FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Yee, KL Rodriguez, M Thompson, OA Fu, CX Wang, ZY Davison, BH Mielenz, JR AF Yee, Kelsey L. Rodriguez, Miguel, Jr. Thompson, Olivia A. Fu, Chunxiang Wang, Zeng-Yu Davison, Brian H. Mielenz, Jonathan R. TI Consolidated bioprocessing of transgenic switchgrass by an engineered and evolved Clostridium thermocellum strain SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Transgenic; Switchgrass; Metabolic engineering; Clostridium thermocellum; Consolidated bioprocessing; Feedstock; Cellulosic ethanol ID BIOFUEL PRODUCTION; SIMULTANEOUS SACCHARIFICATION; LIGNIN MODIFICATION; CELLULOSIC BIOMASS; FERMENTATION; ETHANOL; RECALCITRANCE; IMPROVEMENT; CONVERSION; YIELDS AB Background: Switchgrass is an abundant and dedicated bioenergy feedstock, however its inherent recalcitrance is one of the economic hurdles for producing biofuels. The downregulation of the caffeic acid O-methyl transferase (COMT) gene in the lignin pathway of switchgrass reduced lignin content and S/G ratio, and the transgenic lines showed improved fermentation yield with Saccharomyces cerevisiae and wild-type Clostridium thermocellum (ATCC 27405) in comparison to the wild-type switchgrass. Results: Here we examine the conversion and yield of the COMT transgenic and wild-type switchgrass lines with an engineered and evolved C. thermocellum (M1570) strain. The fermentation of the transgenic switchgrass by M1570 had superior conversion relative to the wild-type control switchgrass line with an increase in conversion of approximately 20% and ethanol being the primary product accounting for 90% of the total metabolites measured by HPLC analysis. Conclusions: The engineered and evolved C. thermocellum M1570 was found to respond to the apparent reduced recalcitrance of the COMT switchgrass with no substrate inhibition, producing more ethanol on the transgenic feedstock than the wild-type substrate. Since ethanol was the main fermentation metabolite produced by an engineered and evolved C. thermocellum strain, its ethanol yield on a transgenic switchgrass substrate (gram/gram (g/g) glucan liberated) is the highest produced thus far. This result indicates that the advantages of a modified feedstock can be combined with a modified consolidated bioprocessing microorganism as anticipated. C1 [Yee, Kelsey L.; Rodriguez, Miguel, Jr.; Thompson, Olivia A.; Davison, Brian H.; Mielenz, Jonathan R.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Yee, Kelsey L.; Rodriguez, Miguel, Jr.; Thompson, Olivia A.; Wang, Zeng-Yu; Davison, Brian H.; Mielenz, Jonathan R.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Fu, Chunxiang; Wang, Zeng-Yu] Samuel Roberts Noble Fdn Inc, Forage Improvement Div, Ardmore, OK 73401 USA. [Mielenz, Jonathan R.] White Cliff Biosyst, Rockwood, TN 37854 USA. RP Davison, BH (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM davisonbh@ornl.gov RI Davison, Brian/D-7617-2013 OI Davison, Brian/0000-0002-7408-3609 FU Bioenergy Science Center (BESC) [ERKP695]; US Department of Energy (DOE) Bioenergy Research Center; Office of Biological and Environmental Research in the DOE Office of Science; US Government [DE-AC05-00OR22725] FX We would like to thank Mrs Choo Y Hamilton for her technical assistance and support to this project. We would also like to thank D Aaron Argyros for his assistance and support and the Mascoma Corporation for providing the C. thermocellum M1570 strain. This research was funded by the Bioenergy Science Center (BESC) under grant ERKP695, which is a US Department of Energy (DOE) Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. This manuscript has been authored by a contractor of the US Government under contract DE-AC05-00OR22725. NR 28 TC 15 Z9 15 U1 1 U2 34 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAY 22 PY 2014 VL 7 AR 75 DI 10.1186/1754-6834-7-75 PG 6 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AI4SH UT WOS:000336854600001 PM 24876889 ER PT J AU Yang, SH Pan, CL Hurst, GB Dice, L Davison, BH Brown, SD AF Yang, Shihui Pan, Chongle Hurst, Gregory B. Dice, Lezlee Davison, Brian H. Brown, Steven D. TI Elucidation of Zymomonas mobilis physiology and stress responses by quantitative proteomics and transcriptomics SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE Zymomonas mobilis; microarray; proteomics and metabolomics; acetate; pretreatment inhibitor; stress responses; quantitative proteomics; systems biology ID FUEL ETHANOL-PRODUCTION; GENOME SEQUENCE; SACCHAROMYCES-CEREVISIAE; HOPANOID BIOSYNTHESIS; STRAIN; IDENTIFICATION; METABOLISM; TOLERANCE; PATHWAY; GROWTH AB Zymomonas mobilis is an excellent ethanologenic bacterium. Biomass pretreatment and saccharification provides access to simple sugars, but also produces inhibitors such as acetate and furfural. Our previous work has identified and confirmed the genetic change of a 1.5-kb deletion in the sodium acetate tolerant Z. mobilis mutant (AcR) leading to constitutively elevated expression of a sodium proton antiporter encoding gene nhaA, which contributes to the sodium acetate tolerance of AcR mutant. In this study, we further investigated the responses of AcR and wild-type ZM4 to sodium acetate stress in minimum media using both transcriptomics and a metabolic labeling approach for quantitative proteomics the first time. Proteomic measurements at two time points identified about eight hundreds proteins, or about half of the predicted proteome. Extracellular metabolite analysis indicated AcR overcame the acetate stress quicker than ZM4 with a concomitant earlier ethanol production in AcR mutant, although the final ethanol yields and cell densities were similar between two strains. Transcriptomic samples were analyzed for four time points and revealed that the response of Z mobilis to sodium acetate stress is dynamic, complex, and involved about one-fifth of the total predicted genes from all different functional categories. The modest correlations between proteomic and transcriptomic data may suggest the involvement of posttranscriptional control. In addition, the transcriptomic data of forty-four microarrays from four experiments for ZM4 and AcR under different conditions were combined to identify strain-specific, media-responsive, growth phase-dependent, and treatment-responsive gene expression profiles. Together this study indicates that minimal medium has the most dramatic effect on gene expression compared to rich medium followed by growth phase, inhibitor, and strain background. Genes involved in protein biosynthesis, glycolysis and fermentation as well as ATP synthesis and stress response play key roles in Z. mobilis metabolism with consistently strong expression levels under different conditions. C1 [Yang, Shihui; Dice, Lezlee; Davison, Brian H.; Brown, Steven D.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Yang, Shihui; Dice, Lezlee; Davison, Brian H.; Brown, Steven D.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN USA. [Yang, Shihui] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Pan, Chongle] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN USA. [Pan, Chongle; Hurst, Gregory B.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA. RP Yang, SH (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM shihui.yang@nrel.gov; brownsd@ornl.gov RI Davison, Brian/D-7617-2013; OI Davison, Brian/0000-0002-7408-3609; Yang, Shihui/0000-0002-9394-9148; Hurst, Gregory/0000-0002-7650-8009 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL); Office of Biological and Environmental Research in the DOE Office of Science; UT-Battelle, LLC [DE-ACO5-000R22725]; U.S. Department of Energy FX We thank Miguel Rodriguez Jr. for assistance with HPLC analyses. This work was sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL) and concluded under the BioEnergy Science Center which is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-ACO5-000R22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 60 TC 7 Z9 7 U1 3 U2 26 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAY 22 PY 2014 VL 5 AR 246 DI 10.3389/fmicb.2014.00246 PG 13 WC Microbiology SC Microbiology GA AI1ZW UT WOS:000336656100002 PM 24904559 ER PT J AU Agrawal, P Rentala, V AF Agrawal, Prateek Rentala, Vikram TI Identifying dark matter interactions in monojet searches SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Dark Matter and Double Beta Decay; Jet substructure; Jets ID RAY POSITRON FRACTION; E(+)E(-) COLLISIONS; MISSING ENERGY; SINGLE-PHOTON; EVENTS; CONSTRAINTS AB We study the discrimination of quark-initiated jets from gluon-initiated jets in monojet searches for dark matter using the technique of averaged jet energy profiles. We demonstrate our results in the context of effective field theories of dark matter interactions with quarks and gluons, but our methods apply more generally to a wide class of models. Different effective theories of dark matter and the standard model backgrounds each have a characteristic quark/gluon fraction for the leading jet. When used in conjunction with the traditional cut-and-count monojet search, the jet energy profile can be used to set stronger bounds on contact interactions of dark matter. In the event of a discovery of a monojet excess at the 14 TeV LHC, contact interactions between dark matter with quarks or with gluons can be differentiated at the 95% confidence level. For a given rate at the LHC, signal predictions at direct detection experiments for different dark matter interactions can span five orders of magnitude. The ability to identify these interactions allows us to make a tighter connection between LHC searches and direct detection experiments. C1 [Agrawal, Prateek] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Rentala, Vikram] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. RP Agrawal, P (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. EM prateek@fnal.gov; rentala@pa.msu.edu OI Agrawal, Prateek/0000-0001-9947-0632 FU NSF [PHY-0855561]; National Science Foundation [PHYS-1066293]; Fermi Research Alliance; LLC with the United States Department of Energy [AC02-07CH11359]; hospitality of the Aspen Center for Physics FX We would like to acknowledge useful discussions with Patrick Fox, Claudia Frugiuele, Roni Harnik, Sonia El Hedri, Raoul Rontsch, Ciaran Williams, and C.-P. Yuan. VR is supported by NSF Grant No. PHY-0855561. PA would like to acknowledge support by the National Science Foundation under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics, where a part of this work was completed. VR would like to thank Fermilab for hospitality during the completion of this work. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE- AC02-07CH11359 with the United States Department of Energy. NR 71 TC 4 Z9 4 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. 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Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P 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Hidas, D. Lath, A. Panwalkar, S. Park, M. Patel, R. Rekovic, V. Robles, J. Salur, S. Schnetzer, S. Seitz, C. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. Yang, Z. C. York, A. Bouhali, O. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Safonov, A. Sakuma, T. Suarez, I. Tatarinov, A. Toback, D. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Wood, J. Gollapinni, S. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Belknap, D. A. Borrello, L. Carlsmith, D. Cepeda, M. Cooperstein, S. Dasu, S. Duric, S. Friis, E. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Klukas, J. Lanaro, A. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Woods, N. TI Evidence for the 125 GeV Higgs boson decaying to a pair of tau leptons SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Higgs physics ID HADRON COLLIDERS; PP COLLISIONS; ELECTROWEAK CORRECTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; QCD CORRECTIONS; ROOT-S=7 TEV; NNLO QCD; MODEL; SEARCH AB A search for a standard model Higgs boson decaying into a pair of tau leptons is performed using events recorded by the CMS experiment at the LHC in 2011 and 2012. The dataset corresponds to an integrated luminosity of 4.9 fb(-1) at a centre-of-mass energy of 7 TeV and 19.7 fb(-1) at 8 TeV. Each tau lepton decays hadronically or leptonically to an electron or a muon, leading to six different final states for the tau-lepton pair, all considered in this analysis. An excess of events is observed over the expected background contributions, with a local significance larger than 3 standard deviations for m (H) values between 115 and 130 GeV. The best fit of the observed H -> tau tau signal cross section times branching fraction for m(H) = 125 GeV is 0.78 +/- 0.27 times the standard model expectation. These observations constitute evidence for the 125 GeV Higgs boson decaying to a pair of tau leptons. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Mahrous, A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Rebane, L.; Tiko, A.; Eerola, P.; Fedi, G.; Voutilainen, M.; Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Agram, J. -L.; Andrea, J.; Bloch, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.] Univ Strasbourg, Univ Haute Alsace Mulhouse, CNRS, Inst Pluridisciplinaire Hubert Curien,IN3P3, Strasbourg, France. [Beluffi, C.; Gadrat, S.] Inst Natl Phys Nucl & Phys Particules, CNRS, Ctr Calcul, IN2P3, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Alvarez, J. D. Ruiz; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.; Xiao, H.; Tsamalaidze, Z.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Klein, B.; Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Geiser, A.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Kraemer, M.; Krucker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Ntomari, E.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Ron, E.; Sahin, M. O.; Salfeld-Nebgen, J.; Saxena, P.; Schmidt, R.; Schoerner-Sadenius, T.; Schroeder, M.; Stein, M.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.; Reid, I. D.; Perry, T.] Deutsch Elekt Synchrotron, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M. G.; Gosselink, M.; Haller, J.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbruck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Caspart, R.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Friese, R.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.; Kroeger, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-giotis, I.; Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Jones, J.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Kumar, A.; Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Banerjee, S.; Guchait, M.; Dewanjee, R. K.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Nespolo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Licata, C. La; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; Licata, C. La; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potos, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Asghar, M. I.; Butt, J.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Golutvin, I.; Gorbunov, I.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Smirnov, V.; Zarubin, A.] Dubna Joint Nucl Res Inst, Dubna 141980, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Iglesias, L. Lloret] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Contardo, D.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Evangelou, I.; Foudas, C.; Bencze, G.; Sharma, A.; Mohanty, A. K.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; Palla, F.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. 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Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Guelmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yuecel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Richardson, C.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.; Cox, B.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois Chicago UIC, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. 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O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. EM cms-publication-committee-chair@cern.ch RI Novaes, Sergio/D-3532-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Moon, Chang-Seong/J-3619-2014; Gregores, Eduardo/F-8702-2012; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Gonzalez Caballero, Isidro/E-7350-2010; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Popov, Andrey/E-1052-2012; OI Novaes, Sergio/0000-0003-0471-8549; Scodellaro, Luca/0000-0002-4974-8330; Montanari, Alessandro/0000-0003-2748-6373; Moon, Chang-Seong/0000-0001-8229-7829; Cerrada, Marcos/0000-0003-0112-1691; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Marzocchi, Badder/0000-0001-6687-6214; Gerosa, Raffaele/0000-0001-8359-3734; Costa, Salvatore/0000-0001-9919-0569; Kasemann, Matthias/0000-0002-0429-2448; Tosi, Nicolo/0000-0002-0474-0247; WANG, MIN-ZU/0000-0002-0979-8341; Popov, Andrey/0000-0002-1207-0984; Margaroli, Fabrizio/0000-0002-3869-0153; Landsberg, Greg/0000-0002-4184-9380; Rizzi, Andrea/0000-0002-4543-2718; Gershtein, Yuri/0000-0002-4871-5449; Malik, Sudhir/0000-0002-6356-2655; Blekman, Freya/0000-0002-7366-7098; Barbieri, Richard/0000-0002-7945-005X; Staiano, Amedeo/0000-0003-1803-624X; Tonelli, Guido Emilio/0000-0003-2606-9156; Androsov, Konstantin/0000-0003-2694-6542; Toback, David/0000-0003-3457-4144; Abbiendi, Giovanni/0000-0003-4499-7562; HSIUNG, YEE/0000-0003-4801-1238; Vidal Marono, Miguel/0000-0002-2590-5987; Goldstein, Joel/0000-0003-1591-6014; Grassi, Marco/0000-0003-2422-6736; ORTONA, Giacomo/0000-0001-8411-2971; Ulrich, Ralf/0000-0002-2535-402X; Verdier, Patrice/0000-0003-3090-2948; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Jacob, Jeson/0000-0001-6895-5493 NR 91 TC 36 Z9 36 U1 7 U2 82 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 22 PY 2014 IS 5 AR 104 DI 10.1007/JHEP05(2014)104 PG 72 WC Physics, Particles & Fields SC Physics GA AI3BU UT WOS:000336734300001 ER PT J AU Alva, G Kim, C Yi, TH Cook, JB Xu, LP Nolis, GM Cabana, J AF Alva, Gabriela Kim, Chunjoong Yi, Tanghong Cook, John B. Xu, Linping Nolis, Gene M. Cabana, Jordi TI Surface Chemistry Consequences of Mg-Based Coatings on LiNi0.5Mn1.5O4 Electrode Materials upon Operation at High Voltage SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-ION BATTERIES; RAY-ABSORPTION SPECTROSCOPY; TRANSITION-METAL OXIDES; X-RAY; LITHIUM BATTERIES; CATHODE MATERIAL; SPINEL CATHODES; ELECTROCHEMICAL PROPERTIES; ELEVATED-TEMPERATURES; CHARGE COMPENSATION AB LiNi(0.5)Mni(1.5)O(4) epitomizes the challenges imposed by high electrochemical potential reactivity on the durability of high energy density Li-ion batteries. Postsynthesis coatings have been explored as a solution to these challenges, but the fundamentals of their function have not been ascertained. To contribute to this understanding, the surface of LiNi0.5Mn1.5O4 microparticles was modified with Mg2+, a coating component of literature relevance, using two different heat treatment temperatures, 500 and 800 degrees C. A combination of characterization tools revealed that Me2+ was introduced mainly as an inhomogeneous MgO coating in the sample treated at 500 degrees C, and into the spinel lattice at the subsurface of the particles at 800 degrees C. Comparing the properties of these two different materials with an unmodified baseline afforded the opportunity to evaluate the effect of varying surface chemistries. Coulometry in Li metal half cells was used as a macroscopic measure of side reactions at the electrode electrolyte interfaces. This magnitude was comparable in all the materials at room temperature. In contrast, a significant drop in efficiency was observed in the untreated material when the cycling temperature was raised to 50 degrees C, but not in the modified materials. The origin of the reduced reactivity of the materials after introducing Mg-based modifications was evaluated by probing the chemical changes at the Ni-O bonds using soft XAS. Taken together, the results of this study revealed that incorporation of Mg stabilizes highly oxidized Ni-O species, which can be related to the better stability toward the electrolyte. They point to a pathway toward the guided design of efficient surface modifications to yield battery electrode materials with increased stability against the electrolyte. C1 [Alva, Gabriela; Kim, Chunjoong; Yi, Tanghong; Cook, John B.; Xu, Linping; Nolis, Gene M.; Cabana, Jordi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm & Energy Technol Div, Berkeley, CA 94720 USA. [Alva, Gabriela] Univ Calif Berkeley, Coll Chem, Berkeley, CA 94720 USA. [Kim, Chunjoong; Cabana, Jordi] Univ Illinois, Dept Chem, Chicago, IL 60607 USA. RP Cabana, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm & Energy Technol Div, One Cyclotron Rd, Berkeley, CA 94720 USA. EM jcabana@uic.edu RI Cabana, Jordi/G-6548-2012; Cook, John/J-3730-2016 OI Cabana, Jordi/0000-0002-2353-5986; Cook, John/0000-0002-2886-3276 FU Office of Vehicle Technologies of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; LBNL through the Science Undergraduate Laboratory Internship program from the DOE; United States Government FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231, as part of the Batteries for Advanced Transportation Technologies (BATT) Program. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. G.M.N. was supported by LBNL through the Science Undergraduate Laboratory Internship program from the DOE. The authors wish to thank Dr. Dennis Nordlund (SSRL) for his assistance during the XAS measurements, and Dr. Marca M. Doeff (LBNL) for valuable interactions. This document was prepared as an account of work sponsored by the United States Government. While this document is believed to contain correct information, neither the United States Government nor any agency thereof, nor the Regents of the University of California, nor any of their employees, makes any warranty, express or implied, or assumes any legal responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by its trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof, or the Regents of the University of California. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof or the Regents of the University of California. NR 58 TC 15 Z9 15 U1 9 U2 85 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 22 PY 2014 VL 118 IS 20 BP 10596 EP 10605 DI 10.1021/jp5003148 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AI0AU UT WOS:000336509400009 ER PT J AU Barile, CJ Spatney, R Zavadil, KR Gewirth, AA AF Barile, Christopher J. Spatney, Russell Zavadil, Kevin R. Gewirth, Andrew A. TI Investigating the Reversibility of in Situ Generated Magnesium Organohaloalurninates for Magnesium Deposition and Dissolution SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-ION BATTERIES; ELECTROLYTE-SOLUTIONS; ELECTROCHEMISTRY; TECHNOLOGY; EFFICIENCY; PROGRESS; SYSTEMS; SALTS AB We compare the electrochemistry of Mg deposition and stripping from Mg(AlCl2EtBu)(2) in THF, a common electrolyte used in Mg-ion battery prototypes, with EtMgBr, a simple Grignard reagent. Electrochemical quartz crystal microbalance measurements demonstrate that mass is gained and lost from the electrode with relatively high efficiency. However, the corresponding Coulombic efficiency is considerably less than the expected 100% for early stage cycles. SEM-EDS analysis shows accumulation of Mg and electrolyte constituents after stripping, highlighting the irreversibility of the Mg deposition and stripping process. GC-MS and NMR analysis of electrolytes reveal decomposition of the solvent-electrolyte system. These findings suggest that Mg organohaloaluminates are not ideal for use in robust Mg-ion batteries. C1 [Barile, Christopher J.; Spatney, Russell; Gewirth, Andrew A.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Zavadil, Kevin R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Gewirth, AA (reprint author), Univ Illinois, Dept Chem, Urbana, IL 61801 USA. EM agewirth@illinois.edu FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; National Science Foundation Graduate Research Fellowship [NSF DGE-1144245]; Springborn Fellowship FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. C.J.B. acknowledges a National Science Foundation Graduate Research Fellowship (No. NSF DGE-1144245) and a Springborn Fellowship. This work was carried out in part in the Frederick Seitz Materials Research Laboratory Central Facilities, University of Illinois at Urbana-Champaign. NR 21 TC 25 Z9 25 U1 4 U2 89 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 22 PY 2014 VL 118 IS 20 BP 10694 EP 10699 DI 10.1021/jp503506c PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AI0AU UT WOS:000336509400020 ER PT J AU Wang, HW DelloStritto, MJ Kumar, N Kolesnikov, AI Kent, PRC Kubicki, JD Wesolowski, DJ Sofo, JO AF Wang, Hsiu-Wen DelloStritto, Mark J. Kumar, Nitin Kolesnikov, Alexander I. Kent, Paul R. C. Kubicki, James D. Wesolowski, David J. Sofo, Jorge O. TI Vibrational Density of States of Strongly H-Bonded Interfacial Water: Insights from Inelastic Neutron Scattering and Theory SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; HYDROGEN-BOND; SURFACE-WATER; THERMODYNAMIC PROPERTIES; ORIENTED ANALYSIS; PROGRAM PACKAGE; NANOPARTICLES; CASSITERITE; ADSORPTION; RUTILE AB The molecular scale interaction between water and an oxide surface depends on the strength of the surface hydrogen bonds (H-bonds) through a subtle interplay among surface structure, surface atom polarity, and orientation of sorbed species. Tin oxide (SnO2) in the rutile structure is an important catalytic and gas-sensing material, and its surface properties have been the subject of intense scrutiny. Here we show that the vibrational dynamics of H2O and OH sorbed on SnO2 nanoparticles, probed with inelastic neutron scattering and analyzed with ab initio molecular dynamics, reveals very strong surface H-bonds, with a formation enthalpy twice that of liquid water. This unusually strong interaction results in (i) decoupling of the hydrated surface from additional water layers due to an epitaxial screening layer of H2O and OH species, (ii) high energy of OH wagging modes that provides an experimental indicator of surface H-bond strengths, and (iii) high proton exchange rates at the interface. H-bonding energetics and interfacial structures also control the average degree of dissociation of sorbed water. The close agreement in the vibrational density of states measured experimentally and generated in silico provides validation of the theory, while the atomistic simulations provide atomic/molecular-level details of individual species contributions to the observed spectrum. Together, these integrated studies provide definitive insights into the role of H-bonds in controlling the structure, dynamics, and reactivity of metal oxide/water interfaces. C1 [Wang, Hsiu-Wen; Wesolowski, David J.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Kolesnikov, Alexander I.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [DelloStritto, Mark J.; Kumar, Nitin; Sofo, Jorge O.] Penn State Univ, Dept Phys & Mat Res, University Pk, PA 16802 USA. [Kubicki, James D.] Penn State Univ, Dept Geosci, University Pk, PA 16802 USA. RP Sofo, JO (reprint author), Penn State Univ, Dept Phys & Mat Res, University Pk, PA 16802 USA. EM sofo@psu.edu RI Kent, Paul/A-6756-2008; Kumar, Nitin/M-5778-2014; Kolesnikov, Alexander/I-9015-2012; Kubicki, James/I-1843-2012 OI Kent, Paul/0000-0001-5539-4017; Kumar, Nitin/0000-0002-1064-1659; Kolesnikov, Alexander/0000-0003-1940-4649; Kubicki, James/0000-0002-9277-9044 FU Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE); Scientific User Facilitates Division, BES, DOE; Materials Simulation Center, a Penn State Center for Nanoscale Science [MRSEC-NSF DMR-08-20404]; Penn State Materials Research Institute; National Science Foundation [OCI-0821527] FX This research was sponsored by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE). The research at the Spallation Neutron Source, and P.R.C.K's work at the Center for Nanophase Materials Science, conducted at Oak Ridge National Laboratory, were supported by the Scientific User Facilitates Division, BES, DOE. This work was supported in part by the Materials Simulation Center, a Penn State Center for Nanoscale Science (MRSEC-NSF DMR-08-20404), the Penn State Materials Research Institute facility, and through instrumentation funded by the National Science Foundation through Grant OCI-0821527. NR 53 TC 12 Z9 12 U1 8 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 22 PY 2014 VL 118 IS 20 BP 10805 EP 10813 DI 10.1021/jp500954v PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AI0AU UT WOS:000336509400032 ER PT J AU Alushin, GM Lander, GC Kellogg, EH Zhang, R Baker, D Nogales, E AF Alushin, Gregory M. Lander, Gabriel C. Kellogg, Elizabeth H. Zhang, Rui Baker, David Nogales, Eva TI High-Resolution Microtubule Structures Reveal the Structural Transitions in alpha beta-Tubulin upon GTP Hydrolysis SO CELL LA English DT Article ID SLOWLY HYDROLYZABLE ANALOG; NDC80 KINETOCHORE COMPLEX; STATHMIN-LIKE DOMAIN; ELECTRON CRYSTALLOGRAPHY; CRYOELECTRON MICROSCOPY; DYNAMIC INSTABILITY; GAMMA-TUBULIN; DENSITY MAPS; UCSF CHIMERA; BINDING AB Dynamic instability, the stochastic switching between growth and shrinkage, is essential for microtubule function. This behavior is driven by GTP hydrolysis in the microtubule lattice and is inhibited by anticancer agents like Taxol. We provide insight into the mechanism of dynamic instability, based on high-resolution cryo-EM structures (4.7-5.6 angstrom) of dynamic microtubules and microtubules stabilized by GMPCPP or Taxol. We infer that hydrolysis leads to a compaction around the E-site nucleotide at longitudinal interfaces, as well as movement of the alpha-tubulin intermediate domain and H7 helix. Displacement of the C-terminal helices in both alpha- and beta-tubulin subunits suggests an effect on interactions with binding partners that contact this region. Taxol inhibits most of these conformational changes, allosterically inducing a GMPCPP-like state. Lateral interactions are similar in all conditions we examined, suggesting that microtubule lattice stability is primarily modulated at longitudinal interfaces. C1 [Alushin, Gregory M.] Univ Calif Berkeley, Biophys Grad Program, Berkeley, CA 94720 USA. [Lander, Gabriel C.; Zhang, Rui; Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Kellogg, Elizabeth H.; Baker, David] Univ Washington, Dept Biochem, Howard Hughes Med Inst, Seattle, WA 98105 USA. [Nogales, Eva] Univ Calif Berkeley, Dept Mol & Cell Biol, Howard Hughes Med Inst, Berkeley, CA 94720 USA. RP Nogales, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM enogales@lbl.gov RI Baker, David/K-8941-2012 OI Baker, David/0000-0001-7896-6217 FU National Institute of General Medical Sciences [GM051487]; Damon Runyon Cancer Research Foundation [DRG 2055-10] FX We thank Patricia Grob and Tom Houweling for electron microscopy and computer support, respectively, Tom Goddard for help with UCSF Chimera, Yifan Song and Frank DiMaio for making code available for use prior to publication, and Stuart Howes for assistance with kinesin purification. We are grateful to Robert Glaeser for assistance with data collection and many discussions. The kinesin expression construct was the gift of Erik Jonsson and Ron Vale. This work was funded by the National Institute of General Medical Sciences (GM051487) (to E.N.) and a Damon Runyon Cancer Research Foundation fellowship (DRG 2055-10) (to G. C. L.). E.N. and D. B. are Howard Hughes Medical Institute Investigators. NR 56 TC 111 Z9 111 U1 9 U2 81 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD MAY 22 PY 2014 VL 157 IS 5 BP 1117 EP 1129 DI 10.1016/j.cell.2014.03.053 PG 13 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA AH9CG UT WOS:000336437200014 PM 24855948 ER PT J AU De Re, E Schlau-Cohen, GS Leverenz, RL Huxter, VM Oliver, TAA Mathies, RA Fleming, GR AF De Re, Eleonora Schlau-Cohen, Gabriela S. Leverenz, Ryan L. Huxter, Vanessa M. Oliver, Thomas A. A. Mathies, Richard A. Fleming, Graham R. TI Insights into the Structural Changes Occurring upon Photoconversion in the Orange Carotenoid Protein from Broadband Two-Dimensional Electronic Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID LIGHT-HARVESTING COMPLEX; SYNECHOCYSTIS PCC 6803; CHARGE-TRANSFER STATE; PHOTOSYSTEM-II; CYANOBACTERIAL PHOTOPROTECTION; ARTHROSPIRA-MAXIMA; ENERGY-DISSIPATION; MOLECULAR SWITCH; EXCITED-STATES; MECHANISM AB Carotenoids play an essential role in photoprotection, interacting with other pigments to safely dissipate excess absorbed energy as heat. In cyanobacteria, the short time scale photoprotective mechanisms involve the photoactive orange carotenoid protein (OCP), which binds a single carbonyl carotenoid. Blue-green light induces the photoswitching of OCP from its ground state form (OCPO) to a metastable photoproduct (OCPR). OCPR can bind to the phycobilisome antenna and induce fluorescence quenching. The photoswitching is accompanied by structural and functional changes at the level of the protein and of the bound carotenoid. Here, we use broadband two-dimensional electronic spectroscopy to study the differences in excited state dynamics of the carotenoid in the two forms of OCP. Our results provide insight into the origin of the pronounced vibrational lineshape and oscillatory dynamics observed in linear absorption and 2D electronic spectroscopy of OCPO and the large inhomogeneous broadening in OCPR, with consequences for the chemical function of the two forms. C1 [De Re, Eleonora; Fleming, Graham R.] Univ Calif Berkeley, Appl Sci & Technol Grad Grp, Berkeley, CA 94720 USA. [De Re, Eleonora; Schlau-Cohen, Gabriela S.; Huxter, Vanessa M.; Oliver, Thomas A. A.; Fleming, Graham R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Schlau-Cohen, Gabriela S.; Leverenz, Ryan L.; Huxter, Vanessa M.; Oliver, Thomas A. A.; Mathies, Richard A.; Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Fleming, GR (reprint author), Univ Calif Berkeley, Appl Sci & Technol Grad Grp, Berkeley, CA 94720 USA. EM grfleming@lbl.gov FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences [DE-AC03-76SF000098] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231 and the Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences through Grant DE-AC03-76SF000098 (at LBNL and U.C. Berkeley). The authors acknowledge J. Zaks for helpful comments on the manuscript. The authors also thank Dr. Gerald Cysewski for the gift of A. platensis cells. NR 57 TC 6 Z9 6 U1 1 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 22 PY 2014 VL 118 IS 20 BP 5382 EP 5389 DI 10.1021/jp502120h PG 8 WC Chemistry, Physical SC Chemistry GA AI0BD UT WOS:000336510300011 PM 24779893 ER PT J AU Gal-Yam, A Arcavi, I Ofek, EO Ben-Ami, S Cenko, SB Kasliwal, MM Cao, Y Yaron, O Tal, D Silverman, JM Horesh, A De Cia, A Taddia, F Sollerman, J Perley, D Vreeswijk, PM Kulkarni, SR Nugent, PE Filippenko, AV Wheeler, JC AF Gal-Yam, Avishay Arcavi, I. Ofek, E. O. Ben-Ami, S. Cenko, S. B. Kasliwal, M. M. Cao, Y. Yaron, O. Tal, D. Silverman, J. M. Horesh, A. De Cia, A. Taddia, F. Sollerman, J. Perley, D. Vreeswijk, P. M. Kulkarni, S. R. Nugent, P. E. Filippenko, A. V. Wheeler, J. C. TI A Wolf-Rayet-like progenitor of SN 2013cu from spectral observations of a stellar wind SO NATURE LA English DT Article ID SUPERNOVA PROGENITORS; IIB SUPERNOVA; MASSIVE STARS; DISCOVERY; 2011DH; TELESCOPE; EVOLUTION; GALAXY; MODEL; IB/C AB The explosive fate of massive Wolf-Rayet stars(1) (WRSs) is a key open question in stellar physics. An appealing option is that hydrogen-deficient WRSs are the progenitors of some hydrogen-poor supernova explosions of types IIb, Ib and Ic (ref. 2). A blue object, having luminosity and colours consistent with those of some WRSs, has recently been identified in pre-explosion images at the location of a supernova of type Ib (ref. 3), but has not yet been conclusively determined to have been the progenitor. Similar work has so far only resulted in non-detections(4). Comparison of early photometric observations of type Ic supernovae with theoretical models suggests that the progenitor stars had radii of less than 1012 centimetres, as expected for some WRSs(5). The signature of WRSs, their emission line spectra, cannot be probed by such studies. Here we report the detection of strong emission lines in a spectrum of type IIb supernova 2013cu (iPTF13ast) obtained approximately 15.5 hours after explosion (by 'flash spectroscopy', which captures the effects of the supernova explosion shock breakout flash on material surrounding the progenitor star). We identify Wolf-Rayet-like wind signatures, suggesting a progenitor of the WN(h) subclass (those WRSs with winds dominated by helium and nitrogen, with traces of hydrogen). The extent of this dense wind may indicate increased mass loss from the progenitor shortly before its explosion, consistent with recent theoretical predictions(6). C1 [Gal-Yam, Avishay; Arcavi, I.; Ofek, E. O.; Ben-Ami, S.; Yaron, O.; Tal, D.; De Cia, A.; Vreeswijk, P. M.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. [Cenko, S. B.] NASA, Astrophys Sci Div, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Kasliwal, M. M.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Cao, Y.; Horesh, A.; Perley, D.; Kulkarni, S. R.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Silverman, J. M.; Wheeler, J. C.] Univ Texas Austin, Dept Astron, Austin, TX 78712 USA. [Taddia, F.; Sollerman, J.] Stockholm Univ, Oskar Klein Ctr, Dept Astron, AlbaNova, S-10691 Stockholm, Sweden. [Nugent, P. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Filippenko, A. V.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94701 USA. RP Gal-Yam, A (reprint author), Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. EM avishay.gal-yam@weizmann.ac.il RI Horesh, Assaf/O-9873-2016; OI Horesh, Assaf/0000-0002-5936-1156; Sollerman, Jesper/0000-0003-1546-6615 FU I-CORE programme 'The Quantum Universe' of the Planning and Budgeting Committee; Israel Science Foundation; ISF; BSF; GIF; Minerva; FP7/ERC; Kimmel Investigator award; Hubble fellowship; Israeli MOST; NSF; TABASGO Foundation; Richard and Rhoda Goldman Fund; Christopher R. Redlich Fund; Swedish Research Council; W. M. Keck Foundation; Carnegie-Princeton fellowship FX This research was supported by the I-CORE programme 'The Quantum Universe' of the Planning and Budgeting Committee and The Israel Science Foundation. A.G.-Y. acknowledges support by grants from the ISF, BSF, GIF, Minerva and FP7/ERC, and a Kimmel Investigator award. M. M. K. acknowledges support from Hubble and Carnegie-Princeton fellowships. E.O.O. acknowledges the Arye Dissentshik Career Development Chair and a grant from the Israeli MOST. J.C.W. is supported in part by the NSF. J.M.S. is supported by an NSF Postdoctoral Fellowship. A. V. F. acknowledges financial support from the TABASGO Foundation, the Richard and Rhoda Goldman Fund, the Christopher R. Redlich Fund and the NSF. The National Energy Research Scientific Computing Center, supported by the Office of Science of the US Department of Energy, provided staff, computational resources and data storage for this project. The Oskar Klein Centre is funded by the Swedish Research Council. We thank K. Clubb, O. Fox, P. Kelly, S. Tang and B. Sesar for their help with observations, and J. Groh, P. Crowther, M. Bersten, C. Fransson and E. Nakar for advice. Some of the data presented here were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California and NASA. The observatory was made possible by the generous financial support of the W. M. Keck Foundation. NR 40 TC 54 Z9 54 U1 0 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 22 PY 2014 VL 509 IS 7501 BP 471 EP + DI 10.1038/nature13304 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH4VE UT WOS:000336126000034 PM 24848059 ER PT J AU Patel, SS Min, MS Uga, KC Lee, T AF Patel, Saumil Sudhir Min, Misun Uga, Kalu Chibueze Lee, Taehun TI A spectral-element discontinuous Galerkin lattice Boltzmann method for simulating natural convection heat transfer in a horizontal concentric annulus SO COMPUTERS & FLUIDS LA English DT Article DE Thermal lattice Boltzmann method; Spectral-element method; Discontinuous Galerkin method; Natural convection flow ID HIGH RAYLEIGH NUMBER; SQUARE CAVITY; INCOMPRESSIBLE LIMIT; BGK MODELS; FLOWS; EQUATION AB We present a spectral-element discontinuous Galerkin lattice Boltzmann method to solve incompressible natural convection flows based on the Bousinessq approximation. A passive-scalar thermal lattice Boltzmann model is used to resolve flows for variable Prandtl number. In our model, we solve the lattice Boltzmann equation for the velocity field and the advection-diffusion equation for the temperature field. As a result, we reduce the degrees of freedom when compared with the passive-scalar double-distribution model, which requires the solution of several equations to resolve the temperature field. Our numerical solution is represented by the tensor product basis of the one-dimensional Legendre-Lagrange interpolation polynomials. A high-order discretization is employed on body-conforming hexahedral elements with Gauss-Lobatto-Legendre quadrature nodes. Within the discontinuous Galerkin framework, we weakly impose boundary and element-interface conditions through the numerical flux. A fourth-order Runge-Kutta scheme is used for time integration with no additional cost for mass matrix inversion due to fully diagonal mass matrices. We study natural convection fluid flows in a square cavity and a horizontal concentric annulus for Rayleigh numbers in the range of Ra = 10(3)-10(8). We validate our numerical approach by comparing it with finite-difference, finite-volume, multiple-relaxation-time lattice Boltzmann, and spectral-element methods. Our computational results show good agreement in temperature profiles and Nusselt numbers using relatively coarse resolutions. (c) 2014 Elsevier Ltd. All rights reserved. C1 [Patel, Saumil Sudhir; Uga, Kalu Chibueze; Lee, Taehun] CUNY City Coll, Dept Mech Engn, New York, NY 10031 USA. [Min, Misun] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Lee, T (reprint author), CUNY City Coll, Dept Mech Engn, New York, NY 10031 USA. EM saumil.patel134@gmail.com; mmin@mcs.anl.gov; uga.kalu@gmail.com; thlee@ccny.cuny.edu RI Lee, Taehun/G-2695-2010 OI Lee, Taehun/0000-0001-9965-5637 FU U.S. Department of Energy, Office of Nuclear Energy's Nuclear Energy University Programs; U.S. Department of Energy [DE-ACO2-O6CH11357] FX This work is supported in part by the U.S. Department of Energy, Office of Nuclear Energy's Nuclear Energy University Programs, and in part by the U.S. Department of Energy, under Contract DE-ACO2-O6CH11357. We thank Alexsandr Obabko for his help and guidance in the proper execution of the Nek5000 code. NR 42 TC 4 Z9 4 U1 0 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD MAY 22 PY 2014 VL 95 BP 197 EP 209 DI 10.1016/j.compfluid.2014.02.021 PG 13 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA AG7WP UT WOS:000335629800014 ER PT J AU Seraydaryan, H Amaryan, MJ Gavalian, G Baghdasaryan, H Weinstein, L Adhikari, KP Adikaram, D Aghasyan, M Anderson, MD Pereira, SA Avakian, H Ball, J Baltzell, NA Battaglieri, M Batourine, V Bedlinskiy, I Bennett, RP Biselli, AS Bono, J Boiarinov, S Briscoe, WJ Brooks, WK Bultmann, S Burkert, VD Carman, DS Celentano, A Chandavar, S Collins, P Contalbrigo, M Cortes, O Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Doughty, D Dugger, M Dupre, R El Fassi, L Eugenio, P Fedotov, G Fegan, S Fersch, R Fleming, JA Gevorgyan, N Giovanetti, KL Girod, FX Goetz, JT Gohn, W Golovatch, E Gothe, RW Griffioen, KA Guidal, M Guler, N Guo, L Hafidi, K Hakobyan, H Hanretty, C Harrison, N Heddle, D Hicks, K Ho, D Holtrop, M Hyde, CE Ilieva, Y Ireland, DG Ishkhanov, BS Isupov, EL Jo, HS Joo, K Keller, D Khandaker, M Kim, A Kim, W Klein, FJ Koirala, S Kubarovsky, A Kubarovsky, V Kuhn, SE Kuleshov, SV Lewis, S Livingston, K Lu, HY MacGregor, IJD Martinez, D Mayer, M McKinnon, B Mineeva, T Mirazita, M Mokeev, V Montgomery, RA Moutarde, H Munevar, E Camacho, CM Nadel-Turonski, P Nasseripour, R Niccolai, S Niculescu, I Osipenko, M Ostrovidov, AI Pappalardo, LL Paremuzyan, R Park, K Park, S Pasyuk, E Phelps, E Phillips, JJ Pisano, S Pogorelko, O Pozdniakov, S Price, JW Protopopescu, D Puckett, AJR Rimal, D Ripani, M Ritchie, BG Rizzo, A Rosner, G Rossi, P Sabatie, F Saini, MS Salgado, C Schott, D Schumacher, RA Seder, E Sharabian, YG Smith, GD Sober, DI Sokhan, D Stepanyan, S Stoler, P Strakovsky, II Strauch, S Tang, W Taylor, CE Tian, Y Tkachenko, S Ungaro, M Vineyard, MF Voskanyan, H Voutier, E Walford, NK Watts, DP Weinstein, LB Wood, MH Zachariou, N Zana, L Zhang, J Zhao, ZW AF Seraydaryan, H. Amaryan, M. J. Gavalian, G. Baghdasaryan, H. Weinstein, L. Adhikari, K. P. Adikaram, D. Aghasyan, M. Anderson, M. D. Pereira, S. Anefalos Avakian, H. Ball, J. Baltzell, N. A. Battaglieri, M. Batourine, V. Bedlinskiy, I. Bennett, R. P. Biselli, A. S. Bono, J. Boiarinov, S. Briscoe, W. J. Brooks, W. K. Bueltmann, S. Burkert, V. D. Carman, D. S. Celentano, A. Chandavar, S. Collins, P. Contalbrigo, M. Cortes, O. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Doughty, D. Dugger, M. Dupre, R. El Fassi, L. Eugenio, P. Fedotov, G. Fegan, S. Fersch, R. Fleming, J. A. Gevorgyan, N. Giovanetti, K. L. Girod, F. X. Goetz, J. T. Gohn, W. Golovatch, E. Gothe, R. W. Griffioen, K. A. Guidal, M. Guler, N. Guo, L. Hafidi, K. Hakobyan, H. Hanretty, C. Harrison, N. Heddle, D. Hicks, K. Ho, D. Holtrop, M. Hyde, C. E. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Isupov, E. L. Jo, H. S. Joo, K. Keller, D. Khandaker, M. Kim, A. Kim, W. Klein, F. J. Koirala, S. Kubarovsky, A. Kubarovsky, V. Kuhn, S. E. Kuleshov, S. V. Lewis, S. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Martinez, D. Mayer, M. McKinnon, B. Mineeva, T. Mirazita, M. Mokeev, V. Montgomery, R. A. Moutarde, H. Munevar, E. Camacho, C. Munoz Nadel-Turonski, P. Nasseripour, R. Niccolai, S. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Pappalardo, L. L. Paremuzyan, R. Park, K. Park, S. Pasyuk, E. Phelps, E. Phillips, J. J. Pisano, S. Pogorelko, O. Pozdniakov, S. Price, J. W. Protopopescu, D. Puckett, A. J. R. Rimal, D. Ripani, M. Ritchie, B. G. Rizzo, A. Rosner, G. Rossi, P. Sabatie, F. Saini, M. S. Salgado, C. Schott, D. Schumacher, R. A. Seder, E. Sharabian, Y. G. Smith, G. D. Sober, D. I. Sokhan, D. Stepanyan, S. Stoler, P. Strakovsky, I. I. Strauch, S. Tang, W. Taylor, C. E. Tian, Ye Tkachenko, S. Ungaro, M. Vineyard, M. F. Voskanyan, H. Voutier, E. Walford, N. K. Watts, D. P. Weinstein, L. B. Wood, M. H. Zachariou, N. Zana, L. Zhang, J. Zhao, Z. W. TI phi-meson photoproduction on hydrogen in the neutral decay mode SO PHYSICAL REVIEW C LA English DT Article ID LARGE MOMENTUM-TRANSFER; DRIFT CHAMBER SYSTEM; PERTURBATIVE QCD; BARYON RESONANCES; NEAR-THRESHOLD; CLAS; DETECTOR; SPECTROMETER AB We report the first measurement of the photoproduction cross section of the phi meson in its neutral decay mode in the reaction gamma p -> p phi(KSKL). The experiment was performed with a tagged photon beam of energy 1.6 <= E-gamma <= 3.6 GeV incident on a liquid hydrogen target of the CLAS spectrometer at the Thomas Jefferson National Accelerator Facility. The p phi final state is identified via reconstruction of K-S in the invariant mass of two oppositely charged pions and by requiring the missing particle in the reaction gamma p -> pK(S)X to be K-L. The presented results significantly enlarge the existing data on phi photoproduction. These data, combined with the data from the charged decay mode, will help to constrain different mechanisms of phi photoproduction. C1 [Seraydaryan, H.; Amaryan, M. J.; Gavalian, G.; Weinstein, L.; Adhikari, K. P.; Adikaram, D.; Bennett, R. P.; Bueltmann, S.; Guler, N.; Hyde, C. E.; Koirala, S.; Kuhn, S. E.; Mayer, M.; Tkachenko, S.; Weinstein, L. B.] Old Dominion Univ, Norfolk, VA 23529 USA. [Baghdasaryan, H.] Univ Virginia, Charlottesville, VA 22904 USA. [Aghasyan, M.; Pereira, S. Anefalos; De Sanctis, E.; Mirazita, M.; Pisano, S.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Anderson, M. D.; Ireland, D. G.; Lewis, S.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Montgomery, R. A.; Phillips, J. J.; Protopopescu, D.; Rosner, G.; Smith, G. D.; Sokhan, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Avakian, H.; Batourine, V.; Boiarinov, S.; Brooks, W. K.; Burkert, V. D.; Carman, D. S.; Deur, A.; Doughty, D.; Girod, F. X.; Guo, L.; Heddle, D.; Kubarovsky, V.; Mokeev, V.; Nadel-Turonski, P.; Park, K.; Pasyuk, E.; Puckett, A. J. R.; Rossi, P.; Sharabian, Y. G.; Stepanyan, S.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Ball, J.; Girod, F. X.; Moutarde, H.; Sabatie, F.] CEA, Ctr Saclay, Irfu Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Baltzell, N. A.; El Fassi, L.; Hafidi, K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Baltzell, N. A.; Djalali, C.; Fedotov, G.; Gothe, R. W.; Lu, H. Y.; Nasseripour, R.; Phelps, E.; Strauch, S.; Tian, Ye; Wood, M. H.; Zachariou, N.] Univ S Carolina, Columbia, SC 29208 USA. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Batourine, V.; Kim, A.; Kim, W.; Park, K.] Kyungpook Natl Univ, Daegu 702701, South Korea. [Bedlinskiy, I.; Kuleshov, S. V.; Pogorelko, O.; Pozdniakov, S.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Biselli, A. S.] Fairfield Univ, Fairfield, CT 06824 USA. [Bono, J.; Guo, L.; Rimal, D.] Florida Int Univ, Miami, FL 33199 USA. [Briscoe, W. J.; Ilieva, Y.; Munevar, E.; Schott, D.; Strakovsky, I. I.; Strauch, S.] George Washington Univ, Washington, DC 20052 USA. [Brooks, W. K.; Hakobyan, H.; Kuleshov, S. V.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Chandavar, S.; Goetz, J. T.; Hicks, K.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Collins, P.; Klein, F. J.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Contalbrigo, M.; Pappalardo, L. L.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Cortes, O.; Martinez, D.; Taylor, C. E.] Idaho State Univ, Pocatello, ID 83209 USA. [Crede, V.; Eugenio, P.; Hanretty, C.; Ostrovidov, A. I.; Park, S.; Saini, M. S.] Florida State Univ, Tallahassee, FL 32306 USA. [D'Angelo, A.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [D'Angelo, A.; Rizzo, A.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Dashyan, N.; Gevorgyan, N.; Hakobyan, H.; Paremuzyan, R.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Doughty, D.; Heddle, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Dugger, M.; Pasyuk, E.; Ritchie, B. G.] Arizona State Univ, Tempe, AZ 85287 USA. [Dupre, R.; Guidal, M.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.] ORSAY, Inst Phys Nucl, Orsay, France. [Fedotov, G.; Golovatch, E.; Ishkhanov, B. S.; Isupov, E. L.; Kubarovsky, A.; Mokeev, V.] Skobeltsyn Nucl Phys Inst, Moscow 119899, Russia. [Fersch, R.; Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Fleming, J. A.; Sokhan, D.; Watts, D. P.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Giovanetti, K. L.; Nasseripour, R.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Gohn, W.; Harrison, N.; Joo, K.; Kubarovsky, A.; Mineeva, T.; Seder, E.] Univ Connecticut, Storrs, CT 06269 USA. [Hanretty, C.; Keller, D.; Tkachenko, S.; Zhao, Z. W.] Univ Virginia, Charlottesville, VA 22901 USA. [Ho, D.; Lu, H. Y.; Schumacher, R. A.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Holtrop, M.; Zana, L.] Univ New Hampshire, Durham, NH 03824 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Kubarovsky, V.; Stoler, P.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Vineyard, M. F.] Union Coll, Schenectady, Schenectady, NY 12308 USA. [Voutier, E.] Univ Joseph Fourier, LPSC, CNRS IN2P3, INPG, Grenoble, France. [Wood, M. H.] Canisius Coll, Buffalo, NY 14208 USA. RP Amaryan, MJ (reprint author), Old Dominion Univ, Norfolk, VA 23529 USA. EM mamaryan@odu.edu RI MacGregor, Ian/D-4072-2011; Sabatie, Franck/K-9066-2015; Osipenko, Mikhail/N-8292-2015; Zhang, Jixie/A-1461-2016; Adikaram, Dasuni/D-1539-2016; Adikaram, D/H-7128-2016; Celentano, Andrea/J-6190-2012; Schumacher, Reinhard/K-6455-2013; D'Angelo, Annalisa/A-2439-2012; OI Sabatie, Franck/0000-0001-7031-3975; Osipenko, Mikhail/0000-0001-9618-3013; Celentano, Andrea/0000-0002-7104-2983; Schumacher, Reinhard/0000-0002-3860-1827; D'Angelo, Annalisa/0000-0003-3050-4907; Bono, Jason/0000-0002-3018-714X; Hyde, Charles/0000-0001-7282-8120 FU Italian Istituto Nazionale di Fisica Nucleare; French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique; United Kingdom's Science and Technology Facilities Council (STFC); US Department of Energy and National Science Foundation; Korea Science and Engineering Foundation; United States Department of Energy [DEAC05-84ER40150] FX We would like to acknowledge the outstanding efforts of the staff of the Accelerator and the Physics Divisions at Jefferson Lab that made the experiment possible. This work was supported in part by the Italian Istituto Nazionale di Fisica Nucleare, the French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique, the United Kingdom's Science and Technology Facilities Council (STFC), the US Department of Energy and National Science Foundation, and the Korea Science and Engineering Foundation. The Southeastern Universities Research Association (SURA) operates the Thomas Jefferson National Accelerator Facility for the United States Department of Energy under Contract No. DEAC05-84ER40150. NR 47 TC 5 Z9 5 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 22 PY 2014 VL 89 IS 5 AR 055206 DI 10.1103/PhysRevC.89.055206 PG 17 WC Physics, Nuclear SC Physics GA CJ0WI UT WOS:000355199600002 ER PT J AU Brown, JA Goldblum, BL Bernstein, LA Bleuel, DL Brickner, NM Caggiano, JA Daub, BH Kaufman, GS Hatarik, R Phillips, TW Wender, SA van Bibber, K Vujic, J Zaitseva, NP AF Brown, J. A. Goldblum, B. L. Bernstein, L. A. Bleuel, D. L. Brickner, N. M. Caggiano, J. A. Daub, B. H. Kaufman, G. S. Hatarik, R. Phillips, T. W. Wender, S. A. van Bibber, K. Vujic, J. Zaitseva, N. P. TI Relative light yield and temporal response of a stilbene-doped bibenzyl organic scintillator for neutron detection SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TIME AB The neutron time-of-flight (nTOF) diagnostics used to characterize implosions at the National Ignition Facility (NIF) has necessitated the development of novel scintillators that exhibit a rapid temporal response and high light yield. One such material, a bibenzyl-stilbene mixed single-crystal organic scintillator grown in a 99.5:0.5 ratio in solution, has become the standard scintillator used for nTOF diagnostics at NIF. The prompt fluorescence lifetime and relative light yield as a function of proton energy were determined to calibrate this material as a neutron detector. The temporal evolution of the intensity of the prompt fluorescent response was modeled using first-order reaction kinetics and the prompt fluorescence decay constant was determined to be 2.46 +/- 0.01 (fit) +/- 0.13 (systematic) ns. The relative response of the bibenzyl-stilbene mixed crystal generated by recoiling protons was measured, and results were analyzed using Birks' relation to quantify the non-radiative quenching of excitation energy in the scintillator. (C) 2014 AIP Publishing LLC. C1 [Brown, J. A.; Goldblum, B. L.; Brickner, N. M.; Daub, B. H.; Kaufman, G. S.; van Bibber, K.; Vujic, J.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Bernstein, L. A.; Bleuel, D. L.; Caggiano, J. A.; Hatarik, R.; Phillips, T. W.; Zaitseva, N. P.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Wender, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Goldblum, BL (reprint author), Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. EM bethany@nuc.berkeley.edu OI Wender, Stephen/0000-0002-2446-5115 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; National Nuclear Security Administration [DE-NA0000979]; Nuclear Science and Security Consortium; University of California Office of the President Laboratory Fees Research Program FX The authors would like to thank the 88-in. Cyclotron operations and facilities staff for their help in performing this experiment. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231, the National Nuclear Security Administration under Award No. DE-NA0000979, The Nuclear Science and Security Consortium, and the University of California Office of the President Laboratory Fees Research Program under Award No. 12-LR-238745. NR 15 TC 6 Z9 6 U1 1 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 21 PY 2014 VL 115 IS 19 AR 193504 DI 10.1063/1.4878238 PG 5 WC Physics, Applied SC Physics GA AI5PA UT WOS:000336920200016 ER PT J AU Lara-Curzio, E May, AF Delaire, O McGuire, MA Lu, X Liu, CY Case, ED Morelli, DT AF Lara-Curzio, E. May, A. F. Delaire, O. McGuire, M. A. Lu, X. Liu, Cheng-Yun Case, E. D. Morelli, D. T. TI Low-temperature heat capacity and localized vibrational modes in natural and synthetic tetrahedrites SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID CU12SB4S13 AB The heat capacity of natural (Cu12-x (Fe, Zn, Ag) x(Sb, As)(4)S-13) and synthetic (Cu12-xZnxSb4S13 with x = 0, 1, 2) tetrahedrite compounds was measured between 2K and 380 K. It was found that the temperature dependence of the heat capacity can be described using a Debye term and three Einstein oscillators with characteristic temperatures that correspond to energies of similar to 1.0 meV, similar to 2.8 meV, and similar to 8.4 meV. The existence of localized vibrational modes, which are assigned to the displacements of the trigonally coordinated Cu atoms in the structure, is discussed in the context of anharmonicity and its effect on the low lattice thermal conductivity exhibited by these compounds. (C) 2014 AIP Publishing LLC. C1 [Lara-Curzio, E.; May, A. F.; Delaire, O.; McGuire, M. A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Lu, X.; Liu, Cheng-Yun; Case, E. D.; Morelli, D. T.] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. RP Lara-Curzio, E (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM laracurzioe@ornl.gov RI McGuire, Michael/B-5453-2009; May, Andrew/E-5897-2011 OI McGuire, Michael/0000-0003-1762-9406; May, Andrew/0000-0003-0777-8539 FU Center on Revolutionary Materials for Solid State Energy Conversion, an Energy Frontier Research Center - U. S. Department of Energy, Office of Basic Energy Sciences [DE-SC0001054]; U. S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX This study was funded through the Center on Revolutionary Materials for Solid State Energy Conversion, an Energy Frontier Research Center funded by the U. S. Department of Energy, Office of Basic Energy Sciences under Award No. DE-SC0001054. A.F.M., O.D., and M.A.M. acknowledge funding from the U. S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. The authors thank their colleagues Bryan Chakoumakos and Hsin Wang of ORNL for reviewing the manuscript and for providing valuable comments. NR 7 TC 22 Z9 22 U1 3 U2 50 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 21 PY 2014 VL 115 IS 19 AR 193515 DI 10.1063/1.4878676 PG 6 WC Physics, Applied SC Physics GA AI5PA UT WOS:000336920200027 ER PT J AU Merritt, TR Meeker, MA Magill, BA Khodaparast, GA McGill, S Tischler, JG Choi, SG Palmstrom, CJ AF Merritt, T. R. Meeker, M. A. Magill, B. A. Khodaparast, G. A. McGill, S. Tischler, J. G. Choi, S. G. Palmstrom, C. J. TI Photoluminescence lineshape and dynamics of localized excitonic transitions in InAsP epitaxial layers SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MOLECULAR-BEAM EPITAXY; CHEMICAL-VAPOR-DEPOSITION; QUANTUM-WELL STRUCTURES; TEMPERATURE-DEPENDENCE; SEMICONDUCTOR ALLOYS; AL(X)GA1-XN ALLOYS; MAGNETIC-FIELD; PHASE EPITAXY; GROWTH; ALXGA1-XAS AB The excitonic radiative transitions of InAsxP1-x (x = 0.13 and x = 0.40) alloy epitaxial layers were studied through magnetic field and temperature dependent photoluminescence and time-resolved photoluminescence spectroscopy. While the linewidth and lineshape of the exciton transition for x = 0.40 indicate the presence of alloy broadening due to random anion distribution and the existence of localized exciton states, those of x = 0.13 suggest that this type of compositional disorder is absent in x = 0.13. This localization is further supported by the behavior of the exciton transitions at low temperature and high magnetic fields. InAs0.4P0.6 exhibits anomalous "S-shaped" temperature dependence of the excition emission peak below 100K as well as linewidth broadening at high magnetic fields due to the compression of the excitonic volume amid compositional fluctuations. Finally, photoluminescence decay patterns suggest that the excitons radiatively relax through two channels, a fast and a slow decay. While the lifetime of the fast decay is comparable for both compositions (similar to 30 ps), that of the slow decay increases from 206 ps to 427 ps as x increases from 0.13 to 0.40, attributable to carrier migration between the localization states of InAs0.4P0.6. (C) 2014 AIP Publishing LLC. C1 [Merritt, T. R.; Meeker, M. A.; Magill, B. A.; Khodaparast, G. A.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [McGill, S.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Tischler, J. G.] Naval Res Lab, Washington, DC 20375 USA. [Choi, S. G.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Palmstrom, C. J.] Univ Calif Santa Barbara, Dept Elect & Comp Engn, Santa Barbara, CA 93106 USA. RP Khodaparast, GA (reprint author), Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. EM khoda@vt.edu RI Choi, Sukgeun/J-2345-2014 FU NSF-Career Award [DMR-0846834]; NSF [DMR-1157490]; State of Florida; U.S. Department of Energy; UCGP; Institute of Critical Technology and Applied Sciences (ICTAS) at Virginia Tech. FX This work was supported by NSF-Career Award DMR-0846834, and a portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement No. DMR-1157490, the State of Florida, the U.S. Department of Energy, and through a UCGP. G. A. Khodaparast thanks the inputs from Professor Alexey Belyanin and the funding from the Institute of Critical Technology and Applied Sciences (ICTAS) at Virginia Tech. NR 37 TC 3 Z9 3 U1 2 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 21 PY 2014 VL 115 IS 19 AR 193503 DI 10.1063/1.4876121 PG 8 WC Physics, Applied SC Physics GA AI5PA UT WOS:000336920200015 ER PT J AU Huntley, RP Harris, MA Alam-Faruque, Y Blake, JA Carbon, S Dietze, H Dimmer, EC Foulger, RE Hill, DP Khodiyar, VK Lock, A Lomax, J Lovering, RC Mutowo-Meullenet, P Sawford, T Van Auken, K Wood, V Mungall, CJ AF Huntley, Rachael P. Harris, Midori A. Alam-Faruque, Yasmin Blake, Judith A. Carbon, Seth Dietze, Heiko Dimmer, Emily C. Foulger, Rebecca E. Hill, David P. Khodiyar, Varsha K. Lock, Antonia Lomax, Jane Lovering, Ruth C. Mutowo-Meullenet, Prudence Sawford, Tony Van Auken, Kimberly Wood, Valerie Mungall, Christopher J. TI A method for increasing expressivity of Gene Ontology annotations using a compositional approach SO BMC BIOINFORMATICS LA English DT Article DE Gene Ontology; Functional annotation; Annotation extension; Manual curation ID RESOURCE; DATABASE; GENOMES AB Background: The Gene Ontology project integrates data about the function of gene products across a diverse range of organisms, allowing the transfer of knowledge from model organisms to humans, and enabling computational analyses for interpretation of high-throughput experimental and clinical data. The core data structure is the annotation, an association between a gene product and a term from one of the three ontologies comprising the GO. Historically, it has not been possible to provide additional information about the context of a GO term, such as the target gene or the location of a molecular function. This has limited the specificity of knowledge that can be expressed by GO annotations. Results: The GO Consortium has introduced annotation extensions that enable manually curated GO annotations to capture additional contextual details. Extensions represent effector-target relationships such as localization dependencies, substrates of protein modifiers and regulation targets of signaling pathways and transcription factors as well as spatial and temporal aspects of processes such as cell or tissue type or developmental stage. We describe the content and structure of annotation extensions, provide examples, and summarize the current usage of annotation extensions. Conclusions: The additional contextual information captured by annotation extensions improves the utility of functional annotation by representing dependencies between annotations to terms in the different ontologies of GO, external ontologies, or an organism's gene products. These enhanced annotations can also support sophisticated queries and reasoning, and will provide curated, directional links between many gene products to support pathway and network reconstruction. C1 [Huntley, Rachael P.; Alam-Faruque, Yasmin; Dimmer, Emily C.; Foulger, Rebecca E.; Lomax, Jane; Mutowo-Meullenet, Prudence; Sawford, Tony] European Bioinformat Inst EMBL EBI, European Mol Biol Lab, Cambridge CB10 1SD, England. [Harris, Midori A.; Lock, Antonia; Wood, Valerie] Univ Cambridge, Dept Biochem, Cambridge Syst Biol Ctr, Cambridge CB2 1GA, England. [Blake, Judith A.; Hill, David P.] Jackson Lab, Bar Harbor, ME 04609 USA. [Carbon, Seth; Dietze, Heiko; Mungall, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Khodiyar, Varsha K.; Lovering, Ruth C.] UCL, Inst Cardiovasc Sci, Ctr Cardiovasc Genet, London, England. [Van Auken, Kimberly] CALTECH, Div Biol, Pasadena, CA 91125 USA. RP Mungall, CJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. EM cjmungall@lbl.gov RI Huntley, Rachael/R-1036-2016; OI Huntley, Rachael/0000-0001-6718-3559; Khodiyar, Varsha/0000-0002-2743-6918; Wood, Valerie/0000-0001-6330-7526; Foulger, Rebecca/0000-0001-8682-8754; Mutowo, Prudence/0000-0002-4646-4172 FU National Human Genome Research Institute (NHGRI); British Heart Foundation grants [SP/07/007/23671, RG/13/5/30112]; Wellcome Trust grant [WT090548MA]; Kidney Research UK [RP26/2008]; European Molecular Biology Laboratory; NIH [4U41HG006104-04]; US National Human Genome Research Institute [U41-HG002223]; British Medical Research Council [G070119]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; [U41-HG22073] FX We thank Mark McDowall and Kim Rutherford for producing the PomBase annotation display. We also thank Mais Ammari, Rama Balakrishnan, Lionel Breuza, Leonardo Briganti, Fiona Broackes-Carter, Nancy Campbell, Karen Christie, Gayatri Chavali, Carol Chen, Maria Costanzo, Janos Demeter, Paul Denny, Robert Dodson, Harold Drabkin, Margaret Duesbury, Marine Dumousseau, Selina Dwight, Stacia Engel, Petra Fey, Dianna Fisk, Reija Hieta, Ursula Hinz, Marta Iannuccelli, Diane Inglis, Sruthi Jagannathan, Jyoti Khadake, Astrid Lagreid, Luana Licata, Paul Lloyd, Birgit Meldal, Anna Melidoni, Mila Milagros, Robert Nash, Li Ni, Sandra Orchard, Livia Perfetto, Pablo Porras Millan, Arathi Raghunath, Silvie Ricard-Blum, Bernd Roechert, Kim van Roey, Aleksandra Shypitsyna, Dmitry Sitnikov, Marek Skrzypek, Andre Stutz, Michael Tognolli and Edith Wong for additional contributions to the currently available annotation extension data set. The Gene Ontology Consortium is supported by National Human Genome Research Institute (NHGRI) U41 grant HG22073 to PIs JA Blake, JM Cherry, S Lewis, PW Sternberg and P Thomas. This grant supports all authors except those listed hereafter. RC Lovering, VK Khodiyar and T Sawford: British Heart Foundation grants SP/07/007/23671 and RG/13/5/30112. MA Harris, V Wood and A Lock: Wellcome Trust grant WT090548MA. Y Alam-Faruque: Kidney Research UK [RP26/2008] and European Molecular Biology Laboratory core funding. T Sawford and P Mutowo-Muellenet: NIH grant 4U41HG006104-04 to UniProt. K Van Auken: US National Human Genome Research Institute [U41-HG002223] and British Medical Research Council [G070119]. The work performed by H Dietze, S Carbon and CJ Mungall was additionally supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The article processing charge was funded by National Human Genome Research Institute (NHGRI) U41 grant HG22073. NR 22 TC 19 Z9 20 U1 1 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2105 J9 BMC BIOINFORMATICS JI BMC Bioinformatics PD MAY 21 PY 2014 VL 15 AR 155 DI 10.1186/1471-2105-15-155 PG 11 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Mathematical & Computational Biology SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Mathematical & Computational Biology GA AI2KA UT WOS:000336685300002 PM 24885854 ER PT J AU Akimov, AV Long, R Prezhdo, OV AF Akimov, Alexey V. Long, Run Prezhdo, Oleg V. TI Coherence penalty functional: A simple method for adding decoherence in Ehrenfest dynamics SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID NONADIABATIC MOLECULAR-DYNAMICS; QUANTIZED-HAMILTON-DYNAMICS; BORN-OPPENHEIMER TRAJECTORIES; QUANTUM-CLASSICAL DYNAMICS; PROTON-TRANSFER REACTIONS; DEPENDENT SCHRODINGER-EQUATION; ADIABATIC COLLISION PROCESSES; GREEN FLUORESCENT PROTEIN; HYDROGEN-BONDED PHENOLS; DOMAIN AB-INITIO AB We present a new semiclassical approach for description of decoherence in electronically nonadiabatic molecular dynamics. The method is formulated on the grounds of the Ehrenfest dynamics and the Meyer-Miller-Thoss-Stock mapping of the time-dependent Schrodinger equation onto a fully classical Hamiltonian representation. We introduce a coherence penalty functional (CPF) that accounts for decoherence effects by randomizing the wavefunction phase and penalizing development of coherences in regions of strong non-adiabatic coupling. The performance of the method is demonstrated with several model and realistic systems. Compared to other semiclassical methods tested, the CPF method eliminates artificial interference and improves agreement with the fully quantum calculations on the models. When applied to study electron transfer dynamics in the nanoscale systems, the method shows an improved accuracy of the predicted time scales. The simplicity and high computational efficiency of the CPF approach make it a perfect practical candidate for applications in realistic systems. (C) 2014 AIP Publishing LLC. C1 [Akimov, Alexey V.; Prezhdo, Oleg V.] Univ Rochester, Dept Chem, Rochester, NY 14627 USA. [Akimov, Alexey V.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Long, Run] Univ Coll Dublin, Sch Phys, Complex & Adapt Syst Lab, Dublin 4, Ireland. RP Akimov, AV (reprint author), Univ Rochester, Dept Chem, Rochester, NY 14627 USA. EM alexvakimov@gmail.com; oleg.prezhdo@rochester.edu RI Akimov, Alexey/H-9547-2014 FU Computational Materials and Chemical Sciences Network (CMCSN) project at the Brookhaven National Laboratory [DE-AC02-98CH10886]; U.S. Department of Energy; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences; Science Foundation Ireland (SFI) SIRG Program [11/SIRG/E2172]; U.S. Department of Energy [DE-SC0006527] FX A.V.A. was funded by the Computational Materials and Chemical Sciences Network (CMCSN) project at the Brookhaven National Laboratory under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy and supported by its Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences. R. L. thanks the Science Foundation Ireland (SFI) SIRG Program (Grant No. 11/SIRG/E2172). O.V.P. acknowledges financial support of the U.S. Department of Energy, Grant No. DE-SC0006527. NR 134 TC 23 Z9 23 U1 3 U2 29 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2014 VL 140 IS 19 AR 194107 DI 10.1063/1.4875702 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI4JY UT WOS:000336832700009 PM 24852530 ER PT J AU De, AK Monahan, D Dawlaty, JM Fleming, GR AF De, Arijit K. Monahan, Daniele Dawlaty, Jahan M. Fleming, Graham R. TI Two-dimensional fluorescence-detected coherent spectroscopy with absolute phasing by confocal imaging of a dynamic grating and 27-step phase-cycling SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID FOURIER-TRANSFORM SPECTROSCOPY; WAVE-PACKET INTERFEROMETRY; LIGHT-HARVESTING COMPLEXES; QUANTUM COHERENCE; SINGLE MOLECULES; ROOM-TEMPERATURE; FEMTOSECOND SPECTROSCOPY; ELECTRONIC SPECTROSCOPY; OPTICAL SPECTROSCOPY; ENERGY-TRANSFER AB We present a novel experimental scheme for two-dimensional fluorescence-detected coherent spectroscopy (2D-FDCS) using a non-collinear beam geometry with the aid of "confocal imaging" of dynamic (population) grating and 27-step phase-cycling to extract the signal. This arrangement obviates the need for distinct experimental designs for previously developed transmission detected non-collinear two-dimensional coherent spectroscopy (2D-CS) and collinear 2D-FDCS. We also describe a novel method for absolute phasing of the 2D spectrum. We apply this method to record 2D spectra of a fluorescent dye in solution at room temperature and observe "spectral diffusion." (C) 2014 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [De, Arijit K.; Fleming, Graham R.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94702 USA. [De, Arijit K.; Monahan, Daniele; Dawlaty, Jahan M.; Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94702 USA. RP De, AK (reprint author), Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94702 USA. EM akde@lbl.gov; grfleming@lbl.gov FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC03-76SF000098]; DARPA [N66001-09-1-2026]; National Science Foundation FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC03-76SF000098, and by DARPA under Grant No. N66001-09-1-2026. D. M. was supported by National Science Foundation's Graduate Research Fellowship Program. We thank Lukas Whaley-Mayda for his help. NR 63 TC 5 Z9 5 U1 1 U2 46 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2014 VL 140 IS 19 AR 194201 DI 10.1063/1.4874697 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI4JY UT WOS:000336832700010 PM 24852531 ER PT J AU Dholabhai, PP Aguiar, JA Misra, A Uberuaga, BP AF Dholabhai, Pratik P. Aguiar, Jeffery A. Misra, Amit Uberuaga, Blas P. TI Defect interactions with stepped CeO2/SrTiO3 interfaces: Implications for radiation damage evolution and fast ion conduction SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID OXYGEN VACANCY FORMATION; SRTIO3 SINGLE-CRYSTALS; AB-INITIO; MOLECULAR-DYNAMICS; GRAIN-BOUNDARIES; POINT-DEFECTS; CEO2; DIFFUSION; IRRADIATION; TOLERANCE AB Due to reduced dimensions and increased interfacial content, nanocomposite oxides offer improved functionalities in a wide variety of advanced technological applications, including their potential use as radiation tolerant materials. To better understand the role of interface structures in influencing the radiation damage tolerance of oxides, we have conducted atomistic calculations to elucidate the behavior of radiation-induced point defects (vacancies and interstitials) at interface steps in a model CeO2/SrTiO3 system. We find that atomic-scale steps at the interface have substantial influence on the defect behavior, which ultimately dictate the material performance in hostile irradiation environments. Distinctive steps react dissimilarly to cation and anion defects, effectively becoming biased sinks for different types of defects. Steps also attract cation interstitials, leaving behind an excess of immobile vacancies. Further, defects introduce significant structural and chemical distortions primarily at the steps. These two factors are plausible origins for the enhanced amorphization at steps seen in our recent experiments. The present work indicates that comprehensive examination of the interaction of radiation-induced point defects with the atomic-scale topology and defect structure of heterointerfaces is essential to evaluate the radiation tolerance of nanocomposites. Finally, our results have implications for other applications, such as fast ion conduction. (C) 2014 AIP Publishing LLC. C1 [Dholabhai, Pratik P.; Aguiar, Jeffery A.; Uberuaga, Blas P.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Misra, Amit] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Dholabhai, PP (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. EM pdholabhai@lanl.gov; blas@lanl.gov RI Dholabhai, Pratik/A-2366-2015; Misra, Amit/H-1087-2012; OI Aguiar, Jeffery/0000-0001-6101-4762 FU Center for Materials at Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396] FX This work was supported by Center for Materials at Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under the Award No. 2008LANL1026. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under Contract No. DE-AC52-06NA25396. NR 91 TC 6 Z9 6 U1 1 U2 32 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2014 VL 140 IS 19 AR 194701 DI 10.1063/1.4876225 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI4JY UT WOS:000336832700030 PM 24852551 ER PT J AU Evans, JW Liu, DJ AF Evans, James W. Liu, Da-Jiang TI Statistical mechanical models for dissociative adsorption of O-2 on metal(100) surfaces with blocking, steering, and funneling SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RANDOM SEQUENTIAL ADSORPTION; STICKING PROBABILITIES; CO OXIDATION; LATTICE-GAS; SQUARE LATTICE; FILM GROWTH; OXYGEN; PD(100); CHEMISORPTION; KINETICS AB We develop statistical mechanical models amenable to analytic treatment for the dissociative adsorption of O-2 at hollow sites on fcc(100) metal surfaces. The models incorporate exclusion of nearest-neighbor pairs of adsorbed O. However, corresponding simple site-blocking models, where adsorption requires a large ensemble of available sites, exhibit an anomalously fast initial decrease in sticking. Thus, in addition to blocking, our models also incorporate more facile adsorption via orientational steering and funneling dynamics (features supported by ab initio Molecular Dynamics studies). Behavior for equilibrated adlayers is distinct from those with finite adspecies mobility. We focus on the low-temperature limited-mobility regime where analysis of the associated master equations readily produces exact results for both short-and long-time behavior. Kinetic Monte Carlo simulation is also utilized to provide a more complete picture of behavior. These models capture both the initial decrease and the saturation of the experimentally observed sticking versus coverage, as well as features of non-equilibrium adlayer ordering as assessed by surface-sensitive diffraction. (C) 2014 AIP Publishing LLC. C1 [Evans, James W.; Liu, Da-Jiang] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Evans, James W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Evans, JW (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. FU U.S. Department of Energy (USDOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics program; USDOE [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (USDOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics program. We acknowledge use of NERSC computational resources. The work was performed at Ames Laboratory which is operated for the USDOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 48 TC 6 Z9 6 U1 2 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2014 VL 140 IS 19 AR 194704 DI 10.1063/1.4875813 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI4JY UT WOS:000336832700033 PM 24852554 ER PT J AU Randazzo, JB Croteau, P Kostko, O Ahmed, M Boering, KA AF Randazzo, John B. Croteau, Philip Kostko, Oleg Ahmed, Musahid Boering, Kristie A. TI Isotope effects and spectroscopic assignments in the non-dissociative photoionization spectrum of N-2 SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RESOLUTION ABSORPTION-SPECTRUM; DOUBLE-RESONANCE SPECTROSCOPY; MOLECULAR NITROGEN; CROSS-SECTIONS; SYNCHROTRON-RADIATION; IONIZATION THRESHOLD; EXTREME-ULTRAVIOLET; TITANS ATMOSPHERE; NEAR-THRESHOLD; RYDBERG STATES AB Photoionization efficiency spectra of N-14(2), (NN)-N-15-N-14, and N-15(2) from 15.5 to 18.9 eV were measured using synchrotron radiation at the Advanced Light Source at Lawrence Berkeley National Laboratory with a resolution of 6 meV, and significant changes in peak energies and intensities upon isotopic substitution were observed. Previously, we reported the isotope shifts and their applications to Titan's atmosphere. Here, we report more extensive experimental details and tabulate the isotope shifts of many transitions in the N-2 spectrum, including those for (NN)-N-15-N-14, which have not been previously reported. The isotope shifts are used to address several long-standing ambiguities in spectral peak assignments just above the ionization threshold of N-2. The feature at 15.677 eV (the so-called second "cathedral" peak) is of particular interest in this respect. The measured isotope shifts for this peak relative to N-14(2) are 0.015 +/- 0.001 eV for N-15(2) and 0.008 +/- 0.001 eV for (NN)-N-15-N-14, which match most closely with the isotope shifts predicted for transitions to the (A (2)Pi(u) v' = 2) 4s sigma g (1)Pi(u) state using Herzberg equations for the isotopic differences in harmonic oscillator energy levels plus the first anharmonic correction of 0.0143 eV for N-15(2) and 0.0071 eV for (NN)-N-15-N-14. More generally, the isotope shifts measured for both N-15(2) and (NN)-N-15-N-14 relative to N-14(2) provide new benchmarks for theoretical calculations of interferences between direct and indirect autoionization states which can interact to produce intricate resonant structures in molecular photoionization spectra in regions near ionization thresholds. (C) 2014 AIP Publishing LLC. C1 [Randazzo, John B.; Croteau, Philip; Boering, Kristie A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Kostko, Oleg; Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Boering, Kristie A.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. RP Randazzo, JB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RI Ahmed, Musahid/A-8733-2009; Kostko, Oleg/B-3822-2009 OI Kostko, Oleg/0000-0003-2068-4991 FU NASA Planetary Atmospheres [NNX08AE69G]; Dreyfus Teacher-Scholar Award; Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge support from NASA Planetary Atmospheres grant NNX08AE69G to UC Berkeley, the Dreyfus Teacher-Scholar Award for K. A. B. and from the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 for O.K., M. A., and the A.L.S. NR 69 TC 3 Z9 3 U1 2 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2014 VL 140 IS 19 AR 194303 DI 10.1063/1.4873717 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI4JY UT WOS:000336832700013 PM 24852534 ER PT J AU Salerno, KM Ismail, AE Lane, JMD Grest, GS AF Salerno, K. Michael Ismail, Ahmed E. Lane, J. Matthew D. Grest, Gary S. TI Coating thickness and coverage effects on the forces between silica nanoparticles in water SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; POLYMER-GRAFTED NANOPARTICLES; SELF-ASSEMBLED MONOLAYERS; 2ND VIRIAL-COEFFICIENT; POLY(ETHYLENE OXIDE); GOLD NANOPARTICLES; QUANTUM-CHEMISTRY; AQUEOUS-SOLUTION; SURFACE; LIQUID AB The structure and interactions of coated silica nanoparticles have been studied in water using molecular dynamics simulations. For 5 nm diameter amorphous silica nanoparticles, we studied the effects of varying the chain length and grafting density of polyethylene oxide on the nanoparticle coating's shape and on nanoparticle-nanoparticle effective forces. For short ligands of length n = 6 and n = 20 repeat units, the coatings are radially symmetric while for longer chains (n = 100) the coatings are highly anisotropic. This anisotropy appears to be governed primarily by chain length, with coverage playing a secondary role. For the largest chain lengths considered, the strongly anisotropic shape makes fitting to a simple radial force model impossible. For shorter ligands, where the coatings are isotropic, we found that the force between pairs of nanoparticles is purely repulsive and can be fit to the form (R/2r(core) -1)(-b) where R is the separation between the center of the nanoparticles, r(core) is the radius of the silica core, and b is measured to be between 2.3 and 4.1. (C) 2014 AIP Publishing LLC. C1 [Salerno, K. Michael; Lane, J. Matthew D.; Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Ismail, Ahmed E.] Rhein Westfal TH Aachen, Aachener Verfahrenstech Mol Simulat & Transformat, Fac Mech Engn, D-52056 Aachen, Germany. RP Salerno, KM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU Cluster of Excellence "Tailor-Made Fuels from Biomass"; Excellence Initiative by the German federal and state governments to promote science and research at German universities; (U.S.) Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX A.E.I. was supported by the Cluster of Excellence "Tailor-Made Fuels from Biomass," which is funded by the Excellence Initiative by the German federal and state governments to promote science and research at German universities. This work was performed, in part, at the Center for Integrated Nanotechnology, a (U.S.) Department of Energy (DOE) and Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the (U.S.) Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 59 TC 6 Z9 6 U1 5 U2 49 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2014 VL 140 IS 19 AR 194904 DI 10.1063/1.4874638 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI4JY UT WOS:000336832700039 PM 24852560 ER PT J AU Treske, U Khoshkhoo, MS Roth, F Knupfer, M Bauer, ED Sarrao, JL Buchner, B Koitzsch, A AF Treske, U. Khoshkhoo, M. S. Roth, F. Knupfer, M. Bauer, E. D. Sarrao, J. L. Buechner, B. Koitzsch, A. TI X-ray photoemission study of CeTIn5 (T = Co, Rh, Ir) SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE x-ray photoemission spectroscopy; heavy fermion superconductors; Anderson impurity model; strongly correlated electrons ID ELECTRONIC-STRUCTURE; CE COMPOUNDS; XPS; SUPERCONDUCTIVITY; SURFACE; MODEL AB We investigated CeTIn5 (T = Co, Rh, Ir) using temperature- and angle-dependent x-ray photoemission spectroscopy. The Ce 3d core level has a very similar shape for all three materials and is indicative of weak f-hybridization. The spectra were analyzed using a simplified version of the Anderson impurity model, which yields a Ce 4f occupancy that is larger than 0.9. The temperature dependence shows a continuous, irreversible and exclusive broadening of the Ce 3d peaks, due to oxidation of Ce at the surface. C1 [Treske, U.; Khoshkhoo, M. S.; Roth, F.; Knupfer, M.; Buechner, B.; Koitzsch, A.] IFW Dresden, Inst Solid State Res, DE-01171 Dresden, Germany. [Roth, F.] Ctr Free Electron Laser Sci DESY, D-22607 Hamburg, Germany. [Bauer, E. D.; Sarrao, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Buechner, B.] Tech Univ Dresden, Inst Festkorperphys, D-01062 Dresden, Germany. RP Treske, U (reprint author), IFW Dresden, Inst Solid State Res, POB 270116, DE-01171 Dresden, Germany. EM a.koitzsch@ifw-dresden.de RI Roth, Friedrich/J-3084-2015; Samadi Khoshkhoo, Mahdi/M-7940-2015; Buchner, Bernd/E-2437-2016; OI Samadi Khoshkhoo, Mahdi/0000-0003-0393-4768; Buchner, Bernd/0000-0002-3886-2680; Bauer, Eric/0000-0003-0017-1937 FU DFG [KO 3831/1-1]; US Department of Energy, Office of Science, Division of Materials Science and Engineering FX We thank R Hubel, R Schonfelder and S Leger for technical assistance and the DFG for financial support (grant no. KO 3831/1-1). Work at Los Alamos was performed under the auspices of the US Department of Energy, Office of Science, Division of Materials Science and Engineering. NR 28 TC 3 Z9 3 U1 3 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 21 PY 2014 VL 26 IS 20 AR 205601 DI 10.1088/0953-8984/26/20/205601 PG 5 WC Physics, Condensed Matter SC Physics GA AH6ML UT WOS:000336244900008 PM 24786193 ER PT J AU Manthiram, K Surendranath, Y Alivisatos, AP AF Manthiram, Karthish Surendranath, Yogesh Alivisatos, A. Paul TI Dendritic Assembly of Gold Nanoparticles during Fuel-Forming Electrocatalysis SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID DIFFUSION-LIMITED AGGREGATION; ELECTROCHEMICAL DESORPTION; AU NANOPARTICLES; METAL-ELECTRODES; CO2 REDUCTION; CLUSTERS; SURFACE; OXIDE AB We observe the dendritic assembly of alkanethiol-capped gold nanoparticles on a glassy carbon support during electrochemical reduction of protons and CO2. We find that the primary mechanism by which surfactant-ligated gold nanoparticles lose surface area is by taking a random walk along the support, colliding with their neighbors, and fusing to form dendrites, a type of fractal aggregate. A random walk model reproduces the fractal dimensionality of the dendrites observed experimentally. The rate at which the dendrites form is strongly dependent on the solubility of the surfactant in the electrochemical double layer under the conditions of electrolysis. Since alkanethiolate surfactants reductively desorb at potentials close to the onset of CO2 reduction, they do not poison the catalytic activity of the gold nanoparticles. Although catalyst mobility is typically thought to be limited for room-temperature electrochemistry, our results demonstrate that nanoparticle mobility is significant under conditions at which they electrochemically catalyze gas evolution, even in the presence of a high surface area carbon and binder. A careful understanding of the electrolyte- and polarization-dependent nanoparticle aggregation kinetics informs strategies for maintaining catalyst dispersion during fuel-forming electrocatalysis. C1 [Manthiram, Karthish] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Surendranath, Yogesh; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Manthiram, Karthish; Surendranath, Yogesh; Alivisatos, A. Paul] Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. [Surendranath, Yogesh] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Manthiram, Karthish; Surendranath, Yogesh; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM alivis@berkeley.edu RI Foundry, Molecular/G-9968-2014; Alivisatos , Paul /N-8863-2015 OI Alivisatos , Paul /0000-0001-6895-9048 FU Dow Chemical Co. [20120984]; Office of Science, Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; U.S. DOE Office of Science Graduate Fellowship; Miller Institute for Basic Research in Science; U.S. DOE [DE-AC02-05CH11231] FX We thank David Grauer for conducting XPS measurements and Virginia Altoe, David Barton, Brandon Beberwyck, Trevor Ewers, Eric Granlund, Kendra Kuhl, Li-Chiang Lin, Matt Lucas, Pete Nickias, Fadekemi Oba, and Rachel Segalman for useful discussions and experimental assistance. This work was supported by the Dow Chemical Co. under contract 20120984. SEM was conducted at the Molecular Foundry, supported by the Office of Science, Basic Energy Sciences, of the U.S. Department of Energy (DOE) under contract DE-AC02-05CH11231. K.M. acknowledges the support of the U.S. DOE Office of Science Graduate Fellowship. Y.S. acknowledges the Miller Institute for Basic Research in Science for a postdoctoral fellowship. A.PA was supported by the U.S. DOE under contract DE-AC02-05CH11231. NR 24 TC 18 Z9 19 U1 11 U2 130 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 21 PY 2014 VL 136 IS 20 BP 7237 EP 7240 DI 10.1021/ja502628r PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AH8VP UT WOS:000336416600013 PM 24766431 ER PT J AU Schrauben, JN Ryerson, JL Michl, J Johnson, JC AF Schrauben, Joel N. Ryerson, Joseph L. Michl, Josef Johnson, Justin C. TI Mechanism of Singlet Fission in Thin Films of 1,3-Diphenylisobenzofuran SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID EXCIMER-FORMING CRYSTAL; EXCITON FISSION; TETRACENE; PENTACENE; DYNAMICS; PHOTOPHYSICS; YIELD; SPECTROSCOPY; ANTHRACENE; DIFFUSION AB In order to elucidate the mechanism of singlet fission in thin films of 1,3-diphenylisobenzofuran (1) we have performed ultrafast transient absorption spectroscopy as a function of sample temperature and excitation fluence on polycrystalline thin films composed of two polymorphs. Our earlier investigations revealed that films enriched in a particular polymorph of 1 displayed near 200% efficiency for triplet formation at 77 K, while films composed primarily of a second polymorph had a very low triplet quantum yield. Present data confirm the triplet yield disparities in the two polymorphs and demonstrate the distinct fates of the initially prepared singlets in films of different structure. Singlet fission is inhibited in the more stable polymorph due to rapid excimer formation and trapping. The less stable polymorph undergoes highly efficient singlet fission with a dominant time constant of 10-30 ps and without strong thermal activation. Transient absorption measurements with varying excitation fluence indicate that singlet-singlet annihilation is a primary competitor of singlet fission at higher fluence and that fission from higher-lying states can also contribute to the triplet formation process. Measurements employing different excitation energies and sample temperatures reveal the role that trapping processes play in attenuating the triplet quantum yield to produce the complex temperature dependence of the singlet fission yield. The rate constants for singlet fission itself are essentially temperature independent. C1 [Schrauben, Joel N.; Ryerson, Joseph L.; Johnson, Justin C.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ryerson, Joseph L.; Michl, Josef] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80301 USA. [Michl, Josef] Acad Sci Czech Republic, Inst Organ Chem & Biochem, CR-16610 Prague 6, Czech Republic. RP Johnson, JC (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Justin.Johnson@nrel.gov RI Michl, Josef/G-9376-2014 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences; NREL [DE-AC36-08GO28308]; [DOE DE-SC0007004] FX This work has been supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences. J.N.S., J.R., and J.C.J acknowledge contract no. DE-AC36-08GO28308 with NREL, and J.M. acknowledges Award Number DOE DE-SC0007004. NR 40 TC 30 Z9 30 U1 6 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 21 PY 2014 VL 136 IS 20 BP 7363 EP 7373 DI 10.1021/ja501337b PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA AH8VP UT WOS:000336416600031 PM 24735403 ER PT J AU Kumara, C Zuo, XB Ilavsky, J Chapman, KW Cullen, DA Dass, A AF Kumara, Chanaka Zuo, Xiaobing Ilavsky, Jan Chapman, Karena W. Cullen, David A. Dass, Amala TI Super-Stable, Highly Monodisperse Plasmonic Faradaurate-500 Nanocrystals with 500 Gold Atoms: Au-similar to 500(SR)(similar to 120) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PAIR DISTRIBUTION FUNCTION; THEORETICAL-ANALYSIS; ALLOY NANOMOLECULES; CLUSTER COMPOUNDS; CRYSTAL-STRUCTURE; SOLAR-CELLS; NANOPARTICLES; NANOCLUSTERS; RESOLUTION; AU-38 AB Determining the composition of plasmonic nanoparticles is challenging due to a lack of tools to accurately quantify the number of atoms within the particle. Mass spectrometry plays a significant role in determining the nanoparticle composition at the atomic level. Significant progress has been made in understanding ultrasmall gold nanoparticles such as Au-25(SR)(18) and Au-38(SR)(24), which have Au core diameters of 0.97 and 1.3 nm, respectively. However, progress in 2-5 nm-diameter small plasmonic nanoparticles is currently impeded, partially because of the challenges in synthesizing monodisperse nanoparticles. Here, we report a plasmonic nanocrystal that is highly monodisperse, with unprecedentedly small size variability. The composition of the superstable plasmonic nanocrystals at 115 kDa was determined as Au500 +/- 10SR120 +/- 3. The Au-similar to 500 system, named Faradaurate-500, is the largest system to be characterized using high resolution electrospray (ESI) mass spectrometry. Atomic pair distribution function (PDF) data indicate that the local atomic structure is consistent with a face-centered cubic (fcc) or Marks decahedral arrangement. High resolution scanning transmission electron microscopy (STEM) images show that the diameter is 2.4 +/- 0.1 nm. The size and the shape of the molecular envelope measured by small-angle X-ray scattering (SAXS) confirms the STEM and PDF analysis. C1 [Kumara, Chanaka; Dass, Amala] Univ Mississippi, Dept Chem & Biochem, University, MS 38677 USA. [Zuo, Xiaobing; Ilavsky, Jan; Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Cullen, David A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Dass, A (reprint author), Univ Mississippi, Dept Chem & Biochem, University, MS 38677 USA. EM amal@olemiss.edu RI Cullen, David/A-2918-2015; Ilavsky, Jan/D-4521-2013 OI Cullen, David/0000-0002-2593-7866; Ilavsky, Jan/0000-0003-1982-8900 FU U.S. DOE [DE-AC02-06CH11357]; ORNL's Center for Nanophase Materials Sciences (CNMS); Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; [NSF-CHE-1255519] FX A.D. and C.K. were funded through NSF-CHE-1255519. Work performed at Argonne and use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Electron microscopy was supported through a user project at ORNL's Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. We thank Riccardo Ferrando for assistance with theoretical models and Miguel Yacaman, Robert Whetten, and Daniel Bahenas for preliminary STEM results. We thank Pavol Juhas for help with python script used in calculating atomic PDF. NR 39 TC 22 Z9 22 U1 2 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 21 PY 2014 VL 136 IS 20 BP 7410 EP 7417 DI 10.1021/ja502327a PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA AH8VP UT WOS:000336416600036 PM 24814044 ER PT J AU Gao, CB Hu, YX Wang, MS Chi, MF Yin, YD AF Gao, Chuanbo Hu, Yongxing Wang, Mingsheng Chi, Miaofang Yin, Yadong TI Fully Alloyed Ag/Au Nanospheres: Combining the Plasmonic Property of Ag with the Stability of Au SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID GOLD-SILVER NANOPARTICLES; SEEDED GROWTH; METAL NANOSTRUCTURES; SIZE; SPECTROSCOPY; NANORODS; LAYER; ABSORPTION; NANOPRISMS; DEPOSITION AB We report that fully alloyed Ag/Au nanospheres with high compositional homogeneity ensured by annealing at elevated temperatures show large extinction cross sections, extremely narrow bandwidths, and remarkable stability in harsh chemical environments. Nanostructures of Ag are known to have much stronger surface plasmon resonance than Au, but their applications in many areas have been very limited by their poor chemical stability against nonideal chemical environments. Here we address this issue by producing fully alloyed Ag/Au nanospheres through a surface-protected annealing process. A critical temperature has been found to be around 930 degrees C, below which the resulting alloy nanospheres, although significantly more stable than pure silver nanoparticles, can still gradually decay upon extended exposure to a harsh etchant. Nanospheres annealed above the critical temperature show a homogeneous distribution of Ag and Au, minimal crystallographic defects, and the absence of structural and compositional interfaces, which account for the extremely narrow bandwidths of the surface plasmon resonance and may enable many plasmonic applications with high performance and long lifetime, especially for those involving corrosive species. C1 [Gao, Chuanbo] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Ctr Mat Chem, Xian 710054, Shaanxi, Peoples R China. [Gao, Chuanbo; Wang, Mingsheng; Yin, Yadong] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. [Hu, Yongxing] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Chi, Miaofang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Gao, CB (reprint author), Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Ctr Mat Chem, Xian 710054, Shaanxi, Peoples R China. EM gaochuanbo@mail.xjtu.edu.cn; yadong.yin@ucr.edu RI Wang, Mingsheng/J-9252-2013; Gao, Chuanbo/D-6121-2011; Yin, Yadong/D-5987-2011; Chi, Miaofang/Q-2489-2015 OI Wang, Mingsheng/0000-0003-1049-8917; Gao, Chuanbo/0000-0003-3429-3473; Yin, Yadong/0000-0003-0218-3042; Chi, Miaofang/0000-0003-0764-1567 FU National Science Foundation [CHE-1308587]; Xi'an Jiaotong University; ORNL's Center for Nanophase Materials Sciences (CNMS); Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Y.Y. acknowledges support from the National Science Foundation (CHE-1308587). This work was also supported partly by the startup fund for C.G. and the operational fund for the Center for Materials Chemistry from Xi'an Jiaotong University. The electron microscopy studies were conducted through a user project supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors also thank X. Zhong and Prof. Z. Li at the Institute of Physics, CAS, for helpful discussions. NR 41 TC 67 Z9 67 U1 12 U2 201 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 21 PY 2014 VL 136 IS 20 BP 7474 EP 7479 DI 10.1021/ja502890c PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AH8VP UT WOS:000336416600043 PM 24821567 ER PT J AU Zhou, K Xu, N Xu, Z Zhuang, PF AF Zhou, Kai Xu, Nu Xu, Zhe Zhuang, Pengfei TI Medium effects on charmonium production at ultrarelativistic energies available at the CERN Large Hadron Collider SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; PB-PB COLLISIONS; NUCLEAR COLLISIONS; J/PSI SUPPRESSION; TRANSVERSE-MOMENTUM; PP COLLISIONS; ROOT-S=7 TEV; RAPIDITY; GENERATION; DEPENDENCE AB We investigate with a transport approach the cold and hot nuclear matter effects on the charmonium transverse momentum distributions in relativistic heavy ion collisions. The newly defined nuclear modification factor r(AA) = < p(T)(2)>(AA)/< p(T)(2)>(pp) and elliptic flow v(2) for J/psi are sensitive to the nature of the hot medium and the thermalization of heavy quarks. From Super Proton Synchrotron (SPS) through Relativistic Heavy Ion Collider (RHIC) to Large Hadron Collider (LHC) colliding energies, we observe dramatic changes in the centrality dependence of r(AA). We find that, at LHC energy, the finally observed charmonia are dominated by the regeneration from thermalized heavy quarks. C1 [Zhou, Kai; Xu, Zhe; Zhuang, Pengfei] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Zhou, Kai; Xu, Zhe; Zhuang, Pengfei] Collaborat Innovat Ctr Quantum Matter, Beijing 100084, Peoples R China. [Xu, Nu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Xu, Nu] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Xu, Nu] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. RP Zhou, K (reprint author), Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. FU NSFC; MOST; DOE [11221504, 11335005, 11275103, 2013CB922000, 2014CB845400, DE-AC03-76SF00098] FX The work is supported by the NSFC, the MOST and DOE Grants No. 11221504, No. 11335005, No. 11275103, No. 2013CB922000, No. 2014CB845400, and No. DE-AC03-76SF00098. NR 78 TC 32 Z9 32 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 21 PY 2014 VL 89 IS 5 AR 054911 DI 10.1103/PhysRevC.89.054911 PG 11 WC Physics, Nuclear SC Physics GA AH6NX UT WOS:000336248700004 ER PT J AU Dodin, IY Fisch, NJ AF Dodin, I. Y. Fisch, N. J. TI Ponderomotive Forces on Waves in Modulated Media SO PHYSICAL REVIEW LETTERS LA English DT Article ID LINEAR-MODE CONVERSION; CHARGED-PARTICLES; ELECTROMAGNETIC-WAVES; NEUTRAL PARTICLES; MAXWELL DEMON; LASER-BEAMS; ATOM DIODE; BARRIER; FIELD; MANIPULATION AB Nonlinear interactions of waves via instantaneous cross-phase modulation can be cast in the same way as ponderomotive wave-particle interactions in high-frequency fields. The ponderomotive effect arises when rays of a probe wave scatter off perturbations of the underlying medium produced by a second, modulation wave, much like charged particles scatter off an oscillating electromagnetic field. Parallels with the point-particle dynamics, which itself is subsumed under this theory, lead to new methods of wave manipulation, including asymmetric barriers for light. C1 [Dodin, I. Y.; Fisch, N. J.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Dodin, IY (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. FU NNSA [DE274-FG52-08NA28553]; DOE [DE-AC02-09CH11466]; DTRA [HDTRA1-11-1-0037] FX The work was supported by NNSA Grant No. DE274-FG52-08NA28553, DOE Contract No. DE-AC02-09CH11466, and DTRA Grant No. HDTRA1-11-1-0037. NR 70 TC 5 Z9 5 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 21 PY 2014 VL 112 IS 20 AR 205002 DI 10.1103/PhysRevLett.112.205002 PG 5 WC Physics, Multidisciplinary SC Physics GA AH6OK UT WOS:000336250100008 ER PT J AU Edwards, MJ Baiden, NA Johs, A Tomanicek, SJ Liang, LY Shi, L Fredrickson, JK Zachara, JM Gates, AJ Butt, JN Richardson, DJ Clarke, TA AF Edwards, Marcus J. Baiden, Nanakow A. Johs, Alexander Tomanicek, Stephen J. Liang, Liyuan Shi, Liang Fredrickson, Jim K. Zachara, John M. Gates, Andrew J. Butt, Julea N. Richardson, David J. Clarke, Thomas A. TI The X-ray crystal structure of Shewanella oneidensis OmcA reveals new insight at the microbe-mineral interface SO FEBS LETTERS LA English DT Article DE Multiheme cytochrome; Mineral respiration; Electron transfer; Shewanella; c-Type heme; Outer membrane; Metalloprotein ID MEMBRANE CYTOCHROMES MTRC; C-TYPE CYTOCHROMES; ELECTRON-TRANSFER; IRON REDUCTION; MR-1; BINDING; SYSTEM; SCATTERING; HEMATITE; SURFACE AB The X-ray crystal structure of Shewanella oneidensis OmcA, an extracellular decaheme cytochrome involved in mineral reduction, was solved to a resolution of 2.7 angstrom. The four OmcA molecules in the asymmetric unit are arranged so the minimum distance between heme 5 on adjacent OmcA monomers is 9 angstrom, indicative of a transient OmcA dimer capable of intermolecular electron transfer. A previously identified hematite binding motif was identified near heme 10, forming a hydroxylated surface that would bring a heme 10 electron egress site to similar to 10 degrees of a mineral surface. Structured summary of protein interactions: OmcA and OmcA bind by X-ray crystallography (View interaction) (C) 2014 Federation of European Biochemical Societies. Published by Elsevier B. V. All rights reserved. C1 [Edwards, Marcus J.; Baiden, Nanakow A.; Gates, Andrew J.; Butt, Julea N.; Richardson, David J.; Clarke, Thomas A.] Univ E Anglia, Sch Biol Sci, Ctr Mol & Struct Biochem, Norwich NR4 7TJ, Norfolk, England. [Johs, Alexander; Tomanicek, Stephen J.; Liang, Liyuan] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Shi, Liang; Fredrickson, Jim K.; Zachara, John M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Richardson, DJ (reprint author), Univ E Anglia, Sch Biol Sci, Ctr Mol & Struct Biochem, Norwich NR4 7TJ, Norfolk, England. EM d.richardson@uea.ac.uk; tom.clarke@uea.ac.uk RI Gates, Andrew/F-8218-2011; Liang, Liyuan/O-7213-2014; clarke, tom/D-1837-2009; Butt, Julea/E-2133-2011 OI Gates, Andrew/0000-0002-4594-5038; Liang, Liyuan/0000-0003-1338-0324; clarke, tom/0000-0002-6234-1914; Butt, Julea/0000-0002-9624-5226 FU Biotechnology and Biological Sciences Research Council [BB/K00929X/1, BB/H007288/1]; Subsurface Biogeochemical Research program (SBR)/Office of Biological and Environmental Research (BER); U.S. Department of Energy (DOE) FX DJR is a Royal Society Wolfson Foundation Merit Award holder. This research was supported by the Biotechnology and Biological Sciences Research Council (BB/K00929X/1 and BB/H007288/1) and sponsored by the Subsurface Biogeochemical Research program (SBR)/Office of Biological and Environmental Research (BER), U.S. Department of Energy (DOE), and is a contribution of the Pacific Northwest National Laboratory (PNNL) Scientific Focus Area and the Mercury Scientific Focus Area at Oak Ridge National Laboratory (ORNL). The PNNL and ORNL are operated for the DOE by Battelle under contracts DE-AC05-76RLO1830 and DE-AC05-00OR22725 NR 33 TC 24 Z9 24 U1 6 U2 77 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0014-5793 EI 1873-3468 J9 FEBS LETT JI FEBS Lett. PD MAY 21 PY 2014 VL 588 IS 10 BP 1886 EP 1890 DI 10.1016/j.febslet.2014.04.013 PG 5 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA AH3OL UT WOS:000336033700005 PM 24747425 ER PT J AU Nguyen, JH Akin, MC Chau, R Fratanduono, DE Ambrose, WP Fat'yanov, OV Asimow, PD Holmes, NC AF Nguyen, Jeffrey H. Akin, Minta C. Chau, Ricky Fratanduono, Dayne E. Ambrose, W. Patrick Fat'yanov, Oleg V. Asimow, Paul D. Holmes, Neil C. TI Molybdenum sound velocity and shear modulus softening under shock compression SO PHYSICAL REVIEW B LA English DT Article ID PHASE-TRANSITIONS; CORE CONDITIONS; HIGH-PRESSURES; TANTALUM; IRON; MO; ALUMINUM; EQUATION; COPPER; STATE AB We measured the longitudinal sound velocity in Mo shock compressed up to 4.4 Mbars on the Hugoniot. Its sound speed increases linearly with pressure up to 2.6 Mbars; the slope then decreases up to the melting pressure of similar to 3.8 Mbars. This suggests a decrease of shear modulus before the melt. A linear extrapolation of our data to 1 bar agrees with the ambient sound speed. The results suggest that Mo remains in the bcc phase on the Hugoniot up to the melting pressure. There is no statistically significant evidence for a previously reported bcc -> hcp phase transition on the Hugoniot. C1 [Nguyen, Jeffrey H.; Akin, Minta C.; Chau, Ricky; Fratanduono, Dayne E.; Ambrose, W. Patrick; Holmes, Neil C.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Fat'yanov, Oleg V.; Asimow, Paul D.] CALTECH, Pasadena, CA 91125 USA. RP Nguyen, JH (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM nguyen29@llnl.gov FU U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344] FX We thank R. Hixson and M. Ross for their useful discussions, and Papo Gelle, Mike Long, Russ Oliver, Bob Nafzinger, Paul Benevento, Sam Weaver, and Cory McLean for their dedicated effort. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344. NR 36 TC 16 Z9 18 U1 2 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 21 PY 2014 VL 89 IS 17 AR 174109 DI 10.1103/PhysRevB.89.174109 PG 6 WC Physics, Condensed Matter SC Physics GA AH6NL UT WOS:000336247500001 ER PT J AU Buras, AJ Gerard, JM Bardeen, WA AF Buras, Andrzej J. Gerard, Jean-Marc Bardeen, William A. TI Large N approach to Kaon decays and mixing 28 years later: Delta I=1/2 rule, (B)over-cap(K), and Delta M-K SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CHIRAL PERTURBATION-THEORY; HADRONIC MATRIX-ELEMENTS; NONLEPTONIC DECAYS; LEADING LOGARITHMS; MASS DIFFERENCE; STANDARD MODEL; GAUGE-THEORIES; 1/N EXPANSION; QUANTUM CHROMODYNAMICS; PENGUIN CONTRIBUTION AB We review and update our results for K -> pi pi decays and K-0-(K) over bar (0) mixing obtained by us in the 1980s within an analytic approximate approach based on the dual representation of QCD as a theory of weakly interacting mesons for large N, where N is the number of colors. In our analytic approach the Standard Model dynamics behind the enhancement of ReA(0) and suppression of ReA(2), the so-called Delta I = 1/2 rule for K -> pi pi decays, has a simple structure: the usual octet enhancement through the long but slow quark-gluon renormalization group evolution down to the scales O(1 GeV) is continued as a short but fast meson evolution down to zeromomentum scales at which the factorization of hadronic matrix elements is at work. The inclusion of lowest-lying vector meson contributions in addition to the pseudoscalar ones and of Wilson coefficients in a momentum scheme improves significantly the matching between quark-gluon and meson evolutions. In particular, the anomalous dimension matrix governing the meson evolution exhibits the structure of the known anomalous dimension matrix in the quark-gluon evolution. While this physical picture did not yet emerge from lattice simulations, the recent results on ReA(2) and ReA(0) from the RBC-UKQCD collaboration give support for its correctness. In particular, the signs of the two main contractions found numerically by these authors follow uniquely from our analytic approach. Though the current-current operators dominate the Delta I = 1/2 rule, working with matching scales O(1 GeV) we find that the presence of QCD-penguin operator Q(6) is required to obtain satisfactory result for ReA(0). At NLO in 1/N we obtain R = ReA(0)/ReA(2) = 16.0 +/- 1.5 which amounts to an order of magnitude enhancement over the strict large N limit value root 2. We also update our results for the parameter (B) over cap (K), finding (B) over cap (K) = 0.73 +/- 0.02. The smallness of 1/N corrections to the large N value (B) over cap (K) = 3/4 results within our approach from an approximate cancelation between pseudoscalar and vector meson one-loop contributions. We also summarize the status of Delta MK in this approach. C1 [Buras, Andrzej J.] TUM Inst Adv Study, D-85747 Garching, Germany. [Buras, Andrzej J.] Tech Univ Munich, Dept Phys, D-85747 Garching, Germany. [Gerard, Jean-Marc] Catholic Univ Louvain, Ctr Cosmol Particle Phys & Phenomenol CP3, B-1348 Louvain, Belgium. [Bardeen, William A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Buras, AJ (reprint author), TUM Inst Adv Study, Lichtenbergstr 2a, D-85747 Garching, Germany. EM aburas@ph.tum.de FU ERC Advanced Grant project "FLAVOUR" [267104]; Belgian IAP Program [BELSPO P7/37]; DFG cluster of excellence "Origin and Structure of the Universe"; United States Department of Energy [DE-AC02- 07CH11359] FX AJB would like to thank Gino Isidori and Heiri Leutwyler for very encouraging comments on the first version of the paper and Jure Drobnak and Robert Ziegler for checking numerically the values of the Wilson coefficients zi. We would like to thank Jennifer Girrbach, Chris Sachrajda and Amarjit Soni for discussions and Nuria Carrasco, Luca Silvestrini and Vittorio Lubicz for E-mail exchanges. This research was financially supported by the ERC Advanced Grant project "FLAVOUR" (267104) and the Belgian IAP Program BELSPO P7/37. It was also partially supported by the DFG cluster of excellence "Origin and Structure of the Universe". Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02- 07CH11359 with the United States Department of Energy. NR 100 TC 26 Z9 26 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY 20 PY 2014 VL 74 IS 5 AR 2871 DI 10.1140/epjc/s10052-014-2871-x PG 30 WC Physics, Particles & Fields SC Physics GA CD0DM UT WOS:000350740600001 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Aielli, G Akesson, TP Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bolnet, NM Bomben, M Bona, M Boonekamp, M Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A 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Zimine, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. CA ATLAS Collaboration TI Search for Invisible Decays of a Higgs Boson Produced in Association with a Z Boson in ATLAS SO PHYSICAL REVIEW LETTERS LA English DT Article ID DARK-MATTER; MAJORON MODELS; LEPTON NUMBER; PARTICLES; VIOLATION; DETECTOR; MASSES; LHC AB A search for evidence of invisible-particle decay modes of a Higgs boson produced in association with a Z boson at the Large Hadron Collider is presented. No deviation from the standard model expectation is observed in 4.5 fb(-1) (20.3 fb(-1)) of 7 (8) TeV pp collision data collected by the ATLAS experiment. Assuming the standard model rate for ZH production, an upper limit of 75%, at the 95% confidence level is set on the branching ratio to invisible-particle decay modes of the Higgs boson at a mass of 125.5 GeV. The limit on the branching ratio is also interpreted in terms of an upper limit on the allowed dark matter-nucleon scattering cross section within a Higgs-portal dark matter scenario. Within the constraints of such a scenario, the results presented in this Letter provide the strongest available limits for low-mass dark matter candidates. Limits are also set on an additional neutral Higgs boson, in the mass range 110 < m(H) < 400 GeV, produced in association with a Z boson and decaying to invisible particles. C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. 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[Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Backes, M.; Banfi, D.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Franchino, S.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; PommSs, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, Y.; Peng, H.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Willis, W.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Dano Hoffmann, M.; Galster, G.; Gregersen, K.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Milan, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwasaki, H.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Dallas, TX 75230 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Naumann, T.; Peschke, R.; Peters, R. F. Y.; Petit, E.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Peters, R. F. Y.; Petit, E.; Piec, S. M.; Radeka, V.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Bunse, M.; Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Univ Dortmund, Inst Expt Phys 4, D-44227 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Schnoor, U.; Socher, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Kajomovitz, E.; Kotwal, A.; Kruse, A.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Miucci, A.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Caso, C.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Milan, Italy. [Barberis, D.; Caso, C.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Ivane Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, J.; Smith, K. M.; St. Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Meyer, J.; Morel, J.; Nackenhorst, O.; Nadal, J.; Peters, R. F. Y.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, G.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Guimaraes da Costa, J. Barreiro; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; Della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lange, C.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, Y.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Milan, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salerno, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, A.; Span, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Martyniuk, A. C.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjonmark, J. U.; Smirnova, O.; Viazlo, O.; Wielers, M.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bertella, C.; Bousson, N.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bertella, C.; Bousson, N.; Chen, L.; Clemens, J. C.; Coadou, Y.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubacek, Z.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, P.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Ge, P.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Stelzer, H. J.; Ta, D.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Moscow Engn Phys Inst, MEPhI, Moscow 115409, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Milan, Italy. [Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluth, S.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Scifo, E.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Milan, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Milan, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao Fis Expt Particula, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Bohm, C.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Dos Santos, D. Roda; Ruzicka, P.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Milan, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Liu, L.; Luci, C.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Milan, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Milan, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Laporte, J. F.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Migas, S.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwegler, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Inst Rech Lois Fondament Univers, DSM IRFU, Gif Sur Yvette, France. [Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Chen, X.; Huang, Y.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg 2050, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, B.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Bee, C. P.; Chen, K.; Engelmann, R.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Bee, C. P.; Chen, K.; Engelmann, R.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Intt Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, N.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Shimmin, C. O.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Milan, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] IFIC, Inst Fis Corpuscular, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Gonzalez Parra, G.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elec, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrari, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, A.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. 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[Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaidan, R.] Technol State Univ, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. 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Kuleshov, Sergey/D-9940-2013; Gabrielli, Alessandro/H-4931-2012; Juste, Aurelio/I-2531-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Grinstein, Sebastian/N-3988-2014; la rotonda, laura/B-4028-2016; Monzani, Simone/D-6328-2017; Fullana Torregrosa, Esteban/A-7305-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Canelli, Florencia/O-9693-2016; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016 OI White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Moraes, Arthur/0000-0002-5157-5686; Smirnova, Oxana/0000-0003-2517-531X; Smirnov, Sergei/0000-0002-6778-073X; Belanger-Champagne, Camille/0000-0003-2368-2617; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Walsh, Brian/0000-0003-1689-2309; Price, Darren/0000-0003-2750-9977; Filthaut, Frank/0000-0003-3338-2247; Terzo, Stefano/0000-0003-3388-3906; Warburton, Andreas/0000-0002-2298-7315; Castro, Nuno/0000-0001-8491-4376; Ferrando, James/0000-0002-1007-7816; Bosman, Martine/0000-0002-7290-643X; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Gabrielli, Alessandro/0000-0001-5346-7841; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Wang, Kuhan/0000-0002-6151-0034; Grohsjean, Alexander/0000-0003-0748-8494; La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Cristinziani, Markus/0000-0003-3893-9171; Qian, Jianming/0000-0003-4813-8167; Haas, Andrew/0000-0002-4832-0455; Galhardo, Bruno/0000-0003-0641-301X; Della Volpe, Domenico/0000-0001-8530-7447; Pina, Joao /0000-0001-8959-5044; Hays, Chris/0000-0003-2371-9723; Dell'Asta, Lidia/0000-0002-9601-4225; Sawyer, Lee/0000-0001-8295-0605; Juste, Aurelio/0000-0002-1558-3291; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Grinstein, Sebastian/0000-0002-6460-8694; la rotonda, laura/0000-0002-6780-5829; Coccaro, Andrea/0000-0003-2368-4559; Monzani, Simone/0000-0002-0479-2207; Chromek-Burckhart, Doris/0000-0003-4243-3288; Begel, Michael/0000-0002-1634-4399; Mincer, Allen/0000-0002-6307-1418; Troncon, Clara/0000-0002-7997-8524; Bailey, David C/0000-0002-7970-7839; Chen, Hucheng/0000-0002-9936-0115; Nisati, Aleandro/0000-0002-5080-2293; Fullana Torregrosa, Esteban/0000-0003-3082-621X; Vari, Riccardo/0000-0002-2814-1337; Gray, Heather/0000-0002-5293-4716; Thomson, Mark/0000-0002-2654-9005; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Canelli, Florencia/0000-0001-6361-2117; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; NSRF; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America; ERC; European Union; Geneva, Switzerland FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 70 TC 106 Z9 106 U1 13 U2 135 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2014 VL 112 IS 20 AR 201802 DI 10.1103/PhysRevLett.112.201802 PG 19 WC Physics, Multidisciplinary SC Physics GA AM0RS UT WOS:000339554800003 ER PT J AU Hayes, AC Friar, JL Garvey, GT Jungman, G Jonkmans, G AF Hayes, A. C. Friar, J. L. Garvey, G. T. Jungman, Gerard Jonkmans, G. TI Systematic Uncertainties in the Analysis of the Reactor Neutrino Anomaly SO PHYSICAL REVIEW LETTERS LA English DT Article ID FISSION-PRODUCTS; ANTINEUTRINO SPECTRA; DECAY; HYDROGEN; PU-239 AB We examine uncertainties in the analysis of the reactor neutrino anomaly, wherein it is suggested that only about 94% of the emitted antineutrino flux was detected in short baseline experiments. We find that the form of the corrections that lead to the anomaly are very uncertain for the 30% of the flux that arises from forbidden decays. This uncertainty was estimated in four ways, is as large as the size of the anomaly, and is unlikely to be reduced without accurate direct measurements of the antineutrino flux. Given the present lack of detailed knowledge of the structure of the forbidden transitions, it is not possible to convert the measured aggregate fission beta spectra to antineutrino spectra to the accuracy needed to infer an anomaly. Neutrino physics conclusions based on the original anomaly need to be revisited, as do oscillation analyses that assumed that the antineutrino flux is known to better than approximately 4%. C1 [Hayes, A. C.; Friar, J. L.; Garvey, G. T.; Jungman, Gerard] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Jonkmans, G.] AECL Res, Chalk River Labs, Chalk River, ON K0J 1J0, Canada. RP Hayes, AC (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. NR 22 TC 49 Z9 49 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2014 VL 112 IS 20 AR 202501 DI 10.1103/PhysRevLett.112.202501 PG 5 WC Physics, Multidisciplinary SC Physics GA AM0RS UT WOS:000339554800004 ER PT J AU Lee, D Mitchell, B Fujiwara, Y Dierolf, V AF Lee, Donghwa Mitchell, Brandon Fujiwara, Y. Dierolf, V. TI Thermodynamics and Kinetics of Three Mg-H-V-N Complexes in Mg:GaN from Combined First-Principles Calculation and Experiment SO PHYSICAL REVIEW LETTERS LA English DT Article ID DOPED GAN; COMPENSATION; MECHANISM; POINTS; FILMS AB An understanding of the formation and dissociation process of Mg-H defects in GaN is of paramount importance for high efficient GaN-based solid-state lighting. Through a combination of first-principle calculations and experimental observations, we find the existence of three types of Mg related centers forming different Mg-H-V-N complexes in Mg:GaN. Our study shows that the three different arrangements, which differ by the relative position of the H, determine the degree of acceptor passivation by changing their charge state from +3 to +1. The energetic study demonstrates that the relative stability of the defect complexes can vary with the location of the Fermi level, as well as thermal annealing and electron beam irradiation. The inclusion of a V-N is shown to produce an additional variance in optical spectra associated with Mg acceptor activation, resulting from changes in the defect configurations and charge states. Our study shows that these three Mg-H-V-N complexes are key components for understanding the Mg acceptor activation and passivation processes. C1 [Lee, Donghwa] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Mitchell, Brandon; Dierolf, V.] Lehigh Univ, Dept Phys, Bethlehem, PA 18015 USA. [Fujiwara, Y.] Osaka Univ, Div Mat & Mfg Sci, Suita, Osaka 5650871, Japan. RP Lee, D (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave L-413, Livermore, CA 94550 USA. EM lee1004@llnl.gov RI Lee, Donghwa/G-7934-2012; Fujiwara, Yasufumi/D-9052-2012 OI Lee, Donghwa/0000-0002-8956-3648; FU NSF [ECCS-140038]; Japan Society for the Promotion of Science [24226009]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The experimental work performed by B. M. and V. D. was supported by NSF Grant No. ECCS-140038. The experimental work performed by Y. F. was supported by a Grant-in-Aid for Scientific Research (S) (Grant No. 24226009) from the Japan Society for the Promotion of Science. Part of the work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 29 TC 2 Z9 2 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2014 VL 112 IS 20 AR 205501 DI 10.1103/PhysRevLett.112.205501 PG 5 WC Physics, Multidisciplinary SC Physics GA AM0RS UT WOS:000339554800009 ER PT J AU Mak, KF da Jornada, FH He, KL Deslippe, J Petrone, N Hone, J Shan, J Louie, SG Heinz, TF AF Mak, Kin Fai da Jornada, Felipe H. He, Keliang Deslippe, Jack Petrone, Nicholas Hone, James Shan, Jie Louie, Steven G. Heinz, Tony F. TI Tuning Many-Body Interactions in Graphene: The Effects of Doping on Excitons and Carrier Lifetimes SO PHYSICAL REVIEW LETTERS LA English DT Article ID OPTICAL-SPECTRA; BAND-GAPS; SEMICONDUCTORS; INSULATORS AB The optical properties of graphene are strongly affected by electron-electron (e-e) and electron-hole (e-h) interactions. Here we tune these many-body interactions through varying the density of free charge carriers. Measurements from the infrared to the ultraviolet reveal significant changes in the optical conductivity of graphene for both electron and hole doping. The shift, broadening, and modification in shape of the saddle-point exciton resonance reflect strong screening of the many-body interactions by the carriers, as well as changes in quasiparticle lifetimes. Ab initio calculations by the GW Bethe-Salpeter equation method, which take into account the modification of both the repulsive e-e and the attractive e-h interactions, provide excellent agreement with experiment. Understanding the optical properties and high-energy carrier dynamics of graphene over a wide range of doping is crucial for both fundamental graphene physics and for emerging applications of graphene in photonics. C1 [Mak, Kin Fai; Heinz, Tony F.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Mak, Kin Fai; Heinz, Tony F.] Columbia Univ, Dept Elect Engn, New York, NY 10027 USA. [da Jornada, Felipe H.; Deslippe, Jack; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [da Jornada, Felipe H.; Deslippe, Jack; Louie, Steven G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [He, Keliang; Shan, Jie] Case Western Reserve Univ, Dept Phys, Cleveland, OH 44106 USA. [Deslippe, Jack] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Energy Res Sci Comp Ctr, Berkeley, CA 94720 USA. [Petrone, Nicholas; Hone, James] Columbia Univ, Dept Mech Engn, New York, NY 10027 USA. RP Heinz, TF (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. EM tony.heinz@columbia.edu RI Hone, James/E-1879-2011; Heinz, Tony/K-7797-2015 OI Hone, James/0000-0002-8084-3301; Heinz, Tony/0000-0003-1365-9464 FU U.S. Department of Energy (DOE) through the Energy Frontier Research Center at Columbia University [DESC00001085]; U.S. Office of Naval Research (ONR) at Columbia University; National Science Foundation (NSF) [DMR-0907477, DMR-1106225, DMR-101006184]; ONR under the MURI program at University of California, Berkeley; U.S. Department of Energy, the Office of Basic Energy Sciences and of Advanced Scientific Computing Research [DE-AC02-05CH11231]; Simons Foundation Fellowship in Theoretical Physics FX We acknowledge helpful discussions with Dr. Mark Hybertsen. Support for the growth of the graphene samples was provided by the U.S. Department of Energy (DOE) through the Energy Frontier Research Center at Columbia University (Grant No. DESC00001085). Device fabrication was supported by the U.S. Office of Naval Research (ONR) at Columbia University and by the National Science Foundation (NSF Grant No. DMR-0907477) at Case Western Reserve University. Optical characterization and analysis was supported by the NSF (Grant No. DMR-1106225). The theoretical formulation and study of lifetime effects was supported by the NSF (Grant No. DMR-101006184) and by the ONR under the MURI program at University of California, Berkeley. This research is also supported by the Theory Program (simulation and analysis of the optical absorption) and the SciDAC Program on Excited State Phenomena in Energy Materials (algorithms and code developments) funded by the U.S. Department of Energy, the Office of Basic Energy Sciences and of Advanced Scientific Computing Research, under Contract No. DE-AC02-05CH11231 at the Lawrence Berkeley National Laboratory. S. G. L. acknowledges support of a Simons Foundation Fellowship in Theoretical Physics. Computational resources were provided by the DOE at Lawrence Berkeley National Laboratory's NERSC facility. K. F. M. and F. H. J. contributed equally to this work. NR 37 TC 22 Z9 22 U1 3 U2 58 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2014 VL 112 IS 20 AR 207401 DI 10.1103/PhysRevLett.112.207401 PG 5 WC Physics, Multidisciplinary SC Physics GA AM0RS UT WOS:000339554800013 ER PT J AU Sakai, H Tokunaga, Y Kambe, S Ronning, F Bauer, ED Thompson, JD AF Sakai, H. Tokunaga, Y. Kambe, S. Ronning, F. Bauer, E. D. Thompson, J. D. TI Coexistence of Antiferromagnetism with Superconductivity in CePt2In7: Microscopic Phase Diagram Determined by In-115 NMR and NQR SO PHYSICAL REVIEW LETTERS LA English DT Article ID QUANTUM CRITICALITY; CERHIN5; TRANSITIONS; SYSTEMS AB Single crystals of the heavy-fermion antiferromagnet CePt2In7 with a Neel temperature (T-N) of 5.2 K at ambient pressure have been investigated by zero-field In-115-nuclear magnetic and quadrupole resonance measurements as a function of applied pressure. Within the antiferromagnetic state, the character of Ce's 4f electron appears to change from localized to itinerantlike at P* similar to 2.4 GPa, approximately the pressure where superconductivity first emerges. With increased pressure, the superconducting transition T-c reaches a maximum just at or slightly before antiferromagnetic order disappears, and not at the pressure P-c similar to 3.4 GPa, where the steeply decreasing Neel boundary extrapolates to zero temperature. For P > P-c, the spin relaxation rate drops sharply by more than 2 orders of magnitude at T-c, suggestive of a first-order transition. C1 [Sakai, H.; Tokunaga, Y.; Kambe, S.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Ronning, F.; Bauer, E. D.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Sakai, H (reprint author), Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. EM sakai.hironori@jaea.go.jp FU Reimei Research Program of JAEA; U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX We thank S. Hoshino, N. Tateiwa, Y. Haga, and H. Yasuoka for valuable discussions. Work in Japan was supported by the Reimei Research Program of JAEA. Work at LANL was performed under the auspices of the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 33 TC 8 Z9 8 U1 5 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2014 VL 112 IS 20 AR 206401 DI 10.1103/PhysRevLett.112.206401 PG 5 WC Physics, Multidisciplinary SC Physics GA AM0RS UT WOS:000339554800011 ER PT J AU Polei, S Snijders, PC Meiwes-Broer, KH Barke, I AF Polei, S. Snijders, P. C. Meiwes-Broer, K. -H. Barke, I. TI Current-dependent periodicities of Si(553)-Au SO PHYSICAL REVIEW B LA English DT Article ID ATOM AB We investigate quasi-one-dimensional atomic chains on Si(553)-Au with a scanning tunneling microscope (STM). The observed periodicity at the Si step edge can be altered by the STM and depends on the magnitude of the tunneling current. In a recent report this reversible structural transition was attributed to transient doping with a characteristic time scale of a few milliseconds [S. Polei et al., Phys. Rev. Lett. 111, 156801 (2013)]. Here we explore the evolution of the STM topography as a function of the magnitude of the tunneling current for a wide temperature range. Based on a decomposition of topographic line profiles and a detailed Fourier analysis we conclude that all observed current-dependent STM topographies can be explained by a time-averaged linear combination of two fluctuating step-edge structures. These data also reveal the precise relative alignment of the characteristic STM features for both phases along the step edges. A simple diagram is developed, presenting the relative contribution of these phases to the STM topography as a function of tunneling current and temperature. Time-and current-dependent measurements of fluctuations in the tunneling current reveal two different transition regimes that are related to two specific current injection locations within the surface unit cell. A method based on spatially resolved I (z) curves is presented that enables a quantitative analysis of contributing phases. C1 [Polei, S.; Meiwes-Broer, K. -H.; Barke, I.] Univ Rostock, Inst Phys, D-18055 Rostock, Germany. [Snijders, P. C.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Snijders, P. C.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Polei, S (reprint author), Univ Rostock, Inst Phys, D-18055 Rostock, Germany. EM snijderspc@ornl.gov; ingo.barke@uni-rostock.de OI Meiwes-Broer, Karl-Heinz/0000-0002-8516-0470 FU federal state Mecklenburg-Vorpommern within the project Nano4Hydrogen; Federal Ministry of Education and Research (BMBF) within the project Light2Hydrogen; US DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division, through the Oak Ridge National Laboratory FX Funding by the federal state Mecklenburg-Vorpommern within the project Nano4Hydrogen and by the Federal Ministry of Education and Research (BMBF) within the project Light2Hydrogen is gratefully acknowledged (S. P.). P. C. S. acknowledges support by the US DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division, through the Oak Ridge National Laboratory. NR 32 TC 2 Z9 2 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 20 PY 2014 VL 89 IS 20 AR 205420 DI 10.1103/PhysRevB.89.205420 PG 8 WC Physics, Condensed Matter SC Physics GA AM0RL UT WOS:000339553800004 ER PT J AU Li, QY Fernandez-Martinez, A Lee, B Waychunas, GA Jun, YS AF Li, Qingyun Fernandez-Martinez, Alejandro Lee, Byeongdu Waychunas, Glenn A. Jun, Young-Shin TI Interfacial Energies for Heterogeneous Nucleation of Calcium Carbonate on Mica and Quartz SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID IN-SITU OBSERVATIONS; PRECIPITATION KINETICS; CO2 SEQUESTRATION; FORCE MICROSCOPY; EPITAXIAL-GROWTH; SCALE; STORAGE; BIOMINERALIZATION; CRYSTALLIZATION; THERMODYNAMICS AB Interfacial free energies often control heterogeneous nucleation of calcium carbonate (CaCO3) on mineral surfaces. Here we report an in situ experimental study of CaCO3 nucleation on mica (muscovite) and quartz, which allows us to obtain the interfacial energies governing heterogeneous nucleation. In situ grazing incidence small-angle X-ray scattering (GISAXS) was used to measure nucleation rates at different supersaturations. The rates were incorporated into classical nucleation theory to calculate the effective interfacial energies (alpha'). Ex situ Raman spectroscopy identified both calcite and vaterite as CaCO3 polymorphs; however, vaterite is the most probable heterogeneous nuclei mineral phase. The alpha' was 24 mJ/m(2) for the vaterite mica system and 32 mJ/m(2) for the vaterite quartz system. The smaller alpha' of the CaCO3 mica system led to smaller particles and often higher particle densities on mica. A contributing factor affecting alpha' in our system was the smaller structural mismatch between CaCO3 and mica compared to that between CaCO3 and quartz. The extent of hydrophilicity and the surface charge could not explain the observed CaCO3 nucleation trend on mica and quartz. The findings of this study provide new thermodynamic parameters for subsurface reactive transport modeling and contribute to our understanding of mechanisms where CaCO3 formation on surfaces is of concern. C1 [Li, Qingyun; Jun, Young-Shin] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. [Fernandez-Martinez, Alejandro] CNRS, ISTerre, F-38041 Grenoble, France. [Fernandez-Martinez, Alejandro] Univ Grenoble Alpes, ISTerre, F-38041 Grenoble, France. [Lee, Byeongdu] Argonne Natl Lab, Argonne, IL 60439 USA. [Waychunas, Glenn A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Jun, YS (reprint author), Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. EM ysjun@seas.wustl.edu RI Fernandez-Martinez, Alejandro/B-4042-2010; OI Fernandez-Martinez, Alejandro/0000-0001-5073-9629; Lee, Byeongdu/0000-0003-2514-8805 FU Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]; U.S. DOE [DE-AC02-06CH11357]; National Science Foundation [EAR-1057117] FX The authors acknowledge Dr. Yandi Hu for valuable discussions about the experimental setup and data analysis, Drs. Xiaobing Zuo and Sonke Seifert for helping collect GISAXS data, and Ms. Jessica Ray and Dr. Namhey Lee for helping conducting experiments. We also thank Dr. Carl I. Steefel for insightful discussion about calcium carbonates in GCS field sites. We also appreciate Prof. J. C. Ballard's close reading of the manuscript. The authors also acknowledge support from the Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-AC02-05CH11231. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. This work was also partially supported by the National Science Foundation's Career Award (EAR-1057117). ISTerre is part of Labex OSUG@2020 (ANR10 LABX56). NR 67 TC 8 Z9 8 U1 3 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 20 PY 2014 VL 48 IS 10 BP 5745 EP 5753 DI 10.1021/es405141j PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AH8VB UT WOS:000336415200048 PM 24730716 ER PT J AU Riley, BJ Pierce, DA Chun, J Matyas, J Lepry, WC Garn, TG Law, JD Kanatzidis, MG AF Riley, Brian J. Pierce, David A. Chun, Jaehun Matyas, Josef Lepry, William C. Garn, Troy G. Law, Jack D. Kanatzidis, Mercouri G. TI Polyacrylonitrile-Chalcogel Hybrid Sorbents for Radioiodine Capture SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID RADIOACTIVE IODINE; WASTE FORMS; IMMOBILIZATION; REMEDIATION; AEROGELS; GLASSES; APATITE AB Powders of a Sn2S3 chalcogen-based aerogel (chalcogel) were combined with powdered polyacrylonitrile (PAN) in different mass ratios (SnS33, SnS50, and SnS70; # = mass% of chalcogel), dissolved in dimethyl sulfoxide, and added dropwise to deionized water to form pellets of a porous PAN-chalcogel hybrid material. These pellets, along with pure powdered (SnSp) and granular (SnSg) forms of the chalcogel, were then used to capture iodine gas under both dynamic (dilute) and static (concentrated) conditions. Both SnSp and SnSg chalcogels showed very high iodine loadings at 67.2 and 68.3 mass%, respectively. The SnS50 hybrid sorbent demonstrated strated a high, although slightly reduced, maximum iodine loading (53.5 mass%) with greatly improved mechanical rigidity. In all cases, X-ray diffraction results showed the formation of crystalline SnI4 and SnI4(S-8)(2), revealing that the iodine binding in these materials is mainly due to a chemisorption process, although a small amount of physisorption was observed. C1 [Riley, Brian J.; Pierce, David A.; Chun, Jaehun; Matyas, Josef; Lepry, William C.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Garn, Troy G.; Law, Jack D.] EG&G Idaho Inc, Idaho Natl Engn Lab, Idaho Falls, ID 83401 USA. [Kanatzidis, Mercouri G.] Northwestern Univ, Evanston, IL 60208 USA. RP Riley, BJ (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM brian.riley@pnnl.gov OI Riley, Brian/0000-0002-7745-6730; Law, Jack/0000-0001-7085-7542 FU Department of Energy Office of Nuclear Energy under the Fuel Cycle Research and Development Program; U.S. Department of Energy [DE-AC05-76RL01830]; NEUP program of DOE FX This work was funded by the Department of Energy Office of Nuclear Energy under the Fuel Cycle Research and Development Program. Pacific Northwest National Laboratory is operated by the U.S. Department of Energy under Contract Number DE-AC05-76RL01830. At Northwestern University, this work was supported by the NEUP program of DOE (M.G.K.). The authors thank Denis Strachan for comments on this document. The authors also thank Benjamin Yuhas of Northwestern University for providing the Na4Sn2S6center dot 14H2O precursor that was used to make the Sn2S3 chalcogel, Xiaohong Li for help with BET, Maura Zimmerschied for technical editing, and Michael Perkins for help with the graphics. NR 40 TC 13 Z9 13 U1 4 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 20 PY 2014 VL 48 IS 10 BP 5832 EP 5839 DI 10.1021/es405807w PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AH8VB UT WOS:000336415200058 PM 24779585 ER PT J AU Jeong, S Millstein, D Fischer, ML AF Jeong, Seongeun Millstein, Dev Fischer, Marc L. TI Spatially Explicit Methane Emissions from Petroleum Production and the Natural Gas System in California SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article AB We present a new, spatially resolved inventory of methane (CH4) emissions based on US-EPA emission factors and publically available activity data for 2010 California petroleum production and natural gas production, processing, transmission, and distribution. Compared to official California bottom-up inventories, our initial estimates are 3 to 7 times higher for the petroleum and natural gas production sectors but similar for the natural gas transmission and distribution sectors. Evidence from published "top-down" atmospheric measurement campaigns within Southern California supports our initial emission estimates from production and processing but indicates emission estimates from transmission and distribution are low by a factor of approximately 2. To provide emission maps with more accurate total emissions we scale the spatially resolved inventory by sector-specific results from a Southern California aircraft measurement campaign to all of California. Assuming uncertainties are determined by the uncertainties estimated in the top-down study, our estimated state total CH4 emissions are 541 +/- 144 Gg yr(-1) (as compared with 210.7 Gg yr(-1) in California's current official inventory), where the majority of our reported uncertainty is derived from transmission and distribution. We note uncertainties relative to the mean for a given region are likely larger than that for the State total, emphasizing the need for additional measurements in undersampled regions. C1 [Jeong, Seongeun; Millstein, Dev; Fischer, Marc L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Jeong, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM sjeong@lbl.gov FU California Energy Commissions Public Interest Environmental Research program; US Department of Energy [DE-AC02-05CH11231] FX We thank Stephanie Detwiler, Joseph Fischer, Simone Brant, Guido Franco, Larry Sasadeusz, and Bill Winkler for valuable advice and discussion. This analysis was supported by the California Energy Commissions Public Interest Environmental Research program, with work at LBNL conducted under US Department of Energy Contract DE-AC02-05CH11231. NR 27 TC 10 Z9 10 U1 1 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 20 PY 2014 VL 48 IS 10 BP 5982 EP 5990 DI 10.1021/es4046692 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AH8VB UT WOS:000336415200075 PM 24758763 ER PT J AU Davis, RE Fishman, DB Frank, ED Johnson, MC Jones, SB Kinchin, CM Skaggs, RL Venteris, ER Wigmosta, MS AF Davis, Ryan E. Fishman, Daniel B. Frank, Edward D. Johnson, Michael C. Jones, Susanne B. Kinchin, Christopher M. Skaggs, Richard L. Venteris, Erik R. Wigmosta, Mark S. TI Integrated Evaluation of Cost, Emissions, and Resource Potential for Algal Biofuels at the National Scale SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID HYDROTHERMAL LIQUEFACTION; TECHNOECONOMIC ANALYSIS; NANNOCHLOROPSIS SP; OIL PRODUCTION; RACEWAY PONDS; UNITED-STATES; MICROALGAE; AVAILABILITY; CULTIVATION; CONVERSION AB Costs, emissions, and resource availability were modeled for the production of 5 billion gallons yr(-1) (5 BGY) of renewable diesel in the United States from Chlorella biomass by hydrothermal liquefaction (HTL). The HTL model utilized data from a continuous 1-L reactor including catalytic hydrothermal gasification of the aqueous phase, and catalytic hydrotreatment of the HTL oil. A biophysical algae growth model coupled with weather and pond simulations predicted biomass productivity from experimental growth parameters, allowing site-by-site and temporal prediction of biomass production. The 5 BGY scale required geographically and climatically distributed sites. Even though screening down to 5 BGY significantly reduced spatial and temporal variability, site-to-site, season-to-season, and interannual variations in productivity affected economic and environmental performance. Performance metrics based on annual average or peak productivity were inadequate; temporally and spatially explicit computations allowed more rigorous analysis of these dynamic systems. For example, 3-season operation with a winter shutdown was favored to avoid high greenhouse gas emissions, but economic performance was harmed by underutilized equipment during slow-growth periods. Thus, analysis of algal biofiiel pathways must combine spatiotemporal resource assessment, economic analysis, and environmental analysis integrated over many sites when assessing national scale performance. C1 [Frank, Edward D.; Johnson, Michael C.] Argonne Natl Lab, Ctr Transportat Res, Argonne, IL 60439 USA. [Fishman, Daniel B.] US DOE, Washington, DC 20585 USA. [Davis, Ryan E.; Kinchin, Christopher M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Jones, Susanne B.; Skaggs, Richard L.; Venteris, Erik R.; Wigmosta, Mark S.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Frank, ED (reprint author), Argonne Natl Lab, Ctr Transportat Res, 9700 S Cass Ave, Argonne, IL 60439 USA. EM efrank@anl.gov RI Frank, Edward/A-8865-2012 FU U.S. Department of Energy (DOE); Argonne National Laboratory is a DOE laboratory [DE-AC02-06CH11357]; NREL is a national laboratory of the U.S. Department of Energy, Office of Energy Efficiency & Renewable Energy [DE-AC36-08GO28308]; Pacific Northwest National Laboratory [DE-AC05-76RL01830] FX This work was sponsored by the U.S. Department of Energy (DOE). Argonne National Laboratory is a DOE laboratory managed by UChicago Argonne, LLC under contract DE-AC02-06CH11357. NREL is a national laboratory of the U.S. Department of Energy, Office of Energy Efficiency & Renewable Energy, operated by the Alliance for Sustainable Energy, LLC, under contract DE-AC36-08GO28308. Pacific Northwest National Laboratory is operated by Battelle for DOE under contract DE-AC05-76RL01830. NR 37 TC 28 Z9 28 U1 7 U2 84 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 20 PY 2014 VL 48 IS 10 BP 6035 EP 6042 DI 10.1021/es4055719 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AH8VB UT WOS:000336415200082 PM 24749989 ER PT J AU Gerlits, O Das, A Keshwani, MM Taylor, S Waltman, MJ Langan, P Heller, WT Kovalevsky, A AF Gerlits, Oksana Das, Amit Keshwani, Malik M. Taylor, Susan Waltman, Mary Jo Langan, Paul Heller, William T. Kovalevsky, Andrey TI Metal-Free cAMP-Dependent Protein Kinase Can Catalyze Phosphoryl Transfer SO BIOCHEMISTRY LA English DT Article ID STABLE INHIBITOR PROTEIN; PEPTIDE INHIBITOR; KINETIC MECHANISM; CRYSTAL-STRUCTURE; SITE SPECIFICITY; TRANSITION-STATE; BOVINE HEART; ACTIVE-SITE; SUBUNIT; SUBSTRATE AB X-ray structures of several ternary product complexes of the catalytic subunit of cAMP-dependent protein kinase (PKAc) have been determined with no bound metal ions and with Na+ or K+ coordinated at two metal-binding sites. The metal-free PKAc and the enzyme with alkali metals were able to facilitate the phosphoryl transfer reaction. In all studied complexes, the ATP and the substrate peptide (SP20) were modified into the products ADP and the phosphorylated peptide. The products of the phosphotransfer reaction were also found when ATP-gamma S, a nonhydrolyzable ATP analogue, reacted with SP20 in the PKAc active site containing no metals. Single turnover enzyme kinetics measurements utilizing P-32-labeled ATP confirmed the phosphotransferase activity of the enzyme in the absence of metal ions and in the presence of alkali metals. In addition, the structure of the apo-PKAc binary complex with SP20 suggests that the sequence of binding events may become ordered in a metal-free environment, with SP20 binding first to prime the enzyme for subsequent ATP binding. Comparison of these structures reveals conformational and hydrogen bonding changes that might be important for the mechanism of catalysis. C1 [Gerlits, Oksana; Das, Amit; Langan, Paul; Heller, William T.; Kovalevsky, Andrey] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Keshwani, Malik M.; Taylor, Susan] Univ Calif San Diego, Dept Chem, La Jolla, CA 92093 USA. [Keshwani, Malik M.; Taylor, Susan] Univ Calif San Diego, Dept Biochem & Pharmacol, La Jolla, CA 92093 USA. [Waltman, Mary Jo] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Kovalevsky, A (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. EM kovalevskyay@ornl.gov RI Langan, Paul/N-5237-2015; OI Langan, Paul/0000-0002-0247-3122; Kovalevsky, Andrey/0000-0003-4459-9142 FU UCOP; DOE-OBER; NIH-NIGMS [1R01GM071939-01]; NIH [GM19301]; Laboratory Directed Research and Development grant from ORNL FX O.G., S.T. and A.K. were partly supported by a UCOP grant. M.J.W. was partly supported by a DOE-OBER grant to the neutron Protein Crystallography Station at LANSCE. P.L. was partly supported by an NIH-NIGMS-funded consortium (Grant 1R01GM071939-01) between ORNL and LBNL to develop computational tools for neutron protein crystallography. S.T. and M.M.K. were partly supported by NIH Grant GM19301. A.D. and W.T.H. were supported and O.G. and P.L. were partly supported by a Laboratory Directed Research and Development grant from ORNL. NR 49 TC 10 Z9 10 U1 0 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 20 PY 2014 VL 53 IS 19 BP 3179 EP 3186 DI 10.1021/bi5000965 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AH8UM UT WOS:000336413700012 PM 24786636 ER PT J AU Huang, RK Baxa, U Aldrian, G Ahmed, AB Wall, JS Mizuno, N Antzutkin, O Steven, AC Kajava, AV AF Huang, Rick K. Baxa, Ulrich Aldrian, Gudrun Ahmed, Abdullah B. Wall, Joseph S. Mizuno, Naoko Antzutkin, Oleg Steven, Alasdair C. Kajava, Andrey V. TI Conformational Switching in PolyGln Amyloid Fibrils Resulting from a Single Amino Acid Insertion SO BIOPHYSICAL JOURNAL LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; SOLID-STATE NMR; BETA-SOLENOID PROTEINS; URE2P PRION FILAMENTS; HUNTINGTONS-DISEASE; POLYGLUTAMINE; PARALLEL; IMAGE; FORM; ORGANIZATION AB The established correlation between neurodegenerative disorders and intracerebral deposition of polyglutamine aggregates motivates attempts to better understand their fibrillar structure. We designed polyglutamines with a few lysines inserted to overcome the hindrance of extreme insolubility and two D-lysines to limit the lengths of beta-strands. One is 33 amino acids long (PolyQKd-33) and the other has one fewer glutamine (PolyQKd-32). Both form well-dispersed fibrils suitable for analysis by electron microscopy. Electron diffraction confirmed cross-beta structures in both fibrils. Remarkably, the deletion of just one glutamine residue from the middle of the peptide leads to substantially different amyloid structures. PolyQKd-32 fibrils are consistently 10-20% wider than PolyQKd-33, as measured by negative staining, cryo-electron microscopy, and scanning transmission electron microscopy. Scanning transmission electron microscopy analysis revealed that the PolyQKd-32 fibrils have 50% higher mass-per-length than PolyQKd-33. This distinction can be explained by a superpleated beta-structure model for PolyQKd-33 ;and a model with two beta-solenoid protofibrils for PolyQKd-32. These data provide evidence for beta-arch-containing structures in polyglutamine fibrils and open future possibilities for structure-based drug design. C1 [Huang, Rick K.; Baxa, Ulrich; Mizuno, Naoko; Steven, Alasdair C.] NIAMSD, Struct Biol Lab, NIH, Bethesda, MD 20892 USA. [Baxa, Ulrich] Frederick Natl Lab Canc Res, Electron Microscopy Lab, Canc Res Technol Program, Leidos Biomed Res, Frederick, MD USA. [Aldrian, Gudrun; Ahmed, Abdullah B.; Kajava, Andrey V.] Univ Montpellier 1 & 2, CNRS, Ctr Rech Biochim Macromol, Montpellier, France. [Kajava, Andrey V.] Inst Biol Computat, Montpellier, France. [Kajava, Andrey V.] Univ ITMO, St Petersburg 197101, Russia. [Wall, Joseph S.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Mizuno, Naoko] Max Planck Inst Biochem, Dept Struct Cell Biol, D-82152 Martinsried, Germany. [Antzutkin, Oleg] Lulea Univ Technol, S-95187 Lulea, Sweden. [Antzutkin, Oleg] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. RP Steven, AC (reprint author), NIAMSD, Struct Biol Lab, NIH, Bethesda, MD 20892 USA. EM stevena@mail.nih.gov; andrey.kajava@crbm.cnrs.fr RI Kajava, Andrey/E-1107-2014 OI Kajava, Andrey/0000-0002-2342-6886 FU intramural research program of National Institute of Arthritis and Musculoskeletal and Skin Diseases (NIAMS); NCI [HHSN261200800001E]; Overseas Scholarship Scheme Phase II grant by the Higher Education Commission of Pakistan FX This work was supported in part by the intramural research program of National Institute of Arthritis and Musculoskeletal and Skin Diseases (NIAMS) and by the NCI under contract HHSN261200800001E, and by an Overseas Scholarship Scheme Phase II grant by the Higher Education Commission of Pakistan to A.B.A. NR 41 TC 2 Z9 2 U1 1 U2 8 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD MAY 20 PY 2014 VL 106 IS 10 BP 2134 EP 2142 DI 10.1016/j.bpj.2014.03.047 PG 9 WC Biophysics SC Biophysics GA AH7ZF UT WOS:000336353200008 PM 24853742 ER PT J AU Greene, AC Lord, SJ Tian, AW Rhodes, C Kai, H Groves, JT AF Greene, Adrienne C. Lord, Samuel J. Tian, Aiwei Rhodes, Christopher Kai, Hiroyuki Groves, Jay T. TI Spatial Organization of EphA2 at the Cell-Cell Interface Modulates Trans-Endocytosis of EphrinA1 SO BIOPHYSICAL JOURNAL LA English DT Article ID RECEPTOR TYROSINE KINASE; CLATHRIN-MEDIATED ENDOCYTOSIS; PLANAR SUPPORTED BILAYERS; MONOMERIC EPHRINA1; LIPID-BILAYERS; BREAST-CANCER; MEMBRANES; DYNAMICS; LIGAND; INHIBITION AB EphA2 is a receptor tyrosine kinase (RTK) that is sensitive to spatial and mechanical aspects of the cell's microenvironment. Misregulation of EphA2 occurs in many aggressive cancers. Although its juxtacrine signaling geometry (EphA2's cognate ligand ephrinA1 is expressed on the surface of an apposing cell) provides a mechanism by which the receptor may experience extracellular forces, this also renders the system challenging to decode. By depositing living cells on synthetic supported lipid membranes displaying ephrinA1, we have reconstituted key features of the juxtacrine EphA2-ephrinA1 signaling system while maintaining the ability to perturb the spatial and mechanical properties of the membrane-cell interface with precision. In addition, we developed a trans-endocytosis assay to monitor internalization of ephrinA1 from a supported membrane into the apposing cell using a quantitative three-dimensional fluorescence microscopy assay. Using this experimental platform to mimic a cell-cell junction, we found that the signaling complex is not efficiently internalized when lateral reorganization at the membrane-cell contact sites is physically hindered. This suggests that EphA2-ephrinA1 trans-endocytosis is sensitive to the mechanical properties of a cell's microenvironment and may have implications in physical aspects of tumor biology. C1 [Greene, Adrienne C.; Lord, Samuel J.; Tian, Aiwei; Rhodes, Christopher; Kai, Hiroyuki; Groves, Jay T.] Univ Calif Berkeley, Dept Chem, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Greene, Adrienne C.; Lord, Samuel J.; Tian, Aiwei; Rhodes, Christopher; Kai, Hiroyuki; Groves, Jay T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Greene, Adrienne C.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Rhodes, Christopher] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Groves, Jay T.] Natl Univ Singapore, Mechanobiol Inst, Singapore 117548, Singapore. RP Groves, JT (reprint author), Univ Calif Berkeley, Dept Chem, Howard Hughes Med Inst, Berkeley, CA 94720 USA. EM jtgroves@lbl.gov RI Lord, Samuel/B-2531-2008 OI Lord, Samuel/0000-0002-2785-989X FU Department of Defense National Defense Science and Engineering Graduate Fellowship; American Chemical Society Irving S. Sigal Postdoctoral Fellowship; Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; Department of Defense [W81XWH-11-1-0256]; National Institutes of Health National Cancer Institute Integrative Cancer Biology Program [1-U54-CA143836] FX We thank I. Jeena Lee for assisting with preliminary experiments, and Dr. Aaron Cheng and Dr. David Drubin for many useful discussions, help, and reagents. We also thank the Mechanobiology Institute in Singapore for providing some nanofabricated substrates. We acknowledge the financial support from Department of Defense National Defense Science and Engineering Graduate Fellowship (A.C.G.) and the American Chemical Society Irving S. Sigal Postdoctoral Fellowship (S.J.L.).; This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division and the Materials Sciences and Engineering Division of the U.S. Department of Energy under contract number DE-AC02-05CH11231; the Department of Defense W81XWH-11-1-0256; and the National Institutes of Health National Cancer Institute Integrative Cancer Biology Program grant number 1-U54-CA143836. The content is solely the responsibility of the authors and does not necessarily represent the official views of the NCI or the NIH. NR 72 TC 12 Z9 12 U1 0 U2 6 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD MAY 20 PY 2014 VL 106 IS 10 BP 2196 EP 2205 DI 10.1016/j.bpj.2014.03.043 PG 10 WC Biophysics SC Biophysics GA AH7ZF UT WOS:000336353200014 PM 24853748 ER PT J AU Guan, P Wang, GX Luo, CH Yan, KP Cairns, EJ Hu, XS AF Guan, Peng Wang, Guixin Luo, Chunhui Yan, Kangping Cairns, Elton J. Hu, Xueshan TI Comparisons of heat treatment on the electrochemical performance of different carbons for lithium-oxygen cells SO ELECTROCHIMICA ACTA LA English DT Article DE Lithium-oxygen cells; Carbon catalysis; Heat treatment; Oxygen reduction reaction; Microstructure ID LI-AIR BATTERIES; ACTIVATED CARBON; REDUCTION REACTION; CATHODE CATALYSTS; RECENT PROGRESS; NUT-SHELL; NANOTUBES; ELECTRODES; GRAPHENE; CAPACITY AB Lithium-oxygen (Li-O-2) cells are a promising power source, and carbons are an attractive non-metal catalyst for air electrodes. To improve the electrochemical performance, various carbons are heated in an inert atmosphere. It is found that heat treatment at 900 degrees C can differently improve the electrochemical performance of multiwalled carbon nanotubes (CNTs), acetylene carbon black (AB) and activated carbon (AC), but the improvement of CNTs is the most obvious. After heat treatment, the peak current density of the oxygen reduction reaction (ORR) and the 1st discharge capacity of CNTs increase similar to 30% and similar to 125%, respectively, while the charge transfer reaction resistance and the Warburg diffusion resistance decrease similar to 7.0% and similar to 11.1%, respectively. AC has the highest charge capacities and capacity retention ratio in spite of little influence by heat treatment. The possible mechanism and reasons are analyzed using different techniques. Microstructure is superior to conductivity for enhancing the rechargeability and the cyclability, and heat treatment is effective for some carbon materials in improving the electrochemical performance of Li-O-2 cells. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Guan, Peng; Wang, Guixin; Luo, Chunhui; Yan, Kangping] Sichuan Univ, Coll Chem Engn, Chengdu 610065, Peoples R China. [Cairns, Elton J.