION; MOISTURE ABSORPTION; ADHESIVE; CURE; DIFFUSION; CHEMISTRY; KINETICS AB We present an experimental study on the rheological properties of a commonly used epoxy resin system (EPIKOTE-862 resin and EPIKURE-W curing agent), exposed to a variety of fluids typical of aerospace operations (jet fuel, hydraulic fluids, deicing, detergents, etc.), for a period of up to 6 months, at room temperature for most conditions, and with no concurrent mechanical loading or prior degradation. The specimens were subjected to stress and frequency sweeps with a shear rheometer, while a limited set received also a temperature sweep in a range consistent with aircraft operations. Results indicate that the treated resin samples are linear viscoelastic under these testing conditions. The resin has reasonable chemical resistance to most contaminants of this study, with the exception of two commonly used detergents: an aircraft surface cleaning compound, Penair C5572, and a nonionic detergent, Methyl Ethyl Ketone (MEK). The durability change of the first compound appears triggered by high temperatures only, while the second compound causes a very drastic stiffness loss under several conditions. This drop of performance occurs within a 3-months period, with no apparent color change or fracture that could prompt visual inspection and repair. (c) 2013 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 130: 3961-3971, 2013 C1 [Moffet, Mitchell L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [La Saponara, Valeria] Univ Calif Davis, Davis, CA 95616 USA. RP La Saponara, V (reprint author), Univ Calif Davis, Davis, CA 95616 USA. EM vlasaponara@ucdavis.edu NR 29 TC 3 Z9 3 U1 0 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0021-8995 EI 1097-4628 J9 J APPL POLYM SCI JI J. Appl. Polym. Sci. PD DEC 15 PY 2013 VL 130 IS 6 BP 3961 EP 3971 DI 10.1002/app.39654 PG 11 WC Polymer Science SC Polymer Science GA 282EO UT WOS:000329153300016 ER PT J AU King, BV Moore, JF Veryovkin, IV Pellin, MJ AF King, B. V. Moore, J. F. Veryovkin, I. V. Pellin, M. J. TI High sensitivity sputter neutral mass spectrometry - Sputtering of neutral mixed clusters from gold-aluminum alloys SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 19th International Workshop on Inelastic Ion-Surface Collisions (IISC) CY SEP 16-21, 2012 CL GERMANY DE Sputtering; Sputter neutral mass spectrometry; Clusters ID METAL-CLUSTERS; INTERNAL ENERGY; SILVER; AL AB We have used the surface sensitivity of laser sputter neutral mass spectrometry to make measurements of clusters sputtered from AuAl alloys surfaces with high dynamic range. Polycrystalline AuAl4 and Au4Al were bombarded with 15 keV Ar+ at 60 degrees incidence, and the resulting secondary neutral yield distributions were measured using laser postionization mass spectrometry. Neutral clusters containing up to 28 atoms were observed and exhibited an odd-even variation in signal dependent on the stability of the photoion. Clusters sputtered from Au4Al were gold rich compared to the substrate and the yield of neutral clusters containing n atoms, Y-n, was found to follow a power in n, i.e. Y-n proportional to n(-delta), where the exponent delta was approximately 3.4. 2013 Elsevier B.V. All rights reserved. C1 [King, B. V.] Univ Newcastle, Callaghan, NSW 2308, Australia. [King, B. V.; Veryovkin, I. V.; Pellin, M. J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Moore, J. F.] MassThink LLC, Naperville, IL 60563 USA. RP King, BV (reprint author), Univ Newcastle, Callaghan, NSW 2308, Australia. EM bruce.king@newcastle.edu.au RI Pellin, Michael/B-5897-2008 OI Pellin, Michael/0000-0002-8149-9768 NR 33 TC 2 Z9 2 U1 1 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD DEC 15 PY 2013 VL 317 BP 115 EP 120 DI 10.1016/j.nimb.2013.06.026 PN A PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 285FC UT WOS:000329378100022 ER PT J AU Xu, CG AF Xu, Chonggang TI Decoupling correlated and uncorrelated parametric uncertainty contributions for nonlinear models SO APPLIED MATHEMATICAL MODELLING LA English DT Article DE Uncertainty analysis; Sensitivity analysis; Correlation; Nonlinear model; Nonlinear dependence; Fourier Amplitude Sensitivity Test ID GLOBAL SENSITIVITY-ANALYSIS; COUPLED REACTION SYSTEMS; RANDOM BALANCE DESIGNS; RATE COEFFICIENTS; WASTE-DISPOSAL; INDEXES AB For models with correlated parameters, the amount of uncertainty (generally measured by variance) in a model output contributed by a specific parameter encompasses two components: (1) the uncertainty contributed by the variations (used to represent uncertainty in the parameter) correlated with other parameters; and (2) the uncertainty contributed by the variations unique to the parameter of interest (i.e., uncorrelated variations or variations that cannot be explained by any other parameters in the model). A regression-based method has been proposed previously by Xu and Gertner (2008) [1] to decouple the correlated and uncorrelated contributions to uncertainties in model outputs by each parameter for linear models. Based on a modified version of the popular Fourier Amplitude Sensitivity Test (FAST), this paper develops a general approach for the quantification of the correlated and uncorrelated parametric uncertainty contributions in linear, nonlinear and non-monotonic models with linear or nonlinear dependence among parameters. The decoupling of correlated and uncorrelated contributions can help us determine if the uncertainty contributed by a specific parameter results from the uncertainty in itself or from its correlations with other parameters. Thus, this decoupling can be very useful in improving the understanding our modeled systems. Published by Elsevier Inc. C1 Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. RP Xu, CG (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, MS J495,EES-14, Los Alamos, NM 87545 USA. EM cxu@lanl.gov OI Xu, Chonggang/0000-0002-0937-5744 FU Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) Program; UC Lab Research Program [2012UCLRP0IT00000068990] FX This work is funded by Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) Program and UC Lab Research Program (Award ID: 2012UCLRP0IT00000068990). This submission is under public release with the approved LA-UR number of LA-UR-13-21764. NR 35 TC 5 Z9 5 U1 1 U2 7 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0307-904X EI 1872-8480 J9 APPL MATH MODEL JI Appl. Math. Model. PD DEC 15 PY 2013 VL 37 IS 24 BP 9950 EP 9969 DI 10.1016/j.apm.2013.05.036 PG 20 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Engineering; Mathematics; Mechanics GA 277GC UT WOS:000328806000011 ER PT J AU Lentine, A Grzybowski, R Shalf, JM AF Lentine, Anthony Grzybowski, Richard Shalf, John M. TI Introduction to the JLT Special Issue on Optical Interconnects SO JOURNAL OF LIGHTWAVE TECHNOLOGY LA English DT Editorial Material C1 [Lentine, Anthony] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Grzybowski, Richard] Photon Controls, Horseheads, NY 14830 USA. [Shalf, John M.] Lawrence Berkeley Natl Labs, Berkeley, CA 94720 USA. RP Lentine, A (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jshalf@lbl.gov NR 0 TC 0 Z9 0 U1 1 U2 1 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0733-8724 EI 1558-2213 J9 J LIGHTWAVE TECHNOL JI J. Lightwave Technol. PD DEC 15 PY 2013 VL 31 IS 24 BP 3905 EP 3906 DI 10.1109/JLT.2013.2290201 PG 2 WC Engineering, Electrical & Electronic; Optics; Telecommunications SC Engineering; Optics; Telecommunications GA 275KU UT WOS:000328675800001 ER PT J AU Shankaran, H Adeshina, F Teeguarden, JG AF Shankaran, Harish Adeshina, Femi Teeguarden, Justin G. TI Physiologically-based pharmacokinetic model for Fentanyl in support of the development of Provisional Advisory Levels SO TOXICOLOGY AND APPLIED PHARMACOLOGY LA English DT Article DE Computational modeling; Inhalation; Oral transmucosal; Anesthetic; Route-to-route extrapolation; Risk assessment ID DRUG-INTERACTIONS; INTERINDIVIDUAL VARIABILITY; DOSE PROPORTIONALITY; HEALTHY-VOLUNTEERS; BIOMONITORING DATA; CANCER-PATIENTS; BUCCAL TABLETS; DOUBLE-BLIND; CHRONIC PAIN; BLOOD-FLOW AB Provisional Advisory Levels (PALs) are tiered exposure limits for toxic chemicals in air and drinking water that are developed to assist in emergency responses. Physiologically-based pharmacokinetic (PBPK) modeling can support this process by enabling extrapolations across doses, and exposure routes, thereby addressing gaps in the available toxicity data. Here, we describe the development of a PBPK model for Fentanyl - a synthetic opioid used clinically for pain management - to support the establishment of PALS. Starting from an existing model for intravenous Fentanyl, we first optimized distribution and clearance parameters using several additional IV datasets. We then calibrated the model using pharmacokinetic data for various formulations, and determined the absorbed fraction, F, and time taken for the absorbed amount to reach 90% of its final value, t90. For aerosolized pulmonary Fentanyl, F = 1 and t90 < 1 min indicating complete and rapid absorption. The F value ranged from 0.35 to 0.74 for oral and various transmucosal routes. Oral Fentanyl was absorbed the slowest (t90 similar to 300 min); the absorption of intranasal Fentanyl was relatively rapid (t90 similar to 20-40 min); and the various oral transmucosal routes had intermediate absorption rates (t90 similar to 160-300 min). Based on these results, for inhalation exposures, we assumed that all of the Fentanyl inhaled from the air during each breath directly, and instantaneously enters the arterial circulation. We present model predictions of Fentanyl blood concentrations in oral and inhalation scenarios relevant for PAL development, and provide an analytical expression that can be used to extrapolate between oral and inhalation routes for the derivation of PALs. Published by Elsevier Inc. C1 [Shankaran, Harish] Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA 99352 USA. [Adeshina, Femi] US EPA, Natl Homeland Secur Res Ctr, Washington, DC 20460 USA. [Teeguarden, Justin G.] Pacific NW Natl Lab, Syst Toxicol Grp, Richland, WA 99352 USA. RP Shankaran, H (reprint author), Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, POB 999,MS J4-33, Richland, WA 99352 USA. EM harish.shankaran@pnnl.gov OI Teeguarden, Justin/0000-0003-3817-4391 FU US EPA under Battelle Prime Contract [EP-C-09-0006]; Battelle for the U.S. Department of Energy [DE-AC06-76RL01830] FX This work was funded by the US EPA under Battelle Prime Contract EP-C-09-0006. Pacific Northwest National Laboratory is a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC06-76RL01830. NR 73 TC 8 Z9 8 U1 1 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0041-008X EI 1096-0333 J9 TOXICOL APPL PHARM JI Toxicol. Appl. Pharmacol. PD DEC 15 PY 2013 VL 273 IS 3 BP 464 EP 476 DI 10.1016/j.taap.2013.05.024 PG 13 WC Pharmacology & Pharmacy; Toxicology SC Pharmacology & Pharmacy; Toxicology GA 275XC UT WOS:000328711700005 PM 23732079 ER PT J AU Bowman, RC Payzant, EA Wilson, PR Pearson, DP Ledovskikh, A Danilov, D Notten, PHL An, K Skorpenske, HD Wood, DL AF Bowman, R. C., Jr. Payzant, E. A. Wilson, P. R. Pearson, D. P. Ledovskikh, A. Danilov, D. Notten, P. H. L. An, K. Skorpenske, H. D. Wood, D. L. TI Characterization and analyses of degradation and recovery of LaNi4.78Sn0.22 hydrides following thermal aging SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE La-Ni-Sn alloys; Pressure-composition isotherms; Hydride degradation behavior; Statistical thermodynamics modeling; Neutron powder diffraction ID ELECTROCHEMICAL CYCLING STABILITY; PRODUCE 20 K; FORMING COMPOUNDS; HYDROGEN ABSORPTION; METAL-HYDRIDES; ALLOYS AB LaNi4.78Sn0.22Hx hydride samples were held at a hydrogen content of x>5.0 (x is H/La atomic ratio) and temperatures above 465 K to accelerate the intrinsic degradation processes. Although Sn-substituted alloys are much more resistant to disproportionation than nearly all other LaNi5 alloys, the present test conditions did produce substantial degradation. Effects observed included reduction in hydrogen storage capacity, decreases in the plateau pressures, increased slopes of the plateaus, and smaller hysteresis ratios. A regeneration process nearly completely restored the behavior of the degraded LaNi4.78Sn0.22 hydride to its initial value. First-principles chemical reaction kinetics and statistical thermodynamics simulations have replicated experimental pressure-composition hydrogen gas absorption isotherms for both initial and degraded LaNi4.75Sn0.22 hydride. Neutron diffraction characterization of phase compositions, crystal structures, and hydrogen content have been performed on undamaged, degraded, and regenerated LaNi4.78Sn0.22 deuterides. (C) 2013 Elsevier B.V. All rights reserved. C1 [Bowman, R. C., Jr.; Payzant, E. A.; An, K.; Skorpenske, H. D.; Wood, D. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Wilson, P. R.; Pearson, D. P.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Ledovskikh, A.; Danilov, D.; Notten, P. H. L.] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. RP Bowman, RC (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM rcbjr1967@gmail.com RI Payzant, Edward/B-5449-2009; An, Ke/G-5226-2011; OI Payzant, Edward/0000-0002-3447-2060; An, Ke/0000-0002-6093-429X; Bowman, Robert/0000-0002-2114-1713 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Aeronautics and Space Administration (NASA) FX We wish to thank J.W. Reiter for supporting isotope exchange processing and Dr. A.D. Stoica, R.A. Mills, and R.W. Connatser for assistance with the neutron experiments. This work was partially supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy. A portion of this research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The Jet Propulsion Laboratory is operated by California Institute of Technology, under a contract with the National Aeronautics and Space Administration (NASA). NR 26 TC 3 Z9 3 U1 1 U2 12 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 SU 1 BP S207 EP S210 DI 10.1016/j.jallcom.2013.03.129 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 268LO UT WOS:000328172400054 ER PT J AU Cantelli, R Paolone, A Palumbo, O Leardini, F Autrey, T Karkamkar, A Luedtke, AT AF Cantelli, R. Paolone, A. Palumbo, O. Leardini, F. Autrey, T. Karkamkar, A. Luedtke, A. T. TI Rotational dynamics in ammonia borane: Evidence of strong isotope effects SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Hydrogen absorbing materials; Ultrasonics ID HYDROGEN STORAGE; ANELASTIC SPECTROSCOPY; ORTHORHOMBIC PHASE; CHEMICAL-REACTIONS; DIHYDROGEN BOND; HIGH-PRESSURE; DIFFRACTION; BH3NH3; DECOMPOSITION; TRANSITION AB This work reports anelastic spectroscopy measurements on the partially deuterated (ND3BH3 and NH3BD3) and perdeuterated (ND3BD3) ammonia borane (NH3BH3) compounds. The relaxations previously reported in NH3BH3 are observed in all the samples, and are ascribed to the rotational and torsional dynamics of NH(D)(3)BH(D)(3) complexes. A new thermally activated peak appears at 70 K (for a vibration frequency of similar to 1 kHz) in the spectrum of NH3BD3 and ND3BD3. The peak is practically a single-time Debye process, indicating absence of interaction between the relaxing units, and has a strikingly high intensity. A secondary relaxation process is also detected around 55 K. The anelastic spectrum of the ND3BH3 only displays this less intense process at 55 K. The analysis of the peaks supplies information about the dynamics of the relaxing species, and the obtained results provide indications on the effect of partial and selective deuteration on the hydrogen (deuterium) dynamics. (C) 2013 Elsevier B.V. All rights reserved. C1 [Cantelli, R.; Leardini, F.] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. [Paolone, A.; Palumbo, O.] CNR, ISC, I-00185 Rome, Italy. [Autrey, T.; Karkamkar, A.; Luedtke, A. T.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Cantelli, R (reprint author), Univ Roma La Sapienza, Dept Phys, Piazzale A Moro 5, I-00185 Rome, Italy. EM Rosario.Cantelli@roma1.infn.it RI Leardini, Fabrice/K-2451-2014; Paolone, Annalisa/B-7701-2015; Palumbo, Oriele/B-7694-2015; OI Paolone, Annalisa/0000-0002-4839-7815; Palumbo, Oriele/0000-0003-4968-1049 FU Italian Ministry of Economic Development; Regione Lazio FX This work was supported by the Italian Ministry of Economic Development through the Industria 2015 Project "Hydrostore". PNNL is operated by Battelle for the US DOE. One of the authors (F. L.) wishes to thank Regione Lazio for a grant. NR 26 TC 4 Z9 4 U1 0 U2 16 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 SU 1 BP S63 EP S66 DI 10.1016/j.jallcom.2013.03.148 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 268LO UT WOS:000328172400018 ER PT J AU Corgnale, C Motyka, T Greenway, S Perez-Berrios, JM Nakano, A Ito, H Maeda, T AF Corgnale, Claudio Motyka, Theodore Greenway, Scott Perez-Berrios, Jose M. Nakano, Akihiro Ito, Hiroshi Maeda, Tetsuhiko TI Metal hydride bed system model for renewable source driven Regenerative Fuel Cell SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Hydrogen storage; Metal hydride; AB5 material; System simulation; Regenerative Fuel Cell ID 2-DIMENSIONAL HEAT; HYDROGEN REACTOR; MASS-TRANSFER AB A Regenerative Fuel Cell system, driven by renewable energy sources, has the potential to overcome the intermittent nature of renewable energy and become a reliable and feasible solution for small power stationary systems, producing electricity without pollutants. The present work describes a new system model for a metal hydride hydrogen storage bed (based on an AB5-type material) integrated into a Regenerative Fuel Cell system. The model has been validated against experimental data obtained from a Savannah River National Laboratory metal hydride bed at different operating conditions and has been integrated into a Regenerative Fuel Cell system using TRNSYS to simulate the behavior of the overall system for selected scenarios. Results show the technical feasibility of the Regenerative Fuel Cell concept with short term energy storage (i.e. hydrogen storage) and suggest useful solutions to make the system adaptable to long term storage scenarios as well. (C) 2013 Published by Elsevier B.V. C1 [Corgnale, Claudio; Motyka, Theodore] SRNL, Aiken, SC 29808 USA. [Greenway, Scott; Perez-Berrios, Jose M.] Greenway Energy LLC, Aiken, SC 29808 USA. [Nakano, Akihiro; Ito, Hiroshi; Maeda, Tetsuhiko] Energy Technol Res Inst, Natl Inst Adv Ind Sci & Technol AIST, Tsukuba, Ibaraki 3058564, Japan. RP Corgnale, C (reprint author), SRNL, Savannah River Site, Aiken, SC 29808 USA. EM claudio.corgnale@gmail.com FU DOE; METI FX A part of this study was supported by the Clean Energy Partnership Technology Program between DOE and METI. The authors also wish to thank the technical staff of TRNSYS (R) and in particular Mr. Matt Duffy for useful interactions. NR 7 TC 8 Z9 8 U1 0 U2 7 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 SU 1 BP S406 EP S409 DI 10.1016/j.jallcom.2013.03.010 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 268LO UT WOS:000328172400101 ER PT J AU Paolone, A Palumbo, O Leardini, F Cantelli, R Knight, DA Teprovich, JA Zidan, R AF Paolone, A. Palumbo, O. Leardini, F. Cantelli, R. Knight, D. A. Teprovich, J. A., Jr. Zidan, R. TI A spectroscopic investigation of hydrogenated Li doped fullerane SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Hydrogen absorbing materials; Ultrasonics ID ANELASTIC SPECTROSCOPY; RELAXATION PROCESSES; CHEMICAL-REACTIONS; AMMONIA BORANE; DYNAMICS; STORAGE AB We investigated two samples of Li6C60Hx, with different crystal structures, by means of anelastic and infrared spectroscopy. In both compounds the elastic energy loss does not display the relaxation peak, which in pure fullerene was attributed to the rotations of the buckyballs between energetically nearly-equivalent positions. We suggest that the disappearance of the relaxation process is due to bonding between bucicyballs. The optical density of both specimens show new phonon lines appearing in the mid-infrared range, which in the previous literature were found in polymerized fullerenes. The results obtained by means of both spectroscopies clearly indicate the presence of chemical bonding between C-60 molecules in the Li6C60Hx, independently of their crystal structure. (C) 2013 Elsevier B.V. All rights reserved. C1 [Leardini, F.; Cantelli, R.] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. [Paolone, A.; Palumbo, O.] CNR, ISC, I-00185 Rome, Italy. [Knight, D. A.; Teprovich, J. A., Jr.; Zidan, R.] Savannah River Natl Lab, Clean Energy Directorate, Aiken, SC 29801 USA. RP Cantelli, R (reprint author), Univ Roma La Sapienza, Dept Phys, Piazzale A Moro 5, I-00185 Rome, Italy. EM Rosario.Cantelli@roma1.infn.it RI Leardini, Fabrice/K-2451-2014; Paolone, Annalisa/B-7701-2015; Palumbo, Oriele/B-7694-2015; OI Palumbo, Oriele/0000-0003-4968-1049; Paolone, Annalisa/0000-0002-4839-7815; Knight, David/0000-0001-5510-6265 FU Italian Ministry of Economic Development; US-DOE, Office of Basic Energy Science; Regione Lazio FX This work was supported by the Italian Ministry of Economic Development through the Industria 2015 Project "Hydrostore". D.A.K., J.A.T., and R.Z. would like to thank the US-DOE, Office of Basic Energy Science for funding. One of the authors (F.L.) wishes to thank Regione Lazio for a grant. NR 14 TC 3 Z9 3 U1 2 U2 22 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 SU 1 BP S67 EP S69 DI 10.1016/j.jallcom.2013.03.162 PG 3 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 268LO UT WOS:000328172400019 ER PT J AU Stetson, NT Ordaz, G Adams, J Randolph, K McWhorter, S AF Stetson, Ned T. Ordaz, Grace Adams, Jesse Randolph, Katie McWhorter, Scott TI The use of application-specific performance targets and engineering considerations to guide hydrogen storage materials development SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Alane; Mischmetal; Sodium alanate; TiCrMn ID HIERARCHICAL METHODOLOGY; HYDRIDE; MODELS AB The Hydrogen and Fuel Cells Technologies Office, carried out through the DOE Office of Energy Efficiency and Renewable Energy, maintains a broad portfolio of activities to enable the commercialization of fuel cells across a range of near, mid and long-term applications. Improved, advanced hydrogen storage technologies are seen as a critical need for successful implementation of hydrogen fuel cells in many of these applications. To guide and focus materials development efforts, the DOE develops system performance targets for the specific applications of interest, and carries out system engineering analyses to determine the system-level performance delivered when the materials are incorporated into a complete system. To meet the needs of applications, it is important to consider the system-level performance, not just the material-level properties. An overview of the DOE's hydrogen storage efforts in developing application-specific performance targets and systems engineering to guide hydrogen storage materials identification and development is herein provided. Published by Elsevier B.V. C1 [Stetson, Ned T.; Ordaz, Grace; Adams, Jesse; Randolph, Katie] US DOE, Washington, DC 20585 USA. [McWhorter, Scott] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Stetson, NT (reprint author), US DOE, 1000 Independence Ave SW,EE-2H, Washington, DC 20585 USA. EM ned.stetson@ee.doe.gov NR 20 TC 3 Z9 3 U1 1 U2 8 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 SU 1 BP S333 EP S336 DI 10.1016/j.jallcom.2013.03.227 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 268LO UT WOS:000328172400085 ER PT J AU Teprovich, JA Knight, DA Peters, B Zidan, R AF Teprovich, Joseph A., Jr. Knight, Douglas A. Peters, Brent Zidan, Ragaiy TI Comparative study of reversible hydrogen storage in alkali-doped fulleranes SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE C-60; Alkali doped; Fullerane; XRD; Reversible hydrogen storage; Polymer ID THERMAL-DECOMPOSITION; ELECTRONIC-PROPERTIES; C-60; C60H36; CARBON; FULLERENES; MAGNESIUM; GAS; SUPERCONDUCTIVITY; FRAGMENTATION AB In this report we describe and compare the hydrogen storage properties of lithium and sodium doped fullerenes prepared via a solvent-assisted mixing process. For the preparation of these samples either NaH or LiH was utilized as the alkali metal source to make material based on either a Na6C60 or Li6C60. Both of the alkali-doped materials can reversibly absorb and desorb hydrogen at much milder conditions than the starting materials used to make them (decomposition temperatures of NaH > 420 degrees C, LiH > 670 degrees C, and fullerane > 500 degrees C). The hydrogen storage properties of the materials were compared by TGA, isothermal desorption, and XRD analysis. It was determined that the sodium-doped material can reversibly store 4.0 wt.% H-2 while the lithium doped material can reversibly store 5.0 wt.% H-2 through a chemisorption mechanism indicated by the formation and measurement of C-H bonds. XRD analysis of the material demonstrated that a reversible phase transition between fcc and bcc occurs depending on the temperature at which the hydrogenation is performed. In either system the active hydrogen storage material resembles a hydrogenated fullerene (fullerane). (C) 2013 Elsevier B.V. All rights reserved. C1 [Teprovich, Joseph A., Jr.; Knight, Douglas A.; Peters, Brent; Zidan, Ragaiy] Savannah River Natl Lab, Clean Energy Directorate, Aiken, SC 29801 USA. RP Zidan, R (reprint author), Savannah River Natl Lab, Clean Energy Directorate, Aiken, SC 29801 USA. EM ragaiy.zidan@srnl.doe.gov OI Knight, David/0000-0001-5510-6265 FU U.S. DOE, Office of Basic Energy Science FX J.A.T., D.A.K., B.P., and R.Z. would like to thank the U.S. DOE, Office of Basic Energy Science for funding as well as Mr. David Missimer (SRNL) for his help with the XRD measurements and Mr. Joseph Wheeler (SRNL) for his assistance with the laboratory operations. NR 48 TC 8 Z9 8 U1 2 U2 39 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 SU 1 BP S364 EP S367 DI 10.1016/j.jallcom.2013.02.024 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 268LO UT WOS:000328172400091 ER PT J AU Seo, YJ Muench, L Reid, A Chen, JZ Kang, YN Hooker, JM Volkow, ND Fowler, JS Kim, SW AF Seo, Young Jun Muench, Lisa Reid, Alicia Chen, Jinzhu Kang, Yeona Hooker, Jacob M. Volkow, Nora D. Fowler, Joanna S. Kim, Sung Won TI Radionuclide labeling and evaluation of candidate radioligands for PET imaging of histone deacetylase in the brain SO BIOORGANIC & MEDICINAL CHEMISTRY LETTERS LA English DT Article DE Carbon-11; Positron emission tomography; SAHA; Brain; Epigenetics; Brain permeability ID TRICHOSTATIN-A; INHIBITORS; POTENT; RADIOSYNTHESIS; MECHANISMS; DISORDERS; EFFICIENT; ESTERS; MS-275 AB Histone deacetylases (HDACs) regulate gene expression by inducing conformational changes in chromatin. Ever since the discovery of a naturally occurring HDAC inhibitor, trichostatin A (TSA) stimulated the recent development of suberoylanilide (SAHA, Zolinza (R)), HDAC has become an important molecular target for drug development. This has created the need to develop specific in vivo radioligands to study epigenetic regulation and HDAC engagement for drug development for diseases including cancer and disorders. 6-([F-18]Fluoroacetamido)-1-hexanoicanilide ([F-18]FAHA) was recently developed as a HDAC substrate and shows moderate blood-brain barrier (BBB) permeability and specific signal (by metabolic trapping/or deacetylation) but rapid metabolism. Here, we report the radiosynthesis of two carbon-11 labeled candidate radiotracers (substrate-and inhibitor-based radioligand) for HDAC and their evaluation in non-human primate brain. PET studies showed very low brain uptake and rapid metabolism of both labeled compounds but revealed a surprising enhancement of brain penetration by F for H substitution when comparing one of these to [F-18]FAHA. Further structural refinement is needed for the development of brain-penetrant, metabolically stable HDAC radiotracers and to understand the role of fluorine substitution on brain penetration. Published by Elsevier Ltd. C1 [Seo, Young Jun; Chen, Jinzhu; Kang, Yeona; Fowler, Joanna S.] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. [Seo, Young Jun] Chonbuk Natl Univ, Dept Chem, Jeonju 561756, South Korea. [Muench, Lisa; Volkow, Nora D.; Kim, Sung Won] NIAAA, Lab Neuroimaging, Bethesda, MD 20892 USA. [Reid, Alicia] CUNY Medgar Evers Coll, Dept Phys Environm & Comp Sci, Brooklyn, NY 11225 USA. [Hooker, Jacob M.] Harvard Univ, Sch Med, Massachusetts Gen Hosp, Athinoula A Martinos Ctr Biomed Imaging,Dept Radi, Charlestown, MA 02129 USA. [Volkow, Nora D.] NIDA, Rockville, MD 20852 USA. RP Hooker, JM (reprint author), NIAAA, 10 Ctr Dr,Rm B2L304, Bethesda, MD 20892 USA. EM hooker@nmr.mgh.harvard.edu; sunny.kim@nih.gov OI Hooker, Jacob/0000-0002-9394-7708 FU DOE [BR KP1503010]; NIH [1R01DA030321]; U.S. Department of Energy [DEAC02-98CH10886]; National Institute on Alcohol Abuse and Alcoholism FX This work was supported by DOE grant B&R KP1503010 and NIH grant 1R01DA030321. In addition, the work at Brookhaven National Laboratory was performed under contract DEAC02-98CH10886 with the U.S. Department of Energy, and with infrastructure support from its Office of Biological and Environmental Research. Salary support for SWK and LM was provided by the intramural program of the National Institute on Alcohol Abuse and Alcoholism. We are grateful to the PET radiotracer and imaging team at BNL (Dr. Michael Schueller, David Alexoff, Colleen Shea, Youwen Xu, Pauline Carter, Payton King, Barbara Hubbard and Don Warner) for carrying out primate imaging experiments. We used two computational chemistry programs available in the Center for Molecular Modeling (http://cmm.cit.nih.gov) and the Helix Systems (http://helix.nih.gov) at the National Institutes of Health, Bethesda, MD. NR 30 TC 10 Z9 10 U1 3 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-894X EI 1464-3405 J9 BIOORG MED CHEM LETT JI Bioorg. Med. Chem. Lett. PD DEC 15 PY 2013 VL 23 IS 24 BP 6700 EP 6705 DI 10.1016/j.bmcl.2013.10.038 PG 6 WC Chemistry, Medicinal; Chemistry, Organic SC Pharmacology & Pharmacy; Chemistry GA 263DU UT WOS:000327787700033 PM 24210501 ER PT J AU Zenone, T Gelfand, I Chen, JQ Hamilton, SK Robertson, GP AF Zenone, Terenzio Gelfand, Ilya Chen, Jiquan Hamilton, Stephen K. Robertson, G. Philip TI From set-aside grassland to annual and perennial cellulosic biofuel crops: Effects of land use change on carbon balance SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Land use change; Conservation Reserve Program; Switchgrass; Restored prairie; Corn; Soil carbon ID NET ECOSYSTEM EXCHANGE; ENERGY-BALANCE; SOIL CARBON; DIOXIDE EXCHANGE; EDDY COVARIANCE; INTERANNUAL VARIABILITY; SONIC ANEMOMETER; CO2 FLUXES; FOREST; WATER AB Increasing demand for agricultural commodities such as grain for feed and feedstocks for biofuels are driving rapid land use change. We studied the effect of agricultural land-use change on two historical land use types for three different cropping systems using eddy covariance and ecosystem carbon balance approaches. We quantified the consequences of establishing corn, switchgrass, and mixed prairie species on cropland under a recent corn-soybean rotation and on set-aside land planted for 20 years to smooth bromegrass (Bromus inermis Leyss) enrolled in the USDA Conservation Reserve Program (CRP). We converted three CRP and three cropland fields to no-till soybeans in 2009 (conversion year) and then established fields of corn, switchgrass, and mixed prairie species in fields formerly cropland or CRP. In addition, one CRP perennial grassland site was kept undisturbed as a reference. We measured the harvestable biomass during the conversion and over the two following years. To account for C removed in harvestable biomass we calculated adjusted Net Ecosystem Production (NEPadj; g C m(-2) yr(-1)) as NEP measured by eddy covariance plus harvested biomass. During the conversion year, fields converted from historical CRP grassland exhibited net C emissions between 261 and 340 g C m(-2) yr(-1). The sites established on recent cropland emitted 37-42 g Cm-2 yr(-1). The undisturbed reference site sequestered (rather than emitted) 35 g C m(-2) yr(-1). Cumulative NEPadj over the entire 3-year period at the sites converted from CRP grasslands was 170, 740, and 885 g C m(-2) for switchgrass, corn, and mixed prairie systems, respectively. At the former cropland sites, cumulative NEPadj was 214, 364, and 446 g C m(-2) for mixed prairie, corn, and switchgrass systems, respectively. Over this period the reference site had an NEP of 260 30 g C m(-2). Land use change to biofuel crops thus induced large C emissions, even when renewable energy production was included as a fossil fuel carbon offset. The most productive perennial systems had lowest overall C losses. Accounting for fossil fuel offset credits generated from harvested biomass completely attenuated CO2 emissions in the CRP site converted to switchgrass and partially attenuated emissions in all other converted sites. These results can be readily incorporated into management recommendations for future establishment of biofuels feedstock and row agriculture systems with different management intensities. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zenone, Terenzio; Chen, Jiquan] Univ Toledo, Dept Environm Sci, Toledo, OH 43606 USA. [Zenone, Terenzio; Gelfand, Ilya; Chen, Jiquan; Hamilton, Stephen K.; Robertson, G. Philip] Michigan State Univ, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Gelfand, Ilya; Hamilton, Stephen K.; Robertson, G. Philip] Michigan State Univ, WK Kellogg Biol Stn, Hickory Corners, MI 49060 USA. [Hamilton, Stephen K.] Michigan State Univ, Dept Zool, E Lansing, MI 48824 USA. [Robertson, G. Philip] Michigan State Univ, Dept Plant Soil & Microbial Sci, E Lansing, MI 48824 USA. RP Zenone, T (reprint author), Univ Antwerp, Dept Biol, Res Grp Plant & Vegetat Ecol, B-2610 Antwerp, Belgium. EM Terenzio.Zenone@ua.ac.be RI Chen, Jiquan/D-1955-2009; Gelfand, Ilya/J-9017-2012; Hamilton, Stephen/N-2979-2014; OI Gelfand, Ilya/0000-0002-8576-0978; Hamilton, Stephen/0000-0002-4702-9017; Robertson, G/0000-0001-9771-9895 FU DOE Office of Science [DE-FC02-07ER64494]; Office of Energy Efficiency and Renewable Energy [DE-AC05-76RL01830]; U.S. National Science Foundation LTER program [DEB 1027253]; MSU AgBioResearch FX Financial support for this work was provided by the DOE Office of Science (DE-FC02-07ER64494) and Office of Energy Efficiency and Renewable Energy (DE-AC05-76RL01830), the U.S. National Science Foundation LTER program (DEB 1027253), and MSU AgBioResearch. We thank K. Kahmark, M. Deal, C. Shao, and J. Xu for help with the EC towers and L. Delp Taylor for editorial assistance. J. Bronson and J. Simmons assisted with field data acquisition. We also thank A. Noormets for use of the EC processor software NR 45 TC 14 Z9 15 U1 5 U2 106 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD DEC 15 PY 2013 VL 182 SI SI BP 1 EP 12 DI 10.1016/j.agrformet.2013.07.015 PG 12 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA 252JE UT WOS:000327000200001 ER PT J AU Burgess, WA Tapriyal, D Morreale, BD Soong, Y Baled, HO Enick, RM Wu, Y Bamgbade, BA McHugh, MA AF Burgess, Ward A. Tapriyal, Deepak Morreale, Bryan D. Soong, Yee Baled, Hseen O. Enick, Robert M. Wu, Yue Bamgbade, Babatunde A. McHugh, Mark A. TI Volume-translated cubic EoS and PC-SAFT density models and a free volume-based viscosity model for hydrocarbons at extreme temperature and pressure conditions SO FLUID PHASE EQUILIBRIA LA English DT Article; Proceedings Paper CT 1st International Conference on Upstream Engineering and Flow Assurance (ICUEFA) at the Spring Meeting of the American-Institute-of-Chemical-Engineers (AIChE) CY APR 01-05, 2012 CL Houston, TX SP Amer Inst Chem Engineers DE SAFT; Peng-Robinson; Soave-Redlich-Kwong; Reservoir engineering ID EQUATION-OF-STATE; PERTURBED-CHAIN SAFT; FRICTION THEORY; ASSOCIATING MOLECULES; TRANSPORT-PROPERTIES; SRK EQUATION; N-ALKANES; FLUIDS; PREDICTION; MIXTURES AB This research focuses on providing the petroleum reservoir engineering community with robust models of hydrocarbon density and viscosity at the extreme temperature and pressure conditions (up to 533 K and 276 MPa, respectively) characteristic of ultra-deep reservoirs, such as those associated with the deep-water wells in the Gulf of Mexico. Our strategy is to base the volume-translated (VT) Peng-Robinson (PR) and Soave-Redlich-Kwong (SRK) cubic equations of state (EoSs) and perturbed-chain, statistical associating fluid theory (PC-SAFT) on an extensive data base of high temperature (278-533 K), high pressure (6.9-276 MPa) density rather than fitting the models to low pressure saturated liquid density data. This high-temperature, high-pressure (HTHP) data base consists of literature data for hydrocarbons ranging from methane to C-40. The three new models developed in this work, HTHP VT-PR EoS, HTHP VT-SRK EoS, and hybrid PC-SAFT, yield mean absolute percent deviation values (MAPD) for HTHP hydrocarbon density of similar to 2.0%, similar to 1.5%, and <1.0%, respectively. An effort was also made to provide accurate hydrocarbon viscosity models based on literature data. Viscosity values are estimated with the frictional theory (f-theory) and free volume (FV) theory of viscosity. The best results were obtained when the PC-SAFT equation was used to obtain both the attractive and repulsive pressure inputs to f-theory, and the density input to FV theory. Both viscosity models provide accurate results at pressures to 100 MPa but experimental and model results can deviate by more than 25% at pressures above 200 MPa. (C) 2013 Elsevier B.V. All rights reserved. C1 [Burgess, Ward A.; Tapriyal, Deepak; Morreale, Bryan D.; Soong, Yee; Baled, Hseen O.; Enick, Robert M.; Wu, Yue; Bamgbade, Babatunde A.; McHugh, Mark A.] US DOE, NETL, Off Res & Dev, Pittsburgh, PA 15236 USA. [Tapriyal, Deepak] URS, NETL, Pittsburgh, PA 15236 USA. [Baled, Hseen O.; Enick, Robert M.] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. [Wu, Yue; Bamgbade, Babatunde A.; McHugh, Mark A.] Virginia Commonwealth Univ, Dept Chem & Life Sci Engn, Richmond, VA 23284 USA. RP Burgess, WA (reprint author), US DOE, NETL, Off Res & Dev, Pittsburgh, PA 15236 USA. EM Ward.Burgess@or.netl.doe.gov NR 36 TC 12 Z9 12 U1 2 U2 54 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-3812 EI 1879-0224 J9 FLUID PHASE EQUILIBR JI Fluid Phase Equilib. PD DEC 15 PY 2013 VL 359 SI SI BP 38 EP 44 DI 10.1016/j.fluid.2013.07.016 PG 7 WC Thermodynamics; Chemistry, Physical; Engineering, Chemical SC Thermodynamics; Chemistry; Engineering GA 261TR UT WOS:000327688000005 ER PT J AU Smith, BD Jewett, A Burt, RD Zibbell, JE Yartel, AK DiNenno, E AF Smith, Bryce D. Jewett, Amy Burt, Richard D. Zibbell, Jon E. Yartel, Anthony K. DiNenno, Elizabeth TI "To Share or Not to Share?" Serosorting by Hepatitis C Status in the Sharing of Drug Injection Equipment Among NHBS-IDU2 Participants SO JOURNAL OF INFECTIOUS DISEASES LA English DT Article DE hepatitis C virus; serosorting; injection drug use; sharing injection equipment ID VIRUS-INFECTION; HIV-INFECTION; RISK BEHAVIOR; UNITED-STATES; USERS; PREVALENCE; SURVEILLANCE; POPULATION; MEN AB Background. Persons who inject drugs (PWID) are at high risk for acquiring hepatitis C virus (HCV) infection. The Centers for Disease Control and Prevention estimates there are 17 000 new infections per year, mainly among PWID. This study examines injection equipment serosorting-considering HCV serostatus when deciding whether and with whom to share injection equipment. Objective. To examine whether injection equipment serosorting is occurring among PWID in selected cities. Methods. Using data from the National HIV Behavioral Surveillance System-Injection Drug Users (NHBS-IDU2, 2009), we developed multivariate logistic regression models to examine the extent to which participants' self-reported HCV status is associated with their injection equipment serosorting behavior and knowledge of last injecting partner's HCV status. Results. Participants who knew their HCV status were more likely to know the HCV status of their last injecting partner, compared to those who did not know their status (HCV+: adjusted odds ratio [aOR] 4.1, 95% confidence interval [CI], 3.4-4.9; HCV-: aOR 2.5, 95% CI, 2.0-3.0). Participants who reported being HCV+, relative to those of unknown HCV status, were 5 times more likely to share injection equipment with a partner of HCV-positive status (aOR 4.8, 95% CI, 3.9-6.0). Conclusions. Our analysis suggests PWID are more likely to share injection equipment with persons of concordant HCV status. C1 [Smith, Bryce D.; Zibbell, Jon E.] Ctr Dis Control & Prevent, Div Viral Hepatitis, Atlanta, GA USA. [Jewett, Amy] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Burt, Richard D.] Publ Hlth Seattle & King Cty, Seattle, WA USA. [Yartel, Anthony K.] Ctr Dis Control & Prevent Fdn, Atlanta, GA USA. [DiNenno, Elizabeth] Ctr Dis Control & Prevent, Div HIV AIDS Prevent, Atlanta, GA USA. RP Smith, BD (reprint author), 1600 Clifton Rd,MS G-37, Atlanta, GA 30333 USA. EM bsmith6@cdc.gov OI Yartel, Anthony/0000-0001-6586-9362 FU Division of Viral Hepatitis at the Centers for Disease Control and Prevention; Division of HIV/AIDS Prevention at the Centers for Disease Control and Prevention FX Funding for this study was provided by Divisions of Viral Hepatitis and HIV/AIDS Prevention at the Centers for Disease Control and Prevention. NR 37 TC 7 Z9 7 U1 0 U2 2 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0022-1899 EI 1537-6613 J9 J INFECT DIS JI J. Infect. Dis. PD DEC 15 PY 2013 VL 208 IS 12 BP 1934 EP 1942 DI 10.1093/infdis/jit520 PG 9 WC Immunology; Infectious Diseases; Microbiology SC Immunology; Infectious Diseases; Microbiology GA 259RS UT WOS:000327544600003 PM 24136794 ER PT J AU Lee, SS Fenter, P Nagy, KL Sturchio, NC AF Lee, Sang Soo Fenter, Paul Nagy, Kathryn L. Sturchio, Neil C. TI Changes in adsorption free energy and speciation during competitive adsorption between monovalent cations at the muscovite (001)- water interface SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID X-RAY REFLECTIVITY; MOLECULAR-DYNAMICS SIMULATIONS; SURFACE STRUCTURAL APPROACH; HYDRATION FORCES; ION ADSORPTION; (001)-SOLUTION INTERFACE; ELECTROLYTE-SOLUTIONS; CHARGE-DISTRIBUTION; HOFMEISTER SERIES; MINERAL SURFACES AB The relationships between the adsorption free energy and speciation of monovalent cations (Li+, Na-+,Na- K+, Rb+, and Cs+) at the muscovite (001)-solution interface were investigated using in situ resonant anomalous X-ray reflectivity. The Gibbs free energies of adsorption (Delta G(ads)(o)) for the cations and the changes in adsorbed Rb+ speciation during competitive adsorption were measured by monitoring changes in the coverage of reference-cation Rb+ as a function of molar ratio between Rb+ and other cations in binary solutions at fixed ionic strengths (0.003 m and 0.03 m). Larger adsorption free energies (Delta G(ads)(o) = -22.2 +/- 0.7, -23.5 +/- 0.6, and -21.2 +/- 0.8 kJ/mol, respectively) were observed for K+, Rb+, and Cs+, which form mainly inner-sphere (IS) complexes at the interface, compared to those for more strongly hydrated cations Na+ and Li+ (Delta G(ads)(o) = -16.7 perpendicular to 0.6 and -14.3 +/- 0.8 kJ/mol, respectively) which form dominantly outer-sphere (OS) complexes. The relative coverage of OS Rb+ with respect to IS Rb+ increased with increasing adsorbed coverages of the competing cation. This effect depends on the competing ion, with a larger increase in OS:IS ratio observed with Li+ or Cs+ compared to that with Na+ or K+. The change in proportions of OS to IS Rb+ is explained by systematic perturbation of the interfacial water structure caused by different hydration free energy and hydration structures of the competing cation. These results illustrate the complexity in the speciation and thermodynamics of cation adsorption in natural aqueous systems, and are discussed in the context of the Hofmeister effect. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Lee, Sang Soo; Fenter, Paul] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Nagy, Kathryn L.; Sturchio, Neil C.] Univ Illinois, Dept Earth & Environm Sci, Chicago, IL 60607 USA. RP Lee, SS (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM sslee@anl.gov FU Geosciences Research Program, Office of Basic Energy Sciences, United States Department of Energy [DE-AC02-06CH11357, DE-FG02-03ER15381]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Geosciences Research Program, Office of Basic Energy Sciences, United States Department of Energy under Contracts DE-AC02-06CH11357 to UChicago Argonne, LLC as operator of Argonne National Laboratory and DE-FG02-03ER15381 to the University of Illinois at Chicago. The reflectivity data were collected at beamlines 6-ID-B and 33-ID-D, Advanced Photon Source. Use of the Advanced Photon Source was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357 to UChicago Argonne, LLC as operator of Argonne National Laboratory. We are grateful to Dr. Ian C. Bourg and one anonymous reviewer for thoughtful comments. NR 62 TC 9 Z9 9 U1 7 U2 60 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD DEC 15 PY 2013 VL 123 BP 416 EP 426 DI 10.1016/j.gca.2013.07.033 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 250RM UT WOS:000326871400026 ER PT J AU Turchyn, AV Alt, JC Brown, ST DePaolo, DJ Coggon, RM Chi, GX Bedard, JH Skulski, T AF Turchyn, Alexandra V. Alt, Jeffrey C. Brown, Shaun T. DePaolo, Donald J. Coggon, Rosalind M. Chi, Guoxiang Bedard, Jean H. Skulski, Thomas TI Reconstructing the oxygen isotope composition of late Cambrian and Cretaceous hydrothermal vent fluid SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID SEA-SURFACE TEMPERATURES; CRUSTAL RESIDENCE TIME; BAIE-VERTE PENINSULA; BETTS COVE OPHIOLITE; UPPER OCEANIC-CRUST; CANADIAN APPALACHIANS; STABLE-ISOTOPE; PLEISTOCENE TEMPERATURES; PHANEROZOIC SEAWATER; JOSEPHINE OPHIOLITE AB Oxygen isotope analyses (delta O-18) of 16 quartz-epidote pairs from late Cambrian (Betts Cove and Mings Bight, Newfoundland), Ordovician (Thetford Mines, Quebec, Canada) and Cretaceous (Troodos, Cyprus) ophiolites are used to calculate the delta O-18 of the hydrothermal fluids from which they crystallized. We combine these with 3 quartz-fluid inclusion measurements and 3 quartz-magnetite measurements from the Cambrian ophiolites to explore how the range in the delta O-18 of submarine hydrothermal vent fluid has varied between the late Cambrian, Cretaceous and today. The range of calculated delta O-18 values of vent fluid (-4 to + 7.4) is larger than that of modern seafloor hydrothermal vent fluid (0 to + 4). We employ two numerical models to ascertain whether this range is most consistent with changes in paleo-seawater delta O-18 or with changes in the reactive flow path in ancient hydrothermal systems. A static calculation of the vent fluid oxygen isotope composition as a function of the water-rock ratio suggests that in an ocean with a lower delta O-18 than today, the range of vent fluid delta O-18 should be larger. Our data, however, show little evidence that the delta O-18 of the ocean was much lower than the global ice-free value of -1.2. A dual porosity model for reactive flow through fractured and porous media is used to model the relative evolution of the Sr-87/Sr-86 and delta O-18 of vent fluid in contact with rock. Our Sr-87/Sr-86 and delta O-18 for Cretaceous epidotes suggest the strontium concentration of the Cretaceous oceans may have been much higher than at present. The Sr-87/(86) Sr and delta O-18 data from Cambrian epidotes are strikingly different from the younger samples, and are difficult to model unless fluid-rock interaction in the Cambrian hydrothermal systems was substantially different. It is also possible that some of the quartz-epidote veins have been reset by obduction-related metamorphism. Our data suggest that the high calcium-to-sulfate ratio in early (and Cretaceous) seawater may have affected the degree of strontium isotope exchange, causing hydrothermal fluids to have Sr-87/(86) Sr closer to that of seawater than in modern systems. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Turchyn, Alexandra V.] Univ Cambridge, Dept Earth Sci, Cambridge CB2 3EQ, England. [Alt, Jeffrey C.] Univ Michigan, Dept Earth & Environm Sci, Ann Arbor, MI 48109 USA. [Brown, Shaun T.; DePaolo, Donald J.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Brown, Shaun T.; DePaolo, Donald J.] EO Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Coggon, Rosalind M.] Univ London Imperial Coll Sci Technol & Med, Dept Earth Sci & Engn, London, England. [Chi, Guoxiang] Univ Regina, Dept Geol, Regina, SK S4S 0A2, Canada. [Bedard, Jean H.] Geol Survey Canada, Quebec City, PQ, Canada. [Skulski, Thomas] Geol Survey Canada, Ottawa, ON K1A 0E8, Canada. RP Turchyn, AV (reprint author), Univ Cambridge, Dept Earth Sci, Cambridge CB2 3EQ, England. EM avt25@cam.ac.uk RI Brown, Shaun/E-9398-2015 OI Brown, Shaun/0000-0002-2159-6718 FU U.S. Department of Energy [DE-AC02-05CH11231] FX The authors wish to thank the Miller Institute for Basic Research (fellowship to AVT) and the Canadian Institute for Advanced Research (support for AVT). This manuscript benefited greatly from the comments of Graham Shields and two anonymous reviewers. Field assistance for sample collection was provided by Connor and Danny Lees (Cyprus), Yves Moussallam and Stephen Hinchey (Betts Cove, Newfoundland). Support for STB and DJD was provided by the Director, Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 99 TC 2 Z9 2 U1 5 U2 28 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD DEC 15 PY 2013 VL 123 BP 440 EP 458 DI 10.1016/j.gca.2013.08.015 PG 19 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 250RM UT WOS:000326871400028 ER PT J AU Hibbs, MR AF Hibbs, Michael R. TI Alkaline Stability of Poly(phenylene)-Based Anion Exchange Membranes with Various Cations SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE alkaline fuel cell; anion exchange membrane; guanidinium; imidazolium; ionomers; membrane; sidechain; stability; stabilization ID FUEL-CELL APPLICATIONS; HYDROXIDE; POLYELECTROLYTE; IONOMER AB Anion exchange membranes comprised of a poly(phenylene) backbone and one of five different cationic head-groups are prepared, briefly characterized, and tested for stability in 4 M KOH at 90 degrees C. The two membranes with resonance-stabilized cations (benzyl pentamethylguanidinium and benzyl N-methylimidazolium) show large (>25%) decreases in both conductivity and ion exchange capacity (IEC) after just one day of testing. The membrane with benzyl trimethylammonium cations shows a 33% loss of conductivity (14% decrease in IEC) after 14 days while the membrane with trimethylammonium cations attached by a hexamethylene spacer shows the least degradation: a 5% loss of conductivity over 14 days with no accompanying loss in IEC. A similar membrane which has a six-carbon spacer and a ketone adjacent to the phenyl ring shows much lower stability, suggesting that the ketone takes part in degradation reactions. (c) 2012 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2013, 51, 1736-1742, 2013 C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Hibbs, MR (reprint author), Sandia Natl Labs, POB 5800,MS 0888, Albuquerque, NM 87185 USA. EM mhibbs@sandia.gov FU Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 32 TC 68 Z9 68 U1 5 U2 136 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD DEC 15 PY 2013 VL 51 IS 24 SI SI BP 1736 EP 1742 DI 10.1002/polb.23149 PG 7 WC Polymer Science SC Polymer Science GA 248JR UT WOS:000326696200002 ER PT J AU Janarthanan, R Horan, JL Caire, BR Ziegler, ZC Yang, Y Zuo, XB Liberatore, MW Hibbs, MR Herring, AM AF Janarthanan, Rajeswari Horan, James L. Caire, Benjamin R. Ziegler, Zachary C. Yang, Yuan Zuo, Xiaobing Liberatore, Matthew W. Hibbs, Michael R. Herring, Andrew M. TI Understanding Anion Transport in an Aminated Trimethyl Polyphenylene with High Anionic Conductivity SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE ionomer; polyaromatics; diffusion; SAXS; alkaline exchange membrane; fuel cell; anion conductivity; anion diffusion ID ALKALINE FUEL-CELLS; X-RAY-SCATTERING; SMALL-ANGLE SCATTERING; EXCHANGE MEMBRANES; DIFFUSION MEASUREMENTS; STIMULATED ECHO; SELF-DIFFUSION; NMR-DIFFUSION; WATER-UPTAKE; IONOMER AB An alkaline exchange membrane (AEM) based on an aminated trimethyl poly(phenylene) is studied in detail. This article reports hydroxide ion conductivity through an in situ method that allows for a more accurate measurement. The ionic conductivities of the membrane in bromide and carbonate forms at 90 degrees C and 95% RH are found to be 13 and 17 mS cm(-1) respectively. When exchanged with hydroxide, conductivity improved to 86 mS cm(-1) under the same experimental conditions. The effect of relative humidity on water uptake and the SAXS patterns of the AEM membranes were investigated. SAXS analysis revealed a rigid aromatic structure of the AEM membrane with no microphase separation. The synthesized AEM is shown to be mechanically stable as seen from the water uptake and SAXS studies. Diffusion NMR studies demonstrated a steady state long-range diffusion constant, D of 9.8 x 10(-6) cm(2) s(-1) after 50-100 ms. (c) 2012 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2013, 51, 1743-1750, 2013 C1 [Janarthanan, Rajeswari; Horan, James L.; Caire, Benjamin R.; Ziegler, Zachary C.; Liberatore, Matthew W.; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Yang, Yuan] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Zuo, Xiaobing] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Hibbs, Michael R.] Sandia Natl Labs, Dept Mat Devices & Energy Technol, Albuquerque, NM 87123 USA. RP Herring, AM (reprint author), Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. EM aherring@mines.edu RI Liberatore, Matthew/B-6828-2008; OI Caire, Benjamin/0000-0003-3379-7733; Herring, Andrew/0000-0001-7318-5999 FU LDRD grant from Sandia National Laboratories; ARO through a MURI award [W911NF-10-1-0520]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by a LDRD grant from Sandia National Laboratories and in part by the ARO through a MURI award, W911NF-10-1-0520. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 39 TC 21 Z9 22 U1 3 U2 68 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD DEC 15 PY 2013 VL 51 IS 24 SI SI BP 1743 EP 1750 DI 10.1002/polb.23164 PG 8 WC Polymer Science SC Polymer Science GA 248JR UT WOS:000326696200003 ER PT J AU Tsai, TH Maes, AM Vandiver, MA Versek, C Seifert, S Tuominen, M Liberatore, MW Herring, AM Coughlin, EB AF Tsai, Tsung-Han Maes, Ashley M. Vandiver, Melissa A. Versek, Craig Seifert, Soenke Tuominen, Mark Liberatore, Matthew W. Herring, Andrew M. Coughlin, E. Bryan TI Synthesis and Structure-Conductivity Relationship of Polystyrene-block-Poly(vinyl benzyl trimethylammonium) for Alkaline Anion Exchange Membrane Fuel Cells SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE amphiphilic block copolymers; anion exchange membrane fuel cell; atom transfer radical polymerization (ATRP); phase separation; polymeric electrolyte membranes; polystyrene; poly(vinyl benzyl trimethylammonium); structure; conductivity relationship ID RADICAL POLYMERIZATION; VINYLBENZYL CHLORIDE; TRANSPORT-PROPERTIES; IONIC-CONDUCTIVITY; BLOCK-COPOLYMERS; ORDER-DISORDER; PHASE-BEHAVIOR; HYDROXIDE; PERFORMANCE; METHANOL AB Block copolymers of polystyrene-b-poly(vinyl benzyl trimethylammonium tetrafluoroborate) (PS-b-[PVBTMA][BF4]) were synthesized by sequential monomer addition using atom transfer radical polymerization. Membranes of the block copolymers were prepared by drop casting from dimethylformamide. Initial evaluation of the microphase separation in these PS-b-[PVBTMA][BF4] materials via SAXS revealed the formation of spherical, cylindrical, and lamellar morphologies. Block copolymers of polystyrene-b-poly(vinyl benzyl trimethylammonium hydroxide) (PS-b-[PVBTMA][OH]) were prepared as polymeric alkaline anion exchange membranes materials by ion exchange from PS-b-[PVBTMA][BF4] with hydroxide in order to investigate the relationship between morphology and ionic conductivity. Studies of humidity [relative humidity (RH)]-dependent conductivity at 80 degrees C showed that the conductivity increases with increasing humidity. Moreover, the investigation of the temperature-dependent conductivity at RH = 50, 70, and 90% showed a significant effect of grain boundaries in the membranes against the formation of continuous conductive channels, which is an important requirement for achieving high ion conductivity. (c) 2012 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2013, 51, 1751-1760, 2013 C1 [Tsai, Tsung-Han; Coughlin, E. Bryan] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Maes, Ashley M.; Vandiver, Melissa A.; Liberatore, Matthew W.; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Versek, Craig; Tuominen, Mark] Univ Massachusetts, Dept Phys, Hasbrouck Lab 411, Amherst, MA 01003 USA. [Seifert, Soenke] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Coughlin, EB (reprint author), Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. EM coughlin@mail.pse.umass.edu RI Liberatore, Matthew/B-6828-2008; Tuominen, Mark/A-6129-2012; OI Herring, Andrew/0000-0001-7318-5999 FU US Army MURI on Ion Transport in Complex Heterogeneous Organic Materials [W911NF-10-1-0520]; National Science Foundation Center for Hierarchical Manufacturing [CMMI-1025020]; IGERT program [DGE-0504485]; US DOE [DE-AC02-06CH11357] FX Funding was provided by the US Army MURI on Ion Transport in Complex Heterogeneous Organic Materials (W911NF-10-1-0520). Partial support was provided by the National Science Foundation Center for Hierarchical Manufacturing (CMMI-1025020) and an IGERT program (DGE-0504485). The use of Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under contract no. DE-AC02-06CH11357. NR 49 TC 31 Z9 32 U1 9 U2 116 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD DEC 15 PY 2013 VL 51 IS 24 SI SI BP 1751 EP 1760 DI 10.1002/polb.23170 PG 10 WC Polymer Science SC Polymer Science GA 248JR UT WOS:000326696200004 ER PT J AU Vandiver, MA Horan, JL Yang, Y Tansey, ET Seifert, S Liberatore, MW Herring, AM AF Vandiver, Melissa A. Horan, James L. Yang, Yuan Tansey, Emily T. Seifert, Soeenke Liberatore, Matthew W. Herring, Andrew M. TI Synthesis and Characterization of Perfluoro Quaternary Ammonium Anion Exchange Membranes SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE ionomers; fluoropolymers; NMR; SAXS ID POLYMER ELECTROLYTE MEMBRANES; ALKALINE FUEL-CELLS; IONOMER MEMBRANES; DIFFUSION; WATER; NAFION; CONDUCTIVITY; SCATTERING; STATE; NMR AB In this study, new alkaline exchange membranes were prepared from the perfluorinated 3M ionomer with various quaternary ammonium cations attached with sulfonamide linkage. The degree of functionalization varied depending on the cation species, resulting in different ion exchange capacities (IECs), 0.33-0.72 meq g(-1). There was evidence of polymer degradation when the films were exposed to hydroxide, and hence all membrane characterization was performed in the chloride form. Conductivity was dependent on cation species and IEC, E-a = 36-59 kJ mol(-1). Diffusion of water through the membrane was relatively high 1.6 x 10(-5) cm(2) s(-1) and indicated restriction over a range of diffusion times, 6-700 ms. Water uptake (WU) in the membranes was generally low and the hydration level varied based on cation species, = 6-11. Small-angle scattering experiments suggested ionic aggregation, 37-42 angstrom, independent of cation species but slight differences in long-range order with cation species. (c) 2012 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2013, 51, 1761-1769, 2013 C1 [Vandiver, Melissa A.; Horan, James L.; Tansey, Emily T.; Liberatore, Matthew W.; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Yang, Yuan] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Seifert, Soeenke] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Herring, AM (reprint author), Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. EM aherring@mines.edu RI Liberatore, Matthew/B-6828-2008; OI Herring, Andrew/0000-0001-7318-5999 FU Army Research Laboratory under MURI [W911NF-10-1-0520]; U.S. DOE [DE-AC02-06CH11357] FX The authors thank the Army Research Laboratory for support of this research under the MURI grant number #W911NF-10-1-0520. The authors thank Steven J. Hamrock of 3M Company for useful discussions and supplying the 3M ionomer. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 39 TC 11 Z9 11 U1 3 U2 62 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD DEC 15 PY 2013 VL 51 IS 24 SI SI BP 1761 EP 1769 DI 10.1002/polb.23171 PG 9 WC Polymer Science SC Polymer Science GA 248JR UT WOS:000326696200005 ER PT J AU Yan, JL Moore, HD Hibbs, MR Hickner, MA AF Yan, Jingling Moore, Hunter D. Hibbs, Michael R. Hickner, Michael A. TI Synthesis and Structure-Property Relationships of Poly(sulfone)s for Anion Exchange Membranes SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE anion exchange membrane; conductivity; fuel cell; ionomers; membranes; polycondensation; poly(sulfone); water uptake ID ETHER SULFONE) COPOLYMERS; FUEL-CELL APPLICATIONS; POLYMER ELECTROLYTE; PERFORMANCE; HYDROXIDE; CHLOROMETHYLATION; CONDUCTIVITY; TRANSPORT; IONOMER; SERIES AB Membranes based on cationic polymers that conduct anions are important for enabling alkaline membrane fuel cells and other solid-state electrochemical devices that operate at high pH. Anion exchange membranes with poly(arylene ether sulfone) backbones are demonstrated by two routes: chloromethylation of commercially available poly(sulfone)s or radical bromination of benzylmethyl moieties in poly(sulfone)s containing tetramethylbisphenol A monomer residues. Polymers with tethered trimethylbenzyl ammonium moieties resulted from conversion of the halomethyl groups by quaternization with trimethyl amine. The water uptake of the chloromethylated polymers was dependent on the type of poly(sulfone) backbone for a given IEC. Bisphenol A-based Udel (R) poly(sulfone) membranes swelled in water to a large extent while membranes from biphenol-based Radel (R) poly(sulfone), a stiffer backbone than Udel, only showed moderate water uptake. The water uptake of cationic poly(sulfone)s was further reduced by synthesizing tetramethylbisphenol A and 4,4-biphenol-containing poly(sulfone) copolymers where the ionic groups were clustered on the tetramethylbisphenol A residues. The conductivity of all samples scaled with the bulk water uptake. The hydration number of the membranes could be increased by casting membranes from the ionic form polymers versus converting the halomethyl form cast polymers to ionic form in the solid state. (c) 2013 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2013, 51, 1790-1798, 2013 C1 [Yan, Jingling; Moore, Hunter D.; Hickner, Michael A.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Hibbs, Michael R.] Sandia Natl Labs, Fuel & Energy Transit Dept, Albuquerque, NM 87123 USA. RP Hickner, MA (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. EM hickner@matse.psu.edu RI Yan, Jingling/F-8512-2011 FU Office of Naval Research [N00014-08-1-0730, N00014-10-1-0875]; Advanced Research Projects Agency-Energy (ARPA-E), US Department of Energy [DE-AR0000121]; United States Department of Energy's National Nuclear Security Administration [DEAC04-94AL85000] FX The authors acknowledge support of the Office of Naval Research through grants N00014-08-1-0730 and N00014-10-1-0875 and the Advanced Research Projects Agency-Energy (ARPA-E), US Department of Energy, under Award No. DE-AR0000121. Sandia is a multiprogram laboratory operated by Sandia Corp., a Lockheed Martin Co., for the United States Department of Energy's National Nuclear Security Administration under Contract DEAC04-94AL85000. The authors further acknowledge Solvay Advanced Polymers for kind donations of the Udel (R) and Radel (R) poly(sulfone) starting materials. NR 25 TC 15 Z9 15 U1 2 U2 78 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD DEC 15 PY 2013 VL 51 IS 24 SI SI BP 1790 EP 1798 DI 10.1002/polb.23331 PG 9 WC Polymer Science SC Polymer Science GA 248JR UT WOS:000326696200008 ER PT J AU Cai, YF Bai, ZJ Pask, JE Sukumar, N AF Cai, Yunfeng Bai, Zhaojun Pask, John E. Sukumar, N. TI Hybrid preconditioning for iterative diagonalization of ill-conditioned generalized eigenvalue problems in electronic structure calculations SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Hybrid preconditioning; Iterative diagonalization; Ill conditioned GHEP; Steepest descent method; Electronic structure calculation ID FINITE-ELEMENT-METHOD; DIFFERENCE-PSEUDOPOTENTIAL METHOD; DENSITY-FUNCTIONAL THEORY; INDEFINITE SYSTEMS; LINEAR-EQUATIONS; BASIS-SET; ACCELERATION; MATRICES AB The iterative diagonalization of a sequence of large ill-conditioned generalized eigenvalue problems is a computational bottleneck in quantum mechanical methods employing a nonorthogonal basis for ab initio electronic structure calculations. We propose a hybrid preconditioning scheme to effectively combine global and locally accelerated preconditioners for rapid iterative diagonalization of such eigenvalue problems. In partition-of-unity finite-element (PUFE) pseudopotential density-functional calculations, employing a nonorthogonal basis, we show that the hybrid preconditioned block steepest descent method is a cost-effective eigensolver, outperforming current state-of-the-art global preconditioning schemes, and comparably efficient for the ill-conditioned generalized eigenvalue problems produced by PUFE as the locally optimal block preconditioned conjugate-gradient method for the well-conditioned standard eigenvalue problems produced by planewave methods. (c) 2013 Elsevier Inc. All rights reserved. C1 [Cai, Yunfeng] Peking Univ, LMAM, Beijing 100871, Peoples R China. [Cai, Yunfeng] Peking Univ, Sch Math Sci, Beijing 100871, Peoples R China. [Cai, Yunfeng; Bai, Zhaojun] Univ Calif Davis, Dept Comp Sci, Davis, CA 95616 USA. [Bai, Zhaojun] Univ Calif Davis, Dept Math, Davis, CA 95616 USA. [Pask, John E.] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. [Sukumar, N.] Univ Calif Davis, Dept Civil & Environm Engn, Davis, CA 95616 USA. RP Cai, YF (reprint author), Peking Univ, LMAM, Beijing 100871, Peoples R China. EM yfcai@math.pku.edu.cn; bai@cs.ucdavis.edu; pask1@llnl.gov; nsukumar@ucdavis.edu RI Sukumar, N/B-1660-2008 FU UC Lab Fees Research Program [118128]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Supported in part by award no. 118128 from the UC Lab Fees Research Program. This work performed, in part, under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 60 TC 3 Z9 3 U1 0 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD DEC 15 PY 2013 VL 255 BP 16 EP 30 DI 10.1016/j.jcp.2013.07.020 PG 15 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 232XF UT WOS:000325527100002 ER PT J AU Cook, AW AF Cook, Andrew W. TI Effects of heat conduction on artificial viscosity methods for shock capturing SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Large-eddy simulation; Subgrid-scale models; Shocks; Turbulence; Artificial viscosity; Thermal conductivity; Stagnation enthalpy ID SCHEMES; HYPERVISCOSITY; RESOLUTION; WAVE AB We investigate the efficacy of artificial thermal conductivity for shock capturing. The conductivity model is derived from artificial bulk and shear viscosities, such that stagnation enthalpy remains constant across shocks. By thus fixing the Prandtl number, more physical shock profiles are obtained, only on a larger scale. The conductivity model does not contain any empirical constants. It increases the net dissipation of a computational algorithm but is found to better preserve symmetry and produce more robust solutions for strong-shock problems. (c) 2013 Elsevier Inc. All rights reserved. C1 Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Cook, AW (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM awcook@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 18 TC 0 Z9 0 U1 1 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD DEC 15 PY 2013 VL 255 BP 48 EP 52 DI 10.1016/j.jcp.2013.08.003 PG 5 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 232XF UT WOS:000325527100004 ER PT J AU Chen, L He, YL Kang, QJ Tao, WQ AF Chen, Li He, Ya-Ling Kang, Qinjun Tao, Wen-Quan TI Coupled numerical approach combining finite volume and lattice Boltzmann methods for multi-scale multi-physicochemical processes SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Multi-scale simulation; Lattice Boltzmann method; Finite volume method; Coupling (hybrid); Multi-physicochemical processes; Reconstruction operator ID MEMBRANE FUEL-CELL; GAS-DIFFUSION LAYER; EFFICIENT SEGREGATED ALGORITHM; INCOMPRESSIBLE FLUID-FLOW; HEAT-TRANSFER PROBLEMS; NATURAL-CONVECTION; MOLECULAR-DYNAMICS; AMMONIA DECOMPOSITION; RECTANGULAR ENCLOSURE; DIFFERENCE SCHEME AB A coupled (hybrid) simulation strategy spatially combining the finite volume method (FVM) and the lattice Boltzmann method (LBM), called CFVLBM, is developed to simulate coupled multi-scale multi-physicochemical processes. In the CFVLBM, computational domain of multi-scale problems is divided into two sub-domains, i.e., an open, free fluid region and a region filled with porous materials. The FVM and LBM are used for these two regions, respectively, with information exchanged at the interface between the two sub-domains. A general reconstruction operator (RO) is proposed to derive the distribution functions in the LBM from the corresponding macro scalar, the governing equation of which obeys the convection-diffusion equation. The CFVLBM and the RO are validated in several typical physicochemical problems and then are applied to simulate complex multi-scale coupled fluid flow, heat transfer, mass transport, and chemical reaction in a wall-coated micro reactor. The maximum ratio of the grid size between the FVM and LBM regions is explored and discussed. (c) 2013 Elsevier Inc. All rights reserved. C1 [Chen, Li; He, Ya-Ling; Tao, Wen-Quan] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Thermo Fluid Sci & Engn, Shaanxi 710049, Peoples R China. [Kang, Qinjun] Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM USA. RP Tao, WQ (reprint author), Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Thermo Fluid Sci & Engn, Shaanxi 710049, Peoples R China. EM wqtao@mail.xjtu.edu.cn RI Chen, Li/P-4886-2014; Kang, Qinjun/A-2585-2010 OI Chen, Li/0000-0001-7956-3532; Kang, Qinjun/0000-0002-4754-2240 FU key project of NNSFC [51136004] FX This work was supported by the key project of NNSFC (51136004). NR 62 TC 27 Z9 27 U1 6 U2 89 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD DEC 15 PY 2013 VL 255 BP 83 EP 105 DI 10.1016/j.jcp.2013.07.034 PG 23 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 232XF UT WOS:000325527100006 ER PT J AU Velechovsky, J Kucharik, M Liska, R Shashkov, M Vachal, P AF Velechovsky, J. Kucharik, M. Liska, R. Shashkov, M. Vachal, P. TI Symmetry- and essentially-bound-preserving flux-corrected remapping of momentum in staggered ALE hydrodynamics SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Staggered hydrodynamics; ALE; Remap of vectors; Symmetric reconstruction ID LAGRANGIAN-EULERIAN METHOD; MULTIMATERIAL ALE; COMPUTING METHOD; REPAIR PARADIGM; FLOW SPEEDS; ALGORITHM; COMPUTATIONS; CONSERVATION; TRANSPORT; EQUATIONS AB We present a new flux-corrected approach for remapping of velocity in the framework of staggered arbitrary Lagrangian-Eulerian methods. The main focus of the paper is the definition and preservation of coordinate invariant local bounds for velocity vector and development of momentum remapping method such that the radial symmetry of the radially symmetric flows is preserved when remapping from one equiangular polar mesh to another. The properties of this new method are demonstrated on a set of selected numerical cyclic remapping tests and a full hydrodynamic example. (C) 2013 Elsevier Inc. All rights reserved. C1 [Velechovsky, J.; Kucharik, M.; Liska, R.; Vachal, P.] Czech Tech Univ, FNSPE, Prague 11519 1, Czech Republic. [Shashkov, M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Velechovsky, J (reprint author), Czech Tech Univ, FNSPE, Brehova 7, Prague 11519 1, Czech Republic. EM velecjan@fjfi.cvut.cz RI Liska, Richard/C-3142-2009; Vachal, Pavel/G-2131-2011; OI Liska, Richard/0000-0002-6149-0440; Vachal, Pavel/0000-0002-6668-9045 FU US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; US Department of Energy Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research; US Department of Energy National Nuclear Security Administration Advanced Simulation and Computing (ASC) Program; Czech Technical University [5G513/220/OHK4/3T/14]; Czech Science Foundation project [P201/12/P554, RVO: 68407700] FX This work was performed under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The authors gratefully acknowledge the partial support of the US Department of Energy Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research and the partial support of the US Department of Energy National Nuclear Security Administration Advanced Simulation and Computing (ASC) Program. This research was supported in parts by the Czech Technical University grant 5G513/220/OHK4/3T/14, the Czech Science Foundation project P201/12/P554 and RVO: 68407700. We thank both anonymous referees for their useful comments. NR 39 TC 8 Z9 8 U1 2 U2 27 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD DEC 15 PY 2013 VL 255 BP 590 EP 611 DI 10.1016/j.jcp.2013.08.037 PG 22 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 232XF UT WOS:000325527100032 ER PT J AU Rycroft, CH Wilkening, J AF Rycroft, Chris H. Wilkening, Jon TI Computation of three-dimensional standing water waves SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Water waves; Multigrid methods; Optimization ID TIME-PERIODIC SOLUTIONS; ALMOST-HIGHEST WAVE; GRAVITY-WAVES; DEEP-WATER; FINITE DEPTH; NUMERICAL-SIMULATION; SURFACE-TENSION; WILTON RIPPLES; FARADAY WAVES; EXTREME FORM AB We develop a method for computing three-dimensional gravity-driven water waves, which we use to search for time-periodic standing wave solutions. We simulate an inviscid, irrotational, incompressible fluid bounded below by a flat wall, and above by an evolving free surface. The computations make use of spectral derivatives on the surface, but also require computing a velocity potential in the bulk, which we carry out using a finite element method with fourth-order elements that are curved to match the free surface. This computationally expensive step is solved using a parallel multigrid algorithm, which is discussed in detail. Time-periodic solutions are searched for using a previously developed overdetermined shooting method. Several families of large-amplitude three-dimensional standing waves are found in both shallow and deep regimes, and their physical characteristics are examined and compared to previously known two-dimensional solutions. Published by Elsevier Inc. C1 [Rycroft, Chris H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Rycroft, Chris H.; Wilkening, Jon] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Rycroft, Chris H.; Wilkening, Jon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Math, Berkeley, CA 94720 USA. [Rycroft, Chris H.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. RP Rycroft, CH (reprint author), Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. EM chr@seas.harvard.edu; wilken@math.berkeley.edu OI Rycroft, Chris/0000-0003-4677-6990 FU Office of Science, Computational and Technology Research, U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMS-0955078] FX This work was supported by the Director, Office of Science, Computational and Technology Research, U.S. Department of Energy under contract number DE-AC02-05CH11231, and by the National Science Foundation through grant DMS-0955078. NR 53 TC 6 Z9 6 U1 2 U2 20 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD DEC 15 PY 2013 VL 255 BP 612 EP 638 DI 10.1016/j.jcp.2013.08.026 PG 27 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 232XF UT WOS:000325527100033 ER PT J AU Ge, XX Zhang, WY Lin, YH Du, D AF Ge, Xiaoxiao Zhang, Weiying Lin, Yuehe Du, Dan TI Magnetic Fe3O4@TiO2 nanoparticles-based test strip immunosensing device for rapid detection of phosphorylated butyrylcholinesterase SO BIOSENSORS & BIOELECTRONICS LA English DT Article DE Test strip; Immunosensor; Organophosphorous pesticides; Biomarker; Phosphorylated butyrylcholinesterase ID FLOW TEST STRIP; GOLD NANOPARTICLES; ELECTROCHEMICAL IMMUNOSENSOR; ORGANOPHOSPHORUS PESTICIDES; CHOLINESTERASE ACTIVITY; ENZYME-ACTIVITY; NERVE AGENTS; EXPOSURE; BIOMARKER; AMPLIFICATION AB An integrated magnetic nanoparticles-based test strip immunosensing device was developed for rapid and sensitive quantification of phosphorylated butyrylcholinesterase (BChE), the biomarker of exposure to organophosphorous pesticides (OP), in human plasma. In order to overcome the difficulty in scarce availability of OP-specific antibody, here magnetic Fe3O4@TiO2 nanoparticles were used and adsorbed on the test strip through a small magnet inserted in the device to capture target OP-BChE through selective binding between TiO2 and OP moiety. Further recognition was completed by horseradish peroxidase (HRP) and anti-BChE antibody (Ab) co-immobilized gold nanoparticles (GNPs). Their strong affinities among Fe3O4@TiO2, OP-BChE and HRP/Ab-GNPs were characterized by quartz crystal microbalance (QCM), surface plasmon resonance (SPR) and square wave voltammetry (SWV) measurements. After cutting off from test strip, the resulted immunocomplex (HRP/Ab-GNPs/OP-BChE/Fe3O4@TiO2) was measured by SWV using a screen printed electrode under the test zone. Greatly enhanced sensitivity was achieved by introduction of GNPs to link enzyme and antibody at high ratio, which amplifies electrocatalytic signal significantly. Moreover, the use of test strip for fast immunoreactions reduces analytical time remarkably. Under the optimized conditions, the developed device shows a broader linear response over the concentration of OP-BChE from 0.05 nM to 10 nM within 15 min, with a detection limit of 0.01 nM. Coupling with a portable electrochemical detector, the integrated device with advanced nanotechnology displays great promise for sensitive, rapid and on-site evaluation of OP poisoning. (C) 2013 Elsevier B.V. All rights reserved. C1 [Ge, Xiaoxiao; Du, Dan] Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Coll Chem, Wuhan 430079, Peoples R China. [Zhang, Weiying; Lin, Yuehe; Du, Dan] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Du, D (reprint author), Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Coll Chem, Wuhan 430079, Peoples R China. EM dan.du@mail.ccnu.edu.cn RI Du, Dan (Annie)/G-3821-2012; Lin, Yuehe/D-9762-2011 OI Lin, Yuehe/0000-0003-3791-7587 FU National Natural Science Foundation of China [21275062, 21075047]; Program for New Century Excellent Talents in University [NCET-12-0871]; US-DOE [DE-AC05-76RL01830] FX This work was supported by the National Natural Science Foundation of China (21275062, 21075047) and the Program for New Century Excellent Talents in University (NCET-12-0871). Pacific Northwest National Laboratory is operated by Battelle for US-DOE under Contract DE-AC05-76RL01830. We specially thank Prof. Chunming Yang in Hunan Normal University for preparation and characterization of the nanoparticles. NR 34 TC 23 Z9 24 U1 13 U2 239 PU ELSEVIER ADVANCED TECHNOLOGY PI OXFORD PA OXFORD FULFILLMENT CENTRE THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0956-5663 J9 BIOSENS BIOELECTRON JI Biosens. Bioelectron. PD DEC 15 PY 2013 VL 50 BP 486 EP 491 DI 10.1016/j.bios.2013.07.017 PG 6 WC Biophysics; Biotechnology & Applied Microbiology; Chemistry, Analytical; Electrochemistry; Nanoscience & Nanotechnology SC Biophysics; Biotechnology & Applied Microbiology; Chemistry; Electrochemistry; Science & Technology - Other Topics GA 228LL UT WOS:000325188200075 PM 23911770 ER PT J AU Kim, JH Lee, JH Min, JY Kim, SW Park, CH Yeom, JT Byun, TS AF Kim, Jeoung Han Lee, Jae Hoon Min, Jeon Yeong Kim, Seong Woong Park, Chan Hee Yeom, Jong Taek Byun, Thak Sang TI Cryomilling effect on the mechanical alloying behaviour of ferritic oxide dispersion strengthened powder with Y2O3 SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Oxide dispersion strengthened alloy; Mechanical alloying; Grain refinement; Nuclear reactor materials; X-ray diffraction ID ELECTRON BACKSCATTER DIFFRACTION; NANOSTRUCTURED MATERIALS; STEELS AB Cryogenic cooling effect on mechanical alloying of the mixture of Fe-14Cr-3W-0.1Ti and Y2O3 powders was investigated. The powder mixtures were ball milled for 40 h at room-temperature and -150 degrees C. Cryomilling produced much finer particle/grain size than conventional room-temperature milling. XRD diffraction peak intensity was much lower under cryomilling conditions due to formation of nano-size grains and increased residual microstrain. Absorption amounts of interstitial elements were considerably higher under cryomilling conditions. (C) 2013 Elsevier B.V. All rights reserved. C1 [Kim, Jeoung Han; Min, Jeon Yeong; Kim, Seong Woong; Park, Chan Hee; Yeom, Jong Taek] Korea Inst Mat Sci, Special Alloys Grp, Chang Won, South Korea. [Lee, Jae Hoon] POSCO Tech Res Labs, Gwangyang Si 545090, Jeonnam, South Korea. [Byun, Thak Sang] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Kim, JH (reprint author), Korea Inst Mat Sci, Special Alloys Grp, Chang Won, South Korea. EM kjh1754@kims.re.kr FU Korea Institute of Materials Science; U.S. Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; UT-Battelle, LLC FX This research was sponsored by the in-house research project of the Korea Institute of Materials Science. It was also sponsored by U.S. Department of Energy, Office of Nuclear Energy under Contract DE-AC05-00OR22725 with UT-Battelle, LLC. Special thanks go to Dr. Heung Man Kim and Ms. Sang Mi Woo. NR 16 TC 9 Z9 9 U1 1 U2 30 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 BP 125 EP 130 DI 10.1016/j.jallcom.2013.04.165 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 219RH UT WOS:000324525800019 ER PT J AU Khatkhatay, F Jian, J Jiao, L Su, Q Gan, J Cole, JI Wang, HY AF Khatkhatay, Fauzia Jian, Jie Jiao, Liang Su, Qing Gan, Jian Cole, James I. Wang, Haiyan TI Diffusion barrier properties of nitride-based coatings on fuel cladding SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE TiN; ZrN; Cladding tube; Diffusion barrier ID IRON; CERIUM; INTERDIFFUSION; REACTORS; DIAMOND; FILMS AB In this work, titanium nitride (TiN) and zirconium nitride (ZrN) coatings are proposed as diffusion barriers between stainless steel nuclear fuel cladding and lanthanide fission products. TiN and ZrN have been coated as barrier materials between pure Fe and Ce, i.e. diffusion couples of Fe/TiN/Ce and Fe/ZrN/Ce, annealed up to a temperature of 600 degrees C, and compared to the diffusion behavior of uncoated Fe/Ce. Back-scattered electron images and energy dispersive X-ray spectroscopy measurements confirm that, with a 500 nm TiN or ZrN layer, no obvious diffusion is observed between Fe and Ce. Basic diffusion characteristics of the Fe/Ce couple have also been measured and compared with the TiN and ZrN coated ones. These preliminary results strongly advocate that TiN and ZrN coatings may be feasible as diffusion barriers against Ce and possibly other lanthanide fission products. (C) 2013 Elsevier B.V. All rights reserved. C1 [Khatkhatay, Fauzia; Jian, Jie; Wang, Haiyan] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Jiao, Liang; Su, Qing; Wang, Haiyan] Texas A&M Univ, Mat Sci & Engn Program, College Stn, TX 77843 USA. [Gan, Jian; Cole, James I.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Wang, HY (reprint author), Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. EM wangh@ece.tamu.edu RI Su, Qing/N-2518-2014; Wang, Haiyan/P-3550-2014; OI Wang, Haiyan/0000-0002-7397-1209; Su, Qing/0000-0003-2477-0002; Cole, James/0000-0003-1178-5846 FU Idaho National Laboratory through subcontract under the Department of Energy's (DOE) Fuel Cycle Research and Development Program FX This work was funded by the Idaho National Laboratory through subcontract under the Department of Energy's (DOE) Fuel Cycle Research and Development Program. NR 21 TC 8 Z9 8 U1 6 U2 47 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 15 PY 2013 VL 580 BP 442 EP 448 DI 10.1016/j.jallcom.2013.06.108 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 219RH UT WOS:000324525800069 ER PT J AU Dong, JP Yu, XQ Sun, Y Liu, L Yang, XQ Huang, XJ AF Dong, Jinping Yu, Xiqian Sun, Yang Liu, Lei Yang, Xiaoqing Huang, Xuejie TI Trip lite LiFeSO4F as cathode material for Li-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Fluorosulphate; Cathode material; Lithium ion batteries; Cation mixing ID RECHARGEABLE LITHIUM BATTERIES; ELECTRODE AB Monoclinic phase LiFeSO4F has a triplite like structure in which Li+/Fe2+ is fully mixing. Not 100% Li can be extracted from the lattice easily even at a rate of C/20, and the valence of Fe changes between ca +2 and +2.5 observed by XANES for a Li/LiFeSO4F cell cycled between 2.2 and 4.6 V. Two-phase reaction mechanism is verified by GITT due to the appearance of a flat plateau, and large polarization appears after more than 50% Li extracted from triplite-LiFeSO4F. A core shell model has been mentioned to explain its extreme polarization. In the fully mixing structure, there is no intact long-range pathway for Li+, so leading to sluggish kinetics effect and "inert" Li+ in the lattice. (C) 2012 Elsevier B.V. All rights reserved. C1 [Dong, Jinping; Sun, Yang; Liu, Lei; Huang, Xuejie] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Yu, Xiqian; Yang, Xiaoqing] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Huang, XJ (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. EM xjhuang@iphy.ac.cn RI Yu, Xiqian/B-5574-2014; liu, lei/M-6396-2016 OI Yu, Xiqian/0000-0001-8513-518X; liu, lei/0000-0003-3631-1874 FU Hi-tech Research and Development Program of China [2009AA033101]; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. DOE [DE-AC02-98CH10886]; U.S. DOE FX This work was supported by Hi-tech Research and Development Program of China (2009AA033101). The work at Brookhaven National Lab, was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. DOE under Contract No. DE-AC02-98CH10886. Research at beam line X14A and X18A were partially sponsored by the U.S. DOE. The authors thank the help from Dr. Steven N. Ehrlich. NR 13 TC 7 Z9 7 U1 7 U2 122 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD DEC 15 PY 2013 VL 244 SI SI BP 716 EP 720 DI 10.1016/j.jpowsour.2012.11.084 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 219MR UT WOS:000324511600114 ER PT J AU Alexander, CS Key, CT Schumacher, SC AF Alexander, C. S. Key, C. T. Schumacher, S. C. TI Dynamic response and modeling of a carbon fiber-epoxy composite subject to shock loading SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID IMPACT; BEHAVIOR AB Unidirectional carbon fiber reinforced epoxy composite samples were tested to determine their response to one dimensional shock loading with the ultimate goal of developing a micromechanics based numerical model of the dynamic response. The material tested had high fiber content (62-68% by volume) and low porosity. Wave speeds for shocks traveling along the carbon fibers are significantly higher than for those traveling transverse to the fibers or through the bulk epoxy. As a result, the dynamic material response is dependent on the relative shock-fiber orientation; a complication that must be captured in the numerical models. Shocks traveling transverse to the fibers show an inelastic response consistent with the material constituent parts. Shocks traveling along the fiber direction travel faster and exhibit both elastic and plastic characteristics over the stress range tested; up to 15 GPa. Results presented detail the anisotropic material response, which is governed by different mechanisms along each of the two principle directions in the composite. Finally, numerical modeling of this response is described in detail and validated against the experimental data. (C) 2013 AIP Publishing LLC. C1 [Alexander, C. S.; Schumacher, S. C.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Key, C. T.] HI TEST Labs, Appl Technol Grp, Arvonia, VA 23004 USA. RP Alexander, CS (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU Joint DoD/DOE Munitions Technology Development Program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors wish to thank the STAR experimental team consisting of Bill Reinhart, Tom Thornhill, Keith Hodge, John Martinez, and Rocky Palomino for their hard work in fielding these tests; and Patricia Cizan from Hexcel and Gerald Geil and Lee Underwood from AFRL for their assistance in acquiring and manufacturing the test samples. This work was supported by the Joint DoD/DOE Munitions Technology Development Program.; Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 22 TC 0 Z9 0 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223515 DI 10.1063/1.4846116 PG 10 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400024 ER PT J AU Barron, SC Kelly, ST Kirchhoff, J Knepper, R Fisher, K Livi, KJT Dufresne, EM Fezzaa, K Barbee, TW Hufnagel, TC Weihs, TP AF Barron, S. C. Kelly, S. T. Kirchhoff, J. Knepper, R. Fisher, K. Livi, K. J. T. Dufresne, E. M. Fezzaa, K. Barbee, T. W. Hufnagel, T. C. Weihs, T. P. TI Self-propagating reactions in Al/Zr multilayers: Anomalous dependence of reaction velocity on bilayer thickness SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID HETEROGENEOUS FLAME PROPAGATION; SYNTHESIS SHS PROCESS; THIN-FILMS; COMBUSTION SYNTHESIS; HIGH-TEMPERATURE; SURFACE-ENERGY; X-RAY; AL-ZR; EXOTHERMIC REACTIONS; GASLESS COMBUSTION AB High temperature, self-propagating reactions are observed in vapor-deposited Al/Zr multilayered foils of overall atomic ratios 3 Al:1 Zr and 2 Al:1 Zr and nanoscale layer thicknesses; however, the reaction velocities do not exhibit the inverse dependence on bilayer thickness that is expected based on changes in the average diffusion distance. Instead, for bilayer thicknesses of 20-30 nm, the velocity is essentially constant at similar to 7.7 m/s. We explore several possible explanations for this anomalous behavior, including microstructural factors, changes in the phase evolution, and phase transformations in the reactant layers, but find no conclusive explanations. We determine that the phase evolution during self-propagating reactions in foils with a 3 Al:1 Zr stoichiometry is a rapid transformation from Al/Zr multilayers to the equilibrium intermetallic Al3Zr compound with no intermediate crystalline phases. This phase evolution is the same for foils of 90 nm bilayer thicknesses and foils of bilayer thicknesses in the range of 27 nm to 35 nm. Further, for foils with a bilayer thickness of 90 nm and a 3 Al:1 Zr overall chemistry, the propagation front is planar and steady, in contrast to unsteady reaction fronts in foils with 1 Al:1 Zr overall chemistry and similar bilayer thicknesses. (C) 2013 AIP Publishing LLC. C1 [Barron, S. C.; Kelly, S. T.; Kirchhoff, J.; Knepper, R.; Fisher, K.; Hufnagel, T. C.; Weihs, T. P.] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. [Livi, K. J. T.] Johns Hopkins Univ, Integrated Imaging Ctr, Dept Earth & Planetary Sci, Baltimore, MD 21218 USA. [Dufresne, E. M.; Fezzaa, K.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Barbee, T. W.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Condensed Matter & Mat Div, Livermore, CA 94550 USA. RP Weihs, TP (reprint author), Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. EM weihs@jhu.edu RI Weihs, Timothy/A-3313-2010; Hufnagel, Todd/A-3309-2010 OI Hufnagel, Todd/0000-0002-6373-9377 FU U.S. Department of Energy (DOE) [DE-SC002509]; U.S. DOE [DE-AC02-06CH11357]; U.S. Office of Naval Research [N00014-07-1-0740] FX The authors acknowledge financial support from the U.S. Department of Energy (DOE) (Grant No. DE-SC002509) during the in-situ diffraction experiments at the Advanced Photon Source (APS). The APS is an Office of Science User Facility operated for the U.S. DOE Office of Science by Argonne National Laboratory; its use is supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. S. C. B., R. K., and T. P. W. also acknowledge the financial support of the U.S. Office of Naval Research (Grant No. N00014-07-1-0740) during material fabrication and velocity, temperature, and calorimetry studies at JHU. NR 67 TC 5 Z9 5 U1 4 U2 34 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223517 DI 10.1063/1.4840915 PG 10 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400026 ER PT J AU Beringer, DB Roach, WM Clavero, C Reece, CE Lukaszew, RA AF Beringer, D. B. Roach, W. M. Clavero, C. Reece, C. E. Lukaszew, R. A. TI Characterization of two different orientations of epitaxial niobium thin films grown on MgO(001) surfaces SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID HETEROSTRUCTURES; MGO AB Epitaxial Nb thin films deposited onto the same crystalline insulating surface can evolve in very different fashions depending on specific deposition conditions, thereby affecting their microstructure, surface morphology and superconducting properties. Here, we examine and compare the microstructure and ensuing surface morphology from two distinct Nb/MgO series each with its own epitaxial registry-namely Nb(001)/MgO(001) and Nb(110)/MgO(001)-leading to distinct surface anisotropy and we closely examine the dynamical scaling of the surface features during growth. We compare our findings with those in other metal/MgO epitaxial systems and for the first time, general scaling formalism is applied to analyze anisotropic surfaces exhibiting biaxial symmetry. Further, Power Spectral Density is applied to the specific problem of thin film growth and surface evolution to qualify the set of deposition conditions leading to smoother surfaces. We find good correlation between the surface morphology and microstructure of the various Nb films with superconducting properties such as their residual resistance ratio and lower critical field. (C) 2013 AIP Publishing LLC. C1 [Beringer, D. B.; Lukaszew, R. A.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Roach, W. M.; Clavero, C.] Coll William & Mary, Dept Appl Sci, Williamsburg, VA 23187 USA. [Reece, C. E.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Beringer, DB (reprint author), Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. EM dbberinger@email.wm.edu RI Clavero, Cesar/C-4391-2008 OI Clavero, Cesar/0000-0001-6665-3141 FU Defense Threat Reduction Agency [HDTRA1-10-1-0072]; U.S. Department of Energy [DE-AC05-06OR23177] FX This work was funded by the Defense Threat Reduction Agency (HDTRA1-10-1-0072) and the U.S. Department of Energy (DE-AC05-06OR23177). NR 29 TC 2 Z9 2 U1 0 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223502 DI 10.1063/1.4837595 PG 7 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400011 ER PT J AU Brown, JL Alexander, CS Asay, JR Vogler, TJ Ding, JL AF Brown, J. L. Alexander, C. S. Asay, J. R. Vogler, T. J. Ding, J. L. TI Extracting strength from high pressure ramp-release experiments SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ISENTROPIC COMPRESSION EXPERIMENTS; SHOCK-WAVE; MODEL; ALUMINUM; TANTALUM; SOLIDS; INSTABILITY; BEHAVIOR; METALS AB Unloading from a plastically deformed state has long been recognized as a sensitive measure of a material's deviatoric response. In the case of a ramp compression and unload, time resolved particle velocity measurements of a sample/window interface may be used to gain insight into the sample material's strength. Unfortunately, measurements of this type are often highly perturbed by wave interactions associated with impedance mismatches. Additionally, wave attenuation, the finite pressure range over which the material elastically unloads, and rate effects further complicate the analysis. Here, we present a methodology that overcomes these shortcomings to accurately calculate a mean shear stress near peak compression for experiments of this type. A new interpretation of the self-consistent strength analysis is presented and then validated through the analysis of synthetic data sets on tantalum to 250 GPa. The synthetic analyses suggest that the calculated shear stresses are within 3% of the simulated values obtained using both rate-dependent and rate-independent constitutive models. Window effects are addressed by a new technique referred to as the transfer function approach, where numerical simulations are used to define a mapping to transform the experimental measurements to in situ velocities. The transfer function represents a robust methodology to account for complex wave interactions and a dramatic improvement over the incremental impedance matching methods traditionally used. The technique is validated using experiments performed on both lithium fluoride and tantalum ramp compressed to peak stresses of 10 and 15 GPa, respectively. In each case, various windows of different shock impedance are used to ensure consistency within the transfer function analysis. The data are found to be independent of the window used and in good agreement with previous results. (C) 2013 AIP Publishing LLC. C1 [Brown, J. L.; Alexander, C. S.; Asay, J. R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Vogler, T. J.] Sandia Natl Labs, Livermore, CA 94450 USA. [Ding, J. L.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Brown, JL (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We would like to thank R. J. Hickman, A. C. Bowers, N. M. Cofer, J. J. Lynch, and D. M. Pariza for their technical support in designing, fabricating, and conducting the experiments. We also thank T. Ao for the useful discussions and for supplying the LiF samples. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 62 TC 10 Z9 12 U1 5 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223518 DI 10.1063/1.4847535 PG 16 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400027 ER PT J AU Hagmann, MJ Stenger, FS Yarotski, DA AF Hagmann, Mark J. Stenger, Frank S. Yarotski, Dmitry A. TI Linewidth of the harmonics in a microwave frequency comb generated by focusing a mode-locked ultrafast laser on a tunneling junction SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NOISE AB Previous analyses suggest that microwave frequency combs (MFCs) with harmonics having extremely narrow linewidths could be produced by photodetection with a mode-locked ultrafast laser. In the MFC generated by focusing a passively mode-locked ultrafast laser on a tunneling junction, 200 harmonics from 74.254 MHz to 14.85 GHz have reproducible measured linewidths approximating the 1Hz resolution bandwidth (RBW) of the spectrum analyzer. However, in new measurements at a RBW of 0.1 Hz, the linewidths are distributed from 0.12 to 1.17 Hz. Measurements and analysis suggest that, because the laser is not stabilized, the stochastic drift in the pulse repetition rate is the cause for the distribution in measured linewidths. It appears that there are three cases in which the RBW is (1) greater than, (2) less than, or (3) comparable with the intrinsic linewidth. The measured spectra in the third class are stochastic and may show two or more peaks at a single harmonic. (C) 2013 AIP Publishing LLC. C1 [Hagmann, Mark J.] Univ Utah, Dept Elect & Comp Engn, Salt Lake City, UT 84112 USA. [Stenger, Frank S.] Univ Utah, Sch Comp, Salt Lake City, UT 84112 USA. [Yarotski, Dmitry A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Hagmann, MJ (reprint author), Univ Utah, Dept Elect & Comp Engn, Salt Lake City, UT 84112 USA. RI Yarotski, Dmitry/G-4568-2010 FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; Department of Energy [DE-SC0006339] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, U.S. Department of Energy, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, L.L.C., for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. We also acknowledge support from the Department of Energy under Award No. DE-SC0006339. NR 12 TC 3 Z9 3 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223107 DI 10.1063/1.4831952 PG 6 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400007 ER PT J AU Monti, M Sanz, M Oujja, M Rebollar, E Castillejo, M Pedrosa, FJ Bollero, A Camarero, J Cunado, JLF Nemes, NM Mompean, FJ Garcia-Hernandez, M Nie, S McCarty, KF N'Diaye, AT Chen, G Schmid, AK Marco, JF de la Figuera, J AF Monti, Matteo Sanz, Mikel Oujja, Mohamed Rebollar, Esther Castillejo, Marta Pedrosa, Francisco J. Bollero, Alberto Camarero, Julio Cunado, Jose Luis F. Nemes, Norbert M. Mompean, Federico J. Garcia-Hernandez, Mar Nie, Shu McCarty, Kevin F. N'Diaye, Alpha T. Chen, Gong Schmid, Andreas K. Marco, Jose F. de la Figuera, Juan TI Room temperature in-plane (100) magnetic easy axis for Fe3O4/SrTiO3(001):Nb grown by infrared pulsed laser deposition SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ENERGY-ELECTRON MICROSCOPY; MOLECULAR-BEAM EPITAXY; FE3O4 FILMS; TRANSPORT-PROPERTIES; SPIN-POLARIZATION; OXIDE-FILMS; THIN-FILMS; ANISOTROPY; INTERFACE; BEHAVIOR AB We examine the magnetic easy-axis directions of stoichiometric magnetite films grown on SrTiO3: Nb by infrared pulsed-laser deposition. Spin-polarized low-energy electron microscopy reveals that the individual magnetic domains are magnetized along the in-plane <100> film directions. Magneto-optical Kerr effect measurements show that the maxima of the remanence and coercivity are also along in-plane <100> film directions. This easy-axis orientation differs from bulk magnetite and films prepared by other techniques, establishing that the magnetic anisotropy can be tuned by film growth. (C) 2013 AIP Publishing LLC. C1 [Monti, Matteo; Sanz, Mikel; Oujja, Mohamed; Rebollar, Esther; Castillejo, Marta; Marco, Jose F.; de la Figuera, Juan] CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain. [Pedrosa, Francisco J.; Bollero, Alberto; Camarero, Julio; Cunado, Jose Luis F.] Inst Madrileno Estudios Avanzados Nanociencia, IMDEA Nanociencia, E-28049 Madrid, Spain. [Camarero, Julio; Cunado, Jose Luis F.] Univ Autonoma Madrid, Dpto Fis Materia Condensada, E-28049 Madrid, Spain. [Nemes, Norbert M.] Univ Complutense Madrid, Dpto Fis Aplicada 3, E-28040 Madrid, Spain. [Mompean, Federico J.; Garcia-Hernandez, Mar] CSIC, Inst Ciencia Mat Madrid, E-28049 Madrid, Spain. [Nie, Shu; McCarty, Kevin F.] Sandia Natl Labs, Livermore, CA 94550 USA. [N'Diaye, Alpha T.; Chen, Gong; Schmid, Andreas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP de la Figuera, J (reprint author), CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain. EM juan.delafiguera@iqfr.csic.es RI Castillejo, Marta/D-7448-2014; Oujja, Mohamed/F-8573-2013; Camarero, Julio/C-4375-2014; Garcia-Hernandez, Mar/J-9520-2014; Mompean, Federico/B-8713-2011; de la Figuera, Juan/E-7046-2010; Marco, Jose/N-3176-2014; Rebollar, Esther/N-4065-2014; Sanz, Mikel/M-5349-2014; Chen, Gong/H-3074-2015; Foundry, Molecular/G-9968-2014 OI Oujja, Mohamed/0000-0003-3757-4043; Monti, Matteo/0000-0003-3595-4472; Castillejo, Marta/0000-0002-5870-4380; Garcia-Hernandez, Mar/0000-0002-5987-0647; de la Figuera, Juan/0000-0002-7014-4777; Marco, Jose/0000-0002-5147-1449; Rebollar, Esther/0000-0002-1144-7102; Sanz, Mikel/0000-0001-6160-3583; FU MICINN [CTQ2010-15680, MAT2009-14578-C03-01, MAT2011-27470-C02- 02]; MINECO [MAT2012-38045-C04-01, MAT2011-25598]; EU-FP7 NANOPYME [310516]; Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. Department of Energy [DE-AC04-94AL85000]; National Center for Electron Microscopy, Lawrence Berkeley National Laboratory; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02- 05CH11231]; Alexander von Humboldt Foundation and a contract through the MICINN FPI Programme [S2009/Mat-1629] FX Authors acknowledge fruitful discussions with Professor M. Ziese. This research was supported by Projects CTQ2010-15680, MAT2009-14578-C03-01 (MICINN), MAT2012-38045-C04-01 (MINECO), MAT2011-27470-C02- 02 (MICINN), MAT2011-25598 (MINECO), the EU-FP7 NANOPYME Project (No. 310516) and by the Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. Department of Energy under Contract No. DE-AC04-94AL85000 (Sandia National Laboratories). Experiments performed at the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, were supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02- 05CH11231. E. R., M. O., M. S., A. T. N., and M. M. gratefully thank financial support from the Ramon y Cajal Programme (MINECO), a CSIC contract, a Geomateriales (CAM, S2009/Mat-1629) contract, a Feodor Lynen Postdoctoral Fellowship from the Alexander von Humboldt Foundation and a contract through the MICINN FPI Programme, respectively. We are grateful to Professor T. Ezquerra (IEM, CSIC) for the use of the AFM system and M. Juanco (ICA, CSIC) for XRD measurements. NR 53 TC 14 Z9 14 U1 1 U2 48 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223902 DI 10.1063/1.4837656 PG 5 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400047 ER PT J AU Saha, B Ramanathan, M Ren, C Appusamy, K McCarter, MK Guruswamy, S Cook, R Miller, DJ AF Saha, B. Ramanathan, M. Ren, C. Appusamy, K. McCarter, M. K. Guruswamy, S. Cook, R. Miller, D. J. TI Acoustic emission and changes in dislocation structure and magnetostriction accompanying plastic deformation of [126]-oriented Fe-Ga alloy single crystals SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID BANDS; ZN; MG AB Controlled compressive deformation of [126]-oriented Fe-20 at.% Ga alloy single crystal along [126] direction results in large and asymmetric changes in the magnetostriction of the sample. This is in contrast to a much smaller change in magnetostriction observed in [100]-oriented single crystal deformed along [001] direction. Deformation of [126]-oriented crystal along [126] direction involved operation of only one of the slip systems. This is confirmed by TEM examination that showed only a single set of dislocation array which introduces asymmetric strain modulation in the crystal. The [100]-oriented crystal deformation involved operation of multiple slip systems and formation of several sets of dislocation arrays which introduce more symmetric strain modulations. The results suggest that the nature of strain modulation introduced by the dislocation arrays has a strong influence on the magnetostrictive behavior. Several sudden load drops accompanied by acoustic emissions and formation of slip bands were observed during [126]-oriented crystal deformation, while no such load drops or audible acoustic emissions were seen during the [001]-oriented crystal deformation. (C) 2013 AIP Publishing LLC. C1 [Saha, B.; Ramanathan, M.; Ren, C.; Appusamy, K.; McCarter, M. K.; Guruswamy, S.] Univ Utah, Salt Lake City, UT 84112 USA. [Cook, R.; Miller, D. J.] Argonne Natl Lab, Elect Microscopy Ctr, Argonne, IL 60439 USA. RP Saha, B (reprint author), Univ Utah, Salt Lake City, UT 84112 USA. FU National Science Foundation under NSF DMR [DMR-0854166]; NSF-MRSEC at the University of Utah [DMR-1121252]; University of Utah; Electron Microscopy Center at Argonne National Laboratory, a U.S. Department of Energy, Office of Science Laboratory by University of Chicago, Argonne, LLC [DE-AC02_06CH11357] FX The authors are grateful for the financial support of this work by the National Science Foundation under NSF DMR Award No. DMR-0854166 and under NSF-MRSEC at the University of Utah (Grant No. DMR-1121252). Support of this work by the University of Utah was also gratefully acknowledged. The electron microscopy was accomplished at the Electron Microscopy Center at Argonne National Laboratory, a U.S. Department of Energy, Office of Science Laboratory operated under Contract No DE-AC02_06CH11357 by University of Chicago, Argonne, LLC. NR 17 TC 1 Z9 1 U1 2 U2 16 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223910 DI 10.1063/1.4846815 PG 6 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400055 ER PT J AU Smith, RF Eggert, JH Swift, DC Wang, J Duffy, TS Braun, DG Rudd, RE Reisman, DB Davis, JP Knudson, MD Collins, GW AF Smith, R. F. Eggert, J. H. Swift, D. C. Wang, J. Duffy, T. S. Braun, D. G. Rudd, R. E. Reisman, D. B. Davis, J-P Knudson, M. D. Collins, G. W. TI Time-dependence of the alpha to epsilon phase transformation in iron SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ISENTROPIC COMPRESSION EXPERIMENTS; SHOCK-WAVE; HIGH-PRESSURE; TRANSITIONS; DYNAMICS; STATE; EQUATIONS; CRYSTALS; KINETICS; STRESS AB Iron was ramp-compressed over timescales of 3 <= t(ns) <= 300 to study the time-dependence of the alpha ->epsilon (bcc -> hcp) phase transformation. Onset stresses (sigma(alpha ->epsilon)) for the transformation similar to 14.8-38.4 GPa were determined through laser and magnetic ramp-compression techniques where the transition strain-rate was varied between 10(6) <= (mu) over dot(alpha ->epsilon)(s(-1)) <= 5 x 10(8). We find sigma(alpha ->epsilon) = 10.8+0.55 ln ((mu) over dot(alpha ->epsilon)) for (mu) over dot(alpha ->epsilon) < 10(6)/s and sigma(alpha ->epsilon) - 1.15 ((mu) over dot(alpha ->epsilon))(0.18) for (mu) over dot(alpha ->epsilon) > 10(6)/s. This (mu) over dot response is quite similar to recent results on incipient plasticity in Fe [Smith et al., J. Appl. Phys. 110, 123515 (2011)] suggesting that under high rate ramp compression the alpha ->epsilon phase transition and plastic deformation occur through similar mechanisms, e. g., the rate limiting step for (mu) over dot > 10(6)/s is due to phonon scattering from defects moving to relieve strain. We show that over-pressurization of equilibrium phase boundaries is a common feature exhibited under high strain-rate compression of many materials encompassing many orders of magnitude of strain-rate. (C) 2013 AIP Publishing LLC. C1 [Smith, R. F.; Eggert, J. H.; Swift, D. C.; Braun, D. G.; Rudd, R. E.; Reisman, D. B.; Collins, G. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Wang, J.; Duffy, T. S.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. [Davis, J-P; Knudson, M. D.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Smith, RF (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94550 USA. RI Wang, Jue/I-4705-2014; Duffy, Thomas/C-9140-2017 OI Wang, Jue/0000-0001-9206-4367; Duffy, Thomas/0000-0002-5357-1259 FU U.S. Dept. of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; NNSA/DOE through the National Laser Users Facility Program [DE-NA0000856, DE-FG52-09NA29037] FX This work was performed under the auspices of the U.S. Dept. of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The research was supported by NNSA/DOE through the National Laser Users Facility Program under contracts DE-NA0000856 and DE-FG52-09NA29037. NR 60 TC 12 Z9 13 U1 5 U2 37 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223507 DI 10.1063/1.4839655 PG 11 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400016 ER PT J AU Taylor, CN Dadras, J Luitjohan, KE Allain, JP Krstic, PS Skinner, CH AF Taylor, C. N. Dadras, J. Luitjohan, K. E. Allain, J. P. Krstic, P. S. Skinner, C. H. TI The role of oxygen in the uptake of deuterium in lithiated graphite SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID BREAKDOWN; MICROPLASMAS; DISCHARGES AB We investigate the mechanism of deuterium retention by lithiated graphite and its relationship to the oxygen concentration through surface sensitive experiments and atomistic simulations. Deposition of lithium on graphite yielded 5%-8% oxygen surface concentration and when subsequently irradiated with D ions at energies between 500 and 1000 eV/amu and fluences over 10(16) cm(-2) the oxygen concentration rose to between 25% and 40%. These enhanced oxygen levels were reached in a few seconds compared to about 300 h when the lithiated graphite was allowed to adsorb oxygen from the ambient environment under equilibrium conditions. Irradiating graphite without lithium deposition, however, resulted in complete removal of oxygen to levels below the detection limit of XPS (e. g., <1%). These findings confirm the predictions of atomistic simulations, which had concluded that oxygen was the primary component for the enhanced hydrogen retention chemistry on the lithiated graphite surface. (C) 2013 AIP Publishing LLC. C1 [Taylor, C. N.; Luitjohan, K. E.; Allain, J. P.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA. [Dadras, J.; Krstic, P. S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37998 USA. [Allain, J. P.] Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Krstic, P. S.] Univ Tennessee, Joint Inst Computat Sci, Knoxville, TN 37998 USA. [Krstic, P. S.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Skinner, C. H.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Taylor, CN (reprint author), Idaho Natl Lab, Fus Safety Program, Idaho Falls, ID 83415 USA. EM chase.taylor@inl.gov OI Allain, Jean Paul/0000-0003-1348-262X NR 23 TC 4 Z9 4 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 14 PY 2013 VL 114 IS 22 AR 223301 DI 10.1063/1.4841115 PG 16 WC Physics, Applied SC Physics GA 281HI UT WOS:000329090400009 ER PT J AU Hanson, DE Barber, JL Subramanian, G AF Hanson, David E. Barber, John L. Subramanian, Gopinath TI The entropy of the rotational conformations of (poly)isoprene molecules and its relationship to rubber elasticity and temperature increase for moderate tensile or compressive strains SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID POLYMER NETWORKS; STRESSED RUBBER; NATURAL-RUBBER; RETRACTION; MODEL AB Molecular networks comprised of crosslinked cis-1,4 polyisoprene, often referred to as "natural rubber," are one of the most common systems for the study of rubber elasticity. Under moderate tensile or compressive strain, network chains begin to assume straighter paths, as local molecular kinks are removed. Isoprene units along the chain backbone are mechanically forced from their equilibrium distributions of 18 possible rotational states into a smaller subset of states, restricted to more linear conformations with the greatest end-to-end distances. There are two consequences to this change: both the configurational entropy and average internal energy decrease. We find that the change in entropy, and resulting change in free energy, gives rise to an elastic force. We derive an expression for a chain extension force constant that we have incorporated in an explicit, three-dimensional meso-scale network simulation code. Using this force model, our simulations predict a macroscopic stress-strain relationship that closely matches published experimental values. We also predict a slight increase in temperature resulting from the change in average internal energy in the affected isoprene units that is consistent with experiments. (C) 2013 AIP Publishing LLC. C1 [Hanson, David E.; Barber, John L.; Subramanian, Gopinath] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Hanson, DE (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; DOE-DOD Joint Munitions Program FX This work was performed under the auspices of Los Alamos National Laboratory, which is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. We wish to gratefully acknowledge the support of the DOE-DOD Joint Munitions Program. We also thank Dr. Paul Welch for helpful comments and suggestions. NR 33 TC 1 Z9 1 U1 2 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD DEC 14 PY 2013 VL 139 IS 22 DI 10.1063/1.4840096 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 276DT UT WOS:000328729000046 PM 24329092 ER PT J AU Lei, HP Wang, CZ Yao, YX Wang, YG Hupalo, M McDougall, D Tringides, M Ho, KM AF Lei, Huaping Wang, Caizhuang Yao, Yongxin Wang, Yangang Hupalo, Myron McDougall, Dan Tringides, Michael Ho, Kaiming TI Strain effect on the adsorption, diffusion, and molecular dissociation of hydrogen on Mg (0001) surface SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; METAL-SURFACES; AB-INITIO; MG(0001) SURFACE; SADDLE-POINTS; THIN-FILMS; STORAGE; MAGNESIUM; H-2 AB The adsorption, diffusion, and molecular dissociation of hydrogen on the biaxially strained Mg (0001) surface have been systematically investigated by the first principle calculations based on density functional theory. When the strain changes from the compressive to tensile state, the adsorption energy of H atom linearly increases while its diffusion barrier linearly decreases oppositely. The dissociation barrier of H-2 molecule linearly reduces in the tensile strain region. Through the chemical bonding analysis including the charge density difference, the projected density of states and the Mulliken population, the mechanism of the strain effect on the adsorption of H atom and the dissociation of H-2 molecule has been elucidated by an s-p charge transfer model. With the reduction of the orbital overlap between the surface Mg atoms upon the lattice expansion, the charge transfers from p to s states of Mg atoms, which enhances the hybridization of H s and Mg s orbitals. Therefore, the bonding interaction of H with Mg surface is strengthened and then the atomic diffusion and molecular dissociation barriers of hydrogen decrease accordingly. Our works will be helpful to understand and to estimate the influence of the lattice deformation on the performance of Mg-containing hydrogen storage materials. (C) 2013 AIP Publishing LLC. C1 [Lei, Huaping; Wang, Caizhuang; Yao, Yongxin; Wang, Yangang; Hupalo, Myron; McDougall, Dan; Tringides, Michael; Ho, Kaiming] US DOE, Ames Lab, Ames, IA 50011 USA. [Wang, Yangang] Chinese Acad Sci, Supercomp Ctr Comp Network Informat Ctr, Beijing 100190, Peoples R China. [McDougall, Dan; Tringides, Michael; Ho, Kaiming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Lei, HP (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. FU U. S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358] FX This work was supported by the U. S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering under the Contract No. DE-AC02-07CH11358 including the computer time support from the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. NR 48 TC 2 Z9 2 U1 4 U2 35 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD DEC 14 PY 2013 VL 139 IS 22 DI 10.1063/1.4839595 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 276DT UT WOS:000328729000032 ER PT J AU Sassi, P Perticaroli, S Comez, L Giugliarelli, A Paolantoni, M Fioretto, D Morresi, A AF Sassi, Paola Perticaroli, Stefania Comez, Lucia Giugliarelli, Alessandra Paolantoni, Marco Fioretto, Daniele Morresi, Assunta TI Volume properties and spectroscopy: A terahertz Raman investigation of hen egg white lysozyme SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID INELASTIC NEUTRON-SCATTERING; DEPOLARIZED LIGHT-SCATTERING; GLOBULAR-PROTEINS; THERMODYNAMIC INVESTIGATIONS; THERMAL-EXPANSION; TEMPERATURE; DYNAMICS; WATER; HYDRATION; MOTIONS AB The low frequency depolarized Raman spectra of 100 mg/ml aqueous solutions of hen egg white lysozyme (HEWL) have been collected in the 25-85 degrees C range. Short and long exposures to high temperatures have been used to modulate the competition between the thermally induced reversible and irreversible denaturation processes. A peculiar temperature evolution of spectra is evidenced under prolonged exposure of the protein solution at temperatures higher than 65 degrees C. This result is connected to the self-assembling of polypeptide chains and testifies the sensitivity of the technique to the properties of both protein molecule and its surrounding. Solvent free spectra have been obtained after subtraction of elastic and solvent components and assigned to a genuine vibrational contribution of hydrated HEWL. A straight similarity is observed between the solvent-free THz Raman feature and the vibrational density of states as obtained by molecular dynamics simulations; according to this, we verify the relation between this spectroscopic observable and the effective protein volume, and distinguish the properties of this latter respect to those of the hydration shell in the pre-melting region. (C) 2013 AIP Publishing LLC. C1 [Sassi, Paola; Giugliarelli, Alessandra; Paolantoni, Marco; Morresi, Assunta] Univ Perugia, Dipartimento Chim, I-06123 Perugia, Italy. [Perticaroli, Stefania] Oak Ridge Natl Lab, Div Chem & Mat Sci, Oak Ridge, TN 37831 USA. [Perticaroli, Stefania] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Comez, Lucia] Univ Perugia, Dipartimento Fis, IOM CNR, I-06123 Perugia, Italy. [Comez, Lucia; Fioretto, Daniele] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Fioretto, Daniele] Univ Perugia, CEMIN, I-06123 Perugia, Italy. RP Sassi, P (reprint author), Univ Perugia, Dipartimento Chim, Via Elce Sotto 8, I-06123 Perugia, Italy. EM paola.sassi@unipg.it RI Sassi, Paola/F-1141-2014; Paolantoni, Marco /G-1646-2014; Morresi, Assunta/M-7359-2014 OI Sassi, Paola/0000-0002-4920-2784; Paolantoni, Marco /0000-0002-6266-3497; Morresi, Assunta/0000-0002-0481-6424 NR 40 TC 1 Z9 1 U1 5 U2 47 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD DEC 14 PY 2013 VL 139 IS 22 DI 10.1063/1.4838355 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 276DT UT WOS:000328729000047 PM 24329093 ER PT J AU Abdallah, J Colgan, J Rohringer, N AF Abdallah, J., Jr. Colgan, J. Rohringer, N. TI Time-dependent calculations of electron energy distribution functions for neon gas in the presence of intense XFEL radiation SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article ID X-RAY LASER AB Boltzmann electron kinetic simulations are performed to study the time development of the electron energy distribution function (EEDF) in plasma resulting from neon gas subject to a 40 fs x-ray free electron laser radiation source. The simulations are performed without any assumptions of electron temperature. The distributions are calculated as a function of time through 40 fs using Boltzmann kinetics, including the appropriate processes that alter state populations and electron energy. The calculations are also extended into the picosecond regime, after the laser pulse, to track the thermalization of free electrons. Results are presented that predict the evolution of the charge-state distribution, effective temperature, the photon spectrum, as well as the EEDF. C1 [Abdallah, J., Jr.; Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Rohringer, N.] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. [Rohringer, N.] Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany. RP Abdallah, J (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM abd@lanl.gov RI Rohringer, Nina/N-3238-2014; OI Rohringer, Nina/0000-0001-7905-3567; Colgan, James/0000-0003-1045-3858 FU National Nuclear Security Administration of the US Department of Energy [DE-AC5206NA25396] FX The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the US Department of Energy under contract no. DE-AC5206NA25396. NR 30 TC 3 Z9 3 U1 2 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD DEC 14 PY 2013 VL 46 IS 23 AR 235004 DI 10.1088/0953-4075/46/23/235004 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 263NB UT WOS:000327814200005 ER PT J AU da Rocha, UN Plugge, CM George, I van Elsas, JD van Overbeek, LS AF da Rocha, Ulisses Nunes Plugge, Caroline M. George, Isabelle van Elsas, Jan Dirk van Overbeek, Leonard Simon TI The Rhizosphere Selects for Particular Groups of Acidobacteria and Verrucomicrobia SO PLOS ONE LA English DT Article ID 16S RIBOSOMAL-RNA; BACTERIAL COMMUNITY STRUCTURE; HITHERTO-UNCULTURED BACTERIA; ALLIUM-PORRUM RHIZOSPHERE; SOIL MICROBIAL COMMUNITY; PHYLUM ACIDOBACTERIA; GEN. NOV.; SUBDIVISION 1; FOREST SOILS; DIVERSITY AB There is a lack in our current understanding on the putative interactions of species of the phyla of Acidobacteria and Verrucomicrobia with plants. Moreover, progress in this area is seriously hampered by the recalcitrance of members of these phyla to grow as pure cultures. The purpose of this study was to investigate whether particular members of Acidobacteria and Verrucomicrobia are avid colonizers of the rhizosphere. Based on previous work, rhizosphere competence was demonstrated for the Verrucomicrobia subdivision 1 groups of Luteolibacter and Candidatus genus Rhizospheria and it was hypothesized that the rhizosphere is a common habitat for Acidobacteria subdivision 8 (class Holophagae). We assessed the population densities of Bacteria, Verrucomicrobia subdivision 1 groups Luteolibacter and Candidatus genus Rhizospheria and Acidobacteria subdivisions 1, 3, 4, 6 and Holophagae in bulk soil and in the rhizospheres of grass, potato and leek in the same field at different points in time using real-time quantitative PCR. Primers of all seven verrucomicrobial, acidobacterial and holophagal PCR systems were based on 16S rRNA gene sequences of cultivable representatives of the different groups. Luteolibacter, Candidatus genus Rhizospheria, subdivision 6 acidobacteria and Holophaga showed preferences for one or more rhizospheres. In particular, the Holophaga 16S rRNA gene number were more abundant in the leek rhizosphere than in bulk soil and the rhizospheres of grass and potato. Attraction to, and colonization of, leek roots by Holophagae strain CHC25 was further shown in an experimental microcosm set-up. In the light of this remarkable capacity, we propose to coin strain CHC25 Candidatus Porrumbacterium oxyphilus (class Holophagae, Phylum Acidobacteria), the first cultured representative with rhizosphere competence. C1 [da Rocha, Ulisses Nunes; van Overbeek, Leonard Simon] Univ Wageningen & Res Ctr, Wageningen, Netherlands. [da Rocha, Ulisses Nunes] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Environm Biotechnol, Berkeley, CA 94720 USA. [Plugge, Caroline M.] Univ Wageningen & Res Ctr, Microbiol Lab, Wageningen, Netherlands. [George, Isabelle] Univ Libre Brussels, Lab Ecol Syst Aquat, Brussels, Belgium. [van Elsas, Jan Dirk] Univ Groningen, Dept Microbial Ecol, Ctr Ecol & Evolutionary Studies, Groningen, Netherlands. RP van Overbeek, LS (reprint author), Univ Wageningen & Res Ctr, Wageningen, Netherlands. EM leo.vanoverbeek@wur.nl FU Netherlands Genomic Initiative(NGI); Dutch Ministry of Agriculture, Nature and Food Quality [KB4] FX This research was conducted within the Netherlands Genomic Initiative(NGI)-financed program of 'Ecogenomics', and the Research Program on Sustainable Agriculture (KB4), financed by the Dutch Ministry of Agriculture, Nature and Food Quality. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 55 TC 13 Z9 13 U1 6 U2 41 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 13 PY 2013 VL 8 IS 12 AR UNSP e82443 DI 10.1371/journal.pone.0082443 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 276FP UT WOS:000328734200043 ER PT J AU Johnson, MT Childers, AS De Carlo, F Xiao, X Faber, KT AF Johnson, M. T. Childers, A. S. De Carlo, F. Xiao, X. Faber, K. T. TI Wood-derived copper-graphite composites produced via additive-assisted electrodeposition SO COMPOSITES SCIENCE AND TECHNOLOGY LA English DT Article DE Electroplating; Functional composites; Porosity/Voids; Scanning electron microscopy (SEM) ID SILICON CARBIDE COMPOSITES; X-RAY MICROTOMOGRAPHY; MECHANICAL-PROPERTIES; THERMAL-CONDUCTIVITY; WETTABILITY; CERAMICS; ALLOY AB An additive-assisted copper electroplating technique designed for infiltrating high-aspect-ratio pores was adapted to work with three-dimensional wood-derived graphitic scaffolds with aspect ratios ranging from 15 to 300. The poor wettability of the carbon/copper system necessitates the development of alternative infiltration techniques to produce composite structures from highly porous precursors such as wood-derived graphite. By incorporating electrolyte additives, copper infiltration was demonstrated into red oak-derived graphite scaffolds, producing a composite with a biologically-derived microstructure. Copper infiltration was studied as a function of electrolyte chemistry and deposition time in two dimensions using electron microscopy techniques and in three dimensions using X-ray computed tomography. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Johnson, M. T.; Childers, A. S.; Faber, K. T.] Northwestern Univ, Robert R McCormick Sch Engn & Appl Sci, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [De Carlo, F.; Xiao, X.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Faber, KT (reprint author), Northwestern Univ, Robert R McCormick Sch Engn & Appl Sci, Dept Mat Sci & Engn, 2220 N Campus Dr, Evanston, IL 60208 USA. EM k-faber@northwestern.edu RI Faber, Katherine/B-6741-2009 FU National Science Foundation [DMR-0710630]; NSF-NSEC; NSF-MRSEC; Keck Foundation; State of Illinois, and Northwestern University; MRSEC program of the National Science Foundation, at the Materials Research Center of Northwestern University [DMR-0520513]; United States Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the National Science Foundation, DMR-0710630. SEM work was performed in the EPIC facility of the NUANCE Center at Northwestern University, supported by NSF-NSEC, NSF-MRSEC, The Keck Foundation, The State of Illinois, and Northwestern University. Portions of this work made use of the Optical Microscopy and Metallography Facility, supported by the MRSEC program of the National Science Foundation, DMR-0520513, at the Materials Research Center of Northwestern University. XCT work made use of the Advanced Photon Source at Argonne National Laboratory. Use of the Advanced Photon Source is supported by the United States Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 27 TC 2 Z9 2 U1 2 U2 35 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0266-3538 EI 1879-1050 J9 COMPOS SCI TECHNOL JI Compos. Sci. Technol. PD DEC 13 PY 2013 VL 89 BP 61 EP 68 DI 10.1016/j.compscitech.2013.09.010 PG 8 WC Materials Science, Composites SC Materials Science GA 275YO UT WOS:000328715500009 ER PT J AU Pan, LH Li, J Tai, YY Graf, MJ Zhu, JX Ting, CS AF Pan, Lihua Li, Jian Tai, Yuan-Yen Graf, Matthias J. Zhu, Jian-Xin Ting, C. S. TI Evolution of the Fermi surface topology in doped 122 iron pnictides SO PHYSICAL REVIEW B LA English DT Article ID NODELESS SUPERCONDUCTING GAPS; SPIN-DENSITY-WAVE; BA0.6K0.4FE2AS2; COEXISTENCE; PHASE AB Based on the minimum two-orbital model and the phase diagram recently proposed by Tai et al. [Europhys. Lett. 103, 67001 (2013)] for both electron-and hole-doped 122 iron-based superconducting compounds, we use the Bogoliubov-de-Gennes equations to perform a comprehensive investigation of the evolution of the Fermi surface (FS) topology in the presence of the collinear spin-density-wave (SDW) order as the doping is changed. In the parent compound, the ground state is the SDW order, where the FS is not completely gapped, and two types of Dirac cones, one electron-doped and the other hole-doped emerge in the magnetic Brillouin zone. Our findings are qualitatively consistent with recent angle-resolved photoemission spectroscopy and magnetoresistivity measurements. We also examine the FS evolution of both electron-and hole-doped cases and compare them with measurements, as well as with those obtained by other model Hamiltonians. C1 [Pan, Lihua; Li, Jian; Tai, Yuan-Yen; Ting, C. S.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Pan, Lihua; Li, Jian; Tai, Yuan-Yen; Ting, C. S.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Pan, Lihua] Yangzhou Univ, Sch Phys Sci & Technol, Yangzhou 225002, Peoples R China. [Graf, Matthias J.; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Pan, LH (reprint author), Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. OI Zhu, Jianxin/0000-0001-7991-3918 FU Texas Center for Superconductivity at the University of Houston; Robert A. Welch Foundation [E-1146]; US DOE [DE-AC52-06NA25396]; Office of Basic Energy Sciences (BES), Division of Materials Sciences Engineering; Center for Integrated Nanotechnologies, a BES user facility; NSF [PHYS-1066293] FX This work was supported in part by the Texas Center for Superconductivity at the University of Houston and by the Robert A. Welch Foundation under Grant No. E-1146 (L. P., J.L., Y.-Y.T., and C. S. T.). Work at Los Alamos was performed under the auspices of the US DOE Contract No. DE-AC52-06NA25396 through the LDRD program (Y.-Y.T.), the Office of Basic Energy Sciences (BES), Division of Materials Sciences & Engineering (M.J.G.), and the Center for Integrated Nanotechnologies, a BES user facility (J.-X.Z.). M.J.G. also thanks the Aspen Center for Physics for its hospitality, which is supported by the NSF under Grant No. PHYS-1066293. NR 54 TC 6 Z9 6 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 13 PY 2013 VL 88 IS 21 AR 214510 DI 10.1103/PhysRevB.88.214510 PG 7 WC Physics, Condensed Matter SC Physics GA 275MU UT WOS:000328682100002 ER PT J AU Shulenburger, L Mattsson, TR AF Shulenburger, Luke Mattsson, Thomas R. TI Quantum Monte Carlo applied to solids SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; AUGMENTED-WAVE METHOD; ELECTRON-GAS; NONLOCAL PSEUDOPOTENTIALS; GROUND-STATE; SYSTEMS AB We apply diffusion quantum Monte Carlo to a broad set of solids, benchmarking the method by comparing bulk structural properties (equilibrium volume and bulk modulus) to experiment and density functional theory (DFT) based theories. The test set includes materials with many different types of binding including ionic, metallic, covalent, and van der Waals. We show that, on average, the accuracy is comparable to or better than that of DFT when using the new generation of functionals, including one hybrid functional and two dispersion corrected functionals. The excellent performance of quantum Monte Carlo on solids is promising for its application to heterogeneous systems and high-pressure/high-density conditions. Important to the results here is the application of a consistent procedure with regards to the several approximations that are made, such as finite-size corrections and pseudopotential approximations. This test set allows for any improvements in these methods to be judged in a systematic way. C1 [Shulenburger, Luke; Mattsson, Thomas R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Shulenburger, L (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM lshulen@sandia.gov; trmatts@sandia.gov FU NNSA Science Campaigns; Predictive Theory and Modeling for Materials and Chemical Science program by the Basic Energy Science (BES), Department of Energy (DOE); U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We thank Jeongnim Kim, Mike Desjarlais, Miguel Morales, and Paul Kent for stimulating discussions and the Cielo Capability Computing Campaign for computer time. The work was supported by the NNSA Science Campaigns and L. S. was supported through the Predictive Theory and Modeling for Materials and Chemical Science program by the Basic Energy Science (BES), Department of Energy (DOE). Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 50 TC 38 Z9 38 U1 0 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 13 PY 2013 VL 88 IS 24 AR 245117 DI 10.1103/PhysRevB.88.245117 PG 8 WC Physics, Condensed Matter SC Physics GA 275NF UT WOS:000328683400002 ER PT J AU Berger, EL Sullivan, Z Zhang, H AF Berger, Edmond L. Sullivan, Zack Zhang, Hao TI LHC and Tevatron constraints on a W ' model interpretation of the top quark forward-backward asymmetry SO PHYSICAL REVIEW D LA English DT Article ID T(T)OVER-BAR; SEARCH AB Aspects of a flavor-changing W' model with right-handed couplings are addressed in this paper in light of Tevatron and LHC data. Our fit to the Tevatron top-quark forward-backward asymmetry and the t (t) over bar inclusive cross section includes higher-order loop effects in the effective interaction. The higher-order corrections change the best-fit value of the W' effective coupling strength as a function of the W' mass. The consistency of the model is checked against the shape of the t (t) over bar invariant mass distribution. We use these updated W' parameters to compute the expected contributions from W't associated production and, for the first time, W'W' pair production at the LHC. We do a full Monte Carlo simulation of the t (t) over barX final state, including interference between the tW'-induced t (t) over barj process and the standard model t (t) over barj process. Interference effects are shown to be quantitatively important, particularly when the W' mass is large. The jet-multiplicity distribution in t (t) over bar jet production at 8 TeV constrains the W' model severely. C1 [Berger, Edmond L.; Zhang, Hao] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Sullivan, Zack; Zhang, Hao] IIT, Dept Phys, Chicago, IL 60616 USA. RP Berger, EL (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. EM berger@anl.gov; Zack.Sullivan@IIT.edu; zhanghao@physics.ucsb.edu RI ZHANG, Hao/G-6430-2015 FU U.S. DOE [DE-AC0206CH11357]; DOE [DE-SC0008347]; National Science Foundation [PHYS-1066293]; Aspen Center for Physics FX The work of E.L.B. and H.Z. at Argonne is supported in part by the U.S. DOE under Contract No. DE-AC0206CH11357. Z.S. and H.Z. are supported at IIT by the DOE under Contract No. DE-SC0008347. Part of this work was done while E.L.B. was visiting the Aspen Center for Physics and was supported there in part by the National Science Foundation under Contract No. PHYS-1066293. E.L.B. is pleased to recognize this support and the hospitality of the Aspen Center for Physics. NR 55 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD DEC 13 PY 2013 VL 88 IS 11 AR 114026 DI 10.1103/PhysRevD.88.114026 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 275QN UT WOS:000328692300002 ER PT J AU Pelton, M Chakraborty, D Malachosky, E Guyot-Sionnest, P Sader, JE AF Pelton, Matthew Chakraborty, Debadi Malachosky, Edward Guyot-Sionnest, Philippe Sader, John E. TI Viscoelastic Flows in Simple Liquids Generated by Vibrating Nanostructures SO PHYSICAL REVIEW LETTERS LA English DT Article ID ATOMIC-FORCE MICROSCOPE; METAL NANOPARTICLES; ACOUSTIC VIBRATIONS; VISCOUS FLUIDS; GOLD NANOPARTICLES; FREQUENCY-RESPONSE; DYNAMICS; WATER; BIPYRAMIDS; SCATTERING AB Newtonian fluid mechanics, in which the shear stress is proportional to the strain rate, is synonymous with the flow of simple liquids such as water. We report the measurement and theoretical verification of non-Newtonian, viscoelastic flow phenomena produced by the high-frequency (20 GHz) vibration of gold nanoparticles immersed in water-glycerol mixtures. The observed viscoelasticity is not due to molecular confinement, but is a bulk continuum effect arising from the short time scale of vibration. This represents the first direct mechanical measurement of the intrinsic viscoelastic properties of simple bulk liquids, and opens a new paradigm for understanding extremely high frequency fluid mechanics, nanoscale sensing technologies, and biophysical processes. C1 [Pelton, Matthew] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Chakraborty, Debadi; Sader, John E.] Univ Melbourne, Dept Math & Stat, Melbourne, Vic 3010, Australia. [Malachosky, Edward; Guyot-Sionnest, Philippe] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Sader, John E.] CALTECH, Kavli Nanosci Inst, Pasadena, CA 91125 USA. [Sader, John E.] CALTECH, Dept Phys, Pasadena, CA 91125 USA. RP Sader, JE (reprint author), Univ Melbourne, Dept Math & Stat, Melbourne, Vic 3010, Australia. EM jsader@unimelb.edu.au RI Pelton, Matthew/H-7482-2013 OI Pelton, Matthew/0000-0002-6370-8765 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; NSF [CHE1111799]; Australian Research Council; Caltech's Kavli Nanoscience Institute; Center for Nanoscale Materials FX We thank D. Gosztola for valuable assistance with the transient-absorption measurements. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. E. M. was supported by NSF Grant No. CHE1111799. This research was supported by the Australian Research Council Grants Scheme and by Caltech's Kavli Nanoscience Institute. NR 29 TC 23 Z9 24 U1 9 U2 55 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 13 PY 2013 VL 111 IS 24 AR 244502 DI 10.1103/PhysRevLett.111.244502 PG 5 WC Physics, Multidisciplinary SC Physics GA 275TQ UT WOS:000328700900002 PM 24483667 ER PT J AU Homes, CC Tu, JJ Li, J Gu, GD Akrap, A AF Homes, C. C. Tu, J. J. Li, J. Gu, G. D. Akrap, A. TI Optical conductivity of nodal metals SO SCIENTIFIC REPORTS LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; FERMI-LIQUID; PSEUDOGAP; ELECTRODYNAMICS; STATE; PHASE AB Fermi liquid theory is remarkably successful in describing the transport and optical properties of metals; at frequencies higher than the scattering rate, the optical conductivity adopts the well-known power law behavior sigma(1)(omega) proportional to omega(-2). We have observed an unusual non-Fermi liquid response sigma(1)(omega) proportional to omega(-1 +/- 0.2) in the ground states of several cuprate and iron-based materials which undergo electronic or magnetic phase transitions resulting in dramatically reduced or nodal Fermi surfaces. The identification of an inverse (or fractional) power-law behavior in the residual optical conductivity now permits the removal of this contribution, revealing the direct transitions across the gap and allowing the nature of the electron-boson coupling to be probed. The non-Fermi liquid behavior in these systems may be the result of a common Fermi surface topology of Dirac cone-like features in the electronic dispersion. C1 [Homes, C. C.; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Tu, J. J.; Li, J.] CUNY City Coll, Dept Phys, New York, NY 10031 USA. [Akrap, A.] Univ Geneva, Ecole Phys, CH-1211 Geneva 4, Switzerland. RP Homes, CC (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM homes@bnl.gov; jtu@sci.ccny.cuny.edu RI Akrap, Ana/G-1409-2013 OI Akrap, Ana/0000-0003-4493-5273 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-98CH10886] FX The authors would like to acknowledge useful discussions with P. W. Anderson, Y.M. Dai, D.N. Basov, D.A. Bonn, S. V. Borisenko, G. Kotliar, P. Phillips, J.D. Rameau, D. Schmeltzer and C. Varma. Research supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-98CH10886. C.C.H. would like to acknowledge the hospitality of the Theory Institute for Strongly Correlated and Complex Systems. NR 38 TC 5 Z9 5 U1 2 U2 15 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD DEC 13 PY 2013 VL 3 AR 3446 DI 10.1038/srep03446 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 273BZ UT WOS:000328509500001 PM 24336241 ER PT J AU Tessmer, OL Jiao, YH Cruz, JA Kramer, DM Chen, J AF Tessmer, Oliver L. Jiao, Yuhua Cruz, Jeffrey A. Kramer, David M. Chen, Jin TI Functional approach to high-throughput plant growth analysis SO BMC SYSTEMS BIOLOGY LA English DT Article; Proceedings Paper CT 24th International Conference on Genome Informatics (GIW) CY DEC 16-18, 2013 CL Singapore, SINGAPORE ID ARABIDOPSIS-THALIANA; CHLOROPHYLL FLUORESCENCE; IMAGE-ANALYSIS; EQUATIONS AB Method: Taking advantage of the current rapid development in imaging systems and computer vision algorithms, we present HPGA, a high-throughput phenotyping platform for plant growth modeling and functional analysis, which produces better understanding of energy distribution in regards of the balance between growth and defense. HPGA has two components, PAE (Plant Area Estimation) and GMA (Growth Modeling and Analysis). In PAE, by taking the complex leaf overlap problem into consideration, the area of every plant is measured from top-view images in four steps. Given the abundant measurements obtained with PAE, in the second module GMA, a nonlinear growth model is applied to generate growth curves, followed by functional data analysis. Results: Experimental results on model plant Arabidopsis thaliana show that, compared to an existing approach, HPGA reduces the error rate of measuring plant area by half. The application of HPGA on the cfq mutant plants under fluctuating light reveals the correlation between low photosynthetic rates and small plant area (compared to wild type), which raises a hypothesis that knocking out cfq changes the sensitivity of the energy distribution under fluctuating light conditions to repress leaf growth. C1 [Tessmer, Oliver L.; Chen, Jin] Michigan State Univ, Dept Comp Sci & Engn, E Lansing, MI 48864 USA. [Kramer, David M.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48864 USA. [Jiao, Yuhua; Cruz, Jeffrey A.; Kramer, David M.; Chen, Jin] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48864 USA. RP Kramer, DM (reprint author), Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48864 USA. EM kramerd8@msu.edu; jinchen@msu.edu NR 35 TC 21 Z9 22 U1 0 U2 27 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1752-0509 J9 BMC SYST BIOL JI BMC Syst. Biol. PD DEC 13 PY 2013 VL 7 SU 6 AR S17 DI 10.1186/1752-0509-7-S6-S17 PG 13 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA 270NY UT WOS:000328326600018 PM 24565437 ER PT J AU Greene, DL Lin, ZH Dong, J AF Greene, David L. Lin, Zhenhong Dong, Jing TI Analyzing the sensitivity of hydrogen vehicle sales to consumers' preferences SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen vehicles; Market penetration; Vehicle choice; Vehicle technology ID EFFICIENCY AB The success of hydrogen vehicles will depend on consumer behavior as well as technology, energy prices and public policy. This study examines the sensitivity of the future market shares of hydrogen-powered vehicles to alternative assumptions about consumers' preferences. The Market Acceptance of Advanced Automotive Technologies model was used to project future market shares. The model has 1458 market segments, differentiated by travel behavior, geography, and tolerance to risk, among other factors, and it estimates market shares for twenty advanced power-train technologies. The market potential of hydrogen vehicles is most sensitive to the improvement of drive train technology, especially cost reduction. The long-run market success of hydrogen vehicles is less sensitive to the price elasticity of vehicle choice, how consumers evaluate future fuel costs, and the importance of fuel availability and limited driving range. The importance of these factors will likely be greater in the early years following initial commercialization of hydrogen vehicles. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Greene, David L.; Lin, Zhenhong] Oak Ridge Natl Lab, Knoxville, TN 37932 USA. [Dong, Jing] Iowa State Univ, Ames, IA 50011 USA. RP Greene, DL (reprint author), Oak Ridge Natl Lab, 2360 Cherahala Blvd, Knoxville, TN 37932 USA. EM dlgreene@ornl.gov; linz@ornl.gov; jingdong@iastate.edu OI Dong, Jing/0000-0002-7304-8430 NR 24 TC 4 Z9 4 U1 0 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD DEC 13 PY 2013 VL 38 IS 36 BP 15857 EP 15867 DI 10.1016/j.ijhydene.2013.08.099 PG 11 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 264TS UT WOS:000327904500001 ER PT J AU Su, Q Yoon, D Sisman, Z Khatkhatay, F Jia, QX Manthiram, A Wang, HY AF Su, Qing Yoon, Daeil Sisman, Zeynep Khatkhatay, Fauzia Jia, Quanxi Manthiram, Arumugam Wang, Haiyan TI Vertically aligned nanocomposite La0.8Sr0.2MnO3-delta/Zr0.92Y0.08O1.96 thin films as electrode/electrolyte interfacial layer for solid oxide reversible fuel cells SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE LSM/YSZ oxygen electrode; Interlayer; Vertically aligned nanocomposite; SORFC; SOFC ID PULSED-LASER DEPOSITION; ELECTROLYSIS CELLS; SOFC CATHODE; IMPEDANCE; MICROSTRUCTURE; TECHNOLOGIES; MECHANISM; ENERGY AB A thin layer with a vertically aligned nanocomposite (VAN) structure of La0.8Sr0.2MnO3-delta (LSM) and Zr0.32Y0 O-08(1.96) (YSZ) between the oxygen electrode and the electrolyte has been fabricated by a pulsed laser deposition (PLD) technique for solid oxide reversible fuel cells (SORFCs). The high quality epitaxial growth of VAN structured LSM/YSZ has been achieved on single crystal SrTiO3 substrate at high-deposition temperatures. The symmetric cells with the VAN interlayer are found to have a lower area specific resistance compared to that without the interlayer. The enhancement in performance has been demonstrated by increased oxygen electrode catalytic properties and porous oxygen electrode microstructure. The cell with the VAN interlayer shows an open circuit voltage (OCV) of 1.00 V at 650 degrees C and maximum power densities of 0.22, 0.32, 0.43 and 0.55 W cm(-2) at 650, 700, 750 and 800 degrees C, respectively. Compared with the cell without an interlayer, the cells with the interlayer have similar to 2 times of the overall maximum power density at the measured temperature range, demonstrating that the VAN interlayer significantly enhances the oxygen electrode performance. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Su, Qing; Sisman, Zeynep; Wang, Haiyan] Texas A&M Univ, Mat Sci & Engn Program, College Stn, TX 77843 USA. [Yoon, Daeil; Manthiram, Arumugam] Univ Texas Austin, Electrochem Energy Lab, Austin, TX 78712 USA. [Yoon, Daeil; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Khatkhatay, Fauzia; Wang, Haiyan] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. RP Wang, HY (reprint author), Texas A&M Univ, Mat Sci & Engn Program, College Stn, TX 77843 USA. EM wangh@ece.tamu.edu RI Jia, Q. X./C-5194-2008; Su, Qing/N-2518-2014; Wang, Haiyan/P-3550-2014; OI Wang, Haiyan/0000-0002-7397-1209; Su, Qing/0000-0003-2477-0002 FU National Science Foundation [NSF-0846504, NSF-1007969]; Welch Foundation [F-1254]; U.S. Department of Energy through the Center for Integrated Nanotechnologies; U.S. Department of Energy, Office of Basic Energy Sciences FX The work at the Texas A&M University was supported by the National Science Foundation (NSF-0846504 and NSF-1007969). The work at the University of Texas at Austin was supported by the Welch Foundation grant F-1254. The work at Los Alamos was supported in part by the U.S. Department of Energy through the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory. NR 33 TC 7 Z9 7 U1 4 U2 64 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD DEC 13 PY 2013 VL 38 IS 36 BP 16320 EP 16327 DI 10.1016/j.ijhydene.2013.09.128 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 264TS UT WOS:000327904500050 ER PT J AU Shan, YP Tiwari, PB Krishnakumar, P Vlassiouk, I Li, WZ Wang, XW Darici, Y Lindsay, SM Wang, HD Smirnov, S He, J AF Shan, Y. P. Tiwari, P. B. Krishnakumar, P. Vlassiouk, I. Li, W. Z. Wang, X. W. Darici, Y. Lindsay, S. M. Wang, H. D. Smirnov, S. He, J. TI Surface modification of graphene nanopores for protein translocation SO NANOTECHNOLOGY LA English DT Article ID SOLID-STATE NANOPORES; DNA TRANSLOCATION; SINGLE; TRANSPORT; MOLECULES; SENSORS AB Studies of DNA translocation through graphene nanopores have revealed their potential for DNA sequencing. Here we report a study of protein translocation through chemically modified graphene nanopores. A transmission electron microscope (TEM) was used to cut nanopores with diameters between 5 and 20 nm in multilayer graphene prepared by chemical vapor deposition (CVD). After oxygen plasma treatment, the dependence of the measured ionic current on salt concentration and pH was consistent with a small surface charge induced by the formation of carboxyl groups. While translocation of gold nanoparticles (10 nm) was readily detected through such treated pores of a larger diameter, translocation of the protein ferritin was not observed either for oxygen plasma treated pores, or for pores modified with mercaptohexadecanoic acid. Ferritin translocation events were reliably observed after the pores were modified with the phospholipid-PEG (DPPE-PEG750) amphiphile. The ion current signature of translocation events was complex, suggesting that a series of interactions between the protein and pores occurs during the process. C1 [Shan, Y. P.; Tiwari, P. B.; Li, W. Z.; Wang, X. W.; Darici, Y.; He, J.] Florida Int Univ, Dept Phys, Miami, FL 33199 USA. [Krishnakumar, P.; Lindsay, S. M.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Vlassiouk, I.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Lindsay, S. M.] Arizona State Univ, Biodesign Inst, Tempe, AZ 85287 USA. [Lindsay, S. M.] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Wang, H. D.] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Jilin, Peoples R China. [Smirnov, S.] New Mexico State Univ, Dept Chem & Biochem, Las Cruces, NM 88003 USA. RP Shan, YP (reprint author), Florida Int Univ, Dept Phys, Miami, FL 33199 USA. EM snsm@nmsu.edu; jinhe@fiu.edu RI Smirnov, Sergei/H-8774-2016; Li, Wenzhi/J-6797-2016; Vlassiouk, Ivan/F-9587-2010 OI Li, Wenzhi/0000-0001-8442-2232; Vlassiouk, Ivan/0000-0002-5494-0386 FU FIU CAS; DNA Sequencing Technology Program of the National Human Genome Research Institute [1RC2HG005625-01, 1R21HG004770-01]; China NSFC [21073181]; China CAS '100 Talent Program'; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX We acknowledge the use of the nanofab at the Center for Solid State Electronic Research (CSSER) and SEM and TEM at the Center for Solid State Science (CSSS) at Arizona State University, and the nanofab at AMERI at Florida International University (FIU). This work was supported by the start-up funds and 2012 faculty summer research award (JH) from FIU CAS and the DNA Sequencing Technology Program of the National Human Genome Research Institute (1RC2HG005625-01, 1R21HG004770-01), China NSFC (grant no 21073181) and China CAS '100 Talent Program' (to HW). P Tiwari would also like to thank FIU School of Integrated Science and Humanity, College of Arts and Sciences for the research assistantship. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 40 TC 12 Z9 12 U1 6 U2 79 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD DEC 13 PY 2013 VL 24 IS 49 AR 495102 DI 10.1088/0957-4484/24/49/495102 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 269BN UT WOS:000328215300002 PM 24231385 ER PT J AU Timilsina, R Rack, PD AF Timilsina, Rajendra Rack, Philip D. TI Monte Carlo simulations of nanoscale focused neon ion beam sputtering SO NANOTECHNOLOGY LA English DT Article ID INDUCED DEPOSITION; MICROSCOPE; TARGETS; PROGRAM AB A Monte Carlo simulation is developed to model the physical sputtering of aluminum and tungsten emulating nanoscale focused helium and neon ion beam etching from the gas field ion microscope. Neon beams with different beam energies (0.5-30 keV) and a constant beam diameter (Gaussian with full-width-at-half-maximum of 1 nm) were simulated to elucidate the nanostructure evolution during the physical sputtering of nanoscale high aspect ratio features. The aspect ratio and sputter yield vary with the ion species and beam energy for a constant beam diameter and are related to the distribution of the nuclear energy loss. Neon ions have a larger sputter yield than the helium ions due to their larger mass and consequently larger nuclear energy loss relative to helium. Quantitative information such as the sputtering yields, the energy-dependent aspect ratios and resolution-limiting effects are discussed. C1 [Timilsina, Rajendra; Rack, Philip D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Rack, Philip D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Timilsina, R (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM prack@utk.edu OI Rack, Philip/0000-0002-9964-3254 FU Division of Scientific User Facilities, US Department of Energy FX The authors would like to acknowledge the support of the Semiconductor Research Corporation (Bob Havemann, Program Manager). PDR also acknowledges that part of the original algorithms for the secondary electron and gas handling were developed at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, US Department of Energy. NR 37 TC 6 Z9 6 U1 1 U2 24 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD DEC 13 PY 2013 VL 24 IS 49 AR 495303 DI 10.1088/0957-4484/24/49/495303 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 269BN UT WOS:000328215300008 PM 24231648 ER PT J AU Li, X Shu, C Yi, GH Chaton, CT Shelton, CL Diao, JS Zuo, XB Kao, CC Herr, AB Li, PW AF Li, Xin Shu, Chang Yi, Guanghui Chaton, Catherine T. Shelton, Catherine L. Diao, Jiasheng Zuo, Xiaobing Kao, C. Cheng Herr, Andrew B. Li, Pingwei TI Cyclic GMP-AMP Synthase Is Activated by Double-Stranded DNA-Induced Oligomerization SO IMMUNITY LA English DT Article ID INNATE IMMUNE-RESPONSE; CYTOSOLIC DNA; DI-GMP; ANTIVIRAL RESPONSE; SIGNALING PATHWAY; STRUCTURAL BASIS; RECOGNITION; CGAS; 2ND-MESSENGER; DINUCLEOTIDE AB Cyclic GMP-AMP synthase (cGAS) is a cytosolic DNA sensor mediating innate antimicrobial immunity. It catalyzes the synthesis of a noncanonical cyclic dinucleotide, 20,50 cGAMP, that binds to STING and mediates the activation of TBK1 and IRF-3. Activated IRF-3 translocates to the nucleus and initiates the transcription of the IFN-beta gene. The structure of mouse cGAS bound to an 18 bp dsDNA revealed that cGAS interacts with dsDNA through two binding sites, forming a 2: 2 complex. Enzyme assays and IFN-beta reporter assays of cGAS mutants demonstrated that interactions at both DNA binding sites are essential for cGAS activation. Mutagenesis and DNA binding studies showed that the two sites bind dsDNA cooperatively and that site B plays a critical role in DNA binding. The structure of mouse cGAS bound to dsDNA and 20,50 cGAMP provided insight into the catalytic mechanism of cGAS. These results demonstrated that cGAS is activated by dsDNA-induced oligomerization. C1 [Li, Xin; Shu, Chang; Diao, Jiasheng; Li, Pingwei] Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. [Yi, Guanghui; Kao, C. Cheng] Indiana Univ, Dept Mol & Cellular Biochem, Bloomington, IN 47405 USA. [Chaton, Catherine T.; Shelton, Catherine L.; Herr, Andrew B.] Univ Cincinnati, Coll Med, Dept Mol Genet Biochem & Microbiol, Cincinnati, OH 45267 USA. [Zuo, Xiaobing] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Li, PW (reprint author), Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. EM pingwei@tamu.edu RI shu, chang/H-4452-2015; OI shu, chang/0000-0002-6738-8973; Herr, Andrew/0000-0002-3598-3399; Herr, Amy/0000-0002-6906-2985 FU National Institutes of Health [AI 087741]; Welch Foundation [A-1816] FX The diffraction data of the hcGAS crystals were collected the Stanford Synchrotron Radiation Lightsource (SSRL). The SAXS studies of cGAS were conducted at the Advanced Photon Source (APS). We thank L. Tong from Columbia University for suggestions on structural determination and J.-Y. Ji from Texas A&M University for critical reading of the manuscript and valuable discussions. This research was supported by the National Institutes of Health (grant AI 087741 to P. L.) and the Welch Foundation (grant A-1816 to P. L.). This work is dedicated to the memory of Y.-X. Wang (1914-2008) of Peking University. NR 41 TC 56 Z9 60 U1 2 U2 16 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1074-7613 EI 1097-4180 J9 IMMUNITY JI Immunity PD DEC 12 PY 2013 VL 39 IS 6 BP 1019 EP 1031 DI 10.1016/j.immuni.2013.10.019 PG 13 WC Immunology SC Immunology GA AA2UZ UT WOS:000330951000009 PM 24332030 ER PT J AU Li, XY Chen, X Hu, BX Navon, IM AF Li, Xinya Chen, Xiao Hu, Bill X. Navon, I. Michael TI Model reduction of a coupled numerical model using proper orthogonal decomposition SO JOURNAL OF HYDROLOGY LA English DT Article DE Model reduction; Proper orthogonal decomposition; Single value decomposition; Galerkin projection; Variable density flow ID GROUNDWATER-FLOW MODELS; WATER EQUATIONS MODEL; KARHUNEN-LOEVE EXPANSION; VARIABLE-DENSITY FLOW; HENRY PROBLEM; ORDER REDUCTION; POROUS MEDIUM; IDENTIFICATION; WORTHINESS; SIMULATION AB Numerical models for variable-density flow and solute transport (VDFST) are widely used to simulate seawater intrusion and related problems. The mathematical model for VDFST is a coupled nonlinear dynamical system, so the numerical discretizations in time and space are usually required to be as fine as possible. As a result, fine-scale transient models require large computational time, which is a disadvantage for state estimation, forward prediction or model inversion. The purpose of this research is to develop mathematical and numerical methods to simulate VDFST via a model order reduction technique called Proper Orthogonal Decomposition (POD) designed for nonlinear dynamical systems. POD was applied to extract leading "model features" (basis functions) through singular value decomposition (SVD) from observational data or simulations (snapshots) of high-dimensional systems. These basis functions were then used in the Galerkin projection procedure that yielded low-dimensional (reduced-order) models. The original full numerical models were also discretized by the Galerkin Finite-Element Method (GFEM). The implementation of the POD reduced-order method was straightforward when applied to the full order model to the complex model. The developed GFEM-POD model was applied to solve two classic VDFST cases, the Henry problem and the Elder problem, in order to investigate the accuracy and efficiency of the POD model reduction method. Once the snapshots from full model results are obtained, the reduced-order model can reproduce the full model results with acceptable accuracy but with less computational cost in comparison with the full model, which is useful for model calibration and data assimilation problems. We found that the accuracy and efficiency of the POD reduced-order model is mainly determined by the optimal selection of snapshots and POD bases. Validation and verification experiments confirmed our POD model reduction procedure. (C) 2013 Elsevier B.V. All rights reserved. C1 [Li, Xinya] Pacific NW Natl Lab, Hydrol Energy & Environm Directorate, Richland, WA 99352 USA. [Chen, Xiao] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA. [Hu, Bill X.] Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. [Navon, I. Michael] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. RP Chen, X (reprint author), Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA. EM chen73@llnl.gov RI Navon, Ionel/A-5173-2008; Chen, Xiao/K-3070-2014 OI Navon, Ionel/0000-0001-7830-7094; FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; NSF [ATM-0931198] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Prof. Navon acknowledges the support of NSF Grant ATM-0931198. NR 47 TC 1 Z9 1 U1 1 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD DEC 12 PY 2013 VL 507 BP 227 EP 240 DI 10.1016/j.jhydrol.2013.09.011 PG 14 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA 300UY UT WOS:000330490700019 ER PT J AU Armstrong, MR Zaug, JM Goldman, N Kuo, IFW Crowhurst, JC Howard, WM Carter, JA Kashgarian, M Chesser, JM Barbee, TW Bastea, S AF Armstrong, Michael R. Zaug, Joseph M. Goldman, Nir Kuo, I-Feng W. Crowhurst, Jonathan C. Howard, W. Michael Carter, Jeffrey A. Kashgarian, Michaele Chesser, John M. Barbee, Troy W. Bastea, Sorin TI Ultrafast Shock Initiation of Exothermic Chemistry in Hydrogen Peroxide SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MOLECULAR-DYNAMICS; HIGH-PRESSURES; DENSITY; WAVES; NITROMETHANE; ALUMINUM; BEHAVIOR; FILMS AB We report observations of shock compressed, unreacted hydrogen peroxide at pressures up to the von Neumann pressure for a steady detonation wave, using ultrafast laser-driven shock wave methods. At higher laser drive energy we find evidence of exothermic chemical reactivity occurring in less than 100 ps after the arrival of the shock wave in the sample. The results are consistent with our MD simulations and analysis and suggest that reactivity in hydrogen peroxide is initiated on a sub-100 ps time scale under conditions found just subsequent to the lead shock in a steady detonation wave. C1 [Armstrong, Michael R.; Zaug, Joseph M.; Goldman, Nir; Kuo, I-Feng W.; Crowhurst, Jonathan C.; Howard, W. Michael; Carter, Jeffrey A.; Kashgarian, Michaele; Chesser, John M.; Barbee, Troy W.; Bastea, Sorin] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Armstrong, MR (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. EM armstrong30@llnl.gov; zaug1@llnl.gov RI Armstrong, Michael/I-9454-2012 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development grant [11ERD067] FX We acknowledge useful conversations with L. E. Fried, S. McGrane, C. Tarver, and R. Manaa. We also recognize the friendship and achievements of W. Michael Howard, who will be greatly missed. This research was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and it was funded by Laboratory Directed Research and Development grant 11ERD067 with S.B. as principal investigator. NR 56 TC 9 Z9 9 U1 3 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD DEC 12 PY 2013 VL 117 IS 49 BP 13051 EP 13058 DI 10.1021/jp407595u PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 273IU UT WOS:000328529300002 PM 24102452 ER PT J AU Wagner, AF AF Wagner, Albert F. TI Improved Multidimensional Semiclassical Tunneling Theory SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TRANSITION-STATE THEORY; FORCE-FIELDS; BARRIER AB We show that the analytic multidimensional semiclassical tunneling formula of Miller et al. [Miller, W. H.; Hernandez, R.; Handy, N. C.; Jayatilaka, D.; Willets, A. Chem. Phys. Lett. 1990, 172, 62] is qualitatively incorrect for deep tunneling at energies well below the top of the barrier. The origin of this deficiency is that the formula uses an effective barrier weakly related to the true energetics but correctly adjusted to reproduce the harmonic description and anharmonic corrections of the reaction path at the saddle point as determined by second order vibrational perturbation theory. We present an analytic improved semiclassical formula that correctly includes energetic information and allows a qualitatively correct representation of deep tunneling. This is done by constructing a three segment composite Eckart potential that is continuous everywhere in both value and derivative. This composite potential has an analytic barrier penetration integral from which the semiclassical action can be derived and then used to define the semiclassical tunneling probability. The middle segment of the composite potential by itself is superior to the original formula of Miller et al. because it incorporates the asymmetry of the reaction barrier produced by the known reaction exoergicity. Comparison of the semiclassical and exact quantum tunneling probability for the pure Eckart potential suggests a simple threshold multiplicative factor to the improved formula to account for quantum effects very near threshold not represented by semiclassical theory. The deep tunneling limitations of the original formula are echoed in semiclassical high-energy descriptions of bound vibrational states perpendicular to the reaction path at the saddle point. However, typically ab initio energetic information is not available to correct it. The Supporting Information contains a Fortran code, test input, and test output that implements the improved semiclassical tunneling formula. C1 Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Wagner, AF (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. EM wagner@anl.gov FU Office of Basic Energy Sciences, Division of Chemical Sciences, U.S. Department of Energy [DE-AC02-06CH11357] FX We thank John Stanton (University of Texas) and John Barker (University of Michigan) for many valuable discussions of this work. We thank a reviewer for alerting us to a more general context for semiclassical transition state theory. This work was supported by a grant from the Office of Basic Energy Sciences, Division of Chemical Sciences, U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 16 TC 10 Z9 10 U1 2 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD DEC 12 PY 2013 VL 117 IS 49 BP 13089 EP 13100 DI 10.1021/jp409720s PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 273IU UT WOS:000328529300006 PM 24224758 ER PT J AU Kashyap, HK Santos, CS Murthy, NS Hettige, JJ Kerr, K Ramati, S Gwon, J Gohdo, M Lall-Ramnarine, SI Wishart, JF Margulis, CJ Castner, EW AF Kashyap, Hemant K. Santos, Cherry S. Murthy, N. Sanjeeva Hettige, Jeevapani J. Kerr, Kijana Ramati, Sharon Gwon, JinHee Gohdo, Masao Lall-Ramnarine, Sharon I. Wishart, James F. Margulis, Claudio J. Castner, Edward W., Jr. TI Structure of 1-Alky1-1-methylpyrrolidinium Bis(trifluoromethylsulfonyl)amide Ionic Liquids with Linear, Branched, and Cyclic Alkyl Groups SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID X-RAY-SCATTERING; MOLECULAR-DYNAMICS SIMULATIONS; PARTICLE MESH EWALD; ORIENTATIONAL DYNAMICS; CATION SYMMETRY; CHAIN-LENGTH; FORCE-FIELD; TEMPERATURE; IMIDAZOLIUM; BIS(TRIFLUOROMETHANESULFONYL)AMIDE AB X-ray scattering and molecular dynamics simulations have been carried out to investigate structural differences and similarities in the condensed phase between pyrrolidinium-based ionic liquids paired with the bis(trifluoromethylsulfonyl)amide (NTf2-) anion where the cationic tail is linear, branched, or cyclic. This is important in light of the charge and polarity type alternations that have recently been shown to be present in the case of liquids with cations of moderately long linear tails. For this study, we have chosen to use the 1-alkyl-1-methylpyrrolidinium, Pyrri(1,n)(+) with n = 5 or 7, as systems with linear tails, 1-(2ethylhexyl)-1-methylpyrrolidinium, Pyrr(1,Ethx)(+), as a system with a branched tail, and 1-(cyclohexylmethyl)-1-methylpyrrolidinium, Pyrr(1,Ethx)(+), as a system with a cyclic tail. We put these results into context by comparing these data with recently published results for the Pyrr(1,n)(+)/NTf2- ionic liquids with n = 4, 6, 8, and 10.(1,2) General methods for interpreting the structure function S(q) in terms of q-dependent natural partitionings are described. This allows for an in-depth analysis of the scattering data based on molecular dynamics (MD) trajectories that highlight the effect of modifying the cationic tail. C1 [Kashyap, Hemant K.; Hettige, Jeevapani J.; Margulis, Claudio J.] Univ Iowa, Dept Chem, Iowa City, IA 52242 USA. [Santos, Cherry S.; Castner, Edward W., Jr.] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. [Murthy, N. Sanjeeva] Rutgers State Univ, New Jersey Ctr Biomat, Piscataway, NJ 08854 USA. [Kerr, Kijana; Gohdo, Masao; Wishart, James F.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Ramati, Sharon; Gwon, JinHee; Lall-Ramnarine, Sharon I.] CUNY Queensborough Community Coll, Dept Chem, New York, NY 11364 USA. RP Margulis, CJ (reprint author), Univ Iowa, Dept Chem, Iowa City, IA 52242 USA. EM claudio-margulis@uiowa.edu; ed.castner@rutgers.edu RI Wishart, James/L-6303-2013 OI Wishart, James/0000-0002-0488-7636 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-SC0001780, DE-SC0008644, DE-AC02-98CH10886]; BNL by the DOE Office of Nuclear Energy from Queensborough Community College; PSC-CUNY Research Award Grants; Louis Stokes Alliance for Minority Participation; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors thank Prof. Mark Maroncelli for the sample of Pyrr1,5+/NTf2-, Dr. Tomasz Szreder for measuring the density of Pyrr1,4+/NTf2-, Dr. Alison Funston for measuring the density of Pyrr1,5+/NTf2-, and Jasmine Hatcher for assistance preparing scattering samples. We thank Dr. Chris Benmore and Dr. Yang Ren for help in the X-ray measurements and data analysis at APS beamline 11-ID-C. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under contracts DE-SC0001780 (E.W.C.), DE-SC0008644 (CJ.M.), and DE-AC02-98CH10886 (J.F.W.). Preparation of Pyrr1,ChxMe+ and Pyrr1,7+ salts by K.K. was supported at BNL by the DOE Office of Nuclear Energy. Researchers (S.L.-R., S.R., J.G.) from Queensborough Community College were supported by PSC-CUNY Research Award Grants and the Louis Stokes Alliance for Minority Participation. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 83 TC 51 Z9 51 U1 1 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD DEC 12 PY 2013 VL 117 IS 49 SI SI BP 15328 EP 15337 DI 10.1021/jp403518j PG 10 WC Chemistry, Physical SC Chemistry GA 273IR UT WOS:000328529000011 PM 23750608 ER PT J AU Lu, YC Crumlin, EJ Carney, TJ Baggetto, L Veith, GM Dudney, NJ Liu, Z Shao-Horn, Y AF Lu, Yi-Chun Crumlin, Ethan J. Carney, Thomas J. Baggetto, Loic Veith, Gabriel M. Dudney, Nancy J. Liu, Zhi Shao-Horn, Yang TI Influence of Hydrocarbon and CO2 on the Reversibility of Li-O-2 Chemistry Using In Situ Ambient Pressure X-ray Photoelectron Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-AIR BATTERIES; LITHIUM-OXYGEN BATTERIES; ETHER-BASED ELECTROLYTE; CARBONATE ELECTROLYTES; DISCHARGE PRODUCTS; ION BATTERIES; CELLS; SALTS; LI2O2; ELECTROCHEMISTRY AB Identifying fundamental barriers that hinder reversible lithium-oxygen (Li-O-2) redox reaction is essential for developing efficient and long-lasting rechargeable Li-O-2 batteries. Addressing these challenges is being limited by parasitic reactions in the carbon-based O-2-electrode with aprotic electrolytes. Understanding the mechanisms of these parasitic reactions is hampered by the complexity that multiple and coupled parasitic reactions involving carbon, electrolytes, and Li-O-2 reaction intermediates/products can occur simultaneously. In this work, we employed solid-state cells free of carbon and aprotic electrolytes to probe the influence of surface adventitious hydrocarbons and carbon dioxide (CO2) on the reversibility of the Li-O-2 redox chemistry using in situ synchrotron-based ambient pressure X-ray photoelectron spectroscopy. Direct evidence was provided, for the first time, that surface hydrocarbons and CO2 irreversibly react with Li-O-2 reaction intermediates/products such as Li2O2 and Li2O, forming carboxylate and carbonate-based species, which cannot be removed fully upon recharge. The slower Li2O2 oxidation kinetics was correlated with increasing coverage of surface carbonate/carboxylate species. Our work critically points out that materials design that mitigates the reactivity between Li-O-2 reaction products and common impurities in the atmosphere is needed to achieve long cycle-life Li-O-2 batteries. C1 [Lu, Yi-Chun; Shao-Horn, Yang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Lu, Yi-Chun; Carney, Thomas J.; Shao-Horn, Yang] MIT, Electrochem Energy Lab, Cambridge, MA 02139 USA. [Crumlin, Ethan J.; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Carney, Thomas J.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Baggetto, Loic; Veith, Gabriel M.; Dudney, Nancy J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Shao-Horn, Y (reprint author), MIT, Dept Mech Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM shaohorn@mit.edu RI Liu, Zhi/B-3642-2009; Lu, Yi-Chun/J-1841-2015; Dudney, Nancy/I-6361-2016; Baggetto, Loic/D-5542-2017 OI Liu, Zhi/0000-0002-8973-6561; Lu, Yi-Chun/0000-0003-1607-1615; Dudney, Nancy/0000-0001-7729-6178; Baggetto, Loic/0000-0002-9029-2363 FU MRSEC Program of the National Science Foundation [DMR- 0819762]; Office of FreedomCAR and Vehicle Technologies of the U.S. Department of Energy [DE-AC03-76SF00098]; Lawrence Berkeley National Laboratory; U.S. Department of Energy's U.S.-China Clean Energy Research Center for Clean Vehicles [DE-PI0000012]; Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; UT-Battelle, LLC.; ALS Postdoctoral Fellowship Program FX This work was supported in part by the MRSEC Program of the National Science Foundation under Award DMR- 0819762, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of FreedomCAR and Vehicle Technologies of the U.S. Department of Energy, under Contract DE-AC03-76SF00098 with the Lawrence Berkeley National Laboratory, the U.S. Department of Energy's U.S.-China Clean Energy Research Center for Clean Vehicles, Grant DE-PI0000012, and the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. Research conducted at ORNL was supported by the U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering, under contract with UT-Battelle, LLC. E.J.C. is grateful for the financial support from the ALS Postdoctoral Fellowship Program. NR 50 TC 25 Z9 25 U1 5 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 12 PY 2013 VL 117 IS 49 BP 25948 EP 25954 DI 10.1021/jp409453s PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 273IZ UT WOS:000328529800010 ER PT J AU Rodovsky, DB Peet, J Shao, N Azoulay, JD Bazan, GC Drolet, N Wu, Q Sfeir, MY AF Rodovsky, Deanna B. Peet, Jeff Shao, Nan Azoulay, Jason D. Bazan, Guillermo C. Drolet, Nicolas Wu, Qin Sfeir, Matthew Y. TI Quantifying the Relationship between the Maximum Achievable Voltage and Current Levels in Low-Bandgap Polymer Photovoltaics SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; DONOR-ACCEPTOR POLYMERS; EXCITON DISSOCIATION; ELECTRON-TRANSFER; CHARGE-TRANSFER; GAP POLYMERS; ENERGY; DYNAMICS; EFFICIENCY; OFFSETS AB A critical problem in the design of materials for organic photovoltaics is quantifying the driving force needed for efficient charge separation without losses associated with a large overpotential. Here, we directly measured the effect of the molecular driving force on the charge transfer rate in films of low-bandgap push-pull type polymers mixed with a series of fullerene-based molecular acceptors using broadband near-infrared transient absorption spectroscopy. By systematically tuning the absolute energy levels of the donor and acceptor, as well as the relative offset between them, we determine the minimum voltage loss required to achieve a high short circuit current. A molecular donor-acceptor framework provides a quantitative description of the charge transfer rate constants in our system and describes the scaling of the photogenerated current with S-1-LUMO energy offset. These results point to potential efficiency gains for high performing polymer devices through recovery of additional voltage without sacrificing current output. C1 [Rodovsky, Deanna B.; Peet, Jeff; Drolet, Nicolas] Konarka Technol, Lowell, MA 01852 USA. [Rodovsky, Deanna B.] NIST, Gaithersburg, MD 20899 USA. [Shao, Nan; Wu, Qin; Sfeir, Matthew Y.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Azoulay, Jason D.; Bazan, Guillermo C.] Univ Calif Santa Barbara, Ctr Polymers & Organ Solids, Santa Barbara, CA 93106 USA. RP Sfeir, MY (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM msfeir@bnl.gov RI Wu, Qin/C-9483-2009; Bazan, Guillermo/B-7625-2014; OI Wu, Qin/0000-0001-6350-6672; Sfeir, Matthew/0000-0001-5619-5722 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. NR 31 TC 3 Z9 3 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 12 PY 2013 VL 117 IS 49 BP 25955 EP 25960 DI 10.1021/jp410234u PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 273IZ UT WOS:000328529800011 ER PT J AU Skripov, AV Babanova, OA Soloninin, AV Stavila, V Verdal, N Udovic, TJ Rush, JJ AF Skripov, Alexander V. Babanova, Olga A. Soloninin, Alexei V. Stavila, Vitalie Verdal, Nina Udovic, Terrence J. Rush, John J. TI Nuclear Magnetic Resonance Study of Atomic Motion in A(2)B(12)H(12) (A = Na, K, Rb, Cs): Anion Reorientations and Na+ Mobility SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DODECAHYDRO-CLOSO-DODECABORATE; HYDROGEN DIFFUSION; METAL BOROHYDRIDES; PHASE-TRANSITION; LIBH4; NMR; LI2B12H12; DECOMPOSITION; DESORPTION; STABILITY AB To study the reorientational motion of icosahedral [B12H12](2-) anions in A(2)B(12)H(12) (A = Na, K, Rb, Cs) and the translational diffusion of Na+ cations in Na2B12H12, we have measured the H-1, B-11, and Na-23 NMR spectra and spin-lattice relaxation rates in these compounds over the temperature range of 170-580 K. For cubic compounds K2B12H12, Rb2B12H12, and Cs2B12H12, the measured H-1 and B-11 spin-lattice relaxation rates are governed by thermally activated reorientations of the [B12H12](2-) anions. The activation energy of this reorientational motion is found to decrease with increasing cation radius, changing from 800 meV for K2B12H12 to 549 meV for Rb2B12H12 and 427 meV for Cs2B12H12. For Na2B12H12, the first-order transition from the low-temperature monoclinic to the high-temperature cubic phase near 520 K is accompanied by a 2 orders of magnitude increase in the reorientational jump rate, and the corresponding activation energy changes from 770 meV for the low-T phase to 270 meV for the high-T phase. Measurements of the Na-23 NMR spectra and spin-lattice relaxation rates show that the transition from the low-T to the high-T phase of Na2B12H12 is also accompanied by the onset of the fast translational diffusion of Na+ ions. Just above the transition point, the lower limit of the Na+ jump rate estimated from the Na-23 spin-lattice relaxation data is 2 x 10(8) s(-1), and the corresponding activation energy for Na+ diffusion is about 410 meV. C1 [Skripov, Alexander V.; Babanova, Olga A.; Soloninin, Alexei V.] Russian Acad Sci, Ural Div, Inst Met Phys, Ekaterinburg 620990, Russia. [Stavila, Vitalie] Sandia Natl Labs, Livermore, CA 94551 USA. [Verdal, Nina; Udovic, Terrence J.; Rush, John J.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Verdal, Nina; Rush, John J.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Skripov, AV (reprint author), Russian Acad Sci, Ural Div, Inst Met Phys, S Kovalevskoi 18, Ekaterinburg 620990, Russia. EM skripov@imp.uran.ru RI Babanova, Olga/J-4821-2013; Skripov, Alexander/K-4525-2013; Soloninin, Alexey/J-8580-2013 OI Babanova, Olga/0000-0002-2422-3263; Skripov, Alexander/0000-0002-0610-5538; Soloninin, Alexey/0000-0001-7127-9641 FU U.S. Department of Energy EERE [DE-EE0002978, DE-AI-01-05EE11104, DE-AC04-94AL85000]; Russian Foundation for Basic Research [12-03-00078]; Russian Academy of Sciences (RAS) [12-P-2-1050]; Ural Branch of RAS [RUP1-7076-EK-12]; U.S. Civilian Research & Development Foundation (CRDF Global); U.S. Department of State FX This work was supported by the U.S. Department of Energy EERE (Grants DE-EE0002978, DE-AI-01-05EE11104, and DE-AC04-94AL85000), the Russian Foundation for Basic Research (Grant 12-03-00078), the Priority Program 12-P-2-1050 "Physico-technical principles of development of technologies and devices for smart adaptive electrical networks" of the Russian Academy of Sciences (RAS), and the collaborative Grant RUP1-7076-EK-12 from the Ural Branch of RAS and the U.S. Civilian Research & Development Foundation (CRDF Global) with funding from the U.S. Department of State. The opinions, findings and conclusions stated herein are those of the authors and do not necessarily reflect those of CRDF Global or the U.S. Department of State. NR 26 TC 22 Z9 22 U1 4 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 12 PY 2013 VL 117 IS 49 BP 25961 EP 25968 DI 10.1021/jp4106585 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 273IZ UT WOS:000328529800012 ER PT J AU Thompson, CM Carl, LM Somorjai, GA AF Thompson, Christopher M. Carl, Lindsay M. Somorjai, Gabor A. TI Sum Frequency Generation Study of the Interfacial Layer in Liquid-Phase Heterogeneously Catalyzed Oxidation of 2-Propanol on Platinum: Effect of the Concentrations of Water and 2-Propanol at the Interface SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MULTIPLE STEADY-STATES; VIBRATIONAL SPECTROSCOPY; METAL-CATALYSTS; ETHANOL ELECTROOXIDATION; SELECTIVE OXIDATION; MOLECULAR-OXYGEN; AQUEOUS-ETHANOL; CARBON; SFG; SURFACES AB Sum frequency generation (SFG) vibrational spectroscopy was applied to study the solid-liquid interface in the heterogeneously catalyzed oxidation of 2-propanol to acetone by dissolved dioxygen in aqueous solution on platinum. The mole fraction of alcohol was varied from 0 to 1. At 2-propanol mole fractions less than 0.14 and above 0.23, the TOF for acetone is approximately 20 h(-1). A 3-fold increase in the reaction rate is seen when 2-propanol is present with concentrations in this intermediate range (0.14-0.23). SFG spectra indicate that in aqueous mixtures of 2-propanol the solid-liquid interface is dominated by the alcohol, even at low mole fractions of alcohol, but resonant features from molecular 2-propanol not bound to the platinum surface appear only above 0.14 mole fraction. At 2-propanol concentrations where the highest reaction rates are observed, SFG shows the presence of water and alcohol at the catalyst interface, whereas, above and below these concentrations, either water or 2-propanol is not detectable at the surface. When water is excluded totally from the surface, the reaction rate is decreased. We attribute this correlation of surface concentrations to a dependence of the reaction rate on both alcohol and water, and our results demonstrate the importance of considering the interfacial concentration in liquid-phase heterogeneous catalysts. C1 [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 33 TC 5 Z9 5 U1 1 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 12 PY 2013 VL 117 IS 49 BP 26077 EP 26083 DI 10.1021/jp408123u PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 273IZ UT WOS:000328529800025 ER PT J AU Hummer, DR Kubicki, JD Kent, PRC Heaney, PJ AF Hummer, Daniel R. Kubicki, James D. Kent, Paul R. C. Heaney, Peter J. TI Single-Site and Monolayer Surface Hydration Energy of Anatase and Rutile Nanoparticles Using Density Functional Theory SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TIO2 ULTRAFINE POWDERS; NANOCRYSTALLINE TIO2; PHASE-STABILITY; TITANIUM-DIOXIDE; WATER; ENERGETICS; PRECIPITATION; TEMPERATURE; ADSORPTION; SIMULATION AB Models of 1, 2, and 3 nm diameter anatase and rutile particles, with either a surface monolayer of water or a single water molecule at different surface sites, were subjected to energy minimizations using density functional theory (DFT). The optimized structures show that H2O molecules bind covalently to both anatase and rutile particles via undercoordinated Ti atoms at the surface of the particle, with a significant degree of hydrogen bonding to other surface waters and bridging oxygens. Ti-OH2 bonds are more highly ordered on anatase surfaces but are stronger on rutile surfaces. Energies of the fully optimized structures with and without water show that hydration of rutile surfaces is more strongly exothermic than is the hydration of anatase surfaces, and this effect becomes more pronounced as particle size decreases. Individual surface sites exhibit a wide range of hydration energies, explaining the strong experimental dependence of hydration energy on water coverage. The less exothermic surface hydration energy of anatase offsets its lower vacuum surface energy and makes ruble nanoparticles thermodynamically competitive with anatase in low-temperature aqueous solutions. C1 [Hummer, Daniel R.; Kubicki, James D.; Heaney, Peter J.] Penn State Univ, Dept Geosci, University Pk, PA 16802 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Hummer, DR (reprint author), Univ Calif Los Angeles, Dept Earth & Space Sci, Los Angeles, CA 90095 USA. EM dhummer@ess.ucla.edu RI Kent, Paul/A-6756-2008; Kubicki, James/I-1843-2012 OI Kent, Paul/0000-0001-5539-4017; Kubicki, James/0000-0002-9277-9044 FU National Science Foundation [EAR07-45374, EAR11-47728]; Center for Environmental Kinetics Analysis (CEKA); NSF; DOE [NSF CHE-0431328]; respective facilities divisions of the Advanced Scientific Computing Research; Basic Energy Sciences of the U.S. Department of Energy FX This work was made possible by National Science Foundation Grants EAR07-45374, EAR11-47728 and by the Center for Environmental Kinetics Analysis (CEKA), an NSF- and DOE-sponsored Environmental Molecular Science Institute (NSF CHE-0431328). This research used resources of the National Energy Research Scientific Computing Center, National Center for Computational Sciences, and the Center for Nanophase Materials Sciences, which are sponsored by the respective facilities divisions of the Advanced Scientific Computing Research and Basic Energy Sciences of the U.S. Department of Energy. We also thank Andrei Bandura and Jorge Sofo for their assistance with the GULP and VASP calculations utilized in this study. NR 38 TC 5 Z9 5 U1 1 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 12 PY 2013 VL 117 IS 49 BP 26084 EP 26090 DI 10.1021/jp408345v PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 273IZ UT WOS:000328529800026 ER PT J AU Ugeda, MM Yu, M Bradley, AJ Doak, P Liu, WJ Moore, GF Sharp, ID Tilley, TD Neaton, JB Crommie, MF AF Ugeda, Miguel M. Yu, Min Bradley, Aaron J. Doak, Peter Liu, Wenjun Moore, Gary F. Sharp, Ian D. Tilley, T. D. Neaton, Jeffrey B. Crommie, Michael F. TI Adsorption and Stability of pi-Bonded Ethylene on GaP(110) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; AUGMENTED-WAVE METHOD; III-V SEMICONDUCTORS; 110 SURFACES; ELECTRONIC-PROPERTIES; DECOMPOSITION; SPECTROSCOPY; GAAS AB We have investigated the structural and electronic properties of individual ethylene molecules on the GaP(110) surface by combining low-temperature scanning tunneling microscopy and spectroscopy (LT-STM/STS) with density functional theory (DFT) calculations. Isolated molecules were adsorbed on in situ cleaved GaP(110) surfaces through ethylene exposures at 300 K and 15 K. DFT calculations suggest two possible stable adsorption geometries for a single ethylene molecule on GaP(110) at low temperature. High-resolution STM images, however, reveal only one adsorption geometry for this system, consistent with the site having the largest computed binding energy. Unlike adsorption of ethylene on other metallic and semiconducting surfaces, ethylene physisorbs to GaP(110) through a weak hybridization of molecular pi-states with substrate surface states, leaving the frontier molecular orbitals largely unperturbed. Differential conductivity spectra acquired on single molecules are consistent with self-energy corrected DFT calculations. C1 [Ugeda, Miguel M.; Bradley, Aaron J.; Crommie, Michael F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ugeda, Miguel M.; Yu, Min; Liu, Wenjun; Moore, Gary F.; Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.; Crommie, Michael F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Yu, Min; Doak, Peter; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Doak, Peter; Liu, Wenjun; Tilley, T. D.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Ugeda, MM (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM mmorenougeda@lbl.gov; crommie@berkeley.edu RI Liu, Wenjun/J-8679-2012; Sharp, Ian/I-6163-2015; Doak, Peter/A-1910-2016; Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014; Moore, Gary/L-6828-2016; Moreno Ugeda, Miguel/N-3006-2016 OI Sharp, Ian/0000-0001-5238-7487; Doak, Peter/0000-0001-6039-9752; Neaton, Jeffrey/0000-0001-7585-6135; Moore, Gary/0000-0003-3369-9308; FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. A.J.B. was supported by the Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We are grateful to J. I. Pascual for fruitful discussions. Experimental data and simulated STM images were analyzed and rendered using WSxM software.35 NR 34 TC 2 Z9 2 U1 0 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 12 PY 2013 VL 117 IS 49 BP 26091 EP 26096 DI 10.1021/jp408539x PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 273IZ UT WOS:000328529800027 ER PT J AU Zhang, L Cole, JM Liu, XG AF Zhang, Lei Cole, Jacqueline M. Liu, Xiaogang TI Tuning Solvatochromism of Azo Dyes with Intramolecular Hydrogen Bonding in Solution and on Titanium Dioxide Nanoparticles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SENSITIZED SOLAR-CELLS; NONLINEAR-OPTICAL MATERIALS; QUANTUM-CHEMICAL CALCULATIONS; HYDRAZONE TAUTOMERISM; MOLECULAR-ORIGINS; OPTOELECTRONIC PROPERTIES; ABSORPTION; NMR; PHOTOISOMERIZATION; SPECTROSCOPY AB "Smart tuning" of optical properties in three azo dyes containing intramolecular hydrogen bonding is realized by the judicious control of solvents, when the dyes are in solution or adsorbed onto titanium dioxide nanoparticles. In solution, certain solvents destabilizing intramolecular hydrogen bonding induce a distinctive approximate to 70 nm "blue-shifted" absorption peak, compared with other solvents. In parallel, the optical properties of azo dye/TiO2 nanocomposites can be tuned using solvents with different hydrogen-bond accepting/donating abilities, giving insights into smart materials and dye-sensitized solar cell device design. It is proposed that intramolecular hydrogen bonding alone plays the leading role in such phenomena, which is fundamentally different to other mechanisms, such as tautomerism and cis-trans isomerization, that explain the optical control of azo dyes. Hybrid density functional theory (DFT) is employed in order to trace the origin of this optical control, and these calculations support the mechanism involving intramolecular hydrogen bonding. Two complementary studies are also reported: H-1 NMR spectroscopy is conducted in order to further understand the solvent effects on intramolecular hydrogen bonding; crystal structure analysis from associated research indicates the importance of intramolecular hydrogen bonding on intramolecular charge transfer. C1 [Zhang, Lei; Cole, Jacqueline M.; Liu, Xiaogang] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Cole, Jacqueline M.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Cole, JM (reprint author), Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England. EM jmc61@cam.ac.uk RI Cole, Jacqueline/C-5991-2008; Liu, Xiaogang/H-2189-2011; OI Liu, Xiaogang/0000-0002-2553-2068; Zhang, Lei/0000-0001-6873-7314 FU Fulbright Commission; DOE Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; EPSRC U.K.; Singapore Economic Development Board FX J.M.C. thanks the Fulbright Commission for a UK-US Fulbright Scholar Award and Argonne National Laboratory where work done was supported by DOE Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. X.L. is indebted to the Singapore Economic Development Board for a Clean Energy Scholarship. The authors acknowledge support from the EPSRC U.K. National Service for Computational Chemistry Software (NSCCS), based at Imperial College London, and contributions from its staff in assisting with this work. The authors also thank Chi Hu for her technical assistance in NMR experiments. NR 53 TC 7 Z9 7 U1 2 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 12 PY 2013 VL 117 IS 49 BP 26316 EP 26323 DI 10.1021/jp4088783 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 273IZ UT WOS:000328529800051 ER PT J AU Bisset, RN Ticknor, C Blakie, PB AF Bisset, R. N. Ticknor, C. Blakie, P. B. TI Finite-resolution fluctuation measurements of a trapped Bose-Einstein condensate SO PHYSICAL REVIEW A LA English DT Article ID PARTICLE FLUCTUATIONS; COHERENCE; GAS AB We consider the fluctuations in atom number that occur within finite-sized measurement cells in a trapped Bose-Einstein condensate. These approximate the fluctuation measurements made in current experiments with finite-resolution in situ imaging. A numerical scheme is developed to calculate these fluctuations using the quasiparticle modes of a cylindrically symmetric three-dimensionally trapped condensate with either contact or dipole-dipole interactions. We use this scheme to study the properties of a pancake-shaped condensate using cylindrical cells. The extension of the theory to washer-shaped cells with azimuthal weighting ismade and used to discriminate between the low-energy roton modes in a dipolar condensate according to their projection of angular momentum. Our results are based on the Bogoliubov approach valid for zero and small finite temperatures. C1 [Bisset, R. N.; Blakie, P. B.] Univ Otago, Dept Phys, Jack Dodd Ctr Quantum Technol, Dunedin, New Zealand. [Bisset, R. N.; Ticknor, C.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Bisset, R. N.; Ticknor, C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Bisset, RN (reprint author), Univ Otago, Dept Phys, Jack Dodd Ctr Quantum Technol, Dunedin, New Zealand. RI Ticknor, Christopher/B-8651-2014; Blakie, Peter/A-1554-2009; Bisset, Russell/H-1750-2012; OI Blakie, Peter/0000-0003-4772-6514; Ticknor, Christopher/0000-0001-9972-4524 FU Marsden Fund of New Zealand [UOO1220]; CNLS; LDRD; U.S. DOE [DE-AC52-06NA25396] FX We acknowledge fruitful discussions with J. Armijo. P.B.B. and R.N.B. acknowledge support by the Marsden Fund of New Zealand (Contract No. UOO1220). R.N.B. and C.T. acknowledge support from CNLS, LDRD, and LANL, which is operated by LANS, LLC for the NNSA of the U.S. DOE (Contract No. DE-AC52-06NA25396). NR 57 TC 1 Z9 1 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD DEC 12 PY 2013 VL 88 IS 6 AR 063624 DI 10.1103/PhysRevA.88.063624 PG 10 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 275JX UT WOS:000328673200008 ER PT J AU Grutter, AJ Wong, FJ Jenkins, CA Arenholz, E Vailionis, A Suzuki, Y AF Grutter, A. J. Wong, F. J. Jenkins, C. A. Arenholz, E. Vailionis, A. Suzuki, Y. TI Stabilization of spin-zero Ru4+ through epitaxial strain in SrRuO3 thin films SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC-STRUCTURE; MAGNETIC-PROPERTIES; SINGLE-CRYSTAL AB We report the stabilization of a nonmagnetic spin-zero state of Ru4+ in SrRuO3 thin films under tensile strain, resulting in suppression of the saturation magnetization relative to bulk. The magnitude of suppression as a function of strain magnitude agrees well with density functional theory predictions of the magnetic ground state of (100) oriented films. In addition to the (100) orientation, we report on the effects of tensile strain on the magnetic properties of (110) and (111) oriented SrRuO3 thin films. All films show reduced saturation magnetization as well as enhancement of the Curie temperature, a universal in-plane magnetic easy axis, and anisotropy of the saturation magnetization. Films of all orientations exhibit characteristics of a magnetic easy axis as well as higher saturation magnetizations when magnetized in the film plane rather than along the film normal. We show that all of these effects can be attributed to the tensile strain induced by growth on KTaO3 substrates and explain them in terms of an anisotropic modification of the crystal field. C1 [Grutter, A. J.; Wong, F. J.; Suzuki, Y.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Grutter, A. J.; Suzuki, Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Grutter, A. J.; Vailionis, A.; Suzuki, Y.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Jenkins, C. A.; Arenholz, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Vailionis, A.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. RP Grutter, AJ (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RI Vailionis, Arturas/C-5202-2008 OI Vailionis, Arturas/0000-0001-5878-1864 FU Office of Science, Office of Basic Energy Sciences, US Department of Energy (DOE) [DE-SC0008505, DE-AC02-05CH11231]; Army Research Office [MURI W911NF-08-1-0317] FX We would like to thank K. M. Yu for assistance with Rutherford backscattering spectrometry measurements as well as J. Rondinelli and N. Spaldin for fruitful discussions. This work and the Advanced Light Source are supported by the Director, Office of Science, Office of Basic Energy Sciences, US Department of Energy (DOE) (Grants No. DE-SC0008505 and No. DE-AC02-05CH11231). F.J.W. is supported by the Army Research Office under Grant No. MURI W911NF-08-1-0317. NR 19 TC 6 Z9 6 U1 1 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 12 PY 2013 VL 88 IS 21 AR 214410 DI 10.1103/PhysRevB.88.214410 PG 5 WC Physics, Condensed Matter SC Physics GA 275MJ UT WOS:000328680800001 ER PT J AU Fotiades, N Cizewski, JA Higashiyama, K Yoshinaga, N Teruya, E Krucken, R Clark, RM Fallon, P Lee, IY Macchiavelli, AO Younes, W AF Fotiades, N. Cizewski, J. A. Higashiyama, K. Yoshinaga, N. Teruya, E. Kruecken, R. Clark, R. M. Fallon, P. Lee, I. Y. Macchiavelli, A. O. Younes, W. TI Medium-spin states in Cs-135 SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; S-PROCESS; EXCITATIONS; ISOTOPES AB Limited information is currently known on medium-and higher-spin states for Cs-135, a neutron-rich nucleus amenable to shell-model calculations due to its proximity to the shell closures in Sn-132. In order to extend the level structure of Cs-135 to higher excitations, this nucleus was studied via prompt gamma-ray spectroscopy of fragments following the fission of the compound nucleus Th-226 formed in the O-18 (91 MeV) + Pb-208 fusion-fission reaction. Medium-spin states up to spin (23/2) and similar to 3.3 MeV excitation energy have been established. The observed states were compared with those in the neighboring N = 82(137)Cs nucleus, as well as with states in the neighboring N = 80 isotones. The coupling of the odd proton occupying the g(7/2) orbital to the yrast states in the Xe-134 and Ba-136 cores could account for the lower excited states of Cs-135. The experimental results are compared with predictions from shell-model calculations. C1 [Fotiades, N.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Cizewski, J. A.] Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. [Higashiyama, K.] Chiba Inst Technol, Dept Phys, Narashino, Chiba 2750023, Japan. [Yoshinaga, N.; Teruya, E.] Saitama Univ, Dept Phys, Saitama 3388570, Japan. [Kruecken, R.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Younes, W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Fotiades, N (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM fotia@lanl.gov RI Kruecken, Reiner/A-1640-2013; OI Kruecken, Reiner/0000-0002-2755-8042; Fotiadis, Nikolaos/0000-0003-1410-3871 FU U.S. Department of Energy [DE-AC52-06NA25396, DE-AC52-07NA27344, AC03-76SF00098]; National Science Foundation (Rutgers); Japan Society for the Promotion of Science [24540251, 25400267] FX This work has been supported in part by the U.S. Department of Energy under Contracts No. DE-AC52-06NA25396 (LANL), No. DE-AC52-07NA27344 (LLNL), and No. AC03-76SF00098 (LBNL), by the National Science Foundation (Rutgers), and by the Japan Society for the Promotion of Science under grants in aid for scientific research No. 24540251 and No. 25400267. NR 35 TC 2 Z9 2 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD DEC 12 PY 2013 VL 88 IS 6 AR 064315 DI 10.1103/PhysRevC.88.064315 PG 5 WC Physics, Nuclear SC Physics GA 275PO UT WOS:000328689500002 ER PT J AU Brown, CM Ramirez-Cuesta, AJ Johnson, MR Garcia-Sakai, V AF Brown, Craig M. Ramirez-Cuesta, Anibal (Timmy) J. Johnson, Mark R. Garcia-Sakai, Victoria TI Chemical spectroscopy using neutrons Preface SO CHEMICAL PHYSICS LA English DT Editorial Material ID MOLECULAR VIBRATIONS; COMPTON-SCATTERING; INELASTIC-SCATTERING; SPECTRUM; HYDROGEN; DYNAMICS; CARBON; STATES; INS C1 [Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Ramirez-Cuesta, Anibal (Timmy) J.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Johnson, Mark R.] Inst Max Von Laue Paul Langevin, F-38042 Grenoble, France. [Garcia-Sakai, Victoria] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. RP Brown, CM (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. RI Brown, Craig/B-5430-2009; Ramirez-Cuesta, Timmy/A-4296-2010 OI Brown, Craig/0000-0002-9637-9355; Ramirez-Cuesta, Timmy/0000-0003-1231-0068 NR 33 TC 1 Z9 1 U1 2 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD DEC 12 PY 2013 VL 427 BP 1 EP 2 DI 10.1016/j.chemphys.2013.11.009 PG 2 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262YN UT WOS:000327773900001 ER PT J AU Brown, CM Ramirez-Cuesta, AJ Her, JH Wheatley, PS Morris, RE AF Brown, Craig M. Ramirez-Cuesta, Anibal Javier Her, Jae-Hyuk Wheatley, Paul S. Morris, Russell E. TI Structure and spectroscopy of hydrogen adsorbed in a nickel metal-organic framework SO CHEMICAL PHYSICS LA English DT Article DE Neutron scattering; Hydrogen storage; Metal-organic framework; Porous crystal ID NEUTRON POWDER DIFFRACTION; HIGH H-2 ADSORPTION; COORDINATION POLYMER; STORAGE; SITES; SCATTERING; CENTERS; SORPTION; BINDING; MOF-74 AB The structure of Ni-2(dobdc) (dobdc(4) = 2,5-dioxido-1,4-benzenedicarboxylate) as a function of deuterium adsorption has been determined through the application of in situ neutron powder diffraction. Detailed information concerning the local adsorption potential for hydrogen at each site has also been probed using inelastic neutron scattering techniques. These results are compared to those previously published on isostructural analogs and the Ni2+ variant shows the shortest deuterium-metal distance in the M-2(dobdc) series (M = Mg, Zn, Co, Fe) that have been studied so far. Published by Elsevier B.V. C1 [Brown, Craig M.; Her, Jae-Hyuk] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Brown, Craig M.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. [Ramirez-Cuesta, Anibal Javier] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Her, Jae-Hyuk] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Wheatley, Paul S.; Morris, Russell E.] Univ St Andrews, EaStCHEM Sch Chem, St Andrews KY16 9ST, Fife, Scotland. RP Brown, CM (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM craig.brown@nist.gov RI Brown, Craig/B-5430-2009; Morris, Russell/G-4285-2010; Ramirez-Cuesta, Timmy/A-4296-2010 OI Brown, Craig/0000-0002-9637-9355; Morris, Russell/0000-0001-7809-0315; Ramirez-Cuesta, Timmy/0000-0003-1231-0068 FU Office of Energy Efficiency and Renewable Energy (EERE) through the Hydrogen and Fuel Cells Program; EPSRC [EP/K005499/1, EP/K025112/1] FX This research was partially supported by the Office of Energy Efficiency and Renewable Energy (EERE) through the Hydrogen and Fuel Cells Program. We thank Dr. Y. Liu for experimental assistance at NIST and M. Kibble and C. Goodway from ISIS for their help in gas loading experiments performed on TOSCA. REM thanks the EPSRC for funding (EP/K005499/1 and EP/K025112/1). REM is also a Royal Society Industry Fellow. NR 47 TC 10 Z9 10 U1 0 U2 45 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD DEC 12 PY 2013 VL 427 BP 3 EP 8 DI 10.1016/j.chemphys.2013.08.010 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262YN UT WOS:000327773900002 ER PT J AU Gremaud, R Zuttel, A Borgschulte, A Ramirez-Cuesta, AJ Refson, K Colognesi, D AF Gremaud, R. Zuettel, A. Borgschulte, A. Ramirez-Cuesta, A. J. Refson, K. Colognesi, D. TI Origin of the large anharmonicity in the phonon modes of LiBH4 SO CHEMICAL PHYSICS LA English DT Article DE Inelastic neutron scattering; Raman spectroscopy; Infrared spectroscopy; Complex hydride; Anharmonicity; Density functional theory ID INELASTIC NEUTRON-SCATTERING; HYDROGEN-STORAGE MATERIALS; RAMAN-SPECTROSCOPY; LIBRON; BOROHYDRIDES AB The dynamics and bonding of the complex hydride LiBH4 have been investigated by vibrational spectroscopy and density functional theory (DFT). The combination of infrared, Raman, and inelastic neutron-scattering (INS) spectroscopies on hydrided and deuterated samples reveals a complete picture of the dynamics of the BH4 ions as well as of the lattice. Particular emphasis is laid on a comparison between experiment and theory, revealing significant discrepancy between the two approaches for vibrations with high anharmonicity, which is related to large vibrational amplitudes. The latter is typical for librational modes in molecular crystals and pseudo-ionic crystals such as complex hydrides. The presented strategy for anharmonic frequency corrections might thus be generally applicable for this kind of materials. (C) 2013 Elsevier B. V. All rights reserved. C1 [Gremaud, R.; Zuettel, A.; Borgschulte, A.] Empa, Swiss Fed Labs Mat Sci & Technol, Lab Hydrogen & Energy 505, CH-8600 Dubendorf, Switzerland. [Ramirez-Cuesta, A. J.; Refson, K.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN USA. [Colognesi, D.] CNR, Sez Firenze, Ist Sistemi Complessi, I-50019 Sesto Fiorentino, FI, Italy. RP Borgschulte, A (reprint author), Empa, Swiss Fed Labs Mat Sci & Technol, Lab Hydrogen & Energy 505, Uberlandstr 129, CH-8600 Dubendorf, Switzerland. EM andreas.borgschulte@empa.ch RI Ramirez-Cuesta, Timmy/A-4296-2010; Borgschulte, Andreas/D-5168-2016; OI Ramirez-Cuesta, Timmy/0000-0003-1231-0068; Borgschulte, Andreas/0000-0001-6250-4667; Refson, Keith/0000-0002-8715-5835 FU Swiss federal office for Energy via the CompHy project; Swiss federal office for Energy via the ACH project; European Commission [FP7-284522] FX This work was financially supported by the Swiss federal office for Energy via the CompHy and ACH projects and by the European Commission, Grant agreement No. FP7-284522 (infrastructure program H2FC). Computing resources provided by the UK e-Science Centre, STFC (SCARF) are gratefully acknowledged. NR 42 TC 2 Z9 2 U1 1 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD DEC 12 PY 2013 VL 427 BP 22 EP 29 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262YN UT WOS:000327773900005 ER PT J AU Ogilvie, AD Makepeace, JW Hore, K Ramirez-Cuesta, AJ Apperley, DC Mitchels, JM Edwards, PP Sartbaeva, A AF Ogilvie, Alexander D. Makepeace, Joshua W. Hore, Katie Ramirez-Cuesta, Anibal J. Apperley, David C. Mitchels, John M. Edwards, Peter P. Sartbaeva, Asel TI Catalyst-free synthesis of sodium amide nanoparticles encapsulated in silica gel SO CHEMICAL PHYSICS LA English DT Article DE Sodium amide; Encapsulation; Nanoparticle; Inelastic neutron spectroscopy; INS ID ALKALI-METALS AB Crystalline sodium amide nanoparticles encapsulated in an amorphous silica framework were formed by ammoniation of a precursor material, silica gel loaded with metallic sodium, under mild conditions and without catalysis. This ammoniation was performed in situ on TOSCA beamline at ISIS, RAL, using anhydrous gaseous ammonia. The resulting material exhibits no pyrophoricity and much reduced air- and moisture-sensitivity compared to the bulk amide. The nanoparticles formed will offer a greatly increased surface area for chemical reactions where amide is currently used as an important ingredient for industrial applications. We anticipate that this method of sodium amide production will have a diversity of applications. (C) 2013 Elsevier B. V. All rights reserved. C1 [Ogilvie, Alexander D.; Makepeace, Joshua W.; Hore, Katie; Edwards, Peter P.] Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England. [Apperley, David C.] Univ Durham, Dept Chem, EPSRC UK Natl Solid State NMR Serv, Durham DH1 3LE, England. [Ramirez-Cuesta, Anibal J.] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Ramirez-Cuesta, Anibal J.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN USA. [Mitchels, John M.] Univ Bath, Bath BA2 7AY, Avon, England. [Sartbaeva, Asel] Univ Bath, Dept Chem, Bath BA2 7AY, Avon, England. RP Ogilvie, AD (reprint author), Univ Oxford, Inorgan Chem Lab, S Parks Rd, Oxford OX1 3QR, England. EM alexander.ogilvie@chem.oxon.org; josh.make-peace@chem.ox.ac.uk; katie.hore@chem.ox.ac.uk; tim-my.ramirez-cuesta@stfc.ac.uk; d.c.apperley@dur.ac.uk; J.M.Mitchels@bath.ac.uk; peter.edwards@chem.ox.ac.uk; a.sartbaeva@bath.ac.uk RI Ramirez-Cuesta, Timmy/A-4296-2010; OI Ramirez-Cuesta, Timmy/0000-0003-1231-0068; Makepeace, Joshua/0000-0002-7107-0845 FU Royal Society FX We would like to acknowledge Dr S. Rudic for help with INS data collection. We thank the STFC for beamtime at ISIS (RAL), National Solid-state NMR Service at Durham University for SS-NMR data, and Microscopy and Analysis Suite Service (MAS) at the University of Bath for TEM data and Dr P. Manuel and Dr D. Khalyavin for collecting neutron diffraction data on WISH at ISIS. Dr A. Sartbaeva would like to thank the Royal Society for funding. NR 23 TC 0 Z9 0 U1 3 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD DEC 12 PY 2013 VL 427 BP 61 EP 65 DI 10.1016/j.chemphys.2013.06.003 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262YN UT WOS:000327773900011 ER PT J AU White, CE Kearley, GJ Provis, JL Riley, DP AF White, Claire E. Kearley, Gordon J. Provis, John L. Riley, Daniel P. TI Inelastic neutron scattering analysis of the thermal decomposition of kaolinite to metakaolin SO CHEMICAL PHYSICS LA English DT Article DE Inelastic neutron scattering; Kaolinite dehydroxylation; Metakaolin; Hydrogen atom dynamics ID RIETVELD REFINEMENT; KINETIC-ANALYSIS; DEHYDROXYLATION; DICKITE; MULLITE; 1ST-PRINCIPLES; ORIENTATION; MECHANISM; DYNAMICS; NACRITE AB Understanding the formation of metakaolin via kaolinite dehydroxylation is extremely important for the optimization of various industrial processes. Recent investigations have reported that the different types of hydrogen atoms in kaolinite are removed concurrently during the dehydroxylation process. Here, inelastic neutron scattering (INS) is used to analyze the location and dynamics of hydrogen atoms in kaolinite, together with the changes induced during dehydroxylation. This is achieved by using prior knowledge of how the inner and inner surface hydrogen atoms contribute to the kaolinite INS spectrum in the 200-1200 cm(-1) range, in combination with a semi-quantitative analysis of the experimental INS spectra. Overall, it is seen that there is a distinct preferential loss of inner surface hydrogen-atom types during the dehydroxylation process, as determined from analysis of the Al-O-H vibrational modes (consisting of deformation and torsion) in the INS spectrum. (C) 2013 Elsevier B. V. All rights reserved. C1 [White, Claire E.] Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [White, Claire E.] Los Alamos Natl Lab, Los Alamos, NM USA. [White, Claire E.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [White, Claire E.; Provis, John L.] Univ Melbourne, Dept Chem & Biomol Engn, Parkville, Vic 3052, Australia. [Kearley, Gordon J.] Australian Nucl Sci & Technol Org, Bragg Inst, Lucas Heights, Australia. [Provis, John L.] Univ Sheffield, Dept Mat Sci & Engn, Sheffield, S Yorkshire, England. [Riley, Daniel P.] Australian Nucl Sci & Technol Org, Inst Mat Engn, Lucas Heights, Australia. [Riley, Daniel P.] Univ Melbourne, Dept Mech Engn, Parkville, Vic 3052, Australia. RP White, CE (reprint author), Princeton Univ, Dept Civil & Environm Engn, Andlinger Ctr Energy & Environm, Princeton, NJ 08544 USA. EM whitece@princeton.edu RI White, Claire/A-1722-2011; OI White, Claire/0000-0002-4800-7960; Provis, John/0000-0003-3372-8922 FU DOE [DE-AC52-06NA25396]; U.S. Department of Energy through the LANL/LDRD Program; Australian Research Council (ARC) via the Particulate Fluids Processing Centre, a Special Research Centre of the ARC; Centre for Sustainable Resource Processing via the Geopolymer Alliance; ANSTO Access to Major Research Facilities Program FX The authors would like to thank Dr. Stewart Parker and Dr. Timmy Ramirez-Cuesta for assistance with sample loading, data acquisition and data reduction on TOSCA at ISIS, Rutherford Appleton Laboratory, UK. The participation of CEW in this work was supported by Los Alamos National Laboratory, which is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. Furthermore, CEW gratefully acknowledges the support of the U.S. Department of Energy through the LANL/LDRD Program. This work was funded in part by the Australian Research Council (ARC) (including some funding via the Particulate Fluids Processing Centre, a Special Research Centre of the ARC), and in part by a studentship paid to Claire White by the Centre for Sustainable Resource Processing via the Geopolymer Alliance. Travel funding for the experiments at ISIS was provided through the ANSTO Access to Major Research Facilities Program. NR 33 TC 4 Z9 4 U1 2 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD DEC 12 PY 2013 VL 427 BP 82 EP 86 DI 10.1016/j.chemphys.2013.08.009 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262YN UT WOS:000327773900014 ER PT J AU Hartl, M Daemen, L Hartl, H Brudgam, I Eckert, J AF Hartl, Monika Daemen, Luke Hartl, Hans Bruedgam, Irene Eckert, Juergen TI Short hydrogen bonds in 2,4-dinitrobenzoic acid complexed with pyridine SO CHEMICAL PHYSICS LA English DT Article DE Short hydrogen bonds; Single crystal XRD; FT-IR; IINS; DFT ID INELASTIC NEUTRON-SCATTERING; N-OXIDE; DISSOCIATION-CONSTANTS; COMPUTATIONAL APPROACH; LOW-TEMPERATURE; X-RAY; DYNAMICS; CRYSTAL; DIFFRACTION; IR AB The aim of this work was to describe the vibrations connected with the short hydrogen bonds of differing geometries in 2,4-dinitrobenzoic acid and in 2,4-dinitrobenzoic acid complexed in two ratios with pyridine. All three compounds contain short hydrogen bonds either between two acid molecules (OH center dot center dot center dot O bond) or between acid and pyridine (NH center dot center dot center dot O bonds) or both. We selectively deuterated the proton of the 2,4-dinitrobenzoic acid molecule involved in the proton transfer to aid in the assignment of the H-bond protonic modes. The compounds have been characterized with single crystal X-ray diffraction, CHN elemental analysis, FT-IR and IINS spectroscopy. We show that our combination of analytical methods with DFT calculations represents a fruitful approach to observe the relationship between the geometries of hydrogen bonds and their dynamics. Published by Elsevier B.V. C1 [Hartl, Monika; Daemen, Luke] Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Hartl, Hans; Bruedgam, Irene] Free Univ Berlin, Inst Chem & Biochem, D-14195 Berlin, Germany. [Eckert, Juergen] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. RP Hartl, M (reprint author), Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA. EM hartl@lanl.gov RI Hartl, Monika/F-3094-2014; Hartl, Monika/N-4586-2016 OI Hartl, Monika/0000-0002-6601-7273; Hartl, Monika/0000-0002-6601-7273 FU DOE [DE-AC52-06NA25396] FX This work has benefitted from the use of the Manuel Lujan, Jr. Neutron Scattering Center at Los Alamos National Laboratory, which is funded by the Department of Energys Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. NR 26 TC 0 Z9 0 U1 1 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD DEC 12 PY 2013 VL 427 BP 87 EP 94 DI 10.1016/j.chemphys.2013.10.016 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 262YN UT WOS:000327773900015 ER PT J AU Zhang, YB Wong, CH Birnbaum, RY Li, GL Favaro, R Ngan, CY Lim, J Tai, E Poh, HM Wong, E Mulawadi, FH Sung, WK Nicolis, S Ahituv, N Ruan, YJ Wei, CL AF Zhang, Yubo Wong, Chee-Hong Birnbaum, Ramon Y. Li, Guoliang Favaro, Rebecca Ngan, Chew Yee Lim, Joanne Tai, Eunice Poh, Huay Mei Wong, Eleanor Mulawadi, Fabianus Hendriyan Sung, Wing-Kin Nicolis, Silvia Ahituv, Nadav Ruan, Yijun Wei, Chia-Lin TI Chromatin connectivity maps reveal dynamic promoter-enhancer long-range associations SO NATURE LA English DT Article ID NEURAL STEM-CELLS; REGULATORY SEQUENCES; GENE-EXPRESSION; MOUSE; PLURIPOTENT; INTERACTOME; VERTEBRATE; CIRCUITRY; GENOME AB In multicellular organisms, transcription regulation is one of the central mechanisms modelling lineage differentiation and cell-fate determination(1). Transcription requires dynamic chromatin configurations between promoters and their corresponding distal regulatory elements(2). It is believed that their communication occurs within large discrete foci of aggregated RNA polymerases termed transcription factories in three-dimensional nuclear space(3). However, the dynamic nature of chromatin connectivity has not been characterized at the genome-wide level. Here, through a chromatin interaction analysis with paired-end tagging approach(3-5) using an antibody that primarily recognizes the pre-initiation complexes of RNA polymerase II6, we explore the transcriptional interactomes of three mouse cells of progressive lineage commitment, including pluripotent embryonic stem cells(7), neural stem cells(8) and neurosphere stem/progenitor cells(9). Our global chromatin connectivity maps reveal approximately 40,000 long-range interactions, suggest precise enhancer-promoter associations and delineate cell-type-specific chromatin structures. Analysis of the complex regulatory repertoire shows that there are extensive colocalizations among promoters and distal-acting enhancers. Most of the enhancers associate with promoters located beyond their nearest active genes, indicating that the linear juxtaposition is not the only guiding principle driving enhancer target selection. Although promoter-enhancer interactions exhibit high cell-type specificity, promoters involved in interactions are found to be generally common and mostly active among different cells. Chromatin connectivity networks reveal that the pivotal genes of reprogramming functions are transcribed within physical proximity to each other in embryonic stem cells, linking chromatin architecture to coordinated gene expression. Our study sets the stage for the full-scale dissection of spatial and temporal genome structures and their roles in orchestrating development. C1 [Zhang, Yubo; Wong, Chee-Hong; Ngan, Chew Yee; Wei, Chia-Lin] Lawrence Berkeley Natl Lab, Joint Genome Inst, Sequencing Technol Grp, Walnut Creek, CA 94598 USA. [Birnbaum, Ramon Y.; Ahituv, Nadav] UCSF, Inst Human Genet, Dept Bioengn & Therapeut Sci, San Francisco, CA 94158 USA. [Li, Guoliang; Ruan, Yijun] Univ Connecticut, Jackson Lab Genom Med, Farmington, CT 06030 USA. [Li, Guoliang; Ruan, Yijun] Univ Connecticut, Dept Genet & Dev Biol, Farmington, CT 06030 USA. [Li, Guoliang; Lim, Joanne; Tai, Eunice; Poh, Huay Mei; Wong, Eleanor; Mulawadi, Fabianus Hendriyan; Sung, Wing-Kin; Wei, Chia-Lin] Genome Inst Singapore, Singapore 138672, Singapore. [Favaro, Rebecca; Nicolis, Silvia] Univ Milano Bicocca, Dept Biol Sci & Biotechnol, I-20126 Milan, Italy. RP Wei, CL (reprint author), Lawrence Berkeley Natl Lab, Joint Genome Inst, Sequencing Technol Grp, Walnut Creek, CA 94598 USA. EM cwei@lbl.gov OI Favaro, Rebecca/0000-0002-6195-5711; Ahituv, Nadav/0000-0002-7434-8144 FU ASTIL Regione Lombardia (SAL-19) [16874]; Telethon [GGP12152]; Cariplo [2010-0673]; AIRC [IG-5801]; NINDS [R01NS079231]; NICHD [R01HD059862]; NHGRI [R01HG005058, R01HG006768]; NIDDK [R01DK090382]; NIGMS [GM61390]; Simons Foundation SFARI [256769]; UCSF Program for Biomedical Breakthrough Research (PBBR); Agency for Science, Technology and Research (A*STAR), Singapore; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; National Institutes of Health ENCODE [R01 HG004456-01, R01HG003521-01, 1U54HG004557-01] FX The authors thank J. Mariani for the preparation of RNA from NPC; K. Murphy and A. Ku for their assistance with zebrafish enhancer assays; and A. Visel and A. Nord for discussion and their comments on the manuscript. S.N. and R. F. were supported by grants from ASTIL Regione Lombardia (SAL-19 ref. no. 16874), Telethon (GGP12152), Cariplo (Rif. 2010-0673) and AIRC (IG-5801). N.A. is supported by NINDS grant number R01NS079231, NICHD grant number R01HD059862, NHGRI grant numbers R01HG005058 and R01HG006768, NIDDK award number R01DK090382, NIGMS award number GM61390 and Simons Foundation SFARI no. 256769. R.Y.B. is supported by NINDS grant number R01NS079231 and the UCSF Program for Biomedical Breakthrough Research (PBBR). This work was supported by Agency for Science, Technology and Research (A*STAR), Singapore, the Office of Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231 and National Institutes of Health ENCODE grants (R01 HG004456-01, R01HG003521-01 and 1U54HG004557-01) to Y.R. and C.-L.W. NR 30 TC 138 Z9 141 U1 8 U2 56 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD DEC 12 PY 2013 VL 504 IS 7479 BP 306 EP + DI 10.1038/nature12716 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 267TQ UT WOS:000328121500042 PM 24213634 ER PT J AU Reyes-Gil, KR Robinson, DB AF Reyes-Gil, Karla R. Robinson, David B. TI WO3-Enhanced TiO2 Nanotube Photoanodes for Solar Water Splitting with Simultaneous Wastewater Treatment SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE TiO2 nanotubes; WO3; photodegradation; water splitting H-2 production; water pollutants ID ENHANCED ELECTROCHROMIC PROPERTIES; VISIBLE-LIGHT ILLUMINATION; TUNGSTEN TRIOXIDE FILMS; PHOTOCATALYTIC ACTIVITY; ENERGY-CONVERSION; WO3 FILMS; ARRAYS; ELECTRODEPOSITION; TEMPERATURE; ULTRAVIOLET AB Composite WO3/TiO2 nanostructures with optimal properties that enhance solar photoconversion reactions were developed, characterized, and tested. The TiO2 nanotubes were prepared by anodization of Ti foil and used as substrates for WO3 electrodeposition. The WO3 electrodeposition parameters were controlled to develop unique WO3 nanostructures with enhanced photoelectrochemical properties. Scanning electron microscopy (SEM) images showed that the nanomaterials with optimal photocurrent density have the same ordered structure as TiO2 nanotubes, with an external tubular nanostnictured WO3 layer. Diffuse reflectance spectra showed an increase in the visible absorption relative to bare TiO2 nanotubes and in the UV absorption relative to bare WO3 films. Incident simulated solar photon-to-current efficiency (IPCE) increased from 30% (for bare WO3) to 50% (for tubular WO3/TiO2 composites). With the addition of diverse organic pollutants, the photocurrent densities exhibited more than a 5-fold increase. Chemical oxygen demand measurements showed the simultaneous photodegradation of organic pollutants. The results of this work showed that the unique structure and composition of these composite WO3/TiO2 materials enhance the IPCE efficiencies, optical properties, and photodegradation performance compared with the parent materials. C1 [Reyes-Gil, Karla R.; Robinson, David B.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Reyes-Gil, KR (reprint author), Sandia Natl Labs, POB 969, Livermore, CA 94551 USA. EM krreyes@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Early Career Laboratory Directed Research and Development program at Sandia National Laboratories FX The authors thank Zachary D. Stephens for his technical work during the summer 2012, Dr. Vitalie Stavila for his valuable help in the XRD data collection, and Jeffery M. Chames for the SEM and EDS data collection. The authors also want to thank Brian Patterson, Paul Schrader, and Dr. John Goldsmith for their contribution in the instrumental setup for IPCE measurements. This work was funded by the Early Career Laboratory Directed Research and Development program at Sandia National Laboratories, a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 35 TC 32 Z9 35 U1 8 U2 126 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD DEC 11 PY 2013 VL 5 IS 23 BP 12400 EP 12410 DI 10.1021/am403369p PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 272DD UT WOS:000328439600026 PM 24195676 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaitia, Y Acharya, BS Adamczyka, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Artamonov, A Artoni, G Arutinov, D Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, 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Wrona, B. Wu, S. L. Wu, X. Wu, Y. Wulf, E. Wynne, B. M. Xella, S. Xiao, M. Xie, S. Xu, C. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yamada, M. Yamaguchi, H. Yamaguchi, Y. Yamamoto, A. Yamamoto, K. Yamamoto, S. Yamamura, T. Yamanaka, T. Yamauchi, K. Yamazaki, T. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, U. K. Yang, Y. Yang, Z. Yanush, S. Yao, L. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yen, A. L. Yildirim, E. Yilmaz, M. Yoosoofmiya, R. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. Yu, D. R. Yu, J. Yu, J. Yuan, L. Yurkewicz, A. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zambito, S. Zanello, L. Zanzi, D. Zaytsev, A. Zeitnitz, C. Zeman, M. Zemla, A. Zenin, O. Zenis, T. Zerwas, D. della Porta, G. Zevi Zhang, D. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, N. Zhou, Y. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccoli, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurement of jet shapes in top-quark pair events at root s=7 TeV using the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID DEEP-INELASTIC SCATTERING; PRODUCTION CROSS-SECTION; COLLISIONS; HERA; ALGORITHM; DISTRIBUTIONS; PHYSICS; CHANNEL; QCD AB A measurement of jet shapes in top-quark pair events using 1.8 fb(-1) of pp collision data recorded by the ATLAS detector at the LHC is presented. Samples of top-quark pair events are selected in both the single-lepton and dilepton final states. The differential and integrated shapes of the jets initiated by bottom-quarks from the top-quark decays are compared with those of the jets originated by light-quarks from the hadronic W-boson decays in the single-lepton channel. 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[Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C-M; Dinut, F.; Dita, P.; Dita, S.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Fabre, C.; Facini, G.; Farthouat, P.; Fassnacht, P.; Franchino, S.; Francis, D.; Franz, S.; Froidevaux, D.; Gabaldon, C.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Koeneke, K.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lua, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] IN2P3, CNRS, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN, Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyka, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Pinto Firmino Da Costa, J. Goncalves; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Mattig, S.; Medinnis, M.; Monig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Pinto Firmino Da Costa, J. Goncalves; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Mattig, S.; Medinnis, M.; Monig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Li, S.; Liu, M.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Ahles, F.; Amoroso, S.; Barber, T.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobavab, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] IN2P3, CNRS, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Henke, M.; Hofmann, J. I.; Khomich, A.; Kluge, E-E; Laier, H.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] IN2P3, CNRS, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] IN2P3, CNRS, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Xu, L.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Ge, P.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F; Asbah, N.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F; Asbah, N.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koetsveld, F.; Koenig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 7008530, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] IN2P3, CNRS, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Colombo, T.; Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, Lphea Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J-B; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay Commissariat Energie Atom & Energie Al, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenecb, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Garcia, B. R. Mellado; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaitia, Y.; Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaitia, Y.; Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Petridis, A.; Plucinski, P.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G-Y; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Ahmad, A.; Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Cheung, S. L.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rosenbaum, G. A.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirouta, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] INFN, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Fassi, F.; Ferrer, A.; Fuster, J.; Garcia, C.; Irles Quiles, A.; Lacasta, C.; Oliver Garcia, E.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; Higon-Rodriguez, E.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Astbury, A.; Berghaus, F.; Marino, C. P.; Martyniuk, A. C.; Ouellette, E. A.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. 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[Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Smirnova, L. N.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Ventura, Andrea/A-9544-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Franco , Fernando /D-5021-2013; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Warburton, Andreas/N-8028-2013; Moraes, Arthur/F-6478-2010; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Gutierrez, Phillip/C-1161-2011; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; Nozka, Libor/G-5550-2014; Kepka, Oldrich/G-6375-2014; Nemecek, Stanislav/G-5931-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Snesarev, Andrey/H-5090-2013; Tomasek, Lukas/G-6370-2014; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Ferrando, James/A-9192-2012; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Smirnova, Oxana/A-4401-2013; Gabrielli, Alessandro/H-4931-2012; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012 OI Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Coccaro, Andrea/0000-0003-2368-4559; Haas, Andrew/0000-0002-4832-0455; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Karyukhin, Andrey/0000-0001-9087-4315; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Franco , Fernando /0000-0002-5829-3155; SULIN, VLADIMIR/0000-0003-3943-2495; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; Svatos, Michal/0000-0002-7199-3383; Warburton, Andreas/0000-0002-2298-7315; Moraes, Arthur/0000-0002-5157-5686; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Castro, Nuno/0000-0001-8491-4376; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Mikestikova, Marcela/0000-0003-1277-2596; Tomasek, Lukas/0000-0002-5224-1936; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Ferrando, James/0000-0002-1007-7816; Doyle, Anthony/0000-0001-6322-6195; Boyko, Igor/0000-0002-3355-4662; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Lee, Jason/0000-0002-2153-1519; Kuday, Sinan/0000-0002-0116-5494; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Fabbri, Laura/0000-0002-4002-8353 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; AvH Foundation, Germany; MPG, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MIN-ERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MIN-ERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 70 TC 4 Z9 4 U1 10 U2 171 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. 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APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Silveira, G Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, E Lagana, C Mercadante, PG 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Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Swanson, J. CA CMS Collaboration TI Jet and underlying event properties as a function of charged-particle multiplicity in proton-proton collisions at root s=7 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PHYSICS; LHC; QCD AB Characteristics of multi-particle production in proton-proton collisions at root s = 7 TeV are studied as a function of the charged-particle multiplicity, N (ch). The produced particles are separated into two classes: those belonging to jets and those belonging to the underlying event. Charged particles are measured with pseudorapidity |eta|< 2.4 and transverse momentum p (T)> 0.25 GeV/c. Jets are reconstructed from charged-particles only and required to have p (T)> 5 GeV/c. The distributions of jet p (T), average p (T) of charged particles belonging to the underlying event or to jets, jet rates, and jet shapes are presented as functions of N (ch) and compared to the predictions of the pythia and herwig event generators. Predictions without multi-parton interactions fail completely to describe the N (ch)-dependence observed in the data. For increasing N (ch), pythia systematically predicts higher jet rates and harder p (T) spectra than seen in the data, whereas herwig shows the opposite trends. At the highest multiplicity, the data-model agreement is worse for most observables, indicating the need for further tuning and/or new model ingredients. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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T.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoameri, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dudko, L.; Gribushin, A.; Khein, L.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Proskuryakov, A.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Gomez-Reino Garrido, R.; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Palencia Cortezon, E.; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. 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A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Calderon De La Barca Sanchez, M.; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Magana Villalba, R.; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Luiggi Lopez, E.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Nicolas Kaufman, G.; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Butler, P. H.; Harris, P.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. 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Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; My, Salvatore/0000-0002-9938-2680; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Ragazzi, Stefano/0000-0001-8219-2074; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Montanari, Alessandro/0000-0003-2748-6373; Moon, Chang-Seong/0000-0001-8229-7829; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Codispoti, Giuseppe/0000-0003-0217-7021; Dudko, Lev/0000-0002-4462-3192; de Jesus Damiao, Dilson/0000-0002-3769-1680; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Heredia De La Cruz, Ivan/0000-0002-8133-6467; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Varela, Joao/0000-0003-2613-3146; Heath, Helen/0000-0001-6576-9740 FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU; Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 41 TC 7 Z9 8 U1 5 U2 108 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD DEC 11 PY 2013 VL 73 IS 12 AR 2674 DI 10.1140/epjc/s10052-013-2674-5 PG 26 WC Physics, Particles & Fields SC Physics GA 270TT UT WOS:000328342400001 ER PT J AU Mathias, PM Jasperson, LV VonNiederhausern, D Bearden, MD Koech, PK Freeman, CJ Heldebrant, DJ AF Mathias, Paul M. Jasperson, Louis V. VonNiederhausern, David Bearden, Mark D. Koech, Phillip K. Freeman, Charles J. Heldebrant, David J. TI Assessing Anhydrous Tertiary Alkanolamines for High-Pressure Gas Purifications SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CO2 CAPTURE; MIXTURES AB Anhydrous tertiary alkanolamines chemically react with CO2 and H2S, with greater selectivity for the latter. This is in direct contrast to aqueous amine-based solvent systems, which exhibit higher selectivity for CO2 over H2S. Anhydrous tertiary alkanolamines exhibit pressure-induced chemical fixation of CO2 to form zwitterionic ammonium alkylcarbonate ionic liquids, while the same tertiary alkanolamines react with H2S at atmospheric pressures to form hydrosulfide ionic liquids. This difference in capture pressure implies that certain anhydrous alkanolamines could be chemically selective for H2S over CO2. We present here the first published vapor liquid liquid equilibrium (VLLE) data of anhydrous ethyldiethanolamine (EDEA) with CH4, C3H8, H2S, and CO2 at 10-50 degrees C measured by the TPx and TPxy methods. The data are modeled in Aspen Plus using an NRTL-with-solvation model. Data trends and the underlying phenomena are discussed for each gas. We also present process simulations that compare anhydrous EDEA's performance for CO2 and H2S high-pressure separations to other solvents such as Fluor Solvent (propylene carbonate), Selexol, and aqueous methyldiethanolamine (MDEA) for a representative gas-purification absorber. This work indicates that a niche for anhydrous EDEA in high-pressure gas purifications may be its stronger absorption for CO2 and H2S (relative to physical solvents) and its selectivity for H2S over CO2 (relative to chemical solvents). C1 [Mathias, Paul M.] Fluor Corp, Aliso Viejo, CA 92698 USA. [Jasperson, Louis V.; VonNiederhausern, David] Wiltec Res Co, Provo, UT 84601 USA. [Bearden, Mark D.; Koech, Phillip K.; Freeman, Charles J.; Heldebrant, David J.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Mathias, PM (reprint author), Fluor Corp, 3 Polaris Way, Aliso Viejo, CA 92698 USA. EM Paul.Mathias@Fluor.com OI Koech, Phillip/0000-0003-2996-0593 FU PNNL Laboratory Directed Research and Development (LDRD) FX PNNL acknowledges funding from PNNL Laboratory Directed Research and Development (LDRD) and Mike Elliot for his engineering support. Wiltec acknowledges Lane Gardner for his conscientious assistance in obtaining the measured data. NR 19 TC 2 Z9 2 U1 3 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD DEC 11 PY 2013 VL 52 IS 49 BP 17562 EP 17572 DI 10.1021/ie4020974 PG 11 WC Engineering, Chemical SC Engineering GA 272CV UT WOS:000328438800025 ER PT J AU Levitskaia, TG Peterson, JM Campbell, EL Casella, AJ Peterman, DR Bryan, SA AF Levitskaia, Tatiana G. Peterson, James M. Campbell, Emily L. Casella, Amanda J. Peterman, Dean R. Bryan, Samuel A. TI Fourier Transform Infrared Spectroscopy and Multivariate Analysis for Online Monitoring of Dibutyl Phosphate Degradation Product in Tributyl Phosphate/n-Dodecane/Nitric Acid Solvent SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID MONOBUTYL PHOSPHATE; LEAST-SQUARES; NITRIC-ACID; CHROMATOGRAPHY; SYSTEM AB In liquid-liquid extraction separation processes, accumulation of organic solvent degradation products is detrimental to the process robustness, and frequent solvent analysis is warranted. Our research explores the feasibility of online monitoring of the organic solvents relevant to used nuclear fuel reprocessing. This paper describes the first phase of developing a system for monitoring the tributyl phosphate (TBP)/n-dodecane solvent commonly used to separate used nuclear fuel. In this investigation, the effect of extraction of nitric acid from aqueous solutions of variable concentrations on the quantification of TBP and its major degradation product dibutylphosphoric acid (HDBP) was assessed. Fourier transform infrared (FTIR) spectroscopy was used to discriminate between HDBP and TBP in the nitric acid-containing TBP/n-dodecane solvent. Multivariate analysis of the spectral data facilitated the development of regression models for HDBP and TBP quantification in real time, enabling online implementation of the monitoring system. The predictive regression models were validated using TBP/n-dodecane solvent samples subjected to high-dose external gamma-irradiation. The predictive models were translated to flow conditions using a hollow fiber FTIR probe installed in a centrifugal contactor extraction apparatus, demonstrating the applicability of the FTIR technique coupled with multivariate analysis for the online monitoring of the organic solvent degradation products. C1 [Levitskaia, Tatiana G.; Peterson, James M.; Campbell, Emily L.; Casella, Amanda J.; Bryan, Samuel A.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Peterman, Dean R.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Levitskaia, TG (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Tatiana.Levitskaia@pnnl.gov; Sam.Bryan@pnnl.gov RI Bryan, Samuel/D-5457-2015 OI Bryan, Samuel/0000-0001-5664-3249 FU Separations and Waste Forms Campaign within the U.S. Department of Energy's Fuel Cycle Research and Development Program; U.S. Department of Energy [DE-AC05-76RL01830] FX This research was supported by the Separations and Waste Forms Campaign within the U.S. Department of Energy's Fuel Cycle Research and Development Program and conducted at the Pacific Northwest National Laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. NR 26 TC 7 Z9 7 U1 4 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD DEC 11 PY 2013 VL 52 IS 49 BP 17607 EP 17617 DI 10.1021/ie402722n PG 11 WC Engineering, Chemical SC Engineering GA 272CV UT WOS:000328438800030 ER PT J AU Borges, I Aquino, AJA Kohn, A Nieman, R Hase, WL Chen, LX Lischka, H AF Borges, Itamar, Jr. Aquino, Adelia J. A. Koehn, Andreas Nieman, Reed Hase, William L. Chen, Lin X. Lischka, Hans TI Ab Initio Modeling of Excitonic and Charge-Transfer States in Organic Semiconductors: The PTB1/PCBM Low Band Gap System SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID DENSITY-FUNCTIONAL THEORY; ELECTRONICALLY EXCITED-STATES; DONOR-ACCEPTOR COMPLEXES; SOLAR-CELLS; TRANSFER EXCITATIONS; MOLECULAR-COMPLEXES; APPROXIMATION; TETRACYANOETHYLENE; POLYMERS; EXCHANGE AB A detailed quantum chemical simulation of the excitonic and charge-transfer (CT) states of a bulk heterojunction model containing poly(thieno[3,4-b]-thiophene benzodithiophene) (PTB1)/[6,6]-phenyl-C-61-butyric acid methyl ester (PCBM) is reported. The largest molecular model contains two stacked PTB1 trimer chains interacting with C-60 positioned on top of and lateral to the (PTB1)(3) stack. The calculations were performed using the algebraic diagrammatic construction method to second order (ADC(2)). One main result of the calculations is that the CT states are located below the bright inter-chain excitonic state, directly accessible via internal conversion processes. The other important aspects of the calculations are the formation of discrete bands of CT states originating from the lateral C-60's and the importance of inter-chain charge delocalization for the stability of the CT states. A simple model for the charge separation step is also given, revealing the energetic feasibility of the overall photovoltaic process. C1 [Borges, Itamar, Jr.; Aquino, Adelia J. A.; Nieman, Reed; Hase, William L.; Lischka, Hans] Texas Tech Univ, Dept Chem & Biochem, Lubbock, TX 79409 USA. [Borges, Itamar, Jr.] Inst Mil Engn, Dept Quim, BR-22290270 Rio De Janeiro, Brazil. [Koehn, Andreas] Johannes Gutenberg Univ Mainz, Inst Phys Chem, D-55099 Mainz, Germany. [Chen, Lin X.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Lischka, Hans] Univ Vienna, Inst Theoret Chem, A-1090 Vienna, Austria. RP Borges, I (reprint author), Texas Tech Univ, Dept Chem & Biochem, Lubbock, TX 79409 USA. EM itamar@ime.eb.br; hans.lischka@ttu.edu RI Borges, Itamar/B-9535-2009; Lischka, Hans/A-8802-2015; Aquino, Adelia/F-3226-2016 OI Borges, Itamar/0000-0002-8492-1223; FU National Science Foundation [CHE-1213263, OISE-0730114]; Robert A. Welch Foundation [D-0005]; Center for Integrated Nanotechnologies [C2013A0070]; U.S. Department of Energy Office of Science [DE-AC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000]; Vienna Scientific Cluster [70019]; Fulbright Foundation; CAPES; DFG [KO 2337/3-1] FX This material is based upon work supported by the National Science Foundation under Project No. CHE-1213263 and Grant No. OISE-0730114 for the Partnerships in International Research and Education. Support was also provided by the Robert A. Welch Foundation under Grant No. D-0005 and by the Center for Integrated Nanotechnologies (Project No. C2013A0070), an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract DE-AC04-94AL85000). Computer time at the Vienna Scientific Cluster (Project No. 70019) is gratefully acknowledged. I.B. thanks the Fulbright Foundation and CAPES for a fellowship to visit the Texas Tech University. A.K. acknowledges a Heisenberg Fellowship of the DFG (Grant No. KO 2337/3-1). NR 31 TC 23 Z9 23 U1 5 U2 69 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 11 PY 2013 VL 135 IS 49 BP 18252 EP 18255 DI 10.1021/ja4081925 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 272CU UT WOS:000328438700003 PM 24215627 ER PT J AU Berweger, S Nguyen, DM Muller, EA Bechtel, HA Perkins, TT Raschke, MB AF Berweger, Samuel Nguyen, Duc M. Muller, Eric A. Bechtel, Hans A. Perkins, Thomas T. Raschke, Markus B. TI Nano-Chemical Infrared Imaging of Membrane Proteins in Lipid Bilayers SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ATOMIC-FORCE MICROSCOPY; NEAR-FIELD MICROSCOPY; OPTICAL MICROSCOPY; PURPLE MEMBRANES; SPECTROSCOPY; RESOLUTION; BACTERIORHODOPSIN; LIMIT; SCATTERING; STABILITY AB The spectroscopic characterization of biomolecular structures requires nanometer spatial resolution and chemical specificity. We perform full spatio-spectral imaging of dried purple membrane patches purified from Halobacterium salinarum with infrared vibrational scattering-type scanning near-field optical microscopy (s-SNOM). Using near-field spectral phase contrast based on the Amide I resonance of the protein backbone, we identify the protein distribution with 20 nm spatial resolution and few-protein sensitivity. This demonstrates the general applicability of s-SNOM vibrational nanospectroscopy, with potential extension to a wide range of biomolecular systems. C1 [Berweger, Samuel; Muller, Eric A.; Raschke, Markus B.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Berweger, Samuel; Muller, Eric A.; Raschke, Markus B.] Univ Colorado, Dept Chem, Boulder, CO 80309 USA. [Nguyen, Duc M.] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80309 USA. [Perkins, Thomas T.] Univ Colorado, Dept Mol Cellular & Dev Biol, Boulder, CO 80309 USA. [Berweger, Samuel; Muller, Eric A.; Perkins, Thomas T.; Raschke, Markus B.] Univ Colorado, NIST, Joint Inst Lab Astrophys, Boulder, CO 80309 USA. [Berweger, Samuel; Muller, Eric A.; Perkins, Thomas T.; Raschke, Markus B.] Univ Colorado, Boulder, CO 80309 USA. [Bechtel, Hans A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source Div, Berkeley, CA 94720 USA. RP Raschke, MB (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA. EM markus.raschke@colorado.edu RI Muller, Eric/J-2161-2012; Raschke, Markus/F-8023-2013; OI Muller, Eric/0000-0002-9629-1767; Perkins, Thomas/0000-0003-4826-9490 FU National Science Foundation [CHE-0748226, DBI-0923544, Phys-1125844]; NIST; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Linda Randall for providing the halobacterium and protocols for preparing the bR sample, and Craig Prater from Anasys Instruments for technical scanning probe support. M.B.R. acknowledges support from the National Science Foundation (CHE-0748226). T.T.P. acknowledges support from the NSF (DBI-0923544, Phys-1125844) and NIST. T.T.P. is a staff member of the Quantum Physics Division of NIST. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 28 TC 23 Z9 23 U1 6 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 11 PY 2013 VL 135 IS 49 BP 18292 EP 18295 DI 10.1021/ja409815g PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 272CU UT WOS:000328438700013 PM 24251914 ER PT J AU Dutta, A Lense, S Hou, JB Engelhard, MH Roberts, JAS Shaw, WJ AF Dutta, Arnab Lense, Sheri Hou, Jianbo Engelhard, Mark H. Roberts, John A. S. Shaw, Wendy J. TI Minimal Proton Channel Enables H-2 Oxidation and Production with a Water-Soluble Nickel-Based Catalyst SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OUTER-COORDINATION SPHERE; HYDROGEN-PRODUCTION; PENDANT AMINES; MOLECULAR CATALYSTS; ELECTRON-TRANSFER; COMPLEXES; ELECTROCATALYSTS; EVOLUTION; SYSTEMS; DESIGN AB Hydrogenase enzymes use first-row transition metals to interconvert H-2 with protons and electrons, reactions that are important for the storage and recovery of energy from intermittent sources such as solar, hydroelectric, and wind. Here we present Ni((P2N2Gly)-N-Cy)(2), a water-soluble molecular electrocatalyst with the amino acid glycine built into the diphosphine ligand framework. Proton transfer between the outer coordination sphere carboxylates and the second coordination sphere pendant amines is rapid, as observed by cyclic voltammetry and FTIR spectroscopy, indicating that the carboxylate groups may participate in proton transfer during catalysis. This complex oxidizes H-2 (1-33 s(-1)) at low overpotentials (150-365 mV) over a range of pH values (0.1-9.0) and produces H-2 under identical solution conditions (>2400 s(-1) at pH 0.5). Enzymes employ proton channels for the controlled movement of protons over long distances-the results presented here demonstrate the effects of a simple two-component proton channel in a synthetic molecular electrocatalyst. C1 [Dutta, Arnab; Lense, Sheri; Hou, Jianbo; Engelhard, Mark H.; Roberts, John A. S.; Shaw, Wendy J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Roberts, JAS (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM john.roberts@pnnl.gov; wendy.shaw@pnnl.gov OI Engelhard, Mark/0000-0002-5543-0812 FU Office of Science Early Career Research Program through U.S. Department of Energy (DOE), Basic Energy Sciences (BES); Center for Molecular Electrocatalysis, an Energy Frontier Research Center; U.S. DOE, BES; U.S. DOE's Office of Biological and Environmental Research program FX This work was funded by the Office of Science Early Career Research Program through the U.S. Department of Energy (DOE), Basic Energy Sciences (BES) (A.D., S.L., W.J.S.), and the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. DOE, BES (J.H., J.A.S.R). Part of the research was conducted at the W.R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by U.S. DOE's Office of Biological and Environmental Research program located at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the U.S. DOE. NR 45 TC 55 Z9 55 U1 5 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 11 PY 2013 VL 135 IS 49 BP 18490 EP 18496 DI 10.1021/ja407826d PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 272CU UT WOS:000328438700043 PM 24206187 ER PT J AU Young, KC Blume-Kohout, R Lidar, DA AF Young, Kevin C. Blume-Kohout, Robin Lidar, Daniel A. TI Adiabatic quantum optimization with the wrong Hamiltonian SO PHYSICAL REVIEW A LA English DT Article ID CODES AB Analog models of quantum information processing, such as adiabatic quantum computation and analog quantum simulation, require the ability to subject a system to precisely specified Hamiltonians. Unfortunately, the hardware used to implement these Hamiltonians will be imperfect and limited in its precision. Even small perturbations and imprecisions can have profound effects on the nature of the ground state. Here we consider an imperfect implementation of adiabatic quantum optimization and show that, for a widely applicable random control noise model, quantum stabilizer encodings are able to reduce the effective noise magnitude and thus improve the likelihood of a successful computation or simulation. This reduction builds upon two design principles: summation of equivalent logical operators to increase the energy scale of the encoded optimization problem, and the inclusion of a penalty term comprising the sum of the code stabilizer elements. We illustrate our findings with an Ising ladder and show that classical repetition coding drastically increases the probability that the ground state of a perturbed model is decodable to that of the unperturbed model, while using only realistic two-body interaction. Finally, we note that the repetition encoding is a special case of quantum stabilizer encodings, and show that this in principle allows us to generalize our results to many types of analog quantum information processing, albeit at the expense of many-body interactions. C1 [Young, Kevin C.] Sandia Natl Labs, Scalable & Secure Syst Res 08961, Livermore, CA 94550 USA. [Blume-Kohout, Robin] Sandia Natl Labs, Adv Device Technol 01425, Albuquerque, NM 87185 USA. [Lidar, Daniel A.] Univ So Calif, Dept Chem, Dept Elect Engn, Dept Phys, Los Angeles, CA 90089 USA. [Lidar, Daniel A.] Univ So Calif, Ctr Quantum Informat Sci & Technol, Los Angeles, CA 90089 USA. RP Young, KC (reprint author), Sandia Natl Labs, Scalable & Secure Syst Res 08961, Livermore, CA 94550 USA. EM kyoung@sandia.gov FU ARO-MURI [W911NF-11-1-0268]; ARO-QA [W911NF-12-1-0523]; Lockheed Martin Corporation; NSF [PHY-969969, PHY-803304] FX The authors thank Alexey Gorshkov for calling attention to the problem of control errors on the final Hamiltonian in adiabatic quantum computing. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. DAL's research was supported by ARO-MURI Grant No. W911NF-11-1-0268, by ARO-QA Grant No. W911NF-12-1-0523, by the Lockheed Martin Corporation, and by NSF Grants No. PHY-969969 and No. PHY-803304. NR 22 TC 12 Z9 12 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD DEC 11 PY 2013 VL 88 IS 6 AR 062314 DI 10.1103/PhysRevA.88.062314 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 275JU UT WOS:000328672900001 ER PT J AU Busser, CA Martins, GB Feiguin, AE AF Buesser, C. A. Martins, G. B. Feiguin, A. E. TI Lanczos transformation for quantum impurity problems in d-dimensional lattices: Application to graphene nanoribbons SO PHYSICAL REVIEW B LA English DT Article ID LOCAL ATOMIC ENVIRONMENT; TIGHT-BINDING BANDS; RENORMALIZATION-GROUP; ELECTRONIC-STRUCTURE; MAGNETIC IMPURITY; ANDERSON MODEL; FERMI SYSTEMS; KONDO PROBLEM; TRANSPORT; FIELD AB We present a completely unbiased and controlled numerical method to solve quantum impurity problems in d-dimensional lattices. This approach is based on a canonical transformation, of the Lanczos form, where the complete lattice Hamiltonian is exactly mapped onto an equivalent one-dimensional system, in the same spirit as Wilson's numerical renormalization, and Haydock's recursion method. We introduce many-body interactions in the form of a Kondo or Anderson impurity and we solve the low-dimensional problem using the density matrix renormalization group. The technique is particularly suited to study systems that are inhomogeneous, and/or have a boundary. The resulting dimensional reduction translates into a reduction of the scaling of the entanglement entropy by a factor Ld-1, where L is the linear dimension of the original d-dimensional lattice. This allows one to calculate the ground state of a magnetic impurity attached to an L x L square lattice and an L x L x L cubic lattice with L up to 140 sites. We also study the localized edge states in graphene nanoribbons by attaching a magnetic impurity to the edge or the center of the system. For armchair metallic nanoribbons we find a slow decay of the spin correlations as a consequence of the delocalized metallic states. In the case of zigzag ribbons, the decay of the spin correlations depends on the position of the impurity. If the impurity is situated in the bulk of the ribbon, the decay is slow as in the metallic case. On the other hand, if the adatom is attached to the edge, the decay is fast, within few sites of the impurity, as a consequence of the localized edge states, and the short correlation length. The mapping can be combined with ab initio band structure calculations to model the system, and to understand correlation effects in quantum impurity problems starting from first principles. C1 [Buesser, C. A.] Univ Munich, Dept Phys, D-81377 Munich, Germany. [Buesser, C. A.] Univ Munich, Arnold Sommerfeld Ctr Theoret Phys, D-81377 Munich, Germany. [Martins, G. B.] Oakland Univ, Dept Phys, Rochester, MI 48309 USA. [Martins, G. B.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Feiguin, A. E.] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. RP Busser, CA (reprint author), Univ Munich, Dept Phys, Marchioninistr 15, D-81377 Munich, Germany. EM carlos.busser@gmail.com RI Busser, Carlos/K-1017-2014; Martins, George/C-9756-2012 OI Busser, Carlos/0000-0002-0353-7490; Martins, George/0000-0001-7846-708X FU Deutsche Forschungsgemeinschaft (DFG) [FOR 912, HE5242/2-2]; NSF [DMR-0710529, DMR-1107994, MRI-0922811, DMR-1339564]; DAAD FX We thank K. Al-Hassanieh, F. Heidrich Meisner, L. Vidmar, and C. Batista for helpful discussions. C. A. B. was supported by the Deutsche Forschungsgemeinschaft (DFG) through FOR 912 under Grant No. HE5242/2-2. G. B. M. acknowledges financial support from the NSF under Grant Nos. DMR-0710529, DMR-1107994, and MRI-0922811. G. B. M. also thanks the hospitality of the Institut fur Theorie der Statistischen Physik, RWTH Aachen University, Aachen, Germany, where part of this work was performed under a DAAD fellowship. A. E. F. acknowledges NSF support through Grant No. DMR-1339564. NR 94 TC 7 Z9 7 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 11 PY 2013 VL 88 IS 24 AR 245113 DI 10.1103/PhysRevB.88.245113 PG 13 WC Physics, Condensed Matter SC Physics GA 275MG UT WOS:000328680500002 ER PT J AU Knizek, K Hejtmanek, J Marysko, M Novak, P Santava, E Jirak, Z Naito, T Fujishiro, H de la Cruz, C AF Knizek, K. Hejtmanek, J. Marysko, M. Novak, P. Santava, E. Jirak, Z. Naito, T. Fujishiro, H. de la Cruz, Clarina TI Spin-state crossover and low-temperature magnetic state in yttrium-doped Pr0.7Ca0.3CoO3 SO PHYSICAL REVIEW B LA English DT Article ID ENERGY-LEVELS; TRANSITION; LA1-XSRXCOO3; RESONANCE; ORDER AB The structural and magnetic properties of two mixed-valence cobaltites with a formal population of 0.30 Co4+ ions per f.u., (Pr1-yYy)(0.7)Ca0.3CoO3 (y = 0 and 0.15), have been studied down to very low temperatures by means of high-resolution neutron diffraction, SQUID magnetometry, and heat-capacity measurements. The results are interpreted within the scenario of the spin-state crossover from a room-temperature mixture of the intermediate-spin Co3+ and low-spin Co4+ (IS/LS) to the LS/LS mixture in the sample ground states. In contrast to the yttrium-free y = 0 that retains the metallic-like character and exhibits ferromagnetic (FM) ordering below 55 K, the doped system y = 0.15 undergoes a first-order metal-insulator transition at 132 K, during which not only the crossover to low-spin states but also a partial electron transfer from Pr3+ 4f to cobalt 3d states takes place simultaneously. Taking into account the nonmagnetic character of LS Co3+, such a valence shift electronic transition causes a magnetic dilution, formally to 0.12 LS Co4+ or 0.12 t(2g) hole spins per f.u., which is the reason for an insulating, highly nonuniform magnetic ground state without long-range order. Nevertheless, even in that case there exists a relatively strong molecular field distributed over all the crystal lattice. It is argued that the spontaneous FM order in y = 0 and the existence of strong FM correlations in y = 0.15 apparently contradict the single t(2g) band character of LS/LS phase. The explanation we suggest relies on a model of the defect-induced, itinerant hole-mediated magnetism, where the defects are identified with the magnetic high-spin Co3+ species stabilized near oxygen vacancies. C1 [Knizek, K.; Hejtmanek, J.; Marysko, M.; Novak, P.; Santava, E.; Jirak, Z.] Inst Phys ASCR, Prague 16200 6, Czech Republic. [Naito, T.; Fujishiro, H.] Iwate Univ, Fac Engn, Morioka, Iwate 0208551, Japan. [de la Cruz, Clarina] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Knizek, K (reprint author), Inst Phys ASCR, Cukrovarnicka 10, Prague 16200 6, Czech Republic. RI Knizek, Karel/G-5270-2014; Hejtmanek, Jiri/G-5591-2014; Jirak, Zdenek/G-6281-2014; Marysko, Miroslav/G-6464-2014; Novak, Pavel/G-6692-2014; dela Cruz, Clarina/C-2747-2013 OI Knizek, Karel/0000-0002-0725-0331; Hejtmanek, Jiri/0000-0001-8248-3912; dela Cruz, Clarina/0000-0003-4233-2145 FU Grant Agency of the Czech Republic [204/11/0713] FX We thank J. Kunes and C. Leighton for stimulating comments. This work was supported by Project No. 204/11/0713 of the Grant Agency of the Czech Republic. NR 30 TC 10 Z9 10 U1 2 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 11 PY 2013 VL 88 IS 22 AR 224412 DI 10.1103/PhysRevB.88.224412 PG 8 WC Physics, Condensed Matter SC Physics GA 275MB UT WOS:000328679700003 ER PT J AU Hlophe, L Elster, C Johnson, RC Upadhyay, NJ Nunes, FM Arbanas, G Eremenko, V Escher, JE Thompson, IJ AF Hlophe, L. Elster, Ch. Johnson, R. C. Upadhyay, N. J. Nunes, F. M. Arbanas, G. Eremenko, V. Escher, J. E. Thompson, I. J. CA TORUS Collaboration TI Separable representation of phenomenological optical potentials of Woods-Saxon type SO PHYSICAL REVIEW C LA English DT Article ID FADDEEV CALCULATIONS; 2-BODY INTERACTIONS; MODEL; APPROXIMATIONS; SCATTERING; STATE AB Background: One important ingredient for many applications of nuclear physics to astrophysics, nuclear energy, and stockpile stewardship are the cross sections for reactions of neutrons with rare isotopes. Since direct measurements are often not feasible, indirect methods, e. g., (d, p) reactions, should be used. Those (d, p) reactions may be viewed as three-body reactions and described with Faddeev techniques. Purpose: Faddeev equations in momentum space have a long tradition of utilizing separable interactions in order to arrive at sets of coupled integral equations in one variable. While there exist several separable representations for the nucleon-nucleon interaction, the optical potential between a neutron (proton) and a nucleus is not readily available in separable form. The purpose of this paper is to introduce a separable representation for complex phenomenological optical potentials of Woods-Saxon type. Results: Starting from a global optical potential, a separable representation thereof is introduced based on the Ernst-Shakin-Thaler (EST) scheme. This scheme is generalized to non-Hermitian potentials. Applications to n + Ca-48, n + Sn-132, and n + Pb-208 are investigated for energies from 0 to 50 MeV and the quality of the representation is examined. Conclusions: We find a good description of the on-shell t matrix for all systems with rank up to 5. The required rank depends inversely on the angular momentum. The resulting separable interaction exhibits a different off-shell behavior compared to the original potential, reducing the high-momentum contributions. C1 [Hlophe, L.; Elster, Ch.; Eremenko, V.] Ohio Univ, Inst Nucl & Particle Phys, Athens, OH 45701 USA. [Hlophe, L.; Elster, Ch.; Eremenko, V.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Johnson, R. C.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Upadhyay, N. J.; Nunes, F. M.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Upadhyay, N. J.; Nunes, F. M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Arbanas, G.] Oak Ridge Natl Lab, Nucl Sci & Technol Div, Oak Ridge, TN 37831 USA. [Escher, J. E.; Thompson, I. J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Eremenko, V.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. RP Hlophe, L (reprint author), Ohio Univ, Inst Nucl & Particle Phys, Athens, OH 45701 USA. EM lh421709@ohio.edu; elster@ohio.edu RI Elster, Charlotte/N-9845-2015 FU U.S. Department of Energy [DE-FG02-93ER40756, DE-FG52-08NA28552, DE-SC0004084, DE-SC0004087]; Ohio University; Michigan State University; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Science Foundation [PHY-0800026] FX This work was performed in part under the auspices of the U.S. Department of Energy under Contract No. DE-FG02-93ER40756 with Ohio University and Contract No. DE-FG52-08NA28552 with Michigan State University and under Contracts No. DE-SC0004084 and No. DE-SC0004087 (TORUS Collaboration) and by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. F. M. Nunes also acknowledges support from the National Science Foundation under Grant No. PHY-0800026. R. C. Johnson thanks the NSCL for their hospitality and support during his visits. NR 33 TC 8 Z9 8 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD DEC 11 PY 2013 VL 88 IS 6 AR 064608 DI 10.1103/PhysRevC.88.064608 PG 11 WC Physics, Nuclear SC Physics GA 275PN UT WOS:000328689400001 ER PT J AU Deshmukh, S Kamath, G Ramanathan, S Sankaranarayanan, SKRS AF Deshmukh, Sanket Kamath, Ganesh Ramanathan, Shriram Sankaranarayanan, Subramanian K. R. S. TI Chloride ions induce order-disorder transition at water-oxide interfaces SO PHYSICAL REVIEW E LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; PITTING CORROSION; LIQUID; GROWTH; SPECTROSCOPY; SURFACES; COPPER; STAGE; FILMS AB Water can form quasi-two-dimensional ordered layers near a solid interface. The solvation dynamics and ionic transport phenomena through this ordered water structure is of direct relevance to a variety of problems in interface science. Molecular dynamics simulations are used to study the impact of local fluctuation of the chloride ion density in the vicinity of an oxide surface on the structure and dynamics of water layers. We demonstrate that local increase in chloride ions beyond a threshold concentration near the water-MgO ( 100) interface introduces an order-disorder transition of this two-dimensional layered network into bulklike water, leading to increased diffusional characteristics and reduced hydrogen bonding lifetimes. We find that the extent of this order-disorder transition can be tuned by modifying the defect chemistry and nature of the underlying substrate. The kinetic fluidity resulting from order-disorder transition at high chloride ion concentration has significance for a broad range of phenomena, ranging from freezing point depression of brine to onset of aqueous corrosion. C1 [Deshmukh, Sanket; Sankaranarayanan, Subramanian K. R. S.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Kamath, Ganesh] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Ramanathan, Shriram] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. RP Sankaranarayanan, SKRS (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM skrssank@anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; ONR [N00014-10-1-0346] FX Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. S.R. acknowledges the ONR for support under Grant No. N00014-10-1-0346. NR 28 TC 2 Z9 2 U1 4 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD DEC 11 PY 2013 VL 88 IS 6 AR 062119 DI 10.1103/PhysRevE.88.062119 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 275RM UT WOS:000328695100001 PM 24483398 ER PT J AU Liu, YH Cuellar, FA Sefrioui, Z Freeland, JW Fitzsimmons, MR Leon, C Santamaria, J te Velthuis, SGE AF Liu, Yaohua Cuellar, F. A. Sefrioui, Z. Freeland, J. W. Fitzsimmons, M. R. Leon, C. Santamaria, J. te Velthuis, S. G. E. TI Emergent Spin Filter at the Interface between Ferromagnetic and Insulating Layered Oxides SO PHYSICAL REVIEW LETTERS LA English DT Article ID METALLIC FERROMAGNET; TUNNEL-JUNCTIONS; TRANSPORT; MAGNETISM; FILMS AB We report a strong effect of interface-induced magnetization on the transport properties of magnetic tunnel junctions consisting of ferromagnetic manganite La0.7Ca0.3MnO3 and insulating cuprate PrBa2Cu3O7. Contrary to the typically observed steady increase of the tunnel magnetoresistance with decreasing temperature, this system exhibits a sudden anomalous decrease at lowtemperatures. Interestingly, this anomalous behavior can be attributed to the competition between the positive spin polarization of the manganite contacts and the negative spin-filter effect from the interface-induced Cu magnetization. C1 [Liu, Yaohua; te Velthuis, S. G. E.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Cuellar, F. A.; Sefrioui, Z.; Leon, C.; Santamaria, J.] Univ Complutense Madrid, Dept Fis Aplicada 3, GFMC, ES-28040 Madrid, Spain. [Freeland, J. W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Fitzsimmons, M. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Liu, YH (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Leon, Carlos/A-5587-2008; te Velthuis, Suzanne/I-6735-2013; Liu, Yaohua/B-2529-2009; Santamaria, Jacobo/N-8783-2016; Sefrioui, Zouhair/C-2728-2017; OI Leon, Carlos/0000-0002-3262-1843; te Velthuis, Suzanne/0000-0002-1023-8384; Liu, Yaohua/0000-0002-5867-5065; Santamaria, Jacobo/0000-0003-4594-2686; Sefrioui, Zouhair/0000-0002-6703-3339; Cuellar Jimenez, Fabian Andres/0000-0002-2891-6198 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; SpanishMICINN [MAT2011-27470-C02]; Consolider Ingenio [CSD2009-00013]; CAM [S2009/MAT-1756]; Department of Energy's Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396] FX Work at Argonne National Laboratory and use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. Work at UCM was supported by the SpanishMICINN through Grant No. MAT2011-27470-C02, Consolider Ingenio 2010 -CSD2009-00013 (Imagine), and by CAM through Grant No. S2009/MAT-1756 (Phama). This work has benefited from the use of the Lujan Neutron Scattering Center at LANSCE, which is funded by the Department of Energy's Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE through Contract No. DE-AC52-06NA25396. NR 37 TC 14 Z9 14 U1 2 U2 48 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 11 PY 2013 VL 111 IS 24 AR 247203 DI 10.1103/PhysRevLett.111.247203 PG 5 WC Physics, Multidisciplinary SC Physics GA 275TF UT WOS:000328699800019 PM 24483696 ER PT J AU Beria, M Brandino, GP Lepori, L Konik, RM Sierra, G AF Beria, M. Brandino, G. P. Lepori, L. Konik, R. M. Sierra, G. TI Truncated conformal space approach for perturbed Wess-Zumino-Witten SU(2)(k) models SO NUCLEAR PHYSICS B LA English DT Article ID NONLINEAR INTEGRAL-EQUATION; SINE-GORDON THEORY; 2 DIMENSIONS; FIELD-THEORIES; RENORMALIZATION-GROUP; HEISENBERG CHAIN; MAGNETIC-FIELD; EXCITED-STATES; ISING-MODEL; ENERGY AB We outline the application of the truncated conformal space approach (TCSA) to perturbations of SU(2)(k) Wess-Zumino-Witten theories. As examples of this methodology, we consider two distinct perturbations of SU (2)(1) and one of SU(2)(2). SU (2)(1) is first perturbed by its spin-1/2 field, a model which is equivalent to the sine-Gordon model at a particular value of its coupling beta. The sine-Gordon spectrum is correctly reproduced as well as the corresponding finite-size corrections. We next study SU (2)(1) with a marginal current current perturbation. The TCSA results can be matched to perturbation theory within an appropriate treatment of the UV divergences. We find however that these results do not match field theoretic computations on the same model performed with a Lorentz invariant regulator. Finally, we consider SU(2)2 perturbed by its spin-1 field, which is equivalent to three decoupled massive Majorana fermions. In this case as well the TCSA reproduces accurately the known spectrum. (C) 2013 Elsevier B.V. All rights reserved. C1 [Beria, M.] SISSA Int Sch Adv Studies, I-34136 Trieste, Italy. [Beria, M.] Ist Nazl Fis Nucl, Sez Trieste, Rome, Italy. [Brandino, G. P.] Univ Amsterdam, Inst Theoret Phys, NL-1090 GL Amsterdam, Netherlands. [Lepori, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Bellaterra, Spain. [Lepori, L.] IPCMS, UMR 7504, Strasbourg, France. [Lepori, L.] Univ Strasbourg, ISIS, UMR 7006, Strasbourg, France. [Lepori, L.] CNRS, Strasbourg, France. [Konik, R. M.] Brookhaven Natl Lab, Condensed Matter & Mat Sci Dept, Upton, NY 11973 USA. [Sierra, G.] UAM CSIC, Inst Fis Teor, Madrid, Spain. RP Beria, M (reprint author), SISSA Int Sch Adv Studies, Via Bonomea 265, I-34136 Trieste, Italy. RI Konik, Robert/L-8076-2016 OI Konik, Robert/0000-0003-1209-6890 FU European Regional Development Fund; US DOE [DE-AC02-98CH10886]; NSF [PHY 1208521]; QUITEMAD [FIS2009-11654]; Severo-Ochoa Program; Netherlands Organisation for Scientific Research (NWO) FX We thank J. Cardy, F.H.L. Essler, G. Mussardo and G. Takacs for useful discussions. L.L. acknowledges a grant awarded by Banco de Santander and financial support from European Regional Development Fund. R.M.K. acknowledges support by the US DOE under contract DE-AC02-98CH10886 and NSF under grant no. PHY 1208521. G.S. acknowledges support from the grants FIS2009-11654, QUITEMAD and the Severo-Ochoa Program. G.P.B. acknowledges support from the Netherlands Organisation for Scientific Research (NWO). NR 63 TC 11 Z9 11 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0550-3213 EI 1873-1562 J9 NUCL PHYS B JI Nucl. Phys. B PD DEC 11 PY 2013 VL 877 IS 2 BP 457 EP 483 DI 10.1016/j.nuclphysb.2013.10.005 PG 27 WC Physics, Particles & Fields SC Physics GA 266DP UT WOS:000328003100011 ER PT J AU Liu, Y Nelson, J Holzner, C Andrews, JC Pianetta, P AF Liu, Y. Nelson, J. Holzner, C. Andrews, J. C. Pianetta, P. TI Recent advances in synchrotron-based hard x-ray phase contrast imaging SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article ID COMPUTED TOMOGRAPHIC RECONSTRUCTION; 30 NM-RESOLUTION; TALBOT INTERFEROMETRY; CONFIGURED DETECTOR; ZONE PLATES; MICROSCOPY; DIFFRACTION; TRANSMISSION; RETRIEVAL; PROPAGATION AB Ever since the first demonstration of phase contrast imaging (PCI) in the 1930s by Frits Zernike, people have realized the significant advantage of phase contrast over conventional absorption-based imaging in terms of sensitivity to 'transparent' features within specimens. Thus, x-ray phase contrast imaging (XPCI) holds great potential in studies of soft biological tissues, typically containing low Z elements such as C, H, O and N. Particularly when synchrotron hard x-rays are employed, the favourable brightness, energy tunability, monochromatic characteristics and penetration depth have dramatically enhanced the quality and variety of XPCI methods, which permit detection of the phase shift associated with 3D geometry of relatively large samples in a non-destructive manner. In this paper, we review recent advances in several synchrotron-based hard x-ray XPCI methods. Challenges and key factors in methodological development are discussed, and biological and medical applications are presented. C1 [Liu, Y.; Nelson, J.; Andrews, J. C.; Pianetta, P.] SLAC Natl Accelerator Ctr, Stanford Synchrotron Radiat Lab, Menlo Pk, CA 94025 USA. [Holzner, C.] Xradia Inc, Pleasanton, CA 94588 USA. RP Liu, Y (reprint author), SLAC Natl Accelerator Ctr, Stanford Synchrotron Radiat Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM pianetta@slac.stanford.edu RI Liu, Yijin/O-2640-2013; Nelson Weker, Johanna/J-4159-2015 OI Liu, Yijin/0000-0002-8417-2488; Nelson Weker, Johanna/0000-0001-6856-3203 NR 118 TC 16 Z9 16 U1 2 U2 60 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD DEC 11 PY 2013 VL 46 IS 49 AR 494001 DI 10.1088/0022-3727/46/49/494001 PG 13 WC Physics, Applied SC Physics GA 264OH UT WOS:000327887500002 ER PT J AU Wu, SR Lin, CH Chen, YS Chen, YY Hwu, Y Chu, YS Margaritondo, G AF Wu, S. R. Lin, C. H. Chen, Y. S. Chen, Y. Y. Hwu, Y. Chu, Y. S. Margaritondo, G. TI At the frontiers of high-resolution hard-x-ray microscopy: an international programme SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article ID FRESNEL ZONE PLATES; FREE-ELECTRON LASER; ORIENTED PYROLYTIC-GRAPHITE; ZERNIKE PHASE-CONTRAST; E-BEAM LITHOGRAPHY; 30 NM RESOLUTION; ELECTROCHEMICAL NUCLEATION; DIFFRACTION MICROSCOPY; GROWTH-MECHANISM; ELECTRODEPOSITION AB We review the recent progress achieved by our international collaboration on novel imaging techniques based on high-brightness and highly coherent synchrotron sources. After outlining the background, we will discuss the technical progress of recent years. Then, we will exemplify the applications with a number of cases in materials science and life sciences, in particular neurobiology. New results on metal electrodeposition will be used to practically illustrate the impact of the techniques in this important technological area and in general its potential for materials research. Finally, we will briefly comment on the foreseeable technical improvements and on their positive consequences. C1 [Wu, S. R.; Lin, C. H.; Chen, Y. S.; Chen, Y. Y.; Hwu, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Wu, S. R.; Hwu, Y.] Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 300, Taiwan. [Hwu, Y.] Natl Cheng Kung Univ, Adv Optoelect Technol Ctr, Tainan 701, Taiwan. [Chu, Y. S.] Brookhaven Natl Lab, NSLS 2, Upton, NY 11973 USA. [Margaritondo, G.] Ecole Polytech Fed Lausanne, Fac Sci Base, CH-1015 Lausanne, Switzerland. RP Hwu, Y (reprint author), Acad Sinica, Inst Phys, Taipei 115, Taiwan. EM phhwu@sinica.edu.tw RI Centre d'imagerie Biomedicale, CIBM/B-5740-2012 FU National Science and Technology Programme for Nanoscience and Nanotechnology; National Science Council; Academia Sinica; Fonds National Suisse pour la Recherche Scientifique; EPFL; Center for Biomedical Imaging (CIBM); Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; US Department of Energy, Office of Basic Energy Sciences, [DE-AC02-06CH11357] FX The authors thank all the colleagues from the Academia Sinica, the Mackay Memorial Hospital, the Tri-Service General Hospital, the Tsing Hua University, the National Synchrotron Radiation Research Center, the Argonne Advanced Photon Source, the Brookhaven National Synchrotron Light Source, the University of Bordeaux, the Ecole Polytechnique Federale de Lausanne (EPFL) and the Paul-Scherrer-Institut who participated in different stages of their imaging programmes. The research was supported by the National Science and Technology Programme for Nanoscience and Nanotechnology, the National Science Council, the Academia Sinica, the Fonds National Suisse pour la Recherche Scientifique, the EPFL, the Center for Biomedical Imaging (CIBM) and the Brookhaven Science Associates, LLC under Contract No DE-AC02-98CH10886. Use of the Advanced Photon Source is supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract No DE-AC02-06CH11357. NR 94 TC 4 Z9 4 U1 1 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD DEC 11 PY 2013 VL 46 IS 49 AR 494005 DI 10.1088/0022-3727/46/49/494005 PG 14 WC Physics, Applied SC Physics GA 264OH UT WOS:000327887500006 ER PT J AU Garcia-Sciveres, M Mekkaoui, A Ganani, D AF Garcia-Sciveres, M. Mekkaoui, A. Ganani, D. TI Towards third generation pixel readout chips SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 6th International Workshop on Semiconductor Pixel Detectors for Particles and Imaging (PIXEL) CY SEP 03-07, 2012 CL Inawashiro, JAPAN SP High Energy Accelerator Res Org, Japan Synchrotron Radiat Res Inst, RIKEN SPring 8 Ctr DE Hybrid pixel detectors; Readout integrated circuits; 65 im CMOS; Silicon detectors; LHC detectors AB We present concepts and prototyping results towards a third generation pixel readout chip. We consider the 130 am feature size FE-14 chip, in production for the ATLAS IBL upgrade, to be a second generation chip. A third generation chip would have to go significantly further. A possible direction is to make the IC design generic so that different experiments can configure it to meet significantly different requirements, without the need for everybody to develop their own ASIC from the ground up. In terms of target technology, a demonstrator 500-pixel matrix containing analog front ends only (no complex functionality), was designed and fabricated in 65 nm CMOS and irradiated with protons in December 2011 and May 2012. (C) 2013 Elsevier B.V. All rights reserved. C1 [Garcia-Sciveres, M.; Mekkaoui, A.; Ganani, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Garcia-Sciveres, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM mgarcia-sciveres@lbl.gov RI Gnani, Dario/J-6426-2012 OI Gnani, Dario/0000-0003-0464-9176 NR 10 TC 6 Z9 6 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 11 PY 2013 VL 731 BP 83 EP 87 DI 10.1016/j.nima.2013.04.023 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258VT UT WOS:000327487500017 ER PT J AU Aruntinov, D Barbero, M Gonella, L Hemperek, T Hugging, F Kruger, H Wermes, N Breugnon, P Chantepie, B Clemens, JC Fei, R Fougeron, D Godiot, S Pangaud, P Rozanov, A Garcia-Sciveres, M Mekkaoui, A AF Aruntinov, D. Barbero, M. Gonella, L. Hemperek, T. Huegging, F. Krueger, H. Wermes, N. Breugnon, P. Chantepie, B. Clemens, J. C. Fei, R. Fougeron, D. Godiot, S. Pangaud, P. Rozanov, A. Garcia-Sciveres, M. Mekkaoui, A. TI Experience with 3D integration technologies in the framework of the ATLAS pixel detector upgrade for the HL-LHC SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 6th International Workshop on Semiconductor Pixel Detectors for Particles and Imaging (PIXEL) CY SEP 03-07, 2012 CL Inawashiro, JAPAN SP High Energy Accelerator Res Org, Japan Synchrotron Radiat Res Inst, RIKEN SPring 8 Ctr DE 3D electronics; TSV; Pixel detector; ATLAS; HL-LHC AB 3D technologies are investigated for the upgrade of the ATLAS pixel detector at the HL-LHC. R&D focuses on both, IC design in 3D, as well as On post-processing 3D technologies such as Through Silicon Via (TSV). The first one uses a so-called via first technology, featuring the insertion of small aspect ratio TSV at the pixel level. As discussed in the paper, this technology can still present technical challenges for the industrial partners. The second one consists of etching the TSV via last. This technology is investigated to enable 4-side abuttable module concepts, using today's pixel detector technology. Both approaches are presented in this paper and results from first available prototypes are discussed. (C) 2013 Elsevier B.V. All rights reserved. C1 [Aruntinov, D.; Barbero, M.; Gonella, L.; Hemperek, T.; Huegging, F.; Krueger, H.; Wermes, N.] Univ Bonn, Inst Phys, Bonn, Germany. [Breugnon, P.; Chantepie, B.; Clemens, J. C.; Fei, R.; Fougeron, D.; Godiot, S.; Pangaud, P.; Rozanov, A.] CPPM, Marseille, France. [Garcia-Sciveres, M.; Mekkaoui, A.] Lawrence Berkeley Natl Lab, Oakland, CA 94611 USA. RP Gonella, L (reprint author), Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. EM gonella@physik.uni-bonn.de NR 10 TC 3 Z9 3 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 11 PY 2013 VL 731 BP 97 EP 102 DI 10.1016/j.nima.2013.04.044 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258VT UT WOS:000327487500020 ER PT J AU Peric, I Fischer, P Kreidl, C Nguyen, HH Augustin, H Berger, N Kiehn, M Perrevoort, AK Schoning, A Wiedner, D Feigl, S Heim, T Meng, LX Munstermann, D Benoit, M Dannheim, D Bompard, F Breugnon, P Clemens, JC Fougeron, D Liu, J Pangaud, P Rozanov, A Barbero, M Backhaus, M Hugging, F Kruger, H Lutticke, F Marinas, C Obermann, T Garcia-Sciveres, M Schwenker, B Dierlamm, A La Rosa, A Miucci, A AF Peric, Ivan Fischer, Peter Kreidl, Christian Hong Hanh Nguyen Augustin, Heiko Berger, Niklaus Kiehn, Moritz Perrevoort, Ann-Kathrin Schoening, Andre Wiedner, Dirk Feigl, Simon Heim, Timon Meng, Lingxin Muenstermann, Daniel Benoit, Mathieu Dannheim, Dominik Bompard, Frederic Breugnon, Patrick Clemens, Jean-Claude Fougeron, Denis Liu, Jian Pangaud, Patrick Rozanov, Alexandre Barbero, Marlon Backhaus, Malte Huegging, Fabian Krueger, Hans Luetticke, Florian Marinas, Carlos Obermann, Theresa Garcia-Sciveres, Maurice Schwenker, Benjamin Dierlamm, Alexander La Rosa, Alessandro Miucci, Antonio TI High-voltage pixel detectors in commercial CMOS technologies for ATLAS, CLIC and Mu3e experiments SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 6th International Workshop on Semiconductor Pixel Detectors for Particles and Imaging (PIXEL) CY SEP 03-07, 2012 CL Inawashiro, JAPAN SP High Energy Accelerator Res Org, Japan Synchrotron Radiat Res Inst, RIKEN SPring 8 Ctr DE High-voltage pixel detector; Smart-diode array; Capacitive coupled pixel detector; Mu3e ID PARTICLE-DETECTOR AB High-voltage particle detectors in commercial CMOS technologies are a detector family that allows implementation of low-cost, thin and radiation-tolerant detectors with a high time resolution. In the R/D phase of the development, a radiation tolerance of 10(15) n(eq)/cm(2), nearly 100% detection efficiency and a spatial resolution of about 3 mu m were demonstrated. Since 2011 the HV detectors have first applications: the technology is presently the main option for the pixel detector of the planned Mu3e experiment at PSI (Switzerland). Several prototype sensors have been designed in a standard 180 urn HV CMOS process and successfully tested. Thanks to its high radiation tolerance, the HV detectors are also seen at CERN as a promising alternative to the standard options for ATLAS upgrade and CLIC. In order to test the concept, within ATLAS upgrade R/D, we are currently exploring an active pixel detector demonstrator HV2FEl4; also implemented in the 180 nm HV process. (C ) 2013 Elsevier B.V. All rights reserved. C1 [Peric, Ivan; Fischer, Peter; Kreidl, Christian; Hong Hanh Nguyen] Heidelberg Univ, Inst Comp Engn, Mannheim, Germany. [Augustin, Heiko; Berger, Niklaus; Kiehn, Moritz; Perrevoort, Ann-Kathrin; Schoening, Andre; Wiedner, Dirk] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Feigl, Simon; Heim, Timon; Meng, Lingxin; Muenstermann, Daniel; Benoit, Mathieu; Dannheim, Dominik] CERN, Geneva, Switzerland. [Bompard, Frederic; Breugnon, Patrick; Clemens, Jean-Claude; Fougeron, Denis; Liu, Jian; Pangaud, Patrick; Rozanov, Alexandre; Barbero, Marlon] CPPM, Marseille, France. [Backhaus, Malte; Huegging, Fabian; Krueger, Hans; Luetticke, Florian; Marinas, Carlos; Obermann, Theresa] Univ Bonn, Inst Phys, Bonn, Germany. [Garcia-Sciveres, Maurice] LBNL, Berkeley, CA USA. [Schwenker, Benjamin] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Dierlamm, Alexander] KIT, Karlsruhe, Germany. [La Rosa, Alessandro; Miucci, Antonio] Univ Geneva, CH-1211 Geneva 4, Switzerland. RP Peric, I (reprint author), Heidelberg Univ, Inst Comp Engn, Mannheim, Germany. EM ivan.peric@ziti.uni-heidelberg.de OI La Rosa, Alessandro/0000-0001-6291-2142; Benoit, Mathieu/0000-0002-8623-1699 NR 12 TC 22 Z9 22 U1 2 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 11 PY 2013 VL 731 BP 131 EP 136 DI 10.1016/j.nima.2013.05.006 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258VT UT WOS:000327487500026 ER PT J AU Da Via, C Boscardin, M Dalla Betta, GF Haughton, I Grenier, P Grinstein, S Hansen, TE Hasi, J Kenney, C Kok, A Parker, S Pellegrini, G Povoli, M Tzhnevyi, V Watts, SJ AF Da Via, Cinzia Boscardin, Maurizio Dalla Betta, Gian-Franco Haughton, Iain Grenier, Philippe Grinstein, Sebastian Hansen, Thor-Erik Hasi, Jasmine Kenney, Christopher Kok, Angela Parker, Sherwood Pellegrini, Giulio Povoli, Marco Tzhnevyi, Vladislav Watts, Stephen J. TI Future trends of 3D silicon sensors SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 6th International Workshop on Semiconductor Pixel Detectors for Particles and Imaging (PIXEL) CY SEP 03-07, 2012 CL Inawashiro, JAPAN SP High Energy Accelerator Res Org, Japan Synchrotron Radiat Res Inst, RIKEN SPring 8 Ctr DE 3D silicon sensor; ATLAS IBL; LHC upgrade; Pixels; Radiation hardness; Micro-channel cooling ID DETECTORS AB Vertex detectors for the next LHC experiments upgrades will need to have low mass while at the same Lime be radiation hard and with sufficient granularity to fulfil the physics challenges of the next decade. Based on the gained experience with 3D silicon sensors for the ATLAS IBL project and the oil going developments on light materials, interconnectivity and cooling, this paper will discuss possible solutions to these requirements. (C) 2013 Elsevier B.V. All rights reserved. C1 [Da Via, Cinzia; Haughton, Iain; Tzhnevyi, Vladislav; Watts, Stephen J.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Boscardin, Maurizio] FBK CMM, Fdn Bruno Kessler, I-38123 Trento, Italy. [Dalla Betta, Gian-Franco; Povoli, Marco] Univ Trento, DISI, I-38123 Trento, Italy. [Dalla Betta, Gian-Franco; Povoli, Marco] Ist Nazl Fis Nucl, I-38123 Trento, Italy. [Grenier, Philippe; Hasi, Jasmine; Kenney, Christopher] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Grinstein, Sebastian] UAB, IFAE, E-08193 Bellaterra, Barcelona, Spain. [Grinstein, Sebastian] UAB, ICREA, E-08193 Bellaterra, Barcelona, Spain. [Hansen, Thor-Erik; Kok, Angela] SINTEF MiNaLab, N-0314 Oslo, Norway. [Parker, Sherwood] Univ Hawaii, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Pellegrini, Giulio] CNM IMB CSIC, Ctr Nacl Microelect, E-08193 Barcelona, Spain. RP Da Via, C (reprint author), Univ Manchester, Sch Phys & Astron, Oxford Rd, Manchester M13 9PL, Lancs, England. EM cinzia.da.via@cern.ch RI Boscardin, Maurizio/A-4420-2014; Dalla Betta, Gian-Franco/I-1783-2012; Grinstein, Sebastian/N-3988-2014; Pellegrini, Giulio/F-4921-2011 OI Dalla Betta, Gian-Franco/0000-0001-5516-9282; Grinstein, Sebastian/0000-0002-6460-8694; Pellegrini, Giulio/0000-0002-1606-3546 NR 17 TC 5 Z9 5 U1 0 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD DEC 11 PY 2013 VL 731 BP 201 EP 204 DI 10.1016/j.nima.2013.05.048 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258VT UT WOS:000327487500039 ER PT J AU Ehlers, G Podlesnyak, AA Frontzek, M Freitas, RS Ghivelder, L Gardner, JS Shiryaev, SV Barilo, S AF Ehlers, G. Podlesnyak, A. A. Frontzek, M. Freitas, R. S. Ghivelder, L. Gardner, J. S. Shiryaev, S. V. Barilo, S. TI A detailed study of the magnetic phase transition in CuCrO2 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID SPIN-ECHO SPECTROSCOPY AB The phase transition in CuCrO2 to an ordered magnetic state is studied with bulk measurements and elastic and inelastic neutron scattering techniques. The reported onset of spontaneous electric polarization at T D 23.5 K coincides with the appearance, on cooling, of elastic magnetic scattering. At higher temperatures long range magnetic correlations gradually develop but they are dynamic. The ground state is characterized by three-dimensional long range magnetic ordering but along the c direction the correlation length remains limited to similar to 200 angstrom. C1 [Ehlers, G.; Podlesnyak, A. A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Frontzek, M.] Paul Scherrer Inst, Neutron Scattering Lab, CH-5232 Villigen, Switzerland. [Freitas, R. S.] Univ Sao Paulo, Inst Fis, BR-05314970 Sao Paulo, Brazil. [Ghivelder, L.] Univ Fed Rio de Janeiro, Inst Fis, BR-21941972 Rio De Janeiro, RJ, Brazil. [Gardner, J. S.] Indiana Univ, Dept Phys, Bloomington, IN 47408 USA. [Gardner, J. S.] NIST, NCNR, Gaithersburg, MD 20899 USA. [Gardner, J. S.] Natl Synchrotron Radiat Res Ctr, Neutron Grp, Hsinchu 30077, Taiwan. [Shiryaev, S. V.; Barilo, S.] Inst Solid State & Semicond Phys, Minsk 220072, Byelarus. RP Ehlers, G (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. EM ehlersg@ornl.gov RI Freitas, Rafael/K-1034-2013; GHIVELDER, LUIS/L-1820-2015; Instrument, CNCS/B-4599-2012; Ehlers, Georg/B-5412-2008; Podlesnyak, Andrey/A-5593-2013; Frontzek, Matthias/C-5146-2012 OI GHIVELDER, LUIS/0000-0002-5667-6531; Ehlers, Georg/0000-0003-3513-508X; Podlesnyak, Andrey/0000-0001-9366-6319; Frontzek, Matthias/0000-0001-8704-8928 FU National Science Foundation [DMR-0944772]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; FAPESP; CNPq-Brazil FX The authors are grateful to the local support staff at SNS and at NIST. The NCNR is in part funded by the National Science Foundation under Agreement No. DMR-0944772. The identification of any commercial product or trade name does not imply endorsement or recommendation by the National Institute of Standards and Technology. Research at Oak Ridge National Laboratory's Spallation Neutron Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. RSF acknowledges support from FAPESP and CNPq-Brazil. NR 21 TC 0 Z9 0 U1 4 U2 25 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD DEC 11 PY 2013 VL 25 IS 49 DI 10.1088/0953-8984/25/49/49600 PG 6 WC Physics, Condensed Matter SC Physics GA 254QU UT WOS:000327181400022 ER PT J AU Van Ginhoven, RM Schultz, PA AF Van Ginhoven, R. M. Schultz, P. A. TI Off-center Tl and Na dopant centers in CsI SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID EXCITED-STATE STRUCTURE; DECAY KINETICS; ALKALI HALIDES; CESIUM-HALIDES; LUMINESCENCE; ABSORPTION; CRYSTALS; PSEUDOPOTENTIALS; SCINTILLATORS; DISTORTIONS AB We use density functional theory calculations to characterize the electronic and structural properties of the Tl and Na dopant centers in CsI. We find that the Tl and Na centers can accept one or two electrons and couple to long-range relaxations in the surrounding crystal lattice to distort strongly off-center to multiple distinct minima, even without a triplet excitation. The long-range distortions are a mechanism to couple to phonon modes in the crystal, and are expected to play an important role in the phonon-assisted transport of polarons in activated CsI and subsequent light emission in this scintillator. C1 [Van Ginhoven, R. M.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Schultz, P. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Van Ginhoven, RM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Renee.VanGinhoven@pnnl.gov; paschul@sandia.gov FU Office of Nuclear Nonproliferation Research and Engineering [NA22]; US Department of Energy; Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory; Sandia Corporation; Lockheed Martin Corporation; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This project is supported by Office of Nuclear Nonproliferation Research and Engineering (NA22), the US Department of Energy. The research was performed in part using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 32 TC 0 Z9 0 U1 1 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD DEC 11 PY 2013 VL 25 IS 49 AR 495504 DI 10.1088/0953-8984/25/49/495504 PG 6 WC Physics, Condensed Matter SC Physics GA 254QU UT WOS:000327181400009 PM 24196783 ER PT J AU Huang, ZS Arovas, DP Balatsky, AV AF Huang, Zhoushen Arovas, Daniel P. Balatsky, Alexander V. TI Impurity scattering in Weyl semimetals and their stability classification SO NEW JOURNAL OF PHYSICS LA English DT Article ID TOPOLOGICAL INSULATORS; SUPERCONDUCTORS; PHASE AB Weyl semimetals (WS) are a new class of Dirac-type materials exhibiting a phase with bulk energy nodes and an associated vanishing density of states (DOS). We investigate the stability of this nodal DOS suppression in the presence of local impurities and consider whether or not such a suppression can be lifted by impurity-induced resonances. We find that while a scalar (chemical potential type) impurity can always induce a resonance at arbitrary energy and hence lift the DOS suppression at Dirac/Weyl nodes, for many other impurity types (e.g. magnetic or orbital mixing), resonances are forbidden in a wide range of energy. We investigate a four-band tight-binding model of WS adapted from a physical heterostructure construction due to Burkov et al (2011 Phys. Rev. B 84 235126), and represent a local impurity potential by a strength g as well as a matrix structure Lambda. A general framework is developed to analyze this resonance dichotomy and make connection with the phase shift picture in scattering theory, as well as to determine the relation between resonance energy and impurity strength g. A complete classification of impurities based on Lambda, based on their effect on nodal DOS suppression, is tabulated. We also discuss the differences between continuum and lattice approaches. C1 [Huang, Zhoushen; Arovas, Daniel P.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Balatsky, Alexander V.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] Nord Inst Theoret Phys NORDITA, S-10691 Stockholm, Sweden. RP Huang, ZS (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM zhohuang@physics.ucsd.edu FU NSF [DMR-1007028]; US DoE Basic Energy Sciences; Center for Integrated Nanotechnologies; US Department of Energy [DE-AC52-06NA25396]; [ERC-DM321031]; [VR-621-2012-2983] FX We are grateful to A Black-Schaffer, Tanmoy Das and Da Wang for useful discussions. This work was supported in part by the NSF through grant DMR-1007028. Work at LANL was supported by US DoE Basic Energy Sciences and in part by the Center for Integrated Nanotechnologies, operated by LANS, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. Work at Nordita was supported by ERC-DM321031 and VR-621-2012-2983. NR 32 TC 14 Z9 14 U1 4 U2 24 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD DEC 10 PY 2013 VL 15 AR 123019 DI 10.1088/1367-2630/15/12/123019 PG 29 WC Physics, Multidisciplinary SC Physics GA 286BB UT WOS:000329438400003 ER PT J AU Jiang, YY Lu, GR Trescott, LR Hou, YN Guan, XQ Wang, S Stamenkovich, A Brunzelle, J Sirinupong, N Li, CY Yang, Z AF Jiang, Yuanyuan Lu, Guorong Trescott, Laura R. Hou, Yuning Guan, Xiaoqing Wang, Shuo Stamenkovich, Angelique Brunzelle, Joseph Sirinupong, Nualpun Li, Chunying Yang, Zhe TI New Conformational State of NHERF1-CXCR2 Signaling Complex Captured by Crystal Lattice Trapping SO PLOS ONE LA English DT Article ID TRANSMEMBRANE CONDUCTANCE REGULATOR; CXCR2 MACROMOLECULAR COMPLEX; PDZ DOMAINS; BINDING SELECTIVITY; PROTEIN; FLEXIBILITY; DYNAMICS; PROMISCUITY; RECOGNITION; SPECIFICITY AB NHERF1 is a PDZ adaptor protein that scaffolds the assembly of diverse signaling complexes and has been implicated in many cancers. However, little is known about the mechanism responsible for its scaffolding promiscuity or its ability to bind to multiple targets. Computational studies have indicated that PDZ promiscuity may be attributed to its conformational dynamics, but experimental evidence for this relationship remains very limited. Here we examine the conformational flexibility of the NHERF1 PDZ1 domain using crystal lattice trapping via solving PDZ1 structure of a new crystal form. The structure, together with prior PDZ1 structures of a different space group, reveals that 4 of 11 ligand-interacting residues undergo significant crystal packing-induced structural changes. Most of these residues correspond to the residues involved in allosteric transition when a peptide ligand binds. In addition, a subtle difference in ligand conformations causes the same peptide to bind in slightly different modes in different crystal forms. These findings indicate that substantial structural flexibility is present in the PDZ1 peptide-binding pocket, and the structural substate trapped in the present crystal form can be utilized to represent the conformational space accessible to the protein. Such knowledge will be critical for drug design against the NHERF1 PDZ1 domain, highlighting the continued need for experimentally determined PDZ1-ligand complexes. C1 [Jiang, Yuanyuan; Lu, Guorong; Trescott, Laura R.; Hou, Yuning; Guan, Xiaoqing; Wang, Shuo; Stamenkovich, Angelique; Li, Chunying; Yang, Zhe] Wayne State Univ, Sch Med, Dept Biochem & Mol Biol, Detroit, MI 48202 USA. [Brunzelle, Joseph] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Sirinupong, Nualpun] Prince Songkla Univ, Nutraceut & Funct Food Res & Dev Ctr, Hat Yai, Songkhla, Thailand. RP Li, CY (reprint author), Wayne State Univ, Sch Med, Dept Biochem & Mol Biol, Detroit, MI 48202 USA. EM cl@med.wayne.edu; zyang@med.wayne.edu FU Leukemia Research Foundation; Aplastic Anemia & MDS International Foundation; Elsa U. Pardee Foundation; American Heart Association; American Cancer Society [11-053-01-IRG] FX This study was supported by the Leukemia Research Foundation (to ZY) and the Aplastic Anemia & MDS International Foundation (to ZY), as well as the Elsa U. Pardee Foundation (to CL), American Heart Association (to CL), and American Cancer Society Institutional Research Grant (# 11-053-01-IRG) (to CL). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 43 TC 3 Z9 3 U1 0 U2 3 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 10 PY 2013 VL 8 IS 12 AR e81904 DI 10.1371/journal.pone.0081904 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 275VW UT WOS:000328707400052 PM 24339979 ER PT J AU Legros, M Xu, CG Morrison, A Scott, TW Lloyd, AL Gould, F AF Legros, Mathieu Xu, Chonggang Morrison, Amy Scott, Thomas W. Lloyd, Alun L. Gould, Fred TI Modeling the Dynamics of a Non- Limited and a Self-Limited Gene Drive System in Structured Aedes aegypti Populations SO PLOS ONE LA English DT Article ID MOSQUITO-BORNE DISEASES; ENGINEERED UNDERDOMINANCE; CULICIDAE PRODUCTION; INSECT POPULATIONS; RNA INTERFERENCE; PEST POPULATIONS; VIRUS-RESISTANCE; MEIOTIC DRIVE; TRANSGENES; DIPTERA AB Recently there have been significant advances in research on genetic strategies to control populations of disease-vectoring insects. Some of these strategies use the gene drive properties of selfish genetic elements to spread physically linked anti-pathogen genes into local vector populations. Because of the potential of these selfish elements to spread through populations, control approaches based on these strategies must be carefully evaluated to ensure a balance between the desirable spread of the refractoriness-conferring genetic cargo and the avoidance of potentially unwanted outcomes such as spread to non-target populations. There is also a need to develop better estimates of the economics of such releases. We present here an evaluation of two such strategies using a biologically realistic mathematical model that simulates the resident Aedes aegypti mosquito population of Iquitos, Peru. One strategy uses the selfish element Medea, a non-limited element that could permanently spread over a large geographic area; the other strategy relies on Killer-Rescue genetic constructs, and has been predicted to have limited spatial and temporal spread. We simulate various operational approaches for deploying these genetic strategies, and quantify the optimal number of released transgenic mosquitoes needed to achieve definitive spread of Medea-linked genes and/or high frequencies of Killer-Rescue-associated elements. We show that for both strategies the most efficient approach for achieving spread of anti-pathogen genes within three years is generally to release adults of both sexes in multiple releases over time. Even though females in these releases should not transmit disease, there could be public concern over such releases, making the less efficient male-only release more practical. This study provides guidelines for operational approaches to population replacement genetic strategies, as well as illustrates the use of detailed spatial models to assist in safe and efficient implementation of such novel genetic strategies. C1 [Legros, Mathieu; Xu, Chonggang; Gould, Fred] N Carolina State Univ, Dept Entomol, Raleigh, NC 27695 USA. [Legros, Mathieu; Morrison, Amy; Scott, Thomas W.] Univ Calif Davis, Dept Entomol, Davis, CA 95616 USA. [Legros, Mathieu] ETH, Inst Integrat Biol, Zurich, Switzerland. [Xu, Chonggang] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Morrison, Amy; Scott, Thomas W.; Lloyd, Alun L.; Gould, Fred] NIH, Fogarty Int Ctr, Bethesda, MD 20892 USA. [Lloyd, Alun L.] N Carolina State Univ, Dept Math, Raleigh, NC 27695 USA. [Lloyd, Alun L.] N Carolina State Univ, Biomath Grad Program, Raleigh, NC 27695 USA. RP Legros, M (reprint author), N Carolina State Univ, Dept Entomol, Raleigh, NC 27695 USA. EM legros.mathieu@gmail.com RI Legros, Mathieu/E-6767-2011; OI Legros, Mathieu/0000-0003-3807-8594; Xu, Chonggang/0000-0002-0937-5744 FU National Institutes of Health [R01-AI54954-0IA2]; Regents of the University of California from the Foundation for the National Institutes of Health Grand Challenges in Global Health initiative FX This work was funded by National Institutes of Health grant R01-AI54954-0IA2, and through the Regents of the University of California from the Foundation for the National Institutes of Health Grand Challenges in Global Health initiative. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 36 TC 5 Z9 5 U1 3 U2 10 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 10 PY 2013 VL 8 IS 12 AR UNSP e83354 DI 10.1371/journal.pone.0083354 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 275VW UT WOS:000328707400130 PM 24340097 ER PT J AU Aliu, E Archambault, S Behera, B Berger, K Beilicke, M Benbow, W Bird, R Bouvier, A Bugaev, V Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Dumm, J Falcone, A Federici, S Feng, Q Finley, JP Fortin, P Fortson, L Furniss, A Galante, N Gillanders, GH Griffin, S Griffiths, ST Grube, J Gyuk, G Hanna, D Holder, J Hughes, G Humensky, TB Kaaret, P Kertzman, M Khassen, Y Kieda, D Krennrich, F Lang, MJ Maier, G Majumdar, P McArthur, S McCann, A Moriarty, P Mukherjee, R de Bhroithe, AO Ong, RA Otte, AN Park, N Perkins, JS Pohl, M Popkow, A Prokoph, H Quinn, J Ragan, K Rajotte, J Ratliff, G Reynolds, PT Richards, GT Roache, E Sembroski, GH Sheidaei, F Skole, C Smith, AW Staszak, D Telezhinsky, I Tyler, J Varlotta, A Vincent, S Wakely, SP Weekes, TC Weinstein, A Welsing, R Zajczyk, A Zitzer, B AF Aliu, E. Archambault, S. Behera, B. Berger, K. Beilicke, M. Benbow, W. Bird, R. Bouvier, A. Bugaev, V. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Dumm, J. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortin, P. Fortson, L. Furniss, A. Galante, N. Gillanders, G. H. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krennrich, F. Lang, M. J. Maier, G. Majumdar, P. McArthur, S. McCann, A. Moriarty, P. Mukherjee, R. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Prokoph, H. Quinn, J. Ragan, K. Rajotte, J. Ratliff, G. Reynolds, P. T. Richards, G. T. Roache, E. Sembroski, G. H. Sheidaei, F. Skole, C. Smith, A. W. Staszak, D. Telezhinsky, I. Tyler, J. Varlotta, A. Vincent, S. Wakely, S. P. Weekes, T. C. Weinstein, A. Welsing, R. Zajczyk, A. Zitzer, B. TI MULTIWAVELENGTH OBSERVATIONS OF THE TeV BINARY LS I+61 degrees 303 WITH VERITAS, Fermi-LAT, AND Swift/XRT DURING A TeV OUTBURST SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; binaries: general; gamma rays: stars; relativistic processes; X-rays: binaries ID GAMMA-RAY BINARY; X-RAY; EMISSION; +61-DEGREES-303; TELESCOPE; SPECTRUM; STAR AB We present the results of a multiwavelength observational campaign on the TeV binary system LS I +61 degrees 303 with the VERITAS telescope array (>200 GeV), Fermi-LAT (0.3-300 GeV), and Swift/XRT (2-10 keV). The data were taken from 2011 December through 2012 January and show a strong detection in all three wavebands. During this period VERITAS obtained 24.9 hr of quality selected livetime data in which LS I +61 degrees 303 was detected at a statistical significance of 11.9 sigma. These TeV observations show evidence for nightly variability in the TeV regime at a post-trial significance of 3.6 sigma. The combination of the simultaneously obtained TeV and X-ray fluxes do not demonstrate any evidence for a correlation between emission in the two bands. For the first time since the launch of the Fermi satellite in 2008, this TeV detection allows the construction of a detailed MeV-TeV spectral energy distribution from LS I +61 degrees 303. This spectrum shows a distinct cutoff in emission near 4 GeV, with emission seen by the VERITAS observations following a simple power-law above 200 GeV. This feature in the spectrum of LS I +61 degrees 303, obtained from overlapping observations with Fermi-LAT and VERITAS, may indicate that there are two distinct populations of accelerated particles producing the GeV and TeV emission. C1 [Aliu, E.; Humensky, T. B.; Mukherjee, R.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Archambault, S.; Griffin, S.; Hanna, D.; Ragan, K.; Rajotte, J.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Behera, B.; Chen, X.; Federici, S.; Hughes, G.; Maier, G.; Pohl, M.; Prokoph, H.; Skole, C.; Telezhinsky, I.; Vincent, S.; Welsing, R.] DESY, D-15738 Zeuthen, Germany. [Berger, K.; Holder, J.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Berger, K.; Holder, J.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Beilicke, M.; Bugaev, V.; Zajczyk, A.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Cerruti, M.; Fortin, P.; Galante, N.; Roache, E.; Weekes, T. C.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Bird, R.; Khassen, Y.; de Bhroithe, A. O'Faolain; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Bouvier, A.; Furniss, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Bouvier, A.; Furniss, A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Chen, X.; Federici, S.; Pohl, M.; Telezhinsky, I.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.; Ratliff, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Gillanders, G. H.; Lang, M. J.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Cui, W.; Feng, Q.; Finley, J. P.; Sembroski, G. H.; Varlotta, A.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Dumm, J.; Fortson, L.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Griffiths, S. T.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Kieda, D.; Sheidaei, F.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Krennrich, F.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Majumdar, P.; Ong, R. A.; Popkow, A.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Majumdar, P.] Saha Inst Nucl Phys, Kolkata 700064, W Bengal, India. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Galway, Ireland. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Perkins, J. S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. [Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Aliu, E (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. EM sheidaei@physics.utah.edu; aw.smith@utah.edu RI Khassen, Yerbol/I-3806-2015; OI Khassen, Yerbol/0000-0002-7296-3100; Cui, Wei/0000-0002-6324-5772 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the U.K. FX This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748) and by STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. We thank the Swift Team for scheduling contemporaneous observations and providing data and analysis tools. The authors would also like to thank Jeremy Perkins for his tireless assistance with Fermi-LAT data analysis. NR 40 TC 5 Z9 5 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 10 PY 2013 VL 779 IS 1 AR UNSP 88 DI 10.1088/0004-637X/779/1/88 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268HD UT WOS:000328160100088 ER PT J AU Bothwell, MS Aguirre, JE Chapman, SC Marrone, DP Vieira, JD Ashby, MLN Aravena, M Benson, BA Bock, JJ Bradford, CM Brodwin, M Carlstrom, JE Crawford, TM De Breuck, C Downes, TP Fassnacht, CD Gonzalez, AH Greve, TR Gullberg, B Hezaveh, Y Holder, GP Holzapfel, WL Ibar, E Ivison, R Kamenetzky, J Keisler, R Lupu, RE Ma, J Malkan, M McIntyre, V Murphy, EJ Nguyen, HT Reichardt, CL Rosenman, M Spilker, JS Stalder, B Stark, AA Strandet, M Vernet, J Weiss, A Welikala, N AF Bothwell, M. S. Aguirre, J. E. Chapman, S. C. Marrone, D. P. Vieira, J. D. Ashby, M. L. N. Aravena, M. Benson, B. A. Bock, J. J. Bradford, C. M. Brodwin, M. Carlstrom, J. E. Crawford, T. M. De Breuck, C. Downes, T. P. Fassnacht, C. D. Gonzalez, A. H. Greve, T. R. Gullberg, B. Hezaveh, Y. Holder, G. P. Holzapfel, W. L. Ibar, E. Ivison, R. Kamenetzky, J. Keisler, R. Lupu, R. E. Ma, J. Malkan, M. McIntyre, V. Murphy, E. J. Nguyen, H. T. Reichardt, C. L. Rosenman, M. Spilker, J. S. Stalder, B. Stark, A. A. Strandet, M. Vernet, J. Weiss, A. Welikala, N. TI SPT 0538-50: PHYSICAL CONDITIONS IN THE INTERSTELLAR MEDIUM OF A STRONGLY LENSED DUSTY STAR-FORMING GALAXY AT z=2.8 SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: evolution; galaxies: formation; galaxies: high-redshift; galaxies: individual; gravitational lensing: strong; submillimeter: galaxies ID ULTRALUMINOUS INFRARED GALAXIES; SOUTH-POLE TELESCOPE; LUMINOUS SUBMILLIMETER GALAXIES; HERSCHEL-SPIRE SPECTROSCOPY; SCIENCE DEMONSTRATION PHASE; SPITZER-SPACE-TELESCOPE; INITIAL MASS FUNCTION; MOLECULAR GAS; HIGH-REDSHIFT; FORMATION HISTORY AB We present observations of SPT-S J053816-5030.8, a gravitationally lensed dusty star-forming galaxy (DSFG) at z = 2.7817 that was first discovered at millimeter wavelengths by the South Pole Telescope. SPT 0538-50 is typical of the brightest sources found by wide-field millimeter-wavelength surveys, being lensed by an intervening galaxy at moderate redshift (in this instance, at z = 0.441). We present a wide array of multi-wavelength spectroscopic and photometric data on SPT 0538-50, including data from ALMA, Herschel PACS and SPIRE, Hubble, Spitzer, the Very Large Telescope, ATCA, APEX, and the Submillimeter Array. We use high-resolution imaging from the Hubble Space Telescope to de-blend SPT 0538-50, separating DSFG emission from that of the foreground lens. Combined with a source model derived from ALMA imaging (which suggests a magnification factor of 21+/-4), we derive the intrinsic properties of SPT 0538-50, including the stellar mass, far-IR luminosity, star formation rate, molecular gas mass, and-using molecular line fluxes-the excitation conditions within the interstellar medium. The derived physical properties argue that we arewitnessing compact, merger-driven star formation in SPT 0538-50 similar to local starburst galaxies and unlike that seen in some other DSFGs at this epoch. C1 [Bothwell, M. S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HA, England. [Bothwell, M. S.; Marrone, D. P.; Spilker, J. S.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [Aguirre, J. E.; Lupu, R. E.; Rosenman, M.] Univ Penn, Philadelphia, PA 19104 USA. [Chapman, S. C.] Dalhousie Univ, Halifax, NS, Canada. [Vieira, J. D.; Bock, J. J.; Downes, T. P.] CALTECH, Pasadena, CA 91125 USA. [Ashby, M. L. N.; Stalder, B.; Stark, A. A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Aravena, M.; De Breuck, C.; Gullberg, B.; Vernet, J.] European So Observ, Casilla 19001, Vitacura Santia, Chile. [Aravena, M.] Univ Diego Portales, Fac Ingn, Santiago, Chile. [Benson, B. A.; Carlstrom, J. E.; Keisler, R.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Benson, B. A.; Carlstrom, J. E.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Bock, J. J.; Bradford, C. M.; Nguyen, H. T.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Brodwin, M.] Univ Missouri, Dept Phys & Astron, Kansas City, MO 64110 USA. [Carlstrom, J. E.; Keisler, R.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Carlstrom, J. E.; Crawford, T. M.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Carlstrom, J. E.] Argonne Natl Lab, Argonne, IL 60439 USA. [Fassnacht, C. D.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Gonzalez, A. H.; Ma, J.] Univ Florida, Dept Astron, Gainesville, FL 32611 USA. [Greve, T. R.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Hezaveh, Y.; Holder, G. P.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Holzapfel, W. L.; Reichardt, C. L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ibar, E.] Pontificia Univ Catolica Chile, Fac Fis, Inst Astrofis, Santiago 22, Chile. [Ivison, R.] Inst Astron, Edinburgh EH9 3HJ, Midlothian, Scotland. [Kamenetzky, J.] Univ Colorado, Ctr Astrophys & Space Astron, Boulder, CO 80309 USA. [Malkan, M.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [McIntyre, V.] CSIRO, Australia Telescope Natl Facil, Epping, NSW 1710, Australia. [Murphy, E. J.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Strandet, M.; Weiss, A.] Max Planck Inst Radioastron, D-53121 Bonn, Germany. [Welikala, N.] Univ Paris Diderot, CNRS IN2P3, CEA Irfu, Observ Paris,Sorbonne Paris Cite, F-75205 Paris 13, France. RP Bothwell, MS (reprint author), Univ Cambridge, Cavendish Lab, JJ Thompson Ave, Cambridge CB3 0HA, England. RI Aravena, Manuel/O-2361-2014; Lupu, Roxana/P-9060-2014; Holzapfel, William/I-4836-2015; Ivison, R./G-4450-2011; OI Lupu, Roxana/0000-0003-3444-5908; Ivison, R./0000-0001-5118-1313; Marrone, Daniel/0000-0002-2367-1080; Reichardt, Christian/0000-0003-2226-9169; Vernet, Joel/0000-0002-8639-8560; De Breuck, Carlos/0000-0002-6637-3315; Stark, Antony/0000-0002-2718-9996 FU Smithsonian Institution; Academia Sinica; National Science Foundation [AST-1009649, ANT-0638937, PHY-1125897, PHYS-1066293]; NASA from the Space Telescope Science Institute [HST-GO-12659]; JPL/Caltech [OT1_dmarrone_1, OT1_jvieira_4, OT2_jvieira_5] FX We thank the anonymous referee who provided comments that helped improve the clarity of this manuscript. The authors would like to thank N. Rangwala for sharing the M82 CO flux densities. M. S. B. would like to acknowledge the hospitality of the Aspen Center for Physics, where some of this manuscript was written. The Submillimeter Array is a joint project between the Smithsonian Astrophysical Observatory and the Academia Sinica Institute of Astronomy and Astrophysics and is funded by the Smithsonian Institution and the Academia Sinica. Support is provided by National Science Foundation grants AST-1009649, ANT-0638937, PHY-1125897, and PHYS-1066293. This paper makes use of the following ALMA data: ADS/JAO. ALMA #2011.0.00957.S and #2011.0.00958.S. ALMA is a partnership of ESO (representing its member states), NSF (USA) and NINS (Japan), together with NRC (Canada) and NSC and ASIAA (Taiwan), in cooperation with the Republic of Chile. The Joint ALMA Observatory is operated by ESO, AUI/NRAO, and NAOJ. The National Radio Astronomy Observatory is a facility of the National Science Foundation operated under a cooperative agreement by Associated Universities, Inc. Partial support for this work was provided by NASA through grant HST-GO-12659 from the Space Telescope Science Institute and awards for Herschel analysis issued by JPL/Caltech for OT1_dmarrone_1, OT1_jvieira_4, and OT2_jvieira_5. NR 86 TC 17 Z9 17 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 10 PY 2013 VL 779 IS 1 AR 67 DI 10.1088/0004-637X/779/1/67 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268HD UT WOS:000328160100067 ER PT J AU Dominik, M Belczynski, K Fryer, C Holz, DE Berti, E Bulik, T Mandel, I O'Shaughnessy, R AF Dominik, Michal Belczynski, Krzysztof Fryer, Christopher Holz, Daniel E. Berti, Emanuele Bulik, Tomasz Mandel, Ilya O'Shaughnessy, Richard TI DOUBLE COMPACT OBJECTS. II. COSMOLOGICAL MERGER RATES SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: miscellaneous; stars: black holes; stars: neutron ID GAMMA-RAY BURSTS; STAR-FORMATION HISTORY; STELLAR BLACK-HOLES; CLOSE BINARY STARS; MASSIVE STARS; GRAVITATIONAL-WAVES; EXPLOSION MECHANISM; COMMON ENVELOPE; TIDAL EVOLUTION; METALLICITY AB The development of advanced gravitational wave (GW) observatories, such as Advanced LIGO and Advanced Virgo, provides impetus to refine theoretical predictions for what these instruments might detect. In particular, with the range increasing by an order of magnitude, the search for GWsources is extending beyond the "local" universe and out to cosmological distances. Double compact objects (neutron star-neutron star (NS-NS), black hole-neutron star (BH-NS), and black hole-black hole (BH-BH) systems) are considered to be the most promising GW sources. In addition, NS-NS and/or BH-NS systems are thought to be the progenitors of gamma-ray bursts and may also be associated with kilonovae. In this paper, we present the merger event rates of these objects as a function of cosmological redshift. We provide the results for four cases, each one investigating a different important evolution parameter of binary stars. Each case is also presented for two metallicity evolution scenarios. We find that (1) in most cases NS-NS systems dominate the merger rates in the local universe, while BH-BH mergers dominate at high redshift, (2) BH-NS mergers are less frequent than other sources per unit volume, for all time, and (3) natal kicks may alter the observable properties of populations in a significant way, allowing the underlying models of binary evolution and compact object formation to be easily distinguished. This is the second paper in a series of three. The third paper will focus on calculating the detection rates of mergers by GW telescopes. C1 [Dominik, Michal; Belczynski, Krzysztof; Bulik, Tomasz] Univ Warsaw, Astron Observ, PL-00478 Warsaw, Poland. [Belczynski, Krzysztof] Univ Texas Brownsville, Ctr Gravitat Wave Astron, Brownsville, TX 78520 USA. [Fryer, Christopher] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Holz, Daniel E.] Univ Chicago, Dept Phys, Enrico Fermi Inst, Chicago, IL 60637 USA. [Holz, Daniel E.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Berti, Emanuele] Univ Mississippi, Dept Phys & Astron, University, MS 38677 USA. [Berti, Emanuele] CALTECH, Pasadena, CA 91109 USA. [Mandel, Ilya] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [O'Shaughnessy, Richard] Univ Wisconsin, Milwaukee, WI 53217 USA. RP Dominik, M (reprint author), Univ Warsaw, Astron Observ, Al Ujazdowskie 4, PL-00478 Warsaw, Poland. RI Berti, Emanuele/C-9331-2016; OI Berti, Emanuele/0000-0003-0751-5130; O'Shaughnessy, Richard/0000-0001-5832-8517; Mandel, Ilya/0000-0002-6134-8946 FU National Science Foundation CAREER [PHY-1151836, PHY-1055103]; MSHE [N203 404939, N203 511238]; NASA [NNX09AV06A]; Polish Science Foundation; National Science Center [DEC-2011/01/N/ST9/00383]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AO52-06NA25396]; [DPN/N176/VIRGO/2009] FX We thank Alexander Heger for a helpful discussion on pair-instability supernovae. We also thank the N. Copernicus Astronomical Centre in Warsaw, Poland and the University Of Texas, Brownsville, TX, for providing computational resources. D. E. H. acknowledges support from National Science Foundation CAREER grant PHY-1151836. K. B. and M. D. acknowledge support from MSHE grant N203 404939 and N203 511238, NASA Grant NNX09AV06A to the UTB, Polish Science Foundation Master 2013 Subsidy and National Science Center DEC-2011/01/N/ST9/00383. T. B. was supported by the DPN/N176/VIRGO/2009 grant. E. B. acknowledges support from National Science Foundation CAREER grant No. PHY-1055103. Work by C. L. F. was done under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy under contract No. DE-AO52-06NA25396. NR 62 TC 69 Z9 69 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 10 PY 2013 VL 779 IS 1 AR 72 DI 10.1088/0004-637X/779/1/72 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268HD UT WOS:000328160100072 ER PT J AU Furst, F Grefenstette, BW Staubert, R Tomsick, JA Bachetti, M Barret, D Bellm, EC Boggs, SE Chenevez, J Christensen, FE Craig, WW Hailey, CJ Harrison, F Klochkov, D Madsen, KK Pottschmidt, K Stern, D Walton, DJ Wilms, J Zhang, W AF Fuerst, Felix Grefenstette, Brian W. Staubert, Ruediger Tomsick, John A. Bachetti, Matteo Barret, Didier Bellm, Eric C. Boggs, Steven E. Chenevez, Jerome Christensen, Finn E. Craig, William W. Hailey, Charles J. Harrison, Fiona Klochkov, Dmitry Madsen, Kristin K. Pottschmidt, Katja Stern, Daniel Walton, Dominic J. Wilms, Joern Zhang, William TI THE SMOOTH CYCLOTRON LINE IN HER X-1 AS SEEN WITH NUCLEAR SPECTROSCOPIC TELESCOPE ARRAY SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; pulsars: individual (Her X-1); stars: neutron; X-rays: binaries ID X-RAY PULSARS; PHASE-RESOLVED SPECTROSCOPY; 35 DAY EVOLUTION; ACCRETION DISK; MAGNETIC-FIELDS; NEUTRON-STAR; HERCULES X-1; LIGHT-CURVE; MAIN-ON; RXTE AB Her X-1, one of the brightest and best studied X-ray binaries, shows a cyclotron resonant scattering feature (CRSF) near 37 keV. This makes it an ideal target for a detailed study with the Nuclear Spectroscopic Telescope Array (NuSTAR), taking advantage of its excellent hard X-ray spectral resolution. We observed Her X-1 three times, coordinated with Suzaku, during one of the high flux intervals of its 35 day superorbital period. This paper focuses on the shape and evolution of the hard X-ray spectrum. The broadband spectra can be fitted with a power law with a high-energy cutoff, an iron line, and a CRSF. We find that the CRSF has a very smooth and symmetric shape in all observations and at all pulse phases. We compare the residuals of a line with a Gaussian optical-depth profile to a Lorentzian optical-depth profile and find no significant differences, strongly constraining the very smooth shape of the line. Even though the line energy changes dramatically with pulse phase, we find that its smooth shape does not. Additionally, our data show that the continuum only changes marginally between the three observations. These changes can be explained with varying amounts of Thomson scattering in the hot corona of the accretion disk. The average, luminosity-corrected CRSF energy is lower than in past observations and follows a secular decline. The excellent data quality of NuSTAR provides the best constraint on the CRSF energy to date. C1 [Fuerst, Felix; Grefenstette, Brian W.; Bellm, Eric C.; Harrison, Fiona; Madsen, Kristin K.; Walton, Dominic J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Staubert, Ruediger; Klochkov, Dmitry] Univ Tubingen IAAT, Inst Astron & Astrophys, D-72076 Tubingen, Germany. [Tomsick, John A.; Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Bachetti, Matteo; Barret, Didier] Univ Toulouse, UPS OMP, IRAP, F-31028 Toulouse, France. [Bachetti, Matteo; Barret, Didier] CNRS, Inst Rech Astrophys & Planetol, F-31028 Toulouse 4, France. [Chenevez, Jerome; Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Pottschmidt, Katja] UMBC, CRESST, Greenbelt, MD 20771 USA. [Pottschmidt, Katja; Zhang, William] NASA GSFC, Greenbelt, MD 20771 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Wilms, Joern] Dr Karl Remeis Sternwarte, D-96049 Bamberg, Germany. [Wilms, Joern] ECAP, D-96049 Bamberg, Germany. RP Furst, F (reprint author), CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. RI Wilms, Joern/C-8116-2013; Boggs, Steven/E-4170-2015; XRAY, SUZAKU/A-1808-2009; OI Wilms, Joern/0000-0003-2065-5410; Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337; Madsen, Kristin/0000-0003-1252-4891 FU NASA [NNG08FD60C]; NASA Astrophysics Data Analysis Program [NNX13AE98G]; Centre National d'Etudes Spatiales (CNES) FX This work was supported under NASA contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTAR-DAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). We would like to thank John E. Davis for the slxfig module, which was used to produce all figures in this work. F. F. would also like to thank the Remeis-Observatory Bamberg for their hospitality. J.A.T. acknowledges partial support from NASA Astrophysics Data Analysis Program grant NNX13AE98G. M. B. was supported by the Centre National d'Etudes Spatiales (CNES). NR 55 TC 18 Z9 18 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 10 PY 2013 VL 779 IS 1 AR UNSP 69 DI 10.1088/0004-637X/779/1/69 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268HD UT WOS:000328160100069 ER PT J AU McComas, DJ Angold, N Elliott, HA Livadiotis, G Schwadron, NA Skoug, RM Smith, CW AF McComas, D. J. Angold, N. Elliott, H. A. Livadiotis, G. Schwadron, N. A. Skoug, R. M. Smith, C. W. TI WEAKEST SOLAR WIND OF THE SPACE AGE AND THE CURRENT "MINI" SOLAR MAXIMUM SO ASTROPHYSICAL JOURNAL LA English DT Article DE dynamo; solar wind; Sun: activity; Sun: corona; Sun: heliosphere; sunspots ID INTERPLANETARY MAGNETIC-FIELD; LOCAL INTERSTELLAR-MEDIUM; TERMINATION SHOCK; OUTER HELIOSPHERE; SCALING LAW; ULYSSES; EXPLORER; PLASMA; FLUX; HELIOSHEATH AB The last solar minimum, which extended into 2009, was especially deep and prolonged. Since then, sunspot activity has gone through a very small peak while the heliospheric current sheet achieved large tilt angles similar to prior solar maxima. The solar wind fluid properties and interplanetary magnetic field (IMF) have declined through the prolonged solar minimum and continued to be low through the current mini solar maximum. Compared to values typically observed from the mid-1970s through the mid-1990s, the following proton parameters are lower on average from 2009 through day 79 of 2013: solar wind speed and beta (similar to 11%), temperature (similar to 40%), thermal pressure (similar to 55%), mass flux (similar to 34%), momentum flux or dynamic pressure (similar to 41%), energy flux (similar to 48%), IMF magnitude (similar to 31%), and radial component of the IMF (similar to 38%). These results have important implications for the solar wind's interaction with planetary magnetospheres and the heliosphere's interaction with the local interstellar medium, with the proton dynamic pressure remaining near the lowest values observed in the space age: similar to 1.4 nPa, compared to similar to 2.4 nPa typically observed from the mid-1970s through the mid-1990s. The combination of lower magnetic flux emergence from the Sun (carried out in the solar wind as the IMF) and associated low power in the solar wind points to the causal relationship between them. Our results indicate that the low solar wind output is driven by an internal trend in the Sun that is longer than the similar to 11 yr solar cycle, and they suggest that this current weak solar maximum is driven by the same trend. C1 [McComas, D. J.; Angold, N.; Elliott, H. A.; Livadiotis, G.] SW Res Inst, San Antonio, TX 78228 USA. [McComas, D. J.] Univ Texas San Antonio, San Antonio, TX 78249 USA. [Schwadron, N. A.; Smith, C. W.] Univ New Hampshire, Durham, NH 03824 USA. [Skoug, R. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP McComas, DJ (reprint author), SW Res Inst, 6220 Culebra Rd, San Antonio, TX 78228 USA. FU ACE mission, part of NASA's Explorer program FX We thank the WSO for providing the heliospheric current sheet tilt model results and various plasma and magnetometer teams (especially from IMP-8, WIND, and ACE) for providing the solar wind data, along with OMNI-2 for assembling and intercalibrating these data. Work at LANL was performed under the auspices of the U. S. DOE. This work was funded by the ACE mission, which is part of NASA's Explorer program. NR 44 TC 38 Z9 39 U1 4 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 10 PY 2013 VL 779 IS 1 DI 10.1088/0004-637X/779/1/2 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268HD UT WOS:000328160100002 ER PT J AU Mocanu, LM Crawford, TM Vieira, JD Aird, KA Aravena, M Austermann, JE Benson, BA Bethermin, M Bleem, LE Bothwell, M Carlstrom, JE Chang, CL Chapman, S Cho, HM Crites, AT de Haan, T Dobbs, MA Everett, WB George, EM Halverson, NW Harrington, N Hezaveh, Y Holder, GP Holzapfel, WL Hoover, S Hrubes, JD Keisler, R Knox, L Lee, AT Leitch, EM Lueker, M Luong-Van, D Marrone, DP McMahon, JJ Mehl, J Meyer, SS Mohr, JJ Montroy, TE Natoli, T Padin, S Plagge, T Pryke, C Rest, A Reichardt, CL Ruhl, JE Sayre, JT Schaffer, KK Shirokoff, E Spieler, HG Spilker, JS Stalder, B Staniszewski, Z Stark, AA Story, KT Switzer, ER Vanderlinde, K Williamson, R AF Mocanu, L. M. Crawford, T. M. Vieira, J. D. Aird, K. A. Aravena, M. Austermann, J. E. Benson, B. A. Bethermin, M. Bleem, L. E. Bothwell, M. Carlstrom, J. E. Chang, C. L. Chapman, S. Cho, H. -M. Crites, A. T. de Haan, T. Dobbs, M. A. Everett, W. B. George, E. M. Halverson, N. W. Harrington, N. Hezaveh, Y. Holder, G. P. Holzapfel, W. L. Hoover, S. Hrubes, J. D. Keisler, R. Knox, L. Lee, A. T. Leitch, E. M. Lueker, M. Luong-Van, D. Marrone, D. P. McMahon, J. J. Mehl, J. Meyer, S. S. Mohr, J. J. Montroy, T. E. Natoli, T. Padin, S. Plagge, T. Pryke, C. Rest, A. Reichardt, C. L. Ruhl, J. E. Sayre, J. T. Schaffer, K. K. Shirokoff, E. Spieler, H. G. Spilker, J. S. Stalder, B. Staniszewski, Z. Stark, A. A. Story, K. T. Switzer, E. R. Vanderlinde, K. Williamson, R. TI EXTRAGALACTIC MILLIMETER-WAVE POINT-SOURCE CATALOG, NUMBER COUNTS AND STATISTICS FROM 771 deg(2) OF THE SPT-SZ SURVEY SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: high-redshift; submillimeter: galaxies; surveys ID SOUTH-POLE TELESCOPE; SUBMILLIMETER-SELECTED GALAXIES; STAR-FORMING GALAXIES; DEEP-FIELD-SOUTH; ALL-SKY SURVEY; REDSHIFT DISTRIBUTION; INFRARED GALAXIES; MU-M; LENSED GALAXIES; LOCKMAN HOLE AB We present a point-source catalog from 771 deg(2) of the South Pole Telescope Sunyaev-Zel'dovich survey at 95, 150, and 220 GHz. We detect 1545 sources above 4.5 sigma significance in at least one band. Based on their relative brightness between survey bands, we classify the sources into two populations, one dominated by synchrotron emission from active galactic nuclei, and one dominated by thermal emission from dust-enshrouded star-forming galaxies. We find 1238 synchrotron and 307 dusty sources. We cross-match all sources against external catalogs and find 189 unidentified synchrotron sources and 189 unidentified dusty sources. The dusty sources without counterparts are good candidates for high-redshift, strongly lensed submillimeter galaxies. We derive number counts for each population from 1 Jy down to roughly 11, 4, and 11 mJy at 95, 150, and 220 GHz. We compare these counts with galaxy population models and find that none of the models we consider for either population provide a good fit to the measured counts in all three bands. The disparities imply that these measurements will be an important input to the next generation of millimeter-wave extragalactic source population models. C1 [Mocanu, L. M.; Crawford, T. M.; Benson, B. A.; Bleem, L. E.; Carlstrom, J. E.; Chang, C. L.; Crites, A. T.; Hoover, S.; Keisler, R.; Leitch, E. M.; Mehl, J.; Meyer, S. S.; Natoli, T.; Padin, S.; Plagge, T.; Schaffer, K. K.; Story, K. T.; Williamson, R.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Mocanu, L. M.; Crawford, T. M.; Carlstrom, J. E.; Crites, A. T.; Leitch, E. M.; Meyer, S. S.; Padin, S.; Plagge, T.; Williamson, R.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Vieira, J. D.; Lueker, M.; Padin, S.] CALTECH, Pasadena, CA 91125 USA. [Aird, K. A.; Hrubes, J. D.; Luong-Van, D.] Univ Chicago, Chicago, IL 60637 USA. [Aravena, M.] European So Observ, Alonso De Cordova 3107, Vitacura Santia, Chile. [Aravena, M.] Univ Diego Portales, Fac Engn, Santiago, Chile. [Austermann, J. E.; Everett, W. B.; Halverson, N. W.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80309 USA. [Austermann, J. E.; Everett, W. B.; Halverson, N. W.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Benson, B. A.; Carlstrom, J. E.; Chang, C. L.; Meyer, S. S.; Schaffer, K. K.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Bethermin, M.] CEA DSM Irfu CNRS Univ Paris Diderot, CEA Saclay, Lab AIM Paris Saclay, F-91191 Gif Sur Yvette, France. [Bleem, L. E.; Carlstrom, J. E.; Hoover, S.; Keisler, R.; Meyer, S. S.; Natoli, T.; Story, K. T.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Bothwell, M.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Carlstrom, J. E.; Chang, C. L.; Mehl, J.] Argonne Natl Lab, Argonne, IL 60439 USA. [Chapman, S.] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS B3H 3J5, Canada. [Chapman, S.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Cho, H. -M.] NIST, Quantum Devices Grp, Boulder, CO 80305 USA. [de Haan, T.; Dobbs, M. A.; Hezaveh, Y.; Holder, G. P.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [George, E. M.; Harrington, N.; Holzapfel, W. L.; Lee, A. T.; Reichardt, C. L.; Shirokoff, E.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Knox, L.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Lee, A. T.; Spieler, H. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Marrone, D. P.; Spilker, J. S.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [McMahon, J. J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Mohr, J. J.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Mohr, J. J.] Excellence Cluster Universe, D-85748 Garching, Germany. [Mohr, J. J.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Montroy, T. E.; Ruhl, J. E.; Sayre, J. T.; Staniszewski, Z.] Case Western Reserve Univ, Dept Phys, Ctr Educ & Res Cosmol & Astrophys, Cleveland, OH 44106 USA. [Pryke, C.] Univ Minnesota, Dept Phys, Minneapolis, MN 55455 USA. [Rest, A.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Schaffer, K. K.] Sch Art Inst Chicago, Liberal Arts Dept, Chicago, IL 60603 USA. [Stalder, B.; Stark, A. A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Switzer, E. R.] Univ Toronto, Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. [Vanderlinde, K.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Vanderlinde, K.] Univ Toronto, Dept Astron & Astrophys, Toronto, ON M5S 3H4, Canada. RP Mocanu, LM (reprint author), Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. EM lmocanu@uchicago.edu RI Aravena, Manuel/O-2361-2014; Williamson, Ross/H-1734-2015; Holzapfel, William/I-4836-2015; OI Williamson, Ross/0000-0002-6945-2975; Marrone, Daniel/0000-0002-2367-1080; Aird, Kenneth/0000-0003-1441-9518; Reichardt, Christian/0000-0003-2226-9169; Bethermin, Matthieu/0000-0002-3915-2015; Stark, Antony/0000-0002-2718-9996 FU National Science Foundation [ANT-0638937, PHY-1125897]; Kavli Foundation; Gordon and Betty Moore Foundation; Marie Curie Actions of the European Commission (FP7-COFUND); NASA Hubble Fellowship [HF-51275] FX The SPT is supported by the National Science Foundation through grant ANT-0638937, with partial support provided by NSF grant PHY-1125897, the Kavli Foundation, and the Gordon and Betty Moore Foundation. M. Aravena was co-funded under the Marie Curie Actions of the European Commission (FP7-COFUND). R. Keisler acknowledges support from NASA Hubble Fellowship grant HF-51275. NR 83 TC 40 Z9 40 U1 1 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 10 PY 2013 VL 779 IS 1 AR 61 DI 10.1088/0004-637X/779/1/61 PG 22 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268HD UT WOS:000328160100061 ER PT J AU Story, KT Reichardt, CL Hou, Z Keisler, R Aird, KA Benson, BA Bleem, LE Carlstrom, JE Chang, CL Cho, HM Crawford, TM Crites, AT de Haan, T Dobbs, MA Dudley, J Follin, B George, EM Halverson, NW Holder, GP Holzapfel, WL Hoover, S Hrubes, JD Joy, M Knox, L Lee, AT Leitch, EM Lueker, M Luong-Van, D McMahon, JJ Mehl, J Meyer, SS Millea, M Mohr, JJ Montroy, TE Padin, S Plagge, T Pryke, C Ruhl, JE Sayre, JT Schaffer, KK Shaw, L Shirokoff, E Spieler, HG Staniszewski, Z Stark, AA van Engelen, A Vanderlinde, K Vieira, JD Williamson, R Zahn, O AF Story, K. T. Reichardt, C. L. Hou, Z. Keisler, R. Aird, K. A. Benson, B. A. Bleem, L. E. Carlstrom, J. E. Chang, C. L. Cho, H. -M. Crawford, T. M. Crites, A. T. de Haan, T. Dobbs, M. A. Dudley, J. Follin, B. George, E. M. Halverson, N. W. Holder, G. P. Holzapfel, W. L. Hoover, S. Hrubes, J. D. Joy, M. Knox, L. Lee, A. T. Leitch, E. M. Lueker, M. Luong-Van, D. McMahon, J. J. Mehl, J. Meyer, S. S. Millea, M. Mohr, J. J. Montroy, T. E. Padin, S. Plagge, T. Pryke, C. Ruhl, J. E. Sayre, J. T. Schaffer, K. K. Shaw, L. Shirokoff, E. Spieler, H. G. Staniszewski, Z. Stark, A. A. van Engelen, A. Vanderlinde, K. Vieira, J. D. Williamson, R. Zahn, O. TI MEASUREMENT OF THE COSMIC MICROWAVE BACKGROUND DAMPING TAIL FROM THE 2500-SQUARE-DEGREE SPT-SZ SURVEY SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic background radiation; cosmology: observations; large-scale structure of universe ID SOUTH-POLE TELESCOPE; ATACAMA COSMOLOGY TELESCOPE; BARYON ACOUSTIC-OSCILLATIONS; INFLATIONARY UNIVERSE SCENARIO; DIGITAL SKY SURVEY; POWER SPECTRUM; GALAXY CLUSTERS; SYMMETRY-BREAKING; DARK ENERGY; 148 GHZ AB We present a measurement of the cosmic microwave background (CMB) temperature power spectrum using data from the recently completed South Pole Telescope Sunyaev-Zel'dovich (SPT-SZ) survey. This measurement is made from observations of 2540 deg(2) of sky with arcminute resolution at 150 GHz, and improves upon previous measurements using the SPT by tripling the sky area. We report CMB temperature anisotropy power over the multipole range 650 < l < 3000. We fit the SPT bandpowers, combined with the 7 yr Wilkinson Microwave Anisotropy Probe (WMAP7) data, with a six-parameter Lambda CDM cosmological model and find that the two datasets are consistent and well fit by the model. Adding SPT measurements significantly improves Lambda CDM parameter constraints; in particular, the constraint on theta(s) tightens by a factor of 2.7. The impact of gravitational lensing is detected at 8.1 sigma, the most significant detection to date. This sensitivity of the SPT+WMAP7 data to lensing by large-scale structure at low redshifts allows us to constrain the mean curvature of the observable universe with CMB data alone to be Omega(k) = -0.003(-0.018)(+0.014). Using the SPT+ WMAP7 data, we measure the spectral index of scalar fluctuations to be n(s) = 0.9623 +/- 0.0097 in the Lambda CDM model, a 3.9 sigma preference for a scale-dependent spectrum with n(s) < 1. The SPT measurement of the CMB damping tail helps break the degeneracy that exists between the tensor-to-scalar ratio r and ns in large-scale CMB measurements, leading to an upper limit of r < 0.18 (95% C. L.) in the Lambda CDM+r model. Adding low-redshift measurements of the Hubble constant (H-0) and the baryon acoustic oscillation (BAO) feature to the SPT+ WMAP7 data leads to further improvements. The combination of SPT+WMAP7+H-0+BAO constrains n(s) = 0.9538 +/- 0.0081 in the Lambda CDM model, a 5.7 sigma detection of n(s) < 1, and places an upper limit of r < 0.11 (95% C. L.) in the Lambda CDM+r model. These new constraints on ns and r have significant implications for our understanding of inflation, which we discuss in the context of selected single-field inflation models. C1 [Story, K. T.; Keisler, R.; Benson, B. A.; Bleem, L. E.; Carlstrom, J. E.; Chang, C. L.; Crawford, T. M.; Crites, A. T.; Hoover, S.; Leitch, E. M.; Mehl, J.; Meyer, S. S.; Padin, S.; Plagge, T.; Schaffer, K. K.; Williamson, R.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Story, K. T.; Keisler, R.; Bleem, L. E.; Carlstrom, J. E.; Hoover, S.; Meyer, S. S.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Reichardt, C. L.; George, E. M.; Holzapfel, W. L.; Lee, A. T.; Shirokoff, E.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Hou, Z.; Follin, B.; Knox, L.; Millea, M.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Aird, K. A.; Hrubes, J. D.; Luong-Van, D.] Univ Chicago, Chicago, IL 60637 USA. [Benson, B. A.; Carlstrom, J. E.; Chang, C. L.; Meyer, S. S.; Schaffer, K. K.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carlstrom, J. E.; Crawford, T. M.; Crites, A. T.; Leitch, E. M.; Meyer, S. S.; Padin, S.; Plagge, T.; Williamson, R.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Carlstrom, J. E.; Chang, C. L.; Mehl, J.] Argonne Natl Lab, Argonne, IL 60439 USA. [Cho, H. -M.] NIST, Quantum Devices Grp, Boulder, CO 80305 USA. [de Haan, T.; Dobbs, M. A.; Dudley, J.; Holder, G. P.; Shaw, L.; van Engelen, A.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Halverson, N. W.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80309 USA. [Halverson, N. W.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Joy, M.] NASA, George C Marshall Space Flight Ctr, Dept Space Sci, Huntsville, AL 35812 USA. [Lee, A. T.; Spieler, H. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Lueker, M.; Padin, S.; Vieira, J. D.] CALTECH, Pasadena, CA 91125 USA. [McMahon, J. J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Mohr, J. J.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Mohr, J. J.] Excellence Cluster Universe, D-85748 Garching, Germany. [Mohr, J. J.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Montroy, T. E.; Ruhl, J. E.; Sayre, J. T.; Staniszewski, Z.] Case Western Reserve Univ, Dept Phys, Ctr Educ & Res Cosmol & Astrophys, Cleveland, OH 44106 USA. [Pryke, C.] Univ Minnesota, Dept Phys, Minneapolis, MN 55455 USA. [Schaffer, K. K.] Sch Art Inst Chicago, Liberal Arts Dept, Chicago, IL 60603 USA. [Stark, A. A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Vanderlinde, K.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Vanderlinde, K.] Univ Toronto, Dept Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Zahn, O.] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Zahn, O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Story, KT (reprint author), Univ Chicago, Kavli Inst Cosmol Phys, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM kstory@uchicago.edu RI Williamson, Ross/H-1734-2015; Holzapfel, William/I-4836-2015; OI Williamson, Ross/0000-0002-6945-2975; Stark, Antony/0000-0002-2718-9996 FU National Science Foundation [ANT-0638937]; NSF [PHY-1125897, 0709498]; Kavli Foundation; Gordon and Betty Moore Foundation; National Sciences and Engineering Research Council of Canada; Canada Research Chairs program; Canadian Institute for Advanced Research; NASA Hubble Fellowship [HF-51275.01]; KICP Fellowship; Alfred P. Sloan Research Fellowship; BCCP fellowship; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Open Science Grid, NSF [NSF PHY 1148698]; NASA Office of Space Science; [AST-1009012] FX We thank Scott Dodelson, John Peacock, David Baumann, and Antonio Riotto for useful conversations. The SPT is supported by the National Science Foundation through grant ANT-0638937, with partial support provided by NSF grant PHY-1125897, the Kavli Foundation, and the Gordon and Betty Moore Foundation. The McGill group acknowledges funding from the National Sciences and Engineering Research Council of Canada, Canada Research Chairs program, and the Canadian Institute for Advanced Research. Work at Harvard is supported by grant AST-1009012. R. Keisler acknowledges support from NASA Hubble Fellowship grant HF-51275.01, B. A. Benson a KICP Fellowship, M. Dobbs an Alfred P. Sloan Research Fellowship, O. Zahn a BCCP fellowship, M. Millea and L. Knox a NSF grant 0709498. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under contract No. DE-AC02-05CH11231, and the resources of the University of Chicago Computing Cooperative (UC3), supported in part by the Open Science Grid, NSF grant NSF PHY 1148698. Some of the results in this paper have been derived using the HEALPix (Gorski et al. 2005) package. We acknowledge the use of the Legacy Archive for Microwave Background Data Analysis (LAMBDA). Support for LAMBDA is provided by the NASA Office of Space Science. NR 79 TC 133 Z9 133 U1 2 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD DEC 10 PY 2013 VL 779 IS 1 AR 86 DI 10.1088/0004-637X/779/1/86 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 268HD UT WOS:000328160100086 ER PT J AU Fan, F Wang, YY Sokolov, AP AF Fan, Fei Wang, Yangyang Sokolov, Alexei P. TI Ionic Transport, Microphase Separation, and Polymer Relaxation in Poly(propylene glycol) and Lithium Perchlorate Mixtures SO MACROMOLECULES LA English DT Article ID POLY(ETHYLENE OXIDE); MOLECULAR-WEIGHT; CONDUCTIVITY BEHAVIOR; DIELECTRIC-RELAXATION; BRILLOUIN-SCATTERING; MODE RELAXATION; END-GROUPS; ELECTROLYTES; LICLO4; COMPLEXES AB By combining broadband dielectric spectroscopy (BDS) and differential scanning calorimetry (DSC), the ionic transport, microphase separation, and polymer relaxation in poly(propylene glycol) (PPG) and lithium perchlorate (LiClO4) mixtures have been systematically examined as a function of temperature, pressure, polymer molecular weight, and salt concentration. While the low molecular weight PPG LiClO4 mixtures exhibit only a single phase, microphase separation is observed in the mixtures of higher molecular weight PPGs (1000 and 4000 g/mol). In the samples with microphase separation, BDS and DSC yield consistent glass transition temperatures for ion-rich and ion-depleted domains. Our Walden plot analysis indicates that the ionic transport in PPG-LiClO4 is controlled by the (slow) segmental relaxation, and the data of all PPG-LiClO4 fall close to the "ideal" Walden line. Last, the application of pressure not only suppresses the microphase separation, but also decouples the ionic transport from the segmental relaxation. C1 [Fan, Fei; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Wang, Yangyang; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Wang, YY (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM yywang@utk.edu RI Wang, Yangyang/A-5925-2010 OI Wang, Yangyang/0000-0001-7042-9804 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy; NSF Polymer Program [DMR-1104824] FX This research was sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. F.F. thanks the NSF Polymer Program (DMR-1104824) for funding. The authors are grateful to M. Paluch for the help with the high-pressure dielectric device. NR 66 TC 9 Z9 9 U1 3 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD DEC 10 PY 2013 VL 46 IS 23 BP 9380 EP 9389 DI 10.1021/ma401238k PG 10 WC Polymer Science SC Polymer Science GA 272CB UT WOS:000328436800023 ER PT J AU Edmunds, C Tang, L Cervantes, M Shirazi-HD, M Shao, J Grier, A Valavanis, A Cooper, JD Li, D Gardner, G Zakharov, DN Ikonic, Z Indjin, D Harrison, P Manfra, MJ Malis, O AF Edmunds, C. Tang, L. Cervantes, M. Shirazi-HD, M. Shao, J. Grier, A. Valavanis, A. Cooper, J. D. Li, D. Gardner, G. Zakharov, D. N. Ikonic, Z. Indjin, D. Harrison, P. Manfra, M. J. Malis, O. TI Comparative study of intersubband absorption in AlGaN/GaN and AlInN/GaN superlattices: Impact of material inhomogeneities SO PHYSICAL REVIEW B LA English DT Article ID LATTICE-MATCHED ALINN/GAN; QUANTUM-WELLS; SCATTERING AB We report a systematic and quantitative study of near-infrared intersubband absorption in strained AlGaN/GaN and lattice-matched AlInN/GaN superlattices grown by plasma-assisted molecular-beam epitaxy as a function of Si-doping profile with and without delta doping. For AlGaN/GaN, we obtained good theoretical agreement with experimental measurements of transition energy, integrated absorbance and linewidth by considering many-body effects, interface roughness, and calculations of the transition lifetime that include dephasing. For the AlInN/GaN system, experimental measurements of the integrated absorbance due to the superlattice transitions produced values more than one order of magnitude lower than AlGaN/GaN heterostructures at similar doping levels. Furthermore, observed transition energies were roughly 150 meV higher than expected. The weak absorption and high transition energies measured in these structures is attributed to columnar alloy inhomogeneity in the AlInN barriers observed in high-angle annular dark-field scanning transmission electron microscopy. We simulated the effect of these inhomogeneities using three-dimensional band-structure calculations. The inhomogeneities were modeled as AlInN nanorods with radially varying In composition embedded in the barrier material of the superlattice. We show that inclusion of the nanorods leads to the depletion of the quantum wells (QWs) due to localization of charge carriers in high-In-containing regions. The higher energy of the intersubband transitions was attributed to the relatively uniform regions of the QWs surrounded by high Al (95%) composition barriers. The calculated transition energy assuming Al0.95In0.05N barriers was in good agreement with experimental results. C1 [Edmunds, C.; Tang, L.; Cervantes, M.; Shao, J.; Li, D.; Manfra, M. J.; Malis, O.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Tang, L.; Shirazi-HD, M.; Shao, J.; Li, D.; Gardner, G.; Manfra, M. J.] Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Shirazi-HD, M.; Manfra, M. J.] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Grier, A.; Valavanis, A.; Cooper, J. D.; Ikonic, Z.; Indjin, D.; Harrison, P.] Univ Leeds, Sch Elect & Elect Engn, Inst Microwaves & Photon, Leeds LS2 9JT, W Yorkshire, England. [Gardner, G.; Manfra, M. J.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Zakharov, D. N.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Malis, O (reprint author), Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. EM omalis@purdue.edu RI Zakharov, Dmitri/F-4493-2014; Valavanis, Alexander/C-1617-2009 OI Valavanis, Alexander/0000-0001-5565-0463 FU NSF awards [ECCS-1001431, ECCS-1253720, DMR-1206919]; Defense Advanced Research Project Agency (DARPA) [D11PC20027]; Univ. Leeds FIRC grant FX This work was supported by the NSF awards ECCS-1001431, ECCS-1253720, and DMR-1206919; the Defense Advanced Research Project Agency (DARPA) under Contract No. D11PC20027; and the Univ. Leeds FIRC 2011 grant. NR 27 TC 12 Z9 12 U1 8 U2 59 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 10 PY 2013 VL 88 IS 23 AR 235306 DI 10.1103/PhysRevB.88.235306 PG 10 WC Physics, Condensed Matter SC Physics GA 275LO UT WOS:000328678200009 ER PT J AU Fan, YC Wei, ZY Li, HQ Chen, H Soukoulis, CM AF Fan, Yuancheng Wei, Zeyong Li, Hongqiang Chen, Hong Soukoulis, Costas M. TI Photonic band gap of a graphene-embedded quarter-wave stack SO PHYSICAL REVIEW B LA English DT Article ID CRYSTAL; LIGHT AB Here, we present a mechanism for tailoring the photonic band structure of a quarter-wave stack without changing its physical periods by embedding conductive sheets. Graphene is utilized and studied as a realistic, two-dimensional conductive sheet. In a graphene-embedded quarter-wave stack, the synergic actions of Bragg scattering and graphene conductance contributions open photonic gaps at the center of the reduced Brillouin zone that are nonexistent in conventional quarter-wave stacks. Such photonic gaps show giant, loss-independent density of optical states at the fixed lower-gap edges, of even-multiple characteristic frequency of the quarter-wave stack. The conductive sheet-induced photonic gaps provide a platform for the enhancement of light-matter interactions. C1 [Fan, Yuancheng; Soukoulis, Costas M.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Fan, Yuancheng; Soukoulis, Costas M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Fan, Yuancheng; Wei, Zeyong; Li, Hongqiang; Chen, Hong] Tongji Univ, Key Lab Adv Microstruct Mat MOE, Shanghai 200092, Peoples R China. [Fan, Yuancheng; Wei, Zeyong; Li, Hongqiang; Chen, Hong] Tongji Univ, Sch Phys Sci & Engn, Shanghai 200092, Peoples R China. [Soukoulis, Costas M.] FORTH, Inst Elect Struct & Laser, Iraklion 71110, Crete, Greece. RP Fan, YC (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM phyfan@ameslab.gov; hqlee@tongji.edu.cn; soukoulis@ameslab.gov RI Soukoulis, Costas/A-5295-2008; OI Fan, Yuancheng/0000-0002-7919-4148 FU US Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) [DE-AC02-07CH11358]; Greek GSRT [ERC-02 EXEL]; NSFC [11174221, 10974144]; CNKBRSF [2011CB922001]; China Scholarship Council [201206260055] FX Work at Ames Laboratory was partially supported by the US Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) under Contract No. DE-AC02-07CH11358. This work was partially supported by the Greek GSRT through the project ERC-02 EXEL. The work was supported by NSFC (Grants Nos. 11174221 and 10974144) and CNKBRSF (Grant No. 2011CB922001). Y.F. acknowledges Y. Chen and P. Zhang for helpful discussions and the China Scholarship Council (No. 201206260055) for financial support. NR 41 TC 17 Z9 17 U1 2 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD DEC 10 PY 2013 VL 88 IS 24 AR 241403 DI 10.1103/PhysRevB.88.241403 PG 5 WC Physics, Condensed Matter SC Physics GA 275LS UT WOS:000328678600005 ER PT J AU Melkov, GA Kobljanskyj, Y Novosad, V Slavin, AN Guslienko, KY AF Melkov, G. A. Kobljanskyj, Y. Novosad, V. Slavin, A. N. Guslienko, K. Y. TI Probing the energy barriers in nonuniform magnetization states of circular dots by broadband ferromagnetic resonance SO PHYSICAL REVIEW B LA English DT Article ID THERMAL FLUCTUATIONS; VORTEX STATE; FIELD AB The time evolution of the ferromagnetic resonance output signal in the arrays of permalloy circular dots of submicron sizes was measured near the critical fields of the vortex nucleation and annihilation. Surprisingly short times of the transition from the quasiuniform to the vortex magnetization state (several milliseconds) were detected. The observed effects are explained by overcoming the field dependent energy barriers in the process of vortex core nucleation. The energy barrier values found from the time dependences of the ferromagnetic resonance peak intensities were compared with the ones calculated within the rigid vortex model. The rigid vortex model overestimates the nucleation barriers and a more adequate magnetization reversal model is needed. There is a strong dependence of the stable, metastable energy minima and energy barriers on the magnetic field and dot geometrical parameters. C1 [Melkov, G. A.; Kobljanskyj, Y.] Taras Shevchenko Natl Univ Kyiv, Fac Radiophys, UA-01601 Kiev, Ukraine. [Novosad, V.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Slavin, A. N.] Oakland Univ, Dept Phys, Rochester, MI 48309 USA. [Guslienko, K. Y.] Univ Basque Country, Dept Fis Mat, San Sebastian 20018, Spain. [Guslienko, K. Y.] Basque Fdn Sci, IKERBASQUE, Bilbao 48011, Spain. RP Melkov, GA (reprint author), Taras Shevchenko Natl Univ Kyiv, Fac Radiophys, UA-01601 Kiev, Ukraine. RI Novosad, Valentyn/C-2018-2014; Novosad, V /J-4843-2015 FU State Fund for Fundamental Research of Ukraine [UU34/008]; MES of Ukraine [M/90-2010]; National Science Foundation of the USA [DMR-1015175]; US DOE Office of Science [DE-AC02-06CH11357]; Spanish MEC [PIB2010US-00153, FIS2010-20979-C02-01]; IKERBASQUE (the Basque Foundation for Science) FX This work was supported by the State Fund for Fundamental Research of Ukraine (Project No. UU34/008), by the MES of Ukraine (Grant No. M/90-2010), by the National Science Foundation of the USA (Grant No. DMR-1015175), by the US DOE Office of Science (Contract No. DE-AC02-06CH11357), and by the Spanish MEC Grants No. PIB2010US-00153 and No. FIS2010-20979-C02-01. K. G. acknowledges support by IKERBASQUE (the Basque Foundation for Science). NR 24 TC 3 Z9 3 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 10 PY 2013 VL 88 IS 22 AR 220407 DI 10.1103/PhysRevB.88.220407 PG 5 WC Physics, Condensed Matter SC Physics GA 275LK UT WOS:000328677800001 ER PT J AU Randrup, J Moller, P AF Randrup, J. Moeller, P. TI Energy dependence of fission-fragment mass distributions from strongly damped shape evolution SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-FISSION AB The recently developed treatment of Brownian shape evolution is refined to take account of the gradual decrease in microscopic effects as the nuclear excitation energy is raised. We construct effective potential-energy surfaces by multiplying the shell-plus-pairing correction term by a suppression factor that depends on the local excitation energy. While this approach is equivalent to the modification of the Fermi-gas level density parameter suggested by Ignatyuk et al. [Sov. J. Nucl. Phys. 29, 450 (1979)], we adopt a more general functional form for the suppression factor, which is adjusted to measured charge yields for U-234 (E* approximate to 11 MeV). The resulting model is benchmarked by comparison with 70 measured yields. C1 [Randrup, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Moeller, P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Randrup, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. OI Moller, Peter/0000-0002-5848-3565 FU Office of Energy Research, Office of High Energy and Nuclear Physics, Nuclear Physics Division of the U.S. Department of Energy [DE-AC02-05CH11231]; JUSTIPEN/UT Grant [DE-FG02-06ER41407]; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX During this work, we have benefited from discussions with many colleagues, in particular, A. N. Andreyev, M. Brack, T. Dossing, F. Farget, H. Feldmeier, D. Hinde, T. Ichikawa, A. V. Ignatyuk, A. Iwamoto, K. Nishio, K.-H. Schmidt, A. J. Sierk, and R. Vogt. We also thank K.-H. Schmidt for providing computer-readable files of the experimental data in Ref. [17]. This work was supported by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Nuclear Physics Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (J. R.) and JUSTIPEN/UT Grant No. DE-FG02-06ER41407 (P. M.) and by the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 (P.M.). NR 25 TC 29 Z9 29 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD DEC 10 PY 2013 VL 88 IS 6 AR 064606 DI 10.1103/PhysRevC.88.064606 PG 16 WC Physics, Nuclear SC Physics GA 275PM UT WOS:000328689300006 ER PT J AU Sadhukhan, J Mazurek, K Baran, A Dobaczewski, J Nazarewicz, W Sheikh, JA AF Sadhukhan, Jhilam Mazurek, K. Baran, A. Dobaczewski, J. Nazarewicz, W. Sheikh, J. A. TI Spontaneous fission lifetimes from the minimization of self-consistent collective action SO PHYSICAL REVIEW C LA English DT Article ID HARTREE-FOCK THEORY; SUPERHEAVY NUCLEI; MASS PARAMETERS; HALF-LIVES; APPROXIMATION; SHAPES; MOTION; FORCE AB The spontaneous fission lifetime of Fm-264 has been studied within nuclear density functional theory by minimizing the collective action integral for fission in a two-dimensional quadrupole collective space representing elongation and triaxiality. The collective potential and inertia tensor are obtained self-consistently using the Skyrme energy density functional and density-dependent pairing interaction. The resulting spontaneous fission lifetimes are compared with the static result obtained with the minimum-energy pathway. We show that fission pathways strongly depend on assumptions underlying collective inertia. With the nonperturbative mass parameters, the dynamic fission pathway becomes strongly triaxial and it approaches the static fission valley. On the other hand, when the standard perturbative cranking inertia tensor is used, axial symmetry is restored along the path to fission; an effect that is an artifact of the approximation used. C1 [Sadhukhan, Jhilam; Mazurek, K.; Baran, A.; Dobaczewski, J.; Nazarewicz, W.; Sheikh, J. A.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Sadhukhan, Jhilam; Mazurek, K.; Baran, A.; Dobaczewski, J.; Nazarewicz, W.; Sheikh, J. A.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Mazurek, K.] Niewodniczanski Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Baran, A.] Marie Curie Sklodowska Univ, Inst Phys, PL-20031 Lublin, Poland. [Dobaczewski, J.; Nazarewicz, W.] Univ Warsaw, Inst Theoret Phys, Fac Phys, PL-00681 Warsaw, Poland. [Dobaczewski, J.] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland. RP Sadhukhan, J (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM jhilam@utk.edu FU National Institute for Nuclear Theory in Seattle [INT-13-3]; US Department of Energy [DE-FG02-96ER40963, DE-FG52-09NA29461, DE-SC0008499]; Academy of Finland; University of Jyvaskyla within the FIDIPRO program; Polish National Science Center [2012/07/B/ST2/03907, 2011/01/B/ST2/03667] FX Useful discussions with L. Prochniak and A. Staszczak are gratefully acknowledged. This work was finalized during the Program INT-13-3 "Quantitative Large Amplitude Shape Dynamics: fission and heavy ion fusion" at the National Institute for Nuclear Theory in Seattle; it was supported by by the US Department of Energy under Contracts No. DE-FG02-96ER40963 (University of Tennessee), No. DE-FG52-09NA29461 (the Stewardship Science Academic Alliances program), and No. DE-SC0008499 (NUCLEI Sci-DAC Collaboration), by the Academy of Finland and University of Jyvaskyla within the FIDIPRO program, and by the Polish National Science Center under Contracts No. 2012/07/B/ST2/03907 and No. 2011/01/B/ST2/03667. Computer time was provided by the National Institute for Computational Sciences (NICS) and the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program using resources of the OLCF facility. NR 36 TC 29 Z9 29 U1 1 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD DEC 10 PY 2013 VL 88 IS 6 AR 064314 DI 10.1103/PhysRevC.88.064314 PG 5 WC Physics, Nuclear SC Physics GA 275PM UT WOS:000328689300005 ER PT J AU Xu, LS Chen, CH Wang, FQ AF Xu, Lingshan Chen, Chin-Hao Wang, Fuqiang TI Event mixing does not reproduce single-particle acceptance convolutions for nonuniform pseudorapidity distributions SO PHYSICAL REVIEW C LA English DT Article ID ANGULAR-CORRELATIONS; LONG-RANGE; COLLISIONS; COLLABORATION; SIDE AB We point out that the mixed-event method for two-particle acceptance correction, widely used in particle correlation measurements at the BNL Realtivistic Heavy Ion Collider and the CERN Large Hadron Collider (LHC), is wrong in cases where the single-particle pseudorapidity distribution is significantly nonuniform. The correct acceptance should be the convolution of two single-particle efficiency x acceptance functions. The error of themixed-event method, which guarantees a uniform Delta eta two-particle combinatorial density, is, however, small in correlation analyses where the two particles are integrated over an extended pseudorapidity eta range. With one particle fixed in eta and the right acceptance correction, the background-subtracted correlated pair density may reveal not only a short-range but also a long-range Delta eta dependence. This has important physics implication and may provide crucial information to disentangle physics mechanisms for the recently observed long-range ridge correlation in asymmetric proton-lead collisions at the LHC. C1 [Xu, Lingshan; Wang, Fuqiang] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Chen, Chin-Hao] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Xu, LS (reprint author), Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. FU US Department of Energy [DE-FG02-88ER40412]; RIKEN-BNL Memorandum of Understanding on spin physics projects FX L.X. and F. W. are supported by the US Department of Energy under Grant No. DE-FG02-88ER40412. C. H. C. is supported by the RIKEN-BNL Memorandum of Understanding on spin physics projects. NR 17 TC 4 Z9 4 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD DEC 10 PY 2013 VL 88 IS 6 AR 064907 DI 10.1103/PhysRevC.88.064907 PG 3 WC Physics, Nuclear SC Physics GA 275PM UT WOS:000328689300009 ER PT J AU Briceno, RA Davoudi, Z Luu, TC Savage, MJ AF Briceno, Raul A. Davoudi, Zohreh Luu, Thomas C. Savage, Martin J. TI Two-nucleon systems in a finite volume. II.S-3(1)-D-3(1) coupled channels and the deuteron SO PHYSICAL REVIEW D LA English DT Article ID NUCLEON-NUCLEON POTENTIALS; QUADRUPOLE-MOMENT; LATTICE QCD; S-MATRIX; SCATTERING; STATES; BOX; SIMULATIONS; DIAGRAMS AB The energy spectra of two nucleons in a cubic volume provide access to the two phase shifts and one mixing angle that define the S matrix in the S-3(1)-D-3(1) coupled channels containing the deuteron. With the aid of recently derived energy quantization conditions for such systems, and the known scattering parameters, these spectra are predicted for a range of volumes. It is found that extractions of the infinite-volume deuteron binding energy and leading scattering parameters, including the S-D mixing angle at the deuteron pole, are possible from lattice QCD calculations of two-nucleon systems with boosts of vertical bar P vertical bar <= 2 pi/L root 3 in volumes with 10 fm less than or similar to L less than or similar to 14 fm. The viability of extracting the asymptotic D/S ratio of the deuteron wave function from lattice QCD calculations is discussed. C1 [Briceno, Raul A.] Jefferson Lab, Newport News, VA 23606 USA. [Davoudi, Zohreh; Savage, Martin J.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Davoudi, Zohreh; Savage, Martin J.] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Luu, Thomas C.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany. [Luu, Thomas C.] Forschungszentrum Julich, Inst Kernphys, D-52425 Julich, Germany. [Luu, Thomas C.] Forschungszentrum Julich, Julich Ctr Hadron Phys, D-52425 Julich, Germany. RP Briceno, RA (reprint author), Jefferson Lab, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM rbriceno@jlab.org; davoudi@uw.edu; t.luu@fz-juelich.de; mjs5@uw.edu OI Briceno, Raul/0000-0003-1109-1473 FU DOE [DE-FG02-97ER41014, DE-FG02-00ER41132]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX R. B., Z. D., and M. J. S. were supported in part by the DOE Grant No. DE-FG02-97ER41014. Z. D. and M. J. S. were also supported in part by DOE Grant No. DE-FG02-00ER41132. The work of T. L. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 59 TC 27 Z9 27 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 10 PY 2013 VL 88 IS 11 AR 114507 DI 10.1103/PhysRevD.88.114507 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 275QF UT WOS:000328691300001 ER PT J AU Wu, LJ Meng, QP Jooss, C Zheng, JC Inada, H Su, D Li, Q Zhu, YM AF Wu, Lijun Meng, Qingping Jooss, Christian Zheng, Jin-Cheng Inada, H. Su, Dong Li, Qiang Zhu, Yimei TI Origin of Phonon Glass-Electron Crystal Behavior in Thermoelectric Layered Cobaltate SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE thermoelectric materials; layered structures; thermal vibration; crystal structures ID THERMAL-CONDUCTIVITY; OXIDES; THERMOPOWER; INTERFACE; STEM; SI AB Measurement of local disorder and lattice vibrations is of great importance for understanding the mechanisms whereby thermoelectric materials efficiently convert heat to electricity. Attaining high thermoelectric power requires minimizing thermal conductivity while keeping electric conductivity high. This situation is achievable by enhancing phonon scattering through specific structural disorder (phonon glass) that also retains sufficient electron mobility (electron crystal). It is demonstrated that the quantitative acquisition of multiple annular-dark-field images via scanning transmission electron microscopy at different scattering-angles simultaneously allows not only the separation but also the accurate determination of static and thermal atomic displacements in crystals. Applying the unique method to the layered thermoelectric material (Ca2CoO3)(0.62)CoO2 discloses the presence of large incommensurate displacive modulation and enhanced local vibration of atoms, largely confined within its Ca2CoO3 sublayers. Relating the refined disorder to ab initio calculations of scattering rates is a tremendeous challenge. Based on an approximate calculation of scattering rates, it is suggested that this well-defined deterministic disorder engenders static displacement-induced scattering and vibrational-induced resonance scattering of phonons as the origin of the phonon glass. Concurrently, the crystalline CoO2 sublayers provide pathways for highly conducting electrons and large thermal voltages. C1 [Wu, Lijun; Meng, Qingping; Su, Dong; Li, Qiang; Zhu, Yimei] Brookhaven Natl Lab, Upton, NY 11973 USA. [Jooss, Christian] Univ Gottingen, D-37077 Gottingen, Germany. [Zheng, Jin-Cheng] Xiamen Univ, Dept Phys, Xiamen 361005, Peoples R China. [Inada, H.] Hitachi High Technol, Ibaraki 3120032, Japan. RP Wu, LJ (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM zhu@bnl.gov RI Zheng, JC/G-3383-2010; Su, Dong/A-8233-2013 OI Zheng, JC/0000-0002-6292-3236; Su, Dong/0000-0002-1921-6683 FU U.S. Department of Energy, Office of Basic Energy Science, Material Science and Engineering Division [DE-AC02-98CH10886]; DFG [SPP 1386]; SRFDP [20090121120028] FX The authors would like to thank P. B. Allen for his stimulating discussions on phonon scattering and thermal conductivity. Work at Brookhaven, including the use of Center for Functional Nanomaterials, was supported by the U.S. Department of Energy, Office of Basic Energy Science, Material Science and Engineering Division, under Contract No. DE-AC02-98CH10886 and the work of C.J. was supported by DFG SPP 1386. J.C.Z. was supported by SRFDP No. 20090121120028. NR 33 TC 8 Z9 8 U1 7 U2 86 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD DEC 10 PY 2013 VL 23 IS 46 BP 5728 EP 5736 DI 10.1002/adfm.201301098 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 268EG UT WOS:000328151000005 ER PT J AU Tan, K Canepa, P Gong, QH Liu, J Johnson, DH Dyevoich, A Thallapally, PK Thonhauser, T Li, J Chabal, YJ AF Tan, Kui Canepa, Pieremanuele Gong, Qihan Liu, Jian Johnson, Daniel H. Dyevoich, Allison Thallapally, Praveen K. Thonhauser, Timo Li, Jing Chabal, Yves J. TI Mechanism of Preferential Adsorption of SO2 into Two Microporous Paddle Wheel Frameworks M(bdc)(ted)(0.5) SO CHEMISTRY OF MATERIALS LA English DT Article DE metal organic frameworks; paddlewheel; sulfur dioxide; adsorption isotherm; in situ infrared spectroscopy; DFT calculations ID METAL-ORGANIC FRAMEWORKS; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; SULFUR-DIOXIDE; HIGH-CAPACITY; CARBON-DIOXIDE; BASIS-SET; SEPARATION; CO2 AB The selective adsorption of a corrosive gas, SO2, into two microporous pillared paddle-wheel frameworks M(bdc)(ted)(0.5) [M = Ni, Zn; bdc =1,4-benzenedicarboxylate; ted = triethylenediamine] is studied by volumetric adsorption measurements and a combination of in situ infrared spectroscopy and ab initio density functional theory (DFT) calculations. The uptake of SO2 in M(bdc)(ted)(0.5) at room temperature is quite significant, 9.97 mol/kg at 1.13 bar. The major adsorbed SO2 molecules contributing to the isotherm measurements are characterized by stretching bands at 1326 and 1144 cm(-1). Theoretical calculations including van der Waals interactions (based on vdW-DF) suggest that two adsorption configurations are possible for these SO2 molecules. One geometry involves an SO2 molecule bonded through its sulfur atom to the oxygen atom of the paddle-wheel building unit and its two oxygen atoms to the C-H groups of the organic linkers by formation of hydrogen bonds. Such a configuration results in a distortion of the benzene rings, which is consistent with the experimentally observed shift of the ring deformation mode. In the other geometry, SO2 establishes hydrogen bonding with -CH2, group of the ted linker through its two oxygen atoms simultaneously. The vdW-DF-simulated frequency shifts of the SO2 stretching bands in these two configurations are similar and in good agreement with spectroscopically measured values of physisorbed SO2. In addition, the IR spectra reveal the presence of another minor species, characterized by stretching modes at 1242 and 1105 cm(-1) and causing significant perturbations of MOFs vibrational modes (CHx and carboxylate groups). This species is more strongly bound, requiring a higher temperature (similar to 150 degrees C) to remove it than for the main physisorbed species. The adsorption configurations of SO2 into M(bdc)(ted)(0.5) derived by infrared spectroscopy and vdW-DF calculations provide the initial understanding to develop microporous metal organic frameworks materials based on paddlewheel secondary-building units for SO2 removal in industrial processes. C1 [Tan, Kui; Chabal, Yves J.] Univ Texas Dallas, Dept Mat Sci & Engn, Richardson, TX 75080 USA. [Canepa, Pieremanuele; Johnson, Daniel H.; Thonhauser, Timo] Wake Forest Univ, Dept Phys, Winston Salem, NC 27109 USA. [Gong, Qihan; Dyevoich, Allison; Li, Jing] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. [Liu, Jian; Thallapally, Praveen K.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Chabal, YJ (reprint author), Univ Texas Dallas, Dept Mat Sci & Engn, Richardson, TX 75080 USA. EM chabal@utdallas.edu RI thallapally, praveen/I-5026-2014; Canepa, Pieremanuele/O-2344-2013; Liu, Jian/C-4707-2011; Liu, Jian/D-3393-2009 OI thallapally, praveen/0000-0001-7814-4467; Canepa, Pieremanuele/0000-0002-5168-9253; Liu, Jian/0000-0001-5329-7408; Liu, Jian/0000-0001-5329-7408 FU Department of Energy, Basic Energy Sciences, division of Materials Sciences and Engineering (DOE) [DE-FG02-08ER46491]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [KC020105-FWP12152]; U.S. Department of Energy [DE-AC05-76RL01830] FX The synthesis, spectroscopic characterization, and modeling work performed at Rutgers, UT Dallas, and Wake Forest was supported in its totality by the Department of Energy, Basic Energy Sciences, division of Materials Sciences and Engineering (DOE Grant No. DE-FG02-08ER46491). The isotherm measurements, performed at PNNL, were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (Award No. KC020105-FWP12152). Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy under Contract No. DE-AC05-76RL01830. NR 62 TC 20 Z9 20 U1 10 U2 108 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD DEC 10 PY 2013 VL 25 IS 23 BP 4653 EP 4662 DI 10.1021/cm401270b PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 272CG UT WOS:000328437300002 ER PT J AU Chen, QL El Gabaly, F Akgul, FA Liu, Z Mun, BS Yamaguchi, S Braun, A AF Chen, Qianli El Gabaly, Farid Akgul, Funda Alcsoy Liu, Zhi Mun, Bongjin Simon Yamaguchi, Shu Braun, Artur TI Observation of Oxygen Vacancy Filling under Water Vapor in Ceramic Proton Conductors in Situ with Ambient Pressure XPS SO CHEMISTRY OF MATERIALS LA English DT Article DE proton conductor; perovskite; proton diffusivity; oxygen vacancy; AP-XPS; ambient pressure XPS; valence band; in situ spectroscopy; impedance spectroscopy; resonant photoemission ID OPTICAL-ABSORPTION SPECTRA; X-RAY SPECTROSCOPY; ELECTRONIC-STRUCTURE; BULK STATE; BACE0.90Y0.10O3-DELTA; OXIDES; CERIUM AB The interaction of metal oxides with their ambient environment at elevated temperatures is of significant relevance for the functionality and operation of ceramic fuel cells, electrolyzers, and gas sensors. Proton conductivity in metal oxides is a subtle transport process which is based on formation of oxygen vacancies by cation doping and substitution and oxygen vacancy filling upon hydration in water vapor atmosphere. We have investigated the conductivity and electronic structure of the BaCeY-oxide proton conductor under realistic operation conditions from 373 to 593 K and water vapor pressures up to 200 mTorr in situ by combining ambient pressure Xray photoelectron spectroscopy and electrochemical impedance spectroscopy. We provide element specific spectroscopic evidence that oxygen vacancies are filled by oxygen upon water exposure and partly oxidize Ce3+ and Y2+ toward Ce4+ and Y3+. Moreover, the resonant valence band spectra of dry and hydrated samples show that oxygen ligand holes in the proximity of the Y dopant are by around 0.5 eV closer to the Fermi level than the corresponding hole states from Ce. Both hole states become substantially depleted upon hydration, while the proton conductivity sets on and increases systematically. Charge redistribution between lattice oxygen, Ce, and Y when BCY is exposed to water vapor at ambient and high temperature provides insight in the complex mechanism for proton incorporation in BCY. C1 [Chen, Qianli; Braun, Artur] Empa Swiss Fed Labs Mat Sci & Technol, Lab High Performance Ceram, CH-8600 Dubendorf, Switzerland. [Chen, Qianli] ETH, Dept Phys, Swiss Fed Inst Technol, CH-8057 Zurich, Switzerland. [El Gabaly, Farid] Sandia Natl Labs, Livermore, CA 94551 USA. [Akgul, Funda Alcsoy; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Mun, Bongjin Simon] Gwangju Inst Sci & Technol, Ertl Ctr Electrochem & Catalysis, Sch Phys & Chem, Dept Phys & Photon Sci, Kwangju 500712, Chonnam, South Korea. [Yamaguchi, Shu] Univ Tokyo, Dept Mat Engn, Tokyo 1138656, Japan. RP Braun, A (reprint author), Empa Swiss Fed Labs Mat Sci & Technol, Lab High Performance Ceram, CH-8600 Dubendorf, Switzerland. EM artur.braun@alumni.ethz.ch RI Liu, Zhi/B-3642-2009; BRAUN, Artur/A-1154-2009 OI Liu, Zhi/0000-0002-8973-6561; BRAUN, Artur/0000-0002-6992-7774 FU European Community's Sixth Framework Marie Curie International Reintegration Programme [042095]; Swiss National Science Foundation [200021-124812]; Korean-Swiss Cooperative Program in Science and Technology project "Spectroscopy on Photoelectrochemical Electrode Materials (SOPEM) [NRF-2013K1A3A1A14055158]; Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. DOE [DE-AC04-94AL85000]; Director, Office of Science/BES, of the U.S. DoE [DE-AC02-05CH11231] FX The research leading to these results received funding from the European Community's Sixth Framework Marie Curie International Reintegration Programme grant no. 042095 (HiTempE-chem - X-ray and Electrochemical Studies on Solid Oxide Fuel Cells and Related Materials), Swiss National Science Foundation project # 200021-124812 (Effect of lattice volume and imperfections on the proton-phonon coupling in proton conducting lanthanide transition metal oxides: High pressure and high temperature neutron and impedance studies) and by the Korean-Swiss Cooperative Program in Science and Technology project "Spectroscopy on Photoelectrochemical Electrode Materials (SOPEM)" (Call 2010), NRF-2013K1A3A1A14055158. We are grateful to Selma Erat (Empa, ETHZ) and William Chueh (Stanford University) for assistance at the beamline, and Songhak Yoon (Empa) for the high temperature XRD measurements. F.E.G. was supported by the Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. DOE, under contract no. DE-AC04-94AL85000. The ALS is supported by the Director, Office of Science/BES, of the U.S. DoE, No. DE-AC02-05CH11231. NR 24 TC 10 Z9 10 U1 11 U2 90 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD DEC 10 PY 2013 VL 25 IS 23 BP 4690 EP 4696 DI 10.1021/cm401977p PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 272CG UT WOS:000328437300006 ER PT J AU Song, J Wolinsky, M Wren, M Burr, T Li, PE Doggett, N AF Song, Jian Wolinsky, Murray Wren, Melinda Burr, Tom Li, Po-E Doggett, Norman TI Forensic signatures for Marburgviruses SO FORENSIC SCIENCE INTERNATIONAL LA English DT Article DE Forensic science; Hemorrhagic fever virus; Marburgvirus; Canonical SNPs; SNP genotyping; TaqMan-MGB allelic discrimination assay ID HYBRID OLIGONUCLEOTIDE PRIMERS; HEMORRHAGIC-FEVER; VIRUS-INFECTION; SEQUENCE; MODEL; PROTEIN; LETHAL; GLYCOPROTEIN; OUTBREAK; MONKEYS AB Marburgvirus is one of the most important hemorrhagic fever viruses with extremely high infectivity and fatality rate (similar to 90%). It is transmitted easily in human populations through a respiratory route and therefore considered as a major biothreat agent. Although detection assays have been developed, no assay is available for forensic analysis. Here we report development of forensic assays for Marburgvirus. We performed detailed phylogenetic analysis of strains and isolates from all known Marburg virus outbreaks as well as from several laboratory strains and identified canonical SNPs for all major clades (outbreaks) and strains. TaqMan-MGB allelic discrimination assays targeting these SNPs were designed and experimentally screened against synthetic RNA templates and genomic RNAs. A total of 45 assays were validated to provide 100% coverage of the clades (outbreaks) and 91% at the strain level (21 out of the 23 targeted Marburgvirus strains) with built-in redundancy for increased robustness. Using these validated assays, we were able to provide accurate forensic analysis on 3 "unknown" Marburgviruses. These high-resolution forensic assays allow rapid and accurate genotyping of Marburgviruses for forensic investigations. (C) 2013 Elsevier Ireland Ltd. All rights reserved. C1 [Song, Jian; Wolinsky, Murray; Wren, Melinda; Li, Po-E; Doggett, Norman] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Burr, Tom] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM 87545 USA. RP Doggett, N (reprint author), Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87545 USA. EM doggett@lanl.gov OI Wren, Melinda/0000-0003-4714-2287 NR 46 TC 1 Z9 1 U1 0 U2 6 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0379-0738 EI 1872-6283 J9 FORENSIC SCI INT JI Forensic Sci.Int. PD DEC 10 PY 2013 VL 233 IS 1-3 BP 338 EP 347 DI 10.1016/j.forsciint.2013.09.026 PG 10 WC Medicine, Legal SC Legal Medicine GA 264PT UT WOS:000327892400048 PM 24314539 ER PT J AU Kouveliotou, C Granot, J Racusin, JL Bellm, E Vianello, G Oates, S Fryer, CL Boggs, SE Christensen, FE Craig, WW Dermer, CD Gehrels, N Hailey, CJ Harrison, FA Melandri, A McEnery, JE Mundell, CG Stern, DK Tagliaferri, G Zhang, WW AF Kouveliotou, C. Granot, J. Racusin, J. L. Bellm, E. Vianello, G. Oates, S. Fryer, C. L. Boggs, S. E. Christensen, F. E. Craig, W. W. Dermer, C. D. Gehrels, N. Hailey, C. J. Harrison, F. A. Melandri, A. McEnery, J. E. Mundell, C. G. Stern, D. K. Tagliaferri, G. Zhang, W. W. TI NuSTAR OBSERVATIONS OF GRB 130427A ESTABLISH A SINGLE COMPONENT SYNCHROTRON AFTERGLOW ORIGIN FOR THE LATE OPTICAL TO MULTI-GEV EMISSION SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE acceleration of particles; gamma-ray burst: individual (GRB 130427A); magnetic fields; radiation mechanisms: non-thermal; shock waves ID GAMMA-RAY BURSTS; INTERGALACTIC MAGNETIC-FIELDS; HIGH-ENERGY EMISSION; CRAB-NEBULA; PARTICLE-ACCELERATION; RELATIVISTIC SHOCKS; RECONNECTION; FLARES; FERMI; SPECTRUM AB GRB 130427A occurred in a relatively nearby galaxy; its prompt emission had the largest GRB fluence ever recorded. The afterglow of GRB 130427A was bright enough for the Nuclear Spectroscopic Telescope ARray (NuSTAR) to observe it in the 3-79 keV energy range long after its prompt emission (similar to 1.5 and 5 days). This range, where afterglow observations were previously not possible, bridges an important spectral gap. Combined with Swift, Fermi, and ground-based optical data, NuSTAR observations unambiguously establish a single afterglow spectral component from optical to multi-GeV energies a day after the event, which is almost certainly synchrotron radiation. Such an origin of the late-time Fermi/Large Area Telescope >10 GeV photons requires revisions in our understanding of collisionless relativistic shock physics. C1 [Kouveliotou, C.] NASA, George C Marshall Space Flight Ctr, Astrophys Off ZP12, Huntsville, AL 35812 USA. [Granot, J.] Open Univ Israel, Dept Nat Sci, IL-43537 Raanana, Israel. [Racusin, J. L.; Gehrels, N.; McEnery, J. E.; Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Bellm, E.; Harrison, F. A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Vianello, G.] Stanford Univ, Dept Phys, Kavli Inst Particle Astrophys & Cosmol, W Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Vianello, G.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Oates, S.] Univ Coll London, Mullard Space Sci Lab, Dorking RH5 6NT, Surrey, England. [Fryer, C. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Dermer, C. D.] Natl Res Lab, Washington, DC 20375 USA. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Melandri, A.; Tagliaferri, G.] INAF Osservatorio Astron Brera, I-23807 Merate, Italy. [Mundell, C. G.] Liverpool John Moores Univ, Astrophys Res Inst, Liverpool L3 5RF, Merseyside, England. [Stern, D. K.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP Kouveliotou, C (reprint author), NASA, George C Marshall Space Flight Ctr, Astrophys Off ZP12, Huntsville, AL 35812 USA. EM chryssa.kouveliotou@nasa.gov; granot@openu.ac.il; judith.racusin@nasa.gov RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bellm, Eric/0000-0001-8018-5348; Tagliaferri, Gianpiero/0000-0003-0121-0723 FU NASA [NNG08FD60C]; INAF in Italy; CNES in France for science FX This work was supported under NASA Contract NNG08FD60C, and made use of data from the NuSTAR mission, a project led by CalTech, managed by JPL, and funded by NASA. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and CalTech. This work made use of data supplied by the UK Swift Science Data Centre at the University of Leicester. The Fermi/LAT Collaboration acknowledges support from NASA and DOE (U. S.), CEA/Irfu and IN2P3/CNRS (France), ASI and INFN (Italy), MEXT, KEK, and JAXA (Japan), and the K. A. Wallenberg Foundation, the Swedish Research Council and the National Space Board in Sweden. Additional support from INAF in Italy and CNES in France for science analysis during the operations phase is also gratefully acknowledged. The Liverpool Telescope is operated by Liverpool John Moores University at the Observatorio del Roque de los Muchachos of the Instituto de Astrofisica de Canarias. C. G. M. acknowledges support from the Royal Society. NR 41 TC 25 Z9 26 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD DEC 10 PY 2013 VL 779 IS 1 AR L1 DI 10.1088/2041-8205/779/1/L1 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 263ZA UT WOS:000327845400001 ER PT J AU Miller, JM Parker, ML Fuerst, F Bachetti, M Barret, D Grefenstette, BW Tendulkar, S Harrison, FA Boggs, SE Chakrabarty, D Christensen, FE Craig, WW Fabian, AC Hailey, CJ Natalucci, L Paerels, F Rana, V Stern, DK Tomsick, JA Zhang, WW AF Miller, J. M. Parker, M. L. Fuerst, F. Bachetti, M. Barret, D. Grefenstette, B. W. Tendulkar, S. Harrison, F. A. Boggs, S. E. Chakrabarty, D. Christensen, F. E. Craig, W. W. Fabian, A. C. Hailey, C. J. Natalucci, L. Paerels, F. Rana, V. Stern, D. K. Tomsick, J. A. Zhang, W. W. TI CONSTRAINTS ON THE NEUTRON STAR AND INNER ACCRETION FLOW IN SERPENS X-1 USING NuSTAR SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE accretion, accretion disks; equation of state; relativistic processes; X-rays: binaries ID X-RAY BINARIES; IRON EMISSION-LINES; 4U 1705-44; MASS; SPECTROSCOPY; REFLECTION; RADIUS; CLUSTERS; SPECTRUM; BURSTS AB We report on an observation of the neutron star low-mass X-ray binary Serpens X-1, made with NuSTAR. The extraordinary sensitivity afforded by NuSTAR facilitated the detection of a clear, robust, relativistic Fe K emission line from the inner disk. A relativistic profile is required over a single Gaussian line from any charge state of Fe at the 5 sigma level of confidence, and any two Gaussians of equal width at the same confidence. The Compton back-scattering "hump" peaking in the 10-20 keV band is detected for the first time in a neutron star X-ray binary. Fits with relativistically blurred disk reflection models suggest that the disk likely extends close to the innermost stable circular orbit (ISCO) or stellar surface. The best-fit blurred reflection models constrain the gravitational redshift from the stellar surface to be z(NS) >= 0.16. The data are broadly compatible with the disk extending to the ISCO; in that case, z(NS) >= 0.22 and R-NS <= 12.6 km (assuming M-NS = 1.4 M-circle dot and a = 0, where a = cJ/GM(2)). If the star is as large or larger than its ISCO, or if the effective reflecting disk leaks across the ISCO to the surface, the redshift constraints become measurements. We discuss our results in the context of efforts to measure fundamental properties of neutron stars, and models for accretion onto compact objects. C1 [Miller, J. M.] Univ Michigan, Dept Astron, 500 Church St, Ann Arbor, MI 48109 USA. [Parker, M. L.; Fabian, A. C.] Univ Cambridge, Inst Astron, Cambridge CB3 OHA, England. [Fuerst, F.; Grefenstette, B. W.; Tendulkar, S.; Harrison, F. A.; Rana, V.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Bachetti, M.; Barret, D.] Univ Toulouse, UPS OMP, Toulouse, France. [Bachetti, M.; Barret, D.] CNRS, Inst Rech Astrophys & Planetol, F-31028 Toulouse 4, France. [Boggs, S. E.; Craig, W. W.; Tomsick, J. A.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Chakrabarty, D.] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Christensen, F. E.] Danish Tech Univ, Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, C. J.; Paerels, F.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Hailey, C. J.; Paerels, F.] Columbia Univ, Dept Astron, New York, NY 10027 USA. [Natalucci, L.] Ist Astrofis & Planetol Spaziali INAF, I-00133 Rome, Italy. [Stern, D. K.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Miller, JM (reprint author), Univ Michigan, Dept Astron, 500 Church St, Ann Arbor, MI 48109 USA. EM jonmm@umich.edu RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337; Rana, Vikram/0000-0003-1703-8796 FU NASA [NNG08FD60C]; California Institute of Technology; NASA FX This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. NR 32 TC 25 Z9 25 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD DEC 10 PY 2013 VL 779 IS 1 AR L2 DI 10.1088/2041-8205/779/1/L2 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 263ZA UT WOS:000327845400002 ER PT J AU Miller, SM Wofsy, SC Michalak, AM Kort, EA Andrews, AE Biraud, SC Dlugokencky, EJ Eluszkiewicz, J Fischer, ML Janssens-Maenhout, G Miller, BR Miller, JB Montzka, SA Nehrkorn, T Sweeney, C AF Miller, Scot M. Wofsy, Steven C. Michalak, Anna M. Kort, Eric A. Andrews, Arlyn E. Biraud, Sebastien C. Dlugokencky, Edward J. Eluszkiewicz, Janusz Fischer, Marc L. Janssens-Maenhout, Greet Miller, Ben R. Miller, John B. Montzka, Stephen A. Nehrkorn, Thomas Sweeney, Colm TI Anthropogenic emissions of methane in the United States SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE climate change policy; geostatistical inverse modeling ID GEOSTATISTICAL APPROACH; ATMOSPHERIC METHANE; NITROUS-OXIDE; STILT MODEL; CO2; POLLUTION; DECADES AB This study quantitatively estimates the spatial distribution of anthropogenic methane sources in the United States by combining comprehensive atmospheric methane observations, extensive spatial datasets, and a high-resolution atmospheric transport model. Results show that current inventories from the US Environmental Protection Agency (EPA) and the Emissions Database for Global Atmospheric Research underestimate methane emissions nationally by a factor of similar to 1.5 and similar to 1.7, respectively. Our study indicates that emissions due to ruminants and manure are up to twice the magnitude of existing inventories. In addition, the discrepancy in methane source estimates is particularly pronounced in the south-central United States, where we find total emissions are similar to 2.7 times greater than in most inventories and account for 24 +/- 3% of national emissions. The spatial patterns of our emission fluxes and observed methane-propane correlations indicate that fossil fuel extraction and refining are major contributors (45 +/- 13%) in the south-central United States. This result suggests that regional methane emissions due to fossil fuel extraction and processing could be 4.9 +/- 2.6 times larger than in EDGAR, the most comprehensive global methane inventory. These results cast doubt on the US EPA's recent decision to downscale its estimate of national natural gas emissions by 25-30%. Overall, we conclude that methane emissions associated with both the animal husbandry and fossil fuel industries have larger greenhouse gas impacts than indicated by existing inventories. C1 [Miller, Scot M.; Wofsy, Steven C.] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Michalak, Anna M.] Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94305 USA. [Kort, Eric A.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Andrews, Arlyn E.; Dlugokencky, Edward J.; Montzka, Stephen A.] NOAA, Global Monitoring Div, Earth Syst Res Lab, Boulder, CO 80305 USA. [Biraud, Sebastien C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Fischer, Marc L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Eluszkiewicz, Janusz; Nehrkorn, Thomas] Atmospher & Environm Res, Lexington, MA 02421 USA. [Janssens-Maenhout, Greet] Commiss European Communities, Joint Res Ctr, Inst Environm & Sustainabil, I-21027 Ispra, Italy. [Miller, Ben R.; Miller, John B.; Sweeney, Colm] Univ Colorado Boulder, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. RP Miller, SM (reprint author), Harvard Univ, Dept Earth & Planetary Sci, 20 Oxford St, Cambridge, MA 02138 USA. EM scot.m.miller@gmail.com RI Kort, Eric/F-9942-2012; Andrews, Arlyn/K-3427-2012; Biraud, Sebastien/M-5267-2013; OI Kort, Eric/0000-0003-4940-7541; Biraud, Sebastien/0000-0001-7697-933X; Miller, Benjamin/0000-0003-1647-0122; Montzka, Stephen/0000-0002-9396-0400; Nehrkorn, Thomas/0000-0003-0637-3468 FU American Meteorological Society Graduate Student Fellowship/Department of Energy (DOE) Atmospheric Radiation Measurement Program, a DOE Computational Science Graduate Fellowship; National Science Foundation Graduate Research Fellowship Program; Atmospheric Composition and Climate Program of NOAA's Climate Program Office; Carbon Cycle Program of NOAA's Climate Program Office; NASA [NNX08AR47G, NNX11AG47G]; NOAA [NA09OAR4310122, NA11OAR4310158]; National Science Foundaton (NSF) [ATM-0628575]; Environmental Defense Fund [0146-10100]; California Energy Commission Public Interest Environmental Research Program through US Department of Energy [DE-AC02-05CH11231]; Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231]; Office of Biological and Environmental Research of the US Department of Energy as part of the Atmospheric Radiation Measurement Program (ARM); Office of Biological and Environmental Research of the US Department of Energy as part of ARM Aerial Facility; Office of Biological and Environmental Research of the US Department of Energy as part of Terrestrial Ecosystem Science Program; NSF [ATM-0836153]; NASA; NOAA; US intelligence community FX For advice and support, we thank Roisin Commane, Elaine Gottlieb, and Matthew Hayek (Harvard University); Robert Harriss (Environmental Defense Fund); Hanqin Tian and Bowen Zhang (Auburn University); Jed Kaplan (Ecole Polytechnique Federale de Lausanne); Kimberly Mueller and Christopher Weber (Institute for Defense Analyses Science and Technology Policy Institute); Nadia Oussayef; and Gregory Berger. In addition, we thank the National Aeronautics and Space Administration (NASA) Advanced Supercomputing Division for computing help; P. Lang, K. Sours, and C. Siso for analysis of National Oceanic and Atmospheric Administration (NOAA) flasks; and B. Hall for calibration standards work. This work was supported by the American Meteorological Society Graduate Student Fellowship/Department of Energy (DOE) Atmospheric Radiation Measurement Program, a DOE Computational Science Graduate Fellowship, and the National Science Foundation Graduate Research Fellowship Program. NOAA measurements were funded in part by the Atmospheric Composition and Climate Program and the Carbon Cycle Program of NOAA's Climate Program Office. Support for this research was provided by NASA Grants NNX08AR47G and NNX11AG47G, NOAA Grants NA09OAR4310122 and NA11OAR4310158, National Science Foundaton (NSF) Grant ATM-0628575, and Environmental Defense Fund Grant 0146-10100 (to Harvard University). Measurements at Walnut Grove were supported in part by a California Energy Commission Public Interest Environmental Research Program grant to Lawrence Berkeley National Laboratory through the US Department of Energy under Contract DE-AC02-05CH11231. DOE flights were supported by the Office of Biological and Environmental Research of the US Department of Energy under Contract DE-AC02-05CH11231 as part of the Atmospheric Radiation Measurement Program (ARM), ARM Aerial Facility, and Terrestrial Ecosystem Science Program. Weather Research and Forecasting-Stochastic Time-Inverted Lagrangian Transport model development at Atmospheric and Environmental Research has been funded by NSF Grant ATM-0836153, NASA, NOAA, and the US intelligence community. NR 43 TC 156 Z9 161 U1 10 U2 136 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD DEC 10 PY 2013 VL 110 IS 50 BP 20018 EP 20022 DI 10.1073/pnas.1314392110 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 266YY UT WOS:000328061700028 PM 24277804 ER PT J AU Tisserant, E Malbreil, M Kuo, A Kohler, A Symeonidi, A Balestrini, R Charron, P Duensing, N Frey, NFD Gianinazzi-Pearson, V Gilbert, LB Handa, Y Herr, JR Hijri, M Koul, R Kawaguchi, M Krajinski, F Lammers, PJ Masclauxm, FG Murat, C Morin, E Ndikumana, S Pagni, M Petitpierre, D Requena, N Rosikiewicz, P Riley, R Saito, K Clemente, HS Shapiro, H Van Tuinen, D Becard, G Bonfante, P Paszkowski, U Shachar-Hill, YY Tuskan, GA Young, PW Sanders, IR Henrissat, B Rensing, SA Grigoriev, IV Corradi, N Roux, C Martin, F AF Tisserant, Emilie Malbreil, Mathilde Kuo, Alan Kohler, Annegret Symeonidi, Aikaterini Balestrini, Raffaella Charron, Philippe Duensing, Nina Frey, Nicolas Frei Dit Gianinazzi-Pearson, Vivienne Gilbert, Luz B. Handa, Yoshihiro Herr, Joshua R. Hijri, Mohamed Koul, Raman Kawaguchi, Masayoshi Krajinski, Franziska Lammers, Peter J. Masclauxm, Frederic G. Murat, Claude Morin, Emmanuelle Ndikumana, Steve Pagni, Marco Petitpierre, Denis Requena, Natalia Rosikiewicz, Pawel Riley, Rohan Saito, Katsuharu Clemente, Helene San Shapiro, Harris Van Tuinen, Diederik Becard, Guillaume Bonfante, Paola Paszkowski, Uta Shachar-Hill, Yair Y. Tuskan, Gerald A. Young, Peter W. Sanders, Ian R. Henrissat, Bernard Rensing, Stefan A. Grigoriev, Igor V. Corradi, Nicolas Roux, Christophe Martin, Francis TI Genome of an arbuscular mycorrhizal fungus provides insight into the oldest plant symbiosis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbohydrate-active enzymes; effector; fungal evolution; glomales; mutualism ID GLOMUS-INTRARADICES; GENES; RECOMBINATION; INDIVIDUALS; TRADEOFFS; EVOLUTION; GENETICS; BIOLOGY AB The mutualistic symbiosis involving Glomeromycota, a distinctive phylum of early diverging Fungi, is widely hypothesized to have promoted the evolution of land plants during the middle Paleozoic. These arbuscular mycorrhizal fungi (AMF) perform vital functions in the phosphorus cycle that are fundamental to sustainable crop plant productivity. The unusual biological features of AMF have long fascinated evolutionary biologists. The coenocytic hyphae host a community of hundreds of nuclei and reproduce clonally through large multinucleated spores. It has been suggested that the AMF maintain a stable assemblage of several different genomes during the life cycle, but this genomic organization has been questioned. Here we introduce the 153-Mb haploid genome of Rhizophagus irregularis and its repertoire of 28,232 genes. The observed low level of genome polymorphism (0.43 SNP per kb) is not consistent with the occurrence of multiple, highly diverged genomes. The expansion of mating-related genes suggests the existence of cryptic sex-related processes. A comparison of gene categories confirms that R. irregularis is close to the Mucoromycotina. The AMF obligate biotrophy is not explained by genome erosion or any related loss of metabolic complexity in central metabolism, but is marked by a lack of genes encoding plant cell wall-degrading enzymes and of genes involved in toxin and thiamine synthesis. A battery of mycorrhiza-induced secreted proteins is expressed in symbiotic tissues. The present comprehensive repertoire of R. irregularis genes provides a basis for future research on symbiosis-related mechanisms in Glomeromycota. C1 [Tisserant, Emilie; Kohler, Annegret; Herr, Joshua R.; Murat, Claude; Morin, Emmanuelle; Petitpierre, Denis; Martin, Francis] Univ Lorraine, INRA, Unite Mixte Rech 1136, Ctr Nancy, F-54280 Champenoux, France. [Malbreil, Mathilde; Frey, Nicolas Frei Dit; Gilbert, Luz B.; Clemente, Helene San; Becard, Guillaume; Roux, Christophe] Univ Toulouse 3, CNRS, Unite Mixte Rech 5546, Lab Rech Sci Vegetales,Univ Toulouse, F-31326 Castanet Tolosan, France. [Kuo, Alan; Shapiro, Harris; Grigoriev, Igor V.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Symeonidi, Aikaterini; Rensing, Stefan A.] Univ Freiburg, BIOSS Ctr Biol Signalling Studies, D-79104 Freiburg, Germany. [Symeonidi, Aikaterini; Rensing, Stefan A.] Univ Freiburg, Fac Biol, D-79104 Freiburg, Germany. [Symeonidi, Aikaterini; Rensing, Stefan A.] Univ Marburg, Fac Biol, D-35043 Marburg, Germany. [Balestrini, Raffaella; Bonfante, Paola] CNR, Ist Protez Piante, Dipartimento Sci Vita & Biol Sistemi, I-10125 Turin, Italy. [Charron, Philippe; Ndikumana, Steve; Riley, Rohan; Corradi, Nicolas] Univ Ottawa, Dept Biol, Canadian Inst Adv Res, Ottawa, ON K1N 6N5, Canada. [Duensing, Nina; Krajinski, Franziska] Max Planck Inst Mol Pflanzenphysiol, D-14476 Potsdam, Germany. [Gianinazzi-Pearson, Vivienne] Univ Bourgogne, Unite Mixte Rech 1347, INRA, F-21065 Dijon, France. [Handa, Yoshihiro; Kawaguchi, Masayoshi] Natl Inst Basic Biol, Div Symbiot Syst, Dept Evolutionary Biol & Biodivers, Okazaki, Aichi 4448585, Japan. [Hijri, Mohamed] Univ Montreal, Inst Rech Biol Vegetale, Dept Sci Biol, Montreal, PQ H1X 2B2, Canada. [Koul, Raman; Lammers, Peter J.; Van Tuinen, Diederik] New Mexico State Univ, Dept Chem & Biochem, Las Cruces, NM 88003 USA. [Masclauxm, Frederic G.; Pagni, Marco; Rosikiewicz, Pawel; Sanders, Ian R.] Univ Lausanne, Dept Ecol & Evolut, CH-1015 Lausanne, Switzerland. [Masclauxm, Frederic G.] Swiss Inst Bioinformat, Vital IT Grp, CH-1015 Lausanne, Switzerland. [Requena, Natalia] Karlsruhe Inst Technol, Bot Inst, D-76187 Karlsruhe, Germany. [Saito, Katsuharu] Shinshu Univ, Fac Agr, Nagano 3994598, Japan. [Paszkowski, Uta] Univ Cambridge, Dept Plant Sci, Cambridge CB2 3EA, England. [Shachar-Hill, Yair Y.] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. [Tuskan, Gerald A.] Oak Ridge Natl Lab, Biosci Dept, Oak Ridge, TN 37831 USA. [Young, Peter W.] Univ York, Dept Biol, York YO10 5DD, N Yorkshire, England. [Henrissat, Bernard] Aix Marseille Univ, F-13288 Marseille 9, France. [Henrissat, Bernard] Aix Marseille Univ, Unite Mixte Rech 7257, CNRS, F-13288 Marseille 9, France. [Henrissat, Bernard] Univ Copenhagen, Fac Hlth & Med Sci, Dept Cellular & Mol Med, DK-2200 Copenhagen N, Denmark. RP Martin, F (reprint author), Univ Lorraine, INRA, Unite Mixte Rech 1136, Ctr Nancy, F-54280 Champenoux, France. EM fmartin@nancy.inra.fr RI Young, Peter/C-1446-2012; Henrissat, Bernard/J-2475-2012; Requena Sanchez, Natalia/I-4738-2016; Saito, Katsuharu/I-9304-2014; Tuskan, Gerald/A-6225-2011; Balestrini, Raffaella/Q-1106-2015; OI Young, Peter/0000-0001-5259-4830; Requena Sanchez, Natalia/0000-0001-5406-0015; Bonfante, Paola/0000-0003-3576-8530; Hijri, Mohamed/0000-0001-6112-8372; Saito, Katsuharu/0000-0003-2557-1726; Tuskan, Gerald/0000-0003-0106-1289; Balestrini, Raffaella/0000-0001-7958-7681; Herr, Joshua/0000-0003-3425-292X; Pagni, Marco/0000-0001-9292-9463 FU European Commission [EcoFINDERS FP7-264465]; French National Research Agency through the Clusters of Excellence ARBRE (Advanced Research on the Biology of Tree and Forest Ecosystems) [ANR-11-LABX-0002-01]; French National Research Agency through TULIP (Toward a Unified Theory of Biotic Interactions: Role of Environmental Perturbations) [ANR-10-LABX-41]; US Department of Energy's Oak Ridge National Laboratory Scientific Focus Area for Genomics Foundational Sciences; Conseil Regional Midi-Pyrenees; Natural Sciences and Engineering Research Council of Canada; German Federal Ministry of Education and Research; Swiss National Science Foundation; Italian Regional Project Converging Technologies-BIOBIT; Ministry of Education, Culture, Sports, Science, and Technology of Japan; Programme for Promotion of Basic and Applied Researches for Innovations in Bio-oriented Industry; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX We acknowledge Y.C. Li, H. Niculita-Herzel, and A. Brachman (from the former Joint Genome Institute Glomus consortium) for their genome analyses that were not included in this study. We also thank the Lausanne University Genomic Technologies Facility, especially K. Harshman and E. Beaudoing, for PacBio sequencing support, and the Genome et Transcriptome-Plateforme Genomique (GeT-PlaGE) Facility of Toulouse, especially N. Marsaud and N. Ladouce, for Illumina sequencing support. The computations were performed at the Institut National de la Recherche Agronomique Nancy Ecogenomics facilities and in part at the Vital-IT Center for high-performance computing of the Swiss Institute of Bioinformatics. E.T. is supported by a postdoctoral fellowship from the European Commission (project EcoFINDERS FP7-264465). This work was supported by the French National Research Agency through the Clusters of Excellence ARBRE (Advanced Research on the Biology of Tree and Forest Ecosystems) (ANR-11-LABX-0002-01) and TULIP (Toward a Unified Theory of Biotic Interactions: Role of Environmental Perturbations) (ANR-10-LABX-41). This work was also funded by grants from the US Department of Energy's Oak Ridge National Laboratory Scientific Focus Area for Genomics Foundational Sciences (to F.M. and G.A.T.); the Conseil Regional Midi-Pyrenees (to C.R.); the Natural Sciences and Engineering Research Council of Canada (to N.C.); the German Federal Ministry of Education and Research (to S.A.R.); the Swiss National Science Foundation (to I.R.S.); the Italian Regional Project Converging Technologies-BIOBIT (to P.B.); the Ministry of Education, Culture, Sports, Science, and Technology of Japan (to M.K.); and the Programme for Promotion of Basic and Applied Researches for Innovations in Bio-oriented Industry (to K.S.). The work conducted by the US Department of Energy's Joint Genome Institute is supported by the Office of Science of the US Department of Energy under Contract DE-AC02-05CH11231. NR 32 TC 149 Z9 158 U1 21 U2 289 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD DEC 10 PY 2013 VL 110 IS 50 BP 20117 EP 20122 DI 10.1073/pnas.1313452110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 266YY UT WOS:000328061700045 PM 24277808 ER PT J AU Remillieux, MC Pasareanu, SM Svensson, UP AF Remillieux, Marcel C. Pasareanu, Stephanie M. Svensson, U. Peter TI Numerical modeling of the exterior-to-interior transmission of impulsive sound through three-dimensional, thin-walled elastic structures SO JOURNAL OF SOUND AND VIBRATION LA English DT Article ID ACOUSTIC PULSE-PROPAGATION; CLOSED RECTANGULAR CAVITY; EDGE-DIFFRACTION; URBAN-ENVIRONMENT; COUPLED FINITE; FORMULATION; NOISE; PLATE; SIMULATIONS; VIBRATIONS AB Exterior propagation of impulsive sound and its transmission through three-dimensional, thin walled elastic structures, into enclosed cavities, are investigated numerically in the framework of linear dynamics. A model was developed in the time domain by combining two numerical tools: (i) exterior sound propagation and induced structural loading are computed using the image source method for the reflected field (specular reflections) combined with an extension of the Biot-Tolstoy-Meclyvin method for the diffracted field, (ii) the fully coupled vibro-acoustic response of the interior fluid-structure system is computed using a truncated modal-decomposition approach. In the model for exterior sound propagation, it is assumed that: all surfaces are acoustically rigid. Since coupling between the structure and the exterior fluid is not enforced, the model is applicable to the case of a light exterior fluid and arbitrary interior fluid(s). The structural modes are computed with the finite-element method using shell elements. Acoustic modes are computed analytically assuming acoustically rigid boundaries and rectangular geometries of the enclosed cavities. This model is verified against finite-element solutions for the cases of rectangular structures containing one and two cavities, respectively. Published by Elsevier Ltd. C1 [Remillieux, Marcel C.; Pasareanu, Stephanie M.] Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA. [Svensson, U. Peter] Norwegian Univ Sci & Technol, Dept Elect & Telecommun, Acoust Res Ctr, NO-7491 Trondheim, Norway. RP Remillieux, MC (reprint author), Los Alamos Natl Lab, Geophys Grp EES 17, MS D446, Los Alamos, NM 87545 USA. EM mremilli@vt.edu; psteph7@vt.edu; svensson@iet.ntnu.no RI Svensson, Peter/B-4593-2011 OI Svensson, Peter/0000-0002-2286-7305 FU NASA Langley Research Center [NNL10AA05C] FX The authors would like to acknowledge the financial support from NASA Langley Research Center under Grant number NNL10AA05C. NR 37 TC 2 Z9 2 U1 1 U2 3 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-460X EI 1095-8568 J9 J SOUND VIB JI J. Sound Vibr. PD DEC 9 PY 2013 VL 332 IS 25 BP 6725 EP 6742 DI 10.1016/j.jsv.2013.08.003 PG 18 WC Acoustics; Engineering, Mechanical; Mechanics SC Acoustics; Engineering; Mechanics GA AR4NL UT WOS:000343563400012 ER PT J AU Kawano, DT Morzfeld, M Ma, F AF Kawano, Daniel T. Morzfeld, Matthias Ma, Fai TI The decoupling of second-order linear systems with a singular mass matrix SO JOURNAL OF SOUND AND VIBRATION LA English DT Article ID COORDINATE TRANSFORMATIONS; EQUATIONS; MOTION AB It was demonstrated in earlier work that a nondefective, linear dynamical system with an invertible mass matrix in free or forced motion may be decoupled in the configuration space by a real and isospectral transformation. We extend this work by developing a procedure for decoupling a linear dynamical system with a singular mass matrix in the configuration space, transforming the original differential-algebraic system into decoupled sets of real, independent, first- and second order differential equations. Numerical examples are provided to illustrate the application of the decoupling procedure. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Kawano, Daniel T.] Rose Hulman Inst Technol, Dept Mech Engn, Terre Haute, IN 47803 USA. [Morzfeld, Matthias] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Math, Berkeley, CA 94720 USA. [Ma, Fai] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. RP Kawano, DT (reprint author), Rose Hulman Inst Technol, Dept Mech Engn, Terre Haute, IN 47803 USA. EM kawano@rose-hulman.edu NR 21 TC 5 Z9 5 U1 0 U2 7 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-460X EI 1095-8568 J9 J SOUND VIB JI J. Sound Vibr. PD DEC 9 PY 2013 VL 332 IS 25 BP 6829 EP 6846 DI 10.1016/j.jsv.2013.08.005 PG 18 WC Acoustics; Engineering, Mechanical; Mechanics SC Acoustics; Engineering; Mechanics GA AR4NL UT WOS:000343563400019 ER PT J AU Zhang, XH Zhang, Y Liao, QL Song, Y Ma, SW AF Zhang, Xiaohui Zhang, Yue Liao, Qingliang Song, Yu Ma, Siwei TI Reduced Graphene Oxide-Functionalized High Electron Mobility Transistors for Novel Recognition Pattern Label-Free DNA Sensors SO SMALL LA English DT Article ID FIELD-EFFECT-TRANSISTOR; BIOSENSORS; GRAPHITE; FILMS AB We designed and constructed reduced graphene oxide (rGO) functionalized high electron mobility transistor (HEMT) for rapid and ultra-sensitive detection of label-free DNA in real time. The micrometer sized rGO sheets with structural defects helped absorb DNA molecules providing a facile and robust approach to functionalization. DNA was immobilized onto the surface of HEMT gate through rGO functionalization, and changed the conductivity of HEMT. The real time monitor and detection of DNA hybridization by rGO functionalized HEMT presented interesting current responses: a "two steps" signal enhancement in the presence of target DNA; and a "one step" signaling with random DNA. These two different recognition patterns made the HEMT capable of specifically detecting target DNA sequence. The working principle of the rGO functionalized HEMT can be demonstrated as the variation of the ambience charge distribution. Furthermore, the as constructed DNA sensors showed excellent sensitivity of detect limit at 0.07 fM with linear detect range from 0.1 fM to 0.1 pM. The results indicated that the HEMT functionalized with rGO paves a new avenue to design novel electronic devices for high sensitive and specific genetic material assays in biomedical applications. C1 [Zhang, Xiaohui; Zhang, Yue; Liao, Qingliang; Song, Yu; Ma, Siwei] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Zhang, Xiaohui] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zhang, Y (reprint author), Univ Sci & Technol Beijing, Sch Mat Sci & Engn, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. EM yuezhang@ustb.edu.cn FU National Major Research Program of China [2013CB932600]; Major Project of International Cooperation and Exchanges [2012DFA50990]; NSFC [51232001, 51172022, 51002008]; Beijing Municipal Commission of Education; Fundamental Research Funds for Central Universities [FRF-TP-12-030A]; Program for Changjiang Scholars and Innovative Research Team in University FX This work was supported by the National Major Research Program of China (2013CB932600), the Major Project of International Cooperation and Exchanges (2012DFA50990), NSFC (51232001, 51172022, and 51002008), the Research Fund of Co-construction Program from the Beijing Municipal Commission of Education, the Fundamental Research Funds for Central Universities (FRF-TP-12-030A), and Program for Changjiang Scholars and Innovative Research Team in University. We also special thanks to Yuehe Lin and Zhiwen Tang from Pacific Northwest National Laboratory for the kind and valuable discussion and assistance during the paper writing. NR 40 TC 15 Z9 15 U1 2 U2 60 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD DEC 9 PY 2013 VL 9 IS 23 BP 4045 EP 4050 DI 10.1002/smll.201300793 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AA7MV UT WOS:000331282400020 PM 23828864 ER PT J AU Gardner, SN Hall, BG AF Gardner, Shea N. Hall, Barry G. TI When Whole-Genome Alignments Just Won't Work: kSNP v2 Software for Alignment-Free SNP Discovery and Phylogenetics of Hundreds of Microbial Genomes SO PLOS ONE LA English DT Article ID TREES; EPIDEMIOLOGY; EVOLUTION AB Effective use of rapid and inexpensive whole genome sequencing for microbes requires fast, memory efficient bioinformatics tools for sequence comparison. The kSNP v2 software finds single nucleotide polymorphisms (SNPs) in whole genome data. kSNP v2 has numerous improvements over kSNP v1 including SNP gene annotation; better scaling for draft genomes available as assembled contigs or raw, unassembled reads; a tool to identify the optimal value of k; distribution of packages of executables for Linux and Mac OS X for ease of installation and user-friendly use; and a detailed User Guide. SNP discovery is based on k-mer analysis, and requires no multiple sequence alignment or the selection of a single reference genome. Most target sets with hundreds of genomes complete in minutes to hours. SNP phylogenies are built by maximum likelihood, parsimony, and distance, based on all SNPs, only core SNPs, or SNPs present in some intermediate user-specified fraction of targets. The SNP-based trees that result are consistent with known taxonomy. kSNP v2 can handle many gigabases of sequence in a single run, and if one or more annotated genomes are included in the target set, SNPs are annotated with protein coding and other information (UTRs, etc.) from Genbank file(s). We demonstrate application of kSNP v2 on sets of viral and bacterial genomes, and discuss in detail analysis of a set of 68 finished E. coli and Shigella genomes and a set of the same genomes to which have been added 47 assemblies and four "raw read'' genomes of H104:H4 strains from the recent European E. coli outbreak that resulted in both bloody diarrhea and hemolytic uremic syndrome (HUS), and caused at least 50 deaths. C1 [Gardner, Shea N.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hall, Barry G.] Bellingham Res Inst, Bellingham, WA USA. RP Gardner, SN (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM gardner26@llnl.gov FU US Department of Homeland Security Science and Technology Directorate [HSHQPM-10-X-00078 P00001, HSHQPM-10-X-00099 P00002]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the US Department of Homeland Security Science and Technology Directorate via awards HSHQPM-10-X-00078 P00001 and HSHQPM-10-X-00099 P00002. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 26 TC 64 Z9 64 U1 1 U2 16 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 9 PY 2013 VL 8 IS 12 AR e81760 DI 10.1371/journal.pone.0081760 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 275VD UT WOS:000328705200048 PM 24349125 ER PT J AU Mohan, S Das, D Bauer, RJ Heroux, A Zalewski, JK Heber, S Dosunmu-Ogunbi, AM Trakselis, MA Hildebrand, JD VanDemark, AP AF Mohan, Swarna Das, Debamitra Bauer, Robert J. Heroux, Annie Zalewski, Jenna K. Heber, Simone Dosunmu-Ogunbi, Atinuke M. Trakselis, Michael A. Hildebrand, Jeffrey D. VanDemark, Andrew P. TI Structure of a Highly Conserved Domain of Rock1 Required for Shroom-Mediated Regulation of Cell Morphology SO PLOS ONE LA English DT Article ID SMOOTH-MUSCLE MYOSIN; RHO-ASSOCIATED KINASE; NEURAL-TUBE CLOSURE; APICAL CONSTRICTION; PROTEIN-KINASE; COILED-COIL; LIGHT-CHAIN; CRYSTAL-STRUCTURE; BINDING PROTEIN; FAMILY PROTEINS AB Rho-associated coiled coil containing protein kinase (Rho-kinase or Rock) is a well-defined determinant of actin organization and dynamics in most animal cells characterized to date. One of the primary effectors of Rock is non-muscle myosin II. Activation of Rock results in increased contractility of myosin II and subsequent changes in actin architecture and cell morphology. The regulation of Rock is thought to occur via autoinhibition of the kinase domain via intramolecular interactions between the N-terminus and the C-terminus of the kinase. This autoinhibited state can be relieved via proteolytic cleavage, binding of lipids to a Pleckstrin Homology domain near the C-terminus, or binding of GTP-bound RhoA to the central coiled-coil region of Rock. Recent work has identified the Shroom family of proteins as an additional regulator of Rock either at the level of cellular distribution or catalytic activity or both. The Shroom-Rock complex is conserved in most animals and is essential for the formation of the neural tube, eye, and gut in vertebrates. To address the mechanism by which Shroom and Rock interact, we have solved the structure of the coiled-coil region of Rock that binds to Shroom proteins. Consistent with other observations, the Shroom binding domain is a parallel coiled-coil dimer. Using biochemical approaches, we have identified a large patch of residues that contribute to Shrm binding. Their orientation suggests that there may be two independent Shrm binding sites on opposing faces of the coiled-coil region of Rock. Finally, we show that the binding surface is essential for Rock colocalization with Shroom and for Shroom-mediated changes in cell morphology. C1 [Mohan, Swarna; Das, Debamitra; Zalewski, Jenna K.; Heber, Simone; Dosunmu-Ogunbi, Atinuke M.; Hildebrand, Jeffrey D.; VanDemark, Andrew P.] Univ Pittsburgh, Dept Biol Sci, Pittsburgh, PA 15260 USA. [Bauer, Robert J.; Trakselis, Michael A.] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Heroux, Annie] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Hildebrand, JD (reprint author), Univ Pittsburgh, Dept Biol Sci, Pittsburgh, PA 15260 USA. EM jeffh@pitt.edu; andyv@pitt.edu OI Bauer, Robert/0000-0001-6317-6933; Trakselis, Michael/0000-0001-7054-8475 FU National Institutes of Health [GM097204] FX This work was supported by funding from the National Institutes of Health (GM097204) to JH and AV. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 59 TC 5 Z9 5 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 9 PY 2013 VL 8 IS 12 AR e81075 DI 10.1371/journal.pone.0081075 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 275VD UT WOS:000328705200016 PM 24349032 ER PT J AU Williams, PT AF Williams, Paul T. TI Breast Cancer Mortality vs. Exercise and Breast Size in Runners and Walkers SO PLOS ONE LA English DT Article ID BODY-MASS INDEX; PHYSICAL-ACTIVITY; POSTMENOPAUSAL WOMEN; WEIGHT-GAIN; RISK; SELECTION; ASSOCIATION; SURVIVAL; DENSITY; ADIPOSITY AB Purpose: Identify predictors of breast cancer mortality in women who exercised below (<7.5 metabolic equivalent hours/week, MET-hours/wk), at (7.5 to 12.5 MET-hours/wk), or above (>= 12.5 MET-hours/wk) recommended levels. Methods: Cox proportional hazard analyses of baseline pre-diagnosis MET-hours/wk vs. breast cancer mortality adjusted for follow-up age, race, baseline menopause, and estrogen and oral contraceptive use in 79,124 women (32,872 walkers, 46,252 runners) from the National Walkers' and Runners' Health Studies. Results: One-hundred eleven women (57 walkers, 54 runners) died from breast cancer during the 11-year follow-up. The decline in mortality in women who exercised >= 7.5 MET-hours/wk was not different for walking and running (P = 0.34), so running and walking energy expenditures were combined. The risk for breast cancer mortality was 41.5% lower for >= 7.5 vs. <7.5 MET-hours/wk (HR: 0.585, 95%Cl: 0.382 to 0.924, P = 0.02), which persisted when adjusted for BMI (HR: 0.584, 95%Cl: 0.368 to 0.956, P = 0.03). Other than age and menopause, baseline bra cup size was the strongest predictor of breast cancer mortality, i.e., 57.9% risk increase per cup size when adjusted for MET-hours/wk and the other covariates (HR: 1.579, 95%Cl: 1.268 to 1.966, P<0.0001), and 70.4% greater when further adjusted for BMI (HR: 1.704, 95%Cl: 1.344 to 2.156, P = 10(-5)). Breast cancer mortality was 4.0-fold greater (HR: 3.980, 95%Cl: 1.894 to 9.412, P = 0.0001) for C-cup, and 4.7-fold greater (HR: 4.668, 95%Cl: 1.963 to 11.980, P = 0.0004) for >= D-cup vs. A-cup when adjusted for BMI and other covariates. Adjustment for cup size and BM I did not eliminate the association between breast cancer mortality and >= 7.5 MET-hour/wk walked or run (HR: 0.615, 95%Cl: 0.389 to 1.004, P = 0.05). Conclusion: Breast cancer mortality decreased in association with both meeting the exercise recommendations and smaller breast volume. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Williams, PT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM ptwilliams@lbl.gov FU National Heart, Lung, and Blood Institute [HL094717] FX This research was supported by grant HL094717 from the National Heart, Lung, and Blood Institute and was conducted at the Ernest Orlando Lawrence Berkeley National Laboratory (Department of Energy DE-AC03-76SF00098 to the University of California). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 43 TC 7 Z9 8 U1 0 U2 9 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 9 PY 2013 VL 8 IS 12 AR e80616 DI 10.1371/journal.pone.0080616 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 275VD UT WOS:000328705200008 PM 24349006 ER PT J AU Beninato, A Emery, T Baglio, S Ando, B Bulsara, AR Jenkins, C Palkar, V AF Beninato, A. Emery, T. Baglio, S. Ando, B. Bulsara, A. R. Jenkins, C. Palkar, V. TI A concept for a magnetic field detector underpinned by the nonlinear dynamics of coupled multiferroic devices SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILMS; FERROELECTRICITY; PROGRESS AB Multiferroic (MF) composites, in which magnetic and ferroelectric orders coexist, represent a very attractive class of materials with promising applications in areas, such as spintronics, memories, and sensors. One of the most important multiferroics is the perovskite phase of bismuth ferrite, which exhibits weak magnetoelectric properties at room temperature; its properties can be enhanced by doping with other elements such as dysprosium. A recent paper has demonstrated that a thin film of Bi0.7Dy0.3FeO3 shows good magnetoelectric coupling. In separate work it has been shown that a carefully crafted ring connection of N (N odd and N >= 3) ferroelectric capacitors yields, past a critical point, nonlinear oscillations that can be exploited for electric (E) field sensing. These two results represent the starting point of our work. In this paper the (electrical) hysteresis, experimentally measured in the MF material Bi0.7Dy0.3FeO3, is characterized with the applied magnetic field (B) taken as a control parameter. This yields a "blueprint" for a magnetic (B) field sensor: a ring-oscillator coupling of N = 3 Sawyer-Tower circuits each underpinned by a mutliferroic element. In this configuration, the changes induced in the ferroelectric behavior by the external or "target" B-field are quantified, thus providing a pathway for very low power and high sensitivity B-field sensing. (C) 2013 AIP Publishing LLC. C1 [Beninato, A.; Baglio, S.; Ando, B.] Univ Catania, Dipartimento Ingn Elettr Elettron & Sistemi, I-95125 Catania, Italy. [Emery, T.; Bulsara, A. R.] Space & Naval Warfare Syst Ctr, San Diego, CA 92152 USA. [Jenkins, C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Palkar, V.] Indian Inst Technol, Dept Elect Engn, Ctr Excellence Nanoelect, Bombay 400076, Maharashtra, India. RP Beninato, A (reprint author), Univ Catania, Dipartimento Ingn Elettr Elettron & Sistemi, Viale A Doria 6, I-95125 Catania, Italy. FU SSC Pacific Naval Innovative Science and Engineering (NISE) Program; US Office of Naval Research [30]; Office of Naval Research-Global FX A.R.B. and T. E. were supported and funded by the SSC Pacific Naval Innovative Science and Engineering (NISE) Program, as well as the US Office of Naval Research (code 30); S. B., A. B., and B. A. acknowledge funding from the Office of Naval Research-Global. V. P. would like to thank K. Prashanthi for experimental help. NR 21 TC 0 Z9 0 U1 0 U2 29 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 244107 DI 10.1063/1.4846315 PG 4 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500110 ER PT J AU Cai, S Schaffer, JE Ren, Y Yu, C AF Cai, S. Schaffer, J. E. Ren, Y. Yu, C. TI Texture evolution during nitinol martensite detwinning and phase transformation SO APPLIED PHYSICS LETTERS LA English DT Article ID SHAPE-MEMORY ALLOY; NEUTRON-DIFFRACTION; THIN-FILMS; DEFORMATION; STENTS; DURABILITY; FATIGUE; STRAIN; TWIN AB Nitinol has been widely used to make medical devices for years due to its unique shape memory and superelastic properties. However, the texture of the nitinol wires has been largely ignored due to inherent complexity. In this study, in situ synchrotron X-ray diffraction has been carried out during uniaxial tensile testing to investigate the texture evolution of the nitinol wires during martensite detwinning, variant reorientation, and phase transformation. It was found that the thermal martensitic nitinol wire comprised primarily an axial ((1) over bar 20), (120), and (102)-fiber texture. Detwinning initially converted the (120) and (102) fibers to the ((1) over bar 20) fiber and progressed to a ((1) over bar 30)-fiber texture by rigid body rotation. At strains above 10%, the ((1) over bar 30)-fiber was shifted to the (110) fiber by (2 (1) over bar0) deformation twinning. The austenitic wire exhibited an axial (334)-fiber, which transformed to the near-((1) over bar 30) martensite texture after the stress-induced phase transformation. (C) 2013 AIP Publishing LLC. C1 [Cai, S.; Schaffer, J. E.] Ft Wayne Met Res Prod Corp, Ft Wayne, IN 46809 USA. [Ren, Y.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Yu, C.] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. RP Cai, S (reprint author), Ft Wayne Met Res Prod Corp, 9609 Ardmore Ave, Ft Wayne, IN 46809 USA. OI Yu, Cun/0000-0003-0084-6746 FU U.S. Department of Energy, Office of Science [DEAC02-06CH11357] FX Use of the synchrotron X-ray at APS was granted by the U.S. Department of Energy, Office of Science, under Contract No. DEAC02-06CH11357. Data analysis was performed by using the FIT2D and Maud software. S. C. and E. S. thank their colleague J. Kolhoff for DSC testing and gratefully acknowledge Fort Wayne Metals management for the continuous support of this research. NR 26 TC 3 Z9 3 U1 0 U2 30 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 241909 DI 10.1063/1.4846495 PG 4 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500027 ER PT J AU Ge, WW Luo, CT Devreugd, CP Zhang, QH Ren, Y Li, JF Luo, HS Viehland, D AF Ge, Wenwei Luo, Chengtao Devreugd, Christopher P. Zhang, Qinhui Ren, Yang Li, Jiefang Luo, Haosu Viehland, D. TI Direct evidence of correlations between relaxor behavior and polar nano-regions in relaxor ferroelectrics: A case study of lead-free piezoelectrics Na0.5Bi0.5TiO3-x%BaTiO3 SO APPLIED PHYSICS LETTERS LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; GLASSY POLARIZATION BEHAVIOR; SODIUM-BISMUTH TITANATE; PHASE-TRANSITIONS; SINGLE-CRYSTALS; MAGNESIUM NIOBATE; NA0.5BI0.5TIO3; CERAMICS AB Diffuse scattering and relaxor behavior in Na0.5Bi0.5TiO3 (NBT) and NBT-5.6 at. % BaTiO3 (NBT-5.6%BT) were investigated. X-ray diffraction revealed two types of diffuse scattering in NBT: (i) broad and (ii) asymmetric L-shaped. After modification with 5.6%BT, the broad diffuse scattering patterns became narrow, and the asymmetric L-shaped ones were replaced by symmetric ones. The symmetric diffuse scattering in NBT-5.6%BT disappeared with increasing dc electric field (E) for E >= 9.5 kV/cm where the frequency dispersion in the dielectric constant disappeared. These results demonstrate that the relaxor characteristics are directly correlated with the diffuse scattering and the presence polar nano-regions. (C) 2013 AIP Publishing LLC. C1 [Ge, Wenwei; Luo, Chengtao; Devreugd, Christopher P.; Li, Jiefang; Viehland, D.] Virginia Tech, Dept Mat Sci & Engn, Blacksburg, VA 24061 USA. [Zhang, Qinhui; Luo, Haosu] Chinese Acad Sci, Shanghai Inst Ceram, Key Lab Inorgan Funct Mat & Device, Shanghai 201800, Peoples R China. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Ge, WW (reprint author), Virginia Tech, Dept Mat Sci & Engn, Blacksburg, VA 24061 USA. EM wenweige@gmail.com FU Department of Energy [DE-FG02-07ER46480]; Office of Naval Research [N00014-13-1-0049]; Natural Science Foundation of China [51332009]; Shanghai Rising-Star Program [11QA1407500]; U.S. Department of Energy Office of Science [DE-AC02-06CH11357] FX This work was supported by the Department of Energy under No. DE-FG02-07ER46480 (DV), Office of Naval Research under No. N00014-13-1-0049 (JFL), the Natural Science Foundation of China under Grant No. 51332009, and the Shanghai Rising-Star Program No. 11QA1407500. Use of the APS was supported by the U.S. Department of Energy Office of Science, under Contract No. DE-AC02-06CH11357. NR 40 TC 14 Z9 14 U1 12 U2 86 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 241914 DI 10.1063/1.4846655 PG 5 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500032 ER PT J AU Liu, R Zheng, SJ Baldwin, JK Kuthuru, M Mara, N Antoniou, A AF Liu, Ran Zheng, Shijian Baldwin, Jon Kevin Kuthuru, Mary Mara, Nathan Antoniou, Antonia TI Synthesis and mechanical behavior of nanoporous nanotwinned copper SO APPLIED PHYSICS LETTERS LA English DT Article ID ELASTIC-MODULUS; STRENGTH; FOAMS; CU; GOLD; INDENTATION; NANOWIRES; COMPOSITE; PLATINUM; HARDNESS AB We synthesize nanoporous copper (NP Cu) through electrochemical dealloying of amorphous Cu0.41Si0.59 under compressive residual stress. Transmission Electron Microscopy reveals that struts are nanocrystalline with grain size equal to the strut thickness. Moreover, a significant population of twins with spacing similar to 7 nm is present within each imaged grain. The hardness of this nanocrystalline, nanotwinned NP Cu is approximately one order of magnitude greater than reports on NP Cu in the literature. The yield strength of individual struts inferred through dimensional analysis is approximately an order of magnitude greater than bulk copper and compares well with other nanostructured copper systems. (C) 2013 AIP Publishing LLC. C1 [Liu, Ran; Antoniou, Antonia] Georgia Inst Technol, Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Zheng, Shijian; Baldwin, Jon Kevin; Mara, Nathan] Los Alamos Natl Lab, MPA CINT, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Kuthuru, Mary] Cross Keys High Sch, Atlanta, GA 30319 USA. RP Antoniou, A (reprint author), Georgia Inst Technol, Woodruff Sch Mech Engn, 801 Ferst Dr, Atlanta, GA 30332 USA. EM antonia.antoniou@me.gatech.edu RI zheng, shijian/F-2453-2012; Mara, Nathan/J-4509-2014; OI Mara, Nathan/0000-0002-9135-4693 FU NSF [CMMI-1200857, CMMI-1301268]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; NSF through RET [DMR-0851574] FX We are grateful to NSF for support through Grant Nos. CMMI-1200857 and CMMI-1301268. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract DE-AC52-06NA25396. Contributions from M. K. were supported by NSF through RET Program No. DMR-0851574. NR 40 TC 4 Z9 5 U1 3 U2 53 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 241907 DI 10.1063/1.4841455 PG 5 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500025 ER PT J AU Mitchell, B Lee, D Lee, D Fujiwara, Y Dierolf, V AF Mitchell, B. Lee, D. Lee, D. Fujiwara, Y. Dierolf, V. TI Vibrationally induced center reconfiguration in co-doped GaN:Eu, Mg epitaxial layers: Local hydrogen migration vs. activation of non-radiative channels SO APPLIED PHYSICS LETTERS LA English DT Article ID ELECTRON-BEAM IRRADIATION; CHEMICAL-VAPOR-DEPOSITION; P-TYPE GAN; LUMINESCENCE; FILMS; BAND AB Europium doped gallium nitride (GaN:Eu) is a promising candidate as a material for red light emitting diodes. When Mg was co-doped into GaN: Eu, additional incorporation environments were discovered that show high excitation efficiency at room temperature and have been attributed to the coupling of Mg-H complexes to the majority Eu site. Electron beam irradiation, indirect and resonant (direct) laser excitation were found to modify these complexes, indicating that vibrational energy alone can trigger the migration of the H while the presence of additional charges and excess energy controls the type of reconfiguration and the activation of non-radiative decay channels. (C) 2013 AIP Publishing LLC. C1 [Mitchell, B.; Dierolf, V.] Lehigh Univ, Bethlehem, PA 18015 USA. [Lee, D.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Lee, D.; Fujiwara, Y.] Osaka Univ, Suita, Osaka 5650871, Japan. RP Mitchell, B (reprint author), Lehigh Univ, 16 Mem Dr E, Bethlehem, PA 18015 USA. RI Fujiwara, Yasufumi/D-9052-2012; Lee, Donghwa/G-7934-2012; OI Lee, Donghwa/0000-0002-8956-3648; Lee, Dong-gun/0000-0002-5339-9364 FU National Science Foundation [ECCS-1140038]; Japan Society for the Promotion of Science [19GS1209, 24226009]; U.S. Department of Energy at Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The work at Lehigh was supported by the National Science Foundation grant (ECCS-1140038). The work at Osaka was partly supported by a Grant-in-Aid for Creative Scientific Research (Grant No. 19GS1209) and a Grant-in-Aid for Scientific Research (S) (Grant No. 24226009) from the Japan Society for the Promotion of Science. Computational work was performed under the auspices of the U.S. Department of Energy at Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 23 TC 5 Z9 5 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 242105 DI 10.1063/1.4846575 PG 4 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500038 ER PT J AU Schultes, FJ Christian, T Jones-Albertus, R Pickett, E Alberi, K Fluegel, B Liu, T Misra, P Sukiasyan, A Yuen, H Haegel, NM AF Schultes, F. J. Christian, T. Jones-Albertus, R. Pickett, E. Alberi, K. Fluegel, B. Liu, T. Misra, P. Sukiasyan, A. Yuen, H. Haegel, N. M. TI Temperature dependence of diffusion length, lifetime and minority electron mobility in GaInP SO APPLIED PHYSICS LETTERS LA English DT Article ID LIQUID-PHASE EPITAXY; P-TYPE GAAS; CARRIER MOBILITY; DEVICE SIMULATION; TRANSPORT; MAJORITY; MODEL AB The mobility of electrons in double heterostructures of p-type Ga0.50In0.50P has been determined by measuring minority carrier diffusion length and lifetime. The minority electron mobility increases monotonically from 300 K to 5 K, limited primarily by optical phonon and alloy scattering. Comparison to majority electron mobility over the same temperature range in comparably doped samples shows a significant reduction in ionized impurity scattering at lower temperatures, due to differences in interaction of repulsive versus attractive carriers with ionized dopant sites. These results should be useful in modeling and optimization for multi-junction solar cells and other optoelectronic devices. (C) 2013 AIP Publishing LLC. C1 [Schultes, F. J.; Haegel, N. M.] Naval Postgrad Sch, Dept Phys, Monterey, CA 93943 USA. [Christian, T.; Alberi, K.; Fluegel, B.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Jones-Albertus, R.; Pickett, E.; Liu, T.; Misra, P.; Sukiasyan, A.; Yuen, H.] Solar Junct Inc, San Jose, CA 95131 USA. RP Haegel, NM (reprint author), Naval Postgrad Sch, Dept Phys, Monterey, CA 93943 USA. EM nmhaegel@nps.edu FU Naval Postgraduate School in part by National Science Foundation [DMR-0804527]; NPS Energy Academic Group; Navy Energy Coordination Office; Department of Energy, Office of Science Graduate Fellowship Program (DOE SCGF); Department of Energy Office of Science, Basic Energy Sciences [DE-AC36-08GO28308] FX This work was supported at the Naval Postgraduate School in part by National Science Foundation Grant No. DMR-0804527 and in part by the NPS Energy Academic Group with funding from the Navy Energy Coordination Office. T. C. acknowledges support from the Department of Energy, Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under Control No. DE-AC05-06OR23100. TRPL work at NREL was supported by the Department of Energy Office of Science, Basic Energy Sciences under DE-AC36-08GO28308. NR 16 TC 11 Z9 11 U1 1 U2 20 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 242106 DI 10.1063/1.4847635 PG 4 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500039 ER PT J AU Sinsheimer, J Callori, SJ Ziegler, B Bein, B Chinta, PV Ashrafi, A Headrick, RL Dawber, M AF Sinsheimer, J. Callori, S. J. Ziegler, B. Bein, B. Chinta, P. V. Ashrafi, A. Headrick, R. L. Dawber, M. TI In-situ x-ray diffraction study of the growth of highly strained epitaxial BaTiO3 thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID CRITICAL THICKNESS; FERROELECTRICITY; ENHANCEMENT AB In-situ synchrotron x-ray diffraction was performed during the growth of BaTiO3 thin films on SrTiO3 substrates using both off-axis RF magnetron sputtering and pulsed laser deposition techniques. It was found that the films were ferroelectric during the growth process, and the presence or absence of a bottom SrRuO3 electrode played an important role in the growth of the films. Pulsed laser deposited films on SrRuO3 displayed an anomalously high tetragonality and unit volume, which may be connected to the previously predicted negative pressure phase of BaTiO3. (C) 2013 AIP Publishing LLC. C1 [Sinsheimer, J.; Callori, S. J.; Ziegler, B.; Bein, B.; Dawber, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Chinta, P. V.; Ashrafi, A.; Headrick, R. L.] Univ Vermont, Dept Phys, Burlington, VT 05405 USA. RP Sinsheimer, J (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM matthew.dawber@stonybrook.edu FU NSF [DMR 1055413]; DOE [DE-FG02-07ER46380]; MRI-R2 grant [NSF DMR 0959486]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by NSF DMR 1055413 (SBU) and DOE DE-FG02-07ER46380 (UVM). The experimental apparatus used at X21 was partially developed under an MRI-R2 grant (NSF DMR 0959486). Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 19 TC 3 Z9 3 U1 2 U2 52 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 242904 DI 10.1063/1.4848779 PG 4 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500066 ER PT J AU Tselev, A Sangwan, VK Jariwala, D Marks, TJ Lauhon, LJ Hersam, MC Kalinin, SV AF Tselev, Alexander Sangwan, Vinod K. Jariwala, Deep Marks, Tobin J. Lauhon, Lincoln J. Hersam, Mark C. Kalinin, Sergei V. TI Near-field microwave microscopy of high-kappa oxides grown on graphene with an organic seeding layer SO APPLIED PHYSICS LETTERS LA English DT Article ID EPITAXIAL GRAPHENE; DEPOSITION; DIELECTRICS; TRANSISTORS; MONOLAYERS; FILMS AB Near-field scanning microwave microscopy (SMM) is used for non-destructive nanoscale characterization of Al2O3 and HfO2 films grown on epitaxial graphene on SiC by atomic layer deposition using a self-assembled perylene-3,4,9,10-tetracarboxylic dianhydride seeding layer. SMM allows imaging of buried inhomogeneities in the dielectric layer with a spatial resolution close to 100 nm. The results indicate that, while topographic features on the substrate surface cannot be eliminated as possible sites of defect nucleation, the use of a vertically heterogeneous Al2O3/ HfO2 stack suppresses formation of large outgrowth defects in the oxide film, ultimately improving lateral uniformity of the dielectric film. (C) 2013 AIP Publishing LLC. C1 [Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Sangwan, Vinod K.; Jariwala, Deep; Marks, Tobin J.; Lauhon, Lincoln J.; Hersam, Mark C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Marks, Tobin J.; Hersam, Mark C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Tselev, A (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM tseleva@ornl.gov RI Hersam, Mark/B-6739-2009; Lauhon, Lincoln/B-7526-2009; Lauhon, Lincoln/H-2976-2015; Tselev, Alexander/L-8579-2015; Jariwala, Deep/E-9913-2013; Kalinin, Sergei/I-9096-2012 OI Lauhon, Lincoln/0000-0001-6046-3304; Tselev, Alexander/0000-0002-0098-6696; Kalinin, Sergei/0000-0001-5354-6152 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U. S. Department of Energy; Office of Naval Research [N00014-11-1-0463]; W. M. Keck Foundation Science and Engineering Grant; Materials Research Science and Engineering Center (MRSEC) of Northwestern University [DMR-1121262] FX A portion of this research (A.T., S.V.K.) was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U. S. Department of Energy. This research was also supported by the Office of Naval Research (N00014-11-1-0463), a W. M. Keck Foundation Science and Engineering Grant, and the Materials Research Science and Engineering Center (MRSEC) of Northwestern University (NSF DMR-1121262). NR 25 TC 4 Z9 5 U1 4 U2 27 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 243105 DI 10.1063/1.4847675 PG 5 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500072 ER PT J AU Yang, MY Allard, LF Ji, N Zhang, XW Yu, GH Wang, JP AF Yang, Meiyin Allard, Lawrence F. Ji, Nian Zhang, Xiaowei Yu, Guang-Hua Wang, Jian-Ping TI The effect of strain induced by Ag underlayer on saturation magnetization of partially ordered Fe16N2 thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID MOMENT; NITRIDE; IRON AB Partially ordered Fe-N thin films were grown by a facing target sputtering process on the surface of a (001) Ag underlayer on MgO substrates. It was confirmed by x-ray diffraction that the Ag layer enlarged the in-plane lattice of the Fe-N thin films. Domains of the ordered alpha''-Fe16N2 phase within an epitaxial (001) alpha'-FexN phase were identified by electron diffraction and high-resolution aberration-corrected scanning transmission electron microscopy (STEM) methods. STEM dark-field and bright-field images showed the fully ordered structure of the alpha''-Fe16N2 at the atomic column level. High saturation magnetization(Ms) of 1890 emu/cc was obtained for alpha''-Fe16N2 on the Ag underlayer, while only 1500 emu/cc was measured for Fe-N on the Fe underlayer. The results are likely due to a tensile strain induced in the alpha''-Fe16N2 phase by the Ag structure at the interface. (C) 2013 AIP Publishing LLC. C1 [Yang, Meiyin; Yu, Guang-Hua] Univ Sci & Technol Beijing, Dept Mat Phys & Chem, Beijing 100083, Peoples R China. [Yang, Meiyin; Ji, Nian; Zhang, Xiaowei; Wang, Jian-Ping] Univ Minnesota, Ctr Micromagnet & Informat Technol MINT, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. [Allard, Lawrence F.] Oak Ridge Natl Lab, Mat Sci & Technol Div, High Temp Mat Lab, Oak Ridge, TN 37831 USA. RP Wang, JP (reprint author), Univ Sci & Technol Beijing, Dept Mat Phys & Chem, Beijing 100083, Peoples R China. EM jpwang@umn.edu FU DOE ARPA-E REACT Program [DE-AR0000199]; National Science Foundation of China [51331002, 51371027] FX This work was partially supported by a DOE ARPA-E REACT Program, DE-AR0000199, and National Science Foundation of China, Grant Nos. 51331002 and 51371027. NR 20 TC 6 Z9 6 U1 3 U2 34 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 242412 DI 10.1063/1.4847315 PG 4 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500053 ER PT J AU Zhang, W Vlaminck, V Pearson, JE Divan, R Bader, SD Hoffmann, A AF Zhang, Wei Vlaminck, Vincent Pearson, John E. Divan, Ralu Bader, Samuel D. Hoffmann, Axel TI Determination of the Pt spin diffusion length by spin-pumping and spin Hall effect SO APPLIED PHYSICS LETTERS LA English DT Article ID RESONANCE AB The spin diffusion length of Pt at room temperature and at 8 K is experimentally determined via spin pumping and spin Hall effect in permalloy/Pt bilayers. Voltages generated during excitation of ferromagnetic resonance from the inverse spin Hall effect and anisotropic magnetoresistance effect were investigated with a broadband approach. Varying the Pt layer thickness gives rise to an evolution of the voltage line shape due to the superposition of the above two effects. By studying the ratio of the two voltage components with the Pt layer thickness, the spin diffusion length of Pt can be directly extracted. We obtain a spin diffusion length of similar to 1.2 nm at room temperature and similar to 1.6 nm at 8 K. (C) 2013 AIP Publishing LLC. C1 [Zhang, Wei; Vlaminck, Vincent; Pearson, John E.; Bader, Samuel D.; Hoffmann, Axel] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Vlaminck, Vincent] Univ San Fransciso Quito, Colegio Ciencias & Ingn, Quito, Ecuador. [Divan, Ralu; Bader, Samuel D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Zhang, W (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Zhang, Wei/G-1523-2012; Hoffmann, Axel/A-8152-2009 OI Zhang, Wei/0000-0002-5878-3090; Hoffmann, Axel/0000-0002-1808-2767 FU U. S. Department of Energy, Office of Science, Basic Energy Science [DE-AC02-06CH11357] FX This work and the use of the Center for Nanoscale Materials at Argonne National Laboratory were supported by the U. S. Department of Energy, Office of Science, Basic Energy Science under Contract No. DE-AC02-06CH11357. NR 38 TC 44 Z9 44 U1 6 U2 62 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 9 PY 2013 VL 103 IS 24 AR 242414 DI 10.1063/1.4848102 PG 4 WC Physics, Applied SC Physics GA 275VO UT WOS:000328706500055 ER PT J AU Aschenauer, EC Burton, T Stratmann, M Martini, T Spiesberger, H AF Aschenauer, Elke C. Burton, Thomas Stratmann, Marco Martini, Till Spiesberger, Hubert TI Prospects for charged current deep-inelastic scattering off polarized nucleons at a future electron-ion collider SO PHYSICAL REVIEW D LA English DT Article ID WEAK STRUCTURE FUNCTIONS; MONTE-CARLO GENERATOR; TO-LEADING-ORDER; PARTON DISTRIBUTIONS; SPIN ASYMMETRIES; HERA ENERGIES; PROTON; QCD; PHYSICS; SIMULATION AB We present a detailed phenomenological study of charged-current-mediated deep-inelastic scattering off longitudinally polarized nucleons at a future electron-ion collider. A new version of the event generator package DJANGOH, extended by capabilities to handle processes with polarized nucleons, is introduced and used to simulate charged current deep-inelastic scattering including QED, QCD, and electroweak radiative effects. We carefully explore the range of validity and the accuracy of the Jacquet-Blondel method to reconstruct the relevant kinematic variables from the measured hadronic final state in charged current events, assuming realistic detector performance parameters. Finally, we estimate the impact of the simulated charged current single-spin asymmetries on determinations of helicity parton distributions in the context of a global QCD analysis at next-to-leading order accuracy. C1 [Aschenauer, Elke C.; Burton, Thomas; Stratmann, Marco] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Martini, Till] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Spiesberger, Hubert] Johannes Gutenberg Univ Mainz, Inst Phys, PRISMA Cluster Excellence, D-55099 Mainz, Germany. RP Aschenauer, EC (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM elke@bnl.gov; tpb@bnl.gov; marco@bnl.gov; martinit@physik.hu-berlin.de; spiesber@uni-mainz.de FU U.S. Department of Energy [DE-AC02-98CH10886]; Brookhaven National Laboratory [LDRD 12-034]; DFG [SFB 1044] FX We are grateful to W. Vogelsang for useful discussions about the results shown in the EIC White Paper. We acknowledge support by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886 and by a "Laboratory Research and Development'' grant (LDRD 12-034) from Brookhaven National Laboratory. H. S. has been supported in part by the DFG in the SFB 1044. NR 70 TC 6 Z9 6 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 9 PY 2013 VL 88 IS 11 AR 114025 DI 10.1103/PhysRevD.88.114025 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 275QD UT WOS:000328691000002 ER PT J AU Perez, F Kemp, AJ Divol, L Chen, CD Patel, PK AF Perez, F. Kemp, A. J. Divol, L. Chen, C. D. Patel, P. K. TI Deflection of MeV Electrons by Self-Generated Magnetic Fields in Intense Laser-Solid Interactions SO PHYSICAL REVIEW LETTERS LA English DT Article ID TRANSPORT; IGNITION; TARGETS; PLASMAS AB We show that the interaction of relativistic-intensity, picosecond laser pulses with solid targets is affected by the reflected light through the strong currents and 10(4) T magnetic fields it produces. Three-dimensional particle-in-cell simulations, with the axisymmetry broken by a small angle of incidence, show that these magnetic fields deflect the laser-accelerated electrons away from the incident laser axis. This directly impacts the interpretation of electron divergence and directionality in applications such as laser-driven ion acceleration or fast-ignition inertial fusion. C1 [Perez, F.; Kemp, A. J.; Divol, L.; Chen, C. D.; Patel, P. K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Perez, F (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM perez75@llnl.gov RI Patel, Pravesh/E-1400-2011 FU U.S. Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Simulations were carried out on the Livermore Computing Center's Sierra cluster under a LLNL Grand Challenge allocation. This work was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 35 TC 10 Z9 10 U1 4 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 9 PY 2013 VL 111 IS 24 AR 245001 DI 10.1103/PhysRevLett.111.245001 PG 5 WC Physics, Multidisciplinary SC Physics GA 275SZ UT WOS:000328699200017 PM 24483668 ER PT J AU Barling, A Swaminathan, K Mitros, T James, BT Morris, J Ngamboma, O Hall, MC Kirkpatrick, J Alabady, M Spence, AK Hudson, ME Rokhsar, DS Moose, SP AF Barling, Adam Swaminathan, Kankshita Mitros, Therese James, Brandon T. Morris, Juliette Ngamboma, Ornella Hall, Megan C. Kirkpatrick, Jessica Alabady, Magdy Spence, Ashley K. Hudson, Matthew E. Rokhsar, Daniel S. Moose, Stephen P. TI A detailed gene expression study of the Miscanthus genus reveals changes in the transcriptome associated with the rejuvenation of spring rhizomes SO BMC GENOMICS LA English DT Article DE Transcriptome; Miscanthus; Illumina; Short read sequencing; RNA sequencing; Development ID ARABIDOPSIS-THALIANA PLANTS; JASMONIC ACID; HYDROPHOBIC PROTEINS; INDUCIBLE GENES; MESSENGER-RNA; SINENSIS; SORGHUM; GENOME; ANDROPOGONEAE; INTERPROSCAN AB Background: The Miscanthus genus of perennial C4 grasses contains promising biofuel crops for temperate climates. However, few genomic resources exist for Miscanthus, which limits understanding of its interesting biology and future genetic improvement. A comprehensive catalog of expressed sequences were generated from a variety of Miscanthus species and tissue types, with an emphasis on characterizing gene expression changes in spring compared to fall rhizomes. Results: Illumina short read sequencing technology was used to produce transcriptome sequences from different tissues and organs during distinct developmental stages for multiple Miscanthus species, including Miscanthus sinensis, Miscanthus sacchariflorus, and their interspecific hybrid Miscanthus x giganteus. More than fifty billion base-pairs of Miscanthus transcript sequence were produced. Overall, 26,230 Sorghum gene models (i.e., similar to 96% of predicted Sorghum genes) had at least five Miscanthus reads mapped to them, suggesting that a large portion of the Miscanthus transcriptome is represented in this dataset. The Miscanthus x giganteus data was used to identify genes preferentially expressed in a single tissue, such as the spring rhizome, using Sorghum bicolor as a reference. Quantitative real-time PCR was used to verify examples of preferential expression predicted via RNA-Seq. Contiguous consensus transcript sequences were assembled for each species and annotated using InterProScan. Sequences from the assembled transcriptome were used to amplify genomic segments from a doubled haploid Miscanthus sinensis and from Miscanthus x giganteus to further disentangle the allelic and paralogous variations in genes. Conclusions: This large expressed sequence tag collection creates a valuable resource for the study of Miscanthus biology by providing detailed gene sequence information and tissue preferred expression patterns. We have successfully generated a database of transcriptome assemblies and demonstrated its use in the study of genes of interest. Analysis of gene expression profiles revealed biological pathways that exhibit altered regulation in spring compared to fall rhizomes, which are consistent with their different physiological functions. The expression profiles of the subterranean rhizome provides a better understanding of the biological activities of the underground stem structures that are essentials for perenniality and the storage or remobilization of carbon and nutrient resources. C1 [Barling, Adam; Swaminathan, Kankshita; James, Brandon T.; Morris, Juliette; Ngamboma, Ornella; Kirkpatrick, Jessica; Alabady, Magdy; Hudson, Matthew E.; Moose, Stephen P.] Univ Illinois, Inst Genom Biol, Energy Biosci Inst, Urbana, IL 61801 USA. [Barling, Adam; James, Brandon T.; Kirkpatrick, Jessica; Hudson, Matthew E.; Moose, Stephen P.] Univ Illinois, Urbana, IL 61801 USA. [Mitros, Therese; Hall, Megan C.; Rokhsar, Daniel S.] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94720 USA. [Mitros, Therese; Rokhsar, Daniel S.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Spence, Ashley K.] Univ Illinois, Dept Plant Biol, Edward R Madigan Lab, Urbana, IL 61801 USA. [Rokhsar, Daniel S.] DOE Joint Genome Inst, Walnut Creek, CA 94598 USA. RP Moose, SP (reprint author), Univ Illinois, Inst Genom Biol, Energy Biosci Inst, 1206 West Gregory Dr, Urbana, IL 61801 USA. EM smoose@illinois.edu RI Hudson, Matthew/A-4438-2008 OI Hudson, Matthew/0000-0002-4737-0936 FU Energy Biosciences Institute; Department of Energy [DE-SC0005433]; USDA Feedstock Genomics program FX Funding was provided by the Energy Biosciences Institute to SPM, MEH, DSR, AB, KS, TM, BTJ, JM, ON, MCH, JK, and MA. Some of the RNA-Seq data used was funded by Award DE-SC0005433 from the joint Department of Energy and USDA Feedstock Genomics program. We would like to thank Dr. Thomas Voigt and members of the EBI Agronomy Program for growing and maintaining the accessions used in this study. We would also like to thank Won Byoung Chae and John A. Juvik for the greenhouse-grown M. sinensis leaf tissue samples and Katarzyna Glowacka and Stanislaw Jezowski, from the Institute of Plant Genetics, Polish Academy of Sciences, Strzeszynska 34, 60-479 Poznan, Poland, for leaf tissue from the M. sinensis double haploid lines (DH1 and DH2) and their parents (DH1P and DH2P). We thank Alvaro Hernandez and the UIUC Keck Center for Illumina RNA sequencing, Kranthi Varala for sharing scripts to aid the assembly, and David Goodstein and the JGI Phytozome team for database access and numerous pipeline scripts. NR 58 TC 7 Z9 9 U1 5 U2 28 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD DEC 9 PY 2013 VL 14 AR 864 DI 10.1186/1471-2164-14-864 PG 16 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA 275AY UT WOS:000328648800001 PM 24320546 ER PT J AU Zhang, B Huang, YF McDermott, JE Posey, RH Xu, H Zhao, ZM AF Zhang, Bing Huang, Yufei McDermott, Jason E. Posey, Rebecca H. Xu, Hua Zhao, Zhongming TI Interdisciplinary dialogue for education, collaboration, and innovation: Intelligent Biology and Medicine in and beyond 2013 SO BMC GENOMICS LA English DT Article; Proceedings Paper CT International Conference on Intelligent Biology and Medicine (ICIBM) CY AUG 11-13, 2013 CL Nashville, TN AB The 2013 International Conference on Intelligent Biology and Medicine (ICIBM 2013) was held on August 11-13, 2013 in Nashville, Tennessee, USA. The conference included six scientific sessions, two tutorial sessions, one workshop, two poster sessions, and four keynote presentations that covered cutting-edge research topics in bioinformatics, systems biology, computational medicine, and intelligent computing. Here, we present a summary of the conference and an editorial report of the supplements to BMC Genomics and BMC Systems Biology that include 19 research papers selected from ICIBM 2013. C1 [Zhang, Bing; Posey, Rebecca H.; Zhao, Zhongming] Vanderbilt Univ, Sch Med, Dept Biomed Informat, Nashville, TN 37232 USA. [Zhang, Bing; Zhao, Zhongming] Vanderbilt Univ, Sch Med, Dept Canc Biol, Nashville, TN 37232 USA. [Zhang, Bing; Zhao, Zhongming] Vanderbilt Univ, Ctr Quantitat Sci, Nashville, TN 37232 USA. [Huang, Yufei] Univ Texas San Antonio, Dept Elect & Comp Engn, San Antonio, TX 78249 USA. [McDermott, Jason E.] Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA 99352 USA. [Xu, Hua] Univ Texas Houston, Hlth Sci Ctr, Sch Biomed Informat, Houston, TX 77030 USA. [Zhao, Zhongming] Vanderbilt Univ, Sch Med, Dept Psychiat, Nashville, TN 37212 USA. RP Zhang, B (reprint author), Vanderbilt Univ, Sch Med, Dept Biomed Informat, Nashville, TN 37232 USA. EM bing.zhang@vanderbilt.edu; zhongming.zhao@vanderbilt.edu FU NCI NIH HHS [U24 CA160019] NR 22 TC 0 Z9 0 U1 1 U2 9 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD DEC 9 PY 2013 VL 14 SU 8 AR S1 DI 10.1186/1471-2164-14-S8-S1 PG 6 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA 270MS UT WOS:000328323100001 PM 24564388 ER PT J AU Franz, JA O'Hagan, M Ho, MH Liu, T Helm, ML Lense, S DuBois, DL Shaw, WJ Appel, AM Raugei, S Bullock, RM AF Franz, James A. O'Hagan, Molly Ho, Ming-Hsun Liu, Tianbiao Helm, Monte L. Lense, Sheri DuBois, Daniel L. Shaw, Wendy J. Appel, Aaron M. Raugei, Simone Bullock, R. Morris TI Conformational Dynamics and Proton Relay Positioning in Nickel Catalysts for Hydrogen Production and Oxidation SO ORGANOMETALLICS LA English DT Article ID H-2 PRODUCTION; PENDANT AMINES; ELECTROCATALYTIC OXIDATION; NMR-SPECTROSCOPY; COMPLEXES; ENERGY; COORDINATION; MODEL; PSEUDOPOTENTIALS; APPROXIMATION AB The [Ni((P2NR)-N-R'2)2](2+) complexes (where PR2NR'2 is 1,5-R'-3,7-R-1,5-diaza-3,7-diphosphacyclooctane) are fast electrocatalysts for H2 production and oxidation. Binding of a fifth ligand (CH3CN or BF4) or chair/boat isomerization has the potential to slow catalysis by blocking the addition of H-2 or by incorrectly positioning the pendant amines. We report the structural dynamics of a series of nickel complexes characterized by NMR spectroscopy and theoretical modeling to examine the effects of the fifth ligand for the Ni(II) complexes, including CH3CN, BF4, Cl, and H, as well as the differences in dynamics between the Ni(II) and Ni(0) oxidation states. A fast exchange process was observed for the [Ni(CH3CN)((P2NR)-N-R'2)2](2+) complexes, with rates ranging from 104 to 107 s1 depending on the phosphorus and nitrogen substituents on the PR2NR'2 ligand. This exchange process was identified to occur through a multistep mechanism, which consists of dissociation of the acetonitrile, boat/chair isomerization of each of the four rings (including nitrogen inversion), and reassociation of an acetonitrile on the opposite side of the complex. The rate of the chair/boat inversion was found to be influenced by varying the substituent on the nitrogen atom, but the rate of the overall exchange process is at least an order of magnitude faster than the catalytic rate in acetonitrile, demonstrating that the structural dynamics of the [Ni(CH3CN)((P2NR)-N-R'2)2](2+) complexes do not hinder catalysis. Possible catalytic implications of the coordination of a fifth ligand to the Ni(II) complex are discussed. C1 [Franz, James A.; O'Hagan, Molly; Ho, Ming-Hsun; Liu, Tianbiao; Helm, Monte L.; Lense, Sheri; DuBois, Daniel L.; Shaw, Wendy J.; Appel, Aaron M.; Raugei, Simone; Bullock, R. Morris] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Richland, WA 99352 USA. RP Appel, AM (reprint author), Pacific NW Natl Lab, Ctr Mol Electrocatalysis, POB 999,K2-57, Richland, WA 99352 USA. EM aaron.appel@pnnl.gov; simone.raugei@pnnl.gov RI Liu, Tianbiao/A-3390-2011; Bullock, R. Morris/L-6802-2016; OI Bullock, R. Morris/0000-0001-6306-4851; Appel, Aaron/0000-0002-5604-1253 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; U.S. Department of Energy, Office of Science; DOE Office of Science Early Career Research Program through the Office of Basic Energy Sciences; Department of Energy; Office of Science of the U.S. DOE [DE-AC05000R22725] FX We dedicate this paper to the memory of Dr. James A. Franz (1948-2010): a great scientist, mentor, and friend. Research by JAF., M.O., M.-H.H., M.L.H., D.L.D., A.M.A., SR., and R.M.B. was supported as part of the Center for Molecular Electro-catalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science. W.J.S. and S.L. were funded by the DOE Office of Science Early Career Research Program through the Office of Basic Energy Sciences. T.L. was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for the DOE by Battelle. Computational resources were provided at W. R Wiley Environmental Molecular Science Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory, the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory, and the Jaguar supercomputer at Oak Ridge National Laboratory (INCITE 2008-2011 award supported by the Office of Science of the U.S. DOE under Contract No. DE-AC05000R22725). NR 52 TC 18 Z9 18 U1 2 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD DEC 9 PY 2013 VL 32 IS 23 BP 7034 EP 7042 DI 10.1021/om400695w PG 9 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA 269KM UT WOS:000328240200023 ER PT J AU Beekman, M Disch, S Rouvimov, S Kasinathan, D Koepernik, K Rosner, H Zschack, P Neumann, WS Johnson, DC AF Beekman, Matt Disch, Sabrina Rouvimov, Sergei Kasinathan, Deepa Koepernik, Klaus Rosner, Helge Zschack, Paul Neumann, Wolfgang S. Johnson, David C. TI Controlling Size-Induced Phase Transformations Using Chemically Designed Nanolaminates SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE chalcogenides; layered compounds; metastable compounds; nanostructures; phase transitions ID TRANSITION-METAL DICHALCOGENIDES; MISFIT LAYER COMPOUNDS; FERECRYSTALLINE COMPOUNDS; SNSE; NANOCRYSTALS; STABILITY; DEPENDENCE; TEMPERATURE; DIFFRACTION; SYMMETRY C1 [Beekman, Matt] Oregon Inst Technol, Dept Nat Sci, Klamath Falls, OR 97601 USA. [Disch, Sabrina; Neumann, Wolfgang S.; Johnson, David C.] Univ Oregon, Dept Chem, Eugene, OR 97403 USA. [Rouvimov, Sergei] Univ Notre Dame, Dept Elect Engn, Notre Dame, IN 46556 USA. [Kasinathan, Deepa; Rosner, Helge] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Koepernik, Klaus] IFW Dresden, D-01171 Dresden, Germany. [Zschack, Paul] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Beekman, M (reprint author), Oregon Inst Technol, Dept Nat Sci, Klamath Falls, OR 97601 USA. EM matt.beekman@oit.edu; davej@uoregon.edu RI Beekman, Matt/I-4470-2014; Kasinathan, Deepa/M-8825-2015; Disch, Sabrina/K-7185-2013 OI Beekman, Matt/0000-0001-9694-2286; Kasinathan, Deepa/0000-0002-9063-6867; Disch, Sabrina/0000-0002-4565-189X FU NSF through CCI [CHE-1102637]; NSF [MRI 0923577, DMR 0907049]; ONR [N000141110193]; U.S. DOE [DE-AC02-06CH11357] FX This work was supported by the NSF through CCI grant CHE-1102637, and grant MRI 0923577 provided equipment used in this investigation. M. B. acknowledges support from the NSF under grant DMR 0907049. S. R. and W.S.N. acknowledge support from ONR Award No. N000141110193. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The authors thank J. Karapatrova and D. Robinson for their assistance in collection of the synchrotron X-ray diffraction data, and C. Heideman and D. Moore for useful discussions. NR 39 TC 16 Z9 16 U1 5 U2 40 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD DEC 9 PY 2013 VL 52 IS 50 BP 13211 EP 13214 DI 10.1002/anie.201305377 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 263IO UT WOS:000327802100009 PM 24133018 ER PT J AU Zhang, JY Yan, Y Chance, MW Chen, JH Hayat, J Ma, SG Tang, CB AF Zhang, Jiuyang Yan, Yi Chance, Michael W. Chen, Jihua Hayat, Jeffery Ma, Shuguo Tang, Chuanbing TI Charged Metallopolymers as Universal Precursors for Versatile Cobalt Materials SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE cobalt; ion exchange; metallopolymers; nanomaterials; phase transfer ID NANOSTRUCTURED MATERIALS; CARBON NANOTUBES; THIN-FILMS; SUPERCRITICAL FLUIDS; ALLOY NANOPARTICLES; MAGNETIC-PROPERTIES; GOLD NANOPARTICLES; BLOCK-COPOLYMERS; PHASE-TRANSFER; IONIC LIQUID C1 [Zhang, Jiuyang; Yan, Yi; Chance, Michael W.; Hayat, Jeffery; Tang, Chuanbing] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. [Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Ma, Shuguo] Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. RP Tang, CB (reprint author), Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. EM tang4@mailbox.sc.edu RI Chen, Jihua/F-1417-2011; Yan, Yi/A-9071-2015; Zhang, Jiuyang/H-2195-2016; OI Chen, Jihua/0000-0001-6879-5936; Yan, Yi/0000-0003-4119-9047; Tang, Chuanbing/0000-0002-0242-8241 FU National Science Foundation [CHE-1151479]; Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. Department of Energy FX The support from National Science Foundation (CHE-1151479) is acknowledged. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. Department of Energy. NR 54 TC 27 Z9 27 U1 8 U2 59 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD DEC 9 PY 2013 VL 52 IS 50 BP 13387 EP 13391 DI 10.1002/anie.201306432 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 263IO UT WOS:000327802100049 PM 24133033 ER PT J AU Yue, YF Mayes, RT Kim, J Fulvio, PF Sun, XG Tsouris, C Chen, JH Brown, S Dai, S AF Yue, Yanfeng Mayes, Richard T. Kim, Jungseung Fulvio, Pasquale F. Sun, Xiao-Guang Tsouris, Costas Chen, Jihua Brown, Suree Dai, Sheng TI Seawater Uranium Sorbents: Preparation from a Mesoporous Copolymer Initiator by Atom-Transfer Radical Polymerization SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE amidoxime; atom-transfer radical polymerization; mesoporous copolymers; seawater; uranium extraction ID GROUP-CONTAINING ADSORBENT; SEA-WATER; AMIDOXIME GROUPS; EXTRACTION; RECOVERY; ADSORPTION; CARBON; FIBER; PRECONCENTRATION; EQUILIBRIUM C1 [Yue, Yanfeng; Mayes, Richard T.; Fulvio, Pasquale F.; Sun, Xiao-Guang; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Kim, Jungseung; Tsouris, Costas] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Brown, Suree; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM dais@ornl.gov RI Chen, Jihua/F-1417-2011; Fulvio, Pasquale/B-2968-2014; Tsouris, Costas/C-2544-2016; Dai, Sheng/K-8411-2015; Mayes, Richard/G-1499-2016 OI Chen, Jihua/0000-0001-6879-5936; Fulvio, Pasquale/0000-0001-7580-727X; Tsouris, Costas/0000-0002-0522-1027; Dai, Sheng/0000-0002-8046-3931; Mayes, Richard/0000-0002-7457-3261 FU US Department of Energy, Office of Nuclear Energy [E-AC05-00OR22725]; Oak Ridge National Laboratory; Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy FX This research was sponsored by the US Department of Energy, Office of Nuclear Energy under contract DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy. The JAEA adsorbent was kindly donated for testing by the Japan Atomic Energy Agency. We acknowledge Dr. Tomonori Saito for constructive discussions and advice on ATRP reactions. NR 51 TC 63 Z9 65 U1 21 U2 157 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD DEC 9 PY 2013 VL 52 IS 50 BP 13458 EP 13462 DI 10.1002/anie.201307825 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 263IO UT WOS:000327802100064 PM 24174429 ER PT J AU Harding, LB Klippenstein, SJ Lischka, H Shepard, R AF Harding, Lawrence B. Klippenstein, Stephen J. Lischka, Hans Shepard, Ron TI Comparison of multireference configuration interaction potential energy surfaces for H + O-2 -> HO2: the effect of internal contraction SO THEORETICAL CHEMISTRY ACCOUNTS LA English DT Article DE MRCI; Internal contraction; H + O-2 ID H/MU+O-2 ADDITION-REACTIONS; PRESSURE RATE CONSTANTS; BASIS-SETS; DEPENDENCE; TEMPERATURES; PROGRAM; AR AB A comparison is presented of uncontracted multireference singles and doubles configuration interaction (MRCI) and internally contracted MRCI potential energy surfaces for the reaction H(S-2) + O-2 ((3)Sigma(-)(g)) -> HO2((2)A ''). It is found that internal contraction leads to significant differences in the reaction kinetics relative to the uncontracted calculations. C1 [Harding, Lawrence B.; Klippenstein, Stephen J.; Lischka, Hans; Shepard, Ron] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Lischka, Hans] Texas Tech Univ, Dept Chem & Biochem, Lubbock, TX 79409 USA. RP Harding, LB (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM harding@anl.gov RI Lischka, Hans/A-8802-2015; OI Klippenstein, Stephen/0000-0001-6297-9187 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357]; National Science Foundation [CHE-1213263]; Robert A. Welch Foundation [D-0005] FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract Numbers DE-AC02-06CH11357. HL was also supported by the National Science Foundation under Project No. CHE-1213263 and by the Robert A. Welch Foundation under Grant No. D-0005. NR 29 TC 8 Z9 8 U1 1 U2 36 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1432-881X EI 1432-2234 J9 THEOR CHEM ACC JI Theor. Chem. Acc. PD DEC 8 PY 2013 VL 133 IS 2 AR 1429 DI 10.1007/s00214-013-1429-6 PG 7 WC Chemistry, Physical SC Chemistry GA 277RX UT WOS:000328838100001 ER PT J AU Boschen, JS Theis, D Ruedenberg, K Windus, TL AF Boschen, Jeffery S. Theis, Daniel Ruedenberg, Klaus Windus, Theresa L. TI Accurate ab initio potential energy curves and spectroscopic properties of the four lowest singlet states of C-2 SO THEORETICAL CHEMISTRY ACCOUNTS LA English DT Article DE Diatomic carbon; Ab initio electronic structure; Dissociation; Configuration interaction; Spectroscopic properties; Multi-configurational wave functions ID MOLECULAR ELECTRONIC WAVEFUNCTIONS; GAUSSIAN-BASIS SETS; MULTIREFERENCE CONFIGURATION-INTERACTION; PHILLIPS SYSTEM; CORRELATED CALCULATIONS; NITROGEN MOLECULE; COUPLED-CLUSTER; INFRARED BANDS; GROUND-STATE; C2 MOLECULE AB The diatomic carbon molecule has a complex electronic structure with a large number of low-lying electronic excited states. In this work, the potential energy curves (PECs) of the four lowest lying singlet states (X-1 Sigma(+)(g), A(1)Pi(u), B-1 Delta(g), and B'(1)Sigma(+)(g)) were obtained by high-level ab initio calculations. Valence electron correlation was accounted for by the correlation energy extrapolation by intrinsic scaling (CEEIS) method. Additional corrections to the PECs included core-valence correlation and relativistic effects. Spin-orbit corrections were found to be insignificant. The impact of using dynamically weighted reference wave functions in conjunction with CEEIS was examined and found to give indistinguishable results from the even weighted method. The PECs showed multiple curve crossings due to the B-1 Delta(g) state as well as an avoided crossing between the two (1)Sigma(+)(g) states. Vibrational energy levels were computed for each of the four electronic states, as well as rotational constants and spectroscopic parameters. Comparison between the theoretical and experimental results showed excellent agreement overall. Equilibrium bond distances are reproduced to within 0.05 %. The dissociation energies of the states agree with experiment to within similar to 0.5 kcal/mol, achieving "chemical accuracy." Vibrational energy levels show average deviations of similar to 20 cm(-1) or less. The B-1 Delta(g) state shows the best agreement with a mean absolute deviation of 2.41 cm(-1). Calculated rotational constants exhibit very good agreement with experiment, as do the spectroscopic constants. C1 [Boschen, Jeffery S.; Theis, Daniel; Ruedenberg, Klaus; Windus, Theresa L.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Boschen, Jeffery S.; Theis, Daniel; Ruedenberg, Klaus; Windus, Theresa L.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Windus, TL (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM twindus@iastate.edu FU US Department of Energy [DE-AC02-07CH11358]; US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory FX The authors thank Dr. Laimutis Bytautas and Dr. Luke Roskop for helpful discussions related to this work. This research is supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory. The Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 74 TC 17 Z9 17 U1 2 U2 41 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1432-881X EI 1432-2234 J9 THEOR CHEM ACC JI Theor. Chem. Acc. PD DEC 7 PY 2013 VL 133 IS 2 AR 1425 DI 10.1007/s00214-013-1425-x PG 12 WC Chemistry, Physical SC Chemistry GA 277RV UT WOS:000328837900001 ER PT J AU Charnvanichborikarn, S Myers, MT Shao, L Kucheyev, SO AF Charnvanichborikarn, S. Myers, M. T. Shao, L. Kucheyev, S. O. TI Enhanced radiation tolerance of non-polar-terminated ZnO SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID CRYSTAL ORIENTATION; OPTICAL ACTIVATION; DAMAGE FORMATION; SINGLE-CRYSTALS; 15 K; SAPPHIRE; FILMS; MGO; MICROSTRUCTURE; IMPLANTATION AB Room-temperature heavy-ion bombardment of polar (0001) ZnO leads to the formation of intermediate peak and step features in damage-depth profiles measured by ion channeling. Here, we show that these anomalous disorder effects are strongly suppressed for crystals with (11 (2) over bar0) and (10 (1) over bar0) non-polar surface terminations. Possible defect interaction scenarios responsible for the enhanced radiation tolerance of non-polar-terminated ZnO are discussed. (C) 2013 AIP Publishing LLC. C1 [Charnvanichborikarn, S.; Myers, M. T.; Kucheyev, S. O.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Shao, L.] Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. RP Kucheyev, SO (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM kucheyev@llnl.gov FU U.S. DOE by LLNL [DE-AC52-07NA27344]; NSF [0846835]; LLNL Lawrence Scholar Program FX This work was performed under the auspices of the U.S. DOE by LLNL under Contract No. DE-AC52-07NA27344. L. S. thanks the support from NSF Grant No. 0846835, and M. T. M. would like to acknowledge the LLNL Lawrence Scholar Program for funding. NR 37 TC 3 Z9 3 U1 1 U2 11 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 7 PY 2013 VL 114 IS 21 AR 213512 DI 10.1063/1.4842116 PG 5 WC Physics, Applied SC Physics GA 274VZ UT WOS:000328635600019 ER PT J AU Medvedev, NN Starostenkov, MD Manley, ME AF Medvedev, N. N. Starostenkov, M. D. Manley, M. E. TI Energy localization on the Al sublattice of Pt3Al with L1(2) order SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DISCRETE BREATHERS; MODES; GENERATION; EXISTENCE; CRYSTALS; METALS AB A three-dimensional molecular-dynamics model of Pt3Al with L1(2) order was developed and found to support the excitation of discrete breathers (DBs) and energy localization on the Al sublattice. For an initial lattice temperature of 0K, large-amplitude DBs polarized along [100] are found to be very weakly damped, retaining most of their initial energy for more than 1000 cycles, while DBs polarized along [111] damped out over similar to 15 cycles. Because the DBs and their dissipation channels are confined to the Al sublattice, long-lived nonequilibrium states with large energy differences between the Al and Pt sublattices occur. Since collisions during irradiation more efficiently generate lattice vibrations in light atoms than heavy atoms, such nonequilibrium states may occur and alter the relaxation processes occurring during radiation damage. (C) 2013 AIP Publishing LLC. C1 [Medvedev, N. N.; Starostenkov, M. D.] Altay State Tech Univ, Barnaul 656038, Altay Territory, Russia. [Manley, M. E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Medvedev, NN (reprint author), Altay State Tech Univ, Barnaul 656038, Altay Territory, Russia. RI Manley, Michael/N-4334-2015 FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX Research sponsored in part (MEM) by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. NR 33 TC 12 Z9 17 U1 0 U2 4 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 7 PY 2013 VL 114 IS 21 AR 213506 DI 10.1063/1.4837598 PG 4 WC Physics, Applied SC Physics GA 274VZ UT WOS:000328635600013 ER PT J AU Morelock, CR Greve, BK Gallington, LC Chapman, KW Wilkinson, AP AF Morelock, Cody R. Greve, Benjamin K. Gallington, Leighanne C. Chapman, Karena W. Wilkinson, Angus P. TI Negative thermal expansion and compressibility of Sc1-xYxF3 (x <= 0.25) SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; CUBIC PHASE-TRANSITION; FERROELASTIC PROPERTIES; POWDER DIFFRACTION; FLUORIDE GLASSES; RAY-DIFFRACTION; MECHANISM; FEF3; SCF3; PEROVSKITES AB Scandium fluoride displays isotropic negative thermal expansion (NTE) from at least 10 to 1100 K and retains a cubic ReO3-type structure over this range; the NTE is most pronounced at low temperatures. Control of thermal expansion was explored by forming Sc1-xYxF3 (x <= 0.25), which were characterized with synchrotron powder diffraction at ambient pressure from 100 to 800 K. The behavior of the solid solutions under pressure (<= 0.276 GPa) was also examined while heating from 298 to 523 K. Insertion of the relatively large Y3+ ion into ScF3 results in a cubic-to-rhombohedral phase transition upon cooling from ambient temperature to 100 K, even at low substitution levels (5%). The coefficient of thermal expansion (CTE) of the solid solutions in the rhombohedral phase is strongly dependent on both composition and temperature; however, above 400 K, where all samples are cubic, the CTE appears to be largely independent of composition. The isothermal bulk modulus and CTE of ScF3, but not those of the solid solutions, are independent of temperature and pressure, respectively. Yttrium substitution lowers the bulk modulus, even at temperatures where the samples are cubic. Finally, the solid solutions stiffen upon heating. (C) 2013 AIP Publishing LLC. C1 [Morelock, Cody R.; Greve, Benjamin K.; Gallington, Leighanne C.; Wilkinson, Angus P.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Wilkinson, Angus P.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. RP Wilkinson, AP (reprint author), Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. EM angus.wilkinson@chemistry.gatech.edu RI Morelock, Cody/C-2831-2012; Wilkinson, Angus/C-3408-2008; Gallington, Leighanne/G-9341-2011 OI Wilkinson, Angus/0000-0003-2904-400X; Gallington, Leighanne/0000-0002-0383-7522 FU National Science Foundation [DMR-0905842]; United States Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX A.P.W. is grateful for support from the National Science Foundation under Grant No. DMR-0905842. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the United States Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors are grateful for the assistance of G. J. Halder at beamline 1-BM-C of the APS, as well as R. E. Josefsberg of Georgia Tech for assistance in data collection at beamline 11-ID-B. NR 78 TC 22 Z9 23 U1 10 U2 48 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD DEC 7 PY 2013 VL 114 IS 21 AR 213501 DI 10.1063/1.4836855 PG 8 WC Physics, Applied SC Physics GA 274VZ UT WOS:000328635600008 ER PT J AU Halverson, JD Lee, WB Grest, GS Grosberg, AY Kremer, K AF Halverson, Jonathan D. Lee, Won Bo Grest, Gary S. Grosberg, Alexander Y. Kremer, Kurt TI Response to "Comment on 'Molecular dynamics simulation study of nonconcatenated ring polymers in a melt. I. Statics"' [J. Chem. Phys. 139, 217101 (2013)] SO JOURNAL OF CHEMICAL PHYSICS LA English DT Editorial Material C1 [Halverson, Jonathan D.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Lee, Won Bo] Sogang Univ, Dept Chem & Biomol Engn, Seoul, South Korea. [Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Grosberg, Alexander Y.] NYU, Dept Phys, New York, NY 10003 USA. [Grosberg, Alexander Y.] NYU, Ctr Soft Matter Res, New York, NY 10003 USA. [Kremer, Kurt] Max Planck Inst Polymer Res, D-55128 Mainz, Germany. RP Halverson, JD (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RI Kremer, Kurt/G-5652-2011; MPIP, Theory/I-9884-2014; Grosberg, Alexander/O-2122-2015 OI Grosberg, Alexander/0000-0002-4230-8690 NR 9 TC 1 Z9 1 U1 4 U2 25 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD DEC 7 PY 2013 VL 139 IS 21 AR 217102 DI 10.1063/1.4833175 PG 2 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 274WH UT WOS:000328636400051 PM 24320406 ER PT J AU Souvatzis, P Niklasson, AMN AF Souvatzis, Petros Niklasson, Anders M. N. TI Extended Lagrangian Born-Oppenheimer molecular dynamics in the limit of vanishing self-consistent field optimization SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-MATRIX; GAUSSIAN-ORBITALS; HARTREE-FOCK; TRAJECTORIES; SIMULATIONS AB We present an efficient general approach to first principles molecular dynamics simulations based on extended Lagrangian Born-Oppenheimer molecular dynamics [A. M. N. Niklasson, Phys. Rev. Lett. 100, 123004 (2008)] in the limit of vanishing self-consistent field optimization. The reduction of the optimization requirement reduces the computational cost to a minimum, but without causing any significant loss of accuracy or long-term energy drift. The optimization-free first principles molecular dynamics requires only one single diagonalization per time step, but is still able to provide trajectories at the same level of accuracy as "exact," fully converged, Born-Oppenheimer molecular dynamics simulations. The optimization-free limit of extended Lagrangian Born-Oppenheimer molecular dynamics therefore represents an ideal starting point for robust and efficient first principles quantum mechanical molecular dynamics simulations. (C) 2013 AIP Publishing LLC. C1 [Souvatzis, Petros] Uppsala Univ, Div Mat Theory, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Niklasson, Anders M. N.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Souvatzis, P (reprint author), Uppsala Univ, Div Mat Theory, Dept Phys & Astron, Box 516, SE-75120 Uppsala, Sweden. EM petros.souvatsiz@fysik.uu.se; amn@lanl.gov FU (U.S.) Department of Energy (DOE) Office of Basic Energy Sciences; NNSA of the U.S. DOE [DE-AC52-06NA25396]; Goran Gustafsson's Foundation FX P.S. wants to thank L.S. for her eternal patience. A.M.N.N. acknowledges support by the (U.S.) Department of Energy (DOE) Office of Basic Energy Sciences as well as discussions with M. Cawkwell, E. Chisolm, and C. J. Tymczak and stimulating contributions by T. Peery at the T-Division Ten Bar Java group. LANL is operated by Los Alamos National Security, LLC, for the NNSA of the U.S. DOE under Contract No. DE-AC52-06NA25396. Support from Goran Gustafsson's Foundation is acknowledged. NR 41 TC 4 Z9 4 U1 2 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD DEC 7 PY 2013 VL 139 IS 21 AR 214102 DI 10.1063/1.4834015 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 274WH UT WOS:000328636400004 PM 24320359 ER PT J AU Xu, H Pratt, ST AF Xu, Hong Pratt, S. T. TI A new look at the photodissociation of methyl iodide at 193 nm SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MOLECULAR RYDBERG TRANSITIONS; MAGNETIC CIRCULAR-DICHROISM; MULTIPHOTON IONIZATION; EMISSION-SPECTROSCOPY; ATOMIC IODINE; QUANTUM YIELD; B-STATE; CH3I; DYNAMICS; PHOTOIONIZATION AB A new measurement of the photodissociation of CH3I at 193 nm is reported in which we use a combination of vacuum ultraviolet photoionization and velocity map ion imaging. The iodine photofragments are probed by single-photon ionization at photon energies above and below the photoionization threshold of I(P-2(3/2)). The relative I(P-2(3/2)) and I*(P-2(1/2)) photoionization cross sections are determined at these wavelengths by using the known branching fractions for the photodissociation at 266 nm. Velocity map ion images indicate that the branching fraction for I(P-2(3/2)) atoms is non-zero, and yield a value of 0.07 +/- 0.01. Interestingly, the translational energy distribution extracted from the image shows that the translational energy of the I(P-2(3/2)) fragments is significantly smaller than that of the I*(P-2(1/2)) atoms. This observation indicates the internal rotational/vibrational energy of the CH3 co-fragment is very high in the I(P-2(3/2)) channel. The results can be interpreted in a manner consistent with the previous measurements, and provide a more complete picture of the dissociation dynamics of this prototypical molecule. (C) 2013 AIP Publishing LLC. C1 [Xu, Hong; Pratt, S. T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Xu, H (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX We would like to thank Dr. A. Alekseyev for providing the theoretical CH3I potential curves in digital form, and for comments on the manuscript. We would also like to thank S. R. Leone and W. P. Hess for helpful comments. This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Contract No. DE-AC02-06CH11357. NR 63 TC 3 Z9 3 U1 2 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD DEC 7 PY 2013 VL 139 IS 21 AR 214310 DI 10.1063/1.4829747 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 274WH UT WOS:000328636400028 PM 24320383 ER PT J AU Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, Z Masoodi, AA Ahmed, I Ahn, SA Ahn, SU Aimo, I Aiola, S Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alexandre, D Alici, A Alkin, A Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Augustinus, A Averbeck, R Awes, TC Aysto, J Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, PC Baumann, C 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Urciuoli, G. M. Usai, G. L. Vajzer, M. Vala, M. Palomo, L. Valencia Vande Vyvre, P. Vannucci, L. Van Hoorne, J. W. van Leeuwen, M. Vargas, A. Varma, R. Vasileiou, M. Vasiliev, A. Vechernin, V. Veldhoen, M. Venaruzzo, M. Vercellin, E. Vergara, S. Vernet, R. Verweij, M. Vickovic, L. Viesti, G. Viinikainen, J. Vilakazi, Z. Baillie, O. Villalobos Vinogradov, A. Vinogradov, L. Vinogradov, Y. Virgili, T. Viyogi, Y. P. Vodopyanov, A. Voelkl, M. A. Voloshin, S. Voloshin, K. Volpe, G. von Haller, B. Vorobyev, I. Vranic, D. Vrlakova, J. Vulpescu, B. Vyushin, A. Wagner, B. Wagner, V. Wagner, J. Wang, Y. Wang, Y. Wang, M. Watanabe, D. Watanabe, K. Weber, M. Wessels, J. P. Westerhoff, U. Wiechula, J. Wikne, J. Wilde, M. Wilk, G. Wilkinson, J. Williams, M. C. S. Windelband, B. Winn, M. Xiang, C. Yaldo, C. G. Yamaguchi, Y. Yang, H. Yang, P. Yang, S. Yano, S. Yasnopolskiy, S. Yi, J. Yin, Z. Yoo, I.-K. Yushmanov, I. Zaccolo, V. Zach, C. Zampolli, C. Zaporozhets, S. Zarochentsev, A. Zavada, P. Zaviyalov, N. Zbroszczyk, H. Zelnicek, P. Zgura, I. S. Zhalov, M. Zhang, F. Zhang, Y. Zhang, H. Zhang, X. Zhou, D. Zhou, Y. Zhou, F. Zhu, X. Zhu, J. Zhu, J. Zhu, H. Zichichi, A. Zimmermann, M. B. Zimmermann, A. Zinovjev, G. Zoccarato, Y. Zynovyev, M. Zyzak, M. CA ALICE Collab TI Energy dependence of the transverse momentum distributions of charged particles in pp collisions measured by ALICE SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PROTON-PROTON COLLISIONS; PB-PB COLLISIONS; ROOT-S(NN)=2.76 TEV; DIFFRACTION; SUPPRESSION; LHC AB Differential cross sections of charged particles in inelastic pp collisions as a function of pT have been measured at root s = 0.9, 2.76 and 7 TeV at the LHC. The pT spectra are compared to NLO-pQCD calculations. Though the differential cross section for an individual root s cannot be described by NLO-pQCD, the relative increase of cross section with root s is in agreement with NLO-pQCD. 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T.; Ketzer, B.; Kramer, F.; Kulakov, I.; Lehnert, J.; Luettig, P.; Marquard, M.; Pitz, N.; Rascanu, B. T.; Reichelt, P.; Renfordt, R.; Schuchmann, S.; Peloni, A. Tarantola; Ulery, J.; Zyzak, M.] Goethe Univ Frankfurt, Inst Kernphys, Frankfurt, Germany. [Oeschler, H.] Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. [Anielski, J.; Bathen, B.; Dietel, T.; Emschermann, D.; Feldkamp, L.; Haake, R.; Heide, M.; Klein-Bosing, C.; Passfeld, A.; Wessels, J. P.; Westerhoff, U.; Wilde, M.; Zimmermann, M. B.] Univ Munster, Inst Kernphys, Munster, Germany. [Belikov, I.; Hippolyte, B.; Kuhn, C.; Molnar, L.; Roy, C.; Sanchez Castro, X.] Univ Strasbourg, CNRS, IN2P3, IPHC, Strasbourg, France. [Bogolyubsky, M.; Evdokimov, S.; Kharlov, Y.; Patalakha, D. I.; Polichtchouk, B.; Sadovsky, S.; Stolpovskiy, M.] Inst High Energy Phys, Protvino, Russia. [Finogeev, D.; Guber, F.; Karavichev, O.; Karavicheva, T.; Karpechev, E.; Konevskikh, A.; Kurepin, A. 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W.; Barret, V.; Bastid, N.; Crochet, P.; Dupieux, P.; Ichou, R.; Li, S.; Lopez, X.; Manso, F.; Marchisone, M.; Porteboeuf-Houssais, S.; Rosnet, P.; Silvestre, C.; Vulpescu, B.; Zhang, X.] Univ Clermont Ferrand, Clermont Univ, CNRS, IN2P3,LPC, Clermont Ferrand, France. [Arbor, N.; Balbastre, G. Conesa; Faivre, J.; Furget, C.; Guernane, R.; Kox, S.; Real, J. S.] Univ Grenoble 1, Inst Polytech Grenoble, CNRS, IN2P3,LPSC, Grenoble, France. [Bianchi, N.; Diaz, A. Casanova; Cunqueiro, L.; Di Nezza, P.; Fantoni, A.; Gianotti, P.; Muccifora, V.; Reolon, R. A.; Ronchetti, F.; Sakai, S.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Ricci, R. A.; Vannucci, L.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Legnaro, Italy. [Bock, F.; Braidot, E.; Cosentino, M. R.; Loizides, C.; Jacobs, P. M.; Ploskon, M.; Sakai, S.; Symons, T. J. M.; Zhang, X.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Abelev, B.; Garishvili, I.; Soltz, R.] Lawrence Livermore Natl Lab, Livermore, CA USA. 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[Anguelov, V.; Bock, F.; Busch, O.; Fasel, M.; Glassel, P.; Grajcarek, R.; Herrmann, N.; Klein, J.; Kweon, M. J.; Lohner, D.; Lu, X. G.; Maire, A.; Perez, J. Mercado; Oeschler, H.; Oyama, K.; Pachmayer, Y.; Reidt, F.; Reygers, K.; Schicker, R.; Stiller, J. H.; Baillie, O. Villalobos; Voelkl, M. A.; Wang, Y.; Wilkinson, J.; Windelband, B.; Winn, M.; Zimmermann, A.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Agnello, M.; Aimo, I.; Bedda, C.] Politecn Torino, Turin, Italy. [Browning, T. A.; Scharenberg, R. P.; Srivastava, B. K.] Purdue Univ, W Lafayette, IN USA. [Chung, S. U.; Seo, J.; Song, J.; Yi, J.; Yoo, I.-K.] Pusan Natl Univ, Pusan, South Korea. [Andronic, A.; Arsene, I. C.; Averbeck, R.; Braun-Munzinger, P.; Donigus, B.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Knichel, M. L.; Koehler, M. K.; Krzewicki, M.; Lenhardt, M.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Otwinowski, J.; Park, W. J.; Romita, R.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Thaeder, J.; Vranic, D.; Wagner, J.] GSI Helmholtzzentrum Schwerionenforsch, Res Div, Darmstadt, Germany. [Andronic, A.; Arsene, I. C.; Averbeck, R.; Braun-Munzinger, P.; Donigus, B.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Knichel, M. L.; Koehler, M. K.; Krzewicki, M.; Lenhardt, M.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Otwinowski, J.; Park, W. J.; Romita, R.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, Darmstadt, Germany. [Anticic, T.; Planinic, M.; Poljak, N.; Simatovic, G.; Susa, T.] Rudjer Boskovic Inst, Zagreb, Croatia. [Budnikov, D.; Filchagin, S.; Ilkaev, R.; Kuryakin, A.; Mamonov, A.; Nazarenko, S.; Punin, V.; Tumkin, A.; Vinogradov, Y.; Vyushin, A.; Zaviyalov, N.] Russian Fed Nucl Ctr VNIIEF, Sarov, Russia. 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Martinez; Martin Blanco, J.; Mas, A.; Massacrier, L.; Pillot, P.; Schutz, Y.; Shabetai, A.; Stocco, D.] Univ Nantes, CNRS, IN2P3, Ecole Mines Nantes,SUBATECH, Nantes, France. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Knospe, A. G.; Markert, C.] Univ Texas, Phys Dept, Austin, TX USA. [Gomez, R.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Prado, C. Alves Garcia; Deppman, A.; de Barros, G. O. V.; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Moreira De Godoy, D. A.; Munhoz, M. G.; Oliveira Da Silva, A. C.; Pereira De Oliveira Filho, E.; Suaide, A. A. P.; Szanto de Toledo, A.] Univ Sao Paulo, Sao Paulo, Brazil. [Dash, A.; Takahashi, J.] Univ Estadual Campinas UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Blanco, F.; Chinellato, D. D.; Jayarathna, P. H. S. Y.; Jena, S.; Pinsky, L.; Piyarathna, D. B.; Pluta, J.; Timmins, A. R.; Weber, M.] Univ Houston, Houston, TX USA. [Aysto, J.; Chang, B.; Kalliokoski, T.; Kim, D. J.; Kral, J.; Loo, K. K.; Morreale, A.; Rak, J.; Trzaska, W. H.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Martashvili, I.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.] Univ Tennessee, Knoxville, TN USA. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Hori, Y.; Torii, H.; Tsuji, T.; Yamaguchi, Y.] Univ Tokyo, Tokyo, Japan. [Masoodi, A. Ahmad; Bhom, J.; Chujo, T.; Esumi, S.; Inaba, M.; Miake, Y.; Sakata, D.; Sano, M.; Watanabe, D.; Watanabe, K.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. Y.; Guilbaud, M.; Tieulent, R.; Uras, A.; Zoccarato, Y.] Univ Lyon 1, Univ Lyon, IPN Lyon, CNRS IN2P3, Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Vorobyev, I.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg, Russia. [Ahammed, Z.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; De, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata, India. [Langoy, R.; Lien, J.] Vestfold Univ Coll, Tonsberg, Norway. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pawlak, T.; Peryt, W.; Szymanski, M.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Borissov, A.; Cormier, T. M.; Dobrin, A.; Loggins, V. R.; Mlynarz, J.; Prasad, S. K.; Pruneau, C. A.; Putschke, J.; Voloshin, S.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Agocs, A. G.; Barnafoldi, G. 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RI Mitu, Ciprian/E-6733-2011; Sevcenco, Adrian/C-1832-2012; Ahmed, Ijaz/E-9144-2015; Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014; Bregant, Marco/I-7663-2012; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Altsybeev, Igor/K-6687-2013; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Takahashi, Jun/B-2946-2012; Kovalenko, Vladimir/C-5709-2013; Barnby, Lee/G-2135-2010; Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Rui, Rinaldo/L-1926-2015; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Zarochentsev, Andrey/J-6253-2013; Graczykowski, Lukasz/O-7522-2015; Janik, Malgorzata/O-7520-2015; feofilov, grigory/A-2549-2013; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008 OI Sevcenco, Adrian/0000-0002-4151-1056; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Altsybeev, Igor/0000-0002-8079-7026; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; Takahashi, Jun/0000-0002-4091-1779; Kovalenko, Vladimir/0000-0001-6012-6615; Barnby, Lee/0000-0001-7357-9904; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; van Leeuwen, Marco/0000-0002-5222-4888; Murray, Sean/0000-0003-0548-588X; Masera, Massimo/0000-0003-1880-5467; Gaardhoje, Jens-Jorgen/0000-0001-6122-4698; Fernandez Tellez, Arturo/0000-0001-5092-9748; Zhou, You/0000-0002-7868-6706; Guerzoni, Barbara/0000-0003-3187-7051; Beole', Stefania/0000-0003-4673-8038; Fiore, Enrichetta Maria/0000-0002-3548-2690; Di Bari, Domenico/0000-0002-5559-8906; Feliciello, Alessandro/0000-0001-5823-9733; Martynov, Yevgen/0000-0003-0753-2205; Read, Kenneth/0000-0002-3358-7667; Monteno, Marco/0000-0002-3521-6333; Bhasin, Anju/0000-0002-3687-8179; SANTORO, ROMUALDO/0000-0002-4360-4600; Scarlassara, Fernando/0000-0002-4663-8216; Rui, Rinaldo/0000-0002-6993-0332; Virgili, Tiziano/0000-0003-0471-7052; Christiansen, Peter/0000-0001-7066-3473; Scomparin, Enrico/0000-0001-9015-9610; Gago Medina, Alberto Martin/0000-0002-0019-9692; Riggi, Francesco/0000-0002-0030-8377; Lemmon, Roy/0000-0002-1259-979X; Dainese, Andrea/0000-0002-2166-1874; Paticchio, Vincenzo/0000-0002-2916-1671; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Turrisi, Rosario/0000-0002-5272-337X; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Zarochentsev, Andrey/0000-0002-3502-8084; Janik, Malgorzata/0000-0002-3356-3438; feofilov, grigory/0000-0003-3700-8623; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748 FU State Committee of Science; World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); the Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; the Carlsberg Foundation; Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; 'Region Pays de Loire'; 'Region Alsace'; 'Region Auvergne'; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology; Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science; Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi- Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC; EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research-NASR; (Autoritatea Nationala pentru Cercetare Stiintifica-ANCS); Ministry of Education and Science of Russian Federation; Russian Academy of ScienceS; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN, Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC);; The United States Department of Energy; the United States National Science Foundation; the State of Texas; the State of Ohio FX The ALICE collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector:; State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia;; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP);; National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC);; Ministry of Education and Youth of the Czech Republic;; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation;; The European Research Council under the European Community's Seventh Framework Programme;; Helsinki Institute of Physics and the Academy of Finland;; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France;; German BMBF and the Helmholtz Association;; General Secretariat for Research and Technology, Ministry of Development, Greece;; Hungarian OTKA and National Office for Research and Technology (NKTH);; Department of Atomic Energy and Department of Science and Technology of the Government of India;; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi",Italy;; MEXT Grant-in-Aid for Specially Promoted Research, Japan;; Joint Institute for Nuclear Research, Dubna;; National Research Foundation of Korea (NRF);; CONACYT, DGAPA, Mexico, ALFA-EC and the EPLANET Progam (European Particle Physics Latin American Network);; Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands;; Research Council of Norway (NFR);; Polish Ministry of Science and Higher Education;; National Authority for Scientific Research-NASR (Autoritatea Nationala pentru Cercetare Stiintifica-ANCS);; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research;; Ministry of Education of Slovakia;; Department of Science and Technology, South Africa;; CIEMAT, EELA, Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency);; Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW);; Ukraine Ministry of Education and Science;; United Kingdom Science and Technology Facilities Council (STFC);; The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 19 TC 33 Z9 33 U1 0 U2 49 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD DEC 6 PY 2013 VL 73 IS 12 AR 2662 DI 10.1140/epjc/s10052-013-2662-9 PG 12 WC Physics, Particles & Fields SC Physics GA 264RH UT WOS:000327897500002 ER PT J AU Cheng, XL Hiras, J Deng, K Bowen, B Simmons, BA Adams, PD Singer, SW Northen, TR AF Cheng, Xiaoliang Hiras, Jennifer Deng, Kai Bowen, Benjamin Simmons, Blake A. Adams, Paul D. Singer, Steven W. Northen, Trent R. TI High throughput nanostructure-initiator mass spectrometry screening of microbial growth conditions for maximal beta-glucosidase production SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE NIMS; high throughput; beta-glucosidase; enzymatic activity screening; microbial communities ID CONTINUOUS FLUOROMETRIC-DETERMINATION; WAVELENGTH FLUORESCENT SUBSTRATE; GLYCOSIDE HYDROLASE ACTIVITIES; ENZYME-ACTIVITY ASSAY; PLANT BIOMASS; BISPORA; INHIBITION; HYDROLYSIS; FUELS; NIMS AB Production of biofuels via enzymatic hydrolysis of complex plant polysaccharides is a subject of intense global interest. Microbial communities are known to express a wide range of enzymes necessary for the saccharification of lignocellulosic feedstocks and serve as a powerful reservoir for enzyme discovery. However, the growth temperature and conditions that yield high cellulase activity vary widely, and the throughput to identify optimal conditions has been limited by the slow handling and conventional analysis. A rapid method that uses small volumes of isolate culture to resolve specific enzyme activity is needed. In this work, a high throughput nanostructure-initiator mass spectrometry (NIMS)based approach was developed for screening a thermophilic cellulolytic actinomycete, Thermobispora bispora, for beta-glucosidase production under various growth conditions. Media that produced high beta-glucosidase activity were found to be I/S + glucose or microcrystalline cellulose (MCC), Medium 84 + rolled oats, and M9TE + MCC at 45 degrees C. Supernatants of cell cultures grown in M9TE + 1% MCC cleaved 2.5 times more substrate at 45 degrees C than at all other temperatures. While T bispora is reported to grow optimally at 60 degrees C in Medium 84 + rolled oats and M9TE + 1% MCC, approximately 40% more conversion was observed at 45 degrees C. This high throughput NIMS approach may provide an important tool in discovery and characterization of enzymes from environmental microbes for industrial and biofuel applications. C1 [Cheng, Xiaoliang; Deng, Kai; Adams, Paul D.; Northen, Trent R.] Joint BioEnergy Inst, Div Technol, Emeryville, CA USA. [Cheng, Xiaoliang; Bowen, Benjamin; Northen, Trent R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Dept Bioenergy GTL & Struct Biol, Berkeley, CA 94720 USA. [Hiras, Jennifer; Simmons, Blake A.; Singer, Steven W.] Joint BioEnergy Inst, Deconstruct Div, Emeryville, CA USA. [Hiras, Jennifer; Adams, Paul D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Deng, Kai; Simmons, Blake A.] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA USA. [Singer, Steven W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Geochem, Berkeley, CA 94720 USA. [Singer, Steven W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Ecol, Berkeley, CA 94720 USA. RP Northen, TR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Dept Bioenergy GTL & Struct Biol, Berkeley, CA 94720 USA. EM trnorthen@lbl.gov RI Adams, Paul/A-1977-2013 OI Adams, Paul/0000-0001-9333-8219 FU US Department of Energy; Office of Science, Office of Biological and Environmental Research [DE-AC02-050411231] FX This work was performed as part of the DOE Joint BioEnergy Institute (hrttp://www.jbei.org) supported by the US Department of Energy. Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-050411231 between Lawrence Berkeley National Laboratory and the US Department of Energy. NR 31 TC 6 Z9 6 U1 1 U2 41 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD DEC 6 PY 2013 VL 4 AR 365 DI 10.3389/fmicb.2013.00365 PG 7 WC Microbiology SC Microbiology GA AB1II UT WOS:000331544300001 PM 24367356 ER PT J AU Peden, EA Boehm, M Mulder, DW Davis, R Old, WM King, PW Ghirardi, ML Dubini, A AF Peden, Erin A. Boehm, Marko Mulder, David W. Davis, ReAnna Old, William M. King, Paul W. Ghirardi, Maria L. Dubini, Alexandra TI Identification of Global Ferredoxin Interaction Networks in Chlamydomonas reinhardtii SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Bioenergetics; Electron Transfer Complex; Chlamydomonas; Energy Metabolism; Protein-Protein Interactions; Redox; Ferredoxin; Network ID AMINO-ACID SEQUENCE; GREEN-ALGA; STATE TRANSITIONS; ELECTRON-TRANSFER; ESCHERICHIA-COLI; REDOX REGULATION; PHOTOSYSTEM-II; FATTY-ACIDS; IN-VITRO; DESATURATION AB Background:Chlamydomonas contains six chloroplast ferredoxins (FDXs) whose function is still unclear. Results: A global FDX interactome was obtained where FDX1 has a predominant role and is the most relevant electron donor to FNR1 and HYDA1. Conclusion: FDXs have distinct but also overlapping function. Significance: We discovered new FDX interaction partners and specific roles for each FDX isoform. Ferredoxins (FDXs) can distribute electrons originating from photosynthetic water oxidation, fermentation, and other reductant-generating pathways to specific redox enzymes in different organisms. The six FDXs identified in Chlamydomonas reinhardtii are not fully characterized in terms of their biological function. In this report, we present data from the following: (a) yeast two-hybrid screens, identifying interaction partners for each Chlamydomonas FDX; (b) pairwise yeast two-hybrid assays measuring FDX interactions with proteins from selected biochemical pathways; (c) affinity pulldown assays that, in some cases, confirm and even expand the interaction network for FDX1 and FDX2; and (d) in vitro NADP(+) reduction and H-2 photo-production assays mediated by each FDX that verify their role in these two pathways. Our results demonstrate new potential roles for FDX1 in redox metabolism and carbohydrate and fatty acid biosynthesis, for FDX2 in anaerobic metabolism, and possibly in state transition. Our data also suggest that FDX3 is involved in nitrogen assimilation, FDX4 in glycolysis and response to reactive oxygen species, and FDX5 in hydrogenase maturation. Finally, we provide experimental evidence that FDX1 serves as the primary electron donor to two important biological pathways, NADPH and H-2 photo-production, whereas FDX2 is capable of driving these reactions at less than half the rate observed for FDX1. C1 [Peden, Erin A.; Boehm, Marko; Mulder, David W.; Davis, ReAnna; King, Paul W.; Ghirardi, Maria L.; Dubini, Alexandra] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Old, William M.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. RP Dubini, A (reprint author), Natl Renewable Energy Lab, Mail Stop 3313,15013 Denver West Pkwy, Golden, CO 80401 USA. EM alexandra.dubini@nrel.gov RI King, Paul/D-9979-2011; dubini, alexandra /A-7252-2016; OI King, Paul/0000-0001-5039-654X; dubini, alexandra /0000-0001-8825-3915; OLD, WILLIAM/0000-0002-9499-8478 FU United States Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; Biological and Environmental Research program, Division of Energy Biosciences, Office of Science; United States Department of Energy; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the United States Department of Energy FX This work was supported by the United States Department of Energy under Contract DE-AC36-08GO28308 from the National Renewable Energy Laboratory, a grant from the Biological and Environmental Research program, Division of Energy Biosciences, Office of Science, the United States Department of Energy (to M. L G.), and the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the United States Department of Energy (to P. W. K.). NR 69 TC 19 Z9 19 U1 1 U2 31 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD DEC 6 PY 2013 VL 288 IS 49 BP 35192 EP 35209 DI 10.1074/jbc.M113.483727 PG 18 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 291YA UT WOS:000329867600020 PM 24100040 ER PT J AU Kopaskie, KS Ligtenberg, KG Schneewind, O AF Kopaskie, Karyl S. Ligtenberg, Katherine Given Schneewind, Olaf TI Translational Regulation of Yersinia enterocolitica mRNA Encoding a Type Ill Secretion Substrate SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Bacterial Pathogenesis; mRNA; Ribosomes; Secretion; Translation Regulation ID III PROTEIN SECRETION; TARGET-CELL CONTACT; YOP PROTEINS; HELA-CELLS; POSTTRANSCRIPTIONAL MECHANISM; EUKARYOTIC CELLS; TIP COMPLEX; CHAPERONE; PSEUDOTUBERCULOSIS; EXPRESSION AB Background:Yersinia enterocolitica yopD, lcrH, and yscM1 control the expression of yopQ encoding a secretion substrate. Results: YopD associates with 30 S ribosomal particles, and YopD, LcrH, and YscM1 block yopQ mRNA translation. Conclusion: In response to environmental signals, Yersinia prevent yopQ expression by blocking the translation of its transcripts. Significance: These results demonstrate translational regulation for the Yersinia type III secretion pathway. Yersinia enterocolitica type III secretion machines transport YopQ and other Yop effectors into host immune cells. YopD and its chaperone LcrH are essential components of the Yersinia type III pathway, enabling effector translocation into host cells. YopD, LcrH, and YscM1 also regulate yop expression post-transcriptionally in response to environmental signals; however, the molecular mechanisms for this regulation and Yop secretion are unknown. We show here that YopD associates with 30 S ribosomal particles in a manner requiring LcrH. When added to ribosomes, YopD, LcrH, and YscM1 block the translation of yopQ mRNA. We propose a model whereby LcrH-dependent association of YopD with 30 S ribosomal particles enables YscM1 to block yopQ translation unless type III machines are induced to secrete the effector. C1 Argonne Natl Lab, Howard Taylor Ricketts Lab, Argonne, IL 60439 USA. [Schneewind, Olaf] Univ Chicago, Dept Microbiol, Chicago, IL 60637 USA. RP Schneewind, O (reprint author), Univ Chicago, Dept Microbiol, 920 E 58th St, Chicago, IL 60637 USA. EM oschnee@bsd.uchicago.edu FU NICHD, National Institutes of Health; Region V "Great Lakes" Regional Center of Excellence in Biodefense and Emerging Infectious Diseases Consortium (National Institutes of Health) [1-U54-AI-057153] FX We thank Antoni P.A. Hendrickx for training in transmission electron microscopy and members of our laboratory for discussion and critical comments on the manuscript The S3 monoclonal antibody developed by L. Kahan was obtained from the Developmental Studies Hybridoma Bank developed under the auspices of the NICHD, National Institutes of Health, and maintained by The University of Iowa, Department of Biology, Iowa City, IA 52242. O. S. acknowledges membership within and support from the Region V "Great Lakes" Regional Center of Excellence in Biodefense and Emerging Infectious Diseases Consortium (National Institutes of Health Award 1-U54-AI-057153). NR 66 TC 8 Z9 8 U1 0 U2 0 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD DEC 6 PY 2013 VL 288 IS 49 BP 35478 EP 35488 DI 10.1074/jbc.M113.504811 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 291YA UT WOS:000329867600043 PM 24158443 ER PT J AU Gluzman, S Karpeev, DA Berlyand, LV AF Gluzman, Simon Karpeev, Dmitry A. Berlyand, Leonid V. TI Effective viscosity of puller-like microswimmers: a renormalization approach SO JOURNAL OF THE ROYAL SOCIETY INTERFACE LA English DT Article DE pullers; effective viscosity; active and passive suspensions ID RANDOM CLOSE PACKING; SPHERICAL-PARTICLES; BULK STRESS; SUSPENSION; SPHERES; DISPERSIONS; MODEL; MOTION; FLUID AB Effective viscosity (EV) of suspensions of puller-like microswimmers (pullers), for example Chlamydamonas algae, is difficult to measure or simulate for all swimmer concentrations. Although there are good reasons to expect that the EV of pullers is similar to that of passive suspensions, analytical determination of the passive EV for all concentrations remains unsatisfactory. At the same time, the EV of bacterial suspensions is closely linked to collective motion in these systems and is biologically significant. We develop an approach for determining analytical EV estimates at all concentrations for suspensions of pullers as well as for passive suspensions. The proposed methods are based on the ideas of renormalization group (RG) theory and construct the EV formula based on the known asymptotics for small concentrations and near the critical point (i.e. approaching dense packing). For passive suspensions, the method is verified by comparison against known theoretical results. We find that the method performs much better than an earlier RG-based technique. For pullers, the validation is done by comparing them to experiments conducted on Chlamydamonas suspensions. C1 [Gluzman, Simon; Berlyand, Leonid V.] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Karpeev, Dmitry A.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Gluzman, S (reprint author), Penn State Univ, Dept Math, University Pk, PA 16802 USA. EM simon.gluzman@gmail.com FU NIH/NIGMS [1R01GM104978-01] FX The work of all three authors was supported by NIH/NIGMS R01 grant no. 1R01GM104978-01. The authors express their gratitude to I. Aronson for his explanations of puller experiments, to P. Peyla for useful discussions and to S. Ryan for multiple useful suggestions. NR 36 TC 5 Z9 5 U1 1 U2 9 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1742-5689 EI 1742-5662 J9 J R SOC INTERFACE JI J. R. Soc. Interface PD DEC 6 PY 2013 VL 10 IS 89 AR 20130720 DI 10.1098/rsif.2013.0720 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 298CU UT WOS:000330302400008 PM 24068178 ER PT J AU Abelev, B Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, Z Ahmad, N Masoodi, AA Ahmed, I Ahn, SA Ahn, SU Aimo, I Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alexandre, D Alici, A Alkin, A Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Andrei, C Andronic, A Anguelov, V Anielski, J Anson, C Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Arend, A Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Asryan, A Augustinus, A Averbeck, R Awes, TC Aysto, J Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, PC Baumann, C Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bergognon, AAE Bertens, RA Berzano, D Betev, L Bhasin, A Bhati, AK Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Bjelogrlic, S Blanco, F Blanco, F Blau, D Blume, C Boccioli, M Bock, F Bottger, S Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bossu, F Botje, M Botta, E Braidot, E Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brun, R Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Caffarri, D Cai, X Caines, H Caliva, A Villar, EC Camerini, P Roman, VC Romeo, GC Carena, F Carena, W Carlin, N Carminati, F Diaz, AC Castellanos, JC Hernandez, JFC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JL Chattopadhyay, S Chattopadhyay, S Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Chochula, P Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Balbastre, GC del Valle, ZC Connors, ME Contin, G Contreras, JG Cormier, TM Morales, YC Cortese, P Maldonado, IC Cosentino, MR Costa, F Cotallo, ME Crescio, E Crochet, P Alaniz, EC Albino, RC Cuautle, E Cunqueiro, L Czopowicz, TR Dainese, A Dang, R Danu, A Das, D Das, I Das, S Das, K Dash, A Dash, S De, S de Barros, GOV De Caro, A de Cataldo, G De Cuveland, J De Falco, A De Gruttola, D Delagrange, H Deloff, A De Marco, N Denes, E De Pasquale, S Deppman, A D'Erasmo, G de Rooij, R Corchero, MAD Di Bari, D Dietel, T Di Giglio, C Di Liberto, S Di Mauro, A Di Nezza, P Divia, R Djuvsland, O Dobrin, A Dobrowolski, T Donigus, B Dordic, O Dubey, AK Dubla, A Ducroux, L Dupieux, P Majumdar, AKD Elia, D Elwood, BG Emschermann, D Engel, H Erazmus, B Erdal, HA Eschweiler, D Espagnon, B Estienne, M Esumi, S Evans, D Evdokimov, S Eyyubova, G Fabris, D Faivre, J Falchieri, D Fantoni, A Fasel, M Fehlker, D Feldkamp, L Felea, D Feliciello, A Fenton-Olsen, B Feofilov, G Telez, AF Ferretti, A Festanti, A Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Floratos, E Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Girard, MF Gaardhoje, JJ Gagliardi, M Gago, A Gallio, M Gangadharan, DR Ganoti, P Garabatos, C Garcia-Solis, E Gargiulo, C Garishvili, I Gerhard, J Germain, M Gheata, A Gheata, M Ghidini, B Ghosh, P Gianotti, P Giubellino, P Gladysz-Dziadus, E Glassel, P Goerlich, L Gomez, R Ferreiro, EG Gonzalez-Zamora, P Gorbunov, S Goswami, A Gotovac, S Graczykowski, LK Grajcarek, R Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Gros, P Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Guilbaud, M Gulbrandsen, K Gulkanyan, H Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Han, BH Hanratty, LD Hansen, A Harris, JW Harton, A Hatzifotiadou, D Hayashi, S Hayrapetyan, A Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Herrmann, N Hess, BA Hetland, KF Hicks, B Hippolyte, B Hori, Y Hristov, P Hrivnacova, I Huang, M Humanic, TJ Hwang, DS Ichou, R Ilkaev, R Ilkiv, I Inaba, M Incani, E Innocenti, PG Innocenti, GM Ionita, C Ippolitov, M Irfan, M Ivanov, V Ivanov, M Ivanov, A Ivanytskyi, O Jacholkowski, A Jacobs, PM Jahnke, C Jang, HJ Janik, MA Jayarathna, PHSY Jena, S Jha, DM Bustamante, RTJ Jones, PG Jung, H Jusko, A Kaidalov, AB Kalcher, S Kalina, P Kalliokoski, T Kalweit, A Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karpechev, E Kazantsev, A Kebschull, U Keidel, R Ketzer, B Khan, MM Khan, P Khan, KH Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, JS Kim, B Kim, T Kim, DJ Kim, S Kim, M Kim, DW Kim, JH 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P Lunardon, M Luo, J Luparello, G Luzzi, C Ma, R Ma, K Madagodahettige-Don, DM Maevskaya, A Mager, M Mahapatra, DP Maire, A Malaev, M Cervantes, IM Malinina, L Mal'Kevich, D Malzacher, P Mamonov, A Manceau, L Mangotra, L Manko, V Manso, F Manzari, V Marchisone, M Mares, J Margagliotti, GV Margotti, A Marin, A Markert, C Marquard, M Martashvili, I Martin, NA Blanco, JM Martinengo, P Martinez, MI Garcia, Gi Martynov, Y Mas, A Masciocchi, S Masera, M Masoni, A Massacrier, L Mastroserio, A Matyja, A Mayer, C Mazer, J Mazumder, R Mazzoni, MA Meddi, F Menchaca-Rocha, A Perez, JM Meres, M Miake, Y Mikhaylov, K Milano, L Milosevic, J Mischke, A Mishra, AN Miskowiec, D Mitu, C Mlynarz, J Mohanty, B Molnar, L Zetina, LM Monteno, M Montes, E Moon, T Morando, M De Godoy, DAM Moretto, S Morreale, A Morsch, A Muccifora, V Mudnic, E Muhuri, S Mukherjee, M Muller, H Munhoz, MG Murray, S Musa, L Musinsky, J Nandi, BK Nania, R Nappi, E Nasar, M Nattrass, C Nayak, TK Nazarenko, S Nedosekin, A Nicassio, M 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CA ALICE Collaboration TI Directed Flow of Charged Particles at Midrapidity Relative to the Spectator Plane in Pb-Pb Collisions at root s(NN)=2.76TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; ELLIPTIC FLOW; AU+AU COLLISIONS; COLLECTIVE FLOW; DEPENDENCE; ANISOTROPY; LHC; TEV AB The directed flow of charged particles at midrapidity is measured in Pb-Pb collisions at root s(NN) p 2: 76 TeV relative to the collision symmetry plane defined by the spectator nucleons. A negative slope of the rapidity-odd directed flow component with approximately 3 times smaller magnitude than found at the highest RHIC energy is observed. This suggests a smaller longitudinal tilt of the initial system and disfavors the strong fireball rotation predicted for the LHC energies. The rapidity-even directed flow component is measured for the first time with spectators and found to be independent of pseudorapidity with a sign change at transverse momenta p(T) between 1.2 and 1: 7 GeV/c. Combined with the observation of a vanishing rapidity-even p(T) shift along the spectator deflection this is strong evidence for dipolelike initial density fluctuations in the overlap zone of the nuclei. Similar trends in the rapidity-even directed flow and the estimate from two-particle correlations at midrapidity, which is larger by about a factor of 40, indicate a weak correlation between fluctuating participant and spectator symmetry planes. These observations open new possibilities for investigation of the initial conditions in heavy-ion collisions with spectator nucleons. C1 [Abelev, B.; Garishvili, I.; Soltz, R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. 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V.; Piano, S.; Rachevski, A.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Gomez, R.; Monzon, I. Leon; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Goswami, A.; Mishra, A. N.; Raniwala, S.; Raniwala, R.] Univ Rajasthan, Dept Phys, Jaipur 302004, Rajasthan, India. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Grigoryan, A.; Gulkanyan, H.; Hayrapetyan, A.; Papikyan, V.] AI Alikhanyan Natl Sci Lab Yerevan Phys Inst Fdn, Yerevan, Armenia. [Agostinelli, A.; Gunji, T.; Hamagaki, H.; Hayashi, S.; Hori, Y.; Ozawa, K.; Torii, H.; Tsuji, T.; Yamaguchi, Y.] Univ Tokyo, Tokyo, Japan. [Han, B. H.; Hwang, D. S.; Kim, S.; Kim, J. H.] Sejong Univ, Dept Phys, Seoul, South Korea. [Hess, B. A.; Schmidt, H. R.; Wiechula, J.] Univ Tubingen, Tubingen, Germany. [Uysal, A. Karasu] KTO Karatay Univ, Konya, Turkey. [Keidel, R.] Fachhsch Worms, ZTT, Worms, Germany. Tech Univ Munich, D-80290 Munich, Germany. [Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Knospe, A. G.; Markert, C.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Langoy, R.; Lien, J.] Vestfold Univ Coll, Tonsberg, Norway. [Lemmon, R. C.; Romita, R.] STFC Daresbury Lab, Nucl Phys Grp, Daresbury, England. [Mager, M.; Oeschler, H.] Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Mares, J.; Polak, K.; Zavada, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Martashvili, I.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.] Univ Tennessee, Knoxville, TN USA. [Mazumder, R.; Mishra, A. N.; Sahoo, R.] Indian Inst Technol Indore, Indore, Madhya Pradesh, India. [Meddi, F.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Meddi, F.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Milosevic, J.] Univ Belgrade, Fac Phys & Vinca, Inst Nucl Sci, Belgrade, Serbia. [Mohanty, B.; Singha, S.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Nasar, M.] ASRT, Cairo, Egypt. [Pestov, Y.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Redlich, K.] Univ Wroclaw, Inst Theoret Phys, PL-50138 Wroclaw, Poland. [Ricci, R. A.; Vannucci, L.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Sakaguchi, H.; Shigaki, K.; Sugitate, T.; Yano, S.] Hiroshima Univ, Hiroshima, Japan. [Vernet, R.] IN2P3, Ctr Calcul, Villeurbanne, France. RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Vajzer, Michal/G-8469-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Takahashi, Jun/B-2946-2012; Barnby, Lee/G-2135-2010; Kovalenko, Vladimir/C-5709-2013; Guber, Fedor/I-4271-2013; Castillo Castellanos, Javier/G-8915-2013; Bregant, Marco/I-7663-2012; Wagner, Vladimir/G-5650-2014; Sevcenco, Adrian/C-1832-2012; Kucera, Vit/G-8459-2014; Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Ahmed, Ijaz/E-9144-2015; Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Kompaniets, Mikhail/F-5025-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Zarochentsev, Andrey/J-6253-2013; Janik, Malgorzata/O-7520-2015; Graczykowski, Lukasz/O-7522-2015; feofilov, grigory/A-2549-2013; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; OI Takahashi, Jun/0000-0002-4091-1779; Barnby, Lee/0000-0001-7357-9904; Kovalenko, Vladimir/0000-0001-6012-6615; Guber, Fedor/0000-0001-8790-3218; Castillo Castellanos, Javier/0000-0002-5187-2779; Sevcenco, Adrian/0000-0002-4151-1056; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Kompaniets, Mikhail/0000-0001-8831-0553; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Zarochentsev, Andrey/0000-0002-3502-8084; Janik, Malgorzata/0000-0002-3356-3438; feofilov, grigory/0000-0003-3700-8623; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Gago Medina, Alberto Martin/0000-0002-0019-9692; Dainese, Andrea/0000-0002-2166-1874; Paticchio, Vincenzo/0000-0002-2916-1671; Monteno, Marco/0000-0002-3521-6333; Bhasin, Anju/0000-0002-3687-8179; SANTORO, ROMUALDO/0000-0002-4360-4600; Scarlassara, Fernando/0000-0002-4663-8216; Turrisi, Rosario/0000-0002-5272-337X; D'Erasmo, Ginevra/0000-0003-3407-6962; Beole', Stefania/0000-0003-4673-8038 FU State Committee of Science, World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia,; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao, a o de Amparo a Pesquisa do Estado de Sa o Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi-Museo Storico della Fisica e Centro Studie Ricerche ``Enrico Fermi,'' Italy; Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico; ALFA-ECEPLANET Program (European Particle Physics Latin American Network) FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao, a o de Amparo a Pesquisa do Estado de Sa o Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE), and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the ``Region Pays de Loire,'' ``Region Alsace,'' ``Region Auvergne,'' and CEA, France; German BMBF and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studie Ricerche ``Enrico Fermi,'' Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC, and the EPLANET Program (European Particle Physics Latin American Network) Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific ResearchNASR (Autoritatea Nationala pentru Cercetare Stiintifica-ANCS); Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations, and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); USA Department of Energy, USA National Science Foundation, the State of Texas, and the State of Ohio. NR 52 TC 22 Z9 22 U1 1 U2 82 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 6 PY 2013 VL 111 IS 23 AR 232302 DI 10.1103/PhysRevLett.111.232302 PG 11 WC Physics, Multidisciplinary SC Physics GA 274PK UT WOS:000328618300006 PM 24476260 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, 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CA CMS Collaboration TI Measurement of the cross section and angular correlations for associated production of a Z boson with b hadrons in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID ATLAS DETECTOR; LHC AB A study of proton-proton collisions in which two b hadrons are produced in association with a Z boson is reported. The collisions were recorded at a centre-of-mass energy of 7 TeVwith the CMS detector at the LHC, for an integrated luminosity of 5.2 fb(-1). The b hadrons are identified by means of displaced secondary vertices, without the use of reconstructed jets, permitting the study of b-hadron pair production at small angular separation. Differential cross sections are presented as a function of the angular separation of the b hadrons and the Z boson. In addition, inclusive measurements are presented. 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[Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Radics, B.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.; Majumder, D.] Tata Inst Fundamental Res EHEP, Mumbai, Maharashtra, India. [Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Tabarelli de Fatis, T.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; Tabarelli de Fatis, T.] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; De Cosa, A.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Fantinel, S.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Ortona, G.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; David, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Gomez-Reino Garrido, R.; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Palencia Cortezon, E.; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. 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[Amsler, C.; Chiochia, V.; Favaro, C.; Ivova Rikova, M.; Kilminster, B.; Millan Mejias, B.; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Buchmann, M. A.; Bainbridge, R.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Calderon De La Barca Sanchez, M.; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Hanson, G.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Williams, G.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. 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[Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Basso, L.; Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Ragazzi, Stefano/D-2463-2009; Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Petrushanko, Sergey/D-6880-2012; da Cruz e Silva, Cristovao/K-7229-2013; Dudko, Lev/D-7127-2012; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Bellan, Riccardo/G-2139-2014; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Janssen, Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Bartalini, Paolo/E-2512-2014; Ligabue, Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; OI Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Ragazzi, Stefano/0000-0001-8219-2074; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Dudko, Lev/0000-0002-4462-3192; de Jesus Damiao, Dilson/0000-0002-3769-1680; Montanari, Alessandro/0000-0003-2748-6373; Novaes, Sergio/0000-0003-0471-8549; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Heath, Helen/0000-0001-6576-9740; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235 FU Austrian Federal Ministry of Science and Research; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education, Youth and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Science and Innovation, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Science and Technological Development of Serbia; Secretaria de Estado de Investigacion; Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education, Youth and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Science and Innovation, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, co-financed by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 35 TC 3 Z9 3 U1 3 U2 97 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD DEC 6 PY 2013 IS 12 AR 039 DI 10.1007/JHEP12(2013)039 PG 38 WC Physics, Particles & Fields SC Physics GA 270WJ UT WOS:000328349600001 ER PT J AU Ren, J AF Ren, Jie TI Predicted rectification and negative differential spin Seebeck effect at magnetic interfaces SO PHYSICAL REVIEW B LA English DT Article ID FERROMAGNET; INSULATOR AB We study the nonequilibrium Seebeck spin transport acrossmetal-magnetic insulator interfaces. The conjugate-converted thermal-spin transport is assisted by the exchange interaction at the interface, between conduction electrons in the metal lead and localized spins in the insulating magnet lead. We predict the rectification and negative differential spin Seebeck effect and resolve their microscopic mechanism, as a consequence of the strongly fluctuated electronic density of states in the metal lead. The rectification of spin Peltier effect is also discussed. The phenomena predicted here are relevant for designing efficient spin/magnon diode and transistor, which could play crucial roles in controlling energy and information in functional devices. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ren, J (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM renjie@lanl.gov RI Ren, Jie/G-5314-2010 OI Ren, Jie/0000-0003-2806-7226 FU National Nuclear Security Administration of the US DOE at LANL through the LDRD Program [DE-AC52-06NA25396] FX J.R. acknowledges the support from National Nuclear Security Administration of the US DOE at LANL under Contract No. DE-AC52-06NA25396 through the LDRD Program. NR 39 TC 20 Z9 20 U1 3 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 6 PY 2013 VL 88 IS 22 AR 220406 DI 10.1103/PhysRevB.88.220406 PG 5 WC Physics, Condensed Matter SC Physics GA 274AU UT WOS:000328578200001 ER PT J AU Consolati, G Franco, D Hans, S Jollet, C Meregaglia, A Perasso, S Tonazzo, A Yeh, M AF Consolati, G. Franco, D. Hans, S. Jollet, C. Meregaglia, A. Perasso, S. Tonazzo, A. Yeh, M. TI Characterization of positronium properties in doped liquid scintillators SO PHYSICAL REVIEW C LA English DT Article AB Orthopositronium (o-Ps) formation and decay can replace the annihilation process, when a positron interacts in liquid scintillator media. The delay induced by the positronium decay represents either a potential signature for antineutrino detection, via inverse beta decay, or to identify and suppress positron background, as recently demonstrated by the Borexino experiment. The formation probability and decay time of o-Ps depend strongly on the surrounding material. In this paper, we characterize the o-Ps properties in liquid scintillators as function of concentrations of gadolinium, lithium, neodymium, and tellurium dopers used by present and future neutrino experiments. In particular, gadolinium and lithium are high neutron cross section isotopes, widely used in reactor antineutrino experiments, while neodymium and tellurium are double beta decay emitters, employed to investigates the Majorana neutrino nature. Future neutrino experiments may profit from the performed measurements to tune the preparation of the scintillator in order to maximize the o-Ps signature, and therefore the discrimination power. C1 [Consolati, G.] Politecn Milan, Dept Aerosp Sci & Technol, I-20156 Milan, Italy. [Franco, D.; Perasso, S.; Tonazzo, A.] Univ Paris Diderot, CNRS, IN2P3,Sorbonne Paris Cite, APC,AstroParticule & Cosmol,CEA,Irfu,Observ Paris, F-75205 Paris 13, France. [Hans, S.; Yeh, M.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Jollet, C.; Meregaglia, A.] Univ Strasbourg, IPHC, CNRS, IN2P3, F-67037 Strasbourg, France. RP Consolati, G (reprint author), Politecn Milan, Dept Aerosp Sci & Technol, Via La Masa 34, I-20156 Milan, Italy. RI Consolati, Giovanni/C-5680-2013; OI Consolati, Giovanni/0000-0003-3614-245X; Franco, Davide/0000-0001-5604-2531 FU ANR NuToPs project [2011-JS04-009-01]; UnivEarthS Labex program of Sorbonne Paris Cite [ANR-10-LABX-0023, ANR-11-IDEX-0005-02]; US Department of Energy [DE-AC02-98CH10886] FX We acknowledge the financial support from the ANR NuToPs project (Grant No. 2011-JS04-009-01) and from the UnivEarthS Labex program of Sorbonne Paris Cite (nos. ANR-10-LABX-0023 and ANR-11-IDEX-0005-02). The work conducted at Brookhaven National Laboratory was supported by the US Department of Energy under Contract No. DE-AC02-98CH10886. We thank P. Crivelli for useful discussions on positronium physics. NR 18 TC 8 Z9 8 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD DEC 6 PY 2013 VL 88 IS 6 AR 065502 DI 10.1103/PhysRevC.88.065502 PG 5 WC Physics, Nuclear SC Physics GA 274CJ UT WOS:000328582400008 ER PT J AU Sharapov, EI Morris, CL Makela, M Saunders, A Adamek, ER Broussard, LJ Cude-Woods, CB Fellers, DE Geltenbort, P Hartl, M Hasan, SI Hickerson, KP Hogan, G Holley, AT Lavelle, CM Liu, CY Mendenhall, MP Ortiz, J Pattie, RW Phillips , DG Ramsey, J Salvat, DJ Seestrom, SJ Shaw, E Sjue, S Sondheim, WE Dick, BV Wang, Z Womack, TL Young, AR Zeck, BA AF Sharapov, E. I. Morris, C. L. Makela, M. Saunders, A. Adamek, Evan R. Broussard, L. J. Cude-Woods, C. B. Fellers, Deion E. Geltenbort, Peter Hartl, M. Hasan, S. I. Hickerson, K. P. Hogan, G. Holley, A. T. Lavelle, C. M. Liu, Chen-Yu Mendenhall, M. P. Ortiz, J. Pattie, R. W., Jr. Phillips, D. G., II Ramsey, J. Salvat, D. J. Seestrom, S. J. Shaw, E. Sjue, Sky Sondheim, W. E. Dick, B. Vorn Wang, Z. Womack, T. L. Young, A. R. Zeck, B. A. TI Upscattering of ultracold neutrons from the polymer [C6H12](n) SO PHYSICAL REVIEW C LA English DT Article ID SLOW-NEUTRONS; POLYETHYLENE; STORAGE AB It is generally accepted that the main cause of ultracold neutron (UCN) losses in storage traps is upscattering to the thermal energy range by hydrogen adsorbed on the surface of the trap walls. However, the data on which this conclusion is based are poor and contradictory. Here we report a measurement, performed at the Los Alamos National Laboratory UCN source, of the average energy of the flux of upscattered neutrons after the interaction of UCN with hydrogen bound in the semicrystalline polymer PMP (trade name TPX), [C6H12](n). Our analysis, performed with the MCNP code which applies the neutron-scattering law to UCN upscattered by bound hydrogen in semicrystalline polyethylene, [C2H4](n), leads us to a flux average energy value of 26 +/- 3 meV, in contradiction to previously reported experimental values of 10 to 13 meV and in agreement with the theoretical models of neutron heating implemented in MCNP. C1 [Sharapov, E. I.] Joint Inst Nucl Res, Dubna 141980, Russia. [Morris, C. L.; Makela, M.; Saunders, A.; Broussard, L. J.; Cude-Woods, C. B.; Fellers, Deion E.; Hartl, M.; Hogan, G.; Ortiz, J.; Ramsey, J.; Seestrom, S. J.; Shaw, E.; Sjue, Sky; Sondheim, W. E.; Wang, Z.; Womack, T. L.; Zeck, B. A.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Adamek, Evan R.; Cude-Woods, C. B.; Holley, A. T.; Liu, Chen-Yu; Salvat, D. J.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Geltenbort, Peter] Inst Laue Langevin, F-38042 Grenoble 9, France. [Hasan, S. I.] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA. [Hickerson, K. P.; Mendenhall, M. P.] CALTECH, Kellogg Radiat Lab, Pasadena, CA 91125 USA. [Lavelle, C. M.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Pattie, R. W., Jr.; Phillips, D. G., II; Dick, B. Vorn; Young, A. R.; Zeck, B. A.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. RP Morris, CL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. EM cmorris@lanl.gov RI Hartl, Monika/F-3094-2014; Hartl, Monika/N-4586-2016; OI Hartl, Monika/0000-0002-6601-7273; Hartl, Monika/0000-0002-6601-7273; Broussard, Leah/0000-0001-9182-2808; Makela, Mark/0000-0003-0592-3683; Morris, Christopher/0000-0003-2141-0255 FU U.S. Department of Energy [DE-AC52-06NA25396]; DOE Office of Science; American Recovery and Reinvestment Act [DE-AC05-06OR23100] FX We thank L. Daemen for help in acquiring x-ray diffraction data for our samples. This work was performed under the auspices of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. Author D.J.S. is supported by the DOE Office of Science Graduate Fellowship Program, made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under Contract No. DE-AC05-06OR23100. NR 21 TC 1 Z9 1 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD DEC 6 PY 2013 VL 88 IS 6 AR 064605 DI 10.1103/PhysRevC.88.064605 PG 4 WC Physics, Nuclear SC Physics GA 274CJ UT WOS:000328582400006 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, 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Will, J. Z. Williams, E. Williams, H. H. Williams, S. Willis, W. Willocq, S. Wilson, J. A. Wilson, A. Wingerter-Seez, I. Winkelmann, S. Winklmeier, F. Wittgen, M. Wittig, T. Wittkowski, J. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wong, W. C. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wraight, K. Wright, M. Wu, S. L. Wu, X. Wu, Y. Wulf, E. Wyatt, T. R. Wynne, B. M. Xella, S. Xiao, M. Xu, C. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yamada, M. Yamaguchi, H. Yamaguchi, Y. Yamamoto, A. Yamamoto, K. Yamamoto, S. Yamamura, T. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, U. K. Yang, Y. Yang, Z. Yanush, S. Yao, L. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yen, A. L. Yildirim, E. Yilmaz, M. Yoosoofmiya, R. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. Yuan, L. Yurkewicz, A. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zambito, S. Zanello, L. Zanzi, D. Zaytsev, A. Zeitnitz, C. Zeman, M. Zemla, A. Zenin, O. Zenis, T. Zerwas, D. della Porta, G. Zevi Zhang, D. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, L. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. Zur Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Search for charginos nearly mass degenerate with the lightest neutralino based on a disappearing-track signature in pp collisions at root(s)=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article AB A search is presented for direct chargino production based on a disappearing-track signature using 20.3 fb(-1) of proton-proton collisions at root s = 8 TeV collected with the ATLAS experiment at the LHC. In anomaly-mediated supersymmetry breaking (AMSB) models, the lightest chargino is nearly mass degenerate with the lightest neutralino and its lifetime is long enough to be detected in the tracking detectors by identifying decays that result in tracks with no associated hits in the outer region of the tracking system. Some models with supersymmetry also predict charginos with a significant lifetime. This analysis attains sensitivity for charginos with a lifetime between 0.1 and 10 ns, and significantly surpasses the reach of the LEP experiments. No significant excess above the background expectation is observed for candidate tracks with large transverse momentum, and constraints on chargino properties are obtained. In the AMSB scenarios, a chargino mass below 270 GeV is excluded at 95% confidence level. C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. 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[Bindi, M.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, A. P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Abajyan, T.; Arslan, O.; Backhaus, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Glatzer, J.; Haefner, P.; Hageboeck, S.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Amundsen, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.; Zambito, S.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Backes, M.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Baines, J. T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zhou, L.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Hoffmann, M. Dano; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Milan, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Socher, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Kajomovitz, E.; Ko, B. R.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Olivares Pino, S. A.; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Vu Anh, T.; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Alexander, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Milan, Italy. [Barberis, D.; Caso, C.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subat & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. 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F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Milan, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, A. M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. 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J.; Ta, D.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. 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E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Milan, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Oussoren, K. P.; Pani, P.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Oussoren, K. P.; Pani, P.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Milan, Italy. [Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Milan, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Dos Santos, D. Roda; Ruzicka, P.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Particle Phys Dept, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Milan, Italy. [Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Milan, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Milan, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Mountricha, E.; Nguyen Thi Hong, V.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay, DSM IRFU, Inst Rech Lois Fondamentales Univers, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Huang, Y.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Grout, Z. J.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Gough Eschrich, I.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Milan, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, Freiburg, Germany. RI la rotonda, laura/B-4028-2016; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Ventura, Andrea/A-9544-2015; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gutierrez, Phillip/C-1161-2011; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Deliot, Frederic/F-3321-2014; Nozka, Libor/G-5550-2014; Kepka, Oldrich/G-6375-2014; Nemecek, Stanislav/G-5931-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Snesarev, Andrey/H-5090-2013; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Smirnova, Oxana/A-4401-2013; Gabrielli, Alessandro/H-4931-2012; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Ferrando, James/A-9192-2012 OI la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Karpov, Sergey/0000-0002-2230-5353; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Warburton, Andreas/0000-0002-2298-7315; Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Castro, Nuno/0000-0001-8491-4376; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Mikestikova, Marcela/0000-0003-1277-2596; Doyle, Anthony/0000-0001-6322-6195; Boyko, Igor/0000-0002-3355-4662; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Lee, Jason/0000-0002-2153-1519; Kuday, Sinan/0000-0002-0116-5494; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Fabbri, Laura/0000-0002-4002-8353; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Ferrando, James/0000-0002-1007-7816 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan;; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular, from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA), and in the Tier-2 facilities worldwide. NR 38 TC 36 Z9 36 U1 8 U2 130 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 6 PY 2013 VL 88 IS 11 AR 112006 DI 10.1103/PhysRevD.88.112006 PG 23 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274KE UT WOS:000328604400001 ER PT J AU Aartsen, MG Abbasi, R Abdou, Y Ackermann, M Adams, J Aguilar, JA Ahlers, M Altmann, D Auffenberg, J Bai, X Baker, M Barwick, SW Baum, V Bay, R Beatty, JJ Bechet, S Tjus, JB Becker, KH Benabderrahmane, ML BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Bertrand, D Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohaichuk, S Bohm, C Bose, D Boser, S Botner, O Brayeur, L Bretz, HP Brown, AM Bruijn, R Brunner, J Carson, M Casey, J Casier, M Chirkin, D Christov, A Christy, B Clark, K Clevermann, F Coenders, S Cohen, S Cowen, DF Silva, AHC Danninger, M Daughhetee, J Davis, JC Day, M De Clercq, C De Ridder, S Desiati, P de Vries, KD de With, M DeYoung, T Diaz-Velez, JC Dunkman, M Eagan, R Eberhardt, B Eisch, J Ellsworth, RW Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feintzeig, J Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Flis, S Franckowiak, A Frantzen, K Fuchs, T Gaisser, TK Gallagher, J Gerhardt, L Gladstone, L Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grandmont, DT Grant, D Gross, A Ha, C Ismail, AH Hallen, P Hallgren, A Halzen, F Hanson, K Heereman, D Heinen, D Helbing, K Hellauer, R Hickford, S Hill, GC Hoffman, KD Hoffmann, R Homeier, A Hoshina, K Huelsnitz, W Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobi, E Jacobsen, J Jagielski, K Japaridze, GS Jero, K Jlelati, O Kaminsky, B Kappes, A Karg, T Karle, A Kelley, JL Kiryluk, J Klas, J Klein, SR Kohne, JH Kohnen, G Kolanoski, H Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krasberg, M Krings, K Kroll, G Kunnen, J Kurahashi, N Kuwabara, T Labare, M Landsman, H Larson, MJ Lesiak-Bzdak, M Leuermann, M Leute, J Lunemann, J Macias, O Madsen, J Maggi, G Maruyama, R Mase, K Matis, HS McNally, F Meagher, K Merck, M Meures, T Miarecki, S Middell, E Milke, N Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Odrowski, S Olivas, A Omairat, A O'Murchadha, A Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Radel, L Rameez, M Rawlins, K Redl, P Reimann, R Resconi, E Rhode, W Ribordy, M Richman, M Riedel, B Rodrigues, JP Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Salameh, T Sander, HG Santander, M Sarkar, S Schatto, K Scheriau, F Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schukraft, A Schulte, L Schulz, O Seckel, D Sestayo, Y Seunarine, S Shanidze, R Sheremata, C Smith, MWE Soldin, D Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Sullivan, GW Taavola, H Taboada, I Tamburro, A Tepe, A Ter-Antonyan, S Tesic, G Tilav, S Toale, PA Toscano, S Unger, E Usner, M Vallecorsa, S van Eijndhoven, N Van Overloop, A van Santen, J Vehring, M Voge, M Vraeghe, M Walck, C Waldenmaier, T Wallraff, M Weaver, C Wellons, M Wendt, C Westerhoff, S Whitehorn, N Wiebe, K Wiebusch, CH Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Ziemann, J Zierke, S Zoll, M AF Aartsen, M. G. Abbasi, R. Abdou, Y. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Altmann, D. Auffenberg, J. Bai, X. Baker, M. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Bechet, S. Tjus, J. Becker Becker, K. -H. Benabderrahmane, M. L. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Bertrand, D. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohaichuk, S. Bohm, C. Bose, D. Boeser, S. Botner, O. Brayeur, L. Bretz, H. -P. Brown, A. M. Bruijn, R. Brunner, J. Carson, M. Casey, J. Casier, M. Chirkin, D. Christov, A. Christy, B. Clark, K. Clevermann, F. Coenders, S. Cohen, S. Cowen, D. F. Silva, A. H. Cruz Danninger, M. Daughhetee, J. Davis, J. C. Day, M. De Clercq, C. De Ridder, S. Desiati, P. de Vries, K. D. de With, M. DeYoung, T. Diaz-Velez, J. C. Dunkman, M. Eagan, R. Eberhardt, B. Eisch, J. Ellsworth, R. W. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feintzeig, J. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Franckowiak, A. Frantzen, K. Fuchs, T. Gaisser, T. K. Gallagher, J. Gerhardt, L. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grandmont, D. T. Grant, D. Gross, A. Ha, C. Ismail, A. Haj Hallen, P. Hallgren, A. Halzen, F. Hanson, K. Heereman, D. Heinen, D. Helbing, K. Hellauer, R. Hickford, S. Hill, G. C. Hoffman, K. D. Hoffmann, R. Homeier, A. Hoshina, K. Huelsnitz, W. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobi, E. Jacobsen, J. Jagielski, K. Japaridze, G. S. Jero, K. Jlelati, O. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kelley, J. L. Kiryluk, J. Klaes, J. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krasberg, M. Krings, K. Kroll, G. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Landsman, H. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leute, J. Luenemann, J. Macias, O. Madsen, J. Maggi, G. Maruyama, R. Mase, K. Matis, H. S. McNally, F. Meagher, K. Merck, M. Meures, T. Miarecki, S. Middell, E. Milke, N. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Odrowski, S. Olivas, A. Omairat, A. O'Murchadha, A. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Reimann, R. Resconi, E. Rhode, W. Ribordy, M. Richman, M. Riedel, B. Rodrigues, J. P. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Salameh, T. Sander, H. -G. Santander, M. Sarkar, S. Schatto, K. Scheriau, F. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Schulz, O. Seckel, D. Sestayo, Y. Seunarine, S. Shanidze, R. Sheremata, C. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Strom, R. Sullivan, G. W. Taavola, H. Taboada, I. Tamburro, A. Tepe, A. Ter-Antonyan, S. Tesic, G. Tilav, S. Toale, P. A. Toscano, S. Unger, E. Usner, M. Vallecorsa, S. van Eijndhoven, N. Van Overloop, A. van Santen, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Waldenmaier, T. Wallraff, M. Weaver, Ch. Wellons, M. Wendt, C. Westerhoff, S. Whitehorn, N. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Ziemann, J. Zierke, S. Zoll, M. CA IceCube Collaboration TI IceCube search for dark matter annihilation in nearby galaxies and galaxy clusters SO PHYSICAL REVIEW D LA English DT Article ID CONSTRAINTS; PARTICLES; EVOLUTION; SIGNALS; HALOES; SYSTEM AB We present the results of a first search for self-annihilating dark matter in nearby galaxies and galaxy clusters using a sample of high-energy neutrinos acquired in 339.8 days of live time during 2009/10 with the IceCube neutrino observatory in its 59-string configuration. The targets of interest include the Virgo and Coma galaxy clusters, the Andromeda galaxy, and several dwarf galaxies. We obtain upper limits on the cross section as a function of the weakly interacting massive particle mass between 300 GeV and 100 TeV for the annihilation into b (b) over bar, W+(W) over bar (-), tau(+)tau(-), mu(+)mu(-) , and nu(nu) over bar. 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R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Bay, R.; Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Altmann, D.; de With, M.; Kappes, A.; Kolanoski, H.; Schoeneberg, S.; Unger, E.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Tjus, J. Becker; Fedynitch, A.; Saba, S. M.; Schoeneberg, S.; Unger, E.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Boeser, S.; Franckowiak, A.; Homeier, A.; Kowalski, M.; Schulte, L.; Stasik, A.; Usner, M.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Bechet, S.; Bertrand, D.; Hanson, K.; Heereman, D.; Meures, T.; O'Murchadha, A.; Pinat, E.] Univ Libre Bruxelles, B-1050 Brussels, Belgium. [Bose, D.; Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; Golup, G.; Kunnen, J.; Maggi, G.; Miller, J.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Ishihara, A.; Mase, K.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Adams, J.; Brown, A. M.; Hickford, S.; Macias, O.] Univ Canterbury, Dept Phys & Astron, Christchurch 8140, New Zealand. [Berley, D.; Blaufuss, E.; Christy, B.; Ellsworth, R. W.; Goodman, J. A.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Meagher, K.; Olivas, A.; Redl, P.; Richman, M.; Schmidt, T.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Clevermann, F.; Frantzen, K.; Fuchs, T.; Koehne, J. -H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.; Scheriau, F.; Schmitz, M.; Ziemann, J.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Bohaichuk, S.; Grandmont, D. T.; Grant, D.; Nowicki, S. C.; Odrowski, S.; Sheremata, C.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Aguilar, J. A.; Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [Abdou, Y.; Carson, M.; De Ridder, S.; Feusels, T.; Ismail, A. Haj; Jlelati, O.; Labare, M.; Ryckbosch, D.; Van Overloop, A.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Barwick, S. W.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Bruijn, R.; Cohen, S.; Ribordy, M.] Ecole Polytech Fed Lausanne, High Energy Phys Lab, CH-1015 Lausanne, Switzerland. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Abbasi, R.; Ahlers, M.; Auffenberg, J.; Baker, M.; BenZvi, S.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kelley, J. L.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Abbasi, R.; Ahlers, M.; Auffenberg, J.; Baker, M.; BenZvi, S.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kelley, J. L.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Baum, V.; Eberhardt, B.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Bernhard, A.; Gross, A.; Leute, J.; Resconi, E.; Schulz, O.; Sestayo, Y.] Tech Univ Munich, D-85748 Garching, Germany. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Larson, M. J.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Clark, K.; Cowen, D. F.; DeYoung, T.; Dunkman, M.; Eagan, R.; Koskinen, D. J.; Salameh, T.; Smith, M. W. E.; Tesic, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Boersma, D. J.; Botner, O.; Hallgren, A.; de los Heros, C. Perez; Strom, R.; Taavola, H.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D.; Tepe, A.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Ackermann, M.; Benabderrahmane, M. L.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Brunner, J.; Silva, A. H. Cruz; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Kaminsky, B.; Karg, T.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Stoessl, A.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. [Montaruli, T.] Dipartimento Fis, Sez INFN, I-70126 Bari, Italy. RP Lunemann, J (reprint author), Johannes Gutenberg Univ Mainz, Inst Phys, Staudinger Weg 7, D-55099 Mainz, Germany. EM jan.luenemann@uni-mainz.de RI Taavola, Henric/B-4497-2011; Wiebusch, Christopher/G-6490-2012; Auffenberg, Jan/D-3954-2014; Koskinen, David/G-3236-2014; Brunner, Juergen/G-3540-2015; Aguilar Sanchez, Juan Antonio/H-4467-2015; Maruyama, Reina/A-1064-2013; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; Tjus, Julia/G-8145-2012 OI Taavola, Henric/0000-0002-2604-2810; Carson, Michael/0000-0003-0400-7819; Perez de los Heros, Carlos/0000-0002-2084-5866; Benabderrahmane, Mohamed Lotfi/0000-0003-4410-5886; Wiebusch, Christopher/0000-0002-6418-3008; Auffenberg, Jan/0000-0002-1185-9094; Koskinen, David/0000-0002-0514-5917; Brunner, Juergen/0000-0002-5052-7236; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Maruyama, Reina/0000-0003-2794-512X; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Rott, Carsten/0000-0002-6958-6033; Ter-Antonyan, Samvel/0000-0002-5788-1369; Schukraft, Anne/0000-0002-9112-5479; FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison; Open Science Grid (OSG) grid infrastructure; U. S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid; Compute/Calcul Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF) FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; U. S. Department of Energy, National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid, and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF). The research has made use of the SIMBAD database, operated at CDS, Strasbourg, France. NR 57 TC 36 Z9 36 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD DEC 6 PY 2013 VL 88 IS 12 AR UNSP 122001 DI 10.1103/PhysRevD.88.122001 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274KG UT WOS:000328604600002 ER PT J AU Yang, SX Terletska, H Meng, ZY Moreno, J Jarrell, M AF Yang, S. -X. Terletska, H. Meng, Z. Y. Moreno, J. Jarrell, M. TI Mean-field embedding of the dual-fermion approach for correlated electron systems SO PHYSICAL REVIEW E LA English DT Article ID CONSERVING APPROXIMATIONS; MODEL; DIMENSIONS; DYNAMICS AB To reduce the rapidly growing computational cost of the dual-fermion lattice calculation with increasing system size, we introduce two embedding schemes. One is the real fermion embedding, and the other is the dual-fermion embedding. Our numerical tests show that the real fermion and dual-fermion embedding approaches converge to essentially the same result. The application on the Anderson disorder and Hubbard models shows that these embedding algorithms converge more quickly with system size as compared to the conventional dual-fermion method, for the calculation of both single-and two-particle quantities. C1 [Yang, S. -X.; Meng, Z. Y.; Moreno, J.; Jarrell, M.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Yang, S. -X.; Meng, Z. Y.; Moreno, J.; Jarrell, M.] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Terletska, H.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Yang, SX (reprint author), Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. EM yangphysics@gmail.com RI Moreno, Juana/D-5882-2012; Meng, Zi Yang/F-5212-2012 OI Meng, Zi Yang/0000-0001-9771-7494 FU DOE SciDAC grant [DE-FC02-10ER25916]; BES CMCSN grant [DE-AC02-98CH10886]; NSF EPSCoR [EPS-1003897] FX This work is supported by the DOE SciDAC grant DE-FC02-10ER25916 (S.Y. and M.J.) and BES CMCSN grant DE-AC02-98CH10886 (H.T.). Additional support was provided by NSF EPSCoR Cooperative Agreement No. EPS-1003897 (Z.M. and J.M.). NR 27 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD DEC 6 PY 2013 VL 88 IS 6 AR 063306 DI 10.1103/PhysRevE.88.063306 PG 9 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 274KX UT WOS:000328606300014 PM 24483583 ER PT J AU Parker, WD Nakhmanson, SM AF Parker, William D. Nakhmanson, S. M. TI Density functional study of the structural, electronic, and vibrational properties of beta-Ba2TiO4 SO PHYSICAL REVIEW B LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; BORN EFFECTIVE CHARGES; BARIUM ORTHOTITANATE; DIELECTRIC-PROPERTIES; ABSORPTION PROPERTIES; PERTURBATION-THEORY; CRYSTAL-STRUCTURE; BAND-STRUCTURE; TI-O; TITANATE AB Motivated by the reported high dielectric response of monoclinic beta-Ba2TiO4 as well as its affinity for absorbing small molecules, we investigate its structural, electronic, and vibrational properties with density functional theory (DFT). DFT-based structural optimization obtains lattice parameters and bond lengths within a few percent of experimentally observed values, with specific details depending on the choice of exchange-correlation functional. Although, for both the local density approximation (LDA) and generalized gradient approximation (GGA) functionals employed, the DFT calculations produce a wide-band-gap insulating state for beta-Ba2TiO4 (with an indirect gap of 4.1 eV or greater), they do not agree on the energetic ordering of this phase with respect to its perovskite-like Ruddlesden-Popper (RP) polymorph. Simulations that utilize LDA place the beta phase 0.30 eV higher, while those using the Perdew-Burke-Ernzerhof GGA functional place it 0.22 eV lower than the RP one, leaving the question of the degree of perovskite-like phase metastability under epitaxial growth conditions unresolved. Comparison of the formula unit volumes of the A(2)TiO(4) and ATiO(3) polymorphs (A = Sr, Ba) reveals that both Ba2TiO4 structures possess much more open geometries-more so for the beta than for the RP phase-than their isostoichiometric Sr-based counterparts and all of the examined ATiO(3) compounds, in line with the demonstrated propensity of the Ba-based 2-1-4 oxides to capture molecules like CO2 and H2O. However, an analysis of vibrations and their contributions to the static dielectric permittivity tensor of beta-Ba2TiO4 indicates that, unlike the perovskite RP phase, this structure does not exhibit strong polar lattice distortions, which results in a rather low value for its average static dielectric constant. C1 [Parker, William D.] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. [Parker, William D.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Nakhmanson, S. M.] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Nakhmanson, S. M.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. RP Parker, WD (reprint author), Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wparker@anl.gov RI Nakhmanson, Serge/A-6329-2014; Parker, William/B-4970-2012 OI Parker, William/0000-0003-2454-6094 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; American Recovery and Reinvestment Act (ARRA) through the Office of Advanced Scientific Computing Research [DE-AC02-06CH11357] FX This project was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, and by American Recovery and Reinvestment Act (ARRA) funding through the Office of Advanced Scientific Computing Research under Contract No. DE-AC02-06CH11357. NR 54 TC 0 Z9 0 U1 10 U2 45 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 6 PY 2013 VL 88 IS 24 AR 245108 DI 10.1103/PhysRevB.88.245108 PG 8 WC Physics, Condensed Matter SC Physics GA 274BD UT WOS:000328579200001 ER PT J AU Barday, R Burrill, A Jankowiak, A Kamps, T Knobloch, J Kugeler, O Matveenko, A Neumann, A Schmeisser, M Volker, J Kneisel, P Nietubyc, R Schubert, S Smedley, J Sekutowicz, J Will, I AF Barday, R. Burrill, A. Jankowiak, A. Kamps, T. Knobloch, J. Kugeler, O. Matveenko, A. Neumann, A. Schmeisser, M. Voelker, J. Kneisel, P. Nietubyc, R. Schubert, S. Smedley, J. Sekutowicz, J. Will, I. TI Characterization of a superconducting Pb photocathode in a superconducting rf photoinjector cavity SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB Photocathodes are a limiting factor for the next generation of ultrahigh brightness photoinjectors. We studied the behavior of a superconducting Pb cathode in the cryogenic environment of a superconducting rf gun cavity to measure the quantum efficiency, its spatial distribution, and the work function. We will also discuss how the cathode surface contaminants modify the performance of the photocathode as well as the gun cavity and we discuss the possibilities to remove these contaminants. C1 [Barday, R.; Burrill, A.; Jankowiak, A.; Kamps, T.; Knobloch, J.; Kugeler, O.; Matveenko, A.; Neumann, A.; Schmeisser, M.; Voelker, J.] Mat & Energie GmbH, Helmholtz Zentrum Berlin, D-14109 Berlin, Germany. [Kneisel, P.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Nietubyc, R.] Natl Ctr Nucl Res, PL-05400 Otwock, Poland. [Schubert, S.; Smedley, J.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Sekutowicz, J.] DESY, D-22603 Hamburg, Germany. [Will, I.] Max Born Inst, D-12489 Berlin, Germany. RP Barday, R (reprint author), Mat & Energie GmbH, Helmholtz Zentrum Berlin, Hahn Meitner Pl 1, D-14109 Berlin, Germany. EM roman.barday@helmholtz-berlin.de RI Knobloch, Jens/F-1452-2015 FU Bundesministerium fur Bildung und Forschung; Land Berlin; EuCARD FX The authors acknowledge fruitful discussions with K. Aulenbacher, D. Dowell, and V. I. Shvedunov. We would also like to thank M. Schenk for technical support. This work was supported by Bundesministerium fur Bildung und Forschung and Land Berlin. The Pb deposition activity is supported by EuCARD. NR 20 TC 4 Z9 4 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD DEC 6 PY 2013 VL 16 IS 12 AR 123402 DI 10.1103/PhysRevSTAB.16.123402 PG 7 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 274PW UT WOS:000328619500002 ER PT J AU Elizarov, A Litvinenko, V AF Elizarov, Andrey Litvinenko, Vladimir TI Semianalytical description of the modulator section of the coherent electron cooling SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB In the coherent electron cooling, the modern hadron beam cooling technique, each hadron receives an individual kick from the electric field of the amplified electron density perturbation created in the modulator by this hadron in a copropagating electron beam. We developed a method for computing the dynamics of these density perturbations in an infinite electron plasma with any equilibrium velocity distribution-a possible model for the modulator. We derived analytical expressions for the dynamics of the density perturbations in the Fourier-Laplace domain for a variety of 1D, 2D, and 3D equilibrium distributions of the electron beam. To obtain the space-time dynamics, we employed the fast Fourier transform algorithm. We also found an analytical solution in the space-time domain for the 1D Cauchy equilibrium distribution, which serves as a benchmark for our general approach based on numerical evaluation of the integral transforms and as a fast alternative to the numerical computations. We tested the method for various distributions and initial conditions. C1 [Elizarov, Andrey; Litvinenko, Vladimir] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. [Elizarov, Andrey; Litvinenko, Vladimir] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Elizarov, A (reprint author), Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. EM andrey.elizarov@stonybrook.edu; vl@bnl.gov NR 14 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD DEC 6 PY 2013 VL 16 IS 12 AR 124001 DI 10.1103/PhysRevSTAB.16.124001 PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 274PW UT WOS:000328619500003 ER PT J AU Mustapha, B Kolomiets, AA Ostroumov, PN AF Mustapha, B. Kolomiets, A. A. Ostroumov, P. N. TI Full three-dimensional approach to the design and simulation of a radio-frequency quadrupole SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB We have developed a new full 3D approach for the electromagnetic and beam dynamics design and simulation of a radio-frequency quadrupole (RFQ). A detailed full 3D model including vane modulation was simulated, which was made possible by the ever advancing computing capabilities. The electromagnetic (EM) design approach was first validated using experimental measurements on an existing prototype RFQ and more recently on the actual full size RFQ. Two design options have been studied, the original with standard sinusoidal modulation over the full length of the RFQ; in the second design, a trapezoidal modulation was used in the accelerating section of the RFQ to achieve a higher energy gain for the same power and length. A detailed comparison of both options is presented supporting our decision to select the trapezoidal design. The trapezoidal modulation increased the shunt impedance of the RFQ by 34%, the output energy by 15% with a similar increase in the peak surface electric field, but practically no change in the dynamics of the accelerated beam. The beam dynamics simulations were performed using three different field methods. The first uses the standard eight-term potential to derive the fields, the second uses 3D fields from individual cell-by-cell models, and the third uses the 3D fields for the whole RFQ as a single cavity. A detailed comparison of the results from TRACK shows a very good agreement, validating the 3D fields approach used for the beam dynamics studies. The EM simulations were mainly performed using the CST MICROWAVE-STUDIO with the final results verified using other software. Detailed segment-by-segment and full RFQ frequency calculations were performed and compared to the measured data. The maximum frequency deviation is about 100 kHz. The frequencies of higher-order modes have also been calculated and finally the modulation and tuners effects on both the frequency and field flatness have been studied. We believe that with this new full 3D approach, the enhanced computing capabilities and the calculation precision the electromagnetic design software offer, we may be able to skip the prototyping phase and build the final product at once, although we recognize that prototyping is still needed to establish and validate the fabrication procedure. C1 [Mustapha, B.; Kolomiets, A. A.; Ostroumov, P. N.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Mustapha, B (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM brahim@anl.gov FU U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX The authors would like to thank A. Barcikowski and G. Zinkann for the frequency measurements on the individual segments and the full ATLAS upgrade RFQ, and Z. Conway for reading and discussing the manuscript. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. NR 29 TC 4 Z9 4 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD DEC 6 PY 2013 VL 16 IS 12 AR 120101 DI 10.1103/PhysRevSTAB.16.120101 PG 14 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 274PW UT WOS:000328619500001 ER PT J AU Suchowski, H O'Brien, K Wong, ZJ Salandrino, A Yin, XB Zhang, X AF Suchowski, Haim O'Brien, Kevin Wong, Zi Jing Salandrino, Alessandro Yin, Xiaobo Zhang, Xiang TI Phase Mismatch-Free Nonlinear Propagation in Optical Zero-Index Materials SO SCIENCE LA English DT Article ID NEGATIVE-INDEX; 2ND-HARMONIC GENERATION; PARAMETRIC AMPLIFICATION; METAMATERIALS; OSCILLATOR; REFRACTION AB Phase matching is a critical requirement for coherent nonlinear optical processes such as frequency conversion and parametric amplification. Phase mismatch prevents microscopic nonlinear sources from combining constructively, resulting in destructive interference and thus very low efficiency. We report the experimental demonstration of phase mismatch-free nonlinear generation in a zero-index optical metamaterial. In contrast to phase mismatch compensation techniques required in conventional nonlinear media, the zero index eliminates the need for phase matching, allowing efficient nonlinear generation in both forward and backward directions. We demonstrate phase mismatch-free nonlinear generation using intrapulse four-wave mixing, where we observed a forward-to-backward nonlinear emission ratio close to unity. The removal of phase matching in nonlinear optical metamaterials may lead to applications such as multidirectional frequency conversion and entangled photon generation. C1 [Suchowski, Haim; O'Brien, Kevin; Wong, Zi Jing; Salandrino, Alessandro; Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Yin, Xiaobo/A-4142-2011; Zhang, Xiang/F-6905-2011; Salandrino, Alessandro/B-5898-2011; Foundry, Molecular/G-9968-2014 OI Salandrino, Alessandro/0000-0002-8643-9764; FU U.S. Department of Energy, Office of Basic Energy Sciences through the Materials Sciences Division of Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Fulbright Foundation FX Supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract no. DE-AC02-05CH11231 through the Materials Sciences Division of Lawrence Berkeley National Laboratory. H. S. and Z.J.W. acknowledge partial support by the Fulbright Foundation. We thank the Molecular Foundry, Lawrence Berkeley National Laboratory, for technical support in nanofabrication. NR 29 TC 71 Z9 71 U1 9 U2 110 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD DEC 6 PY 2013 VL 342 IS 6163 BP 1223 EP 1226 DI 10.1126/science.1244303 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 264DT UT WOS:000327857900045 PM 24311687 ER PT J AU Shi, XW Clark, JN Xiong, G Huang, XJ Harder, R Robinson, IK AF Shi, Xiaowen Clark, Jesse N. Xiong, Gang Huang, Xiaojing Harder, Ross Robinson, Ian K. TI Mechanical breakdown of bent silicon nanowires imaged by coherent x-ray diffraction SO NEW JOURNAL OF PHYSICS LA English DT Article ID DEFORMATION; NANOSCALE; STRAIN; FIELD; HETEROSTRUCTURES; FRACTURE; STRESS AB We have developed a method of coherent x-ray diffractive imaging to surmount its inability to image the structure of strongly strained crystals. We used calculated models from finite-element analysis to guide an iterative algorithm to fit experimental data from a series of increasingly bent wires cut into silicon-on-insulator films. Just before mechanical fracture, the wires were found to contain new phase structures, which are identified as dislocations associated with crossing the elastic limit. C1 [Shi, Xiaowen; Clark, Jesse N.; Xiong, Gang; Huang, Xiaojing; Robinson, Ian K.] UCL, London Ctr Nanotechnol, London WC1E 6BT, England. [Shi, Xiaowen; Clark, Jesse N.; Xiong, Gang; Huang, Xiaojing; Robinson, Ian K.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Huang, Xiaojing; Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Robinson, Ian K.] Res Complex Harwell, Didcot OX11 0DE, Oxon, England. RP Robinson, IK (reprint author), UCL, London Ctr Nanotechnol, Gower St, London WC1E 6BT, England. EM i.robinson@ucl.ac.uk FU NSF [DMR-9724294]; DOE [DE-AC02-06CH11357]; European Research Council [227711] FX The experimental work was performed at APS beamline 34-ID-C, built with funds from the NSF under grant DMR-9724294 and operated by the DOE, under contract no. DE-AC02-06CH11357. The research was supported by the European Research Council 'Advanced' grant 'Nanosculpture' code 227711. We thank Dr Dorothy Duffy, Bo Chen, Isaac Peterson and Zheng Gu for fruitful discussions on the mechanical breakdown of silicon and the optimization of CDI algorithms. NR 35 TC 3 Z9 3 U1 1 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD DEC 5 PY 2013 VL 15 AR 123007 DI 10.1088/1367-2630/15/12/123007 PG 15 WC Physics, Multidisciplinary SC Physics GA 286AJ UT WOS:000329436600004 ER PT J AU Yan, YH Candreva, J Shi, H Ernst, E Martienssen, R Schwender, J Shanklin, J AF Yan, Yiheng Candreva, Jason Shi, Hai Ernst, Evan Martienssen, Robert Schwender, Jorg Shanklin, John TI Survey of the total fatty acid and triacylglycerol composition and content of 30 duckweed species and cloning of a Delta 6-desaturase responsible for the production of gamma-linolenic and stearidonic acids in Lemna gibba SO BMC PLANT BIOLOGY LA English DT Article DE Desaturase; Fatty acid; Triacylglycerol; Lemnoideae; Duckweed; Lemna; Wolffiela; Renewable feedstock; Biofuel ID DELTA(8)-SPHINGOLIPID DESATURASES; MOLECULAR CHARACTERIZATION; LIPID-SYNTHESIS; HIGHER-PLANTS; ARABIDOPSIS; ACCUMULATION; OIL; PROTEIN; ENZYME; IDENTIFICATION AB Background: Duckweeds, i.e., members of the Lemnoideae family, are amongst the smallest aquatic flowering plants. Their high growth rate, aquatic habit and suitability for bio-remediation make them strong candidates for biomass production. Duckweeds have been studied for their potential as feedstocks for bioethanol production; however, less is known about their ability to accumulate reduced carbon as fatty acids (FA) and oil. Results: Total FA profiles of thirty duckweed species were analysed to assess the natural diversity within the Lemnoideae. Total FA content varied between 4.6% and 14.2% of dry weight whereas triacylglycerol (TAG) levels varied between 0.02% and 0.15% of dry weight. Three FA, 16:0 (palmitic), 18:2 Delta 9,12 (Linoleic acid, or LN) and 18:3 Delta 9,12,15 (a-linolenic acid, or ALA) comprise more than 80% of total duckweed FA. Seven Lemna and two Wolffiela species also accumulate polyunsaturated FA containing Delta 6-double bonds, i.e., GLA and SDA. Relative to total FA, TAG is enriched in saturated FA and deficient in polyunsaturated FA, and only five Lemna species accumulate Delta 6-FA in their TAG. A putative Delta 6-desaturase designated LgDes, with homology to a family of front-end Delta 6-FA and Delta 8-spingolipid desaturases, was identified in the assembled DNA sequence of Lemna gibba. Expression of a synthetic LgDes gene in Nicotiana benthamiana resulted in the accumulation of GLA and SDA, confirming it specifies a Delta 6-desaturase. Conclusions: Total accumulation of FA varies three-fold across the 30 species of Lemnoideae surveyed. Nine species contain GLA and SDA which are synthesized by a Delta 6 front-end desaturase, but FA composition is otherwise similar. TAG accumulates up to 0.15% of total dry weight, comparable to levels found in the leaves of terrestrial plants. Polyunsaturated FA is underrepresented in TAG, and the Delta 6-FA GLA and SDA are found in the TAG of only five of the nine Lemna species that produce them. When present, GLA is enriched and SDA diminished relative to their abundance in the total FA pool. C1 [Yan, Yiheng; Candreva, Jason; Shi, Hai; Schwender, Jorg; Shanklin, John] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. [Ernst, Evan; Martienssen, Robert] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA. RP Shanklin, J (reprint author), Brookhaven Natl Lab, Dept Biosci, 463,50 Bell Ave, Upton, NY 11973 USA. EM shanklin@bnl.gov RI Schwender, Jorg/P-2282-2014 OI Schwender, Jorg/0000-0003-1350-4171 FU Office of Basic Energy Sciences of the U.S. Department of Energy; DOE EERE FX This work was supported by the Office of Basic Energy Sciences of the U.S. Department of Energy (JS and JS), and DOE EERE to JS, JS, YY, EE, RM and HS. We thank Dr. F. W. Studier and Dr. Xiao Hong Yu for critical reading of the manuscript and Dr. Sean McCorkle for technical assistance. NR 41 TC 5 Z9 5 U1 1 U2 41 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2229 J9 BMC PLANT BIOL JI BMC Plant Biol. PD DEC 5 PY 2013 VL 13 AR 201 DI 10.1186/1471-2229-13-201 PG 13 WC Plant Sciences SC Plant Sciences GA 281AN UT WOS:000329072000001 PM 24308551 ER PT J AU Balitsky, I Chirilli, GA AF Balitsky, Ian Chirilli, Giovanni A. TI Rapidity evolution of Wilson lines at the next-to-leading order SO PHYSICAL REVIEW D LA English DT Article ID COLOR GLASS CONDENSATE; NONLINEAR GLUON EVOLUTION; X EVOLUTION; EQUATION AB At high energies, particles move very fast, so the proper degrees of freedom for the fast gluons moving along the straight lines are Wilson-line operators-infinite gauge factors ordered along the line. In the framework of operator expansion in Wilson lines, the energy dependence of the amplitudes is determined by the rapidity evolution of Wilson lines. We present the next-to-leading order hierarchy of the evolution equations for Wilson-line operators. C1 [Balitsky, Ian] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Balitsky, Ian] Jlab, Theory Grp, Newport News, VA 23606 USA. [Chirilli, Giovanni A.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. RP Balitsky, I (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. EM balitsky@jlab.org; chirilli.1@asc.ohio-state.edu FU Jefferson Science Associates, LLC [DE-AC05-06OR23177]; U.S. Department of Energy [DE-SC0004286] FX The authors are grateful to A. Grabovsky, H. Weigert, and M. Lublinsky for valuable discussions. This work was supported by Contract No. DE-AC05-06OR23177, under which the Jefferson Science Associates, LLC operate the Thomas Jefferson National Accelerator Facility and by the U.S. Department of Energy under Grant No. DE-SC0004286. NR 32 TC 32 Z9 32 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 5 PY 2013 VL 88 IS 11 AR 111501 DI 10.1103/PhysRevD.88.111501 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274JX UT WOS:000328603700002 ER PT J AU Weninger, C Purvis, M Ryan, D London, RA Bozek, JD Bostedt, C Graf, A Brown, G Rocca, JJ Rohringer, N AF Weninger, Clemens Purvis, Michael Ryan, Duncan London, Richard A. Bozek, John D. Bostedt, Christoph Graf, Alexander Brown, Gregory Rocca, Jorge J. Rohringer, Nina TI Stimulated Electronic X-Ray Raman Scattering SO PHYSICAL REVIEW LETTERS LA English DT Article ID EMISSION SPECTROSCOPY; LASER; RADIATION; REGIME; EXCITATIONS; IONIZATION; OPERATION AB We demonstrate strong stimulated inelastic x-ray scattering by resonantly exciting a dense gas target of neon with femtosecond, high-intensity x-ray pulses from an x-ray free-electron laser (XFEL). A small number of lower energy XFEL seed photons drive an avalanche of stimulated resonant inelastic x-ray scattering processes that amplify the Raman scattering signal by several orders of magnitude until it reaches saturation. Despite the large overall spectral width, the internal spiky structure of the XFEL spectrum determines the energy resolution of the scattering process in a statistical sense. This is demonstrated by observing a stochastic line shift of the inelastically scattered x-ray radiation. In conjunction with statistical methods, XFELs can be used for stimulated resonant inelastic x-ray scattering, with spectral resolution smaller than the natural width of the core-excited, intermediate state. C1 [Weninger, Clemens; Rohringer, Nina] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. [Weninger, Clemens; Rohringer, Nina] Ctr Free Electron Laser Sci, D-22761 Hamburg, Germany. [Purvis, Michael; Ryan, Duncan; Rocca, Jorge J.] Colorado State Univ, Ft Collins, CO 80523 USA. [London, Richard A.; Graf, Alexander; Brown, Gregory] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Bozek, John D.; Bostedt, Christoph] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA. RP Weninger, C (reprint author), Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. EM nina@pks.mpg.de RI Bozek, John/E-9260-2010; Rohringer, Nina/N-3238-2014; OI Bozek, John/0000-0001-7486-7238; Rohringer, Nina/0000-0001-7905-3567; Ryan, Duncan/0000-0001-7702-8499 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy, Office of Science, Basic Energy Sciences AMOS Program FX , Portions of this work were carried out at the Linac Coherent Light Source, a national user facility operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Science. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory (Contract No. DE-AC52-07NA27344). Support for the work of M. P., D. R., and J. J. R. by the U.S. Department of Energy, Office of Science, Basic Energy Sciences AMOS Program is acknowledged. We thank J. Nilsen and Chul-Min Kim for discussions, J. Dunn for filters, J.-C. Castagna, M. L. Swiggers, M. Messerschmidt, C.-M. Tsai, and S. F. Carron-Montero for their assistance with the experiment, and M. J. Bogan and H. Chapman for the loan of an x-ray CCD camera. We are indebted to the LCLS operating team for their excellent support during beam time. NR 49 TC 35 Z9 35 U1 9 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 5 PY 2013 VL 111 IS 23 AR 233902 DI 10.1103/PhysRevLett.111.233902 PG 5 WC Physics, Multidisciplinary SC Physics GA 274OY UT WOS:000328617100001 PM 24476271 ER PT J AU Ovchinnikov, YN Kresin, VZ AF Ovchinnikov, Yurii N. Kresin, Vladimir Z. TI Networks of Josephson junctions and their synchronization SO PHYSICAL REVIEW B LA English DT Article ID PHASE-LOCKING; ARRAYS; STATE AB One can demonstrate that a 1D Josephson network containing junctions with different tunneling resistances can be synchronized at frequencies, which are multiples of 2eV, where V is the total dc voltage applied across the network. The appearance of such synchronization follows from the law of charge conservation and takes place if charge transfer is dominated by the Josephson channel. One can observe also a subharmonic structure. The result holds for cluster-based arrays as well as for the general case of a tunneling network. C1 [Ovchinnikov, Yurii N.] L Landau Inst Theoret Phys, Moscow 117334, Russia. [Ovchinnikov, Yurii N.] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. [Kresin, Vladimir Z.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. RP Ovchinnikov, YN (reprint author), L Landau Inst Theoret Phys, Moscow 117334, Russia. FU EOARD [097006] FX The authors are grateful to R. Dynes and S. Cybart for fruitful discussions. The research of Y.N.O. is supported by EOARD under Contract No. 097006. NR 17 TC 4 Z9 4 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 5 PY 2013 VL 88 IS 21 AR 214504 DI 10.1103/PhysRevB.88.214504 PG 4 WC Physics, Condensed Matter SC Physics GA 274AF UT WOS:000328576700002 ER PT J AU Petri, A Haiman, Z Hui, L May, M Kratochvil, JM AF Petri, Andrea Haiman, Zoltan Hui, Lam May, Morgan Kratochvil, Jan M. TI Cosmology with Minkowski functionals and moments of the weak lensing convergence field SO PHYSICAL REVIEW D LA English DT Article ID LARGE-SCALE STRUCTURE; NON-GAUSSIANITY; COSMIC SHEAR; UNIVERSE; STATISTICS; TOPOLOGY; PROBE AB We compare the efficiency of moments and Minkowski functionals (MFs) in constraining the subset of cosmological parameters (Omega(m), omega, sigma(8)) using simulated weak lensing convergence maps. We study an analytic perturbative expansion of the MFs [T. Matsubara, Phys. Rev. D 81, 083505 (2010); D. Munshi et al., Mon. Not. R. Astron. Soc. 419, 536 (2012)] in terms of the moments of the convergence field and of its spatial derivatives. We show that this perturbation series breaks down on smoothing scales below 5', while it shows a good degree of convergence on larger scales (similar to 15'). Most of the cosmological distinguishing power is lost when the maps are smoothed on these larger scales. We also show that, on scales comparable to 10, where the perturbation series does not converge, cosmological constraints obtained from the MFs are approximately 1.5-2 times better than the ones obtained from the first few moments of the convergence distribution-provided that the latter include spatial information, either from moments of gradients or by combining multiple smoothing scales. Including a set of either these moments or the MFs can significantly tighten constraints on cosmological parameters, compared to the conventional method of using the power spectrum alone. C1 [Petri, Andrea; Hui, Lam] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Petri, Andrea; May, Morgan] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Haiman, Zoltan; Hui, Lam] Columbia Univ, Dept Astron, New York, NY 10027 USA. [Kratochvil, Jan M.] Univ Miami, Dept Phys, Coral Gables, FL 33146 USA. [Kratochvil, Jan M.] Univ KwaZulu Natal, Astrophys & Cosmol Res Unit, ZA-4000 Durban, South Africa. RP Petri, A (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. EM apetri@phys.columbia.edu FU State of New York; U.S. Department of Energy [DE-AC02-98CH10886, DE-FG02-92-ER40699]; NSF [AST-1210877]; NASA [NNX10AN14G] FX We thank Deepak Munshi and Kevin Huffenberger for useful discussions. We thank the referee for the insightful comments. This research utilized resources at the New York Center for Computational Sciences, a cooperative effort between Brookhaven National Laboratory and Stony Brook University, supported in part by the State of New York. This work is supported in part by the U.S. Department of Energy under Contracts No. DE-AC02-98CH10886 and No. DE-FG02-92-ER40699, by the NSF under Grant No. AST-1210877, and by NASA under Grant No. NNX10AN14G. NR 36 TC 17 Z9 17 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD DEC 5 PY 2013 VL 88 IS 12 AR 123002 DI 10.1103/PhysRevD.88.123002 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274KB UT WOS:000328604100001 ER PT J AU Macridin, A Spentzouris, P Amundson, J AF Macridin, Alexandru Spentzouris, Panagiotis Amundson, James TI Nonperturbative algorithm for the resistive wall impedance of general cross-section beam pipes SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID COUPLING IMPEDANCE AB We present an algorithm for calculating the impedance of infinitely long beam pipes with arbitrary cross section. The method is not restricted to ultrarelativistic beams or perturbative approximations with respect to the wall surface impedance or skin penetration depth. We exemplify our algorithm with a calculation of the impedance for rectangular metallic beam pipes. Unlike the situation in the perturbative regime, where the beam pipe geometry modifies the metallic resistive wall impedances by only a multiplicative factor, the beam pipe geometry has a more complex influence on the impedance when nonultrarelativistic effects are significant and in the ultrarelativistic regime at both small and large frequencies. Since our algorithm requires the boundary conditions at the beam pipe wall to be provided as linear relations between the transverse components of the electromagnetic field, we discuss a general algorithm to calculate these boundary conditions for multilayer beam pipes with arbitrary cross section. C1 [Macridin, Alexandru; Spentzouris, Panagiotis; Amundson, James] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Macridin, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. FU United States Department of Energy [De-AC02-07CH11359]; ComPASS project; Scientific Discovery through Advanced Computing program in the DOE Office of High Energy Physics FX This work was performed at Fermilab, operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. It was also supported by the ComPASS project, funded through the Scientific Discovery through Advanced Computing program in the DOE Office of High Energy Physics. NR 25 TC 3 Z9 3 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD DEC 5 PY 2013 VL 16 IS 12 AR 121001 DI 10.1103/PhysRevSTAB.16.121001 PG 14 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 274PS UT WOS:000328619100001 ER PT J AU Polino, D Klippenstein, SJ Harding, LB Georgievskii, Y AF Polino, Daniela Klippenstein, Stephen J. Harding, Lawrence B. Georgievskii, Yuri TI Predictive Theory for the Addition and Insertion Kinetics of (CH2)-C-1 Reacting with Unsaturated Hydrocarbons SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MULTIREFERENCE PERTURBATION-THEORY; RESONANCE-STABILIZED RADICALS; FLEXIBLE TRANSITION-STATES; SINGLET METHYLENE REMOVAL; BENZYL DECOMPOSITION; ELEMENTARY REACTIONS; AB-INITIO; AROMATIC-HYDROCARBONS; THERMAL-DECOMPOSITION; CORRELATION-ENERGY AB The reactions of singlet methylene, (CH2)-C-1, with unsaturated hydrocarbons are of considerable significance to the formation and growth of polycyclic aromatic hydrocarbons (PAHs). In this work, we employ high level ab initio transition state theory to predict the high pressure rate coefficient for singlet methylene reacting with acetylene (C2H2), ethylene (C2H4), propyne (CH3CCH), propene (CH3CHCH2), allene (CH2CCH2), 1,3-butadiene (CH2CHCHCH2), 2-butyne (CH3CCCH3), and benzene (C6H6). Both addition and insertion channels are found to contribute significantly to the kinetics, with the insertion kinetics of increasing importance for larger hydrocarbons due to the increasing number of CH bonds and increasingly attractive interactions. We treat the addition kinetics with direct CASPT2 based variable-reaction-coordinate transition state theory. One-dimensional corrections to the CASPT2 interaction energies are obtained from geometry relaxation calculations and CCSD(T)/CBS evaluations. The insertion kinetics is treated with traditional variational TST methods employing CCSD(T)/CBS energies obtained along the CASPT2/cc-pVTZ distinguished coordinate reaction paths. The overall rate constant and branching fractions are obtained from a multiple transition state model that accounts for the physical distinction between tight inner and loose outer transition states. The predicted rate constants, which cover the range from 200 to 2000 K, are found to be in excellent agreement with the available experimental data, with a maximum observed discrepancy of about 40%. C1 [Polino, Daniela; Klippenstein, Stephen J.; Harding, Lawrence B.; Georgievskii, Yuri] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Polino, Daniela] Politecn Milan, Dipartimento Chim Mat & Ingn Chim G Natta, I-20131 Milan, Italy. RP Klippenstein, SJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. OI Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX The work at Argonne was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract No. DE-AC02-06CH11357. NR 73 TC 8 Z9 8 U1 1 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD DEC 5 PY 2013 VL 117 IS 48 BP 12677 EP 12692 DI 10.1021/jp406246y PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 267MB UT WOS:000328100800001 PM 24093491 ER PT J AU Chatterjee, S Del Negro, AS Smith, FN Wang, ZM Hightower, SE Sullivan, BP Heineman, WR Seliskar, CJ Bryan, SA AF Chatterjee, Sayandev Del Negro, Andrew S. Smith, Frances N. Wang, Zheming Hightower, Sean E. Sullivan, B. Patrick Heineman, William R. Seliskar, Carl J. Bryan, Samuel A. TI Photophysics and Luminescence Spectroelectrochemistry of [Tc(dmpe)(3)](+/2+) (dmpe=1,2-bis(dimethylphosphino)ethane) SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID DENSITY-FUNCTIONAL THEORY; RUTHENIUM DIIMINE COMPLEXES; MOLECULAR-ORBITAL METHODS; ELECTRON-TRANSFER; TECHNETIUM COMPLEXES; EXCITED-STATE; URANYL-ION; FLUORESCENCE; PHOTOCHEMISTRY; POTENTIALS AB The ligand-to-metal charge transfer (LMCT) excited state luminescence of [Tc(dmpe)(3)](2+) (dmpe is 1,2-bis(dimethylphosphino)ethane) has been measured in solution at room temperature and is compared to its Re analogue. Surprisingly, both [M(dmpe)(3)](2+)* (M = Re, Tc) species have extremely large excited-state potentials (ESPs) as oxidants, the highest for any simple coordination complex of a transition metal. Furthermore, this potential is available using a photon of visible light (calculated for M = Tc; E degrees'* = +2.48 V versus SCE; lambda(max) = 585 nm). Open shell time-dependent density functional theory (TDDFT) calculations support the assignment of the lowest energy transition in both the technetium and rhenium complexes to be a doublet-doublet process that involves predominantly LMCT (dmpe-to-metal) character and is in agreement with past assignments for the Re system. As expected for highly oxidizing excited state potentials, quenching is observed for the excited states of both the rhenium and technetium complexes. Stern-Volmer analysis resulted in quenching parameters for both the rhenium and technetium complexes under identical conditions and are compared using Rehm-Weller analysis. Of particular interest is the fact that both benzene and toluene are oxidized by both the Re and Tc systems. C1 [Chatterjee, Sayandev; Del Negro, Andrew S.; Smith, Frances N.; Hightower, Sean E.; Bryan, Samuel A.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Wang, Zheming] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Sullivan, B. Patrick] Univ Wyoming, Dept Chem, Laramie, WY 82071 USA. [Heineman, William R.; Seliskar, Carl J.] Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA. RP Seliskar, CJ (reprint author), Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA. EM seliskcj@ucmail.uc.edu; Sam.Bryan@pnnl.gov RI Wang, Zheming/E-8244-2010; Bryan, Samuel/D-5457-2015; OI Wang, Zheming/0000-0002-1986-4357; Bryan, Samuel/0000-0001-5664-3249; Chatterjee, Sayandev/0000-0003-2218-5635 FU Office of Biological and Environmental Research (OBER) of the U.S. Department of Energy [DE-FG0799ER62331]; U.S. Department of Energy by Battelle [DE-AC06-76RLO 1830] FX Support from the Office of Biological and Environmental Research (OBER) of the U.S. Department of Energy (Grant DE-FG0799ER62331) is greatly acknowledged. Part of this research was performed at EMSL, a national scientific user facility at PNNL managed by the Department of Energy's Office of Biological and Environmental Research. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle under Contract DE-AC06-76RLO 1830. NR 46 TC 3 Z9 3 U1 1 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD DEC 5 PY 2013 VL 117 IS 48 BP 12749 EP 12758 DI 10.1021/jp406365c PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 267MB UT WOS:000328100800008 PM 24256024 ER PT J AU Koziol, L Kumar, N Wong, SE Lightstone, FC AF Koziol, Lucas Kumar, Neeraj Wong, Sergio E. Lightstone, Felice C. TI Molecular Recognition of Aromatic Rings by Flavin: Electrostatics and Dispersion Determine Ring Positioning above Isoalloxazine SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID FRAGMENT POTENTIAL METHOD; PI-PI-INTERACTIONS; FERREDOXIN-NADP(+) REDUCTASE; INTERACTION ENERGIES; CRYSTAL-STRUCTURE; BENZENE-PYRIDINE; MODEL SYSTEMS; DNA-REPAIR; CHEMISTRY; DIMER AB Aromatic stacking interactions between isoalloxazine (ISA) of flavin and three prototypical aromatics (benzene, pyridine, chlorobenzene) were investigated using electronic structure calculations with Monte Carlo simulated annealing. The Effective Fragment Potential (EFP) method was used to locate the low-energy equilibrium configurations for the three dimer systems. These structures were further characterized through DFT (M06-2X) and MP2 calculations. One equilibrium configuration exists for ISA-benzene; characterizing the stacked dimer surface revealed a steep, single-welled potential that funnels benzene directly between rings II and III, positioning a substituent hydrogen adjacent to the redox-active N5. ISA-pyridine and ISA-chlorobenzene minimum-energy structures contain the aromatic ring in very similar position to that in ISA-benzene. However, the added rotational degree of freedom leads to two distinct binding motifs, having approximately antiparallel or parallel dipole moment alignment with ISA. The existence of the latter binding configuration was unexpected but is explained by the shape of the ISA electrostatic potential. Dispersion is the primary noncovalent interaction driving the positioning of aromatic rings above ISA, while electrostatics determine the orientation in dipole-containing substituted benzenes. The interplay of these interactions can be used to tune molecular recognition properties of synthetic redox cofactors, including positioning desired functional groups adjacent to the redox-active N5. C1 [Koziol, Lucas; Wong, Sergio E.; Lightstone, Felice C.] Lawrence Livermore Natl Lab, Phys & Life Sci Div, Livermore, CA 94550 USA. [Kumar, Neeraj] Univ Louisville, Dept Chem, Louisville, KY 40208 USA. RP Lightstone, FC (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Div, 7000 East Ave, Livermore, CA 94550 USA. EM lightstone1@llnl.gov RI Kumar, Neeraj/M-3279-2015 OI Kumar, Neeraj/0000-0001-6713-2129 FU Defense Threat Reduction Agency [CBM.THERB.02.11.LLNL.047]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-ACS2-07NA27344] FX We thank the Defense Threat Reduction Agency for funding (CBM.THERB.02.11.LLNL.047). We also thank Livermore Computing for the computer time. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-ACS2-07NA27344. NR 38 TC 3 Z9 3 U1 3 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD DEC 5 PY 2013 VL 117 IS 48 BP 12946 EP 12952 DI 10.1021/jp407193c PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 267MB UT WOS:000328100800028 PM 24229368 ER PT J AU He, QP Suraweera, NS Joy, DC Keffer, DJ AF He, Qianping Suraweera, Nethika S. Joy, David C. Keffer, David J. TI Structure of the lonomer Film in Catalyst Layers of Proton Exchange Membrane Fuel Cells SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY-SCATTERING; PERFLUORINATED IONOMER MEMBRANES; MOLECULAR-DYNAMICS SIMULATION; SUPPORTED PLATINUM CATALYST; PERFLUOROSULFONIC ACID MEMBRANES; POLYMER ELECTROLYTE MEMBRANES; OXYGEN REDUCTION REACTION; ELECTROCHEMICAL OXIDATION; NANOPARTICLE ADHESION; PT3CO NANOPARTICLES AB The nanoscale structure of the ionomer film located in the catalyst layer of polymer exchange membrane fuel cells (PEMFCs) is of vital importance to proton transport and catalyst utilization. Classical molecular dynamic simulations are conducted to explore the molecular-level structure as well as the structure-property relationships in the ionomer film. Twenty-four systems are simulated to investigate the effect of (i) hydration, (ii) ionomer film thickness, (iii) oxidation of the carbon support surface, and (iv) the presence of catalyst nanoparticles on film adhesion and morphology. The ionomer does not form a continuous film on the carbon surface; rather, the ionomer forms irregular patches through which proton transport from the catalyst to the membrane must occur. These ionomer films are not able to retain water to the same extent as bulk ionomer membranes. However, thicker films retain proportionally more water than thinner films, allowing for a larger and better connected aqueous domain required for proton transport. Oxidation of the carbon support surface through either epoxidation or hydroxylation strongly impacts the water distribution throughout the film and thus the film adhesion. Hydroxylation enhances adhesion of the film relative to a pristine surface. Epoxidation can result in partial delamination of the film, an effect that is more pronounced for thinner films. The presence of Pt or PtO nanoparticles impacts the distribution of water and the ionomer. An aqueous layer forms around the nanoparticles and provides pathways for protons into the film. These insights provide a molecular-level basis for the experimental observations such as the inhomogeneous distribution of the Nafion film on the carbon support, the existence of an optimal content of recast ionomer in the catalyst layer, and the impact of surface oxidation on the restructuring of polymer chains and thus on PEMFC performance. This work also implies that oxidation during operation can result in ionomer film delamination, which reduces the binding energy of the catalysts, a possible precursor to catalyst detachment. C1 [He, Qianping; Suraweera, Nethika S.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Joy, David C.; Keffer, David J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Joy, David C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Keffer, DJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM dkeffer@utk.edu RI Keffer, David/C-5133-2014 OI Keffer, David/0000-0002-6246-0286 FU Sustainable Energy and Education Research Center at the University of Tennessee; National Science Foundation [DGE-0801470]; NSF [OCI 07-11134.5] FX This research was supported by the Sustainable Energy and Education Research Center at the University of Tennessee and by a grant from the National Science Foundation (DGE-0801470). This research project used resources of the National Institute for Computational Sciences (NICS) supported by NSF under Agreement Number OCI 07-11134.5. NR 85 TC 13 Z9 13 U1 9 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 5 PY 2013 VL 117 IS 48 BP 25305 EP 25316 DI 10.1021/jp408653f PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 267ME UT WOS:000328101200011 ER PT J AU Nie, MY Abraham, DP Seo, DM Chen, YJ Bose, A Lucht, BL AF Nie, Mengyun Abraham, Daniel P. Seo, Daniel M. Chen, Yanjing Bose, Arijit Lucht, Brett L. TI Role of Solution Structure in Solid Electrolyte lnterphase Formation on Graphite with LiPF6 in Propylene Carbonate SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; LITHIUM-ION BATTERIES; LI-ION; SURFACE-FILMS; INTERPHASIAL CHEMISTRY; SOLVATION; ANODE; ACETONITRILE; INTERCALATION; DECOMPOSITION AB An investigation of the interrelationship of cycling performance, solution structure, and electrode surface film structure has been conducted for electrolytes composed of different concentrations of LiPF6 in propylene carbonate (PC) with a binder- free (BF) graphite electrode. Varying the concentration of LiPF6 changes the solution structure, altering the predominant mechanism of electrolyte reduction at the electrode interface. The change in mechanism results in a change in the structure of the solid electrolyte interface (SEI) and the reversible cycling of the cell. At low concentrations of LiPF6 in PC (1.2 M), electrochemical cycling and cyclic voltammetry (CV) of BF graphite electrodes reveal continuous electrolyte reduction and no lithiation/delithiation of the graphite. The solution structure is dominated by solvent-separated ion pairs (Li+(PC)(4)//PF6-), and the primary reduction product of the electrolyte is lithium propylene dicarbonate (LPDC). At high concentrations of LiPF6 in PC (3.0-3.5 M), electrochemical cycling and CV reveal reversible lithiation/delithiation of the graphite electrode. The solution structure is dominated by contact ion pairs (Li+(PC)(3)PF6-), and the primary reduction product of the electrolyte is LiF. C1 [Nie, Mengyun; Seo, Daniel M.; Chen, Yanjing; Bose, Arijit; Lucht, Brett L.] Univ Rhode Isl, Kingston, RI 02881 USA. [Abraham, Daniel P.] Argonne Natl Lab, Argonne, IL 60438 USA. RP Lucht, BL (reprint author), Univ Rhode Isl, Kingston, RI 02881 USA. EM blucht@chm.uri.edu RI Nie, Mengyun/F-4981-2015 OI Nie, Mengyun/0000-0002-8546-5215 FU Department of Energy Office of Basic Energy Sciences EPSCoR Implementation [DE-SC0007074] FX We gratefully acknowledge funding from the Department of Energy Office of Basic Energy Sciences EPSCoR Implementation award (DE-SC0007074). NR 42 TC 42 Z9 42 U1 4 U2 92 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 5 PY 2013 VL 117 IS 48 BP 25381 EP 25389 DI 10.1021/jp409765w PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 267ME UT WOS:000328101200020 ER PT J AU Wang, Y Lopata, K Chambers, SA Govind, N Sushko, PV AF Wang, Yong Lopata, Kenneth Chambers, Scott A. Govind, Niranjan Sushko, Peter V. TI Optical Absorption and Band Gap Reduction in (Fe1-xCrx)(2)O-3 Solid Solutions: A First-Principles Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DENSITY-FUNCTIONAL THEORY; AUGMENTED-WAVE METHOD; ELECTRONIC-STRUCTURE; BASIS-SET; TIO2; APPROXIMATION; SIMULATIONS; EXCHANGE; SPECTRUM; RUTILE AB We provide a detailed theoretical analysis of the character of optical transitions and band gap reduction in (Fe1-xCrx)(2)O-3 solid solutions using extensive periodic model and embedded cluster calculations. Time-dependent density functional theory is used to calculate and assign optical absorption bands for x = 0.0, 0.5, and 1.0 and photon energies up to 5 eV. Consistent with recent experimental data, a band gap reduction of as much as 0.7 eV with respect to that of pure alpha-Fe2O3 is found. This result is attributed predominantly to two effects: (i) the higher valence band edge for x approximate to 0.5, as compared to those in pure alpha-Fe2O3 and alpha-Cr2O3, and (ii) the onset of Cr -> Fe d-d excitations in the solid solutions. Broadening of the valence band due to hybridization of O 2p with Fe and Cr 3d states also contributes to band gap reduction. C1 [Wang, Yong; Chambers, Scott A.