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Cairns, Elton J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Hu, Xueshan] Novolyte Technol Co Ltd, Suzhou 215123, Jiangsu, Peoples R China. RP Wang, GX (reprint author), Sichuan Univ, Coll Chem Engn, Chengdu 610065, Peoples R China. EM guixinwang1@gmail.com RI Wang, Guixin wang/I-8445-2014; Cairns, Elton/E-8873-2012 OI Wang, Guixin wang/0000-0002-4850-9207; Cairns, Elton/0000-0002-1179-7591 FU National Science Foundation of China [21206099] FX We gratefully acknowledge financial support from the National Science Foundation of China (Grant No. 21206099) and helps from the Analytical & Testing Center of Sichuan University. NR 56 TC 3 Z9 3 U1 1 U2 57 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD MAY 20 PY 2014 VL 129 BP 318 EP 326 DI 10.1016/j.electacta.2014.02.079 PG 9 WC Electrochemistry SC Electrochemistry GA AH9MI UT WOS:000336466100041 ER PT J AU Tannenbaum, MJ AF Tannenbaum, M. J. TI Highlights from BNL-RHIC 2011-2013 SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Review DE RHIC; LHC; sQGP; heavy ion collisions; jet quenching; thermal radiation; collective flow; QCD critical point; cumulants; J/Psi suppression; deconfinement ID NUCLEUS-NUCLEUS COLLISIONS; QUARK-GLUON PLASMA; ANOMALOUS MAGNETIC-MOMENT; LARGE-TRANSVERSE-MOMENTUM; HEAVY-ION COLLISIONS; PB-PB COLLISIONS; MULTIPLICITY DISTRIBUTIONS; QUANTUM CHROMODYNAMICS; ROOT-S(NN)=2.76 TEV; J/PSI SUPPRESSION AB Highlights from Brookhaven National Laboratory (BNL) and experiments at the BNL Relativistic Heavy Ion Collider (RHIC) are presented for the years 2011-2013. This review is a combination of lectures which discussed the latest results each year at a three year celebration of the 50th anniversary of the International School of Subnuclear Physics in Erice, Sicily, Italy. Since the first collisions in the year 2000, RHIC has provided nucleus-nucleus and polarized proton-proton collisions over a range of nucleonnucleon center-of-mass energies (root sNN) from 7.7 GeV to 510 GeV with nuclei from deuterium to uranium, most often gold. The objective was the discovery of the Quark Gluon Plasma, which was achieved, and the measurement of its properties, which were much different than expected, namely a "perfect fluid" of quarks and gluons with their color charges exposed rather than a gas. Topics including quenching of light and heavy quarks at large transverse momentum, thermal photons, search for a QCD critical point as well as measurements of collective flow, two-particle correlations and J/Psi suppression are presented. During this period, results from the first and subsequent heavy ion measurements at the Large Hadron Collider (LHC) at CERN became available. These confirmed and extended the RHIC discoveries and have led to ideas for new and improved measurements. C1 Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Tannenbaum, MJ (reprint author), Brookhaven Natl Lab, Dept Phys, 510c, Upton, NY 11973 USA. EM mjt@bnl.gov OI Tannenbaum, Michael/0000-0002-8840-5314 FU US Department of Energy [DE-AC02-98CH1088]; LLC [DE-AC02-98CH10886]; US Department of Energy FX This research was supported by US Department of Energy, DE-AC02-98CH1088. This manuscript has been authored by employees of Brookhaven Science Associates, LLC under Contract No. DE-AC02-98CH10886 with the US Department of Energy. The publisher by accepting the manuscript for publication acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 140 TC 3 Z9 3 U1 0 U2 8 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD MAY 20 PY 2014 VL 29 IS 13 AR 1430017 DI 10.1142/S0217751X14300178 PG 53 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AH8JM UT WOS:000336384100001 ER PT J AU Chen, Y Du, GH Feng, L Feng, SW Kong, XL Guo, F Wang, B Li, G AF Chen, Yao Du, Guohui Feng, Li Feng, Shiwei Kong, Xiangliang Guo, Fan Wang, Bing Li, Gang TI A SOLAR TYPE II RADIO BURST FROM CORONAL MASS EJECTION-CORONAL RAY INTERACTION: SIMULTANEOUS RADIO AND EXTREME ULTRAVIOLET IMAGING SO ASTROPHYSICAL JOURNAL LA English DT Article DE shock waves; Sun: corona; Sun: coronal mass ejections (CMEs); Sun: radio radiation ID NOVEMBER 2003; SOHO MISSION; SHOCK; ELECTRONS; ACCELERATION; WAVES; DIAGNOSTICS; DYNAMICS; FLARE; CMES AB Simultaneous radio and extreme ultraviolet (EUV)/white-light imaging data are examined for a solar type II radio burst occurring on 2010 March 18 to deduce its source location. Using a bow-shock model, we reconstruct the three-dimensional EUV wave front (presumably the type-II-emitting shock) based on the imaging data of the two Solar TErrestrial RElations Observatory spacecraft. It is then combined with the Nancay radio imaging data to infer the three-dimensional position of the type II source. It is found that the type II source coincides with the interface between the coronal mass ejection (CME) EUV wave front and a nearby coronal ray structure, providing evidence that the type II emission is physically related to the CME-ray interaction. This result, consistent with those of previous studies, is based on simultaneous radio and EUV imaging data for the first time. C1 [Chen, Yao; Du, Guohui; Feng, Shiwei; Kong, Xiangliang; Wang, Bing] Shandong Univ, Shandong Prov Key Lab Opt Astron & Solar Terr Env, Weihai 264209, Peoples R China. [Chen, Yao; Du, Guohui; Feng, Shiwei; Kong, Xiangliang; Wang, Bing] Shandong Univ, Inst Space Sci, Weihai 264209, Peoples R China. [Feng, Li] Chinese Acad Sci, Purple Mt Observ, Key Lab Dark Matter & Space Astron, Nanjing 210008, Jiangsu, Peoples R China. [Guo, Fan] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Li, Gang] Univ Alabama, Dept Space Sci, Huntsville, AL 35899 USA. [Li, Gang] Univ Alabama, CSPAR, Huntsville, AL 35899 USA. RP Chen, Y (reprint author), Shandong Univ, Shandong Prov Key Lab Opt Astron & Solar Terr Env, Weihai 264209, Peoples R China. EM yaochen@sdu.edu.cn RI Kong, Xiangliang/D-9855-2012; Chen, Yao/B-7255-2011; Guo, Fan/H-1723-2013; Feng, Li/G-2100-2015; OI Guo, Fan/0000-0003-4315-3755 FU NSF [ATM0847719, AGS1135432]; [NSBRSF 2012CB825601]; [NNSFC 41274175]; [41331068]; [NNSFC 11003047]; [11233008]; [BK2012889] FX We thank the referee for constructive comments. This work was supported by grants NSBRSF 2012CB825601, NNSFC 41274175, and 41331068. Li Feng's work was supported by grants NNSFC 11003047, 11233008, and BK2012889. Gang Li's work at UAHuntsivlle was supported by NSF grants ATM0847719 and AGS1135432. NR 41 TC 15 Z9 16 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2014 VL 787 IS 1 AR 59 DI 10.1088/0004-637X/787/1/59 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH2AX UT WOS:000335924200059 ER PT J AU Islam, T AF Islam, Tanim TI THE COLLISIONLESS MAGNETOVISCOUS-THERMAL INSTABILITY SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disk; Galaxy: center; instabilities; magnetic fields; magnetohydrodynamics (MHD); plasmas ID SAGITTARIUS-A-ASTERISK; FLUID KINETIC DESCRIPTION; MAGNETOROTATIONAL INSTABILITY; MAGNETIZED DISKS; PLASMA MICROINSTABILITIES; LINEAR-POLARIZATION; ACCRETION DISKS; SIMULATIONS; TRANSPORT; EQUILIBRIUM AB It is likely that nearly all central galactic massive and supermassive black holes are nonradiative: their accretion luminosities are orders of magnitude below what can be explained by efficient black hole accretion within their ambient environments. These objects, of which Sagittarius A* is the best-known example, are also dilute (mildly collisional to highly collisionless) and optically thin. In order for accretion to occur, magnetohydrodynamic (MHD) instabilities must develop that not only transport angular momentum, but also gravitational energy generated through matter infall, outward. A class of new magnetohydrodynamical fluid instabilities-the magnetoviscous-thermal instability (MVTI)-was found to transport angular momentum and energy along magnetic field lines through large (fluid) viscosities and thermal conductivities. This paper describes the analog to the MVTI, the collisionless MVTI (CMVTI), that similarly transports energy and angular momentum outward, expected to be important in describing the flow properties of hot, dilute, and radiatively inefficient accretion flows around black holes. We construct a local equilibrium for MHD stability analysis in this differentially rotating disk. We then find and characterize specific instabilities expected to be important in describing their flow properties, and show their qualitative similarities to instabilities derived using the fluid formalism. We conclude with further work needed in modeling this class of accretion flow. C1 Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Islam, T (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. EM islam5@llnl.gov NR 43 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2014 VL 787 IS 1 AR 53 DI 10.1088/0004-637X/787/1/53 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH2AX UT WOS:000335924200053 ER PT J AU Marinucci, A Matt, G Miniutti, G Guainazzi, M Parker, ML Brenneman, L Fabian, AC Kara, E Arevalo, P Ballantyne, DR Boggs, SE Cappi, M Christensen, FE Craig, WW Elvis, M Hailey, CJ Harrison, FA Reynolds, CS Risaliti, G Stern, DK Walton, DJ Zhang, W AF Marinucci, A. Matt, G. Miniutti, G. Guainazzi, M. Parker, M. L. Brenneman, L. Fabian, A. C. Kara, E. Arevalo, P. Ballantyne, D. R. Boggs, S. E. Cappi, M. Christensen, F. E. Craig, W. W. Elvis, M. Hailey, C. J. Harrison, F. A. Reynolds, C. S. Risaliti, G. Stern, D. K. Walton, D. J. Zhang, W. TI THE BROADBAND SPECTRAL VARIABILITY OF MCG-6-30-15 OBSERVED BY NUSTAR AND XMM-NEWTON SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; galaxies: active; galaxies: Seyfert; X-rays: individual (MCG-6-30-015) ID ACTIVE GALACTIC NUCLEI; 1 GALAXY MCG-6-30-15; X-RAY VARIABILITY; K-ALPHA LINE; PHOTON IMAGING CAMERA; DUSTY WARM ABSORBER; BLACK-HOLE; IRON LINE; SUZAKU OBSERVATIONS; SEYFERT-1 GALAXIES AB MCG-6-30-15, at a distance of 37 Mpc (z = 0.008), is the archetypical Seyfert 1 galaxy showing very broad Fe K alpha emission. We present results from a joint NuSTAR and XMM-Newton observational campaign that, for the first time, allows a sensitive, time-resolved spectral analysis from 0.35 keV up to 80 keV. The strong variability of the source is best explained in terms of intrinsic X-ray flux variations and in the context of the light-bending model: the primary, variable emission is reprocessed by the accretion disk, which produces secondary, less variable, reflected emission. The broad Fe K alpha profile is, as usual for this source, well explained by relativistic effects occurring in the innermost regions of the accretion disk around a rapidly rotating black hole. We also discuss the alternative model in which the broadening of the Fe K alpha is due to the complex nature of the circumnuclear absorbing structure. Even if this model cannot be ruled out, it is disfavored on statistical grounds. We also detected an occultation event likely caused by broad-line region clouds crossing the line of sight. C1 [Marinucci, A.; Matt, G.] Univ Rome, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Marinucci, A.; Miniutti, G.] ESAC, Dep Astrofis, Ctr Astrobiol CSIC INTA, Madrid, Spain. [Guainazzi, M.] European Space Astron Ctr ESA, E-28080 Madrid, Spain. [Parker, M. L.; Fabian, A. C.; Kara, E.] Univ Cambridge, Inst Astron, Cambridge CB3 OHA, England. [Brenneman, L.; Elvis, M.; Risaliti, G.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Arevalo, P.] Pontificia Univ Catolica Chile, Inst Astrofis, Santiago 22, Chile. [Arevalo, P.] Univ Valparaiso, Inst Fis & Astron, Valparaiso, Chile. [Ballantyne, D. R.] Georgia Inst Technol, Sch Phys, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Boggs, S. E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Cappi, M.] IASF Bologna, INAF, I-40129 Bologna, Italy. [Christensen, F. E.] Danish Tech Univ, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Craig, W. W.; Hailey, C. J.; Walton, D. J.] Columbia Univ, New York, NY 10027 USA. [Harrison, F. A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Reynolds, C. S.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Risaliti, G.] INAF Osservatorio Astrofis Arcetri, I-50125 Florence, Italy. [Stern, D. K.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Marinucci, A (reprint author), Univ Rome, Dipartimento Matemat & Fis, Via Vasca Navale 84, I-00146 Rome, Italy. RI Miniutti, Giovanni/L-2721-2014; Boggs, Steven/E-4170-2015; Cappi, Massimo/F-4813-2015 OI Miniutti, Giovanni/0000-0003-0707-4531; Cappi, Massimo/0000-0001-6966-8920; Boggs, Steven/0000-0001-9567-4224; Risaliti, Guido/0000-0002-3556-977X; FU Fondazione Angelo Della Riccia.; Italian Space Agency [ASI/INAF I/037/12/0-011/13]; European Union Seventh Framework Programme (FP7) [312789]; Anillo [ACT1101]; NASA [NNG08FD60C]; California Institute of Technology; National Aeronautics and Space Administration.; NuSTAR Operations, Software, and Calibration; NuSTAR Data Analysis Software (NuSTARDAS); ASI Science Data Center (ASDC, Italy); California Institute of Technology (USA) FX A. M. acknowledges financial support from Fondazione Angelo Della Riccia. A. M. and G. M. acknowledge financial support from Italian Space Agency under grant ASI/INAF I/037/12/0-011/13. A. M., G. Matt, G. Miniutti, A. C. F., and E. K. acknowledge financial support from the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 312789. P. A. acknowledges financial support from Anillo ACT1101. This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). NR 76 TC 26 Z9 26 U1 2 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2014 VL 787 IS 1 AR 83 DI 10.1088/0004-637X/787/1/83 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH2AX UT WOS:000335924200083 ER PT J AU Mesler, RA Whalen, DJ Smidt, J Fryer, CL Lloyd-Ronning, NM Pihlstrom, YM AF Mesler, R. A. Whalen, Daniel J. Smidt, Joseph Fryer, Chris L. Lloyd-Ronning, N. M. Pihlstroem, Y. M. TI THE FIRST GAMMA-RAY BURSTS IN THE UNIVERSE SO ASTROPHYSICAL JOURNAL LA English DT Article DE early universe; galaxies: high-redshift; gamma-ray burst: general; hydrodynamics; radiative transfer; stars: early-type; stars: winds, outflows; supernovae: general ID PAIR-INSTABILITY SUPERNOVAE; SUPERMASSIVE BLACK-HOLES; RELATIVISTIC BLAST WAVES; PRIMORDIAL HII-REGIONS; METAL-POOR STARS; POPULATION-III; HIGH-REDSHIFT; LIGHT CURVES; PROTOSTELLAR FEEDBACK; SYNCHROTRON EMISSION AB Gamma-ray bursts (GRBs) are the ultimate cosmic lighthouses, capable of illuminating the universe at its earliest epochs. Could such events probe the properties of the first stars at z similar to 20, the end of the cosmic Dark Ages? Previous studies of Population III (Pop III) GRBs only considered explosions in the diffuse relic H II regions of their progenitors or bursts that are far more energetic than those observed to date. However, the processes that produce GRBs at the highest redshifts likely reset their local environments, creating much more complicated structures than those in which relativistic jets have been modeled so far. These structures can greatly affect the luminosity of the afterglow and hence the redshift at which it can be detected. We have now simulated Pop III GRB afterglows in H II regions, winds, and dense shells ejected by the star during the processes that produce the burst. We find that GRBs with E-iso,E-gamma = 10(51)-10(53) erg will be visible at z greater than or similar to 20 to the next generation of near infrared and radio observatories. In many cases, the environment of the burst, and hence progenitor type, can be inferred from the afterglow light curve. Although some Pop III GRBs are visible to Swift and the Very Large Array now, the optimal strategy for their detection will be future missions like the proposed EXIST and JANUS missions with large survey areas and onboard X-ray and infrared telescopes that can track their near-infrared flux from the moment of the burst, thereby identifying their redshifts. C1 [Mesler, R. A.; Pihlstroem, Y. M.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Whalen, Daniel J.; Smidt, Joseph; Fryer, Chris L.; Lloyd-Ronning, N. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Whalen, Daniel J.] Heidelberg Univ, Zentrum Astron, Inst Theoret Astrophys, D-69120 Heidelberg, Germany. RP Mesler, RA (reprint author), Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. FU LANL IGPP [10-150]; Baden-Wurttemberg-Stiftung via the programme Internationale Spitzenforschung II [P-LS-SPII/18]; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX R.M. was supported by LANL IGPP grant 10-150. D.J.W. acknowledges support from the Baden-Wurttemberg-Stiftung by contract research via the programme Internationale Spitzenforschung II (grant P-LS-SPII/18). Work at LANL was done under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. All ZEUS-MP simulations were performed with allocations from Institutional Computing (IC) on the Pinto cluster at LANL. NR 131 TC 17 Z9 17 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2014 VL 787 IS 1 AR 91 DI 10.1088/0004-637X/787/1/91 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH2AX UT WOS:000335924200091 ER PT J AU Morley, CV Marley, MS Fortney, JJ Lupu, R Saumon, D Greene, T Lodders, K AF Morley, Caroline V. Marley, Mark S. Fortney, Jonathan J. Lupu, Roxana Saumon, Didier Greene, Tom Lodders, Katharina TI WATER CLOUDS IN Y DWARFS AND EXOPLANETS SO ASTROPHYSICAL JOURNAL LA English DT Article DE brown dwarfs; planets and satellites: atmospheres; planets and satellites: detection; stars: atmospheres ID EXTRASOLAR GIANT PLANETS; COOLEST BROWN DWARFS; COLLISION-INDUCED ABSORPTION; HR 8799 PLANETS; T-DWARFS; ATMOSPHERIC CHEMISTRY; CHEMICAL-EQUILIBRIUM; MODEL ATMOSPHERES; CARBON-MONOXIDE; L/T TRANSITION AB The formation of clouds affects brown dwarf and planetary atmospheres of nearly all effective temperatures. Iron and silicate condense in L dwarf atmospheres and dissipate at the L/T transition. Minor species such as sulfides and salts condense in mid- to late T dwarfs. For brown dwarfs below T-eff similar to 450 K, water condenses in the upper atmosphere to form ice clouds. Currently, over a dozen objects in this temperature range have been discovered, and few previous theoretical studies have addressed the effect of water clouds on brown dwarf or exoplanetary spectra. Here we present a new grid of models that include the effect of water cloud opacity. We find that they become optically thick in objects below T-eff similar to 350-375 K. Unlike refractory cloud materials, water-ice particles are significantly nongray absorbers; they predominantly scatter at optical wavelengths through the J band and absorb in the infrared with prominent features, the strongest of which is at 2.8 mu m. H2O, NH3, CH4, and H-2 CIA are dominant opacity sources; less abundant species may also be detectable, including the alkalis, H2S, and PH3. PH3, which has been detected in Jupiter, is expected to have a strong signature in the mid-infrared at 4.3 mu m in Y dwarfs around T-eff = 450 K; if disequilibrium chemistry increases the abundance of PH3, it may be detectable over a wider effective temperature range than models predict. We show results incorporating disequilibrium nitrogen and carbon chemistry and predict signatures of low gravity in planetary mass objects. Finally, we make predictions for the observability of Y dwarfs and planets with existing and future instruments, including the James Webb Space Telescope and Gemini Planet Imager. C1 [Morley, Caroline V.; Fortney, Jonathan J.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Marley, Mark S.; Lupu, Roxana; Greene, Tom] NASA, Ames Res Ctr, Naval Air Stn, Mountain View, CA 94035 USA. [Saumon, Didier] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lodders, Katharina] Washington Univ, St Louis, MO 63130 USA. RP Morley, CV (reprint author), Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. EM cmorley@ucolick.org RI Marley, Mark/I-4704-2013; Lupu, Roxana/P-9060-2014; OI Lupu, Roxana/0000-0003-3444-5908; Marley, Mark/0000-0002-5251-2943 FU NSF [AST-1312545]; NASA Astrophysics Theory [NNH11AQ54I]; NASA Astrophysics Theory and Origins Programs FX The authors acknowledge Gregory Mace, Michael Liu, and the anonymous referee for comments that improved the paper. We also thank Andy Skemer for information on the observing capabilities of the LBT. We also acknowledge the Database of Ultracool Parallaxes maintained by Trent Dupuy. J.J.F. acknowledges the support of NSF grant AST-1312545, D.S. acknowledges the support of NASA Astrophysics Theory grant NNH11AQ54I, and M.S.M. and K.L. acknowledge the support of the NASA Astrophysics Theory and Origins Programs. We thank Ian Crossfield for identifying an error in a figure within a previous version of this manuscript. NR 102 TC 40 Z9 40 U1 1 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2014 VL 787 IS 1 AR 78 DI 10.1088/0004-637X/787/1/78 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH2AX UT WOS:000335924200078 ER PT J AU Naud, ME Artigau, E Malo, L Albert, L Doyon, R Lafreniere, D Gagne, J Saumon, D Morley, CV Allard, F Homeier, D Beichman, CA Gelino, CR Boucher, A AF Naud, Marie-Eve Artigau, Etienne Malo, Lison Albert, Loic Doyon, Rene Lafreniere, David Gagne, Jonathan Saumon, Didier Morley, Caroline V. Allard, France Homeier, Derek Beichman, Charles A. Gelino, Christopher R. Boucher, Anne TI DISCOVERY OF A WIDE PLANETARY-MASS COMPANION TO THE YOUNG M3 STAR GU PSC SO ASTROPHYSICAL JOURNAL LA English DT Article DE infrared: planetary systems; planetary systems; planets and satellites: detection; stars: imaging; stars: individual (GU Psc); stars: low-mass ID VERY-LOW-MASS; DIGITAL SKY SURVEY; ANGULAR-MOMENTUM EVOLUTION; COLOR-MAGNITUDE DIAGRAMS; BRIGHT SOURCE CATALOG; DORADUS MOVING GROUP; INFRARED FILTER SET; T-DWARF TRANSITION; GAS GIANT PLANETS; BROWN DWARFS AB We present the discovery of a comoving planetary-mass companion similar to 42 '' (similar to 2000AU) from a young M3 star, GU Psc, a likely member of the young AB Doradus Moving Group (ABDMG). The companion was first identified via its distinctively red i - z color (> 3.5) through a survey made with Gemini-S/GMOS. Follow-up Canada-France-Hawaii Telescope/WIRCam near-infrared (NIR) imaging, Gemini-N/GNIRS NIR spectroscopy and Wide-field Infrared Survey Explorer photometry indicate a spectral type of T3.5 +/- 1 and reveal signs of low gravity which we attribute to youth. Keck/Adaptive Optics NIR observations did not resolve the companion as a binary. A comparison with atmosphere models indicates T-eff = 1000-1100 K and log g = 4.5-5.0. Based on evolution models, this temperature corresponds to a mass of 9-13 M-Jup for the age of ABDMG (70-130 Myr). The relatively well-constrained age of this companion and its very large angular separation to its host star will allow its thorough characterization and will make it a valuable comparison for planetary-mass companions that will be uncovered by forthcoming planet-finder instruments such as Gemini Planet Imager and SPHERE. C1 [Naud, Marie-Eve; Artigau, Etienne; Malo, Lison; Albert, Loic; Doyon, Rene; Lafreniere, David; Gagne, Jonathan; Boucher, Anne] Univ Montreal, Dept Phys, Montreal, PQ H3C 3J7, Canada. [Naud, Marie-Eve; Artigau, Etienne; Malo, Lison; Albert, Loic; Doyon, Rene; Lafreniere, David; Gagne, Jonathan; Boucher, Anne] Univ Montreal, Observ Mt Megantic, Montreal, PQ H3C 3J7, Canada. [Saumon, Didier] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Morley, Caroline V.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Allard, France; Homeier, Derek] Univ Lyon, Ecole Normale Super Lyon, UMR CNRS 5574, Ctr Rech Astrophys Lyon, F-69364 Lyon 07, France. [Beichman, Charles A.; Gelino, Christopher R.] CALTECH, Ctr Infrared Proc & Anal, Pasadena, CA 91125 USA. [Gelino, Christopher R.] CALTECH, NASA, Exoplanet Sci Inst, Pasadena, CA 91125 USA. RP Naud, ME (reprint author), Univ Montreal, Dept Phys, CP 6128, Montreal, PQ H3C 3J7, Canada. EM naud@astro.umontreal.ca OI Homeier, Derek/0000-0002-8546-9128; Gagne, Jonathan/0000-0002-2592-9612; Boucher, Anne/0000-0001-9427-1642; Lafreniere, David/0000-0002-6780-4252 FU Natural Sciences and Engineering Research Council (NSERC) of Canada; Fond de Recherche Quebecois-Nature et Technologie (FRQNT; Quebec); NASA [NNH11AQ54I]; European Research Council under the European Community [247060]; Gemini-S/PHOENIX: program [GS-2010B-Q-89]; Gemini-S/GMOS: program [GS-2011B-Q-74]; Gemini-S/NICI [GS-2011BQ-24, GS-2012B-Q-54]; Gemini-N/GNIRS: program [GN-2012B-Q-58]; European Southern Observatory Very Large Telescope under program [087.D-0510, 091.D-0641]; Universite de Montreal; Universite Laval and the Canada Foundation for Innovation; W.M. Keck Foundation; NASA InfraRed Telescope Facility, with SpeX [2013B025]; National Aeronautics and Space Administration, from the Two Micron All Sky Survey; National Aeronautics and Space Administration; National Science Foundation, of the NASA's Astrophysics Data System Bibliographic Services, SIMBAD database, the VizieR catalog access tool and the SIMBAD database operated at CDS, Strasbourg, France FX We would like to thank the anonymous referee for constructive comments and suggestions that greatly improved the overall quality of the paper. This work was financially supported by the Natural Sciences and Engineering Research Council (NSERC) of Canada and the Fond de Recherche Quebecois-Nature et Technologie (FRQNT; Quebec). D.S. is supported by NASA Astrophysics Theory grant NNH11AQ54I. D.H. acknowledges support from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013 Grant Agreement no. 247060). Based on observations obtained at the Gemini Observatory (Gemini-S/PHOENIX: program GS-2010B-Q-89, Gemini-S/GMOS: program GS-2011B-Q-74, Gemini-S/NICI: programs GS-2011BQ-24 and GS-2012B-Q-54 and Gemini-N/GNIRS: program GN-2012B-Q-58), which is operated by the Association of Universities for Research in Astronomy, Inc., under a cooperative agreement with the NSF on behalf of the Gemini partnership: the National Science Foundation (United States), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), Ministerio da Cincia, Tecnologia e Inovacao (Brazil) and Ministerio de Ciencia, Tecnologa e Innovacin Productiva (Argentina). Observations were also collected at CFHT with WIRCam (run IDs: 11BC20 and 12BC20) and ESPaDOnS (run ID: 12AC23), at the European Southern Observatory Very Large Telescope under program ID: 087.D-0510, 091.D-0641 and on CPAPIR infrared camera, at Observatoire du mont Megantic, which is funded by the Universite de Montreal, Universite Laval and the Canada Foundation for Innovation. Some of the data presented herein were obtained at the W.M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W.M. Keck Foundation. The authors recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate to have the opportunity to conduct observations from this mountain. Finally, we also obtained data from the NASA InfraRed Telescope Facility, with SpeX, under the program number 2013B025. This publication makes use of data products from the Wide-field Infrared Survey Explorer, which is a joint project of the University of California, Los Angeles, and the Jet Propulsion Laboratory/ California Institute of Technology, funded by the National Aeronautics and Space Administration, from the Two Micron All Sky Survey, which is a joint project of the University of Massachusetts and the Infrared Processing and Analysis Center, and funded by the National Aeronautics and Space Administration and the National Science Foundation, of the NASA's Astrophysics Data System Bibliographic Services, SIMBAD database, the VizieR catalog access tool and the SIMBAD database operated at CDS, Strasbourg, France. The BT-Settl model atmospheres have been computed at the Pole Scientifique de Modelisation Numerique of the ENS de Lyon, and at the Gesellschaft fur Wissenschaftliche Datenverarbeitung Gottingen in co-operation with the Institut fur Astrophysik Gottingen. This publication has made use of the L and T dwarf data archive, http://staff.gemini.edu/similar to sleggett/LTdata.html. NR 147 TC 39 Z9 39 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2014 VL 787 IS 1 AR 5 DI 10.1088/0004-637X/787/1/5 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH2AX UT WOS:000335924200005 ER PT J AU Gnedin, NY Tasker, EJ Fujimoto, Y AF Gnedin, Nickolay Y. Tasker, Elizabeth J. Fujimoto, Yusuke TI EMERGENCE OF THE KENNICUTT-SCHMIDT RELATION FROM THE SMALL-SCALE SFR-DENSITY RELATION SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE cosmology: theory; galaxies: evolution; galaxies: formation; methods: numerical; stars: formation ID STAR-FORMATION RELATION; GIANT MOLECULAR CLOUDS; NEARBY DISK GALAXIES; GAS DEPLETION TIME; KPC SCALES; TURBULENCE; ORIGIN; II.; LAW AB We use simulations of isolated galaxies with a few parsec resolution to explore the connection between the small-scale star formation rate (SFR)-gas density relation and the induced large-scale correlation between the SFR surface density and the surface density of the molecular gas (the Kennicutt-Schmidt relation). We find that, in the simulations, a power-law small-scale "star formation law" directly translates into an identical power-law Kennicutt-Schmidt relation. If this conclusion holds in the reality as well, it implies that the observed approximately linear Kennicutt-Schmidt relation must reflect the approximately linear small-scale "star formation law." C1 [Gnedin, Nickolay Y.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gnedin, Nickolay Y.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Gnedin, Nickolay Y.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Tasker, Elizabeth J.; Fujimoto, Yusuke] Hokkaido Univ, Fac Sci, Dept Phys, Kita Ku, Sapporo, Hokkaido 0600810, Japan. RP Gnedin, NY (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM gnedin@fnal.gov NR 26 TC 2 Z9 2 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD MAY 20 PY 2014 VL 787 IS 1 AR L7 DI 10.1088/2041-8205/787/1/L7 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH3PE UT WOS:000336035800007 ER PT J AU Bechtel, HA Muller, EA Olmon, RL Martin, MC Raschke, MB AF Bechtel, Hans A. Muller, Eric A. Olmon, Robert L. Martin, Michael C. Raschke, Markus B. TI Ultrabroadband infrared nanospectroscopic imaging SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE nano-FTIR; chemical identification; bioimaging ID NEAR-FIELD SPECTROSCOPY; SYNCHROTRON-RADIATION; MICROSCOPY; LIGHT; RESOLUTION; SCATTERING; SCALE; SPECTROMICROSCOPY; ABSORPTION; CHEMISTRY AB Characterizing and ultimately controlling the heterogeneity underlying biomolecular functions, quantum behavior of complex matter, photonic materials, or catalysis requires large-scale spectroscopic imaging with simultaneous specificity to structure, phase, and chemical composition at nanometer spatial resolution. However, as with any ultrahigh spatial resolution microscopy technique, the associated demand for an increase in both spatial and spectral bandwidth often leads to a decrease in desired sensitivity. We overcome this limitation in infrared vibrational scattering-scanning probe near-field optical microscopy using synchrotron midinfrared radiation. Tip-enhanced localized light-matter interaction is induced by low-noise, broadband, and spatially coherent synchrotron light of high spectral irradiance, and the near-field signal is sensitively detected using heterodyne interferometric amplification. We achieve sub-40-nm spatially resolved, molecular, and phonon vibrational spectroscopic imaging, with rapid spectral acquisition, spanning the full midinfrared (700-5,000 cm(-1)) with few cm(-1) spectral resolution. We demonstrate the performance of synchrotron infrared nanospectroscopy on semiconductor, biomineral, and protein nanostructures, providing vibrational chemical imaging with subzeptomole sensitivity. C1 [Bechtel, Hans A.; Martin, Michael C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source Div, Berkeley, CA 94720 USA. [Muller, Eric A.; Olmon, Robert L.; Raschke, Markus B.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Muller, Eric A.; Olmon, Robert L.; Raschke, Markus B.] Univ Colorado, Dept Chem, Boulder, CO 80309 USA. [Muller, Eric A.; Olmon, Robert L.; Raschke, Markus B.] Univ Colorado, JILA, Boulder, CO 80309 USA. [Muller, Eric A.; Olmon, Robert L.; Raschke, Markus B.] NIST, Boulder, CO 80309 USA. RP Bechtel, HA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source Div, Berkeley, CA 94720 USA. EM habechtel@lbl.gov; mcmartin@lbl.gov; markus.raschke@colorado.edu RI Muller, Eric/J-2161-2012; Raschke, Markus/F-8023-2013; Foundry, Molecular/G-9968-2014 OI Muller, Eric/0000-0002-9629-1767; FU Berkeley Synchrotron Infrared Structural Biology (BSISB) program; Office of Science, Office of Basic Energy Sciences the US Department of Energy (DOE) [DE-AC02-05CH11231]; Office of Biological and Environmental Research through the US Department of Energy (DOE) [DE-AC02-05CH11231]; US DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-12ER46893]; DOE Office of Biological and Environmental Research at Pacific Northwest National Laboratory (PNNL); US DOE [DEAC06-76RL01830] FX The authors thank Gloria K. Oliver for the synthesis and provision of peptide loop-displaying peptoid nanosheets, which was performed at The Molecular Foundry (TMF), Sun Choi for providing dried protein samples, which was supported by the Berkeley Synchrotron Infrared Structural Biology (BSISB) program, and Pupa Gilbert for providing the shell sample. The authors also thank Andrew Jones and Erik Josberger for contributions to the modifications of the AFM, as well as Jaroslaw Syzdek and Benjamin Pollard for helpful discussions. The ALS and TMF are supported by the Director, Office of Science, Office of Basic Energy Sciences, and the BSISB is supported by the Office of Biological and Environmental Research, all through the US Department of Energy (DOE) under Contract DE-AC02-05CH11231. A portion of the research was supported by the US DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-FG02-12ER46893 (to E.A.M., R.L.O., and M.B.R.). Funding was provided by a partner proposal with the Environmental Molecular Sciences Laboratory, a national scientific user facility from the DOE Office of Biological and Environmental Research at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the US DOE under Contract DEAC06-76RL01830. NR 51 TC 59 Z9 60 U1 14 U2 103 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 20 PY 2014 VL 111 IS 20 BP 7191 EP 7196 DI 10.1073/pnas.1400502111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH5KP UT WOS:000336168100019 PM 24803431 ER PT J AU Kaushal, PS Sharma, MR Booth, TM Haque, EM Tung, CS Sanbonmatsu, KY Spremulli, LL Agrawal, RK AF Kaushal, Prem S. Sharma, Manjuli R. Booth, Timothy M. Haque, Emdadul M. Tung, Chang-Shung Sanbonmatsu, Karissa Y. Spremulli, Linda L. Agrawal, Rajendra K. TI Cryo-EM structure of the small subunit of the mammalian mitochondrial ribosome SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE mammalian mitochondrial ribosomal SSU; cryo-electron microscopy; mito-12S rRNA; mammalian MRPs ID ANGSTROM RESOLUTION; TRANSLATIONAL APPARATUS; CRYOELECTRON MICROSCOPY; PROTEIN-SYNTHESIS; RNA; IDENTIFICATION; DISEASES; FEATURES; REVEALS; MEMBERS AB The mammalian mitochondrial ribosomes (mitoribosomes) are responsible for synthesizing 13 membrane proteins that form essential components of the complexes involved in oxidative phosphorylation or ATP generation for the eukaryotic cell. The mammalian 55S mitoribosome contains significantly smaller rRNAs and a large mass of mitochondrial ribosomal proteins (MRPs), including large mito-specific amino acid extensions and insertions in MRPs that are homologous to bacterial ribosomal proteins and an additional 35 mito-specific MRPs. Here we present the cryo-EM structure analysis of the small (28S) subunit (SSU) of the 55S mitoribosome. We find that the mito-specific extensions in homologous MRPs generally are involved in inter-MRP contacts and in contacts with mito-specific MRPs, suggesting a stepwise evolution of the current architecture of the mitoribosome. Although most of the mito-specific MRPs and extensions of homologous MRPs are situated on the peripheral regions, they also contribute significantly to the formation of linings of the mRNA and tRNA paths, suggesting a tailor-made structural organization of the mito-SSU for the recruitment of mito-specific mRNAs, most of which do not possess a 5' leader sequence. In addition, docking of previously published coordinates of the large (39S) subunit (LSU) into the cryo-EM map of the 55S mitoribosome reveals that mito-specific MRPs of both the SSU and LSU are involved directly in the formation of six of the 15 intersubunit bridges. C1 [Kaushal, Prem S.; Sharma, Manjuli R.; Booth, Timothy M.; Agrawal, Rajendra K.] New York State Dept Hlth, Wadsworth Ctr, Div Translat Med, Albany, NY 12201 USA. [Haque, Emdadul M.; Spremulli, Linda L.] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA. [Tung, Chang-Shung; Sanbonmatsu, Karissa Y.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Agrawal, Rajendra K.] SUNY Albany, Sch Publ Hlth, Dept Biomed Sci, Albany, NY 12222 USA. RP Agrawal, RK (reprint author), New York State Dept Hlth, Wadsworth Ctr, Div Translat Med, Albany, NY 12201 USA. EM agrawal@wadsworth.org FU National Institutes of Health [R01 GM061576, R01 GM072686] FX We thank the staff of the New York Structural Biology Center for help with cryo-EM data collection on their 300 kV FEG JEOL electron microscope; Kae Yokoyama for help with manual screening of particle images; Nilesh Banavali for helpful discussions on MRP modeling; and Wadsworth Center computing facilities for all image processing and MDFF simulations. This work was supported by National Institutes of Health Grants R01 GM061576 (to R. K. A.) and R01 GM072686 (to K.Y.S.). NR 44 TC 21 Z9 21 U1 3 U2 15 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 20 PY 2014 VL 111 IS 20 BP 7284 EP 7289 DI 10.1073/pnas.1401657111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH5KP UT WOS:000336168100035 PM 24799711 ER PT J AU Huang, B Deng, HX Lee, H Yoon, M Sumpter, BG Liu, F Smith, SC Wei, SH AF Huang, Bing Deng, Hui-Xiong Lee, Hoonkyung Yoon, Mina Sumpter, Bobby G. Liu, Feng Smith, Sean C. Wei, Su-Huai TI Exceptional Optoelectronic Properties of Hydrogenated Bilayer Silicene SO PHYSICAL REVIEW X LA English DT Article ID HEXAGONAL BORON-NITRIDE; SOLAR-CELL; 1ST-PRINCIPLES CALCULATION; TEMPERATURE-DEPENDENCE; GRAPHENE; EFFICIENCY; STATE; SEMICONDUCTORS; PHOTOVOLTAICS; ADSORPTION AB Silicon is arguably the best electronic material, but it is not a good optoelectronic material. By employing first-principles calculations and the cluster-expansion approach, we discover that hydrogenated bilayer silicene (BS) shows promising potential as a new kind of optoelectronic material. Most significantly, hydrogenation converts the intrinsic BS, a strongly indirect semiconductor, into a direct-gap semiconductor with a widely tunable band gap. At low hydrogen concentrations, four ground states of single-and double-sided hydrogenated BS are characterized by dipole-allowed direct (or quasidirect) band gaps in the desirable range from 1 to 1.5 eV, suitable for solar applications. At high hydrogen concentrations, three well-ordered double-sided hydrogenated BS structures exhibit direct (or quasidirect) band gaps in the color range of red, green, and blue, affording white light-emitting diodes. Our findings open opportunities to search for new silicon-based light-absorption and light-emitting materials for earth-abundant, high-efficiency, optoelectronic applications. C1 [Huang, Bing; Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Huang, Bing; Yoon, Mina; Sumpter, Bobby G.; Smith, Sean C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Deng, Hui-Xiong] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China. [Lee, Hoonkyung] Konkuk Univ, Sch Phys, Div Quantum Phases & Devices, Seoul 143701, South Korea. [Liu, Feng] Univ Utah, Dept Mat Sci & Engn, Salt Lake City, UT 84112 USA. RP Huang, B (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM huangb@ornl.gov; suhuai.wei@nrel.gov RI Smith, Sean/H-5003-2015; Sumpter, Bobby/C-9459-2013; Yoon, Mina/A-1965-2016 OI Smith, Sean/0000-0002-5679-8205; Sumpter, Bobby/0000-0001-6341-0355; Yoon, Mina/0000-0002-1317-3301 FU U.S. Department of Energy [DE-AC36-08GO28308]; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Basic Science Research Program through the National Research Foundation of Korea - Ministry of Education, Science and Technology [KRF-2012R1A1A1013124] FX The research at NREL is sponsored by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. The research at ORNL is sponsored by the the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. H.L. is supported by the Basic Science Research Program (Grant No. KRF-2012R1A1A1013124) through the National Research Foundation of Korea, funded by the Ministry of Education, Science and Technology. All the calculations were carried out at the DOE REDMESA and NERSC facilities. NR 68 TC 27 Z9 29 U1 4 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAY 19 PY 2014 VL 4 IS 2 AR 021029 DI 10.1103/PhysRevX.4.021029 PG 12 WC Physics, Multidisciplinary SC Physics GA CB3TV UT WOS:000349552700001 ER PT J AU Haendel, MA Balhoff, JP Bastian, FB Blackburn, DC Blake, JA Bradford, Y Comte, A Dahdul, WM Dececchi, TA Druzinsky, RE Hayamizu, TF Ibrahim, N Lewis, SE Mabee, PM Niknejad, A Robinson-Rechavi, M Sereno, PC Mungall, CJ AF Haendel, Melissa A. Balhoff, James P. Bastian, Frederic B. Blackburn, David C. Blake, Judith A. Bradford, Yvonne Comte, Aurelie Dahdul, Wasila M. Dececchi, Thomas A. Druzinsky, Robert E. Hayamizu, Terry F. Ibrahim, Nizar Lewis, Suzanna E. Mabee, Paula M. Niknejad, Anne Robinson-Rechavi, Marc Sereno, Paul C. Mungall, Christopher J. TI Unification of multi-species vertebrate anatomy ontologies for comparative biology in Uberon SO JOURNAL OF BIOMEDICAL SEMANTICS LA English DT Article DE Evolutionary biology; Morphological variation; Phenotype; Semantic integration; Bio-ontology ID DEVELOPMENTAL ANATOMY; EVOLUTIONARY; SKELETON; LIMB; INFORMATICS; ZEBRAFISH; DATABASE; ORIGIN; GENES AB Background: Elucidating disease and developmental dysfunction requires understanding variation in phenotype. Single-species model organism anatomy ontologies (ssAOs) have been established to represent this variation. Multi-species anatomy ontologies (msAOs; vertebrate skeletal, vertebrate homologous, teleost, amphibian AOs) have been developed to represent 'natural' phenotypic variation across species. Our aim has been to integrate ssAOs and msAOs for various purposes, including establishing links between phenotypic variation and candidate genes. Results: Previously, msAOs contained a mixture of unique and overlapping content. This hampered integration and coordination due to the need to maintain cross-references or inter-ontology equivalence axioms to the ssAOs, or to perform large-scale obsolescence and modular import. Here we present the unification of anatomy ontologies into Uberon, a single ontology resource that enables interoperability among disparate data and research groups. As a consequence, independent development of TAO, VSAO, AAO, and vHOG has been discontinued. Conclusions: The newly broadened Uberon ontology is a unified cross-taxon resource for metazoans (animals) that has been substantially expanded to include a broad diversity of vertebrate anatomical structures, permitting reasoning across anatomical variation in extinct and extant taxa. Uberon is a core resource that supports single-and cross-species queries for candidate genes using annotations for phenotypes from the systematics, biodiversity, medical, and model organism communities, while also providing entities for logical definitions in the Cell and Gene Ontologies. C1 [Haendel, Melissa A.] Oregon Hlth & Sci Univ, Dept Med Informat & Epidemiol, Portland, OR 97201 USA. [Balhoff, James P.] Univ N Carolina, Dept Biol, Chapel Hill, NC 27599 USA. [Balhoff, James P.; Dahdul, Wasila M.] Natl Evolutionary Synth Ctr, Durham, NC USA. [Bastian, Frederic B.; Comte, Aurelie; Niknejad, Anne; Robinson-Rechavi, Marc] Univ Lausanne, Dept Ecol & Evolut, Lausanne, Switzerland. [Blackburn, David C.] Calif Acad Sci, Dept Vertebrate Zool & Anthropol, San Francisco, CA 94118 USA. [Blake, Judith A.; Hayamizu, Terry F.] Jackson Lab, Bar Harbor, ME 04609 USA. [Bradford, Yvonne] Univ Oregon, Zebrafish Model Organism Database, Eugene, OR 97403 USA. [Dahdul, Wasila M.; Dececchi, Thomas A.; Mabee, Paula M.] Univ S Dakota, Dept Biol, Vermillion, SD 57069 USA. [Druzinsky, Robert E.] Univ Illinois, Dept Oral Biol, Chicago, IL 60612 USA. [Ibrahim, Nizar; Sereno, Paul C.] Univ Chicago, Dept Organismal Biol & Anat, Chicago, IL 60637 USA. [Lewis, Suzanna E.; Mungall, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bastian, Frederic B.; Comte, Aurelie; Niknejad, Anne; Robinson-Rechavi, Marc] Swiss Inst Bioinformat, Lausanne, Switzerland. RP Haendel, MA (reprint author), Oregon Hlth & Sci Univ, Dept Med Informat & Epidemiol, Portland, OR 97201 USA. EM haendel@ohsu.edu RI Robinson-Rechavi, Marc/E-9727-2011; OI Robinson-Rechavi, Marc/0000-0002-3437-3329; Blackburn, David/0000-0002-1810-9886; Bradford, Yvonne/0000-0002-9900-7880; Lewis, Suzanna/0000-0002-8343-612X; Dahdul, Wasila/0000-0003-3162-7490; Balhoff, James/0000-0002-8688-6599 FU National Science Foundation [DBI-0641025, DBI-1062404, DBI-1062350, DBI-1062542]; National Evolutionary Synthesis Center [NSF EF-0423641]; NSF [EF-0905606]; NIH [R24OD011883]; Phenotype Ontology Research Coordination Network [NSF-DEB-0956049]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Swiss Institute of Bioinformatics (SIB); Swiss National Science Foundation [31003A 133011/1]; Etat de Vaud FX This material is based in part upon work supported by the National Science Foundation under Grant Numbers DBI-0641025, DBI-1062404, DBI-1062350, and DBI-1062542, and supported by the National Evolutionary Synthesis Center under NSF EF-0423641 and NSF #EF-0905606. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the National Science Foundation. Aligning to human and model organism sources was supported by the NIH under R24OD011883. We acknowledge the support of the Phenotype Ontology Research Coordination Network (NSF-DEB-0956049) for bringing together the participants to develop key areas of the ontology. CJM acknowledges the support of the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Bgee is supported by the Swiss Institute of Bioinformatics (SIB), the Swiss National Science Foundation (grant number 31003A 133011/1), and Etat de Vaud. We also acknowledge the many contributors to Uberon via our tracker and the constructive comments of the reviewers. NR 45 TC 25 Z9 25 U1 1 U2 4 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 2041-1480 J9 J BIOMED SEMANT JI J. Biomed. Semant. PD MAY 19 PY 2014 VL 5 AR 21 DI 10.1186/2041-1480-5-21 PG 13 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA AR6RL UT WOS:000343710500001 PM 25009735 ER PT J AU Sheikh, JA Hinohara, N Dobaczewski, J Nakatsukasa, T Nazarewicz, W Sato, K AF Sheikh, J. A. Hinohara, N. Dobaczewski, J. Nakatsukasa, T. Nazarewicz, W. Sato, K. TI Isospin-invariant Skyrme energy-density-functional approach with axial symmetry SO PHYSICAL REVIEW C LA English DT Article ID FOCK-BOGOLYUBOV EQUATIONS; HARMONIC-OSCILLATOR BASIS; MEAN-FIELD DESCRIPTION; MANY-BODY PROBLEM; DRIP-LINE NUCLEI; DEFORMED SOLUTION; PROGRAM; N=Z AB Background: Density functional theory (DFT) is the microscopic tool of choice to describe properties of nuclei over the entire nuclear landscape, with a focus on medium-mass and heavy complex systems. Modern energy density functionals (EDFs) often offer a level of accuracy typical of phenomenological approaches based on parameters locally fitted to the data. It is clear, however, that in order to achieve high quality of predictions to guide spectroscopic studies, current functionals must be improved, especially in the isospin channel. In this respect, experimental studies of short-lived nuclei far from stability offer a unique test of isospin aspects of the many-body theory. Purpose: We develop the isospin-invariant Skyrme-EDF method by considering local densities in all possible isospin channels and proton-neutron (p-n) mixing terms as mandated by the isospin symmetry. The EDF employed has the most general form that depends quadratically on the isoscalar and isovector densities. We test and benchmark the resulting p-n EDF approach, and study the general properties of the new scheme by means of the cranking in the isospin space. Methods: We extend the existing axial DFT solver HFBTHO to the case of isospin-invariant EDF approach with all possible p-n mixing terms. Explicit expressions have been derived for all the densities and potentials that appear in the isospin representation. In practical tests, we consider the Skyrme EDF SkM* and, as a first application, concentrate on Hartree-Fock aspects of the problem, i.e., pairing has been disregarded. Results: Calculations have been performed for the (A = 78, T similar or equal to 11), (A = 40, T similar or equal to 8), and (A = 48, T similar or equal to 4) isobaric analog chains. Isospin structure of self-consistent p-n mixed solutions has been investigated with and without the Coulomb interaction, which is the sole source of isospin symmetry breaking in our approach. The extended axial HFBTHO solver has been benchmarked against the symmetry-unrestricted HFODD code for deformed and spherical states. Conclusions: We developed and tested a general isospin-invariant Skyrme-EDF framework. The new approach permits spin-isospin densities that may give rise to hitherto unexplored modes in the excitation spectrum. The new formalism has been tested in the Hartree-Fock limit. A systematic comparison between HFODD and HFBTHO results show a maximum deviation of about 10 keV on the total binding energy for deformed nuclei when the Coulomb term is included. Without this term, the results of both solvers agree down to a similar to 10 eV level. C1 [Sheikh, J. A.; Hinohara, N.; Dobaczewski, J.; Nazarewicz, W.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Sheikh, J. A.; Hinohara, N.] Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. [Sheikh, J. A.] Univ Kashmir, Dept Phys, Srinagar 190006, Jammu & Kashmir, India. [Hinohara, N.] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC 27599 USA. [Dobaczewski, J.; Nazarewicz, W.] Univ Warsaw, Inst Theoret Phys, Fac Phys, PL-00681 Warsaw, Poland. [Dobaczewski, J.] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland. [Nakatsukasa, T.; Sato, K.] RIKEN Nishina Ctr, Wako, Saitama 3510198, Japan. [Nakatsukasa, T.] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058571, Japan. [Nazarewicz, W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Sheikh, JA (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RI Nakatsukasa, Takashi/O-9995-2014; OI Hinohara, Nobuo/0000-0001-9562-0189 FU U.S. Department of Energy [DE-FG02-96ER40963, DE-SC0008499, DE-FG02-06ER41407]; Academy of Finland; University of Jyvaskyla within the FIDIPRO program; Polish National Science Center [2012/07/B/ST2/03907]; JSPS KAKENHI [20105003, 24105006, 25287065, 25287066] FX We would like to express our deep gratitude to our friend and colleague, Mario Stoitsov, for his contributions in the initial stages of this work. J.A.S. would like to acknowledge I. Maqbool and P. A. Ganai for discussions. This work was supported by the U.S. Department of Energy under Contracts No. DE-FG02-96ER40963 (University of Tennessee), No. DE-SC0008499 (NUCLEI SciDAC Collaboration), and No. DE-FG02-06ER41407 (JUSTIPEN, Japan-U.S. Theory Institute for Physics with Exotic Nuclei); by the Academy of Finland and University of Jyvaskyla within the FIDIPRO program; by the Polish National Science Center under Contract No. 2012/07/B/ST2/03907; and by JSPS KAKENHI (Grants No. 20105003, No. 24105006, No. 25287065, and No. 25287066). Computational resources were provided through an INCITE award "Computational Nuclear Structure" by the National Center for Computational Sciences (NCCS) and the National Institute for Computational Sciences (NICS) at Oak Ridge National Laboratory. A part of the numerical calculations were also carried out on SR16000 at the Yukawa Institute for Theoretical Physics in Kyoto University and on the RIKEN Integrated Cluster of Clusters (RICC) facility. NR 40 TC 4 Z9 4 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 19 PY 2014 VL 89 IS 5 AR 054317 DI 10.1103/PhysRevC.89.054317 PG 12 WC Physics, Nuclear SC Physics GA AP2EE UT WOS:000341884500004 ER PT J AU Gibbons, SM Jones, E Bearquiver, A Blackwolf, F Roundstone, W Scott, N Hooker, J Madsen, R Coleman, ML Gilbert, JA AF Gibbons, Sean M. Jones, Edwin Bearquiver, Angelita Blackwolf, Frederick Roundstone, Wayne Scott, Nicole Hooker, Jeff Madsen, Robert Coleman, Maureen L. Gilbert, Jack A. TI Human and Environmental Impacts on River Sediment Microbial Communities SO PLOS ONE LA English DT Article ID GRAVEL-BED RIVER; HYPORHEIC-ZONE; BACTERIAL PRODUCTION; SEASONAL DYNAMICS; DIVERSITY; ECOSYSTEM; MAGNITUDE; SEQUENCES; TAXONOMY; GENES AB Sediment microbial communities are responsible for a majority of the metabolic activity in river and stream ecosystems. Understanding the dynamics in community structure and function across freshwater environments will help us to predict how these ecosystems will change in response to human land-use practices. Here we present a spatiotemporal study of sediments in the Tongue River (Montana, USA), comprising six sites along 134 km of river sampled in both spring and fall for two years. Sequencing of 16S rRNA amplicons and shotgun metagenomes revealed that these sediments are the richest (similar to 65,000 microbial 'species' identified) and most novel (93% of OTUs do not match known microbial diversity) ecosystems analyzed by the Earth Microbiome Project to date, and display more functional diversity than was detected in a recent review of global soil metagenomes. Community structure and functional potential have been significantly altered by anthropogenic drivers, including increased pathogenicity and antibiotic metabolism markers near towns and metabolic signatures of coal and coalbed methane extraction byproducts. The core (OTUs shared across all samples) and the overall microbial community exhibited highly similar structure, and phylogeny was weakly coupled with functional potential. Together, these results suggest that microbial community structure is shaped by environmental drivers and niche filtering, though stochastic assembly processes likely play a role as well. These results indicate that sediment microbial communities are highly complex and sensitive to changes in land use practices. C1 [Gibbons, Sean M.; Gilbert, Jack A.] Univ Chicago, Grad Program Biophys Sci, Chicago, IL 60637 USA. [Gibbons, Sean M.; Scott, Nicole; Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Lemont, IL USA. [Gibbons, Sean M.; Jones, Edwin; Bearquiver, Angelita; Blackwolf, Frederick; Roundstone, Wayne; Hooker, Jeff; Madsen, Robert] Chief Dull Knife Coll, Dept Biol, Lame Deer, MT USA. [Coleman, Maureen L.] Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. RP Gilbert, JA (reprint author), Univ Chicago, Grad Program Biophys Sci, Chicago, IL 60637 USA. EM gilbertjack@anl.gov OI Gibbons, Sean/0000-0002-8724-7916 FU U.S. Department of Energy [DE-AC02-06CH11357]; National Science Foundation EPSCoR; U.S. Nuclear Regulatory Commission [NRC-27-10-1124]; EPA STAR Graduate Fellowship FX This work was supported in part by the U.S. Department of Energy under Contract DE-AC02-06CH11357, by National Science Foundation EPSCoR funds, and by the U.S. Nuclear Regulatory Commission under the grant number NRC-27-10-1124. S.M.G. was supported by an EPA STAR Graduate Fellowship. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 46 TC 18 Z9 19 U1 10 U2 66 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 19 PY 2014 VL 9 IS 5 AR e97435 DI 10.1371/journal.pone.0097435 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN9SK UT WOS:000340948600032 PM 24841417 ER PT J AU Budker, D Graham, PW Ledbetter, M Rajendran, S Sushkov, AO AF Budker, Dmitry Graham, Peter W. Ledbetter, Micah Rajendran, Surjeet Sushkov, Alexander O. TI Proposal for a Cosmic Axion Spin Precession Experiment (CASPEr) SO PHYSICAL REVIEW X LA English DT Article ID ODD ELECTROMAGNETIC MOMENTS; ELECTRIC-DIPOLE MOMENT; CP CONSERVATION; INVISIBLE-AXION; HARMLESS AXION; INVARIANCE; PARTICLES; COSMOLOGY; NUCLEI; THETA AB We propose an experiment to search for QCD axion and axionlike-particle dark matter. Nuclei that are interacting with the background axion dark matter acquire time-varying CP-odd nuclear moments such as an electric dipole moment. In analogy with nuclear magnetic resonance, these moments cause precession of nuclear spins in a material sample in the presence of an electric field. Precision magnetometry can be used to search for such precession. An initial phase of this experiment could cover many orders of magnitude in axionlike-particle parameter space beyond the current astrophysical and laboratory limits. And with established techniques, the proposed experimental scheme has sensitivity to QCD axion masses m(a) less than or similar to 10(-9) eV, corresponding to theoretically well-motivated axion decay constants f(a) greater than or similar to 10(16) GeV. With further improvements, this experiment could ultimately cover the entire range of masses m(a) less than or similar to mu V, complementary to cavity searches. C1 [Budker, Dmitry] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Budker, Dmitry] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Graham, Peter W.; Rajendran, Surjeet] Stanford Univ, Stanford Inst Theoret Phys, Dept Phys, Stanford, CA 94305 USA. [Ledbetter, Micah] AOSense, Sunnyvale, CA 94085 USA. [Sushkov, Alexander O.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Sushkov, Alexander O.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. [Budker, Dmitry] Johannes Gutenberg Univ Mainz, Helmholtz Inst Mainz, D-55099 Mainz, Germany. RP Budker, D (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RI Budker, Dmitry/F-7580-2016; OI Budker, Dmitry/0000-0002-7356-4814; Graham, Peter/0000-0002-1600-1601 FU ERC Grant BSMOXFORD [228169]; National Science Foundation [PHY-1068875]; Miller Institute for Basic Research in Science; NSF [PHY-1316706]; Hellman Faculty Scholars program; Terman Fellowship FX We thank Blas Cabrera, Savas Dimopoulos, Matt Pyle, and Scott Thomas for valuable discussions. S. R. was supported by ERC Grant BSMOXFORD No. 228169. This work has been supported in part by the National Science Foundation under Grant No. PHY-1068875. D. B. acknowledges support by the Miller Institute for Basic Research in Science. PWG acknowledges the support of NSF Grant No. PHY-1316706, the Hellman Faculty Scholars program, and the Terman Fellowship. NR 63 TC 63 Z9 63 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAY 19 PY 2014 VL 4 IS 2 AR 021030 DI 10.1103/PhysRevX.4.021030 PG 10 WC Physics, Multidisciplinary SC Physics GA AN5UZ UT WOS:000340658200001 ER PT J AU Lu, YM Lee, DH AF Lu, Yuan-Ming Lee, Dung-Hai TI Gapped symmetric edges of symmetry-protected topological phases SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM HALL STATES; INSULATORS AB Symmetry-protected topological (SPT) phases are gapped quantum phases which host symmetry-protected gapless edge excitations. On the other hand, the edge states can be gapped by spontaneously breaking symmetry. We show that topological defects on the symmetry-broken edge cannot proliferate due to their fractional statistics. A gapped symmetric boundary, however, can be achieved between an SPT phase and certain fractionalized phases by condensing the bound state of a topological defect and an anyon. We demonstrate this by two examples in two dimensions: an exactly solvable model for the boundary between a topological Ising paramagnet and the double-semion model, and a fermionic example about the quantum spin Hall edge. Such a hybrid structure containing both SPT phase and fractionalized phase generally support ground-state degeneracy on a torus. C1 [Lu, Yuan-Ming] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Lu, YM (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RI Lu, Yuan-Ming/D-7554-2017 OI Lu, Yuan-Ming/0000-0001-6275-739X FU Office of Basic Energy Sciences, Materials Sciences Division, of the US DOE [DE-AC02-05CH11231]; National Science Foundation [PHYS-1066293] FX This work was supported by the Office of Basic Energy Sciences, Materials Sciences Division, of the US DOE under Contract No. DE-AC02-05CH11231 (Y.M.L., D.H.L.) and in part by the National Science Foundation under Grant No. PHYS-1066293 (Y.M.L.). We thank Taylor L. Hughes and Ashvin Vishwanath for helpful conversations. Y.M.L. is grateful for the hospitality of the Aspen Center for Physics where he presented this work in the 2013 summer program "Disorder, Dynamics, Frustration, and Topology in Quantum Condensed Matter," and for the hospitality of the Institute for Advance Study in Tsinghua University, where part of this work was finished. NR 31 TC 10 Z9 10 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 19 PY 2014 VL 89 IS 20 AR 205117 DI 10.1103/PhysRevB.89.205117 PG 6 WC Physics, Condensed Matter SC Physics GA AM1SW UT WOS:000339629600004 ER PT J AU Lancaster, T Goddard, PA Blundell, SJ Foronda, FR Ghannadzadeh, S Moller, JS Baker, PJ Pratt, FL Baines, C Huang, L Wosnitza, J McDonald, RD Modic, KA Singleton, J Topping, CV Beale, TAW Xiao, F Schlueter, JA Barton, AM Cabrera, RD Carreiro, KE Tran, HE Manson, JL AF Lancaster, T. Goddard, P. A. Blundell, S. J. Foronda, F. R. Ghannadzadeh, S. Moeller, J. S. Baker, P. J. Pratt, F. L. Baines, C. Huang, L. Wosnitza, J. McDonald, R. D. Modic, K. A. Singleton, J. Topping, C. V. Beale, T. A. W. Xiao, F. Schlueter, J. A. Barton, A. M. Cabrera, R. D. Carreiro, K. E. Tran, H. E. Manson, J. L. TI Controlling Magnetic Order and Quantum Disorder in Molecule-Based Magnets SO PHYSICAL REVIEW LETTERS LA English DT Article ID INSULATORS AB We investigate the structural and magnetic properties of two molecule-based magnets synthesized from the same starting components. Their different structural motifs promote contrasting exchange pathways and consequently lead to markedly different magnetic ground states. Through examination of their structural and magnetic properties we show that [Cu(pyz)(H2O)(gly)(2)](ClO4)(2) may be considered a quasi-one-dimensional quantum Heisenberg antiferromagnet whereas the related compound [Cu(pyz)(gly)](ClO4), which is formed from dimers of antiferromagnetically interacting Cu2+ spins, remains disordered down to at least 0.03 K in zero field but shows a field-temperature phase diagram reminiscent of that seen in materials showing a Bose-Einstein condensation of magnons. C1 [Lancaster, T.; Beale, T. A. W.; Xiao, F.] Univ Durham, Ctr Phys Mat, Durham DH1 3LE, England. [Goddard, P. A.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Blundell, S. J.; Foronda, F. R.; Ghannadzadeh, S.; Moeller, J. S.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Baker, P. J.; Pratt, F. L.] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Baines, C.] Paul Scherrer Inst, Lab Muon Spin Spect, CH-5232 Villigen, Switzerland. [Huang, L.; Wosnitza, J.] Helmholtz Zentrum Dresden Rossendorf, Dresden High Magnet Field Lab, D-01314 Dresden, Germany. [McDonald, R. D.; Modic, K. A.; Singleton, J.; Topping, C. V.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. [Schlueter, J. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Barton, A. M.; Cabrera, R. D.; Carreiro, K. E.; Tran, H. E.; Manson, J. L.] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. RP Lancaster, T (reprint author), Univ Durham, Ctr Phys Mat, South Rd, Durham DH1 3LE, England. EM tom.lancaster@durham.ac.uk; jmanson@ewu.edu RI Baker, Peter/E-4216-2010; Goddard, Paul/A-8638-2015 OI Baker, Peter/0000-0002-2306-2648; Goddard, Paul/0000-0002-0666-5236 FU EPSRC (UK); U.S. National Science Foundation [DMR-1005825, 1306158]; Independent Research/Development program at the National Science Foundation; National Science Foundation [DMR-1157490]; State of Florida; U.S. Department of Energy (DoE) FX Part of this work was carried out at the STFC ISIS facility and at the Swiss Muon Source, Paul Scherrer Institute, Switzerland, and we are grateful for the provision of beam time. This work is supported by EPSRC (UK). We are grateful to R. Williams and D. S Yufit for experimental assistance. The work at EWU was supported in part by the U.S. National Science Foundation under Grants No. DMR-1005825 and No. 1306158. J. A. S. acknowledges support from the Independent Research/Development program while serving at the National Science Foundation. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement No. DMR-1157490, the State of Florida, and the U.S. Department of Energy (DoE) and through the DoE Basic Energy Science Field Work Proposal "Science in 100 T." NR 19 TC 6 Z9 6 U1 1 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 19 PY 2014 VL 112 IS 20 AR 207201 DI 10.1103/PhysRevLett.112.207201 PG 5 WC Physics, Multidisciplinary SC Physics GA AM1RM UT WOS:000339625800004 ER PT J AU Kindervater, J Haussler, W Janoschek, M Pfleiderer, C Boni, P Garst, M AF Kindervater, J. Haeussler, W. Janoschek, M. Pfleiderer, C. Boeni, P. Garst, M. TI Critical spin-flip scattering at the helimagnetic transition of MnSi SO PHYSICAL REVIEW B LA English DT Article ID NEUTRON POLARIMETRY; FEGE AB We report spherical neutron polarimetry (SNP) and discuss the spin-flip scattering cross sections as well as the chiral fraction. close to the helimagnetic transition in MnSi. For our study we have developed a miniaturized SNP device that allows fast data collection when used in small angle scattering geometry with an area detector. Critical spin-flip scattering is found to be governed by chiral paramagnons that soften on a sphere in momentum space. Carefully accounting for the incoherent spin-flip background, we find that the resulting chiral fraction. decreases gradually above the helimagnetic transition reflecting a strongly renormalized chiral correlation length with a temperature dependence in excellent quantitative agreement with the Brazovskii theory for a fluctuation-induced first order transition. C1 [Kindervater, J.; Haeussler, W.; Pfleiderer, C.; Boeni, P.] Tech Univ Munich, Phys Dept E21, D-85748 Garching, Germany. [Haeussler, W.] Tech Univ Munich, Heinz Maier Leibnitz Zentrum, D-85748 Garching, Germany. [Janoschek, M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Garst, M.] Univ Cologne, Inst Theoret Phys, D-50937 Cologne, Germany. RP Kindervater, J (reprint author), Tech Univ Munich, Phys Dept E21, D-85748 Garching, Germany. RI Garst, Markus/B-6740-2012; Pfleiderer, Christian/P-3575-2014; Janoschek, Marc/M-8871-2015 OI Garst, Markus/0000-0001-5390-3316; Janoschek, Marc/0000-0002-2943-0173 FU TUM Graduate School; DFG [TRR80, FOR960]; ERC-AdG [291079 TOPFIT] FX We wish to thank A. Rosch, K. Pappas, and S. Grigoriev for helpful discussions, and M. Schulz and P. Schmakat for contributions at early stages of this work. J. K. acknowledges financial support through the TUM Graduate School. Financial support through DFG TRR80, FOR960, and ERC-AdG (291079 TOPFIT) are gratefully acknowledged. NR 36 TC 11 Z9 11 U1 2 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 19 PY 2014 VL 89 IS 18 AR 180408 DI 10.1103/PhysRevB.89.180408 PG 5 WC Physics, Condensed Matter SC Physics GA AL6XD UT WOS:000339276100001 ER PT J AU Huneeus, N Boucher, O Alterskjaer, K Cole, JNS Curry, CL Ji, DY Jones, A Kravitz, B Kristjansson, JE Moore, JC Muri, H Niemeier, U Rasch, P Robock, A Singh, B Schmidt, H Schulz, M Tilmes, S Watanabe, S Yoon, JH AF Huneeus, Nicolas Boucher, Olivier Alterskjaer, Kari Cole, Jason N. S. Curry, Charles L. Ji, Duoying Jones, Andy Kravitz, Ben Kristjansson, Jon Egill Moore, John C. Muri, Helene Niemeier, Ulrike Rasch, Phil Robock, Alan Singh, Balwinder Schmidt, Hauke Schulz, Michael Tilmes, Simone Watanabe, Shingo Yoon, Jin-Ho TI Forcings and feedbacks in the GeoMIP ensemble for a reduction in solar irradiance and increase in CO2 SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID CLIMATE SENSITIVITY; MODELS; RESPONSES; CMIP5 AB The effective radiative forcings (including rapid adjustments) and feedbacks associated with an instantaneous quadrupling of the preindustrial CO2 concentration and a counterbalancing reduction of the solar constant are investigated in the context of the Geoengineering Model Intercomparison Project (GeoMIP). The forcing and feedback parameters of the net energy flux, as well as its different components at the top-of-atmosphere (TOA) and surface, were examined in 10 Earth System Models to better understand the impact of solar radiation management on the energy budget. In spite of their very different nature, the feedback parameter and its components at the TOA and surface are almost identical for the two forcing mechanisms, not only in the global mean but also in their geographical distributions. This conclusion holds for each of the individual models despite intermodel differences in how feedbacks affect the energy budget. This indicates that the climate sensitivity parameter is independent of the forcing (when measured as an effective radiative forcing). We also show the existence of a large contribution of the cloudy-sky component to the shortwave effective radiative forcing at the TOA suggesting rapid cloud adjustments to a change in solar irradiance. In addition, the models present significant diversity in the spatial distribution of the shortwave feedback parameter in cloudy regions, indicating persistent uncertainties in cloud feedback mechanisms. C1 [Huneeus, Nicolas; Boucher, Olivier] UPMC, CNRS, IPSL, Lab Meteorol Dynam, Paris, France. [Alterskjaer, Kari; Kristjansson, Jon Egill; Muri, Helene] Univ Oslo, Dept Geosci, Oslo, Norway. [Cole, Jason N. S.] Environm Canada, Canadian Ctr Climate Modelling & Anal, Toronto, ON, Canada. [Curry, Charles L.] Univ Victoria, Sch Earth & Ocean Sci, Victoria, BC, Canada. [Ji, Duoying; Moore, John C.] Beijing Normal Univ, Coll Global Change & Earth Syst Sci, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China. [Jones, Andy] Met Off Hadley Ctr, Exeter, Devon, England. [Kravitz, Ben; Rasch, Phil; Singh, Balwinder; Yoon, Jin-Ho] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Niemeier, Ulrike; Schmidt, Hauke] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Robock, Alan] Rutgers State Univ, Dept Environm Sci, New Brunswick, NJ 08903 USA. [Schulz, Michael] Norwegian Meteorol Inst, Oslo, Norway. [Tilmes, Simone] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Watanabe, Shingo] Japan Agcy Marine Earth Sci & Technol, Yokohama, Kanagawa, Japan. RP Huneeus, N (reprint author), Univ Chile, Dept Geophys, Santiago, Chile. EM nhuneeus@dgf.uchile.cl RI Moore, John/B-2868-2013; YOON, JIN-HO/A-1672-2009; Kravitz, Ben/P-7925-2014; Muri, Helene/D-4845-2015; Schulz, Michael/A-6930-2011; Robock, Alan/B-6385-2016; Huneeus, Nicolas/J-4994-2016; Watanabe, Shingo/L-9689-2014 OI Huneeus, Nicolas/0000-0002-6214-5518; Moore, John/0000-0001-8271-5787; YOON, JIN-HO/0000-0002-4939-8078; Cole, Jason/0000-0003-0450-2748; Kravitz, Ben/0000-0001-6318-1150; Muri, Helene/0000-0003-4738-493X; Schulz, Michael/0000-0003-4493-4158; Watanabe, Shingo/0000-0002-2228-0088 FU European Commission under the EU Seventh Research Framework Programme (MACC II) [283576]; French Ministere de l'Ecologie, du Developpement Durable, des Transports et du Logement (MEDDE) under the GMES-MDD program; GENCI-TGCC [2013-t2013012201]; Fund for Innovative Climate and Energy Research (FICER); U.S. Department of Energy [DE-AC05-76RL01830]; NSF [AGS-1157525, CBET-1240507]; Joint UK DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; European Commission's Seventh Framework Programme through the IMPLICC project [FP7-ENV-2008-1-226567]; European Union's Seventh Framework Programme (FP7) [226567-IMPLICC]; European Commission under the EU Seventh Research Framework Programme (EuTRACE) [306395]; National Science Foundation; Office of Science (BER) of the U.S. Department of Energy FX We thank all participants of the Geoengineering Model Intercomparison Project and their model development teams, the CLIVAR/WCRP Working Group on Coupled Modeling for endorsing GeoMIP, and the scientists managing the Earth System Grid data nodes who have assisted with making GeoMIP output available. We further acknowledge the World Climate Research Programme's Working Group on Coupled Modelling, which is responsible for CMIP, and we thank the climate modeling groups for producing and making available their model output. For CMIP, the U.S. Department of Energy's Program for Climate Model Diagnosis and Intercomparison provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals. This study was co-funded by the European Commission under the EU Seventh Research Framework Programme (grant agreement No. 283576, MACC II) and by the French Ministere de l'Ecologie, du Developpement Durable, des Transports et du Logement (MEDDE) under the GMES-MDD program. This work was partly performed using HPC resources from GENCI-TGCC (grant 2013-t2013012201). Simulations performed by Ben Kravitz were supported by the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center. Ben Kravitz is supported by the Fund for Innovative Climate and Energy Research (FICER). The Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RL01830. Alan Robock is supported by NSF grants AGS-1157525 and CBET-1240507. Andy Jones was supported by the Joint UK DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). U. Niemeier and H. Schmidt have received funding from the European Commission's Seventh Framework Programme through the IMPLICC project (FP7-ENV-2008-1-226567). K. Alterskjaer and J.E. Kristjansson received support from the European Union's Seventh Framework Programme (FP7/2007-2013) under grant agreement 226567-IMPLICC, as well as from the Norwegian Research Council's Programme for Supercomputing (NOTUR) through a grant of computing time. Helene Muri was supported by the European Commission under the EU Seventh Research Framework Programme (grant agreement 306395, EuTRACE). The CESM project (and therefore CCSM) is supported by the National Science Foundation and the Office of Science (BER) of the U.S. Department of Energy. The National Center for Atmospheric Research is funded by the National Science Foundation. NR 35 TC 7 Z9 8 U1 1 U2 17 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 19 PY 2014 VL 119 IS 9 BP 5226 EP 5239 DI 10.1002/2013JD021110 PG 14 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3QS UT WOS:000338340400013 ER PT J AU Zhao, CF Xie, SC Chen, X Jensen, MP Dunn, M AF Zhao, Chuanfeng Xie, Shaocheng Chen, Xiao Jensen, Michael P. Dunn, Maureen TI Quantifying uncertainties of cloud microphysical property retrievals with a perturbation method SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID ICE WATER-CONTENT; MICROWAVE RADIOMETER; RADIATIVE PROPERTIES; RADAR MEASUREMENTS; MILLIMETER RADAR; REMOTE SENSORS; CIRRUS CLOUDS; STRATUS CLOUD; BEAUFORT SEA; PART I AB Quantifying the uncertainty of cloud retrievals is an emerging topic important for both cloud process studies and modeling studies. This paper presents a general approach to estimate uncertainties in ground-based retrievals of cloud properties. This approach, called the perturbation method, quantifies the cloud retrieval uncertainties by perturbing the cloud retrieval influential factors (like inputs and parameters) within their error ranges. The error ranges for the cloud retrieval inputs and parameters are determined by either instrument limitations or comparisons against aircraft observations. With the knowledge from observations and the retrieval algorithms, the perturbation method can provide an estimate of the cloud retrieval uncertainties, regardless of the complexity (like nonlinearity) of the retrieval algorithm. The relative contribution to the uncertainties of retrieved cloud properties from the inputs, assumptions, and parameterizations can also be assessed with this perturbation method. As an example, we apply this approach to the Atmospheric Radiation Measurement Program baseline retrieval, MICROBASE. Only nonprecipitating single-phase (liquid or ice) clouds have been examined in this study. Results reveal that different influential factors play the dominant contributing role to the uncertainties of different cloud properties. To reduce uncertainties in cloud retrievals, future efforts should be emphasized on the major contributing factors for considered cloud properties. This study also shows high sensitivity of cloud retrieval uncertainties to different cloud types, with the largest uncertainties for deep convective clouds. Limitations and further efforts for this uncertainty quantification method are discussed. C1 [Zhao, Chuanfeng] Beijing Normal Univ, Coll Global Change & Earth Syst Sci, Beijing 100875, Peoples R China. [Xie, Shaocheng; Chen, Xiao] Lawrence Livermore Natl Lab, Livermore, CA USA. [Jensen, Michael P.; Dunn, Maureen] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Zhao, CF (reprint author), Beijing Normal Univ, Coll Global Change & Earth Syst Sci, Beijing 100875, Peoples R China. EM czhao@bnu.edu.cn RI Zhao, Chuanfeng/G-8546-2013; Xie, Shaocheng/D-2207-2013 OI Xie, Shaocheng/0000-0001-8931-5145 FU Atmospheric Radiation Measurement Program of the U.S. Department of Energy's Climate and Earth System Division of the Office of Science; Ministry of Science and Technology of China [2012AA120901, 2013CB955802]; Chinese Program for New Century Excellent Talents in University (NCET); Fundamental Research Funds for the Central Universities; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research by Brookhaven National Laboratory [DE-AC02-98CH10886] FX This work was supported by the Atmospheric Radiation Measurement Program of the U.S. Department of Energy's Climate and Earth System Division of the Office of Science and the Ministry of Science and Technology of China through grant 2012AA120901 and 2013CB955802, the Chinese Program for New Century Excellent Talents in University (NCET), and the Fundamental Research Funds for the Central Universities. The study in LLNL and BNL is performed under the auspices of the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 and by Brookhaven National Laboratory under contract DE-AC02-98CH10886, respectively. We thank X. Dong for providing us the aircraft data for stratus clouds on 17 March 2000 at SGP site, and thank Y. Zhang and R. McCoy for valuable communications. NR 37 TC 8 Z9 8 U1 0 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 19 PY 2014 VL 119 IS 9 BP 5375 EP 5385 DI 10.1002/2013JD021112 PG 11 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3QS UT WOS:000338340400023 ER PT J AU Creekmore, TN Joseph, E Long, CN Li, SW AF Creekmore, Torreon N. Joseph, Everette Long, Charles N. Li, Siwei TI Quantifying aerosol direct effects from broadband irradiance and spectral aerosol optical depth observations SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID GENERAL-CIRCULATION MODEL; ACTIVE SOLAR IRRADIANCE; RADIATIVE-TRANSFER; CLEAR SKIES; PARAMETERIZATION; CLIMATE; CLOUDS AB We outline a methodology using broadband and spectral irradiances to quantify aerosol direct effects on the surface diffuse shortwave (SW) irradiance. Best Estimate Flux data span a 13 year timeframe at the Department of Energy Atmospheric Radiation Measurement Program's Southern Great Plains (SGP) site. Screened clear-sky irradiances and aerosol optical depth (AOD), for solar zenith angles <= 65 degrees, are used to estimate clear-sky diffuse irradiances. We validate against detected clear-sky observations from SGP's Basic Radiation System (BRS). BRS diffuse irradiances were in accordance with estimates, producing a root-mean-square error and mean bias errors of 4.0 W/m(2) and -1.4 W/m(2), respectively. Absolute differences show 99% of estimates within +/- 10 W/m(2) (10%) of the mean BRS observations. Clear-sky diffuse estimates are used to derive quantitative estimates of aerosol radiative effects, represented as the aerosol diffuse irradiance (ADI). ADI is the contribution of diffuse SW to global SW, attributable to scattering of atmospheric transmission by natural plus anthropogenic aerosols. Estimated slope for the ADI as a function of AOD indicates an increase of similar to 22 W/m(2) in diffuse SW for every 0.1 increase in AOD. Such significant increases in the diffuse fraction could possibly increase photosynthesis. Annual mean ADI is 28.2 W/m(2), and heavy aerosol loading at SGP provides up to a maximum increase of 120 W/m(2) in diffuse SW over background conditions. With regard to seasonal variation, the mean diffuse forcings are 17.2, 33.3, 39.0, and 23.6 W/m(2) for winter, spring, summer, and fall, respectively. C1 [Creekmore, Torreon N.] Natl Geospatial Intelligence Agcy, InnoVison Basic & Appl Res Off, Springfield, VA 22150 USA. [Joseph, Everette; Li, Siwei] Howard Univ, Beltsville Ctr Climate Syst Observat, Washington, DC 20059 USA. [Joseph, Everette] Howard Univ, Dept Phys & Astron, Washington, DC 20059 USA. [Long, Charles N.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Creekmore, TN (reprint author), Natl Geospatial Intelligence Agcy, InnoVison Basic & Appl Res Off, Springfield, VA 22150 USA. EM torreon.n.creekmore@nga.mil FU Office of Science of the U.S. Department of Energy FX The authors are grateful to the data provided by the AERONET network and ARM program. Additionally, the authors express their appreciation to the operators running the instruments at the SGP site. Long acknowledges support from the Office of Science of the U.S. Department of Energy as part of the Atmospheric System Research Program. The data for this paper are available at the following links: http://aeronet.gsfc.nasa.gov and http://www.arm.gov. NR 45 TC 1 Z9 1 U1 1 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 19 PY 2014 VL 119 IS 9 BP 5464 EP 5474 DI 10.1002/2013JD021217 PG 11 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3QS UT WOS:000338340400029 ER PT J AU Riihimaki, LD Long, CN AF Riihimaki, Laura D. Long, Charles N. TI Spatial variability of surface irradiance measurements at the Manus ARM site SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID TROPICAL WESTERN PACIFIC; ATMOSPHERIC RADIATION; MODEL VALIDATION; SOLAR-RADIATION; CLOUD; NETWORK; BUDGET AB The location of the Atmospheric Radiation Measurement (ARM) site on Manus island was chosen because it is very close to the coast, in a flat, near-sea level area of the island, hopefully minimizing the impact of local island effects on the meteorology of the measurements. In this study, we confirm that the Manus site is indeed less impacted by the island meteorology than slightly inland by comparing over a year of broadband surface irradiance and ceilometer measurements and derived quantities at the standard Manus site and a second location 7 km away as part of the ARM Madden Julian Oscillation Investigation Experiment (AMIE)-Manus campaign. The two sites show statistically similar distributions of irradiance and other derived quantities for all wind directions except easterly winds, when the inland site is downwind from the standard Manus site. Under easterly wind conditions, which occur 17% of the time, there is a higher occurrence of cloudiness at the downwind site likely due to land heating and orographic effects. This increased cloudiness is caused by scattered clouds often with bases around 700 m in altitude. While the central Manus site consistently measures a frequency of occurrence of low clouds (cloud base height less than 1200 m) about 25% of the time regardless of wind direction, the AMIE site has higher frequencies of low clouds (38%) when winds are from the east. This increase in low, locally produced clouds causes an additional -20 W/m(2) shortwave surface cloud radiative effect at the AMIE site than the Manus site. C1 [Riihimaki, Laura D.; Long, Charles N.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Riihimaki, LD (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM laura.riihimaki@pnnl.gov FU Office of Science of the U.S. Department of Energy as part of the Atmospheric Systems Research Program; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830] FX This research was supported by the Office of Science of the U.S. Department of Energy as part of the Atmospheric Systems Research Program and used data and facilities from the Atmospheric Radiation Measurement Climate Research Facility. All data products are available online at the ARM website: http://www.arm.gov. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. Recognition is also extended to those responsible for the operation and maintenance of the instruments that produced the data used in this study; their diligent and dedicated efforts are often underappreciated. The authors also thank Larry Berg for helpful discussions which improved the manuscript. NR 35 TC 4 Z9 4 U1 1 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 19 PY 2014 VL 119 IS 9 BP 5475 EP 5491 DI 10.1002/2013JD021187 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3QS UT WOS:000338340400030 ER PT J AU Pfister, GG Walters, S Lamarque, JF Fast, J Barth, MC Wong, J Done, J Holland, G Bruyere, CL AF Pfister, G. G. Walters, S. Lamarque, J. -F. Fast, J. Barth, M. C. Wong, J. Done, J. Holland, G. Bruyere, C. L. TI Projections of future summertime ozone over the US SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID COMMUNITY ATMOSPHERE MODEL; REGIONAL AIR-POLLUTION; CLIMATE-CHANGE; UNITED-STATES; SURFACE OZONE; TROPOSPHERIC OZONE; PARTICULATE MATTER; ISOPRENE EMISSIONS; EASTERN-EUROPE; SYSTEM MODEL AB We use a regional coupled chemistry-transport model to assess changes in surface ozone over the summertime U.S. between present and a 2050 future time period at high spatial resolution under the A2 climate and Representative Concentration Pathway (RCP) 8.5 anthropogenic precursor emission scenarios. Predicted changes in regional climate and globally enhanced ozone are estimated to increase surface ozone over most of the U.S.; the 95th percentile for daily 8 h maximum surface ozone increases from 79 ppb to 87 ppb. The analysis suggests that changes in meteorological drivers likely will add to increasing ozone, but the simulations do not allow separating meteorological feedbacks from that due to enhanced global ozone. Stringent emission controls can counteract these feedbacks; if implemented as in RCP8.5, the 95th percentile for surface ozone is reduced to 55 ppb. A comparison of regional to global model projections shows that the global model is biased high in surface ozone compared to the regional model and compared to observations. On average, both the global and the regional model predict similar future changes but reveal pronounced differences in urban and rural regimes that cannot be resolved at the coarse resolution of the considered global model. This study confirms the key role of emission control strategies in future air quality projections and demonstrates the need for considering degradation of air quality with future climate change in policy making. It also illustrates the need for high-resolution modeling when the objective is to address regional and local air quality or establish links to human health and society. C1 [Pfister, G. G.; Walters, S.; Lamarque, J. -F.; Barth, M. C.; Wong, J.] NCAR, Div Atmospher Chem, Boulder, CO 80305 USA. [Fast, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Barth, M. C.; Done, J.; Holland, G.; Bruyere, C. L.] NCAR, Boulder, CO USA. [Wong, J.] Univ Colorado, Dept Atmospher & Ocean Sci, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Bruyere, C. L.] North West Univ, Potchefstroom, South Africa. RP Pfister, GG (reprint author), NCAR, Div Atmospher Chem, Boulder, CO 80305 USA. EM pfister@ucar.edu RI Lamarque, Jean-Francois/L-2313-2014 OI Lamarque, Jean-Francois/0000-0002-4225-5074 FU NSF-EaSM [AGS-1048829]; NCAR Accelerated Scientific Discovery (ASD) grant; National Science Foundation; Office of Science (BER) of the U.S. Department of Energy; DOE's Office of Science/Biological and Environmental Research through the Atmospheric System Research program at Pacific Northwest National Laboratory (PNNL); DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830] FX We would like to acknowledge the three reviewers for their valuable and constructive input. This work was supported by NSF-EaSM grant AGS-1048829 "Developing a Next-Generation Approach to Regional Climate Prediction at High Resolution." Model simulations were made possible by an NCAR Accelerated Scientific Discovery (ASD) grant. The CESM project (which includes CAM-Chem) is supported by the National Science Foundation and the Office of Science (BER) of the U.S. Department of Energy. NCAR is operated by the University Corporation of Atmospheric Research under sponsorship of the National Science Foundation. Jerome Fast was supported by the DOE's Office of Science/Biological and Environmental Research, through the Atmospheric System Research program at Pacific Northwest National Laboratory (PNNL). PNNL is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. NR 89 TC 21 Z9 21 U1 2 U2 44 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 19 PY 2014 VL 119 IS 9 BP 5559 EP 5582 DI 10.1002/2013JD020932 PG 24 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3QS UT WOS:000338340400035 ER PT J AU Pinto, JP Dibb, J Lee, BH Rappengluck, B Wood, EC Levy, M Zhang, RY Lefer, B Ren, XR Stutz, J Tsai, C Ackermann, L Golovko, J Herndon, SC Oakes, M Meng, QY Munger, JW Zahniser, M Zheng, J AF Pinto, J. P. Dibb, J. Lee, B. H. Rappenglueck, B. Wood, E. C. Levy, M. Zhang, R. -Y. Lefer, B. Ren, X. -R. Stutz, J. Tsai, C. Ackermann, L. Golovko, J. Herndon, S. C. Oakes, M. Meng, Q. -Y. Munger, J. W. Zahniser, M. Zheng, J. TI Intercomparison of field measurements of nitrous acid (HONO) during the SHARP campaign SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID TEXAS AIR-QUALITY; NITRIC-ACID; CHEMISTRY; HOUSTON; OZONE; INSTRUMENT; ABSORPTION; ATMOSPHERE; SULFATE; IMPACT AB Because of the importance of HONO as a radical reservoir, consistent and accurate measurements of its concentration are needed. As part of SHARP (Study of Houston Atmospheric Radical Precursors), time series of HONO were obtained by six different measurement techniques on the roof of the Moody Tower at the University of Houston. Techniques used were long path differential optical absorption spectroscopy (DOAS), stripping coil-visible absorption photometry (SC-AP), long path absorption photometry (LOPAP (R)), mist chamber/ion chromatography (MC-IC), quantum cascade-tunable infrared laser differential absorption spectroscopy (QC-TILDAS), and ion drift-chemical ionization mass spectrometry (ID-CIMS). Various combinations of techniques were in operation from 15 April through 31 May 2009. All instruments recorded a similar diurnal pattern of HONO concentrations with higher median and mean values during the night than during the day. Highest values were observed in the final 2 weeks of the campaign. Inlets for the MC-IC, SC-AP, and QC-TILDAS were collocated and agreed most closely with each other based on several measures. Largest differences between pairs of measurements were evident during the day for concentrations similar to 100 parts per trillion (ppt). Above similar to 200 ppt, concentrations from the SC-AP, MC-IC, and QC-TILDAS converged to within about 20%, with slightly larger discrepancies when DOAS was considered. During the first 2 weeks, HONO measured by ID-CIMS agreed with these techniques, but ID-CIMS reported higher values during the afternoon and evening of the final 4 weeks, possibly from interference from unknown sources. A number of factors, including building related sources, likely affected measured concentrations. C1 [Pinto, J. P.] US EPA, Natl Ctr Environm Assessment, Durham, NC 27711 USA. [Dibb, J.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Lee, B. H.] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. [Rappenglueck, B.; Lefer, B.; Ackermann, L.; Golovko, J.] Univ Houston, Dept Earth & Atmospher Sci, Houston, TX USA. [Wood, E. C.] Univ Massachusetts, Dept Environm Hlth Sci, Amherst, MA 01003 USA. [Wood, E. C.; Herndon, S. C.; Zahniser, M.] Aerodyne Res Inc, Billerica, MA USA. [Levy, M.; Zhang, R. -Y.; Zheng, J.] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX USA. [Ren, X. -R.] Univ Miami, Rosentiel Sch Marine & Atmospher Sci, Coral Gables, FL 33124 USA. [Stutz, J.; Tsai, C.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA USA. [Oakes, M.] Oak Ridge Inst Sci Educ, Oak Ridge, TN USA. [Meng, Q. -Y.] Univ Med & Dent New Jersey, Dept Environm & Occupat Hlth, Piscataway, NJ 08854 USA. [Munger, J. W.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. RP Pinto, JP (reprint author), US EPA, Natl Ctr Environm Assessment, Durham, NC 27711 USA. EM pinto.joseph@epa.gov RI Ren, Xinrong/E-7838-2015; Lee, Ben/G-7007-2014; Stutz, Jochen/K-7159-2014; Levy, Misti/G-8660-2014; Zhang, Renyi/A-2942-2011; Zheng, Jun/E-6772-2010; Munger, J/H-4502-2013 OI Ren, Xinrong/0000-0001-9974-1666; Lee, Ben/0000-0002-5057-2168; Levy, Misti/0000-0002-4832-7753; Munger, J/0000-0002-1042-8452 FU State of Texas under the Texas Emissions Reduction Plan (TERP) through the Texas Environmental Research Consortium (TERC); Office of Research and Development, U.S. EPA; Robert A. Welch Foundation [A-1417]; National Science Foundation [AGS-0914619]; National Natural Science Foundation of China [41275142] FX We would like to acknowledge the various participants in the SHARP campaign who made data available and Stephen McDow and David Svendsgaard for useful discussions. Funding for SHARP was provided by the State of Texas under the Texas Emissions Reduction Plan (TERP) through the Texas Environmental Research Consortium (TERC). The information in this document has been subjected to review by the National Center for Environmental Assessment, U.S. Environmental Protection Agency, and approved for publication. Approval does not signify that the contents reflect the views of the Agency, nor does mention of trade names or commercial products constitute endorsement or recommendation for use. In addition to data presented in the manuscript and SI, additional information can be obtained from the individual investigators cross referenced in the author list and Table 1. M.O. was supported by an appointment to the Research Participation Program at the Office of Research and Development, U.S. EPA, administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement between the U.S. DOE and EPA. R.Z. acknowledges additional support from the Robert A. Welch Foundation (A-1417). X. R. acknowledges partial support from the National Science Foundation (AGS-0914619). J.Z. acknowledges support from the National Natural Science Foundation of China (41275142). NR 43 TC 10 Z9 10 U1 8 U2 54 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 19 PY 2014 VL 119 IS 9 BP 5583 EP 5601 DI 10.1002/2013JD020287 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3QS UT WOS:000338340400036 ER PT J AU Jin, K Xiao, HY Zhang, Y Weber, WJ AF Jin, K. Xiao, H. Y. Zhang, Y. Weber, W. J. TI Effects of boron-nitride substrates on Stone-Wales defect formation in graphene: An ab initio molecular dynamics study SO APPLIED PHYSICS LETTERS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; ELECTRONIC-PROPERTIES; SIMULATION; SILICENE AB Ab initio molecular dynamics simulations are performed to investigate the effects of a boron nitride (BN) substrate on Stone-Wales (SW) defect formation and recovery in graphene. It is found that SW defects can be created by an off-plane recoil atom that interacts with the BN substrate. A mechanism with complete bond breakage for formation of SW defects in suspended graphene is also revealed for recoils at large displacement angles. In addition, further irradiation can result in recovery of the SW defects through a bond rotation mechanism in both graphene and graphene/BN, and the substrate has little effect on the recovery process. This study indicates that the BN substrate enhances the irradiation resistance of graphene. (C) 2014 AIP Publishing LLC. C1 [Jin, K.; Xiao, H. Y.; Zhang, Y.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Zhang, Y.; Weber, W. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Weber, WJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM wjweber@utk.edu RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division FX This work was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division. The simulations were performed using the supercomputer resources at the National Energy Research Scientific Computing Center located at Lawrence Berkeley National Laboratory. NR 35 TC 4 Z9 4 U1 1 U2 37 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 19 PY 2014 VL 104 IS 20 AR 203106 DI 10.1063/1.4879258 PG 4 WC Physics, Applied SC Physics GA AI8EQ UT WOS:000337140800059 ER PT J AU Middey, S Kareev, M Meyers, D Liu, X Cao, Y Tripathi, S Yazici, D Maple, MB Ryan, PJ Freeland, JW Chakhalian, J AF Middey, S. Kareev, M. Meyers, D. Liu, X. Cao, Y. Tripathi, S. Yazici, D. Maple, M. B. Ryan, P. J. Freeland, J. W. Chakhalian, J. TI Epitaxial stabilization of ultra thin films of electron doped manganites SO APPLIED PHYSICS LETTERS LA English DT Article ID PULSED-LASER DEPOSITION; X-RAY-ABSORPTION; PHASE-DIAGRAM; TRANSPORT; LA1-XCEXMNO3; PHYSICS; ND AB Ultra-thin films of the electron doped manganite La0.8Ce0.2MnO3 were grown in a layer-by-layer growth mode on SrTiO3 (001) substrates by pulsed laser interval deposition. High structural quality and surface morphology were confirmed by a combination of synchrotron based x-ray diffraction and atomic force microscopy. Resonant X-ray absorption spectroscopy measurements confirm the presence of Ce4+ and Mn2+ ions. In addition, the electron doping signature was corroborated by Hall effect measurements. All grown films show a ferromagnetic ground state as revealed by both dc magnetization and x-ray magnetic circular dichroism measurements and remain insulating contrary to earlier reports of a metal-insulator transition. Our results hint at the possibility of electron-hole asymmetry in the colossal magnetoresistive manganite phase diagram akin to the high-T-c cuprates. (C) 2014 AIP Publishing LLC. C1 [Middey, S.; Kareev, M.; Meyers, D.; Liu, X.; Cao, Y.; Tripathi, S.; Chakhalian, J.] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA. [Yazici, D.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Ryan, P. J.; Freeland, J. W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Middey, S (reprint author), Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA. EM smiddey@uark.edu RI Chakhalian, Jak/F-2274-2015; Middey, Srimanta/D-9580-2013 OI Middey, Srimanta/0000-0001-5893-0946 FU DOD-ARO [0402-17291]; U.S. Department of Energy, Office of Science [DEAC02-06CH11357]; U.S. Department of Energy [DE-FG02-04-ER46105] FX J.C. was supported by DOD-ARO under Grant No. 0402-17291. Work at the Advanced Photon Source, Argonne was supported by the U.S. Department of Energy, Office of Science under Grant No. DEAC02-06CH11357. Research at UCSD was supported by the U.S. Department of Energy under Grant No. DE-FG02-04-ER46105. NR 30 TC 3 Z9 3 U1 1 U2 39 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 19 PY 2014 VL 104 IS 20 AR 202409 DI 10.1063/1.4879456 PG 4 WC Physics, Applied SC Physics GA AI8EQ UT WOS:000337140800044 ER PT J AU Singh, S Fitzsimmons, MR Jeen, H Biswas, A AF Singh, Surendra Fitzsimmons, M. R. Jeen, H. Biswas, A. TI Influence of the magnitude and direction of applied elastic stress on the transport properties of (La0.4Pr0.6)(0.67)Ca0.33MnO3 thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID MANGANITES; PHYSICS AB We measured the electrical transport properties of single crystalline (La0.4Pr0.6)(0.67)Ca0.33MnO3 films grown on NdGaO3 (110) substrates as functions of temperature and applied stress. The metal-to-insulator transition (MIT) shifts to higher temperature with compressive stress and lower temperature with tensile stress. The resistance of the film in the metallic phase was strongly dependent upon the sign and direction of applied stress. We observed anisotropy in the responses of the MIT and resistance in the sample plane with current. The observed anisotropic response of the resistance to the bending stress can be explained by stress-induced rotation and growth of stripe ferromagnetic (metallic) domains. (C) 2014 AIP Publishing LLC. C1 [Singh, Surendra] Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. [Fitzsimmons, M. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Jeen, H.; Biswas, A.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Jeen, H.] Pusan Natl Univ, Dept Phys, Pusan 609735, South Korea. RP Singh, S (reprint author), Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. EM surendra@barc.gov.in RI Singh, Surendra/E-5351-2011 OI Singh, Surendra/0000-0001-5482-9744 FU Office of Basic Energy Science, U.S. Department of Energy, BES-DMS - Department of Energy's Office of Basic Energy Science; National Science Foundation [DMR-0804452]; DOE [DE-AC52-06NA25396] FX We thank J. Won for SEM measurements on our LPCMO film. This work was supported by the Office of Basic Energy Science, U.S. Department of Energy, BES-DMS funded by the Department of Energy's Office of Basic Energy Science and the National Science Foundation (DMR-0804452) (H. J. and A. B.). Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. NR 28 TC 4 Z9 4 U1 2 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 19 PY 2014 VL 104 IS 20 AR 201602 DI 10.1063/1.4879282 PG 5 WC Physics, Applied SC Physics GA AI8EQ UT WOS:000337140800017 ER PT J AU Kenanakis, G Zhao, R Katsarakis, N Kafesaki, M Soukoulis, CM Economou, EN AF Kenanakis, G. Zhao, R. Katsarakis, N. Kafesaki, M. Soukoulis, C. M. Economou, E. N. TI Optically controllable THz chiral metamaterials SO OPTICS EXPRESS LA English DT Article ID CIRCULAR-DICHROISM; PHOTONIC METAMATERIAL; DESIGNS AB Switchable and tunable chiral metamaterial response is numerically demonstrated here in different uniaxial chiral metamaterial structures operating in the THz regime. The structures are based on the bilayer conductor design and the tunable/switchable response is achieved by replacing parts of the metallic components of the structures by photoconducting Si, which can be transformed from an insulating to an almost conducting state through photoexcitation, achievable under external optical pumping. All the structures proposed and discussed here exhibit frequency regions with giant tunable circular dichroism, as well as regions with giant tunable optical activity, showing unique potential in the achievement of active THz polarization components, like tunable polarizers and polarization filters. (C) 2014 Optical Society of America C1 [Kenanakis, G.; Katsarakis, N.; Kafesaki, M.; Soukoulis, C. M.; Economou, E. N.] Fdn Res & Technol Hellas, Inst Elect Struct & Laser, Iraklion 71110, Crete, Greece. [Kenanakis, G.; Katsarakis, N.] Technol Educ Inst Crete, Sch Appl Technol, Dept Sci, Iraklion 71004, Crete, Greece. [Zhao, R.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, Blackett Lab, London SW7 2AZ, England. [Kafesaki, M.] Univ Crete, Dept Mat Sci & Technol, Iraklion 71003, Crete, Greece. [Soukoulis, C. M.] Iowa State Univ, USDOE, Ames Lab, Ames, IA 50011 USA. [Soukoulis, C. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Kenanakis, G (reprint author), Fdn Res & Technol Hellas, Inst Elect Struct & Laser, POB 1385, Iraklion 71110, Crete, Greece. EM gkenanak@iesl.forth.gr RI Kafesaki, Maria/E-6843-2012; Soukoulis, Costas/A-5295-2008; Kenanakis, George/G-1283-2010; Zhao, Rongkuo/B-5731-2008; Economou, Eleftherios /E-6374-2010 OI Kafesaki, Maria/0000-0002-9524-2576; Kenanakis, George/0000-0001-5843-3712; FU Greek GSRT project [ERC02-EXEL]; EU-project ENSEMBLE [213669]; EU-project By-Nanoera; Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) [DE-AC02-07CH11358]; Leverhulme Trust; Royal Commission for the Exhibition of 1851 Research Fellowship in Science or Engineering FX This work was supported by Greek GSRT project ERC02-EXEL and by the EU-projects ENSEMBLE (grant no 213669) and By-Nanoera. Work at Ames Laboratory was partially supported by the Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) under Contract No. DE-AC02-07CH11358 (computational studies). Author R. Z. acknowledges financial support by the Leverhulme Trust and the Royal Commission for the Exhibition of 1851 Research Fellowship in Science or Engineering. Author M. K. acknowledges useful discussions with Prof. Sergei Tretyakov. NR 29 TC 24 Z9 24 U1 5 U2 74 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 19 PY 2014 VL 22 IS 10 BP 12149 EP 12159 DI 10.1364/OE.22.012149 PG 11 WC Optics SC Optics GA AI6CP UT WOS:000336957700077 PM 24921336 ER PT J AU Zhang, P Goodwin, PM Werner, JH AF Zhang, P. Goodwin, P. M. Werner, J. H. TI Fast, super resolution imaging via Bessel-beam stimulated emission depletion microscopy SO OPTICS EXPRESS LA English DT Article ID OPTICAL RECONSTRUCTION MICROSCOPY; FIELD FLUORESCENCE MICROSCOPY; SINGLE-MOLECULE LOCALIZATION; ILLUMINATION MICROSCOPY; STRUCTURED ILLUMINATION; DIFFRACTION-LIMIT; PLANE ILLUMINATION; STED MICROSCOPY; THICK MEDIA; CELLS AB A substantial advantage of stimulated emission depletion (STED) microscopy over other super-resolution methods is that images can be acquired in real-time without any post-processing. However imaging speed and photodamage are two major concerns for STED imaging of whole cells. Here we propose a new microscopy method we have termed Bessel-Beam STED (or BB-STED) that overcomes both of these limitations of conventional STED microscopy. In the proposed method, rather than exciting a single STED spot in the sample, an entire line of the sample is illuminated. This line-scanning technique dramatically increases the speed of STED. In addition, plane-illumination by scanning of the line across the focal plane of a detection objective limits the light to a thin layer of the sample and thus significantly reduces photobleaching and photodamage above and below the focal plane compared to epi-illumination. Using the organic dye Atto647N as an example, we calculated the STED power required to break the diffraction limit. The results presented here will be used to guide future experimental designs. (C) 2014 Optical Society of America C1 [Zhang, P.; Goodwin, P. M.; Werner, J. H.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Werner, JH (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM jwerner@lanl.gov FU Los Alamos National Laboratory Directed Research and Development (LDRD); Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC52-06NA25396] FX This work was supported through Los Alamos National Laboratory Directed Research and Development (LDRD) and was performed at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory (Contract DE-AC52-06NA25396). NR 38 TC 11 Z9 11 U1 2 U2 48 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 19 PY 2014 VL 22 IS 10 BP 12398 EP 12409 DI 10.1364/OE.22.012398 PG 12 WC Optics SC Optics GA AI6CP UT WOS:000336957700100 PM 24921358 ER PT J AU Davids, PS Intravaia, F Dalvit, DAR AF Davids, P. S. Intravaia, F. Dalvit, D. A. R. TI Spoof polariton enhanced modal density of states in planar nanostructured metallic cavities SO OPTICS EXPRESS LA English DT Article ID FORMULATION; SURFACES; GRATINGS; LASER AB Spoof surface modes on nanostructured metallic surfaces are known to have tailorable dispersion dependent on the geometric characteristics of the periodic pattern. Here we examine the spoof plasmon dispersion on an isolated grating and a grating-planar mirror cavity configuration. The spoof polariton dispersion in the cavity is obtained using the scattering matrix approach, and the related differential modal density of states is introduced to obtain the mode dispersion and classify the cavity polariton modes. The grating-mirror cavity geometry is an example of periodically nanostructured metals above a planar ground plane. The properties discussed here are relevant for applications ranging from thin electromagnetic perfect absorbers to near-field radiative heat transfer. (C) 2014 Optical Society of America C1 [Davids, P. S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Intravaia, F.] Max Born Inst, D-12489 Berlin, Germany. [Dalvit, D. A. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Davids, PS (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM pdavids@sandia.gov RI Intravaia, Francesco/E-6500-2010 OI Intravaia, Francesco/0000-0001-7993-4698 FU Sandia's and Los Alamos' Laboratory Directed Research and Development (LDRD) program; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NNSA of the U.S. DOE at LANL [DEAC52-06NA25396]; European Union Marie Curie People program through the Career Integration Grant [631571] FX This research was funded by Sandia's and Los Alamos' Laboratory Directed Research and Development (LDRD) program. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Award No. DEAC52-06NA25396. F. I. acknowledges financial support from the European Union Marie Curie People program through the Career Integration Grant No. 631571. NR 37 TC 5 Z9 5 U1 0 U2 18 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 19 PY 2014 VL 22 IS 10 BP 12424 EP 12437 DI 10.1364/OE.22.012424 PG 14 WC Optics SC Optics GA AI6CP UT WOS:000336957700102 PM 24921360 ER PT J AU Huang, XJ Yan, HF Harder, R Hwu, YK Robinson, IK Chu, YS AF Huang, Xiaojing Yan, Hanfei Harder, Ross Hwu, Yeukuang Robinson, Ian K. Chu, Yong S. TI Optimization of overlap uniformness for ptychography SO OPTICS EXPRESS LA English DT Article ID PHASE RETRIEVAL; WAVE-FIELD; DIFFRACTION; MICROSCOPY; ERRORS; FOCUS AB We demonstrate the advantages of imaging with ptychography scans that follow a Fermat spiral trajectory. This scan pattern provides a more uniform coverage and a higher overlap ratio with the same number of scan points over the same area than the presently used mesh and concentric [13] patterns. Under realistically imperfect measurement conditions, numerical simulations show that the quality of the reconstructed image is improved significantly with a Fermat spiral compared with a concentric scan pattern. The result is confirmed by the performance enhancement with experimental data, especially under low-overlap conditions. These results suggest that the Fermat spiral pattern increases the quality of the reconstructed image and tolerance to data with imperfections. (C) 2014 Optical Society of America C1 [Huang, Xiaojing; Yan, Hanfei; Chu, Yong S.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Hwu, Yeukuang] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Robinson, Ian K.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. RP Huang, XJ (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM xjhuang@bnl.gov RI Huang, Xiaojing/K-3075-2012; Yan, Hanfei/F-7993-2011 OI Huang, Xiaojing/0000-0001-6034-5893; Yan, Hanfei/0000-0001-6824-0367 FU Department of Energy, Office of Basic Energy Sciences [DE-AC-02-98CH10886]; European Resarch Council [227711]; EPSRC; Thematic Project (Academia Sinica); National Program for Nanoscience and Nanotechnology (the National Science Council, Taiwan); US National Science Foundation [DMR-9724294]; US Department of Energy, Office of Basic Energy Sciences [DE-AC-02-06CH11357] FX Work at Brookhaven was supported by the Department of Energy, Office of Basic Energy Sciences under contract DE-AC-02-98CH10886. I. K. R. is supported by the European Resarch Council "nanosculpture" advanced grant 227711 and additional support from EPSRC. Work performed at Academia Sinica was supported by the Thematic Project (Academia Sinica), National Program for Nanoscience and Nanotechnology (the National Science Council, Taiwan). The measurements were carried out at APS beamline 34-ID-C, built with US National Science Foundation grant DMR-9724294 and operated by the US Department of Energy, Office of Basic Energy Sciences, under contract no. DE-AC-02-06CH11357. NR 30 TC 19 Z9 19 U1 1 U2 20 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 19 PY 2014 VL 22 IS 10 BP 12634 EP 12644 DI 10.1364/OE.22.012634 PG 11 WC Optics SC Optics GA AI6CP UT WOS:000336957700122 PM 24921380 ER PT J AU Stubben, CJ Micheva-Viteva, SN Shou, YL Buddenborg, SK Dunbar, JM Hong-Geller, E AF Stubben, Chris J. Micheva-Viteva, Sofiya N. Shou, Yulin Buddenborg, Sarah K. Dunbar, John M. Hong-Geller, Elizabeth TI Differential expression of small RNAs from Burkholderia thailandensis in response to varying environmental and stress conditions SO BMC GENOMICS LA English DT Article DE Small RNAs; Burkholderia; Microarray; Stress conditions; Bacterial adaptation; Gene expression ID ALKYL HYDROPEROXIDE REDUCTASE; SMALL NONCODING RNAS; ESCHERICHIA-COLI; HIGH-THROUGHPUT; VIRULENCE; MACROPHAGES; PREDICTION; RESISTANCE; MECHANISM; DISCOVERY AB Background: Bacterial small RNAs (sRNAs) regulate gene expression by base-pairing with downstream target mRNAs to attenuate translation of mRNA into protein at the post-transcriptional level. In response to specific environmental changes, sRNAs can modulate the expression levels of target genes, thus enabling adaptation of cellular physiology. Results: We profiled sRNA expression in the Gram-negative bacteria Burkholderia thailandensis cultured under 54 distinct growth conditions using a Burkholderia-specific microarray that contains probe sets to all intergenic regions greater than 90 bases. We identified 38 novel sRNAs and performed experimental validation on five sRNAs that play a role in adaptation of Burkholderia to cell stressors. In particular, the trans-encoded BTH_ s1 and s39 exhibited differential expression profiles dependent on growth phase and cell stimuli, such as antibiotics and serum. Furthermore, knockdown of the highly-expressed BTH_ s39 by antisense transcripts reduced B. thailandensis cell growth and attenuated host immune response upon infection, indicating that BTH_ s39 functions in bacterial metabolism and adaptation to the host. In addition, expression of cis-encoded BTH_ s13 and s19 found in the 5' untranslated regions of their cognate genes correlated with tight regulation of gene transcript levels. This sRNA-mediated downregulation of gene expression may be a conserved mechanism of post-transcriptional gene dosage control. Conclusions: These studies provide a broad analysis of differential Burkholderia sRNA expression profiles and illustrate the complexity of bacterial gene regulation in response to different environmental stress conditions. C1 [Stubben, Chris J.; Micheva-Viteva, Sofiya N.; Shou, Yulin; Buddenborg, Sarah K.; Dunbar, John M.; Hong-Geller, Elizabeth] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87544 USA. RP Hong-Geller, E (reprint author), Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87544 USA. EM ehong@lanl.gov FU LANL Laboratory-Directed Research and Development Directed Research Grants FX This work was supported by LANL Laboratory-Directed Research and Development Directed Research Grants to EH-G and JMD. NR 42 TC 3 Z9 4 U1 3 U2 13 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD MAY 19 PY 2014 VL 15 AR 385 DI 10.1186/1471-2164-15-385 PG 18 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA AI2HX UT WOS:000336679500001 PM 24884623 ER PT J AU Liu, TB Wang, XP Hoffmann, C DuBois, DL Bullock, RM AF Liu, Tianbiao Wang, Xiaoping Hoffmann, Christina DuBois, Daniel L. Bullock, R. Morris TI Heterolytic Cleavage of Hydrogen by an Iron Hydrogenase Model: An Fe-H H- N Dihydrogen Bond Characterized by Neutron Diffraction SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE enzyme models; hydrogen; hydrogenases; iron; neutron diffraction ID ASYMMETRIC TRANSFER HYDROGENATION; ACTIVE-SITE; ONLY HYDROGENASE; H-2; COMPLEX; ACTIVATION; RESOLUTION; REDUCTION; OXIDATION; CRYSTAL AB Hydrogenase enzymes in nature use hydrogen as a fuel, but the heterolytic cleavage of HH bonds cannot be readily observed in enzymes. Here we show that an iron complex with pendant amines in the diphosphine ligand cleaves hydrogen heterolytically. The product has a strong Fe-HH-N dihydrogen bond. The structure was determined by single-crystal neutron diffraction, and has a remarkably short HH distance of 1.489(10)angstrom between the protic N-H+ and hydridic Fe-H- part. The structural data for [CpC5F4NFeH((P2N2H)-N-tBu-H-tBu)](+) provide a glimpse of how the HH bond is oxidized or generated in hydrogenase enzymes. These results now provide a full picture for the first time, illustrating structures and reactivity of the dihydrogen complex and the product of the heterolytic cleavage of H-2 in a functional model of the active site of the [FeFe] hydrogenase enzyme. C1 [Liu, Tianbiao; DuBois, Daniel L.; Bullock, R. Morris] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Richland, WA 99352 USA. [Wang, Xiaoping; Hoffmann, Christina] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Liu, TB (reprint author), Pacific NW Natl Lab, Ctr Mol Electrocatalysis, POB 999, Richland, WA 99352 USA. EM Tianbiao.Liu@pnnl.gov; morris.bullock@pnnl.gov RI Wang, Xiaoping/E-8050-2012; Liu, Tianbiao/A-3390-2011; Bullock, R. Morris/L-6802-2016; hoffmann, christina/D-2292-2016 OI Wang, Xiaoping/0000-0001-7143-8112; Bullock, R. Morris/0000-0001-6306-4851; hoffmann, christina/0000-0002-7222-5845 FU Center for Molecular Electrocatalysis, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy. We thank Dr. Molly O'Hagan for assistance with HSQC NMR experiments and Dr. John A. S. Roberts for assistance with the electrochemical studies. Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract No. DE-AC05-00OR22725. NR 40 TC 47 Z9 47 U1 4 U2 82 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAY 19 PY 2014 VL 53 IS 21 BP 5300 EP 5304 DI 10.1002/anie.201402090 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA AH0KQ UT WOS:000335809200006 PM 24757087 ER PT J AU Baber, AE Yang, XF Kim, HY Mudiyanselage, K Soldemo, M Weissenrieder, J Senanayake, SD Al-Mahboob, A Sadowski, JT Evans, J Rodriguez, JA Liu, P Hoffmann, FM Chen, JGG Stacchiola, DJ AF Baber, Ashleigh E. Yang, Xiaofang Kim, Hyun You Mudiyanselage, Kumudu Soldemo, Markus Weissenrieder, Jonas Senanayake, Sanjaya D. Al-Mahboob, Abdullah Sadowski, Jerzy T. Evans, Jaime Rodriguez, Jose A. Liu, Ping Hoffmann, Friedrich M. Chen, Jingguang G. Stacchiola, Dario J. TI Stabilization of Catalytically Active Cu plus Surface Sites on TitaniumCopper Mixed-Oxide Films** SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE CO oxidation; IR spectroscopy; mixed oxides; scanning tunneling microscopy; surface chemistry ID TRANSITION-METAL OXIDES; PHOTOELECTRON-SPECTROSCOPY; PHOTOCATALYTIC ACTIVITY; AMBIENT-PRESSURE; CARBON-MONOXIDE; OXIDATION; COPPER; CO; ADSORPTION AB The oxidation of CO is the archetypal heterogeneous catalytic reaction and plays a central role in the advancement of fundamental studies, the control of automobile emissions, and industrial oxidation reactions. Copper-based catalysts were the first catalysts that were reported to enable the oxidation of CO at room temperature, but a lack of stability at the elevated reaction temperatures that are used in automobile catalytic converters, in particular the loss of the most reactive Cu+ cations, leads to their deactivation. Using a combined experimental and theoretical approach, it is shown how the incorporation of titanium cations in a Cu2O film leads to the formation of a stable mixed-metal oxide with a Cu+ terminated surface that is highly active for CO oxidation. C1 [Baber, Ashleigh E.; Yang, Xiaofang; Mudiyanselage, Kumudu; Senanayake, Sanjaya D.; Rodriguez, Jose A.; Chen, Jingguang G.; Stacchiola, Dario J.] BNL, Dept Chem, Upton, NY 11973 USA. [Soldemo, Markus; Weissenrieder, Jonas] KTH Royal Inst Technol, Stockholm, Sweden. [Kim, Hyun You; Al-Mahboob, Abdullah; Sadowski, Jerzy T.; Liu, Ping] BNL, CFN, Upton, NY 11973 USA. [Evans, Jaime] Cent Univ Venezuela, Fac Ciencias, Caracas 1020A, Venezuela. [Hoffmann, Friedrich M.] BMCC CUNY, Dept Sci, New York, NY 10007 USA. [Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. RP Stacchiola, DJ (reprint author), BNL, Dept Chem, Upton, NY 11973 USA. EM djs@bnl.gov RI Stacchiola, Dario/B-1918-2009; Senanayake, Sanjaya/D-4769-2009; Mudiyanselage, Kumudu/B-2277-2013 OI Stacchiola, Dario/0000-0001-5494-3205; Senanayake, Sanjaya/0000-0003-3991-4232; Mudiyanselage, Kumudu/0000-0002-3539-632X FU US DOE, Office of BES [DE-AC02-98CH10086]; Swedish Research Council (VR) FX Work carried out at BNL was supported by the US DOE, Office of BES (DE-AC02-98CH10086). Calculations were performed at the CFN. We are thankful to the Swedish Research Council (VR) for financial support. Jan Knudsen, Joachim Schnadt, and the Max-lab staff are acknowledged for their support. NR 20 TC 13 Z9 13 U1 9 U2 96 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAY 19 PY 2014 VL 53 IS 21 BP 5336 EP 5340 DI 10.1002/anie.201402435 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA AH0KQ UT WOS:000335809200014 PM 24719231 ER PT J AU Yaprak, D Spielberg, ET Backer, T Richter, M Mallick, B Klein, A Mudring, AV AF Yaprak, Damla Spielberg, Eike T. Baecker, Tobias Richter, Mark Mallick, Bert Klein, Axel Mudring, Anja-Verena TI A Roadmap to Uranium Ionic Liquids: Anti-Crystal Engineering SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE crystal structure; density functional calculations; ionic liquids; IR spectroscopy; uranium ID SOLUBILIZING METAL-OXIDES; URANYL COMPLEXES; 1-BUTYL-3-METHYLIMIDAZOLIUM CHLORIDE; BASIS-SETS; SPECTRA; DITHIOCARBAMATE; EXTRACTION; BEHAVIOR; RN AB In the search for uranium-based ionic liquids, tris(N,N-dialkyldithiocarbamato)uranylates have been synthesized as salts of the 1-butyl-3-methylimidazolium (C(4)mim) cation. As dithiocarbamate ligands binding to the UO22+ unit, tetra-, penta-, hexa-, and heptamethylenedithiocarbamates, N,N-diethyldithiocarbamate, N-methyl-N-propyldithiocarbamate, N-ethyl-N-propyldithiocarbamate, and N-methyl-N-butyldithiocarbamate have been explored. X-ray single-crystal diffraction allowed unambiguous structural characterization of all compounds except N-methyl-N-butyldithiocarbamate, which is obtained as a glassy material only. In addition, powder X-ray diffraction as well as vibrational and UV/Vis spectroscopy, supported by computational methods, were used to characterize the products. Differential scanning calorimetry was employed to investigate the phase-transition behavior depending on the N,N-dialkyldithiocarbamato ligand with the aim to establish structure-property relationships regarding the ionic liquid formation capability. Compounds with the least symmetric N,N-dialkyldithiocarbamato ligand and hence the least symmetric anions, tris(N-methyl-N-propyldithiocarbamato)uranylate, tris(N-ethyl-N-propyldithiocarbamato)uranylate, and tris(N-methyl-N-butyldithiocarbamato)uranylate, lead to the formation of (room-temperature) ionic liquids, which confirms that low-symmetry ions are indeed suitable to suppress crystallization. These materials combine low melting points, stable complex formation, and hydrophobicity and are therefore excellent candidates for nuclear fuel purification and recovery. C1 [Yaprak, Damla; Spielberg, Eike T.; Baecker, Tobias; Richter, Mark; Mallick, Bert; Mudring, Anja-Verena] Ruhr Univ Bochum, D-44801 Bochum, Germany. [Klein, Axel] Univ Cologne, Inst Anorgan Chem, D-50939 Cologne, Germany. [Mudring, Anja-Verena] Iowa State Univ, Ames Lab, Ames, IA 50014 USA. [Mudring, Anja-Verena] Crit Mat Inst, Ames Lab, Ames, IA 50014 USA. RP Mudring, AV (reprint author), Ruhr Univ Bochum, Univ Str 150, D-44801 Bochum, Germany. EM anja.mudring@rub.de RI Spielberg, Eike/D-9890-2015; OI Spielberg, Eike/0000-0002-3333-5814; Klein, Axel/0000-0003-0093-9619 FU Ruhr-Universitat Bochum; RUBION; Zentrale Einrichtung fur Ionenstrahlen und Radionuklide; DFG Excellence Cluster RESOLV FX A.-V.M. thanks the Ruhr-Universitat Bochum, in particular the RUBION, Zentrale Einrichtung fur Ionenstrahlen und Radionuklide, and DFG Excellence Cluster RESOLV for support. We thank Patrick Balzerowski for practical work during his internship. NR 47 TC 7 Z9 7 U1 4 U2 33 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD MAY 19 PY 2014 VL 20 IS 21 BP 6482 EP 6493 DI 10.1002/chem.201303333 PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA AG9XR UT WOS:000335773800036 PM 24737451 ER PT J AU Katukuri, VM Roszeitis, K Yushankhai, V Mitrushchenkov, A Stoll, H van Veenendaal, M Fulde, P van den Brink, J Hozoi, L AF Katukuri, Vamshi M. Roszeitis, Karla Yushankhai, Viktor Mitrushchenkov, Alexander Stoll, Hermann van Veenendaal, Michel Fulde, Peter van den Brink, Jeroen Hozoi, Liviu TI Electronic Structure of Low-Dimensional 4d(5) Oxides: Interplay of Ligand Distortions, Overall Lattice Anisotropy, and Spin-Orbit Interactions SO INORGANIC CHEMISTRY LA English DT Article ID BRANCHING RATIO; MAGNETIC-PROPERTIES; OPTICAL-ABSORPTION; PARENT COMPOUNDS; WAVE-FUNCTIONS; BASIS-SETS; CLUSTER; ATOMS; NIO; SUPERCONDUCTIVITY AB The electronic structure of the low-dimensional 4d(5) oxides Sr2RhO4 and Ca3CoRhO6 is herein investigated by embedded-cluster quantum chemistry calculations. A negative tetragonal-like t(2g) splitting is computed in Sr2RhO4 and a negative trigonal-like splitting is predicted for Ca3CoRhO6, in spite of having positive tetragonal distortions in the former material and cubic oxygen octahedra in the latter. Our findings bring to the foreground the role of longer-range crystalline anisotropy in generating noncubic potentials that compete with local distortions of the ligand cage, an issue not addressed in standard textbooks on crystal-field theory. We also show that sizable t(2g)(5)-t(2g)(4)e(g)(1) couplings via spin-orbit interactions produce in Sr2RhO4 (Z) = ground-state expectation values significantly larger than 1, quite similar to theoretical and experimental data for 5d(5) spin-orbit-driven oxides such as Sr2IrO4. On the other hand, in Ca3CoRhO6, the (Z) values are lower because of larger t(2g)-e(g) splittings. Future X-ray magnetic circular dichroism experiments on these 4d oxides will constitute a direct test for the (Z) values that we predict here, the importance of many-body t(2g)-e(g) couplings mediated by spin-orbit interactions, and the role of low-symmetry fields associated with the extended surroundings. C1 [Katukuri, Vamshi M.; Roszeitis, Karla; van den Brink, Jeroen; Hozoi, Liviu] IFW Dresden, Inst Theoret Solid State Phys, D-01069 Dresden, Germany. [Roszeitis, Karla; van den Brink, Jeroen] Tech Univ Dresden, Dept Phys, D-01069 Dresden, Germany. [Yushankhai, Viktor] Joint Inst Nucl Res, Dubna 141980, Russia. [Yushankhai, Viktor; Fulde, Peter] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. [Mitrushchenkov, Alexander] Univ Paris Est, Lab Modelisat & Simulat Multi Echelle, F-77454 Marne La Vallee 2, France. [Stoll, Hermann] Univ Stuttgart, Inst Theoret Chem, D-70550 Stuttgart, Germany. [van Veenendaal, Michel] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [van Veenendaal, Michel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Hozoi, L (reprint author), IFW Dresden, Inst Theoret Solid State Phys, Helmholtzstr 20, D-01069 Dresden, Germany. EM l.hozoi@ifw-dresden.de RI van den Brink, Jeroen/E-5670-2011; Katukuri, Vamshi Mohan/J-4048-2015 OI van den Brink, Jeroen/0000-0001-6594-9610; Katukuri, Vamshi Mohan/0000-0001-9355-0594 FU German Research Foundation (Deutsche Forschungsgemeinschaft) FX This article is dedicated to Prof. Ria Broer to honor her devoted career in Theoretical and Computational Chemistry. We thank N. A. Bogdanov and K. Koepernik for useful discussions. L.H. acknowledges financial support from the German Research Foundation (Deutsche Forschungsgemeinschaft). NR 78 TC 11 Z9 11 U1 1 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 19 PY 2014 VL 53 IS 10 BP 4833 EP 4839 DI 10.1021/ic402653f PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AH6KS UT WOS:000336240400008 PM 24779549 ER PT J AU Zheng, FS Logvenov, G Bozovic, I Zhu, YM He, JQ AF Zheng, Fengshan Logvenov, Gennady Bozovic, Ivan Zhu, Yimei He, Jiaqing TI Structural origin of enhanced critical temperature in ultrafine multilayers of cuprate superconducting films SO PHYSICAL REVIEW B LA English DT Article ID INTERFACE SUPERCONDUCTIVITY; THIN-FILMS; EPITAXIAL-STRAIN; TRANSITION; OXIDES; OXYGEN; LA2-XSRXCUO4; LA2CUO4 AB The interface layers of La2-xSrxCuO4 (LSCO) thin films epitaxially grown on LaSrAlO4 substrates by molecular beam epitaxy were investigated using transmission electron microscopy (TEM). In single-phase LSCO film, we observed an irregular layering sequence near the interface between the film and the substrate, as well as an abundance of oxygen vacancies in CuO2 layers. A multilayer LSCO film with a high critical temperature (T-c = 44.5 K) showed perfect interfaces between the sublayers. Furthermore, by combining scanning TEM, electron energy-loss spectroscopy, and electron holography, we show that there is little or no interdiffusion between the sublayers. The interfacial defects and oxygen vacancies reduce T-c, while the compressive strain in high-quality multilayers enhances T-c. C1 [Zheng, Fengshan; He, Jiaqing] South Univ Sci & Technol China, Dept Phys, Shenzhen 518055, Peoples R China. [Logvenov, Gennady; Bozovic, Ivan; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Zheng, FS (reprint author), South Univ Sci & Technol China, Dept Phys, Shenzhen 518055, Peoples R China. EM zhu@bnl.gov; he.jq@sustc.edu.cn RI Zheng, Fengshan/A-8942-2014 OI Zheng, Fengshan/0000-0001-7354-041X FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; South University of Science and Technology of China from the Shenzhen government; National 1000 Plan FX Research was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. J.H. thanks M. Schofield and H. Inada for fruitful discussions. This contribution was also supported by the startup of South University of Science and Technology of China from the Shenzhen government and National 1000 Plan for young scientists (J.H.). NR 33 TC 3 Z9 3 U1 5 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2014 VL 89 IS 18 AR 184509 DI 10.1103/PhysRevB.89.184509 PG 5 WC Physics, Condensed Matter SC Physics GA AM0UC UT WOS:000339561400003 ER PT J AU Chen, CY Davoudiasl, H Kim, D AF Chen, Chien-Yi Davoudiasl, Hooman Kim, Doojin TI Z with missing energy as a warped graviton signal at hadron colliders SO PHYSICAL REVIEW D LA English DT Article ID RANDALL-SUNDRUM MODEL; STANDARD MODEL; GAUGE BOSONS; BULK FIELDS; LHC; PHENOMENOLOGY; HIERARCHY; MODULUS; SEARCH; MASS AB We examine the reach at hadron colliders for the lightest warped Kaluza-Klein graviton G(1) in the Z(-> l(+)l(-))Z (->nu(nu) over bar channel, l = e,mu, within Randall-Sundrum models of hierarchy and flavor where the Standard Model gauge fields and fermions propagate in the 5D bulk. The reconstructed Z and the accompanying large missing energy allow for an efficient suppression of backgrounds. For reasonable parameters, an similar to 2(2.6) TeV G(1) can be discovered at 5s with 300 fb(-1) (3 ab(-1)) of 14 TeV LHC data via our " Z with missing energy" signal. Using this signal, the discovery reach for G(1) at a future 100 TeV pp collider is estimated to be as high as similar to 10 TeV. We discuss mass determination of the singly produced G(1) using the energy distribution of its visible (Z -> l(+)l(-)) decay product by adapting a recently proposed method. Based on our analysis, a mass measurement at the similar to 5% level with similar to 3 ab(-1) of the 14 TeV LHC data can be feasible. C1 [Chen, Chien-Yi; Davoudiasl, Hooman] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Kim, Doojin] Univ Florida, Dept Phys, Inst Fundamental Theory, Gainesville, FL 32611 USA. RP Kim, D (reprint author), Univ Florida, Dept Phys, Inst Fundamental Theory, Gainesville, FL 32611 USA. EM immworry@ufl.edu FU U.S. DOE [DE-AC02-98CH10886]; NSF [PHY-0652363]; LHC Theory Initiative graduate and postdoctoral fellowship (NSF) [PHY-0969510] FX We thank Kaustubh Agashe, James Gainer, Ian Lewis, Konstantin Matchev, Frank Paige, Gilad Perez, and Hong Zhang for helpful comments and discussions, Roberto Franceschini for extensive discussions on the fitting functions, and Hongsuk Kang, Myeonghun Park, and Young Soo Yoon for help with fitting and error estimation. We are especially grateful to Kaustubh Agashe for useful feedback on a draft version of this work and Oleg Antipin and Tuomas Hapola for help with the CalHEP model file. The work of C.-Y. C. and H. D. is supported in part by the U.S. DOE Grant No. DE-AC02-98CH10886. D. K. was supported in part by NSF Grant No. PHY-0652363 and also acknowledges the support from the LHC Theory Initiative graduate and postdoctoral fellowship (NSF Grant No. PHY-0969510). D. K. acknowledges the hospitality of Brookhaven National Laboratory during part of this project. NR 39 TC 9 Z9 9 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 16 PY 2014 VL 89 IS 9 AR 096007 DI 10.1103/PhysRevD.89.096007 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AM0UP UT WOS:000339562700003 ER PT J AU Crivellin, A D'Eramo, F Procura, M AF Crivellin, Andreas D'Eramo, Francesco Procura, Massimiliano TI New Constraints on Dark Matter Effective Theories from Standard Model Loops SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGGS; HEAVY; CANDIDATES; SEARCHES; PHYSICS; LHC AB We consider an effective field theory for a gauge singlet Dirac dark matter particle interacting with the standard model fields via effective operators suppressed by the scale Lambda greater than or similar to 1 TeV. We perform a systematic analysis of the leading loop contributions to spin-independent Dirac dark matter-nucleon scattering using renormalization group evolution between. and the low-energy scale probed by direct detection experiments. We find that electroweak interactions induce operator mixings such that operators that are naively velocity suppressed and spin dependent can actually contribute to spin-independent scattering. This allows us to put novel constraints on Wilson coefficients that were so far poorly bounded by direct detection. Constraints from current searches are already significantly stronger than LHC bounds, and will improve in the near future. Interestingly, the loop contribution we find is isospin violating even if the underlying theory is isospin conserving. C1 [Crivellin, Andreas] CERN, Div Theory, CH-1211 Geneva 23, Switzerland. [Crivellin, Andreas; Procura, Massimiliano] Univ Bern, Inst Theoret Phys, Albert Einstein Ctr Fundamental Phys, CH-3012 Bern, Switzerland. [D'Eramo, Francesco] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [D'Eramo, Francesco] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Crivellin, A (reprint author), CERN, Div Theory, CH-1211 Geneva 23, Switzerland. OI Crivellin, Andreas/0000-0002-6449-5845; D'Eramo, Francesco/0000-0001-8499-7685 FU Marie Curie Intra-European Fellowship of the European Community's 7th Framework Programme [PIEF-GA-2012-326948]; Swiss National Science Foundation; "Innovations-und Kooperationsprojekt C-13" of the Schweizerische Universitatskonferenz SUK/CRUS; Miller Institute for Basic Research in Science FX We acknowledge useful conversations with T. Cohen, U. Haisch, R. Hill, M. Hoferichter, E. Mereghetti, Y. Nomura, W. Shepherd, S. Shirai, M. Solon, T. Tait, J. Thaler, and L. Ubaldi. F. D. thanks the Aspen Center for Physics for hospitality when this work was initiated. A. C. is supported by a Marie Curie Intra-European Fellowship of the European Community's 7th Framework Programme under Contract No. (PIEF-GA-2012-326948). A. C. and M. P. are supported by the Swiss National Science Foundation and by the "Innovations-und Kooperationsprojekt C-13" of the Schweizerische Universitatskonferenz SUK/CRUS. F. D. is supported by the Miller Institute for Basic Research in Science. NR 63 TC 34 Z9 34 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 16 PY 2014 VL 112 IS 19 AR 191304 DI 10.1103/PhysRevLett.112.191304 PG 5 WC Physics, Multidisciplinary SC Physics GA AM0TM UT WOS:000339559700001 PM 24877928 ER PT J AU Anderson, BJ Korth, H Waters, CL Green, DL Merkin, VG Barnes, RJ Dyrud, LP AF Anderson, B. J. Korth, H. Waters, C. L. Green, D. L. Merkin, V. G. Barnes, R. J. Dyrud, L. P. TI Development of large-scale Birkeland currents determined from the Active Magnetosphere and Planetary Electrodynamics Response Experiment SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID FIELD-ALIGNED CURRENTS; MAGNETIC-FIELD; CURRENT DISTRIBUTIONS; MAGNETOMETER DATA; MHD SIMULATIONS; HIGH-LATITUDES; SUBSTORMS; IRIDIUM; SYSTEM; PARAMETERS AB The Active Magnetosphere and Planetary Electrodynamics Response Experiment uses magnetic field data from the Iridium constellation to derive the global Birkeland current distribution every 10 min. We examine cases in which the interplanetary magnetic field (IMF) rotated from northward to southward resulting in onsets of the Birkeland currents. Dayside Region 1/2 currents, totaling similar to 25% of the final current, appear within 20 min of the IMF southward turning and remain steady. Onset of nightside currents occurs 40 to 70 min after the dayside currents appear. Thereafter, the currents intensify at dawn, dusk, and on the dayside, yielding a fully formed Region 1/2 system similar to 30 min after the nightside onset. The results imply that the dayside Birkeland currents are driven by magnetopause reconnection, and the remainder of the system forms as magnetospheric return flows start and progress sunward, ultimately closing the Dungey convection cycle. C1 [Anderson, B. J.; Korth, H.; Merkin, V. G.; Barnes, R. J.; Dyrud, L. P.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Waters, C. L.; Green, D. L.] Univ Newcastle, Sch Math & Phys Sci, Newcastle, NSW 2300, Australia. [Green, D. L.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Dyrud, L. P.] Charles Stark Draper Lab Inc, Cambridge, MA 02139 USA. RP Anderson, BJ (reprint author), Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. EM brian.anderson@jhuapl.edu RI Merkin, Viacheslav/D-5982-2016 OI Merkin, Viacheslav/0000-0003-4344-5424 FU National Science Foundation [ATM-0739864, ATM-1003513] FX The AMPERE project was supported by the National Science Foundation under grant ATM-0739864 to the Johns Hopkins University Applied Physics Laboratory. Additional support was provided by NSF grant ATM-1003513. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the NSF. AMPERE data are available via http://ampere.jhuapl.edu. We thank the ACE team for the use of the MAG and SWEPAM data (http://www.srl.caltech.edu/ACE/ASC/level2/). Auroral and ring current indices are available via http://wdc.kugi.kyoto-u.ac.jp/wdc/Sec3.html. NR 37 TC 28 Z9 28 U1 0 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 16 PY 2014 VL 41 IS 9 BP 3017 EP 3025 DI 10.1002/2014GL059941 PG 9 WC Geosciences, Multidisciplinary SC Geology GA AK1SP UT WOS:000338196700001 ER PT J AU Wang, SY Hipps, L Gillies, RR Yoon, JH AF Wang, S. -Y. Hipps, Lawrence Gillies, Robert R. Yoon, Jin-Ho TI Probable causes of the abnormal ridge accompanying the 2013-2014 California drought: ENSO precursor and anthropogenic warming footprint SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID WESTERN UNITED-STATES; NORTH PACIFIC; REANALYSIS PROJECT; PRECIPITATION; TELECONNECTION; AMERICA; OSCILLATION; VARIABILITY; MODULATION; MECHANISM AB The 2013-2014 California drought was initiated by an anomalous high-amplitude ridge system. The anomalous ridge was investigated using reanalysis data and the Community Earth System Model (CESM). It was found that the ridge emerged from continual sources of Rossby wave energy in the western North Pacific starting in late summer and subsequently intensified into winter. The ridge generated a surge of wave energy downwind and deepened further the trough over the northeast U. S., forming a dipole. The dipole and associated circulation pattern is not linked directly with either El Nino-Southern Oscillation (ENSO) or Pacific Decadal Oscillation; instead, it is correlated with a type of ENSO precursor. The connection between the dipole and ENSO precursor has become stronger since the 1970s, and this is attributed to increased greenhouse gas loading as simulated by the CESM. Therefore, there is a traceable anthropogenic warming footprint in the enormous intensity of the anomalous ridge during winter 2013-2014 and the associated drought. C1 [Wang, S. -Y.; Gillies, Robert R.] Utah State Univ, Utah Climate Ctr, Logan, UT 84322 USA. [Wang, S. -Y.; Hipps, Lawrence; Gillies, Robert R.] Utah State Univ, Dept Plants Soils & Climate, Logan, UT 84322 USA. [Yoon, Jin-Ho] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Wang, SY (reprint author), Utah State Univ, Utah Climate Ctr, Logan, UT 84322 USA. EM simon.wang@usu.edu RI Wang, S.-Y. Simon/G-2566-2010; YOON, JIN-HO/A-1672-2009; OI YOON, JIN-HO/0000-0002-4939-8078; Hipps, Lawrence/0000-0002-7658-8571 FU WaterSMART [R13AC80039]; Utah Agricultural Experiment Station [8652]; Office of Science of the U.S. Department of Energy (DOE) as part of the Earth System Modeling program; DOE by Battelle Memorial Institute [DEAC05-76RLO1830]; National Science Foundation; Office of Science of the DOE; [NNX13AC37G] FX Observational data for this paper are available at NOAA's ESRL and CPC websites. Support came from grants NNX13AC37G and WaterSMART R13AC80039 and the Utah Agricultural Experiment Station (#8652). Jin-Ho Yoon was supported by the Office of Science of the U.S. Department of Energy (DOE) as part of the Earth System Modeling program. PNNL is operated for the DOE by Battelle Memorial Institute under Contract DEAC05-76RLO1830. The CESM project is supported by the National Science Foundation and the Office of Science of the DOE. Computational support from the National Energy Research Scientific Computing Center is greatly appreciated. NR 31 TC 59 Z9 59 U1 5 U2 60 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 16 PY 2014 VL 41 IS 9 BP 3220 EP 3226 DI 10.1002/2014GL059748 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AK1SP UT WOS:000338196700028 ER PT J AU Ceppi, P Zelinka, MD Hartmann, DL AF Ceppi, Paulo Zelinka, Mark D. Hartmann, Dennis L. TI The response of the Southern Hemispheric eddy-driven jet to future changes in shortwave radiation in CMIP5 SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID CLIMATE MODELS; CLOUD FEEDBACKS; POLEWARD SHIFT; LATITUDE AB A strong relationship is found between changes in the meridional gradient of absorbed shortwave radiation (ASR) and Southern Hemispheric jet shifts in 21st century climate simulations of CMIP5 (Coupled Model Intercomparison Project phase 5) coupled models. The relationship is such that models with increases in the meridional ASR gradient around the southern midlatitudes, and therefore increases in midlatitude baroclinicity, tend to produce a larger poleward jet shift. The ASR changes are shown to be dominated by changes in cloud properties, with sea ice declines playing a secondary role. We demonstrate that the ASR changes are the cause, and not the result, of the intermodel differences in jet response by comparing coupled simulations with experiments in which sea surface temperature increases are prescribed. Our results highlight the importance of reducing the uncertainty in cloud feedbacks in order to constrain future circulation changes. C1 [Ceppi, Paulo; Hartmann, Dennis L.] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. [Zelinka, Mark D.] Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA USA. RP Ceppi, P (reprint author), Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. EM ceppi@atmos.washington.edu RI Zelinka, Mark/C-4627-2011; Ceppi, Paulo/N-2282-2016 OI Zelinka, Mark/0000-0002-6570-5445; Ceppi, Paulo/0000-0002-3754-3506 FU National Science Foundation [AGS-0960497]; U.S. Department of Energy (DOE) by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Regional and Global Climate Modeling program of the U.S. DOE's Office of Science FX We thank the reviewers (Ed Gerber and anonymous) for their helpful comments. P. C. and D. L. H were supported by the National Science Foundation under grant AGS-0960497. M.D.Z.'s contribution was performed under the auspices of U.S. Department of Energy (DOE) by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 and was supported by the Regional and Global Climate Modeling program of the U.S. DOE's Office of Science. We acknowledge the World Climate Research Programme's Working Group on Coupled Modelling, which is responsible for CMIP, and we thank the climate modeling groups (listed in Table S1 of this paper) for producing and making available their model output. For CMIP the U. S. Department of Energy's Program for Climate Model Diagnosis and Intercomparison provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals. NR 27 TC 28 Z9 28 U1 0 U2 18 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. 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TI Measurement of the production of a W boson in association with a charm quark in pp collisions at root s=7 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Electroweak interaction; Hadron-Hadron Scattering; Charm physics ID PARTON DISTRIBUTIONS; MONTE-CARLO; LHC; DECAY; TEVATRON; PROTON; QCD AB The production of a W boson in association with a single charm quark is studied using 4.6 fb(-1) of pp collision data at root s = 7 TeV collected with the ATLAS detector at the Large Hadron Collider. In events in which a W boson decays to an electron or muon, the charm quark is tagged either by its semileptonic decay to a muon or by the presence of a charmed meson. The integrated and differential cross sections as a function of the pseudorapidity of the lepton from the W-boson decay are measured. Results are compared to the predictions of next-to-leading-order QCD calculations obtained from various parton distribution function parameterisations. The ratio of the strange-to-down sea-quark distributions is determined to be 0.96(-0.30)(+0.26) at Q (2) = 1.9 GeV2, which supports the hypothesis of an SU(3)-symmetric composition of the light-quark sea. Additionally, the cross-section ratio sigma(W (+) +)/sigma(W (-) + c) is compared to the predictions obtained using parton distribution function parameterisations with different assumptions about the s-(s) over bar quark asymmetry. C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Chan, K.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. 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S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Ancu, L. S.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mclaughlan, T.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Giacobbe, B.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Abajyan, T.; Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Filho, L. Manhaes de Andrade] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Cavendish Lab, Cambridge, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Banfi, D.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; MoEnig, K.; Naumann, T.; Peschke, R.; Petit, E.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Barber, T.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruhr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Miucci, A.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, E.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St. Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Vazquez Schroeder, T.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69115 Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-69115 Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Hasib, A.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; KoEnig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; SchaEfer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S. G.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S. G.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J. -F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Davies, M.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. 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G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Hasib, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C. -L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Hasib, A.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Marchese, F.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J. -P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energie A, Inst Rech Lois Fondamentales Univers, DSM IRFU, Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Huang, Y.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, A.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Ottawa, ON, Canada. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Experimentalphys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. EM atlas.publications@cern.ch RI Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Ferrando, James/A-9192-2012; Boyko, Igor/J-3659-2013; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Mikestikova, Marcela/H-1996-2014; Warburton, Andreas/N-8028-2013; Kuday, Sinan/C-8528-2014; Turchikhin, Semen/O-1929-2013; Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Kuleshov, Sergey/D-9940-2013; Gabrielli, Alessandro/H-4931-2012; Castro, Nuno/D-5260-2011; Staroba, Pavel/G-8850-2014; Lei, Xiaowen/O-4348-2014; Doyle, Anthony/C-5889-2009; Di Domenico, Antonio/G-6301-2011; de Groot, Nicolo/A-2675-2009; Wemans, Andre/A-6738-2012; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; OI Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Ferrando, James/0000-0002-1007-7816; Boyko, Igor/0000-0002-3355-4662; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Warburton, Andreas/0000-0002-2298-7315; Kuday, Sinan/0000-0002-0116-5494; Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Kuleshov, Sergey/0000-0002-3065-326X; Gabrielli, Alessandro/0000-0001-5346-7841; Castro, Nuno/0000-0001-8491-4376; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Coccaro, Andrea/0000-0003-2368-4559 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF Austria; FWF Austria; ANAS, Azerbaijan FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3- CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America.; The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier- 1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier- 2 facilities worldwide. NR 79 TC 1 Z9 1 U1 7 U2 94 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 16 PY 2014 IS 5 BP 1 EP 67 DI 10.1007/JHEP05(2014)068 PG 67 WC Physics, Particles & Fields SC Physics GA AI3XS UT WOS:000336799600001 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, S Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, B Adamczyk, L Adams, D Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, S Ahmad, A Ahmadov, F Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, B Alviggi, MG Amako, K Coutinho, Y Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS 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TI Search for direct production of charginos, neutralinos and sleptons in final states with two leptons and missing transverse momentum in pp collisions at root s=8TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry; Hadron-Hadron Scattering ID DYNAMICAL SUPERSYMMETRY BREAKING; SYMMETRY-BREAKING; HADRON COLLIDERS; SUPERGAUGE TRANSFORMATIONS; E(+)E(-) COLLISIONS; MEASURING MASSES; PARTICLE; MODEL; ENERGY; MSSM AB Searches for the electroweak production of charginos, neutralinos and sleptons in final states characterized by the presence of two leptons (electrons and muons) and missing transverse momentum are performed using 20.3 fb(-1) of proton-proton collision data at root s = 8 TeV recorded with the ATLAS experiment at the Large Hadron Collider. No significant excess beyond Standard Model expectations is observed. 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G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Banfi, D.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gorini, E.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand 2, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Blaise Pascal, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. C.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, S.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Petit, E.; Radescu, V.; Rubinskiy, I.; Ruschke, A.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Ahmad, A.; Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St. Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimares; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69115 Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-69115 Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Morris, J. D.; Piccaro, E.; Salamanna, G.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, C.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Ahmad, A.; Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Koenig, S.; Kowpke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Robinson, D.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, Z.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J. -F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Tikhomirov, V. O.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, B.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Ahmad, A.; Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C. -L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Particle Phys Dept, Rutherford Appleton Lab, Didcot, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J. -P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energie A, Inst Rech Lois Fondamentales Univers, DSM IRFU, Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lobodzinska, E.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, A.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Farooque, T.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, A.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Ahmad, A.; Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; De Sanctis, U.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Jenni, P.] CERN, Geneva, Switzerland. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Sch Phys Sci, Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Nucl & Particle Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Experimentalphys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. 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Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Peleganchuk, Sergey/J-6722-2014; Ferrando, James/A-9192-2012; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Li, Liang/O-1107-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; OI Smirnova, Oxana/0000-0003-2517-531X; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Kuleshov, Sergey/0000-0002-3065-326X; Gabrielli, Alessandro/0000-0001-5346-7841; Castro, Nuno/0000-0001-8491-4376; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Bosman, Martine/0000-0002-7290-643X; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Warburton, Andreas/0000-0002-2298-7315; Kuday, Sinan/0000-0002-0116-5494; Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Peleganchuk, Sergey/0000-0003-0907-7592; Ferrando, James/0000-0002-1007-7816; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Coccaro, Andrea/0000-0003-2368-4559; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Li, Liang/0000-0001-6411-6107; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Walsh, Brian/0000-0003-1689-2309; Filthaut, Frank/0000-0003-3338-2247; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Hays, Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Wang, Kuhan/0000-0002-6151-0034; Grohsjean, Alexander/0000-0003-0748-8494; La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society and Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 104 TC 53 Z9 53 U1 10 U2 98 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 16 PY 2014 IS 5 BP 1 EP 52 AR 071 DI 10.1007/JHEP05(2014)071 PG 52 WC Physics, Particles & Fields SC Physics GA AI1ZJ UT WOS:000336654400001 ER PT J AU Ostoja-Starzewski, M Li, J Joumaa, H Demmie, PN AF Ostoja-Starzewski, Martin Li, Jun Joumaa, Hady Demmie, Paul N. TI From fractal media to continuum mechanics SO ZAMM-ZEITSCHRIFT FUR ANGEWANDTE MATHEMATIK UND MECHANIK LA English DT Article DE Fractals; continuum mechanics; dimensional regularization; balance laws ID FRACTIONAL CALCULUS; SCALING LAWS; DISORDERED MATERIALS; PRODUCT MEASURES; MODEL; SURFACES; GEOMETRY; SOLIDS; FLUID; VISCOELASTICITY AB This paper presents an overview of modeling fractal media by continuum mechanics using the method of dimensional regularization. The basis of this method is to express the balance laws for fractal media in terms of fractional integrals and, then, convert them to integer-order integrals in conventional (Euclidean) space. Following an account of this method, we develop balance laws of fractal media (continuity, linear and angular momenta, energy, and second law) and discuss wave equations in several settings (1d and 3d wave motions, fractal Timoshenko beam, and elastodynamics under finite strains). We then discuss extremum and variational principles, fracture mechanics, and equations of turbulent flow in fractal media. In all the cases, the derived equations for fractal media depend explicitly on fractal dimensions and reduce to conventional forms for continuous media with Euclidean geometries upon setting the dimensions to integers. We also point out relations and potential extensions of dimensional regularization to other models of microscopically heterogeneous physical systems. C1 [Ostoja-Starzewski, Martin] Univ Illinois, Dept Mech Sci & Engn, Inst Condensed Matter Theory, Urbana, IL 61801 USA. [Ostoja-Starzewski, Martin] Univ Illinois, Beckman Inst, Urbana, IL 61801 USA. [Li, Jun] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Joumaa, Hady] Univ Illinois, Dept Mech Sci & Engn, Urbana, IL 61801 USA. Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ostoja-Starzewski, M (reprint author), Univ Illinois, Dept Mech Sci & Engn, Inst Condensed Matter Theory, Urbana, IL 61801 USA. EM martinos@illinois.edu OI Ostoja-Starzewski, Martin/0000-0002-3493-363X FU Sandia-DTRA [HDTRA1-08-10-BRCWMD]; NSF [CMMI-1030940] FX This work was made possible by the support from Sandia-DTRA (grant HDTRA1-08-10-BRCWMD) and the NSF (grant CMMI-1030940). Also, the support of the first author as Timoshenko Distinguished Visitor in the Division of Mechanics and Computation, Stanford University, is gratefully acknowledged. NR 82 TC 12 Z9 12 U1 3 U2 17 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0044-2267 EI 1521-4001 J9 ZAMM-Z ANGEW MATH ME JI ZAMM-Z. Angew. Math. Mech. PD MAY 16 PY 2014 VL 94 IS 5 SI SI BP 373 EP 401 DI 10.1002/zamm.201200164 PG 29 WC Mathematics, Applied; Mechanics SC Mathematics; Mechanics GA AG7DS UT WOS:000335578900002 ER PT J AU Hanke, A Hamann, E Sharma, R Geelhoed, JS Hargesheimer, T Kraft, B Meyer, V Lenk, S Osmers, H Wu, R Makinwa, K Hettich, RL Banfield, JF Tegetmeyer, HE Strous, M AF Hanke, Anna Hamann, Emmo Sharma, Ritin Geelhoed, Jeanine S. Hargesheimer, Theresa Kraft, Beate Meyer, Volker Lenk, Sabine Osmers, Harald Wu, Rong Makinwa, Kofi Hettich, Robert L. Banfield, Jillian F. Tegetmeyer, Halina E. Strous, Marc TI Recoding of the stop codon UGA to glycine by a BD1-5/SN-2 bacterium and niche partitioning between Alpha- and Gammaproteobacteria in a tidal sediment microbial community naturally selected in a laboratory chemostat SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE continuous culture; enrichment; chemostat; Roseobacter; Maritimibacter; stop codon ID TARGETED OLIGONUCLEOTIDE PROBES; IN-SITU HYBRIDIZATION; SINGLE-CELL GENOMICS; PEPTIDE IDENTIFICATION; WADDEN SEA; GEN. NOV.; METABOLISM; SEQUENCES; WATERS; ALIGNMENT AB Sandy coastal sediments are global hotspots for microbial mineralization of organic matter and denitrification. These sediments are characterized by advective porewater flow, tidal cycling and an active and complex microbial community. Metagenomic sequencing of microbial communities sampled from such sediments showed that potential sulfur oxidizing Gammaproteobacteria and members of the enigmatic BD1-5/SN-2 candidate phylum were abundant in situ (> 10% and similar to 2% respectively). By mimicking the dynamic oxic/anoxic environmental conditions of the sediment in a laboratory chemostat, a simplified microbial community was selected from the more complex inoculum. Metagenomics, proteomics and fluorescence in situ hybridization showed that this simplified community contained both a potential sulfur oxidizing Gammaproteobacteria (at 24 +/- 2% abundance) and a member of the BD1-5/SN-2 candidate phylum (at 7 +/- 6% abundance). Despite the abundant supply of organic substrates to the chemostat, proteomic analysis suggested that the selected gammaproteobacterium grew partially autotrophically and performed hydrogen/formate oxidation. The enrichment of a member of the BD1-5/SN-2 candidate phylum enabled, for the first time, direct microscopic observation by fluorescent in situ hybridization and the experimental validation of the previously predicted translation of the stop codon UGA into glycine. C1 [Hanke, Anna; Hamann, Emmo; Geelhoed, Jeanine S.; Hargesheimer, Theresa; Kraft, Beate; Meyer, Volker; Lenk, Sabine; Osmers, Harald; Tegetmeyer, Halina E.; Strous, Marc] Max Planck Inst Marine Microbiol, Microbial Fitness Grp, Bremen, Germany. [Sharma, Ritin; Hettich, Robert L.] Univ Tennessee, UT ORNL Grad Sch Genome Sci & Technol, Knoxville, TN USA. [Sharma, Ritin; Hettich, Robert L.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA. [Wu, Rong; Makinwa, Kofi] Delft Univ Technol, Fac Elect Engn Math & Comp Sci, Delft, Netherlands. [Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Tegetmeyer, Halina E.; Strous, Marc] Univ Bielefeld, Ctr Biotechnol, D-33615 Bielefeld, Germany. [Strous, Marc] Univ Calgary, Dept Geosci, Calgary, AB T2N 1N4, Canada. RP Strous, M (reprint author), Univ Calgary, Dept Geosci, Campus Dr 7200 NW, Calgary, AB T2N 1N4, Canada. EM mstrous@ucalgary.ca RI Hettich, Robert/N-1458-2016; Strous, Marc/B-4064-2017 OI Tegetmeyer, Halina E./0000-0003-1970-4457; Kraft, Beate/0000-0003-0310-5206; Hettich, Robert/0000-0001-7708-786X; Strous, Marc/0000-0001-9600-3828 FU ERC starting grant (MASEM) [242635]; Royal Dutch Society for Arts and Sciences (KNAW); German Federal State North Rhine Westfalia; U.S. Department of Energy, Office of Biological and Environmental Research FX The support of Ines Kattelmann and Regina Varenhorst in metagenomic sequencing and analysis is kindly acknowledged. Also acknowledged is the help of Jessika Fussel with respect to NOx measurements. This research was funded by an ERC starting grant to Marc Strous (MASEM, 242635), the Royal Dutch Society for Arts and Sciences (KNAW) and the German Federal State North Rhine Westfalia. The MS-based proteomics at ORNL was supported by funding from the U.S. Department of Energy, Office of Biological and Environmental Research. NR 60 TC 7 Z9 7 U1 2 U2 16 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAY 16 PY 2014 VL 5 AR 231 DI 10.3389/fmicb.2014.00231 PG 17 WC Microbiology SC Microbiology GA AH4HM UT WOS:000336088000001 PM 24904545 ER PT J AU Ragauskas, AJ Beckham, GT Biddy, MJ Chandra, R Chen, F Davis, MF Davison, BH Dixon, RA Gilna, P Keller, M Langan, P Naskar, AK Saddler, JN Tschaplinski, TJ Tuskan, GA Wyman, CE AF Ragauskas, Arthur J. Beckham, Gregg T. Biddy, Mary J. Chandra, Richard Chen, Fang Davis, Mark F. Davison, Brian H. Dixon, Richard A. Gilna, Paul Keller, Martin Langan, Paul Naskar, Amit K. Saddler, Jack N. Tschaplinski, Timothy J. Tuskan, Gerald A. Wyman, Charles E. TI Lignin Valorization: Improving Lignin Processing in the Biorefinery SO SCIENCE LA English DT Review ID CINNAMYL ALCOHOL-DEHYDROGENASE; CELL-WALL COMPOSITION; IONIC LIQUID; LIGNOCELLULOSIC BIOMASS; KRAFT LIGNIN; BIOSYNTHESIS PERTURBATIONS; HYDROTHERMAL PRETREATMENT; CARBOHYDRATE COMPLEXES; ARABIDOPSIS-THALIANA; BIOFUEL PRODUCTION AB Research and development activities directed toward commercial production of cellulosic ethanol have created the opportunity to dramatically increase the transformation of lignin to value-added products. Here, we highlight recent advances in this lignin valorization effort. Discovery of genetic variants in native populations of bioenergy crops and direct manipulation of biosynthesis pathways have produced lignin feedstocks with favorable properties for recovery and downstream conversion. Advances in analytical chemistry and computational modeling detail the structure of the modified lignin and direct bioengineering strategies for future targeted properties. Refinement of biomass pretreatment technologies has further facilitated lignin recovery, and this coupled with genetic engineering will enable new uses for this biopolymer, including low-cost carbon fibers, engineered plastics and thermoplastic elastomers, polymeric foams, fungible fuels, and commodity chemicals. C1 [Ragauskas, Arthur J.] Georgia Inst Technol, Inst Paper Sci & Technol, Sch Chem & Biochem, BioEnergy Sci Ctr, Atlanta, GA 30332 USA. [Beckham, Gregg T.; Biddy, Mary J.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80402 USA. [Beckham, Gregg T.; Biddy, Mary J.] Natl Renewable Energy Lab, Natl Adv Biofuels Consortium, Golden, CO 80402 USA. [Chandra, Richard; Saddler, Jack N.] Univ British Columbia, Dept Wood Sci, Vancouver, BC V6T 1Z4, Canada. [Chen, Fang; Dixon, Richard A.] Univ N Texas, Dept Biol Sci, BioEnergy Sci Ctr, Denton, TX 76203 USA. [Davis, Mark F.] Natl Renewable Energy Lab, BioEnergy Sci Ctr, Golden, CO 80402 USA. [Davis, Mark F.] Natl Renewable Energy Lab, Natl Adv Biofuels Consortium, Golden, CO 80402 USA. [Davison, Brian H.; Gilna, Paul; Tschaplinski, Timothy J.; Tuskan, Gerald A.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Biosci Div, Oak Ridge, TN 37831 USA. [Keller, Martin] Oak Ridge Natl Lab, Energy & Environm Sci Directorate, Oak Ridge, TN 37831 USA. [Langan, Paul] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Naskar, Amit K.