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Lopata, Kenneth; Govind, Niranjan] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Sushko, Peter V.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Sushko, Peter V.] UCL, London Ctr Nanotechnol, London WC1E 6BT, England. RP Sushko, PV (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM p.sushko@ucl.ac.uk RI Sushko, Peter/F-5171-2013 OI Sushko, Peter/0000-0001-7338-4146 FU U.S. Department of Energy, Office of Science, Division of Chemical Sciences, Geosciences, and Biosciences [48526]; U.S. Department of Energy's Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory (PNNL); Department of Energy by the Battelle Memorial Institute [DE-AC06-76RLO-1830]; William Wiley Postdoctoral Fellowship from EMSL; U.S. Department of Energy, Office of Basic Energy Sciences of the SciDAC program [DESC0008666]; Royal Society; EPSRC [EP/H018328/1] FX Authors thank Sara E. Chamberlin, Tiffany C. Kaspar, Daniel R. Gamelin, and Wei Li Cheah for stimulating discussions. This work was supported by the U.S. Department of Energy, Office of Science, Division of Chemical Sciences, Geosciences, and Biosciences under Award No. 48526, and was performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated for the Department of Energy by the Battelle Memorial Institute under Contract DE-AC06-76RLO-1830. K.L. acknowledges the William Wiley Postdoctoral Fellowship from EMSL. N.G. acknowledges support from the U.S. Department of Energy, Office of Basic Energy Sciences, under Grant No. DESC0008666 of the SciDAC program. P.V.S. acknowledges support from the Royal Society and EPSRC (Grant EP/H018328/1). NR 52 TC 18 Z9 18 U1 3 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 5 PY 2013 VL 117 IS 48 BP 25504 EP 25512 DI 10.1021/jp407496w PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 267ME UT WOS:000328101200034 ER PT J AU Chen, YZ Xi, XX Yim, WL Peng, F Wang, YC Wang, H Ma, YM Liu, GT Sun, CL Ma, CL Chen, ZQ Berger, H AF Chen, Yuanzheng Xi, Xiaoxiang Yim, Wai-Leung Peng, Feng Wang, Yanchao Wang, Hui Ma, Yanming Liu, Guangtao Sun, Chenglin Ma, Chunli Chen, Zhiqiang Berger, H. TI High-Pressure Phase Transitions and Structures of Topological Insulator BiTel SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SINGLE DIRAC CONE; SUPERCONDUCTIVITY; BI2TE3; SURFACE; SB2TE3; BI2SE3; MODEL AB Being a giant bulk Rashba semiconductor, the ambient-pressure phase of BiTeI was predicted to transform into a topological insulator under pressure at 1.7-4.1 GPa [Nat. Commun. 2012, 3, 679]. Because the structure governs the new quantum state of matter, it is essential to establish the high-pressure phase transitions and structures of BiTeI for better understanding its topological nature. Here, we report a joint theoretical and experimental study up to 30 GPa to uncover two orthorhombic high-pressure phases of Pnma and P4/nmm structures named phases II and III, respectively. Phases II (stable at 8.8-18.9 GPa) and III (stable at >18.9 GPa) were first predicted by our first-principles structure prediction calculations based on the calypso method and subsequently confirmed by our high-pressure powder X-ray diffraction experiment. Phase II can be regarded as a partially ionic structure, consisting of positively charged (BiTe)(+) ladders and negatively charged I- ions. Phase III is a typical ionic structure characterized by interconnected cubic building blocks of Te-Bi-I stacking. Application of pressures up to 30 GPa tuned effectively the electronic properties of BiTeI from a topological insulator to a normal semiconductor and eventually a metal having a potential of superconductivity. C1 [Chen, Yuanzheng; Peng, Feng; Wang, Yanchao; Wang, Hui; Ma, Yanming; Liu, Guangtao; Ma, Chunli] Jilin Univ, State Key Lab Superhard Mat, Changchun 130012, Peoples R China. [Chen, Yuanzheng; Sun, Chenglin] Jilin Univ, Coll Phys, Changchun 130012, Peoples R China. [Xi, Xiaoxiang] Brookhaven Natl Lab, Upton, NY 11973 USA. [Yim, Wai-Leung] Agcy Sci Technol & Res, Inst High Performance Comp, Singapore 138632, Singapore. [Ma, Chunli] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Chen, Zhiqiang] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Berger, H.] Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland. RP Wang, YC (reprint author), Jilin Univ, State Key Lab Superhard Mat, Changchun 130012, Peoples R China. EM wyc@calypso.cn; mym@calypso.cn RI Wang, Hui/B-1302-2012; Ma, Yanming/A-7297-2008; Ma, Yanming/A-4982-2009; Wang, Yanchao/A-6634-2015 OI Ma, Yanming/0000-0003-3711-0011; FU China 973 Program [2011CB808200]; Natural Science Foundation of China (NSFC) [51202084, 11274136, 11104104, 11025418, 91022029]; NSFC [11250110051]; Changjiang Scholars Program of China, Changjiang Scholar; Innovative Research Team in University [IRT1132]; U.S. Department of Energy [DE-AC02-98CH10886]; COMPRES (the Consortium for Materials Properties Research in Earth Sciences) under NSF [EAR 11-57758] FX This work is supported by the China 973 Program (2011CB808200), Natural Science Foundation of China (NSFC) under 51202084, 11274136, 11104104, 11025418, and 91022029, NSFC awarded Research Fellowship for International Young Scientists under Grant No. 11250110051, the 2012 Changjiang Scholars Program of China, Changjiang Scholar, and the Innovative Research Team in University (IRT1132). The authors also acknowledge the High Performance Computing Center of Jilin University for supercomputer time. The work at BNL was also supported by the U.S. Department of Energy through Contract DE-AC02-98CH10886. The use of the X17C beamline was partially supported by COMPRES (the Consortium for Materials Properties Research in Earth Sciences) under NSF Cooperative Agreement EAR 11-57758. NR 39 TC 18 Z9 19 U1 5 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 5 PY 2013 VL 117 IS 48 BP 25677 EP 25683 DI 10.1021/jp409824g PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 267ME UT WOS:000328101200054 ER PT J AU Zhou, J Huang, JS Sumpter, BG Kent, PRC Terrones, H Smith, SC AF Zhou, Jia Huang, Jingsong Sumpter, Bobby G. Kent, Paul R. C. Terrones, Humberto Smith, Sean C. TI Structures, Energetics, and Electronic Properties of Layered Materials and Nanotubes of Cadmium Chalcogenides SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INITIO MOLECULAR-DYNAMICS; BORON-NITRIDE NANORIBBONS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CARBON NANOTUBES; SILICON-CARBIDE; BASIS-SET; GRAPHENE; PHASE; CDSE AB Geometric structures, energetics, and electronic properties of single-layer sheets, multilayer stacks, and single-walled nanotubes (SWNTs) of cadmium chalcogenides CdX (X = S, Se, Te) have been studied using ab initio density functional theory, along with spin orbit coupling, van der Waals (vdW) interactions, and the GW approximation. Methodologies applied to the rationally designed materials have been validated through the experimental structural parameters and band gaps of 3D bulk zinc blende and wurtzite phases of CdX. The 2D single-layer sheet of CdS is found to be completely planar, while those of CdSe and CdTe are slightly corrugated, all showing a honeycomb lattice. The 2D sheets are destabilized with respect to the bulk zinc blende and wurtzite phases, but can be significantly stabilized by forming 3D multilayer stacks as a result of interlayer interactions. ID (S,5) armchair and (9,0) zigzag SWNTs are also stabilized from their single-layer sheet counterparts. Both SWNTs consist of two concentric cylinders, with the Cd and X atoms in the inner and the outer cylinders, respectively, and with the intercylinder separations showing the same trend as the degree of nonplanarity in the single-layer sheets. By analogy to quantum dots of CdX, we suggest quantum flakes as interesting targets for experimental synthesis due to the diverse band gaps complementary to those of the bulk phases, allowing a much wider wavelength range, from infrared, visible, to ultraviolet, to be utilized. C1 [Zhou, Jia; Huang, Jingsong; Sumpter, Bobby G.; Kent, Paul R. C.; Terrones, Humberto; Smith, Sean C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Huang, Jingsong; Sumpter, Bobby G.; Kent, Paul R. C.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Zhou, J (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM zhouj1@ornl.gov; smithsc@ornl.gov RI Kent, Paul/A-6756-2008; Sumpter, Bobby/C-9459-2013; Huang, Jingsong/A-2789-2008; Smith, Sean/H-5003-2015 OI Kent, Paul/0000-0001-5539-4017; Sumpter, Bobby/0000-0001-6341-0355; Huang, Jingsong/0000-0001-8993-2506; Smith, Sean/0000-0002-5679-8205 FU Office of Science of the U.S. Department of Energy [DE-AC05-00OR22750, DE-AC02-05CH11231]; Center for Nanophase Materials Sciences; ORNL by the Scientific User Facilities Division, U.S. Department of Energy FX This work used computational resources of the National Center for Computational Sciences at Oak Ridge National laboratory and of the National Energy Research Scientific Computing Center, which are supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22750 and DE-AC02-05CH11231, respectively. We also acknowledge the support from the Center for Nanophase Materials Sciences, which is sponsored at ORNL by the Scientific User Facilities Division, U.S. Department of Energy. NR 63 TC 10 Z9 10 U1 4 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD DEC 5 PY 2013 VL 117 IS 48 BP 25817 EP 25825 DI 10.1021/jp409772r PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 267ME UT WOS:000328101200070 ER PT J AU Knesting, KM Ju, HX Schlenker, CW Giordano, AJ Garcia, A Smith, OL Olson, DC Marder, SR Ginger, DS AF Knesting, Kristina M. Ju, Huanxin Schlenker, Cody W. Giordano, Anthony J. Garcia, Andres Smith, O'Neil L. Olson, Dana C. Marder, Seth R. Ginger, David S. TI ITO Interface Modifiers Can Improve V-OC in Polymer Solar Cells and Suppress Surface Recombination SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID OPEN-CIRCUIT VOLTAGE; INDIUM-TIN OXIDE; SELF-ASSEMBLED MONOLAYERS; WORK FUNCTION; ORGANIC PHOTOVOLTAICS; PHOSPHONIC-ACIDS; TRANSPORT LAYERS; METAL-OXIDE; EFFICIENCY; DEVICES AB We use dipolar phosphonic acid self-assembled monolayers (PA SAMs) to modify the work function of the hole-extracting contact in polymer/fullerene bulk heterojunction solar cells. We observe a linear dependence of the open-circuit voltage (V-OC) of these organic photovoltaic devices on the modified indium tin oxide (ITO) work function when using a donor polymer with a deep-lying ionization energy. With specific SAMs, we can obtain V-OC values exceeding those obtained with the common poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate) (PEDOT:PSS) hole-extraction layer. We measure charge-carrier lifetimes and densities using transient photovoltage and charge extraction in a series of devices with SAM-modified contacts. As expected, these measurements show systematically longer carrier lifetimes in devices with higher V-OC values; however, the trends provide useful distinctions between different hypotheses of how transient photovoltage decays might be controlled by surface chemistry. We interpret our results as being consistent with changes in the band bending at the ITO/bulk heterojunction interface that have the net result of altering the internal electric field to help prevent electrons in fullerene domains from undergoing surface recombination at the hole-extracting electrode. C1 [Knesting, Kristina M.; Ju, Huanxin; Schlenker, Cody W.; Ginger, David S.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Giordano, Anthony J.; Smith, O'Neil L.; Marder, Seth R.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Giordano, Anthony J.; Smith, O'Neil L.; Marder, Seth R.] Georgia Inst Technol, Ctr Organ Photon & Elect, Atlanta, GA 30332 USA. [Garcia, Andres; Olson, Dana C.] Natl Ctr Photovolta, Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ju, Huanxin] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China. RP Ginger, DS (reprint author), Univ Washington, Dept Chem, Seattle, WA 98195 USA. EM ginger@chem.washington.edu RI Zhou, David/N-5367-2015; Ginger, David/C-4866-2011 OI Ginger, David/0000-0002-9759-5447 FU Center for Interface Science: Solar-Electric Materials (CIS:SEM), an Energy Frontier Research Center; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0001084]; National Defense Science and Engineering Graduate Fellowship program; NSF graduate research fellowship [DGE-0644493]; Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF) [DE-AC05-06OR23100]; NSF [DMR-1215753] FX K.M.K. and C.W.S. thank Roy Olund and the University of Washington Chemistry Electronics shop as well as Dr. Rajiv Giridharagopal and Dr. Jennifer Chen for circuit and programming expertise. This paper is based on research partially supported by the Center for Interface Science: Solar-Electric Materials (CIS:SEM), an Energy Frontier Research Center funded through the U.S. Department of Energy, Office of Basic Energy Sciences, under Award Number DE-SC0001084 (K.M.K., A.J.G., A.G., D.C.O., S.R.M., D.S.G.), and the National Defense Science and Engineering Graduate Fellowship program and NSF graduate research fellowship DGE-0644493 (A.J.G.). K.M.K. acknowledges graduate fellowship support from the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under contract no. DE-AC05-06OR23100. C.W.S. was supported by NSF DMR-1215753. NR 63 TC 45 Z9 45 U1 3 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD DEC 5 PY 2013 VL 4 IS 23 BP 4038 EP 4044 DI 10.1021/jz4021525 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 267MC UT WOS:000328101000004 ER PT J AU Akgul, FA Gumus, C Er, AO Farha, AH Akgul, G Ufuktepe, Y Liu, Z AF Akgul, Funda Aksoy Gumus, Cebrail Er, Ali O. Farha, Ashraf H. Akgul, Guvenc Ufuktepe, Yuksel Liu, Zhi TI Structural and electronic properties of SnO2 SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Thin films; Crystal structure; Electronic properties; Optical properties; Synchrotron radiation; X-ray diffraction ID DEPOSITED TIN OXIDE; CHEMICAL-VAPOR-DEPOSITION; X-RAY-PHOTOEMISSION; THIN-FILMS; OPTICAL-PROPERTIES; SPRAY-PYROLYSIS; CORE-LEVEL; TRANSPARENT CONDUCTORS; ION-BOMBARDMENT; DOPED SNO2 AB Highly transparent polycrystalline thin film of SnO2 (tin dioxide) was deposited using a simple and low cost spray pyrolysis method. The film was prepared from an aqueous solution of tin tetrachloride (stannic chloride) onto glass substrates at 400 degrees C. A range of diagnostic techniques including X-ray diffraction (XRD), UV-visible absorption, atomic force microscopy (AFM), scanning electron microscopy (SEM), and synchrotron-based X-ray photoelectron spectroscopy (XPS) were used to investigate structural, optical, and electronic properties of the resulting film. Deposited film was found to be polycrystalline. A mixture of SnO and SnO2 phases was observed. The average crystallite size of similar to 21.3 nm for SnO2 was calculated by Rietveld method using XRD data. The oxidation states of the SnO2 thin film were confirmed by the shape analysis of corresponding XPS O 1s, Sn 3d, and Sn 4d peaks using the decomposition procedure. The analysis of the XPS core level peaks showed that the chemical component is non-stoichiometric and the ratio of oxygen to tin (O/Sn) is 1.85 which is slightly under stoichiometry. (c) 2013 Elsevier B.V. All rights reserved. C1 [Akgul, Funda Aksoy] Nigde Univ, Dept Phys, TR-51240 Nigde, Turkey. [Gumus, Cebrail; Ufuktepe, Yuksel] Cukurova Univ, Dept Phys, TR-01330 Adana, Turkey. [Er, Ali O.] Univ Calif Irvine, Dept Chem, Irvine, CA 92612 USA. [Farha, Ashraf H.] Old Dominion Univ, Norfolk, VA 23529 USA. [Akgul, Guvenc] Nigde Univ, Bor Vocat Sch, TR-51700 Nigde, Turkey. [Akgul, Funda Aksoy; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Farha, Ashraf H.] Ain Shams Univ, Dept Phys, Cairo 11566, Egypt. RP Akgul, FA (reprint author), Nigde Univ, Dept Phys, TR-51240 Nigde, Turkey. EM fundaaksoy01@gmail.com; cgumus@cu.edu.tr RI Liu, Zhi/B-3642-2009 OI Liu, Zhi/0000-0002-8973-6561 FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The authors are grateful to the Advanced Light Source, Berkeley, California USA for providing synchrotron-based XPS facility. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 57 TC 13 Z9 14 U1 5 U2 185 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 J9 J ALLOY COMPD JI J. Alloy. Compd. PD DEC 5 PY 2013 VL 579 BP 50 EP 56 DI 10.1016/j.jallcom.2013.05.057 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 219QN UT WOS:000324523500010 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F Da Costa, JBG Bartoldus, R Barton, AE Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buehrer, F Bugge, L Bulekov, O Bundock, AC Bunse, M Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Buscher, V Bussey, P Buszello, CP Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D 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Wolter, M. W. Wolters, H. Wong, W. C. Wooden, G. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wraight, K. Wright, M. Wrona, B. Wu, S. L. Wu, X. Wu, Y. Wulf, E. Wyatt, T. R. Wynne, B. M. Xella, S. Xiao, M. Xu, C. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yamada, M. Yamaguchi, H. Yamaguchi, Y. Yamamoto, A. Yamamoto, K. Yamamoto, S. Yamamura, T. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, U. K. Yang, Y. Yang, Z. Yanush, S. Yao, L. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yen, A. L. Yildirim, E. Yilmaz, M. Yoosoofmiya, R. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. Yuan, L. Yurkewicz, A. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zambito, S. Zanello, L. Zanzi, D. Zaytsev, A. Zeitnitz, C. Zeman, M. Zemla, A. Zenin, O. Zenis, T. Zerwas, D. della Porta, G. Zevi Zhang, D. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurement of Top Quark Polarization in Top-Antitop Events from Proton- Proton Collisions at root s=7 TeV Using the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID PAIR PRODUCTION; DECAY AB This Letter presents measurements of the polarization of the top quark in top-antitop quark pair events, using 4: 7 fb(-1) of proton-proton collision data recorded with the ATLAS detector at the Large Hadron Collider at root s = 7 TeV. Final states containing one or two isolated leptons ( electrons or muons) and jets are considered. Two measurements of alpha P-l, the product of the leptonic spin-analyzing power and the top quark polarization, are performed assuming that the polarization is introduced by either a CP conserving or a maximally CP violating production process. The measurements obtained, alpha P-l(CPC) = -0: 035 +/- 0: 014(stat) +/- 0: 037(syst) and alpha P-l(CPV) = 0: 020 +/- 0: 016(stat)(-0.017)(+0.013)(syst), are in good agreement with the standard model prediction of negligible top quark polarization. C1 [Jackson, P.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. 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R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Backes, M.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. 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A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salek, D.; Salzburger, A.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Huang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Milan, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hillert, S.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Ahmad, A.; Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Armbruster, A. J.; Brock, R.; Bromberg, C.; Caughron, S.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Hauser, R.; Hayden, D.; Holzbauer, J. L.; Huston, J.; Koll, J.; Levin, D.; Li, X.; Linnemann, J. T.; Liu, L.; Martin, B.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Pope, B. G.; Qian, J.; Scheirich, D.; Schwienhorst, R.; Searcy, J.; Stelzer, B.; Thun, R. P.; Tollefson, K.; True, P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Xu, L.; Zhang, D.; Zhang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Ge, P.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Messina, A.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Solodkov, A. A.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Ahmad, A.; Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. 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M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Dos Santos, D. Roda; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. 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[Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, Lphea Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Mountricha, E.; Nguyen Thi Hong, V.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, DSM IRFU, Inst Rech Lois Fondamentales Univers, F-91191 Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, A.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. 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D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Mitani, T.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Hard, A. S.; Jared, R. 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Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, IN2P3, Ctr Calcul, Villeurbanne, France. [Aguilar-Saavedra, J. A.] Kings Coll London, Dept Phys, London, England. [Apolle, R.; Davies, E.; Mattravers, C.; Nash, M.; Wielers, M.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Apolle, R.; Davies, E.; Mattravers, C.; Nash, M.; Wielers, M.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Novosibirsk State Univ, Novosibirsk 630090, Russia. 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[Nessi, M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Minho, Dept Fis, Braga, Portugal. [Pasztor, G.; Toth, J.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Peters, R. F. Y.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Purohit, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Smirnova, L. N.; Turchikhin, S.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Spousta, M.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Ventura, Andrea/A-9544-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Gabrielli, Alessandro/H-4931-2012; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Ferrando, James/A-9192-2012; Smirnova, Oxana/A-4401-2013; Deliot, Frederic/F-3321-2014; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; 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Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; EPLANET, ERC; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS., Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS., Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular, from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 51 TC 24 Z9 24 U1 8 U2 138 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. 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TI Observation of D-0-(D)over-bar(0) Mixing Using the CDF II Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID CONSTRAINTS AB We measure the time dependence of the ratio of decay rates for D-0 -> K+ pi(-) to the Cabibbo- favored decay D-0 -> K- pi(+). The charge conjugate decays are included. A signal of 3: 3 x 10(4) D*(+) -> pi D-+(0), D-0 -> K+ pi(-) decays is obtained with D-0 proper decay times between 0.75 and 10 mean D-0 lifetimes. The data were recorded with the CDF II detector at the Fermilab Tevatron and correspond to an integrated luminosity of 9: 6 fb(-1) for p (p) over bar collisions at root s = 1: 96 TeV. Assuming CP conservation, we search for D-0-(D) over bar (0) mixing and measure the mixing parameters to be R-D = (3: 51 +/- 0: 35) x 10(-3), y' = (4: 3 +/- 4: 3) x 10(-3), and x'(2) = (0: 08 +/- 0: 18) x 10(-3). 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[Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Clarke, C.; Harr, R. F.; Karchin, P. E.; Kulkarni, N.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; Kim, Soo-Bong/B-7061-2014; Robson, Aidan/G-1087-2011; maestro, paolo/E-3280-2010; Chiarelli, Giorgio/E-8953-2012; Lysak, Roman/H-2995-2014; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Cavalli-Sforza, Matteo/H-7102-2015 OI Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399; maestro, paolo/0000-0002-4193-1288; Chiarelli, Giorgio/0000-0001-9851-4816; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A.P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, U.K.; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A.P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, U.K.; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 16 TC 20 Z9 20 U1 2 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 4 PY 2013 VL 111 IS 23 AR 231802 DI 10.1103/PhysRevLett.111.231802 PG 8 WC Physics, Multidisciplinary SC Physics GA 274OQ UT WOS:000328616300011 ER PT J AU Albert, F Pollock, BB Shaw, JL Marsh, KA Ralph, JE Chen, YH Alessi, D Pak, A Clayton, CE Glenzer, SH Joshi, C AF Albert, F. Pollock, B. B. Shaw, J. L. Marsh, K. A. Ralph, J. E. Chen, Y. -H. Alessi, D. Pak, A. Clayton, C. E. Glenzer, S. H. Joshi, C. TI Angular Dependence of Betatron X-Ray Spectra from a Laser-Wakefield Accelerator SO PHYSICAL REVIEW LETTERS LA English DT Article ID THOMSON SCATTERING; ELECTRON-BEAMS; CHANNEL AB We present the first measurements of the angular dependence of the betatron x-ray spectrum produced by electrons inside the cavity of a laser-wakefield accelerator. Electrons accelerated up to 300 MeV energies produce a beam of broadband, forward-directed betatron x-ray radiation extending up to 80 keV. The angular resolved spectrum from an image plate-based spectrometer with differential filtering provides data in a single laser shot. The simultaneous spectral and spatial x-ray analysis allows for a three-dimensional reconstruction of electron trajectories with micrometer resolution, and we find that the angular dependence of the x-ray spectrum is showing strong evidence of anisotropic electron trajectories. C1 [Albert, F.; Pollock, B. B.; Ralph, J. E.; Chen, Y. -H.; Alessi, D.; Pak, A.] Lawrence Livermore Natl Lab, NIF, Livermore, CA 94550 USA. [Albert, F.; Pollock, B. B.; Ralph, J. E.; Chen, Y. -H.; Alessi, D.; Pak, A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Shaw, J. L.; Marsh, K. A.; Clayton, C. E.; Joshi, C.] Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA. [Glenzer, S. H.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. RP Albert, F (reprint author), Lawrence Livermore Natl Lab, NIF, 7000 East Ave, Livermore, CA 94550 USA. EM albert6@llnl.gov RI Chen, Yu-hsin/I-3400-2012; Albert, Felicie/G-2645-2013 OI Chen, Yu-hsin/0000-0002-9603-7371; FU U.S. Department of Energy at UCLA [DE-AC52-07NA27344, DE-FG02-92-ER40727]; Laboratory Directed Research and Development (LDRD) Program [13-LW-076]; DOE Office of Science, Fusion Energy Sciences [FWP 100182] FX This work was performed under the auspices of the U.S. Department of Energy under Contracts No. DE-AC52-07NA27344 at LLNL, and No. DE-FG02-92-ER40727 at UCLA, and supported by the Laboratory Directed Research and Development (LDRD) Program under tracking code 13-LW-076. This work was partially supported by the DOE Office of Science, Fusion Energy Sciences under FWP 100182. The authors thank R. C. Cauble, J. Bonlie, and S. Maricle for their support of the Callisto laser system at the Jupiter Laser Facility and C. Haefner for advice on lasers. F. A. acknowledges discussions with F. V. Hartemann on theory and modeling and thanks C. D. Chen for discussions on the spectrometer layout. NR 35 TC 29 Z9 29 U1 7 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 4 PY 2013 VL 111 IS 23 AR 235004 DI 10.1103/PhysRevLett.111.235004 PG 5 WC Physics, Multidisciplinary SC Physics GA 274OQ UT WOS:000328616300021 PM 24476282 ER PT J AU Balasubramanian, V Bernamonti, A de Boer, J Craps, B Franti, L Galli, F Keski-Vakkuri, E Muller, B Schafer, A AF Balasubramanian, V. Bernamonti, A. de Boer, J. Craps, B. Franti, L. Galli, F. Keski-Vakkuri, E. Mueller, B. Schaefer, A. TI Inhomogeneous Thermalization in Strongly Coupled Field Theories SO PHYSICAL REVIEW LETTERS LA English DT Article ID PB-PB COLLISIONS; ROOT-S(NN)=2.76 TEV; FLOW AB To describe theoretically the creation and evolution of the quark-gluon plasma, one typically employs three ingredients: a model for the initial state, nonhydrodynamic early time evolution, and hydrodynamics. In this Letter we study the nonhydrodynamic early time evolution using the AdS/CFT correspondence in the presence of inhomogeneities. We find that the AdS description of the early time evolution is well matched by free streaming. Near the end of the early time interval where our analytic computations are reliable, the stress tensor agrees with the second order hydrodynamic stress tensor computed from the local energy density and fluid velocity. Our techniques may also be useful for the study of far-from-equilibrium strongly coupled systems in other areas of physics. C1 [Balasubramanian, V.] Univ Penn, David Rittenhouse Lab, Philadelphia, PA 19104 USA. [Balasubramanian, V.] Ecole Normale Super, Phys Theor Lab, F-75005 Paris, France. [Bernamonti, A.] Katholieke Univ Leuven, Inst Theoret Fys, B-3001 Louvain, Belgium. [de Boer, J.] Univ Amsterdam, Inst Theoret Phys, NL-1090 GL Amsterdam, Netherlands. [Craps, B.; Galli, F.] Vrije Univ Brussel, B-1050 Brussels, Belgium. [Craps, B.; Galli, F.] Int Solvay Inst, B-1050 Brussels, Belgium. [Franti, L.; Keski-Vakkuri, E.] Univ Helsinki, Helsinki Inst Phys, FIN-00014 Helsinki, Finland. [Franti, L.; Keski-Vakkuri, E.] Univ Helsinki, Dept Phys, FIN-00014 Helsinki, Finland. [Keski-Vakkuri, E.] Uppsala Univ, Dept Phys & Astron, SE-75108 Uppsala, Sweden. [Mueller, B.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Mueller, B.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Schaefer, A.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. RP Balasubramanian, V (reprint author), Univ Penn, David Rittenhouse Lab, Philadelphia, PA 19104 USA. RI Craps, Ben/J-8429-2016; Keski-Vakkuri, Esko/B-6747-2017 OI Craps, Ben/0000-0002-0805-0403; Keski-Vakkuri, Esko/0000-0002-6737-6067 FU Belgian Federal Science Policy Office; FWO-Vlaanderen; Foundation of Fundamental Research on Matter (FOM); Finnish Academy of Science and Letters; U.S. Department of Energy; BMBF; Academy of Finland FX We thank M. Heller, K. Rajagopal, and especially S. Minwalla for discussions. This research is supported by the Belgian Federal Science Policy Office, by FWO-Vlaanderen, by the Foundation of Fundamental Research on Matter (FOM), by Finnish Academy of Science and Letters, by the U.S. Department of Energy, by the BMBF, and by the Academy of Finland. A. B. is a Postdoctoral Researcher FWO and F. G. is Aspirant FWO. NR 36 TC 21 Z9 23 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 4 PY 2013 VL 111 IS 23 AR 231602 DI 10.1103/PhysRevLett.111.231602 PG 5 WC Physics, Multidisciplinary SC Physics GA 274OQ UT WOS:000328616300010 PM 24476254 ER PT J AU Bennett, MB Wrede, C Chipps, KA Jose, J Liddick, SN Santia, M Bowe, A Chen, AA Cooper, N Irvine, D McNeice, E Montes, F Naqvi, F Ortez, R Pain, SD Pereira, J Prokop, C Quaglia, J Quinn, SJ Schwartz, SB Shanab, S Simon, A Spyrou, A Thiagalingam, E AF Bennett, M. B. Wrede, C. Chipps, K. A. Jose, J. Liddick, S. N. Santia, M. Bowe, A. Chen, A. A. Cooper, N. Irvine, D. McNeice, E. Montes, F. Naqvi, F. Ortez, R. Pain, S. D. Pereira, J. Prokop, C. Quaglia, J. Quinn, S. J. Schwartz, S. B. Shanab, S. Simon, A. Spyrou, A. Thiagalingam, E. TI Classical-Nova Contribution to the Milky Way's Al-26 Abundance: Exit Channel of the Key Al-25(p,gamma)Si-26 Resonance SO PHYSICAL REVIEW LETTERS LA English DT Article ID THERMONUCLEAR REACTION-RATES; FRAGMENT SEPARATOR; NUCLEOSYNTHESIS; EMISSION; MG-25(P,GAMMA)AL-26; GALAXY; STATES; STARS; FE-60 AB Classical novae are expected to contribute to the 1809-keV Galactic gamma-ray emission by producing its precursor Al-26, but the yield depends on the thermonuclear rate of the unmeasured Al-25(p,gamma)Si-26 reaction. Using the beta decay of P-26 to populate the key J(pi) = 3(+) resonance in this reaction, we report the first evidence for the observation of its exit channel via a 1741: 6 +/- 0.6(stat) +/- 0: 3(syst) keV primary gamma-ray, where the uncertainties are statistical and systematic, respectively. By combining the measured gamma-ray energy and intensity with other experimental data on Si-26, we find the center-of-mass energy and strength of the resonance to be E-r = 414: 9 +/- 0: 6(stat) +/- 0: 3(syst) +/- 0: 6(lit.) keV and omega gamma = 23 +/- 6(stat)(-10)(+11)(lit.) meV, respectively, where the last uncertainties are from adopted literature data. We use hydrodynamic nova simulations to model Al-26 production showing that these measurements effectively eliminate the dominant experimental nuclear-physics uncertainty and we estimate that novae may contribute up to 30% of the Galactic Al-26. C1 [Bennett, M. B.; Wrede, C.; Santia, M.; Bowe, A.; Ortez, R.; Quinn, S. J.; Schwartz, S. B.; Shanab, S.; Spyrou, A.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Bennett, M. B.; Wrede, C.; Liddick, S. N.; Santia, M.; Bowe, A.; Montes, F.; Ortez, R.; Pereira, J.; Prokop, C.; Quaglia, J.; Quinn, S. J.; Schwartz, S. B.; Shanab, S.; Simon, A.; Spyrou, A.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Wrede, C.; Ortez, R.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Chipps, K. A.] Colorado Sch Mines, Dept Phys, Golden, CO 08401 USA. [Jose, J.] Dept Fis & Engn Nucl UPC, E-08034 Barcelona, Spain. [Jose, J.] Inst Estudis Espacials Catalunya, E-08034 Barcelona, Spain. [Liddick, S. N.; Prokop, C.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Bowe, A.] Kalamazoo Coll, Dept Phys, Kalamazoo, MI 49006 USA. [Chen, A. A.; Irvine, D.; McNeice, E.; Thiagalingam, E.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Cooper, N.; Naqvi, F.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Cooper, N.; Naqvi, F.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06520 USA. [Montes, F.; Pereira, J.; Quaglia, J.; Quinn, S. J.; Simon, A.; Spyrou, A.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Pain, S. D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Quaglia, J.] Michigan State Univ, Dept Elect Engn, E Lansing, MI 48824 USA. [Schwartz, S. B.] Univ So Indiana, Geol & Phys Dept, Evansville, IN 47712 USA. RP Bennett, MB (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM bennettm@nscl.msu.edu; wrede@nscl.msu.edu RI Pain, Steven/E-1188-2011 OI Pain, Steven/0000-0003-3081-688X FU U.S. National Science Foundation [PHY-1102511, PHY Q7 08-22648]; U.S. Department of Energy [DE-FG02-97ER41020]; U.S. National Nuclear Security Agency [DE-NA0000979]; MEC [AYA2010-15685]; ESF EUROCORES Program EuroGENESIS [EUI2009-04167] FX This work was supported by the U.S. National Science Foundation under Grants No. PHY-1102511 and No. PHY Q7 08-22648, the U.S. Department of Energy under Contract No. DE-FG02-97ER41020, the U. S. National Nuclear Security Agency under Contract No. DE-NA0000979, MEC Grant No. AYA2010-15685, and the ESF EUROCORES Program EuroGENESIS through Grant No. EUI2009-04167. We gratefully acknowledge A. Garcia for advice during the preparation of our experimental proposal and the NSCL Operations staff for delivering the beam. NR 48 TC 17 Z9 17 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 4 PY 2013 VL 111 IS 23 AR 232503 DI 10.1103/PhysRevLett.111.232503 PG 6 WC Physics, Multidisciplinary SC Physics GA 274OQ UT WOS:000328616300014 PM 24476263 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T DeWolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, X Wang, Z Xiao, H Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Benhabib, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Heracleous, N Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Flucke, G Geiser, A Glushkov, I Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G Horton, D Jung, H Kasemann, M Katsas, P Kleinwort, C Kluge, H Kramer, M Krucker, D Kuznetsova, E Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Olzem, J Perrey, H Petrukhin, A Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Riedl, C Ron, E Sahin, MO Salfeld-Nebgen, J Schmidt, R Schoerner-Sadenius, T Sen, N Stein, M Walsh, R Wissing, C Martin, MA Blobel, V Enderle, H Erfle, J Garutti, E Gebbert, U Gorner, M Gosselink, M Haller, J Heine, K Hoing, RS Kaussen, G Kirschenmann, H Klanner, R Kogler, R Lange, J Marchesini, I Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schroder, M Schum, T Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Thomsen, J Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hartmann, F Hauth, T Held, H Hoffmann, KH Husemann, U Katkov, I Komaragiri, JR Kornmayer, A Pardo, PL Martschei, D Muller, T Niegel, M Nurnberg, A Oberst, O Ott, J Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Ntomari, E Topsis-giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Mittal, M Nishu, N Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Malhotra, S Naimuddin, M Ranjan, K Saxena, P Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, 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Mohapatra, A. Mozer, M. U. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Swanson, J. CA CMS Collaboration TI Measurement of the differential and double-differential Drell-Yan cross sections in proton-proton collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; LHC AB Measurements of the differential and double-differential Drell-Yan cross sections are presented using an integrated luminosity of 4.5 (4.8) fb(-1) in the dimuon (dielectron) channel of proton-proton collision data recorded with the CMS detector at the LHC at = 7 TeV. The measured inclusive cross section in the Z-peak region (60-120 GeV) is sigma(a""a"") = 986.4 +/- 0.6 (stat.) +/- 5.9 (exp. syst.) +/- 21.7 (th. syst.) +/- 21.7 (lum.) pb for the combination of the dimuon and dielectron channels. Differential cross sections d sigma/dm for the dimuon, dielectron, and combined channels are measured in the mass range 15 to 1500 GeV and corrected to the full phase space. Results are also presented for the measurement of the double-differential cross section d(2)sigma/dm d|y| in the dimuon channel over the mass range 20 to 1500 GeV and absolute dimuon rapidity from 0 to 2.4. These measurements are compared to the predictions of perturbative QCD calculations at next-to-leading and next-to-next-to-leading orders using various sets of parton distribution functions. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C-E] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Bansal, M.; Bansal, S.; Cornelis, T.; DeWolf, E. A.; Janssen, X.; Knutsson, A.; Luyckx, S.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Staykova, Z.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Kalogeropoulos, A.; Keaveney, J.; Maes, M.; Olbrechts, A.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Hreus, T.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, B-1348 Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; Correa Martins Junior, M.; Martins, T.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Alda Junior, W. L.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Malek, M.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dias, F. A.; Fernandez Perez Tomei, T. R.; Lagana, C.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Genchev, V.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Tcholakov, V.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, X.; Wang, Z.; Xiao, H.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, Q.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Carrillo Montoya, C. A.; Chaparro Sierra, L. F.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.; Tikvica, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Abdelalim, A. A.; Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Radi, A.] Egyptian Network High Energy Phys, Acad Sci Res & Technol Arab Republ Egypt, Cairo, Egypt. [Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Rebane, L.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Baffioni, S.; Beaudette, F.; Benhabib, L.; Bluj, M.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Florent, A.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Agram, J-L; Andrea, J.; Bloch, D.; Brom, J-M; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J-C; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, P.; Le Bihan, A. -C; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Gadrat, S.] IN2P3, CNRS, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I-A; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. O.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Stein, M.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Gebbert, U.; Goerner, M.; Gosselink, M.; Haller, J.; Heine, K.; Hoeing, R. S.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Marchesini, I.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Kornmayer, A.; Pardo, P. Lobelle; Martschei, D.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F-P; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Topsis-giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Abdulsalam, A.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, EHEP, Mumbai 400005, Maharashtra, India. [Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res, HECR, Mumbai 400005, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.; Tosi, M.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; De Cosa, A.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Fantinel, S.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Gulmini, M.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Maron, G.; Meneguzzo, A. T.; Michelotto, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Montoya, C. A.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Andreev, V.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Abdulsalam, A.; Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Sci, Belgrade 11000, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Gomez-Reino Garrido, R.; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Palencia Cortezon, E.; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rojo, J.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Erdmann, M.; Bertl, W.; Deiters, K.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. 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Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; Moon, Chang-Seong/J-3619-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014 OI Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Dudko, Lev/0000-0002-4462-3192; de Jesus Damiao, Dilson/0000-0002-3769-1680; Novaes, Sergio/0000-0003-0471-8549; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Codispoti, Giuseppe/0000-0003-0217-7021; Montanari, Alessandro/0000-0003-2748-6373; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; da Cruz e silva, Cristovao/0000-0002-1231-3819; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Heath, Helen/0000-0001-6576-9740; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; Michelotto, Michele/0000-0001-6644-987X; My, Salvatore/0000-0002-9938-2680; Lo Vetere, Maurizio/0000-0002-6520-4480; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Ragazzi, Stefano/0000-0001-8219-2074; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; Moon, Chang-Seong/0000-0001-8229-7829; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787 FU Austrian Federal Ministry of Science and Research; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes co financed by EU-ESF and the Greek NSRF. NR 51 TC 10 Z9 10 U1 4 U2 98 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD DEC 4 PY 2013 IS 12 AR 030 DI 10.1007/JHEP12(2013)030 PG 62 WC Physics, Particles & Fields SC Physics GA 270WI UT WOS:000328349500001 ER PT J AU Sakai, Y Nguyen, GD Capaz, RB Coh, S Pechenezhskiy, IV Hong, XP Wang, F Crommie, MF Saito, S Louie, SG Cohen, ML AF Sakai, Yuki Nguyen, Giang D. Capaz, Rodrigo B. Coh, Sinisa Pechenezhskiy, Ivan V. Hong, Xiaoping Wang, Feng Crommie, Michael F. Saito, Susumu Louie, Steven G. Cohen, Marvin L. TI Intermolecular interactions and substrate effects for an adamantane monolayer on a Au(111) surface SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-FUNCTIONAL THEORY; INFRARED-SPECTROSCOPY; DIAMONDOID MOLECULES; ELECTRON-GAS; VIBRATIONS; SPECTRA; SYSTEMS; PHASE AB We study theoretically and experimentally the infrared (IR) spectrum of an adamantane monolayer on a Au(111) surface. Using a STM-based IR spectroscopy technique (IRSTM) we are able to measure both the nanoscale structure of an adamantane monolayer on Au(111) as well as its infrared spectrum, while DFT-based ab initio calculations allow us to interpret the microscopic vibrational dynamics revealed by our measurements. We find that the IR spectrum of an adamantane monolayer on Au(111) is substantially modified with respect to the gas-phase IR spectrum. The first modification is caused by the adamantane-adamantane interaction due to monolayer packing, and it reduces the IR intensity of the 2912 cm(-1) peak (gas phase) by a factor of 3.5. The second modification originates from the adamantane-gold interaction, and it increases the IR intensity of the 2938 cm(-1) peak (gas phase) by a factor of 2.6 and reduces its frequency by 276 cm(-1). We expect that the techniques described here can be used for an independent estimate of substrate effects and intermolecular interactions in other diamondoid molecules and for other metallic substrates. C1 [Sakai, Yuki; Saito, Susumu] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Sakai, Yuki; Nguyen, Giang D.; Capaz, Rodrigo B.; Coh, Sinisa; Pechenezhskiy, Ivan V.; Hong, Xiaoping; Wang, Feng; Crommie, Michael F.; Louie, Steven G.; Cohen, Marvin L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Capaz, Rodrigo B.] Univ Fed Rio de Janeiro, Inst Fis, BR-21941972 Rio De Janeiro, RJ, Brazil. [Coh, Sinisa; Pechenezhskiy, Ivan V.; Wang, Feng; Crommie, Michael F.; Louie, Steven G.; Cohen, Marvin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Sakai, Y (reprint author), Tokyo Inst Technol, Dept Phys, Meguro Ku, 2-12-1 Oh Okayama, Tokyo 1528551, Japan. RI Hong, Xiaoping/G-8673-2013; B, Rodrigo/N-7595-2014; wang, Feng/I-5727-2015; Nguyen, Giang/R-1287-2016 OI Hong, Xiaoping/0000-0002-5864-4533; Nguyen, Giang/0000-0003-4125-8203 FU NSF [DMR-10-1006184]; Nanomachines Program at the Lawrence Berkeley National Lab; office of Basic Energy Sciences, DOE [DE-AC02-05CH11231]; Nanomachines Program of the Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy [DE-AC02-05CH11231]; Department of Energy [DESC0003949]; Japan Society for the Promotion of Science; CNPq; FAPERJ; INCT -Nanomateriais de Carbono and Rede de Pesquisa e Instrumentacao em NanoEspectroscopia Optica; Simons Foundation FX Computational resources were provided by the DOE at Lawrence Berkeley National Laboratory's NERSC facility. Numerical calculations were also carried out on the TSUB-AME2.0 supercomputer in the Tokyo Institute of Technology. The theoretical part of the work was supported by NSF Grant No. DMR-10-1006184 (structural determination) and by the Nanomachines Program at the Lawrence Berkeley National Lab funded by the office of Basic Energy Sciences, DOE under Contract No. DE-AC02-05CH11231 (infrared spectra simulations and analyses). The experimental part of the study was supported by the Nanomachines Program of the Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy under Contract No. DE-AC02-05CH11231 (STM measurements) and by the Department of Energy Early Career Award DESC0003949 (development of IR laser source). Y. S. acknowledges financial support from Japan Society for the Promotion of Science. R. B. C. acknowledges financial support from Brazilian agencies CNPq, FAPERJ, INCT -Nanomateriais de Carbono and Rede de Pesquisa e Instrumentacao em NanoEspectroscopia Optica. S. G. L. acknowledges the support of a Simons Foundation Fellowship in Theoretical Physics. NR 35 TC 2 Z9 2 U1 1 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 4 PY 2013 VL 88 IS 23 AR 235407 DI 10.1103/PhysRevB.88.235407 PG 9 WC Physics, Condensed Matter SC Physics GA 274AA UT WOS:000328576200004 ER PT J AU Di Sante, D Stroppa, A Jain, P Picozzi, S AF Di Sante, Domenico Stroppa, Alessandro Jain, Prashant Picozzi, Silvia TI Tuning the Ferroelectric Polarization in a Multiferroic Metal-Organic Framework SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IMPROPER FERROELECTRICITY; MECHANICAL-PROPERTIES; FORMATE FRAMEWORKS; MOLECULAR-CRYSTAL; PEROVSKITE; INSTABILITIES; TRANSITION; ENERGY; ROOM; M=MN AB We perform density functional theory calculations on a recently synthesized metal-organic framework (MOP) with a perovskite-like topology ABX(3), i.e., [CH3CH2NH3]Mn(HCOO)(3), and predict a multiferroic behavior, i.e., a coexistence of ferroelectricity and ferromagnetism. A peculiar canted ordering of the organic A-cation dipole moments gives rise to a ferroelectric polarization of similar to 2 mu C/cm(2). Starting from these findings, we show that by choosing different organic A cations, it is possible to tune the ferroelectric polarization and increase it up. to 6 mu C/cm(2). The possibility of changing the magnitude and/or the canting of the organic molecular dipole opens new routes toward engineering ferroelectric polarization in the new class of multiferroic metal-organic frameworks. C1 [Di Sante, Domenico] Univ Aquila, Dept Phys & Chem Sci, I-67100 Laquila, Italy. [Di Sante, Domenico; Stroppa, Alessandro; Picozzi, Silvia] CNR SPIN, Laquila, Italy. [Jain, Prashant] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Di Sante, D (reprint author), Univ Aquila, Dept Phys & Chem Sci, Via Vetoio, I-67100 Laquila, Italy. EM domenico.disante@aquila.infn.it; alessandro.stroppa@spin.cnr.it RI Stroppa, Alessandro/E-7702-2010; Picozzi, Silvia/E-2374-2011; SPIN-CNR, L'Aquila/C-7274-2011; Di Sante, Domenico/L-8931-2013 OI Stroppa, Alessandro/0000-0003-1000-4745; Picozzi, Silvia/0000-0002-3232-788X; FU MIUR-FIRB project [RBAP117RWN]; SPIN-CNR SEED project [PAQSE001]; U.S. Department of Energy through the LANL/LDRD Program; U.S. National Science Foundation I2CAM International Materials Institute Award [DMR-0844115] FX The work is supported by the MIUR-FIRB project RBAP117RWN. We acknowledge support from SPIN-CNR SEED project PAQSE001 Metal-Organic Frameworks, New Routes to Multiferroicity and Magnetoelectricity. We acknowledge that the results in this paper have been achieved using the PRACE Research Infrastructure resource FERMI based in Italy at CINECA-Bologna under grant agreement MEMOIR-Multi-ferroic and magnetoElectric Metal Organic Frameworks of the fifth PRACE Regular Call for Proposals. We also thankfully acknowledge the computer resources from MareNostrum, technical expertise, and prompt assistance provided by the Spanish Supercomputing Network (RES) and the Barcelona Supercomputing Center. A.S. and D.D.S. thanks Prof. M. Aschi and Dr. T. Bucko for useful discussions. A.S. greatly thanks Prof. C. J. Fennie, Prof. J. M. Rondinelli, and Prof. V. Zapf for invitations to Cornell, Drexel University, and Los Alamos National Laboratory, respectively, and for useful discussions. A.S. thanks Prof. A. Sayede for the kind invitation to Universite d'Artois, Faculte des Sciences Jean Perrin, where this work was finalized. P.J. acknowledges the support of the U.S. Department of Energy through the LANL/LDRD Program as well as support of the U.S. National Science Foundation I2CAM International Materials Institute Award, Grant DMR-0844115. The authors greatly acknowledge the careful reading and useful comments by Prof. J. R. Long (University of California, Berkeley). A.S. gratefully acknowledges Prof. A. K. Cheetham and Dr. Wei Li for the invitation to Cambridge University (Functional Inorganics and Hybrid Materials group) and for useful discussions. A.S. thanks Prof. M. H. Whangbo for the warm hospitality at Department of Chemistry, North Carolina State University, and for interesting discussions. NR 52 TC 87 Z9 87 U1 21 U2 228 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 4 PY 2013 VL 135 IS 48 BP 18126 EP 18130 DI 10.1021/ja408283a PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 267LU UT WOS:000328100000022 PM 24191632 ER PT J AU Drisdell, WS Poloni, R McDonald, TM Long, JR Smit, B Neaton, JB Prendergast, D Kortright, JB AF Drisdell, Walter S. Poloni, Roberta McDonald, Thomas M. Long, Jeffrey R. Smit, Berend Neaton, Jeffrey B. Prendergast, David Kortright, Jeffrey B. TI Probing Adsorption Interactions in Metal-Organic Frameworks using X-ray Spectroscopy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CARBON-DIOXIDE CAPTURE; NEAR-EDGE STRUCTURE; ABSORPTION-SPECTRA; ALKALI-HALIDES; CO2 ADSORPTION; SITES; GAS; DIFFRACTION; MAGNESIUM; CELLS AB We explore the local electronic signatures of molecular adsorption at coordinatively unsaturated binding sites in the metal organic framework Mg-MOF-74 using X-ray spectroscopy and first-principles calculations. In situ measurements at the Mg K-edge reveal distinct pre-edge absorption features associated with the unique, open coordination of the Mg sites which are suppressed upon adsorption of CO2 and N,N'-dimethylformamide. Density functional theory shows that these spectral changes arise from modifications of local symmetry around the Mg sites upon gas uptake and are strongly dependent on the metal-adsorbate binding strength. The expanded MOP Mg-2(dobpdc) displays the same behavior upon adsorption of CO2 and N,N'-dimethylethylenediamine. Similar sensitivity to local symmetry is expected for any open metal site, making X-ray spectroscopy an ideal tool for examining adsorption in such MOFs. Qualitative agreement between ambient-temperature experimental and 0 K theoretical spectra is good, with minor discrepancies thought to result from framework vibrational motion. C1 [Drisdell, Walter S.; Poloni, Roberta; McDonald, Thomas M.; Long, Jeffrey R.; Neaton, Jeffrey B.; Prendergast, David; Kortright, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Poloni, Roberta; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Poloni, Roberta; McDonald, Thomas M.; Long, Jeffrey R.; Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Poloni, Roberta] Grenoble INP, UMR CNRS 5266, Lab Sci & Ingn Mat & Procedes SIMaP, F-38402 St Martin Dheres, France. RP Kortright, JB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM jbkortright@lbl.gov RI Smit, Berend/B-7580-2009; EFRC, CGS/I-6680-2012; Stangl, Kristin/D-1502-2015; Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014 OI Smit, Berend/0000-0003-4653-8562; Neaton, Jeffrey/0000-0001-7585-6135; FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award Number DE-SC0001015. Portions of this work were performed as User Projects at the Advanced Light Source and Molecular Foundry, both at Lawrence Berkeley National Laboratory and supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Calculations used LBNL Lawrencium, the National Energy Research Scientific Computing Center, LBNL, and the Molecular Foundry computing resources nano and vulcan, managed by the High Performance Computing Services Group, LBNL. NR 46 TC 25 Z9 25 U1 6 U2 137 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD DEC 4 PY 2013 VL 135 IS 48 BP 18183 EP 18190 DI 10.1021/ja408972f PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 267LU UT WOS:000328100000028 PM 24224556 ER PT J AU Sagaram, US El-Mounadi, K Buchko, GW Berg, HR Kaur, J Pandurangi, RS Smith, TJ Shah, DM AF Sagaram, Uma Shankar El-Mounadi, Kaoutar Buchko, Garry W. Berg, Howard R. Kaur, Jagdeep Pandurangi, Raghu S. Smith, Thomas J. Shah, Dilip M. TI Structural and Functional Studies of a Phosphatidic Acid-Binding Antifungal Plant Defensin MtDef4: Identification of an RGFRRR Motif Governing Fungal Cell Entry SO PLOS ONE LA English DT Article ID 3-DIMENSIONAL SOLUTION STRUCTURE; HUMAN IMMUNODEFICIENCY VIRUS; PISUM-SATIVUM DEFENSIN-1; DAHLIA DAHLIA-MERCKII; ANIMAL HOST-CELLS; ANTIMICROBIAL PEPTIDES; EFFECTOR PROTEINS; FUSARIUM-GRAMINEARUM; GROWTH-INHIBITION; CHEMICAL-SHIFT AB MtDef4 is a 47-amino acid cysteine-rich evolutionary conserved defensin from a model legume Medicago truncatula. It is an apoplast-localized plant defense protein that inhibits the growth of the ascomycetous fungal pathogen Fusarium graminearum in vitro at micromolar concentrations. Little is known about the mechanisms by which MtDef4 mediates its antifungal activity. In this study, we show that MtDef4 rapidly permeabilizes fungal plasma membrane and is internalized by the fungal cells where it accumulates in the cytoplasm. Furthermore, analysis of the structure of MtDef4 reveals the presence of a positively charged Upsilon-core motif composed of beta(2) and beta(3) strands connected by a positively charged RGFRRR loop. Replacement of the RGFRRR sequence with AAAARR or RGFRAA abolishes the ability of MtDef4 to enter fungal cells, suggesting that the RGFRRR loop is a translocation signal required for the internalization of the protein. MtDef4 binds to phosphatidic acid (PA), a precursor for the biosynthesis of membrane phospholipids and a signaling lipid known to recruit cytosolic proteins to membranes. Amino acid substitutions in the RGFRRR sequence which abolish the ability of MtDef4 to enter fungal cells also impair its ability to bind PA. These findings suggest that MtDef4 is a novel antifungal plant defensin capable of entering into fungal cells and affecting intracellular targets and that these processes are mediated by the highly conserved cationic RGFRRR loop via its interaction with PA. C1 [Sagaram, Uma Shankar; El-Mounadi, Kaoutar; Berg, Howard R.; Kaur, Jagdeep; Pandurangi, Raghu S.; Smith, Thomas J.; Shah, Dilip M.] Donald Danforth Plant Sci Ctr, St Louis, MO USA. [Buchko, Garry W.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Shah, DM (reprint author), Donald Danforth Plant Sci Ctr, St Louis, MO USA. EM dshah@danforthcenter.org RI Shah, Dilip/M-2850-2013; Buchko, Garry/G-6173-2015; Kaur, Jagdeep/C-4155-2015; Berg, R. Howard/M-2839-2013 OI Buchko, Garry/0000-0002-3639-1061; Kaur, Jagdeep/0000-0002-3238-4825; Berg, R. Howard/0000-0001-5081-2769 FU NSF [MCB-0924124] FX This research has been supported by the NSF grant MCB-0924124. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 70 TC 29 Z9 29 U1 2 U2 29 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 4 PY 2013 VL 8 IS 12 AR UNSP e82485 DI 10.1371/journal.pone.0082485 PG 22 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 265KD UT WOS:000327949300154 PM 24324798 ER PT J AU Williams, PT AF Williams, Paul T. TI Inadequate Exercise as a Risk Factor for Sepsis Mortality SO PLOS ONE LA English DT Article ID TYPE-2 DIABETES-MELLITUS; CORONARY-HEART-DISEASE; PHYSICAL-ACTIVITY; IMMUNE-SYSTEM; VIGOROUS EXERCISE; CONSCIOUS RATS; SEPTIC SHOCK; RUNNERS; ASSOCIATION; CHOLESTEROL AB Objective: Test whether inadequate exercise is related to sepsis mortality. Research Design and Methods: Mortality surveillance of an epidemiological cohort of 155,484 National Walkers' and Runners' Health Study participants residing in the United States. Deaths were monitored for an average of 11.6-years using the National Death index through December 31, 2008. Cox proportional hazard analyses were used to compare sepsis mortality (ICD-10 A40-41) to inadequate exercise (<1.07 METh/d run or walked) as measured on their baseline questionnaires. Deaths occurring within one year of the baseline survey were excluded. Results: Sepsis was the underlying cause in 54 deaths (sepsis(underlying)) and a contributing cause in 184 deaths (sepsis(contributing)), or 238 total sepsis-related deaths (sepsis(total)). Inadequate exercise was associated with 2.24-fold increased risk for sepsisunderlying (95%CI: 1.21 to 4.07-fold, P=0.01), 2.11-fold increased risk for sepsis(contributing) (95%CI: 1.51- to 2.92-fold, P<10(-4)), and 2.13-fold increased risk for sepsis(total) (95%CI: 1.59- to 2.84-fold, P, 10 26) when adjusted for age, sex, race, and cohort. The risk increase did not differ significantly between runners and walkers, by sex, or by age. Sepsistotal risk was greater in diabetics (P=10(-5)), cancer survivors (P=0.0001), and heart attack survivors (P=0.003) and increased with waist circumference (P=0.0004). The sepsis(total) risk associated with inadequate exercise persisted when further adjusted for diabetes, prior cancer, prior heart attack and waist circumference, and when excluding deaths with cancer, or cardiovascular, respiratory, or genitourinary disease as the underlying cause. Inadequate exercise also increased sepsistotal risk in 2163 baseline diabetics (4.78-fold, 95%CI: 2.1- to 13.8-fold, P=0.0001) when adjusted, which was significantly greater (P=0.03) than the adjusted risk increase in non-diabetics (1.80-fold, 95%CI: 1.30- to 2.46-fold, P=0.0006). Conclusion: Inadequate exercise is a risk factor for sepsis mortality, particular in diabetics. C1 Ernest Orlando Lawrence Berkeley Natl Lab, Donner Lab, Div Life Sci, Berkeley, CA USA. RP Williams, PT (reprint author), Ernest Orlando Lawrence Berkeley Natl Lab, Donner Lab, Div Life Sci, Berkeley, CA USA. EM ptwilliams@lbl.gov FU National Heart, Lung, and Blood Institute [HL094717] FX This research was supported by grant HL094717 from the National Heart, Lung, and Blood Institute and was conducted at the Ernest Orlando Lawrence Berkeley National Laboratory (Department of Energy DE-AC03-76SF00098 to the University of California). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 44 TC 2 Z9 2 U1 0 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD DEC 4 PY 2013 VL 8 IS 12 AR e79344 DI 10.1371/journal.pone.0079344 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 265KD UT WOS:000327949300008 PM 24324580 ER PT J AU Liu, B Xiao, HY Zhang, Y Aidhy, DS Weber, WJ AF Liu, B. Xiao, H. Y. Zhang, Y. Aidhy, D. S. Weber, W. J. TI Ab initio molecular dynamics simulations of threshold displacement energies in SrTiO3 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID ELECTRONIC-STRUCTURE; STRONTIUM-TITANATE; CERAMICS; PSEUDOPOTENTIALS; PEROVSKITES; IRRADIATION; DISORDER; BATIO3; CATIO3; OXIDES AB Ab initio molecular dynamics simulations have been carried out to study low energy recoil events in SrTiO3. The threshold displacement energies are shown to be strongly dependent on both the orientation and the corresponding atomic arrangement. The minimum threshold displacement energies are 13 eV for an O recoil along the < 100 > O-O chain, 25 eV for a Sr recoil along the < 100 > Sr-Sr chain and 38 eV for a Ti recoil along the < 110 > Ti-Ti chain. The weighted average threshold displacement energies along the primary crystallographic directions are 35.7, 53.5 and >64.9 eV for O, Sr and Ti, respectively. The interstitial configurations produced by the recoil events are < 100 > and < 111 > split interstitials for O and Sr, respectively, together with a Ti interstitial occupying a distorted bridge position between two Sr sites. It is found that the recoil events in SrTiO3 are partial-charge transfer assisted processes, and the partial-charge transfer plays an important role in these recoil events. C1 [Liu, B.; Zhang, Y.; Aidhy, D. S.; Weber, W. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Xiao, H. Y.; Zhang, Y.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Liu, B (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM liub2@ornl.gov; wjweber@utk.edu RI Weber, William/A-4177-2008; Liu, Bin/N-9955-2014 OI Weber, William/0000-0002-9017-7365; FU US Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division FX This work was supported by the US Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division. The theoretical calculations were performed using the supercomputer resources at the National Energy Research Scientific Computing Center located at Lawrence Berkeley National Laboratory. NR 40 TC 5 Z9 5 U1 4 U2 37 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD DEC 4 PY 2013 VL 25 IS 48 AR 485003 DI 10.1088/0953-8984/25/48/485003 PG 8 WC Physics, Condensed Matter SC Physics GA 254CB UT WOS:000327138300013 PM 24162447 ER PT J AU Palacio, I Monti, M Marco, JF McCarty, KF de la Figuera, J AF Palacio, I. Monti, M. Marco, J. F. McCarty, K. F. de la Figuera, J. TI Initial stages of FeO growth on Ru(0001) SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID ENERGY-ELECTRON-DIFFRACTION; CO OXIDATION; IRON; SURFACE; FILMS; OXIDES; ADSORPTION; NUCLEATION; DIFFUSION; CATALYSIS AB We study how FeO wustite films on Ru(0001) grow by oxygen-assisted molecular beam epitaxy at elevated temperatures (800-900 K). The nucleation and growth of FeO islands are observed in real time by low-energy electron microscopy (LEEM). When the growth is performed in an oxygen pressure of 10(-6) Torr, the islands are of bilayer thickness (Fe-O-Fe-O). In contrast, under a pressure of 10(-8) Torr, the islands are a single FeO layer thick. We propose that the film thickness is controlled by the concentration of oxygen adsorbed on the Ru. More specifically, when monolayer growth increases the adsorbed oxygen concentration above a limiting value, its growth is suppressed. Increasing the temperature at a fixed oxygen pressure decreases the density of FeO islands. However, the nucleation density is not a monotonic function of oxygen pressure. C1 [Palacio, I.] Univ Complutense Madrid, Dept Fis Mat, E-28040 Madrid, Spain. [Palacio, I.] Unidad Asociada IQFR CSIC UCM, E-28040 Madrid, Spain. [Monti, M.; Marco, J. F.; de la Figuera, J.] CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain. [McCarty, K. F.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Palacio, I (reprint author), Synchroton Soleil, F-91190 St Aubin, France. EM juan.delafiguera@iqfr.csic.es RI de la Figuera, Juan/E-7046-2010; Marco, Jose/N-3176-2014 OI de la Figuera, Juan/0000-0002-7014-4777; Marco, Jose/0000-0002-5147-1449 FU Spanish Ministry of Education and Science [MAT2009-14578-C03-01, MAT2009-14578-C03-02]; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC04-94AL85000]; Spanish Ministry of Science and Innovation through FPI fellowships FX This research was supported by the Spanish Ministry of Education and Science under project nos MAT2009-14578-C03-01 and MAT2009-14578-C03-02, and by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under contract no. .DE-AC04-94AL85000. IP and MM thank the Spanish Ministry of Science and Innovation for support through FPI fellowships NR 42 TC 6 Z9 6 U1 2 U2 48 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD DEC 4 PY 2013 VL 25 IS 48 AR 484001 DI 10.1088/0953-8984/25/48/484001 PG 10 WC Physics, Condensed Matter SC Physics GA 254CB UT WOS:000327138300003 PM 24200910 ER PT J AU Yuen, CD Miller, GJ Lei, HP Wang, CZ Thiel, PA AF Yuen, Chad D. Miller, Gordon J. Lei, Huaping Wang, Cai-Zhuang Thiel, Patricia A. TI Structure of the clean Gd5Ge4(010) surface SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID MAGNETOCALORIC MATERIALS; MAGNETIC REFRIGERATION; CRYSTAL-STRUCTURES; GD(0001) SURFACE; GERMANIUM; SYSTEM; ALLOYS; GD; GD-5(SIXGE1-X)(4); IDENTIFICATION AB We have characterized the (010) surface of Gd5Ge4 using scanning tunneling microscopy (STM) and x-ray photoelectron spectroscopy. Data from different samples have the following features in common: (1) the surface composition equals the bulk composition to within 5 at.%, both after ion etching and after annealing at temperatures of 400-1200 K; and (2) the surface exhibits terraces of two types. The height of the steps between similar terraces corresponds well to the separation between equivalent layers along the < 010 > direction in the bulk structure. Density functional theory (DFT) shows that the surface energy of the (0001) plane of hexagonal close-packed Gd is lower than that of the (111) plane of diamond-type Ge, suggesting that surfaces of Gd5Ge4 (for comparable density) should be rich in Gd. Indeed, DFT shows that among the bulk terminations of Gd5Ge4, a pure Ge termination is not favored. Each of the three remaining terminations (two pure Gd and one mixed, Gd-Ge) has its minimum surface energy in a different range of the possible Gd chemical potentials, indicating that different terminations may be stable under different conditions. DFT shows that the heights of the steps between dissimilar terraces, measured in STM, are consistent with the two pure Gd terminations. C1 [Yuen, Chad D.; Miller, Gordon J.; Lei, Huaping; Wang, Cai-Zhuang; Thiel, Patricia A.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Yuen, Chad D.; Miller, Gordon J.; Thiel, Patricia A.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Thiel, Patricia A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Yuen, CD (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM pthiel@iastate.edu FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX This research was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-07CH11358. James W Anderegg, Mark Wallingford, and Holly Walen assisted with some of the experiments. D L Schlagel expertly grew, oriented, and polished the samples, and performed optical microscopy and x-ray diffraction. Shalabh Gupta and Srinivasa Thimmaiah gave insights into the bulk structure, and assisted in its representation. We thank them all. NR 46 TC 1 Z9 1 U1 2 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD DEC 4 PY 2013 VL 25 IS 48 AR 485002 DI 10.1088/0953-8984/25/48/485002 PG 9 WC Physics, Condensed Matter SC Physics GA 254CB UT WOS:000327138300012 PM 24162383 ER PT J AU Sayre, R AF Sayre, Richard TI Iron biofortification and homeostasis in transgenic cassava roots expressing an algal iron assimilatory protein, FEA1 (vol 3, pg 171, 2012) SO FRONTIERS IN PLANT SCIENCE LA English DT Correction C1 Los Alamos Natl Labs, New Mexico Consortium, Los Alamos, NM 87545 USA. RP Sayre, R (reprint author), Los Alamos Natl Labs, New Mexico Consortium, Los Alamos, NM 87545 USA. EM rsayre@newmexicoconsortium.org OI Sayre, Richard/0000-0002-3153-7084 NR 1 TC 0 Z9 0 U1 0 U2 6 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. 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CA ATLAS Collaboration TI Search for long-lived stopped R-hadrons decaying out of time with pp collisions using the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID DYNAMICAL SUPERSYMMETRY BREAKING; SUPERGAUGE TRANSFORMATIONS; PARTICLES; MODEL; SIMULATION; EXTENSION; COLLIDERS; CURRENTS; SQUARK; WEAK AB An updated search is performed for gluino, top squark, or bottom squark R-hadrons that have come to rest within the ATLAS calorimeter, and decay at some later time to hadronic jets and a neutralino, using 5.0 and 22.9 fb(-1) of pp collisions at 7 and 8 TeV, respectively. Candidate decay events are triggered in selected empty bunch crossings of the LHC in order to remove pp collision backgrounds. Selections based on jet shape and muon system activity are applied to discriminate signal events from cosmic ray and beam-halo muon backgrounds. In the absence of an excess of events, improved limits are set on gluino, stop, and sbottom masses for different decays, lifetimes, and neutralino masses. With a neutralino of mass 100 GeV, the analysis excludes gluinos with mass below 832 GeV (with an expected lower limit of 731 GeV), for a gluino lifetime between 10 mu s and 1000 s in the generic R-hadron model with equal branching ratios for decays to q (q) over bar(chi) over tilde (0) and g (chi) over tilde (0). Under the same assumptions for the neutralino mass and squark lifetime, top squarks and bottom squarks in the Regge R-hadron model are excluded with masses below 379 and 344 GeV, respectively. C1 [Corriveau, F.; Jackson, P.; McPherson, R. A.; Sobie, R.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. 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S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Ancu, L. S.; Beck, H. P.; Borer, C.; Cervelli, A.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Mahout, G.; Mclaughlan, T.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, E.; Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Bindi, M.; Boscherini, D.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Gabrielli, A.; Giacobbe, B.; Grafstrom, P.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] INFN Sezione Bologna, Bologna, Italy. [Bindi, M.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Gabrielli, A.; Grafstrom, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis Astron, Bologna, Italy. [Abajyan, T.; Arslan, O.; Backhaus, M.; Bechtle, P.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Hageboeck, S.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Physikal Inst, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.; Zambito, S.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Univ Fed Juiz de Fora, Juiz de Fora, Brazil. [do Vale, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Backes, M.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianco, M.; Bogaerts, J. A.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Chen, S.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Laboratoire Phys Corpusculaire, Clermont Ferrand, France. [Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Blaise Pascal, Laboratoire Phys Corpusculaire, Clermont Ferrand, France. [Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Laboratoire Phys Corpusculaire, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zhou, L.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Gruppo Collegato Cosenza, Milan, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Bunse, M.; Burmeister, I.; Esch, H.; Gossling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Experimentelle Phys IV, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphysik, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Kajomovitz, E.; Ko, B. R.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Ludwig, D.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Demichev, M.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Buehrer, F.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; dit Latour, B. Martin; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] INFN Sezione Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Joseph Fourier, Laboratoire Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Laboratoire Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytechn Grenoble, Laboratoire Phys Subatom & Cosmol, Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informatik, Heidelberg, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphysik, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, Inst Fis La Plata, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sezione Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Dept Phys, Ljubljana 61000, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London E1 4NS, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Cantrill, R.; Cooper-Smith, N. J.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.] Univ London Royal Holloway, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Lab Phys Nucl & Hautes Energies, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.; Venturi, M.] Univ Aix Marseille 1, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.; Venturi, M.] CNRS, IN2P3, CPPM, Marseille, France. [Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Xu, L.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Caughron, S.; Ge, P.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Ta, D.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] INFN Sezione Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] PN Lebedev Phys Inst, Acad Sci, Moscow 117924, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Moscow Engn & Phys Inst, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; De Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst Phys, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Grad Sch Sci, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sezione Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, LAL, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sezione Pavia, Pavia, Italy. [Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] INFN Sezione Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Sargedas De Sousa, M. J. Da Cunha; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Dos Santos, D. Roda; Ruzicka, P.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] INFN Sezione Roma 1, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] INFN Sezione Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] INFN Sezione Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies Univ, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucleaires, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Fac Sci, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Mountricha, E.; Thi Hong, V. Nguyen; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.; Xu, C.] DSM IRFU, CEA Saclay, Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Huang, Y.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron & Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Grout, Z. J.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Israel Inst Technol, Dept PhysTechn, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bangert, A.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Bangert, A.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Centro Investigaciones, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] INFN Gruppo Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernanandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, IFIC, CSIC, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernanandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dep Fisica Atom Mol & Nucl, CSIC, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernanandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingenieri Elect, CSIC, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernanandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, IMB CNM, CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astronomie, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Physik, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr IN2P3, Villeurbanne, France. Kings Coll London, Dept Phys, London WC2R 2LS, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Nova Lisboa, Faculdade Ciencias & CFNUL, P-1200 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Robertson, S. H.; Teuscher, R. J.] Inst Particle Phys, Toronto, ON, Canada. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC Faculdade Ciencias Tecnologia, Caparica, Portugal. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Tech Univ, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Wildt, M. A.] Univ Hamburg, Inst Experimentalphys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Chudoba, Jiri/G-7737-2014; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Snesarev, Andrey/H-5090-2013; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Ferrando, James/A-9192-2012; Deliot, Frederic/F-3321-2014; Doyle, Anthony/C-5889-2009; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Nozka, Libor/G-5550-2014; Kuday, Sinan/C-8528-2014; Smirnova, Oxana/A-4401-2013; Gabrielli, Alessandro/H-4931-2012; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Karyukhin, Andrey/J-3904-2014; Juste, Aurelio/I-2531-2015; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Fullana Torregrosa, Esteban/A-7305-2016; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; O'Shea, Val/G-1279-2010; Carvalho, Joao/M-4060-2013; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011 OI Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Warburton, Andreas/0000-0002-2298-7315; Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Castro, Nuno/0000-0001-8491-4376; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Mikestikova, Marcela/0000-0003-1277-2596; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Ferrando, James/0000-0002-1007-7816; Doyle, Anthony/0000-0001-6322-6195; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Lee, Jason/0000-0002-2153-1519; Kuday, Sinan/0000-0002-0116-5494; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Belanger-Champagne, Camille/0000-0003-2368-2617; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Walsh, Brian/0000-0003-1689-2309; Price, Darren/0000-0003-2750-9977; Filthaut, Frank/0000-0003-3338-2247; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Wang, Kuhan/0000-0002-6151-0034; Grohsjean, Alexander/0000-0003-0748-8494; La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Salamanna, Giuseppe/0000-0002-0861-0052; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Haas, Andrew/0000-0002-4832-0455; Galhardo, Bruno/0000-0003-0641-301X; Della Volpe, Domenico/0000-0001-8530-7447; Casadei, Diego/0000-0002-3343-3529; Mendes Saraiva, Joao Gentil/0000-0002-7006-0864; Pina, Joao /0000-0001-8959-5044; Hays, Chris/0000-0003-2371-9723; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Cristinziani, Markus/0000-0003-3893-9171; Qian, Jianming/0000-0003-4813-8167; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Juste, Aurelio/0000-0002-1558-3291; Karpov, Sergey/0000-0002-2230-5353; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Vari, Riccardo/0000-0002-2814-1337; Gray, Heather/0000-0002-5293-4716; Thomson, Mark/0000-0002-2654-9005; Grancagnolo, Francesco/0000-0002-9367-3380; Dell'Asta, Lidia/0000-0002-9601-4225; Cataldi, Gabriella/0000-0001-8066-7718; Sawyer, Lee/0000-0001-8295-0605; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Chromek-Burckhart, Doris/0000-0003-4243-3288; Begel, Michael/0000-0002-1634-4399; Mincer, Allen/0000-0002-6307-1418; Troncon, Clara/0000-0002-7997-8524; Bailey, David C/0000-0002-7970-7839; Chen, Hucheng/0000-0002-9936-0115; Nisati, Aleandro/0000-0002-5080-2293; Fullana Torregrosa, Esteban/0000-0003-3082-621X; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; O'Shea, Val/0000-0001-7183-1205; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM; Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular, from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 65 TC 22 Z9 22 U1 9 U2 116 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD DEC 3 PY 2013 VL 88 IS 11 AR 112003 DI 10.1103/PhysRevD.88.112003 PG 30 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274JF UT WOS:000328601900002 ER PT J AU Sun, P Yuan, F AF Sun, Peng Yuan, Feng TI Transverse momentum dependent evolution: Matching semi-inclusive deep inelastic scattering processes to Drell-Yan and W/Z boson production SO PHYSICAL REVIEW D LA English DT Article ID SINGLE-SPIN ASYMMETRIES; LEPTON PAIRS; SIVERS ASYMMETRIES; DISTRIBUTIONS; COLLISIONS; QCD; UNIVERSALITY; COLLINS; DIS AB We examine the QCD evolution for the transverse momentum dependent observables in hard processes of semi-inclusive hadron production in deep inelastic scattering and Drell-Yan lepton pair production in pp collisions, including the spin-average cross sections and Sivers single transverse spin asymmetries. We show that the evolution equations derived by a direct integral of the Collins-Soper-Sterman evolution kernel from low to high Q can describe well the transverse momentum distributions of the unpolarized cross sections in the Q(2) range from 2 to 100 GeV2. In addition, the matching is established between our evolution and the Collins-Soper-Sterman resummation with b(*) prescription and Konychev-Nodalsky parametrization of the nonperturbative form factors, which are formulated to describe the Drell-Yan lepton pair and W/Z boson production in hadronic collisions. With these results, we present the predictions for the Sivers single transverse spin asymmetries in Drell-Yan lepton pair production and W-+/- boson production in polarized pp and pi(-) p collisions for several proposed experiments. We emphasize that these experiments will not only provide crucial test of the sign change of the Sivers asymmetry but also provide important opportunities to study the QCD evolution effects. C1 [Sun, Peng; Yuan, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Sun, Peng; Yuan, Feng] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China. RP Sun, P (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RI Yuan, Feng/N-4175-2013 FU U. S. Department of Energy [DE-AC02-05CH11231] FX We thank Z. Kang and B. Xiao for early collaboration related to Ref. [21]. We thank A. Bressan, A. Martin, and G. Schnell for communications concerning HERMES and COMPASS experimental data. We thank X. Jiang, Z. Kang, A. Martin, and A. Prokudin for comments and discussions. We also thank the Center of High Energy Physics, Peking University, for warm hospitality during our visits, when this paper was finished. This work was partially supported by the U. S. Department of Energy via Grant No. DE-AC02-05CH11231. NR 82 TC 41 Z9 41 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 3 PY 2013 VL 88 IS 11 AR 114012 DI 10.1103/PhysRevD.88.114012 PG 31 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274JF UT WOS:000328601900008 ER PT J AU Park, SR Cao, Y Wang, Q Fujita, M Yamada, K Mo, SK Dessau, DS Reznik, D AF Park, S. R. Cao, Y. Wang, Q. Fujita, M. Yamada, K. Mo, S. -K. Dessau, D. S. Reznik, D. TI Broken relationship between superconducting pairing interaction and electronic dispersion kinks in La2-xSrxCuO4 measured by angle-resolved photoemission SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; COPPER-OXIDE SUPERCONDUCTORS; T-C SUPERCONDUCTOR; TRANSITION TEMPERATURE; SPIN; BI2SR2CACU2O8+DELTA; EXCITATIONS; STATE AB Electronic band dispersions in copper oxide superconductors have kinks around 70 meV that are typically attributed to coupling of electrons to a bosonic mode. We performed angle-resolved photoemission spectroscopy experiments on overdoped cuprate high temperature superconductors to test the relationship between the superconducting transition temperature and electron-bosonic mode coupling. Remarkably, the kinks remain strong in the heavily overdoped region of the doping phase diagram of strong in the heavily overdoped region of the doping phase diagram of La2-xSrxCuO4, even when the superconductivity completely disappears. This unexpected observation is incompatible with the conventional picture of superconductivity mediated by the sharp bosonic modes that are responsible for the kink unless extra doping strongly suppresses their d-wave projection but not the overall spectral weight. Our results favor pairing mediated by a very broad electronic spectrum or an unconventional mechanism without pairing glue. C1 [Park, S. R.; Cao, Y.; Wang, Q.; Dessau, D. S.; Reznik, D.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Park, S. R.] Incheon Natl Univ, Dept Phys, Inchon 406772, South Korea. [Fujita, M.] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan. [Yamada, K.] KEK, Inst Mat Struct Sci, Oho, Ibaraki 3050801, Japan. [Mo, S. -K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Park, SR (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA. EM dmitry.reznik@colorado.edu RI Fujita, Masaki/D-8430-2013; Mo, Sung-Kwan/F-3489-2013; OI Mo, Sung-Kwan/0000-0003-0711-8514; Cao, Yue/0000-0002-3989-158X FU DOE, Office of Basic Energy Sciences, Office of Science, [DE-SC0006939]; DOE [DE-FG02-03ER46066]; MEXT of Japan [22244039] FX The authors thank Ted Reber for valuable discussions. The Advanced Light Source is operated by the DOE, Office of Basic Energy Sciences. S. R. P. and D. R. were supported by the DOE, Office of Basic Energy Sciences, Office of Science, under Contract No. DE-SC0006939. Y. C., Q. W., and D. S. D. were supported by the DOE under Contract No. DE-FG02-03ER46066. The work at Tohoku University was supported by the Grant-In-Aid for Science Research A (22244039) from the MEXT of Japan. NR 63 TC 8 Z9 8 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD DEC 3 PY 2013 VL 88 IS 22 AR 220503 DI 10.1103/PhysRevB.88.220503 PG 6 WC Physics, Condensed Matter SC Physics GA 273YP UT WOS:000328572500003 ER PT J AU Metere, A Oppelstrup, T Sarman, S Laaksonen, A Dzugutov, M AF Metere, A. Oppelstrup, T. Sarman, S. Laaksonen, A. Dzugutov, M. TI Formation of the smectic-B crystal from a simple monatomic liquid SO PHYSICAL REVIEW E LA English DT Article ID COMPUTER-SIMULATION; PHASE; SYSTEMS; MODEL AB We report a molecular dynamics simulation demonstrating that the smectic-B crystalline phase (Cry-B), commonly observed in mesogenic systems of anisotropic molecules, can be formed by a system of identical particles interacting via a spherically symmetric potential. The Cry-B phase forms as a result of a first-order transition from an isotropic liquid phase upon isochoric cooling at appropriate number density. Its structure, determined by the design of the pair potential, corresponds to the Cry-B structure formed by elongated particles with the aspect ratio 1.8. The diffraction pattern and the real-space structure inspection demonstrate dominance of the ABC-type of axial layer stacking. This result opens a general possibility of producing smectic phases using isotropic interparticle interaction both in simulations and in colloidal systems. C1 [Metere, A.; Sarman, S.; Laaksonen, A.] Stockholm Univ, Dept Mat & Environm Chem, S-10691 Stockholm, Sweden. [Oppelstrup, T.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Dzugutov, M.] Royal Inst Technol, Dept Math, S-10044 Stockholm, Sweden. [Dzugutov, M.] Royal Inst Technol, Ctr Parallel Comp, S-10044 Stockholm, Sweden. RP Metere, A (reprint author), Stockholm Univ, Dept Mat & Environm Chem, Arrhenius Vag 16C, S-10691 Stockholm, Sweden. RI Metere, Alfredo/M-9399-2014 OI Metere, Alfredo/0000-0003-0237-7250 FU Swedish e-Science Research Center; Swedish Science Council VR; LLNL [DE-AC52-07NA27344] FX We gratefully acknowledge the valuable assistance of Michael Schliephake and other staff members of the Centre for Parallel Computers (PDC), KTH. This study was supported by the Swedish e-Science Research Center. We thank the Swedish Science Council VR for funding support. This work has been approved for release under Lawrence Livermore Release No. LLNL-JRNL-639781; prepared by LLNL under Contract No. DE-AC52-07NA27344. NR 26 TC 3 Z9 3 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD DEC 3 PY 2013 VL 88 IS 6 AR 062502 DI 10.1103/PhysRevE.88.062502 PG 4 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 274KO UT WOS:000328605400003 PM 24483463 ER PT J AU Awe, TJ McBride, RD Jennings, CA Lamppa, DC Martin, MR Rovang, DC Slutz, SA Cuneo, ME Owen, AC Sinars, DB Tomlinson, K Gomez, MR Hansen, SB Herrmann, MC McKenney, JL Nakhleh, C Robertson, GK Rochau, GA Savage, ME Schroen, DG Stygar, WA AF Awe, T. J. McBride, R. D. Jennings, C. A. Lamppa, D. C. Martin, M. R. Rovang, D. C. Slutz, S. A. Cuneo, M. E. Owen, A. C. Sinars, D. B. Tomlinson, K. Gomez, M. R. Hansen, S. B. Herrmann, M. C. McKenney, J. L. Nakhleh, C. Robertson, G. K. Rochau, G. A. Savage, M. E. Schroen, D. G. Stygar, W. A. TI Observations of Modified Three-Dimensional Instability Structure for Imploding z-Pinch Liners that are Premagnetized with an Axial Field SO PHYSICAL REVIEW LETTERS LA English DT Article ID FUSION AB Novel experimental data are reported that reveal helical instability formation on imploding z-pinch liners that are premagnetized with an axial field. Such instabilities differ dramatically from the mostly azimuthally symmetric instabilities that form on unmagnetized liners. The helical structure persists at nearly constant pitch as the liner implodes. This is surprising since, at the liner surface, the azimuthal drive field presumably dwarfs the axial field for all but the earliest stages of the experiment. These fundamentally 3D results provide a unique and challenging test for 3D-magnetohydrodynamics simulations. C1 [Awe, T. J.; McBride, R. D.; Jennings, C. A.; Lamppa, D. C.; Martin, M. R.; Rovang, D. C.; Slutz, S. A.; Cuneo, M. E.; Owen, A. C.; Sinars, D. B.; Gomez, M. R.; Hansen, S. B.; Herrmann, M. C.; McKenney, J. L.; Robertson, G. K.; Rochau, G. A.; Savage, M. E.; Stygar, W. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Tomlinson, K.; Schroen, D. G.] Gen Atom, San Diego, CA 92121 USA. [Nakhleh, C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Awe, TJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tjawe@sandia.gov FU Sandia's Laboratory Directed Research and Development Program [141537, 165736]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank the ABZ Team, the MagLIF Team, the Z Operations Team, the Z-Beamlet Operations Team, Center Section personnel, the Z Diagnostics Team, The Neutron Team, CMDAS personnel, Lab 101 personnel, the VISAR team, the Gas Fill Team, the Target Fabrication Team, J. Greenly, D. Johnson, M. Jones, R. Kamm, J. Moore, S. Radovich, G. Smith, and I. Smith. This project was funded in part by Sandia's Laboratory Directed Research and Development Program (Projects No. 141537 and No. 165736). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 24 TC 34 Z9 35 U1 1 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 3 PY 2013 VL 111 IS 23 AR 235005 DI 10.1103/PhysRevLett.111.235005 PG 5 WC Physics, Multidisciplinary SC Physics GA 274OL UT WOS:000328615700013 PM 24476283 ER PT J AU Li, CK Ryutov, DD Hu, SX Rosenberg, MJ Zylstra, AB Seguin, FH Frenje, JA Casey, DT Johnson, MG Manuel, MJE Rinderknecht, HG Petrasso, RD Amendt, PA Park, HS Remington, BA Wilks, SC Betti, R Froula, DH Knauer, JP Meyerhofer, DD Drake, RP Kuranz, CC Young, R Koenig, M AF Li, C. K. Ryutov, D. D. Hu, S. X. Rosenberg, M. J. Zylstra, A. B. Seguin, F. H. Frenje, J. A. Casey, D. T. Johnson, M. Gatu Manuel, M. J. -E. Rinderknecht, H. G. Petrasso, R. D. Amendt, P. A. Park, H. S. Remington, B. A. Wilks, S. C. Betti, R. Froula, D. H. Knauer, J. P. Meyerhofer, D. D. Drake, R. P. Kuranz, C. C. Young, R. Koenig, M. TI Structure and Dynamics of Colliding Plasma Jets SO PHYSICAL REVIEW LETTERS LA English DT Article ID LASER-PRODUCED PLASMAS; INERTIAL CONFINEMENT FUSION; HIGH-POWER LASERS; DIRECT-DRIVE; COLLISIONLESS SHOCKS; MAGNETIC-FIELDS; ASTROPHYSICS; IMPLOSIONS; GENERATION; OMEGA AB Monoenergetic-proton radiographs of laser-generated, high-Mach-number plasma jets colliding at various angles shed light on the structures and dynamics of these collisions. The observations compare favorably with results from 2D hydrodynamic simulations of multistream plasma jets, and also with results from an analytic treatment of electron flow and magnetic field advection. In collisions of two noncollinear jets, the observed flow structure is similar to the analytic model's prediction of a characteristic feature with a narrow structure pointing in one direction and a much thicker one pointing in the opposite direction. Spontaneous magnetic fields, largely azimuthal around the colliding jets and generated by the well-known del T-e X del n(e) Biermann battery effect near the periphery of the laser spots, are demonstrated to be "frozen in'' the plasma (due to high magnetic Reynolds number Re-M similar to 5 X 10(4)) and advected along the jet streamlines of the electron flow. These studies provide novel insight into the interactions and dynamics of colliding plasma jets. C1 [Li, C. K.; Rosenberg, M. J.; Zylstra, A. B.; Seguin, F. H.; Frenje, J. A.; Casey, D. T.; Johnson, M. Gatu; Manuel, M. J. -E.; Rinderknecht, H. G.; Petrasso, R. D.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Ryutov, D. D.; Amendt, P. A.; Park, H. S.; Remington, B. A.; Wilks, S. C.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hu, S. X.; Betti, R.; Froula, D. H.; Knauer, J. P.; Meyerhofer, D. D.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Drake, R. P.; Kuranz, C. C.; Young, R.] Univ Michigan, Ann Arbor, MI 48109 USA. [Koenig, M.] Univ Paris 06, CEA, CNRS, Lab Utilisat Lasers Intenses,UMR 7605,Ecole Polyt, F-91128 Palaiseau, France. RP Li, CK (reprint author), MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. EM ckli@mit.edu RI Hu, Suxing/A-1265-2007; Manuel, Mario/L-3213-2015; Drake, R Paul/I-9218-2012; OI Hu, Suxing/0000-0003-2465-3818; Manuel, Mario/0000-0002-5834-1161; Drake, R Paul/0000-0002-5450-9844; /0000-0003-4969-5571 FU U.S. DOE and LLE National Laser User's Facility [DE-FG52-07NA28 059, DE-FG03-03SF22691]; LLNL [B543881, LDRD-08-ER-062]; LLE [414090-G]; FSC at the University of Rochester [412761-G] FX This work was supported in part by the U.S. DOE and LLE National Laser User's Facility (No. DE-FG52-07NA28 059 and No. DE-FG03-03SF22691), LLNL (No. B543881 and No. LDRD-08-ER-062), LLE (No. 414090-G), and FSC at the University of Rochester (No. 412761-G). NR 41 TC 10 Z9 10 U1 7 U2 67 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 3 PY 2013 VL 111 IS 23 AR 235003 DI 10.1103/PhysRevLett.111.235003 PG 5 WC Physics, Multidisciplinary SC Physics GA 274OL UT WOS:000328615700012 PM 24476281 ER PT J AU Fabbris, G Matsuoka, T Lim, J Mardegan, JRL Shimizu, K Haskel, D Schilling, JS AF Fabbris, G. Matsuoka, T. Lim, J. Mardegan, J. R. L. Shimizu, K. Haskel, D. Schilling, J. S. TI Different routes to pressure-induced volume collapse transitions in gadolinium and terbium metals SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-NONMAGNETIC TRANSITION; PHASE-TRANSITION; CERIUM; SUPERCONDUCTIVITY; IMPURITIES; GPA; TEMPERATURE; IFEFFIT; YTTRIUM; SYSTEM AB The sudden decrease in molar volume exhibited by most lanthanides under high pressure is often attributed to changes in the degree of localization of their 4f electrons. We give evidence, based on electrical resistivity measurements of dilute Y(Gd) and Y(Tb) alloys to 120 GPa, that the volume collapse transitions in Gd and Tb metals have different origins, despite their being neighbors in the periodic table. Remarkably, the change under pressure in the magnetic state of isolated Pr or Tb impurity ions in the nonmagnetic Y host appears to closely mirror corresponding changes in pure Pr or Tb metals. The collapse in Tb appears to be driven by an enhanced negative exchange interaction between 4f and conduction electrons under pressure (Kondo resonance) which, in the case of Y(Tb), dramatically alters the superconducting properties of the Y host, much like previously found for Y(Pr). In Gd, our resistivity measurements suggest that a Kondo resonance is not the main driver for its volume collapse. X-ray absorption and emission spectroscopies clearly show that 4f local moments remain largely intact across both volume collapse transitions ruling out 4f band formation (delocalization) and valence transition models as possible drivers. The results highlight the richness of behavior behind the volume collapse transition in lanthanides and demonstrate the stability of the 4f level against band formation to extreme pressure. C1 [Fabbris, G.; Mardegan, J. R. L.; Haskel, D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Fabbris, G.; Matsuoka, T.; Lim, J.; Schilling, J. S.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Matsuoka, T.; Shimizu, K.] Osaka Univ, KYOKUGEN, Toyonaka, Osaka 5608531, Japan. [Matsuoka, T.] Gifu Univ, Dept Mat Sci & Technol, Gifu 5011193, Japan. [Mardegan, J. R. L.] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Campinas, SP, Brazil. RP Schilling, JS (reprint author), Washington Univ, Dept Phys, St Louis, MO 63130 USA. EM jss@wuphys.wustl.edu RI Fabbris, Gilberto/F-3244-2011; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Fabbris, Gilberto/0000-0001-8278-4985; FU National Science Foundation [DMR-1104742]; Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE [DE-FC52-08NA28554]; US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-AC-02-06CH11357]; FAPESP (SP-Brazil) [2011/24166-0] FX Research at both Washington University and the APS was supported by the National Science Foundation through grant DMR-1104742 and by the Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE Grant No. DE-FC52-08NA28554. Work at Argonne is supported by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC-02-06CH11357. J. R. L. Mardegan was supported by FAPESP (SP-Brazil) under Contract No. 2011/24166-0. The authors would like to thank Anup Gangopadhyay for assistance in sample preparation, as well as Borje Johansson and James Hamlin for critically reading the manuscript. We thank Steve Heald and Chengjun Sun for their support at Advanced Photon Source (APS) 20-BM, Yuming Xiao, Paul Chow and Genevieve Boman for their support at APS HPCAT 16-ID-D, and Sergey Tkachev for his help in using the APS GSECARS gas loading system. NR 60 TC 11 Z9 11 U1 2 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 3 PY 2013 VL 88 IS 24 AR 245103 DI 10.1103/PhysRevB.88.245103 PG 7 WC Physics, Condensed Matter SC Physics GA 273YX UT WOS:000328573300001 ER PT J AU Butorin, SM Shuh, DK Kvashnina, KO Guo, JH Werme, L Nordgren, J AF Butorin, Sergei M. Shuh, David K. Kvashnina, Kristina O. Guo, Jinghua Werme, Lars Nordgren, Joseph TI Chemical Reduction of Actinides Probed by Resonant Inelastic X-ray Scattering SO ANALYTICAL CHEMISTRY LA English DT Article ID ELECTRONIC-STRUCTURE; EMISSION AB The study addresses the possibilities of immobilizing the mobile species of actinides in the geosphere using metallic iron. Sorption on corroding iron is well-known, but there have been uncertainties with regard to the possibilities of reducing the actinyl species to sparingly soluble oxides and, thereby, permanently immobilizing them. Resonant inelastic X-ray scattering (RIXS) measurements at the actinide 5d edges on Fe foils exposed to uranium(VI) and neptunium(V) solutions in groundwater unambigiously indicate reduction of actinides to, respectively, uranium(IV) and neptunium(IV) on iron surfaces. The reduction manifests itself in an appearance of distinct specific signatures of uranium(IV) and neptunium(IV) in the RIXS profile of 5f-5f excitations. Such signatures and RIXS intensity/cross-section behavior with varying energy of incident photons can be reproduced by model atomic-multiplet calculations of the RIXS spectra. By normalizing the RIXS signal of corresponding 5f-5f excitations to core-to-core 6p-to-5d characteristic fluorescence transitions of actinides, their reduction rates on Fe samples with different exposure to actinide solutions can be estimated. Observed reduction implies similar processes in the nuclear waste canister thus suggesting reduced probability of nuclear waste release with ground waters from the canister. C1 [Butorin, Sergei M.; Kvashnina, Kristina O.; Werme, Lars; Nordgren, Joseph] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Shuh, David K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Butorin, SM (reprint author), Uppsala Univ, Dept Phys & Astron, Box 516, SE-75120 Uppsala, Sweden. EM sergei.butorin@physics.uu.se RI Kvashnina, Kristina/O-2374-2016 OI Kvashnina, Kristina/0000-0003-4447-4542 FU European Commission [EU FIKW-CT-2000-00019]; U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX We would like to thank K. Ollila and Y. Albinsson for preparation of samples. This work was financially supported by the European Commission (under Contract No. EU FIKW-CT-2000-00019). The work at the Advanced Light Source was supported by the Director, Office of Science, and the research performed by D.K.S. was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Heavy Element Chemistry Program, both of the U.S. Department of Energy at Lawrence Berkeley National Laboratory (under Contract No. DE-AC02-05CH11231). NR 13 TC 4 Z9 4 U1 2 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD DEC 3 PY 2013 VL 85 IS 23 BP 11196 EP 11200 DI 10.1021/ac4020534 PG 5 WC Chemistry, Analytical SC Chemistry GA 266CL UT WOS:000327999800007 PM 24187957 ER PT J AU Wilk, A Carter, JC Chrisp, M Manuel, AM Mirkarimi, P Alameda, JB Mizaikoff, B AF Wilk, Andreas Carter, J. Chance Chrisp, Michael Manuel, Anastacia M. Mirkarimi, Paul Alameda, Jennifer B. Mizaikoff, Boris TI Substrate-Integrated Hollow Waveguides: A New Level of Integration in Mid-Infrared Gas Sensing SO ANALYTICAL CHEMISTRY LA English DT Article ID QUANTUM-CASCADE LASERS; EXHALED MOUSE BREATH; CARBON-MONOXIDE; AQUEOUS-SOLUTIONS; DELIVERY-SYSTEMS; CO2-LASER LIGHT; CAPILLARY CELL; NITRIC-OXIDE; ER-YAG; SENSORS AB A new generation of hollow waveguide (HWG) gas cells of unprecedented compact dimensions facilitating low sample volumes suitable for broad- and narrow-band mid-infrared (MIR; 2.5-20 mu m) sensing applications is reported: the substrate-integrated hollow waveguide (iHWG). iHWGs are layered structures providing light guiding channels integrated into a solid-state substrate material, which are competitive if not superior in performance to conventional leaky-mode fiber optic silica HWGs having similar optical pathlengths. In particular, the provided flexibility in device and optical design and the wide variety of manufacturing strategies, substrate materials, access to the optical channel, and optical coating options highlight the advantages of iHWGs in terms of robustness, compactness, and cost-effectiveness. Finally, the unmatched modularity of this novel waveguide approach facilitates tailoring iHWGs to almost any kind of gas sensor technology providing adaptability to the specific demands of a wide range of sensing scenarios. Device fabrication is demonstrated for the example of a yin-yang-shaped gold-coated iHWG fabricated within an aluminum substrate with a footprint of only 75 mm x 50 mm x 12 mm (L x W x H), yet providing a nominal optical absorption path length of more than 22 cm. The analytical utility of this device for advanced MIR gas sensing applications is demonstrated for the gaseous constituents butane, carbon dioxide, cyclopropane, isobutylene, and methane. C1 [Wilk, Andreas; Mizaikoff, Boris] Univ Ulm, Inst Analyt & Bioanalyt Chem, D-89081 Ulm, Germany. [Carter, J. Chance; Chrisp, Michael; Manuel, Anastacia M.; Mirkarimi, Paul; Alameda, Jennifer B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Mizaikoff, B (reprint author), Univ Ulm, Inst Analyt & Bioanalyt Chem, Albert Einstein Allee 11, D-89081 Ulm, Germany. EM boris.mizaikoff@uni-ulm.de RI Mizaikoff, Boris/G-9959-2013 OI Mizaikoff, Boris/0000-0002-5583-7962 FU U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; LLNL [B598643, B603018] FX The authors acknowledge support by the Machine Shop at the University of Ulm during iHWG device development and fabrication. This work was performed in part under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344. This project was funded under LLNL Subcontract Nos. B598643 and B603018. NR 55 TC 25 Z9 25 U1 4 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD DEC 3 PY 2013 VL 85 IS 23 BP 11205 EP 11210 DI 10.1021/ac402391m PG 6 WC Chemistry, Analytical SC Chemistry GA 266CL UT WOS:000327999800009 PM 24059493 ER PT J AU Qin, LH Zhang, WJ Lu, JW Stack, AG Wang, LJ AF Qin, Lihong Zhang, Wenjun Lu, Jianwei Stack, Andrew G. Wang, Lijun TI Direct Imaging of Nanoscale Dissolution of Dicalcium Phosphate Dihydrate by an Organic Ligand: Concentration Matters SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ATOMIC-FORCE MICROSCOPY; OXALATE MONOHYDRATE CRYSTALLIZATION; NEAR-MOLECULAR LEVEL; CRYSTAL-GROWTH; CALCITE DISSOLUTION; COORDINATION CHEMISTRY; AQUEOUS SUSPENSIONS; SURFACE SPECIATION; LUPINUS-ALBUS; CITRIC-ACID AB Unraveling the kinetics and mechanisms of sparingly soluble calcium orthophosphate (Ca-P) dissolution in the presence of organic acids at microscopic levels is important for an improved understanding in determining the effectiveness of organic acids present in most rhizosphere environments. Herein, we use in situ atomic force microscopy (AFM) coupled with a fluid reaction cell to image dissolution on the (010) face of brushite, CaHPO4 center dot 2H(2)O, in citrate-bearing solutions over a broad concentration range. We directly measure the dependence of molecular step retreat rate on citrate concentration at various pH values and ionic strengths, relevant to soil solution conditions. We find that low concentrations of citrate (10-100 mu M) induced a reduction in step retreat rates along both the [(1) over bar 00]Cc and [10 ($) over bar1]Cc directions. However, at higher concentrations (exceeding 0.1 mM), this inhibitory effect was reversed with step retreat speeds increasing rapidly. These results demonstrate that the concentration-dependent modulation of nanoscale Ca-P phase dissolution by citrate may be applied to analyze the controversial role of organic acids in enhancing Ca-P mineral dissolution in a more complex rhizosphere environment. These in situ observations may contribute to resolving the previously unrecognized interactions of root exudates (low molecular weight organic acids) and sparingly soluble Ca-P minerals. C1 [Qin, Lihong; Zhang, Wenjun; Lu, Jianwei; Wang, Lijun] Huazhong Agr Univ, Coll Resources & Environm, Wuhan 430070, Peoples R China. [Stack, Andrew G.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Wang, LJ (reprint author), Huazhong Agr Univ, Coll Resources & Environm, Wuhan 430070, Peoples R China. EM ljwang@mail.hzau.edu.cn FU National Natural Science Foundation of China [41071208]; Huazhong Agricultural University [2010BQ063, 2012MBDX014, 2011JQ008]; Fundamental Research Funds for the Central Universities [2011PY150]; Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the National Natural Science Foundation of China (Grant No. 41071208) and a startup grant (2010BQ063) and two Independent Innovation Foundation (2012MBDX014, 2011JQ008) from the Huazhong Agricultural University to Lijun Wang. It is also supported in part by the Fundamental Research Funds for the Central Universities (2011PY150). Research is sponsored by the Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy to AGS. NR 70 TC 11 Z9 13 U1 2 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD DEC 3 PY 2013 VL 47 IS 23 BP 13365 EP 13374 DI 10.1021/es402748t PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 266CH UT WOS:000327999400023 PM 24251349 ER PT J AU Ratcliff, MA Luecke, J Williams, A Christensen, E Yanowitz, J Reek, A McCormick, RL AF Ratcliff, Matthew A. Luecke, Jon Williams, Aaron Christensen, Earl Yanowitz, Janet Reek, Aaron McCormick, Robert L. TI Impact of Higher Alcohols Blended in Gasoline on Light-Duty Vehicle Exhaust Emissions SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID JET-STIRRED REACTOR; OXIDATION; ISOBUTANOL; BUTANOL; FUELS; E85 AB Certification gasoline was splash blended with alcohols to produce four blends: ethanol (16 vol%), n-butanol (17 vol%), i-butanol (21 vol%), and an i-butanol (12 vol%)/ethanol (7 vol%) mixture; these fuels were tested in a 2009 Honda Odyssey (a Tier 2 Bin 5 vehicle) over triplicate LA92 cycles. Emissions of oxides of nitrogen, carbon monoxide, non-methane organic gases (NMOG), unburned alcohols, carbonyls, and C-1 C-8 hydrocarbons (particularly 1,3-butadiene and benzene) were determined. Large, statistically significant fuel effects on regulated emissions were a 29% reduction in CO from E16 and a 60% increase in formaldehyde emissions from i-butanol, compared to certification gasoline. Ethanol produced the highest unburned alcohol emissions of 1.38 mg/mile ethanol, while butanols produced much lower unburned alcohol emissions (0.17 mg/mile n-butanol, and 0.30 mg/mile i-butanol); these reductions were offset by higher emissions of carbonyls. Formaldehyde, acetaldehyde, and butyraldehyde were the most significant carbonyls from the n-butanol blend, while formaldehyde, acetone, and 2-methylpropanal were the most significant from the i-butanol blend. The 12% i-butanol/7% ethanol blend was designed to produce no increase in gasoline vapor pressure. This fuel's exhaust emissions contained the lowest total oxygenates among the alcohol blends and the lowest NMOG of all fuels tested. C1 [Ratcliff, Matthew A.; Luecke, Jon; Williams, Aaron; Christensen, Earl; McCormick, Robert L.] US DOE, Natl Renewable Energy Lab, Golden, CO 80401 USA. [Yanowitz, Janet] EcoEngineering Inc, Boulder, CO 80304 USA. [Reek, Aaron] SGS Environm Testing Corp, Aurora, CO 80011 USA. RP Ratcliff, MA (reprint author), US DOE, Natl Renewable Energy Lab, Golden, CO 80401 USA. EM matthew.ratcliff@nrel.gov RI McCormick, Robert/B-7928-2011 FU U.S. Department of Energy [DE-AC36-99GO10337]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-99GO10337 with the National Renewable Energy Laboratory. NR 42 TC 9 Z9 9 U1 0 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD DEC 3 PY 2013 VL 47 IS 23 BP 13865 EP 13872 DI 10.1021/es402793p PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 266CH UT WOS:000327999400081 PM 24180630 ER PT J AU Dallmann, TR Kirchstetter, TW DeMartini, SJ Harley, RA AF Dallmann, Timothy R. Kirchstetter, Thomas W. DeMartini, Steven J. Harley, Robert A. TI Quantifying On-Road Emissions from Gasoline-Powered Motor Vehicles: Accounting for the Presence of Medium- and Heavy-Duty Diesel Trucks SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID REMOTE-SENSING MEASUREMENTS; PARTICULATE MATTER; FINE-PARTICLE; BLACK CARBON; CALIFORNIA; EXHAUST; TUNNEL; AEROSOLS; INVENTORIES; POLLUTION AB Vehicle emissions of nitrogen oxides (NOx), carbon monoxide (CO), fine particulate matter (PM2.5), organic aerosol (OA), and black carbon (BC) were measured at the Caldecott tunnel in the San Francisco Bay Area. Measurements were made in bore 2 of the tunnel, where light-duty (LD) vehicles accounted for >99% of total traffic and heavy-duty trucks were not allowed. Prior emission studies conducted in North America have often assumed that route- or weekend-specific prohibitions on heavy-duty truck traffic imply that diesel contributions to pollutant concentrations measured in on-road settings can be neglected. However, as light-duty vehicle emissions have declined, this assumption can lead to biased results, especially for pollutants such as NOx, OA, and BC, for which diesel-engine emission rates are high compared to corresponding values for gasoline engines. In this study, diesel vehicles (mostly medium-duty delivery trucks with two axles and six tires) accounted for <1% of all vehicles observed in the tunnel but were nevertheless responsible for (18 +/- 3)%, (22 +/- 6)%, and (45 +/- 8)% of measured NOx, OA, and BC concentrations. Fleet-average OA and BC emission factors for light-duty vehicles are, respectively, 10 and 50 times lower than for heavy-duty diesel trucks. Using measured emission factors from this study and publicly available data on taxable fuel sales, as of 2010, LD gasoline vehicles were estimated to be responsible for 85%, 18%, 18%, and 6% of emissions of CO, NOx, OA, and BC, respectively, from on-road motor vehicles in the United States. C1 [Dallmann, Timothy R.; Kirchstetter, Thomas W.; DeMartini, Steven J.; Harley, Robert A.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Kirchstetter, Thomas W.; Harley, Robert A.] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Harley, RA (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. EM harley@ce.berkeley.edu RI Harley, Robert/C-9177-2016; OI Harley, Robert/0000-0002-0559-1917; Dallmann, Timothy/0000-0002-6520-7796 FU EPA [RD834553] FX The authors thank Drew Gentner, Allen Goldstein, Gabriel Isaacman, Eric Stevenson, David Worton, and Caltrans staff at the Caldecott tunnel for their assistance and helpful discussions. In-kind support was provided by the Bay Area Air Quality Management District. This research was made possible by EPA Grant RD834553. Its contents are solely the responsibility of the grantee and do not necessarily represent the official views of the EPA. Further, EPA does not endorse purchase of commercial products or services mentioned herein. NR 45 TC 21 Z9 21 U1 4 U2 70 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD DEC 3 PY 2013 VL 47 IS 23 BP 13873 EP 13881 DI 10.1021/es402875u PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 266CH UT WOS:000327999400082 PM 24215572 ER PT J AU Lovingood, DD Salter, WB Griffith, KR Simpson, KM Hearn, JD Owens, JR AF Lovingood, Derek D. Salter, W. Bruce Griffith, Kara R. Simpson, Katherine M. Hearn, John D. Owens, Jeffery R. TI Fabrication of Liquid and Vapor Protective Cotton Fabrics SO LANGMUIR LA English DT Article ID SILICA NANOPARTICLES; DIMETHYL METHYLPHOSPHONATE; SURFACES; WATER; ADSORPTION; DESIGN; FILMS; WETTABILITY; COATINGS; DROPLETS AB Through microwave-assisted techniques, cotton textiles treated with heptadecafluoro-1,1,2,2-tetrahydrodecyltrimethoxysilane in the presence of high surface area silica nanoparticles create a material capable of repelling bulk liquid challenges while simultaneously adsorbing organic vapors from bulk liquid droplets. Characterizing the contradictory behavior of adsorption of vapors and repellency of liquids is the primary focus of this article. These procedures reveal a quick and simple method for a one-step deposition of a vapor-sorptive, liquid-repellent, Cassie-Baxter surface onto textiles. Packed column breakthrough and single swatch permeation experiments showed that treated materials possess a high affinity for 3-hepten-2-one vapor, while goniometry revealed contact angles in excess of 120 degrees for surface-deposited, 5 mu L droplets of several test liquids. Scanning electron micrograph images confirm a lotus-like, nanorough surface, while ATR-FTIR spectra confirm surface fluorocarbon moieties. The performance of so-treated materials lends itself to the application of chemical protective apparel, while the simplicity of the treatment bodes well for potential commercialization. C1 [Lovingood, Derek D.] Oak Ridge Inst Sci & Educ, Belcamp, MD 21017 USA. [Salter, W. Bruce; Griffith, Kara R.; Simpson, Katherine M.] Univesal Technol Corp, Dayton, OH 45432 USA. [Hearn, John D.; Owens, Jeffery R.] Air Force Res Lab, Airbase Technol Div, Tyndall AFB, FL 32403 USA. RP Lovingood, DD (reprint author), Oak Ridge Inst Sci & Educ, 4692 Millennium Dr,Ste 101, Belcamp, MD 21017 USA. EM derek.lovingood.ctr@us.af.mil FU Postgraduate Research Participation Program at the Air Force Research Laboratory FX This research was supported in part by an appointment to the Postgraduate Research Participation Program at the Air Force Research Laboratory administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement between the U.S. Department of Energy and the Air Force Research Laboratory, Materials and Manufacturing Directorate, Airbase Technologies Division (AFRL/RXQ). NR 33 TC 8 Z9 8 U1 0 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD DEC 3 PY 2013 VL 29 IS 48 BP 15043 EP 15050 DI 10.1021/la403266r PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 266CJ UT WOS:000327999600036 PM 24219872 ER PT J AU Ismail, HM O'Neill, PM Hong, DW Finn, RD Henderson, CJ Wright, AT Cravatt, BF Hemingway, J Paine, MJI AF Ismail, Hanafy M. O'Neill, Paul M. Hong, David W. Finn, Robert D. Henderson, Colin J. Wright, Aaron T. Cravatt, Benjamin F. Hemingway, Janet Paine, Mark J. I. TI Pyrethroid activity-based probes for profiling cytochrome P450 activities associated with insecticide interactions SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE insecticide resistance; drug metabolism; interactome; malaria ID IN-VIVO; PROTEIN; B(5); DELETION; RAT; IDENTIFICATION; METABOLISM; MECHANISMS; EXPRESSION; CHEMISTRY AB Pyrethroid insecticides are used to control diseases spread by arthropods. We have developed a suite of pyrethroid mimetic activity-based probes (PyABPs) to selectively label and identify P450s associated with pyrethroid metabolism. The probes were screened against pyrethroid-metabolizing and nonmetabolizing mosquito P450s, as well as rodent microsomes, to measure labeling specificity, plus cytochrome P450 oxidoreductase and b(5) knockout mouse livers to validate P450 activation and establish the role for b5 in probe activation. Using PyABPs, we were able to profile active enzymes in rat liver microsomes and identify pyrethroid-metabolizing enzymes in the target tissue. These included P450s as well as related detoxification enzymes, notably UDP-glucuronosyltransferases, suggesting a network of associated pyrethroid-metabolizing enzymes, or "pyrethrome." Considering the central role P450s play in metabolizing insecticides, we anticipate that PyABPs will aid in the identification and profiling of P450s associated with insecticide pharmacology in a wide range of species, improving understanding of P450-insecticide interactions and aiding the development of unique tools for disease control. C1 [Ismail, Hanafy M.; Hemingway, Janet; Paine, Mark J. I.] Univ Liverpool Liverpool Sch Trop Med, Liverpool L3 5QA, Merseyside, England. [Ismail, Hanafy M.] Univ Alexandria, Dept Chem & Technol Pesticides, Alexandria, Egypt. [O'Neill, Paul M.; Hong, David W.] Univ Liverpool, Dept Chem, Liverpool L69 7ZD, Merseyside, England. [Finn, Robert D.; Henderson, Colin J.] Univ Dundee, Med Res Inst, Div Canc Res, Dundee DD1 9SY, Scotland. [Finn, Robert D.] Northumbria Univ, Dept Appl Sci, Newcastle Upon Tyne NE1 8ST, Tyne & Wear, England. [Wright, Aaron T.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Cravatt, Benjamin F.] Scripps Res Inst, Skaggs Inst Chem Biol, La Jolla, CA 92037 USA. [Cravatt, Benjamin F.] Scripps Res Inst, Dept Physiol Chem, La Jolla, CA 92037 USA. RP Hemingway, J (reprint author), Univ Liverpool Liverpool Sch Trop Med, Liverpool L3 5QA, Merseyside, England. EM hemingway@liverpool.ac.uk; M.J.Paine@liverpool.ac.uk RI Paine, Mark John Ingraham/D-3360-2013; OI Hemingway, Janet/0000-0002-3200-7173; Henderson, Colin/0000-0002-4764-639X; Wright, Aaron/0000-0002-3172-5253; Paine, Mark John Ingraham/0000-0003-2061-7713; Ismail , Hanafy /0000-0002-9953-9588 FU Innovative Vector Control Consortium; William Hesketh Leverhulme foundation; Cancer Research UK programme grant [C4639/A12330]; National Institutes of Health [CA87660, GM103493, CA087660] FX The authors were funded by the Innovative Vector Control Consortium (M.J.I.P., H. M. I., J.H.), the William Hesketh Leverhulme foundation (H. M. I.), a Cancer Research UK programme grant (C4639/A12330 to C.J.H. and R. D. F.) and National Institutes of Health CA87660 (to B. F. C. and A. T. W.), GM103493 (to A. T. W.) and CA087660 (to B.F.C.). NR 35 TC 8 Z9 8 U1 3 U2 48 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD DEC 3 PY 2013 VL 110 IS 49 BP 19766 EP 19771 DI 10.1073/pnas.1320185110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 262OJ UT WOS:000327744900036 PM 24248381 ER PT J AU Rath, P Huang, CD Wang, T Wang, TZ Li, HL Prados-Rosales, R Elemento, O Casadevall, A Nathan, CF AF Rath, Poonam Huang, Chengdong Wang, Tao Wang, Tianzhi Li, Huilin Prados-Rosales, Rafael Elemento, Olivier Casadevall, Arturo Nathan, Carl F. TI Genetic regulation of vesiculogenesis and immunomodulation in Mycobacterium tuberculosis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE TLR2; macrophages ID OUTER-MEMBRANE VESICLES; PROTEIN EXPORT; PSEUDOMONAS-AERUGINOSA; IN-VITRO; MACROPHAGES; PROTECTION; RESPONSES; DEFENSE; VACCINATION; ACTIVATION AB Mycobacterium tuberculosis (Mtb) restrains immune responses well enough to escape eradication but elicits enough immunopathology to ensure its transmission. Here we provide evidence that this host-pathogen relationship is regulated in part by a cytosolic, membrane-associated protein with a unique structural fold, encoded by the Mtb gene rv0431. The protein acts by regulating the quantity of Mtb-derived membrane vesicles bearing Toll-like receptor 2 ligands, including the lipoproteins LpqH and SodC. We propose that rv0431 be named "vesiculogenesis and immune response regulator." C1 [Rath, Poonam; Nathan, Carl F.] Weill Cornell Med Coll, Dept Immunol & Microbiol, New York, NY 10065 USA. [Elemento, Olivier] Weill Cornell Med Coll, Dept Physiol & Biophys, New York, NY 10065 USA. [Rath, Poonam; Nathan, Carl F.] Cornell Univ, Weill Grad Sch Med Sci, Program Immunol & Microbial Pathogenesis, New York, NY 10065 USA. [Huang, Chengdong; Li, Huilin] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [Wang, Tao; Li, Huilin] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. [Wang, Tianzhi] Univ Texas Med Branch, Sealy Ctr Struct Biol & Mol Biophys, Galveston, TX 77555 USA. [Prados-Rosales, Rafael; Casadevall, Arturo] Albert Einstein Coll Med, Dept Microbiol & Immunol, Bronx, NY 10461 USA. RP Nathan, CF (reprint author), Weill Cornell Med Coll, Dept Immunol & Microbiol, New York, NY 10065 USA. EM cnathan@med.cornell.edu RI Prados-Rosales, Rafael/B-1240-2016 FU Milstein Program in Chemical Biology of Infectious Disease; National Institutes of Health [R01 AI70285]; Bill and Melinda Gates Foundation; William Randolph Hearst Foundation FX We thank X. Jiang for help with mouse experiments, K. Burns-Huang and A. Ding for discussions, R. Bryk, M. Braunstein and J. Belisle for antibodies, E. Pamer for TLR2-knockout mice, D. Schnappinger and S. Ehrt for gateway vectors, and J. Schneider and M. Glickman for backbone plasmids pMVB and pJSMG. This work was supported by the Milstein Program in Chemical Biology of Infectious Disease (C.N.) and National Institutes of Health Grant R01 AI70285 (to H. L.). A. C. and R.P.-R. were supported by a grant from the Bill and Melinda Gates Foundation. The Weill Cornell Medical College Department of Microbiology and Immunology is supported by the William Randolph Hearst Foundation. NR 48 TC 19 Z9 19 U1 1 U2 14 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD DEC 3 PY 2013 VL 110 IS 49 BP E4790 EP E4797 DI 10.1073/pnas.1320118110 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 262OJ UT WOS:000327744900011 PM 24248369 ER PT J AU Bartolome, F Bonilla, CM Herrero-Albillos, J Calvo-Almazan, I Castan, C Weschke, E Schmitz, D Paudyal, D Mudryk, Y Pecharsky, V Gschneidner, KA Stunault, A Garcia, LM AF Bartolome, F. Bonilla, C. M. Herrero-Albillos, J. Calvo-Almazan, I. Castan, C. Weschke, E. Schmitz, D. Paudyal, D. Mudryk, Y. Pecharsky, V. Gschneidner, K. A., Jr. Stunault, A. Garcia, L. M. TI Short-range magnetic correlations and parimagnetism in RCo2 SO EUROPEAN PHYSICAL JOURNAL B LA English DT Article ID POLARIZED NEUTRON-DIFFRACTION; QUANTUM PHASE-TRANSITIONS; SPIN FLUCTUATIONS; PARAMAGNETIC ERCO2; RARE REGIONS; BEHAVIOR; SCATTERING; TEMPERATURE; ALLOYS; HOCO2 AB X-ray circular magnetic dichroism, polarized neutron diffraction, ac susceptibility, and Seebeck effect have been measured for several members of the RCo2 series (R = Ho, Tm, Er) as a function of temperature and applied magnetic field. The experimental results show robust parimagnetism (a general behaviour along the RCo2 series with R being a heavy rare earth ion) and two reversal temperatures in some systems, which is an unexpected result. Polarised neutron diffraction show differences between results obtained on single crystals or polycrystalline ingots. We propose an interpretation of parimagnetic RCo2 as a Griffiths phase of the high temperature, magnetically ordered, amorphous RCo2 phase. C1 [Bartolome, F.; Bonilla, C. M.; Herrero-Albillos, J.; Calvo-Almazan, I.; Castan, C.; Garcia, L. M.] Univ Zaragoza, CSIC, Inst Ciencia Mat Aragon, E-50009 Zaragoza, Spain. [Bartolome, F.; Bonilla, C. M.; Herrero-Albillos, J.; Calvo-Almazan, I.; Castan, C.; Garcia, L. M.] Univ Zaragoza, CSIC, Dept Fis Mat Condensada, E-50009 Zaragoza, Spain. [Herrero-Albillos, J.] Fdn ARAID, Zaragoza 50004, Spain. [Herrero-Albillos, J.] Ctr Univ Defensa, Zaragoza 50090, Spain. [Calvo-Almazan, I.; Stunault, A.] Inst Max Von Laue Paul Langevin, F-38042 Grenoble, France. [Weschke, E.; Schmitz, D.] Helmholtz Zentrum Berlin Mat & Energie GmbH, D-12489 Berlin, Germany. [Paudyal, D.; Mudryk, Y.; Pecharsky, V.; Gschneidner, K. A., Jr.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Mudryk, Y.; Pecharsky, V.; Gschneidner, K. A., Jr.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Bartolome, F (reprint author), Univ Zaragoza, CSIC, Inst Ciencia Mat Aragon, Pedro Cerbuna 12, E-50009 Zaragoza, Spain. EM bartolom@unizar.es RI Bartolome, Fernando/K-1700-2014; Herrero-Albillos, Julia/I-5462-2012; Garcia Vinuesa, Luis Miguel /L-5226-2014; Herrero-Albillos, Julia/B-9837-2009 OI Bartolome, Fernando/0000-0002-0047-1772; Herrero-Albillos, Julia/0000-0002-0901-8341; Herrero-Albillos, Julia/0000-0002-0901-8341 FU MINECO [MAT2011/23791]; DGA IMANA; FEDER program; European Social Fund; FPI; Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the Office of Science, U.S. Department of Energy [DE-AC02-07CH11358]; Iowa State University FX Finantial support from MINECO MAT2011/23791 and DGA IMANA projects, partially funded by the FEDER program and the European Social Fund is acknowledged. C. M. Bonilla acknowledges a FPI predoctoral grant. Work at the Ames Laboratory is supported by the Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the Office of Science, U.S. Department of Energy under Contract No. DE-AC02-07CH11358 with Iowa State University. Authors would like to acknowledge the use of Servicio General de Apoyo a la Investigacion-SAI, Universidad de Zaragoza. NR 56 TC 4 Z9 4 U1 4 U2 39 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6028 EI 1434-6036 J9 EUR PHYS J B JI Eur. Phys. J. B PD DEC 2 PY 2013 VL 86 IS 12 AR 489 DI 10.1140/epjb/e2013-30968-7 PG 9 WC Physics, Condensed Matter SC Physics GA AH2VM UT WOS:000335979900002 ER PT J AU Wilson, CM Rodriguez, M Johnson, CM Martin, SL Chu, TM Wolfinger, RD Hauser, LJ Land, ML Klingeman, DM Syed, MH Ragauskas, AJ Tschaplinski, TJ Mielenz, JR Brown, SD AF Wilson, Charlotte M. Rodriguez, Miguel, Jr. Johnson, Courtney M. Martin, Stanton L. Chu, Tzu Ming Wolfinger, Russ D. Hauser, Loren J. Land, Miriam L. Klingeman, Dawn M. Syed, Mustafa H. Ragauskas, Arthur J. Tschaplinski, Timothy J. Mielenz, Jonathan R. Brown, Steven D. TI Global transcriptome analysis of Clostridium thermocellum ATCC 27405 during growth on dilute acid pretreated Populus and switchgrass SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Genome; Reannotation; Biomass; Elemental composition; RNA-seq; Microarray; Phosphate; Normalization; Transcriptomics ID QUANTITATIVE PROTEOMIC ANALYSIS; RNA-SEQ DATA; BIOMASS RECALCITRANCE; CELLULOSE UTILIZATION; BIOFUELS PRODUCTION; ESCHERICHIA-COLI; RE-ANNOTATION; BIO-ETHANOL; PST OPERON; GENOME AB Background: The thermophilic anaerobe Clostridium thermocellum is a candidate consolidated bioprocessing (CBP) biocatalyst for cellulosic ethanol production. The aim of this study was to investigate C. thermocellum genes required to ferment biomass substrates and to conduct a robust comparison of DNA microarray and RNA sequencing (RNA-seq) analytical platforms. Results: C. thermocellum ATCC 27405 fermentations were conducted with a 5 g/L solid substrate loading of either pretreated switchgrass or Populus. Quantitative saccharification and inductively coupled plasma emission spectroscopy (ICP-ES) for elemental analysis revealed composition differences between biomass substrates, which may have influenced growth and transcriptomic profiles. High quality RNA was prepared for C. thermocellum grown on solid substrates and transcriptome profiles were obtained for two time points during active growth (12 hours and 37 hours postinoculation). A comparison of two transcriptomic analytical techniques, microarray and RNA-seq, was performed and the data analyzed for statistical significance. Large expression differences for cellulosomal genes were not observed. We updated gene predictions for the strain and a small novel gene, Cthe_3383, with a putative AgrD peptide quorum sensing function was among the most highly expressed genes. RNA-seq data also supported different small regulatory RNA predictions over others. The DNA microarray gave a greater number (2,351) of significant genes relative to RNA-seq (280 genes when normalized by the kernel density mean of M component (KDMM) method) in an analysis of variance (ANOVA) testing method with a 5% false discovery rate (FDR). When a 2-fold difference in expression threshold was applied, 73 genes were significantly differentially expressed in common between the two techniques. Sulfate and phosphate uptake/utilization genes, along with genes for a putative efflux pump system were some of the most differentially regulated transcripts when profiles for C. thermocellum grown on either pretreated switchgrass or Populus were compared. Conclusions: Our results suggest that a high degree of agreement in differential gene expression measurements between transcriptomic platforms is possible, but choosing an appropriate normalization regime is essential. C1 [Wilson, Charlotte M.; Rodriguez, Miguel, Jr.; Johnson, Courtney M.; Hauser, Loren J.; Land, Miriam L.; Klingeman, Dawn M.; Syed, Mustafa H.; Tschaplinski, Timothy J.; Mielenz, Jonathan R.; Brown, Steven D.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Wilson, Charlotte M.; Rodriguez, Miguel, Jr.; Johnson, Courtney M.; Hauser, Loren J.; Land, Miriam L.; Klingeman, Dawn M.; Syed, Mustafa H.; Ragauskas, Arthur J.; Tschaplinski, Timothy J.; Mielenz, Jonathan R.; Brown, Steven D.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Martin, Stanton L.; Chu, Tzu Ming; Wolfinger, Russ D.] SAS Inst, Cary, NC 27513 USA. [Ragauskas, Arthur J.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. RP Brown, SD (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM brownsd@ornl.gov RI Klingeman, Dawn/B-9415-2012; Land, Miriam/A-6200-2011; Brown, Steven/A-6792-2011; OI Klingeman, Dawn/0000-0002-4307-2560; Land, Miriam/0000-0001-7102-0031; Brown, Steven/0000-0002-9281-3898; Tschaplinski, Timothy/0000-0002-9540-6622; Ragauskas, Arthur/0000-0002-3536-554X FU Office of Biological and Environmental Research in the DOE Office of Science through the BESC; DOE [DE-AC05-00OR22725]; DOE Bioenergy Research Center FX The authors gratefully acknowledge Brian Davison (ORNL) for critical review of the manuscript. The authors thank Kelsey Yee (ORNL), Janet Westpheling (University of Georgia, Athens, GA, USA), Lee Lynd (Dartmouth College, Hanover, NH, USA), and Edward Bayer (Weizmann Institute of Science, Rehovot, Israel) for helpful discussions. Sagar Utturkar (University of Tennessee, Knoxville, TN, USA) provided technical assistance with sequence data. This work was supported by the Office of Biological and Environmental Research in the DOE Office of Science through the BESC, a DOE Bioenergy Research Center. ORNL is managed by UT-Battelle, LLC, Oak Ridge, TN, USA, for the DOE under contract DE-AC05-00OR22725. NR 69 TC 25 Z9 25 U1 1 U2 52 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD DEC 2 PY 2013 VL 6 AR 179 DI 10.1186/1754-6834-6-179 PG 18 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA 292PD UT WOS:000329913300001 PM 24295562 ER PT J AU Baer, H Barger, V Huang, PS Mickelson, D Mustafayev, A Sreethawong, W Tata, X AF Baer, Howard Barger, Vernon Huang, Peisi Mickelson, Dan Mustafayev, Azar Sreethawong, Warintorn Tata, Xerxes TI Radiatively-driven natural supersymmetry at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology; Hadronic Colliders ID FERMILAB TEVATRON COLLIDER; CONSTRAINED MINIMAL SUPERSYMMETRY; NONUNIVERSAL HIGGS MASSES; GRAND UNIFIED THEORIES; LOCAL SUPERSYMMETRY; PBARP COLLIDERS; STANDARD MODEL; PPBAR COLLIDER; SQUARK DECAYS; SUPERGRAVITY AB Radiatively-driven natural supersymmetry (RNS) potentially reconciles the Z and Higgs boson masses close to similar to 100GeV with gluinos and squarks lying beyond the TeV scale. Requiring no large cancellations at the electroweak scale in constructing M-Z = 91.2 GeV while maintaining a light Higgs scalar with m(h) similar or equal to 125 GeV implies a sparticle mass spectrum including light higgsinos with mass similar to 100 - 300 GeV, electroweak gauginos in the 300 - 1200 GeV range, gluinos at 1-4 TeV and top/bottom squarks in the 1-4 TeV range (probably beyond LHC reach), while first/second generation matter scalars can exist in the 5-30 TeV range (far beyond LHC reach). We investigate several characteristic signals for RNS at LHC14. Gluino pair production yields a reach up to m((g) over tilde) similar to 1.7 TeV for 300 fb(-1). Wino pair production - pp -> (W) over tilde (2)(Z) over tilde (4) and (W) over tilde (2)(W) over tilde (2) - leads to a unique same-sign diboson (SSdB) signature accompanied by modest jet activity from daughter higgsino decays; this signature provides the best reach up to m((g) over tilde) similar to 2.1 TeV within this framework. Wino pair production also leads to final states with (WZ -> 3l) + E-T(miss) as well as 4l + E-T(miss) which give confirmatory signals up to m((g) over tilde) similar to 1.4 TeV. Directly produced light higgsinos yield a clean, soft trilepton signature (due to very low visible energy release) which can be visible, but only for a not-too-small a (Z) over tilde (2)-(Z) over tilde (1) mass gap. The clean SSdB signal -as well as the distinctive mass shape of the dilepton mass distribution from (Z) over tilde (2,3)->(Z) over tilde (1)ll decays if this is accessible - will mark the presence of light higgsinos which are necessary for natural SUSY. While an e(+)e(-) collider operating with root s similar to 600GeV should unequivocally reveal the predicted light higgsinos, the RNS model with m(1/2) greater than or similar to 1 TeV may elude all LHC14 search strategies even while maintaining a high degree of electroweak naturalness. C1 [Baer, Howard; Mickelson, Dan] Univ Oklahoma, Dept Phys & Astron, Norman, OK 73019 USA. [Barger, Vernon] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Huang, Peisi] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Huang, Peisi] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Mustafayev, Azar; Tata, Xerxes] Univ Hawaii, Dept Phys & Astron, Honolulu, HI 96822 USA. [Sreethawong, Warintorn] Suranaree Univ Technol, Sch Phys, Nakhon Ratchasima 30000, Thailand. RP Baer, H (reprint author), Univ Oklahoma, Dept Phys & Astron, Norman, OK 73019 USA. EM baer@nhn.ou.edu; barger@pheno.wisc.edu; peisi@uchicago.edu; mickelso@nhn.ou.edu; azar@phys.hawaii.edu; wsreethawong@hotmail.com; tata@phys.hawaii.edu OI Huang, Peisi/0000-0003-3360-2641 FU U.S. Department of Energy; Suranaree University of Technology; Higher Education Research Promotion and National Research University Project of Thailand, Office of the Higher Education Commission FX AM would like to thank FTPI at the University of Minnesota for hospitality during final stages of the project. This work was supported in part by grants from the U.S. Department of Energy, by Suranaree University of Technology, and by the Higher Education Research Promotion and National Research University Project of Thailand, Office of the Higher Education Commission. NR 100 TC 25 Z9 25 U1 0 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD DEC 2 PY 2013 IS 12 AR UNSP 013 DI 10.1007/JHEP12(2013)013 PG 35 WC Physics, Particles & Fields SC Physics GA 278MI UT WOS:000328894000008 ER PT J AU Armstrong, AM Kelchner, K Nakamura, S DenBaars, SP Speck, JS AF Armstrong, A. M. Kelchner, K. Nakamura, S. DenBaars, S. P. Speck, J. S. TI Influence of growth temperature and temperature ramps on deep level defect incorporation in m-plane GaN SO APPLIED PHYSICS LETTERS LA English DT Article ID CARBON; SILICON AB The dependence of deep level defect incorporation in m-plane GaN films grown by metal-organic chemical vapor deposition on bulk m-plane GaN substrates as a function of growth temperature (T-g) and T-g ramping method was investigated using deep level optical spectroscopy. Understanding the influence of T-g on GaN deep level incorporation is important for InGaN/GaN multi-quantum well (MQW) light emitting diodes (LEDs) and laser diodes (LDs) because GaN quantum barrier (QB) layers are grown much colder than thin film GaN to accommodate InGaN QW growth. Deep level spectra of low T-g (800 degrees C) GaN films grown under QB conditions were compared to deep level spectra of high T-g (1150 degrees C) GaN. Reducing T-g, increased the defect density significantly (>50x) through introduction of emergent deep level defects at 2.09 eV and 2.9 eV below the conduction band minimum. However, optimizing growth conditions during the temperature ramp when transitioning from high to low T-g substantially reduced the density of these emergent deep levels by approximately 40%. The results suggest that it is important to consider the potential for non-radiative recombination in QBs of LED or LD active regions, and tailoring the transition from high T-g GaN growth to active layer growth can mitigate such non-radiative channels. (C) 2013 AIP Publishing LLC. C1 [Armstrong, A. M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Kelchner, K.; Nakamura, S.; DenBaars, S. P.] Univ Calif Santa Barbara, Dept Elect & Comp Engn, Santa Barbara, CA 93106 USA. [Nakamura, S.; DenBaars, S. P.; Speck, J. S.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. RP Armstrong, AM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM aarmstr@sandia.gov FU Sandia's Solid-State Lighting Science Energy Frontier Research Center; Department of Energy Office of Basic Energy Science; Center for Energy Efficient Materials (CEEM), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001009]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The DLOS work at SNL was supported by Sandia's Solid-State Lighting Science Energy Frontier Research Center, sponsored by the Department of Energy Office of Basic Energy Science. The semiconductor epitaxy work at UCSB is supported by the Center for Energy Efficient Materials (CEEM), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001009. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 14 TC 8 Z9 8 U1 6 U2 48 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 2 PY 2013 VL 103 IS 23 AR 232108 DI 10.1063/1.4841575 PG 4 WC Physics, Applied SC Physics GA 274VS UT WOS:000328634900043 ER PT J AU Moseley, J Al-Jassim, MM Moutinho, HR Guthrey, HL Metzger, WK Ahrenkiel, RK AF Moseley, J. Al-Jassim, M. M. Moutinho, H. R. Guthrey, H. L. Metzger, W. K. Ahrenkiel, R. K. TI Explanation of red spectral shifts at CdTe grain boundaries SO APPLIED PHYSICS LETTERS LA English DT Article ID RADIATIVE RECOMBINATION; CADMIUM TELLURIDE; SOLAR-CELLS; EFFICIENCY; BAND; PHOTOLUMINESCENCE; DISLOCATIONS; EMISSION; DEFECTS; DONORS AB We use cathodoluminescence spectrum imaging to investigate the nanoscale properties of CdTe thin-films for solar cells deposited by close-spaced sublimation. Luminescence emission is detected (bands) at similar to 1.32 eV and similar to 1.50 eV, which are consistent with Z- and Y-bands. For the grains in the as-deposited films, there is a significant redshift in the transition energies near the grain boundaries. The high grain boundary recombination velocity and the donor-acceptor pair (DAP) mechanism of the Z-band transition account for the contrast between grain boundaries and the grain interior. By applying DAP theory, we estimate the concentration of the shallow donor species participating in the Z-band transition to be similar to 10(17) cm(-3). (C) 2013 AIP Publishing LLC. C1 [Moseley, J.; Al-Jassim, M. M.; Moutinho, H. R.; Guthrey, H. L.; Metzger, W. K.; Ahrenkiel, R. K.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Moseley, J.; Ahrenkiel, R. K.] Colorado Sch Mines, Golden, CO 80401 USA. RP Moseley, J (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. The authors acknowledge the late Manuel Jesus (M.J.) Romero for his pioneering work to establish the CL spectrum imaging technique at NREL. NR 26 TC 6 Z9 6 U1 0 U2 30 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 2 PY 2013 VL 103 IS 23 AR 233103 DI 10.1063/1.4838015 PG 4 WC Physics, Applied SC Physics GA 274VS UT WOS:000328634900071 ER PT J AU Shao, JY Zakharov, DN Edmunds, C Malis, O Manfra, MJ AF Shao, Jiayi Zakharov, Dmitri N. Edmunds, Colin Malis, Oana Manfra, Michael J. TI Homogeneous AlGaN/GaN superlattices grown on free-standing (1(1)over-bar00) GaN substrates by plasma-assisted molecular beam epitaxy SO APPLIED PHYSICS LETTERS LA English DT Article ID LIGHT-EMITTING-DIODES; NITRIDE AB Two-dimensional and homogeneous growth of m-plane AlGaN by plasma-assisted molecular beam epitaxy has been realized on free-standing (1 (1) over bar 00) GaN substrates by implementing high metal-to-nitrogen (III/N) flux ratio. AlN island nucleation, often reported for m-plane AlGaN under nitrogen-rich growth conditions, is suppressed at high III/N flux ratio, highlighting the important role of growth kinetics for adatom incorporation. The homogeneity and microstructure of m-plane AlGaN/GaN superlattices are assessed via a combination of scanning transmission electron microscopy and high resolution transmission electron microscopy (TEM). The predominant defects identified in dark field TEM characterization are short basal plane stacking faults (SFs) bounded by either Frank-Shockley or Frank partial dislocations. In particular, the linear density of SFs is approximately 5 x 10(-5) cm(-1), and the length of SFs is less than 15 nm. (C) 2013 AIP Publishing LLC. C1 [Shao, Jiayi; Malis, Oana; Manfra, Michael J.] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Shao, Jiayi; Edmunds, Colin; Malis, Oana; Manfra, Michael J.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Zakharov, Dmitri N.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Manfra, Michael J.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Manfra, Michael J.] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. RP Shao, JY (reprint author), Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. RI Zakharov, Dmitri/F-4493-2014 FU NSF [ECCS-1001431, ECCS 1253720, DMR-1206919]; Defense Advanced Research Project Agency (DARPA) [D11PC20027]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the NSF awards ECCS-1001431, ECCS 1253720, and DMR-1206919 and from the Defense Advanced Research Project Agency (DARPA) under Contract No. D11PC20027. Part of this research was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 28 TC 7 Z9 7 U1 2 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 2 PY 2013 VL 103 IS 23 AR UNSP 232103 DI 10.1063/1.4836975 PG 4 WC Physics, Applied SC Physics GA 274VS UT WOS:000328634900038 ER PT J AU Zakutayev, A Perry, NH Mason, TO Ginley, DS Lany, S AF Zakutayev, Andriy Perry, Nicola H. Mason, Thomas O. Ginley, David S. Lany, Stephan TI Non-equilibrium origin of high electrical conductivity in gallium zinc oxide thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID PULSED-LASER DEPOSITION; GA-DOPED ZNO; DEFECTS; TEMPERATURE; BULK AB Non-equilibrium state defines physical properties of materials in many technologies, including architectural, metallic, and semiconducting amorphous glasses. In contrast, crystalline electronic and energy materials, such as transparent conductive oxides (TCO), are conventionally thought to be in equilibrium. Here, we demonstrate that high electrical conductivity of crystalline Ga-doped ZnO TCO thin films occurs by virtue of metastable state of their defects. These results imply that such defect metastability may be important in other functional oxides. This finding emphasizes the need to understand and control non-equilibrium states of materials, in particular, their metastable defects, for the design of novel functional materials. (C) 2013 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [Zakutayev, Andriy; Ginley, David S.; Lany, Stephan] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Perry, Nicola H.; Mason, Thomas O.] Northwestern Univ, Evanston, IL 60208 USA. RP Zakutayev, A (reprint author), Natl Renewable Energy Lab, 15013 Denver W Pkwy, Golden, CO 80401 USA. EM andriy.zakutayev@nrel.gov RI Mason, Thomas/B-7528-2009 OI Zakutayev, Andriy/0000-0002-3054-5525; Lany, Stephan/0000-0002-8127-8885; FU U.S. Department of Energy [DE-AC36-08GO28308] FX This research was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 to the National Renewable Energy Laboratory (NREL). The theoretical calculations and the thin film experiments were supported by the Office of Energy Efficiency and Renewable Energy, Solar Energy Technology Program. The in-situ van der Pauw measurements were supported by the Office of Science, Basic Energy Science Program, as a part of the Energy Frontier Research Center "Center for Inverse Design". Useful discussions with P. F. Ndione, A. Adler, and J. D. Perkins are gratefully acknowledged. NR 30 TC 28 Z9 28 U1 5 U2 48 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD DEC 2 PY 2013 VL 103 IS 23 AR 232106 DI 10.1063/1.4841355 PG 4 WC Physics, Applied SC Physics GA 274VS UT WOS:000328634900041 ER PT J AU Cheung, C Roberts, HL AF Cheung, Clifford Roberts, Hannes L. TI Higgs mass from D-terms: a litmus test SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology AB We explore supersymmetric theories in which the Higgs mass is boosted by the non-decoupling D-terms of an extended U(1)(X) gauge symmetry, defined here to be a general linear combination of hypercharge, baryon number, and lepton number. Crucially, the gauge coupling, g(X), is bounded from below to accommodate the Higgs mass, while the quarks and leptons are required by gauge invariance to carry non-zero charge under U(1)(X). This induces an irreducible rate, sigma BR, for pp -> X -> ll relevant to existing and future resonance searches, and gives rise to higher dimension operators that are stringently constrained by precision electroweak measurements. Combined, these bounds define a maximally allowed region in the space of observables, (sigma BR, m(X)), outside of which is excluded by naturalness and experimental limits. If natural supersymmetry utilizes non-decoupling D-terms, then the associated X boson can only be observed within this window, providing a model independent 'litmus test' for this broad class of scenarios at the LHC. Comparing limits, we find that current LHC results only exclude regions in parameter space which were already disfavored by precision electroweak data. C1 [Cheung, Clifford] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Cheung, C (reprint author), Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. EM clifford.cheung@caltech.edu; alexlewisroberts@gmail.com FU Office of Science, Office of High Energy and Nuclear Physics, of the US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-0855653] FX C.C. and H. R. are supported by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the US Department of Energy under Contract DE-AC02-05CH11231, and by the National Science Foundation under grant PHY-0855653. C. C. would like to thank Josh Ruderman for useful comments. NR 23 TC 8 Z9 8 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD DEC 2 PY 2013 IS 12 AR 018 DI 10.1007/JHEP12(2013)018 PG 15 WC Physics, Particles & Fields SC Physics GA 278MM UT WOS:000328894400002 ER PT J AU Weber, CTM Leefer, N Budker, D AF Weber, C. T. M. Leefer, N. Budker, D. TI Investigation of ac Stark shifts in excited states of dysprosium relevant to testing fundamental symmetries SO PHYSICAL REVIEW A LA English DT Article ID ATOMIC DYSPROSIUM; POLARIZABILITIES; SEARCH AB We report on measurements of the differential polarizability between the nearly degenerate, opposite parity states in atomic dysprosium at 19 797.96 cm(-1), and the differential blackbody radiation induced Stark shift of these states. The differential scalar and tensor polarizabilities due to additional states were measured for the vertical bar M vertical bar = 7, ... ,10 sublevels in Dy-164 and Dy-162 and determined to be alpha((0))(BA) = 180 (45)(stat)(8)(sys) mHz/(V/cm)(2) and alpha((2))(BA) = -163 (65)(stat)(5)(sys) mHz/(V/cm)(2), respectively. The average blackbody radiation induced Stark shift of the Zeeman spectrum was measured around 300 K and found to be -34(4) mHz/K and + 29(4) mHz/K for Dy-164 and 162Dy, respectively. We conclude that ac Stark related systematics will not limit a search for variation of the fine-structure constant, using dysprosium, down to the level of |. alpha/alpha| = 2.6 x 10(-17) yr(-1), for two measurements of the transition frequency one year apart. C1 [Weber, C. T. M.] Tech Univ Berlin, D-10623 Berlin, Germany. [Weber, C. T. M.; Leefer, N.; Budker, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Budker, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Weber, CTM (reprint author), Tech Univ Berlin, D-10623 Berlin, Germany. EM ChristianTMWeber@gmail.com; naleefer@berkeley.edu; budker@berkeley.edu RI Budker, Dmitry/F-7580-2016; OI Budker, Dmitry/0000-0002-7356-4814; Leefer, Nathan/0000-0002-4940-8432 FU NSF [PHY-1068875] FX We thank Arman Cingoz, Valeriy Yashchuck, Alain Lapierre, and Tuan Nguyen for designing the Dy atomicbeam apparatus, and Justin Torgerson and Ed Marti for their assistance with the MOPA system. This project has been founded in part by NSF Grant No. PHY-1068875, NIST, LANL, and FQXi. NR 35 TC 4 Z9 4 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD DEC 2 PY 2013 VL 88 IS 6 AR 062503 DI 10.1103/PhysRevA.88.062503 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 273WV UT WOS:000328567900008 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapelain, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cutts, D Das, A Davies, G de Jong, SJ De la Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, VN Falkowski, A Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besancon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Brandt, A. Brandt, O. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapelain, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cutts, D. Das, A. Davies, G. de Jong, S. J. De la Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, V. N. Falkowski, A. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De la Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Osta, J. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Smirnov, D. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Measurement of the asymmetry in angular distributions of leptons produced in dilepton t(t)over-bar final states in p(p)over-bar collisions at root s=1.96 TeV SO PHYSICAL REVIEW D LA English DT Article ID FORWARD-BACKWARD ASYMMETRY; QUARK PAIR PRODUCTION; TO-LEADING ORDER; CHARGE ASYMMETRY; DETECTOR; TEVATRON; LHC AB We present measurements of asymmetries in angular distributions of leptons produced in t (t) over bar events in proton-antiproton collisions at the Fermilab Tevatron Collider. We consider final states where the W-+/- bosons from top quark and antiquark decays both decay into l nu (l = e, mu) resulting in oppositely charged dilepton final states with accompanying jets. Using 9.7 fb(-1) of integrated luminosity collected with the D0 detector, we find the asymmetries in lepton pseudorapidity compatible with predictions based on the standard model. C1 [Maciel, A. K. A.; Santos, A. S.] LAFEX, Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Begalli, M.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Han, L.; Jiang, P.; Liu, Y.; Yang, S.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota, Colombia. [Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, Prague, Czech Republic. [Augsten, K.; Hubacek, Z.; Hynek, V.; Simak, V.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Alton, A.; Kupco, A.; Lokajicek, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Hoeneisen, B.] Univ San Francisco, Quito, Ecuador. [Badaud, F.; Gris, Ph.] Univ Clermont Ferrand, CNRS, IN2P3, LPC, Clermont, France. [Sajot, G.; Stark, J.] Univ Grenoble 1, CNRS, IN2P3, Inst Natl Polytech Grenoble,LPSC, Grenoble, France. [Cousinou, M. -C.; Duperrin, A.; Geng, W.; Kajfasz, E.; Kermiche, S.; Nagy, E.; Osman, N.] Aix Marseille Univ, CNRS, IN2P3, CPPM, Marseille, France. 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[Brandt, O.; Deterre, C.; Hensel, C.; Mansour, J.; Meyer, J.; Peters, Y.; Quadt, A.; Shabalina, E.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Buescher, V.; Fiedler, F.; Hohlfeld, M.; Weichert, J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Nunnemann, T.; Sanders, M. P.] Univ Munich, Munich, Germany. [Beri, S. B.; Bhatnagar, V.; Dutt, S.; Kohli, J. M.] Panjab Univ, Chandigarh 160014, India. [Choudhary, B.; Dubey, A.] Univ Delhi, Delhi 110007, India. [Acharya, B. S.; Banerjee, S.; Mondal, N. K.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Gruenewald, M. W.] Univ Coll Dublin, Dublin 2, Ireland. [Cho, S. W.; Choi, S.; Jeong, M. S.; Lee, H. S.; Lim, J. K.; Park, S. K.] Korea Univ, Korea Detector Lab, Seoul, South Korea. [Camacho-Perez, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Garcia-Gonzalez, J. A.; Heredia-De la Cruz, I.; Luna-Garcia, R.; Magana-Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.] CINVESTAV, Mexico City 14000, DF, Mexico. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.; van Leeuwen, W. M.] Nikhef, Amsterdam, Netherlands. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.] Radboud Univ Nijmegen, NL-6525 ED Nijmegen, Netherlands. [Abazov, V. M.; Alexeev, G. D.; Golovanov, G.; Kharzheev, Y. N.; Malyshev, V. L.; Tokmenin, V. V.; Verkheev, A. Y.; Vertogradov, L. S.; Yatsunenko, Y. A.] Joint Inst Nucl Res, Dubna, Russia. [Gavrilov, V.; Kiselevich, I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E. E.; Bunichev, V.; Dudko, L. V.; Karmanov, D.; Kuzmin, V. A.; Merkin, M.; Perfilov, M.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Denisov, S. P.; Evdokimov, V. N.; Kozelov, A. V.; Lipaev, V. V.; Popov, A. V.; Prokopenko, N.; Razumov, I.; Shchukin, A. A.; Stoyanova, D. A.; Vasilyev, I. A.] Inst High Energy Phys, Protvino, Russia. 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V.; Blessing, S.; Hoang, T.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Bagby, L.; Baldin, B.; Bartlett, J. F.; Bellantoni, L.; Bhat, P. C.; Boehnlein, A.; Bross, A.; Bu, X. B.; Buehler, M.; Casey, B. C. K.; Cihangir, S.; Cooke, M.; Cooper, W. E.; Denisov, D.; Desai, S.; Diehl, H. T.; Diesburg, M.; Elvira, V. D.; Fisk, H. E.; Fuess, S.; Garbincius, P. H.; Ginther, G.; Greenlee, H.; Gruenendahl, S.; Gutierrez, G.; Herner, K.; Illingworth, R.; Ito, A. S.; Johnson, M.; Jonckheere, A.; Jung, A. W.; Khalatyan, N.; Lee, W. M.; Li, Q. Z.; Lincoln, D.; Lipton, R.; Lyon, A. L.; Melnitchouk, A.; Penning, B.; Podstavkov, V. M.; Rominsky, M.; Rubinov, P.; Savage, G.; Verzocchi, M.; Wang, M. H. L. S.; Xie, Y.; Yamada, R.; Yasuda, T.; Ye, Z.; Yin, H.; Youn, S. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, M.; Bazterra, V.; Gerber, C. E.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. 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[Brock, R.; Caughron, S.; Edmunds, D.; Fisher, W.; Geng, W.; Johnson, E.; Linnemann, J.; Schwienhorst, R.; Shaw, S.] Michigan State Univ, E Lansing, MI 48824 USA. [Bhatia, S.; Holzbauer, J. L.; Kraus, J.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Katsanos, I.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; de Sa, R. Lopes; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Haley, J.; Jayasinghe, A.; Severini, H.; Skubic, P.; Strauss, M.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cutts, D.; Heintz, U.; Jabeen, S.; Narain, M.; Parihar, V.; Partridge, R.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Howley, I.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), LAFEX, Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. RI Deliot, Frederic/F-3321-2014; Sharyy, Viatcheslav/F-9057-2014; Lokajicek, Milos/G-7800-2014; Dudko, Lev/D-7127-2012; Fisher, Wade/N-4491-2013; Santos, Angelo/K-5552-2012; Kupco, Alexander/G-9713-2014; Kozelov, Alexander/J-3812-2014; Lei, Xiaowen/O-4348-2014; Gutierrez, Phillip/C-1161-2011; Merkin, Mikhail/D-6809-2012; Li, Liang/O-1107-2015 OI Sharyy, Viatcheslav/0000-0002-7161-2616; Dudko, Lev/0000-0002-4462-3192; Lei, Xiaowen/0000-0002-2564-8351; Li, Liang/0000-0001-6411-6107 FU DOE, (USA); NSF (USA); CEA, (France); CNRS/IN2P3 (France); MON, (Russia); NRC KI, (Russia); RFBR (Russia); CNPq, (Brazil); FAPERJ, (Brazil); FAPESP, (Brazil); FUNDUNESP (Brazil); DAE, (India); DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (The Netherlands); STFC, (United Kingdom); Royal Society (United Kingdom); MSMT, (Czech Republic); GACR (Czech Republic); BMBF, (Germany); DFG (Germany); SFI (Ireland); Swedish Research Council (Sweden); CAS, (China); CNSF (China) FX We thank the staffs at Fermilab and collaborating institutions, and acknowledge support from the DOE and NSF (USA); CEA and CNRS/IN2P3 (France); MON, NRC KI and RFBR (Russia); CNPq, FAPERJ, FAPESP and FUNDUNESP (Brazil); DAE and DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (The Netherlands); STFC and the Royal Society (United Kingdom); MSMT and GACR (Czech Republic); BMBF and DFG (Germany); SFI (Ireland); The Swedish Research Council (Sweden); and CAS and CNSF (China). NR 67 TC 37 Z9 37 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 2 PY 2013 VL 88 IS 11 AR 112002 DI 10.1103/PhysRevD.88.112002 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274CX UT WOS:000328583800001 ER PT J AU Boughezal, R Schulze, M AF Boughezal, Radja Schulze, Markus TI t(t)over-bar + large missing energy from top-quark partners: A comprehensive study at next-to-leading order QCD SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS AB We perform a detailed study of top-quark partner production in the t (t) over bar plus large missing energy final state at the LHC, presenting results for both scalar and fermionic top-quark partners in the semileptonic and dileptonic decay modes of the top quarks. We compare the results of several simulation tools: leading order matrix elements, next-to-leading order (NLO) matrix elements, leading order plus parton shower simulations, and merged samples that contain the signal process with an additional hard jet radiated. We find that predictions from leading order plus parton shower simulations can significantly deviate from NLO QCD or LO merged samples and do not correctly model the kinematics of the t (t) over bar + E-T,E-miss signature. They are therefore not a good framework for modeling this new physics signature. On the other hand, the acceptances obtained with a merged sample of the leading-order process together with the radiation of an additional hard jet are in agreement with the NLO predictions. We also demonstrate that the scale variation of the inclusive cross section, plus that of the acceptance, does not accurately reflect the uncertainty of the cross section after cuts, which is typically larger. We show the importance of including higher-order QCD corrections when using kinematic distributions to determine the spin of the top-quark partner. C1 [Boughezal, Radja; Schulze, Markus] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. RP Boughezal, R (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. EM rboughezal@anl.gov; markus.schulze@anl.gov FU US DOE [DE-AC02-06CH11357] FX We thank Till Eifert for useful communications and input. We thank the Erwin Schrodinger International Institute for Mathematical Physics (ESI) and the Aspen Center for Physics for kind hospitality while this work was being completed. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory (Argonne). This research is supported by the US DOE under Contract No. DE-AC02-06CH11357. NR 33 TC 10 Z9 10 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 2 PY 2013 VL 88 IS 11 AR 114002 DI 10.1103/PhysRevD.88.114002 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274CX UT WOS:000328583800003 ER PT J AU Mueller, AH Xiao, BW Yuan, F AF Mueller, A. H. Xiao, Bo-Wen Yuan, Feng TI Sudakov double logarithms resummation in hard processes in the small-x saturation formalism SO PHYSICAL REVIEW D LA English DT Article ID COLOR GLASS CONDENSATE; QUASI-CLASSICAL APPROXIMATION; NONLINEAR GLUON EVOLUTION; SMALL TRANSVERSE-MOMENTUM; NUCLEUS COLLISIONS; PARTON SATURATION; BOSON PRODUCTION; PA-COLLISIONS; QCD; SCATTERING AB In this manuscript, we present a complete study of the Sudakov double logarithms resummation for various hard processes in eA and pA collisions in the small-x saturation formalism. We first employ a couple of slightly different formalisms to perform the one-loop analysis of the Higgs boson production process in pA collisions, and demonstrate that Sudakov-type logarithms arise as the leading correction and that they can be systematically resummed in addition to the usual small-x resummation. We further study the Sudakov double logarithms for other processes such as heavy quark pair production and back-to-back dijet production in eA and pA collisions through detailed calculation of the corresponding one-loop diagrams. As the most important contribution from the one-loop correction, the Sudakov factor should play an important role in the phenomenological study of saturation physics in the pA programs at RHIC and the LHC. C1 [Mueller, A. H.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Xiao, Bo-Wen] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Yuan, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Mueller, AH (reprint author), Columbia Univ, Dept Phys, New York, NY 10027 USA. RI Yuan, Feng/N-4175-2013 FU U.S. Department of Energy [DE-AC02-05CH11231] FX We thank J. W. Qiu for useful comments and discussions. This work was supported in part by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. B. X. wishes to thank Dr. S. Munier, Dr. B. Pire and the CPHT at the Ecole Polytechnique for hospitality and support during his visit when this work was finalized. NR 59 TC 32 Z9 32 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 2 PY 2013 VL 88 IS 11 AR 114010 DI 10.1103/PhysRevD.88.114010 PG 38 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274CX UT WOS:000328583800009 ER PT J AU Thorne, F Schwanda, C Adachi, I Aihara, H Asner, DM Aulchenko, V Aushev, T Bakich, AM Bala, A Bhuyan, B Bonvicini, G Bracko, M Chang, MC Chekelian, V Chen, A Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, SK Choi, Y Cinabro, D Dalseno, J Dolezal, Z Drasal, Z Dutta, D Eidelman, S Esen, S Farhat, H Fast, JE Feindt, M Ferber, T Gaur, V Gabyshev, N Gillard, R Glattauer, R Goh, YM Golob, B Haba, J Hara, T Hayasaka, K Hayashii, H Hoshi, Y Hou, WS Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Iwashita, T Jaegle, I Julius, T Kah, DH Kang, JH Kato, E Kiesling, C Kim, DY Kim, HO Kim, JB Kim, JH Kim, MJ Kim, YJ Klucar, J Ko, BR Kodys, P Krizan, P Krokovny, P Kuhr, T Lange, JS Lee, SH Libby, J Liu, C Liu, Y Lukin, P Matvienko, D Miyata, H Mizuk, R Mohanty, GB Moll, A Mori, T Nagasaka, Y Nakano, E Nakao, M Natkaniec, Z Nayak, M Ng, C Nishida, S Nitoh, O Okuno, S Oswald, C Pakhlova, G Park, H Park, HK Pestotnik, R Petric, M Piilonen, LE Prim, M Ritter, M Rostomyan, A Ryu, S Sahoo, H Saito, T Sakai, Y Sandilya, S Santelj, L Sanuki, T Savinov, V Schneider, O Schnell, G Semmler, D Senyo, K Sevior, ME Shapkin, M Shen, CP Shibata, TA Shiu, JG Shwartz, B Sibidanov, A Simon, F Sohn, YS Sokolov, A Solovieva, E Stanic, S Staric, M Tamponi, U Tanida, K Tatishvili, G Teramoto, Y Uchida, M Unno, Y Uno, S Urquijo, P Vahsen, SE Varner, G Varvell, KE Vorobyev, V Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, Y Williams, KM Won, E Yamaoka, J Yamashita, Y Yashchenko, S Yuan, CZ Zhang, ZP Zhilich, V Zupanc, A AF Thorne, F. Schwanda, C. Adachi, I. Aihara, H. Asner, D. M. Aulchenko, V. Aushev, T. Bakich, A. M. Bala, A. Bhuyan, B. Bonvicini, G. Bracko, M. Chang, M. -C. Chekelian, V. Chen, A. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, S. -K. Choi, Y. Cinabro, D. Dalseno, J. Dolezal, Z. Drasal, Z. Dutta, D. Eidelman, S. Esen, S. Farhat, H. Fast, J. E. Feindt, M. Ferber, T. Gaur, V. Gabyshev, N. Gillard, R. Glattauer, R. Goh, Y. M. Golob, B. Haba, J. Hara, T. Hayasaka, K. Hayashii, H. Hoshi, Y. Hou, W. -S. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Iwashita, T. Jaegle, I. Julius, T. Kah, D. H. Kang, J. H. Kato, E. Kiesling, C. Kim, D. Y. Kim, H. O. Kim, J. B. Kim, J. H. Kim, M. J. Kim, Y. J. Klucar, J. Ko, B. R. Kodys, P. Krizan, P. Krokovny, P. Kuhr, T. Lange, J. S. Lee, S. -H. Libby, J. Liu, C. Liu, Y. Lukin, P. Matvienko, D. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Mori, T. Nagasaka, Y. Nakano, E. Nakao, M. Natkaniec, Z. Nayak, M. Ng, C. Nishida, S. Nitoh, O. Okuno, S. Oswald, C. Pakhlova, G. Park, H. Park, H. K. Pestotnik, R. Petric, M. Piilonen, L. E. Prim, M. Ritter, M. Rostomyan, A. Ryu, S. Sahoo, H. Saito, T. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Savinov, V. Schneider, O. Schnell, G. Semmler, D. Senyo, K. Sevior, M. E. Shapkin, M. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Sibidanov, A. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Stanic, S. Staric, M. Tamponi, U. Tanida, K. Tatishvili, G. Teramoto, Y. Uchida, M. Unno, Y. Uno, S. Urquijo, P. Vahsen, S. E. Varner, G. Varvell, K. E. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, Y. Williams, K. M. Won, E. Yamaoka, J. Yamashita, Y. Yashchenko, S. Yuan, C. Z. Zhang, Z. P. Zhilich, V. Zupanc, A. CA Belle Collaboration TI Measurement of the decays B-s(0) -> J/psi phi(1020), B-s(0) -> J/psi f(2)'(1525) and B-s(0) -> J/psi K+K- at Belle SO PHYSICAL REVIEW D LA English DT Article AB We report a measurement of the branching fraction of the decay B-s(0) -> J/psi phi(1020), evidence and a branching fraction measurement for B-s(0) -> J/psi f(2)'(1525), and the determination of the total B-s(0) -> J/psi K+K- branching fraction, including the resonant and nonresonant contributions to the K+K- channel. We also determine the S-wave contribution within the phi(1020) mass region. The absolute branching fractions are B[B-s(0) -> J/psi phi(1020)] = (1.25 +/- 0.07(stat) +/- 0.08(syst) +/- 0.22(f(s))) x 10(-3), B[B-s(0) -> J/psi f(2)'(1525)] = (0.26 +/- 0.06(stat) +/- 0.02(syst) +/- 0.05(f(s))) x 10(-3), and B[B-s(0) -> J/psi K+K-] = (1.01 +/- 0.09(stat) +/- 0.10(syst) +/- 0.18(f(s))) x 10(-3), where the last systematic error is due to the branching fraction of b (b) over bar -> B-s(()*()) B-s(()*()). The branching fraction ratio is found to be B[B-s(0) -> J/psi f(2)'(1525)]/B[B-s(0) -> J/psi phi(1020)] = (21.5 +/- 4.9(stat) +/- 2.6(syst))%. All results are based on a 121. 4 fb(-1) data sample collected at the Upsilon(5S) resonance by the Belle experiment at the KEKB asymmetric-energy e(+)e(-) collider. C1 [Schnell, G.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Oswald, C.; Urquijo, P.] Univ Bonn, D-53115 Bonn, Germany. [Aulchenko, V.; Eidelman, S.; Ferber, T.; Gabyshev, N.; Krokovny, P.; Lukin, P.; Matvienko, D.; Shwartz, B.; Vorobyev, V.; Zhilich, V.] SB RAS, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, Prague 12116, Czech Republic. [Esen, S.; Liu, Y.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Rostomyan, A.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Chang, M. -C.] Fu Jen Catholic Univ, Dept Phys, Taipei 24205, Taiwan. [Lange, J. S.; Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Choi, S. -K.] Gyeongsang Natl Univ, Chinju 660701, South Korea. [Cheon, B. G.; Goh, Y. M.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Jaegle, I.; Sahoo, H.; Vahsen, S. E.; Varner, G.; Yamaoka, J.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Hara, T.; Itoh, R.; Iwasaki, Y.; Nakao, M.; Nishida, S.; Sakai, Y.; Uno, S.] High Energy Accelerator Org, KEK, Tsukuba, Ibaraki 3050801, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Hiroshima 7315193, Japan. [Schnell, G.] Ikerbasque, Bilbao 48011, Spain. [Bhuyan, B.; Dutta, D.] Indian Inst Technol, Gauhati, Assam 781039, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.; Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Thorne, F.; Schwanda, C.; Glattauer, R.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chilikin, K.; Chistov, R.; Mizuk, R.; Pakhlova, G.; Solovieva, E.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Klucar, J.; Krizan, P.; Pestotnik, R.; Petric, M.; Santelj, L.; Staric, M.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Feindt, M.; Kuhr, T.; Prim, M.; Zupanc, A.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Ko, B. R.; Lee, S. -H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Hyun, H. J.; Kah, D. H.; Kim, H. O.; Kim, M. J.; Park, H.; Park, H. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Bracko, M.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Moll, A.; Ritter, M.; Simon, F.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Mizuk, R.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Iijima, T.; Mori, T.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Iwashita, T.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Natkaniec, Z.] Henryk Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Yamashita, Y.] Nippon Dent Univ, Niigata 9518580, Japan. [Miyata, H.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.] Panjab Univ, Chandigarh 160014, India. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Liu, C.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Ryu, S.; Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Ishikawa, A.; Sibidanov, A.; Varvell, K. E.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Gaur, V.; Mohanty, G. B.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, D-857480 Garching, Germany. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Kato, E.; Saito, T.; Sanuki, T.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Ng, C.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Tokyo 1848588, Japan. [Tamponi, U.] Univ Torino, I-10124 Turin, Italy. [Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kang, J. H.; Sohn, Y. -S.] Yonsei Univ, Seoul 120749, South Korea. RP Thorne, F (reprint author), Inst High Energy Phys, A-1050 Vienna, Austria. RI Pakhlova, Galina/C-5378-2014; Solovieva, Elena/B-2449-2014; Nitoh, Osamu/C-3522-2013; Aihara, Hiroaki/F-3854-2010; Ishikawa, Akimasa/G-6916-2012; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Chilikin, Kirill/B-4402-2014; Chistov, Ruslan/B-4893-2014 OI Pakhlova, Galina/0000-0001-7518-3022; Solovieva, Elena/0000-0002-5735-4059; Aihara, Hiroaki/0000-0002-1907-5964; Krokovny, Pavel/0000-0002-1236-4667; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 10825524]; Ministry of Education, Youth and Sports of the Czech Republic [MSM0021620859]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; BK21; WCU program of the Ministry Education Science and Technology; National Research Foundation of Korea [2010-0021174, 2011-0029457, 2012-0008143, 2012R1A1A2008330]; BRL program under NRF [KRF-2011-0020333]; GSDC of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Federal Agency for Atomic Energy; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); UPV/EHU under program UFI [11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"); JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics") FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid, and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grant No. P 22742-N16; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, and No. 10825524; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. MSM0021620859; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; The BK21 and WCU program of the Ministry Education Science and Technology, National Research Foundation of Korea Grants No. 2010-0021174, No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, BRL program under NRF Grant No. KRF-2011-0020333, and GSDC of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Federal Agency for Atomic Energy; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under program UFI 11/55; the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"), and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 27 TC 3 Z9 3 U1 2 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD DEC 2 PY 2013 VL 88 IS 11 AR 114006 DI 10.1103/PhysRevD.88.114006 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 274CX UT WOS:000328583800006 ER PT J AU McDermott, D Amelang, J Reichhardt, CJO Reichhardt, C AF McDermott, D. Amelang, J. Reichhardt, C. J. Olson Reichhardt, C. TI Dynamic regimes for driven colloidal particles on a periodic substrate at commensurate and incommensurate fillings SO PHYSICAL REVIEW E LA English DT Article ID VORTEX DYNAMICS; PLASTIC-FLOW; ARRAYS; SUPERCONDUCTORS; PHASES; MONOLAYERS; VORTICES; CRYSTALS; FRICTION; DEFECTS AB We numerically examine colloidal particles driven over a muffin tin substrate. Previous studies of this model identified a variety of commensurate and incommensurate static phases in which topological defects can form domain walls, ordered stripes, superlattices, or disordered patchy regimes as a function of the filling fraction. Here, we show that the addition of an external drive to these static phases can produce distinct dynamical responses. At incommensurate fillings the flow occurs in the form of localized pulses or solitons correlated with topological defect structures. Transitions between different modes of motion can occur as a function of increasing drive. We measure the average particle velocity for specific ranges of external drive and show that changes in the velocity response correlate with changes in the topological defect arrangements. We also demonstrate that in the different dynamic phases, the particles have distinct trajectories and velocity distributions. Dynamic transitions between ordered and disordered flows exhibit hysteresis, while in strongly disordered regimes there is no hysteresis and the velocity-force curves are smooth. When stripe patterns are present, transport can occur at an angle to the driving direction. C1 [McDermott, D.; Amelang, J.; Reichhardt, C. J. Olson; Reichhardt, C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [McDermott, D.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Amelang, J.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. RP McDermott, D (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Reichhardt, Cynthia/0000-0002-3487-5089 FU NNSA of the US DoE at LANL [DE-AC52-06NA25396]; ASC Summer Workshop program at LANL FX This work was carried out under the auspices of the NNSA of the US DoE at LANL under Contract No. DE-AC52-06NA25396. D.M. and J.A. received support from the ASC Summer Workshop program at LANL. NR 69 TC 14 Z9 14 U1 2 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD DEC 2 PY 2013 VL 88 IS 6 AR 062301 DI 10.1103/PhysRevE.88.062301 PG 12 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 274KK UT WOS:000328605000008 PM 24483438 ER PT J AU Regev, I Lookman, T Reichhardt, C AF Regev, Ido Lookman, Turab Reichhardt, Charles TI Onset of irreversibility and chaos in amorphous solids under periodic shear SO PHYSICAL REVIEW E LA English DT Article ID SOFT GLASSY MATERIALS; DEFORMATION; DYNAMICS; SYSTEMS; MODEL AB A fundamental problem in the physics of amorphous materials is understanding the transition from reversible to irreversible plastic behavior and its connection to yield. Currently, continuum material modeling relies on phenomenological yield thresholds, however in many cases the transition from elastic to plastic behavior is gradual, which makes it difficult to identify an exact yield criterion. Here we show that under periodic shear, amorphous solids undergo a transition from repetitive, predictable behavior to chaotic, irregular behavior as a function of the strain amplitude. In both the periodic and chaotic regimes, localized particle rearrangements are observed. We associate the point of transition from repetitive to chaotic behavior with the yield strain and suggest that at least for oscillatory shear, yield in amorphous solids is a result of a "transition to chaos." C1 [Regev, Ido] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Regev, I (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. FU U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX We would like to thank Paul Chaikin, Colm Connaughton, Bob Ecke, Nicholas Ouellette, and Eran Bouchbinder for useful discussions. We would like to thank LANL institutional computing for resources. This work was carried out under the auspices of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 33 TC 31 Z9 31 U1 0 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD DEC 2 PY 2013 VL 88 IS 6 AR 062401 DI 10.1103/PhysRevE.88.062401 PG 9 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 274KK UT WOS:000328605000009 PM 24483455 ER PT J AU Dewald, EL Milovich, JL Michel, P Landen, OL Kline, JL Glenn, S Jones, O Kalantar, DH Pak, A Robey, HF Kyrala, GA Divol, L Benedetti, LR Holder, J Widmann, K Moore, A Schneider, MB Doppner, T Tommasini, R Bradley, DK Bell, P Ehrlich, B Thomas, CA Shaw, M Widmayer, C Callahan, DA Meezan, NB Town, RPJ Hamza, A Dzenitis, B Nikroo, A Moreno, K Van Wonterghem, B Mackinnon, AJ Glenzer, SH MacGowan, BJ Kilkenny, JD Edwards, MJ Atherton, LJ Moses, EI AF Dewald, E. L. Milovich, J. L. Michel, P. Landen, O. L. Kline, J. L. Glenn, S. Jones, O. Kalantar, D. H. Pak, A. Robey, H. F. Kyrala, G. A. Divol, L. Benedetti, L. R. Holder, J. Widmann, K. Moore, A. Schneider, M. B. Doeppner, T. Tommasini, R. Bradley, D. K. Bell, P. Ehrlich, B. Thomas, C. A. Shaw, M. Widmayer, C. Callahan, D. A. Meezan, N. B. Town, R. P. J. Hamza, A. Dzenitis, B. Nikroo, A. Moreno, K. Van Wonterghem, B. Mackinnon, A. J. Glenzer, S. H. MacGowan, B. J. Kilkenny, J. D. Edwards, M. J. Atherton, L. J. Moses, E. I. TI Early-Time Symmetry Tuning in the Presence of Cross-Beam Energy Transfer in ICF Experiments on the National Ignition Facility SO PHYSICAL REVIEW LETTERS LA English DT Article ID TARGET EXPERIMENTS; LASER AB On the National Ignition Facility, the hohlraum-driven implosion symmetry is tuned using cross-beam energy transfer (CBET) during peak power, which is controlled by applying a wavelength separation between cones of laser beams. In this Letter, we present early-time measurements of the instantaneous soft x-ray drive at the capsule using reemission spheres, which show that this wavelength separation also leads to significant CBET during the first shock, even though the laser intensities are 30X smaller than during the peak. We demonstrate that the resulting early drive P-2/P-0 asymmetry can be minimized and tuned to < 1% accuracy (well within the +/- 7.5% requirement for ignition) by varying the relative input powers between different cones of beams. These experiments also provide time-resolved measurements of CBET during the first 2 ns of the laser drive, which are in good agreement with radiation-hydrodynamics calculations including a linear CBET model. C1 [Dewald, E. L.; Milovich, J. L.; Michel, P.; Landen, O. L.; Glenn, S.; Jones, O.; Kalantar, D. H.; Pak, A.; Robey, H. F.; Divol, L.; Benedetti, L. R.; Holder, J.; Widmann, K.; Moore, A.; Schneider, M. B.; Doeppner, T.; Tommasini, R.; Bradley, D. K.; Bell, P.; Ehrlich, B.; Thomas, C. A.; Shaw, M.; Widmayer, C.; Callahan, D. A.; Meezan, N. B.; Town, R. P. J.; Hamza, A.; Dzenitis, B.; Van Wonterghem, B.; Mackinnon, A. J.; Glenzer, S. H.; MacGowan, B. J.; Kilkenny, J. D.; Edwards, M. J.; Atherton, L. J.; Moses, E. I.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Kline, J. L.; Kyrala, G. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Nikroo, A.; Moreno, K.] Gen Atom, San Diego, CA 92186 USA. RP Dewald, EL (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94550 USA. RI Michel, Pierre/J-9947-2012; MacKinnon, Andrew/P-7239-2014; Tommasini, Riccardo/A-8214-2009; OI MacKinnon, Andrew/0000-0002-4380-2906; Tommasini, Riccardo/0000-0002-1070-3565; Kline, John/0000-0002-2271-9919 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 28 TC 20 Z9 22 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD DEC 2 PY 2013 VL 111 IS 23 AR 235001 DI 10.1103/PhysRevLett.111.235001 PG 5 WC Physics, Multidisciplinary SC Physics GA 274OE UT WOS:000328615000003 PM 24476279 ER PT J AU Jacobsen, JL Berget, PE Varela, MC Vu, T Schore, NE Martin, KE Shelnutt, JA Santos, LM Medforth, CJ AF Jacobsen, John L. Berget, Patrick E. Varela, Michael C. Vu, Tony Schore, Neil E. Martin, Kathleen E. Shelnutt, John A. Santos, Luis M. Medforth, Craig J. TI Synthesis and nanostructures of 5,10,15,20-tetrakis(4-piperidyl) porphyrin SO TETRAHEDRON LA English DT Article DE Porphyrin; Water-soluble; Self-assembly; Nanostructure ID CATIONIC PORPHYRINS; SELF-METALLIZATION; DNA; COMPLEXES; NANOTUBES; MESO; INTERFACES; REDUCTION; INDUCTION; PORPHINE AB A new water-soluble porphyrin, 5,10,15,20-tetrakis(4-piperidyl)porphyrin (T(4-Pip)P), has been synthesized. T(4-Pip)P is related to the extensively studied water-soluble porphyrin 5,10,15,20-tetrakis(4-pyridyl)porphyrin (T(4-Py)P) but has substituents with different electronic and hydrogen-bonding properties and is soluble over a much larger pH range due to the higher pK(a) of its conjugate acid T(4-H-Pip)P4+. Investigations of the ionic self-assembly reactions of T(4-H-Pip)P4+ with anionic water-soluble porphyrins reveal that it forms nanoscale materials. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Jacobsen, John L.; Berget, Patrick E.; Varela, Michael C.; Vu, Tony; Schore, Neil E.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Martin, Kathleen E.] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. [Shelnutt, John A.] Univ Georgia, Dept Chem, Athens, GA 30602 USA. [Shelnutt, John A.] Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Santos, Luis M.; Medforth, Craig J.] Univ Porto, Fac Ciencias, REQUIMTE Dept Quim & Bioquim, P-4169007 Oporto, Portugal. RP Medforth, CJ (reprint author), Univ Porto, Fac Ciencias, REQUIMTE Dept Quim & Bioquim, P-4169007 Oporto, Portugal. EM craig.medforth@fc.up.pt RI Medforth, Craig/D-8210-2013 OI Medforth, Craig/0000-0003-3046-4909 FU European Union [PCOFUND-GA-2009-246542]; Foundation for Science and Technology of Portugal; Fundacao para a Ciencia e a Tecnologia, Portugal; Marie Curie Action Cofund; National Science Foundation [NSF CHE-0910870]; United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy's National Nuclear Security Administration [DEAC04-94AL85000] FX The research leading to these results has received funding from the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no PCOFUND-GA-2009-246542 and from the Foundation for Science and Technology of Portugal. C.J.M. is the recipient of a Marie Curie Fellowship from the Fundacao para a Ciencia e a Tecnologia, Portugal and the Marie Curie Action Cofund. J.L.J. and N.E.S. acknowledge support from the National Science Foundation (grant NSF CHE-0910870). Research supported by the United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. This work was performed, in part, at the Center for Integrated Nano-technologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DEAC04-94AL85000. We would like to thank Dr. Cynthia Holsclaw and Dr. William Jewell of the UC Davis Campus Mass Spectrometry Facilities for their assistance. NR 53 TC 2 Z9 2 U1 3 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0040-4020 J9 TETRAHEDRON JI Tetrahedron PD DEC 2 PY 2013 VL 69 IS 48 BP 10507 EP 10515 DI 10.1016/j.tet.2013.09.055 PG 9 WC Chemistry, Organic SC Chemistry GA 273FW UT WOS:000328521700042 ER PT J AU Lacerda, M Moore, PL Ngandu, NK Seaman, M Gray, ES Murrell, B Krishnamoorthy, M Nonyane, M Madiga, M Wibmer, CK Sheward, D Bailer, RT Gao, HM Greene, KM Karim, SSA Mascola, JR Korber, BTM Montefiori, DC Morris, L Williamson, C Seoighe, C AF Lacerda, Miguel Moore, Penny L. Ngandu, Nobubelo K. Seaman, Michael Gray, Elin S. Murrell, Ben Krishnamoorthy, Mohan Nonyane, Molati Madiga, Maphuti Wibmer, Constantinos Kurt Sheward, Daniel Bailer, Robert T. Gao, Hongmei Greene, Kelli M. Karim, Salim S. Abdool Mascola, John R. Korber, Bette T. M. Montefiori, David C. Morris, Lynn Williamson, Carolyn Seoighe, Cathal CA CAVD-NSDP Consortium TI Identification of broadly neutralizing antibody epitopes in the HIV-1 envelope glycoprotein using evolutionary models SO VIROLOGY JOURNAL LA English DT Article DE HIV; Antibodies; Neutralization sensitivity; Epitope prediction; Evolutionary model ID IMMUNODEFICIENCY-VIRUS TYPE-1; B-CELL RESPONSES; INFECTION; GP120; PHYLOGENIES; BINDING; RECOMBINATION; INDIVIDUALS; DISCOVERY; ALGORITHM AB Background: Identification of the epitopes targeted by antibodies that can neutralize diverse HIV-1 strains can provide important clues for the design of a preventative vaccine. Methods: We have developed a computational approach that can identify key amino acids within the HIV-1 envelope glycoprotein that influence sensitivity to broadly cross-neutralizing antibodies. Given a sequence alignment and neutralization titers for a panel of viruses, the method works by fitting a phylogenetic model that allows the amino acid frequencies at each site to depend on neutralization sensitivities. Sites at which viral evolution influences neutralization sensitivity were identified using Bayes factors (BFs) to compare the fit of this model to that of a null model in which sequences evolved independently of antibody sensitivity. Conformational epitopes were identified with a Metropolis algorithm that searched for a cluster of sites with large Bayes factors on the tertiary structure of the viral envelope. Results: We applied our method to ID50 neutralization data generated from seven HIV-1 subtype C serum samples with neutralization breadth that had been tested against a multi-clade panel of 225 pseudoviruses for which envelope sequences were also available. For each sample, between two and four sites were identified that were strongly associated with neutralization sensitivity (2ln(BF) > 6), a subset of which were experimentally confirmed using site-directed mutagenesis. Conclusions: Our results provide strong support for the use of evolutionary models applied to cross-sectional viral neutralization data to identify the epitopes of serum antibodies that confer neutralization breadth. C1 [Lacerda, Miguel; Seoighe, Cathal] Natl Univ Ireland Galway, Sch Math Stat & Appl Math, Galway, Ireland. [Lacerda, Miguel] Univ Cape Town, Fac Sci, Dept Stat Sci, ZA-7925 Cape Town, South Africa. [Moore, Penny L.; Gray, Elin S.; Nonyane, Molati; Madiga, Maphuti; Wibmer, Constantinos Kurt; Morris, Lynn] Natl Hlth Lab Serv, Natl Inst Communicable Dis, Ctr HIV & STIs, Johannesburg, South Africa. [Moore, Penny L.; Morris, Lynn] Univ Witwatersrand, Sch Pathol, Johannesburg, South Africa. [Ngandu, Nobubelo K.; Sheward, Daniel; Williamson, Carolyn] Univ Cape Town, Fac Hlth Sci, Div Med Virol, Inst Infect Dis & Mol Med, ZA-7925 Cape Town, South Africa. [Ngandu, Nobubelo K.; Sheward, Daniel; Williamson, Carolyn] NHLS, Cape Town, South Africa. [Seaman, Michael] Beth Israel Deaconess Med Ctr, Div Viral Pathogenesis, Harvard, MA USA. [Murrell, Ben] MRC, eHlth Res & Innovat Platform, Biomed Informat Res Div, Tygerberg, South Africa. [Murrell, Ben] Univ Stellenbosch, Dept Math Sci, Div Comp Sci, ZA-7600 Stellenbosch, South Africa. [Krishnamoorthy, Mohan; Korber, Bette T. M.] Los Alamos Natl Lab, Los Alamos, NM USA. [Bailer, Robert T.; Mascola, John R.] NIAID, Vaccine Res Ctr, NIH, Bethesda, MD 20892 USA. [Gao, Hongmei; Greene, Kelli M.; Montefiori, David C.] Duke Univ, Med Ctr, Dept Surg, Durham, NC 27710 USA. [Karim, Salim S. Abdool] Univ KwaZulu Natal, Ctr AIDS Programme Res South Africa, Durban, South Africa. [Karim, Salim S. Abdool] Columbia Univ, Ctr AIDS Programme Res South Africa, Columbia, NY USA. [Korber, Bette T. M.] Santa Fe Inst, Santa Fe, NM 87501 USA. RP Seoighe, C (reprint author), Natl Univ Ireland Galway, Sch Math Stat & Appl Math, Galway, Ireland. EM cathal.seoighe@nuigalway.ie RI Abdool Karim, Salim Safurdeen/N-5947-2013; OI Abdool Karim, Salim Safurdeen/0000-0002-4986-2133; Moore, Penny/0000-0001-8719-4028; , Carolyn/0000-0003-0125-1226; Korber, Bette/0000-0002-2026-5757; Wibmer, Constantinos Kurt/0000-0003-2329-2280; Gray, Elin/0000-0002-8613-3570 NR 57 TC 6 Z9 6 U1 1 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1743-422X J9 VIROL J JI Virol. J. PD DEC 2 PY 2013 VL 10 AR 347 DI 10.1186/1743-422X-10-347 PG 18 WC Virology SC Virology GA 276YK UT WOS:000328785400001 PM 24295501 ER PT J AU Xu, C Tian, GX Teat, SJ Liu, GK Rao, LF AF Xu, Chao Tian, Guoxin Teat, Simon J. Liu, Guokui Rao, Linfeng TI Thermodynamic and Structural Trends in Hexavalent Actinyl Cations: Complexation of Dipicolinic Acid with NpO22+ and PuO22+ in Comparison with UO22+ SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE actinides; coordination modes; structure elucidation; thermodynamics ID CALORIMETRIC DETERMINATION; INORGANIC LIGANDS; AQUEOUS-SOLUTION; EXTRACTION; PU(VI); IONS; NP(VI); U(VI); DIAMIDES; 25-DEGREES-C AB The complexation of NpO22+ and PuO22+ with dipicolinic acid (DPA) has been investigated in 0.1M NaClO4 by spectrophotometry, microcalorimetry, and single crystal diffractometry. Formation of 1:1 and 1:2 (metal/ligand molar ratio) complexes of DPA with NpO22+ and PuO22+ were identified and the thermodynamic parameters were determined and compared with those of UO22+. All three hexavalent actinyl cations form strong 1:1 DPA complexes with slightly decreasing but comparable stability constants from UO22+ to PuO22+, whereas the stability constants of the 1:2 complexes (log(2)) decrease substantially along the series (16.3 for UO2L22-, 15.17 for NpO2L22-, and 14.17 for PuO2L22- at 25 degrees C). The enthalpies of complexation for the 1:2 complexes become less exothermic from UO2L22- (-28.9kJmol(-1)), through NpO2L22- (-27.2kJmol(-1)), and to PuO2L22- (-22.7kJmol(-1)). The trends in the thermodynamic parameters are discussed in terms of the effective charge of the cations and the steric constraints in the structures of the complexes. In addition, the features of the absorption spectra, including the wavelength and intensity of the absorption bands, are related to the perturbation of the ligand field and the symmetry of the actinyl complexes. C1 [Xu, Chao; Tian, Guoxin; Rao, Linfeng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Xu, Chao] Tsinghua Univ, Inst Nucl & New Energy Technol, Beijing 100084, Peoples R China. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Liu, Guokui] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Rao, LF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM LRao@lbl.gov RI XU, CHAO/S-4253-2016 OI XU, CHAO/0000-0001-5539-4754 FU Office of Science, Office of Basic Energy Science of the US Department of Energy (DOE) at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, US DOE [DE-AC02-05CH11231]; US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences at Argonne National Laboratory [DE-AC02-06CH11357]; National Natural Science Foundation of China [21201107]; China Scholarship Council FX This work was supported by the Director, Office of Science, Office of Basic Energy Science of the US Department of Energy (DOE), under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory. Single-crystal X-ray diffraction data were collected and analyzed at the Advanced Light Source (ALS). ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, US DOE under Contract No. DE-AC02-05CH11231. G.L.'s work on the analysis of the electronic energy levels was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under contract No. DE-AC02-06CH11357 at Argonne National Laboratory. C.X. acknowledges the partial financial support from China Scholarship Council and National Natural Science Foundation of China (Grant No. 21201107). NR 43 TC 2 Z9 2 U1 3 U2 35 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD DEC 2 PY 2013 VL 19 IS 49 BP 16690 EP 16698 DI 10.1002/chem.201302119 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 257RV UT WOS:000327404700027 PM 24382695 ER PT J AU Barros, K Kato, Y AF Barros, Kipton Kato, Yasuyuki TI Efficient Langevin simulation of coupled classical fields and fermions SO PHYSICAL REVIEW B LA English DT Article ID MONTE-CARLO ALGORITHM; DOUBLE EXCHANGE MODEL; TIGHT-BINDING; SYSTEMS; STATES; ORDER; METAL AB We introduce an efficient Langevin method to study bilinear fermionic Hamiltonians interacting with classical fields. Our approach is orders of magnitude faster than previous methods when applied to very large systems with high accuracy requirements. To demonstrate the method, we study complex noncoplanar chiral spin textures on the triangular Kondo lattice model. We also explore nonequilibrium mesoscale physics such as chiral domain coarsening and Z(2) vortex annihilation. C1 [Barros, Kipton; Kato, Yasuyuki] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Barros, Kipton; Kato, Yasuyuki] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. [Kato, Yasuyuki] RIKEN, CEMS, Wako, Saitama 3510198, Japan. RP Barros, K (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kbarros@lanl.gov OI Barros, Kipton/0000-0002-1333-5972 FU NNSA of the U.S. DOE at LANL [DE-AC52-06NA25396]; LANL/LDRD Program FX We thank Ivar Martin and Cristian Batista for useful discussions. This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396 and supported by the LANL/LDRD Program. The calculations were performed using the CCS-7 Darwin cluster. NR 39 TC 12 Z9 12 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 2 PY 2013 VL 88 IS 23 AR 235101 DI 10.1103/PhysRevB.88.235101 PG 6 WC Physics, Condensed Matter SC Physics GA 273YB UT WOS:000328571100001 ER PT J AU Caviglia, AD Forst, M Scherwitzl, R Khanna, V Bromberger, H Mankowsky, R Singla, R Chuang, YD Lee, WS Krupin, O Schlotter, WF Turner, JJ Dakovski, GL Minitti, MP Robinson, J Scagnoli, V Wilkins, SB Cavill, SA Gibert, M Gariglio, S Zubko, P Triscone, JM Hill, JP Dhesi, SS Cavalleri, A AF Caviglia, A. D. Foerst, M. Scherwitzl, R. Khanna, V. Bromberger, H. Mankowsky, R. Singla, R. Chuang, Y. -D. Lee, W. S. Krupin, O. Schlotter, W. F. Turner, J. J. Dakovski, G. L. Minitti, M. P. Robinson, J. Scagnoli, V. Wilkins, S. B. Cavill, S. A. Gibert, M. Gariglio, S. Zubko, P. Triscone, J. -M. Hill, J. P. Dhesi, S. S. Cavalleri, A. TI Photoinduced melting of magnetic order in the correlated electron insulator NdNiO3 SO PHYSICAL REVIEW B LA English DT Article ID CHARGE; SPIN; TRANSITION; NICKELATE; PHASE; FILMS AB Using ultrafast resonant soft x-ray diffraction, we demonstrate photoinduced melting of antiferromagnetic order in the correlated electron insulator NdNiO3. Time-dependent analysis of the resonant diffraction spectra allows us to follow the temporal evolution of the charge imbalance between adjacent Ni sites. A direct correlation between the melting of magnetic order and charge rebalancing is found. Furthermore, we demonstrate that the magnetic ordering on the Ni and Nd sites, which are locked together in equilibrium, become decoupled during this nonthermal process. C1 [Caviglia, A. D.; Foerst, M.; Khanna, V.; Bromberger, H.; Mankowsky, R.; Singla, R.; Cavalleri, A.] Max Planck Inst Struct & Dynam Matter, Hamburg, Germany. [Caviglia, A. D.] Delft Univ Technol, Kavli Inst Nanosci, Delft, Netherlands. [Scherwitzl, R.; Gibert, M.; Gariglio, S.; Zubko, P.; Triscone, J. -M.] Univ Geneva, Dept Phys Mat Condensee, CH-1211 Geneva, Switzerland. [Khanna, V.; Cavalleri, A.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Khanna, V.; Cavill, S. A.] Diamond Light Source, Didcot, Oxon, England. [Chuang, Y. -D.] Lawrence Berkeley Lab, Advanced Light Source, Berkeley, CA 94720 USA. [Lee, W. S.] Stanford Linear Accelerator Ctr, SIMES, Natl Accelerator Lab, Menlo Pk, CA 94305 USA. [Lee, W. S.] Stanford Univ, Menlo Pk, CA 94305 USA. [Krupin, O.] GmbH, European XFEL, Hamburg, Germany. [Schlotter, W. F.; Turner, J. J.; Dakovski, G. L.; Minitti, M. P.; Robinson, J.] Stanford Linear Accelerator Ctr, Linac Coherent Light Source, Natl Accelerator Lab, Menlo Pk, CA 94305 USA. [Scagnoli, V.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, PSI, Switzerland. [Wilkins, S. B.; Hill, J. P.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Caviglia, AD (reprint author), Max Planck Inst Struct & Dynam Matter, Hamburg, Germany. RI Zubko, Pavlo/B-5496-2009; Forst, Michael/D-8924-2012; Caviglia, Andrea/B-4443-2009; scagnoli, valerio/C-6833-2008; Cavill, Stuart/C-5002-2015; Gibert, Marta/A-2317-2016 OI Zubko, Pavlo/0000-0002-7330-3163; Caviglia, Andrea/0000-0001-9650-3371; scagnoli, valerio/0000-0002-8116-8870; Cavill, Stuart/0000-0002-1359-4958; Gibert, Marta/0000-0001-8856-6831 FU LCLS; Stanford University through the Stanford Institute for Materials Energy Sciences (SIMES); Lawrence Berkeley National Laboratory (LBNL); University of Hamburg through the BMBF [FSP 301]; Center for Free Electron Laser Science (CFEL); Diamond Light Source [SI7285, SI8207-1]; SNSF; Advanced Light Source (ALS); Department of Energy [DE-AC02-05CH11231, DE-AC02-98CH10886] FX We thank M. Altarelli for useful discussions and M. Petrich and J. Harms for technical support. Portions of this research were carried out on the SXR Instrument at the Linac Coherent Light Source (LCLS), a division of SLAC National Accelerator Laboratory and an Office of Science user facility operated by Stanford University for the US Department of Energy. The SXR Instrument is funded by a consortium whose membership includes the LCLS, Stanford University through the Stanford Institute for Materials Energy Sciences (SIMES), Lawrence Berkeley National Laboratory (LBNL), University of Hamburg through the BMBF priority program FSP 301, and the Center for Free Electron Laser Science (CFEL). We acknowledge support from the Diamond Light Source for the provision of experimental beamtime under Awards No. SI7285 and No. SI8207-1. A. D. C. acknowledges financial support by the SNSF. Y.D.C. acknowledges support by the Advanced Light Source (ALS). ALS is supported by Department of Energy under Contract No. DE-AC02-05CH11231. Work at Brookhaven National Laboratory is supported by the Department of Energy under Contract No. DE-AC02-98CH10886. NR 37 TC 18 Z9 18 U1 3 U2 65 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 2 PY 2013 VL 88 IS 22 AR 220401 DI 10.1103/PhysRevB.88.220401 PG 5 WC Physics, Condensed Matter SC Physics GA 273XS UT WOS:000328570200001 ER PT J AU Nishida, Y AF Nishida, Yusuke TI Electron spin resonance in a dilute magnon gas as a probe of magnon scattering resonances SO PHYSICAL REVIEW B LA English DT Article ID EFIMOV; SYSTEMS; LENGTH; ATOMS AB We study the electron spin resonance in a dilute magnon gas that is realized in a ferromagnetic spin system at low temperature. A quantum cluster expansion is developed to show that the frequency shift of the single-magnon peak changes its sign and the linewidth reaches its maximum across a scattering resonance between magnons. Such characteristic behaviors are universal and can be used to experimentally locate the two-magnon resonance when an external parameter such as pressure is varied. Future achievement of the two-magnon resonance may have an impact comparable to the Feshbach resonance in ultracold atoms and will open up a rich variety of strongly correlated physics such as the recently proposed Efimov effect in quantum magnets. We also suggest how the emergence of an Efimov state of three magnons and its binding energy may be observed with the electron spin resonance. C1 [Nishida, Yusuke] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Nishida, Yusuke] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. RP Nishida, Y (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Nishida, Yusuke/B-9334-2015 OI Nishida, Yusuke/0000-0003-4350-3161 FU LANL Oppenheimer Fellowship; JSPS KAKENHI [25887020] FX The author thanks C. D. Batista and Y. Kato and acknowledges many valuable discussions during his visit to RIKEN and YITP in the fall of 2012. This work was supported by a LANL Oppenheimer Fellowship and JSPS KAKENHI Grant No. 25887020. NR 24 TC 4 Z9 4 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD DEC 2 PY 2013 VL 88 IS 22 AR 224402 DI 10.1103/physRevB.88.224402 PG 6 WC Physics, Condensed Matter SC Physics GA 273XS UT WOS:000328570200006 ER PT J AU Yang, X Shvyd'ko, Y AF Yang, Xi Shvyd'ko, Yuri TI Maximizing spectral flux from self-seeding hard x-ray free electron lasers SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID SCATTERING; RADIATION; FEL; BANDWIDTH; COHERENT AB Fully coherent x rays can be generated by self-seeding x-ray free electron lasers (XFELs). Self-seeding by a forward Bragg diffraction (FBD) monochromator has been recently proposed [G. Geloni, V. Kocharyan, and E. Saldin, J. Mod. Opt. 58, 1391 (2011)] and demonstrated [J. Amann et al., Nat. Photonics 6, 693 (2012)]. Characteristic time T-0 of FBD determines the power, spectral, and time characteristics of the FBD seed [Yu. Shvyd'ko and R. Lindberg, Phys. Rev. ST Accel. Beams 15, 100702 (2012)]. Here we show that for a given electron bunch with duration sigma(e) the spectral flux of the self-seeding XFEL can be maximized, and the spectral bandwidth can be respectively minimized by choosing T-0 similar to sigma(e)/pi and by optimizing the electron bunch delay tau(e). The choices of T-0 and tau(e) are not unique. In all cases, the maximum value of the spectral flux and the minimum bandwidth are primarily determined by sigma(e). Two-color seeding takes place if T-0 << sigma(e)/pi. The studies are performed, for a Gaussian electron bunch distribution with the parameters, close to those used in the short-bunch (sigma(e) similar or equal to 5 fs) and long-bunch (sigma(e) similar or equal to 20 fs) operation modes of the Linac Coherent Light Source XFEL. C1 [Yang, Xi] Brookhaven Natl Lab, Upton, NY 11973 USA. [Shvyd'ko, Yuri] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Yang, X (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM xiyang@bnl.gov; shvydko@aps.anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH1-886]; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX We gratefully acknowledge useful discussions with ZhiRong Huang, Gregory Penn, L. H. Yu, and Sven Reiche. ZhiRong Huang and Juhao Wu are acknowledged for providing LCLS FEL parameters. Work at Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH1-886. Work at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. NR 38 TC 2 Z9 2 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD DEC 2 PY 2013 VL 16 IS 12 AR 120701 DI 10.1103/PhysRevSTAB.16.120701 PG 14 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 274PP UT WOS:000328618800001 ER PT J AU Wang, XQ Yang, T Cheng, XL Shen, QL AF Wang, Xueqiang Yang, Tao Cheng, Xiaolin Shen, Qilong TI Enantioselective Electrophilic Trifluoromethylthiolation of beta-Ketoesters: A Case of Reactivity and Selectivity Bias for Organocatalysis SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE asymmetric synthesis; fluorine; organocatalysis; quinine; trifluoromethylthiolation ID FRIEDEL-CRAFTS ALKYLATION; ALPHA-FLUORINATED ETHERS; ARYL BORONIC ACIDS; CINCHONA ALKALOIDS; OXIDATIVE TRIFLUOROMETHYLTHIOLATION; ALLYLIC TRIFLUOROMETHYLATION; ETHYL TRIFLUOROPYRUVATE; ASYMMETRIC-SYNTHESIS; CATALYZED SYNTHESIS; ROOM-TEMPERATURE C1 [Wang, Xueqiang; Yang, Tao; Cheng, Xiaolin; Shen, Qilong] Chinese Acad Sci, Key Lab Organofluorine Chem, Shanghai Inst Organ Chem, Shanghai 200032, Peoples R China. [Cheng, Xiaolin] Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37831 USA. RP Shen, QL (reprint author), Chinese Acad Sci, Key Lab Organofluorine Chem, Shanghai Inst Organ Chem, 345 Lingling Rd, Shanghai 200032, Peoples R China. EM shenql@sioc.ac.cn FU National Basic Research Program of China [2012CB821600]; Natural Science Foundation of China [21032006]; National Natural Science Foundation of China [21172245, 21172244, B020304]; Shanghai Pujiang Program [11J1412200]; SIOC FX The authors gratefully acknowledge financial support from the National Basic Research Program of China (2012CB821600), the Key Program of Natural Science Foundation of China (21032006), the National Natural Science Foundation of China (21172245/21172244/B020304), the Shanghai Pujiang Program (11J1412200), and SIOC. NR 73 TC 96 Z9 97 U1 11 U2 110 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD DEC 2 PY 2013 VL 52 IS 49 BP 12860 EP 12864 DI 10.1002/anie.201305075 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 257TS UT WOS:000327410300013 PM 24000200 ER PT J AU Das, AK Engelhard, MH Liu, F Bullock, RM Roberts, JAS AF Das, Atanu K. Engelhard, Mark H. Liu, Fei Bullock, R. Morris Roberts, John A. S. TI The Electrode as Organolithium Reagent: Catalyst-Free Covalent Attachment of Electrochemically Active Species to an Azide-Terminated Glassy Carbon Electrode Surface SO INORGANIC CHEMISTRY LA English DT Article ID DIAZONIUM SALTS; CONDUCTIVE DIAMOND; CLICK CHEMISTRY; REDUCTION; MOLECULES; FERROCENE; SYSTEMS; OXYGEN; FUNCTIONALIZATION; MONOLAYERS AB The reaction of a lithium acetylide-ethylenediamine complex with azide-terminated glassy carbon surfaces affords 1,2,3-triazolyllithium surface groups that are active toward covalent C-C coupling reactions, including salt metathesis with an aliphatic halide and nucleophilic addition at an aldehyde. Surface ferrocenyl groups were introduced by reaction with (6-iodohexyl)ferrocene; the voltammetry of electrode samples shows narrow, symmetric peaks indicating uniform attachment. X-ray photoelectron and reflectance infrared spectroscopic data provide further support for the surface-attached products. Formation of the 1,2,3-triazolyllithium linkage requires neither a catalyst nor a strained alkyne. Coverages obtained by this route are similar to those obtained by the more common Cu(I)-catalyzed alkyne-azide coupling (CuAAC) of ethynylferrocene with surface azides. Preconditioning of the glassy carbon disk electrodes at ambient temperature under nitrogen affords coverages comparable to those reported with preconditioning at 1000 degrees C under hydrogen/nitrogen. C1 [Das, Atanu K.; Bullock, R. Morris; Roberts, John A. S.] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Chem & Mat Sci Div, Richland, WA 99352 USA. [Engelhard, Mark H.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Liu, Fei] Univ Wyoming, Dept Chem, Laramie, WY 82071 USA. [Liu, Fei] Univ Wyoming, Sch Energy Resources, Laramie, WY 82071 USA. RP Roberts, JAS (reprint author), Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Chem & Mat Sci Div, POB 999,K2-57, Richland, WA 99352 USA. EM john.roberts@pnnl.gov RI Bullock, R. Morris/L-6802-2016; OI Bullock, R. Morris/0000-0001-6306-4851; Engelhard, Mark/0000-0002-5543-0812 FU Center for Molecular Electrocatalysis, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory FX This research was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy. The XPS measurements were performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. We thank Thomas Blake and J. Timothy Bays for assistance with surface IR spectroscopic measurements. NR 56 TC 4 Z9 4 U1 1 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 2 PY 2013 VL 52 IS 23 BP 13674 EP 13684 DI 10.1021/ic402247n PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 263TT UT WOS:000327831600047 PM 24228741 ER PT J AU George, NC Birkel, A Brgoch, J Hong, BC Mikhailovsky, AA Page, K Llobet, A Seshadri, R AF George, Nathan C. Birkel, Alexander Brgoch, Jakoah Hong, Byung-Chul Mikhailovsky, Alexander A. Page, Katharine Llobet, Anna Seshadri, Ram TI Average and Local Structural Origins of the Optical Properties of the Nitride Phosphor La3-xCexSi6N11 (0 < x <= 3) SO INORGANIC CHEMISTRY LA English DT Article ID AUGMENTED-WAVE METHOD; LIGHT EMITTING DIODE; SOLID-STATE; LUMINESCENCE PROPERTIES; CRYSTAL-STRUCTURE; RARE-EARTH; MAS NMR; POWDER DIFFRACTION; ENERGY-TRANSFER; WHITE LEDS AB Structural intricacies of the orange-red nitride phosphor system La3-xCexSi6N11 (0 < x <= 3) have been elucidated using a combination of state-of-the art tools, in order to understand the origins of the exceptional optical properties of this important solid-state lighting material. In addition, the optical properties of the end-member (x = 3) compound, Ce3Si6N11, are described for the first time. A combination of synchrotron powder X-ray diffraction and neutron scattering is employed to establish site preferences and the rigid nature of the structure, which is characterized by a high Debye temperature. The high Debye temperature is also corroborated from ab initio electronic structure calculations. Solid-state Si-29 nuclear magnetic resonance, including paramagnetic shifts of Si-29 spectra, are employed in conjunction with low-temperature electron spin resonance studies to probes of the local environments of Ce ions. Detailed wavelength-, time-, and temperature-dependent luminescence properties of the solid solution are presented. Temperature-dependent quantum yield measurements demonstrate the remarkable thermal robustness of luminescence of La2.82Ce0.18Si6Ni11, which shows little sign of thermal quenching, even at temperatures as high as 500 K. This robustness is attributed to the highly rigid lattice. Luminescence decay measurements indicate very short decay times (close to 40 ns). The fast decay is suggested to prevent strong self-quenching of luminescence, allowing even the end-member compound Ce3Si6N11 to display bright luminescence. C1 [George, Nathan C.; Birkel, Alexander; Brgoch, Jakoah; Seshadri, Ram] Univ Calif Santa Barbara, Mitsubishi Chem Ctr Adv Mat, Santa Barbara, CA 93106 USA. [Hong, Byung-Chul] Mitsubishi Chem Corp, Yokohama, Kanagawa 2278502, Japan. [Mikhailovsky, Alexander A.; Seshadri, Ram] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Page, Katharine; Llobet, Anna] Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [George, Nathan C.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Seshadri, Ram] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Seshadri, Ram] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. RP Seshadri, R (reprint author), Univ Calif Santa Barbara, Mitsubishi Chem Ctr Adv Mat, Santa Barbara, CA 93106 USA. EM seshadri@mrl.ucsb.edu RI Brgoch, Jakoah/D-9347-2011; Seshadri, Ram/C-4205-2013; Page, Katharine/C-9726-2009; Llobet, Anna/B-1672-2010 OI Seshadri, Ram/0000-0001-5858-4027; Page, Katharine/0000-0002-9071-3383; FU ConvEne IGERT Program (NSF-DGE) [0801627]; MRSEC Program of the NSF [DMR 1121053]; NSF; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; DOE Office of Basic Energy Sciences; Los Alamos National Security LLC [DE-AC52-06NA25396] FX N.C.G. has been supported by the ConvEne IGERT Program (NSF-DGE No. 0801627). The research carried out here made extensive use of shared experimental facilities of the Materials Research Laboratory: The MRL Central Facilities are supported by the MRSEC Program of the NSF under Award No. DMR 1121053; a member of the NSF-funded Materials Research Facilities Network (www.mrfn.org). Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (under Contract No. DE-AC02-06CH11357). The authors thank Joan Siewenie for assistance with data collection at NPDF. This work has benefited from the use of NPDF and HIPD at the Lujan Center, funded by DOE Office of Basic Energy Sciences; LANL is operated by Los Alamos National Security LLC (under No. DE-AC52-06NA25396). NR 79 TC 21 Z9 21 U1 2 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD DEC 2 PY 2013 VL 52 IS 23 BP 13730 EP 13741 DI 10.1021/ic402318k PG 12 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 263TT UT WOS:000327831600053 PM 24236540 ER PT J AU Luo, YX Rasmussen, JO Hamilton, JH Ramayya, AV Frauendorf, S Hwang, JK Stone, NJ Zhu, SJ Brewer, NT Wang, E Lee, IY Liu, SH TerAkopian, GM Daniel, AV Oganessian, YT Stoyer, MA Donangelo, R Ma, WC Cole, JD Shi, Y Xu, FR AF Luo, Y. X. Rasmussen, J. O. Hamilton, J. H. Ramayya, A. V. Frauendorf, S. Hwang, J. K. Stone, N. J. Zhu, S. J. Brewer, N. T. Wang, E. Lee, I. Y. Liu, S. H. TerAkopian, G. M. Daniel, A. V. Oganessian, Yu. Ts. Stoyer, M. A. Donangelo, R. Ma, W. C. Cole, J. D. Shi, Yue Xu, F. R. TI New insights into the nuclear structure in neutron-rich 112,114,115,116,117,118Pd SO NUCLEAR PHYSICS A LA English DT Article DE 112,114,115,116,117,118Pd; Cf-252; gamma-gamma-gamma and gamma-gamma(theta); Triaxiality; Chirality; Wobbling; Shape transitions ID ION-INDUCED FISSION; COLLECTIVE MODEL DESCRIPTION; HIGH-SPIN STATES; ODD-A NUCLEI; PD-ISOTOPES; PALLADIUM ISOTOPES; WOBBLING MODE; RU-108,RU-110,RU-112; SPECTROSCOPY; EXCITATIONS AB New level schemes of Pd-112,Pd-114,Pd-115,Pd-116,Pd-117,Pd-118 are established by means of gamma-gamma-gamma, gamma-gamma-gamma-gamma and gamma-gamma(theta) measurements of prompt fission gamma rays from Cf-252 using the Gammasphere multi-detector array. Spins/parities were assigned to levels based on gamma-gamma angular correlation measurements, level systematics and decay patterns. In the even-N isotopes Pd-112,Pd-114,Pd-116, two sets of odd-parity bands were identified and extended with spins measured in each band. The odd-parity bands with large level staggerings were interpreted as disturbed chirality with less pronounced triaxial deformations in the Pd isotopes than observed in the chiral symmetry breaking Ru-110,Ru-112 with maximum triaxiality. Onset of wobbling motion was identified from the sign of the signature splitting in the gamma band of even-even Pd-114, and probably also in Pd-116, as first seen in the N = 68 isotone Ru-112. Maximal triaxiality in Ru and Pd isotopes is found to be reached for N = 68, Ru-112 and Pd-114, 4 neutrons more than predicted in the theoretical calculations. The new data and TRS calculations allowed a systematic study of the band crossings in the even-N Pd-112,Pd-114,Pd-116 and odd-N Pd-115,Pd-117 isotopes. Now we find a new overall, more complex shape evolution than previously proposed from triaxial prolate in Pd-110 via triaxial oblate in Pd-112 to nearly oblate in Pd-114,Pd-116 with a large change of the triaxial deformation parameter gamma toward nearly oblate in the (pi g(9/2))(2) alignment in Pd-114,Pd-115,Pd-116,Pd-117,Pd-118, and triaxial-prolate-triaxial-oblate shape coexisting bands in Pd-115. (C) 2013 Elsevier B.V. All rights reserved. C1 [Luo, Y. X.; Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Zhu, S. J.; Brewer, N. T.; Wang, E.; Liu, S. H.; Daniel, A. V.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Luo, Y. X.; Rasmussen, J. O.; Lee, I. Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Rasmussen, J. O.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Frauendorf, S.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Frauendorf, S.] FZD Rossendorf, Inst Strahlenphys, D-01314 Dresden, Germany. [Stone, N. J.] Univ Oxford, Dept Phys, Oxford OX1 3PU, England. [Stone, N. J.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Zhu, S. J.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Liu, S. H.] Oak Ridge Associated Univ, UNIRIB, Oak Ridge, TN 37831 USA. [TerAkopian, G. M.; Daniel, A. V.; Oganessian, Yu. Ts.] Joint Inst Nucl Res, RU-141980 Dubna, Russia. [TerAkopian, G. M.; Daniel, A. V.] Joint Inst Heavy Ion Res, Oak Ridge, TN 37830 USA. [Stoyer, M. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Donangelo, R.] Fac Ingn, Montevideo 11300, Uruguay. [Ma, W. C.] Mississippi State Univ, Mississippi State, MS 39762 USA. [Cole, J. D.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Shi, Yue; Xu, F. R.] Beijing Univ, Dept Phys, Beijing 100871, Peoples R China. RP Hamilton, JH (reprint author), Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. RI Xu, Furong/K-4178-2013; OI Hwang, Jae-Kwang/0000-0002-4100-3473 FU U.S. DOE [DE-FG-05-88ER40407, DE-FG0295ER40934, DE-AC52-07NA27344, DE-FG02-95ER40939, DE-AC07-761O1570, W-7405-ENG48]; Major State Basic Research Development Program [2007CB815005]; NNSF of China [10975082, 11175095]; HESF [20100002110077]; CNPq; FAPERJ FX The work at Vanderbilt University, Lawrence Berkeley National Laboratory, Lawrence Livermore National Laboratory, Mississippi State University and Idaho National Laboratory was supported by the U.S. DOE Grants DE-FG-05-88ER40407, DE-FG0295ER40934, DE-AC52-07NA27344, DE-FG02-95ER40939, DE-AC07-761O1570 and Contract W-7405-ENG48. The work at Tsinghua University in Beijing was supported by the Major State Basic Research Development Program Contract 2007CB815005, the NNSF of China Grant No. 10975082, Grant No. 11175095, and the Special Program of HESF Grant 20100002110077. The Joint Institute for Heavy Ion Research is supported by its members, Vanderbilt University, University of Tennessee and Oak Ridge National Laboratory and the U.S. DOE. The work at the Federal University of Rio de Janeiro was partially supported by CNPq and FAPERJ. NR 66 TC 4 Z9 5 U1 1 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9474 EI 1873-1554 J9 NUCL PHYS A JI Nucl. Phys. A PD DEC 2 PY 2013 VL 919 BP 67 EP 98 DI 10.1016/j.nuclphysa.2013.10.002 PG 32 WC Physics, Nuclear SC Physics GA 263RY UT WOS:000327826900005 ER PT J AU Lee, IJ Sung, NE Chae, KH Conley, R AF Lee, Ik-Jae Sung, Nark-Eon Chae, Keun Hwa Conley, Ray TI Characterization of zinc-tin-oxide films deposited by radio frequency magnetron sputtering at various substrate temperatures SO THIN SOLID FILMS LA English DT Article DE Zinc-tin-oxide; Sputtering; X-ray diffraction; Transmission electron microscopy; Band gap; Hall mobility ID SENSITIZED SOLAR-CELLS; THIN-FILMS; OPTICAL-PROPERTIES; ELECTRONIC-STRUCTURE; TRANSPARENT; STANNATE; TRANSISTORS; ZN2SNO4; ZNO; SEMICONDUCTORS AB Zinc-tin-oxide (ZTO) thin films were grown by radio frequency magnetron sputtering on glass substrates at various substrate temperatures. The effects of substrate temperature on the crystalline behavior and electrical and optical properties of the films were studied. The ZTO films were amorphous and maintained their stable amorphous state up to a substrate temperature of 350 degrees C. With increasing substrate temperature, the ZTO films underwent an amorphous-to-crystalline phase transition. The Hall mobility of the films was in the range of 22.7-23.5 cm(2)/V s in the amorphous phase and 15.4-19.6 cm(2)/V s in the crystalline phase. The carrier concentration reached 8.287 x 10(19) cm(-3), resulting in a minimum resistivity of 8.75 x 10(-3) Omega.cm in the film deposited at 750 degrees C. The average transmittance in the visible region was >= 85%, and the band gap showed a red-shift in the amorphous phase and a blue-shift in the crystalline phase. (C) 2013 Elsevier B. V. All rights reserved. C1 [Lee, Ik-Jae; Sung, Nark-Eon] Pohang Univ Sci & Technol, Pohang Accelerator Lab, Pohang 790784, South Korea. [Chae, Keun Hwa] Korea Inst Sci & Technol, Nano Mat Anal Ctr, Seoul 136791, South Korea. [Lee, Ik-Jae; Conley, Ray] Brookhaven Natl Lab, Photon Sci Div, NSLS 2, Upton, NY 11973 USA. [Conley, Ray] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Conley, R (reprint author), Brookhaven Natl Lab, Photon Sci Div, NSLS 2, Upton, NY 11973 USA. EM rconley@aps.anl.gov RI Chae, Keun Hwa/H-2459-2016 OI Chae, Keun Hwa/0000-0003-3894-670X FU Basic Science Research Program through the National Research Foundation of Korea (NRF); Ministry of Education, Science and Technology [2011-0022268] FX This research was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) founded by the Ministry of Education, Science and Technology (2011-0022268). NR 31 TC 5 Z9 5 U1 2 U2 38 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD DEC 2 PY 2013 VL 548 BP 385 EP 388 DI 10.1016/j.tsf.2013.08.067 PG 4 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 259MF UT WOS:000327530300062 ER PT J AU Buttigieg, PL Morrison, N Smith, B Mungall, CJ Lewis, SE AF Buttigieg, Pier Luigi Morrison, Norman Smith, Barry Mungall, Christopher J. Lewis, Suzanna E. CA ENVO Consortium TI The environment ontology: contextualising biological and biomedical entities SO JOURNAL OF BIOMEDICAL SEMANTICS LA English DT Article DE Environment; Ecosystem; Biome; Ontology ID DATABASE; BIODIVERSITY; INFORMATION; INTEGRATION; MICROBES; METADATA; DISEASE; WORLDS; EARTH; LIFE AB As biological and biomedical research increasingly reference the environmental context of the biological entities under study, the need for formalisation and standardisation of environment descriptors is growing. The Environment Ontology (ENVO; www.environmentontology.org) is a community-led, open project which seeks to provide an ontology for specifying a wide range of environments relevant to multiple life science disciplines and, through an open participation model, to accommodate the terminological requirements of all those needing to annotate data using ontology classes. This paper summarises ENVO's motivation, content, structure, adoption, and governance approach. C1 [Buttigieg, Pier Luigi] Helmholtz Ctr Polar & Marine Res, Alfred Wegener Inst, HGF MPG Res Grp Deep Sea Ecol & Technol, D-27570 Bremerhaven, Germany. [Mungall, Christopher J.; Lewis, Suzanna E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Smith, Barry] SUNY Buffalo, Dept Philosophy, Buffalo, NY 14260 USA. [Morrison, Norman] Univ Manchester, Sch Comp Sci, Manchester M13 9PL, Lancs, England. RP Buttigieg, PL (reprint author), Helmholtz Ctr Polar & Marine Res, Alfred Wegener Inst, HGF MPG Res Grp Deep Sea Ecol & Technol, Handelshafen 12, D-27570 Bremerhaven, Germany. EM pbuttigi@mpi-bremen.de OI Buttigieg, Pier Luigi/0000-0002-4366-3088; Lewis, Suzanna/0000-0002-8343-612X FU European Commission [287589, 283359]; National Human Genome Research Institute [HG004838]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX ENVO would not exist were it not for the vision and scientific ideals of Professor Michael Ashbumer. He single-handedly initiated this project and through sheer dedication brought proto-ENVO into being. Even in retirement he continues to extend and refine the Gazetteer, which has grown thanks to his efforts to close to three-quarter million place-names. His inspiration provides a beacon guiding us in our efforts to create the environment ontology researchers need. PLB is supported by the European Commission under Grant Agreement no287589 (MicroB3). NM is supported by the European Commission 7th Framework Programme (FP7) as part of its e-Infrastructures activity (Grant no. 283359) (BioVeL). SEL and CJM were supported by grant HG004838 from the National Human Genome Research Institute for 'An Ontology of Qualities for the Annotation of Biomedical Data', and also by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 45 TC 37 Z9 37 U1 0 U2 3 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 2041-1480 J9 J BIOMED SEMANT JI J. Biomed. Semant. PD DEC PY 2013 VL 4 AR 43 DI 10.1186/2041-1480-4-43 PG 9 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA AR6PZ UT WOS:000343706700003 PM 24330602 ER PT J AU Bent, ZW Branda, SS Young, GM AF Bent, Zachary W. Branda, Steven S. Young, Glenn M. TI The Yersinia enterocolitica Ysa type III secretion system is expressed during infections both in vitro and in vivo SO MICROBIOLOGYOPEN LA English DT Article DE In vivo expression; T3SS; Y. enterocolitica; Ysa; Ysp ID GENE-EXPRESSION; BIOVAR 1B; PATHOGENICITY; VIRULENCE; IDENTIFICATION; UNIQUE; LOCUS; CELLS; ENTRY AB Yersinia enterocolitica biovar 1B maintains two type III secretion systems (T3SS) that are involved in pathogenesis, the plasmid encoded Ysc T3SS and the chromosomally encoded Ysa T3SS. In vitro, the Ysa T3SS has been shown to be expressed only at 26 degrees C in a high-nutrient medium containing an exceptionally high concentration of salt - an artificial condition that provides no clear insight on the nature of signal that Y. enterocolitica responds to in a host. However, previous research has indicated that the Ysa system plays a role in the colonization of gastrointestinal tissues of mice. In this study, a series of Ysa promoter fusions to green fluorescent protein gene (gfp) were created to analyze the expression of this T3SS during infection. Using reporter strains, infections were carried out in vitro using HeLa cells and in vivo using the mouse model of yer-siniosis. Expression of green fluorescent protein (GFP) was measured from the promoters of yspP (encoding a secreted effector protein) and orf6 (encoding a structural component of the T3SS apparatus) in vitro and in vivo. During the infection of HeLa cells GFP intensity was measured by fluorescence microscopy, while during murine infections GFP expression in tissues was measured by flow cytometry. These approaches, combined with quantification of yspP mRNA transcripts by quantitative reverse transcriptase-polymerase chain reaction (qRT-PCR), demonstrate that the Ysa system is expressed in vitro in a contact-dependent manner, and is expressed in vivo during infection of mice. C1 [Bent, Zachary W.; Young, Glenn M.] Univ Calif Davis, Microbiol Grad Grp, Davis, CA 95616 USA. [Bent, Zachary W.; Branda, Steven S.] Sandia Natl Labs, Livermore, CA 94550 USA. [Young, Glenn M.] Univ Calif Davis, Dept Food Sci & Technol, Davis, CA 95616 USA. RP Bent, ZW (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM zbent@sandia.gov FU National Institutes of Health (NIH) [R21 AI156042]; NIH training grant [T32 AI60555]; Henry A. Jastro and Peter J. Shields Graduate Research Scholarship Award; Sandia National Laboratories' LDRD (Laboratory-Directed Research and Development) [165767, 171001] FX This study was supported by a grant from the National Institutes of Health (NIH), R21 AI156042 to G. M. Y. NIH training grant for graduate research of animal models of human infectious disease T32 AI60555 and the Henry A. Jastro and Peter J. Shields Graduate Research Scholarship Award partially supported Z. W. B. Z. W. B. and S. S. B. were also funded by Sandia National Laboratories' LDRD (Laboratory-Directed Research and Development, grant numbers 165767 and 171001) program. NR 36 TC 5 Z9 5 U1 0 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2045-8827 J9 MICROBIOLOGYOPEN JI MicrobiologyOpen PD DEC PY 2013 VL 2 IS 6 BP 962 EP 975 DI 10.1002/mbo3.136 PG 14 WC Microbiology SC Microbiology GA AP8TM UT WOS:000342351900007 PM 24166928 ER PT J AU Ibragimov, R Jefferson, G Carminati, J AF Ibragimov, Ranis Jefferson, Grace Carminati, John TI Explicit invariant solutions associated with nonlinear atmospheric flows in a thin rotating spherical shell with and without west-to-east jets perturbations SO ANALYSIS AND MATHEMATICAL PHYSICS LA English DT Article ID DIFFERENTIAL-EQUATIONS; WAVES; FLUID; OCEAN; EULER AB A class of non-stationary exact solutions of two-dimensional nonlinear Navier-Stokes (NS) equations within a thin rotating spherical shell were found as invariant and approximately invariant solutions. The model is used to describe a simple zonally averaged atmospheric circulation caused by the difference in temperature between the equator and the poles. Coriolis effects are generated by pseudoforces, which support the stable west-to-east flows providing the achievable meteorological flows. The model is superimposed by a stationary latitude dependent flow. Under the assumption of no friction, the perturbed model describes zonal west-to-east flows in the upper atmosphere between the Ferrel and Polar cells. In terms of nonlinear modeling for the NS equations, two small parameters are chosen for the viscosity and the rate of the earth's rotation and exact solutions in terms of elementary functions are found using approximate symmetry analysis. It is shown that approximately invariant solutions are also valid in the absence of the flow perturbation to a zonally averaged mean flow. C1 [Ibragimov, Ranis] Pacific NW Natl Lab, Richland, WA 99352 USA. [Jefferson, Grace; Carminati, John] Deakin Univ, Sch Informat Technol, Waurn Ponds, Vic, Australia. RP Ibragimov, R (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Ranis.Ibragimov@utb.edu FU U.S. Department of Energy's Visiting Faculty Program FX This research was supported in part by an appointment to the U.S. Department of Energy's Visiting Faculty Program. NR 47 TC 0 Z9 0 U1 0 U2 1 PU SPRINGER BASEL AG PI BASEL PA PICASSOPLATZ 4, BASEL, 4052, SWITZERLAND SN 1664-2368 EI 1664-235X J9 ANAL MATH PHYS JI Anal. Math. Phys. PD DEC PY 2013 VL 3 IS 4 BP 375 EP 391 DI 10.1007/s13324-013-0062-9 PG 17 WC Mathematics, Applied; Mathematics SC Mathematics GA AO8EM UT WOS:000341586200004 ER PT J AU Borland, AM Yang, XH AF Borland, Anne M. Yang, Xiaohan TI Informing the improvement and biodesign of crassulacean acid metabolism via system dynamics modelling SO NEW PHYTOLOGIST LA English DT Editorial Material DE crassulacean acid metabolism (CAM); modelling; photosynthesis; plant productivity; system dynamics ID PHOTOSYNTHESIS; PLANTS; AGAVE; C3 C1 [Borland, Anne M.] Newcastle Univ, Sch Biol, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. [Borland, Anne M.; Yang, Xiaohan] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Borland, AM (reprint author), Newcastle Univ, Sch Biol, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. EM anne.borland@ncl.ac.uk RI Yang, Xiaohan/A-6975-2011 OI Yang, Xiaohan/0000-0001-5207-4210 NR 13 TC 6 Z9 6 U1 1 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0028-646X EI 1469-8137 J9 NEW PHYTOL JI New Phytol. PD DEC PY 2013 VL 200 IS 4 BP 946 EP 949 PG 4 WC Plant Sciences SC Plant Sciences GA AA2WQ UT WOS:000330955300003 PM 24571665 ER PT J AU Parrish, N Anderson, HS Gupta, MR Hsiao, DY AF Parrish, Nathan Anderson, Hyrum S. Gupta, Maya R. Hsiao, Dun Yu TI Classifying With Confidence From Incomplete Information SO JOURNAL OF MACHINE LEARNING RESEARCH LA English DT Article DE classification; sensor networks; signals; reliability ID SPEECH RECOGNITION; DISCRIMINANT-ANALYSIS AB We consider the problem of classifying a test sample given incomplete information. This problem arises naturally when data about a test sample is collected over time, or when costs must be incurred to compute the classification features. For example, in a distributed sensor network only a fraction of the sensors may have reported measurements at a certain time, and additional time, power, and bandwidth is needed to collect the complete data to classify. A practical goal is to assign a class label as soon as enough data is available to make a good decision. We formalize this goal through the notion of reliability-the probability that a label assigned given incomplete data would be the same as the label assigned given the complete data, and we propose a method to classify incomplete data only if some reliability threshold is met. Our approach models the complete data as a random variable whose distribution is dependent on the current incomplete data and the (complete) training data. The method differs from standard imputation strategies in that our focus is on determining the reliability of the classification decision, rather than just the class label. We show that the method provides useful reliability estimates of the correctness of the imputed class labels on a set of experiments on time-series data sets, where the goal is to classify the time-series as early as possible while still guaranteeing that the reliability threshold is met. C1 [Parrish, Nathan] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Anderson, Hyrum S.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Hsiao, Dun Yu] Univ Washington, Dept Elect Engn, Seattle, WA 98195 USA. RP Parrish, N (reprint author), Johns Hopkins Univ, Appl Phys Lab, Johns Hopkins Rd, Laurel, MD 20723 USA. EM PARRISH.NATHAN@GMAIL.COM; HANDER@SANDIA.GOV; MAYAGUPTA@GOOGLE.COM FU United States PECASE Award; Sandia National Laboratories; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by a United States PECASE Award managed by the United States Office of Naval Research, and by the Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy National Nuclear Security Administration under contract DE-AC04-94AL85000. We thank Bela A. Frigyik for helpful discussions. NR 27 TC 4 Z9 4 U1 0 U2 0 PU MICROTOME PUBL PI BROOKLINE PA 31 GIBBS ST, BROOKLINE, MA 02446 USA SN 1532-4435 J9 J MACH LEARN RES JI J. Mach. Learn. Res. PD DEC PY 2013 VL 14 BP 3561 EP 3589 PG 29 WC Automation & Control Systems; Computer Science, Artificial Intelligence SC Automation & Control Systems; Computer Science GA AG5KE UT WOS:000335457100003 ER PT J AU Crease, RP AF Crease, Robert P. TI Critical Point Longing for Laputa SO PHYSICS WORLD LA English DT Editorial Material C1 [Crease, Robert P.] SUNY Stony Brook, Dept Philosophy, Stony Brook, NY 11790 USA. [Crease, Robert P.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Crease, RP (reprint author), SUNY Stony Brook, Dept Philosophy, Stony Brook, NY 11790 USA. EM robert.crease@stonybrook.edu NR 0 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8585 J9 PHYS WORLD JI Phys. World PD DEC PY 2013 VL 26 IS 12 BP 14 EP 14 PG 1 WC Physics, Multidisciplinary SC Physics GA AD3FS UT WOS:000333124300020 ER PT J AU Krommes, JA AF Krommes, J. A. TI The physics of the second-order gyrokinetic magnetohydrodynamic Hamiltonian: mu conservation, Galilean invariance, and ponderomotive potential SO PHYSICS OF PLASMAS LA English DT Article ID PRINCIPLE; EQUATIONS AB Some physical interpretations are given of the well-known second-order gyrokinetic Hamiltonian in the magnetohydrodynamic limit. Its relations to the conservation of the true (Galilean-invariant) magnetic moment and fluid nonlinearities are described. Subtleties about its derivation as a coldion limit are explained; it is important to take that limit in the frame moving with the E x B velocity. The discussion also provides some geometric understanding of certain well-known Lie generating functions, and it makes contact with general discussions of ponderomotive potentials and the thermodynamics of dielectric media. (c) 2013 AIP Publishing LLC. C1 Princeton Univ, Plasma Phys Lab, Princeton, NJ 08543 USA. RP Krommes, JA (reprint author), Princeton Univ, Plasma Phys Lab, MS 28,POB 451, Princeton, NJ 08543 USA. EM krommes@princeton.edu FU U. S. Department of Energy [DE-AC02-09CH11466] FX I am grateful for informative discussions about gyrokinetics with A. Brizard, G. Hammett, and W. W. Lee and about ponderomotive potentials with I. Dodin. Useful comments on the manuscript were received from I. Dodin, G. Hammett, and J. Squire. This work was supported by the U. S. Department of Energy Contract No. DE-AC02-09CH11466. NR 23 TC 4 Z9 4 U1 1 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD DEC PY 2013 VL 20 IS 12 AR 124501 DI 10.1063/1.4851996 PG 4 WC Physics, Fluids & Plasmas SC Physics GA 282MU UT WOS:000329176800092 ER PT J AU Murayama, H AF Murayama, Hitoshi TI Future experimental programs SO PHYSICA SCRIPTA LA English DT Article; Proceedings Paper CT LHC Nobel Symposium CY MAY, 2013 CL Uppsala, SWEDEN ID DARK-MATTER; MASS; SUPERNOVAE; ANARCHY AB I was asked to discuss future experimental programs even though I am a theorist. As a result, I present my own personal views on where the field is, and where it is going, based on what I myself have been working on. In particular, I discuss why we need expeditions into high energies to find clues to where the relevant energy scale is for dark matter, baryon asymmetry and neutrino mass. I also argue that the next energy frontier machine should be justified on the basis of what we know, namely the mass of the Higgs boson, so that we will learn what energy we should aim at once we nail the Higgs sector. Finally, I make remarks on dark energy. C1 [Murayama, Hitoshi] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Murayama, Hitoshi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Murayama, Hitoshi] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. RP Murayama, H (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM hitoshi@berkeley.edu FU US DOE [DEAC03-76SF00098]; NSF [PHY-1002399]; JSPS [23540289]; FIRST program SuMIRe, CSTP; WPI, MEXT, Japan FX This work was supported in part by the US DOE under contract number DEAC03-76SF00098, by the NSF under grant number PHY-1002399, by the JSPS grant (C) number 23540289, by the FIRST program SuMIRe, CSTP and by WPI, MEXT, Japan. NR 35 TC 4 Z9 4 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 EI 1402-4896 J9 PHYS SCRIPTA JI Phys. Scr. PD DEC PY 2013 VL T158 AR 014025 DI 10.1088/0031-8949/2013/T158/014025 PG 8 WC Physics, Multidisciplinary SC Physics GA AC4QF UT WOS:000332505100026 ER PT J AU Parke, S AF Parke, Stephen TI Neutrinos: theory and phenomenology SO PHYSICA SCRIPTA LA English DT Article; Proceedings Paper CT LHC Nobel Symposium CY MAY, 2013 CL Uppsala, SWEDEN ID SUPER-KAMIOKANDE; CP-VIOLATION; OSCILLATIONS; MASS AB The theory and phenomenology of neutrinos will be addressed, especially that relating to the observation of neutrino flavor transformations. The current status and implications for future experiments will be discussed with special emphasis on the experiments that will determine the neutrino mass ordering, the dominant flavor content of the neutrino mass eigenstate with the smallest electron neutrino content and the size of CP violation in the neutrino sector. Beyond the neutrino standard model, the evidence for and a possible definitive experiment to confirm or refute the existence of light sterile neutrinos will be briefly discussed. C1 Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. RP Parke, S (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. EM parke@fnal.gov OI Parke, Stephen/0000-0003-2028-6782 FU European Union [PITNGA-2011-289442]; Fermi Research Alliance [DE-AC02-07CH11359]; US Department of Energy [DE-AC02-07CH11359] FX I wish to thank the organizers and especially Professor Tord Ekelof for this wonderful symposium and the Nobel Symposia Fund for making this symposium possible. I also thank all of my collaborators in neutrino physics who through our discussion and paper writing have helped me better understand the nature of the neutrino. The author acknowledges partial support from the European Union FP7 ITN INVISIBLES (Marie Curie Actions, PITNGA-2011-289442). Fermilab is operated by the Fermi Research Alliance under contract no. DE-AC02-07CH11359 with the US Department of Energy. NR 34 TC 8 Z9 8 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 EI 1402-4896 J9 PHYS SCRIPTA JI Phys. Scr. PD DEC PY 2013 VL T158 AR 014013 DI 10.1088/0031-8949/2013/T158/014013 PG 9 WC Physics, Multidisciplinary SC Physics GA AC4QF UT WOS:000332505100014 ER PT J AU Lu, CS Liu, YG Niu, SJ Zhao, LJ Yu, HY Cheng, MN AF Lu Chunsong Liu Yangang Niu Shengjie Zhao Lijuan Yu Huaying Cheng Muning TI Examination of microphysical relationships and corresponding microphysical processes in warm fogs SO ACTA METEOROLOGICA SINICA LA English DT Article DE fog microphysics; microphysical relationships; physical processes; observations ID QUASI-PERIODIC OSCILLATIONS; ENSEMBLE PREDICTION SYSTEM; PO VALLEY FOG; RADIATION-FOG; SEA FOG; YELLOW SEA; CHEMICAL-COMPOSITION; NUMERICAL-MODEL; EAST-COAST; CHINA SEA AB In this paper, the microphysical relationships of 8 dense fog events collected from a comprehensive fog observation campaign carried out at Pancheng (32.2A degrees N, 118.7A degrees E) in the Nanjing area, China in the winter of 2007 are investigated. Positive correlations are found among key microphysical properties (cloud droplet number concentration, droplet size, spectral standard deviation, and liquid water content) in each case, suggesting that the dominant processes in these fog events are likely droplet nucleation with subsequent condensational growth and/or droplet deactivation via complete evaporation of some droplets. The abrupt broadening of the fog droplet spectra indicates the occurrence of the collision-coalescence processes as well, although not dominating. The combined effects of the dominant processes and collision-coalescence on microphysical relationships are further analyzed by dividing the dataset according to visibility or autoconversion threshold in each case. The result shows that the specific relationships of number concentration to volume-mean radius and spectral standard deviation depend on the competition between the compensation of small droplets due to nucleation-condensation and the loss of small droplets due to collision-coalescence. Generally, positive correlations are found for different visibility or autoconversion threshold ranges in most cases, although negative correlations sometimes appear with lower visibility or larger autoconversion threshold. Therefore, the compensation of small droplets is generally stronger than the loss, which is likely related to the sufficient fog condensation nuclei in this polluted area. C1 [Lu Chunsong; Niu Shengjie; Yu Huaying] Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Forecast & Evaluat Meteoro, China Meteorol Adm, Key Lab Aerosol Cloud Precipitat, Nanjing 210044, Jiangsu, Peoples R China. [Lu Chunsong] Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing 100081, Peoples R China. [Lu Chunsong; Liu Yangang] Brookhaven Natl Lab, Div Atmospher Sci, Upton, NY 11973 USA. [Zhao Lijuan] Xiamen Environm Monitoring Cent Stn, Xiamen 361004, Peoples R China. [Cheng Muning] Jiangsu Prov Acad Environm Sci, Inst Environm Assessment 2, Nanjing 210000, Jiangsu, Peoples R China. RP Lu, CS (reprint author), Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Forecast & Evaluat Meteoro, China Meteorol Adm, Key Lab Aerosol Cloud Precipitat, Nanjing 210044, Jiangsu, Peoples R China. EM luchunsong110@163.com RI Lu, Chunsong/K-7124-2013 OI Lu, Chunsong/0000-0002-8967-0371 FU National Natural Science Foundation of China [41305120, 41030962, 41275151, 41375138, 41375137, 41305034]; Natural Science Foundation of Jiangsu Province [BK20130988, SK201220841]; Specialized Research Fund for the Doctoral Program of Higher Education [20133228120002]; China Meteorological Administration Special Public Welfare Research Fund [GYHY201406007]; Natural Science Foundation of the Higher Education Institutions of Jiangsu Province [13KJB170014]; Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration [KDW1201, KDW1102]; Key Laboratory of Meteorological Disaster of Ministry of Education [KLME1205, KLME1107]; State Key Laboratory of Severe Weather [2013LASW-B06]; Qing-Lan Project for Cloud-Fog-Precipitation-Aerosol Study in Jiangsu Province; Priority Academic Program Development of Jiangsu Higher Education Institutions; U.S. Department of Energy's (DOE) Earth System Modeling (ESM) program via FASTER project; Atmospheric System Research (ASR) program FX Supported by National Natural Science Foundation of China (41305120, 41030962, 41275151, 41375138, 41375137, and 41305034), Natural Science Foundation of Jiangsu Province (BK20130988, SK201220841), Specialized Research Fund for the Doctoral Program of Higher Education (20133228120002), China Meteorological Administration Special Public Welfare Research Fund (GYHY201406007), Natural Science Foundation of the Higher Education Institutions of Jiangsu Province (13KJB170014), Open Funding from Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration (KDW1201, KDW1102), Open Funding from Key Laboratory of Meteorological Disaster of Ministry of Education (KLME1205, KLME1107), Open Funding from State Key Laboratory of Severe Weather (2013LASW-B06), Qing-Lan Project for Cloud-Fog-Precipitation-Aerosol Study in Jiangsu Province, Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions, and U.S. Department of Energy's (DOE) Earth System Modeling (ESM) program via the FASTER project (www.bnl.gov/faster) and Atmospheric System Research (ASR) program. NR 102 TC 4 Z9 6 U1 4 U2 15 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 0894-0525 EI 2191-4788 J9 ACTA METEOROL SIN JI Acta Meteorol. Sin. PD DEC PY 2013 VL 27 IS 6 BP 832 EP 848 DI 10.1007/s13351-013-0610-0 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AA2XA UT WOS:000330956300006 ER PT J AU Ziebell, AL Barb, JG Sandhu, S Moyers, BT Sykes, RW Doeppke, C Gracom, KL Carlile, M Marek, LF Davis, MF Knapp, SJ Burke, JM AF Ziebell, Angela L. Barb, Jessica G. Sandhu, Sukhpreet Moyers, Brook T. Sykes, Robert W. Doeppke, Crissa Gracom, Kristen L. Carlile, Melissa Marek, Laura F. Davis, Mark F. Knapp, Steven J. Burke, John M. TI Sunflower as a biofuels crop: An analysis of lignocellulosic chemical properties SO BIOMASS & BIOENERGY LA English DT Article DE Biomass; Lignocellulosic biofuel; Lignin; S/G-lignin; Sugar content; Pyrolysis Molecular Beam Mass; Spectrometry ID LIGNIN CONTENT; POPULUS; BIOMASS; POPLAR; SWITCHGRASS; HYDROLYSIS; HELIANTHUS; SORGHUM; GENOME; XYLOSE AB Four accessions of cultivated sunflower (Helianthus annuus) and silverleaf sunflower (Hellanthus argophyllus), were each grown in three locations (Georgia, British Columbia, and Iowa) at different planting densities and phenotyped for biomass-related traits and wood biochemistry. In most environments, H. argophyllus produced significantly more biomass than H. annuus. Cell wall chemistry for a subset of plants grown in Georgia and Iowa was assessed using analytical wet chemistry methods to measure lignin and sugar content/composition. The analysis of lignin and the S/G-lignin ratios for a larger number of samples (n > 250) was also assessed by high-throughput pyrolysis Molecular Beam Mass Spectrometry. Average pyMBMS estimated lignin content (i.e., dry weight fraction) for 60 C dried basal stem samples of H. annuus and H. argophyllus was 29.6% (range, 24.0%-34.6%) and 28.6% (range, 24.6%-33.3%), respectively when averaged across all environments. The average S/G lignin mass ratio was 1.5 (range, 1.0-2.0) for H. annuus and 1.7 (range, 1.0-2.4) in H. argophyllus. Stem samples from these two species only differed statistically for a few cell wall chemistry traits; however, accession level differences within each species were apparent. Cell wall chemistry in both species was significantly affected by both location and planting density, thus demonstrating the need to select for these traits in the environment for which the crop will be produced. Overall, these results show that cultivated sunflower and silverleaf sunflower both possess the necessary phenotypic diversity to facilitate the development of a hybrid sunflower with improved lignocellulosic biofuels traits, namely increased biomass, decreased lignin, and increased glucan. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Ziebell, Angela L.; Sykes, Robert W.; Doeppke, Crissa; Gracom, Kristen L.; Carlile, Melissa; Davis, Mark F.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Barb, Jessica G.; Burke, John M.] Univ Georgia, Dept Plant Biol, Athens, GA 30602 USA. [Sandhu, Sukhpreet; Knapp, Steven J.] Univ Georgia, Inst Plant Breeding Genet & Genom, Athens, GA 30602 USA. [Moyers, Brook T.] Univ British Columbia, Dept Bot, Vancouver, BC V6T 1Z4, Canada. [Marek, Laura F.] Iowa State Univ, USDA ARS, North Cent Reg Plant Intro Stn, Ames, IA 50014 USA. RP Burke, JM (reprint author), Univ Georgia, Dept Plant Biol, Miller Plant Sci Bldg, Athens, GA 30602 USA. EM jmburke@uga.edu RI Burke, John/A-3502-2013; OI Burke, John/0000-0002-1412-5539; davis, mark/0000-0003-4541-9852; Moyers, Brook/0000-0003-0340-9488 FU US Department of Agriculture; US Department of Energy; USDA-NIFA [2008-35504-04854]; USDA DOE [ER64664] FX The authors would like to thank the US Department of Agriculture and the US Department of Energy for the funding provided to support this work (USDA-NIFA Award no. 2008-35504-04854, USDA DOE Plant Feedstock Genomics for Bioenergy ER64664). NR 43 TC 4 Z9 4 U1 0 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0961-9534 EI 1873-2909 J9 BIOMASS BIOENERG JI Biomass Bioenerg. PD DEC PY 2013 VL 59 BP 208 EP 217 DI 10.1016/j.biombioe.2013.06.009 PG 10 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA AA2FL UT WOS:000330910400020 ER PT J AU Moon, J Speziale, S Meral, C Kalkan, B Clark, SM Monteiro, PJM AF Moon, Juhyuk Speziale, Sergio Meral, Cagla Kalkan, Bora Clark, Simon M. Monteiro, Paulo J. M. TI Determination of the elastic properties of amorphous materials: Case study of alkali-silica reaction gel SO CEMENT AND CONCRETE RESEARCH LA English DT Article DE Amorphous material; X-ray diffraction; Alkali-aggregate reaction; Elastic moduli ID DIAMOND-ANVIL CELL; REACTION INDUCED EXPANSION; X-RAY-DIFFRACTION; HIGH-PRESSURE; ASR GEL; BRILLOUIN SPECTROSCOPY; SINGLE-CRYSTAL; TOBERMORITE; ETTRINGITE; SCATTERING AB The gel formed during alkali-silica reaction (ASR) can lead to cracking and deterioration of a concrete structure. The elastic properties of the ASR gel using X-ray absorption and Brillouin spectroscopy measurements are reported. X-ray absorption was used to determine the density of the gel as a function of pressure, and the result yields an isothermal bulk modulus of 33 +/- 2 GPa. Brillouin spectroscopy was applied to measure isentropic bulk (24.9-34.0 GPa) and shear moduli (8.7-10.1 GPa) of the gel. The range of values obtained is attributed to the variable composition of samples that were collected under field conditions. Results suggested that amorphous silica becomes expanded and compressible as it absorbs water molecules and alkali ions. This could explain high gel migration rates through the complex pore structures in concrete. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Moon, Juhyuk] SUNY Stony Brook, Dept Mech Engn, Civil Engn Program, Stony Brook, NY 11794 USA. [Speziale, Sergio] Deutsch GeoForschungsZentrum GFZ, D-14473 Potsdam, Germany. [Meral, Cagla; Monteiro, Paulo J. M.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Meral, Cagla] Middle E Tech Univ, Dept Civil Engn, TR-06800 Ankara, Turkey. [Kalkan, Bora; Clark, Simon M.] Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA USA. [Clark, Simon M.] Macquarie Univ, Dept Earth & Planetary Sci, N Ryde, NSW 2109, Australia. RP Monteiro, PJM (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, 725 Davis Hall, Berkeley, CA 94720 USA. EM monteiro@ce.berkeley.edu RI Moon, Juhyuk/B-7009-2016; Meral, Cagla/K-8590-2013; Clark, Simon/B-2041-2013 OI Moon, Juhyuk/0000-0002-7049-892X; Meral, Cagla/0000-0001-8720-1216; Clark, Simon/0000-0002-7488-3438 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 41 TC 7 Z9 7 U1 8 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-8846 EI 1873-3948 J9 CEMENT CONCRETE RES JI Cem. Concr. Res. PD DEC PY 2013 VL 54 BP 55 EP 60 DI 10.1016/j.cemconres.2013.08.012 PG 6 WC Construction & Building Technology; Materials Science, Multidisciplinary SC Construction & Building Technology; Materials Science GA 300UC UT WOS:000330488500007 ER PT J AU Cole, JK Gieler, BA Heisler, DL Palisoc, MM Williams, AJ Dohnalkova, AC Ming, H Yu, TT Dodsworth, JA Li, WJ Hedlund, BP AF Cole, Jessica K. Gieler, Brandon A. Heisler, Devon L. Palisoc, Maryknoll M. Williams, Amanda J. Dohnalkova, Alice C. Ming, Hong Yu, Tian Tian Dodsworth, Jeremy A. Li, Wen-Jun Hedlund, Brian P. TI Kallotenue papyrolyticum gen. nov., sp nov., a cellulolytic and filamentous thermophile that represents a novel lineage (Kallotenuales ord. nov., Kallotenuaceae fam. nov.) within the class Chloroflexia SO INTERNATIONAL JOURNAL OF SYSTEMATIC AND EVOLUTIONARY MICROBIOLOGY LA English DT Article ID BACTERIUM HERPETOSIPHON-AURANTIACUS; PERFORMANCE LIQUID-CHROMATOGRAPHY; EMENDED DESCRIPTION; GLIDING BACTERIUM; SINGLE-CELL; HOT-SPRINGS; KEBRIT DEEP; RED-SEA; PEPTIDOGLYCAN; COMMUNITIES AB Several closely related, thermophilic and cellulolytic bacterial strains, designated JKG1(T), JKG2, JKG3, JKG4 and JKG5, were isolated from a cellulolytic enrichment (corn stover) incubated in the water column of Great Boiling Spring, NV. Strain JKG1(T) had cells of diameter 0.7-0.9 mu m and length similar to 2.0 mu m that formed non-branched, multicellular filaments reaching >300 mu m. Spores were not formed and dense liquid cultures were red. The temperature range for growth was 45-65 degrees C, with an optimum of 55 degrees C. The pH range for growth was pH 5.6-9.0, with an optimum of pH 7.5. JKG1(T) grew as an aerobic heterotroph, utilizing glucose, sucrose, xylose, arabinose, cellobiose, CM-cellulose, filter paper, microcrystalline cellulose, xylan, starch, Casamino acids, tryptone, peptone, yeast extract, acetate, citrate, lactate, pyruvate and glycerol as sole carbon sources, and was not observed to photosynthesize. The cells stained Gram-negative. Phylogenetic analysis using 16S rRNA gene sequences placed the new isolates in the class Chloroflexia, but distant from other cultivated members, with the highest sequence identity of 82.5% to Roseiflexus castenholzii. The major quinone was menaquinone-9; no ubiquinones were detected. The major cellular fatty acids (>5%) were C-18:0, anteiso-C-17:0, iso-C-18:0, iso-C-17:0, C-16:0, iso-C-16:0 and C-17:0. The peptidoglycan amino acids were alanine, ornithine, glutamic acid, serine and asparagine. Whole-cell sugars included mannose, rhamnose, glucose, galactose, ribose, arabinose and xylose. Morphological, phylogenetic and chemotaxonomic results suggest that JKG1(T) is representative of a new lineage within the class Chloroflexia, which we propose to designate Kallotenue papyrolyticum gen. nov., sp. nov., Kallotenuaceae fam. nov., Kallotenuales ord. nov. The type strain of Kallotenue papyrolyticum gen. nov., sp. nov. is JKG1(T) (=DSM 26889(T)=JCM 19132(T)). C1 [Cole, Jessica K.; Gieler, Brandon A.; Heisler, Devon L.; Palisoc, Maryknoll M.; Williams, Amanda J.; Dodsworth, Jeremy A.; Hedlund, Brian P.] Univ Nevada, Sch Life Sci, Las Vegas, NV 89154 USA. [Dohnalkova, Alice C.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Ming, Hong; Yu, Tian Tian; Li, Wen-Jun] Yunnan Univ, Sch Life Sci, Yunnan Inst Microbiol, Kunming 650091, Peoples R China. RP Hedlund, BP (reprint author), Univ Nevada, Sch Life Sci, 4505 S Maryland Pkwy, Las Vegas, NV 89154 USA. EM brian.hedlund@unlv.edu FU Department of Energy's Office of Biological and Environmental Research; National Science Foundation [EPSCoR RII EPS-0814372, REU DBI-1005223, MCB-0546865, OISE-0968421]; US Department of Energy [DE-EE-0000716, Urban 21, JGI CSP-182, EMSL Rapid 47730]; US Department of Energy (Nevada Renewable Energy Consortium); National Basic Research Program of China [2010CB833801]; National Natural Science Foundation of China [31070007]; Key Project of International Cooperation of China Ministry of Science & Technology (MOST) [2013DFA31980]; UNLV Foundation FX The authors thank David and Sandy Jamieson for gracious support and access to GBS, Drs Steve Quake and Paul Blainey for use of the optical tweezers and microfluidic cell-sorting device, Dr James Raymond for use of the lyophilizer, Bruce Dale for providing corn stover, and Dr Jean Euzeby for extensive advice on taxonomic designations. Additional thanks to Duy Trinh and Kelly Orbeck for assistance with cultivation. Electron microscopy was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. This work was supported by grants funded by the National Science Foundation (EPSCoR RII EPS-0814372, REU DBI-1005223, MCB-0546865 and OISE-0968421); the US Department of Energy (DE-EE-0000716, Urban 21, JGI CSP-182, EMSL Rapid 47730 and Nevada Renewable Energy Consortium); National Basic Research Program of China (no. 2010CB833801); National Natural Science Foundation of China (no. 31070007); and Key Project of International Cooperation of China Ministry of Science & Technology (MOST no. 2013DFA31980). B. P. H acknowledges generous funding from Greg Fullmer from a donation through the UNLV Foundation. NR 48 TC 3 Z9 3 U1 1 U2 14 PU SOC GENERAL MICROBIOLOGY PI READING PA MARLBOROUGH HOUSE, BASINGSTOKE RD, SPENCERS WOODS, READING RG7 1AG, BERKS, ENGLAND SN 1466-5026 EI 1466-5034 J9 INT J SYST EVOL MICR JI Int. J. Syst. Evol. Microbiol. PD DEC PY 2013 VL 63 BP 4675 EP 4682 DI 10.1099/ijs.0.053348-0 PN 12 PG 8 WC Microbiology SC Microbiology GA AA2KB UT WOS:000330922400045 PM 23950149 ER PT J AU Depuydt, G Xie, F Petyuk, VA Shanmugam, N Smolders, A Dhondt, I Brewer, HM Camp, DG Smith, RD Braeckman, BP AF Depuydt, Geert Xie, Fang Petyuk, Vladislav A. Shanmugam, Nilesh Smolders, Arne Dhondt, Ineke Brewer, Heather M. Camp, David G. Smith, Richard D. Braeckman, Bart P. TI Reduced Insulin/Insulin-like Growth Factor-1 Signaling and Dietary Restriction Inhibit Translation but Preserve Muscle Mass in Caenorhabditis elegans SO MOLECULAR & CELLULAR PROTEOMICS LA English DT Article ID LIFE-SPAN EXTENSION; MESSENGER-RNA TRANSLATION; CHAIN AMINO-ACIDS; C-ELEGANS; GENE-EXPRESSION; SACCHAROMYCES-CEREVISIAE; RIBOSOMAL-PROTEINS; INDUCED LONGEVITY; DAUER LARVAE; POSTTRANSCRIPTIONAL MECHANISMS C1 [Depuydt, Geert; Shanmugam, Nilesh; Smolders, Arne; Dhondt, Ineke; Braeckman, Bart P.] Univ Ghent, Dept Biol, B-9000 Ghent, Belgium. [Xie, Fang; Petyuk, Vladislav A.; Brewer, Heather M.; Camp, David G.; Smith, Richard D.] Pacific NW Natl Lab, Biol Sci Div, Richland, WA 99352 USA. [Xie, Fang; Petyuk, Vladislav A.; Brewer, Heather M.; Camp, David G.; Smith, Richard D.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Braeckman, BP (reprint author), Univ Ghent, Dept Biol, Proeftuinstr 86 N1, B-9000 Ghent, Belgium. EM Bart.Braeckman@UGent.be RI Smith, Richard/J-3664-2012; OI Smith, Richard/0000-0002-2381-2349; Smolders, Arne/0000-0003-0926-2392; Petyuk, Vladislav/0000-0003-4076-151X FU U.S. Department of Energy [DE-AC05-76RL01830]; Fund for Scientific Research-Flanders [G.04371.0N]; NIH National Center for Research Resources [RR18522]; BOF project of Ghent University [01J04208] FX The strains GA154 glp-4(bn2ts)I; daf-2(e1370)III and GA153 glp-4(bn2ts)I daf-16(mgDf50)I; daf-2(e1370)III were kindly provided by David Gems. We are grateful to Renata Coopman for her assistance in culturing and sampling worm cohorts. We also thank Myriam Claeys and Ineke Dhondt for assisting with TEM imaging. Proteomic analyses were performed in the Environmental Molecular Sciences Laboratory, a U.S. Department of Energy (DOE) national scientific user facility located at the Pacific Northwest National Laboratory in Richland, WA. PNNL is a multi- program national laboratory operated by Battelle Memorial Institute for the U.S. Department of Energy under Contract DE-AC05-76RL01830. HPLC analysis was performed by the NutriFOODchem unit (Department of Food Safety and Food Quality) at Ghent University.; This work was supported by a grant from the Fund for Scientific Research-Flanders (G.04371.0N) to B.P.B. and the NIH National Center for Research Resources (RR18522 to R.D.S.). G.D. was supported by a BOF project of Ghent University (01J04208). NR 160 TC 31 Z9 33 U1 1 U2 24 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 1535-9476 EI 1535-9484 J9 MOL CELL PROTEOMICS JI Mol. Cell. Proteomics PD DEC PY 2013 VL 12 IS 12 BP 3624 EP 3639 DI 10.1074/mcp.M113.027383 PG 16 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA 293SI UT WOS:000329993600016 PM 24002365 ER PT J AU Velarde, L Lu, Z Wang, HF AF Velarde, Luis Lu, Zhou Wang, Hong-fei TI Coherent Vibrational Dynamics and High-resolution Nonlinear Spectroscopy: A Comparison with the Air/DMSO Liquid Interface SO CHINESE JOURNAL OF CHEMICAL PHYSICS LA English DT Article DE Sum-frequency generation vibrational spectroscopy (SFG-VS); High-resolution broadband SFG-VS; Free-induction decay; Dimethyl sulfoxide; Air/DMSO interface ID SUM-FREQUENCY GENERATION; SFG-VS; MOLECULAR-ORIENTATION; DIMETHYL-SULFOXIDE; SURFACE; PROBE; CONFORMATION; METHYLENE; SPECTRA; CO AB We present a comparative study on the C-H stretching vibrations at air/DMSO (dimethyl sulfoxide) interface with both the free-induction decay (FID) coherent vibrational dynamics and the sub-wavenumber high resolution sum-frequency generation vibrational spectroscopy measurements. In principle the frequency-domain and time-domain spectroscopic measurements should generate identical information for a given molecular system. However, when the molecular systems are with several coupled or overlapping vibrational modes, obtaining detailed spectroscopic and coherent dynamics information is not as straightforward and rather difficult from either the time-domain or the frequency domain measurements. For the case of air/DMSO interface that is with moderately complex vibrational spectra, we show that the frequency-domain measurement with sub-wavenumber high-resolution sum-frequency generation vibrational spectroscopy is probably more advantageous than the time-domain measurement in obtaining quantitative understanding of the structure and coherent dynamics of the molecular interface. C1 [Velarde, Luis; Lu, Zhou; Wang, Hong-fei] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. RP Wang, HF (reprint author), Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. EM hongfei.wang@pnnl.gov RI Wang, Hongfei/B-1263-2010; Lu, Zhou/D-3994-2012; Velarde, Luis/D-4929-2011 OI Wang, Hongfei/0000-0001-8238-1641; Lu, Zhou/0000-0001-8527-0381; Velarde, Luis/0000-0001-6329-3486 FU Pacific Northwest National Laboratory (PNNL) LDRD program; Department of Energy's Office of Biological and Environmental Research (BER) FX This work was supported by the Pacific Northwest National Laboratory (PNNL) LDRD program, and was conducted at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at the Pacific Northwest National Laboratory and sponsored by the Department of Energy's Office of Biological and Environmental Research (BER). NR 49 TC 5 Z9 5 U1 1 U2 23 PU CHINESE PHYSICAL SOC PI BEIJING PA P O BOX 603, BEIJING 100080, PEOPLES R CHINA SN 1674-0068 EI 1003-7713 J9 CHINESE J CHEM PHYS JI Chin. J. Chem. Phys. PD DEC PY 2013 VL 26 IS 6 BP 710 EP 720 DI 10.1063/1674-0068/26/06/710-720 PG 11 WC Physics, Atomic, Molecular & Chemical SC Physics GA 302GS UT WOS:000330591600015 ER PT J AU Kerkar, PB Horvat, K Mahajan, D Jones, KW AF Kerkar, Prasad B. Horvat, Kristine Mahajan, Devinder Jones, Keith W. TI Formation and Dissociation of Methane Hydrates from Seawater in Consolidated Sand: Mimicking Methane Hydrate Dynamics beneath the Seafloor SO ENERGIES LA English DT Article DE methane; hydrates; seawater; Ottawa sand; formation; dissociation; enthalpy ID PORE-SIZE DISTRIBUTIONS; CARBON-DIOXIDE; CLATHRATE HYDRATE; POROUS-MEDIA; PHASE-EQUILIBRIA; SILICA-GELS; PROPANE; SEDIMENT; TEMPERATURES; PRESSURES AB Methane hydrate formation and dissociation kinetics were investigated in seawater-saturated consolidated Ottawa sand-pack under sub-seafloor conditions to study the influence of effective pressure on formation and dissociation kinetics. To simulate a sub-seafloor environment, the pore-pressure was varied relative to confining pressure in successive experiments. Hydrate formation was achieved by methane charging followed by sediment cooling. The formation of hydrates was delayed with increasing degree of consolidation. Hydrate dissociation by step-wise depressurization was instantaneous, emanating preferentially from the interior of the sand-pack. Pressure drops during dissociation and in situ temperature controlled the degree of endothermic cooling within sediments. In a closed system, the post-depressurization dissociation was succeeded by thermally induced dissociation and pressure-temperature conditions followed theoretical methane-seawater equilibrium conditions and exhibited excess pore pressure governed by the pore diameter. These post-depressurization equilibrium values for the methane hydrates in seawater saturated consolidated sand-pack were used to estimate the enthalpy of dissociation of 55.83 +/- 1.41 kJ/mol. These values were found to be lower than those reported in earlier literature for bulk hydrates from seawater (58.84 kJ/mol) and pure water (62.61 kJ/mol) due to excess pore pressure generated within confined sediment system under investigation. However, these observations could be significant in the case of hydrate dissociation in a subseafloor environment where dissociation due to depressurization could result in an instantaneous methane release followed by slow thermally induced dissociation. The excess pore pressure generated during hydrate dissociation could be higher within fine-grained sediments with faults and barriers present in subseafloor settings which could cause shifting in geological layers. C1 [Kerkar, Prasad B.] Shell Int Explorat & Prod Inc, Houston, TX 77082 USA. [Horvat, Kristine; Mahajan, Devinder] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Mahajan, Devinder] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Jones, Keith W.] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. RP Kerkar, PB (reprint author), Shell Int Explorat & Prod Inc, 3333 Hwy 6 South,M-1018, Houston, TX 77082 USA. EM prasad.kerkar@shell.com; kristine.horvat@stonybrook.edu; dmahajan@bnl.gov; jones@bnl.gov FU Office of Fossil Energy, US Department of Energy [DE-AC02-98CH10886]; Office of Vice Presidential Research, Stony Brook University FX This work was supported by the Office of Fossil Energy, US Department of Energy under contract No. DE-AC02-98CH10886. Partial support from the Office of Vice Presidential Research, Stony Brook University is also acknowledged. The experimental work was performed at Brookhaven National Laboratory, Upton, NY as a part of Doctoral dissertation of Prasad B. Kerkar, Stony Brook University. NR 26 TC 3 Z9 4 U1 3 U2 24 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 1996-1073 J9 ENERGIES JI Energies PD DEC PY 2013 VL 6 IS 12 BP 6225 EP 6241 DI 10.3390/en6126225 PG 17 WC Energy & Fuels SC Energy & Fuels GA 297YI UT WOS:000330290600006 ER PT J AU Taylor, CN Luitjohan, KE Heim, B Kollar, L Allain, JP Skinner, CH Kugel, HW Kaita, R Roquemore, AL Maingi, R AF Taylor, C. N. Luitjohan, K. E. Heim, B. Kollar, L. Allain, J. P. Skinner, C. H. Kugel, H. W. Kaita, R. Roquemore, A. L. Maingi, R. TI Surface chemistry analysis of lithium conditioned NSTX graphite tiles correlated to plasma performance SO FUSION ENGINEERING AND DESIGN LA English DT Article DE Lithium; Deuterium; Retention; Carbon-facing components; Divertor; X-ray photoelectron spectroscopy; Plasma-surface interactions ID CDX-U; WALL; TFTR; DISCHARGES; INJECTION; TOKAMAKS; LIMITER AB Lithium wall conditioning in NSTX has resulted in reduced divertor recycling, improved energy confinement, and reduced frequency of edge-localized modes (ELMS), up to the point of complete ELM suppression. NSTX tiles were removed from the vessel following the 2008 campaign and subsequently analyzed using X-ray photoelectron spectroscopy as well as nuclear reaction ion beam analysis. In this paper we relate surface chemistry to deuterium retention/recycling, develop methods for cleaning of passivated NSTX tiles, and explore a method to effectively extract bound deuterium from lithiated graphite. Li-O-D and Li-C-D complexes characteristic of deuterium retention that form during NSTX operations are revealed by sputter cleaning and heating. Heating to similar to 850 C desorbed all deuterium complexes observed in the 0 1s and C 1s photoelectron energy ranges. Tile locations within approximately +/- 2.5 cm of the lower vertical/horizontal divertor corner appear to have unused Li-O bonds that are not saturated with deuterium, whereas locations immediately outboard of this region indicate high deuterium recycling. X-ray photo electron spectra of a specific NSTX tile with wide ranging lithium coverage indicate that a minimum lithium dose, 100-500 nm equivalent thickness, is required for effective deuterium retention. This threshold is suspected to be highly sensitive to surface morphology. The present analysis may explain why plasma discharges in NSTX continue to benefit from lithium coating thickness beyond the divertor deuterium ion implantation depth, which is nominally <10 nm. (C) 2013 Elsevier B.V. All rights reserved. C1 [Taylor, C. N.; Luitjohan, K. E.; Heim, B.; Kollar, L.; Allain, J. P.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47906 USA. [Taylor, C. N.; Heim, B.; Allain, J. P.] Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Skinner, C. H.; Kaita, R.; Roquemore, A. L.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Maingi, R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Taylor, CN (reprint author), Idaho Natl Lab, Fus Safety Program, POBox 1625, Idaho Falls, ID 83415 USA. EM chase.taylor@inl.gov OI Allain, Jean Paul/0000-0003-1348-262X FU Purdue University Graduate School; US DOE [DE-FG02-08ER54990, DE-AC02-09CH11466] FX We would like to thank the Purdue University Graduate School for providing student funding, T. Morton for his contributions in running experiments and sample preparation, L. Guttadora at the Princeton Plasma Physics Laboratory for helping with sample core extraction. Work supported by US DOE Contract DE-FG02-08ER54990 and DE-AC02-09CH11466. NR 44 TC 6 Z9 6 U1 5 U2 23 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0920-3796 EI 1873-7196 J9 FUSION ENG DES JI Fusion Eng. Des. PD DEC PY 2013 VL 88 IS 12 BP 3157 EP 3164 DI 10.1016/j.fusengdes.2013.09.007 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 296AW UT WOS:000330158500008 ER PT J AU Tatsuta, T Hosono, M Miura, Y Sugawara, S Kariya, Y Hakomori, S Nitta, K AF Tatsuta, Takeo Hosono, Masahiro Miura, Yuki Sugawara, Shigeki Kariya, Yukiko Hakomori, Senitiroh Nitta, Kazuo TI Involvement of ER stress in apoptosis induced by sialic acid-binding lectin (leczyme) from bullfrog eggs SO INTERNATIONAL JOURNAL OF ONCOLOGY LA English DT Article DE lectin; ribonuclease; leczyme; ER-stress; caspase pathway; mitochondria perturbation ID ENDOPLASMIC-RETICULUM STRESS; UNFOLDED PROTEIN RESPONSE; RANA-CATESBEIANA EGGS; DRUG-INDUCED APOPTOSIS; CANCER-CELLS; TUMOR-CELLS; IN-VIVO; ACTIVATION; JAPONICA; RIBONUCLEASE AB Sialic-acid binding lectin (SBL) isolated from bullfrog (Rana catesbeiana) oocytes is a multifunctional protein which has lectin activity, ribonuclease activity and cancer-selective antitumor activity. It has been reported that SBL induces apoptosis accompanied by rigid mitochondrial perturbation, which indicates mediation of the intrinsic pathway. However, the mechanism of the antitumor effect of SBL has not been fully elucidated. We report, here, that ER stress is evoked in SBL-treated cells. We show that caspase-4, an initiator caspase of ER stress-mediated apoptosis was activated, and inhibition of caspase-4 resulted in significant attenuation of apoptosis induced by SBL. We analyzed the precise mechanism of activation of the caspase cascade induced by SBL, and found that caspase-9 and -4 are activated upstream of activation of caspase-8. Further study revealed that SBL induces the mitochondrial and ER stress-mediated pathways independently. It is noteworthy that SBL can induce cancer-selective apoptosis by multiple apoptotic signaling pathways, and it can serve as a candidate molecule for anticancer drugs in a novel field. C1 [Tatsuta, Takeo; Hosono, Masahiro; Miura, Yuki; Sugawara, Shigeki; Nitta, Kazuo] Tohoku Pharmaceut Univ, Inst Mol Biomembrane & Glycobiol, Div Cell Recognit Study, Sendai, Miyagi 9818558, Japan. [Kariya, Yukiko] Fukushima Med Univ, Fukushima 9601295, Japan. [Hakomori, Senitiroh] Pacific Northwest Res Inst, Div Biomembrane Res, Seattle, WA 98122 USA. RP Nitta, K (reprint author), Tohoku Pharmaceut Univ, Inst Mol Biomembrane & Glycobiol, Div Cell Recognit Study, Aoba Ku, 4-4-1 Komatsushima, Sendai, Miyagi 9818558, Japan. EM knitta@tohoku-pharm.ac.jp FU Ministry of Education, Culture, Sports, Science and Technology of Japan FX This study was supported in part by Grant-in-Aid of the 'Academic Frontier' Project for Private Universities from the Ministry of Education, Culture, Sports, Science and Technology of Japan. NR 44 TC 7 Z9 8 U1 0 U2 8 PU SPANDIDOS PUBL LTD PI ATHENS PA POB 18179, ATHENS, 116 10, GREECE SN 1019-6439 EI 1791-2423 J9 INT J ONCOL JI Int. J. Oncol. PD DEC PY 2013 VL 43 IS 6 BP 1799 EP 1808 DI 10.3892/ijo.2013.2128 PG 10 WC Oncology SC Oncology GA 297AA UT WOS:000330225800008 PM 24100413 ER PT J AU Zhang, MH Bretherton, CS Blossey, PN Austin, PH Bacmeister, JT Bony, S Brient, F Cheedela, SK Cheng, AN Del Genio, AD De Roode, SR Endo, S Franklin, CN Golaz, JC Hannay, C Heus, T Isotta, FA Dufresne, JL Kang, IS Kawai, H Kohler, M Larson, VE Liu, YG Lock, AP Lohmann, U Khairoutdinov, MF Molod, AM Neggers, RAJ Rasch, P Sandu, I Senkbeil, R Siebesma, AP Siegenthaler-Le Drian, C Stevens, B Suarez, MJ Xu, KM von Salzen, K Webb, MJ Wolf, A Zhao, M AF Zhang, Minghua Bretherton, Christopher S. Blossey, Peter N. Austin, Phillip H. Bacmeister, Julio T. Bony, Sandrine Brient, Florent Cheedela, Suvarchal K. Cheng, Anning Del Genio, Anthony D. De Roode, Stephan R. Endo, Satoshi Franklin, Charmaine N. Golaz, Jean-Christophe Hannay, Cecile Heus, Thijs Isotta, Francesco Alessandro Dufresne, Jean-Louis Kang, In-Sik Kawai, Hideaki Koehler, Martin Larson, Vincent E. Liu, Yangang Lock, Adrian P. Lohmann, Ulrike Khairoutdinov, Marat F. Molod, Andrea M. Neggers, Roel A. J. Rasch, Philip Sandu, Irina Senkbeil, Ryan Siebesma, A. Pier Siegenthaler-Le Drian, Colombe Stevens, Bjorn Suarez, Max J. Xu, Kuan-Man von Salzen, Knut Webb, Mark J. Wolf, Audrey Zhao, Ming TI CGILS: Results from the first phase of an international project to understand the physical mechanisms of low cloud feedbacks in single column models SO JOURNAL OF ADVANCES IN MODELING EARTH SYSTEMS LA English DT Article ID GENERAL-CIRCULATION MODELS; GLOBAL CLIMATE MODEL; COMMUNITY ATMOSPHERE MODEL; SHALLOW CUMULUS CLOUDS; BOUNDARY-LAYER CLOUDS; MASS FLUX FRAMEWORK; PDF-BASED MODEL; PART I; MOIST CONVECTION; PARAMETERIZATION AB CGILS-the CFMIP-GASS Intercomparison of Large Eddy Models (LESs) and single column models (SCMs)-investigates the mechanisms of cloud feedback in SCMs and LESs under idealized climate change perturbation. This paper describes the CGILS results from 15 SCMs and 8 LES models. Three cloud regimes over the subtropical oceans are studied: shallow cumulus, cumulus under stratocumulus, and well-mixed coastal stratus/stratocumulus. In the stratocumulus and coastal stratus regimes, SCMs without activated shallow convection generally simulated negative cloud feedbacks, while models with active shallow convection generally simulated positive cloud feedbacks. In the shallow cumulus alone regime, this relationship is less clear, likely due to the changes in cloud depth, lateral mixing, and precipitation or a combination of them. The majority of LES models simulated negative cloud feedback in the well-mixed coastal stratus/stratocumulus regime, and positive feedback in the shallow cumulus and stratocumulus regime. A general framework is provided to interpret SCM results: in a warmer climate, the moistening rate of the cloudy layer associated with the surface-based turbulence parameterization is enhanced; together with weaker large-scale subsidence, it causes negative cloud feedback. In contrast, in the warmer climate, the drying rate associated with the shallow convection scheme is enhanced. This causes positive cloud feedback. These mechanisms are summarized as the "NESTS" negative cloud feedback and the "SCOPE" positive cloud feedback (Negative feedback from Surface Turbulence under weaker Subsidence-Shallow Convection PositivE feedback) with the net cloud feedback depending on how the two opposing effects counteract each other. The LES results are consistent with these interpretations. C1 [Zhang, Minghua; Khairoutdinov, Marat F.] SUNY Stony Brook, Inst Terr & Planetary Atmospheres, Sch Marine & Atmospher Sci, Stony Brook, NY 11794 USA. [Bretherton, Christopher S.; Blossey, Peter N.] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. [Austin, Phillip H.] Univ British Columbia, Dept Earth & Ocean Sci, Vancouver, BC V5Z 1M9, Canada. [Bacmeister, Julio T.; Hannay, Cecile] Natl Ctr Atmospher Res, Earth Syst Lab, Boulder, CO 80307 USA. [Bony, Sandrine; Brient, Florent; Dufresne, Jean-Louis] IPSL, Lab Meteorol Dynam, Paris, France. [Cheedela, Suvarchal K.; Heus, Thijs; Sandu, Irina; Stevens, Bjorn] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Cheng, Anning; Xu, Kuan-Man] NASA, Langley Res Ctr, Hampton, VA 23665 USA. [Del Genio, Anthony D.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [De Roode, Stephan R.] Delft Univ Technol, Dept Geosci & Remote Sensing, Delft, Netherlands. [Endo, Satoshi; Liu, Yangang] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. [Franklin, Charmaine N.] CSIRO, Ctr Australian Weather & Climate Res, Aspendale, Vic, Australia. [Golaz, Jean-Christophe; Zhao, Ming] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Isotta, Francesco Alessandro; Lohmann, Ulrike; Siegenthaler-Le Drian, Colombe] Swiss Fed Inst Technol, Zurich, Switzerland. [Kang, In-Sik] Seoul Natl Univ, Sch Earth & Environm Sci, Seoul, South Korea. [Kawai, Hideaki] Meteorol Res Inst, Tsukuba, Ibaraki 305, Japan. [Koehler, Martin; Sandu, Irina] European Ctr Medium Range Weather Forecasts, Reading RG2 9AX, Berks, England. [Larson, Vincent E.; Senkbeil, Ryan] Univ Wisconsin, Dept Math Sci, Milwaukee, WI 53201 USA. [Lock, Adrian P.; Webb, Mark J.] Met Off Hadley Ctr, Exeter, Devon, England. [Molod, Andrea M.; Suarez, Max J.] NASA, Global Modeling & Assimilat Off, Goddard Space Flight Ctr, Greenbelt, MD USA. [Neggers, Roel A. J.; Siebesma, A. Pier] Royal Netherlands Meteorol Inst KNMI, Div Atmospher Res, De Bilt, Netherlands. [Rasch, Philip] Pacific NW Natl Lab, Richland, WA 99352 USA. [von Salzen, Knut] Canadian Ctr Climate Modelling & Anal, Victoria, BC, Canada. [Wolf, Audrey] Columbia Univ, Goddard Inst Space Studies, New York, NY USA. RP Zhang, MH (reprint author), SUNY Stony Brook, Inst Terr & Planetary Atmospheres, Sch Marine & Atmospher Sci, Stony Brook, NY 11794 USA. EM minghua.zhang@stonybrook.edu RI Stevens, Bjorn/A-1757-2013; Lohmann, Ulrike/B-6153-2009; Golaz, Jean-Christophe/D-5007-2014; Liu, Yangang/H-6154-2011; Dufresne, Jean-Louis/I-5616-2015; Zhao, Ming/C-6928-2014; Heus, Thijs/E-7336-2012; Xu, Kuan-Man/B-7557-2013; 안, 민섭/D-9972-2015 OI Stevens, Bjorn/0000-0003-3795-0475; Lohmann, Ulrike/0000-0001-8885-3785; Golaz, Jean-Christophe/0000-0003-1616-5435; Bony, Sandrine/0000-0002-4791-4438; Dufresne, Jean-Louis/0000-0003-4764-9600; Heus, Thijs/0000-0003-2650-2423; Xu, Kuan-Man/0000-0001-7851-2629; FU Biological and Environmental Research Division in the Office of Sciences of the US Department of Energy (DOE) through its FASTER project; NASA Modeling and Analysis Program (MAP); US National Science Foundation; NSF Center for Multiscale Modeling and Prediction; Canada's NSERC; NASA MAP program; National Science Foundation [AGS-0968640]; US Department of Energy [DE-SC0006927]; DOE ASR program; Joint DECC/Defra Met Office Hadley Centre Climate Program [GA01101]; European Union [244067]; Australian Climate Change Science Program; Department of Climate Change and Energy Efficiency; Bureau of Meteorology; CSIRO; Deutscher Wetter Dienst (DWD) through the Hans-Ertel Centre for Weather Research, as part of the EUCLIPSE project under Framework Program 7 of the European Union; National Computing Facilities Foundation (NCF); National Science Foundation FX We thank two anonymous reviewers whose comments have led to a significant improvement of this paper. Sung-bin Park of the Seoul National University (SNU) participated in the initial phase of the CGILS project. His tragic death disrupted the submission of results from the SNU model. This paper serves as an appreciation and memory of him. Zhang's CGILS research is supported by the Biological and Environmental Research Division in the Office of Sciences of the US Department of Energy (DOE) through its FASTER project, by the NASA Modeling and Analysis Program (MAP) and the US National Science Foundation to the Stony Brook University. Bretherton and Blossey acknowledge support from the NSF Center for Multiscale Modeling and Prediction, Austin is supported by Canada's NSERC. Del Genio is supported by the NASA MAP program. V. Larson gratefully acknowledges support from the National Science Foundation (grant AGS-0968640) and the US Department of Energy (grant DE-SC0006927). Wolf was supported by the DOE ASR program. Webb was supported by the Joint DECC/Defra Met Office Hadley Centre Climate Program (GA01101) and funding from the European Union, Seventh Framework Program (FP7/2007-2013) under grant agreement number 244067 via the EU CLoud Intercomparison and Process Study Evaluation Project (EUCLIPSE). Franklin was supported by the Australian Climate Change Science Program, funded jointly by the Department of Climate Change and Energy Efficiency, the Bureau of Meteorology and CSIRO. Heus was funded by the Deutscher Wetter Dienst (DWD) through the Hans-Ertel Centre for Weather Research, as part of the EUCLIPSE project under Framework Program 7 of the European Union. The simulations with the Dutch LES model were sponsored by the National Computing Facilities Foundation (NCF). The National Center for Atmospheric Research is sponsored by the National Science Foundation. NR 75 TC 37 Z9 37 U1 0 U2 39 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 1942-2466 J9 J ADV MODEL EARTH SY JI J. Adv. Model. Earth Syst. PD DEC PY 2013 VL 5 IS 4 BP 826 EP 842 DI 10.1002/2013MS000246 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AA1BZ UT WOS:000330832600011 ER PT J AU Carpenter, KJ Weber, PK Davisson, ML Pett-Ridge, J Haverty, MI Keeling, PJ AF Carpenter, Kevin J. Weber, Peter K. Davisson, M. Lee Pett-Ridge, Jennifer Haverty, Michael I. Keeling, Patrick J. TI Correlated SEM, FIB-SEM, TEM, and NanoSIMS Imaging of Microbes from the Hindgut of a Lower Termite: Methods for In Situ Functional and Ecological Studies of Uncultivable Microbes SO MICROSCOPY AND MICROANALYSIS LA English DT Article DE bacteria; bioenergy; ecology; focused ion beam; SIMS; protists; scanning electron microscopy; stable isotopes; termites; transmission electron microscopy ID WOOD-FEEDING COCKROACH; COPTOTERMES-FORMOSANUS; ROACH CRYPTOCERCUS; PSEUDOTRICHONYMPHA-GRASSII; RETICULITERMES-SPERATUS; PHYLOGENETIC DIVERSITY; FLAGELLATED PROTISTS; ELECTRON-MICROSCOPY; NITROGEN-FIXATION; NEOTERMES-CUBANUS AB The hindguts of lower termites harbor highly diverse, endemic communities of symbiotic protists, bacteria, and archaea essential to the termite's ability to digest wood. Despite over a century of experimental studies, ecological roles of many of these microbes are unknown, partly because almost none can be cultivated. Many of the protists associate with bacterial symbionts, but hypotheses for their respective roles in nutrient exchange are based on genomes of only two such bacteria. To show how the ecological roles of protists and nutrient transfer with symbiotic bacteria can be elucidated by direct imaging, we combined stable isotope labeling (C-13-cellulose) of live termites with analysis of fixed hindgut microbes using correlated scanning electron microscopy, focused ion beam-scanning electron microscopy (FIB-SEM), transmission electron microscopy, and high resolution imaging mass spectrometry (NanoSIMS). We developed methods to prepare whole labeled cells on solid substrates, whole labeled cells milled with a FIB- SEM instrument to reveal cell interiors, and ultramicrotome sections of labeled cells for NanoSIMS imaging of C-13 enrichment in protists and associated bacteria. Our results show these methods have the potential to provide direct evidence for nutrient flow and suggest the oxymonad protist Oxymonas dimorpha phagocytoses and enzymatically degrades ingested wood fragments, and may transfer carbon derived from this to its surface bacterial symbionts. C1 [Carpenter, Kevin J.; Weber, Peter K.; Davisson, M. Lee; Pett-Ridge, Jennifer] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. [Haverty, Michael I.] Univ Calif Berkeley, Div Organisms & Environm Environm Sci Policy & Ma, Richmond, CA 94804 USA. [Keeling, Patrick J.] Univ British Columbia, Dept Bot, Canadian Inst Adv Res, Vancouver, BC V6T 1Z4, Canada. RP Carpenter, KJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM kjcarpenter@lbl.gov; weber21@llnl.gov FU Lawrence Livermore National Laboratory Laboratory Directed Research and Development program [011-LW-039]; Department of Energy OBER LLNL Biofuels Scientific Focus Area (SFA) program [SCW1039]; US Department of Energy [DE-AC52-07NA27344] FX This work was supported by the Lawrence Livermore National Laboratory Laboratory Directed Research and Development program (011-LW-039) and the Department of Energy OBER LLNL Biofuels Scientific Focus Area (SFA) program (SCW1039). Work at LLNL was performed under the auspices of the US Department of Energy under contract DE-AC52-07NA27344. The authors thank Ian Hutcheon for guidance, Christina Ramon and Nick Teslich of LLNL for technical assistance, and Sarah E. Baker (LLNL), Moriya Ohkuma (RIKEN Bioresource Center, Wako-Saitama, Japan), Andreas Brune (Max Planck Institute for Terrestrial Microbiology, Marburg, Germany), and Brian Leander (University of British Columbia) and Elaine Humphrey (University of Victoria, Canada) for helpful discussions and other assistance. NR 62 TC 11 Z9 11 U1 7 U2 68 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 1431-9276 EI 1435-8115 J9 MICROSC MICROANAL JI Microsc. microanal. PD DEC PY 2013 VL 19 IS 6 BP 1490 EP 1501 DI 10.1017/S1431927613013482 PG 12 WC Materials Science, Multidisciplinary; Microscopy SC Materials Science; Microscopy GA 298SN UT WOS:000330344800014 PM 24119340 ER PT J AU Xin, HLL Niu, KY Alsem, DH Zheng, HM AF Xin, Huolin L. Niu, Kaiyang Alsem, Daan Hein Zheng, Haimei TI In Situ TEM Study of Catalytic Nanoparticle Reactions in Atmospheric Pressure Gas Environment SO MICROSCOPY AND MICROANALYSIS LA English DT Article DE environmental cells; gas flow; in situ TEM; environmental TEM; nanoscale reactions; Kirkendall effects ID TRANSMISSION ELECTRON-MICROSCOPY; THIN-FILMS; INFORMATION LIMIT; RESOLUTION TEM; NANOCRYSTALS; TEMPERATURES; OXIDATION; CELL AB The understanding of solid-gas interactions has been greatly advanced over the past decade on account of the availability of high-resolution transmission electron microscopes (TEMs) equipped with differentially pumped environmental cells. The operational pressures in these differentially pumped environmental TEM (DP- ETEM) instruments are generally limited up to 20 mbar. Yet, many industrial catalytic reactions are operated at pressures equal or higher than 1 bar-50 times higher than that in the DP- ETEM. This poses limitations for in situ study of gas reactions through ETEM and advances are needed to extend in situ TEM study of gas reactions to the higher pressure range. Here, we present a first series of experiments using a gas flow membrane cell TEM holder that allows a pressure up to 4 bar. The built-in membrane heaters enable reactions at a temperature of 95-400 degrees C with flowing reactive gases. We demonstrate that, using a conventional thermionic TEM, 2 angstrom atomic fringes can be resolved with the presence of 1 bar O-2 gases in an environmental cell and we show real-time observation of the Kirkendall effect during oxidation of cobalt nanocatalysts. C1 [Xin, Huolin L.; Niu, Kaiyang; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Alsem, Daan Hein] Hummingbird Sci, Lacey, WA 98516 USA. RP Zheng, HM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM hmzheng@lbl.gov RI Xin, Huolin/E-2747-2010 OI Xin, Huolin/0000-0002-6521-868X FU U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; Bill Smith (Hummingbird Scientific) for development on the temperature measuring method and model; Helios SERC of LBNL; DOE Office of Science Early Career Research Program FX We performed the ex situ TEM experiments at the National Center for Electron Microscopy (NCEM) of the Lawrence Berkeley National Laboratory (LBNL), which is supported by the U.S. Department of Energy (DOE) under Contract # DE-AC02-05CH11231. In situ TEM experiments were done using LBNL Materials Sciences Division TEM facilities. We acknowledge support from Bill Smith (Hummingbird Scientific) for development on the temperature measuring method and model. H.L.X. thanks Dr. Sophie Carenco (Salmeron group) and Dr. Selim Alayoglu (Somorjai group) for supplying nanoparticle samples. H.L.X. was supported by Helios SERC of LBNL. H.Z. thanks the support of the DOE Office of Science Early Career Research Program. NR 36 TC 16 Z9 16 U1 10 U2 86 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 1431-9276 EI 1435-8115 J9 MICROSC MICROANAL JI Microsc. microanal. PD DEC PY 2013 VL 19 IS 6 BP 1558 EP 1568 DI 10.1017/S1431927613013433 PG 11 WC Materials Science, Multidisciplinary; Microscopy SC Materials Science; Microscopy GA 298SN UT WOS:000330344800021 PM 24011167 ER PT J AU Strachan, DC Ruffell, B Oei, Y Bissell, MJ Coussens, LM Pryer, N Daniel, D AF Strachan, Debbie C. Ruffell, Brian Oei, Yoko Bissell, Mina J. Coussens, Lisa M. Pryer, Nancy Daniel, Dylan TI CSF1R inhibition delays cervical and mammary tumor growth in murine models by attenuating the turnover of tumor-associated macrophages and enhancing infiltration by CD8(+) T cells SO ONCOIMMUNOLOGY LA English DT Article DE breast cancer; cervical cancer; CSF1R; M-CSF; tumor-associated macrophages; tumor immune evasion; tumor immunology; transgenic mouse models ID COLONY-STIMULATING FACTOR; BREAST-CANCER; SQUAMOUS CARCINOGENESIS; MONONUCLEAR PHAGOCYTES; TRANSGENIC MICE; PARACRINE LOOP; MYELOID CELLS; PROGRESSION; METASTASIS; MONOCYTES AB Increased numbers of tumor-infiltrating macrophages correlate with poor disease outcome in patients affected by several types of cancer, including breast and prostate carcinomas. The colony stimulating factor 1 receptor (CSF1R) signaling pathway drives the recruitment of tumor-associated macrophages (TAMs) to the neoplastic microenvironment and promotes the differentiation of TAMs toward a pro-tumorigenic phenotype. Twelve clinical trials are currently evaluating agents that target the CSF1/CSF1R signaling pathway as a treatment against multiple malignancies, including breast carcinoma, leukemia, and glioblastoma. The blockade of CSF1R signaling has been shown to greatly decrease the number of macrophages in a tissue-specific manner. However, additional mechanistic insights are needed in order to understand how macrophages are depleted and the global effects of CSF1R inhibition on other tumor-infiltrating immune cells. Using BLZ945, a highly selective small molecule inhibitor of CSF1R, we show that CSF1R inhibition attenuates the turnover rate of TAMs while increasing the number of CD8(+) T cells that infiltrate cervical and breast carcinomas. Specifically, we find that BLZ945 decreased the growth of malignant cells in the mouse mammary tumor virus-driven polyomavirus middle T antigen (MMTV-PyMT) model of mammary carcinogenesis. Furthermore, we show that BLZ945 prevents tumor progression in the keratin 14-expressing human papillomavirus type 16 (K14-HPV-16) transgenic model of cervical carcinogenesis. Our results demonstrate that TAMs undergo a constant turnover in a CSF1R-dependent manner, and suggest that continuous inhibition of the CSF1R pathway may be essential to maintain efficacious macrophage depletion as an anticancer therapy. C1 [Strachan, Debbie C.; Oei, Yoko; Pryer, Nancy; Daniel, Dylan] Novartis Inst Biomed Res, Emeryville, CA USA. [Ruffell, Brian; Coussens, Lisa M.] Oregon Hlth & Sci Univ, Dept Cell & Dev Biol, Portland, OR 97201 USA. [Ruffell, Brian; Coussens, Lisa M.] Oregon Hlth & Sci Univ, Knight Canc Inst, Portland, OR 97201 USA. [Bissell, Mina J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Daniel, D (reprint author), Novartis Inst Biomed Res, Emeryville, CA USA. EM dylan.daniel@novartis.com FU Department of Defense Breast Cancer Research Program (BCRP); NIH/NCI [R01 CA130980, R01CA140943, R01 CA155331, U54 CA163123]; Department of Defense BCRP Era of Hope Scholar Expansion Award [BC10412]; Susan G Komen Foundation [KG111084, KG110560]; Breast Cancer Research Foundation FX The authors would like to thank Cyrus Ghajar and Irene Kuhn for helpful discussions, Nicole Vanasse and Brenda Bartholomew for maintaining the transgenic mice, and Sok Chey, Ruben Flores and Jose Lapitan for their support with animal studies. The authors acknowledge support from the Department of Defense Breast Cancer Research Program (BCRP) to B. R., and grants from the NIH/NCI (R01 CA130980, R01CA140943, R01 CA155331, U54 CA163123), the Department of Defense BCRP Era of Hope Scholar Expansion Award (BC10412), the Susan G Komen Foundation (KG111084, KG110560), and the Breast Cancer Research Foundation to LMC. NR 44 TC 58 Z9 59 U1 2 U2 23 PU LANDES BIOSCIENCE PI AUSTIN PA 1806 RIO GRANDE ST, AUSTIN, TX 78702 USA SN 2162-4011 EI 2162-402X J9 ONCOIMMUNOLOGY JI OncoImmunology PD DEC PY 2013 VL 2 IS 12 AR UNSP e26968 DI 10.4161/onci.26968 PG 12 WC Oncology; Immunology SC Oncology; Immunology GA 299VZ UT WOS:000330425100002 PM 24498562 ER PT J AU Zhang, XB Gou, MY Liu, CJ AF Zhang, Xuebin Gou, Mingyue Liu, Chang-Jun TI Arabidopsis Kelch Repeat F-Box Proteins Regulate Phenylpropanoid Biosynthesis via Controlling the Turnover of Phenylalanine Ammonia-Lyase SO PLANT CELL LA English DT Article ID CELL-SUSPENSION CULTURES; LIGNIN BIOSYNTHESIS; FLAVONOID BIOSYNTHESIS; GENE FAMILY; FLUORESCENCE COMPLEMENTATION; SECONDARY METABOLISM; FUNCTIONAL-ANALYSIS; PLANT DEVELOPMENT; CIRCADIAN CLOCK; SWEET-POTATO AB Phenylalanine ammonia-lyase (PAL) catalyzes the first rate-limiting step in the phenylpropanoid pathway, which controls carbon flux to a variety of bioactive small-molecule aromatic compounds, and to lignin, the structural component of the cell wall. PAL is regulated at both the transcriptional and translational levels. Our knowledge about the transcriptional regulation of PAL is relatively comprehensive, but our knowledge of the molecular basis of the posttranslational regulation of PAL remains limited. Here, we demonstrate that the Arabidopsis thaliana Kelch repeat F-box (KFB) proteins KFB01, KFB20, and KFB50 physically interact with four PAL isozymes and mediate their proteolytic turnover via the ubiquitination-26S proteasome pathway. The KFB genes are differentially expressed in Arabidopsis tissues and respond to developmental and environmental cues. Up- or downregulation of their expression reciprocally affects the stability of the PAL enzymes, consequently altering the levels of phenylpropanoids. These data suggest that the KFB-mediated protein ubiquitination and degradation regulates the proteolysis of PALs, thus posttranslationally regulating phenylpropanoid metabolism. Characterizing the KFB-mediated proteolysis of PAL enzymes may inform future strategies for manipulating the synthesis of bioactive phenolics. C1 [Zhang, Xuebin; Gou, Mingyue; Liu, Chang-Jun] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. RP Liu, CJ (reprint author), Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. EM cliu@bnl.gov RI zhang, xuebin/K-3361-2015 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U. S. Department of Energy [DEAC0298CH10886 (BO-147), DEAC0298CH10886 (BO-157)]; Office of Basic Energy Sciences, U.S. Department of Energy [DEAC02-98CH10886] FX We thank Lise Jouanina (Institut Jean Pierre Bourgin, France) for sharing Lac4/17 double mutant seeds and John Shanklin (Brookhaven National Laboratory, USA) for discussing protein ubiquitylation with us. This work is supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U. S. Department of Energy through Grant DEAC0298CH10886 (BO-147 and 157) to C.-J.L. The use of the confocal microscope in the Center for Nanosciences was supported by the Office of Basic Energy Sciences, U.S. Department of Energy, under Contract DEAC02-98CH10886. NR 74 TC 31 Z9 31 U1 3 U2 43 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 1040-4651 EI 1532-298X J9 PLANT CELL JI Plant Cell PD DEC PY 2013 VL 25 IS 12 BP 4994 EP 5010 DI 10.1105/tpc.113.119644 PG 17 WC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology SC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology GA 302NM UT WOS:000330611200021 PM 24363316 ER PT J AU Lehoczky, JA Thomas, PE Patrie, KM Owens, KM Villarreal, LM Galbraith, K Washburn, J Johnson, CN Gavino, B Borowsky, AD Millen, KJ Wakenight, P Law, W Van Keuren, ML Gavrilina, G Hughes, ED Saunders, TL Brihn, L Nadeau, JH Innis, JW AF Lehoczky, Jessica A. Thomas, Peedikayil E. Patrie, Kevin M. Owens, Kailey M. Villarreal, Lisa M. Galbraith, Kenneth Washburn, Joe Johnson, Craig N. Gavino, Bryant Borowsky, Alexander D. Millen, Kathleen J. Wakenight, Paul Law, William Van Keuren, Margaret L. Gavrilina, Galina Hughes, Elizabeth D. Saunders, Thomas L. Brihn, Lesil Nadeau, Joseph H. Innis, Jeffrey W. TI A Novel Intergenic ETnII-beta Insertion Mutation Causes Multiple Malformations in Polypodia Mice SO PLOS GENETICS LA English DT Article ID LONG TERMINAL REPEAT; EMBRYONIC STEM-CELLS; TRANS-RETINOIC ACID; ALL-TRANS; DEVELOPMENTAL ANOMALIES; TRANSPOSABLE ELEMENTS; PHENOTYPIC VARIATION; PARTIAL DUPLICATION; PROTEIN-KINASE; C57BL/6 MICE AB Mouse early transposon insertions are responsible for similar to 10% of spontaneous mutant phenotypes. We previously reported the phenotypes and genetic mapping of Polypodia, (Ppd), a spontaneous, X-linked dominant mutation with profound effects on body plan morphogenesis. Our new data shows that mutant mice are not born in expected Mendelian ratios secondary to loss after E9.5. In addition, we refined the Ppd genetic interval and discovered a novel ETnII-beta early transposon insertion between the genes for Dusp9 and Pnck. The ETn inserted 1.6 kb downstream and antisense to Dusp9 and does not disrupt polyadenylation or splicing of either gene. Knock-in mice engineered to carry the ETn display Ppd characteristic ectopic caudal limb phenotypes, showing that the ETn insertion is the Ppd molecular lesion. Early transposons are actively expressed in the early blastocyst. To explore the consequences of the ETn on the genomic landscape at an early stage of development, we compared interval gene expression between wild-type and mutant ES cells. Mutant ES cell expression analysis revealed marked upregulation of Dusp9 mRNA and protein expression. Evaluation of the 5' LTR CpG methylation state in adult mice revealed no correlation with the occurrence or severity of Ppd phenotypes at birth. Thus, the broad range of phenotypes observed in this mutant is secondary to a novel intergenic ETn insertion whose effects include dysregulation of nearby interval gene expression at early stages of development. C1 [Lehoczky, Jessica A.; Thomas, Peedikayil E.; Patrie, Kevin M.; Galbraith, Kenneth; Law, William; Innis, Jeffrey W.] Univ Michigan, Dept Human Genet, Ann Arbor, MI 48109 USA. [Thomas, Peedikayil E.; Owens, Kailey M.; Villarreal, Lisa M.; Innis, Jeffrey W.] Univ Michigan, Ann Arbor, MI 48109 USA. [Washburn, Joe; Johnson, Craig N.] Univ Michigan, Biomed Res Core Facil, DNA Sequencing Core Lab, Ann Arbor, MI 48109 USA. [Gavino, Bryant] Univ Calif Davis, MMCL Mouse Biol Program, Murine Mol Constructs Lab, Davis, CA 95616 USA. [Borowsky, Alexander D.] Univ Calif Davis, Ctr Comparat Med, Davis, CA 95616 USA. [Borowsky, Alexander D.] Univ Calif Davis, Dept Pathol & Lab Med, Ctr Comprehens Canc, Davis, CA 95616 USA. [Millen, Kathleen J.; Wakenight, Paul] Seattle Childrens Hosp, Dept Pediat, Div Med Genet, Seattle, WA USA. [Van Keuren, Margaret L.; Gavrilina, Galina; Hughes, Elizabeth D.; Saunders, Thomas L.] Univ Michigan, Transgen Anim Model Core Lab, Ann Arbor, MI 48109 USA. [Brihn, Lesil] Case Western Reserve Univ, Dept Genet, Cleveland, OH 44106 USA. [Nadeau, Joseph H.] Pacific Northwest Res Inst, Seattle, WA USA. RP Lehoczky, JA (reprint author), Harvard Univ, Sch Med, Dept Genet, Boston, MA 02115 USA. EM innis@umich.edu FU NIH [HD053022, HD25389, HD053703]; University of Michigan Endowment for the Basic Sciences; Departments of Human Genetics and Pediatrics at the University of Michigan FX This work was funded in part by NIH HD053022 to JWI, NIH HD25389 to JHN, NIH HD053703 to KJM, the University of Michigan Endowment for the Basic Sciences, and the Departments of Human Genetics and Pediatrics at the University of Michigan. JWI would like to acknowledge support as the Morton S. and Henrietta K. Sellner Professor of Human Genetics. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 64 TC 0 Z9 0 U1 0 U2 4 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7404 J9 PLOS GENET JI PLoS Genet. PD DEC PY 2013 VL 9 IS 12 AR e1003967 DI 10.1371/journal.pgen.1003967 PG 14 WC Genetics & Heredity SC Genetics & Heredity GA 301LH UT WOS:000330533300015 PM 24339789 ER PT J AU Volz, EM Ionides, E Romero-Severson, EO Brandt, MG Mokotoff, E Koopman, JS AF Volz, Erik M. Ionides, Edward Romero-Severson, Ethan O. Brandt, Mary-Grace Mokotoff, Eve Koopman, James S. TI HIV-1 Transmission during Early Infection in Men Who Have Sex with Men: A Phylodynamic Analysis SO PLOS MEDICINE LA English DT Article ID UNITED-STATES; DRUG-RESISTANCE; SURVEILLANCE; NETHERLANDS; POPULATION; PREVALENCE; VIRUS; ADOLESCENTS; PREVENTION; COALESCENT AB Background: Conventional epidemiological surveillance of infectious diseases is focused on characterization of incident infections and estimation of the number of prevalent infections. Advances in methods for the analysis of the population-level genetic variation of viruses can potentially provide information about donors, not just recipients, of infection. Genetic sequences from many viruses are increasingly abundant, especially HIV, which is routinely sequenced for surveillance of drug resistance mutations. We conducted a phylodynamic analysis of HIV genetic sequence data and surveillance data from a US population of men who have sex with men (MSM) and estimated incidence and transmission rates by stage of infection. Methods and Findings: We analyzed 662 HIV-1 subtype B sequences collected between October 14, 2004, and February 24, 2012, from MSM in the Detroit metropolitan area, Michigan. These sequences were cross-referenced with a database of 30,200 patients diagnosed with HIV infection in the state of Michigan, which includes clinical information that is informative about the recency of infection at the time of diagnosis. These data were analyzed using recently developed population genetic methods that have enabled the estimation of transmission rates from the population-level genetic diversity of the virus. We found that genetic data are highly informative about HIV donors in ways that standard surveillance data are not. Genetic data are especially informative about the stage of infection of donors at the point of transmission. We estimate that 44.7% (95% CI, 42.2%-46.4%) of transmissions occur during the first year of infection. Conclusions: In this study, almost half of transmissions occurred within the first year of HIV infection in MSM. Our conclusions may be sensitive to un-modeled intra-host evolutionary dynamics, un-modeled sexual risk behavior, and uncertainty in the stage of infected hosts at the time of sampling. The intensity of transmission during early infection may have significance for public health interventions based on early treatment of newly diagnosed individuals. C1 [Volz, Erik M.] Univ London Imperial Coll Sci Technol & Med, Dept Infect Dis Epidemiol, London, England. [Ionides, Edward] Univ Michigan, Dept Stat, Ann Arbor, MI 48109 USA. [Romero-Severson, Ethan O.] Los Alamos Natl Lab, Los Alamos, NM USA. [Brandt, Mary-Grace; Mokotoff, Eve] Michigan Dept Community Hlth, Detroit, MI USA. [Koopman, James S.] Univ Michigan, Dept Epidemiol, Ann Arbor, MI 48109 USA. RP Volz, EM (reprint author), Univ London Imperial Coll Sci Technol & Med, Dept Infect Dis Epidemiol, London, England. EM e.volz@imperial.ac.uk OI Volz, Erik/0000-0001-6268-8937 FU NIH [K01-AI-091440-01, R01-AI078752, R01-AI087520] FX EMV was supported by NIH K01-AI-091440-01. This work was also supported by NIH R01-AI078752, and ERS had additional support from NIH R01-AI087520. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 52 TC 39 Z9 40 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1549-1676 J9 PLOS MED JI PLos Med. PD DEC PY 2013 VL 10 IS 12 AR UNSP e1001568 DI 10.1371/journal.pmed.1001568 PG 12 WC Medicine, General & Internal SC General & Internal Medicine GA 301LR UT WOS:000330534300007 PM 24339751 ER PT J AU Tomita, T Bzik, DJ Ma, YF Fox, BA Markillie, LM Taylor, RC Kim, K Weiss, LM AF Tomita, Tadakimi Bzik, David J. Ma, Yan Fen Fox, Barbara A. Markillie, Lye Meng Taylor, Ronald C. Kim, Kami Weiss, Louis M. TI The Toxoplasma gondii Cyst Wall Protein CST1 Is Critical for Cyst Wall Integrity and Promotes Bradyzoite Persistence SO PLOS PATHOGENS LA English DT Article ID CRYPTOSPORIDIUM-PARVUM; TISSUE CYST; IN-VIVO; SURFACE; HOST; IDENTIFICATION; GLYCOPROTEIN; SPOROZOITES; INFECTION; BIOLOGY AB Toxoplasma gondii infects up to one third of the world's population. A key to the success of T. gondii as a parasite is its ability to persist for the life of its host as bradyzoites within tissue cysts. The glycosylated cyst wall is the key structural feature that facilitates persistence and oral transmission of this parasite. Because most of the antibodies and reagents that recognize the cyst wall recognize carbohydrates, identification of the components of the cyst wall has been technically challenging. We have identified CST1 (TGME49_064660) as a 250 kDa SRS (SAG1 related sequence) domain protein with a large mucin-like domain. CST1 is responsible for the Dolichos biflorus Agglutinin (DBA) lectin binding characteristic of T. gondii cysts. Deletion of CST1 results in reduced cyst number and a fragile brain cyst phenotype characterized by a thinning and disruption of the underlying region of the cyst wall. These defects are reversed by complementation of CST1. Additional complementation experiments demonstrate that the CST1-mucin domain is necessary for the formation of a normal cyst wall structure, the ability of the cyst to resist mechanical stress, and binding of DBA to the cyst wall. RNA-seq transcriptome analysis demonstrated dysregulation of bradyzoite genes within the various cst1 mutants. These results indicate that CST1 functions as a key structural component that confers essential sturdiness to the T. gondii tissue cyst critical for persistence of bradyzoite forms. C1 [Tomita, Tadakimi; Ma, Yan Fen; Kim, Kami; Weiss, Louis M.] Albert Einstein Coll Med, Dept Pathol, Bronx, NY 10467 USA. [Bzik, David J.; Fox, Barbara A.] Geisel Sch Med Dartmouth, Dept Microbiol & Immunol, Lebanon, NH USA. [Markillie, Lye Meng; Taylor, Ronald C.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kim, Kami; Weiss, Louis M.] Albert Einstein Coll Med, Dept Med, Bronx, NY 10467 USA. [Kim, Kami] Albert Einstein Coll Med, Dept Microbiol & Immunol, Bronx, NY 10467 USA. RP Tomita, T (reprint author), Albert Einstein Coll Med, Dept Pathol, Bronx, NY 10467 USA. EM louis.weiss@einstein.yu.edu OI Taylor, Ronald/0000-0001-9777-9767; Kim, Kami/0000-0003-3384-152X FU NIH [AI39454, AI095094, AI087625, 5T32AI070117, NCI P30CA01333]; Environmental Molecular Sciences Laboratory Pacific Northwest National Laboratory [40070]; Center for AIDS Research at the Albert Einstein College of Medicine and Montefiore Medical Center; National Institutes of Health [NIH AI-051519] FX Research was supported by NIH grants AI39454 (LMW), AI095094 (LMW), AI087625 (KK), 5T32AI070117 (TT), NCI P30CA01333 and by grant 40070 (LMW) from Environmental Molecular Sciences Laboratory Pacific Northwest National Laboratory. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Lab. This work was also supported in part by the Center for AIDS Research at the Albert Einstein College of Medicine and Montefiore Medical Center funded by the National Institutes of Health (NIH AI-051519). The funders had no role in study design, data collection and 'nalysis, decision to publish, or preparation of the manuscript. NR 34 TC 18 Z9 18 U1 1 U2 11 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7374 J9 PLOS PATHOG JI PLoS Pathog. PD DEC PY 2013 VL 9 IS 12 AR e1003823 DI 10.1371/journal.ppat.1003823 PG 15 WC Microbiology; Parasitology; Virology SC Microbiology; Parasitology; Virology GA 301MC UT WOS:000330535400052 PM 24385904 ER PT J AU Zhu, JL Han, W Zhang, JZ Xu, HW Vogel, SC Jin, CQ Izumi, F Momma, K Kawamura, Y Zhao, YS AF Zhu, Jinlong Han, Wei Zhang, Jianzhong Xu, Hongwu Vogel, Sven C. Jin, Changqing Izumi, Fujio Momma, Koichi Kawamura, Yukihiko Zhao, Yusheng TI Nuclear and charge density distributions in ferroelectric PbTiO3: maximum entropy method analysis of neutron and X-ray diffraction data SO POWDER DIFFRACTION LA English DT Article DE ferroelectric materials; neutron diffraction; X-ray diffraction ID POWDER DIFFRACTION; 3-DIMENSIONAL VISUALIZATION; PROFILE REFINEMENT; CRYSTAL-STRUCTURE; DIFFRACTOMETER; DEUTEROHYDRATE; DIFFUSION; TITANATE; HIPPO; ORDER AB We conducted in-situ high-temperature neutron and X-ray diffraction studies on tetragonal PbTiO3. Using a combination of Rietveld analysis and Maximum Entropy Method, the nuclear and charge density distributions were determined as a function of temperature up to 460 degrees C. The ionic states obtained from charge density distributions reveal that the covalency of Pb-O-2 bonds gradually weakens with increasing temperature. The spontaneous polarizations calculated from the contributions of ionic state, ionic displacement, and nuclear polarization, are in good agreement with the experimental measurements. This method provides an effective approach to determine spontaneous polarizations in multiferroics with high-current leakage and low resistance. (C) 2013 International Centre for Diffraction Data. C1 [Zhu, Jinlong; Zhang, Jianzhong; Xu, Hongwu; Vogel, Sven C.; Zhao, Yusheng] Los Alamos Natl Lab, LANSCE, Los Alamos, NM 87545 USA. [Zhu, Jinlong; Zhang, Jianzhong; Xu, Hongwu; Vogel, Sven C.; Zhao, Yusheng] Los Alamos Natl Lab, EES Div, Los Alamos, NM 87545 USA. [Zhu, Jinlong; Han, Wei; Jin, Changqing; Zhao, Yusheng] Chinese Acad Sci, Inst Phys, Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Izumi, Fujio; Momma, Koichi; Kawamura, Yukihiko] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan. [Zhao, Yusheng] Univ Nevada, Dept Phys & Astron, HiPSEC, Las Vegas, NV 89154 USA. RP Jin, CQ (reprint author), Chinese Acad Sci, Inst Phys, Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. EM jin@iphy.ac.cn; Yusheng.Zhao@unlv.edu RI Momma, Koichi/F-1090-2016; OI Xu, Hongwu/0000-0002-0793-6923; Zhang, Jianzhong/0000-0001-5508-1782 FU laboratory-directed research and development (LDRD) program of Los Alamos National Laboratory [DE-AC52-06NA25396]; US Department of Energy's Office of Basic Energy Sciences; NSF; MOST FX This work was supported by the laboratory-directed research and development (LDRD) program of Los Alamos National Laboratory, which is operated by Los Alamos National Security LLC under DOE contract no. DE-AC52-06NA25396. The experimental work has benefited from the use of the Lujan Neutron Scattering Center at Los Alamos Neutron Science Center, which is funded by the US Department of Energy's Office of Basic Energy Sciences. The work at IOPCAS was supported by NSF & MOST through the research projects. NR 23 TC 0 Z9 0 U1 3 U2 15 PU J C P D S-INT CENTRE DIFFRACTION DATA PI NEWTOWN SQ PA 12 CAMPUS BLVD, NEWTOWN SQ, PA 19073-3273 USA SN 0885-7156 EI 1945-7413 J9 POWDER DIFFR JI Powder Diffr. PD DEC PY 2013 VL 28 IS 4 BP 276 EP 280 DI 10.1017/S0885715613000675 PG 5 WC Materials Science, Characterization & Testing SC Materials Science GA 296YN UT WOS:000330221400007 ER PT J AU Toby, BH AF Toby, Brian H. TI The 2013 American Crystallographic Association Meeting SO POWDER DIFFRACTION LA English DT Article C1 Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Toby, BH (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RI Toby, Brian/F-3176-2013 OI Toby, Brian/0000-0001-8793-8285 NR 0 TC 0 Z9 0 U1 0 U2 1 PU J C P D S-INT CENTRE DIFFRACTION DATA PI NEWTOWN SQ PA 12 CAMPUS BLVD, NEWTOWN SQ, PA 19073-3273 USA SN 0885-7156 EI 1945-7413 J9 POWDER DIFFR JI Powder Diffr. PD DEC PY 2013 VL 28 IS 4 BP 325 EP 325 DI 10.1017/S0885715613001309 PG 1 WC Materials Science, Characterization & Testing SC Materials Science GA 296YN UT WOS:000330221400019 ER PT J AU Wang, HY Liu, F Bu, LJ Gao, J Wang, C Wei, W Russell, TP AF Wang, Hongyu Liu, Feng Bu, Laju Gao, Jun Wang, Cheng Wei, Wei Russell, Thomas P. TI The Role of Additive in Diketopyrrolopyrrole-Based Small Molecular Bulk Heterojunction Solar Cells SO ADVANCED MATERIALS LA English DT Article DE organic photovoltaics; morphology; crystallization; X-ray diffraction ID ORGANIC PHOTOVOLTAIC CELLS; PROCESSED SMALL-MOLECULE; BAND-GAP; BENZODITHIOPHENE UNIT; EFFICIENCY; POLYMER; PERFORMANCE; MORPHOLOGY; POLY(3-HEXYLTHIOPHENE); BLENDS C1 [Wang, Hongyu; Gao, Jun] Shanghai Univ, Dept Chem, Shanghai 200444, Peoples R China. [Liu, Feng; Bu, Laju; Russell, Thomas P.] Univ Massachusetts, Polymer Sci & Engn Dept, Amherst, MA USA. [Wei, Wei] Nanjing Univ Posts & Telecommun, Inst Adv Mat, Nanjing 210046, Jiangsu, Peoples R China. [Wang, Cheng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Wang, HY (reprint author), Shanghai Univ, Dept Chem, Shanghai 200444, Peoples R China. EM wanghy@shu.edu.cn; fliu0@polysci.umass.edu; tom.p.russell@gmail.com RI Wang, Cheng/A-9815-2014; Bu, Laju/D-4362-2015; Liu, Feng/J-4361-2014 OI Bu, Laju/0000-0002-7908-9874; Liu, Feng/0000-0002-5572-8512 FU National Natural Science Foundation of China [61204020, 61274054]; Department of Energy [DE-SC0001087]; DOE, Office of Science, and Office of Basic Energy Sciences FX H. Wang and F. Liu contributed equally to this work. This work was financially supported by the National Natural Science Foundation of China (Grant Nos. 61204020, 61274054) and Department of Energy supported Energy Frontier Research Center at the University of Massachusetts (DOE DE-SC0001087). Portions of this research were carried out at the Advanced Light Source, Berkeley National Laboratory, which was supported by the DOE, Office of Science, and Office of Basic Energy Sciences. The authors also thank Dr. H. M. Deng for assistance with NMR measurements at the NMR facility in the Instrumental Analysis and Research Center at Shanghai University. NR 37 TC 38 Z9 38 U1 4 U2 101 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD DEC PY 2013 VL 25 IS 45 BP 6519 EP 6525 DI 10.1002/adma.201302848 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 295HI UT WOS:000330106800003 PM 23996829 ER PT J AU Druzinsky, RE Mungall, C Haendel, M Lapp, H Mabee, P AF Druzinsky, Robert E. Mungall, Christopher Haendel, Melissa Lapp, Hilmar Mabee, Paula TI What is an Anatomy Ontology? SO ANATOMICAL RECORD-ADVANCES IN INTEGRATIVE ANATOMY AND EVOLUTIONARY BIOLOGY LA English DT Letter ID EVOLUTION; INFORMATICS; GENOMICS; BIOLOGY C1 [Druzinsky, Robert E.] Univ Illinois, Coll Med, Dept Oral Biol, Chicago, IL 60612 USA. [Mungall, Christopher] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. [Haendel, Melissa] Oregon Hlth & Sci Univ, Dept Med Informat & Epidemiol, Portland, OR 97201 USA. [Lapp, Hilmar] Natl Evolutionary Synth Ctr NESCent, Durham, NC USA. [Mabee, Paula] Univ S Dakota, Dept Biol, Vermillion, SD 57069 USA. RP Druzinsky, RE (reprint author), Univ Illinois, Coll Med, Dept Oral Biol, M-C 690, Chicago, IL 60612 USA. EM druzinsk@uic.edu OI Mabee, Paula/0000-0002-8455-3213; Druzinsky, Robert/0000-0002-1572-1316; Lapp, Hilmar/0000-0001-9107-0714 FU NIH HHS [R24 OD011883] NR 16 TC 0 Z9 0 U1 0 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1932-8486 EI 1932-8494 J9 ANAT REC JI Anat. Rec. PD DEC PY 2013 VL 296 IS 12 BP 1797 EP 1799 DI 10.1002/ar.22805 PG 3 WC Anatomy & Morphology SC Anatomy & Morphology GA 295RR UT WOS:000330133700001 PM 24127438 ER PT J AU Han, J Elgowainy, A Cai, H Wang, MQ AF Han, Jeongwoo Elgowainy, Amgad Cai, Hao Wang, Michael Q. TI Life-cycle analysis of bio-based aviation fuels SO BIORESOURCE TECHNOLOGY LA English DT Article DE Greenhouse gas emissions; Life-cycle analysis; Bio-based aviation fuels; Well-to-wake analysis ID GREENHOUSE-GAS EMISSIONS; LAND-USE CHANGE; JET FUEL; BIOFUELS; DIESEL AB Well-to-wake (WTWa) analysis of bio-based aviation fuels, including hydroprocessed renewable jet (HRJ) from various oil seeds, Fischer-Tropsch jet (FTJ) from corn-stover and co-feeding of coal and corn-stover, and pyrolysis jet from corn stover, is conducted and compared with petroleum jet. WTWa GHG emission reductions relative to petroleum jet can be 41-63% for HRJ, 68-76% for pyrolysis jet and 89% for FTJ from corn stover. The HRJ production stage dominates WTWa GHG emissions from HRJ pathways. The differences in GHG emissions from HRJ production stage among considered feedstocks are much smaller than those from fertilizer use and N2O emissions related to feedstock collection stage. Sensitivity analyses on FTJ production from coal and corn-stover are also conducted, showing the importance of biomass share in the feedstock, carbon capture and sequestration options, and overall efficiency. For both HRJ and FTJ, co-product handling methods have significant impacts on WTWa results. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Han, Jeongwoo; Elgowainy, Amgad; Cai, Hao; Wang, Michael Q.] Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, Argonne, IL 60439 USA. RP Han, J (reprint author), Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jhan@anl.gov; aelgowainy@anl.gov; hcai@anl.gov; mqwang@anl.gov RI Cai, Hao/A-1975-2016 FU Biomass Energy Technology Office in the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357] FX This study was supported by the Biomass Energy Technology Office in the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy, under Contract DE-AC02-06CH11357. The authors would like to thank Zia Haq, Kristen Johnson, and Alicia Lindauer of that office for their support of this study. The authors are also grateful to James Hileman of Federal Aviation Administration, Matthew Pearlson of Massachusetts Institute of Technology, and David Shonnard and Jiqing Fan of Michigan Technological University for their inputs on HRJ production processes to this WTWa analysis. NR 35 TC 19 Z9 19 U1 3 U2 46 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD DEC PY 2013 VL 150 BP 447 EP 456 DI 10.1016/j.biortech.2013.07.153 PG 10 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA 292HG UT WOS:000329892200058 PM 23978607 ER PT J AU Wu, D Aliprantis, DC AF Wu, Di Aliprantis, Dionysios C. TI Modeling light-duty plug-in electric vehicles for national energy and transportation planning SO ENERGY POLICY LA English DT Article DE Energy planning; Infrastructure; Plug-in electric vehicles ID INTEGRATED ENERGY; DEMAND; IMPACT; DISPATCH; POWER AB This paper sets forth a family of models of light-duty plug-in electric vehicle (PEV) fleets, appropriate for conducting long-term national-level planning studies of the energy and transportation sectors in an integrated manner. Using one of the proposed models, three case studies on the evolution of the U.S. energy and transportation infrastructures are performed, where portfolios of optimum investments over a 40-year horizon are identified, and interdependencies between the two sectors are highlighted. The results indicate that with a gradual but aggressive introduction of PEVs coupled with investments in renewable energy, the total cost from the energy and transportation systems can be reduced by 5%, and that overall emissions from electricity generation and light-duty vehicle (LDV) tailpipes can be reduced by 10% over the 40-year horizon. The annual gasoline consumption from LDVs can be reduced by 66% by the end of the planning horizon, but an additional 800 TWh of annual electricity demand will be introduced. In addition, various scenarios of greenhouse gas (GHG) emissions reductions are investigated. It is found that GHG emissions can be significantly reduced with only a marginal cost increment, by shifting electricity generation from coal to renewable sources. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Wu, Di] Pacific NW Natl Lab, Richland, WA 99352 USA. [Aliprantis, Dionysios C.] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. RP Aliprantis, DC (reprint author), Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. EM di.wu@pnnl.gov; dionysis@purdue.edu OI Wu, Di/0000-0001-6955-4333 FU National Science Foundation [0835989] FX This material is based upon work supported by the National Science Foundation under Grant no. 0835989. NR 75 TC 6 Z9 6 U1 0 U2 20 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD DEC PY 2013 VL 63 BP 419 EP 432 DI 10.1016/j.enpol.2013.07.132 PG 14 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA 294ZC UT WOS:000330085400044 ER PT J AU Dong, CG Wiser, R AF Dong, Changgui Wiser, Ryan TI The impact of city-level permitting processes on residential photovoltaic installation prices and development times: An empirical analysis of solar systems in California cities SO ENERGY POLICY LA English DT Article DE Photovoltaic; Permitting; Installed prices ID LEARNING-CURVE; COST; TECHNOLOGIES; POWER; ELECTRICITY; PROSPECTS; POLICY; MODEL; PV AB With "soft" costs accounting for well over 50% of the installed price of residential photovoltaic (PV) systems in the United States, this study evaluates the effect of city-level permitting processes on the installed price of residential PV systems and on the time required to develop those systems. The study uses a unique dataset from the U.S. Department of Energy's Rooftop Solar Challenge Program, which includes city-level permitting process "scores," plus data from the California Solar Initiative and the U.S. Census. Econometric methods are used to quantify the price and development-time effects of city-level permitting processes on more than 3000 PV installations across 44 California cities in 2011. Results suggest that cities with the most favorable permitting practices can reduce average residential PV prices by $0.27-$0.77/W (4-12% of median PV prices in California) compared with cities with the most onerous permitting practices, depending on the regression model used. Though the empirical models for development times are less robust, results suggest that the most streamlined permitting practices may shorten development times by around 24 days on average (25% of the median development time). These findings illustrate the potential price and development-time benefits of streamlining local permitting procedures for PV systems. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Dong, Changgui; Wiser, Ryan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Elect Markets & Policy Grp, Berkeley, CA 94720 USA. [Dong, Changgui] Univ Texas Austin, LBJ Sch Publ Affairs, Austin, TX 78713 USA. RP Wiser, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Elect Markets & Policy Grp, Berkeley, CA 94720 USA. EM rhwiser@lbl.gov FU Office of Energy Efficiency and Renewable Energy (Solar Energy Technologies Office) of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX The work described in this paper was funded by the Office of Energy Efficiency and Renewable Energy (Solar Energy Technologies Office) of the U.S. Department of Energy (DOE) under Contract no. DE-AC02-05CH11231. For reviewing earlier versions of this work or providing valuable input, we would particularly like to thank Galen Barbose (LBNL), Adam Cohen (DOE), Naim Darghouth (LBNL), Carolyn Davidson (NREL), Kenneth Gillingham (Yale University), Joshua Huneycutt (DOE), Mike Kheyfets (Edgeworth Economics), Gregory Nemet (University of Wisconsin-Madison), Kurt Newick (Sierra Club), Varun Rai (University of Texas, Austin), Gwen Rose (VoteSolar), Joachim Seel (LBNL), and James Tong (Clean Power Finance). We appreciate the substantial editing assistance of Jarett Zuboy (consultant). For their support of this work, we also thank Minh Le, Joshua Huneycutt, Elaine Ulrich, Kelly Knudsen, Christina Nichols, and Adam Cohen (DOE). Of course, the authors are solely responsible for any omissions or errors contained herein. NR 38 TC 10 Z9 10 U1 3 U2 13 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD DEC PY 2013 VL 63 BP 531 EP 542 DI 10.1016/j.enpol.2013.08.054 PG 12 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA 294ZC UT WOS:000330085400055 ER PT J AU Hasanbeigi, A Price, L Fino-Chen, C Lu, HY Ke, J AF Hasanbeigi, Ali Price, Lynn Fino-Chen, Cecilia Lu, Hongyou Ke, Jing TI Retrospective and prospective decomposition analysis of Chinese manufacturing energy use and policy implications SO ENERGY POLICY LA English DT Article DE Energy intensity; Decomposition analysis; Chinese manufacturing ID INTENSITY; INDICATORS; EMISSIONS; INDUSTRY AB Aims: The industrial sector dominates the China's total energy consumption, accounting for about 70% of energy use in 2010. Hence, this study aims to investigate the development path of China's industrial sector which will greatly affect future energy demand and dynamics of not only China, but the entire world. Scope: This study analyzes energy use and the economic structure of the Chinese manufacturing sector. The retrospective (1995-2010) and prospective (2010-2020) decomposition analyses are conducted for manufacturing sectors in order to show how different factors (production growth, structural change, and energy intensity change) influenced industrial energy use trends in China over the last 15 years and how they will do so up to 2020. Conclusions: The forward looking (prospective) decomposition analyses are conducted for three different scenarios. The scenario analysis indicates that if China wants to realize structural change in the manufacturing sector by shifting from energy-intensive and polluting industries to less energy-intensive industries, the value added average annual growth rates (AAGRs) to 2015 and 2020 should be more in line with those shown in scenario 3. The assumed value added AAGRs for scenario 3 are relatively realistic and are informed by possible growth that is foreseen for each subsector. Published by Elsevier Ltd. C1 [Hasanbeigi, Ali; Price, Lynn; Fino-Chen, Cecilia; Lu, Hongyou; Ke, Jing] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, China Energy Grp, Berkeley, CA USA. RP Hasanbeigi, A (reprint author), 1 Cyclotron Rd MS 90R2002, Berkeley, CA 94720 USA. EM AHasanbeigi@lbl.gov RI Ke, Jing/H-4816-2016 OI Ke, Jing/0000-0002-5972-8042 FU China Sustainable Energy Program of the Energy Foundation through the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the China Sustainable Energy Program of the Energy Foundation through the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. We would like to thank Bob Taylor of Energy Pathways for his significant contribution to this study. We are also thankful to Lingbo Kong from State Key Laboratory of Pulp and Paper Engineering, South China University of Technology and Yue Dai from the University of Texas at Austin for their research assistance for this study. We are grateful to Bai Quan of the Energy Research Institute (ERI) of China's National Development and Reform Commission for his valuable comments on the earlier version of the paper. NR 42 TC 15 Z9 15 U1 0 U2 5 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD DEC PY 2013 VL 63 BP 562 EP 574 DI 10.1016/j.enpol.2013.08.067 PG 13 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA 294ZC UT WOS:000330085400058 ER PT J AU Khanna, NZ Zhou, N Fridley, D Fino-Chen, C AF Khanna, Nina Zheng Zhou, Nan Fridley, David Fino-Chen, Cecilia TI Evaluation of China's local enforcement of energy efficiency standards and labeling programs for appliances and equipment SO ENERGY POLICY LA English DT Article DE Appliance standards and labeling; Energy efficiency; Compliance AB Aims: This paper aims to evaluate local enforcement of China's mandatory appliance and equipment energy efficiency standards and labeling programs, two increasingly important policies for meeting national energy and carbon reduction targets. The expected energy savings of efficiency standards and labels can be fully realized only with strong enforcement to ensure compliance for all products sold. This paper provides comprehensive retrospective evaluation of the methodologies, results, progress and remaining challenges in pilot enforcement projects initiated in the absence of consistent national check-testing focused on energy efficiency. Scope: This paper's scope is focused on 2006-2009 pilot local check-tests conducted to verify appliance and equipment compliance with China's mandatory energy label and efficiency standards. Conclusions: This paper finds both improvement and some backsliding in compliance rates over time. Compared to earlier efforts, 2009 check-tests covered a wider regional and product scope but demonstrated greater variation in compliance rates. Labeling display and energy efficiency compliance was generally high across regions and most products, but lower compliance rates were observed in less economically developed regions and for lighting and industrial products. Based on these findings, areas for improvement in local awareness, product sampling methodology, check-testing tools and procedures are identified. Published by Elsevier Ltd. C1 [Khanna, Nina Zheng; Zhou, Nan; Fridley, David; Fino-Chen, Cecilia] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, Berkeley, CA 94720 USA. RP Khanna, NZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, 1 Cyclotron Rd,MS 90R4000, Berkeley, CA 94720 USA. EM XZheng@lbl.gov FU China Sustainable Energy Program of the Energy Foundation; Collaborative Labeling and Appliance Standards Program through the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the China Sustainable Energy Program of the Energy Foundation and the Collaborative Labeling and Appliance Standards Program through the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors are also grateful to the China National Institute of Standardization and the anonymous reviewers for their feedback and input to this work. NR 20 TC 2 Z9 2 U1 3 U2 8 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD DEC PY 2013 VL 63 BP 646 EP 655 DI 10.1016/j.enpol.2013.09.035 PG 10 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA 294ZC UT WOS:000330085400067 ER PT J AU Teeguarden, JG Hanson-Drury, S AF Teeguarden, Justin G. Hanson-Drury, Sesha TI A systematic review of Bisphenol A "low dose" studies in the context of human exposure: A case for establishing standards for reporting "low-dose" effects of chemicals SO FOOD AND CHEMICAL TOXICOLOGY LA English DT Review DE Bisphenol A; Exposure; Risk; Low-dose ID ESTROGEN-RECEPTOR-ALPHA; ENVIRONMENTALLY RELEVANT CONCENTRATIONS; SPRAGUE-DAWLEY RATS; IN-UTERO EXPOSURE; SPERMATOGONIAL CELL-PROLIFERATION; ENDOCRINE-DISRUPTING CHEMICALS; TROUT ONCORHYNCHUS-MYKISS; TANDEM MASS-SPECTROMETRY; FETAL MOUSE PROSTATE; ADULT CD-1 MICE AB Human exposure to the chemical Bisphenol A is almost ubiquitous in surveyed industrialized societies. Structural features similar to estrogen confer the ability of Bisphenol A (BPA) to bind estrogen receptors, giving BPA membership in the group of environmental pollutants called endocrine disruptors. References by scientists, the media, political entities, and non-governmental organizations to many toxicity studies as "low dose" has led to the belief that exposure levels in these studies are similar to humans, implying that BPA is toxic to humans at current exposures. Through systematic, objective comparison of our current, and a previous compilation of the "low-dose" literature to multiple estimates of human external and internal exposure levels, we found that the "low-dose" moniker describes exposures covering 8-12 orders of magnitude, the majority (91-99% of exposures) being greater than the upper bound of human exposure in the general infant, child and adult U.S. Population. "low dose" is therefore a descriptor without specific meaning regarding human exposure. Where human exposure data are available, for BPA and other environmental chemicals, reference to toxicity study exposures by direct comparison to human exposure would be more informative, more objective, and less susceptible to misunderstanding. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Teeguarden, Justin G.; Hanson-Drury, Sesha] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Teeguarden, JG (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM jt@pnl.gov; Sesha.Hanson-Drury@pnl.gov OI Teeguarden, Justin/0000-0003-3817-4391 FU U.S. EPA [R83386701] FX The authors would like to thank the U.S. EPA for providing funding for this work under the STAR program, grant R83386701. The authors would also like to acknowledge Dan Amundson, George Mason University Center for Media and Policy Analysis, for providing copies CMPA's media analysis of the BPA low dose issue and Cortland Johnson, Pacific Northwest National Laboratory for help with graphics. NR 271 TC 37 Z9 37 U1 3 U2 61 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0278-6915 EI 1873-6351 J9 FOOD CHEM TOXICOL JI Food Chem. Toxicol. PD DEC PY 2013 VL 62 BP 935 EP 948 DI 10.1016/j.fct.2013.07.007 PG 14 WC Food Science & Technology; Toxicology SC Food Science & Technology; Toxicology GA 293GW UT WOS:000329960400117 PM 23867546 ER PT J AU Novikova, IV Hennelly, SP Sanbonmatsu, KY AF Novikova, Irina V. Hennelly, Scott P. Sanbonmatsu, Karissa Y. TI Tackling Structures of Long Noncoding RNAs SO INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES LA English DT Review DE long noncoding RNAs; lncRNAs; secondary structure; chemical probing; SHAPE; epigenetics ID SECONDARY STRUCTURE PREDICTION; GENOME-WIDE MEASUREMENT; SAM-I RIBOSWITCH; RIBOSOMAL-RNA; ANGSTROM RESOLUTION; GENE-EXPRESSION; TERTIARY STRUCTURE; SHAPE CHEMISTRY; STRUCTURE MODEL; SERVER AB RNAs are important catalytic machines and regulators at every level of gene expression. A new class of RNAs has emerged called long non-coding RNAs, providing new insights into evolution, development and disease. Long non-coding RNAs (lncRNAs) predominantly found in higher eukaryotes, have been implicated in the regulation of transcription factors, chromatin-remodeling, hormone receptors and many other processes. The structural versatility of RNA allows it to perform various functions, ranging from precise protein recognition to catalysis and metabolite sensing. While major housekeeping RNA molecules have long been the focus of structural studies, lncRNAs remain the least characterized class, both structurally and functionally. Here, we review common methodologies used to tackle RNA structure, emphasizing their potential application to lncRNAs. When considering the complexity of lncRNAs and lack of knowledge of their structure, chemical probing appears to be an indispensable tool, with few restrictions in terms of size, quantity and heterogeneity of the RNA molecule. Probing is not constrained to in vitro analysis and can be adapted to high-throughput sequencing platforms. Significant efforts have been applied to develop new in vivo chemical probing reagents, new library construction protocols for sequencing platforms and improved RNA prediction software based on the experimental evidence. C1 [Novikova, Irina V.; Hennelly, Scott P.; Sanbonmatsu, Karissa Y.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Sanbonmatsu, KY (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM ivn@lanl.gov; sph@lanl.gov; kys@lanl.gov FU US Department of Energy via LANL LDRD FX The work was performed under the auspices of the US Department of Energy via LANL LDRD. NR 86 TC 14 Z9 14 U1 4 U2 45 PU MDPI AG PI BASEL PA ST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND SN 1422-0067 J9 INT J MOL SCI JI Int. J. Mol. Sci. PD DEC PY 2013 VL 14 IS 12 BP 23672 EP 23684 DI 10.3390/ijms141223672 PG 13 WC Biochemistry & Molecular Biology; Chemistry, Multidisciplinary SC Biochemistry & Molecular Biology; Chemistry GA 296XX UT WOS:000330219800032 PM 24304541 ER PT J AU Wirth, M Villeneuve, S Haase, CM Madison, CM Oh, H Landau, SM Rabinovici, GD Jagust, WJ AF Wirth, Miranka Villeneuve, Sylvia Haase, Claudia M. Madison, Cindee M. Oh, Hwamee Landau, Susan M. Rabinovici, Gil D. Jagust, William J. TI Associations Between Alzheimer Disease Biomarkers, Neurodegeneration, and Cognition in Cognitively Normal Older People SO JAMA NEUROLOGY LA English DT Article ID HUMAN CEREBRAL-CORTEX; WHITE-MATTER LESIONS; AMYLOID DEPOSITION; EPISODIC MEMORY; MRI; BRAIN; DEMENTIA; DECLINE; PET AB IMPORTANCE Criteria for preclinical Alzheimer disease (AD) propose beta-amyloid (A beta) plaques to initiate neurodegeneration within AD-affected regions. However, some cognitively normal older individuals harbor neural injury similar to patients with AD, without concurrent A beta burden. Such findings challenge the proposed sequence and suggest that A beta-independent precursors underlie AD-typical neurodegenerative patterns. OBJECTIVE To examine relationships between A beta and non-A beta factors as well as neurodegeneration within AD regions in cognitively normal older adults. The study quantified neurodegenerative abnormalities using imaging biomarkers and examined cross-sectional relationships with A beta deposition; white matter lesions (WMLs), a marker of cerebrovascular disease; and cognitive functions. DESIGN, SETTING, AND PARTICIPANTS Cross-sectional study in a community-based convenience sample of 72 cognitively normal older individuals (mean [SD] age, 74.9 [5.7] years; 48 women; mean [SD] 17.0 [1.9] years of education) of the Berkeley Aging Cohort. INTERVENTION Each individual underwent a standardized neuropsychological test session, magnetic resonance imaging, and positron emission tomography scanning. MAIN OUTCOMES AND MEASURES For each individual, 3 AD-sensitive neurodegeneration biomarkers were measured: hippocampal volume, glucose metabolism, and gray matter thickness, the latter 2 sampled from cortical AD-affected regions. To quantify neurodegenerative abnormalities, each biomarker was age adjusted, dichotomized into a normal or abnormal status (using cutoff thresholds derived from an independent AD sample), and summarized into 0, 1, or more than 1 abnormal neurodegenerative biomarker. Degree and topographic patterns of neurodegenerative abnormalities were assessed and their relationships with cognitive functions, WML volume, and A beta deposition (quantified using carbon 11-labeled Pittsburgh compound B positron emission tomography). RESULTS Of our cognitively normal elderly individuals, 40% (n = 29) displayed at least 1 abnormal neurodegenerative biomarker, 26%(n = 19) of whom had no evidence of elevated Pittsburgh compound B retention. In those people who were classified as having abnormal cortical thickness, degree and topographic specificity of neurodegenerative abnormalities were similar to patients with AD. Accumulation of neurodegenerative abnormalities was related to poor memory and executive functions as well as larger WML volumes but not elevated Pittsburgh compound B retention. CONCLUSIONS AND RELEVANCE Our study confirms that a substantial proportion of cognitively normal older adults harbor neurodegeneration, without A beta burden. Associations of neurodegenerative abnormalities with cerebrovascular disease and cognitive performance indicate that neurodegenerative pathology can emerge through non-A beta pathways within regions most affected by AD. C1 [Wirth, Miranka; Villeneuve, Sylvia; Madison, Cindee M.; Oh, Hwamee; Landau, Susan M.; Rabinovici, Gil D.; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Haase, Claudia M.] Univ Calif Berkeley, Inst Personal & Social Res, Berkeley, CA 94720 USA. [Oh, Hwamee; Landau, Susan M.; Rabinovici, Gil D.; Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Rabinovici, Gil D.] Univ Calif San Francisco, Dept Neurol, Memory & Aging Ctr, San Francisco, CA 94143 USA. RP Wirth, M (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, 132 Barker Hall,Ste 3190, Berkeley, CA 94720 USA. EM miranka.wirth@gmail.com FU National Institutes of Health [P30-AG010129, K01-AG030514, AG034570, K23-AG031861, P01-AG1972403, P50-AG023501]; Alzheimer's Association [NIRG-07-59422]; John Douglas French Alzheimer's Foundation; State of California Department of Health Services Alzheimer's Disease Research Center of California [04-33516]; Swiss National Science Foundation [PA00P1-131515] FX This research was also supported by National Institutes of Health grants P30-AG010129, K01-AG030514, AG034570, K23-AG031861, P01-AG1972403, and P50-AG023501, Alzheimer's Association grant NIRG-07-59422, the John Douglas French Alzheimer's Foundation, State of California Department of Health Services Alzheimer's Disease Research Center of California grant 04-33516, and Swiss National Science Foundation grant PA00P1-131515. NR 34 TC 56 Z9 57 U1 3 U2 12 PU AMER MEDICAL ASSOC PI CHICAGO PA 515 N STATE ST, CHICAGO, IL 60654-0946 USA SN 2168-6149 EI 2168-6157 J9 JAMA NEUROL JI JAMA Neurol. PD DEC PY 2013 VL 70 IS 12 BP 1512 EP 1519 DI 10.1001/jamaneurol.2013.4013 PG 8 WC Clinical Neurology SC Neurosciences & Neurology GA 295LS UT WOS:000330118200008 PM 24166579 ER PT J AU Malikopoulos, AA AF Malikopoulos, Andreas A. TI Impact of Component Sizing in Plug-In Hybrid Electric Vehicles for Energy Resource and Greenhouse Emissions Reduction SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article DE optimization methods; transportation; vehicles; emissions; energy storage ID LIFE-CYCLE ASSESSMENT; POWER MANAGEMENT; PROPULSION SYSTEM; OPTIMIZATION; DESIGN; POWERTRAINS; TRUCK AB Widespread use of alternative hybrid powertrains currently appears inevitable and many opportunities for substantial progress remain. The necessity for environmentally friendly vehicles, in conjunction with increasing concerns regarding U. S. dependency on foreign oil and climate change, has led to significant investment in enhancing the propulsion portfolio with new technologies. Recently, plug-in hybrid electric vehicles (PHEVs) have attracted considerable attention due to their potential to reduce petroleum consumption and greenhouse gas (GHG) emissions in the transportation sector. PHEVs are especially appealing for short daily commutes with excessive stop-and-go driving. However, the high costs associated with their components, and in particular, with their energy storage systems have been significant barriers to extensive market penetration of PHEVs. In the research reported here, we investigated the implications of motor/generator and battery size on fuel economy and GHG emissions in a medium duty PHEV. An optimization framework is proposed and applied to two different parallel powertrain configurations, pretransmission and post transmission, to derive the Pareto frontier with respect to motor/generator and battery size. The optimization and modeling approach adopted here facilitates better understanding of the potential benefits from proper selection of motor/ generator and battery size on fuel economy and GHG emissions. This understanding can help us identify the appropriate sizing of these components and thus reducing the PHEV cost. Addressing optimal sizing of PHEV components could aim at an extensive market penetration of PHEVs. C1 Oak Ridge Natl Lab, Energy & Transportat Sci Div, Knoxville, TN 37932 USA. RP Malikopoulos, AA (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, Knoxville, TN 37932 USA. EM andreas@ornl.gov FU U.S. Department of Energy FX The author appreciates the insightful remarks and suggestions received from C. Stuart Daw and the assistance from David Smith with the Autonomie models. This research was supported by the U.S. Department of Energy. This support is gratefully acknowledged. NR 43 TC 4 Z9 4 U1 2 U2 9 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD DEC PY 2013 VL 135 IS 4 AR 041201 DI 10.1115/1.4023334 PG 9 WC Energy & Fuels SC Energy & Fuels GA 295QH UT WOS:000330130100002 ER PT J AU Vidhi, R Kuravi, S Goswami, DY Stefanakos, E Sabau, AS AF Vidhi, Rachana Kuravi, Sarada Goswami, D. Yogi Stefanakos, Elias Sabau, Adrian S. TI Organic Fluids in a Supercritical Rankine Cycle for Low Temperature Power Generation SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID ENERGY RECOVERY-SYSTEMS; WORKING FLUIDS; THERMODYNAMIC CYCLE; PARAMETRIC OPTIMIZATION; PERFORMANCE ANALYSIS; COOLING CYCLE; SOLAR-ENERGY; HEAT-SOURCE; WASTE HEAT; REFRIGERANTS AB This paper presents a performance analysis of a supercritical organic Rankine cycle (SORC) with various working fluids with thermal energy provided from a geothermal energy source. In the present study, a number of pure fluids (R23, R32, R125, R143a, R134a, R218, and R170) are analyzed to identify the most suitable fluids for different operating conditions. The source temperature is varied between 125 degrees C and 200 degrees C, to study its effect on the efficiency of the cycle for fixed and variable pressure ratios. The energy and exergy efficiencies for each working fluid are obtained and the optimum fluid is selected. It is found that thermal efficiencies as high as 21% can be obtained with 200 degrees C source temperature and 10 degrees C cooling water temperature considered in this study. For medium source temperatures (125-150 degrees C), thermal efficiencies higher than 12% are obtained. C1 [Vidhi, Rachana; Goswami, D. Yogi; Stefanakos, Elias] Univ S Florida, Clean Energy Res Ctr, Tampa, FL 33620 USA. [Kuravi, Sarada] Florida Inst Technol, Dept Mech & Aerosp Engn, Melbourne, FL 32901 USA. [Sabau, Adrian S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Goswami, DY (reprint author), Univ S Florida, Clean Energy Res Ctr, 4202 E Fowler Ave, Tampa, FL 33620 USA. EM rachana@mail.usf.edu; skuravi@fit.edu; goswami@usf.edu; estefana@usf.edu; sabaua@ornl.gov RI Sabau, Adrian/B-9571-2008 OI Sabau, Adrian/0000-0003-3088-6474 FU Geothermal Technologies Program, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy [DE-AC05-00OR22725] FX This work was performed for the project "Working Fluids and Their Effect on Geothermal Turbines" sponsored by the Geothermal Technologies Program, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy under Contract No. DE-AC05-00OR22725, Oak Ridge National Laboratory, managed and operated by UT-Battelle, LLC. NR 49 TC 2 Z9 2 U1 1 U2 25 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD DEC PY 2013 VL 135 IS 4 AR 042002 DI 10.1115/1.4023513 PG 9 WC Energy & Fuels SC Energy & Fuels GA 295QH UT WOS:000330130100007 ER PT J AU Rycroft, CH Dehbi, A Lind, T Guntay, S AF Rycroft, Chris H. Dehbi, Abdel Lind, Terttaliisa Guentay, Salih TI Granular flow in pebble-bed nuclear reactors: Scaling, dust generation, and stress SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID CORE; WEAR; GRAPHITE; MODEL; TRANSITION; PREDICTION; DYNAMICS; BEHAVIOR; CONTACT; MATTER AB In experimental prototypes of pebble-bed reactors, significant quantities of graphite dust have been observed due to rubbing between pebbles as they flow through the core. At the typical operating conditions in these reactors, which feature high temperatures, pressures, and a helium atmosphere, limited data is available on the frictional properties of the pebble surfaces, and as a result, a conceptual design of a scaled-down version of a pebble-bed reactor has been proposed to investigate this issue in detail. However, this raises general questions about how the granular flow in a scaled facility will emulate that in a full-size reactor. To address this, simulations of granular flow in pebble-bed reactors using the discrete-element method (DEM) have been carried out in a full-size geometry (using 440,000 pebbles) and compared to those in geometries scaled down by factors of 3:1 and 6:1. Differences in velocity profiles, pebble ordering, pebble wear, and stresses are examined, and the effect of friction is discussed. The results show complex behavior due to discrete pebble packing effects, although several simple scaling rules can be derived. Published by Elsevier B.V. C1 [Rycroft, Chris H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Rycroft, Chris H.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Rycroft, Chris H.] Lawrence Berkeley Lab, Dept Math, Berkeley, CA 94720 USA. [Rycroft, Chris H.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Dehbi, Abdel; Lind, Terttaliisa; Guentay, Salih] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. RP Rycroft, CH (reprint author), Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. EM chr@seas.harvard.edu; abdel.dehbi@psi.ch; terttaliisa.lind@psi.ch; salih.guentay@psi.ch OI Rycroft, Chris/0000-0003-4677-6990 FU Office of Science, Computational and Technology Research, U.S. Department of Energy [DE-AC02-05CH11231] FX C.H. Rycroft is grateful to L.E. Silbert for useful discussions about the computation of wear within the simulations. C.H. Rycroft was supported by the Director, Office of Science, Computational and Technology Research, U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 65 TC 6 Z9 7 U1 0 U2 9 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD DEC PY 2013 VL 265 BP 69 EP 84 DI 10.1016/j.nucengdes.2013.07.010 PG 16 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 294ZD UT WOS:000330085500010 ER PT J AU Jeremic, B Tafazzoli, N Ancheta, T Orbovic, N Blahoianu, A AF Jeremic, B. Tafazzoli, N. Ancheta, T. Orbovic, N. Blahoianu, A. TI Seismic behavior of NPP structures subjected to realistic 3D, inclined seismic motions, in variable layered soil/rock, on surface or embedded foundations SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID SOIL-STRUCTURE-INTERACTION; PATTERN MULTIFRONTAL METHOD; DOMAIN REDUCTION METHOD; LOCALIZED REGIONS; RESPONSE ANALYSIS AB Presented here is an investigation of the seismic response of a massive NPP structures due to full 3D, inclined, un-correlated input motions for different soil and rock profiles. Of particular interest are the effects of soil and rock layering on the response and the changes of input motions (frequency characteristics) due to such layering. In addition to rock/soil layering effects, investigated are also effects of foundation embedment on dynamic response. Significant differences were observed in dynamic response of containment and internal structure founded on surface and on embedded foundations. These differences were observed for both rock and soil profiles. Select results are used to present most interesting findings. (C) 2013 Elsevier B.V. All rights reserved. C1 [Jeremic, B.; Tafazzoli, N.] Univ Calif Davis, Davis, CA 95616 USA. [Jeremic, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ancheta, T.] Risk Management Solut Inc, Newark, CA USA. [Orbovic, N.; Blahoianu, A.] Canadian Nucl Safety Commiss, Ottawa, ON, Canada. RP Jeremic, B (reprint author), Univ Calif Davis, Davis, CA 95616 USA. EM jeremic@ucdavis.edu FU Canadian Nuclear Safety Commission (SNSC) FX Work presented here was funded by a grant from the Canadian Nuclear Safety Commission (SNSC) and such support is greatly appreciated. NR 41 TC 2 Z9 2 U1 1 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD DEC PY 2013 VL 265 BP 85 EP 94 DI 10.1016/j.nucengdes.2013.07.003 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 294ZD UT WOS:000330085500011 ER PT J AU Morgan, SW King, JC Pope, CL AF Morgan, Sarah W. King, Jeffrey C. Pope, Chad L. TI Beam characterization at the Neutron Radiography Reactor SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID ENERGY-SPECTRUM; FACILITY AB The quality of a neutron-imaging beam directly impacts the quality of radiographic images produced using that beam. Fully characterizing a neutron beam, including determination of the beam's effective length-to-diameter ratio, neutron flux profile, energy spectrum, potential image quality, and beam divergence, is vital for producing quality radiographic images. This paper provides a characterization of the east neutron imaging beamline at the Idaho National Laboratory Neutron Radiography Reactor (NRAD). The experiments which measured the beam's effective length-to-diameter ratio and potential image quality are based on American Society for Testing and Materials (ASTM) standards. An analysis of the image produced by a calibrated phantom measured the beam divergence. The energy spectrum measurements consist of a series of foil irradiations using a selection of activation foils, compared to the results produced by a Monte Carlo n-Particle (MCNP) model of the beamline. The NRAD has an effective collimation ratio greater than 125, a beam divergence of 0.3 +/- 0.1 degrees, and a gold foil cadmium ratio of 2.7. The flux profile has been quantified and the facility is an ASTM Category 1 radiographic facility. Based on bare and cadmium covered foil activation results, the neutron energy spectrum used in the current MCNP model of the radiography beamline over-samples the thermal region of the neutron energy spectrum. (C) 2013 Elsevier B.V. All rights reserved. C1 [Morgan, Sarah W.; King, Jeffrey C.] Colorado Sch Mines, Nucl Sci & Engn Program, Golden, CO 80401 USA. [Pope, Chad L.] Idaho Natl Lab, Scoville, ID 83475 USA. RP King, JC (reprint author), Colorado Sch Mines, Nucl Sci & Engn Program, 1500 Illinois St, Golden, CO 80401 USA. EM kingjc@mines.edu FU Idaho National Laboratory FX The authors wish to acknowledge Doug Porter, Sean Cunningham, Glen Pappiouannou, and Fred Gholson of the Idaho National Laboratory for assistance in completing the experiments necessary for this research. The authors also wish to acknowledge Randy Bachman at the Colorado School of Mines for his assistance fabricating the indicators used in this project. This project was funded by a grant from the Idaho National Laboratory. NR 31 TC 4 Z9 4 U1 2 U2 7 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD DEC PY 2013 VL 265 BP 639 EP 653 DI 10.1016/j.nucengdes.2013.08.059 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 294ZD UT WOS:000330085500065 ER PT J AU Uehara, S Watanabe, Y Nakazawa, H Adachi, I Aihara, H Asner, DM Aulchenko, V Aushev, T Bakich, AM Bala, A Bhardwaj, V Bhuyan, B Bondar, A Bonvicini, G Bozek, A Bracko, M Chekelian, V Chen, A Chen, P Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, SK Choi, Y Cinabro, D Dalseno, J Dingfelder, J Dolezal, Z Dutta, D Eidelman, S Epifanov, D Farhat, H Fast, JE Feindt, M Ferber, T Frey, A Gaur, V Gabyshev, N Ganguly, S Gillard, R Giordano, F Goh, YM Golob, B Haba, J Hayasaka, K Hayashii, H Hoshi, Y Hou, WS Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Julius, T Kah, DH Kang, JH Kato, E Kawai, H Kawasaki, T Kiesling, C Kim, DY Kim, HO Kim, JB Kim, JH Kim, YJ Klucar, J Ko, BR Kodys, P Korpar, S Krizan, P Krokovny, P Kumita, T Kuzmin, A Kwon, YJ Lee, SH Li, J Li, Y Liu, C Liu, ZQ Liventsev, D Lukin, P Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Moll, A Mori, T Muramatsu, N Mussa, R Nagasaka, Y Nakao, M Ng, C Nisar, NK Nishida, S Nitoh, O Ogawa, S Okuno, S Pakhlova, G Park, CW Park, H Park, HK Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Sahoo, H Saito, T Sakai, Y Sandilya, S Santelj, L Sanuki, T Savinov, V Schneider, O Schnell, G Schwanda, C Seidl, R Senyo, K Seon, O Shapkin, M Shen, CP Shibata, TA Shiu, JG Shwartz, B Sibidanov, A Simon, F Sohn, YS Sokolov, A Solovieva, E Staric, M Steder, M Sumihama, M Sumiyoshi, T Tamponi, U Tanida, K Tatishvili, G Teramoto, Y Uchida, M Uglov, T Unno, Y Uno, S Urquijo, P Vahsen, SE Van Hulse, C Varner, G Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Williams, KM Won, E Yamashita, Y Yashchenko, S Yook, Y Yuan, CZ Yusa, Y Zhang, CC Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Uehara, S. Watanabe, Y. Nakazawa, H. Adachi, I. Aihara, H. Asner, D. M. Aulchenko, V. Aushev, T. Bakich, A. M. Bala, A. Bhardwaj, V. Bhuyan, B. Bondar, A. Bonvicini, G. Bozek, A. Bracko, M. Chekelian, V. Chen, A. Chen, P. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, S. -K. Choi, Y. Cinabro, D. Dalseno, J. Dingfelder, J. Dolezal, Z. Dutta, D. Eidelman, S. Epifanov, D. Farhat, H. Fast, J. E. Feindt, M. Ferber, T. Frey, A. Gaur, V. Gabyshev, N. Ganguly, S. Gillard, R. Giordano, F. Goh, Y. M. Golob, B. Haba, J. Hayasaka, K. Hayashii, H. Hoshi, Y. Hou, W. -S. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Julius, T. Kah, D. H. Kang, J. H. Kato, E. Kawai, H. Kawasaki, T. Kiesling, C. Kim, D. Y. Kim, H. O. Kim, J. B. Kim, J. H. Kim, Y. J. Klucar, J. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lee, S. -H. Li, J. Li, Y. Liu, C. Liu, Z. Q. Liventsev, D. Lukin, P. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Moll, A. Mori, T. Muramatsu, N. Mussa, R. Nagasaka, Y. Nakao, M. Ng, C. Nisar, N. K. Nishida, S. Nitoh, O. Ogawa, S. Okuno, S. Pakhlova, G. Park, C. W. Park, H. Park, H. K. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Sahoo, H. Saito, T. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Seidl, R. Senyo, K. Seon, O. Shapkin, M. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Sibidanov, A. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Staric, M. Steder, M. Sumihama, M. Sumiyoshi, T. Tamponi, U. Tanida, K. Tatishvili, G. Teramoto, Y. Uchida, M. Uglov, T. Unno, Y. Uno, S. Urquijo, P. Vahsen, S. E. Van Hulse, C. Varner, G. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Williams, K. M. Won, E. Yamashita, Y. Yashchenko, S. Yook, Y. Yuan, C. Z. Yusa, Y. Zhang, C. C. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI High-statistics study of K-S(0) pair production in two-photon collisions SO PROGRESS OF THEORETICAL AND EXPERIMENTAL PHYSICS LA English DT Article ID GAMMA-GAMMA; SCALAR MESONS; FINAL-STATE; BELLE; KK; EXCITATION; PI(+)PI(-); GLUEBALLS; ENERGIES; SYSTEM AB We report a high-statistics measurement of the differential cross section of the process gamma gamma -> (KSKS0)-K-0 in the range 1.05 GeV <= W <= 4.00 GeV, where W is the center-of-mass energy of the colliding photons, using 972 fb(-1) of data collected with the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider operated at and near the Upsilon-resonance region. The differential cross section is fitted by parameterized S-, D-0-, D-2-, G(0)-, and G(2)-wave amplitudes. In the D-2 wave, the f(2)(1270), a(2)(1320), and f(2)'(1525) are dominant and a resonance, the f(2)(2200), is also present. The f(0)(1710) and possibly the f(0)(2500) are seen in the S wave. The mass, total width, and product of the two-photon partial decay width and decay branching fraction to the K (K) over bar state Gamma(gamma gamma) B(K (K) over bar) are extracted for the f(2)'(1525), f(0)(1710), f(2)(2200), and f(0)(2500). The destructive interference between the f(2)(1270) and a(2)(1320) is confirmed by measuring their relative phase. The parameters of the charmonium states chi(c0) and chi(c2) are updated. Possible contributions from the chi(c0)(2P) and chi(c2)(2P) states are discussed. A new upper limit for the branching fraction of the P- and CP-violating decay channel eta(c) -> (KSKS0)-K-0 is reported. The detailed behavior of the cross section is updated and compared with QCD-based calculations. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Dingfelder, J.; Urquijo, P.] Univ Bonn, D-53115 Bonn, Germany. [Aulchenko, V.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shwartz, B.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Aulchenko, V.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shwartz, B.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Dolezal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Kawai, H.] Chiba Univ, Chiba 2638522, Japan. [Ferber, T.; Rostomyan, A.; Steder, M.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Frey, A.] Univ Gottingen, Phys Inst 2, D-37073 Gottingen, Germany. [Choi, S. -K.] Gyeongsang Natl Univ, Chinju 660701, South Korea. [Cheon, B. G.; Goh, Y. M.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Sahoo, H.; Vahsen, S. E.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Uehara, S.; Adachi, I.; Haba, J.; Itoh, R.; Iwasaki, Y.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Uno, S.] High Energy Accelerator Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Hiroshima 7315193, Japan. [Schnell, G.] Ikerbasque, Bilbao 48011, Spain. [Giordano, F.] Univ Illinois, Urbana, IL 61801 USA. [Bhuyan, B.; Dutta, D.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Liu, Z. Q.; Wang, P.; Yuan, C. Z.; Zhang, C. C.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chilikin, K.; Chistov, R.; Mizuk, R.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Klucar, J.; Korpar, S.; Krizan, P.; Pestotnik, R.; Petric, M.; Santelj, L.; Staric, M.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Watanabe, Y.; Okuno, S.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Feindt, M.; Roehrken, M.; Zupanc, A.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Ko, B. R.; Lee, S. -H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Hyun, H. J.; Kah, D. H.; Kim, H. O.; Park, H.; Park, H. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Moll, A.; Ritter, M.; Simon, F.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Mizuk, R.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Uglov, T.] Moscow Phys Tech Inst, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Mori, T.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Bhardwaj, V.; Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Nakazawa, H.; Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Chen, P.; Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Yamashita, Y.] Nippon Dent Univ, Niigata 9518580, Japan. [Kawasaki, T.; Miyata, H.; Yusa, Y.] Niigata Univ, Niigata 9502181, Japan. [Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.] Panjab Univ, Chandigarh 160014, India. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Muramatsu, N.] Tohoku Univ, Res Ctr Elect Photon Sci, Sendai, Miyagi 9808578, Japan. [Seidl, R.] RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Liu, C.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Li, J.; Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Gaur, V.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Kato, E.; Saito, T.; Sanuki, T.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Epifanov, D.; Ng, C.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Koganei, Tokyo 1848588, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Li, Y.; Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kang, J. H.; Kwon, Y. -J.; Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Uehara, S (reprint author), High Energy Accelerator Org KEK, Tsukuba, Ibaraki 3050801, Japan. EM uehara@post.kek.jp RI Nitoh, Osamu/C-3522-2013; Aihara, Hiroaki/F-3854-2010; Ishikawa, Akimasa/G-6916-2012; Uglov, Timofey/B-2406-2014; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Chilikin, Kirill/B-4402-2014; Chistov, Ruslan/B-4893-2014; Pakhlova, Galina/C-5378-2014; Solovieva, Elena/B-2449-2014 OI Aihara, Hiroaki/0000-0002-1907-5964; Uglov, Timofey/0000-0002-4944-1830; Krokovny, Pavel/0000-0002-1236-4667; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Pakhlova, Galina/0000-0001-7518-3022; Solovieva, Elena/0000-0002-5735-4059 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 10825524]; Ministry of Education, Youth and Sports of the Czech Republic [MSM0021620859]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; Volkswagen-Stiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; BK21 and WCU program of the Ministry Education Science and Technology; National Research Foundation of Korea [2010-0021174, 2011-0029457, 2012-0008143, 2012R1A1A2008330]; BRL program under NRF [KRF-2011-0020333]; GSDC of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Federal Agency for Atomic Energy; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); UPV/EHU [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT; JSPS FX We are grateful to V. Chernyak for fruitful discussions. We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grant No. P 22742-N16; the National Natural Science Foundation of China under contract No. 10575109, 10775142, 10875115, and 10825524; the Ministry of Education, Youth and Sports of the Czech Republic under contract No. MSM0021620859; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the Volkswagen-Stiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the BK21 and WCU program of the Ministry Education Science and Technology, National Research Foundation of Korea Grant No. 2010-0021174, 2011-0029457, 2012-0008143, 2012R1A1A2008330, BRL program under NRF Grant No. KRF-2011-0020333, and GSDC of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Federal Agency for Atomic Energy; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under program UFI 11/55; the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"), and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 49 TC 10 Z9 10 U1 2 U2 26 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 2050-3911 J9 PROG THEOR EXP PHYS JI Prog. Theor. Exp. Phys. PD DEC PY 2013 IS 12 AR 123C01 DI 10.1093/ptep/ptt097 PG 45 WC Physics, Multidisciplinary; Physics, Particles & Fields SC Physics GA 296VA UT WOS:000330212300009 ER PT J AU Hwu, ET Nazaretski, E Chu, YS Chen, HH Chen, YS Xu, WH Hwu, Y AF Hwu, En-Te Nazaretski, Evgeny Chu, Yong S. Chen, Huang-Han Chen, Yu-Sheng Xu, Weihe Hwu, Yeukuang TI Design and characterization of a compact nano-positioning system for a portable transmission x-ray microscope SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID FUEL-CELL ANODE; NANOSCALE; NM AB We have designed and constructed a compact nano-positioning system for a Portable Transmission X-ray Microscope (PTXM). We introduce a concept of PTXM and adopt modular approach which implements identical nano-motion platforms to perform manipulation of PTXM components. Modular design provides higher stiffness of the system and allows for reduction of relative thermal drifts between individual constituents of the PTXM apparatus, ensuring a high degree of stability for nanoscale x-ray imaging. We have measured relative thermal drifts between two identical modules to be as low as 15 nm/h, sufficient to perform nanoscale imaging by TXM. Spatial resolution achieved by developed linear piezo stages was measured to be 3 nm with repeatability of 20 nm over 1 mm travel range. (C) 2013 AIP Publishing LLC. C1 [Hwu, En-Te; Chen, Huang-Han; Chen, Yu-Sheng; Hwu, Yeukuang] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Nazaretski, Evgeny; Chu, Yong S.; Xu, Weihe] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Hwu, ET (reprint author), Acad Sinica, Inst Phys, Taipei 11529, Taiwan. OI Hwu, En-Te/0000-0002-5971-4978 FU Academia Sinica; National Science Council [NSC102-2120-M-001-002]; US Department of Energy [DE-AC02-98CH10886] FX The authors would like to thank the machine shop in Institute of Physics, Academia Sinica for machining of PTXM mechanical parts and Mr. D. Kuhne at Brookhaven National Laboratory for machining parts used for thermal drift measurements. This study is supported by Academia Sinica and National Science Council (NSC102-2120-M-001-002). Work at Brookhaven was supported by the US Department of Energy under Contract No. DE-AC02-98CH10886. NR 24 TC 3 Z9 3 U1 2 U2 13 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD DEC PY 2013 VL 84 IS 12 AR 123702 DI 10.1063/1.4838635 PG 8 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 293PE UT WOS:000329984100034 PM 24387436 ER PT J AU Ping, Y Hicks, DG Yaakobi, B Coppari, F Eggert, J Collins, GW AF Ping, Y. Hicks, D. G. Yaakobi, B. Coppari, F. Eggert, J. Collins, G. W. TI A platform for x-ray absorption fine structure study of dynamically compressed materials above 1 Mbar SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID NEAR-EDGE STRUCTURE AB A platform consisting of a multi-shock drive and an implosion backlighter has been developed for x-ray absorption fine structure (XAFS) measurements on materials compressed to multi-Mbar pressures. The experimental setup, target design, and backlighter characteristics are presented. Extended XAFS (EXAFS) measurements for various materials have been demonstrated. A quintuple-crystal design is described to enhance the efficiency of the x-ray spectrometer, enabling observation of very weak EXAFS signals in a single shot. (C) 2013 AIP Publishing LLC. C1 [Ping, Y.; Hicks, D. G.; Coppari, F.; Eggert, J.; Collins, G. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Yaakobi, B.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. RP Ping, Y (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM ping2@llnl.gov RI Hicks, Damien/B-5042-2015 OI Hicks, Damien/0000-0001-8322-9983 FU U.S. DOE by LLNL [DEAC52-07NA27344] FX We thank Jim Emig, Nick Whiting and the OMEGA team at LLE for excellent laser operation and technical support. We also would like to thank W. Unites, T. Uphaus, S. Uhlich, and R. Wallace for target fabrication. This work was performed under the auspices of U.S. DOE by LLNL under Contract No. DEAC52-07NA27344. NR 16 TC 5 Z9 5 U1 1 U2 13 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD DEC PY 2013 VL 84 IS 12 AR 123105 DI 10.1063/1.4841935 PG 5 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 293PE UT WOS:000329984100015 PM 24387418 ER PT J AU Zhao, JK Robertson, JL Herwig, KW Gallmeier, FX Riemer, BW AF Zhao, J. K. Robertson, J. L. Herwig, Kenneth W. Gallmeier, Franz X. Riemer, Bernard W. TI Optimizing moderator dimensions for neutron scattering at the spallation neutron source SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID PERFORMANCE; TOOL; SNS AB In this work, we investigate the effect of neutron moderator dimensions on the performance of neutron scattering instruments at the Spallation Neutron Source (SNS). In a recent study of the planned second target station at the SNS facility, we have found that the dimensions of a moderator play a significant role in determining its surface brightness. A smaller moderator may be significantly brighter over a smaller viewing area. One of the immediate implications of this finding is that for modern neutron scattering instrument designs, moderator dimensions and brightness have to be incorporated as an integrated optimization parameter. Here, we establish a strategy of matching neutron scattering instruments with moderators using analytical and Monte Carlo techniques. In order to simplify our treatment, we group the instruments into two broad categories: those with natural collimation and those that use neutron guide systems. For instruments using natural collimation, the optimal moderator selection depends on the size of the moderator, the sample, and the moderator brightness. The desired beam divergence only plays a role in determining the distance between sample and moderator. For instruments using neutron optical systems, the smallest moderator available that is larger than the entrance dimension of the closest optical element will perform the best (assuming, as is the case here that smaller moderators are brighter). (C) 2013 AIP Publishing LLC. C1 [Zhao, J. K.; Robertson, J. L.; Herwig, Kenneth W.; Gallmeier, Franz X.; Riemer, Bernard W.] Oak Ridge Natl Lab, Instrument & Source Div, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Zhao, JK (reprint author), Oak Ridge Natl Lab, Instrument & Source Div, Spallat Neutron Source, Oak Ridge, TN 37831 USA. OI Riemer, Bernard/0000-0002-6922-3056 FU U.S. Department of Energy [DE-AC05-00OR22725]; Office of Basic Energy Sciences, US Department of Energy FX This article has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The work was sponsored by the Office of Basic Energy Sciences, US Department of Energy. The authors wish to thank Dr. Erik Iverson of SNS for reading and critiquing the article. NR 18 TC 2 Z9 2 U1 1 U2 8 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD DEC PY 2013 VL 84 IS 12 AR 125104 DI 10.1063/1.4841875 PG 8 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 293PE UT WOS:000329984100063 ER PT J AU Tavakoli, R Yoon, H Delshad, M ElSheikh, AH Wheeler, MF Arnold, BW AF Tavakoli, Reza Yoon, Hongkyu Delshad, Mojdeh ElSheikh, Ahmed H. Wheeler, Mary F. Arnold, Bill W. TI Comparison of ensemble filtering algorithms and null-space Monte Carlo for parameter estimation and uncertainty quantification using CO2 sequestration data SO WATER RESOURCES RESEARCH LA English DT Article DE ensemble Kalman filter; ensemble smoother; null-space Monte Carlo; CO2 sequestration; singular value decomposition ID SEQUENTIAL DATA ASSIMILATION; KALMAN FILTER; PERFORMANCE PREDICTIONS; HYDRAULIC CONDUCTIVITY; TRANSMISSIVITY FIELDS; MODEL CALIBRATION; GROUNDWATER-FLOW; INVERSE PROBLEMS; PILOT POINTS; STATE AB Geological storage of CO2 requires multiphase flow models coupled with key hydrogeologic features to accurately predict the long-term consequences. The prediction uncertainty during geological CO2 storage requires a computationally efficient and practically useful framework. This paper presents a comparative study between ensemble-based filtering algorithms (En-As) and calibration-constrained null-space Monte Carlo (NSMC) methods. For the En-As, we use the ensemble Kalman filter (EnKF), ensemble smoother (ES), ES with multiple data assimilation (ES-MDA), and EnKF and ES with the pilot point method. For the NSMC calibrated models with various parameterization, schemes are tested and single and multiple NSMC (M-NSMC) methods are used. A synthetic case with two layers was developed to mimic an actual CO2 injection pilot test where one injection and two observation wells are located within a short distance. Observed data include bottom hole pressure at injection well and gas saturation (S-g) at two observation wells in the upper layer. Model parameters include horizontal permeability and porosity. Comparison of results shows that both methodologies yield good history match and reasonable prediction results in a computationally efficient way. In particular, the ES-MDA and M-NSMC resulted in smaller objective function values and lower prediction uncertainties of S-g profiles compared to other variants tested in this work. The En-As with the pilot point method have higher variability of permeability compared to those without one, but the En-As show smoother permeability fields compared to the NSMC methods. This is because stochastic randomness at a grid scale was included to generate NSMC fields. Both ensemble-based and NSMC algorithms are unable to correct the structural orientation of the prior ensemble members using only the sparse dynamic data from wells, while they obtain reasonable history match, suggesting that structural uncertainty should be incorporated into prior information. Overall, the ES-MDA has an advantage in terms of computational efficiency, but at the expense of additional computation M-NSMC shows applicability for highly nonlinear problems such as multiphase flow problems. C1 [Tavakoli, Reza; Delshad, Mojdeh; ElSheikh, Ahmed H.; Wheeler, Mary F.] Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA. [Yoon, Hongkyu; Arnold, Bill W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Delshad, Mojdeh] Univ Texas Austin, Ctr Petr & Geosyst Engn, Austin, TX 78712 USA. RP Tavakoli, R (reprint author), Univ Texas Austin, Inst Computat Engn & Sci, 201 East 24th St, Austin, TX 78712 USA. EM tavakoli@ices.utexas.edu FU Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DE-SC0001114. We extend our thanks to the Computer Modeling Group (CMG) for providing licenses to the GEM reservoir simulator and associated software. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors thank the reviewers, the associate editor, and the editor for their valuable and constructive comments and suggestions. NR 87 TC 4 Z9 4 U1 1 U2 18 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD DEC PY 2013 VL 49 IS 12 BP 8108 EP 8127 DI 10.1002/2013WR013959 PG 20 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA 292UX UT WOS:000329929100020 ER PT J AU Klein-Marcuschamer, D Blanch, HW AF Klein-Marcuschamer, Daniel Blanch, Harvey W. TI Survival of the Fittest: An Economic Perspective on the Production of Novel Biofuels SO AICHE JOURNAL LA English DT Article DE biofuels; fermentation; economic analysis ID TECHNOECONOMIC ANALYSIS; ESCHERICHIA-COLI; FERMENTATION; PATHWAYS C1 [Klein-Marcuschamer, Daniel; Blanch, Harvey W.] Joint Bioenergy Inst, Emeryville, CA 94608 USA. [Klein-Marcuschamer, Daniel; Blanch, Harvey W.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Klein-Marcuschamer, Daniel] Univ Queensland, Australian Inst Bioengn & Nanotechnol, St Lucia, Qld 4072, Australia. [Blanch, Harvey W.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Blanch, HW (reprint author), Joint Bioenergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA. EM blanch@berkeley.edu FU U.S. Dept. of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02- 05CH11231]; Australian Institute of Bioengineering and Nanotechnology, at the University of Queensland FX This work was performed as part of the DoE Joint BioEnergy Institute (http://www.jbei.org) supported by the U.S. Dept. of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02- 05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. Support to DKM from the Australian Institute of Bioengineering and Nanotechnology, at the University of Queensland, is also acknowledged. NR 28 TC 9 Z9 9 U1 3 U2 18 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0001-1541 EI 1547-5905 J9 AICHE J JI AICHE J. PD DEC PY 2013 VL 59 IS 12 BP 4454 EP 4460 DI 10.1002/aic.14245 PG 7 WC Engineering, Chemical SC Engineering GA 294IQ UT WOS:000330039200001 ER PT J AU Landau, SM Lu, M Joshi, AD Pontecorvo, M Mintun, MA Trojanowski, JQ Shaw, LM Jagust, WJ AF Landau, Susan M. Lu, Ming Joshi, Abhinay D. Pontecorvo, Michael Mintun, Mark A. Trojanowski, John Q. Shaw, Leslie M. Jagust, William J. CA Alzheimers Dis Neuroimaging TI Comparing Positron Emission Tomography Imaging and Cerebrospinal Fluid Measurements of beta-Amyloid SO ANNALS OF NEUROLOGY LA English DT Article ID MILD COGNITIVE IMPAIRMENT; ALZHEIMERS-DISEASE; CSF BIOMARKERS; DIAGNOSIS; DEMENTIA; MARKERS; PET; NEUROPATHOLOGY; DEPOSITION; AUTOPSY AB ObjectiveWe examined agreement and disagreement between 2 biomarkers of beta-amyloid (A) deposition (amyloid positron emission tomography [PET] and cerebrospinal fluid [CSF] A(1-42)) in normal aging and dementia in a large multicenter study. MethodsConcurrently acquired florbetapir PET and CSF A were measured in cognitively normal, mild cognitive impairment (MCI), and Alzheimer's disease participants (n=374) from the Alzheimer's Disease Neuroimaging Initiative. We also compared A measurements in a separate group with serial CSF measurements over 3.10.8 years that preceded a single florbetapir session. Additional biomarker and cognitive data allowed us to further examine profiles of discordant cases. ResultsFlorbetapir and CSF A were inversely correlated across all diagnostic groups, and dichotomous measurements were in agreement in 86% of subjects. Among subjects showing the most disagreement, the 2 discordant groups had different profiles: the florbetapir(+)/CSF A(-) group was larger (n=13) and was made up of only normal and early MCI subjects, whereas the florbetapir(-)/CSF A(+) group was smaller (n=7) and had poorer cognitive function and higher CSF tau, but no ApoE4 carriers. In the longitudinal sample, we observed both stable longitudinal CSF A trajectories and those actively transitioning from normal to abnormal, but the final CSF A measurements were in good agreement with florbetapir cortical retention. InterpretationCSF and amyloid PET measurements of A were consistent in the majority of subjects in the cross-sectional and longitudinal populations. Based on our analysis of discordant subjects, the available evidence did not show that CSF A regularly becomes abnormal prior to fibrillar A accumulation early in the course of disease. Ann Neurol 2013;74:826-836 C1 [Landau, Susan M.; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Landau, Susan M.; Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Lu, Ming; Joshi, Abhinay D.; Pontecorvo, Michael; Mintun, Mark A.] Avid Radiopharmaceut, Philadelphia, PA USA. [Trojanowski, John Q.; Shaw, Leslie M.] Univ Penn, Dept Pathol & Lab Med, Philadelphia, PA USA. [Jagust, William J.] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA. RP Landau, SM (reprint author), Univ Calif Berkeley, 118 Barker Hall MC 3190, Berkeley, CA 94720 USA. EM slandau@berkeley.edu FU ADNI (NIH grant) [U01 AG024904]; National Institute on Aging; National Institute of Biomedical Imaging and Bioengineering FX This work was supported by the ADNI (NIH grant U01 AG024904, grant recipient, Michael Weiner, principal investigator). ADNI is funded by the National Institute on Aging and National Institute of Biomedical Imaging and Bioengineering, and through generous contributions from the following: Abbott, Alzheimer's Association, Alzheimer's Drug Discovery Foundation, Amorfix Life Sciences, AstraZeneca, Bayer HealthCare, BioClinica, Biogen Idec, Bristol-Myers Squibb, Eisai, Elan Pharmaceuticals, Eli Lilly, F. Hoffmann-La Roche and its affiliated company Genentech, GE Healthcare, Innogenetics, IXICO, Janssen Alzheimer Immunotherapy Research & Development, Johnson & Johnson Pharmaceutical Research & Development, Medpace, Merck, Meso Scale Diagnostics, Novartis Pharmaceuticals, Pfizer, Servier, Synarc, and Takeda Pharmaceutical Company. The Canadian Institutes of Health Research provides funds to support ADNI clinical sites in Canada. Private sector contributions are facilitated by the Foundation for the National Institutes of Health (www.fnih.org). The grantee organization is the Northern California Institute for Research and Education, and the study is coordinated by the Alzheimer's Disease Cooperative Study at the University of California, San Diego. ADNI data are disseminated by the Laboratory for Neuro Imaging at the University of California, Los Angeles. NR 36 TC 77 Z9 77 U1 1 U2 10 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0364-5134 EI 1531-8249 J9 ANN NEUROL JI Ann. Neurol. PD DEC PY 2013 VL 74 IS 6 BP 826 EP 836 DI 10.1002/ana.23908 PG 11 WC Clinical Neurology; Neurosciences SC Neurosciences & Neurology GA 292GV UT WOS:000329891100013 PM 23536396 ER PT J AU Lv, YQ Tan, TW Svec, F AF Lv, Yongqin Tan, Tianwei Svec, Frantisek TI Molecular imprinting of proteins in polymers attached to the surface of nanomaterials for selective recognition of biomacromolecules SO BIOTECHNOLOGY ADVANCES LA English DT Review DE Surface imprinting; Protein; Nanomaterials; Recognition ID TRANSFER RADICAL POLYMERIZATION; BOVINE SERUM-ALBUMIN; MULTIWALLED CARBON NANOTUBES; POLYACRYLAMIDE-GEL BEADS; SOLID-PHASE EXTRACTION; ELECTROSTATIC FUNCTIONAL-GROUPS; CHIRAL STATIONARY PHASES; FAR-INFRARED ABSORPTION; ULTRAFINE AL PARTICLES; ANALOG-BUILT POLYMERS AB This review article summarizes the preparation of polymers imprinted with proteins that exhibit antibody-like specificity due to the presence of well-defined recognition sites. We present the newest developments concerned with use of nanomaterials, such as magnetic and silica nanoparticles, nanowires, carbon nanotubes, and quantum dots as supports enabling the preparation of protein-imprinted polymers via surface imprinting techniques. As an alternative receptor-like synthetic materials, these conjugates are attracting a great deal of interest in various fields including proteomics, genomics, and fabrication of selective sensors. However, imprinting of large biomacromolecules such as proteins still remains a challenge due to the inherent limitations related to protein properties. In the text below, we also describe examples of applications focused on selective recognition of biomacromolecules. (C) 2013 Elsevier Inc. All rights reserved. C1 [Lv, Yongqin; Tan, Tianwei] Beijing Univ Chem Technol, Coll Life Sci & Technol, Beijing Key Lab Bioproc, Beijing 100029, Peoples R China. [Lv, Yongqin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Svec, Frantisek] EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Lv, YQ (reprint author), Beijing Univ Chem Technol, Coll Life Sci & Technol, Beijing Key Lab Bioproc, Beijing 100029, Peoples R China. EM twtan@mail.buct.edu.cn; fsvec@lbl.gov RI Foundry, Molecular/G-9968-2014 FU Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the U.S. Department of Energy [DE-AC02-05CH11231]; special assistance of 973 programs [2013CB733600, 2007CB714300, 2011CB710805, 2007CB714302-2]; National Natural Science Foundation of China [20806006, 21076009, 20636010]; 863 program [2006AA020102, 2007AA10040]; Beijing Educational Committee Joint Construction FX All work on this paper was performed at the Molecular Foundry, Lawrence Berkeley National Laboratory. This work as well as F.S. were supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. Y.L. and T.T. gratefully acknowledge the financial supports from the special assistance of 973 programs (2013CB733600, 2007CB714300, 2011CB710805, and 2007CB714302-2), the National Natural Science Foundation of China (20806006, 21076009, and 20636010), 863 program (2006AA020102 and 2007AA10040), and Beijing Educational Committee Joint Construction. NR 147 TC 73 Z9 76 U1 26 U2 284 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0734-9750 EI 1873-1899 J9 BIOTECHNOL ADV JI Biotechnol. Adv. PD DEC PY 2013 VL 31 IS 8 BP 1172 EP 1186 DI 10.1016/j.biotechadv.2013.02.005 PG 15 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 281DW UT WOS:000329081200005 PM 23466364 ER PT J AU Franzosa, JA Bugel, SM Tal, TL La Du, JK Tilton, SC Waters, KM Tanguay, RL AF Franzosa, Jill A. Bugel, Sean M. Tal, Tamara L. La Du, Jane K. Tilton, Susan C. Waters, Katrina M. Tanguay, Robert L. TI Retinoic acid-dependent regulation of miR-19 expression elicits vertebrate axis defects SO FASEB JOURNAL LA English DT Article DE microRNAs; somitogenesis; zebrafish ID LEFT-RIGHT ASYMMETRY; ANIMAL DEVELOPMENT; CYP26 ENZYMES; EMBRYONIC-DEVELOPMENT; METABOLIZING ENZYME; MICRORNA EXPRESSION; SEGMENTATION CLOCK; GENOME DUPLICATION; MOUSE EMBRYO; ZEBRAFISH AB Retinoic acid (RA) is involved in multifarious and complex functions necessary for vertebrate development. RA signaling is reliant on strict enzymatic regulation of RA synthesis and metabolism. Improper spatiotemporal expression of RA during development can result in vertebrate axis defects. microRNAs (miRNAs) are also pivotal in orchestrating developmental processes. While mechanistic links between miRNAs and axial development are established, the role of miRNAs in regulating metabolic enzymes responsible for RA abundance during axis formation has yet to be elucidated. Our results uncovered a role of miR-19 family members in controlling RA metabolism through the regulation of CYP26A1 during vertebrate axis formation. Global miRNA expression profiling showed that developmental RA exposure suppressed the expression of miR-19 family members during zebrafish somitogenesis. A reporter assay confirmed that cyp26a1 is a bona fide target of miR-19 in vivo. Transient knockdown of miR-19 phenocopied axis defects caused by RA exposure. Exogenous miR-19 rescued the axis defects induced by RA exposure. Taken together, these results indicate that the teratogenic effects of RA exposure result, in part, from repression of miR-19 expression and subsequent misregulation of cyp26a1. This highlights a previously unidentified role of miR-19 in facilitating vertebrate axis development via regulation of RA signaling. C1 [Franzosa, Jill A.; Bugel, Sean M.; Tal, Tamara L.; La Du, Jane K.; Tanguay, Robert L.] Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 97333 USA. [Franzosa, Jill A.; Bugel, Sean M.; Tal, Tamara L.; La Du, Jane K.; Tanguay, Robert L.] Oregon State Univ, Environm Hlth Sci Ctr, Corvallis, OR 97333 USA. [Tilton, Susan C.; Waters, Katrina M.] Pacific NW Natl Lab, Richland, WA USA. RP Tanguay, RL (reprint author), Oregon State Univ, Dept Environm & Mol Toxicol, 28645 East HWY 34, Corvallis, OR 97333 USA. EM robert.tanguay@oregonstate.edu OI Tal, Tamara/0000-0001-8365-9385 FU U.S. National Institute of Environmental Health Sciences (NIEHS) Environmental Health Sciences Core Center [P30 ES000210]; NIEHS [T32 ES007060, P42 ES016465]; Oregon State University Linus Pauling Institute FX The authors thank Leah Wehmas for her experimental and technical assistance. The authors are grateful to Cari Buchner, Carrie Barton, and the staff at the Sinnhuber Aquatic Research Laboratory (Oregon State University) for exemplary fish husbandry and technical expertise. The authors thank Dr. James Patton (Vanderbilt University, Nashville, TN, USA) for sharing the pCS2-GFP vector. The authors appreciate the critical comments on the manuscript provided by Britton Goodale, Katerine Saili, Michael Simonich, and R. L. T. laboratory members. This work was supported by U.S. National Institute of Environmental Health Sciences (NIEHS) Environmental Health Sciences Core Center grant P30 ES000210, NIEHS Training grant T32 ES007060, and an Oregon State University Linus Pauling Institute grant to R. L. T., and by NIEHS Superfund Basic Research Program grant P42 ES016465 to R. L. T. and K. M. W. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. The authors declare no conflicts of interest. J.A.F., S. M. B., T. L. T., and R. L. T designed the research; J.A.F., S. M. B., J.K.L., and T. L. T. performed the research; S. C. T. and K. M. W. contributed analytic tools; J.A.F., S. M. B., T. L. T., S. C. T., K. M. W., and R. L. T. analyzed data; and J.A.F. and R. L. T. wrote the paper. NR 96 TC 3 Z9 3 U1 3 U2 9 PU FEDERATION AMER SOC EXP BIOL PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3998 USA SN 0892-6638 EI 1530-6860 J9 FASEB J JI Faseb J. PD DEC PY 2013 VL 27 IS 12 BP 4866 EP 4876 DI 10.1096/fj.12-225524 PG 11 WC Biochemistry & Molecular Biology; Biology; Cell Biology SC Biochemistry & Molecular Biology; Life Sciences & Biomedicine - Other Topics; Cell Biology GA 293UK UT WOS:000329999000021 PM 23975936 ER PT J AU Alvarez, JA Cook, DG Yee, JL van Hattem, MG Fong, DR Fisher, RN AF Alvarez, Jeff A. Cook, David G. Yee, Julie L. van Hattem, Michael G. Fong, Darren R. Fisher, Robert N. TI COMPARATIVE MICROHABITAT CHARACTERISTICS AT OVIPOSITION SITES OF THE CALIFORNIA RED-LEGGED FROG (RANA DRAYTONII) SO HERPETOLOGICAL CONSERVATION AND BIOLOGY LA English DT Article DE California Red-legged Frog; egg mass; habitat; lentic; lotic; oviposition; Rana draytonii; surveys ID SELECTION; BULLFROGS AB We studied the microhabitat characteristics of 747 egg masses of the federally-threatened Rana draytonii (California red-legged frog) at eight sites in California. our study showed that a broad range of aquatic habitats are utilized by ovipositing R. draytonii, including sites with perennial and ephemeral water sources, natural and constructed wetlands, lentic and lotic hydrology, and sites surrounded by protected lands and nested within modified urban areas. We recorded 45 different egg mass attachment types, although the use of only a few types was common at each site. these attachment types ranged from branches and roots of riparian trees, emergent and submergent wetland vegetation, flooded upland grassland/ruderal vegetation, and debris. eggs were deposited in relatively shallow water (mean 39.7 cm) when compared to maximum site depths. We found that most frogs in artificial pond, natural creek, and artificial channel habitats deposited egg masses within one meter of the shore, while egg masses in a seasonal marsh averaged 27.3 m from the shore due to extensive emergent vegetation. Rana draytonii appeared to delay breeding in lotic habitats and in more inland sites compared to lentic habitats and coastal sites. eggs occurred as early as mid-december at a coastal artificial pond and as late as mid-april in an inland natural creek. We speculate that this delay in breeding may represent a method of avoiding high-flow events and/or freezing temperatures. Understanding the factors related to the reproductive needs of this species can contribute to creating, managing, or preserving appropriate habitat, and promoting species recovery. C1 [Alvarez, Jeff A.] Wildlife Project, Sacramento, CA 95818 USA. [Yee, Julie L.] US Geol Survey, Western Ecol Res Ctr, Sacramento, CA 95819 USA. [van Hattem, Michael G.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [van Hattem, Michael G.] Calif Dept Fish & Wildlife, Eureka, CA 95501 USA. [Fong, Darren R.] Golden Gate Natl Recreat Area, Sausalito, CA 94965 USA. [Fisher, Robert N.] US Geol Survey, Western Ecol Res Ctr, San Diego Field Stn, San Diego, CA 92101 USA. RP Alvarez, JA (reprint author), Wildlife Project, POB 188888, Sacramento, CA 95818 USA. EM jeff@thewildlifeproject.com NR 35 TC 3 Z9 3 U1 3 U2 25 PU HERPETOLOGICAL CONSERVATION & BIOLOGY PI CORVALLIS PA C/O R BRUCE BURY, USGS FOREST & RANGELAND, CORVALLIS, OR 00000 USA SN 2151-0733 EI 1931-7603 J9 HERPETOL CONSERV BIO JI Herpetol. Conserv. Biol. PD DEC PY 2013 VL 8 IS 3 BP 539 EP 551 PG 13 WC Zoology SC Zoology GA 294KD UT WOS:000330043600004 ER PT J AU De Gregorio, BA Weatherhead, PJ Tuberville, TD Sperry, JH AF GreGorio, Brett A. De Weatherhead, Patrick. J. Tuberville, Tracey D. Sperry, Jinelle H. TI TIME IN CAPTIVITY AFFECTS FORAGING BEHAVIOR OF RATSNAKES: IMPLICATIONS FOR TRANSLOCATION SO HERPETOLOGICAL CONSERVATION AND BIOLOGY LA English DT Article DE conservation; Elaphe obsoleta; prey detection; reintroduction; repatriation; snakes ID CONSERVATION TOOL; VISUAL-STIMULI; SURVIVAL; SNAKES; WILD; INDIVIDUALS; ENRICHMENT; EXPERIENCE; RESPONSES; ANIMALS AB As wildlife populations decline or disappear, wildlife professionals are using management tools such as translocation to maintain viable populations, often with mixed results. Wild-to-wild translocations are often more successful than when captive animals are released, raising concerns that captivity may have deleterious effects on animals. although the effects of captivity have been documented on a generational time-scale, effects within the lifetime of an individual have received much less attention. here we examine how time in captivity affects foraging behavior of wild-caught ratsnakes (Elaphe obsoleta). The longer ratsnakes had been in captivity, the less successful and slower they were to react to prey in a simple laboratory discrimination task. snakes that had been captive for a year or more performed no better than expected by chance. Captivity-induced degradation of ecologically important behaviors provides a potential mechanism underlying the poor performance of animals that are released into the wild following prolonged captivity. our results also suggest that research using captive snakes may not always document behaviors representative of wild snakes. C1 [GreGorio, Brett A. De; Weatherhead, Patrick. J.; Sperry, Jinelle H.] Univ Illinois, Dept Nat Resources & Environm Sci, Urbana, IL 61801 USA. [GreGorio, Brett A. De; Tuberville, Tracey D.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Sperry, Jinelle H.] Engineer Res & Dev Ctr, Champaign, IL 61826 USA. RP De Gregorio, BA (reprint author), Univ Illinois, Dept Nat Resources & Environm Sci, 1102 S Goodwin Ave, Urbana, IL 61801 USA. EM Bdegrego@illinois.edu FU Construction Engineering Research Laboratory of the Engineer Research Development Center (ERDC); Department of Energy to the University of Georgia Research Foundation [DE-FC09-07SR22506] FX Funding for this project was provided by the Construction Engineering Research Laboratory of the Engineer Research Development Center (ERDC). We thank Tim Hayden for assistance in arranging funding. This work would not have been possible without the generosity and meticulous record-keeping of Sean Poppy and Angela Tucker in the SREL outreach program. Eric Nordberg, Mary Mack Gray, Brian Metts, Ashley Smith, Patrick Barnhart, Patrick Roberts, Caitlin Kupar, and Phil Vogrinc assisted in snake capture and husbandry. Partial support for manuscript preparation by TDT and use of animal facilities was made possible by Award Number DE-FC09-07SR22506 from Department of Energy to the University of Georgia Research Foundation. Animals were collected under South Carolina Department of Natural Resources permits #G-11-03 and 23-2012A. Animal procedures conformed to permits approved by the University of Illinois (IACUC #11054) and University of Georgia (AUP #A2011 04-007-Y2-A0). NR 38 TC 3 Z9 4 U1 6 U2 46 PU HERPETOLOGICAL CONSERVATION & BIOLOGY PI CORVALLIS PA C/O R BRUCE BURY, USGS FOREST & RANGELAND, CORVALLIS, OR 00000 USA SN 2151-0733 EI 1931-7603 J9 HERPETOL CONSERV BIO JI Herpetol. Conserv. Biol. PD DEC PY 2013 VL 8 IS 3 BP 581 EP 590 PG 10 WC Zoology SC Zoology GA 294KD UT WOS:000330043600008 ER PT J AU Porosoff, MD Yu, WT Chen, JGG AF Porosoff, Marc D. Yu, Weiting Chen, Jingguang G. TI Challenges and opportunities in correlating bimetallic model surfaces and supported catalysts SO JOURNAL OF CATALYSIS LA English DT Article DE Bimetallic catalysis; Model surfaces; Supported catalysts ID TRANSITION-METAL CARBIDES; ETHYLENE-GLYCOL; CYCLOHEXENE HYDROGENATION; CHEMICAL-PROPERTIES; TUNGSTEN CARBIDE; 1ST PRINCIPLES; M/PT(111) M; NI; CHEMISTRY; PLATINUM AB In this paper, we use the hydrogenation and reforming reactions to demonstrate the success and challenges in correlating bimetallic model surfaces with supported catalysts. For hydrogenation reactions, results from ultra-high vacuum (UHV) experiments and density functional theory (DFT) calculations of model surfaces typically show strong correlation with reactor evaluations of the corresponding supported catalysts. However, such correlation is less clear for reforming reactions, which require a strong bonding of oxygenates on the bimetallic surfaces. One of the challenges is to understand the bimetallic structures and their stability under reaction conditions, which would in turn provide critical input for constructing relevant model surfaces for UHV and DFT studies. In order to truly achieve the design of bimetallic catalysts from first principles, it is essential that the structures of model surfaces are as close as possible to those under reaction conditions. (C) 2013 Elsevier Inc. All rights reserved. C1 [Porosoff, Marc D.; Yu, Weiting] Univ Delaware, Dept Biomol & Chem Engn, Newark, DE 19716 USA. [Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. [Chen, Jingguang G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Chen, JGG (reprint author), Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. EM jgchen@columbia.edu RI Porosoff, Marc/N-2816-2015 FU Catalysis Center for Energy Innovation, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001004] FX The authors acknowledge support from the Catalysis Center for Energy Innovation, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001004. NR 49 TC 11 Z9 11 U1 7 U2 55 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD DEC PY 2013 VL 308 BP 2 EP 10 DI 10.1016/j.jcat.2013.05.009 PG 9 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 292DF UT WOS:000329881700002 ER PT J AU Lee, WS Akatay, MC Stach, EA Ribeiro, FH Delgass, WN AF Lee, Wen-Sheng Akatay, M. Cem Stach, Eric A. Ribeiro, Fabio H. Delgass, W. Nicholas TI Enhanced reaction rate for gas-phase epoxidation of propylene using H-2 and O-2 by Cs promotion of Au/TS-1 SO JOURNAL OF CATALYSIS LA English DT Article DE Au/TS-1; Cs promotion; Gold clusters; Propylene epoxidation; Nanoporous materials ID SUPPORTED GOLD NANOPARTICLES; CATALYTIC-ACTIVITY; TITANIUM SILICALITE-1; PROPENE EPOXIDATION; HYDROGEN-PEROXIDE; AU NANOPARTICLES; MOLECULAR-SIEVES; SHIFT CATALYSIS; ACTIVE-SITES; OXIDATION AB Gold clusters supported on titanium silicalite-1 (hereafter denoted as Au/TS-1) with high gold loading at 0.1-0.16 wt%, prepared by the deposition precipitation (DP) method, showed about two times enhancement in the PO rate (similar to 300 versus similar to 150 gpo h(-1) kg(cat)(-1), at 200 degrees C), similar to 10% increase in PO selectivity (similar to 80% versus similar to 70%) and similar to 5-10% increase in H-2 selectivity (-20% versus similar to 10%) when Cs2CO3 instead of Na2CO3 was used as the precipitation agent. Using Cs2CO3 as the precipitation agent caused a fourfold increase in Au uptake efficiency, indicating a strong interaction between Cs and Au in the Au/TS-1 system. XPS/TEM analyses for two Au/TS-1 samples with the same gold loading at similar to 0.16 wt% but different alkali metals (Cs versus Na) indicate that more Au was retained inside the TS-1 nanopores for the Cs sample. The presence of Cs is, therefore, proposed to help stabilize small gold clusters (< 1 nm) inside the TS-1 nanoporous channels at the high gold loading (> 0.1 wt%) due to the Cs/Au interaction, resulting in the promotion of PO rate per gram of catalyst. Furthermore, similar apparent activation energy at 30 kJ mole(-1) observed for the Au/TS-1 catalysts with the presence of either Cs or Na suggests that the number, but not the nature of the active sites, is changed in the Cs-promoted samples. Finally, regardless of the type of alkali metal (Na or Cs) present in the catalysts, lower Ti content (Si/Ti molar ratio 100) for Au/TS-1 catalysts was found to favor PO catalytic performance. (C) 2013 Elsevier Inc. All rights reserved. C1 [Lee, Wen-Sheng; Ribeiro, Fabio H.; Delgass, W. Nicholas] Purdue Univ, W Lafayette, IN 47907 USA. [Akatay, M. Cem; Stach, Eric A.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Akatay, M. Cem; Stach, Eric A.] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Delgass, WN (reprint author), Purdue Univ, Forney Hall Chem Engn, W Lafayette, IN 47907 USA. EM delgass@purdue.edu RI Stach, Eric/D-8545-2011; OI Stach, Eric/0000-0002-3366-2153; Ribeiro, Fabio/0000-0001-7752-461X FU Department of Energy, Office of Basic Energy Sciences, Chemical Sciences [DE-FG02-03ER15408] FX Support from the Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, under Grant DE-FG02-03ER15408 is gratefully acknowledged. The authors would also like to thank the Surface Analysis Facility at Birck Nanotechnology Center for XPS measurements and Mr. Wei-Hsuan Liu for his help and discussion of the kinetic measurements. NR 59 TC 22 Z9 22 U1 11 U2 81 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD DEC PY 2013 VL 308 BP 98 EP 113 DI 10.1016/j.jcat.2013.05.023 PG 16 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 292DF UT WOS:000329881700010 ER PT J AU Chia, M O'Neill, BJ Alamillo, R Dietrich, PJ Ribeiro, FH Miller, JT Dumesic, JA AF Chia, Mei O'Neill, Brandon J. Alamillo, Ricardo Dietrich, Paul J. Ribeiro, Fabio H. Miller, Jeffrey T. Dumesic, James A. TI Bimetallic RhRe/C catalysts for the production of biomass-derived chemicals SO JOURNAL OF CATALYSIS LA English DT Article DE Bifunctional; Rhodium; Rhenium; Hydrogenolysis; Dehydration; Biomass; Fructose; X-ray absorption spectroscopy ID PLATINUM-RHENIUM CATALYSTS; CARBON-SUPPORTED PLATINUM; D-FRUCTOSE FORMATION; BIPHASIC SYSTEM; LEVULINIC ACID; SYNTHESIS GAS; GLYCEROL; HYDROGENOLYSIS; DEHYDRATION; 5-HYDROXYMETHYL-2-FURALDEHYDE AB Pretreatment temperature affects the activity of a RhRe/C catalyst for C-O hydrogenolysis of 2-(hydroxymethyl)tetrahydropyran and for dehydration of fructose. Catalytic activities for both C-O hydrogenolysis and dehydration were observed to decrease with an increase in pretreatment temperature from 393 to 723 K, which coincides with a decrease in the number of sites quantified using NH3 temperature-programmed desorption. Results for the characterization of RhRe/C using X-ray absorption spectroscopy (XAS) are consistent with the formation of Rh-rich particles with a shell of metallic Re islands after reduction at 393 K, which shows penetration of Re into the nanoparticie with increasing reduction temperature. No evidence of rhenium oxide was found from the Re L-III-edge MS spectra after reduction at temperatures above 363 K or under aqueous operando conditions. The apparent acidity of FthRe/C is suggested to be generated from the activation of water molecules over Re atoms on the surface of metallic Rh Re particles. (C) 2013 Elsevier Inc. All rights reserved. C1 [Chia, Mei; O'Neill, Brandon J.; Alamillo, Ricardo; Dumesic, James A.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Dietrich, Paul J.; Ribeiro, Fabio H.] Purdue Univ, Dept Chem Engn, W Lafayette, IN 47907 USA. [Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60429 USA. RP Dumesic, JA (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, 1415 Engn Dr, Madison, WI 53706 USA. EM dumesic@engr.wisc.edu RI BM, MRCAT/G-7576-2011; ID, MRCAT/G-7586-2011; OI Ribeiro, Fabio/0000-0001-7752-461X FU Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center; US Department of Energy, Office of Science, Office of Basic Energy Sciences; National Science Foundation [EEC-0813570]; National Science Foundation Graduate Research Fellowship Program [DGE0718123]; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences [DE-ACO2-06CH11357]; Department of Energy; MRCAT FX X-ray adsorption spectroscopy studies were supported by the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. Fructose dehydration work was supported by the National Science Foundation under the auspices of the Center for Enabling New Technologies through Catalysis (CENTC). All other work was supported by the National Science Foundation under Award No. EEC-0813570. R.A. acknowledges support from the National Science Foundation Graduate Research Fellowship Program under Grant No. DGE0718123. Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences, under Contract DE-ACO2-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. We wish to thank Professors Robert Davis and Matthew Neurock (University of Virginia) for many discussions regarding the catalytic properties of Re-promoted metal catalysts. In addition, we wish to thank Professor Alex Bell for valuable suggestions to us during his visit to the University of Wisconsin to present Hougen Lectures (in February, 2013). NR 27 TC 24 Z9 27 U1 10 U2 122 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD DEC PY 2013 VL 308 BP 226 EP 236 DI 10.1016/j.jcat.2013.08.008 PG 11 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 292DF UT WOS:000329881700021 ER PT J AU Youn, IM Park, SH Roh, HG Lee, CS AF Youn, In Mo Park, Su Han Roh, Hyun Gu Lee, Chang Sik TI Impact of DME as an Oxygenated Alternative Fuel on Combustion and Emissions Reduction in a Transportation Vehicle at Low Load Condition SO JOURNAL OF ENERGY ENGINEERING LA English DT Article DE Dimethyl ether (DME); Pilot injection strategy; Heat release; Combustion duration; Exhaust emission ID DIMETHYL ETHER DME; DIESEL-ENGINE; PERFORMANCE; SYSTEM; SPRAY AB This study investigates the impact of dimethyl ether (DME) on the combustion and exhaust emission characteristics at low engine load operating and pilot injection conditions in a four-cylinder diesel engine that was modified for DME application. The combustion characteristics were analyzed based on the combustion pressure, the rate of heat release, the accumulated heat release, and the premixed combustion characteristics. The emission characteristics were analyzed through the analysis of the nitrogen oxides (NOx), soot, hydrocarbon (HC), and carbon monoxide (CO). The heat release amount per unit crank angle in DME combustion is higher than that in diesel combustion in a pilot injected combustion mode. The accumulated heat release of DME during the main combustion is higher than that of diesel fuel. The pilot injection combustion of DME fuel started earlier than single-injection combustion does. The advanced pilot injection timing caused a decrease of premixed combustion duration and a retardation of premixed combustion phasing. As the pilot injection timing moved to top dead center, the total combustion duration and the heat release amount per unit crank angle decreased. In the emission results, advances of the pilot injection timing caused the decrease of indicated specific (IS) ISNOx emission in both diesel and DME fuels. The advanced pilot injection timing caused a significant increase of HC and CO emission because of an increase of the overmixed region and incomplete combustion. C1 [Youn, In Mo] Korea Inst Energy Technol Evaluat & Planning, R&D Planning Team, Seoul 133502, South Korea. [Park, Su Han] Argonne Natl Lab, Adv Photon Source, XRay Sci Div, Lemont, IL 60439 USA. [Park, Su Han; Lee, Chang Sik] Hanyang Univ, Sch Mech Engn, Seoul 133791, South Korea. [Roh, Hyun Gu] Induk Univ, Dept Mech & Automot Engn, Seoul 139749, South Korea. RP Lee, CS (reprint author), Hanyang Univ, Sch Mech Engn, 17 Haengdang Dong, Seoul 133791, South Korea. EM cslee@hanyang.ac.kr FU Basic Science Research Program through the National Research Foundation of Korea (NRF); Ministry of Education, Science, and Technology [2012007015]; Second Brain Korea 21 Project FX This research was supported in part by the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science, and Technology (2012007015) and the Second Brain Korea 21 Project. NR 37 TC 2 Z9 2 U1 1 U2 5 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 0733-9402 EI 1943-7897 J9 J ENERG ENG JI J. Energy Eng.-ASCE PD DEC 1 PY 2013 VL 139 IS 4 BP 308 EP 315 DI 10.1061/(ASCE)EY.1943-7897.0000124 PG 8 WC Energy & Fuels; Engineering, Civil SC Energy & Fuels; Engineering GA 292OW UT WOS:000329912600008 ER PT J AU Vanderhoof, M Williams, CA Ghimire, B Rogan, J AF Vanderhoof, M. Williams, C. A. Ghimire, B. Rogan, J. TI Impact of mountain pine beetle outbreaks on forest albedo and radiative forcing, as derived from Moderate Resolution Imaging Spectroradiometer, Rocky Mountains, USA SO JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES LA English DT Article DE albedo; radiative forcing; bark beetles; disturbance; lodgepole pine; ponderosa pine ID REFLECTANCE DISTRIBUTION FUNCTION; CLIMATE RESPONSE; MODIS; SURFACE; SCALE; DECOMPOSITION; DISTURBANCES; TEMPERATURES; PRODUCTS; DYNAMICS AB Mountain pine beetle (Dendroctonus ponderosae) outbreaks in North America are widespread and have potentially large-scale impacts on albedo and associated radiative forcing. Mountain pine beetle outbreaks in Colorado and southern Wyoming have resulted in persistent and significant increases in both winter albedo (change peaked 10years post outbreak at 0.060.01 and 0.050.01, in lodgepole pine (Pinus contorta) and ponderosa pine (Pinus ponderosa) stands, respectively) and spring albedo (change peaked 10years post outbreak at 0.060.01 and 0.040.01, in lodgepole pine and ponderosa pine stands, respectively). Instantaneous top-of-atmosphere radiative forcing peaked for both lodgepole pine and ponderosa pine stands in winter at 10years post outbreak at -1.7 +/- 0.2Wm(-2) and -1.4 +/- 0.2Wm(-2), respectively. The persistent increase in albedo with time since mountain pine beetle disturbance combined with the continued progression of the attack across the landscape from 1994-2011 resulted in an exponential increase in winter and annual radiative cooling (MW) over time. In 2011 the rate of radiative forcing within the study area reached -982.7 +/- 139.0MW, -269.8 +/- 38.2MW, -31.1 +/- 4.4MW, and -147.8 +/- 20.9MW in winter, spring, summer, and fall, respectively. An increase in radiative cooling has the potential to decrease sensible and/or latent heat flux by reducing available energy. Such changes could affect current mountain pine beetle outbreaks which are influenced by climatic conditions. C1 [Vanderhoof, M.; Williams, C. A.; Ghimire, B.; Rogan, J.] Clark Univ, Grad Sch Geog, Worcester, MA 01610 USA. [Ghimire, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Vanderhoof, M (reprint author), Clark Univ, Grad Sch Geog, 950 Main St, Worcester, MA 01610 USA. EM mevanderhoof@clarku.edu FU NASA Earth and Space Science Fellowship (NESSF) [11-Earth11F-134, 12-Earth12R-59]; NASA ROSES09 Science of Terra and Aqua program [NNX11AG53G] FX This work was funded by the 2011-2013 NASA Earth and Space Science Fellowship (NESSF) (11-Earth11F-134 and 12-Earth12R-59). Additional financial support was received from the NASA ROSES09 Science of Terra and Aqua program through grant NNX11AG53G. We thank Rocky Mountain National Park for their field support; Marcus Pasay for his assistance with field work; and Jefferey Masek, Crystal Schaaf, Feng Gao, and the anonymous reviewers for their insightful comments. NR 40 TC 8 Z9 8 U1 2 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-8953 EI 2169-8961 J9 J GEOPHYS RES-BIOGEO JI J. Geophys. Res.-Biogeosci. PD DEC PY 2013 VL 118 IS 4 BP 1461 EP 1471 DI 10.1002/jgrg.20120 PG 11 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA 291ZM UT WOS:000329871400010 ER PT J AU Klise, KA Phillips, CA Janke, RJ AF Klise, Katherine A. Phillips, Cynthia A. Janke, Robert J. TI Two-Tiered Sensor Placement for Large Water Distribution Network Models SO JOURNAL OF INFRASTRUCTURE SYSTEMS LA English DT Article DE Water distribution systems; Security; Terrorism; Water quality; Scale effects; Optimization; Public health AB Water distribution network models for large municipalities have tens of thousands of interconnecting pipes and junctions with complex hydraulic controls. Many water security applications, including sensor placement optimization, require detailed simulation of potential contamination incidents. The postsimulation optimization problem can easily exceed memory on standard desktop computers. Large networks can be skeletonized to reduce computation; however, this alters network hydraulics, and therefore sensor placement. The objective of this paper is to evaluate a two-tiered sensor placement approach that combines hydraulic and water quality simulations using all-pipes, or original, network models with subsequent geographic aggregation of time and impact values to reduce memory requirements. The two-tiered approach first places sensors on aggregated regions, then refines the solution to actual nodes in the original model. The two-tiered sensor placement approach is compared to results using the original network and skeletonized networks based on solution quality, memory use, and runtime. Results show that skeletonized networks introduce error in sensor placement. Two-tiered sensor placement using geographic aggregation replicates the original model solution to within 5% in most cases. (C) 2013 American Society of Civil Engineers. C1 [Klise, Katherine A.; Phillips, Cynthia A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Janke, Robert J.] US EPA, Water Infrastruct Protect Div, Cincinnati, OH 45268 USA. RP Klise, KA (reprint author), Sandia Natl Labs, POB 5800 MS 0751, Albuquerque, NM 87185 USA. EM kaklise@sandia.gov; caphill@sandia.gov; Janke.Robert@epamail.epa.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The U.S. EPA, Office of Research and Development funded and participated in the research described here under an interagency agreement. The views expressed in this paper are those of the authors and do not necessarily reflect the views or policies of the U.S. EPA. Mention of trade names or commercial products does not constitute endorsement or recommendation for use. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 15 TC 9 Z9 9 U1 2 U2 9 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 1076-0342 EI 1943-555X J9 J INFRASTRUCT SYST JI J. Infrastruct. Syst. PD DEC 1 PY 2013 VL 19 IS 4 BP 465 EP 473 DI 10.1061/(ASCE)IS.1943-555X.0000156 PG 9 WC Engineering, Civil SC Engineering GA 292PB UT WOS:000329913100012 ER PT J AU Iakovidis, G AF Iakovidis, G. CA MAMMA Collaboration TI The Micromegas project for the ATLAS upgrade SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT 3rd International Conference on Micro Pattern Gaseous Detectors CY JUL 01-06, 2013 CL Zaragoza, SPAIN DE Micropattern gaseous detectors (MSGC, GEM, THGEM, RETHGEM, MHSP, MICROPIC, MICROMEGAS, InGrid, etc); Time projection chambers; Large detector-systems performance; Trigger concepts and systems (hardware and software) AB Micromegas is one of the detector technologies (along with the small Thin Gap Chambers) that has been chosen for precision tracking and triggering purposes of the ATLAS muon forward detectors in the view of LHC luminosity increase. To fulfill the requirements of such an upgrade, several micromegas prototype detectors were tested in recent test beam campaigns with high energy hadron beams at CERN. Performance studies and results on spatial resolution for perpendicular and inclined tracks, efficiency, as well as detector performance and comparison to simulation in a magnetic field are presented. Moreover, an overview of detector performance after neutron, X-ray, gammas and alphas exposure and as well as construction achievements of large area micromegas detectors are presented. C1 [Iakovidis, G.] Natl Tech Univ Athens, GR-15773 Athens, Greece. [Iakovidis, G.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Iakovidis, G (reprint author), Natl Tech Univ Athens, Zografou Campus, GR-15773 Athens, Greece. EM george.iakovidis@cern.ch NR 10 TC 5 Z9 5 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD DEC PY 2013 VL 8 AR C12007 DI 10.1088/1748-0221/8/12/C12007 PG 10 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 292OB UT WOS:000329910500007 ER PT J AU Jones, BJP Alexander, T Back, HO Collin, G Conrad, JM Greene, A Katori, T Pordes, S Toups, M AF Jones, B. J. P. Alexander, T. Back, H. O. Collin, G. Conrad, J. M. Greene, A. Katori, T. Pordes, S. Toups, M. TI The effects of dissolved methane upon liquid argon scintillation light SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Noble liquid detectors (scintillation, ionization, double-phase); Photon detectors for UV, visible and IR photons (vacuum) (photomultipliers, HPDs, others); Photon detectors for UV, visible and IR photons (gas) (gas-photocathodes, solid-photocathodes) AB In this paper we report on measurements of the effects of dissolved methane upon argon scintillation light. We monitor the light yield from an alpha source held 20 cm from a cryogenic photomultiplier tube (PMT) assembly as methane is injected into a high-purity liquid argon volume. We observe significant suppression of the scintillation light yield by dissolved methane at the 10 part per billion (ppb) level. By examining the late scintillation light time constant, we determine that this loss is caused by an absorption process and also see some evidence of methane-induced scintillation quenching at higher concentrations (50-100 ppb). Using a second PMT assembly we look for visible re-emission features from the dissolved methane which have been reported in gas-phase argon methane mixtures, and we find no evidence of visible re-emission from liquid-phase argon methane mixtures at concentrations between 10 ppb and 0.1%. C1 [Jones, B. J. P.; Collin, G.; Conrad, J. M.; Greene, A.; Katori, T.; Toups, M.] MIT, Cambridge, MA 02139 USA. [Alexander, T.] Univ Massachusetts, Amherst, MA 01003 USA. [Back, H. O.] Princeton Univ, Princeton, NJ 08540 USA. [Pordes, S.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Jones, BJP (reprint author), MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM bjpjones@mit.edu OI Katori, Teppei/0000-0002-9429-9482 FU National Science Foundation [NSF-PHY-1205175, NSF PHY-1211308, NSF PHY-1242585]; Department Of Energy [DE-FG02-91ER40661]; Fermi National Accelerator Laboratory [De-AC02-07CH11359] FX We would like to thank Clementine Jones for proofreading this paper, and Bill Miner, Ron Davis and the other technicians who have assisted us at the Proton Assembly Building, Fermilab for their tireless hard work to provide us with cryogenic facilities of the very highest standard. The authors thank the National Science Foundation (NSF-PHY-1205175, NSF PHY-1211308 and NSF PHY-1242585) and Department Of Energy (DE-FG02-91ER40661). This work was supported by the Fermi National Accelerator Laboratory, which is operated by the Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 29 TC 4 Z9 4 U1 2 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD DEC PY 2013 VL 8 AR P12015 DI 10.1088/1748-0221/8/12/P12015 PG 17 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 292OB UT WOS:000329910500064 ER PT J AU Katz, J Ross, JS Sorce, C Froula, DH AF Katz, J. Ross, J. S. Sorce, C. Froula, D. H. TI A reflective image-rotating periscope for spatially resolved Thomson-scattering experiments on OMEGA SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT 16th International Symposium on Laser-Aided Plasma Diagnostics CY SEP 22-26, 2013 CL Madison, WI DE Plasma diagnostics - probes; Plasma diagnostics - interferometry, spectroscopy and imaging ID LASER-PRODUCED PLASMA; ION-ACOUSTIC-WAVES AB A reflective image rotating periscope has been deployed on the Thomson-scattering system at the Laboratory for Laser Energetics, enabling the capability to make spatially resolved measurements of plasma conditions using either the 2 omega (527-nm) or 4 omega (263-nm) probe beam. The spectral content of ion-acoustic and electron plasma wave Thomson-scattering features are analyzed along the probe beam's axis of propagation using a pair of imaging Czerny-Turner spectrometers. A method for calculating image rotation was applied to design a translating periscope mirror assembly that provides fine adjustment of the image orientation at the spectrometer input plane. Spectrally dispersed Thomson-scattering signals are recorded using time-gated intensified charge-coupled-device cameras. Spectral resolution of up to 0.03 nm (0.2 nm) is achieved using a 1-m (0.3-m) spectrometer, allowing for simultaneous measurements of the ion-acoustic and electron plasma wave features. The optical system's 20-mu m m imaging resolution provides excellent noise rejection and spatial definition of the Thomson-scattering volume. C1 [Katz, J.; Sorce, C.; Froula, D. H.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Ross, J. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Katz, J (reprint author), Univ Rochester, Laser Energet Lab, 250 E River Rd, Rochester, NY 14623 USA. EM jkat@lle.rochester.edu NR 21 TC 1 Z9 1 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD DEC PY 2013 VL 8 AR C12009 DI 10.1088/1748-0221/8/12/C12009 PG 9 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 292OB UT WOS:000329910500009 ER PT J AU Ruz, J Asner, DM Baker, RG Bundgaard, J Burgett, E Cunningham, M Deaven, J Duke, DL Greife, U Grimes, S Heffner, M Hill, T Isenhower, D Klay, JL Kleinrath, V Kornilov, N Laptev, AB Loveland, W Massey, TN Meharchand, R Qu, H Sangiorgio, S Seilhan, B Snyder, L Stave, S Tatishvili, G Thornton, RT Tovesson, F Towell, D Towell, RS Watson, S Wendt, B Wood, L AF Ruz, J. Asner, D. M. Baker, R. G. Bundgaard, J. Burgett, E. Cunningham, M. Deaven, J. Duke, D. L. Greife, U. Grimes, S. Heffner, M. Hill, T. Isenhower, D. Klay, J. L. Kleinrath, V. Kornilov, N. Laptev, A. B. Loveland, W. Massey, T. N. Meharchand, R. Qu, H. Sangiorgio, S. Seilhan, B. Snyder, L. Stave, S. Tatishvili, G. Thornton, R. T. Tovesson, F. Towell, D. Towell, R. S. Watson, S. Wendt, B. Wood, L. TI The NIFFTE project SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT 3rd International Conference on Micro Pattern Gaseous Detectors CY JUL 01-06, 2013 CL Zaragoza, SPAIN DE Gaseous detectors; Targets (spallation source targets, radioisotope production, neutrino and muon sources); Micropattern gaseous detectors (MSGC, GEM, THGEM, RETHGEM, MHSP, MICROPIC, MICROMEGAS, InGrid, etc); Particle tracking detectors (Gaseous detectors) AB The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) is a doublesided Time Projection Chamber (TPC) with micromegas readout designed to measure the energy-dependent neutron-induced fission cross sections of the major and minor actinides with unprecedented accuracy. The NIFFTE project addresses the challenge of minimizing major sources of systematic uncertainties from previous fission chamber measurements such as: target and beam non-uniformities, misidentification of alpha and light charged particles as fission fragments, and uncertainties inherent to the reference standards used. In-beam tests of the NIFFTE TPC at the Los Alamos Neutron Science Center (LANSCE) started in 2010 and have continued in 2011, 2012 and 2013. An overview of the NIFFTE TPC status and performance at LANSCE will be presented. C1 [Ruz, J.; Cunningham, M.; Heffner, M.; Sangiorgio, S.; Seilhan, B.; Snyder, L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Asner, D. M.; Stave, S.; Tatishvili, G.; Wood, L.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Baker, R. G.; Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Bundgaard, J.; Duke, D. L.; Greife, U.] Colorado Sch Mines, Golden, CO 80401 USA. [Burgett, E.; Deaven, J.; Kleinrath, V.; Wendt, B.] Idaho State Univ, Pocatello, ID 83209 USA. [Grimes, S.; Kornilov, N.; Massey, T. N.] Ohio Univ, Athens, OH 45701 USA. [Hill, T.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Isenhower, D.; Qu, H.; Thornton, R. T.; Towell, D.; Towell, R. S.; Watson, S.] Abilene Christian Univ, Abilene, TX 79699 USA. [Laptev, A. B.; Meharchand, R.; Tovesson, F.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Loveland, W.] Oregon State Univ, Corvallis, OR 97331 USA. RP Ruz, J (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM ruzarmendari1@llnl.gov RI Sangiorgio, Samuele/F-4389-2014; Laptev, Alexander/D-4686-2009; OI Sangiorgio, Samuele/0000-0002-4792-7802; Laptev, Alexander/0000-0002-9759-9907; Geppert-Kleinrath, Verena/0000-0002-6869-5772 NR 7 TC 0 Z9 0 U1 1 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD DEC PY 2013 VL 8 AR C12018 DI 10.1088/1748-0221/8/12/C12018 PG 7 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 292OB UT WOS:000329910500018 ER PT J AU Cherpak, NT Barannik, AA Prozorov, R Tanatar, M Velichko, AV AF Cherpak, N. T. Barannik, A. A. Prozorov, R. Tanatar, M. Velichko, A. V. TI On the determination of the quasiparticle scattering rate in unconventional superconductors by microwave surface impedance SO LOW TEMPERATURE PHYSICS LA English DT Article AB As found from numerous microwave experiments on the unconventional Fe-based superconductors, the temperature dependence of the quasiparticle scattering rate tau(-1) cannot be accurately described within the framework of standard Drude module in the popular approximation of omega tau << 1, where omega is the signal frequency. To account for the discrepancy, we have extended the classical Drude model for the case of arbitrary values of omega tau, and obtained the expression for tau(-1) as a function of experimentally measurable quantities, namely the real and imaginary parts of the microwave surface impedance. We then show the temperature dependence of tau(-1) in superconducting Ba(Fe1-xCox)(2)As-2 single crystal pnictide derived from the Ka-band surface impedance measurements within the framework of the modified expression. The measurements indicate the extent to which assumption of omega tau << 1 gives results different from those obtained without this restriction, i.e., incorrect results. (C) 2013 AIP Publishing LLC. C1 [Cherpak, N. T.; Barannik, A. A.; Velichko, A. V.] Natl Acad Sci Ukraine, A Usikov Inst Radiophys & Elect, UA-61085 Kharkov, Ukraine. [Prozorov, R.; Tanatar, M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Prozorov, R.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Cherpak, NT (reprint author), Natl Acad Sci Ukraine, A Usikov Inst Radiophys & Elect, 12 Acad Proskura Str, UA-61085 Kharkov, Ukraine. EM cherpak@ire.kharkov.ua NR 25 TC 0 Z9 0 U1 1 U2 4 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1063-777X EI 1090-6517 J9 LOW TEMP PHYS+ JI Low Temp. Phys. PD DEC PY 2013 VL 39 IS 12 BP 1110 EP 1112 DI 10.1063/1.4830422 PG 3 WC Physics, Applied SC Physics GA 293NM UT WOS:000329978800016 ER PT J AU Lykken, J Spiropulu, M AF Lykken, Joseph Spiropulu, Maria TI The future of the Higgs boson SO PHYSICS TODAY LA English DT Article ID BROKEN SYMMETRIES; MASSLESS PARTICLES C1 [Lykken, Joseph] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Spiropulu, Maria] CALTECH, Pasadena, CA 91125 USA. RP Lykken, J (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. NR 11 TC 1 Z9 1 U1 1 U2 7 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0031-9228 EI 1945-0699 J9 PHYS TODAY JI Phys. Today PD DEC PY 2013 VL 66 IS 12 BP 28 EP 33 DI 10.1063/PT.3.2212 PG 6 WC Physics, Multidisciplinary SC Physics GA 293NY UT WOS:000329980200013 ER PT J AU McNeil, A Jonsson, CJ Appelfeld, D Ward, G Lee, ES AF McNeil, A. Jonsson, C. J. Appelfeld, D. Ward, G. Lee, E. S. TI A validation of a ray-tracing tool used to generate bi-directional scattering distribution functions for complex fenestration systems SO SOLAR ENERGY LA English DT Article DE Daylighting; Solar heat gain; Complex fenestration systems; Bi-directional scattering distribution function ID REFLECTANCE AB Fenestration attachments are anticipated to produce significant reductions in building energy use because they can be deployed quickly at low-cost. New software tools enable users to assess the building energy impacts of optically complex fenestration systems (CFS) such as shades, Venetian blinds, or daylighting systems. However, such tools require users to provide bi-directional scattering distribution function (BSDF) data that describe the solar-optical performance of the CFS. A free, open-source Radiance tool genBSDF enables users to generate BSDF data for arbitrary CFS. Prior to genBSDF, BSDF data for arbitrary fenestration systems could only be produced using either expensive software or with expensive equipment. genBSDF outputs CFS data in the Window 6 XML file format and so can be used with CFS-enabled software tools to model multi-layered window systems composed of glazing and shading layers. We explain the basis and use of the genBSDF tool and validate the tool by comparing results for four different cases to BSDF data produced via alternate methods. This validation demonstrates that BSDFs created with genBSDF are comparable to BSDFs generated analytically using TracePro and by measurement with a scanning goniophotometer. This tool is expected to support accelerated adoption of fenestration attachments and daylighting technologies. (C) 2013 Elsevier Ltd. All rights reserved. C1 [McNeil, A.; Jonsson, C. J.; Lee, E. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Bldg Technol & Urban Syst Program, Berkeley, CA 94720 USA. [Appelfeld, D.] Tech Univ Denmark, Dept Civil Engn, DK-2800 Lyngby, Denmark. [Ward, G.] Anyhere Software, Berkeley, CA 94708 USA. RP McNeil, A (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS 90-3111, Berkeley, CA 94611 USA. EM amcneil@lbl.gov RI McNeil, Andrew/I-9530-2014 OI McNeil, Andrew/0000-0001-9994-9002 FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State and Community Programs, Office of Building Research; Standards of the US Department of Energy [DE-AC02-05CH11231]; California Energy Commission through its Public Interest Energy Research (PIER) FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State and Community Programs, Office of Building Research and Standards of the US Department of Energy under Contract No. DE-AC02-05CH11231 and by the California Energy Commission through its Public Interest Energy Research (PIER) Program on behalf of the citizens of California. NR 23 TC 16 Z9 16 U1 0 U2 4 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-092X J9 SOL ENERGY JI Sol. Energy PD DEC PY 2013 VL 98 BP 404 EP 414 DI 10.1016/j.solener.2013.09.032 PN C PG 11 WC Energy & Fuels SC Energy & Fuels GA 293EB UT WOS:000329953100024 ER PT J AU Salazar, JM Diwekar, U Constantinescu, E Zavala, VM AF Salazar, Juan M. Diwekar, Urmila Constantinescu, Emil Zavala, Victor M. TI Stochastic optimization approach to water management in cooling-constrained power plants SO APPLIED ENERGY LA English DT Article DE Stochastic optimization; Power plants; Weather forecasting; Uncertainty; Water constraints ID UNIT COMMITMENT; UNCERTAINTY; GENERATION; FRAMEWORK AB A stochastic optimization framework for water management in cooling-constrained power plants is proposed. The approach determines optimal set-points to maximize power output in the presence of uncertain weather conditions and water intake constraints. Weather uncertainty is quantified in the form of ensembles using the state-of-the-art numerical weather prediction model WRF. The framework enables the handling of first-principles black-box simulation models by using the reweighting scheme implemented in the BONUS solver. In addition, it enables the construction of empirical distributions from limited samples obtained from WRF. Using these computational capabilities, the effects of cooling constraints and weather conditions on generation capacity are investigated. In a pulverized coal power plant study it has been found that weather fluctuations make the maximum plant output vary in the range of 5-10% of the nominal capacity in intraday operations. In addition, it has been found that stochastic optimization can lead to daily capacity gains of as much as 245 MW h over current practice and enables more robust bidding procedures. It is demonstrated that reweighting schemes can enable real-time implementations. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Salazar, Juan M.; Diwekar, Urmila] Ctr Uncertain Syst Tools Optimizat & Management, Vishwamitra Res Inst, Argonne, IL 60439 USA. [Constantinescu, Emil; Zavala, Victor M.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Diwekar, U (reprint author), Ctr Uncertain Syst Tools Optimizat & Management, Vishwamitra Res Inst, Clarendon Hills, Argonne, IL 60439 USA. EM urmila@vri-custom.org FU U.S. Department of Energy [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, under Contract No. DE-AC02-06CH11357. The authors thank Argonne National Laboratory's Laboratory Computing Resource Center for use of the Fusion cluster. NR 29 TC 6 Z9 6 U1 0 U2 1 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD DEC PY 2013 VL 112 SI SI BP 12 EP 22 DI 10.1016/j.apenergy.2013.05.077 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 285FA UT WOS:000329377800002 ER PT J AU Breault, RW Huckaby, ED AF Breault, Ronald W. Huckaby, E. David TI Parametric behavior of a CO2 capture process: CFD simulation of solid-sorbent CO2 absorption in a riser reactor SO APPLIED ENERGY LA English DT Article DE CO2 adsorption; Parametric behavior; CFD simulation ID CIRCULATING FLUIDIZED-BED; CARBON-DIOXIDE CAPTURE; FLOWS; TECHNOLOGY; SYSTEM; MODEL; CYCLE AB The National Energy Technology Laboratory as well as other institutions are developing a variety of technology concepts as alternatives to liquid-amine based absorption processes for post-combustion CO2 capture from large sources such as utility power generation facilities. At low temperature, many of these advanced dry processes are based upon sorbents composed of supported polyamines. In the dry-sorbent process, CO2 from flue gas is absorbed in one reactor, followed by separation of the carbonated particles from the de-carbonated flue gas and in a second reactor the sorbent is regenerated, creating a concentrated stream of pure CO2 for sequestration. In this work, the adsorber performance is simulated using multiphase computational fluid dynamics with chemistry and heat transfer. The three-dimension geometry is based on the lower mixing section of a riser from a recently operated CO2 capture test unit. An eight point test matrix was used to explore the behavior and performance of the riser adsorber with respect to solids circulation rate, gas flow rate and heat removal. It is shown that CO2 adsorption increases with an increase in the solids flow, decreases for an increase in the gas flow. The reactor performance can be summarized as a function of the molar sorbent to CO2 ratio entering the reactor with an R-2 value of 0.9985. Published by Elsevier Ltd. C1 [Breault, Ronald W.; Huckaby, E. David] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Breault, RW (reprint author), US DOE, NETL, POB 880, Morgantown, WV 26507 USA. EM ronald.breault@netl.doe.gov OI Breault, Ronald/0000-0002-5552-4050 FU National Energy Technology Laboratory's Advanced Research program through the Carbon Capture Simulation Initiative FX The authors would like to thank Travis Starns and Holly Krutka from ADA for discussions and information about the 1 kW CO2 capture system. The support from the National Energy Technology Laboratory's Advanced Research program through the Carbon Capture Simulation Initiative is gratefully acknowledged. NR 35 TC 13 Z9 13 U1 5 U2 21 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD DEC PY 2013 VL 112 SI SI BP 224 EP 234 DI 10.1016/j.apenergy.2013.06.008 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 285FA UT WOS:000329377800023 ER PT J AU Abeysekara, AU Alfaro, R Alvarez, C Alvarez, JD Arceo, R Arteaga-Velazquez, JC Solares, HAA Barber, AS Baughman, BM Bautista-Elivar, N Belmont, E BenZvi, SY Berley, D Rosales, MB Braun, J Caballero-Lopez, RA Carraminana, A Castillo, M Cotti, U Cotzmi, J de la Fuente, E De Leon, C DeYoung, T Hernandez, RD Diaz-Velez, JC Dingus, BL DuVernois, MA Ellsworth, RW Fernandez, A Fiorino, DW Fraija, N Galindo, A Garcia-Luna, JL Garcia-Torales, G Garfias, F Gonzalez, LX Gonzalez, MM Goodman, JA Grabski, V Gussert, M Hampel-Arias, Z Hui, CM Huentemeyer, P Imran, A Iriarte, A Karn, P Kieda, D Kunde, GJ Lara, A Lauer, RJ Lee, WH Lennarz, D Vargas, HL Linares, EC Linnemann, JT Longo, M Luna-Garcia, R Marinelli, A Martinez, O Martiinez-Castro, J Matthews, JAJ Miranda-Romagnoli, P Moreno, E Mostafa, M Nava, J Nellen, L Newbold, M Noriega-Papaqui, R Oceguera-Becerra, T Patricelli, B Pelayo, R Perez-Perez, EG Pretz, J Riviere, C Ryan, J Rosa-Gonzalez, D Salazar, H Salesa, F Sandoval, A Santos, E Schneider, M Silich, S Sinnis, G Smith, AJ Sparks, K Springer, RW Taboada, I Toale, PA Tollefson, K Torres, I Ukwatta, TN Villasenor, L Weisgarber, T Westerhoff, S Wisher, IG Wood, J Yodh, GB Younk, PW Zaborov, D Zepeda, A Zhou, H AF Abeysekara, A. U. Alfaro, R. Alvarez, C. Alvarez, J. D. Arceo, R. Arteaga-Velazquez, J. C. Solares, H. A. Ayala Barber, A. S. Baughman, B. M. Bautista-Elivar, N. Belmont, E. BenZvi, S. Y. Berley, D. Bonilla Rosales, M. Braun, J. Caballero-Lopez, R. A. Carraminana, A. Castillo, M. Cotti, U. Cotzmi, J. de la Fuente, E. De Leon, C. DeYoung, T. Diaz Hernandez, R. Diaz-Velez, J. C. Dingus, B. L. DuVernois, M. A. Ellsworth, R. W. Fernandez, A. Fiorino, D. W. Fraija, N. Galindo, A. Garcia-Luna, J. L. Garcia-Torales, G. Garfias, F. Gonzalez, L. X. Gonzalez, M. M. Goodman, J. A. Grabski, V. Gussert, M. Hampel-Arias, Z. Hui, C. M. Huentemeyer, P. Imran, A. Iriarte, A. Karn, P. Kieda, D. Kunde, G. J. Lara, A. Lauer, R. J. Lee, W. H. Lennarz, D. Leon Vargas, H. Linares, E. C. Linnemann, J. T. Longo, M. Luna-Garcia, R. Marinelli, A. Martinez, O. Martinez-Castro, J. Matthews, J. A. J. Miranda-Romagnoli, P. Moreno, E. Mostafa, M. Nava, J. Nellen, L. Newbold, M. Noriega-Papaqui, R. Oceguera-Becerra, T. Patricelli, B. Pelayo, R. Perez-Perez, E. G. Pretz, J. Riviere, C. Ryan, J. Rosa-Gonzalez, D. Salazar, H. Salesa, F. Sandoval, A. Santos, E. Schneider, M. Silich, S. Sinnis, G. Smith, A. J. Sparks, K. Springer, R. W. Taboada, I. Toale, P. A. Tollefson, K. Torres, I. Ukwatta, T. N. Villasenor, L. Weisgarber, T. Westerhoff, S. Wisher, I. G. Wood, J. Yodh, G. B. Younk, P. W. Zaborov, D. Zepeda, A. Zhou, H. TI Sensitivity of the high altitude water Cherenkov detector to sources of multi-TeV gamma rays SO ASTROPARTICLE PHYSICS LA English DT Article DE TeV gamma-ray astronomy; Water cherenkov; Cosmic ray ID CRAB-NEBULA; HIGH-ENERGY; MULTIWAVELENGTH OBSERVATIONS; BLAZAR 1ES-1959+650; SUPERNOVA-REMNANTS; GALACTIC PLANE; CYGNUS REGION; EMISSION; MILAGRO; FLARES AB The High Altitude Water Cherenkov (HAWC) observatory is an array of large water Cherenkov detectors sensitive to gamma rays and hadronic cosmic rays in the energy band between 100 GeV and 100 TeV. The observatory will be used to measure high-energy protons and cosmic rays via detection of the energetic secondary particles reaching the ground when one of these particles interacts in the atmosphere above the detector. HAWC is under construction at a site 4100 meters above sea level on the northern slope of the volcano Sierra Negra, which is located in central Mexico at 19 degrees N latitude. It is scheduled for completion in 2014. In this paper we estimate the sensitivity of the HAWC instrument to point-like and extended sources of gamma rays. The source fluxes are modeled using both unbroken power laws and power Jaws with exponential cutoffs. HAWC, in one year, is sensitive to point sources with integral power-law spectra as low as 5 x 10(-13) cm(-2) sec(-1) above 2 TeV (approximately 50 mCrab) over 5 sr of the sky. This is a conservative estimate based on simple event parameters and is expected to improve as the data analysis techniques are refined. We discuss known TeV sources and the scientific contributions that HAWC can make to our understanding of particle acceleration in these sources. (C) 2013 Elsevier B.V. All rights reserved. C1 [Abeysekara, A. U.; Linnemann, J. T.; Tollefson, K.; Ukwatta, T. N.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alfaro, R.; Belmont, E.; Grabski, V.; Leon Vargas, H.; Marinelli, A.; Oceguera-Becerra, T.; Sandoval, A.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 04510, DF, Mexico. [Alvarez, C.; Arceo, R.; Santos, E.] Univ Autonoma Chiapas, CEFyMAP, Chiapas, Mexico. [Alvarez, J. D.; Arteaga-Velazquez, J. C.; Cotti, U.; Linares, E. C.; Villasenor, L.] Univ Michoacana, Morelia, Michoacan, Mexico. [Solares, H. A. Ayala; Hui, C. M.; Huentemeyer, P.] Michigan Technol Univ, Dept Phys, Houghton, MI 49931 USA. [Barber, A. S.; Kieda, D.; Newbold, M.; Springer, R. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT USA. [Baughman, B. M.; Berley, D.; Ellsworth, R. W.; Goodman, J. A.; Smith, A. J.; Wood, J.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Bautista-Elivar, N.; Perez-Perez, E. G.] Univ Politecn Pachuca, Pachuca, Hgo, Mexico. [BenZvi, S. Y.; Diaz-Velez, J. C.; DuVernois, M. A.; Fiorino, D. W.; Hampel-Arias, Z.; Weisgarber, T.; Westerhoff, S.; Wisher, I. G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Bonilla Rosales, M.; Carraminana, A.; Diaz Hernandez, R.; Galindo, A.; Rosa-Gonzalez, D.; Silich, S.] Inst Nacl Astrofis Opt & Electr, Puebla, Mexico. [Caballero-Lopez, R. A.; Gonzalez, L. X.; Lara, A.] Univ Nacl Autonoma Mexico, Inst Geofis, Mexico City 04510, DF, Mexico. [Castillo, M.; Cotzmi, J.; Fernandez, A.; Martinez, O.; Moreno, E.; Pelayo, R.; Salazar, H.] Benemerita Univ Autonoma Puebla, Fac Ciencias Fis Matemat, Puebla, Mexico. [de la Fuente, E.; Garcia-Luna, J. L.; Garcia-Torales, G.; Oceguera-Becerra, T.] Univ Guadalajara, Phys Mat Phd CUVALLES, IT Phd CUCEA, Dept Fis,Dept Elect CUCEI, Guadalajara, Jalisco, Mexico. [DeYoung, T.; Sparks, K.; Zaborov, D.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Dingus, B. L.; Imran, A.; Kunde, G. J.; Pretz, J.; Sinnis, G.; Younk, P. W.] Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA. [Ellsworth, R. W.] George Mason Univ, Sch Phys Astron & Computat Sci, Fairfax, VA 22030 USA. [Fraija, N.; Garfias, F.; Gonzalez, M. M.; Iriarte, A.; Patricelli, B.; Riviere, C.] Univ Nacl Autonoma Mexico, Inst Astron, Mexico City 04510, DF, Mexico. [Gussert, M.; Longo, M.; Mostafa, M.] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. [Karn, P.; Yodh, G. B.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Lauer, R. J.; Matthews, J. A. J.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Lennarz, D.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. 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EM bbaugh@umdgrb.umd.edu; jpretz@lanl.gov OI Caballero, Rogelio/0000-0001-8954-1927; Lara, Alejandro/0000-0001-6336-5291; Dingus, Brenda/0000-0001-8451-7450 FU National Science Foundation; US Department of Energy Office of High-Energy Physics; LDRD program of Los Alamos National Laboratory; Consejo Nacional de Ciencia y Tecnologia [55155, 103520, 105033, 105666, 122331, 132197]; Red de Fisica de Altas Energias; DGAPA-UNAM [IN105211, IN108713, IN121309, IN115409]; VIEP-BUAP [161-EXC-2011]; University of Wisconsin Alumni Research Foundation; Institute of Geophysics and Planetary Physics at Los Alamos National Lab FX We gratefully acknowledge Scott DeLay his dedicated efforts in the construction and maintenance of the HAWC experiment. This work has been supported by: the National Science Foundation, the US Department of Energy Office of High-Energy Physics, the LDRD program of Los Alamos National Laboratory, Consejo Nacional de Ciencia y Tecnologia (Grants 55155, 103520, 105033, 105666, 122331 and 132197), Red de Fisica de Altas Energias, DGAPA-UNAM (Grants IN105211, IN108713 and IN121309, IN115409), VIEP-BUAP (Grant 161-EXC-2011), the University of Wisconsin Alumni Research Foundation, and the Institute of Geophysics and Planetary Physics at Los Alamos National Lab. NR 43 TC 52 Z9 52 U1 0 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD DEC PY 2013 VL 50-52 BP 26 EP 32 DI 10.1016/j.astropartphys.2013.08.002 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 283TX UT WOS:000329271000004 ER PT J AU Abreu, P Aglietta, M Ahlers, M Ahn, EJ Albuquerque, IFM Allekotte, I Allen, J Allison, P Almela, A Castillo, JA Alvarez-Muniz, J Batista, R Ambrosio, M Aminaei, A Anchordoqui, L Andringa, S Anticic, T Aramo, C Arqueros, F Asorey, H Assis, P Aublin, J Ave, M Avenier, M Avila, G Badescu, AM Barber, KB Barbosa, AF Bardenet, R Baughman, B Bauml, J Baus, C Beatty, JJ Becker, KH Belletoile, A Bellido, JA BenZvi, S Berat, C Bertou, X Biermann, PL Billoir, P Blanco, F Blanco, M Bleve, C Blumer, H Bohacova, M Boncioli, D Bonifazi, C Bonino, R Borodai, N Brack, J Brancus, I Brogueira, P Brown, WC Buchholz, P Bueno, A Buroker, L Burton, RE Buscemi, M Caballero-Mora, KS Caccianiga, B Caccianiga, L Caramete, L Caruso, R Castellina, A Cataldi, G Cazon, L Cester, R Cheng, SH Chiavassa, A Chinellato, JA Chirinos, J Chudoba, J Cilmo, M Clay, RW Cocciolo, G Colalillo, R Collica, L Coluccia, MR Conceicao, R Contreras, F Cook, H Cooper, MJ Coutu, S Covault, CE Criss, A Cronin, J Curutiu, A Dallier, R Daniel, B Dasso, S Daumiller, K Dawson, BR de Almeida, RM De Domenico, M de Jong, SJ De La Vega, G de Mello, WJM Neto, JRTD De Mitri, I de Souza, V de Vries, KD del Peral, L Deligny, O Dembinski, H Dhital, N Di Giulio, C Diaz, JC Castro, MLD Diep, PN Diogo, F Dobrigkeit, C Docters, W D'Olivo, JC Dong, PN Dorofeev, A dos Anjos, JC Dova, MT D'Urso, D Ebr, J Engel, R Erdmann, M Escobar, CO Espadanal, J Etchegoyen, A San Luis, PF Falcke, H Fang, K Farrar, G Fauth, AC Fazzini, N Ferguson, AP Fick, B Figueira, JM Filevich, A Filipcic, A Fliescher, S Fox, BD Fracchiolla, CE Fraenkel, ED Fratu, O Frohlich, U Fuchs, B Gaior, R Gamarra, RF Gambetta, S Garcia, B Roca, STG Garcia-Gamez, D Garcia-Pinto, D Garilli, G Bravo, AG Gemmeke, H Ghia, PL Giller, M Gitto, J Glaser, C Glass, H Golup, G Albarracin, FG Berisso, MG Vitale, PFG Goncalves, P Gonzalez, JG Gookin, B Gorgi, A Gorham, P Gouffon, P Grebe, S Griffith, N Grillo, AF Grubb, TD Guardincerri, Y Guarino, F Guedes, GP Hansen, P Harari, D Harrison, TA Harton, JL Haungs, A Hebbeker, T Heck, D Herve, AE Hill, GC Hojvat, C Hollon, N Holmes, VC Homola, P Horandel, JR Horvath, P Hrabovsky, M Huber, D Huege, T Insolia, A Jansen, S Jarne, C Jiraskova, S Josebachuili, M Kadija, K Kampert, KH Karhan, P Kasper, P Katkov, I Kegl, B Keilhauer, B Keivani, A Kelley, JL Kemp, E Kieckhafer, RM Klages, HO Kleifges, M Kleinfeller, J Knapp, J Krause, R Krohm, N Kromer, O Kruppke-Hansen, D Kuempel, D Kulbartz, JK Kunka, N La Rosa, G LaHurd, D Latronico, L Lauer, R Lauscher, M Lautridou, P Le Coz, S Leao, MSAB Lebrun, D Lebrun, P de Oliveira, MAL Letessier-Selvon, A Lhenry-Yvon, I Link, K Lopez, R Aguera, AL Louedec, K Bahilo, JL Lu, L Lucero, A Ludwig, M Lyberis, H Maccarone, MC Macolino, C Malacari, M Maldera, S Maller, J Mandat, D Mantsch, P Mariazzi, AG Marin, J Marin, V Maris, IC Falcon, HRM Marsella, G Martello, D Martin, L Martinez, H Bravo, OM Martraire, D Meza, JJM Mathes, HJ Matthews, J Matthews, JAJ Matthiae, G Maurel, D Maurizio, D Mayotte, E Mazur, PO Medina-Tanco, G Melissas, M Melo, D Menichetti, E Menshikov, A Messina, S Meyhandan, R Micanovic, S Micheletti, MI Middendorf, L Minaya, IA Mirarrionti, L Mitrica, B Molina-Bueno, L Mollerach, S Monasor, M Ragaigne, DM Montanet, F Morales, B Morello, C Moreno, JC Mostafa, M Moura, CA Muller, MA Muller, G Munchmeyer, M Mussa, R Navarra, G Navarro, JL Navas, S Necesal, P Nellen, L Nelles, A Neuser, TJ Nhung, PT Niechciol, M Niemietz, L Nierstenhoefer, N Niggemann, T Nitz, D Nosek, D Nozka, L Oehlschlager, J Olinto, A Oliveira, M Ortiz, M Pacheco, N Selmi-Dei, DP Palatka, M Pallotta, J Palmieri, N Parente, G Parra, A Pastor, S Paul, T Pech, M Pekala, J Pelayo, R Pepe, IM Perrone, L Pesce, R Petermann, E Petrera, S Petrolini, A Petrov, Y Pfendner, C Piegaia, R Pierog, T Pieroni, P Pimenta, M Pirronello, V Platino, M Plum, M Ponce, VH Pontz, M Porcelli, A Privitera, P Prouza, M Quel, EJ Querchfeld, S Rautenberg, J Ravel, O Ravignani, D Revenu, B Ridky, J Riggi, S Risse, M Ristori, P Rivera, H Rizi, V Roberts, J de Carvalho, WR Cabo, IR Fernandez, GR Martino, JR Rojo, JR Rodriguez-Frias, MD Ros, G Rosado, J Rossler, T Roth, M Rouille-d'Orfeuil, B Roulet, E Rovero, AC Ruhle, C Saffi, SJ Saftoiu, A Salamida, F Salazar, H Greus, FS Salina, G Sanchez, F Santo, CE Santos, E Santos, EM Sarazin, F Sarkar, B Sato, R Scharf, N Scherini, V Schieler, H Schiffer, P Schmidt, A Scholten, O Schoorlemmer, H Schovancova, J Schovanek, P Schroder, FG Schulz, J Schuster, D Sciutto, S Scuderi, M Segreto, A Settimo, M Shadkam, A Shellard, RC Sidelnik, I Sigl, G Sima, O Smialkowski, A Smida, R Snow, GR Sommers, P Sorokin, J Spinka, H Squartini, R Srivastava, YN Stanic, S Stapleton, J Stasielak, J Stephan, M Straub, M Stutz, A Suarez, F Suomijarvi, T Supanitsky, AD Susa, T Sutherland, MS Swain, J Szadkowski, Z Szuba, M Tapia, A Tartare, M Tascau, O Tcaciuc, R Thao, NT Thomas, D Tiffenberg, J Timmermans, C Tkaczyk, W Peixoto, CJT Toma, G Tomankova, L Tome, B Tonachini, A Elipe, GT Machado, DT Travnicek, P Tridapalli, DB Trovato, E Tueros, M Ulrich, R Unger, M Urban, M Galicia, JFV Valino, I Valore, L van Aar, G van den Berg, AM van Velzen, S van Vliet, A Varela, E Cardenas, BV Varner, G Vazquez, JR Vazquez, RA Veberic, D Verzi, V Vicha, J Videla, M Villasenor, L Wahlberg, H Wahrlich, P Wainberg, O Walz, D Watson, AA Weber, M Weidenhaupt, K Weindl, A Werner, F Westerhoff, S Whelan, BJ Widom, A Wieczorek, G Wiencke, L Wilczynska, B Wilczynski, H Will, M Williams, C Winchen, T Wundheiler, B Yamamoto, T Yapici, T Younk, P Yuan, G Yushkov, A Garcia, BZ Zas, E Zavrtanik, D Zavrtanik, M Zaw, I Zepeda, A Zhou, J Zhu, Y Silva, MZ Ziolkowski, M AF Abreu, P. 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Coluccia, M. R. Conceicao, R. Contreras, F. Cook, H. Cooper, M. J. Coutu, S. Covault, C. E. Criss, A. Cronin, J. Curutiu, A. Dallier, R. Daniel, B. Dasso, S. Daumiller, K. Dawson, B. R. de Almeida, R. M. De Domenico, M. de Jong, S. J. De La Vega, G. de Mello, W. J. M., Jr. de Mello Neto, J. R. T. De Mitri, I. de Souza, V. de Vries, K. D. del Peral, L. Deligny, O. Dembinski, H. Dhital, N. Di Giulio, C. Diaz, J. C. Diaz Castro, M. L. Diep, P. N. Diogo, F. Dobrigkeit, C. Docters, W. D'Olivo, J. C. Dong, P. N. Dorofeev, A. dos Anjos, J. C. Dova, M. T. D'Urso, D. Ebr, J. Engel, R. Erdmann, M. Escobar, C. O. Espadanal, J. Etchegoyen, A. San Luis, P. Facal Falcke, H. Fang, K. Farrar, G. Fauth, A. C. Fazzini, N. Ferguson, A. P. Fick, B. Figueira, J. M. Filevich, A. Filipcic, A. Fliescher, S. Fox, B. D. Fracchiolla, C. E. Fraenkel, E. D. Fratu, O. Froehlich, U. Fuchs, B. Gaior, R. Gamarra, R. F. Gambetta, S. Garcia, B. Garcia Roca, S. T. Garcia-Gamez, D. Garcia-Pinto, D. Garilli, G. 