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Wyman, Charles E.] Univ Calif Riverside, BioEnergy Sci Ctr, Ctr Environm Res & Technol, Riverside, CA 92507 USA. [Wyman, Charles E.] Univ Calif Riverside, Dept Chem & Environm Engn, Riverside, CA 92507 USA. RP Ragauskas, AJ (reprint author), Georgia Inst Technol, Inst Paper Sci & Technol, Sch Chem & Biochem, BioEnergy Sci Ctr, Atlanta, GA 30332 USA. EM ragauskas@chemistry.gatech.edu RI Tuskan, Gerald/A-6225-2011; Langan, Paul/N-5237-2015; Davison, Brian/D-7617-2013; Gilna, Paul/I-3608-2016 OI Tuskan, Gerald/0000-0003-0106-1289; Tschaplinski, Timothy/0000-0002-9540-6622; davis, mark/0000-0003-4541-9852; Langan, Paul/0000-0002-0247-3122; Davison, Brian/0000-0002-7408-3609; Gilna, Paul/0000-0002-6542-0191 FU U.S. Department of Energy (DOE); Genomic Science Program, Office of Biological and Environmental Research, DOE [FWP ERKP752]; DOE BioEnergy Technologies Office through American Recovery and Reinvestment Act Funds; DOE; BioEnergy Science Center (BESC); Office of Biological and Environmental Research in the DOE Office of Science FX This work is supported by several agencies, including the Laboratory Directed Research and Development Programs at ORNL and NREL [ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy (DOE); NREL is managed by Alliance for Sustainable Energy, LLC, for DOE]; Genomic Science Program, Office of Biological and Environmental Research, DOE, under FWP ERKP752; National Advanced Biofuels Consortium, which is funded by DOE BioEnergy Technologies Office through American Recovery and Reinvestment Act Funds, and DOE and the BioEnergy Science Center (BESC). BESC is a DOE Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. NR 127 TC 427 Z9 434 U1 154 U2 889 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 16 PY 2014 VL 344 IS 6185 BP 709 EP + AR 1246843 DI 10.1126/science.1246843 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH1WQ UT WOS:000335912900030 PM 24833396 ER PT J AU Jones, AM Xuan, YH Xu, M Wang, RS Ho, CH Lalonde, S You, CH Sardi, MI Parsa, SA Smith-Valle, E Su, TY Frazer, KA Pilot, G Pratelli, R Grossmann, G Acharya, BR Hu, HC Engineer, C Villiers, F Ju, CL Takeda, K Su, Z Dong, QF Assmann, SM Chen, J Kwak, JM Schroeder, JI Albert, R Rhee, SY Frommer, WB AF Jones, Alexander M. Xuan, Yuanhu Xu, Meng Wang, Rui-Sheng Ho, Cheng-Hsun Lalonde, Sylvie You, Chang Hun Sardi, Maria I. Parsa, Saman A. Smith-Valle, Erika Su, Tianying Frazer, Keith A. Pilot, Guillaume Pratelli, Rejane Grossmann, Guido Acharya, Biswa R. Hu, Heng-Cheng Engineer, Cawas Villiers, Florent Ju, Chuanli Takeda, Kouji Su, Zhao Dong, Qunfeng Assmann, Sarah M. Chen, Jin Kwak, June M. Schroeder, Julian I. Albert, Reka Rhee, Seung Y. Frommer, Wolf B. TI Border Control-A Membrane-Linked Interactome of Arabidopsis SO SCIENCE LA English DT Article ID PROTEIN INTERACTIONS; ABSCISIC-ACID; SIGNAL-TRANSDUCTION; GENE-EXPRESSION; YEAST; NETWORK; KINASE; MAP; ENDOCYTOSIS; THALIANA AB Cellular membranes act as signaling platforms and control solute transport. Membrane receptors, transporters, and enzymes communicate with intracellular processes through protein-protein interactions. Using a split-ubiquitin yeast two-hybrid screen that covers a test-space of 6.4 x 10(6) pairs, we identified 12,102 membrane/signaling protein interactions from Arabidopsis. Besides confirmation of expected interactions such as heterotrimeric G protein subunit interactions and aquaporin oligomerization, >99% of the interactions were previously unknown. Interactions were confirmed at a rate of 32% in orthogonal in planta split-green flourescent protein interaction assays, which was statistically indistinguishable from the confirmation rate for known interactions collected from literature (38%). Regulatory associations in membrane protein trafficking, turnover, and phosphorylation include regulation of potassium channel activity through abscisic acid signaling, transporter activity by a WNK kinase, and a brassinolide receptor kinase by trafficking-related proteins. These examples underscore the utility of the membrane/signaling protein interaction network for gene discovery and hypothesis generation in plants and other organisms. C1 [Jones, Alexander M.; Xuan, Yuanhu; Xu, Meng; Ho, Cheng-Hsun; Lalonde, Sylvie; You, Chang Hun; Sardi, Maria I.; Parsa, Saman A.; Smith-Valle, Erika; Su, Tianying; Frazer, Keith A.; Pilot, Guillaume; Pratelli, Rejane; Grossmann, Guido; Chen, Jin; Rhee, Seung Y.; Frommer, Wolf B.] Carnegie Inst Sci, Dept Plant Biol, Stanford, CA 94305 USA. [Wang, Rui-Sheng; Albert, Reka] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Pilot, Guillaume; Pratelli, Rejane] Virginia Polytech Inst & State Univ, Dept Plant Pathol Physiol & Weed Sci, Blacksburg, VA 24061 USA. [Acharya, Biswa R.; Su, Zhao; Assmann, Sarah M.] Penn State Univ, Dept Biol, University Pk, PA 16802 USA. [Hu, Heng-Cheng; Villiers, Florent; Ju, Chuanli; Takeda, Kouji; Kwak, June M.] Univ Maryland, Dept Cell Biol & Mol Genet, College Pk, MD 20742 USA. [Engineer, Cawas; Schroeder, Julian I.] Univ Calif San Diego, Div Biol Sci, Cell & Dev Biol Sect, La Jolla, CA 92093 USA. [Dong, Qunfeng] Univ N Texas, Dept Biol Sci, Denton, TX 76203 USA. [Chen, Jin] Michigan State Univ, US DOE, Plant Res Lab, E Lansing, MI 48824 USA. [Chen, Jin] Michigan State Univ, Dept Comp Sci & Engn, E Lansing, MI 48824 USA. [Kwak, June M.] Daegu Gyeongbuk Inst Sci & Technol, Dept New Biol, Ctr Plant Aging Res, Inst Basic Sci, Taegu 711873, South Korea. RP Rhee, SY (reprint author), Carnegie Inst Sci, Dept Plant Biol, 290 Panama St, Stanford, CA 94305 USA. EM srhee@carnegiescience.edu; wfrommer@stanford.edu RI Albert, Reka/E-2195-2011; Kwak, June/G-8332-2011; Grossmann, Guido/D-3537-2014; Frommer, Wolf B/A-8256-2008; OI Albert, Reka/0000-0002-9485-0828; Grossmann, Guido/0000-0001-7529-9244; Jones, Alexander/0000-0002-3662-2915; Schroeder, Julian/0000-0002-3283-5972; Pilot, Guillaume/0000-0001-7520-1059 FU National Science Foundation (NSF) Arabidopsis grant [MCB-0618402, MCB-1052348]; [NSF-MCB-1021677]; [NSF-MCB-0918220]; [NSF-MCB-1121612] FX We thank W. Monsell (Pennsylvania State University) and Y. S. Han (University of Maryland) for technical assistance and K. Revanna and V. Desu (University of North Texas) for assistance with the MIND web portal development. This work was made possible by a National Science Foundation (NSF) Arabidopsis 2010 grant (MCB-0618402) to W.B.F., S.M.A., R.A., J.M.K., S.Y.R., and J.I.S. and NSF Arabidopsis 2010 grant (MCB-1052348) to W.B.F. and S.Y.R., with partial support from NSF-MCB-1021677 (W.B.F.), NSF-MCB-0918220 (J.I.S.) and NSF-MCB-1121612 (S.M.A. and R.A.). Because of the large number of constructs, we are not able to distribute individual clones. We make split-ubiquitin system vectors and an Arabidopsis ORF collection available through the Arabidopsis Biological Resource Center (https://abrc.osu.edu) and split-GFP assay vectors available through AddGene (www.addgene.org). Instructions for acquiring other materials as well as a materials transfer agreement governing plasmids are provided online at www.associomics.org. Additional materials are included in the suplementary materials. The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest. NR 42 TC 44 Z9 45 U1 7 U2 77 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 16 PY 2014 VL 344 IS 6185 BP 711 EP 716 DI 10.1126/science.1251358 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH1WQ UT WOS:000335912900032 PM 24833385 ER PT J AU Laskin, J Wang, P AF Laskin, Julia Wang, Peng TI Charge retention by organometallic dications on self-assembled monolayer surfaces SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE Soft-landing; Ruthenium trisbipyridine; Ion-surface collisions; Self-assembled monolayer (SAM); Secondary ion mass spectrometry (SIMS); Charge retention ID MASS-SELECTED IONS; LOW-ENERGY COLLISIONS; SLOW POLYATOMIC IONS; LANDED PEPTIDE IONS; CROSS-SECTION DATA; INDUCED DISSOCIATION; CHEMICAL-MODIFICATION; REACTIVE COLLISIONS; COVALENT IMMOBILIZATION; IMPEDANCE SPECTROSCOPY AB Charge retention by mass-selected ruthenium trisbipyridine dications, or Ru(bpy)(3)(2+), soft-landed onto self-assembled monolayer (SAM) surfaces of 1H, 1H, 2H, 2H-perfluorodecane-1-thiol (FSAM), 11-mercaptoundecanoic acid (COOH-SAM), and 11-amino-1-undecanethiol (HSAM) on gold was examined using in situ time-resolved secondary ion mass spectrometry in a Fourier transform ion cyclotron resonance apparatus (FT-ICR SIMS). FT-ICR SIMS analysis was performed during ion soft-landing and for 8-15 h after the ion beam was switched off. Our results demonstrate efficient retention of the doubly charged precursor ion on the FSAM and COOH-SAM surfaces manifested by the abundant Ru(bpy)(3)(2+) ions in the SIMS spectra. In contrast, only the singly charged Ru(bpy)(3)(+) and Ru(bpy)(2)(+) ions were observed on HSAM, indicating rapid loss of at least one charge by the deposited dications. The signal of Ru(bpy)(3)(2+) on COOH-SAM remained almost constant for more than 8 h after the end of ion soft-landing, while a relatively fast decay followed by a plateau region was observed on the FSAM surface. However, we found that SIMS analysis of Ru(bpy)(3)(2+) ions soft-landed onto FSAM is complicated by facile ion-molecule reactivity occurring either on the surface or in the SIMS plume, making it difficult to accurately measure the charge reduction kinetics. Efficient retention of the doubly charged Ru(bpy)(3)(2+) ions on COOH-SAM is remarkably different from facile neutralization of protonated peptides deposited onto this surface reported in previous studies. Our results indicate different mechanisms of charge reduction of protonated molecules and permanent ions, such as Ru(bpy)(3)(2+), on SAM surfaces. Thus, we propose that proton loss is the major charge reduction channel for the protonated species, while electron transfer through the insulating SAM is responsible for the charge loss by permanent ions. Fundamental understanding of charge reduction phenomena is essential for controlled preparation of catalytically active substrates using ion soft-landing. (C) 2014 Published by Elsevier B.V. C1 [Laskin, Julia; Wang, Peng] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Laskin, J (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999 K8-88, Richland, WA 99352 USA. EM Julia.Laskin@pnnl.gov RI Laskin, Julia/H-9974-2012 OI Laskin, Julia/0000-0002-4533-9644 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division; DOE's Office of Biological and Environmental Research; DOE [DE-AC05-76RL01830] FX This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division. The research was performed using EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for DOE under Contract DE-AC05-76RL01830. NR 81 TC 3 Z9 3 U1 2 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD MAY 15 PY 2014 VL 365 SI SI BP 187 EP 193 DI 10.1016/j.ijms.2014.01.012 PG 7 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA AK7QG UT WOS:000338622200031 ER PT J AU Zapf, V Jaime, M Batista, CD AF Zapf, Vivien Jaime, Marcelo Batista, C. D. TI Bose-Einstein condensation in quantum magnets SO REVIEWS OF MODERN PHYSICS LA English DT Article ID GAP SYSTEM TLCUCL3; SHASTRY-SUTHERLAND MODEL; SINGLET GROUND-STATE; ONE-DIMENSIONAL ANTIFERROMAGNETS; FRUSTRATED SQUARE-LATTICE; HIGH-FIELD MAGNETIZATION; CHIRAL CLOCK MODEL; SPIN-GAP; PHASE-TRANSITIONS; CRITICAL-BEHAVIOR AB This article reviews experimental and theoretical work on Bose-Einstein condensation in quantum magnets. These magnets are natural realizations of gases of interacting bosons whose relevant parameters such as dimensionality, lattice geometry, amount of disorder, nature of the interactions, and particle concentration can vary widely between different compounds. The particle concentration can be easily tuned by applying an external magnetic field which plays the role of a chemical potential. This rich spectrum of realizations offers a unique possibility for studying the different physical behaviors that emerge in interacting Bose gases from the interplay between their relevant parameters. The plethora of other bosonic phases that can emerge in quantum magnets, of which the Bose-Einstein condensate is the most basic ground state, is reviewed. The compounds discussed in this review have been intensively studied in the last two decades and have led to important contributions in the area of quantum magnetism. In spite of their apparent simplicity, these systems often exhibit surprising behaviors. The possibility of using controlled theoretical approaches has triggered the discovery of unusual effects induced by frustration, dimensionality, or disorder. C1 [Zapf, Vivien; Jaime, Marcelo] Los Alamos Natl Lab, Mat Phys & Applicat Div, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. [Batista, C. D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Batista, C. D.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RP Zapf, V (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. EM vzapf@lanl.gov; mjaime@lanl.gov; cdb@lanl.gov RI Jaime, Marcelo/F-3791-2015; Batista, Cristian/J-8008-2016 OI Jaime, Marcelo/0000-0001-5360-5220; FU U.S. National Science Foundation [DMR1157490]; State of Florida; U.S. Department of Energy; Laboratory-Directed Research and Development program at LANL; U.S. Department of Energy Basic Energy Sciences "Science at 100 Tesla" project FX The NHMFL-PFF is funded by the U.S. National Science Foundation through Cooperative Grant No. DMR1157490, the State of Florida, and the U.S. Department of Energy. We also acknowledge support from the Laboratory-Directed Research and Development program at LANL and the U.S. Department of Energy Basic Energy Sciences "Science at 100 Tesla" project. NR 321 TC 67 Z9 67 U1 14 U2 89 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0034-6861 EI 1539-0756 J9 REV MOD PHYS JI Rev. Mod. Phys. PD MAY 15 PY 2014 VL 86 IS 2 BP 563 EP 614 DI 10.1103/RevModPhys.86.563 PG 52 WC Physics, Multidisciplinary SC Physics GA AK7ZC UT WOS:000338645900001 ER PT J AU Martinez, RA Glass, DR Ortiz, EG Alvarez, MA Unkefer, CJ AF Martinez, Rodolfo A. Glass, David R. Ortiz, Erick G. Alvarez, Marc A. Unkefer, Clifford J. TI Synthesis of isotopically labeled 1,3-dithiane SO JOURNAL OF LABELLED COMPOUNDS & RADIOPHARMACEUTICALS LA English DT Article DE stable isotope labeling; C-13-labeled synthons ID STABLE-ISOTOPES; SODIUM CYANIDE-C-13; ACETIC-ACID; CARBANIONS; REAGENTS; METHANOL AB The 1,3-dithiane is a protected formaldehyde anion equivalent that could serve as a useful labeled synthon. We report a facile synthesis of 1,3-[2-C-13]- and 1,3-[2-C-13, 2-H-2(2)] dithiane in two steps from [C-13]-or [C-13, H-2(3)] methyl phenyl sulfoxide. We have previously reported the high yield synthesis of [C-13]methyl phenyl sulfide from [C-13]MEOH and the oxidation of [C-13]methyl phenyl sulfide to [C-13]methyl phenyl sulfoxide. Here, we describe the facile exchange of deuterium from (H2O)-H-2 into [C-13]methyl phenyl sulfoxide to yield [C-13, H-2(3)]methyl phenyl sulfoxide. Thus, from [C-13]MEOH and (H2O)-H-2, all possible C2 stable isotopomers of 1,3-dithiane are available. Our synthetic route is also amenable to preparation of radiolabeled 1,3-dithianes. C1 [Martinez, Rodolfo A.; Alvarez, Marc A.; Unkefer, Clifford J.] Los Alamos Natl Lab, Natl Stable Isotope Resource, Biosci Div, Los Alamos, NM 87545 USA. [Martinez, Rodolfo A.; Glass, David R.; Ortiz, Erick G.] New Mexico Highlands Univ, Dept Chem, Las Vegas, NM 87701 USA. RP Martinez, RA (reprint author), New Mexico Highlands Univ, Dept Chem, Box 9000, Las Vegas, NM 87701 USA. EM rudy@nmhu.edu; cju@lanl.gov OI Alvarez, Marc/0000-0002-4679-1106 FU National Stable Isotope Resource at the Los Alamos National Laboratory (NIH) [P41RR02231]; New Mexico Highlands University FX This work was funded in part by the National Stable Isotope Resource at the Los Alamos National Laboratory (NIH grant award P41RR02231) and by the New Mexico Highlands University. NR 31 TC 0 Z9 0 U1 0 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0362-4803 EI 1099-1344 J9 J LABELLED COMPD RAD JI J. Label. Compd. Radiopharm. PD MAY 15 PY 2014 VL 57 IS 5 BP 338 EP 341 DI 10.1002/jlcr.3185 PG 4 WC Biochemical Research Methods; Chemistry, Medicinal; Chemistry, Analytical SC Biochemistry & Molecular Biology; Pharmacology & Pharmacy; Chemistry GA AJ5MY UT WOS:000337729200002 PM 24861982 ER PT J AU Costantini, JM Trautmann, C Weber, WJ Wiss, T AF Costantini, Jean-Marc Trautmann, Christina Weber, William J. Wiss, Thierry TI EMRS 2013 syposium M SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Editorial Material C1 [Costantini, Jean-Marc] CEA Saclay, Gif Sur Yvette, France. [Trautmann, Christina] GSI Helmholtzzentrum, Darmstadt, Germany. [Weber, William J.] Univ Tennessee, ORNL, Knoxville, TN 37996 USA. [Wiss, Thierry] ITU, Karlsruhe, Germany. RP Costantini, JM (reprint author), CEA Saclay, Gif Sur Yvette, France. RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 NR 0 TC 0 Z9 0 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD MAY 15 PY 2014 VL 327 BP 1 EP 1 DI 10.1016/j.nimb.2014.03.006 PG 1 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AI6WA UT WOS:000337016500001 ER PT J AU Schultz, PA Edwards, AH AF Schultz, Peter A. Edwards, Arthur H. TI Modeling charged defects inside density functional theory band gaps SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Defects; Density functional theory; Band gap; Electronic properties; Gallium arsenide; Modeling and simulation ID PERIODIC BOUNDARY-CONDITIONS; ELECTRONIC-STRUCTURE; POINT-DEFECTS; SILICON; SEMICONDUCTORS; BORON; PSEUDOPOTENTIALS; APPROXIMATION; PARAMETERS; VACANCY AB Density functional theory (DFT) has emerged as an important tool to probe microscopic behavior in materials. The fundamental band gap defines the energy scale for charge transition energy levels of point defects in ionic and covalent materials. The eigenvalue gap between occupied and unoccupied states in conventional DFT, the Kohn-Sham gap, is often half or less of the experimental band gap, seemingly precluding quantitative studies of charged defects. Applying explicit and rigorous control of charge boundary conditions in supercells, we find that calculations of defect energy levels derived from total energy differences give accurate predictions of charge transition energy levels in Si and GaAs, unhampered by a band gap problem. The GaAs system provides a good theoretical laboratory for investigating band gap effects in defect level calculations: depending on the functional and pseudopotential, the Kohn-Sham gap can be as large as 1.1 eV or as small as 0.1 eV. We find that the effective defect band gap, the computed range in defect levels, is mostly insensitive to the Kohn-Sham gap, demonstrating it is often possible to use conventional DFT for quantitative studies of defect chemistry governing interesting materials behavior in semiconductors and oxides despite a band gap problem. (C) 2014 Elsevier B.V. All rights reserved. C1 [Schultz, Peter A.] Sandia Natl Labs, Adv Device Technol Dept, Albuquerque, NM 87185 USA. [Edwards, Arthur H.] AFRL RVSE, Air Force Res Lab, Kirtland AFB, NM 87117 USA. RP Schultz, PA (reprint author), Sandia Natl Labs, Adv Device Technol Dept, POB 5800, Albuquerque, NM 87185 USA. EM paschul@sandia.gov FU Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 41 TC 3 Z9 3 U1 5 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD MAY 15 PY 2014 VL 327 BP 2 EP 8 DI 10.1016/j.nimb.2013.09.046 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AI6WA UT WOS:000337016500002 ER PT J AU Zhang, Y Varga, T Ishimaru, M Edmondson, PD Xue, H Liu, P Moll, S Namavar, F Hardiman, C Shannon, S Weber, WJ AF Zhang, Y. Varga, T. Ishimaru, M. Edmondson, P. D. Xue, H. Liu, P. Moll, S. Namavar, F. Hardiman, C. Shannon, S. Weber, W. J. TI Competing effects of electronic and nuclear energy loss on microstructural evolution in ionic-covalent materials SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Ceria; Silicon carbide; Ion irradiation ID MOLECULAR-DYNAMICS SIMULATIONS; SILICON-CARBIDE; DEFECT PRODUCTION; FUSION ENERGY; IRRADIATION; CEO2; DAMAGE; AMORPHIZATION; TEMPERATURE; RECOVERY AB Ever increasing energy needs have raised the demands for advanced fuels and cladding materials that withstand the extreme radiation environments with improved accident tolerance over a long period of time. Ceria (CeO2) is a well known ionic conductor that is isostructural with urania and plutonia-based nuclear fuels. In the context of nuclear fuels, immobilization and transmutation of actinides, CeO2 is a model system for radiation effect studies. Covalent silicon carbide (SIC) is a candidate for use as structural material in fusion, cladding material for fission reactors, and an inert matrix for the transmutation of plutonium and other radioactive actinides. Understanding microstructural change of these ionic-covalent materials to irradiation is important for advanced nuclear energy systems. While displacements from nuclear energy loss may be the primary contribution to damage accumulation in a crystalline matrix and a driving force for the grain boundary evolution in nanostructured materials, local non-equilibrium disorder and excitation through electronic energy loss may, however, produce additional damage or anneal pre-existing defects. At intermediate transit energies where electronic and nuclear energy losses are both significant, synergistic, additive or competitive processes may evolve that affect the dynamic response of materials to irradiation. The response of crystalline and nanostructured CeO2 and SiC to ion irradiation are studied under different nuclear and electronic stopping powers to describe some general material response in this transit energy regime. Although fast radiation-induced grain growth in CeO2 is evident with no phase transformation, different fluence and dose dependence on the growth rate is observed under Si and Au irradiations. While grain shrinkage and amorphization are observed in the nano-engineered 3C SiC with a high-density of stacking faults embedded in nanosize columnar grains, significantly enhanced radiation resistance is attributed to stacking faults that promote efficient point defect annihilation. Moreover, competing effects of electronic and nuclear energy loss on the damage accumulation and annihilation are observed in crystalline 4H-SiC. Systematic experiments and simulation effort are needed to understand the competitive or synergistic effects. (C) 2014 Elsevier B.V. All rights reserved. C1 [Zhang, Y.; Weber, W. J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Zhang, Y.; Xue, H.; Liu, P.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Varga, T.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Ishimaru, M.] Kyushu Inst Technol, Dept Mat Sci & Engn, Fukuoka 8048550, Japan. [Edmondson, P. D.] Univ Oxford, Dept Mat, Oxford OX1 3PH, England. [Liu, P.] Shandong Univ, Key Lab Particle Phys & Particle Irradiat, Sch Phys, Jinan 250100, Peoples R China. [Moll, S.] TN Int AREVA, F-78182 Montigny Le Bretonneux, France. [Namavar, F.] Univ Nebraska, Med Ctr, Omaha, NE 68198 USA. [Hardiman, C.; Shannon, S.] N Carolina State Univ, Dept Nucl Engn, Raleigh, NC 27695 USA. RP Zhang, Y (reprint author), Oak Ridge Natl Lab, 4500S A148,MS 6138, Oak Ridge, TN 37831 USA. EM Zhangy1@ornl.gov RI Weber, William/A-4177-2008; Edmondson, Philip/O-7255-2014; Shannon, Steven/O-3420-2014 OI Weber, William/0000-0002-9017-7365; Edmondson, Philip/0000-0001-8990-0870; Shannon, Steven/0000-0001-8317-6949 FU Materials Science of Actinides; Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Nuclear Engineering University Program; U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory FX The research on ceria was supported as part of the Materials Science of Actinides, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The research on nanostructured silicon carbide was supported by the U.S. Department of Energy, Nuclear Engineering University Program. The research on ion annealing in silicon carbide was supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering. Experimental work was performed at the UT-ORNL Ion Beam Materials Laboratory (IBML) located at the campus of the University of Tennessee, Knoxville and Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory. NR 58 TC 19 Z9 20 U1 7 U2 86 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD MAY 15 PY 2014 VL 327 BP 33 EP 43 DI 10.1016/j.nimb.2013.10.095 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AI6WA UT WOS:000337016500007 ER PT J AU Dow, BA Sukumar, N Matos, JO Choi, M Schulte, A Tatulian, SA Davidson, VL AF Dow, Brian A. Sukumar, Narayanasami Matos, Jason O. Choi, Moonsung Schulte, Alfons Tatulian, Suren A. Davidson, Victor L. TI The sole tryptophan of amicyanin enhances its thermal stability but does not influence the electronic properties of the type 1 copper site SO ARCHIVES OF BIOCHEMISTRY AND BIOPHYSICS LA English DT Article DE Amicyanin; Cupredoxin; Hydrogen bond; Protein structure ID TRANSFER PROTEIN COMPLEX; METHYLAMINE DEHYDROGENASE; PARACOCCUS-DENITRIFICANS; X-RAY; DIRECTED MUTAGENESIS; CRYSTAL-STRUCTURE; SPECTROSCOPIC PROPERTIES; STRUCTURAL DETERMINANTS; ANGSTROM RESOLUTION; MOLECULAR-GRAPHICS AB The cupredoxin amicyanin possesses a single tryptophan residue, Trp45. Its fluorescence is quenched when copper is bound even though it is separated by 10.1 angstrom. Mutation of Trp45 to Ala, Phe, Leu and Lys resulted in undetectable protein expression. A W45Y amicyanin variant was isolated. The W45Y mutation did not alter the spectroscopic properties or intrinsic redox potential of amicyanin, but increased the pK(a) value for the pH-dependent redox potential by 0.5 units. This is due to a hydrogen-bond involving the His95 copper ligand which is present in reduced W45Y amicyanin but not in native amicyanin. The W45Y mutation significantly decreased the thermal stability of amicyanin, as determined by changes in the visible absorbance of oxidized amicyanin and in the circular dichroism spectra for oxidized, reduced and apo forms of amicyanin. Comparison of the crystal structures suggests that the decreased stability of W45Y amicyanin may be attributed to the loss of a strong interior hydrogen bond between Trp45 and Tyr90 in native amicyanin which links two of the beta-sheets that comprise the overall structure of amicyanin. Thus, Trp45 is critical for stabilizing the structure of amicyanin but it does not influence the electronic properties of the copper which quenches its fluorescence. (C) 2014 Elsevier Inc. All rights reserved. C1 [Dow, Brian A.; Matos, Jason O.; Davidson, Victor L.] Univ Cent Florida, Coll Med, Burnett Sch Biomed Sci, Orlando, FL 32827 USA. [Sukumar, Narayanasami] Cornell Univ, Argonne Natl Lab, NE CAT, Argonne, IL 60439 USA. [Sukumar, Narayanasami] Cornell Univ, Argonne Natl Lab, Dept Chem & Chem Biol, Argonne, IL 60439 USA. [Matos, Jason O.; Schulte, Alfons; Tatulian, Suren A.] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. [Choi, Moonsung] Seoul Natl Univ Sci & Technol, Coll Energy & Biotechnol, Dept Optometry, Seoul 139743, South Korea. RP Sukumar, N (reprint author), Cornell Univ, Argonne Natl Lab, APS, Bldg 436E,9700 S Cass Ave, Argonne, IL 60439 USA. EM sukumar@anl.gov; victor.davidson@ucf.edu OI Davidson, Victor/0000-0002-1966-7302 FU National Institute of General Medical Sciences (NIGMS) of the National Institutes of Health (NIH) [R37GM41574, GM103403]; National Institute of Allergy and Infectious Disease, NIH [1R03AI097591]; U.S. DOE, Office of Science, Office of Basic Energy Science [DE-AC02-06CH1 1357] FX This research was supported by the National Institute of General Medical Sciences (NIGMS) of the National Institutes of Health (NIH) under award number R37GM41574 (V.L.D.) and the National Institute of Allergy and Infectious Disease, NIH, under award number 1R03AI097591 (S.A.T). This work and the beamlines 24lD-E and 24lD-C used to collect data and fluorescence scan are supported by award GM103403 from NIGMS at the NIH. Use of the APS is supported by the U.S. DOE, Office of Science, Office of Basic Energy Science, and Contract No. DE-AC02-06CH1 1357. NR 59 TC 3 Z9 3 U1 0 U2 7 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0003-9861 EI 1096-0384 J9 ARCH BIOCHEM BIOPHYS JI Arch. Biochem. Biophys. PD MAY 15 PY 2014 VL 550 BP 20 EP 27 DI 10.1016/j.abb.2014.03.010 PG 8 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA AI3RT UT WOS:000336780300003 PM 24704124 ER PT J AU Le, RK Harris, BJ Iwuchukwu, IJ Bruce, BD Cheng, XL Qian, S Heller, WT O'Neill, H Frymier, PD AF Le, Rosemary K. Harris, Bradley J. Iwuchukwu, Ifeyinwa J. Bruce, Barry D. Cheng, Xiaolin Qian, Shuo Heller, William T. O'Neill, Hugh Frymier, Paul D. TI Analysis of the solution structure of Thermosynechococcus elongatus photosystem I in n-dodecyl-beta-D-maltoside using small-angle neutron scattering and molecular dynamics simulation SO ARCHIVES OF BIOCHEMISTRY AND BIOPHYSICS LA English DT Article DE Small-angle neutron scattering; Membrane protein; Dummy-atom reconstruction; Detergent monolayer ID MEMBRANE-PROTEIN CRYSTALLIZATION; X-RAY-SCATTERING; DETERGENT STRUCTURE; CONTRAST VARIATION; MICELLE STRUCTURE; COMPLEXES; BIOLOGY; SURFACE; SHAPE; WATER AB Small-angle neutron scattering (SANS) and molecular dynamics (MD) simulation were used to investigate the structure of trimeric photosystem I (PSI) from Thermosynechococcus elongatus (T. elongatus) stabilized in n-dodecyl-beta-D-maltoside (DDM) detergent solution. Scattering curves of detergent and protein-detergent complexes were measured at 18% D2O, the contrast match point for the detergent, and 100% D2O, allowing observation of the structures of protein/detergent complexes. It was determined that the maximum dimension of the PSI-DDM complex was consistent with the presence of a monolayer belt of detergent around the periphery of PSI. A dummy-atom reconstruction of the shape of the complex from the SANS data indicates that the detergent envelope has an irregular shape around the hydrophobic periphery of the PSI trimer rather than a uniform, toroidal belt around the complex. A 50 ns MD simulation model (a DDM ring surrounding the PSI complex with extra interstitial DDM) of the PSI-DDM complex was developed for comparison with the SANS data. The results suggest that DDM undergoes additional structuring around the membrane-spanning surface of the complex instead of a simple, relatively uniform belt, as is generally assumed for studies that use detergents to solubilize membrane proteins. (C) 2014 Elsevier Inc. All rights reserved. C1 [Le, Rosemary K.; Harris, Bradley J.; Iwuchukwu, Ifeyinwa J.; Frymier, Paul D.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Bruce, Barry D.; Cheng, Xiaolin] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Bruce, Barry D.; Frymier, Paul D.] Univ Tennessee, Sustainable Energy Educ & Res Ctr, Knoxville, TN 37996 USA. [Cheng, Xiaolin] Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37831 USA. [Qian, Shuo; Heller, William T.; O'Neill, Hugh] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Frymier, PD (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, 419 Dougherty Engn Bldg, Knoxville, TN 37996 USA. EM pdf@utk.edu FU National Science Foundation's IGERT program [DGE-0801470]; NSF-EPSCoR [NSF EPS-1004083]; Photosynthetic Antenna Research Center (PARC), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC 0001035]; U.S. DOE, Office of Science, Office of Biological and Environmental Research Project [ERKP291]; Scientific User Facilities Division, Basic Energy Sciences; U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; National Science Foundation [0711134, 0933959, 1041709, 1041710]; University of Tennessee FX The authors would like to acknowledge financial support for Rosemary Le and Ifeyinwa Iwuchukwu from the National Science Foundation's IGERT program (DGE-0801470), Bradley Harris from the NSF-EPSCoR sponsored TN-SCORE (NSF EPS-1004083) and the University of Tennessee Sustainable Energy Education and Research Center (SEERC) for materials. HON acknowledges the support of Photosynthetic Antenna Research Center (PARC), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC 0001035. The Center for Structural Molecular Biology operates BioSANS and is supported by the U.S. DOE, Office of Science, Office of Biological and Environmental Research Project ERKP291. The High Flux Isotope Reactor is sponsored by the Scientific User Facilities Division, Basic Energy Sciences. Oak Ridge National Laboratory (ORNL) is managed by UT-Battelle, LLC, for the U.S. Department of Energy (DOE) under contract No. DE-AC05-00OR22725. This material is based upon work supported by the National Science Foundation under Grant numbers 0711134, 0933959, 1041709, and 1041710 and the University of Tennessee through the use of the Kraken computing resource at the National Institute for Computational Sciences (http://www.nics.tennessee.edu). NR 96 TC 9 Z9 9 U1 11 U2 40 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0003-9861 EI 1096-0384 J9 ARCH BIOCHEM BIOPHYS JI Arch. Biochem. Biophys. PD MAY 15 PY 2014 VL 550 BP 50 EP 57 DI 10.1016/j.abb.2014.04.005 PG 8 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA AI3RT UT WOS:000336780300007 PM 24769336 ER PT J AU Tovchigrechko, A Venepally, P Payne, SH AF Tovchigrechko, Andrey Venepally, Pratap Payne, Samuel H. TI PGP: parallel prokaryotic proteogenomics pipeline for MPI clusters, high-throughput batch clusters and multicore workstations SO BIOINFORMATICS LA English DT Article ID TOOL AB We present the first public release of our proteogenomic annotation pipeline. We have previously used our original unreleased implementation to improve the annotation of 46 diverse prokaryotic genomes by discovering novel genes, post-translational modifications and correcting the erroneous annotations by analyzing proteomic mass-spectrometry data. This public version has been redesigned to run in a wide range of parallel Linux computing environments and provided with the automated configuration, build and testing facilities for easy deployment and portability. C1 [Tovchigrechko, Andrey; Venepally, Pratap] J Craig Venter Inst, Rockville, MD 20850 USA. [Payne, Samuel H.] Pacific Northwest Natl Lab, Richland, WA 99354 USA. RP Tovchigrechko, A (reprint author), J Craig Venter Inst, 9704 Med Ctr Dr, Rockville, MD 20850 USA. EM atovtchi@jcvi.org OI Payne, Samuel/0000-0002-8351-1994 FU National Science Foundation awards [EF-0949047, 1048199]; XSEDE allocation on the Texas Advanced Computing Center Ranger [DEB100001] FX National Science Foundation awards (EF-0949047 and 1048199), and XSEDE allocation (DEB100001) on the Texas Advanced Computing Center Ranger. The funders had no role in the study design, data collection and analysis, decision to publish or preparation of the manuscript. NR 10 TC 9 Z9 9 U1 0 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1367-4803 EI 1460-2059 J9 BIOINFORMATICS JI Bioinformatics PD MAY 15 PY 2014 VL 30 IS 10 BP 1469 EP 1470 DI 10.1093/bioinformatics/btu051 PG 2 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Computer Science, Interdisciplinary Applications; Mathematical & Computational Biology; Statistics & Probability SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Computer Science; Mathematical & Computational Biology; Mathematics GA AI0IJ UT WOS:000336530000019 PM 24470574 ER PT J AU Jackson, NE Chen, LX Ratner, MA AF Jackson, Nicholas E. Chen, Lin X. Ratner, Mark A. TI Solubility of Nonelectrolytes: A First-Principles Computational Approach SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ADAPTED PERTURBATION-THEORY; HYDRATION FREE-ENERGIES; DRUG-LIKE COMPOUNDS; AQUEOUS SOLUBILITY; COSMO-RS; SOLVATION MODELS; VAPOR-PRESSURES; LIQUID-MIXTURES; WATER CLUSTERS; FORCE-FIELDS AB Using a combination of classical molecular dynamics and symmetry adapted intermolecular perturbation theory, we develop a high-accuracy computational method for examining the solubility energetics of nonelectrolytes. This approach is used to accurately compute the cohesive energy density and Hildebrand solubility parameters of 26 molecular liquids. The energy decomposition of symmetry adapted perturbation theory is then utilized to develop multicomponent Hansen-like solubility parameters. These parameters are shown to reproduce the solvent categorizations (nonpolar, polar aprotic, or polar protic) of all molecular liquids studied while lending quantitative rigor to these qualitative categorizations via the introduction of simple, easily computable parameters. Notably, we find that by monitoring the first-order exchange energy contribution to the total interaction energy, one can rigorously determine the hydrogen bonding character of a molecular liquid. Finally, this method is applied to compute explicitly the Flory interaction parameter and the free energy of mixing for two different small molecule mixtures, reproducing the known miscibilities. This methodology represents an important step toward the prediction of molecular solubility from first principles. C1 [Jackson, Nicholas E.; Chen, Lin X.; Ratner, Mark A.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Ratner, MA (reprint author), Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. EM ratner@northwestern.edu FU NSF [NSF DGE-0824162, NSF CHE-1058896] FX N.E.J. thanks the NSF for the award of a Graduate Research Fellowship (NSF DGE-0824162). N.E.J. would like to thank Brett Savoie and Kevin Kohlstedt for useful discussion and Tomekia Simeon for help with the SAPT calculations. M.A.R. thanks the NSF (NSF CHE-1058896) for support. NR 55 TC 6 Z9 6 U1 2 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 15 PY 2014 VL 118 IS 19 BP 5194 EP 5202 DI 10.1021/jp5024197 PG 9 WC Chemistry, Physical SC Chemistry GA AH5VL UT WOS:000336199100023 PM 24773531 ER PT J AU Lowndes, M Rakshit, S Shafraz, O Borghi, N Harmon, RM Green, KJ Sivasankar, S Nelson, WJ AF Lowndes, Molly Rakshit, Sabyasachi Shafraz, Omer Borghi, Nicolas Harmon, Robert M. Green, Kathleen J. Sivasankar, Sanjeevi Nelson, W. James TI Different roles of cadherins in the assembly and structural integrity of the desmosome complex SO JOURNAL OF CELL SCIENCE LA English DT Article DE Desmosome; Adhesion; Desmocollin; Desmoglein ID RIGHT-VENTRICULAR CARDIOMYOPATHY; CELL-CELL ADHESION; KIDNEY EPITHELIAL-CELLS; EPIDERMAL DIFFERENTIATION; DESMOPLAKIN ORGANIZATION; INTERCELLULAR-ADHESION; PLAKOGLOBIN COMPLEXES; FORCE SPECTROSCOPY; SPATIAL REGULATION; MEMBRANE CORE AB Adhesion between cells is established by the formation of specialized intercellular junctional complexes, such as desmosomes. Desmosomes contain isoforms of two members of the cadherin superfamily of cell adhesion proteins, desmocollins (Dsc) and desmogleins (Dsg), but their combinatorial roles in desmosome assembly are not understood. To uncouple desmosome assembly from other cell-cell adhesion complexes, we used micro-patterned substrates of Dsc2aFc and/or Dsg2Fc and collagen IV; we show that Dsc2aFc, but not Dsg2Fc, was necessary and sufficient to recruit desmosome-specific desmoplakin into desmosome puncta and produce strong adhesive binding. Single-molecule force spectroscopy showed that monomeric Dsc2a, but not Dsg2, formed Ca2+-dependent homophilic bonds, and that Dsg2 formed Ca2+-independent heterophilic bonds with Dsc2a. A W2A mutation in Dsc2a inhibited Ca2+-dependent homophilic binding, similar to classical cadherins, and Dsc2aW2A, but not Dsg2W2A, was excluded from desmosomes in MDCK cells. These results indicate that Dsc2a, but not Dsg2, is required for desmosome assembly through homophilic Ca2+-and W2-dependent binding, and that Dsg2 might be involved later in regulating a switch to Ca2+-independent adhesion in mature desmosomes. C1 [Lowndes, Molly; Nelson, W. James] Stanford Univ, Canc Biol Program, Stanford, CA 94305 USA. [Rakshit, Sabyasachi; Shafraz, Omer; Sivasankar, Sanjeevi] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Rakshit, Sabyasachi; Shafraz, Omer; Sivasankar, Sanjeevi] US DOE, Ames Lab, Ames, IA 50011 USA. [Borghi, Nicolas] CNRS, Inst Jacques Monod, UMR 7592, F-75013 Paris, France. [Borghi, Nicolas] Univ Paris Diderot, F-75013 Paris, France. [Harmon, Robert M.; Green, Kathleen J.] Northwestern Univ, Dept Pathol, Feinberg Sch Med, Chicago, IL 60611 USA. [Nelson, W. James] Stanford Univ, Dept Biol, Stanford, CA 94305 USA. [Nelson, W. James] Stanford Univ, Dept Mol & Cellular Physiol, Stanford, CA 94305 USA. RP Nelson, WJ (reprint author), Stanford Univ, Canc Biol Program, Stanford, CA 94305 USA. EM wjnelson@stanford.edu FU American Heart Association (Scientist Development Grant) [12SDG9320022]; National Institutes of Health (NIH) [R37AR043380, R01 AR41836]; NIH [GM35527]; Human Frontier Science Program [RGP0040/2012]; Genentech Graduate Fellowship; Cancer Biology Training Grant; Mason Case Graduate Fellowship; NIH T32 training grant [GM08061]; American Heart Association predoctoral fellowship FX Work in the S. S. laboratory was partially supported by a grant from the American Heart Association (Scientist Development Grant 12SDG9320022). Work in the K.J.G. laboratory was supported by grants from the National Institutes of Health (NIH) [grant numbers R37AR043380, R01 AR41836]. Work in the W.J.N. laboratory was supported by the NIH [grant number GM35527] and Human Frontier Science Program [grant number RGP0040/2012]. M. L. was supported by a Genentech Graduate Fellowship, Cancer Biology Training Grant and Mason Case Graduate Fellowship. R. M. H. was supported by a NIH T32 training grant [grant number GM08061]; and an American Heart Association predoctoral fellowship. Deposited in PMC for release after 12 months. NR 73 TC 9 Z9 9 U1 3 U2 12 PU COMPANY OF BIOLOGISTS LTD PI CAMBRIDGE PA BIDDER BUILDING CAMBRIDGE COMMERCIAL PARK COWLEY RD, CAMBRIDGE CB4 4DL, CAMBS, ENGLAND SN 0021-9533 EI 1477-9137 J9 J CELL SCI JI J. Cell Sci. PD MAY 15 PY 2014 VL 127 IS 10 BP 2339 EP 2350 DI 10.1242/jcs.146316 PG 12 WC Cell Biology SC Cell Biology GA AH9VS UT WOS:000336493500022 PM 24610950 ER PT J AU Long, H Pivovar, B AF Long, Hai Pivovar, Bryan TI Hydroxide Degradation Pathways for Imidazolium Cations: A DFT Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ANION-EXCHANGE MEMBRANES; ELECTROLYTE FUEL-CELLS; DECOMPOSITION PATHWAYS; POLYMER; STABILITY; THERMOCHEMISTRY; CARBENES; SALTS AB Imidazolium cations are promising candidates as covalently tetherable cations for application in anion exchange membranes. They have generated specific interest in alkaline membrane fuel cell applications where ammonium-based cations have been the most commonly applied but have been found to be susceptible to hydroxide attack. In the search for high stability cations, a detailed understanding of the degradation pathways and reaction barriers is required. In this work, we investigate imidazolium and benzimidazolium cations in the presence of hydroxide using density functional theory calculations for their potential in alkaline membrane fuel cells. The dominant degradation pathway for these cations is predicted to be the nucleophilic addition-elimination pathway at the C-2 atom position on the imidazolium ring. Steric interferences, introduced by substitutions at the C-2, C-4, and C-5 atom positions, were investigated and found to have a significant, positive impact on calculated degradation energy barriers. Benzimidazolium cations, with their larger conjugated systems, are predicted to degrade much faster than their imidazolium counterparts. The reported results provide important insight into designing stable cations for anion exchange membranes. Some of the molecules studied have significantly increased degradation energy barriers suggesting that they could possess significantly improved (several orders of magnitude) durability, compared to traditional cations and potentially enable new applications. C1 [Long, Hai; Pivovar, Bryan] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Pivovar, B (reprint author), Natl Renewable Energy Lab, MS ESIF302,15013 Denver West Pkwy, Golden, CO 80401 USA. EM Bryan.Pivovar@nrel.gov RI Long, Hai/C-5838-2015 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC36-08-GO28308]; Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC36-08-GO28308. This research used capabilities of the National Renewable Energy Laboratory Computational Science Center, which is supported by the Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy. NR 27 TC 19 Z9 19 U1 9 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 15 PY 2014 VL 118 IS 19 BP 9880 EP 9888 DI 10.1021/jp501362y PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH5VJ UT WOS:000336198900003 ER PT J AU Liu, FQ Zhu, K Li, T Xu, T AF Liu, Fa-Qian Zhu, Kai Li, Tao Xu, Tao TI Drift Transport in Al2O3-Sheathed 3-D Transparent Conducting Oxide Photoanodes Observed in Liquid Electrolyte-Based Dye-Sensitized Solar Cells SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MODULATED PHOTOCURRENT SPECTROSCOPY; ATOMIC LAYER DEPOSITION; LITHIUM-ION BATTERIES; CHARGE-TRANSPORT; TIO2 NANOTUBES; POTENTIAL DISTRIBUTION; CONVERSION EFFICIENCY; SNO2; RECOMBINATION; NANOPARTICLES AB It has long been taken for granted that electron transport in liquid-electrolyte-based dye-sensitized solar cells (DSSCs) undergoes an ambipolar diffusive transport due to the strong coupling between electrons in the photoanode and the nearby mobile cations in liquid electrolyte, which, therefore, screens off any electric field in the photoanodes and consequently eliminates the possibility for drift transport. In this work, we demonstrate the existence of drift transport in liquid electrolyte-based DSSCs using a thin Al2O3-sheathed 3-dimentional (3-D) fluorinated tin oxide (FTO), as photoanodes. The electron diffusion rate in such 3-D TCO based DSSC exhibits a striking enhancement to the value of similar to 10(-2) cm(2)/s, about 10(4) times faster than that of the TiO2 nanoparticle-based DSSCs. The electron diffusion coefficient is independent of the photoelectron density, while intensity modulated photocurrent spectroscopy (IMPS) suggests that the time constants of electron transport exhibit a linear dependence on the bias voltage, a strong indication of drift transport behavior in this 3-D FTO hollow nanobeads-based DSSC, despite the use of liquid I-/I-3(-) electrolyte. C1 [Liu, Fa-Qian; Xu, Tao] No Illinois Univ, Dept Chem & Biochem, De Kalb, IL 60115 USA. [Zhu, Kai] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. [Li, Tao] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Zhu, K (reprint author), Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. EM Kai.Zhu@nrel.gov; txu@niu.edu RI li, tao/K-8911-2012 OI li, tao/0000-0001-5454-1468 FU U.S. National Science Foundation [CBET-1150617]; U.S. Department of Energy Office of Science Laboratory by UChicago Argonne, LLC [DE-AC02-06CH11357]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; NSF of China [21371105] FX We acknowledge the support from the U.S. National Science Foundation (CBET-1150617). The electron microscopy was conducted at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. K.Z. acknowledges support by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. F.L. is also partially supported by the NSF of China (no. 21371105). We thank Dr. Alex B. F. Martinson at Materials Science Division, Argonne National Laboratory for his help with atomic layer deposition. NR 48 TC 4 Z9 4 U1 1 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 15 PY 2014 VL 118 IS 19 BP 9951 EP 9957 DI 10.1021/jp502220m PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH5VJ UT WOS:000336198900011 ER PT J AU Taylor, CD AF Taylor, Christopher D. TI Oxidation of Technetium Metal as Simulated by First Principles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; STRUCTURAL STABILITY; NUCLEAR-FUEL; WASTE FORMS; DENSITY; ALGORITHM; BEHAVIOR; ALLOY AB Advanced models for alloy corrosion should take into account the properties of the oxide film that provides the first line of corrosion resistance. Predictive models for alloy corrosion are particularly desirable for the evaluation of candidate alloy forms for the disposition of spent nuclear fuel. Since technetium is one of the long-lived fission products generated in a nuclear reactor, we consider herein the mechanism of technetium oxidation, beginning with computing the properties of the oxide using a number of first-principles approaches, and then moving to oxygen chernisorption and multilayer oxide growth. For TcO2, electronic structure elements were improved with the use of the Hubbard U method, but this choice led to poor structural predictions. Conventional GGA, on the other hand, gave good structural and mechanical agreement with the hybrid density functional calculations. We examined a number of surface terminations for this oxide phase and found that the "striped" nonpolar surface termination was preferred. The surface energy for this configuration was calculated to be 1.41 J/m(2). Oxygen chemisorption to Tc(0001) is very strong, implying that formation of a full surface monolayer of chemisorbed oxygen is preferred to the nucleation of oxide islands. The formation of multilayers of TcO2 on Tc leads to surface configurations that resemble the charge state, bonding patterns, and configuration dependence of TcO2 at an early stage. The films are strongly adherent, with adhesion energies of TcO2(001) on Tc(0001) computed to be -2.50 J/m(2) for 0.50 monolayer (ML), -3.86 J/m(2) for 1.0 ML, and 2.51 J/m(2) for 2.0 ML. C1 [Taylor, Christopher D.] Los Alamos Natl Lab, Mat Sci & Technol Div, Mat Technol Met MST 6, Los Alamos, NM 87545 USA. RP Taylor, CD (reprint author), DNV GL, Strateg Res & Innovat, Dublin, OH 43017 USA. EM Christopher.taylor@dnvgl.com FU U.S. DOE Fuel Cycle RD; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX This study was performed under activity FT-13LA030415 Metal Corrosion Mechanisms under the auspices of the U.S. DOE Fuel Cycle R&D under the direction of John Vienna, Waste Forms Campaign Manager. Helpful discussions with Xiang-Yang (Ben) Liu, Dave Moore, Gordon Jarvinen, Scott Lillard, and Dave Kolman at Los Alamos National Laboratory and Eunja Kim, Philippe Weck (now Sandia National Laboratory), Ken Czerwinski, and Ed Masoulf at University of Nevada-Las Vegas are also acknowledged. High-performance computing resources at LANL were used to complete this research. The Los Alamos National Laboratory is operated by Los Alamos National Security LLC for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 42 TC 5 Z9 5 U1 0 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 15 PY 2014 VL 118 IS 19 BP 10017 EP 10023 DI 10.1021/jp411976s PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH5VJ UT WOS:000336198900019 ER PT J AU Iberi, V Bigelow, NW Mirsaleh-Kohan, N Griffin, S Simmons, PD Guiton, BS Masiello, DJ Camden, JP AF Iberi, Vighter Bigelow, Nicholas W. Mirsaleh-Kohan, Nasrin Griffin, Sarah Simmons, Philip D., Jr. Guiton, Beth S. Masiello, David J. Camden, Jon P. TI Resonance-Rayleigh Scattering and Electron Energy-Loss Spectroscopy of Silver Nanocubes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENHANCED RAMAN-SCATTERING; SURFACE-PLASMON RESONANCES; SINGLE-MOLECULE DETECTION; METAL NANOPARTICLES; FANO RESONANCE; HOT-SPOTS; OPTICAL-PROPERTIES; RHODAMINE 6G; EXCITATIONS; MICROSCOPY AB The Fano interference phenomenon between localized surface plasmon resonances (LSPRs) of individual silver nanocubes is investigated using dark-field optical microscopy and electron-energy loss spectroscopy (EELS) in a scanning transmission electron microscope (STEM). By computing the polarization induced by the electron beam, we show that the hybridized modes responsible for this Fano interference are the same as those present in the resonance-Rayleigh scattering spectrum of an individual nanocube on a substrate. C1 [Iberi, Vighter; Griffin, Sarah; Simmons, Philip D., Jr.; Camden, Jon P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Bigelow, Nicholas W.; Masiello, David J.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Mirsaleh-Kohan, Nasrin] Texas Womans Univ, Dept Chem & Biochem, Denton, TX 76204 USA. [Guiton, Beth S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Guiton, Beth S.] Univ Kentucky, Dept Chem, Lexington, KY 40506 USA. RP Masiello, DJ (reprint author), Univ Washington, Dept Chem, Seattle, WA 98195 USA. EM masiello@chem.washington.edu; jcamden@utk.edu FU University of Tennessee (UT) Office of Research, College of Arts and Sciences; Department of Chemistry; UT/ORNL Joint Institute for Advanced Materials; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0010536]; U.S. National Science Foundation [CHE-1150687, CHE-1253775, PHY-130045]; University of Washington; Eugene P. Wigner Fellowship program of Oak Ridge National Laboratory; U.S. Department of Energy, Office of Basic Energy Sciences (BSG) FX This work was supported by University of Tennessee (UT) Office of Research, College of Arts and Sciences, and Department of Chemistry, the UT/ORNL Joint Institute for Advanced Materials, and the U.S. Department of Energy, Office of Basic Energy Sciences, under Award DE-SC0010536 and the U.S. National Science Foundation under Award CHE-1150687 (V.I., S.G., J.P.C.); the University of Washington and the U.S. National Science Foundation under Awards CHE-1253775 and PHY-130045 (N.W.B., D.J.M.); and the Eugene P. Wigner Fellowship program of Oak Ridge National Laboratory and the U.S. Department of Energy, Office of Basic Energy Sciences (BSG). V.I., N.M.K., and S.G. thank Gerd Duscher for facilitating the STEM/EELS experiments NR 78 TC 7 Z9 7 U1 6 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 15 PY 2014 VL 118 IS 19 BP 10254 EP 10262 DI 10.1021/jp412778y PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH5VJ UT WOS:000336198900047 ER PT J AU Stoerzinger, KA Qiao, L Biegalski, MD Shao-Horn, Y AF Stoerzinger, Kelsey A. Qiao, Liang Biegalski, Michael D. Shao-Horn, Yang TI Orientation-Dependent Oxygen Evolution Activities of Rutile IrO2 and RuO2 SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID WATER; ELECTROCATALYSIS; ELECTROLYSIS; ELECTRODES; MECHANISM; SURFACE; ENERGY; OXIDATION; CORROSION; RUO2(100) AB The activities of the oxygen evolution reaction (OER) on IrO2 and RuO2 catalysts are among the highest known to date. However, the intrinsic OER activities of surfaces with defined crystallographic orientations are not well-established experimentally. Here we report that the (100) surface of IrO2 and RuO2 is more active in alkaline environments (pH 13) than the most thermodynamically stable (110) surface. The OER activity was correlated with the density of coordinatively undersaturated metal sites of each crystallographic facet. The surface-orientation-dependent activities can guide the design of nanoscale catalysts with increased activity for electrolyzers, metal-air batteries, and photoelectrochemical water splitting applications. C1 [Stoerzinger, Kelsey A.; Shao-Horn, Yang] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Stoerzinger, Kelsey A.; Shao-Horn, Yang] MIT, Electrochem Energy Lab, Cambridge, MA 02139 USA. [Shao-Horn, Yang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Qiao, Liang; Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Shao-Horn, Y (reprint author), MIT, Dept Mat Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM shaohorn@mit.edu RI Qiao, Liang/A-8165-2012; OI Stoerzinger, Kelsey/0000-0002-3431-8290 FU MRSEC Program of the National Science Foundation [DMR-0819762]; Eni S.p.A under the Eni-MIT Alliance Solar Frontiers; Skoltech-MIT Center for Electrochemical Energy; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation Graduate Research Fellowship [DGE-1122374] FX This work was partially supported by the MRSEC Program of the National Science Foundation under award number DMR-0819762, by Eni S.p.A under the Eni-MIT Alliance Solar Frontiers, and the Skoltech-MIT Center for Electrochemical Energy. The film growth and structural characterization were performed at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. K.A.S. was supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE-1122374. NR 32 TC 61 Z9 61 U1 24 U2 166 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 15 PY 2014 VL 5 IS 10 BP 1636 EP 1641 DI 10.1021/jz500610u PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH5VK UT WOS:000336199000003 PM 26270358 ER PT J AU Caplins, BW Suich, DE Shearer, AJ Harris, CB AF Caplins, Benjamin W. Suich, David E. Shearer, Alex J. Harris, Charles B. TI Metal/Phthalocyanine Hybrid Interface States on Ag(111) SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ENERGY-LEVEL ALIGNMENT; NOBLE-METAL SURFACES; ELECTRONIC-STRUCTURE; PHTHALOCYANINE; ADSORPTION; ORGANIC/METAL; SUBSTRATE; PTCDA; FILM AB A phthalocyanine/Ag(111) interface state is observed for the first time using time- and angle-resolved two-photon photoemission. For monolayer films of metal-free (H2Pc) and iron phthalocyanine (Fe Pc) on Ag(111), the state exists 0.23 +/- 0.03 and 0.31 +/- 0.03 eV above the Fermi level, respectively. Angle-resolved spectra show the state to be highly dispersive with an effective mass of 0.50 +/- 0.15 m(e) for H2Pc and 0.67 +/- 0.14 m(e) for Fe Pc. Density functional theory calculations on the H2Pc/Ag(111) surface allow us to characterize this state as being a hybrid state resulting from the interaction between the unoccupied molecular states of the phthalocyanine ligand and the Shockley surface state present on the bare Ag(111) surface. This work, when taken together with the extensive literature on the 3,4,9,10-perylene tetracarboxylic dianhydride/Ag interface state, provides compelling evidence that the hybridization of metal surface states with molecular electronic states is a general phenomenon. C1 [Harris, Charles B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Harris, CB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM cbharris@berkeley.edu FU National Energy Research Scientific Computing Center; Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research used resources of the National Energy Research Scientific Computing Center and was supported by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. The authors gratefully acknowledge Dr. James E. Johns for helpful comments and suggestions. NR 37 TC 18 Z9 18 U1 3 U2 69 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 15 PY 2014 VL 5 IS 10 BP 1679 EP 1684 DI 10.1021/jz500571z PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH5VK UT WOS:000336199000011 PM 26270366 ER PT J AU Lopez-Bezanilla, A Zhou, W Idrobo, JC AF Lopez-Bezanilla, Alejandro Zhou, Wu Idrobo, Juan-Carlos TI Electronic and Quantum Transport Properties of Atomically Identified Si Point Defects in Graphene SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID CHEMICAL FUNCTIONALIZATION; ENHANCEMENT; ROUTE AB We report high-resolution scanning transmission electron microscopy images displaying a range of inclusions of isolated silicon atoms at the edges and inner zones of graphene layers. Whereas the incorporation of Si atoms to a graphene armchair edge involves no reconstruction of the neighboring carbon atoms, the inclusion of a Si atom to a zigzag graphene edge entails the formation of five-membered carbon rings. In all the observed atomic edge terminations, a Si atom is found bridging two C atoms in a 2-fold coordinated configuration. The atomic-scale observations are underpinned by first-principles calculations of the electronic and quantum transport properties of the structural anomalies. Experimental estimations of Si-doped graphene band gaps realized by means of transport measurements may be affected by a low doping rate of 2-fold coordinated Si atoms at the graphene edges, and 4-fold coordinated at inner zones due to the apparition of mobility gaps. C1 [Lopez-Bezanilla, Alejandro] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Zhou, Wu] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Idrobo, Juan-Carlos] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci Div, Oak Ridge, TN 37831 USA. RP Lopez-Bezanilla, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 South Cass Ave, Lemont, IL 60439 USA. EM alejandrolb@gmail.com RI Zhou, Wu/D-8526-2011; Lopez-Bezanilla, Alejandro/B-9125-2015; Idrobo, Juan/H-4896-2015 OI Zhou, Wu/0000-0002-6803-1095; Lopez-Bezanilla, Alejandro/0000-0002-4142-2360; Idrobo, Juan/0000-0001-7483-9034 FU Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; NSF [DMR-0938330]; Wigner Fellowship through the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL); Center for Nanophase Materials Sciences (CNMS); ORNL by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE FX We gratefully acknowledge the computing resources provided on the Blues compute cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. This research also used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. This work was supported in part by NSF grant No. DMR-0938330 (W.Z.), by a Wigner Fellowship through the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL), managed by UT-Battelle, LLC, for the U.S. DOE (W.Z.), and the Center for Nanophase Materials Sciences (CNMS), which is sponsored at ORNL by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE (J.-C.L.). NR 27 TC 6 Z9 6 U1 4 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 15 PY 2014 VL 5 IS 10 BP 1711 EP 1718 DI 10.1021/jz500403h PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH5VK UT WOS:000336199000016 PM 26270371 ER PT J AU Sarks, C Jin, MJ Sato, TK Balan, V Dale, BE AF Sarks, Cory Jin, Mingjie Sato, Trey K. Balan, Venkatesh Dale, Bruce E. TI Studying the rapid bioconversion of lignocellulosic sugars into ethanol using high cell density fermentations with cell recycle SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Lignocellulosic biofuel; Ethanol fermentation; Saccharomyces cerevisiae; AFEX; Cell recycling; RaBIT ID CORN STOVER HYDROLYSATE; AMMONIA FIBER EXPANSION; SACCHAROMYCES-CEREVISIAE; ZYMOMONAS-MOBILIS; XYLOSE FERMENTATION; ESCHERICHIA-COLI; PICHIA-STIPITIS; WHEAT-GERM; BIOMASS; PRETREATMENT AB Background: The Rapid Bioconversion with Integrated recycle Technology (RaBIT) process reduces capital costs, processing times, and biocatalyst cost for biochemical conversion of cellulosic biomass to biofuels by reducing total bioprocessing time (enzymatic hydrolysis plus fermentation) to 48 h, increasing biofuel productivity (g/L/h) twofold, and recycling biocatalysts (enzymes and microbes) to the next cycle. To achieve these results, RaBIT utilizes 24-h high cell density fermentations along with cell recycling to solve the slow/incomplete xylose fermentation issue, which is critical for lignocellulosic biofuel fermentations. Previous studies utilizing similar fermentation conditions showed a decrease in xylose consumption when recycling cells into the next fermentation cycle. Eliminating this decrease is critical for RaBIT process effectiveness for high cycle counts. Results: Nine different engineered microbial strains (including Saccharomyces cerevisiae strains, Scheffersomyces (Pichia) stipitis strains, Zymomonas mobilis 8b, and Escherichia coli KO11) were tested under RaBIT platform fermentations to determine their suitability for this platform. Fermentation conditions were then optimized for S. cerevisiae GLBRCY128. Three different nutrient sources (corn steep liquor, yeast extract, and wheat germ) were evaluated to improve xylose consumption by recycled cells. Capacitance readings were used to accurately measure viable cell mass profiles over five cycles. Conclusion: The results showed that not all strains are capable of effectively performing the RaBIT process. Acceptable performance is largely correlated to the specific xylose consumption rate. Corn steep liquor was found to reduce the deleterious impacts of cell recycle and improve specific xylose consumption rates. The viable cell mass profiles indicated that reduction in specific xylose consumption rate, not a drop in viable cell mass, was the main cause for decreasing xylose consumption. C1 [Sarks, Cory; Jin, Mingjie; Balan, Venkatesh; Dale, Bruce E.] Michigan State Univ, Dept Chem Engn & Mat Sci, Biomass Convers Res Lab, Lansing, MI 48910 USA. [Sarks, Cory; Jin, Mingjie; Balan, Venkatesh; Dale, Bruce E.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr GLBRC, E Lansing, MI 48824 USA. [Sato, Trey K.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. RP Sarks, C (reprint author), Michigan State Univ, Dept Chem Engn & Mat Sci, Biomass Convers Res Lab, 3815 Technol Blvd, Lansing, MI 48910 USA. EM sarkscor@egr.msu.edu; jinmingj@egr.msu.edu RI Jin, Mingjie/I-4616-2012; OI Jin, Mingjie/0000-0002-9493-305X FU U.S. Department of Energy through the DOE Great Lakes Bioenergy Research Center (GLBRC) grant [DE-FC02-07ER64494] FX This work was supported by the U.S. Department of Energy through the DOE Great Lakes Bioenergy Research Center (GLBRC) grant DE-FC02-07ER64494. We thank Novozymes and Genencor for supplying the commercial enzymes for this work. We thank Dr. Farzaneh Teymouri from MBI International (Lansing, MI), and Drs. Nancy Ho and Thomas Jeffries for generously providing microbial strains. We thank Dr. Rebecca Garlock-Ong and Charles Donald, Jr. for providing/preparing AFEX-pretreated corn stover. We thank Christa Gunawan for the HPLC analysis. Finally, we thank the members of the GLBRC fermentation group from the University of Wisconsin for their valuable suggestions and input. AFEX is a trademark of MBI, International (Lansing, MI). NR 38 TC 15 Z9 17 U1 5 U2 54 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAY 15 PY 2014 VL 7 AR 73 DI 10.1186/1754-6834-7-73 PG 12 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AH3WC UT WOS:000336055800001 PM 24847379 ER PT J AU Zhang, WK Alonso-Mori, R Bergmann, U Bressler, C Chollet, M Galler, A Gawelda, W Hadt, RG Hartsock, RW Kroll, T Kjaer, KS Kubicek, K Lemke, HT Liang, HYW Meyer, DA Nielsen, MM Purser, C Robinson, JS Solomon, EI Sun, Z Sokaras, D van Driel, TB Vanko, G Weng, TC Zhu, DL Gaffney, KJ AF Zhang, Wenkai Alonso-Mori, Roberto Bergmann, Uwe Bressler, Christian Chollet, Matthieu Galler, Andreas Gawelda, Wojciech Hadt, Ryan G. Hartsock, Robert W. Kroll, Thomas Kjaer, Kasper S. Kubicek, Katharina Lemke, Henrik T. Liang, Huiyang W. Meyer, Drew A. Nielsen, Martin M. Purser, Carola Robinson, Joseph S. Solomon, Edward I. Sun, Zheng Sokaras, Dimosthenis van Driel, Tim B. Vanko, Gyoergy Weng, Tsu-Chien Zhu, Diling Gaffney, Kelly J. TI Tracking excited-state charge and spin dynamics in iron coordination complexes SO NATURE LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; TRANSITION-METAL-COMPLEXES; FREE-ELECTRON LASER; EMISSION SPECTROSCOPY; CROSSOVER DYNAMICS AB Crucial to many light-driven processes in transition metal complexes is the absorption and dissipation of energy by 3d electrons(1-4). But a detailed understanding of such non-equilibrium excited-state dynamics and their interplay with structural changes is challenging: a multitude of excited states and possible transitions result in phenomena too complex to unravel when faced with the indirect sensitivity of optical spectroscopy to spin dynamics(5) and the flux limitations of ultrafast X-ray sources(6,7). Such a situation exists for archetypal poly-pyridyl iron complexes, such as [Fe(2,2'-bipyridine)(3)](2+), where the excited-state charge and spin dynamics involved in the transition from a low-to a high-spin state (spin crossover) have long been a source of interest and controversy(6-15). Here we demonstrate that femtosecond resolution X-ray fluorescence spectroscopy, with its sensitivity to spin state, can elucidate the spin crossover dynamics of [Fe(2,2'-bipyridine)(3)](2+) on photoinduced metal-to-ligand charge transfer excitation. We are able to track the charge and spin dynamics, and establish the critical role of intermediate spin states in the crossover mechanism. We anticipate that these capabilities will make our method a valuable tool for mapping in unprecedented detail the fundamental electronic excited-state dynamics that underpin many useful light-triggered molecular phenomena involving 3d transition metal complexes. C1 [Zhang, Wenkai; Hartsock, Robert W.; Liang, Huiyang W.; Meyer, Drew A.; Purser, Carola; Sun, Zheng; Gaffney, Kelly J.] Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Alonso-Mori, Roberto; Bergmann, Uwe; Chollet, Matthieu; Lemke, Henrik T.; Robinson, Joseph S.; Zhu, Diling] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA. [Bressler, Christian; Galler, Andreas; Gawelda, Wojciech] European XFEL, D-22761 Hamburg, Germany. [Hadt, Ryan G.; Hartsock, Robert W.; Kroll, Thomas; Liang, Huiyang W.; Meyer, Drew A.; Solomon, Edward I.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Kjaer, Kasper S.] Univ Copenhagen, Niels Bohr Inst, Ctr Mol Movies, DK-2100 Copenhagen, Denmark. [Kjaer, Kasper S.; Nielsen, Martin M.; van Driel, Tim B.] Tech Univ Denmark, Dept Phys, Ctr Mol Movies, DK-2800 Lyngby, Denmark. [Kubicek, Katharina] Max Planck Inst Biophys Chem, D-37077 Gottingen, Germany. [Kubicek, Katharina] DESY, D-22607 Hamburg, Germany. [Solomon, Edward I.; Sokaras, Dimosthenis; Weng, Tsu-Chien] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA. [Vanko, Gyoergy] Hungarian Acad Sci, Wigner Res Ctr Phys, H-1525 Budapest, Hungary. RP Gaffney, KJ (reprint author), Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. EM kgaffney@slac.stanford.edu RI Zhang, Wenkai/H-1301-2012; Vanko, Gyorgy/B-8176-2012; Kroll, Thomas/D-3636-2009; Bressler, Christian/G-1864-2010; Gawelda, Wojciech/B-7878-2014; Nielsen, Martin/A-5133-2009; Lemke, Henrik Till/N-7419-2016 OI Vanko, Gyorgy/0000-0002-3095-6551; Gawelda, Wojciech/0000-0001-7824-9197; Nielsen, Martin/0000-0002-8135-434X; Lemke, Henrik Till/0000-0003-1577-8643 FU AMOS programme within the Chemical Sciences, Geosciences and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, US Department of Energy; NSF [CHE-0948211]; German Research Foundation (DFG) [KR3611/2-1]; Danish National Research Foundation; DANSCATT; Volkswagen Foundation [I/85832]; European Research Council [ERC-StG-259709]; Lendulet Programme of the Hungarian Academy of Sciences; DFG [SFB925]; European XFEL FX We thank P. Frank, B. Lin and S. DeBeer for discussion, S. DeBeer for some model iron complex X-ray fluorescence spectra, and D. Stanbury for providing some iron complexes. Experiments were carried out at LCLS and SSRL, which are National User Facilities operated for DOE and OBES respectively by Stanford University. W.Z., R. W. H., H. W. L., D. A. M., Z.S. and K.J.G. acknowledge support from the AMOS programme within the Chemical Sciences, Geosciences and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, US Department of Energy. E. I. S. acknowledges support from the NSF (CHE-0948211). R. G. H. acknowledges a Gerhard Casper Stanford Graduate Fellowship and the Achievements Rewards for College Scientists (ARCS) Foundation. T. K. acknowledges the German Research Foundation (DFG), grant KR3611/2-1. K. S. K., M.M.N. and T. B. v. D. acknowledge support from the Danish National Research Foundation and from DANSCATT. K. K. thanks the Volkswagen Foundation for support under the Peter Paul Ewald fellowship program (I/85832). G. V. acknowledges support from the European Research Council (ERC-StG-259709) and the Lendulet Programme of the Hungarian Academy of Sciences. C. B., W. G. and A. G. thank the DFG (SFB925), as well as the European XFEL, for financial support. NR 40 TC 109 Z9 109 U1 22 U2 215 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 15 PY 2014 VL 509 IS 7500 BP 345 EP + DI 10.1038/nature13252 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH4TM UT WOS:000336121200035 PM 24805234 ER PT J AU Bonawitz, ND Kim, JI Tobimatsu, Y Ciesielski, PN Anderson, NA Ximenes, E Maeda, J Ralph, J Donohoe, BS Ladisch, M Chapple, C AF Bonawitz, Nicholas D. Kim, Jeong Im Tobimatsu, Yuki Ciesielski, Peter N. Anderson, Nickolas A. Ximenes, Eduardo Maeda, Junko Ralph, John Donohoe, Bryon S. Ladisch, Michael Chapple, Clint TI Disruption of Mediator rescues the stunted growth of a lignin-deficient Arabidopsis mutant SO NATURE LA English DT Article ID PLANT-GROWTH; PHENYLPROPANOID BIOSYNTHESIS; DOWN-REGULATION; SALICYLIC-ACID; CELL-WALL; METABOLISM; DEPOSITION; REGULATOR; PATHWAYS; 3-HYDROXYLASE AB Lignin is a phenylpropanoid-derived heteropolymer important for the strength and rigidity of the plant secondary cell wall(1,2). Genetic disruption of lignin biosynthesis has been proposed as a means to improve forage and bioenergy crops, but frequently results in stunted growth and developmental abnormalities, the mechanisms of which are poorly understood(3). Here we show that the phenotype of a lignin-deficient Arabidopsis mutant is dependent on the transcriptional co-regulatory complex, Mediator. Disruption of the Mediator complex subunits MED5a (also known as REF4) and MED5b (also known as RFR1) rescues the stunted growth, lignin deficiency and widespread changes in gene expression seen in the phenylpropanoid pathway mutant ref8, without restoring the synthesis of guaiacyl and syringyl lignin subunits. Cell walls of rescued med5a/5b ref8 plants instead contain a novel lignin consisting almost exclusively of p-hydroxyphenyl lignin subunits, and moreover exhibit substantially facilitated polysaccharide saccharification. These results demonstrate that guaiacyl and syringyl lignin subunits are largely dispensable for normal growth and development, implicate Mediator in an active transcriptional process responsible for dwarfing and inhibition of lignin biosynthesis, and suggest that the transcription machinery and signalling pathways responding to cell wall defects may be important targets to include in efforts to reduce biomass recalcitrance. C1 [Bonawitz, Nicholas D.; Kim, Jeong Im; Anderson, Nickolas A.; Maeda, Junko; Chapple, Clint] Purdue Univ, Dept Biochem, W Lafayette, IN 47907 USA. [Tobimatsu, Yuki; Ralph, John] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA. [Ciesielski, Peter N.; Donohoe, Bryon S.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Ximenes, Eduardo; Ladisch, Michael] Purdue Univ, Dept Agr & Biol Engn, W Lafayette, IN 47907 USA. [Ximenes, Eduardo; Ladisch, Michael] Purdue Univ, Renewable Resources Engn Lab, W Lafayette, IN 47907 USA. [Ralph, John] Univ Wisconsin, Dept Biol Syst Engn, Madison, WI 53706 USA. [Ralph, John] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. [Ralph, John] Univ Wisconsin, Wisconsin Energy Inst, Madison, WI 53726 USA. [Ladisch, Michael] Purdue Univ, Weldon Sch Biomed Engn, W Lafayette, IN 47907 USA. RP Chapple, C (reprint author), Purdue Univ, Dept Biochem, W Lafayette, IN 47907 USA. EM chapple@purdue.edu OI Ximenes, Eduardo/0000-0001-9087-0218 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy (DOE) [DE-FG02-07ER15905]; Life Sciences Research Foundation; US DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64944]; Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio), an Energy Frontier Research Center - US DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0000997]; US DOE [DE-FG02-06ER64301]; Purdue University Office of Agricultural Research Programs; Bioinformatics Core at Purdue University FX This work was primarily funded by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy (DOE) through grant DE-FG02-07ER15905 to C. C. N.D.B. was supported in part by a fellowship from the Life Sciences Research Foundation. Y.T. and J.R. were funded by the US DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64944). J.I.K., P.N.C. and B. S. D. were supported as part of the Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio), an Energy Frontier Research Center funded by the US DOE, Office of Science, Office of Basic Energy Sciences, award number DE-SC0000997. E. X. and M. L. were supported by the US DOE through grant DE-FG02-06ER64301 to M. L. and C. C. and by the Purdue University Office of Agricultural Research Programs. The authors acknowledge the support of the Bioinformatics Core at Purdue University. NR 38 TC 83 Z9 84 U1 11 U2 138 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 15 PY 2014 VL 509 IS 7500 BP 376 EP + DI 10.1038/nature13084 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH4TM UT WOS:000336121200042 PM 24670657 ER PT J AU Reagan, BA Berrill, M Wernsing, KA Baumgarten, C Woolston, M Rocca, JJ AF Reagan, Brendan A. Berrill, Mark Wernsing, Keith A. Baumgarten, Cory Woolston, Mark Rocca, Jorge J. TI High-average-power, 100-Hz-repetition-rate, tabletop soft-x-ray lasers at sub-15-nm wavelengths SO PHYSICAL REVIEW A LA English DT Article ID HZ REPETITION RATE; FREE-ELECTRON LASER; EXTREME-ULTRAVIOLET; NM; PULSES; BEAM; GENERATION; OPERATION; COHERENT; LONG AB Efficient excitation of dense plasma columns at 100-Hz repetition rate using a tailored pump pulse profile produced a tabletop soft-x-ray laser average power of 0.1 mW at lambda = 13.9 nm and 20 mu W at lambda = 11.9 nm from transitions of Ni-like Ag and Ni-like Sn, respectively. Lasing on several other transitions with wavelengths between 10.9 and 14.7 nm was also obtained using 0.9-J pump pulses of 5-ps duration from a compact diode-pumped chirped pulse amplification Yb: YAG laser. Hydrodynamic and atomic plasma simulations show that the pump pulse profile, consisting of a nanosecond ramp followed by two peaks of picosecond duration, creates a plasma with an increased density of Ni-like ions at the time of peak temperature that results in a larger gain coefficient over a temporally and spatially enlarged space leading to a threefold increase in the soft-x-ray laser output pulse energy. The high average power of these compact soft-x-ray lasers will enable applications requiring high photon flux. These results open the path to milliwatt-average-power tabletop soft-x-ray lasers. C1 [Reagan, Brendan A.; Berrill, Mark; Wernsing, Keith A.; Baumgarten, Cory; Woolston, Mark; Rocca, Jorge J.] Colorado State Univ, NSF Engn Res Ctr Extreme Ultraviolet Sci & Techno, Ft Collins, CO 80523 USA. [Reagan, Brendan A.; Wernsing, Keith A.; Woolston, Mark; Rocca, Jorge J.] Colorado State Univ, Dept Elect & Comp Engn, Ft Collins, CO 80523 USA. [Berrill, Mark] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Baumgarten, Cory; Rocca, Jorge J.] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. RP Reagan, BA (reprint author), Colorado State Univ, NSF Engn Res Ctr Extreme Ultraviolet Sci & Techno, Ft Collins, CO 80523 USA. EM brendan.reagan@colostate.edu OI Berrill, Mark/0000-0002-4525-3939 FU AMOS program of the Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation Engineering Research Center for Extreme Ultraviolet Science and Technology [0521649]; NSF [CNS-0923386]; U.S. Department of Energy [DE-AC05-00OR22725] FX The authors acknowledge the contributions of Alden H. Curtis, Federico J. Furch, Brad Luther, Brandon Carr, Anthony Nichols, Leon Durivage, and Chase Salsbury. This work was supported by the AMOS program of the Office of Basic Energy Sciences, U.S. Department of Energy and by the National Science Foundation Engineering Research Center for Extreme Ultraviolet Science and Technology using equipment developed with NSFMRI Grant No. 0521649. Optical coatings for the driver laser were developed by Dinesh Patel and Carmen S. Menoni with the support of the Office of Naval Research and the High Energy Laser Program of the Department of Defense Joint Technology Office. This research used the CSU ISTeC HPC System supported by NSF Grant No. CNS-0923386. M.B. acknowledges support for staff members at Oak Ridge National Laboratory managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. Accordingly, the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U. S. Government purposes. NR 29 TC 14 Z9 14 U1 5 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAY 15 PY 2014 VL 89 IS 5 AR 053820 DI 10.1103/PhysRevA.89.053820 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AH1MO UT WOS:000335885100012 ER PT J AU Sun, SXL Kaduwela, AP Gray, AX Fadley, CS AF Sun, S. X. -L. Kaduwela, A. P. Gray, A. X. Fadley, C. S. TI Progress toward time-resolved molecular imaging: A theoretical study of optimal parameters in static photoelectron holography SO PHYSICAL REVIEW A LA English DT Article ID SCATTERING DIFFRACTION PATTERNS; IMAGES; RECONSTRUCTION; SPECTROSCOPY; SURFACE; WAVE AB The availability of short-pulse free-electron lasers has led to the idea of using photoelectron holography as a method of directly imaging molecular dissociations or reactions in real time, as, e. g., in a recent theoretical study by Krasniqi et al., [ F. Krasniqi, B. Najjari, L. Struder, D. Rolles, A. Voitkiv, and J. Ullrich, Phys. Rev. A 81, 033411 (2010)]. In this paper, we extend this earlier work and in particular look at two critical questions concerning the optimum type of data required for such holographic imaging: the choice of photoelectron kinetic energy (e. g., similar to 300 eV versus similar to 1700 eV as in the prior study), and the use of a single energy or multiple energies. After verifying that our calculations fully duplicate those in this prior paper, we show that using lower energies is preferable to using higher energies for image quality, a conclusion consistent with prior photoelectron holography studies at surfaces, and that multiple lower energies in which the hologram effectively spans a volume in kspace yields the best quality images that should be useful for such "molecular movies." Although the amount of data required for such multi-energy holography is roughly an order of magnitude higher than that for single energy, the reduction of artifacts and the improved quality of the images suggest this as the optimum ultimate future strategy for such dynamic imaging. C1 [Sun, S. X. -L.; Gray, A. X.; Fadley, C. S.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Kaduwela, A. P.] Calif Environm Protect Agcy, Air Resources Board, Sacramento, CA 95814 USA. [Kaduwela, A. P.] Univ Calif Davis, Dept Land Air & Water Resources, Davis, CA 95616 USA. [Gray, A. X.; Fadley, C. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Gray, A. X.] Stanford Univ, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94029 USA. [Gray, A. X.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94029 USA. RP Sun, SXL (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. OI Kaduwela, Ajith/0000-0002-7236-2698 FU Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy [DE-AC02-05CH11231]; Stanford Institute for Materials and Energy Science (SIMES) FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy under Contract No. DE-AC02-05CH11231. Research at Stanford was supported through the Stanford Institute for Materials and Energy Science (SIMES) and the LCLS by the US Department of Energy, Office of Basic Energy Sciences. We also acknowledge helpful comments concerning the software from C. Y. Fong, P. M. Len, and S. Savrasov. NR 27 TC 3 Z9 3 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAY 15 PY 2014 VL 89 IS 5 AR 053415 DI 10.1103/PhysRevA.89.053415 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AH1MO UT WOS:000335885100010 ER PT J AU Okamoto, S Zhu, WG Nomura, Y Arita, R Xiao, D Nagaosa, N AF Okamoto, Satoshi Zhu, Wenguang Nomura, Yusuke Arita, Ryotaro Xiao, Di Nagaosa, Naoto TI Correlation effects in (111) bilayers of perovskite transition-metal oxides SO PHYSICAL REVIEW B LA English DT Article ID INFINITE DIMENSIONS; INSULATOR; SURFACE; STATE; PHASE AB We investigate the correlation-induced Mott, magnetic, and topological phase transitions in artificial (111) bilayers of perovskite transition-metal oxides LaAuO3 and SrIrO3 for which the previous density-functional theory calculations predicted topological insulating states. Using the dynamical-mean-field theory with realistic band structures and Coulomb interactions, LaAuO3 bilayer is shown to be far away from a Mott insulating regime, and a topological-insulating state is robust. On the other hand, SrIrO3 bilayer is on the verge of an orbital-selective topological Mott transition and turns to a trivial insulator by an antiferromagnetic ordering. Oxide bilayers thus provide a novel class of topological materials for which the interplay between the spin-orbit coupling and electron-electron interactions is a fundamental ingredient. C1 [Okamoto, Satoshi] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Zhu, Wenguang] Univ Sci & Technol China, ICQD HFNL, Hefei 230026, Anhui, Peoples R China. [Nomura, Yusuke; Arita, Ryotaro; Nagaosa, Naoto] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Xiao, Di] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [Nagaosa, Naoto] RIKEN, CEMS, Wako, Saitama 3510198, Japan. RP Okamoto, S (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM okapon@ornl.gov RI Okamoto, Satoshi/G-5390-2011; Nagaosa, Naoto/G-7057-2012; Arita, Ryotaro/D-5965-2012; Xiao, Di/B-1830-2008; Nomura, Yusuke/B-8504-2014 OI Okamoto, Satoshi/0000-0002-0493-7568; Arita, Ryotaro/0000-0001-5725-072X; Xiao, Di/0000-0003-0165-6848; FU U. S. Department of Energy; Basic Energy Sciences; Materials Sciences and Engineering Division; National Natural Science Foundation of China [11374273]; AFOSR [FA9550-12-1-0479]; Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan [24224009]; Strategic International Cooperative Program (Joint Research Type) from Japan Science and Technology Agency; World-Leading Innovative R&D on Science and Technology (FIRST Program); [12J08652] FX S.O. thanks M. S. Bahramy, B.-J. Yang, and J. Matsuno for their fruitful discussions and RIKEN CEMS for hospitality during his visit under the FIRST Theory Forum Visiting Scientist program. The research by S.O. is supported by the U. S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. W.Z. is supported by National Natural Science Foundation of China (No. 11374273). Y.N. is supported by Grant-in-Aid for JSPS Fellows (12J08652). D. X. is supported by AFOSR Grant No. FA9550-12-1-0479. N.N. is supported by Grant-in-Aids for Scientific Research (S) (No. 24224009) from the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan, Strategic International Cooperative Program (Joint Research Type) from Japan Science and Technology Agency, and by Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST Program). NR 59 TC 20 Z9 20 U1 3 U2 65 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 15 PY 2014 VL 89 IS 19 AR 195121 DI 10.1103/PhysRevB.89.195121 PG 9 WC Physics, Condensed Matter SC Physics GA AH1MX UT WOS:000335886100003 ER PT J AU Shin, CS Butler, MC Wang, HJ Avalos, CE Seltzer, SJ Liu, RB Pines, A Bajaj, VS AF Shin, Chang S. Butler, Mark C. Wang, Hai-Jing Avalos, Claudia E. Seltzer, Scott J. Liu, Ren-Bao Pines, Alexander Bajaj, Vikram S. TI Optically detected nuclear quadrupolar interaction of N-14 in nitrogen-vacancy centers in diamond SO PHYSICAL REVIEW B LA English DT Article ID ECHO ENVELOPE MODULATION; RESONANCE-SPECTROSCOPY; MAGNETIC-RESONANCE; TRIPLET-STATE; COHERENT DYNAMICS; RAMAN HETERODYNE; ZERO-FIELD; SPIN; ELECTRON; MAGNETOMETRY AB We report sensitive detection of the nuclear quadrupolar interaction of the N-14 nuclear spin of the nitrogen-vacancy (NV) center using the electron spin-echo envelope modulation technique. We applied a weak transverse magnetic field to the spin system so that certain forbidden transitions became weakly allowed due to second-order effects involving the nonsecular terms of the hyperfine interaction. The weak transitions cause modulation of the electron spin-echo signal, and a theoretical analysis suggests that the modulation frequency is primarily determined by the nuclear quadrupolar frequency; numerical simulations confirm the analytical results and show excellent quantitative agreement with experiments. This is an experimentally simple method of detecting quadrupolar interactions, and it can be used to study spin systems with an energy structure similar to that of the NV center. C1 [Shin, Chang S.; Butler, Mark C.; Wang, Hai-Jing; Avalos, Claudia E.; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Shin, Chang S.; Butler, Mark C.; Wang, Hai-Jing; Avalos, Claudia E.; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shin, Chang S.; Butler, Mark C.; Wang, Hai-Jing; Avalos, Claudia E.; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Liu, Ren-Bao] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Liu, Ren-Bao] Chinese Univ Hong Kong, Ctr Quantum Coherence, Shatin, Hong Kong, Peoples R China. RP Bajaj, VS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. EM vikbajaj@gmail.com RI Liu, Ren-Bao/B-3729-2011 OI Liu, Ren-Bao/0000-0002-0620-2370 FU Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [CHE-0957655]; Hong Kong RGC-NSFC [N_CUHK403/11] FX This paper was supported by the Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. M.B. acknowledges salary support from the National Science Foundation under Award No. CHE-0957655. R.L. acknowledges support from Hong Kong RGC-NSFC Project No. N_CUHK403/11. NR 42 TC 5 Z9 5 U1 1 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 15 PY 2014 VL 89 IS 20 AR 205202 DI 10.1103/PhysRevB.89.205202 PG 6 WC Physics, Condensed Matter SC Physics GA AH1NB UT WOS:000335886500006 ER PT J AU Kortelainen, M McDonnell, J Nazarewicz, W Olsen, E Reinhard, PG Sarich, J Schunck, N Wild, SM Davesne, D Erler, J Pastore, A AF Kortelainen, M. McDonnell, J. Nazarewicz, W. Olsen, E. Reinhard, P. -G. Sarich, J. Schunck, N. Wild, S. M. Davesne, D. Erler, J. Pastore, A. TI Nuclear energy density optimization: Shell structure SO PHYSICAL REVIEW C LA English DT Article ID HARTREE-FOCK; MEAN-FIELD; SKYRMES INTERACTION; FUNCTIONAL THEORY; EXOTIC NUCLEI; PARAMETRIZATION; FISSION; FORCES; STATE; MODEL AB Background: Nuclear density functional theory is the only microscopical theory that can be applied throughout the entire nuclear landscape. Its key ingredient is the energy density functional. Purpose: In this work, we propose a new parametrization UNEDF2 of the Skyrme energy density functional. Methods: The functional optimization is carried out using the POUNDerS optimization algorithm within the framework of the Skyrme Hartree-Fock-Bogoliubov theory. Compared to the previous parametrization UNEDF1, restrictions on the tensor term of the energy density have been lifted, yielding a very general form of the energy density functional up to second order in derivatives of the one-body density matrix. In order to impose constraints on all the parameters of the functional, selected data on single-particle splittings in spherical doubly-magic nuclei have been included into the experimental dataset. Results: The agreement with both bulk and spectroscopic nuclear properties achieved by the resulting UNEDF2 parametrization is comparable with UNEDF1. While there is a small improvement on single-particle spectra and binding energies of closed shell nuclei, the reproduction of fission barriers and fission isomer excitation energies has degraded. As compared to previous UNEDF parametrizations, the parameter confidence interval for UNEDF2 is narrower. In particular, our results overlap well with those obtained in previous systematic studies of the spin-orbit and tensor terms. Conclusions: UNEDF2 can be viewed as an all-around Skyrme EDF that performs reasonably well for both global nuclear properties and shell structure. However, after adding new data aiming to better constrain the nuclear functional, its quality has improved only marginally. These results suggest that the standard Skyrme energy density has reached its limits, and significant changes to the form of the functional are needed. C1 [Kortelainen, M.] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland. [Kortelainen, M.; McDonnell, J.; Nazarewicz, W.; Olsen, E.; Schunck, N.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Kortelainen, M.; McDonnell, J.; Nazarewicz, W.; Schunck, N.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [McDonnell, J.; Schunck, N.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94551 USA. [Nazarewicz, W.] Warsaw Univ, Inst Theoret Phys, Warsaw, Poland. [Reinhard, P. -G.] Univ Erlangen Nurnberg, Inst Theoret Phys, D-91054 Erlangen, Germany. [Sarich, J.; Wild, S. M.] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA. [Davesne, D.] Univ Lyon 1, F-69622 Lyon, France. [Davesne, D.] Univ Lyon 1, F-69622 Villeurbanne, France. [Davesne, D.] Inst Phys Nucl, CNRS, IN2P3, Lyon, France. [Erler, J.] German Canc Res Ctr, Div Biophys Macromol, D-69120 Heidelberg, Germany. [Pastore, A.] Univ Libre Bruxelles, Inst Astron & Astrophys, B-1050 Brussels, Belgium. RP Kortelainen, M (reprint author), Univ Jyvaskyla, Dept Phys, POB 35 YFL, FI-40014 Jyvaskyla, Finland. RI Wild, Stefan/P-4907-2016; OI Wild, Stefan/0000-0002-6099-2772; Schunck, Nicolas/0000-0002-9203-6849; Pastore, Alessandro/0000-0003-3354-6432 FU US Department of Energy [DE-SC0008499, DE-FG02-96ER40963, DE-FG52-09NA29461, DE-AC02-06CH11357, DE-AC52-07NA27344]; FIDIPRO program; European Union's Seventh Framework Programme ENSAR (THEXO) [262010]; Livermore Computing Resource Center at Lawrence Livermore National Laboratory; Laboratory Computing Resource Center at Argonne National Laboratory FX We are deeply indebted to the late M. Stoitsov, whose contribution to this work, especially the DFT solver and its interface with the POUNDerS algorithm, was considerable. This work was supported by the US Department of Energy under Contracts No. DE-SC0008499, No. DE-FG02-96ER40963, and No. DE-FG52-09NA29461 (University of Tennessee), No. DE-AC02-06CH11357 (Argonne National Laboratory), and No. DE-AC52-07NA27344 (Lawrence Livermore National Laboratory); by the Academy of Finland under the Centre of Excellence Programme 2012-2017 (Nuclear and Accelerator Based Physics Programme at JYFL) and FIDIPRO program; and by the European Union's Seventh Framework Programme ENSAR (THEXO) under Grant No. 262010. Computational resources were provided through an INCITE award "Computational Nuclear Structure" by the National Center for Computational Sciences (NCCS) and National Institute for Computational Sciences (NICS) at Oak Ridge National Laboratory, through a grant by the Livermore Computing Resource Center at Lawrence Livermore National Laboratory, and through a grant by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 96 TC 54 Z9 54 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 15 PY 2014 VL 89 IS 5 AR 054314 DI 10.1103/PhysRevC.89.054314 PG 16 WC Physics, Nuclear SC Physics GA AH1NF UT WOS:000335886900001 ER PT J AU Watanabe, H Murayama, H AF Watanabe, Haruki Murayama, Hitoshi TI Noncommuting Momenta of Topological Solitons SO PHYSICAL REVIEW LETTERS LA English DT Article ID SKYRMION LATTICE; ALGEBRAS; FORCE AB We show that momentum operators of a topological soliton may not commute among themselves when the soliton is associated with the second cohomology H-2 of the target space. The commutation relation is proportional to the winding number, taking a constant value within each topological sector. The noncommutativity makes it impossible to specify the momentum of a topological soliton, and induces a Magnus force. C1 [Watanabe, Haruki; Murayama, Hitoshi] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Murayama, Hitoshi] Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Murayama, Hitoshi] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. RP Watanabe, H (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM hwatanabe@berkeley.edu; hitoshi@berkeley.edu FU Honjo International Scholarship Foundation; U. S. DOE [DE-AC03-76SF00098]; NSF [PHY-1002399, PHY-1316783]; JSPS Grant [23540289]; WPI, MEXT, Japan FX We thank Masahito Ueda for stimulating suggestions, and Igor Shovkovy, Uwe-Jens Wiese, Yoshimasa Hidaka, and other attendees of the workshop "Effective Field Theory for Quantum Many Body Systems" at IFT UAM-CSIC (the Centro de Excelencia Severo Ochoa Program, under Grant No. SEV-2012-0249) for fruitful comments. We are grateful for useful discussions with Tomoya Hayata, Michikazu Kobayashi, Muneto Nitta, Yasuhiro Tada, Masaki Oshikawa, and Ashvin Vishwanath. H. M. also thanks Scott Carnahan and Yoshitake Hashimoto for useful discussions on cohomology and representation theory. We also thank Grigori Volovik for informing us of Ref. [12]. H. W. appreciates financial support from the Honjo International Scholarship Foundation. The work of H. M. was supported by the U. S. DOE under Contract No. DE-AC03-76SF00098, by the NSF under Grants No. PHY-1002399 and No. PHY-1316783, by the JSPS Grant No. (C) 23540289, and by WPI, MEXT, Japan. NR 37 TC 12 Z9 12 U1 0 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 15 PY 2014 VL 112 IS 19 AR 191804 DI 10.1103/PhysRevLett.112.191804 PG 5 WC Physics, Multidisciplinary SC Physics GA AH1NV UT WOS:000335888700004 PM 24877932 ER PT J AU Zhu, JX Janoschek, M Rosenberg, R Ronning, F Thompson, JD Torrez, MA Bauer, ED Batista, CD AF Zhu, Jian-Xin Janoschek, Marc Rosenberg, Richard Ronning, Filip Thompson, J. D. Torrez, Michael A. Bauer, Eric D. Batista, Cristian D. TI LDA plus DMFT Approach to Magnetocrystalline Anisotropy of Strong Magnets SO PHYSICAL REVIEW X LA English DT Article ID MEAN-FIELD THEORY; RAY CIRCULAR-DICHROISM; ELECTRONIC-STRUCTURE; ORBITAL MAGNETISM; SYSTEMS; ENERGY; YCO5; MAGNETIZATION; TRANSITION; METALS AB The new challenges posed by the need of finding strong rare-earth-free magnets demand methods that can predict magnetization and magnetocrystalline anisotropy energy (MAE). We argue that correlated electron effects, which are normally underestimated in band-structure calculations, play a crucial role in the development of the orbital component of the magnetic moments. Because magnetic anisotropy arises from this orbital component, the ability to include correlation effects has profound consequences on our predictive power of the MAE of strong magnets. Here, we show that incorporating the local effects of electronic correlations with dynamical mean-field theory provides reliable estimates of the orbital moment, the mass enhancement, and the MAE of YCo5. C1 [Zhu, Jian-Xin; Janoschek, Marc; Ronning, Filip; Thompson, J. D.; Torrez, Michael A.; Bauer, Eric D.; Batista, Cristian D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Rosenberg, Richard] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Zhu, JX (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM jxzhu@lanl.gov; cdb@lanl.gov RI Janoschek, Marc/M-8871-2015; Batista, Cristian/J-8008-2016; OI Janoschek, Marc/0000-0002-2943-0173; Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU U.S DOE through LDRD program [DE-AC52- 06NA25396] FX We are grateful to Tomasz Durakiewicz, O. Granas, J. Schweizer, F. Tasset, P. Thunstrom, and J. M. Wills for helpful discussions. Work at the LANL was performed under the auspices of the U.S. DOE Contract No. DE-AC52- 06NA25396 through the LDRD program. Part of the theoretical calculations were carried out on a Linux cluster in the Center for Integrated Nanotechnologies, a DOE Office of Basic Energy Sciences user facility. NR 44 TC 3 Z9 3 U1 1 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAY 15 PY 2014 VL 4 IS 2 AR 021027 DI 10.1103/PhysRevX.4.021027 PG 7 WC Physics, Multidisciplinary SC Physics GA AH1NS UT WOS:000335888300002 ER PT J AU Blau, PJ AF Blau, Peter J. TI A multi-stage wear model for grid-to-rod fretting of nuclear fuel rods SO WEAR LA English DT Article DE Wear; Fretting; Fuel-rods; Zircaloy-4; Impact wear ID BEHAVIOR; ZIRCALOY-4; CORROSION; TUBE AB The wear of fuel rod cladding against the supporting structures in the cores of pressurized water nuclear reactors (PWRs) is an important and potentially costly tribological issue. Grid-to-rod fretting (GTRF), as it is known, involves not only time-varying contact conditions, but also elevated temperatures, flowing hot water, aqueous tribo-corrosion, and the embrittling effects of neutron fluences. The multi-stage, closedform analytical model described in this paper relies on published out-of-reactor wear and corrosion data and a set of simplifying assumptions to portray the conversion of frictional work into wear depth. The cladding material of interest is a zirconium-based alloy called Zircaloy-4 which rubs against dimples or springs on the supporting grid which may be composed of the same or a different alloy. The model involves an incubation stage, a surface oxide wear stage, and a base alloy wear stage. The wear coefficient, which is a measure of the efficiency of conversion of frictional work into wear damage, can change to reflect the evolving metallurgical condition of the alloy. Wear coefficients for Zircaloy-4 and for a polyphase zirconia layer were back-calculated for a range of times required to wear to a critical depth. Inputs for the model, like the friction coefficient, are taken from the tribology literature in lieu of inreactor tribological data. Concepts of classical fretting were used as a basis, but are modified to enable the model to accommodate the complexities of the PWR environment. Factors like grid spring relaxation, pre-oxidation of the cladding, multiple oxide phases, gap formation, impact, and hydrogen embrittlement are part of the problem definition but uncertainties in their relative roles limits the ability to validate the model. Sample calculations of wear depth versus time in the cladding illustrate how GTRF wear might occur in a discontinuous fashion during months-long reactor operating cycles. A means to account for grid/rod gaps and repetitive impact effects on GTRF wear is proposed. 2014 Elsevier B.V. All rights reserved. C1 Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Blau, PJ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, POB 2008,Mail Stop 6063, Oak Ridge, TN 37831 USA. EM weartester@msn.com FU Consortium for Advanced Simulation of Light Water Reactors; Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy [DE-ACO5-000R22725] FX This research was supported by the Consortium for Advanced Simulation of Light Water Reactors (http://www.casl.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy Contract no. DE-ACO5-000R22725. The author wishes to express his appreciation for the comments and advice of R. Lu and Z. Karoutas (Westinghouse Electric Company, LLC), R. Montgomery (Tennessee Valley Authority), Brian Wirth (the University of Tennessee/ORNL), and Jeremy Busby and Theodore Besmann of ORNL The comments and suggestions of the Wear journal reviewers are greatly appreciated. NR 30 TC 10 Z9 10 U1 3 U2 15 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0043-1648 J9 WEAR JI Wear PD MAY 15 PY 2014 VL 313 IS 1-2 BP 89 EP 96 DI 10.1016/j.wear.2014.02.016 PG 8 WC Engineering, Mechanical; Materials Science, Multidisciplinary SC Engineering; Materials Science GA AH3EH UT WOS:000336005900011 ER PT J AU Tang, MJ Marian, J AF Tang, Meijie Marian, Jaime TI Temperature and high strain rate dependence of tensile deformation behavior in single-crystal iron from dislocation dynamics simulations SO ACTA MATERIALIA LA English DT Article DE Dislocation dynamics; High strain rate deformation; Fe single crystals; Materials strength ID CONSTITUTIVE DESCRIPTION; MECHANICAL RESPONSE; FLOW-STRESS; ALUMINUM; METALS; STRENGTH; COPPER; SPALL; MOBILITY; ALLOYS AB We conduct dislocation dynamics simulations of Fe periodic single crystals under tensile load at several high strain rates and temperatures. The simulations are connected to the atomistic scale via recently developed, temperature-dependent dislocation mobility relations. We explore strain rates from 10(4) to 10(6) s(-1) at temperatures of 100, 300 and 600 K. We compute the flow stress as a function of strain rate and temperature, and find very good agreement with experimental data for Fe, suggesting that strain hardening is the dominant materials response mechanism in the range of conditions explored here. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Tang, Meijie; Marian, Jaime] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Marian, J (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave,L-367, Livermore, CA 94551 USA. EM marian1@llnl.gov FU U.S. Department of Energy [DE-AC52-07NA27344]; DOE's Early Career Research Program FX We thank R. Cook for help with visualizing the dislocation microstructure and S. Aubry for helpful discussions. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. J.M. acknowledges support from DOE's Early Career Research Program. NR 34 TC 10 Z9 10 U1 1 U2 29 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2014 VL 70 BP 123 EP 129 DI 10.1016/j.actamat.2014.02.013 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AG7ZE UT WOS:000335636500012 ER PT J AU Gludovatz, B Naleway, SE Ritchie, RO Kruzic, JJ AF Gludovatz, Bernd Naleway, Steven E. Ritchie, Robert O. Kruzic, Jamie J. TI Size-dependent fracture toughness of bulk metallic glasses SO ACTA MATERIALIA LA English DT Article DE Bulk metallic glasses; Fracture toughness; Sample size; Strain softening; Bending ductility ID SUPERCOOLED LIQUID REGION; NI-CU-BE; AMORPHOUS-ALLOYS; RESISTANCE CURVE; SHEAR-BAND; BEHAVIOR; FATIGUE; TEMPERATURE; PLATES AB The fracture toughness is a critical material property that determines engineering performance. However, as is well known for crystalline materials, if certain sample geometry and size requirements are not met, test results become sample-size dependent and difficult to compare between different studies. Here, the room-temperature fracture toughness of the Zr-based bulk metallic glass (BMG) Zr52.5Cu17.9Ni14.6Al10Ti5 (Vitreloy 105) was evaluated using compact-tension, as well as single-edge notched-bend, specimens of different sizes to measure K-Ic values according to ASTM standard E399 and J(Ic) values according to ASTM standard E1820. It is concluded that the ASTM standard E399 sample-size requirements should be cautiously accepted as providing size-independent (valid) K-Ic results for BMGs; however, it is also concluded that small-sized samples may result in a wider scatter in conditional toughness K-Q values, a smaller yield of valid tests and possibly somewhat elevated toughness values. Such behavior is distinct from crystalline metals where the size requirements of ASTM standard E399 are quite conservative. For BMGs, KQ values increase and show a larger scatter with decreasing uncracked ligament width b, which is also distinct from crystalline metals. Samples smaller than required by ASTM standards for Kk testing are allowed by the J-integral-based standard E1820; however, in this study on BMGs, such tests were found to give significantly higher toughness values as compared to valid K-Ic results. Overall, the toughness behavior of BMGs is more sensitive to size requirements than for crystalline metals, an observation that is likely related to the distinct size-dependent bending ductility and strain softening behavior found for metallic glasses. It is concluded that toughness values measured on BMG samples smaller than that required by the K-Ic standard, which are common in the literature, are likely sample size- and geometry-dependent, even when they meet the less restrictive valid J(Ic) requirements. (c) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Gludovatz, Bernd; Ritchie, Robert O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Naleway, Steven E.; Kruzic, Jamie J.] Oregon State Univ, Sch Mech Ind & Mfg Engn, Corvallis, OR 97331 USA. [Ritchie, Robert O.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Kruzic, JJ (reprint author), Oregon State Univ, Sch Mech Ind & Mfg Engn, Corvallis, OR 97331 USA. EM jamie.kruzic@oregonstate.edu RI Ritchie, Robert/A-8066-2008; Kruzic, Jamie/M-3558-2014; Naleway, Steven/K-3497-2016 OI Ritchie, Robert/0000-0002-0501-6998; Gludovatz, Bernd/0000-0002-2420-3879; Kruzic, Jamie/0000-0002-9695-1921; Naleway, Steven/0000-0001-9413-0399 FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231]; Arthur E. Hitsman Faculty Scholarship; Alexander von Humboldt Foundation Friedrich Wilhelm Bessel Award; Mechanical Behavior of Materials Program at the Lawrence Berkeley National Laboratory (LBNL) FX Support for B.G. and R.O.R. was provided by the Mechanical Behavior of Materials Program at the Lawrence Berkeley National Laboratory (LBNL) by the Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. J.J.K. acknowledges the support of the Arthur E. Hitsman Faculty Scholarship and the Alexander von Humboldt Foundation Friedrich Wilhelm Bessel Award. The authors also wish to thank Mr. Bochao Lu for aid in sample preparation at LBNL and Dr. Andy Waniuk of Liquidmetal Technologies for help in preparing the BMG plates. NR 36 TC 28 Z9 28 U1 10 U2 99 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2014 VL 70 BP 198 EP 207 DI 10.1016/j.actamat.2014.01.062 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AG7ZE UT WOS:000335636500018 ER PT J AU Williams, SH Brown, DW Clausen, B Russell, A Gschneidner, KA AF Williams, Scott H. Brown, Donald W. Clausen, Bjorn Russell, Alan Gschneidner, Karl A., Jr. TI Observations of a dynamical-to-kinematic diffraction transition in plastically deformed polycrystalline intermetallic YCu SO ACTA MATERIALIA LA English DT Article DE YCu intermetallic compound; Plastic deformation; Diffraction; dynamic; Diffraction; kinematic; Mosaic structure ID CRYSTALS; DEFORMATION; EXTINCTION; REFINEMENT; FRACTURE; ALLOYS; YAG AB Unlike most intermetallic compounds, polycrystalline YCu, a B2 (CsCl-type) intermetallic, is ductile at room temperature. The mechanisms for this behavior are not fully understood. In situ neutron diffraction was used to investigate whether a stress-induced phase transformation or twinning contribute to the ductility; however, neither mechanism was found to be active in YCu. Surprisingly, this study revealed that the intensities of the diffraction peaks increased after plastic deformation. It is thought that annealing the samples created nearly perfect crystallinity, and subsequent deformation reduced this high degree of lattice coherency, resulting in a modified mosaic structure that decreased or eliminated the extinction effect. Analysis of changes in diffraction peak intensity showed a region of primary plasticity that exhibits significant changes in diffraction behavior. Fully annealed samples initially contain diffracting volumes large enough to follow the dynamical theory of diffraction. When loaded beyond the yield point, dislocation motion disrupts the lattice perfection, and the diffracting volume is reduced to the point that diffraction follows the kinematic theory of diffraction. Since the sample preparation and deformation mechanisms present in this study are common in numerous material systems, this dynamical to kinematic diffraction transition should also be considered in other diffraction experiments. These measurements also suggest the possibility of a new method of investigating structural characteristics. (C) 2014 Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Williams, Scott H.; Russell, Alan; Gschneidner, Karl A., Jr.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Brown, Donald W.; Clausen, Bjorn] Los Alamos Natl Lab, Lujan Ctr, LANSCE 12, Los Alamos, NM 87545 USA. [Russell, Alan; Gschneidner, Karl A., Jr.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RP Gschneidner, KA (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM williams.scott.h@gmail.com; cagey@ameslab.gov RI Clausen, Bjorn/B-3618-2015; OI Clausen, Bjorn/0000-0003-3906-846X; Williams, Scott/0000-0002-1959-3091; Russell, Alan/0000-0001-5264-0104 FU The Ames Laboratory is operated by Iowa State University for the US Department of Energy [DE-ACO2-07CH11358]; Office of Basic Energy of Sciences, Materials Sciences Division of the Office of Science; National Science Foundation's Division of Materials Research [0413616]; National Science Foundation; FWP [2012LANLE389] FX The Ames Laboratory is operated by Iowa State University for the US Department of Energy under Contract No. DE-ACO2-07CH11358. Work at the Ames Laboratory is supported by the Office of Basic Energy of Sciences, Materials Sciences Division of the Office of Science (50% A.R., 100% K.A.G.). The authors wish to thank their colleague Prof. V.K. Pecharsky for useful discussions and the Materials Preparation Center of the Ames Laboratory for their assistance in making the samples. Portions of this research were supported by the National Science Foundation's Division of Materials Research through Grant No. 0413616 (100% S.H.W., 50% A.R.). Any opinions, findings and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation. Much of this research was perfoimed on the SMARTS instrument at the Lujan Center at Los Alamos National Laboratory supported by DOE-Basic Energy Sciences under FWP No. 2012LANLE389 (100% D.B., 100% B.C.). We are grateful to S. Vogel of LANSCE for his invaluable guidance in equipment operation and subsequent diffraction data analysis. NR 32 TC 1 Z9 1 U1 2 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2014 VL 70 BP 307 EP 315 DI 10.1016/j.actamat.2014.01.044 PG 9 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AG7ZE UT WOS:000335636500029 ER PT J AU Schaefer, BT Cheung, J Ihlefeld, JF Jones, JL Nagarajan, V AF Schaefer, Brian T. Cheung, Jeffrey Ihlefeld, Jon F. Jones, Jacob L. Nagarajan, Valanoor TI Stability and dewetting kinetics of thin gold films on Ti, TiOx and ZnO adhesion layers (vol 61, pg 7841, 2013) SO ACTA MATERIALIA LA English DT Correction C1 [Schaefer, Brian T.; Jones, Jacob L.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Schaefer, Brian T.; Cheung, Jeffrey; Jones, Jacob L.; Nagarajan, Valanoor] Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia. [Ihlefeld, Jon F.] Sandia Natl Labs, Elect Opt & Nano Mat Dept, Albuquerque, NM 87185 USA. RP Nagarajan, V (reprint author), Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia. EM nagarajan@unsw.edu.au RI valanoor, nagarajan/B-4159-2012 NR 1 TC 0 Z9 0 U1 0 U2 16 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2014 VL 70 BP 316 EP 317 DI 10.1016/j.actamat.2013.12.024 PG 2 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AG7ZE UT WOS:000335636500030 ER PT J AU Ray, PK Akinc, M Kramer, MJ AF Ray, P. K. Akinc, M. Kramer, M. J. TI Formation of multilayered scale during the oxidation of NiAl-Mo alloy SO APPLIED SURFACE SCIENCE LA English DT Article DE Mo-NiAl; High temperature alloys; Oxidation ID SI-B ALLOYS; MICROSTRUCTURE; TRANSITION; BEHAVIOR; GROWTH AB We have studied the oxidation behavior of a hypereutectic NiAl-Mo alloy. This alloy showed an initial rapid mass loss followed by a relatively steady state behavior. The oxide scale formed during the oxidation process was seen to have a multilayered structure comprising of NiO, NiAl2O4, NiMoO4 and Al2O3 with minor amounts of MoO2 in the sub-scale region. The oxidation behavior is influenced significantly by the formation and stability of the constituent oxides, especially NiMoO4. Hence the decomposition behavior of NiMoO4 in the 1100-1200 degrees C was studied as well. The thermal decomposition of the NiMoO4 was slow at 1100 degrees C, but accelerated at 1200 degrees C, resulting in the formation of NiO, which remained in the oxide scale, and MoO3, which volatilized away. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ray, P. K.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Ray, PK (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM prat@iastate.edu RI Ray, Pratik/C-5383-2008 OI Ray, Pratik/0000-0002-0656-4566 NR 23 TC 5 Z9 5 U1 1 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD MAY 15 PY 2014 VL 301 SI SI BP 107 EP 111 DI 10.1016/j.apsusc.2014.01.148 PG 5 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AG0HD UT WOS:000335095600018 ER PT J AU Dong, XY Li, J Fu, JS Gao, Y Huang, K Zhuang, GS AF Dong, Xinyi Li, Juan Fu, Joshua S. Gao, Yang Huang, Kan Zhuang, Guoshun TI Inorganic aerosols responses to emission changes in Yangtze River Delta, China SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE FM2.5; YRD; Inorganic aerosols sensitivity ID AIR-QUALITY; CONTROL POLICIES; MODELING SYSTEM; POLLUTION; SENSITIVITY; NITRATE; SHANGHAI; IMPACT; CITIES; OZONE AB The new Chinese National Ambient Air Quality standards (CH-NAAQS) published on Feb. 29th, 2012 listed PM2.5 as criteria pollutant for the very first time. In order to probe into PM2.5 pollution over Yangtze River Delta, the integrated MM5/CMAQmodeling system is applied for a full year simulation to examine the PM2.5 concentration and seasonality, and also the inorganic aerosols responses to precursor emission changes. Total PM2.5 concentration over YRD was found to have strong seasonal variation with higher values in winter months (up to 89.9 mu g/m(3) in January) and lower values in summer months (down to 28.8 mu g/m(3) in July). Inorganic aerosols were found to have substantial contribution to PM2.5 over YRD, ranging from 37.1% in November to 52.8% in May. Nocturnal production of nitrate (NO3-) through heterogeneous hydrolysis of N2O5 was found significantly contribute to high NW concentration throughout the year. In winter, NO3- was found to increase under nitrogen oxides (NOx) emission reduction due to higher production of N2O5 from the excessive ozone (O-3) introduced by attenuated titration, which further lead to increase of ammonium (NH4+) and sulfate (SO42-), while other seasons showed decrease response of NO3- Sensitivity responses of NO3- under anthropogenic VOC emission reduction was examined and demonstrated that in urban areas over YRD, NO3- formation was actually more sensitive to VOC than NOx due to the O-3-involved nighttime chemistry of N2O5, while a reduction of NOx emission may have counter-intuitive effect by increasing concentrations of inorganic aerosols. (C) 2014 Elsevier B.V. All rights reserved. C1 [Dong, Xinyi; Fu, Joshua S.; Gao, Yang; Huang, Kan] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Li, Juan] Shanghai Environm Monitoring Ctr, Shanghai 200030, Peoples R China. [Gao, Yang] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99354 USA. [Zhuang, Guoshun] Fudan Univ, Dept Environm Sci & Engn, Ctr Atmospher Chem Study, Shanghai 200433, Peoples R China. RP Fu, JS (reprint author), Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. EM jsfu@utk.edu RI Huang, Kan/E-4824-2011; OI Li, Juan/0000-0002-1555-5397 FU Energy Foundation [G-1208-16611]; National Key Project of Basic Research of China [2006CB403704]; National Natural Science Foundation of China [20877020, 40575062, 40599420]; Office of Science of the U.S. Department of Energy, Regional and Global Climate Modeling Program; Battelle Memorial Institute [DE-AC05-76RL01830] FX This study was supported by the Energy Foundation under Grant No. G-1208-16611. This work was also partially support by the National Key Project of Basic Research of China (Grant No. 2006CB403704) and the National Natural Science Foundation of China (Grant Nos. 20877020, 40575062, and 40599420) of China. Yang Gao is partly supported by the Office of Science of the U.S. Department of Energy as part of the Regional and Global Climate Modeling Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. Any opinions, findings, and conclusions expressed in this material are those of the authors. NR 31 TC 8 Z9 12 U1 5 U2 69 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD MAY 15 PY 2014 VL 481 BP 522 EP 532 DI 10.1016/j.scitotenv.2014.02.076 PG 11 WC Environmental Sciences SC Environmental Sciences & Ecology GA AG0HL UT WOS:000335096400058 PM 24631615 ER PT J AU Cismasu, AC Michel, FM Tcaciuc, AP Brown, GE AF Cismasu, A. Cristina Michel, F. Marc Tcaciuc, A. Patricia Brown, Gordon E., Jr. TI Properties of impurity-bearing ferrihydrite III. Effects of Si on the structure of 2-line ferrihydrite SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; K-EDGE; SYNTHETIC FERRIHYDRITE; 6-LINE FERRIHYDRITE; AQUEOUS-SOLUTIONS; FERRIC OXIDES; PDF ANALYSIS; NANOCRYSTALLINE MATERIAL; POLYHEDRAL APPROACH; IRON OXYHYDROXIDE AB Siliceous ferrihydrites are abundant nanoparticles in natural environments. Although it is well known that the physical properties of ferrihydrite are affected when formed in the presence of silicate oxoanions (SiO44-), the structure of siliceous ferrihydrites (SiFh), and the speciation of Si within these nanosolids are not well understood. In this study we evaluate the effects of Si (at concentrations ranging from 5 to 40 mol% Si) on synthetic ferrihydrite precipitates using structural data derived from synchrotron-based high energy X-ray scattering and pair distribution function (PDF) analysis, in combination with X-ray absorption near edge structure (XANES) spectroscopy, and transmission electron microscopy (TEM). Silicate oxoanions have a major effect on Fe(O,OH)(x) polyhedral polymerization and ferrihydrite particle growth, illustrated by the formation of smaller, poorly crystalline, structurally disordered/strained ferrihydrite nanocrystallites. Variation in Fh unit-cell parameters is suggested to arise from substantial particle size-induced structural disorder. As a result of this significant size-dependent structural disorder, it was not possible to identify evidence for Si4+ for Fe3+ substitution in these samples based on unit cell parameter variations or refinement of different structural models. Principal component analyses (PCA) and linear combination fits carried out on the PDFs suggest that iron partitions between several phases (e. g., ferrihydrite and an Fe-bearing amorphous silica phase (Amorph. SiO2 + Fe)) in these co-precipitates. A mechanism of co-precipitation is proposed, in which silicate binds to Fe polymers and Fh particles, thus inhibiting particle growth at low Si content. At higher Si content, SiO44- polymerization traps significant Fe, and we suggest that the occurrence of this second Fe pool limits further the availability of Fe required for ferrihydrite particle development. Such Si-ferrihydrite co-precipitates are expected to be more stable in natural environments with respect to reductive dissolution or transformation, and to impact the bioavailability of Fe(III). (C) 2014 Elsevier Ltd. All rights reserved. C1 [Cismasu, A. Cristina; Michel, F. Marc; Brown, Gordon E., Jr.] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. [Tcaciuc, A. Patricia] MIT, Woods Hole Oceanog Inst, Cambridge, MA 02139 USA. [Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Dept Photon Sci, Menlo Pk, CA 94025 USA. [Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. RP Cismasu, AC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd Mail Stop 74R316C, Berkeley, CA 94720 USA. EM accismasu@lbl.gov FU DOE-BER [DE-SC0006772]; NSF [EF-0830093]; DOE-BER; Corning Inc. Foundation; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. DOE, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This study was supported by DOE-BER Grant DE-SC0006772 (C. C., G. B.), NSF Grant EF-0830093 (Center for Environmental Implications of Nanotechnology) (G. B., C. C., M. M.), DOE-BER Science Focus Area funding to SLAC (M. M., G. B.), and the Corning Inc. Foundation (C. C., G. B.). The STXM and Si K-edge XANES data reported in this paper were collected at the Advanced Light Source, Lawrence Berkeley National Laboratory. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We are also grateful for access to the Advanced Photon Source, Argonne National Laboratory, where the X-ray scattering studies were carried out. The APS is supported by the U.S. DOE, Office of Basic Energy Sciences under Contract DE-AC02-06CH11357. We wish to thank Peter Chupas and Evan Maxey (APS) for technical support on APS BL ID-11-B, Tolek Tyliszczak (ALS) for support at ALS beamline 11.0.2, and Guangchao Li (Stanford University) for ICP-OES analyses. NR 76 TC 15 Z9 16 U1 14 U2 85 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2014 VL 133 BP 168 EP 185 DI 10.1016/j.gca.2014.02.018 PG 18 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AF6OE UT WOS:000334833600010 ER PT J AU Bishop, ME Glasser, P Dong, HL Arey, B Kovarik, L AF Bishop, Michael E. Glasser, Paul Dong, Hailiang Arey, Bruce Kovarik, Libor TI Reduction and immobilization of hexavalent chromium by microbially reduced Fe-bearing clay minerals SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID ENERGY-LOSS SPECTROSCOPY; CHROMATE REDUCTION; AQUEOUS-SOLUTIONS; CR(VI) REDUCTION; FE(III) REDUCTION; GEOBACTER-SULFURREDUCENS; DRINKING-WATER; NITROAROMATIC COMPOUNDS; DISSIMILATORY FE(III); STRUCTURAL IRON AB Hexavalent chromium (Cr6+) is a major contaminant in the environment. As a redox-sensitive element, the fate and toxicity of chromium is controlled by reduction-oxidation (redox) reactions. Previous research has shown the ability of structural Fe(II) in naturally present and chemically reduced clay minerals to reduce Cr6+ to Cr(III) as a way of immobilization and detoxification. However, it is still poorly known whether or not structural Fe(II) in biologically reduced clay minerals exhibits a similar reactivity and if so, what the kinetics and mechanisms of Cr6+ reduction are. The objective of this study was to determine the kinetics and possible mechanisms of Cr6+ reduction by structural Fe(II) in microbially reduced clay minerals and the nature of reduced Cr(III). Structural Fe(III) in nontronite (NAu-2), montmorillonite (SWy-2), chlorite (CCa-2), and clay-rich sediments from the Ringold Formation of the Hanford site of Washington State, USA was first bioreduced to Fe(II) by an iron-reducing bacterium Geobacter sulfurreducens with acetate as the sole electron donor and anthraquinone-2,6-disulfonate (AQDS) as electron shuttle in synthetic groundwater (pH 7). Biogenic Fe(II) was then used to reduce aqueous Cr6+ at three different temperatures, 10, 20, and 30 degrees C, in order to determine the temperature dependence of the redox reaction between Cr6+ and clay-Fe(II). The results showed that nontronite and montmorillonite were most effective in reducing aqueous Cr6+ at all three temperatures. In contrast, most Fe(II) in chlorite was not reactive towards Cr6+ reduction at 10 degrees C, though at 30 degrees C there was some reduction. For all the clay minerals, the ratio of total Fe(II) oxidized to Cr6+ reduced was close to the expected stoichiometric value of 3. Characterization of the Cr-clay reaction product with scanning electron microscopy with focused ion beam and transmission electron microscopy with electron energy loss spectroscopy revealed that reduced chromium was possibly in the form of sub-nanometer Cr2O3 in association with residual clay minerals as micro-aggregates. This textural association was expected to minimize the chance of Cr(III) reoxidation upon exposure to oxidants. These results are important for our understanding of how various clay minerals may be used to reductively immobilize the heavy metal contaminant Cr in the environment. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Bishop, Michael E.; Glasser, Paul; Dong, Hailiang] Miami Univ, Dept Geol & Environm Earth Sci, Oxford, OH 45056 USA. [Arey, Bruce; Kovarik, Libor] Pacific Northwest Natl Lab, Richland, WA USA. RP Dong, HL (reprint author), Miami Univ, Dept Geol & Environm Earth Sci, Oxford, OH 45056 USA. EM dongh@miamioh.edu RI Kovarik, Libor/L-7139-2016 FU Subsurface Biogeochemical Research (SBR) Program, Office of Science (BER), U.S. Department of Energy (DOE) [DE-SC0005333]; Department of Energy's Office of Biological and Environmental Research FX This research was supported by the Subsurface Biogeochemical Research (SBR) Program, Office of Science (BER), U.S. Department of Energy (DOE) grant no. DE-SC0005333 to H. D. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory. The authors are grateful to Associate Editor and three anonymous reviewers whose comments significantly improved the quality of the manuscript. NR 112 TC 14 Z9 15 U1 16 U2 129 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2014 VL 133 BP 186 EP 203 DI 10.1016/j.gca.2014.02.040 PG 18 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AF6OE UT WOS:000334833600011 ER PT J AU Thakur, P Xiong, YL Borkowski, M Choppin, GR AF Thakur, Punam Xiong, Yongliang Borkowski, Marian Choppin, Gregory R. TI Improved thermodynamic model for interaction of EDTA with trivalent actinides and lanthanide to ionic strength of 6.60 m SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID NUCLEAR-WASTE ISOLATION; NACLO4 MEDIA; AQUEOUS THERMODYNAMICS; CHLORIDE COMPLEXATION; STABILITY-CONSTANTS; NATURAL-WATERS; OXALATE; SOLUBILITY; CITRATE; SYSTEM AB The dissociation constants of ethylenediaminetetraacetic acid (H(4)EDTA), and the stability constants of Am3+, Cm3+ and Eu3+ with EDTA(4-) have been determined at 25 degrees C, over a range of concentration varying from 0.1 to 6.60 m NaClO4 using potentiometric titration and an extraction technique, respectively. The formation of only 1: 1 complex, M(EDTA)(-), where (M = Am3+, Cm3+ and Eu3+), was observed under the experimental conditions. The observed ionic strength dependencies of the dissociation constants and the stability constants have been described successfully over the entire ionic strength range using the Pitzer model. The thermodynamic stability constant: log beta(0)(101) = 20.55 +/- 0.18 for Am3+, log beta(0)(101) = 20.43 +/- 0.20 for Cm3+ and log beta(0)(101) 20.65 +/- 0.19 for Eu3+ were calculated by extrapolation of data to zero ionic strength in an NaClO4 medium. In addition, log beta(0)(101) of 20.05 +/- 0.40 for Am3+ was obtained by simultaneously modeling data both in NaCl and NaClO4 media. For all stability constants, the Pitzer model gives an excellent representation of the data using interaction parameters beta((0)), beta((1)), and C-phi determined in this work. The improved model presented in this work would enable researchers to model accurately the potential mobility of actinides (III) and light rare earth elements to ionic strength of 6.60 m in low temperature environments in the presence of EDTA. Published by Elsevier Ltd. C1 [Thakur, Punam; Choppin, Gregory R.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Xiong, Yongliang] Sandia Natl Labs, Carlsbad Program Grp, Carlsbad, NM 88220 USA. [Borkowski, Marian] Los Alamos Natl Lab, Carlsbad, NM 88220 USA. RP Thakur, P (reprint author), Carlsbad Environm Monitoring & Res Ctr, 1400 Univ Dr, Carlsbad, NM 88220 USA. EM pthakur@cemrc.org FU US Department of Energy, Office of Basic Energy Science; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The support of this work by the US Department of Energy, Office of Basic Energy Science, is gratefully acknowledged. The Pitzer parameter calculations were performed at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The authors thank the anonymous reviewers whose comments have helped to improve this manuscript. NR 73 TC 2 Z9 2 U1 2 U2 28 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2014 VL 133 BP 299 EP 312 DI 10.1016/j.gca.2013.09.040 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AF6OE UT WOS:000334833600017 ER PT J AU Fakhouri, WD Rahimov, F Attanasio, C Kouwenhoven, EN De Lima, RLF Felix, TM Nitschke, L Huver, D Barrons, J Kousa, YA Leslie, E Pennacchio, LA Van Bokhoven, H Visel, A Zhou, HQ Murray, JC Schutte, BC AF Fakhouri, Walid D. Rahimov, Fedik Attanasio, Catia Kouwenhoven, Evelyn N. De Lima, Renata L. Ferreira Felix, Temis Maria Nitschke, Larissa Huver, David Barrons, Julie Kousa, Youssef A. Leslie, Elizabeth Pennacchio, Len A. Van Bokhoven, Hans Visel, Axel Zhou, Huiqing Murray, Jeffrey C. Schutte, Brian C. TI An etiologic regulatory mutation in IRF6 with loss- and gain-of-function effects SO HUMAN MOLECULAR GENETICS LA English DT Article ID DER-WOUDE-SYNDROME; CLEFT-LIP; P63 BINDING; PALATE; EXPRESSION; ENHANCER; VAN; DIFFERENTIATION; MORPHOGENESIS; FAMILIES AB DNA variation in Interferon Regulatory Factor 6 (IRF6) causes Van der Woude syndrome (VWS), the most common syndromic form of cleft lip and palate (CLP). However, an etiologic variant in IRF6 has been found in only 70 of VWS families. To test whether DNA variants in regulatory elements cause VWS, we sequenced three conserved elements near IRF6 in 70 VWS families that lack an etiologic mutation within IRF6 exons. A rare mutation (350dupA) was found in a conserved IRF6 enhancer element (MCS9.7) in a Brazilian family. The 350dupA mutation abrogated the binding of p63 and E47 transcription factors to cis-overlapping motifs, and significantly disrupted enhancer activity in human cell cultures. Moreover, using a transgenic assay in mice, the 350dupA mutation disrupted the activation of MCS9.7 enhancer element and led to failure of lacZ expression in all head and neck pharyngeal arches. Interestingly, disruption of the p63 Motif1 and/or E47 binding sites by nucleotide substitution did not fully recapitulate the effect of the 350dupA mutation. Rather, we recognized that the 350dupA created a CAAAGT motif, a binding site for Lef1 protein. We showed that Lef1 binds to the mutated site and that overexpression of Lef1/-Catenin chimeric protein repressed MCS9.7-350dupA enhancer activity. In conclusion, our data strongly suggest that 350dupA variant is an etiologic mutation in VWS patients and disrupts enhancer activity by a loss- and gain-of-function mechanism, and thus support the rationale for additional screening for regulatory mutations in patients with CLP. C1 [Fakhouri, Walid D.; Nitschke, Larissa; Huver, David; Barrons, Julie; Schutte, Brian C.] Michigan State Univ, E Lansing, MI 48824 USA. [Kousa, Youssef A.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Schutte, Brian C.] Michigan State Univ, Dept Pediat & Human Dev, E Lansing, MI 48824 USA. [Rahimov, Fedik; De Lima, Renata L. Ferreira; Leslie, Elizabeth; Murray, Jeffrey C.] Univ Iowa, Dept Pediat, Iowa City, IA 52242 USA. [Attanasio, Catia; Pennacchio, Len A.; Visel, Axel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Kouwenhoven, Evelyn N.; Van Bokhoven, Hans; Zhou, Huiqing] Radboud Univ Nijmegen, Med Ctr, Nijmegen Ctr Mol Life Sci, Dept Human Genet, NL-6525 ED Nijmegen, Netherlands. [Van Bokhoven, Hans] Radboud Univ Nijmegen, Med Ctr, Donders Inst Brain Cognit & Behav, Dept Cognit Neurosci, NL-6525 ED Nijmegen, Netherlands. [Felix, Temis Maria] Hosp Clin Porto Alegre, Med Genet Serv, Porto Alegre, RS, Brazil. [Zhou, Huiqing] Radboud Univ Nijmegen, Fac Sci, Dept Mol Dev Biol, NL-6525 ED Nijmegen, Netherlands. RP Schutte, BC (reprint author), Michigan State Univ, 5162 Biomed & Phys Sci Bldg, E Lansing, MI 48823 USA. EM schutteb@msu.edu RI Felix, Temis/B-8073-2010; Visel, Axel/A-9398-2009; Zhou, Huiqing/B-1721-2013; Bokhoven, J.H.L.M./H-8015-2014; attanasio, catia/D-5042-2017; OI Felix, Temis/0000-0002-8401-6821; Visel, Axel/0000-0002-4130-7784; Zhou, Huiqing/0000-0002-2434-3986; Kousa, Youssef A/0000-0001-6049-8144 FU NIH/NIDCR [U01DE020060]; SNSF; Department of Energy, University of California [DE-AC02-05CH11231]; [NIH-DE13513]; [F31DE022696] FX Financial support for this research was provided for B. C. S. by NIH-DE13513 and Y.A.K. by F31DE022696. A. V. was supported by NIH/NIDCR FaceBase grant U01DE020060. C.A. was supported by a SNSF advanced researcher fellowship. Research by A. V. and C. A. was conducted at the E.O. Lawrence Berkeley National Laboratory and performed under Department of Energy Contract DE-AC02-05CH11231, University of California. NR 36 TC 15 Z9 15 U1 0 U2 5 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0964-6906 EI 1460-2083 J9 HUM MOL GENET JI Hum. Mol. Genet. PD MAY 15 PY 2014 VL 23 IS 10 BP 2711 EP 2720 DI 10.1093/hmg/ddt664 PG 10 WC Biochemistry & Molecular Biology; Genetics & Heredity SC Biochemistry & Molecular Biology; Genetics & Heredity GA AF4PB UT WOS:000334694800016 PM 24442519 ER PT J AU Schoonen, MA Schoonen, JMT AF Schoonen, Martin A. Schoonen, Jan M. T. TI Removal of crystal violet from aqueous solutions using coal SO JOURNAL OF COLLOID AND INTERFACE SCIENCE LA English DT Article DE Crystal violet; Wastewater; Coal; Sorption; Pyrite ID HYDROXYL RADICALS; HYDROGEN-PEROXIDE; IR SPECTROSCOPY; DYE ADSORPTION; PHASE-ANALYSIS; OXIDATION; DEGRADATION; PYRITE; POROSITY; OXYGEN AB The interaction of crystal violet (CV) and six standard reference coals with varying amounts of pyrite was studied using batch sorption experiments. The experiments were designed to test the hypothesis that pyrite-containing coal removes CV through a combination of sorption and a Fenton-like degradation reaction involving pyrite. While pure pyrite does degrade CV slowly through a Fenton-like mechanism, bituminous coals containing pyrite showed far less CV removal than subbituminous coals without pyrite. Hence, the presence of pyrite in coal does not lead to an enhanced removal of CV from solution. Instead, the surface charge of coal appears to exert a primary role on the uptake of CV. The subbituminous coals tested in this study have a negative surface charge between pH 3 and 8, which facilitates the uptake of the cationic dye. Sorption of cationic CV onto subbituminous coal leads to a charge reversal. Modeling of the sorption kinetics suggest that CV diffuses into pore space within the coal after sorbing onto the surface, which is consistent with the fact that CV is not released after uptake by the coal. The results of this study indicate that subbituminous coal might be a useful sorbent for CV contained in waste streams generated in dye processes. Coal is a cheap bulk commodity, CV does not desorb easily, and the resulting CV-containing coal could be burned to incinerate the contaminant while producing energy. (c) 2014 Elsevier Inc. All rights reserved. C1 [Schoonen, Martin A.; Schoonen, Jan M. T.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Schoonen, Jan M. T.] Stevens Inst Technol, Dept Chem Engn & Mat Sci, Hoboken, NJ 07030 USA. RP Schoonen, MA (reprint author), Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. EM martin.schoonen@stonybrook.edu; jschoone@stevens.edu RI Schoonen, martin/E-7703-2011 OI Schoonen, martin/0000-0002-7133-1160 NR 45 TC 6 Z9 6 U1 1 U2 29 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9797 EI 1095-7103 J9 J COLLOID INTERF SCI JI J. Colloid Interface Sci. PD MAY 15 PY 2014 VL 422 BP 1 EP 8 DI 10.1016/j.jcis.2014.02.008 PG 8 WC Chemistry, Physical SC Chemistry GA AF3ZY UT WOS:000334652400001 PM 24655821 ER PT J AU Neumann, B Gesing, TM Rednyk, A Matolin, V Gash, AE Baumer, M AF Neumann, Bjoern Gesing, Thorsten M. Rednyk, Andrii Matolin, Vladimir Gash, Alexander E. Baeumer, Marcus TI Sol-gel preparation of alumina stabilized rare earth areo- and xerogels and their use as oxidation catalysts SO JOURNAL OF COLLOID AND INTERFACE SCIENCE LA English DT Article DE Sol-gel chemistry; Aerogels; Xerogels; Rare earth oxides; CO oxidation ID OXIDE; AEROGELS; METHANE AB A new sal-gel synthesis route for rare earth (Ce and Pr) alumina hybrid aero- and xerogels is presented which is based on the so-called epoxide addition method. The resulting materials are characterized by TEM, XRD and nitrogen adsorption. The results reveal a different crystallization behavior for the praseodymia/alumina and the ceria/alumina gel. Whereas the first remains amorphous until 875 degrees C, small ceria domains form already after preparation in the second case which grow with increasing calcination temperature. The use of the calcined gels as CO oxidation catalysts was studied in a quartz tube (lab) reactor and in a (slit) microreactor and compared to reference catalysts consisting of the pure rare earth oxides. The Ce/Al hybrid gels exhibit a good catalytic activity and a thermal stability against sintering which was superior to the investigated reference catalyst. In contrast, the Pr/Al hybrid gels show lower CO oxidation activity which, due to the formation of PrAlO3, decreased with increasing calcination temperature. (c) 2014 Elsevier Inc. All rights reserved. C1 [Neumann, Bjoern; Baeumer, Marcus] Univ Bremen, Inst Appl & Phys Chem, D-28359 Bremen, Germany. [Neumann, Bjoern; Baeumer, Marcus] Univ Bremen, Ctr Environm Res & Sustainable Technol, D-28359 Bremen, Germany. [Gesing, Thorsten M.] Univ Bremen, Inst Inorgan Chem, Solid State Chem Crystallog, D-28359 Bremen, Germany. [Rednyk, Andrii; Matolin, Vladimir] Charles Univ Prague, Fac Math & Phys, Dept Surface & Plasma Sci, Prague 18000 8, Czech Republic. [Gash, Alexander E.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. RP Gash, AE (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. EM gash2@llnl.gov; mbaeumer@uni-bremen.de RI Baumer, Marcus/S-5441-2016 OI Baumer, Marcus/0000-0002-8620-1764 FU Deutsche Forschungsgemeinschaft (DFG) [BA1710/19-1]; Heisenberg program [GE1981/3-1]; Deutsche Telekom Stiftung; US Department of Energy by Lawrence Livermore National Laboratory [AC52-07NA27344]; COST Action [MP0903]; Czech Ministry of Education [LD11047] FX We thank Dr. Karsten Thiel (Fraunhofer Institute IFAM, Bremen) and Dr. Willian Menezes (University Bremen) for TEM measurements and Florian Meierhofer and Prof. Dr. Lutz Madler (IWT Foundation) for N2 adsorption. We also gratefully acknowledge financial support for this work provided by the Deutsche Forschungsgemeinschaft (DFG) through grant number BA1710/19-1. TMG especially acknowledges the DFG for a support in the Heisenberg program (GE1981/3-1). BN is grateful for a stipend of the Deutsche Telekom Stiftung. The LLNL work contribution to this report was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. AR acknowledges financial support by the COST Action MP0903 and the COST supporting project LD11047 of the Czech Ministry of Education. NR 17 TC 1 Z9 1 U1 2 U2 48 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9797 EI 1095-7103 J9 J COLLOID INTERF SCI JI J. Colloid Interface Sci. PD MAY 15 PY 2014 VL 422 BP 71 EP 78 DI 10.1016/j.jcis.2014.02.004 PG 8 WC Chemistry, Physical SC Chemistry GA AF3ZY UT WOS:000334652400011 PM 24655831 ER PT J AU Marsh, HS Reid, OG Barnes, G Heeney, M Stingelin, N Rumbles, G AF Marsh, Hilary S. Reid, Obadiah G. Barnes, George Heeney, Martin Stingelin, Natalie Rumbles, Garry TI Control of Polythiophene Film Microstructure and Charge Carrier Dynamics Through Crystallization Temperature SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE conjugated polymers; microwave conductivity; solid-state structure; structure-property relations; thin films ID POLYMER SOLAR-CELLS; CONJUGATED POLYMERS; MORPHOLOGY; POLY(3-HEXYLTHIOPHENE); SEPARATION; CRYSTALS; POLY(3-ALKYLTHIOPHENES); POLYETHYLENE; ABSORPTION; TRANSITION AB The microstructure of neat conjugated polymers is crucial in determining the ultimate morphology and photovoltaic performance of polymer/fullerene blends, yet until recently, little work has focused on controlling the former. Here, we demonstrate that both the long-range order along the (100)-direction and the lamellar crystal thickness along the (001)-direction in neat poly(3-hexylthiophene) (P3HT) and poly[(3,3-didecyl[2,2:5,2-terthiophene]-5,5-diyl)] (PTTT-10) thin films can be manipulated by varying crystallization temperature. Changes in crystalline domain size impact the yield and dynamics of photogenerated charge carriers. Time-resolved microwave conductivity measurements show that neat polymer films composed of larger crystalline domains have longer photoconductance lifetimes and charge carrier yield decreases with increasing crystallite size for P3HT. Our results suggest that the classical polymer science description of temperature-dependent crystallization of polymers from solution can be used to understand thin-film formation in neat conjugated polymers, and hence, should be considered when discussing the structural evolution of organic bulk heterojunctions. (c) 2014 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2014, 52, 700-707 C1 [Marsh, Hilary S.] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80309 USA. [Marsh, Hilary S.; Reid, Obadiah G.; Rumbles, Garry] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Barnes, George; Heeney, Martin] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England. [Barnes, George; Heeney, Martin; Stingelin, Natalie] Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England. [Stingelin, Natalie] Univ London Imperial Coll Sci Technol & Med, Dept Mat, London SW7 2AZ, England. [Rumbles, Garry] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. RP Rumbles, G (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM garry.rumbles@nrel.gov RI Heeney, Martin/O-1916-2013; Stingelin, Natalie/D-6745-2016; OI Heeney, Martin/0000-0001-6879-5020; Stingelin, Natalie/0000-0002-1414-4545; Rumbles, Garry/0000-0003-0776-1462 FU Solar Photochemistry Program, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Laboratory Directed Research and Development (LDRD) Program at the National Renewable Energy Laboratory [06RF1201]; U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; KAUST Global Collaborative Research Academic Excellence Alliance (AEA) grant; European Research Council (ERC) [279587]; EPRSC [EP/G037515/1] FX The TRMC system described here was funded by the Solar Photochemistry Program, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. The experimental development for controlling polymer crystalline domain size was supported by the Laboratory Directed Research and Development (LDRD) Program at the National Renewable Energy Laboratory under task number 06RF1201. This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. The authors also acknowledge Nikos Kopidakis from the National Renewable Energy Laboratory, Neil Treat from Imperial College, London, and Alex Ayzner and Mike Toney from the Stanford Synchrotron Radiation Lightsource (SSRL) for helpful discussions. Alan Sellinger's group at Colorado School of Mines is acknowledged for the use of the TA Q Series DSC 2000 instrument. This work was also supported by a KAUST Global Collaborative Research Academic Excellence Alliance (AEA) grant. NS is in addition supported by a European Research Council (ERC) Starting Independent Research Fellowship under the grant agreement No. 279587. The authors acknowledge EPRSC grant EP/G037515/1 for funding the polymer synthesis portion of this work. NR 47 TC 6 Z9 6 U1 2 U2 65 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD MAY 15 PY 2014 VL 52 IS 10 BP 700 EP 707 DI 10.1002/polb.23471 PG 8 WC Polymer Science SC Polymer Science GA AE3ZX UT WOS:000333918200002 ER PT J AU Staykov, A Yamabe, J Somerday, BP AF Staykov, Aleksandar Yamabe, Junichiro Somerday, Brian P. TI Effect of Hydrogen Gas Impurities on the Hydrogen Dissociation on Iron Surface SO INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY LA English DT Article DE surface chemistry; density functional theory; surface adsorption; Vienna ab initio Simulation Package code ID FATIGUE-CRACK-PROPAGATION; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; AB-INITIO; STRENGTH STEELS; ADSORPTION; MECHANISM; BEHAVIOR; FRACTURE; GROWTH AB A small addition of oxygen to hydrogen gas is known to mitigate the hydrogen embrittlement (HE) of steels. As atomic hydrogen dissolution in steels is responsible for embrittlement, catalysis of molecular hydrogen dissociation by the steel surface is an essential step in the embrittlement process. The most probable role of oxygen in mitigating HE is to inhibit the reactions between molecular hydrogen and the steel surface. To elucidate the mechanism of such surface reaction of hydrogen with the steel in the presence of oxygen, hydrogen, and oxygen adsorption, dissociation, and coadsorption on the Fe(100) surface were investigated using density functional theory. The results show that traces of O-2 would successfully compete with H-2 for surface adsorption sites due to the grater attractive force acting on the O-2 molecule compared to H-2. The H-2 dissociation would be hindered on iron surfaces with predissociated oxygen. Prompted by the notable results for H-2 + O-2, other practical systems were considered, that is, H-2 + CO and CH4. Calculations were performed for the CO chemisorption and H-2 dissociation on iron surface with predissociated CO, as well as, CH4 surface dissociation. The results indicate that CO inhibition of H-2 dissociation proceeds via similar mechanism to O-2 induced inhibition, whereas CH4 traces in the H-2 gas have no effect on H-2 dissociation. (c) 2014 Wiley Periodicals, Inc. C1 [Staykov, Aleksandar; Yamabe, Junichiro; Somerday, Brian P.] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Fukuoka 812, Japan. [Yamabe, Junichiro] Kyushu Univ, Int Res Ctr Hydrogen Energy, Fukuoka 812, Japan. [Somerday, Brian P.] Sandia Natl Labs, Livermore, CA USA. RP Staykov, A (reprint author), Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Fukuoka 812, Japan. EM alex@i2cner.kyushu-u.ac.jp FU World Premier International Research Center Initiative (WPI), Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT), Japan; Sandia National Laboratories [U.S. Department of Energy] [DE-AC04-94AL85000]; JSPS KAKENHI [24560102] FX Contract grant sponsor: World Premier International Research Center Initiative (WPI), Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT), Japan.; Contract grant sponsor: Sandia National Laboratories [(B.P.S.) U.S. Department of Energy]; contract grant number: DE-AC04-94AL85000.; Contract grant sponsor: JSPS KAKENHI (Grant-in-Aid for Scientific Research); contract grant number: 24560102. NR 49 TC 5 Z9 5 U1 4 U2 33 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0020-7608 EI 1097-461X J9 INT J QUANTUM CHEM JI Int. J. Quantum Chem. PD MAY 15 PY 2014 VL 114 IS 10 BP 626 EP 635 DI 10.1002/qua.24633 PG 10 WC Chemistry, Physical; Mathematics, Interdisciplinary Applications; Physics, Atomic, Molecular & Chemical SC Chemistry; Mathematics; Physics GA AD9DI UT WOS:000333564500002 ER PT J AU Kim, JW Travis, JJ Hu, EY Nam, KW Kim, SC Kang, CS Woo, JH Yang, XQ George, SM Oh, KH Cho, SJ Lee, SH AF Kim, Ji Woo Travis, Jonathan J. Hu, Enyuan Nam, Kyung-Wan Kim, Seul Cham Kang, Chan Soon Woo, Jae-Ha Yang, Xiao-Qing George, Steven M. Oh, Kyu Hwan Cho, Sung-Jin Lee, Se-Hee TI Unexpected high power performance of atomic layer deposition coated Li[Ni1/3Mn1/3Co1/3]O-2 cathodes SO JOURNAL OF POWER SOURCES LA English DT Article DE Energy storage; Lithium nickel manganese cobalt oxide; Atomic layer deposition; Rate capability; High temperature cycle-life ID LITHIUM-ION BATTERIES; LI(NI1/3CO1/3MN1/3)O-2; LICO1/3NI1/3MN1/3O2 AB Electric-powered transportation requires an efficient, low-cost, and safe energy storage system with high energy density and power capability. Despite its high specific capacity, the current commercially available cathode material for today's state-of-art Li-ion batteries, lithium nickel manganese cobalt oxide Li[Ni1/3Mn1/3Co1/3]O-2 (NMC), suffers from poor cycle life for high temperature operation and marginal rate capability resulting from irreversible degradation of the cathode material upon cycling. Using an atomicscale surface engineering, the performance of Li[Ni1/3Mn1/3Co1/3]O-2 in terms of rate capability and high temperature cycle-life is significantly improved. The Al2O3 coating deposited by atomic layer deposition (ALD) dramatically reduces the degradation in cell conductivity and reaction kinetics. This durable ultrathin Al2O3-ALD coating layer also improves stability for the NMC at an elevated temperature (55 C). The experimental results suggest that a highly durable and safe cathode material enabled by atomic-scale surface modification could meet the demanding performance and safety requirements of nextgeneration electric vehicles. (c) 2014 Elsevier B.V. All rights reserved. C1 [Kim, Ji Woo; Woo, Jae-Ha; George, Steven M.; Lee, Se-Hee] Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA. [Travis, Jonathan J.; George, Steven M.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Hu, Enyuan; Nam, Kyung-Wan; Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Kim, Seul Cham; Kang, Chan Soon; Oh, Kyu Hwan] Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151742, South Korea. [Cho, Sung-Jin] Johnson Controls Inc, Adv Power Solut, Milwaukee, WI 53209 USA. RP Oh, KH (reprint author), Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151742, South Korea. EM kyuhwan@snu.ac.kr; Sung-Jin.Cho@jci.com; sehee.lee@colorado.edu RI Lee, Sehee/A-5989-2011; Nam, Kyung-Wan/B-9029-2013; Nam, Kyung-Wan/E-9063-2015; George, Steven/O-2163-2013; Hu, Enyuan/D-7492-2016 OI Nam, Kyung-Wan/0000-0001-6278-6369; Nam, Kyung-Wan/0000-0001-6278-6369; George, Steven/0000-0003-0253-9184; Hu, Enyuan/0000-0002-1881-4534 FU National Science Foundation (NSF) [DMR-1206462]; Fundamental R&D Program for Technology of World Premier Materials; Ministry of Knowledge Economy, Republic of Korea [10037919]; U.S. Department of Energy; Office of Vehicle Technologies [DEAC02-98CH10886]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This work was supported by the National Science Foundation (NSF, DMR-1206462). Work at Seoul National University was supported by a grant from the Fundamental R&D Program for Technology of World Premier Materials funded by the Ministry of Knowledge Economy, Republic of Korea (10037919). Work at Brookhaven National Lab. was supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies under Contract No. DEAC02-98CH10886. The authors acknowledge technical supports by the beamline scientist Jianming Bai at beamline X14A of National Synchrotron Light Source, which is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 22 TC 21 Z9 21 U1 9 U2 165 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAY 15 PY 2014 VL 254 BP 190 EP 197 DI 10.1016/j.jpowsour.2013.12.119 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AC4MV UT WOS:000332496300024 ER PT J AU Neuhold, S Vaughey, JT Grogger, C Lopez, CM AF Neuhold, Susanna Vaughey, John T. Grogger, Christa Lopez, Carmen M. TI Enhancement in cycle life of metallic lithium electrodes protected with Fp-silanes SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium; Battery; Coating; Morphology; Silanes ID ELECTROCHEMICAL PERFORMANCE; ION BATTERIES; ANODES; STABILIZATION; CELLS AB Metallic lithium is a promising anode material whose application in rechargeable batteries has been limited by complicated chemical and morphological changes during cycling. These problems can be addressed by the introduction of protective coatings that help to improve the interphasial properties of these electrodes. In this study we used a dip-coating method to generate protective Fp-silane-derived coatings by direct reaction with the surface of metallic lithium. The effect of these coatings has been investigated by comparing the electrochemical performance of coated vs. uncoated electrodes through galvanostatic cycling and electrochemical impedance spectroscopy (EIS). A cycle life enhancement of up to 500% of that of uncoated lithium was observed. Additionally, we observed a trade-off between the value of the obtained stable capacity and the cycle life, which depended on the type of organic substituent on the silane moiety. These results imply that application-tailored protective coatings might, in the near future, enable the efficient use of metallic lithium electrodes in rechargeable batteries. 2013 Elsevier B.V. All rights reserved. C1 [Vaughey, John T.; Lopez, Carmen M.] Argonne Natl Lab, Electrochem Energy Storage Chem Sci & Engn Div, Argonne, IL 60439 USA. [Neuhold, Susanna; Grogger, Christa] Graz Univ Technol, Inst Inorgan Chem, A-8010 Graz, Austria. RP Lopez, CM (reprint author), CIC Energigune, Albert Einstein 48, Minano 01510, Alava, Spain. EM clopez@cicenergigune.com OI Lopez, Carmen M./0000-0002-6096-0674; Vaughey, John/0000-0002-2556-6129 FU Batteries for Advanced Transportation Technologies (BAT!') Program, Office of Vehicle Technologies Program; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, David Howell and Tien Duong FX Support from the Batteries for Advanced Transportation Technologies (BAT!') Program, Office of Vehicle Technologies Program, the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, David Howell and Tien Duong, is gratefully acknowledged. SEM images were recorded using the equipment at the Electron Microscopy Center for Materials Research, Argonne National Laboratory; a US Department of Energy Office of Science Laboratory operated under Contract No. DE-ACO2-06CH11357 by UChicago Argonne, LLC. S. N. would like to acknowledge the support of Gratz University of Technology through the FreChe Materie program. NR 30 TC 2 Z9 2 U1 3 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAY 15 PY 2014 VL 254 BP 241 EP 248 DI 10.1016/j.jpowsour.2013.12.057 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AC4MV UT WOS:000332496300031 ER PT J AU Li, Z Tang, YH Lei, H Caswell, B Karniadakis, GE AF Li, Zhen Tang, Yu-Hang Lei, Huan Caswell, Bruce Karniadakis, George Em TI Energy-conserving dissipative particle dynamics with temperature-dependent properties SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE DPD; Thermal boundary condition; Thermal conductivity; Variable properties; Mesoscopic dynamics ID SLIP BOUNDARY-CONDITIONS; RED-BLOOD-CELLS; TRANSPORT-PROPERTIES; HEAT-CONDUCTION; POISEUILLE FLOW; CONSERVATION; SIMULATION; MECHANICS; MODEL; DPD AB The dynamic properties of fluid, including diffusivity and viscosity, are temperature-dependent and can significantly influence the flow dynamics of mesoscopic non-isothermal systems. To capture the correct temperature-dependence of a fluid, an energy-conserving dissipative particle dynamics (eDPD) model is developed by expressing the weighting terms of the dissipative force and the random force as functions of temperature. The diffusivity and viscosity of liquid water at various temperatures ranging from 273 K to 373 K are used as examples for verifying the proposed model. Simulations of a Poiseuille flow and a steady case of heat conduction for reproducing the Fourier law are carried out to validate the present eDPD formulation and the thermal boundary conditions. Results show that the present eDPD model recovers the standard DPD model when isothermal fluid systems are considered. For non-isothermal fluid systems, the present model can predict the diffusivity and viscosity consistent with available experimental data of liquid water at various temperatures. Moreover, an analytical formula for determining the mesoscopic heat friction is proposed. The validity of the formula is confirmed by reproducing the experimental data for Prandtl number of liquid water at various temperatures. The proposed method is demonstrated in water but it can be readily extended to other liquids. (C) 2014 Elsevier Inc. All rights reserved. C1 [Li, Zhen; Tang, Yu-Hang; Karniadakis, George Em] Brown Univ, Div Appl Math, Providence, RI 02912 USA. [Lei, Huan] Pacific NW Natl Lab, Richland, WA 99352 USA. [Caswell, Bruce] Brown Univ, Sch Engn, Providence, RI 02912 USA. RP Karniadakis, GE (reprint author), Brown Univ, Div Appl Math, Providence, RI 02912 USA. EM george_karniadakis@brown.edu RI Li, Zhen/B-2722-2013 OI Li, Zhen/0000-0002-0936-6928 FU Army Research Laboratory [W911NF-12-2-0023]; new DOE Center on Mathematics for Mesoscopic Modeling of Materials (CM4); INCITE grant FX This work was primarily sponsored by the Army Research Laboratory and was accomplished under Cooperative Agreement Number W911NF-12-2-0023 to University of Utah and partially supported by the new DOE Center on Mathematics for Mesoscopic Modeling of Materials (CM4). Computations were performed at the IBM BG/P with computer time provided by an INCITE grant. NR 34 TC 21 Z9 21 U1 3 U2 52 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 15 PY 2014 VL 265 BP 113 EP 127 DI 10.1016/j.jcp.2014.02.003 PG 15 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AC3KH UT WOS:000332416300007 ER PT J AU Sjogreen, B Yee, HC Vinokur, M AF Sjoegreen, Bjoern Yee, H. C. Vinokur, Marcel TI On high order finite-difference metric discretizations satisfying GCL on moving and deforming grids SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE GCL; High order metric; Moving and deforming grids; High order numerical methods ID GEOMETRIC CONSERVATION LAW; SCHEMES AB In this note we generalize our previous treatment of the discretizations of geometric conservation laws on steady grids (Vinokur and Yee, 2000) to general time dependent grids. The commutative property of mixed difference operators is generalized to apply to time metrics and Jacobians. Our treatment uses half the number of terms as those used in a recent paper by Abe et al. (2012). We also derive the proper temporal discretizations of both Runge-Kutta and linear multistep methods to satisfy the commutativity property for higher than first order. (C) 2014 Published by Elsevier Inc. C1 [Sjoegreen, Bjoern] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Yee, H. C.; Vinokur, Marcel] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. RP Sjogreen, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM Helen.M.Yee@nasa.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Work by the first author performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This is contribution LLNL-TR-637397. NR 10 TC 8 Z9 8 U1 1 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 15 PY 2014 VL 265 BP 211 EP 220 DI 10.1016/j.jcp.2014.01.045 PG 10 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AC3KH UT WOS:000332416300013 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ask, S Aring;sman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Bunse, M Burckhart, H Burdin, S Burgess, T Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Caso, C Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, B Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chavda, V Barajas, CAC Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choudalakis, G Chouridou, S Chow, BKB Christidi, IA Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirilli, M Cirkovic, P Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, B Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coelli, S Coffey, L Cogan, JG Coggeshall, J Colas, J Cole, B Cole, S Colijn, AP Collins-Tooth, C Collot, J Colombo, T Colon, G Compostella, G Muino, PC Coniavitis, E Conidi, MC Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Pedro, RCB Costanzo, D Cote, D Cottin, G Courneyea, L Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Ortuzar, MC Cristinziani, M Crosetti, G Cuciuc, CM Almenar, CC Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dallaire, F Dallapiccola, C Dam, M Damiani, DS Daniells, AC Hoffmann, MD Dao, V Darbo, G Darlea, GL Darmora, S Dassoulas, JA Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S de Graat, J De Groot, N de Jong, P De La Taille, C De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD De Zorzi, G Dearnaley, WJ Debbe, R Debenedetti, C Dechenaux, B Dedovich, DV Degenhardt, J Del Peso, J Del Prete, T Delemontex, T Deliot, F Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C Demers, S Demichev, M Demilly, A Demirkoz, B Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deviveiros, PO Dewhurst, A DeWilde, B Dhaliwal, S Dhullipudi, R Di Ciaccio, A Di Ciaccio, L Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaz, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Yagci, KD Dingfelder, J Dionisi, C Dita, P Dita, S Dittus, F 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CA ATLAS Collaboration TI Measurement of dijet cross-sections in pp collisions at 7 TeV centre-of-mass energy using the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jets; Jet physics; Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; QUARK; LHC; QCD AB Double-differential dijet cross-sections measured in pp collisions at the LHC with a 7 TeV centre-of-mass energy are presented as functions of dijet mass and half the rapidity separation of the two highest-p(T) jets. These measurements are obtained using data corresponding to an integrated luminosity of 4.5 fb(-1), recorded by the ATLAS detector in 2011. The data are corrected for detector effects so that cross-sections are presented at the particle level. Cross-sections are measured up to 5 TeV dijet mass using jets reconstructed with the anti-k(t) algorithm for values of the jet radius parameter of 0.4 and 0.6. The cross-sections are compared with next-to-leading-order perturbative QCD calculations by NLOJet++ corrected to account for non-perturbative effects. Comparisons with POWHEG predictions, using a next-to-leading-order matrix element calculation interfaced to a parton-shower Monte Carlo simulation, are also shown. Electroweak effects are accounted for in both cases. The quantitative comparison of data and theoretical predictions obtained using various parameterizations of the parton distribution functions is performed using a frequentist method. In general, good agreement with data is observed for the NLOJet++ theoretical predictions when using the CT10, NNPDF2.1 and MSTW 2008 PDF sets. Disagreement is observed when using the ABM11 and HERAPDF1.5 PDF sets for some ranges of dijet mass and half the rapidity separation. 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[Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Willis, W.; Wulf, E.; Zhou, L.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Hoffmann, M. Dano; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Dallas, TX 75230 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peschke, R.; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peschke, R.; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Bunse, M.; Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Socher, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Dell'Acqua, A.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Vu Anh, T.; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Martin dit Latour, B.; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St. Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Nadal, J.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1albr, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Whiteson, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.; Wielers, M.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buscher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huettmann, A.; Hulsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. 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E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J. -F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. 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E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. 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P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Vivie De Regie, J. 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[Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Costa Batalha Pedro, R.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. 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T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. 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[Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J. -P.; Mijovic, L.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Inst Rech Lois Fondamentales Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Reece, R.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Huang, Y.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, S.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Ji, H.; Jia, J.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Ahmad, A.; Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Centro Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grpo Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Navarro, G.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn & Elect, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J. -R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Physik, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] CFNUL, Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Ottawa, ON, Canada. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Do Valle Wemans, A.] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] Inst Catalana Recerca & Estudis Avancats, ICREA, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Experimentalphys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Kuday, Sinan/C-8528-2014; Turchikhin, Semen/O-1929-2013; Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Kuleshov, Sergey/D-9940-2013; Ferrando, James/A-9192-2012; Boyko, Igor/J-3659-2013; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Korol, Aleksandr/A-6244-2014; Juste, Aurelio/I-2531-2015; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Monzani, Simone/D-6328-2017; Grinstein, Sebastian/N-3988-2014; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Canelli, Florencia/O-9693-2016; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Ferrer, Antonio/H-2942-2015; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Gabrielli, Alessandro/H-4931-2012; Lokajicek, Milos/G-7800-2014; Castro, Nuno/D-5260-2011; Staroba, Pavel/G-8850-2014; Lei, Xiaowen/O-4348-2014; Doyle, Anthony/C-5889-2009; de Groot, Nicolo/A-2675-2009; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; OI Pina, Joao /0000-0001-8959-5044; Hays, Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Wang, Kuhan/0000-0002-6151-0034; Grohsjean, Alexander/0000-0003-0748-8494; La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Kuday, Sinan/0000-0002-0116-5494; Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Kuleshov, Sergey/0000-0002-3065-326X; Ferrando, James/0000-0002-1007-7816; Boyko, Igor/0000-0002-3355-4662; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Amorim, Antonio/0000-0003-0638-2321; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Cristinziani, Markus/0000-0003-3893-9171; Qian, Jianming/0000-0003-4813-8167; Haas, Andrew/0000-0002-4832-0455; Galhardo, Bruno/0000-0003-0641-301X; Della Volpe, Domenico/0000-0001-8530-7447; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Juste, Aurelio/0000-0002-1558-3291; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Monzani, Simone/0000-0002-0479-2207; Chromek-Burckhart, Doris/0000-0003-4243-3288; Begel, Michael/0000-0002-1634-4399; Mincer, Allen/0000-0002-6307-1418; Grinstein, Sebastian/0000-0002-6460-8694; Bailey, David C/0000-0002-7970-7839; Chen, Hucheng/0000-0002-9936-0115; Nisati, Aleandro/0000-0002-5080-2293; Vari, Riccardo/0000-0002-2814-1337; Gray, Heather/0000-0002-5293-4716; Sawyer, Lee/0000-0001-8295-0605; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Canelli, Florencia/0000-0001-6361-2117; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Ferrer, Antonio/0000-0003-0532-711X; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Gabrielli, Alessandro/0000-0001-5346-7841; Castro, Nuno/0000-0001-8491-4376; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Belanger-Champagne, Camille/0000-0003-2368-2617; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Walsh, Brian/0000-0003-1689-2309; Price, Darren/0000-0003-2750-9977; Filthaut, Frank/0000-0003-3338-2247 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq; FAPESP, Brazil; NSERC; NRC; CFI, Canada; CERN; CONICYT, Chile; CAS; MOST; NSFC, China; COLCIENCIAS, Colombia; MSMT CR; MPO CR; VSC CR, Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany; GSRT; NSRF, Greece; ISF; MINERVA; GIF; DIP; Benoziyo Center, Israel; INFN, Italy; MEXT; JSPS, Japan; CNRST, Morocco; FOM; NWO, Netherlands; BRF; RCN, Norway; MNiSW; NCN, Poland; GRICES; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM; Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS; MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC; Wallenberg Foundation, Sweden; SER; SNSF; Cantons of Bern, Switzerland; Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC; Royal Society; Leverhulme Trust, United Kingdom; DOE; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 71 TC 4 Z9 4 U1 9 U2 96 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 14 PY 2014 IS 5 AR 059 DI 10.1007/JHEP05(2014)059 PG 67 WC Physics, Particles & Fields SC Physics GA AI3DT UT WOS:000336740400001 ER PT J AU Castellanos, S Kivambe, M Hofstetter, J Rinio, M Lai, B Buonassisi, T AF Castellanos, S. Kivambe, M. Hofstetter, J. Rinio, M. Lai, B. Buonassisi, T. TI Variation of dislocation etch-pit geometry: An indicator of bulk microstructure and recombination activity in multicrystalline silicon SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SOLAR-CELLS; DEFECTS AB Dislocation clusters in multicrystalline silicon limit solar cell performance by decreasing minority carrier diffusion length. Studies have shown that the recombination strength of dislocation clusters can vary by up to two orders of magnitude, even within the same wafer. In this contribution, we combine a surface-analysis approach with bulk characterization techniques to explore the underlying root cause of variations in recombination strength among different clusters. We observe that dislocation clusters with higher recombination strength consist of dislocations with a larger variation of line vector, correlated with a higher degree of variation in dislocation etch-pit shapes (ellipticities). Conversely, dislocation clusters exhibiting the lowest recombination strength contain mostly dislocations with identical line vectors, resulting in very similar etch-pit shapes. The disorder of dislocation line vector in high-recombination clusters appears to be correlated with impurity decoration, possibly the cause of the enhanced recombination activity. Based on our observations, we conclude that the relative recombination activity of different dislocation clusters in the device may be predicted via an optical inspection of the distribution and shape variation of dislocation etch pits in the as-grown wafer. (C) 2014 Author(s). C1 [Castellanos, S.; Kivambe, M.; Hofstetter, J.; Buonassisi, T.] MIT, Cambridge, MA 02139 USA. [Rinio, M.] Karlstad Univ, SE-65188 Karlstad, Sweden. [Lai, B.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Castellanos, S (reprint author), MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM sergioc@alum.mit.edu; buonassisi@mit.edu FU U.S. Department of Energy [DE-EE0005314]; National Science Foundation (NSF); Department of Energy under NSF CA [EEC-1041895]; Roberto Rocca Fellowship program; Alexander von Humboldt foundation; NSF [ECS-0335765]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors thank Dr. John Murphy (U. Warwick), David B. Needleman, Sin Cheng Siah, and Dr. Rafael Jaramillo (MIT), Torunn Ervik (NTNU), and Gaute Stokkan (SINTEF) for insightful discussions; Douglas M. Powell (MIT) for his assistance in computer algorithm; David P. Fenning and Ashley E. Morishige (MIT) for synchrotron assistance; Adam T. Paxson (MIT) for figure editing assistance. This work was supported by the U.S. Department of Energy under Contract No. DE-EE0005314, and in part by the National Science Foundation (NSF) and the Department of Energy under NSF CA No. EEC-1041895. S. Castellanos and J. Hofstetter acknowledge support from the Roberto Rocca Fellowship program and the Alexander von Humboldt foundation through a Feodor Lynen postdoctoral fellowship, respectively. Part of this work was performed at the Center for Materials Science and Engineering at MIT, and at the Center for Nanoscale Systems at Harvard University supported by NSF ECS-0335765. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 33 TC 9 Z9 9 U1 2 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2014 VL 115 IS 18 AR 183511 DI 10.1063/1.4876445 PG 7 WC Physics, Applied SC Physics GA AI5OT UT WOS:000336919400015 ER PT J AU Romanenko, A Grassellino, A Melnychuk, O Sergatskov, DA AF Romanenko, A. Grassellino, A. Melnychuk, O. Sergatskov, D. A. TI Dependence of the residual surface resistance of superconducting radio frequency cavities on the cooling dynamics around T-c SO JOURNAL OF APPLIED PHYSICS LA English DT Article AB We report a strong effect of the cooling dynamics through T-c on the amount of trapped external magnetic flux in superconducting niobium cavities. The effect is similar for fine grain and single crystal niobium and all surface treatments including electropolishing with and without 120 degrees C baking and nitrogen doping. Direct magnetic field measurements on the cavity walls show that the effect stems from changes in the flux trapping efficiency: slow cooling leads to almost complete flux trapping and higher residual resistance, while fast cooling leads to the much more efficient flux expulsion and lower residual resistance. (C) 2014 Author(s). C1 [Romanenko, A.; Grassellino, A.; Melnychuk, O.; Sergatskov, D. A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Romanenko, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM aroman@fnal.gov; annag@fnal.gov FU DOE Office of Nuclear Physics; United States Department of Energy [DE-AC02-07CH11359] FX We thank Peter Kneisel from JLab for providing the single crystal cavity for the studies. We acknowledge fruitful discussions with A. Crawford and help with cavity preparation and testing of A. Rowe, D. Bice, M. Wong, Y. Pischalnikov, B. Squires, and all the FNAL cryogenic technical team. The work was partially supported by the DOE Office of Nuclear Physics. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 11 TC 19 Z9 19 U1 2 U2 6 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2014 VL 115 IS 18 AR 184903 DI 10.1063/1.4875655 PG 7 WC Physics, Applied SC Physics GA AI5OT UT WOS:000336919400055 ER PT J AU Berland, K Arter, CA Cooper, VR Lee, K Lundqvist, BI Schroder, E Thonhauser, T Hyldgaard, P AF Berland, Kristian Arter, Calvin A. Cooper, Valentino R. Lee, Kyuho Lundqvist, Bengt I. Schroder, Elsebeth Thonhauser, T. Hyldgaard, Per TI van der Waals density functionals built upon the electron-gas tradition: Facing the challenge of competing interactions SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; GENERALIZED GRADIENT APPROXIMATION; EXCHANGE-CORRELATION ENERGY; SINGLE-PARTICLE SPECTRUM; PHASE-TRANSITIONS; GRAPHITE; ADSORPTION; ACCURATE; FORCES; ADSORBATES AB The theoretical description of sparse matter attracts much interest, in particular for those ground-state properties that can be described by density functional theory. One proposed approach, the van der Waals density functional (vdW-DF) method, rests on strong physical foundations and offers simple yet accurate and robust functionals. A very recent functional within this method called vdW-DF-cx [ K. Berland and P. Hyldgaard, Phys. Rev. B 89, 035412 (2014)] stands out in its attempt to use an exchange energy derived from the same plasmon-based theory from which the nonlocal correlation energy was derived. Encouraged by its good performance for solids, layered materials, and aromatic molecules, we apply it to several systems that are characterized by competing interactions. These include the ferroelectric response in PbTiO3, the adsorption of small molecules within metal-organic frameworks, the graphite/diamond phase transition, and the adsorption of an aromatic-molecule on the Ag(111) surface. Our results indicate that vdW-DF-cx is overall well suited to tackle these challenging systems. In addition to being a competitive density functional for sparse matter, the vdW-DF-cx construction presents a more robust general-purpose functional that could be applied to a range of materials problems with a variety of competing interactions. (C) 2014 AIP Publishing LLC. C1 [Berland, Kristian; Schroder, Elsebeth; Hyldgaard, Per] Chalmers, SE-41296 Gothenburg, Sweden. [Berland, Kristian; Lee, Kyuho] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Arter, Calvin A.; Thonhauser, T.] Wake Forest Univ, Dept Phys, Winston Salem, NC 27109 USA. [Cooper, Valentino R.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Lee, Kyuho] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Lundqvist, Bengt I.] Chalmers, Dept Appl Phys, SE-41296 Gothenburg, Sweden. RP Berland, K (reprint author), Chalmers, MC2, SE-41296 Gothenburg, Sweden. RI Schroder, Elsebeth/A-2030-2011; Cooper, Valentino /A-2070-2012; Foundry, Molecular/G-9968-2014; Hyldgaard, Per/A-2038-2011; OI Schroder, Elsebeth/0000-0003-4995-3585; Cooper, Valentino /0000-0001-6714-4410; Hyldgaard, Per/0000-0001-5810-8119; Berland, Kristian/0000-0002-4655-1233 FU Swedish research council (VR) [VR-2011-4052, VR-2010-4149]; Chalmers Area of Advance, Materials; Swedish pension system; US NSF [DMR-1145968]; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [FG02-12ER16362]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DEAC02-05CH11231] FX The authors thanks H. Rydberg and P. Erhart for useful discussions. Work by K. B., E. S., and P. H. was supported by the Swedish research council (VR) under grants VR-2011-4052 and VR-2010-4149 and by the Chalmers Area of Advance, Materials. Work by B. I. L. was supported via the pension from the Swedish pension system. T. T. acknowledges support from US NSF Grant No. DMR-1145968. V. R. C. was supported by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy. K. L. was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under award DE-FG02-12ER16362. Portions of this work were performed at the Molecular Foundry, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DEAC02-05CH11231. We are also grateful for allocation of computational resources by the Swedish National Infrastructure for Computing (SNIC) and by Wake Forest University. NR 116 TC 26 Z9 26 U1 3 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2014 VL 140 IS 18 AR 18A539 DI 10.1063/1.4871731 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI3SR UT WOS:000336782700042 PM 24832347 ER PT J AU Hao, F Armiento, R Mattsson, AE AF Hao, Feng Armiento, Rickard Mattsson, Ann E. TI Using the electron localization function to correct for confinement physics in semi-local density functional theory SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID GENERALIZED-GRADIENT-APPROXIMATION; SELF-INTERACTION CORRECTION; INITIO MOLECULAR-DYNAMICS; 1ST-PRINCIPLES CALCULATIONS; EXACT EXCHANGE; GROUND-STATE; ENERGY; GAS; TRANSITION; ACCURATE AB We have previously proposed that further improved functionals for density functional theory can be constructed based on the Armiento-Mattsson subsystem functional scheme if, in addition to the uniform electron gas and surface models used in the Armiento-Mattsson 2005 functional, a model for the strongly confined electron gas is also added. However, of central importance for this scheme is an index that identifies regions in space where the correction provided by the confined electron gas should be applied. The electron localization function (ELF) is a well-known indicator of strongly localized electrons. We use a model of a confined electron gas based on the harmonic oscillator to show that regions with high ELF directly coincide with regions where common exchange energy functionals have large errors. This suggests that the harmonic oscillator model together with an index based on the ELF provides the crucial ingredients for future improved semi-local functionals. For a practical illustration of how the proposed scheme is intended to work for a physical system we discuss monoclinic cupric oxide, CuO. A thorough discussion of this system leads us to promote the cell geometry of CuO as a useful benchmark for future semi-local functionals. Very high ELF values are found in a shell around the O ions, and take its maximum value along the Cu-O directions. An estimate of the exchange functional error from the effect of electron confinement in these regions suggests a magnitude and sign that could account for the error in cell geometry. (C) 2014 AIP Publishing LLC. C1 [Hao, Feng; Mattsson, Ann E.] Sandia Natl Labs, Multiscale Sci MS 1322, Albuquerque, NM 87185 USA. [Armiento, Rickard] Linkoping Univ, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden. RP Hao, F (reprint author), Sandia Natl Labs, Multiscale Sci MS 1322, POB 5800, Albuquerque, NM 87185 USA. EM hfeng413@gmail.com; aematts@sandia.gov RI Armiento, Rickard/E-1413-2011 OI Armiento, Rickard/0000-0002-5571-0814 FU Laboratory Directed Research and Development Program; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000]; Swedish Research Council (VR) [621-2011-4249]; Linnaeus Environment at Linkoping on Nanoscale Functional Materials (LiLi-NFM) - VR FX This work was supported by the Laboratory Directed Research and Development Program. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin company, for the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. R. A. acknowledges support from the Swedish Research Council (VR), Grant No. 621-2011-4249 and the Linnaeus Environment at Linkoping on Nanoscale Functional Materials (LiLi-NFM) funded by VR. NR 60 TC 8 Z9 8 U1 0 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2014 VL 140 IS 18 AR 18A536 DI 10.1063/1.4871738 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI3SR UT WOS:000336782700039 PM 24832344 ER PT J AU Lu, DY AF Lu, Deyu TI Evaluation of model exchange-correlation kernels in the adiabatic connection fluctuation-dissipation theorem for inhomogeneous systems SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RANDOM-PHASE-APPROXIMATION; PAIR-DISTRIBUTION FUNCTION; DENSITY-FUNCTIONAL THEORY; ELECTRON-GAS; CORRELATION ENERGIES; METALLIC SURFACE; SOLIDS; LIQUID; ATOMS; STATE AB We investigated the effect of the exchange-correlation kernels of Dobson and Wang (DW) [Phys. Rev. B 62, 10038 (2000)] and Corradini, Del Sole, Onida, and Palummo (CDOP) [Phys. Rev. B 57, 14569 (1998)] in the framework of the adiabatic connection fluctuation-dissipation theorem. The original CDOP kernel was generalized to treat inhomogeneous systems, and an efficient numerical implementation was developed. We found that both kernels improve the correlation energy in bulk silicon as compared to that evaluated from the random phase approximation (RPA). In particular, the correlation energy from the CDOP kernel is in excellent agreement with the diffusion Monte Carlo result. In the case of the Kr dimer, while the DW kernel leads to stronger binding than RPA, the CDOP kernel does the opposite. The cause of this quite different behavior of the two kernels is discussed. Our study suggests that special attention needs to be paid to describe the effective interaction at the low density regions when developing model exchange-correlation kernels. (C) 2014 AIP Publishing LLC. C1 Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Lu, DY (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM dlu@bnl.gov RI Lu, Deyu/O-4418-2016 OI Lu, Deyu/0000-0003-4351-6085 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Research carried out in full at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. D. L. thanks Giulia Galli, Mark Hybertsen, John Dobson, Georg Kresse, and Randy Hood for useful discussions. NR 80 TC 6 Z9 6 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2014 VL 140 IS 18 AR 18A520 DI 10.1063/1.4867538 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI3SR UT WOS:000336782700023 PM 24832328 ER PT J AU Mardirossian, N Head-Gordon, M AF Mardirossian, Narbe Head-Gordon, Martin TI Exploring the limit of accuracy for density functionals based on the generalized gradient approximation: Local, global hybrid, and range-separated hybrid functionals with and without dispersion corrections SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID EXCHANGE-CORRELATION FUNCTIONALS; RARE-GAS ATOMS; THERMOCHEMICAL KINETICS; LONG-RANGE; INTERACTION ENERGIES; NONCOVALENT INTERACTIONS; BENCHMARK DATABASE; BARRIER HEIGHTS; WATER CLUSTERS; DATA SET AB The limit of accuracy for semi-empirical generalized gradient approximation (GGA) density functionals is explored by parameterizing a variety of local, global hybrid, and range-separated hybrid functionals. The training methodology employed differs from conventional approaches in 2 main ways: (1) Instead of uniformly truncating the exchange, same-spin correlation, and opposite-spin correlation functional inhomogeneity correction factors, all possible fits up to fourth order are considered, and (2) Instead of selecting the optimal functionals based solely on their training set performance, the fits are validated on an independent test set and ranked based on their overall performance on the training and test sets. The 3 different methods of accounting for exchange are trained both with and without dispersion corrections (DFT-D2 and VV10), resulting in a total of 491 508 candidate functionals. For each of the 9 functional classes considered, the results illustrate the trade-off between improved training set performance and diminished transferability. Since all 491 508 functionals are uniformly trained and tested, this methodology allows the relative strengths of each type of functional to be consistently compared and contrasted. The range-separated hybrid GGA functional paired with the VV10 nonlocal correlation functional emerges as the most accurate form for the present training and test sets, which span thermochemical energy differences, reaction barriers, and intermolecular interactions involving lighter main group elements. (C) 2014 AIP Publishing LLC. C1 [Mardirossian, Narbe] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Mardirossian, N (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mhg@cchem.berkeley.edu FU Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC0376SF00098]; SciDac Program; NSF [CHE-1048789] FX This work was supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC0376SF00098, and by a grant from the SciDac Program. We acknowledge computational resources obtained under NSF Award No. CHE-1048789. NR 55 TC 20 Z9 20 U1 3 U2 43 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2014 VL 140 IS 18 AR 18A527 DI 10.1063/1.4868117 PG 15 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI3SR UT WOS:000336782700030 PM 24832335 ER PT J AU Yandell, MA King, SB Neumark, DM AF Yandell, Margaret A. King, Sarah B. Neumark, Daniel M. TI Decay dynamics of nascent acetonitrile and nitromethane dipole-bound anions produced by intracluster charge-transfer SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DISSOCIATIVE ELECTRON-ATTACHMENT; RADIATION-INDUCED PHOTODETACHMENT; NEGATIVE-IONS; POLAR-MOLECULES; RELAXATION DYNAMICS; EXCITED-STATES; AUTODETACHMENT SPECTROSCOPY; CLUSTER ANIONS; RYDBERG STATES; CH3CN AB Decay dynamics of nascent dipole bound states of acetonitrile and nitromethane are examined using time-resolved photoelectron imaging of iodide-acetonitrile (I- center dot CH3CN) and iodide-nitromethane (I- center dot CH3NO2) complexes. Dipole-bound anions are created by UV-initiated electron transfer to the molecule of interest from the associated iodide ion at energies just below the vertical detachment energy of the halide-molecule complex. The acetonitrile anion is observed to decay biexponentially with time constants in the range of 4-900 ps. In contrast, the dipole bound state of nitromethane decays rapidly over 400 fs to form the valence bound anion. The nitromethane valence anion species then decays biexponentially with time constants of 2 ps and 1200 ps. The biexponential decay dynamics in acetonitrile are interpreted as iodine atom loss and autodetachment from the excited dipole-bound anion, followed by slower autodetachment of the relaxed metastable ion, while the dynamics of the nitromethane system suggest that a dipole-bound anion to valence anion transition proceeds via intramolecular vibrational energy redistribution to nitro group modes in the vicinity of the iodine atom. (C) 2014 AIP Publishing LLC. C1 [Yandell, Margaret A.; King, Sarah B.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU National Science Foundation (NSF) [CHE-1011819]; NSF Graduate Research Fellowship FX The work described herein was funded by the National Science Foundation (NSF) under Grant No. CHE-1011819. M.A.Y. gratefully acknowledges support from an NSF Graduate Research Fellowship. NR 82 TC 13 Z9 13 U1 6 U2 25 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2014 VL 140 IS 18 AR 184317 DI 10.1063/1.4875021 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AI3SR UT WOS:000336782700081 PM 24832280 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Geiser, A Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G 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A Kuznetsova, E Pardo, PL Martschei, D Mozer, MU Muller, T Niegel, M Nurnberg, A Oberst, O Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Wolf, R Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Ntomari, E Psallidas, A Topsis-giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Mittal, M Nishu, N Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Saxena, P Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K 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CA CMS Collaborat TI Measurement of the properties of a Higgs boson in the four-lepton final state SO PHYSICAL REVIEW D LA English DT Article ID HADRON-HADRON COLLISIONS; ABELIAN GAUGE-THEORIES; ATLAS DETECTOR; PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; WEAK INTERACTIONS; ROOT-S=7 TEV; LHC; MODEL AB The properties of a Higgs boson candidate are measured in the H -> ZZ -> 4l decay channel, with l = e, mu, using data from pp collisions corresponding to an integrated luminosity of 5.1 fb(-1) at the center-of-mass energy of root s = 7 TeV and 19.7 fb(-1) at ffiffiffi root s = 8 TeV, recorded with the CMS detector at the LHC. The new boson is observed as a narrow resonance with a local significance of 6.8 standard deviations, a measured mass of 125.6 +/- 0.4(stat) +/- 0.2(syst) GeV, and a total width <= 3.4 GeV at the 95% confidence level. The production cross section of the new boson times its branching fraction to four leptons is measured to be 0.93(-0.23)(+0.26) (stat)(-0.09)(+0.13) (syst) times that predicted by the standard model. Its spin-parity properties are found to be consistent with the expectations for the standard-model Higgs boson. The hypotheses of a pseudoscalar and all tested spin-1 boson hypotheses are excluded at the 99% confidence level or higher. All tested spin-2 boson hypotheses are excluded at the 95% confidence level or higher. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Gadrat, S.] CNRS, Ctr Calcul, Inst Natl Phys Nucl & Phys Particules, IN2P3, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Alvarez, J. D. Ruiz; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS, Inst Phys Nucl Lyon, IN2P3, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. 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S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Mueller, T.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Psallidas, A.; Topsis-giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, A.; Kumar, A.; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Banerjee, S.; Guchait, M.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, I-56010 Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Machet, M.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Machet, M.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya Jabatan Fiz, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Moreno, S. Carrillo; Valencia, F. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Dubna Joint Nucl Res Inst, Dubna 141980, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Matveev, V.; Andreev, Y.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Sharma, A.; Mohanty, A. K.; Giordano, F.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; Pelliccioni, M.; Seixas, J.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tauscher, L.; Theofilatos, K.; Treille, D.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Cosa, A.; Favaro, C.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Li, W.; Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Bell, K. W.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.; Chen, J.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Johnson, K. F.; Prosper, H.; Tentindo, S.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. 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da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Malik, Sudhir/0000-0002-6356-2655; Gershtein, Yuri/0000-0002-4871-5449; Lazzizzera, Ignazio/0000-0001-5092-7531; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; 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Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Recurrent Financing [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nuclaire et de Physique des Particules/CNRS; Commissariat l'nergie Atomique et aux nergies Alternatives/CEA, France; Bundesministerium fr Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy and the Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Business, Innovation and Employment, New Zealand FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent Financing Contract No. SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nuclaire et de Physique des Particules/CNRS and Commissariat l'nergie Atomique et aux nergies Alternatives/CEA, France; the Bundesministerium fr Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Cincia e a Tecnologia, Portugal; JINR, Dubna, the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretar a de Estado de Investigaci~n, Desarrollo e Innovacin and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey and the Turkish Atomic Energy Authority; the Science and Technology Facilities Council, United Kingdom; the U.S. Department of Energy and the U. S.; National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 150 TC 118 Z9 118 U1 10 U2 102 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 14 PY 2014 VL 89 IS 9 AR 092007 DI 10.1103/PhysRevD.89.092007 PG 45 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH1XK UT WOS:000335914900002 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruehwirth, R Ghete, VM Hoermann, N Hrubec, J Jeitler, M Kiesenhofer, B Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Manganote, EJT Pereira, AV Anjos, TS Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C 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TI Measurement of Inclusive W and Z Boson Production Cross Sections in pp Collisions at root s=8 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID YAN K-FACTOR; P(P)OVER-BAR COLLISIONS; PARTON DISTRIBUTIONS; LHC; ENERGIES AB A measurement of total and fiducial inclusive W and Z boson production cross sections in pp collisions at root s = 8 TeV is presented. Electron and muon final states are analyzed in a data sample collected with the CMS detector corresponding to an integrated luminosity of 18.2 +/- 0.5 pb(-1). The measured total inclusive cross sections times branching fractions are sigma(pp -> WX) x B(W -> l upsilon) = 12.21 +/- 0.03(stat) +/- 0.24(syst) +/- 0.32(lum) nb and sigma(pp -> ZX) x B(Z -> l(+)l(-)) = 1.15 +/- 0.01(stat) +/- 0.02(syst) +/- 0.03(lum) nb for the dilepton mass in the range of 60-120 GeV. The measured values agree with next-to-next-to-leading-order QCD cross section calculations. Ratios of cross sections are reported with a precision of 2%. 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[Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; la Cruz, I. Heredia-de; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. 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[Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, YU-11001 Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, Ctr Invest Energet Medioambient & Tecnol, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. 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Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St. John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Hanson, G.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. 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[Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. 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Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. 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[Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Arfaei, H.; Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Martini, L.] Univ Siena, I-53100 Siena, Italy. [la Cruz, I. Heredia-de] Univ Michoacana, Morelia, Michoacan, Mexico. [Kim, V.] St Petersburg State Polytechn Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. 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RI Ligabue, Franco/F-3432-2014; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Venturi, Andrea/J-1877-2012; Novaes, Sergio/D-3532-2012; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Calvo Alamillo, Enrique/L-1203-2014; Gregores, Eduardo/F-8702-2012; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Gonzalez Caballero, Isidro/E-7350-2010; Yazgan, Efe/A-4915-2015 OI Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Korenkov, Vladimir/0000-0002-2342-7862; Heath, Helen/0000-0001-6576-9740; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Sogut, Kenan/0000-0002-9682-2855; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Novaes, Sergio/0000-0003-0471-8549; Montanari, Alessandro/0000-0003-2748-6373; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Cerrada, Marcos/0000-0003-0112-1691; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Rovelli, Tiziano/0000-0002-9746-4842; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Gonzalez Caballero, Isidro/0000-0002-8087-3199; FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 45 TC 14 Z9 14 U1 5 U2 62 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 14 PY 2014 VL 112 IS 19 AR 191802 DI 10.1103/PhysRevLett.112.191802 PG 17 WC Physics, Multidisciplinary SC Physics GA AH2CR UT WOS:000335928800005 ER PT J AU Wang, ZH Chen, YL Battaglia, V Liu, G AF Wang, Zhihui Chen, Yulin Battaglia, Vincent Liu, Gao TI Improving the performance of lithium-sulfur batteries using conductive polymer and micrometric sulfur powder SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID BOTTOM-UP APPROACH; HIGH-CAPACITY; SILICON NANOWIRES; CATHODE MATERIALS; SHELL; ANODES; ELECTRODES; PARTICLES; NANOTUBES; CELL AB In this study, a conductive polymer, poly(3,4-ethylenedioxythiophene) or PEDOT, was used as binder in the sulfur electrode to study electrochemical performance of lithium-sulfur (Li-S) batteries. PEDOT-based sulfur electrode was compared with that of polyvinylidene difluoride binder based sulfur electrode. Different particle size sulfur materials including commercial micrometric sulfur particles and synthesized colloidal nanometric sulfur powders were chosen as active materials to study the impact of particle size on the cell performance. Different electrolytes including lithium bis(trifluoromethanesulfonyl)imide in polyethylene glycol dimethyl ether (PEGDME) or 1,3-dioxolane-dimethoxy ethane were used in the Li-S batteries to investigate the impact of electrolyte on cell performance. The PEDOT and micrometric sulfur based electrode with PEGDME electrolyte had the best cycle performance, which showed a capacity retention of 68% and specific capacity of 578 mAh/g after 100 cycles. The increased conductivity by conductive polymer and the high viscosity of PEGDME play important roles in the improvement of cycle performance. C1 [Wang, Zhihui; Chen, Yulin; Battaglia, Vincent; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM gliu@lbl.gov FU Vehicle Technologies Office of the U.S. Department of Energy under Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231] FX This research was funded by the Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy under Batteries for Advanced Transportation Technologies (BATT) Program under the contract no. DE-AC02-05CH11231. NR 29 TC 7 Z9 7 U1 8 U2 115 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD MAY 14 PY 2014 VL 29 IS 9 BP 1027 EP 1033 DI 10.1557/jmr.2014.85 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA AH5ZS UT WOS:000336211000001 ER PT J AU An, K Alayoglu, S Musselwhite, N Na, K Somorjai, GA AF An, Kwangjin Alayoglu, Selim Musselwhite, Nathan Na, Kyungsu Somorjai, Gabor A. TI Designed Catalysts from Pt Nanoparticles Supported on Macroporous Oxides for Selective Isomerization of n-Hexane SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID 1-HEXENE ISOMERIZATION; HYDROGENATION; AROMATIZATION; ALUMINA; METALS AB Selective isomerization toward branched hydrocarbons is an important catalytic process in oil refining to obtain high-octane gasoline with minimal content of aromatic compounds. Colloidal Pt nanoparticles with controlled sizes of 1.7, 2.7, and 5.5 nm were deposited onto ordered macroporous oxides of SiO2, Al2O3, TiO2, Nb2O5, Ta2O5, and ZrO2 to investigate Pt size- and support-dependent catalytic selectivity in n-hexane isomerization. Among the macroporous oxides, Nb2O5 and Ta2O5 exhibited the highest product selectivity, yielding predominantly branched C-6 isomers, including 2- or 3-methylpentane, as desired products of n-hexane isomerization (140 Torr n-hexane and 620 Torr H-2 at 360 degrees C). In situ characterizations including X-ray diffraction and ambient-pressure X-ray photoelectron spectroscopy showed that the crystal structures of the oxides in Pt/oxide catalysts were not changed during the reaction and oxidation states of Nb2O5 were maintained under both H-2 and O-2 conditions. Fourier transform infrared spectra of pyridine adsorbed on the oxides showed that Lewis sites were the dominant acidic site of the oxides. Macroporous Nb2O5 and Ta2O5 were identified to play key roles in the selective isomerization by charge transfer at Pt-oxide interfaces. The selectivity was revealed to be Pt size-dependent, with improved isomer production as Pt sizes increased from 1.7 to 5.5 nm. When 5.5 nm Pt nanoparticles were supported on Nb2O5 or Ta2O5, the selectivity toward branched C-6 isomers was further increased, reaching ca. 97% with a minimum content of benzene, due to the combined effects of the Pt size and the strong metal-support interaction. C1 [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu RI Foundry, Molecular/G-9968-2014 FU Office of Basic Energy Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; Chevron Corporation FX This work was supported the Director, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy, under Contract DE-AC02-05CH11231. The user project at the Advanced Light Source and the Molecular Foundry at the Lawrence Berkeley National Laboratory was also supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract DE-AC02-05CH11231. The nanoparticle synthesis was funded by Chevron Corporation. We thank Profs. A. Paul Alivisatos, Peidong Yang, and Omar Yaghi for use of the TEM and XRD instruments; Dr. Gerome Melaet, Walter Ralston, and Stephanus Axnanda for helps in APXPS measurements; Jae-Youn Shin for helping with material preparation; and Jae Hyuck Yoo for the scheme in Figure 1. NR 31 TC 30 Z9 30 U1 23 U2 148 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 14 PY 2014 VL 136 IS 19 BP 6830 EP 6833 DI 10.1021/ja5018656 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AH4EA UT WOS:000336078400014 PM 24773412 ER PT J AU Rangasamy, E Li, JC Sahu, G Dudney, N Liang, CD AF Rangasamy, Ezhiylmurugan Li, Juchuan Sahu, Gayatri Dudney, Nancy Liang, Chengdu TI Pushing the Theoretical Limit of Li-CFx Batteries: A Tale of Bifunctional Electrolyte SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID LITHIUM BATTERIES; IONIC-CONDUCTIVITY; MECHANISM; LI/CFX; CELLS; XPS AB In a typical battery, the inert electrolyte functions solely as the ionic conductor without contribution to the cell capacity. Here we demonstrate that the most energy-dense Li-CFx battery delivers a capacity exceeding the theoretical maximum of CFx with a solid electrolyte of Li3PS4 (LPS) that has dual functions: as the inert electrolyte at the anode and the active component at the cathode. Such a bifunctional electrolyte reconciles both inert and active characteristics through a synergistic discharge mechanism of CFx and LPS. The synergy at the cathode is through LiF, the discharge product of CFx which activates the electrochemical discharge of LPS at a close electrochemical potential of CFx. Therefore, the solid-state Li-CFx batteries output 126.6% energy beyond their theoretic limits without compromising the stability of the cell voltage. The additional energy comes from the electrochemical discharge of LPS, the inert electrolyte. This bifunctional electrolyte revolutionizes the concept of conventional batteries and opens a new avenue for the design of batteries with unprecedented energy density. C1 [Rangasamy, Ezhiylmurugan; Sahu, Gayatri; Liang, Chengdu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Li, Juchuan; Dudney, Nancy] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Liang, CD (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM liangcn@ornl.gov RI Li, Juchuan/A-2992-2009 OI Li, Juchuan/0000-0002-6587-5591 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Division of Scientific User Facilities, U.S. DOE FX This work was sponsored by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The synthesis and characterization of materials were conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. DOE. NR 25 TC 16 Z9 16 U1 14 U2 93 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 14 PY 2014 VL 136 IS 19 BP 6874 EP 6877 DI 10.1021/ja5026358 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AH4EA UT WOS:000336078400025 PM 24730570 ER PT J AU Tan, GJ Zhao, LD Shi, FY Doak, JW Lo, SH Sun, H Wolverton, C Dravid, VP Uher, C Kanatzidis, MG AF Tan, Gangjian Zhao, Li-Dong Shi, Fengyuan Doak, Jeff W. Lo, Shih-Han Sun, Hui Wolverton, Chris Dravid, Vinayak P. Uher, Ctirad Kanatzidis, Mercouri G. TI High Thermoelectric Performance of p-Type SnTe via a Synergistic Band Engineering and Nanostructuring Approach SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID LATTICE THERMAL-CONDUCTIVITY; DENSITY-OF-STATES; BULK THERMOELECTRICS; HIGH FIGURE; PBTE; MERIT; PBS; ALLOYS; SEMICONDUCTOR; ENHANCEMENT AB SnTe is a potentially attractive thermoelectric because it is the lead-free rock-salt analogue of PbTe. However, SnTe is a poor thermoelectric material because of its high hole concentration arising from inherent Sn vacancies in the lattice and its very high electrical and thermal conductivity. In this study, we demonstrate that SnTe-based materials can be controlled to become excellent thermoelectrics for power generation via the successful application of several key concepts that obviate the well-known disadvantages of SnTe. First, we show that Sn self-compensation can effectively reduce the Sn vacancies and decrease the hole carrier density. For example, a 3 mol % self-compensation of Sn results in a 50% improvement in the figure of merit ZT. In addition, we reveal that Cd, nominally isoelectronic with Sn, favorably impacts the electronic band structure by (a) diminishing the energy separation between the light-hole and heavy-hole valence bands in the material, leading to an enhanced Seebeck coefficient, and (b) enlarging the energy band gap. Thus, alloying with Cd atoms enables a form of valence band engineering that improves the high-temperature thermoelectric performance, where p-type samples of SnCd0.03Te exhibit ZT values of similar to 0.96 at 823 K, a 60% improvement over the Cd-free sample. Finally, we introduce endotaxial CdS or ZnS nanoscale precipitates that reduce the lattice thermal conductivity of SnCd0.03Te with no effect on the power factor. We report that SnCd0.03Te that are endotaxially nanostructured with CdS and ZnS have a maximum ZTs of similar to 1.3 and similar to 1.1 at 873 K, respectively. Therefore, SnTe-based materials could be ideal alternatives for p-type lead chalcogenides for high temperature thermoelectric power generation. C1 [Tan, Gangjian; Zhao, Li-Dong; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Shi, Fengyuan; Doak, Jeff W.; Lo, Shih-Han; Wolverton, Chris; Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Sun, Hui; Uher, Ctirad] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Kanatzidis, Mercouri G.] Argonne Natl Lab, Mat Sci Div, Argonne, IL 60439 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM m-kanatzidis@northwestern.edu RI Wolverton, Christopher/B-7542-2009; Dravid, Vinayak/B-6688-2009; Tan, Gangjian/M-3509-2014; Doak, Jeff/P-1366-2014; Sun, Hui/D-3411-2014; Shi, Fengyuan/Q-2584-2015 OI Tan, Gangjian/0000-0002-9087-4048; Doak, Jeff/0000-0001-8576-7304; Sun, Hui/0000-0002-9745-3510; Shi, Fengyuan/0000-0001-9769-3824 FU Revolutionary Materials for Solid State Energy Conversion, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences [DE-SC0001054] FX This work was supported as part of the Revolutionary Materials for Solid State Energy Conversion, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences under Award Number DE-SC0001054. Transmission electron microscopy work was partially performed in the EPIC facility of the NUANCE Center at Northwestern University. NR 85 TC 80 Z9 81 U1 31 U2 270 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 14 PY 2014 VL 136 IS 19 BP 7006 EP 7017 DI 10.1021/ja500860m PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA AH4EA UT WOS:000336078400045 PM 24785377 ER PT J AU Lounis, SD Runnerstrom, EL Bergerud, A Nordlund, D Milliron, DJ AF Lounis, Sebastien D. Runnerstrom, Evan L. Bergerud, Amy Nordlund, Dennis Milliron, Delia J. TI Influence of Dopant Distribution on the Plasmonic Properties of Indium Tin Oxide Nanocrystals SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID DOPED SEMICONDUCTOR NANOCRYSTALS; TRANSPARENT CONDUCTING OXIDES; OPTICAL-PROPERTIES; ELECTRICAL-PROPERTIES; ZNO FILMS; NANOPARTICLES; SPECTROSCOPY; CHEMISTRY; RESONANCE; SCATTERING AB Doped metal oxide nanocrystals represent an exciting frontier for colloidal synthesis of plasmonic materials, displaying unique optoelectronic properties and showing promise for a variety of applications. However, fundamental questions about the nature of doping in these materials remain. In this article, the strong influence of radial dopant distribution on the optoelectronic properties of colloidal indium tin oxide nanocrystals is reported. Comparing elemental depth-profiling by X-ray photoelectron spectroscopy (XPS) with detailed modeling and simulation of the optical extinction of these nanocrystals using the Drude model for free electrons, a correlation between surface segregation of tin ions and the average activation of dopants is observed. A strong influence of surface segregation of tin on the line shape of the localized surface plasmon resonance (LSPR) is also reported. Samples with tin segregated near the surface show a symmetric line shape that suggests weak or no damping of the plasmon by ionized impurities. It is suggested that segregation of tin near the surface facilitates compensation of the dopant ions by electronic defects and oxygen interstitials, thus reducing activation. A core shell model is proposed to explain the observed differences in line shape. These results demonstrate the nuanced role of dopant distribution in determining the optoelectronic properties of semiconductor nanocrystals and suggest that more detailed study of the distribution and structure of defects in plasmonic colloidal nanocrystals is warranted. C1 [Lounis, Sebastien D.; Runnerstrom, Evan L.; Bergerud, Amy; Milliron, Delia J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Lounis, Sebastien D.] Univ Calif Berkeley, Grad Grp Appl Sci & Technol, Berkeley, CA 94720 USA. [Runnerstrom, Evan L.; Bergerud, Amy] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Nordlund, Dennis] Stanford Synchrotron Radiat Lightsource, Stanford, CA 94309 USA. [Milliron, Delia J.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. RP Milliron, DJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM milliron@che.utexas.edu RI Milliron, Delia/D-6002-2012; Nordlund, Dennis/A-8902-2008; Foundry, Molecular/G-9968-2014 OI Nordlund, Dennis/0000-0001-9524-6908; FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; DOE [DE-AC02-76SF00515]; DOE Early Career Research Program grant; DOE ARPA-E grant; National Science Foundation Graduate Student Research Fellowship [DGE 1106400] FX The authors acknowledge A. M. Sawvel and T. C. Weng for useful discussions regarding synchrotron data. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231. Use of the SSRL, SLAC National Accelerator Laboratory, is supported by DOE under Contract No. DE-AC02-76SF00515. S.D.L. and D.J.M. were supported by a DOE Early Career Research Program grant. E.L.R was supported by a DOE ARPA-E grant. A.B. was supported by a National Science Foundation Graduate Student Research Fellowship under Grant No. DGE 1106400. NR 47 TC 36 Z9 36 U1 10 U2 116 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 14 PY 2014 VL 136 IS 19 BP 7110 EP 7116 DI 10.1021/ja502541z PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA AH4EA UT WOS:000336078400056 PM 24786283 ER PT J AU Shan, SY Petkov, V Yang, LF Luo, J Joseph, P Mayzel, D Prasai, B Wang, LY Engelhard, M Zhong, CJ AF Shan, Shiyao Petkov, Valeri Yang, Lefu Luo, Jin Joseph, Pharrah Mayzel, Dina Prasai, Binay Wang, Lingyan Engelhard, Mark Zhong, Chuan-Jian TI Atomic-Structural Synergy for Catalytic CO Oxidation over Palladium-Nickel Nanoalloys SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OXYGEN REDUCTION ELECTROCATALYSTS; SOLVENT-FREE OXIDATION; ETHANOL FUEL-CELLS; ALLOY NANOPARTICLES; METHANE COMBUSTION; PD; GOLD; NI; CU; NANOSTRUCTURE AB Alloying palladium (Pd) with other transition metals at the nanoscale has become an important pathway for preparation of low-cost, highly active and stable catalysts. However, the lack of understanding of how the alloying phase state, chemical composition and atomic-scale structure of the alloys at the nanoscale influence their catalytic activity impedes the rational design of Pd-nanoalloy catalysts. This work addresses this challenge by a novel approach to investigating the catalytic oxidation of carbon monoxide (CO) over palladium nickel (PdNi) nanoalloys with well-defined bimetallic composition, which reveals a remarkable maximal catalytic activity at Pd:Ni ratio of similar to 50:50. Key to understanding the structural-catalytic synergy is the use of high-energy synchrotron X-ray diffraction coupled to atomic pair distribution function (HE-XRD/PDF) analysis to probe the atomic structure of PdNi nanoalloys under controlled thermochemical treatments and CO reaction conditions. Three-dimensional (3D) models of the atomic structure of the nanoalloy particles were generated by reverse Monte Carlo simulations (RMC) guided by the experimental HE-XRD/PDF data. Structural details of the PdNi nanoalloys were extracted from the respective 3D models and compared with the measured catalytic properties. The comparison revealed a strong correlation between the phase state, chemical composition and atomic-scale structure of PdNi nanoalloys and their catalytic activity for CO oxidation. This correlation is further substantiated by analyzing the first atomic neighbor distances and coordination numbers inside the nanoalloy particles and at their surfaces. These findings have provided new insights into the structural synergy of nanoalloy catalysts by controlling the phase state, composition and atomic structure, complementing findings of traditional density functional theory studies. C1 [Shan, Shiyao; Yang, Lefu; Luo, Jin; Joseph, Pharrah; Mayzel, Dina; Wang, Lingyan; Zhong, Chuan-Jian] SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA. [Petkov, Valeri; Prasai, Binay] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Yang, Lefu] Xiamen Univ, Coll Chem & Chem Engn, Xiamen 361005, Peoples R China. [Engelhard, Mark] Pacific NW Natl Lab, EMSL, Richland, WA 99352 USA. RP Zhong, CJ (reprint author), SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA. EM cjzhong@binghamton.edu RI Zhong, Chuan-Jian/D-3394-2013; OI Engelhard, Mark/0000-0002-5543-0812 FU DOE-BES [DE-SC0006877]; DOE [AC02-06CH11357]; DOE's Office of Biological and Environmental Research FX This work was supported by the DOE-BES Grants DE-SC0006877. Work at the Advanced Photon Source was supported by DOE under Contract DE-AC02-06CH11357. Thanks are also due to 11ID beamlines staff for the help with the HE-XRD experiments. The XPS analysis was performed using EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. NR 48 TC 34 Z9 34 U1 18 U2 225 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 14 PY 2014 VL 136 IS 19 BP 7140 EP 7151 DI 10.1021/ja5026744 PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA AH4EA UT WOS:000336078400059 PM 24794852 ER PT J AU Kim, JB Weichman, ML Neumark, DM AF Kim, Jongjin B. Weichman, Marissa L. Neumark, Daniel M. TI Structural Isomers of Ti2O4 and Zr2O4 Anions Identified by Slow Photoelectron Velocity-Map Imaging Spectroscopy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL-OXIDE CLUSTERS; EFFECTIVE CORE POTENTIALS; TITANIUM OXYGEN CLUSTERS; NM SINGLE-PHOTON; GAS-PHASE; ELECTRONIC-STRUCTURE; NEGATIVE-IONS; VIBRATIONAL SPECTROSCOPY; MOLECULAR-STRUCTURES; (TIO2)(N) N=1-4 AB High-resolution anion photoelectron spectra are reported for the group 4 metal dioxide clusters Ti2O4- and Zr2O4-. Slow photoelectron velocity-map imaging (SEVI) spectroscopy of cryogenically cooled, mass-selected anions yields photoelectron spectra with submillielectronvolt resolution, revealing extensive and well-resolved vibrational progressions. By comparison of the spectra with Franck-Condon Ti2O4- and Zr2O4- anions, respectively. Minor contributions from the C-2h isomer of Ti2O4- and the C-2v isomer of Zr2O4- are also seen. The SEVI spectra yield upper bounds for the adiabatic detachment energies, as well as vibrational frequencies for various modes of the neutral Ti2O4 and Zr2O4 species. C1 [Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu OI Weichman, Marissa/0000-0002-2551-9146 FU Air Force Office of Scientific Research [FA9550-12-1-0160]; Defense University Research Instrumentation Program [FA9550-11-1-0330]; National Science Foundation FX This work was funded by the Air Force Office of Scientific Research under Grant FA9550-12-1-0160 and the Defense University Research Instrumentation Program under Grant FA9550-11-1-0330. M.L.W. thanks the National Science Foundation for a graduate research fellowship. NR 64 TC 14 Z9 14 U1 4 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 14 PY 2014 VL 136 IS 19 BP 7159 EP 7168 DI 10.1021/ja502713v PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA AH4EA UT WOS:000336078400061 PM 24794915 ER PT J AU Furukawa, Y Fang, X Kogerler, P AF Furukawa, Y. Fang, X. Koegerler, P. TI Spin dynamics of the giant polyoxometalate molecule {Mn40W224} studied by NMR SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE NMR; molecular magnet; spin dynamics ID MAGNETIZATION; CLUSTER AB Li-7 nuclear magnetic resonance (NMR) studies have been performed to investigate magnetic properties and spin dynamics of Mn3+ (S = 2) spins in the giant polyoxometalate molecule {Mn40W224}. The Li-7-NMR line width is proportional to the external magnetic field H as expected in a paramagnetic state above 3 K. Below this temperature the line width shows a sudden increase and is almost independent of H, which indicates freezing of the local Mn3+ spins. The temperature dependence of T-1 for both H-1 and Li-7 reveals slow spin dynamics at low temperatures, consistent with spin freezing. The slow spin dynamics is also evidenced by the observation of a peak of 1/T-2 around 3 K, where the fluctuation frequency of spins is of the order of similar to 200 kHz. An explicit form of the temperature dependence of the fluctuation frequency of Mn3+ spins is derived from the nuclear relaxation data. C1 [Furukawa, Y.; Fang, X.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Furukawa, Y.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Koegerler, P.] Rhein Westfal TH Aachen, Inst Inorgan Chem, D-52074 Aachen, Germany. RP Furukawa, Y (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM furukawa@ameslab.gov RI Kogerler, Paul/H-5866-2013 OI Kogerler, Paul/0000-0001-7831-3953 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; US Department of Energy by Iowa State University [DE-AC02-07CH11358] FX This research was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 30 TC 0 Z9 0 U1 1 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 14 PY 2014 VL 26 IS 19 AR 196003 DI 10.1088/0953-8984/26/19/196003 PG 6 WC Physics, Condensed Matter SC Physics GA AH0QK UT WOS:000335825000010 PM 24762855 ER PT J AU Carnelli, PFF Almaraz-Calderon, S Rehm, KE Albers, M Alcorta, M Bertone, PF Digiovine, B Esbensen, H Niello, JOF Henderson, D Jiang, CL Lai, J Marley, ST Nusair, O Palchan-Hazan, T Pardo, RC Paul, M Ugalde, C AF Carnelli, P. F. F. Almaraz-Calderon, S. Rehm, K. E. Albers, M. Alcorta, M. Bertone, P. F. Digiovine, B. Esbensen, H. Fernandez Niello, J. O. Henderson, D. Jiang, C. L. Lai, J. Marley, S. T. Nusair, O. Palchan-Hazan, T. Pardo, R. C. Paul, M. Ugalde, C. TI Measurements of Fusion Reactions of Low-Intensity Radioactive Carbon Beams on C-12 and their Implications for the Understanding of X-Ray Bursts SO PHYSICAL REVIEW LETTERS LA English DT Article ID RELATIVISTIC HEAVY-IONS; ENERGIES; CHAMBER; NUCLEI; STARS AB The interaction between neutron-rich nuclei plays an important role for understanding the reaction mechanism of the fusion process as well as for the energy production through pycnonuclear reactions in the crust of neutron stars. We have performed the first measurements of the total fusion cross sections in the systems C-10,C-14,C-15 + C-12 using a new active target-detector system. In the energy region accessible with existing radioactive beams, a good agreement between the experimental and theoretical cross sections is observed. This gives confidence in our ability to calculate fusion cross sections for systems which are outside the range of today's radioactive beam facilities. C1 [Carnelli, P. F. F.; Almaraz-Calderon, S.; Rehm, K. E.; Albers, M.; Alcorta, M.; Bertone, P. F.; Digiovine, B.; Esbensen, H.; Henderson, D.; Jiang, C. L.; Marley, S. T.; Nusair, O.; Palchan-Hazan, T.; Pardo, R. C.; Ugalde, C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Carnelli, P. F. F.; Fernandez Niello, J. O.] Comis Nacl Energia Atom, Lab Tandar, San Martin, Buenos Aires, Argentina. [Carnelli, P. F. F.] Consejo Nacl Invest Cient & Tecn, Buenos Aires, DF, Argentina. [Fernandez Niello, J. O.] Univ San Martin, Escuela Ciencia & Tecnol, San Martin, Buenos Aires, Argentina. [Lai, J.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Paul, M.] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. RP Carnelli, PFF (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RI Alcorta, Martin/G-7107-2011 OI Alcorta, Martin/0000-0002-6217-5004 FU U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Argentina; Universidad Nacional de San Martin [SJ10/39] FX We want to thank S. Umar for providing us with the TDHF cross sections in tabulated form. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics under Contract No. DE-AC02-06CH11357, the Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Argentina, and the Universidad Nacional de San Martin Grant No. SJ10/39. NR 26 TC 13 Z9 13 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 14 PY 2014 VL 112 IS 19 AR 192701 DI 10.1103/PhysRevLett.112.192701 PG 5 WC Physics, Multidisciplinary SC Physics GA AH2CR UT WOS:000335928800009 PM 24877935 ER PT J AU Lu, XC Murayama, H Ruderman, JT Tobioka, K AF Lu, Xiaochuan Murayama, Hitoshi Ruderman, Joshua T. Tobioka, Kohsaku TI Natural Higgs Mass in Supersymmetry from Nondecoupling Effects SO PHYSICAL REVIEW LETTERS LA English DT Article ID STANDARD MODEL; BOSON; COUPLINGS; BREAKING; SECTOR; MSSM; LHC AB The Higgs mass implies fine-tuning for minimal theories of weak-scale supersymmetry (SUSY). Nondecoupling effects can boost the Higgs mass when new states interact with the Higgs boson, but new sources of SUSY breaking that accompany such extensions threaten naturalness. We show that two singlets with a Dirac mass can increase the Higgs mass while maintaining naturalness in the presence of large SUSY breaking in the singlet sector. We explore the modified Higgs phenomenology of this scenario, which we call the "Dirac next-to-minimal supersymmetric standard model." C1 [Lu, Xiaochuan; Murayama, Hitoshi; Ruderman, Joshua T.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lu, Xiaochuan; Murayama, Hitoshi; Ruderman, Joshua T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Murayama, Hitoshi; Tobioka, Kohsaku] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Tobioka, Kohsaku] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. RP Lu, XC (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM luxiaochuan123456@berkeley.edu; hitoshi@berkeley.edu; ruderman@berkeley.edu; tobioka@post.kek.jp FU U.S. DOE [DEAC03-76SF00098]; NSF [PHY-1002399]; JSPS [23540289]; FIRST program Subaru Measurements of Images and Redshifts (SuMIRe); CSTP; WPI; Miller Institute for Basic Research in Science; JSPS Fellows; MEXT, Japan FX We thank Lawrence Hall, Matthew McCullough, Satyanarayan Mukhopadhyay, Tilman Plehn, Filippo Sala, Satoshi Shirai, and Neal Weiner for helpful discussions. We especially thank Yasunori Nomura for discussions and for pointing out that the Dirac mass can be thought of as a new type of portal. The work of H. M. was supported in part by the U.S. DOE under Contract No. DEAC03-76SF00098, by the NSF under Grant No. PHY-1002399, by the JSPS Grant (C) No. 23540289, by the FIRST program Subaru Measurements of Images and Redshifts (SuMIRe), CSTP, and by WPI, MEXT, Japan. J.T.R. is supported by a fellowship from the Miller Institute for Basic Research in Science. The work of K.T. is supported in part by the Grantin-Aid for JSPS Fellows. NR 54 TC 19 Z9 19 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 14 PY 2014 VL 112 IS 19 AR 191803 DI 10.1103/PhysRevLett.112.191803 PG 5 WC Physics, Multidisciplinary SC Physics GA AH2CR UT WOS:000335928800006 PM 24877931 ER PT J AU Salafranca, J Rincon, J Tornos, J Leon, C Santamaria, J Dagotto, E Pennycook, SJ Varela, M AF Salafranca, Juan Rincon, Julian Tornos, Javier Leon, Carlos Santamaria, Jacobo Dagotto, Elbio Pennycook, Stephen J. Varela, Maria TI Competition between Covalent Bonding and Charge Transfer at Complex-Oxide Interfaces SO PHYSICAL REVIEW LETTERS LA English DT Article ID SUPERCONDUCTING OXIDES; YBA2CU3O7-DELTA; SUPERLATTICES; LAYERS AB Here we study the electronic properties of cuprate-manganite interfaces. By means of atomic resolution electron microscopy and spectroscopy, we produce a subnanometer scale map of the transition metal oxidation state profile across the interface between the high Tc superconductor YBa2Cu3O7-delta and the colossal magnetoresistance compound (La,Ca)MnO3. A net transfer of electrons from manganite to cuprate with a peculiar nonmonotonic charge profile is observed. Model calculations rationalize the profile in terms of the competition between standard charge transfer tendencies (due to band mismatch), strong chemical bonding effects across the interface, and Cu substitution into the Mn lattice, with different characteristic length scales. C1 [Salafranca, Juan; Tornos, Javier; Leon, Carlos; Santamaria, Jacobo; Varela, Maria] Univ Complutense Madrid, Grp Fis Mat Complejos, E-28040 Madrid, Spain. [Salafranca, Juan; Rincon, Julian; Dagotto, Elbio; Varela, Maria] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Rincon, Julian] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Pennycook, Stephen J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Salafranca, J (reprint author), Univ Complutense Madrid, Grp Fis Mat Complejos, E-28040 Madrid, Spain. EM jsalafra@ucm.es RI Varela, Maria/H-2648-2012; Leon, Carlos/A-5587-2008; Varela, Maria/E-2472-2014; Santamaria, Jacobo/N-8783-2016 OI Leon, Carlos/0000-0002-3262-1843; Varela, Maria/0000-0002-6582-7004; Santamaria, Jacobo/0000-0003-4594-2686 FU U.S. Department of Energy (DOE); Basic Energy Sciences (BES); Materials Sciences and Engineering Division; Materials Sciences and Engineering Division through the Center for Nanophase Materials Sciences (CNMS); Scientific User Facilities Division; DOE-BES; ERC starting Investigator Award [239739 STEMOX]; Juan de la Cierva program (MICINN-Spain) [JCI-2011-09428]; Spanish MICINN/MINECO [MAT2011-27470-C02]; Consolider Ingenio (Imagine) [CSD2009-00013]; CAM (PHAMA) [S2009/MAT-1756]; National Center for Supercomputing Applications (U. S. Department of Energy) [DEAC02-05CH11231] FX The authors thank Luis Brey for helpful discussions and Masashi Watanabe for the principal component analysis plug-in for Digital Micrograph. Research at ORNL (S.J.P., M.V., E.D., and J.R.) was supported by the U.S. Department of Energy (DOE), Basic Energy Sciences (BES), Materials Sciences and Engineering Division, and through the Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division, DOE-BES. J. Sal. was supported by the ERC starting Investigator Award, Grant No. 239739 STEMOX and Juan de la Cierva program JCI-2011-09428 (MICINN-Spain). Research at UCM (J.T., C.L., J. San.) was supported by the Spanish MICINN/MINECO through Grants No. MAT2011-27470-C02 and Consolider Ingenio 2010 -CSD2009-00013 (Imagine), and by CAM through Grant No. S2009/MAT-1756 (PHAMA). Computations were supported by the National Center for Supercomputing Applications (U. S. Department of Energy, Contract No. DEAC02-05CH11231). NR 37 TC 12 Z9 12 U1 1 U2 61 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 14 PY 2014 VL 112 IS 19 DI 10.1103/PhysRevLett.112.196802 PG 6 WC Physics, Multidisciplinary SC Physics GA AH2CR UT WOS:000335928800020 PM 24877959 ER PT J AU Shukla, N Parihar, A Freeman, E Paik, H Stone, G Narayanan, V Wen, H Cai, Z Gopalan, V Engel-Herbert, R Schlom, DG Raychowdhury, A Datta, S AF Shukla, Nikhil Parihar, Abhinav Freeman, Eugene Paik, Hanjong Stone, Greg Narayanan, Vijaykrishnan Wen, Haidan Cai, Zhonghou Gopalan, Venkatraman Engel-Herbert, Roman Schlom, Darrell G. Raychowdhury, Arijit Datta, Suman TI Synchronized charge oscillations in correlated electron systems SO SCIENTIFIC REPORTS LA English DT Article ID METAL-INSULATOR-TRANSITION; COUPLED OSCILLATORS; CIRCADIAN-RHYTHMS; MOTT TRANSITION; BAND THEORY; VO2; MODEL; MECHANISM; PEIERLS; HUBBARD AB Strongly correlated phases exhibit collective carrier dynamics that if properly harnessed can enable novel functionalities and applications. In this article, we investigate the phenomenon of electrical oscillations in a prototypical MIT system, vanadium dioxide (VO2). We show that the key to such oscillatory behaviour is the ability to induce and stabilize a non-hysteretic and spontaneously reversible phase transition using a negative feedback mechanism. Further, we investigate the synchronization and coupling dynamics of such VO2 based relaxation oscillators and show, via experiment and simulation, that this coupled oscillator system exhibits rich non-linear dynamics including charge oscillations that are synchronized in both frequency and phase. Our approach of harnessing a non-hysteretic reversible phase transition region is applicable to other correlated systems exhibiting metal-insulator transitions and can be a potential candidate for oscillator based non-Boolean computing. C1 [Shukla, Nikhil; Freeman, Eugene; Datta, Suman] Penn State Univ, Dept Elect Engn, University Pk, PA 16802 USA. [Parihar, Abhinav; Raychowdhury, Arijit] Georgia Inst Technol, Sch Elect & Comp Engn, Atlanta, GA 30332 USA. [Paik, Hanjong; Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Stone, Greg; Gopalan, Venkatraman; Engel-Herbert, Roman] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Narayanan, Vijaykrishnan] Penn State Univ, Dept Comp Sci & Engn, University Pk, PA 16802 USA. [Cai, Zhonghou] Argonne Natl Lab, Argonne, IL 60439 USA. [Schlom, Darrell G.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Datta, S (reprint author), Penn State Univ, Dept Elect Engn, University Pk, PA 16802 USA. EM sdatta@engr.psu.edu OI Parihar, Abhinav/0000-0001-8203-5888 FU Office of Naval Research [N00014-11-1-0665]; Intel Corporation; National Science Foundation [DMR-0820404]; National Science Foundation Expeditions in Computing [1317560]; U. S Department of Energy [DE-AC02-06CH1135] FX This work was supported by Office of Naval Research through award N00014-11-1-0665. AP was partially funded by a gift from Intel Corporation. G.S. received partial support from the National Science Foundation award DMR-0820404. SD and VN acknowledge funding, in part, from the National Science Foundation Expeditions in Computing Award-1317560. Work at Argonne National Laboratory was supported by the U.S Department of Energy, under Contract No. DE-AC02-06CH1135. NR 41 TC 31 Z9 31 U1 6 U2 55 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 14 PY 2014 VL 4 AR 4964 DI 10.1038/srep04964 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH0LY UT WOS:000335812600001 ER PT J AU Sava Gallis, DF Rohwer, LES Rodriguez, MA Nenoff, TM AF Sava Gallis, Dorina F. Rohwer, Lauren E. S. Rodriguez, Mark A. Nenoff, Tina M. TI Efficient Photoluminescence via Metal-Ligand Alteration in a New MOFs Family SO CHEMISTRY OF MATERIALS LA English DT Article ID WHITE-LIGHT EMISSION; ORGANIC FRAMEWORKS; COORDINATION POLYMERS; PHOSPHORS AB Here, we introduce a family of metal-organic frameworks (MOFs) whose photoluminescence is tunable through metal and organic ligand substitutions. The compounds in this family are composed of In, In-Eu, or Eu metal centers and organic ligand chromophores. Systematic variations in the metal and organic components resulted in materials with emissions ranging from white to red. The single-component white-light emitter material is made of In, 4,4',4"-s-triazine-2,4,6-triyl-tribenzoic acid (TTB) and oxalic acid. Red-emitting MOFs composed of Eu metal centers and TTB ligands have a room temperature quantum yield (QY) of 50% and a 48% QY at 150 degrees C due to reversible thermal quenching. This is the highest quantum yield measured at elevated temperatures reported for this class of materials. The materials are thermally stable, retaining their high QY after heating at 150 degrees C for several hours. These thermal quenching/stability studies show the potential use of MOFs in devices that operate at elevated temperatures, such as white-light-emitting diodes for solid-state lighting. This is a unique study that correlates the QY, thermal quenching, and thermal stability of MOFs with structural properties. C1 [Sava Gallis, Dorina F.; Nenoff, Tina M.] Sandia Natl Labs, Nanoscale Sci Dept, Albuquerque, NM 87185 USA. [Rohwer, Lauren E. S.] Sandia Natl Labs, Microsyst Integrat Dept, Albuquerque, NM 87185 USA. [Rodriguez, Mark A.] Sandia Natl Labs, Mat Characterizat Dept, Albuquerque, NM 87185 USA. RP Nenoff, TM (reprint author), Sandia Natl Labs, Nanoscale Sci Dept, POB 5800, Albuquerque, NM 87185 USA. EM tmnenof@sandia.gov RI Sava Gallis, Dorina/D-2827-2015 FU US DOE/NE/FCRD-SWG; US DOE's NNSA [DE-AC04-94AL85000]; US DOE [DE-AC02-06CH11357] FX This work was supported by the US DOE/NE/FCRD-SWG. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corp., a wholly owned subsidiary of Lockheed Martin Corporation, for the US DOE's NNSA under contract DE-AC04-94AL85000. We also would like to acknowledge Gregory J. Halder, from the Advanced Photon Source, Argonne National Laboratory for help with collecting synchrotron data on compound 1. Work done at Argonne and the use of the Advanced Photon Source, an Office of Science User Facility operated for the US DOE/Office of Science by Argonne National Laboratory, was supported by the US DOE, Contract No. DE-AC02-06CH11357. NR 36 TC 34 Z9 34 U1 9 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 13 PY 2014 VL 26 IS 9 BP 2943 EP 2951 DI 10.1021/cm500700z PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JY UT WOS:000336020700024 ER PT J AU Uppugundla, N Sousa, LD Chundawat, SPS Yu, XR Simmons, B Singh, S Gao, XD Kumar, R Wyman, CE Dale, BE Balan, V AF Uppugundla, Nirmal Sousa, Leonardo da Costa Chundawat, Shishir P. S. Yu, Xiurong Simmons, Blake Singh, Seema Gao, Xiadi Kumar, Rajeev Wyman, Charles E. Dale, Bruce E. Balan, Venkatesh TI A comparative study of ethanol production using dilute acid, ionic liquid and AFEX (TM) pretreated corn stover SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE AFEX; Dilute acid; Ionic liquid; Pretreatment; Enzymatic hydrolysis; Cellulosic ethanol ID AMMONIA FIBER EXPANSION; LIGNOCELLULOSIC BIOMASS; ENZYMATIC-HYDROLYSIS; CELL-WALL; BETA-GLUCOSIDASE; FERMENTATION; CELLULOSE; INHIBITION; TECHNOLOGIES; SWITCHGRASS AB Background: In a biorefinery producing cellulosic biofuels, biomass pretreatment will significantly influence the efficacy of enzymatic hydrolysis and microbial fermentation. Comparison of different biomass pretreatment techniques by studying the impact of pretreatment on downstream operations at industrially relevant conditions and performing comprehensive mass balances will help focus attention on necessary process improvements, and thereby help reduce the cost of biofuel production. Results: An on-going collaboration between the three US Department of Energy (DOE) funded bioenergy research centers (Great Lakes Bioenergy Research Center (GLBRC), Joint BioEnergy Institute (JBEI) and BioEnergy Science Center (BESC)) has given us a unique opportunity to compare the performance of three pretreatment processes, notably dilute acid (DA), ionic liquid (IL) and ammonia fiber expansion (AFEXTM), using the same source of corn stover. Separate hydrolysis and fermentation (SHF) was carried out using various combinations of commercially available enzymes and engineered yeast (Saccharomyces cerevisiae 424A) strain. The optimal commercial enzyme combination (Ctec2: Htec2: Multifect Pectinase, percentage total protein loading basis) was evaluated for each pretreatment with a microplate-based assay using milled pretreated solids at 0.2% glucan loading and 15 mg total protein loading/g of glucan. The best enzyme combinations were 67:33:0 for DA, 39:33:28 for IL and 67:17:17 for AFEX. The amounts of sugar (kg) (glucose: xylose: total gluco-and xylo-oligomers) per 100 kg of untreated corn stover produced after 72 hours of 6% glucan loading enzymatic hydrolysis were: DA (25:2:2), IL (31:15:2) and AFEX (26: 13: 7). Additionally, the amounts of ethanol (kg) produced per 100 kg of untreated corn stover and the respective ethanol metabolic yield (%) achieved with exogenous nutrient supplemented fermentations were: DA (14.0, 92.0%), IL (21.2, 93.0%) and AFEX (20.5, 95.0%), respectively. The reason for lower ethanol yield for DA is because most of the xylose produced during the pretreatment was removed and not converted to ethanol during fermentation. Conclusions: Compositional analysis of the pretreated biomass solids showed no significant change in composition for AFEX treated corn stover, while about 85% of hemicellulose was solubilized after DA pretreatment, and about 90% of lignin was removed after IL pretreatment. As expected, the optimal commercial enzyme combination was different for the solids prepared by different pretreatment technologies. Due to loss of nutrients during the pretreatment and washing steps, DA and IL pretreated hydrolysates required exogenous nutrient supplementation to ferment glucose and xylose efficiently, while AFEX pretreated hydrolysate did not require nutrient supplementation. C1 [Uppugundla, Nirmal; Sousa, Leonardo da Costa; Chundawat, Shishir P. S.; Dale, Bruce E.; Balan, Venkatesh] Michigan State Univ, Great Lakes Bioenergy Res Ctr, US DOE, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Chundawat, Shishir P. S.] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, US DOE, Dept Biochem, Madison, WI 53706 USA. [Yu, Xiurong] Jilin TuoPai Agr Prod Dev Ltd, Jilin, Jilin, Peoples R China. [Simmons, Blake; Singh, Seema] Joint BioEnergy Inst JBEI, Deconstruct Div, Emeryville, CA 94608 USA. [Simmons, Blake; Singh, Seema] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA 94550 USA. [Gao, Xiadi; Kumar, Rajeev; Wyman, Charles E.] Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, Oak Ridge, TN 37831 USA. [Gao, Xiadi; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Dept Chem & Environm Engn, Riverside, CA 92507 USA. [Gao, Xiadi; Kumar, Rajeev; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol CE CERT, Riverside, CA 92507 USA. RP Balan, V (reprint author), Michigan State Univ, Great Lakes Bioenergy Res Ctr, US DOE, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. EM balan@msu.edu RI da Costa Sousa, Leonardo/A-1536-2016 FU Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BESC at Oak Ridge National Laboratory [DE-PS02-06ER64304]; Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through GLBRC [DE-FC02-07ER64494]; Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through JBEI [DE-AC02-05CH11231] FX We gratefully acknowledge funding support for this research by the Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BESC at Oak Ridge National Laboratory (contract DE-PS02-06ER64304), GLBRC (grant DE-FC02-07ER64494), and JBEI (grant DE-AC02-05CH11231). We would like to thank Professor Nancy Ho at Purdue University (West Lafayette, IN, USA) for providing the 424A yeast strain. We thank Novozymes and DuPont Industrial Biosciences for supplying commercial enzymes for this collaborative work. Also, we thank Charles Donald, Margaret Magyar, Christa Gunawan, Rebecca Garlock, Mingjie Jin and James Humpula (Biomass Conversion Research Laboratory, MSU, Lansing, MI, USA) for additional laboratory assistance. MBI International (Lansing, MI, USA) kindly provided access to their 5 gallon batch reactor for AFEX pretreatment. AFEXTM is a trademark of MBI International. NR 44 TC 45 Z9 46 U1 11 U2 81 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAY 13 PY 2014 VL 7 AR 72 DI 10.1186/1754-6834-7-72 PG 14 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AK4DR UT WOS:000338374700001 PM 24917886 ER PT J AU Gao, XD Kumar, R Singh, S Simmons, BA Balan, V Dale, BE Wyman, CE AF Gao, Xiadi Kumar, Rajeev Singh, Seema Simmons, Blake A. Balan, Venkatesh Dale, Bruce E. Wyman, Charles E. TI Comparison of enzymatic reactivity of corn stover solids prepared by dilute acid, AFEX (TM), and ionic liquid pretreatments SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Corn stover; Enzyme adsorption; Cellulase; Oligomers; Pretreatment; Hydrolysis ID AMMONIA FREEZE-EXPLOSION; CELLULOSE ACCESSIBILITY; STEAM EXPLOSION; LIGNOCELLULOSIC BIOMASS; LEADING TECHNOLOGIES; CELLOBIOHYDROLASE-I; LIGNIN REMOVAL; PINUS-RADIATA; HYDROLYSIS; ADSORPTION AB Background: Pretreatment is essential to realize high product yields from biological conversion of naturally recalcitrant cellulosic biomass, with thermochemical pretreatments often favored for cost and performance. In this study, enzymatic digestion of solids from dilute sulfuric acid (DA), ammonia fiber expansion (AFEX (TM)), and ionic liquid (IL) thermochemical pretreatments of corn stover were followed over time for the same range of total enzyme protein loadings to provide comparative data on glucose and xylose yields of monomers and oligomers from the pretreated solids. The composition of pretreated solids and enzyme adsorption on each substrate were also measured to determine. The extent glucose release could be related to these features. Results: Corn stover solids from pretreatment by DA, AFEX, and IL were enzymatically digested over a range of low to moderate loadings of commercial cellulase, xylanase, and pectinase enzyme mixtures, the proportions of which had been previously optimized for each pretreatment. Avicel (R) cellulose, regenerated amorphous cellulose (RAC), and beechwood xylan were also subjected to enzymatic hydrolysis as controls. Yields of glucose and xylose and their oligomers were followed for times up to 120 hours, and enzyme adsorption was measured. IL pretreated corn stover displayed the highest initial glucose yields at all enzyme loadings and the highest final yield for a low enzyme loading of 3 mg protein/g glucan in the raw material. However, increasing the enzyme loading to 12 mg/g glucan or more resulted in DA pretreated corn stover attaining the highest longer-term glucose yields. Hydrolyzate from AFEX pretreated corn stover had the highest proportion of xylooligomers, while IL produced the most glucooligomers. However, the amounts of both oligomers dropped with increasing enzyme loadings and hydrolysis times. IL pretreated corn stover had the highest enzyme adsorption capacity. Conclusions: Initial hydrolysis yields were highest for substrates with greater lignin removal, a greater degree of change in cellulose crystallinity, and high enzyme accessibility. Final glucose yields could not be clearly related to concentrations of xylooligomers released from xylan during hydrolysis. Overall, none of these factors could completely account for differences in enzymatic digestion performance of solids produced by AFEX, DA, and IL pretreatments. C1 [Gao, Xiadi; Kumar, Rajeev; Wyman, Charles E.] Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, Oak Ridge, TN 37831 USA. [Gao, Xiadi; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Dept Chem & Environm Engn, Riverside, CA 92521 USA. [Gao, Xiadi; Kumar, Rajeev; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol CE CERT, Riverside, CA 92507 USA. [Singh, Seema; Simmons, Blake A.] Joint BioEnergy Inst JBEI, Deconstruct Div, Emeryville, CA 94608 USA. [Singh, Seema; Simmons, Blake A.] Sandia Natl Labs, Livermore, CA 94551 USA. [Balan, Venkatesh; Dale, Bruce E.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr GLBRC, E Lansing, MI 48824 USA. [Balan, Venkatesh; Dale, Bruce E.] Michigan State Univ, Dept Chem Engn & Mat Sci, Biomass Convers Res Lab, Lansing, MI 48910 USA. RP Wyman, CE (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, Oak Ridge, TN 37831 USA. EM cewyman@engr.ucr.edu FU Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BESC at Oak Ridge National Laboratory [DE-PS02-06ER64304]; GLBRC [DE-FC02-07ER64494]; JBEI [DE-AC02-05CH11231]; Ford Motor Company FX We gratefully acknowledge support for this research by the Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BESC at Oak Ridge National Laboratory (contract DE-PS02-06ER64304), GLBRC (grant DE-FC02-07ER64494), and JBEI (grant DE-AC02-05CH11231). We are also grateful to the Center for Environmental Research and Technology of the Bourns College of Engineering (CE-CERT) at UCR for providing key equipment and facilities. We thank Mr. Charles Donald Jr for preparing AFEX pretreated corn stover for this project and Nirmal Uppugundla for having optimized the commercial enzyme formulations for the three different pretreated solids. We also thank Novozymes and DuPont Genencor Science for providing enzymes for this research. The corresponding author is particularly grateful to the Ford Motor Company for funding the Chair in Environmental Engineering at the CE-CERT at UCR that augments support for many projects such as this. NR 63 TC 25 Z9 25 U1 6 U2 76 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAY 13 PY 2014 VL 7 AR 71 DI 10.1186/1754-6834-7-71 PG 13 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AI4RQ UT WOS:000336852900001 PM 24910713 ER PT J AU Skandarajah, A Reber, CD Switz, NA Fletcher, DA AF Skandarajah, Arunan Reber, Clay D. Switz, Neil A. Fletcher, Daniel A. TI Quantitative Imaging with a Mobile Phone Microscope SO PLOS ONE LA English DT Article ID PROCESSING PIPELINE; REAL-TIME; DIAGNOSIS; BANDWIDTH; SYSTEM; RESOLUTION; PATHOLOGY; ACCURACY; CAMERAS; IMAGES AB Use of optical imaging for medical and scientific applications requires accurate quantification of features such as object size, color, and brightness. High pixel density cameras available on modern mobile phones have made photography simple and convenient for consumer applications; however, the camera hardware and software that enables this simplicity can present a barrier to accurate quantification of image data. This issue is exacerbated by automated settings, proprietary image processing algorithms, rapid phone evolution, and the diversity of manufacturers. If mobile phone cameras are to live up to their potential to increase access to healthcare in low-resource settings, limitations of mobile phone-based imaging must be fully understood and addressed with procedures that minimize their effects on image quantification. Here we focus on microscopic optical imaging using a custom mobile phone microscope that is compatible with phones from multiple manufacturers. We demonstrate that quantitative microscopy with micron-scale spatial resolution can be carried out with multiple phones and that image linearity, distortion, and color can be corrected as needed. Using all versions of the iPhone and a selection of Android phones released between 2007 and 2012, we show that phones with greater than 5 MP are capable of nearly diffraction-limited resolution over a broad range of magnifications, including those relevant for single cell imaging. We find that automatic focus, exposure, and color gain standard on mobile phones can degrade image resolution and reduce accuracy of color capture if uncorrected, and we devise procedures to avoid these barriers to quantitative imaging. By accommodating the differences between mobile phone cameras and the scientific cameras, mobile phone microscopes can be reliably used to increase access to quantitative imaging for a variety of medical and scientific applications. C1 [Skandarajah, Arunan; Reber, Clay D.; Fletcher, Daniel A.