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Valore, L. van Aar, G. van den Berg, A. M. van Velzen, S. van Vliet, A. Varela, E. Vargas Cardenas, B. Varner, G. Vazquez, J. R. Vazquez, R. A. Veberic, D. Verzi, V. Vicha, J. Videla, M. Villasenor, L. Wahlberg, H. Wahrlich, P. Wainberg, O. Walz, D. Watson, A. A. Weber, M. Weidenhaupt, K. Weindl, A. Werner, F. Westerhoff, S. Whelan, B. J. Widom, A. Wieczorek, G. Wiencke, L. Wilczynska, B. Wilczynski, H. Will, M. Williams, C. Winchen, T. Wundheiler, B. Yamamoto, T. Yapici, T. Younk, P. Yuan, G. Yushkov, A. Zamorano Garcia, B. Zas, E. Zavrtanik, D. Zavrtanik, M. Zaw, I. Zepeda, A. Zhou, J. Zhu, Y. Zimbres Silva, M. Ziolkowski, M. CA Pierre Auger Collaboration TI Identifying clouds over the Pierre Auger Observatory using infrared satellite data SO ASTROPARTICLE PHYSICS LA English DT Article DE Ultra-high energy cosmic rays; Pierre Auger Observatory; Extensive air showers; Atmospheric monitoring; Clouds; Satellites ID DETECTOR; SYSTEM AB We describe a new method of identifying night-time clouds over the Pierre Auger Observatory using infrared data from the Imager instruments on the GOES-12 and GOES-13 satellites. We compare cloud. identifications resulting from our method to those obtained by the Central Laser Facility of the Auger Observatory. Using our new method we can now develop cloud probability maps for the 3000 km(2) of the Pierre Auger Observatory twice per hour with a spatial resolution of similar to 2.4 km by similar to 5.5 km. Our method could also be applied to monitor cloud cover for other ground-based observatories and for space-based observatories. (C) 2013 Elsevier B.V. All rights reserved. C1 [Allekotte, I.; Asorey, H.; Bertou, X.; Golup, G.; Gomez Berisso, M.; Harari, D.; Mollerach, S.; Ponce, V. H.; Roulet, E.; Sidelnik, I.] Ctr Atom Bariloche, San Carlos De Bariloche, Rio Negro, Argentina. [Allekotte, I.; Asorey, H.; Bertou, X.; Golup, G.; Gomez Berisso, M.; Harari, D.; Mollerach, S.; Ponce, V. H.; Roulet, E.; Sidelnik, I.] CNEA UNCuyo CONICET, Inst Balseiro, San Carlos De Bariloche, Rio Negro, Argentina. [Dasso, S.; Guardincerri, Y.; Masias Meza, J. J.; Piegaia, R.; Pieroni, P.; Tiffenberg, J.] Consejo Nacl Invest Cient & Tecn, RA-1033 Buenos Aires, DF, Argentina. [Dasso, S.; Guardincerri, Y.; Piegaia, R.; Pieroni, P.; Tiffenberg, J.] Univ Buenos Aires, FCEyN, Dept Fis, RA-1053 Buenos Aires, DF, Argentina. [Dova, M. T.; Gomez Albarracin, F.; Jarne, C.; Kruppke-Hansen, D.; Mariazzi, A. G.; Moreno, J. C.; Sciutto, Si.; Wahlberg, H.] Univ Nacl La Plata, IFLP, La Plata, Buenos Aires, Argentina. [Dova, M. T.; Gomez Albarracin, F.; Hansen, P.; Jarne, C.; Mariazzi, A. G.; Sciutto, Si.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Dasso, S.; Rovero, A. C.; Supanitsky, A. D.] CONICET UBA, Inst Astron & Fis Espacio, Buenos Aires, DF, Argentina. [Micheletti, M. I.] CONICET UNR, Inst Fis Rosario IFIR, Rosario, Santa Fe, Argentina. [Micheletti, M. I.] Fac Ciencias Bioquim & Farmaceut UNR, Rosario, Santa Fe, Argentina. [Almela, A.; Etchegoyen, A.; Figueira, J. M.; Filevich, A.; Gamarra, R. F.; Josebachuili, M.; Lucero, A.; Melo, D.; Platino, M.; Ravignani, D.; Sanchez, F.; Schroeder, F. G.; Suarez, F.; Tapia, A.; Wainberg, O.; Wundheiler, B.] CNEA CONICET UNSAM, Inst Tecnol Detecc & Astroparticulas, Buenos Aires, DF, Argentina. [De La Vega, G.; Garcia, B.; Gitto, J.; Videla, M.] Natl Technol Univ, Fac Mendoza, CONICET CNEA, Mendoza, Argentina. [Avila, G.; Contreras, F.; Gomez Vitale, P. F.; Kleinfeller, J.; Marin, J.; Rodriguez Martino, J.; Rodriguez Rojo, J.; Sato, R.; Squartini, R.] Observ Pierre Auger, Malargue, Argentina. [Avila, G.; Gomez Vitale, P. F.] Comis Nacl Energia Atom, Malargue, Argentina. [Almela, A.; Etchegoyen, A.; Wainberg, O.] Univ Tecnol Nacl, Fac Reg Buenos Aires, Buenos Aires, DF, Argentina. [Barber, K. B.; Bellidol, J. A.; Clay, R. W.; Cooper, M. J.; Dawson, B. R.; Grubb, T. D.; Harrison, T. A.; Herve, A. E.; Hill, G. C.; Holmes, V. C.; Malacari, M.; Saffi, S. J.; Sorokin, J.; Wahrlich, P.] Univ Adelaide, Adelaide, SA, Australia. [Barbosa, A. F.; Diaz Castro, M. L.; dos Anjos, J. C.; Maurizio, D.; Shellard, R. C.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, RJ, Brazil. [de Souza, V.; Todero Peixoto, C. J.] Univ Sao Paulo, Inst Fis, Sao Carlos, SP, Brazil. [Albuquerque, I. F. M.; Gouffon, P.; Tridapalli, D. B.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Chinellato, J. A.; Daniel, B.; de Mello, W. J. M., Jr.; Dobrigkeit, C.; Escobar, C. O.; Fauth, A. C.; Goncalves, P.; Kemp, E.; Muller, M. A.; Pakk Selmi-Dei, D.; Zimbres Silva, M.] Univ Estadual Campinas, IFGW, Campinas, SP, Brazil. [Pepe, I. M.] Univ Fed Bahia, Salvador, BA, Brazil. [Leao, M. S. A. B.; Leigui de Oliveira, M. A.; Moura, C. A.] Univ Fed ABC, Santo Andre, SP, Brazil. [Bonifazi, C.; de Mello Neto, J. R. T.; Lyberis, H.; Santos, E. M.] Univ Fed Rio de Janeiro, Inst Fis, Rio De Janeiro, RJ, Brazil. [de Almeida, R. M.] Univ Fed Fluminense, EEIMVR, Volta Redonda, RJ, Brazil. [Anticic, T.; Kadija, K.; Micanovic, S.; Susa, T.] Rudjer Boskovic Inst, Zagreb 10000, Croatia. [Karhan, P.; Nosek, D.] Charles Univ Prague, Fac Math & Phys, Inst Particle & Nucl Phys, Prague, Czech Republic. [Bohacova, M.; Chudoba, J.; Ebr, J.; Hrabovsky, M.; Mandat, D.; Necesal, P.; Nozka, L.; Palatka, M.; Pech, M.; Prouza, M.; Ridky, J.; Schovancova, J.; Travnicek, P.; Vicha, J.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Horvath, P.; Hrabovsky, M.; Rossler, T.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Deligny, O.; Dong, P. N.; Lhenry-Yvon, I.; Lyberis, H.; Martraire, D.; Salamida, F.; Suomijaervi, T.] Univ Paris 11, CNRS, Inst Phys Nucl Orsay, IN2P3, F-91405 Orsay, France. [Bardenet, R.; Garcia-Gamez, D.; Kegl, B.; Louedec, K.; Ragaigne, D. Monnier; Urban, M.] Univ Paris 11, CNRS, Lab Accelerateur Lineaire, IN2P3, Paris, France. [Aublin, J.; Billoir, P.; Blanco, M.; Caccianiga, L.; Gaior, R.; Ghia, P. L.; Letessier-Selvon, A.; Macolino, C.; Maris, I. C.; Muenchmeyer, M.] Univ Paris 06, Lab Phys Nucl & Hautes Energies, Paris, France. [Aublin, J.; Billoir, P.; Blanco, M.; Caccianiga, L.; Gaior, R.; Ghia, P. L.; Letessier-Selvon, A.; Macolino, C.; Maris, I. C.; Muenchmeyer, M.] Univ Paris 07, CNRS, IN2P3, Paris, France. [Avenier, M.; Berat, C.; Le Coz, S.; Lebrun, D.; Louedec, K.; Montanet, F.; Stutz, A.; Tartare, M.] Univ Grenoble 1, CNRS, Grenoble INP, Lab Phys Subatom & Cosmol,IN2P3, F-38041 Grenoble, France. [Dallier, R.; Martin, L.] CNRS INSU, Observ Paris, Stn Radioastron Nancay, Paris, France. [Belletoile, A.; Dallier, R.; Lautridou, P.; Maller, J.; Marin, V.; Martin, L.; Ravel, O.; Revenu, B.; Machado, D. Torres] Univ Nantes, CNRS, IN2P3, Subatech,Ecole Mines Nantes, Nantes, France. [Becker, K. H.; Bleve, C.; Kampert, K. H.; Krohm, N.; Kruppke-Hansen, D.; Neuser, T. J.; Niemietz, L.; Nierstenhoefer, N.; Querchfeld, S.; Rautenberg, J.; Sarkar, B.; Tascau, O.; Zimbres Silva, M.] Berg Univ Wuppertal, Wuppertal, Germany. [Baeuml, J.; Bluemer, H.; Daumiller, K.; Dembinski, H.; Engel, R.; Figueira, J. M.; Haungs, A.; Heck, D.; Huege, T.; Josebachuili, M.; Keilhauer, B.; Klages, H. O.; Kleinfeller, J.; Mathes, H. J.; Maurel, D.; Oehlschlaeger, J.; Pierog, T.; Porcelli, A.; Roth, M.; Schieler, H.; Schroeder, F. G.; Smida, R.; Szuba, M.; Tomankova, L.; Ulrich, R.; Unger, M.; Weindl, A.; Werner, F.; Will, M.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Gemmeke, H.; Kleifges, M.; Kroemer, O.; Kunka, N.; Menshikov, A.; Ruehle, C.; Schmidt, A.; Weber, M.; Zhu, Y.] Karlsruhe Inst Technol, Inst Prozessdatenverarbeitung & Elekt, D-76021 Karlsruhe, Germany. [Baus, C.; Bluemer, H.; Fuchs, B.; Gonzalez, J. G.; Huber, D.; Katkov, I.; Link, K.; Ludwig, M.; Melissas, M.; Palmieri, N.] Karlsruhe Inst Technol, Inst Expt Kernphys IEKP, D-76021 Karlsruhe, Germany. [Biermann, P. L.; Caramete, L.; Curutiu, A.] Max Planck Inst Radioastron, D-53121 Bonn, Germany. [Erdmann, M.; Fliescher, S.; Glaser, C.; Hebbeker, T.; Krause, R.; Kuempel, D.; Lauscher, M.; Middendorf, L.; Mueller, G.; Niggemann, T.; Plum, M.; Scharf, N.; Stephan, M.; Straub, M.; Walz, D.; Weidenhaupt, K.; Winchen, T.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Kulbartz, J. K.; Schiffer, P.; Sigl, G.; van Vliet, A.] Univ Hamburg, Hamburg, Germany. [Buchholz, P.; Froehlich, U.; Niechciol, M.; Pontz, M.; Settimo, M.; Tcaciuc, R.; Younk, P.; Ziolkowski, M.] Univ Siegen, D-57068 Siegen, Germany. [Gambetta, S.; Pesce, R.; Petrolini, A.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Gambetta, S.; Pesce, R.; Petrolini, A.] Ist Nazl Fis Nucl, I-16146 Genoa, Italy. [Petrera, S.; Rizi, V.] Univ Aquila, I-67100 Laquila, Italy. [Petrera, S.; Rizi, V.] INFN, Laquila, Italy. [Caccianiga, B.; Collica, L.; Rivera, H.; Scherini, V.] Univ Milan, Milan, Italy. [Caccianiga, B.; Collica, L.; Mirarrionti, L.; Rivera, H.; Scherini, V.] Sezione Ist Nazl Fis Nucl, Milan, Italy. [Ambrosio, M.; Aramo, C.; Buscemi, M.; Cilmo, M.; Colalillo, R.; D'Urso, D.; Guarino, F.; Valore, L.] Univ Naples Federico II, Naples, Italy. [Ambrosio, M.; Aramo, C.; Buscemi, M.; Cilmo, M.; Colalillo, R.; D'Urso, D.; Guarino, F.; Valore, L.] Sezione Ist Nazl Fis Nucl, Naples, Italy. [Boncioli, D.; Di Giulio, C.; Matthiae, G.; Fernandez, G. Rodriguez; Salina, G.; Verzi, V.] Univ Roma Tor Vergata, I-00173 Rome, Italy. [Boncioli, D.; Di Giulio, C.; Filevich, A.; Matthiae, G.; Fernandez, G. Rodriguez; Salina, G.; Verzi, V.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Caruso, R.; De Domenico, M.; Garilli, G.; Insolia, A.; Pirronello, V.; Scuderi, M.; Trovato, E.] Univ Catania, Catania, Italy. [Caruso, R.; De Domenico, M.; Garilli, G.; Insolia, A.; Pirronello, V.; Scuderi, M.; Trovato, E.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Cester, R.; Maurizio, D.; Menichetti, E.; Mussa, R.; Tonachini, A.] Univ Turin, Turin, Italy. [Cester, R.; Maurizio, D.; Menichetti, E.; Mussa, R.; Tonachini, A.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Cataldi, G.; Cocciolo, G.; Coluccia, M. R.; De Mitri, I.; Marsella, G.; Martello, D.; Perrone, L.; Settimo, M.] E De Giorgi Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Cataldi, G.; Cocciolo, G.; Coluccia, M. R.; De Mitri, I.; Marsella, G.; Martello, D.; Perrone, L.; Settimo, M.] Sezione Ist Nazl Fis Nucl, Lecce, Italy. [La Rosa, G.; Maccarone, M. C.; Riggi, S.; Segreto, A.] Ist Astrofis Spaziale & Fis Cosm Palermo INAF, Palermo, Italy. [Aglietta, M.; Bonino, R.; Castellina, A.; Chiavassa, A.; Gorgi, A.; Latronico, L.; Lucero, A.; Maldera, S.; Marin, J.; Morello, C.; Navarra, G.] Univ Turin, Ist Fis Spazio Interplanetario INAF, Turin, Italy. [Grillo, A. F.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Laquila, Italy. [Lopez, R.; Martinez Bravo, O.; Pelayo, R.; Salazar, H.; Varela, E.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Martinez, H.; Zepeda, A.] Ctr Invest & Estudios Avanzados IPN CINVESTAV, Mexico City, DF, Mexico. [Marquez Falcon, H. R.; Villasenor, L.] Univ Michoacana, Morelia, Michoacan, Mexico. [Alvarez Castillo, J.; D'Olivo, J. C.; Medina-Tanco, G.; Nellen, L.; Valdes Galicia, J. F.; Vargas Cardenas, B.] Univ Nacl Autonoma Mexico, Mexico City 04510, DF, Mexico. [Aminaei, A.; de Jong, S. J.; Falcke, H.; Grebe, S.; Horandel, J. R.; Jansen, S.; Jiraskova, S.; Kelley, J. L.; Nelles, A.; Schoorlemmer, H.; Schulz, J.; Timmermans, C.; van Aar, G.; van Velzen, S.] Radboud Univ Nijmegen, IMAPP, NL-6525 ED Nijmegen, Netherlands. [de Vries, K. D.; Docters, W.; Fraenkel, E. D.; Messina, S.; Scholten, O.; van den Berg, A. M.] Univ Groningen, Kernfys Versneller Inst, Groningen, Netherlands. [de Jong, S. J.; Falcke, H.; Grebe, S.; Horandel, J. R.; Jansen, S.; Nelles, A.; Schoorlemmer, H.; Timmermans, C.] Nikhef, Amsterdam, Netherlands. [Falcke, H.] ASTRON, Dwingeloo, Netherlands. [Borodai, N.; Homola, P.; Pekala, J.; Stasielak, J.; Wilczynska, B.; Wilczynski, H.] Inst Nucl Phys PAN, Krakow, Poland. [Giller, M.; Smialkowski, A.; Szadkowski, Z.; Tkaczyk, W.; Wieczorek, G.] Univ Lodz, PL-90131 Lodz, Poland. [Abreu, P.; Andringa, S.; Assis, P.; Brogueira, P.; Cazon, L.; Conceicao, R.; Diogo, F.; Espadanal, J.; Goncalves, P.; Oliveira, M.; Pimenta, M.; Santo, C. E.; Santos, E.; Tome, B.] Univ Tecn Lisboa, LIP, P-1100 Lisbon, Portugal. [Abreu, P.; Andringa, S.; Assis, P.; Brogueira, P.; Cazon, L.; Conceicao, R.; Diogo, F.; Espadanal, J.; Goncalves, P.; Oliveira, M.; Santo, C. E.; Santos, E.; Tome, B.] Univ Tecn Lisboa, Inst Super Tecn, P-1100 Lisbon, Portugal. [Brancus, I.; Mitrica, B.; Saftoiu, A.; Toma, G.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Sima, O.] Univ Bucharest, Dept Phys, Bucharest, Romania. [Badescu, A. M.; Fratu, O.] Univ Politehn Bucuresti, Bucharest, Romania. [Filipcic, A.; Zavrtanik, D.] J Stefan Inst, Ljubljana, Slovenia. [Pastor, S.] Univ Valencia, Inst Fis Corpuscular, CSIC, Valencia, Spain. [Arqueros, F.; Blanco, F.; Garcia-Pinto, D.; Minaya, I. A.; Ortiz, M.; Rosado, J.; Vazquez, J. R.] Univ Complutense Madrid, Madrid, Spain. [del Peral, L.; Pacheco, N.; Rodriguez-Frias, M. D.; Ros, G.] Univ Alcala de Henares, Alcala De Henares, Madrid, Spain. [Bueno, A.; Gascon Bravo, A.; Lozano Bahilo, J.; Molina-Bueno, L.; Navarro, J. L.; Navas, S.; Zamorano Garcia, B.] Univ Granada, Granada, Spain. [Bueno, A.; Gascon Bravo, A.; Lozano Bahilo, J.; Molina-Bueno, L.; Navarro, J. L.; Navas, S.; Zamorano Garcia, B.] CAFPE, Granada, Spain. [Alvarez-Muniz, J.; Ave, M.; Caballero-Mora, K. S.; Garcia Roca, S. T.; Lopez Agueera, A.; Parente, G.; Parra, A.; Pelayo, R.; Riggi, S.; Rodrigues de Carvalho, W.; Rodriguez Cabo, I.; Fernandez, G. Rodriguez; Torralba Elipe, G.; Tueros, M.; Valino, I.; Vazquez, R. A.; Yushkov, A.; Zas, E.] Univ Santiago Compostela, Santiago De Compostela, Spain. [Cook, H.; Knapp, J.; Lu, L.; Watson, A. A.] Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. [Spinka, H.] Argonne Natl Lab, Argonne, IL 60439 USA. [Burton, R. E.; Covault, C. E.; Ferguson, A. P.; LaHurd, D.] Case Western Reserve Univ, Cleveland, OH 44106 USA. [Mayotte, E.; Sarazin, F.; Schuster, D.; Wiencke, L.] Colorado Sch Mines, Golden, CO 80401 USA. [Brack, J.; Dorofeev, A.; Fracchiolla, C. E.; Gookin, B.; Harton, J. L.; Mostafa, M.; Petrov, Y.; Greus, F. Salesa; Thomas, D.] Colorado State Univ, Ft Collins, CO 80523 USA. [Brown, W. C.] Colorado State Univ, Pueblo, CO USA. [Ahn, E. J.; Escobar, C. O.; Fazzini, N.; Glass, H.; Hojvat, C.; Kasper, P.; Lebrun, P.; Mantsch, P.; Mazur, P. O.; Spinka, H.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Younk, P.] Los Alamos Natl Lab, Los Alamos, NM USA. [Keivani, A.; Matthews, J.; Shadkam, A.; Sutherland, M. S.; Yuan, G.] Louisiana State Univ, Baton Rouge, LA 70803 USA. [Chirinos, J.; Dhital, N.; Diaz, J. C.; Fick, B.; Kieckhafer, R. M.; Nitz, D.; Yapici, T.] Michigan Technol Univ, Houghton, MI 49931 USA. [Allen, J.; Farrar, G.; Roberts, J.; Zaw, I.] NYU, New York, NY USA. [Paul, T.; Srivastava, Y. N.; Swain, J.; Widom, A.] Northeastern Univ, Boston, MA 02115 USA. [Allison, P.; Baughman, B.; Beatty, J. J.; Griffith, N.; Stapleton, J.] Ohio State Univ, Columbus, OH 43210 USA. [Caballero-Mora, K. S.; Cheng, S. H.; Coutu, S.; Criss, A.; Sommers, P.; Whelan, B. J.] Penn State Univ, University Pk, PA 16802 USA. [Cronin, J.; San Luis, P. Facal; Fang, K.; Hollon, N.; Monasor, M.; Olinto, A.; Privitera, P.; Rouille-d'Orfeuil, B.; Williams, C.; Yamamoto, T.; Zhou, J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Fox, B. D.; Gorham, P.; Meyhandan, R.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Petermann, E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Lauer, R.; Matthews, J. A. J.] Univ New Mexico, Albuquerque, NM 87131 USA. [Ahlers, M.; BenZvi, S.; Pfendner, C.; Westerhoff, S.] Univ Wisconsin, Madison, WI USA. [Anchordoqui, L.; Buroker, L.; Paul, T.] Univ Wisconsin, Milwaukee, WI 53201 USA. [Diep, P. N.; Dong, P. N.; Nhung, P. T.; Thao, N. T.] Inst Nucl Sci & Technol, Hanoi, Vietnam. RP Chirinos, J (reprint author), Michigan Technol Univ, Houghton, MI 49931 USA. RI Beatty, James/D-9310-2011; Guarino, Fausto/I-3166-2012; Buscemi, Mario/R-5071-2016; Colalillo, Roberta/R-5088-2016; Bonino, Raffaella/S-2367-2016; Rodriguez Frias, Maria /A-7608-2015; Inst. of Physics, Gleb Wataghin/A-9780-2017; De Mitri, Ivan/C-1728-2017; Mitrica, Bogdan/D-5201-2009; Rodriguez Fernandez, Gonzalo/C-1432-2014; Nosek, Dalibor/F-1129-2017; scuderi, mario/O-7019-2014; Blanco, Francisco/F-1131-2015; zas, enrique/I-5556-2015; Moura Santos, Edivaldo/K-5313-2016; Gouffon, Philippe/I-4549-2012; de Almeida, Rogerio/L-4584-2016; De Domenico, Manlio/B-5826-2014; Abreu, Pedro/L-2220-2014; Navas, Sergio/N-4649-2014; Assis, Pedro/D-9062-2013; Sao Carlos Institute of Physics, IFSC/USP/M-2664-2016; Conceicao, Ruben/L-2971-2014; dos Santos, Eva/N-6351-2013; Alvarez-Muniz, Jaime/H-1857-2015; de souza, Vitor/D-1381-2012; Valino, Ines/J-8324-2012; Carvalho Jr., Washington/H-9855-2015; Espadanal, Joao/I-6618-2015; Vazquez, Jose Ramon/K-2272-2015; Martello, Daniele/J-3131-2012; Insolia, Antonio/M-3447-2015; Petrolini, Alessandro/H-3782-2011; de Mello Neto, Joao/C-5822-2013; Lozano-Bahilo, Julio/F-4881-2016; Pimenta, Mario/M-1741-2013; Chinellato, Carola Dobrigkeit /F-2540-2011; Ros, German/L-4764-2014; Brogueira, Pedro/K-3868-2012; Alves Batista, Rafael/K-6642-2012; Sima, Octavian/C-3565-2011; Torralba Elipe, Guillermo/A-9524-2015; Di Giulio, Claudio/B-3319-2015; Chinellato, Jose Augusto/I-7972-2012; Bueno, Antonio/F-3875-2015; Parente, Gonzalo/G-8264-2015; Travnicek, Petr/G-8814-2014; Smida, Radomir/G-6314-2014; Ridky, Jan/H-6184-2014; Chudoba, Jiri/G-7737-2014; Horvath, Pavel/G-6334-2014; Garcia Pinto, Diego/J-6724-2014; Pastor, Sergio/J-6902-2014; Tome, Bernardo/J-4410-2013; Rosado, Jaime/K-9109-2014; Arqueros, Fernando/K-9460-2014; Espirito Santo, Maria Catarina/L-2341-2014; Todero Peixoto, Carlos Jose/G-3873-2012; Badescu, Alina/B-6087-2012; Cazon, Lorenzo/G-6921-2014; Schovanek, Petr/G-7117-2014; Ebr, Jan/H-8319-2012; Fauth, Anderson/F-9570-2012; Caramete, Laurentiu/C-2328-2011; Prouza, Michael/F-8514-2014; Mandat, Dusan/G-5580-2014; Pech, Miroslav/G-5760-2014; Bohacova, Martina/G-5898-2014; Nozka, Libor/G-5550-2014; Vicha, Jakub/G-8440-2014; OI de Jong, Sijbrand/0000-0002-3120-3367; Sigl, Guenter/0000-0002-4396-645X; Aramo, Carla/0000-0002-8412-3846; Cataldi, Gabriella/0000-0001-8066-7718; Segreto, Alberto/0000-0001-7341-6603; La Rosa, Giovanni/0000-0002-3931-2269; Ravignani, Diego/0000-0001-7410-8522; Matthews, James/0000-0002-1832-4420; Rizi, Vincenzo/0000-0002-5277-6527; Goncalves, Patricia /0000-0003-2042-3759; Beatty, James/0000-0003-0481-4952; Guarino, Fausto/0000-0003-1427-9885; Buscemi, Mario/0000-0003-2123-5434; Colalillo, Roberta/0000-0002-4179-9352; Rodriguez Frias, Maria /0000-0002-2550-4462; De Mitri, Ivan/0000-0002-8665-1730; Rodriguez Fernandez, Gonzalo/0000-0002-4683-230X; Nosek, Dalibor/0000-0001-6219-200X; Knapp, Johannes/0000-0003-1519-1383; scuderi, mario/0000-0001-9026-5317; Blanco, Francisco/0000-0003-4332-434X; zas, enrique/0000-0002-4430-8117; Moura Santos, Edivaldo/0000-0002-2818-8813; Gouffon, Philippe/0000-0001-7511-4115; de Almeida, Rogerio/0000-0003-3104-2724; De Domenico, Manlio/0000-0001-5158-8594; Abreu, Pedro/0000-0002-9973-7314; Navas, Sergio/0000-0003-1688-5758; Assis, Pedro/0000-0001-7765-3606; Conceicao, Ruben/0000-0003-4945-5340; dos Santos, Eva/0000-0002-0474-8863; Alvarez-Muniz, Jaime/0000-0002-2367-0803; Valino, Ines/0000-0001-7823-0154; Carvalho Jr., Washington/0000-0002-2328-7628; Espadanal, Joao/0000-0002-1301-8061; Vazquez, Jose Ramon/0000-0001-9217-5219; Martello, Daniele/0000-0003-2046-3910; Insolia, Antonio/0000-0002-9040-1566; Petrolini, Alessandro/0000-0003-0222-7594; de Mello Neto, Joao/0000-0002-3234-6634; Lozano-Bahilo, Julio/0000-0003-0613-140X; Pimenta, Mario/0000-0002-2590-0908; Chinellato, Carola Dobrigkeit /0000-0002-1236-0789; Ros, German/0000-0001-6623-1483; Brogueira, Pedro/0000-0001-6069-4073; Alves Batista, Rafael/0000-0003-2656-064X; Torralba Elipe, Guillermo/0000-0001-8738-194X; Di Giulio, Claudio/0000-0002-0597-4547; Chinellato, Jose Augusto/0000-0002-3240-6270; Bueno, Antonio/0000-0002-7439-4247; Parente, Gonzalo/0000-0003-2847-0461; Ridky, Jan/0000-0001-6697-1393; Horvath, Pavel/0000-0002-6710-5339; Garcia Pinto, Diego/0000-0003-1348-6735; Tome, Bernardo/0000-0002-7564-8392; Rosado, Jaime/0000-0001-8208-9480; Arqueros, Fernando/0000-0002-4930-9282; Espirito Santo, Maria Catarina/0000-0003-1286-7288; Todero Peixoto, Carlos Jose/0000-0003-3669-8212; Cazon, Lorenzo/0000-0001-6748-8395; Ebr, Jan/0000-0001-8807-6162; Fauth, Anderson/0000-0001-7239-0288; Prouza, Michael/0000-0002-3238-9597; Dembinski, Hans/0000-0003-3337-3850; Del Peral, Luis/0000-0003-2580-5668; Coutu, Stephane/0000-0003-2923-2246; Mussa, Roberto/0000-0002-0294-9071; Ulrich, Ralf/0000-0002-2535-402X; Garcia, Beatriz/0000-0003-0919-2734; Zamorano, Bruno/0000-0002-4286-2835; Bonino, Raffaella/0000-0002-4264-1215; Asorey, Hernan/0000-0002-4559-8785; Petrera, Sergio/0000-0002-6029-1255; Mantsch, Paul/0000-0002-8382-7745; Castellina, Antonella/0000-0002-0045-2467; maldera, simone/0000-0002-0698-4421; Yuan, Guofeng/0000-0002-1907-8815; Marsella, Giovanni/0000-0002-3152-8874; Salamida, Francesco/0000-0002-9306-8447; Navarro Quirante, Jose Luis/0000-0002-9915-1735; Aglietta, Marco/0000-0001-8354-5388; Maccarone, Maria Concetta/0000-0001-8722-0361; Kothandan, Divay/0000-0001-9048-7518 FU Comision Nacional de Energia Atomica; Fundacion Antorchas; Gobierno De La Provincia de Mendoza; Municipalidad de Malargue FX We are very grateful to the following agencies and organizations for financial support: Comision Nacional de Energia Atomica, Fundacion Antorchas, Gobierno De La Provincia de Mendoza, Municipalidad de Malargue, NDM Holdings and Valle Las Lenas, in gratitude for their continuing cooperation over land access, Argentina; the Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacdo de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP), Ministerio de Ciencia e Tecnologia (MCT), Brazil; AVCR AVOZ10100502 and AVOZ10100522, GAAV KJB100100904, MSMT-CR LA08016, LG11044, MEB111003, MSM0021620859, LA08015, TACR TA01010517 and GA UK 119810, Czech Republic; Centre de Calcul IN2P3/CNRS, Centre National de la Recherche Scientifique (CNRS), Conseil Regional Ile-deFrance, Departement Physique Nucleaire et Corpusculaire (PNCIN2P3/CNRS), Departement Sciences de l'Univers (SDU-INSU/CNRS), France; Bundesministerium fur Bildung und Forschung (BMBF), Deutsche Forschungsgemeinschaft (DFG), Finanzministerium Baden-Wurttemberg, Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF), Ministerium fur Wissenschaft und Forschung, Nordrhein-Westfalen, Ministerium fur Wissenschaft, Forschung und Kunst, Baden-Wurttemberg, Germany; Istituto Nazionale di Fisica Nucleare (INFN), Ministero dell'Istruzione, dell'Universitd e della Ricerca (MIUR), Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs, Cultuur en Wetenschap, Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; Ministry of Science and Higher Education, Grant Nos. N N202 200239 and N N202 207238, Poland; Portuguese national funds and FEDER funds within COMPETE - Programa Operacional Factores de Competitividade through Fundacdo para a Ciencia e a Tecnologia, Portugal; Romanian Authority for Scientific Research ANCS, CNDI-UEFISCDI partnership projects nr.20/2012 and nr.194/2012, project nr.1/ASPERA2/2012 ERA-NET and PN-II-RU-PD-2011-3-0145-17, Romania; Ministry for Higher Education, Science, and Technology, Slovenian Research Agency, Slovenia; Comunidad de Madrid, FEDER funds, Ministerio de Ciencia e Innovacion and Consolider-Ingenio 2010 (CPAN), Xunta de Galicia, Spain; The Leverhulme Foundation, Science and Technology Facilities Council, United Kingdom; Department of Energy, Contract Nos. DE-AC02-07CH11359, DE-FR02-04ER41300, DE-FG02-99ER41107, National Science Foundation, Grant No. 0450696, The Grainger Foundation USA; NAFOSTED, Vietnam; Marie Curie-IRSES/EPLANET, European Particle Physics Latin American Network, European Union 7th Framework Program, Grant No. PIRSES-2009-GA-246806; and UNESCO. NR 13 TC 4 Z9 4 U1 3 U2 59 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD DEC PY 2013 VL 50-52 BP 92 EP 101 DI 10.1016/j.astropartphys.2013.09.004 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 283TX UT WOS:000329271000011 ER PT J AU Yoneyama, K Zhang, CD Long, CN AF Yoneyama, Kunio Zhang, Chidong Long, Charles N. TI TRACKING PULSES OF THE MADDEN-JULIAN OSCILLATION SO BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY LA English DT Article ID TROPICAL INTRASEASONAL OSCILLATION; EQUATORIAL INDIAN-OCEAN; STATIC ENERGY BUDGET; CUMULUS CONVECTION; VERTICAL STRUCTURE; RESOLVING MODEL; FORECAST SYSTEM; VARIABILITY; MJO; PREDICTION AB An international field campaign aiming at atmospheric and oceanic processes associated with the Madden-Julian oscillation (MJO) was conducted in and around the tropical Indian Ocean during October 2011-March 2012. The objective of the field campaign was to collect observations urgently needed to expedite the progress of understanding the key processes of the MJO, focusing on its convective initiation but also including propagation and maturation, and ultimately to improve skills of numerical simulation and prediction of the MJO. Primary targets of the field campaign included interaction of atmospheric deep convection with its environmental moisture, evolution of cloud populations, and air- sea interaction. Several MJO events were captured by ground-based, airborne, and oceanic instruments with advanced observing technology. Numerical simulations and real-time forecasts were integrated components of the field campaign in its design and operation. Observations collected during the campaign provide unprecedented opportunities to reveal detailed processes of the MJO and to assist evaluation, improvement, and development of weather and climate models. The data policy of the campaign encourages the broad research community to use the field observations to advance the MJO study. C1 [Yoneyama, Kunio] Japan Agcy Marine Earth Sci & Technol, Yokosuka, Kanagawa 2370061, Japan. [Zhang, Chidong] Univ Miami, Miami, FL USA. [Long, Charles N.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Yoneyama, K (reprint author), Japan Agcy Marine Earth Sci & Technol, 2-15 Natsushima Cho, Yokosuka, Kanagawa 2370061, Japan. EM yoneyamak@jamstec.go.jp FU NSF; DOE (ARM program); DOE (ASR program); ONR; NOAA; NASA; JAMSTEC; Indian MoES; CSIR; France CNES; CNRS, Meteo-France FX We extend recognition and gratitude to all who contributed to the preparation and operation of the field campaign; the success of the field campaign would be impossible without their diligent and dedicated efforts. Nearly 100 students from seven countries volunteered their time to help collect observations onboard ships and aircraft, as well as on the ground. The field campaign provided them with rare opportunities of career experience; they were part of the central force of the success of the field campaign. The DYNAMO Project Office, led by Jim Moore, and NCAR EOL played a crucial role in the logistic support before, during, and after the field campaign with their unmatched experience and skill for instrument deployment and data management. Thanks are owed to local hosts from the Maldives Meteorological Service, Department of Meteorology Sri Lanka, Seychelles National Weather Service, Kenya Meteorological Department, BMKG and BPPT in Indonesia, Meteorological Service Singapore, and Papua New Guinea National Weather Service. The CLIVAR-SSG, ICPO, CLIVAR/AAMP, and CLIVAR/IOC-GOOS Indian Ocean Panel are also acknowledged for their continuous encouragement for the field campaign. Special thanks go to the NSF, DOE (ARM and ASR programs), ONR, NOAA, NASA, JAMSTEC, Indian MoES and CSIR, France CNES and CNRS, Meteo-France, and all other local and participants' funding agencies for their support, as well as the WMO and the JMA who sponsored some of the land-based observations. We appreciate the comments from three anonymous reviewers that helped to improve the manuscript. NR 64 TC 134 Z9 134 U1 2 U2 18 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0003-0007 EI 1520-0477 J9 B AM METEOROL SOC JI Bull. Amer. Meteorol. Soc. PD DEC PY 2013 VL 94 IS 12 BP 1871 EP 1891 DI 10.1175/BAMS-D-12-00157.1 PG 21 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 287OH UT WOS:000329551600010 ER PT J AU Annavarapu, C Hautefeuille, M Dolbow, JE AF Annavarapu, Chandrasekhar Hautefeuille, Martin Dolbow, John E. TI A Nitsche stabilized finite element method for frictional sliding on embedded interfaces. Part II: Intersecting interfaces SO COMPUTER METHODS IN APPLIED MECHANICS AND ENGINEERING LA English DT Article DE Frictional contact; Grain-boundary sliding; Junctions; Nitsche; Polycrystalline; X-FEM ID POLYCRYSTALLINE BRITTLE MATERIALS; GRAIN LEVEL MODEL; COMPUTATIONAL APPROACH; FAILURE INITIATION; X-FEM; BOUNDARY; SIZE; FORMULATION; MICROSTRUCTURES; RESTORATION AB We extend the weighted Nitsche's method proposed in the first part of this study to include multiple intersecting embedded interfaces. These intersections arise either inside a computational domain - where two internal interfaces intersect; or on the boundary of the computational domain - where an internal interface intersects with the external boundary. We propose a variational treatment of both the interfacial kinematics and the external Dirichlet constraints within Nitsche's framework. We modify the numerical analysis to account for these intersections and provide an explicit expression for the weights and the method parameters that arise in the Nitsche variational form in the presence of junctions. Finally, we demonstrate the performance of the method for both perfectly-tied interfaces and perfectly-plastic sliding interfaces through several benchmark examples. (C) 2013 Elsevier B.V. All rights reserved. C1 [Annavarapu, Chandrasekhar] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. [Hautefeuille, Martin] MIT, Dept Aeronaut & Astronaut, Cambridge, MA 02139 USA. [Dolbow, John E.] Duke Univ, Dept Civil & Environm Engn, Durham, NC 27708 USA. [Annavarapu, Chandrasekhar] Duke Univ, Durham, NC 27706 USA. RP Annavarapu, C (reprint author), Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, 7000 East Ave,L-286, Livermore, CA 94550 USA. EM annavarapusr1@llnl.gov RI Hautefeuille, Martin/F-3289-2010; Annavarapu, Chandrasekhar/Q-6512-2016 OI Hautefeuille, Martin/0000-0003-2630-2958; Annavarapu, Chandrasekhar/0000-0003-3608-0500 NR 40 TC 5 Z9 5 U1 1 U2 9 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0045-7825 EI 1879-2138 J9 COMPUT METHOD APPL M JI Comput. Meth. Appl. Mech. Eng. PD DEC 1 PY 2013 VL 267 BP 318 EP 341 DI 10.1016/j.cma.2013.08.008 PG 24 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Engineering; Mathematics; Mechanics GA 287GV UT WOS:000329530900014 ER PT J AU Arkin, AP Fussenegger, M AF Arkin, Adam P. Fussenegger, Martin TI Synthetic biology SO CURRENT OPINION IN CHEMICAL BIOLOGY LA English DT Editorial Material C1 [Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94704 USA. [Arkin, Adam P.] EO Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Fussenegger, Martin] Swiss Fed Inst Technol, Dept Biosyst Sci & Engn, CH-4058 Basel, Switzerland. [Fussenegger, Martin] Univ Basel, CH-4058 Basel, Switzerland. RP Arkin, AP (reprint author), Univ Calif Berkeley, Dept Bioengn, 2151 Berkeley Way, Berkeley, CA 94704 USA. EM aparkin@lbl.gov; martin.fussenegger@bsse.ethz.ch RI Arkin, Adam/A-6751-2008 OI Arkin, Adam/0000-0002-4999-2931 NR 0 TC 1 Z9 1 U1 0 U2 19 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1367-5931 EI 1879-0402 J9 CURR OPIN CHEM BIOL JI Curr. Opin. Chem. Biol. PD DEC PY 2013 VL 17 IS 6 BP 869 EP 870 DI 10.1016/j.cbpa.2013.11.005 PG 2 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA 288GX UT WOS:000329601100001 ER PT J AU Arkin, AP AF Arkin, Adam Paul TI A wise consistency: engineering biology for conformity, reliability, predictability SO CURRENT OPINION IN CHEMICAL BIOLOGY LA English DT Review ID REPLICATING LENTIVIRAL VECTOR; LEBERS CONGENITAL AMAUROSIS; ESCHERICHIA-COLI; GENE-EXPRESSION; PROTEIN EXPRESSION; SYNTHETIC BIOLOGY; MODULAR CONTROL; CANCER-CELLS; LOGIC GATES; T-CELLS AB The next generation of synthetic biology applications will increasingly involve engineered organisms that exist in intimate contact with humans, animals and the rest of the environment. Examples include cellular and viral approaches for maintaining and improving health in humans and animals. The need for reliable and specific function in these environments may require more complex system designs than previously. In these cases the uncertainties in the behavior of biological building blocks, their hosts and their environments present a challenge for design of predictable and safe systems. Here, we review systematic methods for the effective characterization of these uncertainties that are lowering the barriers to predictive design of reliable complex biological systems. C1 [Arkin, Adam Paul] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94704 USA. [Arkin, Adam Paul] EO Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Arkin, AP (reprint author), Univ Calif Berkeley, Dept Bioengn, 2151 Berkeley Way, Berkeley, CA 94704 USA. EM aparkin@lbl.gov RI Arkin, Adam/A-6751-2008 OI Arkin, Adam/0000-0002-4999-2931 FU Department of Energy [DE-FOA-0000640] FX This work was supported by a grant from the Department of Energy grant number DE-FOA-0000640. APA would like to acknowledge V.K. Mutalik for his help with Figure 2. NR 67 TC 16 Z9 16 U1 0 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1367-5931 EI 1879-0402 J9 CURR OPIN CHEM BIOL JI Curr. Opin. Chem. Biol. PD DEC PY 2013 VL 17 IS 6 BP 893 EP 901 DI 10.1016/j.cbpa.2013.09.012 PG 9 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA 288GX UT WOS:000329601100004 PM 24268562 ER PT J AU Uberuaga, BP Andersson, DA Stanek, CR AF Uberuaga, Bias Pedro Andersson, David A. Stanek, Christopher R. TI Defect behavior in oxides: Insights from modern atomistic simulation methods SO CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE LA English DT Review DE Oxides; Defect thermodynamics; Defect chemistry; Electronic defects; Defect kinetics ID GENERALIZED GRADIENT APPROXIMATION; ELECTRONIC-STRUCTURE; RADIATION-DAMAGE; DIELECTRIC-PROPERTIES; STRUCTURAL STABILITY; URANIUM-DIOXIDE; POINT-DEFECTS; PYROCHLORES; DYNAMICS; CONDUCTION AB Oxide ceramics are important for a large number of technological applications. In most cases, the behavior of defects determines the properties of the oxide that make it appealing. Thus, understanding defect properties - thermodynamic and kinetic - is central for optimizing structure/property relationships for oxides. Here, we provide a perspective on the use of modern computational capabilities to interrogate defect properties in complex oxides. We focus on three aspects: the screening of multiple defect reactions in a large set of oxide chemistries to determine dominant defect structure, the interaction of ionic and electronic defects, and the kinetic properties of defects. These examples serve to illustrate the types of insights that can be gained when applying new methodologies, combined with modern computational resources, to advance the understanding of these materials. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Uberuaga, Bias Pedro; Andersson, David A.; Stanek, Christopher R.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Uberuaga, BP (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM blas@lanl.gov; andersson@lanl.gov; stanek@lanl.gov FU Department of Energy (DOE), Office of Nuclear Energy, Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program; DOE Office of Basic Energy Sciences (OBES), Division of Materials Sciences; Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX DAA and CRS acknowledge support by the Department of Energy (DOE), Office of Nuclear Energy, Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program. BPU acknowledges support by the DOE Office of Basic Energy Sciences (OBES), Division of Materials Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under Contract DE-AC52-06NA25396. NR 96 TC 9 Z9 9 U1 10 U2 61 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-0286 EI 1879-0348 J9 CURR OPIN SOLID ST M JI Curr. Opin. Solid State Mat. Sci. PD DEC PY 2013 VL 17 IS 6 SI SI BP 249 EP 256 DI 10.1016/j.cossms.2013.07.003 PG 8 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 286OT UT WOS:000329479300001 ER PT J AU Plimpton, SJ Gale, JD AF Plimpton, Steven J. Gale, Julian D. TI Developing community codes for materials modeling SO CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE LA English DT Review DE Materials modeling; Open source software; Molecular dynamics; Lattice dynamics; Force fields ID UTILITY-LATTICE-PROGRAM; MOLECULAR-DYNAMICS; GULP; ALGORITHMS; SIMULATION AB For this article, we call scientific software a community code if it is freely available, written by a team of developers who welcome user input, and has attracted users beyond the developers. There are obviously many such materials modeling codes. The authors have been part of such efforts for many years in the field of atomistic simulation, specifically for two community codes, the LAMMPS and GULP packages for molecular dynamics and lattice dynamics respectively. Here we highlight lessons we have learned about how to create such codes and the pros and cons of being part of a community effort. Many of our experiences are similar, but we also have some differences of opinion (like modeling vs modelling). Our hope is that readers will find these lessons useful as they design, implement, and distribute their own materials modelling software for others to use. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Plimpton, Steven J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Gale, Julian D.] Curtin Univ, Dept Chem, Nanochem Res Inst, Perth, WA 6845, Australia. RP Plimpton, SJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM sjplimp@sandia.gov; J.Gale@curtin.edu.au RI Gale, Julian/B-7987-2009 OI Gale, Julian/0000-0001-9587-9457 FU Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Australian Research Council FX SJP works at Sandia National Laboratories which is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. JDG acknowledges the support of the Australian Research Council through a Discovery Project. NR 17 TC 3 Z9 3 U1 3 U2 29 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-0286 EI 1879-0348 J9 CURR OPIN SOLID ST M JI Curr. Opin. Solid State Mat. Sci. PD DEC PY 2013 VL 17 IS 6 SI SI BP 271 EP 276 DI 10.1016/j.cossms.2013.09.005 PG 6 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 286OT UT WOS:000329479300004 ER PT J AU Fisher, JA Jacob, DJ Soerensen, AL Amos, HM Corbitt, ES Streets, DG Wang, QQ Yantosca, RM Sunderland, EM AF Fisher, Jenny A. Jacob, Daniel J. Soerensen, Anne L. Amos, Helen M. Corbitt, Elizabeth S. Streets, David G. Wang, Qiaoqiao Yantosca, Robert M. Sunderland, Elsie M. TI Factors driving mercury variability in the Arctic atmosphere and ocean over the past 30 years SO GLOBAL BIOGEOCHEMICAL CYCLES LA English DT Article DE Arctic; mercury ID SEA-ICE; MACKENZIE RIVER; METHYLATED MERCURY; OZONE DEPLETION; GASEOUS MERCURY; 10-YEAR TRENDS; BOUNDARY-LAYER; CLIMATE-CHANGE; MARINE WATERS; BEAUFORT SEA AB Long-term observations at Arctic sites (Alert and Zeppelin) show large interannual variability (IAV) in atmospheric mercury (Hg), implying a strong sensitivity of Hg to environmental factors and potentially to climate change. We use the GEOS-Chem global biogeochemical Hg model to interpret these observations and identify the principal drivers of spring and summer IAV in the Arctic atmosphere and surface ocean from 1979-2008. The model has moderate skill in simulating the observed atmospheric IAV at the two sites (r similar to 0.4) and successfully reproduces a long-term shift at Alert in the timing of the spring minimum from May to April (r=0.7). Principal component analysis indicates that much of the IAV in the model can be explained by a single climate mode with high temperatures, low sea ice fraction, low cloudiness, and shallow boundary layer. This mode drives decreased bromine-driven deposition in spring and increased ocean evasion in summer. In the Arctic surface ocean, we find that the IAV for modeled total Hg is dominated by the meltwater flux of Hg previously deposited to sea ice, which is largest in years with high solar radiation (clear skies) and cold spring air temperature. Climate change in the Arctic is projected to result in increased cloudiness and strong warming in spring, which may thus lead to decreased Hg inputs to the Arctic Ocean. The effect of climate change on Hg discharges from Arctic rivers remains a major source of uncertainty. C1 [Fisher, Jenny A.] Univ Wollongong, Sch Chem, Wollongong, NSW 2522, Australia. [Jacob, Daniel J.; Soerensen, Anne L.; Wang, Qiaoqiao; Yantosca, Robert M.; Sunderland, Elsie M.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Jacob, Daniel J.; Amos, Helen M.; Corbitt, Elizabeth S.] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Soerensen, Anne L.; Sunderland, Elsie M.] Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02115 USA. [Streets, David G.] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Fisher, JA (reprint author), Univ Wollongong, Sch Chem, Northfields Ave, Wollongong, NSW 2522, Australia. EM jennyf@uow.edu.au RI Fisher, Jenny/J-3979-2012; Chem, GEOS/C-5595-2014; Yantosca, Robert/F-7920-2014; Wang, Qiaoqiao/M-3884-2016; Sunderland, Elsie/D-5511-2014; OI Fisher, Jenny/0000-0002-2921-1691; Yantosca, Robert/0000-0003-3781-1870; Sunderland, Elsie/0000-0003-0386-9548; Streets, David/0000-0002-0223-1350 FU NSF Office of Polar Programs; University of Wollongong; Carlsberg Foundation; Northern Contaminants Program, Environment Canada; Arctic Monitoring and Assessment Programme FX This work was supported by the NSF Office of Polar Programs. JAF acknowledges support from a University of Wollongong Vice Chancellor's Postdoctoral Fellowship. ALS acknowledges support from the Carlsberg Foundation. We thank A. Steffen, A. Cole, and the Canadian National Atmospheric Chemistry Database for the collection and provision of the Alert data, with financial support provided by the Northern Contaminants Program, Environment Canada, and the Arctic Monitoring and Assessment Programme. We also thank the European Monitoring and Evaluation Programme, the Finnish Meteorological Institute, and the Norwegian Institute for Air Research for the collection and provision of the Zeppelin and Pallas data. MERRA data used in this study have been provided by the Global Modeling and Assimilation Office at NASA Goddard Space Flight Center through the NASA GES DISC online archive. We thank A. Qureshi for helpful discussions. NR 79 TC 17 Z9 18 U1 3 U2 56 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0886-6236 EI 1944-9224 J9 GLOBAL BIOGEOCHEM CY JI Glob. Biogeochem. Cycle PD DEC PY 2013 VL 27 IS 4 BP 1226 EP 1235 DI 10.1002/2013GB004689 PG 10 WC Environmental Sciences; Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Geology; Meteorology & Atmospheric Sciences GA 289MP UT WOS:000329686900022 ER PT J AU Wu, YH Ren, HY Tang, H AF Wu, Yanhua Ren, Huiying Tang, Hui TI Turbulent flow over a rough backward-facing step SO INTERNATIONAL JOURNAL OF HEAT AND FLUID FLOW LA English DT Article DE Turbulence; Rough-wall turbulent flow; Backward-facing step flow ID PARTICLE IMAGE VELOCIMETRY; IRREGULAR SURFACE-ROUGHNESS; LARGE-EDDY SIMULATION; WALL TURBULENCE; BOUNDARY-LAYER; SHEAR-LAYER; REATTACHMENT; DAMAGE AB This work characterizes the impacts of the realistic roughness due to deposition of foreign materials on the turbulent flows at surface transition from elevated rough-wall to smooth-wall. High resolution PIV measurements were performed in the streamwise-wall-normal (x-y) planes at two different spanwise positions in both smooth and rough backward-facing step flows. The experiment conditions were set at a Reynolds number of 3450 based on the free stream velocity U-infinity and the mean step height h, expansion ratio of 1.01, and the ratio of incoming boundary layer thickness to the step height, delta/h, of 8. The mean flow structures are observed to be modified by the roughness and they illustrate three-dimensional features in rough backward-facing step flows. The mean reattachment length X-r is significantly reduced by the roughness at one PIV measurement position while is slightly increased by the different roughness topography at the other measurement position. The mean velocity profiles at the reattachment point indicate that the studied roughness weakens the perturbation of the step to the incoming turbulent flow. Comparisons of Reynolds normal and shear stresses, productions of normal stresses, quadrant analysis of the instantaneous shear-stress contributing events, and mean spanwise vorticity reveal that the turbulence in the separated shear layer is reduced by the studied roughness. The results also indicate an earlier separation of the turbulent boundary layer over the current rough step, probably due to the adverse pressure gradient produced by the roughness topography even before the step. (C) 2013 Elsevier Inc. All rights reserved. C1 [Wu, Yanhua; Tang, Hui] Nanyang Technol Univ, Sch Mech & Aerosp Engn, Singapore 639798, Singapore. [Ren, Huiying] Pacific NW Natl Lab, Hydrol Tech Grp, Richland, WA 99352 USA. RP Wu, YH (reprint author), Nanyang Technol Univ, Sch Mech & Aerosp Engn, Singapore 639798, Singapore. EM yanhuawu@ntu.edu.sg RI Tang, Hui/B-3890-2010; Wu, Yanhua/A-3839-2011 OI Tang, Hui/0000-0002-6774-507X; NR 35 TC 8 Z9 8 U1 1 U2 27 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0142-727X EI 1879-2278 J9 INT J HEAT FLUID FL JI Int. J. Heat Fluid Flow PD DEC PY 2013 VL 44 BP 155 EP 169 DI 10.1016/j.ijheatfluidflow.2013.05.014 PG 15 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA 288EK UT WOS:000329594600013 ER PT J AU Hazra, DK Shafieloo, A Smoot, GF AF Hazra, Dhiraj Kumar Shafieloo, Arman Smoot, George F. TI Reconstruction of broad features in the primordial spectrum and inflaton potential from Planck SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE inflation; physics of the early universe; cosmological parameters from CMBR; CMBR theory ID PROBE WMAP OBSERVATIONS; POWER SPECTRUM; ANISOTROPY; PERTURBATIONS; COSMOLOGY; MODEL AB With the recently published Cosmic Microwave Background data from Planck we address the optimized binning of the primordial power spectrum. As an important modification to the usual binning of the primordial spectrum, along with the spectral amplitude of the bins, we allow the position of the bins also to vary. This technique enables us to address the location of the possible broad physical features in the primordial spectrum with relatively smaller number of bins compared to the analysis performed earlier. This approach is in fact a reconstruction method looking for broad features in the primordial spectrum and avoiding fitting noise in the data. Performing Markov Chain Monte Carlo analysis we present samples of the allowed primordial spectra with broad features consistent with Planck data. To test how realistic it is to have step-like features in primordial spectrum we revisit an inflationary model, proposed by A. A. Starobinsky which can address the similar features obtained from the binning of the spectrum. Using the publicly available code BINGO, we numerically calculate the local f(NL) for this model in equilateral and arbitrary triangular configurations of wavevectors and show that the obtained non-Gaussianity for this model is consistent with Planck results. In this paper we have also considered different spectral tilts at different bins to identify the cosmological scale that the spectral index needs to have a red tilt and it is interesting to report that spectral index cannot be well constrained up to k approximate to 0.01Mpc(-1). C1 [Hazra, Dhiraj Kumar; Shafieloo, Arman] Asia Pacific Ctr Theoret Phys, Pohang 790784, Gyeongbuk, South Korea. [Shafieloo, Arman] POSTECH, Dept Phys, Pohang 790784, Gyeongbuk, South Korea. [Smoot, George F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Smoot, George F.] Ewha Womans Univ, Inst Early Universe, Seoul 120750, South Korea. [Smoot, George F.] Univ Paris Diderot, Paris Ctr Cosmol Phys, Paris, France. RP Hazra, DK (reprint author), Asia Pacific Ctr Theoret Phys, Pohang 790784, Gyeongbuk, South Korea. EM dhiraj@apctp.org; arman@apctp.org; gfsmoot@lbl.gov FU Korea Ministry of Education, Science and Technology, Gyeongsangbuk-Do; Pohang City for Independent Junior Research Groups at the Asia Pacific Center for Theoretical Physics FX D.K.H and A. S wish to acknowledge support from the Korea Ministry of Education, Science and Technology, Gyeongsangbuk-Do and Pohang City for Independent Junior Research Groups at the Asia Pacific Center for Theoretical Physics. NR 102 TC 19 Z9 19 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD DEC PY 2013 IS 12 AR 035 DI 10.1088/1475-7516/2013/12/035 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 288JV UT WOS:000329609000034 ER PT J AU Linder, EV AF Linder, Eric V. TI How fabulous is Fab 5 cosmology? SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE modified gravity; dark energy theory; physics of the early universe ID FIELD-EQUATIONS; INFLATION; COUPLINGS AB Extended gravity origins for cosmic acceleration can solve some fine tuning issues and have useful characteristics, but generally have little to say regarding the cosmological constant problem. Fab 5 gravity can be ghost free and stable, have attractor solutions in the past and future, and possess self tuning that solves the original cosmological constant problem. Here we show however it does not possess all these qualities at the same time. We also demonstrate that the self tuning is so powerful that it not only cancels the cosmological constant but also all other energy density, and we derive the scalings of its approach to a renormalized de Sitter cosmology. While this strong cancellation is bad for the late universe, it greatly eases early universe inflation. C1 [Linder, Eric V.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Linder, Eric V.] Univ Calif Berkeley, Berkeley Lab, Berkeley, CA 94720 USA. RP Linder, EV (reprint author), Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. EM evlinder@lbl.gov FU Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231] FX I thank Stephen Appleby, Antonio de Felice, and Shinji Mukohyama for helpful discussions, and the Korea Astronomy and Space Science Institute for hospitality. This work has been supported in part by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 30 TC 5 Z9 5 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD DEC PY 2013 IS 12 AR 032 DI 10.1088/1475-7516/2013/12/032 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 288JV UT WOS:000329609000031 ER PT J AU Yu, C Cheng, JJ Kamboj, S AF Yu, C. Cheng, J. -J. Kamboj, S. TI Effects of the new wildlife transfer factors on RESRAD-BIOTA's screening Biota Concentration Guides and previous model comparison studies SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Concentration ratio; Transfer factor; Biv; RESRAD-BIOTA; Biota concentration guide; Radiation dose AB The RESRAD-BIOTA Level 1 default Biota Concentration Guides (BCGs) are generic screening environmental medium concentrations based on reasonably conservative concentration ratios (CRs). These CRs had been identified from available literature for a variety of biota organisms. The International Atomic Energy Agency (IAEA) Technical Report Series (TRS) handbook on radionuclide transfer to wildlife was recently published with data that can be compared with the RESRAD-BIOTA values. In addition, previous IAEA Environmental Modeling for Radiation Safety (EMRAS) II Biota Working Group model comparison results are examined by comparing them with those obtained using the new TRS CR values for wildlife. Since the CR affects only internal doses, the effect on the overall dose depends on the relative contribution from internal and external exposure pathways. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Yu, C.; Cheng, J. -J.; Kamboj, S.] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. RP Yu, C (reprint author), Argonne Natl Lab, Div Environm Sci, 9700 Cass Ave, Argonne, IL 60439 USA. EM cyu@anl.gov FU U.S. Department of Energy [DE-AC02-06CH11357] FX This work was supported by U.S. Department of Energy under contract DE-AC02-06CH11357. NR 13 TC 1 Z9 1 U1 1 U2 5 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD DEC PY 2013 VL 126 SI SI BP 338 EP 351 DI 10.1016/j.jenvrad.2013.01.004 PG 14 WC Environmental Sciences SC Environmental Sciences & Ecology GA 285SR UT WOS:000329415800040 PM 23455002 ER PT J AU Johansen, MP Kamboj, S Kuhne, WW AF Johansen, M. P. Kamboj, S. Kuhne, W. W. TI Whole-organism concentration ratios for plutonium in wildlife from past US nuclear research data SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Concentration ratio; Plutonium; Wildlife; Transfer; Field study ID DEFAULT CONCENTRATION RATIOS; ERICA TOOL; TRANSFER PARAMETERS; BIOTA; RADIONUCLIDES; FACILITY; PU-238; ATOLL; FISH; SOIL AB Whole-organism concentration ratios (CRwo-media) for plutonium (Pu) in wildlife were calculated using data from the broad range of organism types and environmental settings of the US nuclear research program. Original sources included site-specific reports and scientific journal articles typically from 1960s to 80s research. Most of the calculated CRwo-media values are new to existing data sets, and, for some wildlife categories, serve to fill gaps or add to sparse data including those for terrestrial reptile; freshwater bird, crustacean and zooplankton; and marine crustacean and zooplankton. Ratios of Pu concentration in the whole-organism to that in specific tissues and organs are provided here for a range of freshwater and marine fish. The CRwo-media values in fish living in liquid discharge ponds were two orders of magnitude higher than those for similar species living in lakes receiving Pu from atmospheric fallout, suggesting the physico-chemical form of the source Pu can dominate over other factors related to transfer, such as organism size and feeding behavior. Small rodent data indicated one to two order of magnitude increases when carcass, pelt, and gastrointestinal tract were included together in the whole-organism calculation compared to that for carcass alone. Only 4% of Pu resided in the carcass of small rodents compared to 75% in the gastrointestinal tract and 21% in the pelt. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Johansen, M. P.] Australian Nucl Sci & Technol Org, Kirrawee Dc, NSW 2232, Australia. [Kamboj, S.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Johansen, MP (reprint author), Australian Nucl Sci & Technol Org, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia. EM mathew.johansen@ansto.gov.au RI Johansen, Mathew/D-7049-2012 NR 40 TC 5 Z9 6 U1 0 U2 11 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD DEC PY 2013 VL 126 SI SI BP 412 EP 419 DI 10.1016/j.jenvrad.2012.07.015 PG 8 WC Environmental Sciences SC Environmental Sciences & Ecology GA 285SR UT WOS:000329415800046 PM 22939266 ER PT J AU Camporeale, E Delzanno, GL Zaharia, S Koller, J AF Camporeale, E. Delzanno, G. L. Zaharia, S. Koller, J. TI Reply to comment by J. M. Albert on "On the numerical simulation of particle dynamics in the radiation belt. Part I: Implicit and semi-implicit schemes" and "On the numerical simulation of particle dynamics in the radiation belt. Part II: Procedure based on the diagonalization of the diffusion tensor" SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE radiation belt; diffusion code; numerical simulations C1 [Camporeale, E.; Delzanno, G. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zaharia, S.; Koller, J.] Los Alamos Natl Lab, ISR 1, Los Alamos, NM 87545 USA. RP Camporeale, E (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM enrico@lanl.gov RI Koller, Josef/C-5591-2009 OI Koller, Josef/0000-0002-6770-4980 NR 4 TC 4 Z9 4 U1 0 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD DEC PY 2013 VL 118 IS 12 BP 7765 EP 7767 DI 10.1002/2013JA019389 PG 3 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 286ZX UT WOS:000329508900031 ER PT J AU Johansson, LC Arnlund, D Katona, G White, TA Barty, A DePonte, DP Shoeman, RL Wickstrand, C Sharma, A Williams, GJ Aquila, A Bogan, MJ Caleman, C Davidsson, J Doak, RB Frank, M Fromme, R Galli, L Grotjohann, I Hunter, MS Kassemeyer, S Kirian, RA Kupitz, C Liang, MN Lomb, L Malmerberg, E Martin, AV Messerschmidt, M Nass, K Redecke, L Seibert, MM Sjohamn, J Steinbrener, J Stellato, F Wang, DJ Wahlgren, WY Weierstall, U Westenhoff, S Zatsepin, NA Boutet, S Spence, JCH Schlichting, I Chapman, HN Fromme, P Neutze, R AF Johansson, Linda C. Arnlund, David Katona, Gergely White, Thomas A. Barty, Anton DePonte, Daniel P. Shoeman, Robert L. Wickstrand, Cecilia Sharma, Amit Williams, Garth J. Aquila, Andrew Bogan, Michael J. Caleman, Carl Davidsson, Jan Doak, R. Bruce Frank, Matthias Fromme, Raimund Galli, Lorenzo Grotjohann, Ingo Hunter, Mark S. Kassemeyer, Stephan Kirian, Richard A. Kupitz, Christopher Liang, Mengning Lomb, Lukas Malmerberg, Erik Martin, Andrew V. Messerschmidt, Marc Nass, Karol Redecke, Lars Seibert, M. Marvin Sjoehamn, Jennie Steinbrener, Jan Stellato, Francesco Wang, Dingjie Wahlgren, Weixaio Y. Weierstall, Uwe Westenhoff, Sebastian Zatsepin, Nadia A. Boutet, Sebastien Spence, John C. H. Schlichting, Ilme Chapman, Henry N. Fromme, Petra Neutze, Richard TI Structure of a photosynthetic reaction centre determined by serial femtosecond crystallography SO NATURE COMMUNICATIONS LA English DT Article ID PROTEIN-STRUCTURE DETERMINATION; MEMBRANE-PROTEINS; RESOLUTION; NANOCRYSTALLOGRAPHY; CRYSTALLIZATION; DIFFRACTION; LASER AB Serial femtosecond crystallography is an X-ray free-electron-laser-based method with considerable potential to have an impact on challenging problems in structural biology. Here we present X-ray diffraction data recorded from microcrystals of the Blastochloris viridis photosynthetic reaction centre to 2.8 angstrom resolution and determine its serial femtosecond crystallography structure to 3.5 angstrom resolution. Although every microcrystal is exposed to a dose of 33MGy, no signs of X-ray-induced radiation damage are visible in this integral membrane protein structure. C1 [Johansson, Linda C.; Arnlund, David; Katona, Gergely; Wickstrand, Cecilia; Sharma, Amit; Malmerberg, Erik; Sjoehamn, Jennie; Wahlgren, Weixaio Y.; Westenhoff, Sebastian; Neutze, Richard] Univ Gothenburg, Dept Chem & Mol Biol, S-40530 Gothenburg, Sweden. [White, Thomas A.; Barty, Anton; DePonte, Daniel P.; Aquila, Andrew; Caleman, Carl; Galli, Lorenzo; Liang, Mengning; Martin, Andrew V.; Nass, Karol; Stellato, Francesco; Chapman, Henry N.] DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany. [Shoeman, Robert L.; Kassemeyer, Stephan; Lomb, Lukas; Steinbrener, Jan; Schlichting, Ilme] Max Planck Inst Med Res, D-69120 Heidelberg, Germany. [Shoeman, Robert L.; Kassemeyer, Stephan; Lomb, Lukas; Steinbrener, Jan; Schlichting, Ilme] Ctr Free Electron Laser Sci, Max Planck Adv Study Grp, D-22607 Hamburg, Germany. [Williams, Garth J.; Messerschmidt, Marc; Seibert, M. Marvin; Boutet, Sebastien] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. [Bogan, Michael J.] SLAC Natl Accelerator Lab, PULSE Inst, Menlo Pk, CA 94025 USA. [Davidsson, Jan] Uppsala Univ, Dept Chem, Angstrom Lab, S-75120 Uppsala, Sweden. [Doak, R. Bruce; Kirian, Richard A.; Wang, Dingjie; Weierstall, Uwe; Zatsepin, Nadia A.; Spence, John C. H.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Frank, Matthias] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Fromme, Raimund; Grotjohann, Ingo; Hunter, Mark S.; Kupitz, Christopher; Fromme, Petra] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Galli, Lorenzo; Nass, Karol; Chapman, Henry N.] Univ Hamburg, Dept Phys, D-22761 Hamburg, Germany. [Redecke, Lars] Univ Hamburg, Inst Biochem & Mol Biol, Joint Lab Struct Biol Infect & Inflammat, D-22607 Hamburg, Germany. [Redecke, Lars] Univ Lubeck, DESY, Inst Biochem, D-22607 Hamburg, Germany. RP Neutze, R (reprint author), Univ Gothenburg, Dept Chem & Mol Biol, S-40530 Gothenburg, Sweden. EM richard.neutze@chem.gu.se RI Katona, Gergely/B-3491-2008; Johansson, Linda/B-1240-2011; Messerschmidt, Marc/F-3796-2010; Barty, Anton/K-5137-2014; Neutze, Richard/A-7573-2010; Frank, Matthias/O-9055-2014; Schlichting, Ilme/I-1339-2013; Sjohamn, Jennie/A-8266-2011; Fromme, Raimund/C-8885-2012; Chapman, Henry/G-2153-2010; OI Kirian, Richard/0000-0001-7197-3086; Katona, Gergely/0000-0002-2031-8716; MARTIN, ANDREW/0000-0003-3704-1829; Johansson, Linda/0000-0003-4776-5142; Messerschmidt, Marc/0000-0002-8641-3302; Barty, Anton/0000-0003-4751-2727; Neutze, Richard/0000-0003-0986-6153; Fromme, Raimund/0000-0003-4835-1080; Chapman, Henry/0000-0002-4655-1743; Seibert, Mark Marvin/0000-0003-0251-0744 FU Swedish Science Research Council (VR); Swedish Foundation for International Cooperation in Research and Higher Education (STINT); Swedish Strategic Research Foundation (SSF); US National Science Foundation (NSF); bioXFEL Science and Technology Center [NSF 1231306]; US National Institute of Health (NIH); DOE Office of Basic Energy Sciences; Hamburg Ministry of Science and Research; Joachim Herz Stiftung; Deutsche Forschungsgemeinschaft (DFG); German Federal Ministry for Education and Research (BMBF); DFG Cluster of Excellence 'Inflammation at Interfaces' [EXC 306]; Max Planck Society; UCOP Lab Fee Program [118036]; LLNL Lab-directed Research and Development Program [12-ERD-031] FX Experiments were carried out at the LCLS, a national user facility operated by Stanford University on behalf of the U.S. Department of Energy (DOE), Office of Basic Energy Sciences. We gratefully acknowledge financial support from the Swedish Science Research Council (VR), the Swedish Foundation for International Cooperation in Research and Higher Education (STINT), the Swedish Strategic Research Foundation (SSF), the US National Science Foundation (NSF) and its bioXFEL Science and Technology Center (NSF 1231306), the US National Institute of Health (NIH), the DOE Office of Basic Energy Sciences, the Hamburg Ministry of Science and Research, the Joachim Herz Stiftung, the Deutsche Forschungsgemeinschaft (DFG), the German Federal Ministry for Education and Research (BMBF), the DFG Cluster of Excellence 'Inflammation at Interfaces' (EXC 306) and the Max Planck Society. Support for LLNL personnel was provided by the UCOP Lab Fee Program (award number 118036) and the LLNL Lab-directed Research and Development Program (12-ERD-031). NR 37 TC 39 Z9 39 U1 4 U2 69 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD DEC PY 2013 VL 4 AR 2911 DI 10.1038/ncomms3911 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 285LV UT WOS:000329396400012 PM 24352554 ER PT J AU Kim, YS Hofman, GL Ryu, HJ Park, JM Robinson, AB Wachs, DM AF Kim, Yeon Soo Hofman, G. L. Ryu, Ho Jin Park, Jong Man Robinson, A. B. Wachs, D. M. TI MODELING OF INTERACTION LAYER GROWTH BETWEEN U-Mo PARTICLES AND AN Al MATRIX SO NUCLEAR ENGINEERING AND TECHNOLOGY LA English DT Article DE U-Mo; U-Mo/Al; Dispersion Fuel; Interaction Layer; IL Growth; Modeling; In-pile Data ID MO/AL DISPERSION FUEL; URANIUM-MOLYBDENUM/ALUMINUM; ALLOY FUEL; DEGREES-C; IRRADIATION; INTERDIFFUSION; PERFORMANCE; SI; ALUMINUM; BEHAVIOR AB Interaction layer growth between U-Mo alloy fuel particles and Al in a dispersion fuel is a concern due to the volume expansion and other unfavorable irradiation behavior of the interaction product. To reduce interaction layer (IL) growth, a small amount of Si is added to the Al. As a result, IL growth is affected by the Si content in the Al matrix. In order to predict IL growth during fabrication and irradiation, empirical models were developed. For IL growth prediction during fabrication and any follow-on heating process before irradiation, out-of-pile heating test data were used to develop kinetic correlations. Two out-of-pile correlations, one for the pure Al matrix and the other for the Al matrix with Si addition, respectively, were developed, which are Arrhenius equations that include temperature and time. For IL growth predictions during irradiation, the out-of-pile correlations were modified to include a fission-rate term to consider fission enhanced diffusion, and multiplication factors to incorporate the Si addition effect and the effect of the Mo content. The in-pile correlation is applicable for a pure Al matrix and an Al matrix with the Si content up to 8 wt%, for fuel temperatures up to 200 degrees C, and for Mo content in the range of 6 - 10wt%. In order to cover these ranges, in-pile data were included in modeling from various tests, such as the US RERTR-4, -5, -6, -7 and -9 tests and Korea's KOMO-4 test, that were designed to systematically examine the effects of the fission rate, temperature, Si content in Al matrix, and Mo content in U-Mo particles. A model converting the IL thickness to the IL volume fraction in the meat was also developed. C1 [Kim, Yeon Soo; Hofman, G. L.] Argonne Natl Lab, Argonne, IL 60439 USA. [Ryu, Ho Jin] Korea Adv Inst Sci & Technol, Dept Nucl & Quantum Engn, Taejon 305701, South Korea. [Park, Jong Man] Korea Atom Energy Res Inst, Taejon 305353, South Korea. [Robinson, A. B.; Wachs, D. M.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Kim, YS (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM yskim@anl.gov RI RYU, HO JIN/J-2764-2013 OI RYU, HO JIN/0000-0002-3387-7381 FU U.S. Department of Energy, Office of Global Threat Reduction [NA-21]; National Nuclear Security Administration [DE -AC-02-06CH11357] FX This paper contains information obtained from the reduced-size plate tests RERTR-6, -7, and -9 irradiated in the ATR, in the Global Threat Reduction Initiative-Conversion program formerly known as the RERTR program. For design and fabrication of the test samples, Mrs. T. Wiencek, C. Clark, and G. Moore are acknowledged. The physics data were made available by Dr. G. Chang and Ms. M. Lillo at INL. The operation staff at ATR is also acknowledged for the RERTR irradiation tests. The authors appreciate the hands-on PIEs performed at the Materials and Fuels Complex of INL. The authors also thank Dr. J. S. Cheon of KAERI for providing the drawing shown in Fig. 2. This work was supported by the U.S. Department of Energy, Office of Global Threat Reduction (NA-21), National Nuclear Security Administration, under Contract No. DE -AC-02-06CH11357 between UChicago Argonne, LLC and the Department of Energy. NR 61 TC 12 Z9 12 U1 1 U2 6 PU KOREAN NUCLEAR SOC PI DAEJEON PA NUTOPIA BLDG, 342-1 JANGDAE-DONG, DAEJEON, 305-308, SOUTH KOREA SN 1738-5733 J9 NUCL ENG TECHNOL JI Nucl. Eng. Technol. PD DEC PY 2013 VL 45 IS 7 BP 827 EP 838 DI 10.5516/NET.07.2013.713 PG 12 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 289KR UT WOS:000329681900001 ER PT J AU Ryu, HJ Park, JM Jeong, YJ Lee, KH Lee, YS Kim, CK Kim, YS AF Ryu, H. J. Park, J. M. Jeong, Y. J. Lee, K. H. Lee, Y. S. Kim, C. K. Kim, Y. S. TI POST-IRRADIATION ANALYSES OF U-MO DISPERSION FUEL RODS OF KOMO TESTS AT HANARO SO NUCLEAR ENGINEERING AND TECHNOLOGY LA English DT Article DE Irradiation Test; U-Mo Alloys; Post-irradiation Examination; Fuel Performance ID E-FUTURE PLATES; CENTRIFUGAL ATOMIZATION; NONDESTRUCTIVE ANALYSES; LAYER GROWTH; AL-SI; IRRADIATION; ALLOY; PERFORMANCE; MICROSTRUCTURE; INTERDIFFUSION AB Since 2001, a series of five irradiation test campaigns for atomized U-Mo dispersion fuel rods, KOMO-1, -2, -3, -4, and -5, has been conducted at HANARO (Korea) in order to develop high performance low enriched uranium dispersion fuel for research reactors. The KOMO irradiation tests provided valuable information on the irradiation behavior of U-Mo fuel that results from the distinct fuel design and irradiation conditions of the rod fuel for HANARO. Full size U-Mo dispersion fuel rods of 4-5 g-U/cm(3) were irradiated at a maximum linear power of approximately 105 kW/m up to 85% of the initial U-235 depletion burnup without breakaway swelling or fuel cladding failure. Electron probe microanalyses of the irradiated samples showed localized distribution of the silicon that was added in the matrix during fuel fabrication and confirmed its beneficial effect on interaction layer growth during irradiation. The modifications of U-Mo fuel particles by the addition of a ternary alloying element (Ti or Zr), additional protective coatings (silicide or nitride), and the use of larger fuel particles resulted in significantly reduced interaction layers between fuel particles and Al. C1 [Ryu, H. J.] Korea Adv Inst Sci & Technol, Dept Nucl & Quantum Engn, Taejon 305701, South Korea. [Park, J. M.; Jeong, Y. J.; Lee, K. H.; Lee, Y. S.; Kim, C. K.] Korea Atom Energy Res Inst, Res Reactor Fuel Dev Div, Taejon 305353, South Korea. [Kim, Y. S.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Ryu, HJ (reprint author), Korea Adv Inst Sci & Technol, Dept Nucl & Quantum Engn, 291 Daehakro, Taejon 305701, South Korea. EM hojinryu@kaist.ac.kr RI RYU, HO JIN/J-2764-2013 OI RYU, HO JIN/0000-0002-3387-7381 FU National Research Foundation of Korea(NRF); Korea government(MSIP) [2013M2A 8A1041241] FX The authors acknowledge the support of K. H. Kim, D. B. Lee, S. J. Oh, E. S. Kim, S. C. Kweon, and S. J. Jang for the U-Mo powder fabrication; C. G. Seo, C. S. Lee, and H. T. Chae for the neutronic and thermal-hydraulic calculations for the irradiation tests; and Y. H. Jung, Y. S. Choo, D. G. Park, B. O. Yoo, and H. M. Kim for the post, irradiation examination work. This work was supported by the National Research Foundation of Korea(NRF) grant funded by the Korea government(MSIP) (No. 2013M2A 8A1041241). NR 42 TC 7 Z9 7 U1 1 U2 5 PU KOREAN NUCLEAR SOC PI DAEJEON PA NUTOPIA BLDG, 342-1 JANGDAE-DONG, DAEJEON, 305-308, SOUTH KOREA SN 1738-5733 J9 NUCL ENG TECHNOL JI Nucl. Eng. Technol. PD DEC PY 2013 VL 45 IS 7 BP 847 EP 858 DI 10.5516/NET.07.2013.715 PG 12 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 289KR UT WOS:000329681900003 ER PT J AU Chatterjee, P Plesca, D Mazumder, S Boutros, J Yannone, SM Almasan, A AF Chatterjee, Payel Plesca, Dragos Mazumder, Suparna Boutros, Jean Yannone, Steven M. Almasan, Alexandru TI Defective chromatin recruitment and retention of NHEJ core components in human tumor cells expressing a Cyclin E fragment SO NUCLEIC ACIDS RESEARCH LA English DT Article ID DEPENDENT PROTEIN-KINASE; DOUBLE-STRAND BREAKS; DNA-PKCS PHOSPHORYLATIONS; CATALYTIC SUBUNIT; GENOTOXIC STRESS; DAMAGE RESPONSE; REPAIR; END; AUTOPHOSPHORYLATION; RADIATION AB Exposure to genotoxic agents, such as ionizing radiation (IR), produces double-strand breaks, repaired predominantly in mammalian cells by non-homologous end-joining (NHEJ). Ku70 was identified as an interacting partner of a proteolytic Cyclin E (CycE) fragment, p18CycE. p18CycE endogenous generation during IR-induced apoptosis in leukemic cells and its stable expression in epithelial tumor cells sensitized to IR. cH2AX IR-induced foci (IRIFs) and comet assays indicated ineffective NHEJ DNA repair in p18CycE-expressing cells. DNA pull-down and chromatin recruitment assays revealed that retention of NHEJ factors to double-strand breaks, but not recruitment, was diminished. Similarly, IRIFs of phosphorylated T2609 and S2056-DNA-PKcs and its target S1778-53BP1 were greatly decreased in p18CycE-expressing cells. As a result, DNA-PKcs chromatin association was also increased. 53BP1 IRIFs were suppressed when p18CycE was generated in leukemic cells and in epithelial cells stably expressing p18CycE. Ataxia telangiectasia mutated was activated but not its 53BP1 and MDC1 targets. These data indicate a profound influence of p18CycE on NHEJ through its interference with DNA-PKcs conformation and/or dimerization, which is required for effective DNA repair, making the p18CycE-expressing cells more IR sensitive. These studies provide unique mechanistic insights into NHEJ misregulation in human tumor cells, in which defects in NHEJ core components are rare. C1 [Chatterjee, Payel; Plesca, Dragos; Mazumder, Suparna; Boutros, Jean; Almasan, Alexandru] Cleveland Clin, Dept Canc Biol, Lerner Res Inst, Cleveland, OH 44195 USA. [Chatterjee, Payel] Kent State Univ, Sch Biomed Sci, Kent, OH 44234 USA. [Boutros, Jean] Cleveland State Univ, Dept Chem, Cleveland, OH 44115 USA. [Yannone, Steven M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Almasan, Alexandru] Cleveland Clin, Dept Radiat Oncol, Taussig Canc Inst, Cleveland, OH 44195 USA. RP Almasan, A (reprint author), Cleveland Clin, Dept Canc Biol, Lerner Res Inst, Cleveland, OH 44195 USA. EM almasaa@ccf.org OI Almasan, Alex/0000-0002-8916-6650 FU National Institutes of Health (NIH) [CA127264]; US Department of Energy Office of Science [DE-AC02-05CH11231] FX National Institutes of Health (NIH), [CA127264 to A. A.] and by the US Department of Energy Office of Science under contract number [DE-AC02-05CH11231 to S.M.Y.]. Funding for open access: NIH [CA127264]. NR 34 TC 5 Z9 5 U1 0 U2 6 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD DEC PY 2013 VL 41 IS 22 BP 10157 EP 10169 DI 10.1093/nar/gkt812 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 292AQ UT WOS:000329874400020 PM 24021630 ER PT J AU Sheng, J Gan, JH Soares, AS Salon, J Huang, Z AF Sheng, Jia Gan, Jianhua Soares, Alexei S. Salon, Jozef Huang, Zhen TI Structural insights of non-canonical U center dot U pair and Hoogsteen interaction probed with Se atom SO NUCLEIC ACIDS RESEARCH LA English DT Article ID X-RAY CRYSTALLOGRAPHY; LONG NONCODING RNAS; CRYSTAL-STRUCTURE; BASE-PAIR; SELENIUM; ACID; DNA; DERIVATIZATION; COEFFICIENTS; NUCLEOSIDES AB Unlike DNA, in addition to the 2'-OH group, uracil nucleobase and its modifications play essential roles in structure and function diversities of non-coding RNAs. Non-canonical U center dot U base pair is ubiquitous in non-coding RNAs, which are highly diversified. However, it is not completely clear how uracil plays the diversifing roles. To investigate and compare the uracil in U-A and U center dot U base pairs, we have decided to probe them with a selenium atom by synthesizing the novel 4-Se-uridine (U-se) phosphoramidite and Se-nucleobase-modified RNAs (U-se-RNAs), where the exo-4-oxygen of uracil is replaced by selenium. Our crystal structure studies of U-A and U center dot U pairs reveal that the native and Se-derivatized structures are virtually identical, and both U-A and U center dot U pairs can accommodate large Se atoms. Our thermostability and crystal structure studies indicate that the weakened H-bonding in U-A pair may be compensated by the base stacking, and that the stacking of the trans-Hoogsteen U center dot U pairs may stabilize RNA duplex and its junction. Our result confirms that the hydrogen bond (O4...H-C5) of the Hoogsteen pair is weak. Using the Se atom probe, our Se-functionalization studies reveal more insights into the U center dot U interaction and U-participation in structure and function diversification of nucleic acids. C1 [Sheng, Jia; Gan, Jianhua; Salon, Jozef; Huang, Zhen] Georgia State Univ, Dept Chem, Atlanta, GA 30303 USA. [Soares, Alexei S.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Huang, Z (reprint author), Georgia State Univ, Dept Chem, Atlanta, GA 30303 USA. EM huang@gsu.edu RI Soares, Alexei/F-4800-2014 OI Soares, Alexei/0000-0002-6565-8503 FU NIH [R01GM0958811]; Georgia Cancer Coalition (GCC) Distinguished Cancer Clinicians and Scientists FX NIH [R01GM0958811 and Georgia Cancer Coalition (GCC) Distinguished Cancer Clinicians and Scientists. Funding for open access charge: NIH [R01GM0958811 and Georgia Cancer Coalition (GCC) Distinguished Cancer Clinicians and Scientists. NR 55 TC 10 Z9 10 U1 0 U2 9 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD DEC PY 2013 VL 41 IS 22 BP 10476 EP 10487 DI 10.1093/nar/gkt799 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 292AQ UT WOS:000329874400045 PM 24013566 ER PT J AU Chen, Y Balaji, P Vishnu, A AF Chen, Yong Balaji, Pavan Vishnu, Abhinav TI Special issue on programming models, systems software, and tools for High-End Computing SO PARALLEL COMPUTING LA English DT Editorial Material C1 [Chen, Yong] Texas Tech Univ, Dept Comp Sci, Lubbock, TX 79409 USA. [Balaji, Pavan] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Vishnu, Abhinav] Pacific NW Natl Lab, Comp Sci & Math Div, Richland, WA 99352 USA. RP Chen, Y (reprint author), Texas Tech Univ, Dept Comp Sci, Lubbock, TX 79409 USA. EM yong.chen@ttu.edu NR 0 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-8191 EI 1872-7336 J9 PARALLEL COMPUT JI Parallel Comput. PD DEC PY 2013 VL 39 IS 12 SI SI BP 751 EP 752 DI 10.1016/j.parco.2013.09.008 PG 2 WC Computer Science, Theory & Methods SC Computer Science GA 283TD UT WOS:000329269000001 ER PT J AU Tang, W Ren, DX Lan, ZL Desai, N AF Tang, Wei Ren, Dongxu Lan, Zhiling Desai, Narayan TI Toward balanced and sustainable job scheduling for production supercomputers SO PARALLEL COMPUTING LA English DT Article DE Job scheduling; Resource management; Priority balancing; Adaptive policy tuning; Workload characteristic ID STRATEGIES; SYSTEMS AB Job scheduling on production supercomputers is complicated by diverse demands of system administrators and amorphous characteristics of workloads. Specifically, various scheduling goals such as queuing efficiency and system utilization are usually conflicting and thus need to be balanced. Also, changing workload characteristics often impact the effectiveness of the deployed scheduling policies. Thus it is challenging to design a versatile scheduling policy that is effective in all circumstances. In this paper, we propose a novel job scheduling strategy to balance diverse scheduling goals and mitigate the impact of workload characteristics. First, we introduce metric-aware scheduling, which enables the scheduler to balance competing scheduling goals represented by different metrics such as job waiting time, fairness, and system utilization. Second, we design a scheme to dynamically adjust scheduling policies based on feedback information of monitored metrics at runtime. We evaluate our design using real workloads from supercomputer centers. The results demonstrate that our scheduling mechanism can significantly improve system performance in a balanced, sustainable fashion. (C) 2013 Elsevier B.V. All rights reserved. C1 [Tang, Wei; Desai, Narayan] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Ren, Dongxu; Lan, Zhiling] IIT, Dept Comp Sci, Chicago, IL 60616 USA. RP Tang, W (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wtang@mcs.anl.gov; dren1@iit.edu; lan@iit.edu; desai@mcs.anl.gov FU National Science Foundation [CNS-0720549, CCF-0702737]; U.S. Department of Energy [DE-AC02-06CH11357] FX This work is supported in part by National Science Foundation grants CNS-0720549 and CCF-0702737. The work at Argonne National Laboratory is supported by the U.S. Department of Energy under Contract DE-AC02-06CH11357. NR 26 TC 2 Z9 2 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-8191 EI 1872-7336 J9 PARALLEL COMPUT JI Parallel Comput. PD DEC PY 2013 VL 39 IS 12 SI SI BP 753 EP 768 DI 10.1016/j.parco.2013.08.007 PG 16 WC Computer Science, Theory & Methods SC Computer Science GA 283TD UT WOS:000329269000002 ER PT J AU Steinfadt, S AF Steinfadt, Shannon TI Fine-grained parallel implementations for SWAMP plus Smith-Waterman alignment SO PARALLEL COMPUTING LA English DT Article DE SIMD Parallel computing; Bioinformatics; Parallel co-processor; FPGAs; Sequence alignment; Smith-Waterman ID DATABASE SEARCHES; SPEED-UP; ALGORITHM; SEQUENCES AB More sensitive than heuristic methods for searching biological databases, the Smith-Waterman algorithm is widely used but has the drawback of a high quadratic running time. The faster approach extends Smith-Waterman using Associative Massive Parallelism (SWAMP+) for three different parallel architectures: ASsociative Computing (ASC), the ClearSpeed coprocessor, and the Convey Computer FPGA coprocessor. We show that parallel versions of Smith-Waterman can be successfully modified to produce multiple BLAST-like sub-alignments while maintaining the original precision. SWAMP+ combines parallelism and the novel extension producing multiple sub-alignments for pairwise comparisons. Two parallel SWAMP+ implementations for the ASC model and the ClearSpeed CSX-620 use a wavefront approach. Both perform a full traceback in parallel memory, returning multiple sub-alignments. Results show a linear speedup for the 96 processing elements (PEs) on a single ClearSpeed chip. The third SWAMP+ adaptation uses the non-associative Convey Computer FPGA coprocessor. The hybrid system has a Smith-Waterman algorithm suite designed to produce high-speed, high-throughput alignments, optimized for large databases. The Convey Computer Smith-Waterman algorithm suite was extended to produce the additional SWAMP+ sub-alignments efficiently. The parallel sequence alignment algorithms were designed for three different computer systems, all of which contain extensions to produce multiple, additional sub-alignments. This work creates a speedup while providing a deeper exploration of the matched query sequences previously unavailable. (C) 2013 Elsevier B.V. All rights reserved. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Steinfadt, S (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM shannon@lanl.gov NR 40 TC 1 Z9 1 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-8191 EI 1872-7336 J9 PARALLEL COMPUT JI Parallel Comput. PD DEC PY 2013 VL 39 IS 12 SI SI BP 819 EP 833 DI 10.1016/j.parco.2013.08.008 PG 15 WC Computer Science, Theory & Methods SC Computer Science GA 283TD UT WOS:000329269000006 ER PT J AU Farrell, WM Hurley, DM Hodges, RR Killen, RM Halekas, JS Zimmerman, MI Delory, GT AF Farrell, W. M. Hurley, D. M. Hodges, R. R. Killen, R. M. Halekas, J. S. Zimmerman, M. I. Delory, G. T. TI Redistribution of lunar polar water to mid-latitudes and its role in forming an OH veneer SO PLANETARY AND SPACE SCIENCE LA English DT Article; Proceedings Paper CT Workshop on Dust, Atmospheres, and Plasma - The Moon and Small Bodies (DAP) CY JUN 06-08, 2012 CL Boulder, CO SP NASA Lunar Sci Inst, Colorado Ctr Lunar Dust & Atmospher Studies, Moon Express, Ball Aerosp & Technologies Corp, Lockheed Martin Corp DE Moon; Lunar poles; Sputtering; Impact vaporization; Desorption; Transport ID MOON; ICE; REGIONS; ATMOSPHERE; MERCURY AB We suggest that energization processes like ion sputtering and impact vaporization can eject/release polar water molecules residing within cold trapped regions with sufficient velocity to allow their redistribution to mid-latitudes. We consider the possibility that these polar-ejected molecules can contribution to the water/OH veneer observed as a 3 mu m IR absorption feature at mid-latitudes by Chandrayaan-1, Cassini, and EPDXI. We find this source cannot fully account for the observed IR feature, but could be a low intensity additional source. Published by Elsevier Ltd. C1 [Farrell, W. M.; Killen, R. M.; Zimmerman, M. I.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Hurley, D. M.] Johns Hopkins Applied Phys Lab, Laurel, MD USA. [Hodges, R. R.] Univ Colorado, Boulder, CO 80309 USA. [Halekas, J. S.; Delory, G. T.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Farrell, W. M.; Hurley, D. M.; Hodges, R. R.; Killen, R. M.; Halekas, J. S.; Zimmerman, M. I.; Delory, G. T.] NASA, Lunar Sci Inst, Moffett Field, CA USA. [Zimmerman, M. I.] Oak Ridge Associated Univ, Oak Ridge, TN USA. RP Farrell, WM (reprint author), NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. EM william.m.farrell@nasa.gov RI Farrell, William/I-4865-2013; Hurley, Dana/F-4488-2015; OI Hurley, Dana/0000-0003-1052-1494; Halekas, Jasper/0000-0001-5258-6128 NR 30 TC 7 Z9 7 U1 0 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0032-0633 J9 PLANET SPACE SCI JI Planet Space Sci. PD DEC PY 2013 VL 89 BP 15 EP 20 DI 10.1016/j.pss.2013.05.009 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 287QW UT WOS:000329558300003 ER PT J AU Celina, MC AF Celina, Mathew C. TI Review of polymer oxidation and its relationship with materials performance and lifetime prediction SO POLYMER DEGRADATION AND STABILITY LA English DT Review DE Accelerated polymer aging; Lifetime prediction; Thermal oxidation; Polymer degradation; Arrhenius extrapolation; Diffusion limited oxidation ID DIFFUSION-LIMITED OXIDATION; NON-ARRHENIUS BEHAVIOR; DEGRADATION-INDUCED EMBRITTLEMENT; THERMAL-OXIDATION; THERMOGRAVIMETRIC DATA; POLYPROPYLENE FILMS; THERMOOXIDATIVE DEGRADATION; PROFLUORESCENT NITROXIDES; STABILIZED POLYPROPYLENE; SOLID POLYPROPYLENE AB All polymers are intrinsically susceptible to oxidation, which is the underlying process for thermally driven materials degradation and of concern in various applications. There are many approaches for predicting oxidative polymer degradation. Aging studies usually are meant to accelerate oxidation chemistry for predictive purposes. Kinetic models attempt to describe reaction mechanisms and derive rate constants, whereas rapid qualification tests should provide confidence for extended performance during application, and similarly TGA tests are meant to provide rapid guidance for thermal degradation features. What are the underlying commonalities or diverging trends and complications when we approach thermo-oxidative aging of polymers in such different ways? This review presents a brief status report on the important aspects of polymer oxidation and focuses on the complexity of thermally accelerated polymer aging phenomena. Thermal aging and lifetime prediction, the importance of DLO, property correlations, kinetic models, TGA approaches, and a framework for predictive aging models are briefly discussed. An overall perspective is provided showing the challenges associated with our understanding of polymer oxidation as it relates to lifetime prediction requirements. Published by Elsevier Ltd. C1 Sandia Natl Labs, Mat Characterizat & Performance Dept 1819, Albuquerque, NM 87185 USA. RP Celina, MC (reprint author), Sandia Natl Labs, Mat Characterizat & Performance Dept 1819, POB 5800,MS 1411, Albuquerque, NM 87185 USA. EM mccelin@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This paper is an invited contribution based on a plenary address given at the 2012 MODEST conference. All previous and current collaborators, colleagues, mentors, technical staff and students are gratefully acknowledged. Adam Quintana is recognized for creative approaches to DLO modeling. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 122 TC 51 Z9 52 U1 20 U2 116 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0141-3910 EI 1873-2321 J9 POLYM DEGRAD STABIL JI Polym. Degrad. Stabil. PD DEC PY 2013 VL 98 IS 12 BP 2419 EP 2429 DI 10.1016/j.polymdegradstab.2013.06.024 PG 11 WC Polymer Science SC Polymer Science GA 285FT UT WOS:000329379800004 ER PT J AU Von White, G Clough, RL Hochrein, JM Bernstein, R AF Von White, Gregory, II Clough, Roger L. Hochrein, James M. Bernstein, Robert TI Application of isotopic labeling, and gas chromatography mass spectrometry, to understanding degradation products and pathways in the thermal-oxidative aging of Nylon 6.6 SO POLYMER DEGRADATION AND STABILITY LA English DT Article DE Thermal-oxidative degradation; Nylon; Polyamide; Isotopic labels; Free radical mechanisms; Volatile products ID SOLID-PHASE MICROEXTRACTION; THERMOOXIDATIVE DEGRADATION; PARAMAGNETIC RESONANCE; ALIPHATIC POLYAMIDES; POLYPROPYLENE; PYROLYSIS; INSIGHTS; GC/MS; 2-CYCLOPENTYL-CYCLOPENTANONE; CHEMILUMINESCENCE AB Nylon 6.6 containing C-13 isotopic labels at specific positions along the macromolecular backbone has been subjected to extensive thermal-oxidative aging at 138 degrees C for time periods up to 243 days. In complementary experiments, unlabeled Nylon 6.6 was subjected to the same aging conditions under an atmosphere of O-18(2). Volatile organic degradation products were analyzed by cryofocusing gas chromatography mass spectrometry (cryo-GC/MS) to identify the isotopic labeling. The labeling results, combined with basic considerations of free radical reaction chemistry, provided insights to the origin of degradation species, with respect to the macromolecular structure. A number of inferences on chemical mechanisms were drawn, based on 1) the presence (or absence) of the isotopic labels in the various products, 2) the location of the isotope within the product molecule, and 3) the relative abundance of products as indicated by large differences in peak intensities in the gas chromatogram. The overall degradation results can be understood in terms of free radical pathways originating from initial attacks on three different positions along the nylon chain which include hydrogen abstraction from: the (CH2) group adjacent to the nitrogen atom, at the (CH2) adjacent the carbonyl group, and direct radical attack on the carbonyl. Understanding the pathways which lead to Nylon 6.6 degradation ultimately provides new insight into changes that can be leveraged to detect and reduce early aging and minimize problems associated with material degradation. Published by Elsevier Ltd. C1 [Von White, Gregory, II; Clough, Roger L.; Hochrein, James M.; Bernstein, Robert] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Von White, G (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM gvwhite@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Special thanks are given to John L Schroeder, Michael I. White, Donald R. Bradley, and Jonell N. Smith for their contributions to this work. NR 36 TC 2 Z9 2 U1 6 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0141-3910 EI 1873-2321 J9 POLYM DEGRAD STABIL JI Polym. Degrad. Stabil. PD DEC PY 2013 VL 98 IS 12 BP 2452 EP 2465 DI 10.1016/1.polymdegradstab.2013.08.029 PG 14 WC Polymer Science SC Polymer Science GA 285FT UT WOS:000329379800008 ER PT J AU Croft, S Burr, TL Favalli, A AF Croft, S. Burr, T. L. Favalli, A. TI Estimating the half-life of Pu-241 and its uncertainty SO RADIATION MEASUREMENTS LA English DT Article DE Pu-241 decay; Estimation of half-life; Inconsistent measurements; Measurement error model selection; Uncertainty analysis; Data evaluation AB Measuring the double isotope atomic abundance ratio as function of time of a homogenized stock of plutonium using mass spectroscopy provides a means to estimate the half-life of Pu-241, denoted here as t(1/2,241). After a logarithmic transformation, estimating t(1/2,241) along with a justifiable associated uncertainty is reduced to the analysis of a linear relationship, as illustrated in this paper using 15 published data pairs (time, log(double isotope ratio)) of Wellum et al. (2009) that span approximately 31 years (greater than two half-lives). However, as noted by Wellum et al. (2009), the published 15 data pairs exhibit inconsistencies that indicate possible underestimation of individual experimental uncertainties. Similar inconsistencies often arise in multi-experiment comparisons of the same estimated quantity, typically because some components of uncertainty such as individual experimental biases are difficult to identify and assess. It is therefore an important and common problem. In such cases the experimental data must be supplemented with other information to make plausible uncertainty estimates. We therefore analyze the data pairs under several different assumptions regarding total experimental uncertainties and show quantitatively that the best estimate of t(1/2,241) and of its uncertainty depend on the assumptions regarding experimental uncertainties. It is unlikely in this context that the 15 data pairs and associated estimated experimental uncertainties could guide one toward a very certain choice among the reasonable sets of assumptions regarding total experimental uncertainties. Thus a definitive recommendation cannot be singled out. Fortunately, the best estimates and associated uncertainties arising from different yet tenable assumptions regarding experimental uncertainties are all in reasonably close agreement. And, one of those best estimates we provide (with approximately 95% confidence limits) is (14.329 +/- 0.006[fit] +/- 0.029[bias]) years, which uses similar data stratification arguments as in Wellum et al. (2009) but a completely different approach. Furthermore, this estimate of t(1/2,241) agrees closely with the value recommended in Wellum et al. (2009) of (14.325 +/- 0.024) years. We conclude that the value of t(1/2,241) supported by the available data is robust, despite evidence of some non-ideal behavior, and that alternative means of estimating t(1/2,241) and its uncertainty yield reasonably similar results. (c) 2013 Published by Elsevier Ltd. C1 [Croft, S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Burr, T. L.; Favalli, A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Croft, S (reprint author), Oak Ridge Natl Lab, POB 2008,MS-6166, Oak Ridge, TN 37831 USA. EM crofts@ornl.gov; tburr@lanl.gov; afavalli@lanl.gov NR 13 TC 5 Z9 5 U1 1 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1350-4487 J9 RADIAT MEAS JI Radiat. Meas. PD DEC PY 2013 VL 59 BP 94 EP 102 DI 10.1016/j.radmeas.2013.04.010 PG 9 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 285UY UT WOS:000329421700014 ER PT J AU Clark, RA Robertson, JD Schwantes, JM AF Clark, Richard A. Robertson, J. David Schwantes, Jon M. TI Intrinsic dosimetry: Elemental composition effects on the thermoluminescence of commercial borosilicate glass SO RADIATION MEASUREMENTS LA English DT Article DE Borosilicate glass; Intrinsic dosimetry; Thermoluminescence; Nuclear forensics; Elemental analysis; Multivariate analysis ID GAMMA-IRRADIATED PYREX; ALUMINOSILICATE GLASSES; GLOW CURVES; LUMINESCENCE; SPECTROSCOPY; CENTERS; ESR AB Intrinsic dosimetry is the method of measuring total absorbed dose received by the walls of a container holding radioactive material. By considering this dose in tandem with the physical characteristics of the radioactive material housed within the container, this method can provide enhanced pathway information for interdicted radioactive samples. Thermoluminescence (TL) dosimetry was used to measure ionizing radiation dose effects on stock borosilicate glass. Differences in TL glow curve shape and intensity were observed for glasses from different geographical origins. The different TL signatures strongly correlated with the concentration of alkaline earth metals and the ratio of sodium to the total amount of alkali metal present in the borosilicate glass. Published by Elsevier Ltd. C1 [Clark, Richard A.; Robertson, J. David] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Clark, Richard A.; Schwantes, Jon M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Clark, RA (reprint author), Idaho Natl Lab, POB 1625,MS 6180, Idaho Falls, ID 83415 USA. EM richard.clark@inl.gov; robertsonjo@missouri.edu; jon.schwantes@pnnl.gov FU National Technical Nuclear Forensics Center (NTNFC), part of the Domestic Nuclear Detection Office (DNDO) within the Department of Homeland Security; DOE by Battelle [DE-AC05-76RL1830]; U.S. Department of Homeland Security, Domestic Nuclear Detection Office; U.S. Department of Defense, Defense Threat Reduction Agency; Idaho National Laboratory under DOE Idaho Operations Office [DE- 07-05ID14517] FX This research was sponsored by the National Technical Nuclear Forensics Center (NTNFC), part of the Domestic Nuclear Detection Office (DNDO), within the Department of Homeland Security and conducted at the U.S. Department of Energy's Pacific Northwest National Laboratory (PNNL), which is operated for DOE by Battelle under Contract DE-AC05-76RL1830. This research was performed under the Nuclear Forensics Graduate Fellowship Program, which is sponsored by the U.S. Department of Homeland Security, Domestic Nuclear Detection Office and the U.S. Department of Defense, Defense Threat Reduction Agency. Support from Idaho National Laboratory under DOE Idaho Operations Office Contract DE- 07-05ID14517 was provided during the preparation of this article. NR 51 TC 2 Z9 2 U1 0 U2 3 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1350-4487 J9 RADIAT MEAS JI Radiat. Meas. PD DEC PY 2013 VL 59 BP 270 EP 276 DI 10.1016/j.radmeas.2013.07.002 PG 7 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 285UY UT WOS:000329421700041 ER PT J AU Liu, HJ Dai, S Jiang, DE AF Liu, Hongjun Dai, Sheng Jiang, De-en TI Permeance of H-2 through porous graphene from molecular dynamics SO SOLID STATE COMMUNICATIONS LA English DT Article DE Porous graphene; Gas permeation; Molecular dynamics ID NANOPOROUS GRAPHENE; GAS SEPARATION; MEMBRANES; TRANSPORT AB A recent experiment (Koenig et al., 2012 [151) demonstrated the capability of porous graphene as one-atom-thin membrane to separate gases by molecular sieving. A quantitative connection between the measured leak rate and the simulated gas permeance has yet to be established. Using H-2 as a model gas, here we determine its permeance through porous graphene from molecular dynamics (MD) simulations. Trajectories are used to directly obtain H-2 flux, pressure drop across the graphene membrane, and subsequently, H-2 permeance. The permeance is determined to be on the order of 10(5) GPU (gas permeance unit) for pressure driving forces ranging from 2 to 163 atm. By relating to the experimental leak rate, we then use the permeation data to estimate the pore density in the experimentally created porous graphene. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Liu, Hongjun; Dai, Sheng; Jiang, De-en] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37966 USA. RP Jiang, DE (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM jiangd@ornl.gov RI Jiang, De-en/D-9529-2011; Liu, Hongjun /A-2100-2012; Dai, Sheng/K-8411-2015 OI Jiang, De-en/0000-0001-5167-0731; Liu, Hongjun /0000-0003-3326-2640; Dai, Sheng/0000-0002-8046-3931 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy. This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the US Department of Energy under Contract no. DE-AC02-05CH11231. NR 22 TC 18 Z9 19 U1 2 U2 68 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-1098 J9 SOLID STATE COMMUN JI Solid State Commun. PD DEC PY 2013 VL 175 SI SI BP 101 EP 105 DI 10.1016/j.ssc.2013.07.004 PG 5 WC Physics, Condensed Matter SC Physics GA 287JN UT WOS:000329538200013 ER PT J AU Mahadevapuram, RC Carr, JA Chen, YQ Bose, S Nalwa, KS Petrich, JW Chaudharya, S AF Mahadevapuram, Rakesh C. Carr, John A. Chen, Yuqing Bose, Sayantan Nalwa, Kanwar S. Petrich, Jacob W. Chaudharya, Sumit TI Low-boiling-point solvent additives can also enable morphological control in polymer solar cells SO SYNTHETIC METALS LA English DT Article DE Organic solar cells; Solvent additives; Morphology ID EFFICIENCY; PERFORMANCE AB Processing organic photovoltaic (OPV) blend solutions with high-boiling-point solvent additives has recently been used for morphological control in bulk-heterojunction OPV cells. Here we show that even low-boiling-point solvents can be effective additives. When P3HT:PCBM OPV cells were processed with a low-boiling-point solvent tetrahydrafuran as an additive in parent solvent o-dichlorobenzene, charge extraction increased leading to fill factors as high as 69.5%, without low work-function cathodes, electrode buffer layers or thermal treatment. This was attributed to PCBM demixing from P3HT domains and better vertical phase separation, as indicated by photoluminescence lifetimes, hole mobilities, and shunt leakage currents. Dependence on solvent parameters and applicability beyond P3HT system was also investigated. (C) 2013 Elsevier B.V. All rights reserved. C1 [Mahadevapuram, Rakesh C.; Chaudharya, Sumit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Carr, John A.; Chen, Yuqing; Nalwa, Kanwar S.; Chaudharya, Sumit] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Bose, Sayantan; Petrich, Jacob W.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Bose, Sayantan; Petrich, Jacob W.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Chaudharya, S (reprint author), Iowa State Univ, 2124 Coover Hall, Ames, IA 50011 USA. EM sumitc@iastate.edu RI Petrich, Jacob/L-1005-2015 FU National Science Foundation [ECCS-1055930]; U.S. Department of Energy, Office of Basic Energy Sciences, through the Ames Laboratory; U.S. Department of Energy by Iowa State University [DE-ACO2-07CH11358] FX This work was primarily (experimental design, device fabrication and characterization) supported by National Science Foundation (ECCS-1055930). PL lifetime studies were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, through the Ames Laboratory. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-ACO2-07CH11358. NR 15 TC 5 Z9 5 U1 0 U2 25 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0379-6779 J9 SYNTHETIC MET JI Synth. Met. PD DEC 1 PY 2013 VL 185 BP 115 EP 119 DI 10.1016/j.synthmet.2013.10.004 PG 5 WC Materials Science, Multidisciplinary; Physics, Condensed Matter; Polymer Science SC Materials Science; Physics; Polymer Science GA 287NE UT WOS:000329547700018 ER PT J AU Yuan, Y Chen, S Paunesku, T Gleber, SC Liu, WC Doty, CB Mak, R Deng, JJ Jin, QL Lai, B Brister, K Flachenecker, C Jacobsen, C Vogt, S Woloschak, GE AF Yuan, Ye Chen, Si Paunesku, Tatjana Gleber, Sophie Charlotte Liu, William C. Doty, Caroline B. Mak, Rachel Deng, Junjing Jin, Qiaoling Lai, Barry Brister, Keith Flachenecker, Claus Jacobsen, Chris Vogt, Stefan Woloschak, Gayle E. TI Epidermal Growth Factor Receptor Targeted Nuclear Delivery and High-Resolution Whole Cell X-ray Imaging of Fe3O4@TiO2 Nanoparticles in Cancer Cells SO ACS NANO LA English DT Article DE nanoparticles; titanium dioxide; photoactivation; X-ray fluorescence microscopy; epidermal growth factor receptor ID DNA-DAMAGE; COMET ASSAY; TIO2 NANOPARTICLES; OVARIAN-CANCER; EGF RECEPTOR; FLUORESCENCE MICROSCOPY; SIGNALING NETWORK; PROGNOSTIC VALUE; GENE-EXPRESSION; LOCALIZATION AB Sequestration within the cytoplasm often limits the efficacy of therapeutic nanoparticles that have specific subcellular targets. To allow for both cellular and subcellular nanoparticle delivery, we have created epidermal growth factor receptor (EGFR)targeted Fe3O4@TiO2 nanoparticles that use the native intracellular trafficking of EGFR to improve internalization and nuclear translocation in EGFR-expressing He La cells. While bound to EGFR, these nanoparticles do not interfere with the interaction between EGFR and karyopherin-beta, a protein that is critical for the translocation of ligand-bound EGFR to the nucleus. Thus, a portion of the EGFR-targeted nanoparticles taken up by the cells also reaches cell nuclei. We were able to track nanoparticle accumulation in cells by flow cytometry and nanoparticle subcellular distribution by confocal fluorescent microscopy indirectly, using fluorescently labeled nanoparticles. More importantly, we imaged and quantified intracellular nanoparticles directly, by their elemental signatures, using X-ray fluorescence microscopy at the Bionanoprobe, the first instrument of its kind in the world. The Bionanoprobe can focus hard X-rays down to a 30 nm spot size to map the positions of chemical elements tomographically within whole frozen-hydrated cells. Finally, we show that photoactivation of targeted nanoparticles in cell nuclei, dependent on successful EGFR nuclear accumulation, induces significantly more double-stranded DNA breaks than photoactivation of nanoparticles that remain exclusively in the cytoplasm. C1 [Yuan, Ye; Paunesku, Tatjana; Liu, William C.; Doty, Caroline B.; Woloschak, Gayle E.] Northwestern Univ, Dept Radiat Oncol, Chicago, IL 60611 USA. [Chen, Si; Gleber, Sophie Charlotte; Jin, Qiaoling; Lai, Barry; Jacobsen, Chris; Vogt, Stefan] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Mak, Rachel; Deng, Junjing; Jacobsen, Chris] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Brister, Keith] Northwestern Synchrotron Res Ctr, Argonne, IL 60439 USA. [Flachenecker, Claus] Carl Zeiss Xray Microscopy, Pleasanton, CA 94588 USA. RP Woloschak, GE (reprint author), Northwestern Univ, Dept Radiat Oncol, Chicago, IL 60611 USA. EM g-woloschak@northwestern.edu RI Jacobsen, Chris/E-2827-2015; Vogt, Stefan/B-9547-2009; Vogt, Stefan/J-7937-2013; Paunesku, Tatjana/A-3488-2017; Woloschak, Gayle/A-3799-2017 OI Jacobsen, Chris/0000-0001-8562-0353; Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513; Paunesku, Tatjana/0000-0001-8698-2938; Woloschak, Gayle/0000-0001-9209-8954 FU National Institutes of Health [CA107467, EB002100, U54CA119341, GM104530]; NIH/NCI [T32CA09560]; NCI CCSG [P30 CA060553]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NIH ARRA grant [SP0007167] FX This research was supported by the National Institutes of Health under the grant numbers CA107467, EB002100, U54CA119341, and GM104530. Y.Y. was supported in part by NIH/NCI training grant T32CA09560. Flow cytometry was performed at the Northwestern University RHLCCC Flow Cytometry Facility, and confocal microscopy was performed at the Northwestern University Cell Imaging Facility generously supported by NCI CCSG P30 CA060553 awarded to the Robert H. Lurie Comprehensive Cancer Center. Work at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, contract no. DE-AC02-06CH11357. Implementation of the Bionanoprobe is supported by NIH ARRA grant SP0007167. The authors thank Drs. R. Bergan, T. L. Chew, B. Hornberger, R. Omary, and J. Ward for valuable discussions and advice. NR 96 TC 35 Z9 35 U1 6 U2 99 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD DEC PY 2013 VL 7 IS 12 BP 10502 EP 10517 DI 10.1021/nn4033294 PG 16 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 281YO UT WOS:000329137100009 PM 24219664 ER PT J AU Scanlan, LD Reed, RB Loguinov, AV Antczak, P Tagmount, A Aloni, S Nowinski, DT Luong, P Tran, C Karunaratne, N Pham, D Lin, XX Falciani, F Higgins, CP Ranville, JF Vulpe, CD Gilbert, B AF Scanlan, Leona D. Reed, Robert B. Loguinov, Alexandre V. Antczak, Philipp Tagmount, Abderrahmane Aloni, Shaul Nowinski, Daniel Thomas Luong, Pauline Tran, Christine Karunaratne, Nadeeka Don Pham Lin, Xin Xin Falciani, Francesco Higgins, Christopher P. Ranville, James F. Vulpe, Chris D. Gilbert, Benjamin TI Silver Nanowire Exposure Results in Internalization and Toxicity to Daphnia magna SO ACS NANO LA English DT Article DE silver; nanowire; ecotoxicology; Daphnia magna; acute toxicity; transcriptomics; single-particle inductively coupled plasma mass spectrometry ID CARBON NANOTUBES; IN-VITRO; ELECTRON-MICROSCOPY; ZNO NANOPARTICLES; ZEBRAFISH EMBRYOS; GENE-EXPRESSION; SHEDDING LIGHT; THIN-FILMS; SINGLE; CELLS AB Nanowires (NWs), high-aspect-ratio nanomaterials, are increasingly used in technological materials and consumer products and may have toxicological characteristics distinct from nanoparticles. We carried out a comprehensive evaluation of the physicochemical stability of four silver nanowires (AgNWs) of two sizes and coatings and their toxicity to Daphnia magna. Inorganic aluminum-doped silica coatings were less effective than organic poly(vinyl pyrrolidone) coatings at preventing silver oxidation or Ag+ release and underwent a significant morphological transformation within 1 h following addition to low ionic strength Daphnia growth media. All AgNWs were highly toxic to D. magna but less toxic than ionic silver. Toxicity varied as a function of AgNW dimension, coating, and solution chemistry. Ag+ release in the media could not account for observed AgNW toxicity. Single-particle inductively coupled plasma mass spectrometry distinguished and quantified dissolved and nanoparticulate silver in microliter-scale volumes of Daphnia magna hemolymph with a limit of detection of approximately 10 ppb. The silver levels within the hemolymph of Daphnia exposed to both Ag+ and AgNW met or exceeded the initial concentration in the growth medium, indicating effective accumulation during filter feeding. Silver-rich particles were the predominant form of silver in hemolymph following exposure to both AgNWs and Ag+. Scanning electron microscopy imaging of dried hemolymph found both AgNWs and silver precipitates that were not present in the AgNW stock or the growth medium. Both organic and inorganic coatings on the AgNW were transformed during ingestion or absorption. Pathway, gene ontology, and clustering analyses of gene expression response indicated effects of AgNWs distinct from ionic silver on Daphnia magna. C1 [Scanlan, Leona D.; Loguinov, Alexandre V.; Tagmount, Abderrahmane; Nowinski, Daniel Thomas; Luong, Pauline; Tran, Christine; Karunaratne, Nadeeka; Don Pham; Lin, Xin Xin; Vulpe, Chris D.] Univ Calif Berkeley, Dept Nutr Sci & Toxicol, Berkeley, CA 94720 USA. [Reed, Robert B.; Ranville, James F.] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Antczak, Philipp; Falciani, Francesco] Univ Liverpool, Ctr Computat Biol & Modeling, Inst Integrat Biol, Liverpool L69 7ZB, Merseyside, England. [Aloni, Shaul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Div Mat Sci, Berkeley, CA 94720 USA. [Higgins, Christopher P.] Colorado Sch Mines, Dept Civil & Environm Engn, Golden, CO 80401 USA. [Gilbert, Benjamin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Vulpe, CD (reprint author), Univ Calif Berkeley, Dept Nutr Sci & Toxicol, 119 Morgan Hall, Berkeley, CA 94720 USA. EM vulpe@berkeley.edu RI Higgins, Christopher/B-1836-2010; Gilbert, Benjamin/E-3182-2010; Foundry, Molecular/G-9968-2014; OI Higgins, Christopher/0000-0001-6220-8673; ranville, james/0000-0002-4347-4885 FU Center of Integrated Nanomechanical Systems under NSF [EEC-0832819]; NIH Grand Opportunities (RC2) program through NANO-GO NIEHS [DE-FG02-08ER64613]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; [RC2 ES018812] FX This work was funded by the Center of Integrated Nanomechanical Systems under NSF Grant Number EEC-0832819 and by NIH Grand Opportunities (RC2) program through NANO-GO NIEHS Grant DE-FG02-08ER64613. B.G. was supported by RC2 ES018812 to C.V. Part of this work was performed at the Molecular Foundry in Lawrence Berkeley National Laboratory and was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank W. Mickelson for acquiring the TEM image of Figure la. We thank R. Celestre for access to the Nikon microscope. NR 81 TC 38 Z9 38 U1 13 U2 118 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD DEC PY 2013 VL 7 IS 12 BP 10681 EP 10694 DI 10.1021/nn4034103 PG 14 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 281YO UT WOS:000329137100026 PM 24099093 ER PT J AU Goldstein, AP Andrews, SC Berger, RF Radmilovic, VR Neaton, JB Yang, PD AF Goldstein, Anna P. Andrews, Sean C. Berger, Robert F. Radmilovic, Velimir R. Neaton, Jeffrey B. Yang, Peidong TI Zigzag Inversion Domain Boundaries in Indium Zinc Oxide-Based Nanowires: Structure and Formation SO ACS NANO LA English DT Article DE nanowires; EELS; crystal structure; zinc oxide; indium diffusion ID RESOLUTION ELECTRON-MICROSCOPY; HOMOLOGOUS COMPOUNDS; OPTICAL-PROPERTIES; DEFECT STRUCTURES; ZNO-IN2O3 SYSTEM; DIFFUSION; CRYSTALLINE; IRON AB Existing models for the crystal structure of indium zinc oxide (In) and indium iron zinc oxide (IFZO) conflict with electron microscopy data. We propose a model based on imaging and spectroscopy of IZO and IFZO nanowires and verify it using density functional theory. The model features a {1 (2) over bar 1l} "zigzag" layer, which is an inversion domain boundary containing 5-coordinate indium and/or iron atoms. Higher values are observed for greater proportion of iron. We suggest a mechanism of formation in which the basal inclusion and the zigzag diffuse inward together from the surface of the nanowire. C1 [Goldstein, Anna P.; Andrews, Sean C.; Yang, Peidong] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Yang, Peidong] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Berger, Robert F.; Radmilovic, Velimir R.; Neaton, Jeffrey B.; Yang, Peidong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Radmilovic, Velimir R.] Univ Belgrade, Fac Technol & Met, Nanotechnol & Funct Mat Ctr, Belgrade 11120, Serbia. RP Yang, PD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM p_yang@berkeley.edu RI Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014; OI Neaton, Jeffrey/0000-0001-7585-6135; Goldstein, Anna/0000-0002-2710-8228 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Ministry of Education and Science of Republic of Serbia [172054] FX Work performed at NCEM and the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. V.R.R. also acknowledges supports of Ministry of Education and Science of Republic of Serbia, under contract No. 172054. NR 29 TC 5 Z9 5 U1 4 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD DEC PY 2013 VL 7 IS 12 BP 10747 EP 10751 DI 10.1021/nn403836d PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 281YO UT WOS:000329137100033 PM 24237264 ER PT J AU Dong, AG Jiao, YC Milliron, DJ AF Dong, Angang Jiao, Yucong Milliron, Delia J. TI Electronically Coupled Nanocrystal Super lattice Films by in Situ Ligand Exchange at the Liquid-Air Interface SO ACS NANO LA English DT Article DE nanocrystal superlattices; ligand exchange; electronic coupling; in situ treatment; nanocrystal devices; liquid-air interface ID QUANTUM-DOT SOLIDS; COLLOIDAL NANOCRYSTALS; FACILE SYNTHESIS; SURFACE LIGANDS; SUPERLATTICES; NANOPARTICLES; PBSE; FABRICATION; TRANSISTORS; ASSEMBLIES AB The ability to remove long, insulating ligands from nanocrystal (NC) surfaces without deteriorating the structural integrity of NC films is critical to realizing their electronic and optoelectronic applications. Here we report a nondestructive ligand-exchange approach based on in situ chemical treatment of NCs floating at the liquid air interface, enabling strongly coupled NC superlattice films that can be directly transferred to arbitrary substrates for device applications. Ligand-exchange-induced structural defects such as cracks and degraded NC ordering that are commonly observed using previous methods are largely prevented by performing ligand exchange at the liquid air interface. The significantly reduced interparticle spacing arising from ligand replacement leads to highly conductive NC superlattice films, the electrical conductivities and carrier mobilities of which are 1 order of magnitude higher than those of the same NC films subject to substrate-supported exchange using previously reported procedures. The in situ, free-floating exchange approach presented here opens the door for electronically coupled NC superlattices that hold great promise for high-performance, flexible electronic and optoelectronic devices. C1 [Dong, Angang] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China. [Jiao, Yucong] Fudan Univ, Dept Macromol Sci, Shanghai 200433, Peoples R China. [Dong, Angang; Milliron, Delia J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Milliron, Delia J.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. RP Dong, AG (reprint author), Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China. EM agdong@fudan.edu.cn RI Dong, Angang/C-5308-2014; Milliron, Delia/D-6002-2012; Foundry, Molecular/G-9968-2014; OI Dong, Angang/0000-0002-9677-8778 FU U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; DOE Early Career Research Program; Fudan University; Natural National Science Foundation of China [21373052]; 973 Program [2013CB934101, 2014CB845602] FX Work was performed at the Molecular Foundry, Lawrence Berkeley National Laboratory and was supported by the U.S. Department of Energy (DOE) under contract no. DE-AC02-05CH11231. D.J.M. was supported by a DOE Early Career Research Program grant under the same contract. We gratefully acknowledge R. Wang, Y. Zhang, and B. Ma for assistance with FET measurements, Ellen Briggs for PbS NC synthesis, and A. Llordes, E. Chan, and A. Hexemer for assistance with GISAXS, which was carried out at Advanced Light Source (ALS) beamline 7.3.3. A.D. acknowledges startup support from Fudan University, Natural National Science Foundation of China (21373052), and the 973 Program (2013CB934101, 2014CB845602). NR 41 TC 35 Z9 35 U1 17 U2 111 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD DEC PY 2013 VL 7 IS 12 BP 10978 EP 10984 DI 10.1021/nn404566b PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 281YO UT WOS:000329137100058 PM 24252075 ER PT J AU Imai, A Cheng, X Xin, HLL Eliseev, EA Morozovska, AN Kalinin, SV Takahashi, R Lippmaa, M Matsumoto, Y Nagarajan, V AF Imai, Akira Cheng, Xuan Xin, Huolin L. Eliseev, Eugene A. Morozovska, Anna N. Kalinin, Sergei V. Takahashi, Ryota Lippmaa, Mikk Matsumoto, Yuji Nagarajan, Valanoor TI Epitaxial Bi5Ti3FeO15-CoFe2O4 Pillar-Matrix Multiferroic Nanostructures SO ACS NANO LA English DT Article DE oxide film; pulsed laser deposition; nanocomposite; PFM ID THIN-FILMS; FERROELECTRICITY AB Epitaxial self-assembled ferro(i)magnetic spinel (CoFe2O4 (CFO)) and ferroelectric bismuth layered perovskite (Bi5Ti3FeO15 (BTFO)) pillar matrix nanostructures are demonstrated on (001) single-crystalline strontium titanate substrates. The CFO remains embedded in the BTFO matrix as vertical pillars (similar to 50 nm in diameter) up to a volume fraction of 50%. Piezoresponse force microscopy experiments evidence a weak out-of-plane and a strong in-plane ferroelectricity in the BTFO phase, despite previously reported paraelectricity along the c-axis in a pure BTFO film. Phenomenological Landau-Ginzburg-Devonshire-based thermodynamic computations show that the radial stress induced by the CFO nanopillars can influence these ferroelectric phases, thus signifying the importance of the nanopillars. The CFO pillars demonstrate robust ferromagnetic hysteresis loops with little degradation in the saturation magnetization (ca. 4 mu(B)/f.u.). Thus BTFO-CFO nanocomposites show significant promise as a lead-free magnetoelectric materials system. C1 [Imai, Akira; Matsumoto, Yuji] Tokyo Inst Technol, Mat & Struct Lab, Midori Ku, Yokohama, Kanagawa 2268503, Japan. [Imai, Akira; Cheng, Xuan; Nagarajan, Valanoor] Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia. [Xin, Huolin L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Eliseev, Eugene A.; Morozovska, Anna N.] Natl Acad Sci Ukraine, Inst Phys, Inst Problems Mat Sci, UA-03028 Kiev, Ukraine. [Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Takahashi, Ryota; Lippmaa, Mikk] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. [Matsumoto, Yuji] Tohoku Univ, Dept Appl Chem, Sch Engn, Aoba Ku, Sendai, Miyagi 9808579, Japan. RP Matsumoto, Y (reprint author), Tokyo Inst Technol, Mat & Struct Lab, Midori Ku, 4259 Nagatsuta, Yokohama, Kanagawa 2268503, Japan. EM matsumoto@atomol.che.tohoku.ac.jp RI valanoor, nagarajan/B-4159-2012; Takahashi, Ryota/A-8748-2010; Matsumoto, Yuji/H-2056-2011; Kalinin, Sergei/I-9096-2012; Xin, Huolin/E-2747-2010 OI Takahashi, Ryota/0000-0003-2430-2444; Kalinin, Sergei/0000-0001-5354-6152; Xin, Huolin/0000-0002-6521-868X FU New Energy and Industrial Technology Development Organization (NEDO) of Japan; Integrated Doctoral Education Program at Tokyo Tech; Ministry of Education, Culture, Sports, Science, and Technology of Japan [25706022]; ARC Discovery Project; SFFR-NSF project; U.S. National Science Foundation [NSF-DMR-1210588]; State Fund of Fundamental Research of Ukraine [UU48/002]; Center for Functional Nanomaterials at Brookhaven National Laboratory; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We acknowledge funding by the Industrial Technology Research Grant Program in 2007 from New Energy and Industrial Technology Development Organization (NEDO) of Japan, by the Integrated Doctoral Education Program at Tokyo Tech, and partly by a Grant-in-Aid for Scientific Research (grant no. 25706022) from the Ministry of Education, Culture, Sports, Science, and Technology of Japan. This research was carried out by the joint research in the Institute for Solid State Physics at the University of Tokyo. The authors would like to thank Mr. Seiji Takahashi and Dr. Takaharu Ishii at Asylum Technology Co., Ltd. for their kind technical support in PFM measurements to confirm the reproducibility of experimental results. The research at UNSW was supported in part by ARC Discovery Project. E.A.E. and A.N.M. acknowledge the support via the bilateral SFFR-NSF project, namely, U.S. National Science Foundation under NSF-DMR-1210588 and State Fund of Fundamental Research of Ukraine, grant UU48/002. H.L.X. was supported by the Center for Functional Nanomaterials at Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract no. DE-AC02-98CH10886. NR 25 TC 13 Z9 13 U1 10 U2 95 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD DEC PY 2013 VL 7 IS 12 BP 11079 EP 11086 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 281YO UT WOS:000329137100069 PM 24215598 ER PT J AU Pascal, J Ashley, CE Wang, ZH Brocato, TA Butner, JD Carnes, EC Koay, EJ Brinker, CJ Cristini, V AF Pascal, Jennifer Ashley, Carlee E. Wang, Zhihui Brocato, Terisse A. Butner, Joseph D. Carnes, Eric C. Koay, Eugene J. Brinker, C. Jeffrey Cristini, Vittorio TI Mechanistic Modeling Identifies Drug-Uptake History as Predictor of Tumor Drug Resistance and Nano-Carrier-Mediated Response SO ACS NANO LA English DT Article DE drug delivery; mathematical modeling; mesoporous silica nanoparticle; pharmacokinetics-pharmacodynamics model; protocells ID SUPPORTED LIPID-BILAYERS; CELLULAR PHARMACODYNAMICS; MATHEMATICAL-MODEL; CANCER-CELLS; DELIVERY; DOXORUBICIN; NANOPARTICLES; CHEMOTHERAPY; SIMULATION; LIPOSOMES AB A quantitative understanding of the advantages of nanoparticle-based drug delivery vis-a-vis conventional free drug chemotherapy has yet to be established for cancer or other diseases despite numerous investigations. Here, we employ first-principles cell biophysics, drug pharmaco-kinetics, and drug pharmaco-dynamics to model the delivery of doxorubicin (DOX) to hepatocellular carcinoma (HCC) tumor cells and predict the resultant experimental cytotoxicity data. The fundamental, mechanistic hypothesis of our mathematical model is that the integrated history of drug uptake by the cells over time of exposure, which sets the cell death rate parameter, and the uptake rate are the sole determinants of the dose response relationship. A universal solution of the model equations is capable of predicting the entire, nonlinear dose response of the cells to any drug concentration based on just two separate measurements of these cellular parameters. This analysis reveals that nanocarrier-mediated delivery overcomes resistance to the free drug because of improved cellular uptake rates, and that dose response curves to nanocarrier mediated drug delivery are equivalent to those for free-drug, but "shifted to the left;" that is, lower amounts of drug achieve the same cell kill. We then demonstrate the model's general applicability to different tumor and drug types, and cell-exposure time courses by investigating HCC cells exposed to cisplatin and 5-fluorouracil, breast cancer MCF-7 cells exposed to DOX, and pancreatic adenocarcinoma PANC-1 cells exposed to gemcitabine. The model will help in the optimal design of nanocarriers for clinical applications and improve the current, largely empirical understanding of in vivo drug transport and tumor response. C1 [Pascal, Jennifer; Wang, Zhihui; Cristini, Vittorio] Univ New Mexico, Hlth Sci Ctr, Dept Pathol, Albuquerque, NM 87131 USA. [Ashley, Carlee E.; Carnes, Eric C.; Brinker, C. Jeffrey; Cristini, Vittorio] Univ New Mexico, Hlth Sci Ctr, Canc Res & Treatment Ctr, Albuquerque, NM 87131 USA. [Brinker, C. Jeffrey] Univ New Mexico, Hlth Sci Ctr, Dept Mol Genet & Microbiol, Albuquerque, NM 87131 USA. [Ashley, Carlee E.] Sandia Natl Labs, Biotechnol & Bioengn Dept, Livermore, CA 94551 USA. [Carnes, Eric C.] Sandia Natl Labs, Nanobiol Dept, Albuquerque, NM 87185 USA. [Brinker, C. Jeffrey] Sandia Natl Labs, Self Assembled Mat Dept, Albuquerque, NM 87185 USA. [Brocato, Terisse A.; Butner, Joseph D.; Carnes, Eric C.; Brinker, C. Jeffrey; Cristini, Vittorio] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. [Brocato, Terisse A.; Butner, Joseph D.; Carnes, Eric C.; Brinker, C. Jeffrey; Cristini, Vittorio] Univ New Mexico, Ctr Biomed Engn, Albuquerque, NM 87131 USA. [Brinker, C. Jeffrey] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Koay, Eugene J.] Univ Texas MD Anderson Canc Ctr, Dept Radiat Oncol, Houston, TX 77030 USA. [Koay, Eugene J.] Houston Methodist Res Inst, Dept Nanomed, Houston, TX 77030 USA. RP Brinker, CJ (reprint author), Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. EM cjbrink@sandia.gov; VCristini@salud.unm.edu RI Cristini, Vittorio/N-3540-2013 FU NIGMS [K12GM088021]; NSF [DMS-1263742, CTO PSOC-1U54CA143837, TCCN-1U54CA151668, USC PSOC-1U54CA143907, ICBP-1U54-CA149196, EF-0820117]; NSF SBIR [1315372]; Victor and Ruby Hansen Surface Professorship in Molecular Modeling of Cancer; Methodist Hospital Research Institute; Anne Eastland Spears Fellowship; Roadmap for Medical Research [NIH PHS 2 PN2 EY016570B]; NCI [1U01CA151792-01]; DOE BES Materials Science and Engineering Program; Sandia National Laboratories LDRD; NIEHS [1U19ES019528-01]; President Harry S. Truman Fellowship in National Security Science and Engineering at Sandia National Laboratories FX P Dogra, A Day (Cristini lab); H Shen, M Ferrari (partial support for E.J.K). Support NIGMS K12GM088021 (J.P.); NSF Grant DMS-1263742, CTO PSOC-1U54CA143837, TCCN-1U54CA151668, USC PSOC-1U54CA143907, ICBP-1U54-CA149196 (V.C., Z.W.); NSF SBIR 1315372, the Victor and Ruby Hansen Surface Professorship in Molecular Modeling of Cancer (V.C.); Methodist Hospital Research Institute (E.J.K, V.C.); the Anne Eastland Spears Fellowship (E.J.K); the Roadmap for Medical Research under Grant NIH PHS 2 PN2 EY016570B (C.J.B), NCI 1U01CA151792-01(E.C.C., C.J.B.), DOE BES Materials Science and Engineering Program (E.C.C., C.J.B.), Sandia National Laboratories LDRD (E.C.C., C.E.A., C.J.B.), NIEHS 1U19ES019528-01, NSF EF-0820117 (C.E.A., C.J.B.); the President Harry S. Truman Fellowship in National Security Science and Engineering at Sandia National Laboratories (C.E.A.). NR 25 TC 16 Z9 16 U1 2 U2 68 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD DEC PY 2013 VL 7 IS 12 BP 11174 EP 11182 DI 10.1021/nn4048974 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 281YO UT WOS:000329137100080 PM 24187963 ER PT J AU Li, N An, ZN Liu, WJ Wang, YD AF Li, Nan An, Zhinan Liu, Wenjun Wang, Yandong TI Quantification of Compositional and Residual Stress Effects on Lattice Strain in Dual-phase Stainless Steels by Means of Differential Aperture X-ray Micro-diffraction SO ACTA METALLURGICA SINICA-ENGLISH LETTERS LA English DT Article DE Differential aperture X-ray mico-diffraction; Lattice strain; Residual stress; Dual-phase stainless steels ID PARAMETER; DEFORMATION; ALLOY AB Residual stress is an important factor for evaluating the deformation and failure of engineering materials. Diffraction-based measurement assumes that the full measured lattice strain tensor contributes to residual stress according to Hooke's Law. The present work focuses on the lattice strain determination of individual grains in a dual-phase stainless steel (DPSS) by means of differential-aperture X-ray micro-diffraction (DAXM). The results show that the residual stress only takes part of the responsibility of the total measured lattice strain. In fact, the compositional variation inside the material was found to cause greater strain gradient in both ferrite (alpha) and austenite (gamma) phases in DPSS. Therefore, quantification of compositional and residual stress effects on lattice strain was conducted in order to evaluate the true residual stress inside engineering materials. C1 [Li, Nan] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. [An, Zhinan] Univ Tennessee, Dept Mat Engn, Knoxville, TN 37996 USA. [Liu, Wenjun] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Wang, Yandong] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100081, Peoples R China. RP Wang, YD (reprint author), Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100081, Peoples R China. EM ydwang@mail.neu.edu.cn RI wang, yandong/G-9404-2013 FU National Science Foundation of China [51231002]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was financial supported by the National Science Foundation of China (No. 51231002). The authors would like acknowledge that the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 16 TC 0 Z9 0 U1 0 U2 4 PU CHINESE ACAD SCIENCES, INST METAL RESEARCH PI SHENYANG PA 72 WENHUA RD, SHENYANG, 110016, PEOPLES R CHINA SN 1006-7191 EI 2194-1289 J9 ACTA METALL SIN-ENGL JI Acta Metall. Sin.-Engl. Lett. PD DEC PY 2013 VL 26 IS 6 BP 663 EP 668 DI 10.1007/s40195-013-0328-0 PG 6 WC Metallurgy & Metallurgical Engineering SC Metallurgy & Metallurgical Engineering GA 285RC UT WOS:000329411400004 ER PT J AU Tamura, D Nguyen, HT Sleeman, K Levine, M Mishin, VP Yang, H Guo, Z Okomo-Adhiambo, M Xu, XY Stevens, J Gubareva, LV AF Tamura, Daisuke Nguyen, Ha T. Sleeman, Katrina Levine, Marnie Mishin, Vasiliy P. Yang, Hua Guo, Zhu Okomo-Adhiambo, Margaret Xu, Xiyan Stevens, James Gubareva, Larisa V. TI Cell Culture-Selected Substitutions in Influenza A(H3N2) Neuraminidase Affect Drug Susceptibility Assessment SO ANTIMICROBIAL AGENTS AND CHEMOTHERAPY LA English DT Article ID RECEPTOR-BINDING VARIANTS; CANINE KIDNEY-CELLS; SIALIC-ACID; MDCK CELLS; A VIRUSES; LINE VERO; B VIRUSES; RESISTANCE; REPLICATION; INHIBITORS AB Assessment of drug susceptibility has become an integral part of influenza virus surveillance. In this study, we describe the drug resistance profile of influenza A(H3N2) virus, A/Mississippi/05/2011, collected from a patient treated with oseltamivir and detected via surveillance. An MDCK cell-grown isolate of this virus exhibited highly reduced inhibition by the neuraminidase (NA) inhibitors (NAIs) oseltamivir (8,005-fold), zanamivir (813-fold), peramivir (116-fold), and laninamivir (257-fold) in the NA inhibition assay. Sequence analysis of its NA gene revealed a known oseltamivir-resistance marker, the glutamic acid-to-valine substitution at position 119 (E119V), and an additional change, threonine to isoleucine at position 148 (T148I). Unlike E119V, T148I was not detected in the clinical sample but acquired during viral propagation in MDCK cells. Using recombinant proteins, T148I by itself was shown to cause only a 6-fold increase in the zanamivir 50% inhibitory concentration (IC50) and had no effect on inhibition by other drugs. The T148I substitution reduced NA activity by 50%, most likely by affecting the positioning of the 150 loop at the NA catalytic site. Using pyrosequencing, changes at T148 were detected in 35 (23%) of 150 MDCK cell-grown A(H3N2) viruses tested, which was lower than the frequency of changes at D151 (85%), an NA residue previously implicated in cell selection. We demonstrate that culturing of the A(H3N2) viruses (n = 11) at a low multiplicity of infection delayed the emergence of the NA variants with changes at position 148 and/or 151, especially when conducted in MDCK-SIAT1 cells. Our findings highlight the current challenges in monitoring susceptibility of influenza A(H3N2) viruses to the NAI class of antiviral drugs. C1 [Tamura, Daisuke; Nguyen, Ha T.; Sleeman, Katrina; Levine, Marnie; Mishin, Vasiliy P.; Yang, Hua; Guo, Zhu; Okomo-Adhiambo, Margaret; Xu, Xiyan; Stevens, James; Gubareva, Larisa V.] Ctr Dis Control & Prevent, Virus Surveillance & Diag Branch, Influenza Div, Natl Ctr Immunizat & Resp Dis, Atlanta, GA 30333 USA. [Tamura, Daisuke] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Nguyen, Ha T.; Levine, Marnie] Battelle Mem Inst, Atlanta, GA USA. RP Gubareva, LV (reprint author), Ctr Dis Control & Prevent, Virus Surveillance & Diag Branch, Influenza Div, Natl Ctr Immunizat & Resp Dis, Atlanta, GA 30333 USA. EM lqg3@cdc.gov FU Centers for Disease Control and Prevention; Oak Ridge Institute for Science and Education (ORISE) (Oak Ridge, TN); Business of Innovation (Battelle, Atlanta, GA) FX This work was supported by the Centers for Disease Control and Prevention. Financial support for D. T. for this study was provided by the Oak Ridge Institute for Science and Education (ORISE) (Oak Ridge, TN). H.T.N. and M. L. received financial support for this work from the Business of Innovation (Battelle, Atlanta, GA). NR 35 TC 13 Z9 13 U1 1 U2 3 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0066-4804 EI 1098-6596 J9 ANTIMICROB AGENTS CH JI Antimicrob. Agents Chemother. PD DEC PY 2013 VL 57 IS 12 BP 6141 EP 6146 DI 10.1128/AAC.01364-13 PG 6 WC Microbiology; Pharmacology & Pharmacy SC Microbiology; Pharmacology & Pharmacy GA 279KW UT WOS:000328959900040 PM 24080660 ER PT J AU Duncan, BN Yoshida, Y de Foy, B Lamsal, LN Streets, DG Lu, ZF Pickering, KE Krotkov, NA AF Duncan, Bryan N. Yoshida, Yasuko de Foy, Benjamin Lamsal, Lok N. Streets, David G. Lu, Zifeng Pickering, Kenneth E. Krotkov, Nickolay A. TI The observed response of Ozone Monitoring Instrument (OMI) NO2 columns to NOx emission controls on power plants in the United States: 2005-2011 SO ATMOSPHERIC ENVIRONMENT LA English DT Article DE Ozone Monitoring Instrument; Nitrogen dioxide; Air quality; Space-based observations; Power plant emissions; Emission control devices ID RETRIEVAL; SPACE AB We show that Aura Ozone Monitoring Instrument (OMI) nitrogen dioxide (NO2) tropospheric column data may be used to assess changes of the emissions of nitrogen oxides (NOx) from power plants in the United States, though careful interpretation of the data is necessary. There is a clear response for OMI NO2 data to NOx emission reductions from power plants associated with the implementation of mandated emission control devices (ECDs) over the OMI record (2005-2011). This response is scalar for all intents and purposes, whether the reduction is rapid or incremental over several years. However, it is variable among the power plants, even for those with the greatest absolute decrease in emissions. We document the primary causes of this variability, presenting case examples for specific power plants. Published by Elsevier Ltd. C1 [Duncan, Bryan N.; Yoshida, Yasuko; Lamsal, Lok N.; Pickering, Kenneth E.; Krotkov, Nickolay A.] NASA, Goddard Space Flight Ctr, Atmospher Chem & Dynam Lab, Greenbelt, MD 20771 USA. [Yoshida, Yasuko] Sci Syst & Applicat Inc, Lanham, MD USA. [de Foy, Benjamin] St Louis Univ, St Louis, MO 63103 USA. [Lamsal, Lok N.] Univ Space Res Assoc, Goddard Earth Sci Technol Ee Res, Columbia, MD USA. [Streets, David G.; Lu, Zifeng] Argonne Natl Lab, Argonne, IL 60439 USA. RP Duncan, BN (reprint author), NASA, Goddard Space Flight Ctr, Code 614, Greenbelt, MD 20771 USA. EM Bryan.N.Duncan@nasa.gov RI Lu, Zifeng/F-3266-2012; Pickering, Kenneth/E-6274-2012; de Foy, Benjamin/A-9902-2010; Krotkov, Nickolay/E-1541-2012; Duncan, Bryan/A-5962-2011; OI de Foy, Benjamin/0000-0003-4150-9922; Krotkov, Nickolay/0000-0001-6170-6750; Streets, David/0000-0002-0223-1350 FU NASA Air Quality Applied Sciences Team (AQAST) program FX This work was funded by the NASA Air Quality Applied Sciences Team (AQAST) program. We acknowledge the free use of 1) tropospheric NO2 column data from the Aura OMI, 2) NOx emissions data from the US EPA, and 3) EDGAR data, which is maintained as a joint project of the European Commission Joint Research Centre (JRC) and the Netherlands Environmental Assessment Agency (PBL). NR 26 TC 23 Z9 23 U1 2 U2 35 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1352-2310 EI 1873-2844 J9 ATMOS ENVIRON JI Atmos. Environ. PD DEC PY 2013 VL 81 BP 102 EP 111 DI 10.1016/j.atmosenv.2013.08.068 PG 10 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 285EY UT WOS:000329377600013 ER PT J AU Pilath, HM Michener, WE Katahira, R Mittal, A Clark, JM Himmel, ME Nimlos, MR Johnson, DK AF Pilath, Heidi M. Michener, William E. Katahira, Rui Mittal, Ashutosh Clark, Jared M. Himmel, Michael E. Nimlos, Mark R. Johnson, David K. TI Investigation of Xylose Reversion Reactions That Can Occur during Dilute Acid Pretreatment SO ENERGY & FUELS LA English DT Article ID METHYLSULFINYL CARBANION; OXIDATIVE-DEGRADATION; LINKAGE ANALYSIS; SULFURIC-ACID; D-GLUCOSE; HYDROLYSIS; PERMETHYLATION; 2-FURALDEHYDE; METHYLATION; CONVERSION AB Xylose reversion reactions to form xylooligomers represent a potentially important mechanism of sugar loss during dilute acid pretreatment of biomass. We have conducted a study to identify the products that result from these reactions and to determine the kinetics of their formation. A major obstacle is that there are few commercial standards available for xylose disaccharides, which are essential for the identification and quantification of the xylose reversion products formed during these reactions. To overcome this obstacle, we have used GC/MS and NMR analysis of xylose disaccharides isolated by preparative HPLC to identify the reaction products. At the xylose concentration we used (300 g L-1), only xylose disaccharides were observed. As with glucose reversion reactions [Pilath, H. M.; et al. J. Agric. Food Chem. 2010, 58, 6131], the disaccharides contained linkages that involved the anomeric carbon atom of one of the sugar monomers. Eight out of the nine possible disaccharides, including alpha and beta anomers, were observed. Whereas the GC/MS allowed for the identification of the linkages, NMR was needed to distinguish between the alpha and beta isomers of the disaccharides. The kinetics of combined xylose disaccharide formation was measured using HPLC. Arrhenius parameters for the rates of disaccharide formation were calculated by fitting the data to a simple model. C1 [Pilath, Heidi M.; Michener, William E.; Katahira, Rui; Clark, Jared M.; Nimlos, Mark R.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Mittal, Ashutosh; Himmel, Michael E.; Johnson, David K.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. RP Pilath, HM (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. EM Heidi.Pilath@nrel.gov; William.Michener@nrel.gov FU U.S. Department of Energy through the Bioenergy Technologies Office FX This work was supported by the U.S. Department of Energy through the Bioenergy Technologies Office. NR 38 TC 2 Z9 2 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD DEC PY 2013 VL 27 IS 12 BP 7389 EP 7397 DI 10.1021/ef400889u PG 9 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 278WO UT WOS:000328920800022 ER PT J AU Gibson, L Soundarrajan, N Spenik, J Ma, JL Shadle, L Pisupati, SV AF Gibson, LaTosha Soundarrajan, Nari Spenik, James Ma, Jinliang Shadle, Lawrence Pisupati, Sarma V. TI Application of Particle Population Model To Determine the Contribution to Slag, Flyash, and Syngas in Entrained Flow Gasification from Particle Size Distribution SO ENERGY & FUELS LA English DT Article ID PULVERIZED COAL INJECTION; C-S MELTS; BLAST-FURNACE; SLAG/CARBON INTERFACE; MINERAL BEHAVIOR; CFD SIMULATION; CHAR OXIDATION; COMBUSTION; TRANSFORMATIONS; CARBON AB During entrained coal gasification any inefficiency in the slagging process leads to overall process inefficiencies and fouling of downstream equipment. A coal particle population model was developed to evaluate the conversion and partitioning of diverse heterogeneous coal particles into slag and flyash. A Pittsburgh No. 8 coal sample was separated into four gravity fractions by float sink separation. Each density cut was further separated into seven size fractions. These fractions were individually characterized to evaluate the resulting conversion and partitioning into slag and flyash. The sticking probability varied among the four specific gravity fractions as a function of temperature while little or negligible variance among the size fractions was observed for conventional viscosity models. However, this was not the case, when using the contact angle to account for the influence of carbon. By expressing the contact angle as a function of carbon content and the temperature of critical viscosity, the behavior of reacting coal particles striking the gasifier wall could be evaluated. Capture efficiencies were predicted to be higher for particles from smaller size and lower specific gravity fractions. A sensitivity analysis indicated that decreasing the amount of the larger size fractions reduces the formation of flyash since it increases mineral capture in slag, with a slight increase in syngas production due to the larger carbon conversion in smaller size fractions versus larger size fractions. C1 [Gibson, LaTosha; Soundarrajan, Nari; Pisupati, Sarma V.] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. [Gibson, LaTosha; Soundarrajan, Nari; Pisupati, Sarma V.] Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA. [Gibson, LaTosha; Spenik, James; Ma, Jinliang; Shadle, Lawrence; Pisupati, Sarma V.] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Pisupati, SV (reprint author), Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, 110 Hosler Bldg, University Pk, PA 16802 USA. EM sxp17@psu.edu RI Pisupati, Sarma/A-9861-2009; OI Pisupati, Sarma/0000-0002-2098-3302; Shadle, Lawrence/0000-0002-6283-3628 NR 48 TC 5 Z9 5 U1 2 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD DEC PY 2013 VL 27 IS 12 BP 7681 EP 7695 DI 10.1021/ef401414r PG 15 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 278WO UT WOS:000328920800053 ER PT J AU Vegendla, SNP Hasse, C AF Vegendla, S. N. P. Hasse, C. TI Steady Flamelet Progress-Variable (FPV) Modeling and Simulation of a High-Pressure Gasifier SO ENERGY & FUELS LA English DT Article ID LARGE-EDDY SIMULATION; GAS-SOLID FLOW; CHARRING MATERIALS; TURBULENT FLAMES; PYROLYSIS MODEL; COMBUSTION AB A steady computational fluid dynamics (CFD)-flamelet/progress-variable (FPV) model is implemented for the simulation of a gasifier. In this model, the open source code OpenFOAM is used to solve the partial differential equations of mass, momentum, turbulence, fuel mixture fraction mean of fuel and its variance, mean mixture fraction of steam, and progress variable. On the other hand, the species mass fractions are retrieved from a precomputed flamelet look-up table. Finally, the simulation results obtained with the steady CFD FPV are compared to the available pilot plant data. The flame zone shifts toward the inlet when using the FPV model compared to the standard flamelet model without the progress variable. In both models, the observed outlet values are in reasonably good agreement with the experimental values. C1 [Vegendla, S. N. P.; Hasse, C.] TU Bergakad Freiberg, ZIK Virtuhcon, Chair Numer Thermo Fluid Dynam, D-09599 Freiberg, Germany. RP Vegendla, SNP (reprint author), Argonne Natl Lab, Nucl Engn & Anal Div, Lemont, IL 60439 USA. EM svegendla@anl.gov RI Hasse, Christian/A-3587-2011 OI Hasse, Christian/0000-0001-9333-0911 FU Federal Ministry of Education and Research [03Z2FN11] FX The authors gratefully acknowledge financial support during the period of 2010-2011 through the Federal Ministry of Education and Research in the framework of Virtuhcon (Project 03Z2FN11). NR 25 TC 6 Z9 6 U1 0 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD DEC PY 2013 VL 27 IS 12 BP 7772 EP 7777 DI 10.1021/ef4014136 PG 6 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 278WO UT WOS:000328920800060 ER PT J AU Allen, C Valco, D Toulson, E Yoo, JH Lee, T AF Allen, Casey Valco, Daniel Toulson, Elisa Yoo, Ji Hyung Lee, Tonghun TI JP-5 and HRJ-5 Autoignition Characteristics and Surrogate Modeling SO ENERGY & FUELS LA English DT Article ID RAPID COMPRESSION MACHINE; ELEVATED PRESSURES; CHEMICAL-KINETICS; SHOCK-TUBE; JET FUELS; N-HEPTANE; IGNITION; COMBUSTION; TEMPERATURES; CAMELINA AB A heated rapid compression machine has been used to investigate the autoignition behavior of JP-5 and camelina-based hydrotreated renewable jet (HRJ-5) fuels. Testing was conducted at low temperatures (T-c = 627-733 K), low-to-moderate pressures (p(c) = 5, 10, and 20 bar), and lean (phi = 0.25 and 0.50) and stoichiometric mixtures in air. The HRJ-5 fuel, which is 99% paraffinic, exhibited greater reactivity than the JP-5 fuel in the form of shorter ignition delays. The HRJ-5 fuel also exhibited transition into the negative temperature coefficient region at a lower compressed temperature (T-c = 675 K) than the JP-5 fuel (T-c = 700 K). Two surrogate fuel blends and kinetic models intended for Jet-A and kerosene-type fuels are evaluated for their ability to predict JP-5. ignition delay tunes because JP-5 and Jet-A ignition delay times showed close resemblance. The models reproduced the-qualitative trend in the data, including an accurate representation of when the negative temperature coefficient behavior appears. The best agreement between the data and predictions was obtained at p(c) = 5 bar and phi = 1.0, but outside of this region, the disparity was often 2-fold or greater. C1 [Allen, Casey] Marquette Univ, Dept Mech Engn, Milwaukee, WI 53233 USA. [Valco, Daniel] Univ Illinois, Dept Chem & Biomol Engn, Urbana, IL 61801 USA. [Toulson, Elisa] Michigan State Univ, Dept Mech Engn, E Lansing, MI 48824 USA. [Yoo, Ji Hyung] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Knoxville, TN 37932 USA. [Lee, Tonghun] Univ Illinois, Dept Mech Sci & Engn, Urbana, IL 61801 USA. RP Lee, T (reprint author), Univ Illinois, Dept Mech Sci & Engn, Urbana, IL 61801 USA. EM tonghun@illinois.edu FU Office of Naval Research [N00014-12-1-0107] FX The authors gratefully acknowledge the support of the Office of Naval Research under Grant N00014-12-1-0107, with Sharon Beermann-Curtin serving as technical monitor. Additionally, the authors acknowledge Mass Spectrometry Core, Research Technology Support Facility (RTSF), Michigan State University, for graciously providing access to the GC-MS instrumentation. The authors also thank Dr. Robert Morris of the Naval Research Laboratory for assistance with analyzing the fuel compositions. NR 40 TC 6 Z9 6 U1 1 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD DEC PY 2013 VL 27 IS 12 BP 7790 EP 7799 DI 10.1021/ef401629d PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 278WO UT WOS:000328920800062 ER PT J AU Li, TW Chaudhari, K VanEssendelft, D Turton, R Nicoletti, P Shahnam, M Guenther, C AF Li, Tingwen Chaudhari, Kiran VanEssendelft, Dirk Turton, Richard Nicoletti, Philip Shahnam, Mehrdad Guenther, Chris TI Computational Fluid Dynamic Simulations of a Pilot-Scale Transport Coal Gasifier: Evaluation of Reaction Kinetics SO ENERGY & FUELS LA English DT Article ID ENTRAINED FLOW GASIFICATION; CHEMICAL PERCOLATION MODEL; CONVERSION SUBMODELS; DESIGN APPLICATIONS; ELEVATED PRESSURES; HEATING RATE; CFD MODEL; PART I; DEVOLATILIZATION; PYROLYSIS AB The U.S. Department of Energy's National Energy Technology Laboratory has developed a software platform titled Carbonaceous Chemistry for Computational Modeling (C3M) that can be used to seamlessly connect the reaction kinetics typically found in the gasification process to various computational fluid dynamic (CFD) packages, including MFIX, ANSYS-FLUENT, and BARRACUDA, for advanced gasifier simulation. In this study, a pilot-scale transport gasifier was simulated by employing the C3M platform to incorporate various kinetics into the CFD simulation. It was found that appropriate chemical kinetics for gasification reactions are key to the numerical prediction of syngas composition and the kinetics from Niksa Energy Associate's PC Coal Lab yielded reasonable agreement to the experimental data. Using the C3M platform, different chemistry kinetics for coal devolatilization-generated by METC Gasifier Advanced Simulation (MGAS), Niksa Energy Associate's PC Coal Lab (PCCL), Chemical Percolation Model for Coal Devolatilization (CPD), and Advanced Fuel Research's Functional-Group, Depolymerization, Vaporization, Cross-linking (FG-DVC)-were evaluated for the transport gasifier simulation. Results showed that the effect of devolatilization kinetics on the transport gasifier simulation is considered to be secondary comparing to the char gasification reactions because of the relatively long residence time of coal particles in the system. C1 [Li, Tingwen; Chaudhari, Kiran; VanEssendelft, Dirk; Turton, Richard; Nicoletti, Philip; Shahnam, Mehrdad; Guenther, Chris] Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Chaudhari, Kiran; Turton, Richard] W Virginia Univ, Morgantown, WV 26506 USA. [Li, Tingwen; Nicoletti, Philip] URS Corp, Morgantown, WV 26501 USA. RP Li, TW (reprint author), Natl Energy Technol Lab, Morgantown, WV 26507 USA. EM tingwen.li@contr.netl.doe.gov FU National Energy Technology Laboratory [DE-FE0004000]; agency of the United States Government FX This technical report was produced in support of the National Energy Technology Laboratory's ongoing research in advanced numerical simulation of multiphase flow under the RES contract DE-FE0004000. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 50 TC 5 Z9 5 U1 2 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD DEC PY 2013 VL 27 IS 12 BP 7896 EP 7904 DI 10.1021/ef401887r PG 9 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 278WO UT WOS:000328920800073 ER PT J AU Zang, QD Rotroff, DM Judson, RS AF Zang, Qingda Rotroff, Daniel M. Judson, Richard S. TI Binary Classification of a Large Collection of Environmental Chemicals from Estrogen Receptor Assays by Quantitative Structure-Activity Relationship and Machine Learning Methods SO JOURNAL OF CHEMICAL INFORMATION AND MODELING LA English DT Article ID COMPUTATIONAL TOXICOLOGY RESOURCE; ENDOCRINE-DISRUPTING CHEMICALS; THROUGHPUT SCREENING DATA; SUPPORT VECTOR MACHINES; RANDOM FOREST; MOLECULAR DESCRIPTORS; TOXCAST PROGRAM; IMBALANCED DATA; QSAR MODELS; DATA SETS AB There are thousands of environmental chemicals subject to regulatory decisions for endocrine disrupting potential. The ToxCast and Tox21 programs have tested similar to 8200 chemicals in a broad screening panel of in vitro high-throughput screening (HTS) assays for estrogen receptor (ER) agonist and antagonist activity. The present work uses this large data set to develop in silico quantitative structure-activity relationship (QSAR) models using machine learning (ML) methods and a novel approach to manage the imbalanced data distribution. Training compounds from the ToxCast project were categorized as active or inactive (binding or nonbinding) classes based on a composite ER Interaction Score derived from a collection of 13 ER in vitro assays. A total of 1537 chemicals from ToxCast were used to derive and optimize the binary classification models while 5073 additional chemicals from the Tox21 project, evaluated in 2 of the 13 in vitro assays, were used to externally validate the model performance. In order to handle the imbalanced distribution of active and inactive chemicals, we developed a cluster-selection strategy to minimize information loss and increase predictive performance and compared this strategy to three currently popular techniques: cost-sensitive learning, oversampling of the minority class, and undersampling of the majority class. QSAR classification models were built to relate the molecular structures of chemicals to their ER activities using linear discriminant analysis (LDA), classification and regression trees (CART), and support vector machines (SVM) with 51 molecular descriptors from QikProp and 4328 bits of structural fingerprints as explanatory variables. A random forest (RF) feature selection method was employed to extract the structural features most relevant to the ER activity. The best model was obtained using SVM in combination with a subset of descriptors identified from a large set via the RF algorithm, which recognized the active and inactive compounds at the accuracies of 76.1% and 82.8% with a total accuracy of 81.6% on the internal test set and 70.8% on the external test set. These results demonstrate that a combination of high-quality experimental data and ML methods can lead to robust models that achieve excellent predictive accuracy, which are potentially useful for facilitating the virtual screening of chemicals for environmental risk assessment. C1 [Zang, Qingda] US EPA, ORISE, Res Triangle Pk, NC 27711 USA. [Rotroff, Daniel M.; Judson, Richard S.] US EPA, Natl Ctr Computat Toxicol, Res Triangle Pk, NC 27711 USA. [Rotroff, Daniel M.] N Carolina State Univ, Dept Stat, Bioinformat Res Ctr, Raleigh, NC 27695 USA. RP Judson, RS (reprint author), 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA. EM Judson.Richard@epa.gov OI Judson, Richard/0000-0002-2348-9633 FU Office of Research and Development, U.S. Environmental Protection Agency FX This project was supported in part by an appointment to the Research Participation Program at the Office of Research and Development, U.S. Environmental Protection Agency, administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and EPA. We would like to express our appreciation to the anonymous reviewers for their constructive comments and suggestions. NR 66 TC 26 Z9 26 U1 6 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9596 EI 1549-960X J9 J CHEM INF MODEL JI J. Chem Inf. Model. PD DEC PY 2013 VL 53 IS 12 BP 3244 EP 3261 DI 10.1021/ci400527b PG 18 WC Chemistry, Medicinal; Chemistry, Multidisciplinary; Computer Science, Information Systems; Computer Science, Interdisciplinary Applications SC Pharmacology & Pharmacy; Chemistry; Computer Science GA 281YU UT WOS:000329137700015 PM 24279462 ER EF