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Switz, Neil A.; Fletcher, Daniel A.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Fletcher, Daniel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Fletcher, DA (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. EM fletch@berkeley.edu FU Microsoft Research, Intel Corporation; Bill and Melinda Gates Foundation; Blum Center at UC Berkeley; NSF Graduate Research Fellowship; NAS through an NSF IGERT FX This work was supported by grants from Microsoft Research, Intel Corporation, the Bill and Melinda Gates Foundation, and the Blum Center at UC Berkeley. AS has been funded by the NSF Graduate Research Fellowship, and NAS has been supported through an NSF IGERT grant to the UC Berkeley Biophysics Group. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 45 TC 37 Z9 37 U1 10 U2 41 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 13 PY 2014 VL 9 IS 5 AR e96906 DI 10.1371/journal.pone.0096906 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH8EY UT WOS:000336369200040 PM 24824072 ER PT J AU Berges, J Boguslavski, K Schlichting, S Venugopalan, R AF Berges, J. Boguslavski, K. Schlichting, S. Venugopalan, R. TI Basin of attraction for turbulent thermalization and the range of validity of classical-statistical simulations SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Heavy Ion Phenomenology; Phenomenological Models ID COLOR GLASS CONDENSATE; INFLATION; LATTICE; FIELDS; DECAY AB Different thermalization scenarios for systems with large fields have been proposed in the literature based on classical-statistical lattice simulations approximating the underlying quantum dynamics. We investigate the range of validity of these simulations for condensate driven as well as fluctuation dominated initial conditions for the example of a single component scalar field theory. We show that they lead to the same phenomenon of turbulent thermalization for the whole range of (weak) couplings where the classical-statistical approach is valid. In the turbulent regime we establish the existence of a dual cascade characterized by universal scaling exponents and scaling functions. This complements previous investigations where only the direct energy cascade has been studied for the single component theory. A proposed alternative thermalization scenario for stronger couplings is shown to be beyond the range of validity of classical-statistical simulations. C1 [Berges, J.; Boguslavski, K.] Heidelberg Univ, Inst Theoret Phys, D-69120 Heidelberg, Germany. [Berges, J.] GSI Helmholtzzentrum Schwerionenforsch GmbH, ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Schlichting, S.; Venugopalan, R.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Berges, J (reprint author), Heidelberg Univ, Inst Theoret Phys, Philosophenweg 16, D-69120 Heidelberg, Germany. EM j.berges@thphys.uni-heidelberg.de; k.boguslavski@thphys.uni-heidelberg.de; sschlichting@bnl.gov; raju@bnl.gov FU German Research Foundation (DFG); US Department of Energy under DOE [DE-AC02-98CH10886]; Ministry for Education and Research (BMBF); Ministry for Science, Research and Arts Baden-Wuerttemberg (MWK-BW) FX We thank Thomas Epelbaum and Francois Gelis for providing us with their lattice data to make detailed comparisons possible. We also thank Daniil Gelfand, Larry McLerran and Denes Sexty for helpful discussions and suggestions. This work was supported in part by the German Research Foundation (DFG). S.S and R.V. are supported by US Department of Energy under DOE Contract No. DE-AC02-98CH10886. The numerical results presented in this work were obtained on the bwGRiD (http://www.bw-grid.de), member of the German D-Grid initiative, funded by the Ministry for Education and Research (BMBF) and the Ministry for Science, Research and Arts Baden-Wuerttemberg (MWK-BW). NR 53 TC 18 Z9 18 U1 1 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 13 PY 2014 IS 5 AR 054 DI 10.1007/JHEP05(2014)054 PG 23 WC Physics, Particles & Fields SC Physics GA AH8GW UT WOS:000336376000001 ER PT J AU Bielska, AA Olsen, BN Gale, SE Mydock-McGrane, L Krishnan, K Baker, NA Schlesinger, PH Covey, DF Ory, DS AF Bielska, Agata A. Olsen, Brett N. Gale, Sarah E. Mydock-McGrane, Laurel Krishnan, Kathiresan Baker, Nathan A. Schlesinger, Paul H. Covey, Douglas F. Ory, Daniel S. TI Side-Chain Oxysterols Modulate Cholesterol Accessibility through Membrane Remodeling SO BIOCHEMISTRY LA English DT Article ID ENDOPLASMIC-RETICULUM; PHOSPHOLIPID-MEMBRANES; MOLECULAR SIMULATION; LXR-ALPHA; IN-VITRO; HOMEOSTASIS; LY295427; BINDING; CELL; PROTEIN AB Side-chain oxysterols, such as 25-hydroxycholesterol (25-HC), are key regulators of cholesterol homeostasis. New evidence suggests that the alteration of membrane structure by 25-HC contributes to its regulatory effects. We have examined the role of oxysterol membrane effects on :a cholesterol accessibility within the membrane using perfringolysin O (PFO), a cholesterol-dependent cytolysin that g selectively binds accessible cholesterol, as a sensor of membrane cholesterol accessibility. We show that 25-HC increases cholesterol accessibility in a manner dependent on the membrane lipid composition. Structural analysis of molecular dynamics simulations reveals that increased cholesterol accessibility is associated with membrane thinning, and that the effects of 25-HC on cholesterol accessibility are driven by these changes in membrane thickness. Further, we find that the 25-HC antagonist LY295427 (agisterol) abrogates the membrane effects of 25-HC in a nonenantioselective manner, suggesting that agisterol antagonizes the cholesterol-homeostatic effects of 25-HC indirectly through its membrane interactions. These studies demonstrate that oxysterols regulate cholesterol accessibility, and thus the availability of cholesterol to be sensed and transported throughout the cell, by modulating the membrane environment. This work provides new insights into how alterations in membrane structure can be used to relay cholesterol regulatory signals. C1 [Bielska, Agata A.; Olsen, Brett N.; Gale, Sarah E.; Ory, Daniel S.] Washington Univ, Sch Med, Diabet Cardiovasc Dis Ctr, St Louis, MO 63110 USA. [Mydock-McGrane, Laurel; Krishnan, Kathiresan; Covey, Douglas F.] Washington Univ, Sch Med, Dept Dev Biol, St Louis, MO 63110 USA. [Mydock-McGrane, Laurel; Krishnan, Kathiresan; Covey, Douglas F.] Washington Univ, Sch Med, Dept Psychiat, St Louis, MO 63110 USA. [Mydock-McGrane, Laurel; Krishnan, Kathiresan; Covey, Douglas F.] Washington Univ, Sch Med, Dept Anesthesiol, St Louis, MO 63110 USA. [Baker, Nathan A.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Schlesinger, Paul H.] Washington Univ, Sch Med, Dept Cell Biol & Physiol, St Louis, MO 63110 USA. RP Ory, DS (reprint author), Washington Univ, Sch Med, Diabet Cardiovasc Dis Ctr, BJC Inst Hlth Bldg, Suite 10618, St Louis, MO 63110 USA. EM dory@wustl.edu RI Baker, Nathan/A-8605-2010 OI Baker, Nathan/0000-0002-5892-6506 FU National Institutes of Health (NIH) [F30 HL97563]; Cardiovascular Biology Training Grant [T32HL007275]; NIH [HL067773]; Texas Advanced Computing Center through Teragrid [TG-MCB060053, TG-MCA08X003]; National Biomedical Computation Resource (NIH) [P41 RR0860516]; National Science Foundation [OCI-1053575] FX This work was supported by National Institutes of Health (NIH) Grant F30 HL97563 to A.A.B., Cardiovascular Biology Training Grant T32HL007275 to A.A.B. and B.N.O., and NIH Grant HL067773 to D.S.O., D.F.C., P.H.S., and N.A.B. Computational resources were provided by the Texas Advanced Computing Center through Teragrid Grants TG-MCB060053 and TG-MCA08X003 as well as the National Biomedical Computation Resource (NIH Grant P41 RR0860516). This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant OCI-1053575. NR 48 TC 5 Z9 6 U1 0 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 13 PY 2014 VL 53 IS 18 BP 3042 EP 3051 DI 10.1021/bi5000096 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AH3JR UT WOS:000336020000017 PM 24758724 ER PT J AU Kawasaki, H Kumar, S Li, G Zeng, CJ Kauffman, DR Yoshimoto, J Iwasaki, Y Jin, RC AF Kawasaki, Hideya Kumar, Santosh Li, Gao Zeng, Chenjie Kauffman, Douglas R. Yoshimoto, Junya Iwasaki, Yasuhiko Jin, Rongchao TI Generation of Singlet Oxygen by Photoexcited Au-25(SR)(18) Clusters SO CHEMISTRY OF MATERIALS LA English DT Article ID KDA GOLD CLUSTERS; PHOTODYNAMIC THERAPY; QUANTUM DOTS; MOLECULAR-OXYGEN; AU-25 CLUSTERS; OPTICAL-PROPERTIES; CRYSTAL-STRUCTURE; ELECTRON-TRANSFER; NANOCLUSTERS; NANOPARTICLES AB The generation of highly reactive singlet oxygen (O-1(2)) is of major importance for a variety of applications such as photodynamic therapy (PDT) for cancer treatment water treatment catalytic oxidation and others. Herein we demonstrate that O-1(2) can be efficiently produced through the direct photosensitization by Au-25(SR)(18)(-) clusters (H-SR = phenylethanethiol or captopril) without using conventional organic photosensitizers under visible/near-IR (532,650, and 808 nm) irradiation. O-1(2) was successfully detected by direct observation of the characteristic O-1(2) emission around 1276 nm as well as three different O-1(2)-selective probes. Water-soluble Au-25(captopril)(18)(-)clusters were explored for cytocompatibility and photodynamic activity toward cancer cells. In addition selective catalytic oxidation of organic sulfide to sulfoxide by O-1(2) was demonstrated on the photoexcited Au-25(SC2H4Ph)(18)(-)clusters. It is suggested that the optical gap of Au-25(SR)(18) clusters (similar to 1.3 eV) being larger than the energy of O-1(2)(0.97 eV) allows for the eficient energy transfer to O-3(2). In addition the long lifetime of the electronic excited states of Au-25(SR)(18) and the well-defined O-2 adsorption sites are the key factors that promote energy transfer from Au-25(SR)(18)(-) to molecular oxygen thus facilitating the formation of O-1(2). Finally neutral Au-25(SR)(18)(0) can also produce O-1(2) as efficiently as does the anionic Au-25(SR)(18)(-). C1 [Kawasaki, Hideya; Kumar, Santosh; Li, Gao; Zeng, Chenjie; Jin, Rongchao] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15213 USA. [Kawasaki, Hideya; Yoshimoto, Junya; Iwasaki, Yasuhiko] Kansai Univ, Fac Chem Mat & Bioengn, Dept Chem & Mat Engn, Suita, Osaka 5648680, Japan. [Kauffman, Douglas R.] US DOE, NETL, Pittsburgh, PA 15236 USA. RP Kawasaki, H (reprint author), Carnegie Mellon Univ, Dept Chem, 4400 5th Ave, Pittsburgh, PA 15213 USA. EM hkawa@kansai-u.ac.jp; rongchao@andrew.cmu.edu RI Iwasaki, Yasuhiko/D-6870-2011; OI Kauffman, Douglas/0000-0002-7855-3428 FU Kansai University's Overseas Research Program; Japan Society for the Promotion of Science (JSPS) [23360361, 23655074, 22350040]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-12ER16354]; MEXT, Japan [24107524] FX This research was partly supported by Kansai University's Overseas Research Program for 2012 and by Grants-in-Aid for Scientific Research (nos: 23360361, 23655074, and 22350040) from the Japan Society for the Promotion of Science (JSPS) (to H.K.). R.J. thanks support from the U.S. Department of Energy, Office of Basic Energy Sciences, grant no. DE-FG02-12ER16354. Y.I. thanks MEXT, Japan for a Grant-in-Aid for Scientific Research on Innovative Areas "Nanomedicine Molecular Science" (no. 24107524). NR 102 TC 43 Z9 43 U1 10 U2 121 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 13 PY 2014 VL 26 IS 9 BP 2777 EP 2788 DI 10.1021/cm500260z PG 12 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JY UT WOS:000336020700005 ER PT J AU Atkins, R Dolgos, M Fiedler, A Grosse, C Fischer, SF Rudin, SP Johnson, DC AF Atkins, Ryan Dolgos, Michelle Fiedler, Andreas Grosse, Corinna Fischer, Saskia F. Rudin, Sven P. Johnson, David C. TI Synthesis and Systematic Trends in Structure and Electrical Properties of [(SnSe)(1.15)](m) (VSe2)(1), m=1, 2, 3, and 4 SO CHEMISTRY OF MATERIALS LA English DT Article ID CHARGE-DENSITY-WAVE; TRANSITION-METAL DICHALCOGENIDES; SNSE SINGLE-CRYSTALS; TRANSPORT-PROPERTIES; MAGNETIC-PROPERTIES; MOS2 TRANSISTORS; LAYER COMPOUNDS; FILMS; SELENIDE; 1T-VSE2 AB Four compounds [(SnSe)(1.15)],(VSe2)(1) where m = 1-4, were synthesized to explore the effect of increasing the distance between Se-V-Se dichalcogenide layers on electrical transport properties. These kinetically stable compounds were prepared using designed precursors that contained a repeating pattern of elemental layers with the nanoarchitecture of the desired product. XRD and STEM data revealed that the precursors self-assembled into the desired compounds containing a Se-V-Se dichalcogenide layer precisely separated by a SnSe layer. The 001 diffraction data are used to determine the position of the Sn, Se, and V planes along the c-axis, confirming that the average structure is similar to that observed in the STEM images, and the resulting data agrees well with results obtained from calculations based on density functional theory and a semiempirical description of van der Waals interactions. The in-plane diffraction data contains reflections that can be indexed as hk0 reflections coming from the two independent constituents. The SnSe layers diffract independently from one another and are distorted from the bulk structure to lower the surface free energy. All of the samples showed metallic-like behavior in temperature-dependent resistivity between room temperature and about 150 K. The electrical resistivity systematically increases as m increases. Below 150 K the transport data strongly indicates a charge density wave transition whose onset temperature systematically increases as m increases. This suggests increasing quasi-two-dimensional behavior as increasingly thick layers of SnSe separate the Se-V-Se layers. This is supported by electronic structure calculations. C1 [Atkins, Ryan; Johnson, David C.] Univ Oregon, Dept Chem, Eugene, OR 97403 USA. [Atkins, Ryan; Johnson, David C.] Univ Oregon, Inst Mat Sci, Eugene, OR 97403 USA. [Dolgos, Michelle] Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA. [Fiedler, Andreas; Grosse, Corinna; Fischer, Saskia F.] Humboldt Univ, D-12489 Berlin, Germany. [Rudin, Sven P.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Johnson, DC (reprint author), Univ Oregon, Dept Chem, Eugene, OR 97403 USA. EM davej@uoregon.edu FU National Science Foundation [DMR-1266217]; National Science Foundation through CCI [CHE-1102637]; U.S. Department of Energy, Office of Science; Office of Basic Energy Sciences [DE-AC02-06CH11357]; [MRI 0923577] FX The authors thank the staff in CAMCOR for assistance preparing TEM samples and collecting STEM images. The authors acknowledge support from the National Science Foundation under Grant DMR-1266217. Coauthors R.A. and M.D. acknowledge support from the National Science Foundation through CCI Grant CHE-1102637. Grant MRI 0923577 provided funding for the dual beam FIB used to make TEM cross sections. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, and the Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Coauthors A.F., C.G., and S.F.F. thank R. Mitdank for technical help and scientific discussion. NR 76 TC 12 Z9 12 U1 5 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 13 PY 2014 VL 26 IS 9 BP 2862 EP 2872 DI 10.1021/cm5004774 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JY UT WOS:000336020700015 ER PT J AU Ramasamy, K Sims, H Butler, WH Gupta, A AF Ramasamy, Karthik Sims, Hunter Butler, William H. Gupta, Arunava TI Selective Nanocrystal Synthesis and Calculated Electronic Structure of All Four Phases of Copper-Antimony-Sulfide SO CHEMISTRY OF MATERIALS LA English DT Article ID FILM SOLAR-CELLS; INITIO MOLECULAR-DYNAMICS; AUGMENTED-WAVE METHOD; TUNABLE BAND-GAP; SEMICONDUCTOR NANOCRYSTALS; CHALCOSTIBITE CUSBS2; ABSORBER MATERIALS; CRYSTAL-STRUCTURE; EFFICIENCY; SB AB A wide variety of copper-based semiconducting chalcogenides have been investigated in recent years to address the need for sustainable solar cell materials. An attractive class of materials consisting of nontoxic and earth abundant elements is the copper-antimony-sulfides. The copper-antimony- sulfide system consists of four major phases, namely, CuSbS2 (Chalcostibite), Cu12Sb4S13 (Tetrahedrite), Cu3SbS3 (Skinnerite), and Cu3SbS4 (Fematinite). All four phases are p-type semiconductors having energy band gaps between 0.5 and 2 eV, with reported large absorption coefficient values over 105 cm(-1). We have for the first time developed facile colloidal hot-injection methods for the phase-pure synthesis of nanocrystals of all four phases. Cu12Sb4S13 and Cu3SbS3 are found to have direct band gaps (1.6 and 1.4 eV, respectively), while the other two phases display indirect band gaps (1.1 and 1.2 eV for CuSbS2 and Cu3SbS4, respectively). The synthesis methods yield nanocrystals with distinct morphology for the different phases. CuSbS2 is synthesized as nanoplates, and Cu12Sb4S13 is isolated as hollow structures, while uniform spherical Cu3SbS3 and oblate spheroid nanocrystals of Cu3SbS4 are obtained. In order to understand the optical and electrical properties, we have calculated the electronic structures of all four phases using the hybrid functional method (HSE 06) and PBE generalized gradient approximation to density functional theory. Consistent with experimental results, the calculations indicate that CuSbS2 and Cu3SbS4 are indirect band gap materials but with somewhat higher band gap values of 1.6 and 2.5 eV, respectively. Similarly, Cu3SbS3 is determined to be a direct band gap material with a gap of 1.5 eV. Interestingly, both PBE and HSE06 methods predict metallic behavior in fully stoichiometric Cu12Sb4S13 phase, with opening up of bands leading to semiconducting or insulating behavior for off-stoichiometric compositions with a varying number of valence electrons. The absorption coefficient values at visible wavelengths for all the phases are estimated to range between 104 and 105 cm(-1), confirming their potential for solar energy conversion applications. C1 [Ramasamy, Karthik; Gupta, Arunava] Univ Alabama, Dept Chem, Tuscaloosa, AL 35487 USA. [Sims, Hunter; Butler, William H.] Univ Alabama, Dept Phys, Tuscaloosa, AL 35487 USA. [Ramasamy, Karthik; Sims, Hunter; Butler, William H.; Gupta, Arunava] Univ Alabama, Ctr Mat Informat Technol, Tuscaloosa, AL 35487 USA. RP Ramasamy, K (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. EM kramasamy@lanl.gov; agupta@mint.ua.edu OI Sims, Hunter/0000-0001-7631-2754 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-8ER46537] FX This research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Award No. DE-FG02-8ER46537. NR 50 TC 32 Z9 32 U1 9 U2 104 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 13 PY 2014 VL 26 IS 9 BP 2891 EP 2899 DI 10.1021/cm5005642 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JY UT WOS:000336020700018 ER PT J AU Liu, ZW Wang, HL Cotlet, M AF Liu, Zhongwei Wang, Hsing-Lin Cotlet, Mircea TI Energy Transfer from a Cationic Conjugated Polyelectrolyte to a DNA Photonic Wire: Toward Label-Free, Sequence-Specific DNA Sensing SO CHEMISTRY OF MATERIALS LA English DT Article ID DOUBLE-STRANDED DNA; MALACHITE GREEN; CYANINE DYE; OPTICAL-PROPERTIES; LINEAR DICHROISM; NUCLEIC-ACIDS; POLYMERS; COMPLEXES; PLATFORM; SENSORS AB We demonstrate a label-free, sequence specific DNA sensor based on fluorescence resonant energy transfer (FRET) occurring between a cationic conjugated polyelectrolyte and a small intercalating dye, malachite green chloride. The sensor combines (1) conjugated polymer chain conformation changes induced by the binding with DNA, with the conjugated polymer wrapping/twisting around the DNA helical duplex and experiencing a 3-fold increase in its photoluminescence quantum yield and (2) FRET from the conjugated polymer to the intercalated DNA. Owing to its small size, the dye intercalates at maximal, one-to-one dye-to-base pair load, making the intercalated DNA a molecular photonic wire with dyes excitonically coupled and chiroptically active. Any sequence mismatch between probe and target DNA degrades the intercalated DNA photonic wire by decreasing its brightness, excitonic coupling, and chiroptical properties, and this provides a signal transduction method for the DNA sensor. Coupling of intercalated DNA with the conjugated polymer via FRET provides target signal amplification and increased sensitivity toward sequence mismatch, with the FRET efficiency decreasing with added DNA sequence mismatch. C1 [Liu, Zhongwei; Cotlet, Mircea] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Liu, Zhongwei] SUNY Stony Brook, Mat Sci & Engn Dept, Stony Brook, NY 11794 USA. [Wang, Hsing-Lin] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. RP Wang, HL (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM hwang@lanl.gov; cotlet@bnl.gov RI Liu, Zhongwei/F-1327-2017 OI Liu, Zhongwei/0000-0002-2678-3125 FU U.S. Department of Energy, Office of Basic Energy Sciences; Biomaterials Program of the Division of Materials Science and Engineering of the Office of Basic Energy Sciences; [DE-AC02-98CH10886] FX Research carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory and supported by the U.S. Department of Energy, Office of Basic Energy Sciences, by Contract No. DE-AC02-98CH10886 (Z.L., M.C.) and by the Biomaterials Program of the Division of Materials Science and Engineering of the Office of Basic Energy Sciences (H.L.W.). NR 48 TC 11 Z9 11 U1 5 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 13 PY 2014 VL 26 IS 9 BP 2900 EP 2906 DI 10.1021/cm500592j PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JY UT WOS:000336020700019 ER PT J AU Gutierrez, A Qiao, RM Wang, LP Yang, WL Wang, F Manthiram, A AF Gutierrez, Arturo Qiao, Ruimin Wang, Liping Yang, Wanli Wang, Feng Manthiram, Arumugam TI High-Capacity, Aliovalently Doped Olivine LiMn(1-3x/2)Vx square x/2PO4 Cathodes without Carbon Coating SO CHEMISTRY OF MATERIALS LA English DT Article ID LITHIUM-ION BATTERIES; LIFEPO4 CATHODE; X-RAY; ELECTROCHEMICAL PERFORMANCES; CATION SUBSTITUTION; ELECTRODE MATERIALS; ABSORPTION-SPECTRA; SITE SUBSTITUTION; ROOM-TEMPERATURE; PHOSPHO-OLIVINES AB A substantial amount of Mn2+ has been aliovalently substituted by V3+ in cationdeficient LiMn1-3x/2Vx square x/2PO4 (0 <= x <= 0.20) by a low-temperature (<300 degrees C) microwave-assisted solvothermal (MW-ST) process. The necessity of a low-temperature synthesis to achieve higher levels of doping is demonstrated as the solubility of vanadium decreases with the formation of impurity phases on heating the samples to >= 575 degrees C. Soft X-ray absorption spectroscopy reveals enhanced Mn O hybridization in the vanadium-doped samples, which is believed to facilitate an increase in capacity with increasing vanadium content in the lattice. For example, a high capacity of 155 mAh/g is achieved above a cutoff voltage of 3 V without any carbon coating for the x = 0.2 sample. The vanadium substitution enhances the overall kinetics of the material by lowering the charge-transfer impedance and increasing the lithium-diffusion coefficient. C1 [Gutierrez, Arturo; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Qiao, Ruimin; Yang, Wanli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Wang, Liping; Wang, Feng] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. RP Manthiram, A (reprint author), Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. EM manth@austin.utexas.edu RI Qiao, Ruimin/E-9023-2013; Yang, Wanli/D-7183-2011; Wang, Feng/C-1443-2016 OI Yang, Wanli/0000-0003-0666-8063; Wang, Feng/0000-0003-4068-9212 FU Vehicle Technologies of the U.S. Department of Energy [DE-ACO205CH11231]; Welch Foundation [F-1254]; Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-ACO2-05CH11231]; DOE-EERE under the Batteries for Advanced Transportation Technologies (BATT) Program [DE-ACO2-98CH10886]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-ACO2-98CH10886] FX This work was supported by the office of Vehicle Technologies of the U.S. Department of Energy under Contract DE-ACO205CH11231 (BATT Program) and the Welch Foundation Grant F-1254. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-ACO2-05CH11231. The work by L.W. and F.W. was supported by DOE-EERE under the Batteries for Advanced Transportation Technologies (BATT) Program, under Contract No. DE-ACO2-98CH10886. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-ACO2-98CH10886. NR 51 TC 14 Z9 15 U1 1 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 13 PY 2014 VL 26 IS 9 BP 3018 EP 3026 DI 10.1021/cm500924n PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JY UT WOS:000336020700033 ER PT J AU Baxamusa, SH Stadermann, M Aracne-Ruddle, C Nelson, AJ Chea, M Li, SL Youngblood, K Suratwala, TI AF Baxamusa, Salmaan H. Stadermann, Michael Aracne-Ruddle, Chantel Nelson, Art J. Chea, Maverick Li, Shuali Youngblood, Kelly Suratwala, Tayyab I. TI Enhanced Delamination of Ultrathin Free-Standing Polymer Films via Self-Limiting Surface Modification SO LANGMUIR LA English DT Article ID SACRIFICIAL LAYERS; THIN-FILMS; MEMBRANES; MULTILAYERS; MONOLAYERS; ADHESION AB Free-standing polymer thin films are typically fabricated using a sacrificial underlayer (between the film and its deposition substrate) or overlayer (on top of the film to assist peeling) in order to facilitate removal of the thin film from its deposition substrate. We show the direct delamination of extraordinarily thin (as thin as 8 nm) films of poly(vinyl formal) (PVF), polystyrene, and poly(methyl methacrylate). Large (up to 13 cm diameter) films of PVF could be captured on wire supports to produce free-standing films. By modifying the substrate to lower the interfacial energy resisting film substrate separation, the conditions for spontaneous delamination are satisfied even for very thin films. The substrate modification is based on the electrostatic adsorption of a cationic polyelectrolyte. Eliminating the use of sacrificial materials and instead relying on naturally self-limiting adsorption makes this method suitable for large areas. We have observed delamination of films with aspect ratios (ratio of lateral dimension between supports to thickness) of 10(7) and have captured dry, free-standing films with aspect ratios >10(6). Films with an aspect ratio of 10(5) can bear loads up to 10(6) times the mass of the film itself. The presence of the adsorbed layer can be observed using X-ray photoelectron spectroscopy, and this layer is persistent through multiple uses. In the system studied, elimination of sacrificial materials leads to an enhancement in the failure strength of the freestanding thin film. The robustness, persistence, and the self-optimizing nature distinguish this method from various fabrication methods utilizing sacrificial materials and make it a potentially scalable process for the fabrication of ultrathin free-standing or transferrable films for filtration, MEMS, or tissue engineering applications. C1 [Baxamusa, Salmaan H.; Stadermann, Michael; Aracne-Ruddle, Chantel; Nelson, Art J.; Chea, Maverick; Li, Shuali; Youngblood, Kelly; Suratwala, Tayyab I.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Baxamusa, SH (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM baxamusa1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Authors gratefully acknowledge Kedar Shah for providing 15 cm silicon substrates. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 47 TC 9 Z9 9 U1 8 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 13 PY 2014 VL 30 IS 18 BP 5126 EP 5132 DI 10.1021/la5011665 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JZ UT WOS:000336020800011 PM 24784173 ER PT J AU Ewing, CS Bhavsar, S Veser, G McCarthy, JJ Johnson, JK AF Ewing, Christopher S. Bhavsar, Saurabh Veser, Goetz McCarthy, Joseph J. Johnson, J. Karl TI Accurate Amorphous Silica Surface Models from First-Principles Thermodynamics of Surface Dehydroxylation SO LANGMUIR LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; PERIODIC B3LYP CALCULATIONS; LANGMUIR-BLODGETT-FILMS; GAMMA-ALUMINA SURFACES; AB-INITIO; FORCE-FIELD; HYDROXYLATED SURFACES; WATER; DENSITY; SPECTROSCOPY AB Accurate atomically detailed models of amorphous materials have been elusive to-date due to limitations in both experimental data and computational methods. We present an approach for constructing atomistic models of amorphous silica surfaces encountered in many industrial applications (such as catalytic support materials). We have used a combination of classical molecular modeling and density functional theory calculations to develop models having predictive capabilities. Our approach provides accurate surface models for a range of temperatures as measured by the thermodynamics of surface dehydroxylation. We find that a surprisingly small model of an amorphous silica surface can accurately represent the physics and chemistry of real surfaces as demonstrated by direct experimental validation using macroscopic measurements of the silanol number and type as a function of temperature. Beyond accurately predicting the experimentally observed trends in silanol numbers and types, the model also allows new insights into the dehydroxylation of amorphous silica surfaces. Our formalism is transferrable and provides an approach to generating accurate models of other amorphous materials. C1 [Ewing, Christopher S.; Bhavsar, Saurabh; Veser, Goetz; McCarthy, Joseph J.; Johnson, J. Karl] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. [Ewing, Christopher S.; Veser, Goetz] Univ Pittsburgh, Mascaro Ctr Sustainable Innovat, Pittsburgh, PA 15261 USA. [Bhavsar, Saurabh; Veser, Goetz; Johnson, J. Karl] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Johnson, JK (reprint author), Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. EM karlj@pitt.edu RI McCarthy, Joseph/K-6925-2012; Johnson, Karl/E-9733-2013 OI McCarthy, Joseph/0000-0002-2841-3128; Johnson, Karl/0000-0002-3608-8003 FU Department of Education GAANN program [P200A100087]; Mascaro Center for Sustainable Innovation at the University of Pittsburgh FX This work was supported by the Department of Education GAANN program (P200A100087) and the Mascaro Center for Sustainable Innovation at the University of Pittsburgh. Calculations were performed at the University of Pittsburgh Center for Simulation and Modeling. NR 60 TC 19 Z9 19 U1 10 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 13 PY 2014 VL 30 IS 18 BP 5133 EP 5141 DI 10.1021/la500422p PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AH3JZ UT WOS:000336020800012 PM 24793021 ER PT J AU Priftis, D Xia, XX Margossian, KO Perry, SL Leon, L Qin, J de Pablo, JJ Tirrell, M AF Priftis, Dimitrios Xia, Xiaoxing Margossian, Khatcher O. Perry, Sarah L. Leon, Lorraine Qin, Jian de Pablo, Juan J. Tirrell, Matthew TI Ternary, Tunable Polyelectrolyte Complex Fluids Driven by Complex Coacervation SO MACROMOLECULES LA English DT Article ID ELECTROSTATIC FREE-ENERGY; BOVINE SERUM-ALBUMIN; RHEOLOGICAL PROPERTIES; MULTILAYER FILMS; GENE DELIVERY; SYSTEMS; POLYPEPTIDE; MECHANISM; EXCHANGE; CHITOSAN AB Complex coacervation was achieved by combining poly(allylamine) (PAR) or branched poly(ethylenimine) (PEI) with poly(acrylic acid) (PAA) and poly(N,N-dimethylaminoethyl methacrylate) (PDMAEMA). We systematically investigated the effects of stoichiometry, salt concentration, and pH. Ternary coacervates formed over a broader range of stoichiometries compared to the base PAA/PDMAEMA system. An enhanced resistance to salt, that is, resistance to dissolution of the complex with added salt, was observed for ternary coacervates. PEI-containing systems showed a considerable difference in salt resistance at pH 6-8 due to the dramatic change in charge density. This change was interpreted in the context of a theoretical treatment that relies on the Voorn-Overbeek model for free energy. Coacervate stability and viscoelastic behavior were affected by stoichiometry, salt, and pH. Ternary coacervates maintain the characteristics and tunability of typical binary coacervates, but the choice of the third component is important, as it significantly affects the response and material properties. C1 [Priftis, Dimitrios; Xia, Xiaoxing; Margossian, Khatcher O.; Perry, Sarah L.; Leon, Lorraine; Qin, Jian; de Pablo, Juan J.; Tirrell, Matthew] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Leon, Lorraine] Argonne Natl Lab, Inst Mol Engn, Argonne, IL 60439 USA. RP Priftis, D (reprint author), Univ Chicago, Inst Mol Engn, 5735 South Ellis Ave, Chicago, IL 60637 USA. EM dpriftis@uchicago.edu OI Perry, Sarah/0000-0003-2301-6710 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and a Engineering Division FX The authors thank Anna Tropnikova and Patrick McCall for their help with the rheological measurements. This work also benefited from discussions with Dr. Matthew Kade, Dr. Jonathan Whitmer, and Kyle Hoffmann. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and a Engineering Division. NR 50 TC 25 Z9 25 U1 11 U2 88 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 13 PY 2014 VL 47 IS 9 BP 3076 EP 3085 DI 10.1021/ma500245j PG 10 WC Polymer Science SC Polymer Science GA AH3KA UT WOS:000336020900036 ER PT J AU Cao, Z Stevens, MJ Dobrynin, AV AF Cao, Zhen Stevens, Mark J. Dobrynin, Andrey V. TI Adhesion and Wetting of Nanoparticles on Soft Surfaces SO MACROMOLECULES LA English DT Article ID MOLECULAR-DYNAMICS; CELL-ADHESION; CONTACT MECHANICS; ELASTIC SOLIDS; FORCE; PARTICLES AB We study adhesion of spherical and cylindrical nanoparticles on soft (gel-like) substrates using a combination of the molecular dynamics simulations and theoretical calculations. The substrate deformation is obtained as a function of the gel shear modulus, nanoparticle size, surface tension of nanoparticles and substrate, and work of adhesion. It was shown recently that the classical JKR model can only be applied to describe nanoparticle adhesion on relatively stiff substrates. In this so-called adhesion regime the deformation of the substrate is determined by balancing the elastic energy of indentation and the work of adhesion between a nanoparticle and a gel. However, in the case of soft gels when substrates undergo moderate deformations the depth of the indentation produced by a nanoparticle is determined by the surface tension of the gel and the work of adhesion (the wetting regime). We present an analytical model describing crossover between adhesion and wetting regimes. In the framework of this model a crossover between different interaction regimes is controlled by a dimensionless parameter gamma(s)(GR(p))W--2/3(-1/3), where gamma(s) and G are the surface tension and shear modulus of the gel, W is the work of adhesion between gel and nanoparticle, and R-p is the nanoparticle radius. Nanoparticle adhesion regime corresponds to small values of this parameter, gamma(s)(GR(p))W--2/3(-1/3) << 1, while the wetting regime takes place at gamma(s)(GR(p))W--2/3(-1/3) >> 1. We applied our model to obtain work of adhesion between silicon substrates and silica microspheres and to obtain surface tension of silicon gels from particle indentation experiments. C1 [Cao, Zhen; Dobrynin, Andrey V.] Univ Connecticut, Inst Mat Sci, Polyrner Program, Storrs, CT 06269 USA. [Cao, Zhen; Dobrynin, Andrey V.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Stevens, Mark J.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Dobrynin, AV (reprint author), Univ Connecticut, Inst Mat Sci, Polyrner Program, Storrs, CT 06269 USA. EM avd@ims.uconn.edu OI Dobrynin, Andrey/0000-0002-6484-7409 FU National Science Foundation [DMR-1004576]; U.S. Department of Energy, Center for Integrated Nanotechnologies, at Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy [DE-AC04-94AL85000] FX The authors thank Prof. Eric Dufresne and Dr. Robert Style for providing original experimental data sets. This work was supported by the National Science Foundation under Grant DMR-1004576. This work was performed at the U.S. Department of Energy, Center for Integrated Nanotechnologies, at Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94AL85000. NR 40 TC 25 Z9 25 U1 6 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 13 PY 2014 VL 47 IS 9 BP 3203 EP 3209 DI 10.1021/ma500317q PG 7 WC Polymer Science SC Polymer Science GA AH3KA UT WOS:000336020900050 ER PT J AU Agrawal, A Aryal, D Perahia, D Ge, T Grest, GS AF Agrawal, Anupriya Aryal, Dipak Perahia, Dvora Ge, Ting Grest, Gary S. TI Coarse-Graining Atactic Polystyrene and Its Analogues SO MACROMOLECULES LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; POLYMER MELTS; ATOMISTIC SIMULATIONS; MODELS; POTENTIALS; SYSTEMS; LIQUID; BACK AB Capturing large length scales in polymers and soft matter while retaining atomistic properties is imperative to computational studies of dynamic systems. Here we present the results for a coarse-grained model based on atomistic simulation of atactic polystyrene (PS). Similar to previous work by Harmandaris et al. and Fritz et al., each monomer is described by two coarse-grained beads. In contrast to these early studies in which intramolecular potentials were based on Monte Carlo simulations of isotactic and syndiotactic single PS molecules to capture stereochemistry, we obtained intramolecular interactions from a single molecular dynamics simulation of an all-atom atactic PS melt. The nonbonded interactions are obtained using the iterative Boltzmann inversion (IBI) scheme. This methodology has been extended to coarse graining of poly(4-tert-butylstyrene) (PtBS) in which an additional type of coarse-grained bead is used describe the tert-butyl group. Similar to the process for PS, the intramolecular interactions are obtained from a single all-atom melt simulation for atactic PtBS. C1 [Agrawal, Anupriya; Aryal, Dipak; Perahia, Dvora] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. [Ge, Ting] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Perahia, D (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA. EM dperahi@g.clemson.edu RI Agrawal, Anupriya/E-9051-2011 FU DOE [DE-FG02-12ER46843]; NSF [DMR-1006805]; National Science Foundation [NSF PHY11-25915]; Office of Science of the United States Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Kurt Kremer for helpful discussions and gratefully acknowledge financial support from DOE Grant No. DE-FG02-12ER46843 and NSF Grant No. DMR-1006805. This research was supported in part by the National Science Foundation under Grant No. NSF PHY11-25915. This research used resources at the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the United States Department of Energy, under Contract No. DE-AC02-05CH11231. This work was made possible by advanced computational resources deployed and maintained by Clemson Computing and Information Technology. This work was performed, in part, at the Center for Integrated Nanotechnology, a U.S. Department of Energy and Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 51 TC 2 Z9 2 U1 2 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 13 PY 2014 VL 47 IS 9 BP 3210 EP 3218 DI 10.1021/ma500319v PG 9 WC Polymer Science SC Polymer Science GA AH3KA UT WOS:000336020900051 ER PT J AU Tucker, GS Fernandes, RM Pratt, DK Thaler, A Ni, N Marty, K Christianson, AD Lumsden, MD Sales, BC Sefat, AS Bud'ko, SL Canfield, PC Kreyssig, A Goldman, AI McQueeney, RJ AF Tucker, G. S. Fernandes, R. M. Pratt, D. K. Thaler, A. Ni, N. Marty, K. Christianson, A. D. Lumsden, M. D. Sales, B. C. Sefat, A. S. Bud'ko, S. L. Canfield, P. C. Kreyssig, A. Goldman, A. I. McQueeney, R. J. TI Crossover from spin waves to diffusive spin excitations in underdoped Ba(Fe1-xCox)(2)As-2 SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY AB Using inelastic neutron scattering, we show that the onset of superconductivity in underdoped Ba(Fe1-x Co-x) As-2(2) coincides with a crossover from well-defined spin waves to overdamped and diffusive spin excitations. This crossover occurs despite the presence of long-range stripe antiferromagnetic order for samples in a compositional range from x = 0.04 to 0.055, and is a consequence of the shrinking spin-density wave gap and a corresponding increase in the particle-hole (Landau) damping. The latter effect is captured by a simple itinerant model relating Co doping to changes in the hot spots of the Fermi surface. We argue that the overdamped spin fluctuations provide a pairing mechanism for superconductivity in these materials. C1 [Tucker, G. S.; Pratt, D. K.; Thaler, A.; Ni, N.; Bud'ko, S. L.; Canfield, P. C.; Kreyssig, A.; Goldman, A. I.; McQueeney, R. J.] US DOE, Ames Lab, Ames, IA 50011 USA. [Tucker, G. S.; Pratt, D. K.; Thaler, A.; Ni, N.; Bud'ko, S. L.; Canfield, P. C.; Kreyssig, A.; Goldman, A. I.; McQueeney, R. J.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Fernandes, R. M.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Marty, K.; Christianson, A. D.; Lumsden, M. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Sales, B. C.; Sefat, A. S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Tucker, GS (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. RI Canfield, Paul/H-2698-2014; Fernandes, Rafael/E-9273-2010; Thaler, Alexander/J-5741-2014; Tucker, Gregory/L-9357-2013; McQueeney, Robert/A-2864-2016; christianson, andrew/A-3277-2016; Sefat, Athena/R-5457-2016; Lumsden, Mark/F-5366-2012 OI Thaler, Alexander/0000-0001-5066-8904; Tucker, Gregory/0000-0002-2787-8054; McQueeney, Robert/0000-0003-0718-5602; christianson, andrew/0000-0003-3369-5884; Sefat, Athena/0000-0002-5596-3504; Lumsden, Mark/0000-0002-5472-9660 FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; US Department of Energy by Iowa State University [DE-AC02-07CH11358] FX This work was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. A major part of the research was performed at the Ames Laboratory, which is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Neutron scattering was carried out at the High Flux Isotope Reactor at the Oak Ridge National Laboratory, operated for the US Department of Energy by UT-Battelle, LLC. NR 41 TC 6 Z9 6 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 13 PY 2014 VL 89 IS 18 AR 180503 DI 10.1103/PhysRevB.89.180503 PG 5 WC Physics, Condensed Matter SC Physics GA AH0RC UT WOS:000335826900001 ER PT J AU Gursoy, U Kharzeev, D Rajagopal, K AF Gursoy, Umut Kharzeev, Dmitri Rajagopal, Krishna TI Magnetohydrodynamics, charged currents, and directed flow in heavy ion collisions SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR COLLISIONS; BARYON; PP AB The hot QCD matter produced in any heavy ion collision with a nonzero impact parameter is produced within a strong magnetic field. We study the imprint that these fields leave on the azimuthal distributions and correlations of the produced charged hadrons. The magnetic field is time dependent and the medium is expanding, which leads to the induction of charged currents owing to the combination of Faraday and Hall effects. We find that these currents result in a charge-dependent directed flow v(1) that is odd in rapidity and odd under charge exchange. It can be detected by measuring correlations between the directed flow of charged hadrons at different rapidities, < v(1)(+/-)(y(1))v(1)(+/-)(y(2))>. C1 [Gursoy, Umut] Univ Utrecht, Inst Theoret Phys, NL-3584 CE Utrecht, Netherlands. [Kharzeev, Dmitri] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kharzeev, Dmitri] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Rajagopal, Krishna] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. RP Gursoy, U (reprint author), Univ Utrecht, Inst Theoret Phys, Leuvenlaan 4, NL-3584 CE Utrecht, Netherlands. FU US Department of Energy [DE-FG-88ER40388, DE-AC02-98CH10886, DE-FG0205ER41360]; Dutch Ministry of Education, Culture and Science (OCW) FX We are grateful to Sergei Voloshin for helpful suggestions. U.G. and K.R. are grateful to the CERN Theory division for hospitality at the time this research began. The work of D.K. was supported in part by the US Department of Energy under Contracts No. DE-FG-88ER40388 and No. DE-AC02-98CH10886. The work of K.R. was supported by the US Department of Energy under cooperative research Agreement No. DE-FG0205ER41360. This work is part of the D-ITP consortium, a program of the Netherlands Organisation for Scientific Research (NWO) that is funded by the Dutch Ministry of Education, Culture and Science (OCW). NR 42 TC 48 Z9 48 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. 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CA CDF Collaboration TI Study of top quark production and decays involving a tau lepton at CDF and limits on a charged Higgs boson contribution SO PHYSICAL REVIEW D LA English DT Article ID DETECTOR; SEARCH AB We present an analysis of top-antitop quark production and decay into a tau lepton, tau neutrino, and bottom quark using data from 9 fb(-1) of integrated luminosity at the Collider Detector at Fermilab. Dilepton events, where one lepton is an energetic electron or muon and the other a hadronically decaying tau lepton, originating from proton-antiproton collisions at root s = 1.96 TeV, are used. A top-antitop quark production cross section of 8.1 +/- 2.1 pb is measured, assuming standard-model top quark decays. By separately identifying for the first time the single-tau and the ditau components, we measure the branching fraction of C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Nodulman, L.; Wicklund, A. 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RP Aaltonen, T (reprint author), Ctr Invest Energet Medioambient & Tecnol, E-28040 Madrid, Spain. RI song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Martinez, Mario /I-3549-2015; Introzzi, Gianluca/K-2497-2015; Lysak, Roman/H-2995-2014; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Chiarelli, Giorgio/E-8953-2012; Cavalli-Sforza, Matteo/H-7102-2015; OI song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Group, Robert/0000-0002-4097-5254; Simonenko, Alexander/0000-0001-6580-3638; Lancaster, Mark/0000-0002-8872-7292; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; Chiarelli, Giorgio/0000-0001-9851-4816; Hays, Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Dorigo, Mirco/0000-0002-0681-6946; Brucken, Jens Erik/0000-0001-6066-8756; Torre, Stefano/0000-0002-7565-0118; Casarsa, Massimo/0000-0002-1353-8964; Margaroli, Fabrizio/0000-0002-3869-0153; Latino, Giuseppe/0000-0002-4098-3502; iori, maurizio/0000-0002-6349-0380; Jun, Soon Yung/0000-0003-3370-6109; Toback, David/0000-0003-3457-4144; Vidal Marono, Miguel/0000-0002-2590-5987 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A.P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103]; Royal Society, UK FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A.P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, UK; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 46 TC 8 Z9 8 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 13 PY 2014 VL 89 IS 9 AR 091101 DI 10.1103/PhysRevD.89.091101 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH0RX UT WOS:000335829100001 ER PT J AU Celis, A Cirigliano, V Passemar, E AF Celis, Alejandro Cirigliano, Vincenzo Passemar, Emilie TI Model-discriminating power of lepton flavor violating tau decays SO PHYSICAL REVIEW D LA English DT Article ID STANDARD MODEL; LIGHT HIGGS; SEARCH; NUMBER; PHYSICS; MESON AB Within an effective field theory framework, we discuss the possibility to discriminate among different operators that contribute to lepton flavor violating (LFV) tau decays. Correlations among decay rates in different channels are shown to provide a basic handle to unravel the origin of LFV in these processes. More information about the underlying dynamics responsible for LFV can be gathered from differential distributions in three-body decays like tau -> mu pi pi or tau -> 3 mu: these are considered in some detail. We incorporate in our analysis recent developments in the determination of the hadronic form factors for tau -> mu pi pi. Future prospects for the observation of LFV tau decays and its interpretation are also discussed. C1 [Celis, Alejandro] Univ Valencia CSIC, IFIC, E-46071 Valencia, Spain. [Cirigliano, Vincenzo; Passemar, Emilie] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Celis, A (reprint author), Univ Valencia CSIC, IFIC, Apartat Correus 22085, E-46071 Valencia, Spain. EM alejandro.celis@ific.uv.es; cirigliano@lanl.gov; passemar@lanl.gov OI Celis, Alejandro/0000-0002-3045-6696 FU Spanish Government; EU Commission [FPU] [AP2010-0308, FPA2011-23778, CSD2007-00042]; Generalitat Valenciana [PROMETEOII/2013/007]; DOE Office of Science, Nuclear Physics program FX We would like to thank Kiyoshi Hayasaka for clarifications regarding the experimental limits on LFV tau decays and future prospects. The work of A. C. has been supported in part by the Spanish Government and ERDF funds from the EU Commission [FPU Grants No. AP2010-0308, No. FPA2011-23778 and No. CSD2007-00042 (Consolider Project CPAN)] and by Generalitat Valenciana under Grant No. PROMETEOII/2013/007. The work of V. C. and E. P. is supported by the DOE Office of Science, Nuclear Physics program. NR 72 TC 12 Z9 14 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 13 PY 2014 VL 89 IS 9 AR 095014 DI 10.1103/PhysRevD.89.095014 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH0RX UT WOS:000335829100009 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Delaere, C Du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MCM Martins, T Pol, ME Souza, MHG Ald, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E 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CA CMS Collaboration TI Measurement of the W gamma and Z gamma inclusive cross sections in pp collisions at root s=7 TeV and limits on anomalous triple gauge boson couplings SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; QCD CORRECTIONS; HIGGS-BOSON; AMPLITUDES; ZEROS; PHYSICS; SEARCH; SECTOR AB Measurements of W gamma and Z gamma production in proton-proton collisions at root s = 7 TeV are used to extract limits on anomalous triple gauge couplings. The results are based on data recorded by the CMS experiment at the LHC that correspond to an integrated luminosity of 5.0 fb(-1). The cross sections are measured for photon transverse momenta p(T)(gamma) > 15 GeV, and for separations between photons and final-state charged leptons in the pseudorapidity-azimuthal plane of Delta R(l,gamma) > 0.7 in l nu gamma and ll gamma final states, where l refers either to an electron or a muon. A dilepton invariant mass requirement of m(ll) > 50 GeV is imposed for the Z gamma process. 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A.; Janssen, X.; Knutsson, A.; Luyckx, S.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Staykova, Z.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Kalogeropoulos, A.; Keaveney, J.; Maes, M.; Olbrechts, A.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Hreus, T.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Delaere, C.; Du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Selvaggi, M.; Garcia, J. M. Vizan] Catholic Univ Louvain, B-1348 Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; Martins Junior, M. Correa; Martins, T.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Ald Junior, W. L.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; Martins, C. De Oliveira; De Souza, S. Fonseca; Malbouisson, H.; Malek, M.; Figueiredo, D. Matos; Mundim, L.; Nogima, H.; Da Silva, W. L. Prado; Santoro, A.; Sznajder, A.; Manganote, E. J. Tonelli; Pereira, A. Vilela] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dias, F. A.; Fernandez Perez Tomei, T. R.; Lagana, C.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Genchev, V.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Sultanov, G.; Vutova, M.] Inst Nucl Energy Res, Sofia, Bulgaria. [Dimitrov, A.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, J.; Wang, X.; Wang, Z.; Xiao, H.; Xu, M.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, Q.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Carrillo Montoya, C. A.; Chaparro Sierra, L. F.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.] Techn Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Duric, S.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.; Tikvica, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Abdelalim, A. A.; Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Radi, A.] Arab Republ Egypt, Acad Sci Res & Technol, Egyptian Network High Energy Phys, Cairo, Egypt. [Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Rebane, L.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Baffioni, S.; Beaudette, F.; Benhabib, L.; Bluj, M.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Florent, A.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.] CNRS, IN2P3, Ecole Polytech, Lab Leprince Ringuet, Palaiseau, France. [Agram, J. -L.; Andrea, J.; Bloch, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.] Univ Strasbourg, CNRS IN2P3, Univ Haute Alsace Mulhouse, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Gadrat, S.] CNRS, Ctr Calcul, Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sgandurra, L.; Sordini, V.; Tschudi, Y.; Vander Donckt, M.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Nucl Phys, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Calpas, B.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Hoepfner, K.; Klingebiel, D.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Inst Phys A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Inst Phys B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dorland, T.; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. Oe.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Stein, M.; Walsh, R.; Wissing, C.; Kaussen, G.; Kogler, R.] Deutsches Elekt Synchrotron, Hamburg, Germany. [Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Gebbert, U.; Goerner, M.; Gosselink, M.; Haller, J.; Heine, K.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Lange, J.; Marchesini, I.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.] Univ Hamburg, Hamburg, Germany. [Troendle, D.; Usai, E.; Vanelderen, L.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Kornmayer, A.; Pardo, P. Lobelle; Martschei, D.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, C.; Ntomari, E.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Radics, B.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, EHEP, Mumbai 400005, Maharashtra, India. [Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res, HECR, Mumbai 400005, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Barbone, L.; Calabria, C.; De Filippis, N.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Sgaravatto, M.; Torassa, E.; Tosi, M.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Torassa, E.; Tosi, M.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Androsov, K.] Ist Nazl Fis Nucl, Sez Perugia, Pisa, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Amapane, N.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Amapane, N.] Univ Roma, Rome, Italy. [Arneodo, M.; Biino, C.; Costa, M.; Mariotti, C.; Migliore, E.; Musich, M.; Obertino, M. M.; Ortona, G.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Ortona, G.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.] Korea Univ, Seoul, South Korea. [Roh, Y.; Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Abdulsalam, A.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; la Cruz, I. Heredia-De; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Moreno, S. Carrillo; Valencia, F. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico. [Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Linares, E. Casimiro; Pineda, A. Morelos; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Da Cruz E Silva, C. Beirao; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Caudron, A.; Abdulsalam, A.; Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An] Petersburg Nucl Phys Inst, Gatchina, Russia. [Andreev, Yu; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Pelayo, J. Puerta; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; De Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; David, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Bethani, A.; Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Williams, G.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. 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RI Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Gonzalez Caballero, Isidro/E-7350-2010; Novaes, Sergio/D-3532-2012; Scodellaro, Luca/K-9091-2014; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Gregores, Eduardo/F-8702-2012; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Torassa, Ezio/I-1788-2012; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; de la Cruz, Begona/K-7552-2014; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Menasce, Dario Livio/A-2168-2016; Tinoco Mendes, Andre David/D-4314-2011; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011 OI Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Novaes, Sergio/0000-0003-0471-8549; Scodellaro, Luca/0000-0002-4974-8330; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Yazgan, Efe/0000-0001-5732-7950; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Tinoco Mendes, Andre David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Rovelli, Tiziano/0000-0002-9746-4842; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique and Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education, Youth and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology; National Natural Science Foundation of China; Colombian funding agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonian Research Council [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education; University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLPFAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretar a de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, United Kingdom; U.S. Department of Energy; U.S. National Science Foundation; Marie Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS program of the Foundation for Polish Science; European Union Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique and Fonds voor Wetenschappelijk Onderzoek; the Brazilian funding agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education, Youth and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian funding agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and the Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican funding agencies (CINVESTAV, CONACYT, SEP, and UASLPFAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, the Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretar a de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss funding agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey and the Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, United Kingdom; and the U.S. Department of Energy and the U.S. National Science Foundation. Individuals have received support from the Marie Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); and the HOMING PLUS program of the Foundation for Polish Science, cofinanced from the European Union Regional Development Fund; and the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF. NR 48 TC 7 Z9 7 U1 5 U2 60 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 13 PY 2014 VL 89 IS 9 AR 092005 DI 10.1103/PhysRevD.89.092005 PG 32 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH0RX UT WOS:000335829100002 ER PT J AU Geller, M Bar-Shalom, S Soni, A AF Geller, Michael Bar-Shalom, Shaouly Soni, Amarjit TI Higgs-radion unification: Radius stabilization by an SU(2) bulk doublet and the 126 GeV scalar SO PHYSICAL REVIEW D LA English DT Article ID WARPED EXTRA DIMENSIONS AB We investigate a Randall-Sundrum (RS) model with an SU(2) doublet propagating in the bulk. Upon calculating its gravitational effect we find that a stabilized radius can be generated without the use of an additional scalar, as needed for example in the Goldberger-Wise (GW) mechanism, and with no additional fine-tuning other than the inescapable one due to the cosmological constant; similar tuning is also present in the GW mechanism. The lowest scalar excitation in this scenario, the counterpart of the radion of the GW mechanism, has both radionlike and Higgs-like couplings to the Standard Model fields. It, thus, plays a dual role and we, therefore, denote it as the "Higgs radion" (h(r)). As opposed to the GW radion case, our Higgs radion is found to be compatible with the 126 GeV scalar recently discovered at the LHC, at the level of 1 sigma, with a resulting 95% C. L. bound on the KK-gluon mass of 4.48 TeV < M-KKG < 5.44 TeV. An important consequence of our setup should be accentuated: the radion of the traditional RS scenarios simply does not exist, so that our Higgs radion is not the conventional mixed state between the GW radion and the Higgs. C1 [Geller, Michael; Bar-Shalom, Shaouly] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Soni, Amarjit] Brookhaven Natl Lab, Theory Grp, Upton, NY 11973 USA. RP Geller, M (reprint author), Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. EM mic.geller@gmail.com; shaouly@physics.technion.ac.il; adlersoni@gmail.com FU Technion; U.S. DOE [DE-AC02-98CH10886 (BNL)] FX We are extremely grateful to Kaustubh Agashe for many very valuable discussions. We also benefited from useful conversations with Hooman Davoudiasl, Yael Shadmi, Yotam Soreq, John Terning and Tomer Volansky. S. B. S. and M. G. acknowledge research support from the Technion and the work of A. S. is supported in part by the U.S. DOE Contract No. DE-AC02-98CH10886 (BNL). NR 61 TC 9 Z9 9 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 13 PY 2014 VL 89 IS 9 AR 095015 DI 10.1103/PhysRevD.89.095015 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH0RX UT WOS:000335829100010 ER PT J AU Upadhye, A Biswas, R Pope, A Heitmann, K Habib, S Finkel, H Frontiere, N AF Upadhye, Amol Biswas, Rahul Pope, Adrian Heitmann, Katrin Habib, Salman Finkel, Hal Frontiere, Nicholas TI Large-scale structure formation with massive neutrinos and dynamical dark energy SO PHYSICAL REVIEW D LA English DT Article ID MATTER POWER SPECTRUM; MICROWAVE BACKGROUND ANISOTROPIES; COSMOLOGICAL CONSTANT PROBLEM; COSMIC ACCELERATION; CONSTRAINTS; UNIVERSES; PROBE; SUPERNOVAE; DENSITY; MODELS AB Over the next decade, cosmological measurements of the large-scale structure of the Universe will be sensitive to the combined effects of dynamical dark energy and massive neutrinos. The matter power spectrum is a key repository of this information. We extend higher-order perturbative methods for computing the power spectrum to investigate these effects over quasilinear scales. Through comparison with N-body simulations, we establish the regime of validity of a time-renormalization group perturbative treatment that includes dynamical dark energy and massive neutrinos. We also quantify the accuracy of standard, renormalized and Lagrangian resummation (LPT) perturbation theories without massive neutrinos. We find that an approximation that neglects neutrino clustering as a source for nonlinear matter clustering predicts the baryon acoustic oscillation (BAO) peak position to 0.25% accuracy for redshifts 1 <= z <= 3, justifying the use of LPT for BAO reconstruction in upcoming surveys. We release a modified version of the public COPTER code which includes the additional physics discussed in the paper. C1 [Upadhye, Amol; Biswas, Rahul; Pope, Adrian; Heitmann, Katrin; Habib, Salman; Frontiere, Nicholas] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Upadhye, Amol; Heitmann, Katrin; Habib, Salman] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Heitmann, Katrin; Habib, Salman] Argonne Natl Lab, Div Math & Comp Sci, Lemont, IL 60439 USA. [Finkel, Hal] Argonne Natl Lab, ALCF, Lemont, IL 60439 USA. [Frontiere, Nicholas] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. RP Upadhye, A (reprint author), Argonne Natl Lab, Div High Energy Phys, 9700 S Cass Ave, Argonne, IL 60439 USA. FU U.S. Department of Energy, Basic Energy Sciences, Office of Science [DE-AC02-06CH11357]; DOE/SC [DE-AC02-06CH11357, DE-AC05-00OR22725]; Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX We are grateful to J. Kwan, Z. Lukic, and M. Pietroni for insightful conversations. S. H. thanks Masahiro Takada for useful discussions. The authors were supported by the U.S. Department of Energy, Basic Energy Sciences, Office of Science, under Contract No. DE-AC02-06CH11357. This research used resources of the ALCF, which is supported by DOE/SC under Contract No. DE-AC02-06CH11357 and resources of the OLCF, which is supported by DOE/SC under Contract No. DE-AC05-00OR22725.; The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. NR 75 TC 11 Z9 11 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 13 PY 2014 VL 89 IS 10 AR 103515 DI 10.1103/PhysRevD.89.103515 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH0SC UT WOS:000335829600007 ER PT J AU Ota, S Li, TC Li, YM Ye, ZL Labno, AN Yin, XB Alam, MR Zhang, X AF Ota, Sadao Li, Tongcang Li, Yimin Ye, Ziliang Labno, Anna Yin, Xiaobo Alam, Mohammad-Reza Zhang, Xiang TI Brownian motion of tethered nanowires SO PHYSICAL REVIEW E LA English DT Article ID SURFACE; FLUID; PARTICLES; CELL AB Brownian motion of slender particles near a boundary is ubiquitous in biological systems and in nanomaterial assembly, but the complex hydrodynamic interaction in those systems is still poorly understood. Here, we report experimental and computational studies of the Brownian motion of silicon nanowires tethered on a substrate. An optical interference method enabled direct observation of microscopic rotations of the slender bodies in three dimensions with high angular and temporal resolutions. This quantitative observation revealed anisotropic and angle-dependent hydrodynamic wall effects: rotational diffusivity in inclined and azimuth directions follows different power laws as a function of the length, similar to L-2.5 and similar to L-3, respectively, and is more hindered for smaller inclined angles. In parallel, we developed an implicit simulation technique that takes the complex wire-wall hydrodynamic interactions into account efficiently, the result of which agreed well with the experimentally observed angle-dependent diffusion. The demonstrated techniques provide a platform for studying the microrheology of soft condensed matters, such as colloidal and biological systems near interfaces, and exploring the optimal self-assembly conditions of nanostructures. C1 [Ota, Sadao; Li, Tongcang; Li, Yimin; Ye, Ziliang; Labno, Anna; Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr NSEC, Berkeley, CA 94720 USA. [Ota, Sadao; Alam, Mohammad-Reza; Zhang, Xiang] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Li, Tongcang; Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, 3112 Etcheverry Hall, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Li, Yimin/F-5821-2012; Zhang, Xiang/F-6905-2011; Ye, Ziliang/A-2104-2011; Yin, Xiaobo/A-4142-2011 FU National Science Foundation (NSF) Materials World Network [DMR-1210170] FX The authors acknowledge funding support by the National Science Foundation (NSF) Materials World Network (Grant No. DMR-1210170). NR 34 TC 3 Z9 3 U1 2 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD MAY 13 PY 2014 VL 89 IS 5 AR 053010 DI 10.1103/PhysRevE.89.053010 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AH0SN UT WOS:000335830700009 PM 25353883 ER PT J AU Lee, JH Selloni, A AF Lee, Jun Hee Selloni, Annabella TI TiO2/Ferroelectric Heterostructures as Dynamic Polarization-Promoted Catalysts for Photochemical and Electrochemical Oxidation of Water SO PHYSICAL REVIEW LETTERS LA English DT Article ID OXYGEN EVOLUTION; TIO2 PHOTOCATALYSIS; OXIDE SURFACES; ANATASE TIO2; REACTIVITY; STRAIN; FILMS AB Using first-principles density functional theory calculations, we explore the chemical activity of epitaxial heterostructures of TiO2 anatase on strained polar SrTiO3 films focusing on the oxygen evolution reaction (OER), the bottleneck of water splitting. Our results show that the reactivity of the TiO2 surface is tuned by electric dipoles dynamically induced by the adsorbed species during the intermediate steps of the reaction while the initial and final steps remain unaffected. Compared to the OER on unsupported TiO2, the combined effects of the dynamically induced dipoles and epitaxial strain strongly reduce rate-limiting thermodynamic barriers and significantly improve the efficiency of the reaction. C1 [Lee, Jun Hee; Selloni, Annabella] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. RP Lee, JH (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM leej@ornl.gov FU DOE-BES; Geosciences; Biosciences [DE-FG0205ER15702]; Division of Chemical Sciences FX We thank Ye-Fei Li, Jia Chen, Kevin Garrity, Kieron Burke, Morrel H. Cohen, Karin Rabe, Raffaele Resta, and David Vanderbilt for helpful discussions. This work was supported by DOE-BES, Division of Chemical Sciences, Geosciences, and Biosciences under Grant No. DE-FG0205ER15702. We acknowledge the use of computer resources at the TIGRESS high performance computer center of Princeton University, and at the center for Functional Nanomaterials, Brookhaven National Laboratory. NR 41 TC 14 Z9 14 U1 9 U2 135 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 13 PY 2014 VL 112 IS 19 AR 196102 DI 10.1103/PhysRevLett.112.196102 PG 5 WC Physics, Multidisciplinary SC Physics GA AH0TC UT WOS:000335832300002 PM 24877949 ER PT J AU Xiang, HJ Huang, B Kan, E Wei, SH Gong, XG AF Xiang, H. J. Huang, B. Kan, E. Wei, S. -H. Gong, X. G. TI Comment on "Towards Direct-Gap Silicon Phases by the Inverse Band Structure Design Approach" Reply SO PHYSICAL REVIEW LETTERS LA English DT Editorial Material ID SI3ALP C1 [Xiang, H. J.; Gong, X. G.] Fudan Univ, State Key Lab Surface Phys, Minist Educ, Key Lab Computat Phys Sci, Shanghai 200433, Peoples R China. [Xiang, H. J.; Gong, X. G.] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Xiang, H. J.; Huang, B.; Wei, S. -H.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Kan, E.] Nanjing Univ Sci & Technol, Dept Appl Phys, Nanjing 210094, Jiangsu, Peoples R China. RP Xiang, HJ (reprint author), Fudan Univ, State Key Lab Surface Phys, Minist Educ, Key Lab Computat Phys Sci, Shanghai 200433, Peoples R China. EM hxiang@fudan.edu.cn RI Huang, Bing/D-8941-2011; Xiang, Hongjun/I-4305-2016; Kan, Erjun/A-4322-2009; gong, xingao/D-6532-2011 OI Huang, Bing/0000-0001-6735-4637; Xiang, Hongjun/0000-0002-9396-3214; Kan, Erjun/0000-0003-0433-4190; NR 7 TC 1 Z9 1 U1 1 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 13 PY 2014 VL 112 IS 19 AR 199802 DI 10.1103/PhysRevLett.112.199802 PG 1 WC Physics, Multidisciplinary SC Physics GA AH0TC UT WOS:000335832300006 PM 24877973 ER PT J AU Buizert, C Baggenstos, D Jiang, W Purtschert, R Petrenko, VV Lu, ZT Muller, P Kuhl, T Lee, J Severinghaus, JP Brook, EJ AF Buizert, Christo Baggenstos, Daniel Jiang, Wei Purtschert, Roland Petrenko, Vasilii V. Lu, Zheng-Tian Mueller, Peter Kuhl, Tanner Lee, James Severinghaus, Jeffrey P. Brook, Edward J. TI Radiometric Kr-81 dating identifies 120,000-year-old ice at Taylor Glacier, Antarctica SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE geochronology; paleoclimatology; glaciology ID PAST 800,000 YEARS; ATMOSPHERIC CH4; MAGNETOOPTICAL TRAP; GEOMAGNETIC-FIELD; CLIMATE-CHANGE; POLAR ICE; RECORD; CORE; GREENLAND; TERMINATION AB We present successful Kr-81-Kr radiometric dating of ancient polar ice. Krypton was extracted from the air bubbles in four similar to 350-kg polar ice samples from Taylor Glacier in the McMurdo Dry Valleys, Antarctica, and dated using Atom Trap Trace Analysis (ATTA). The Kr-81 radiometric ages agree with independent age estimates obtained from stratigraphic dating techniques with a mean absolute age offset of 6 +/- 2.5 ka. Our experimental methods and sampling strategy are validated by (i) Kr-85 and Ar-39 analyses that show the samples to be free of modern air contamination and (ii) air content measurements that show the ice did not experience gas loss. We estimate the error in the Kr-81 ages due to past geomagnetic variability to be below 3 ka. We show that ice from the previous interglacial period (Marine Isotope Stage 5e, 130-115 ka before present) can be found in abundance near the surface of Taylor Glacier. Our study paves the way for reliable radiometric dating of ancient ice in blue ice areas and margin sites where large samples are available, greatly enhancing their scientific value as archives of old ice and meteorites. At present, ATTA Kr-81 analysis requires a 40-80-kg ice sample; as sample requirements continue to decrease, Kr-81 dating of ice cores is a future possibility. C1 [Buizert, Christo; Lee, James; Brook, Edward J.] Oregon State Univ, Coll Earth Ocean & Atmospher Sci, Corvallis, OR 97331 USA. [Baggenstos, Daniel; Severinghaus, Jeffrey P.] Univ Calif San Diego, Scripps Inst Oceanog, San Diego, CA 92093 USA. [Jiang, Wei; Lu, Zheng-Tian; Mueller, Peter] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Purtschert, Roland] Univ Bern, CH-3012 Bern, Switzerland. [Petrenko, Vasilii V.] Univ Rochester, Dept Earth & Environm Sci, Rochester, NY 14627 USA. [Lu, Zheng-Tian] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Lu, Zheng-Tian] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Kuhl, Tanner] Univ Wisconsin, Madison, WI 53706 USA. RP Buizert, C (reprint author), Oregon State Univ, Coll Earth Ocean & Atmospher Sci, Corvallis, OR 97331 USA. EM buizertc@science.oregonstate.edu RI Purtschert, Roland/N-7108-2016; Jiang, Wei/E-5582-2011; Mueller, Peter/E-4408-2011 OI Purtschert, Roland/0000-0002-4734-7664; Baggenstos, Daniel/0000-0001-9756-6884; Mueller, Peter/0000-0002-8544-8191 FU National Science Foundation Office of Polar Programs [0838936, 0839031]; National Oceanic and Atmospheric Administration Climate and Global Change Fellowship Program; Laboratory for Radiokrypton Dating at Argonne - Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX We want to thank X. Fain, L. Mitchell, H. Schaefer, A. Schilt, T. Bauska, McMurdo Operations, the Berg Field Center (Kate Koons, Martha Story, and Bija Sass), and helicopter crews for support in the field; Jon Edwards for his help with air content calculations; Matthew Puretz for krypton-stable isotope mass spectrometry; and the Polar Geospatial Center for their help with satellite image processing. The Center for Ice and Climate in Copenhagen hosted a seminar that led to the inception of the study. Constructive comments by two anonymous reviewers helped improve the manuscript. This work was funded through National Science Foundation Office of Polar Programs Grants 0838936 (to E.J.B.) and 0839031 (to J.P.S.); C.B. is supported by the National Oceanic and Atmospheric Administration Climate and Global Change Fellowship Program, administered by the University Corporation for Atmospheric Research; W.J., Z.T.L., P.M., and the Laboratory for Radiokrypton Dating at Argonne are supported by Department of Energy, Office of Nuclear Physics, under contract DE-AC02-06CH11357. Development of the ATTA-3 instrument was supported in part by NSF EAR-0651161. NR 65 TC 10 Z9 11 U1 5 U2 40 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 13 PY 2014 VL 111 IS 19 BP 6876 EP 6881 DI 10.1073/pnas.1320329111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH0GS UT WOS:000335798000041 PM 24753606 ER PT J AU Wang, Y Wang, MH Zhang, RY Ghan, SJ Lin, Y Hu, JX Pan, BW Levy, M Jiang, JH Molina, MJ AF Wang, Yuan Wang, Minghuai Zhang, Renyi Ghan, Steven J. Lin, Yun Hu, Jiaxi Pan, Bowen Levy, Misti Jiang, Jonathan H. Molina, Mario J. TI Assessing the effects of anthropogenic aerosols on Pacific storm track using a multiscale global climate model SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE aerosol-cloud-climate interaction; convective storms, cloud invigoration ID LONG-TERM IMPACTS; PNNL-MMF; PRECIPITATION; INTENSIFICATION; MICROPHYSICS; ATMOSPHERE; OXIDATION; PRODUCT; TROPICS; CLOUDS AB Atmospheric aerosols affect weather and global general circulation by modifying cloud and precipitation processes, but the magnitude of cloud adjustment by aerosols remains poorly quantified and represents the largest uncertainty in estimated forcing of climate change. Here we assess the effects of anthropogenic aerosols on the Pacific storm track, using a multiscale global aerosol-climate model (GCM). Simulations of two aerosol scenarios corresponding to the present day and preindustrial conditions reveal long-range transport of anthropogenic aerosols across the north Pacific and large resulting changes in the aerosol optical depth, cloud droplet number concentration, and cloud and ice water paths. Shortwave and long-wave cloud radiative forcing at the top of atmosphere are changed by -2.5 and +1.3 W m(-2), respectively, by emission changes from preindustrial to present day, and an increased cloud top height indicates invigorated midlatitude cyclones. The overall increased precipitation and poleward heat transport reflect intensification of the Pacific storm track by anthropogenic aerosols. Hence, this work provides, for the first time to the authors' knowledge, a global perspective of the effects of Asian pollution outflows from GCMs. Furthermore, our results suggest that the multiscale modeling framework is essential in producing the aerosol invigoration effect of deep convective clouds on a global scale. C1 [Wang, Yuan; Zhang, Renyi; Lin, Yun; Hu, Jiaxi; Pan, Bowen; Levy, Misti] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA. [Wang, Yuan; Jiang, Jonathan H.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Wang, Minghuai; Ghan, Steven J.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Zhang, Renyi] Peking Univ, Coll Environm Sci & Engn, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100871, Peoples R China. [Molina, Mario J.] Univ Calif San Diego, Dept Chem & Biochem, San Diego, CA 92093 USA. RP Zhang, RY (reprint author), Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA. EM renyi-zhang@tamu.edu; mjmolina@ucsd.edu RI Zhang, Renyi/A-2942-2011; Ghan, Steven/H-4301-2011; Levy, Misti/G-8660-2014; Wang, Minghuai/E-5390-2011; Lin, Yun/B-1906-2013 OI Ghan, Steven/0000-0001-8355-8699; Levy, Misti/0000-0002-4832-7753; Lin, Yun/0000-0001-8222-0346; Wang, Minghuai/0000-0002-9179-228X; FU National Aeronautics and Space Administration (NASA) Graduate Student Fellowship in Earth System Science; Ministry of Science and Technology of China [2013CB955800]; NASA Research Opportunities in Space and Earth Sciences Enhancing the Capability of Computational Earth System Models and Using NASA Data for Operation and Assessment program at the Jet Propulsion Laboratory, California Institute of Technology under NASA; Department of Energy (DOE) Office of Science, Decadal and Regional Climate Prediction using Earth System Models program; DOE [DE-AC06-76RLO 1830]; Office of Science of the US Department of Energy [DE-AC05-00OR22725] FX The authors acknowledge T. Yuan and P. Liss for providing additional comments. This work was supported by a National Aeronautics and Space Administration (NASA) Graduate Student Fellowship in Earth System Science (to Y.W.), Ministry of Science and Technology of China Award (2013CB955800 to R.Z.), the NASA Research Opportunities in Space and Earth Sciences Enhancing the Capability of Computational Earth System Models and Using NASA Data for Operation and Assessment program at the Jet Propulsion Laboratory, California Institute of Technology, under contract with NASA (Y.W. and J.H.J.), and the Department of Energy (DOE) Office of Science, Decadal and Regional Climate Prediction using Earth System Models program (M.W. and S.J.G.). PNNL is operated by Battelle for the DOE under Contract DE-AC06-76RLO 1830. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the US Department of Energy under Contract DE-AC05-00OR22725. NR 43 TC 35 Z9 37 U1 10 U2 59 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 13 PY 2014 VL 111 IS 19 BP 6894 EP 6899 DI 10.1073/pnas.1403364111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AH0GS UT WOS:000335798000044 PM 24733923 ER PT J AU Dejoie, C Sciau, P Li, WD Noe, L Mehta, A Chen, K Luo, HJ Kunz, M Tamura, N Liu, Z AF Dejoie, Catherine Sciau, Philippe Li, Weidong Noe, Laure Mehta, Apurva Chen, Kai Luo, Hongjie Kunz, Martin Tamura, Nobumichi Liu, Zhi TI Learning from the past: Rare epsilon-Fe2O3 in the ancient black-glazed Jian (Tenmoku) wares SO SCIENTIFIC REPORTS LA English DT Article ID MAGNETIC-PROPERTIES; WAVE ABSORBER; NANOPARTICLES; OXIDE; STABILIZATION; SPECTROSCOPY AB Ancient Jian wares are famous for their lustrous black glaze that exhibits unique colored patterns. Some striking examples include the brownish colored ``Hare's Fur'' (HF) strips and the silvery ``Oil Spot'' ( OS) patterns. Herein, we investigated the glaze surface of HF and OS samples using a variety of characterization methods. Contrary to the commonly accepted theory, we identified the presence of epsilon-Fe2O3, a rare metastable polymorph of Fe2O3 with unique magnetic properties, in both HF and OS samples. We found that surface crystals of OS samples are up to several micrometers in size and exclusively made of epsilon-Fe2O3. Interestingly, these epsilon-Fe2O3 crystals on the OS sample surface are organized in a periodic two dimensional fashion. These results shed new lights on the actual mechanisms and kinetics of polymorphous transitions of Fe2O3. Deciphering technologies behind the fabrication of ancient Jian wares can thus potentially help researchers improve the epsilon-Fe2O3 synthesis. C1 [Dejoie, Catherine] ETH, Crystallog Lab, CH-8093 Zurich, Switzerland. [Li, Weidong] Chinese Acad Sci, Shanghai Inst Ceram, Shanghai 200050, Peoples R China. [Dejoie, Catherine; Chen, Kai; Kunz, Martin; Tamura, Nobumichi; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Sciau, Philippe; Noe, Laure] Univ Toulouse, CNRS, CEMES, F-31055 Toulouse, France. [Mehta, Apurva] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Chen, Kai] Xi An Jiao Tong Univ, Ctr Adv Mat Performance Nanoscale, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. [Luo, Hongjie] Shanghai Univ, Shanghai 200436, Peoples R China. [Liu, Zhi] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, Shanghai 200050, Peoples R China. RP Li, WD (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, Shanghai 200050, Peoples R China. EM liwd@mail.sic.ac.cn; zliu2@lbl.gov RI Chen, Kai/O-5662-2014; Liu, Zhi/B-3642-2009; xjtu, campnano/Q-1904-2015 OI Chen, Kai/0000-0002-4917-4445; Liu, Zhi/0000-0002-8973-6561; FU key project of Natural Science Foundation of China [51232008]; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the US Department of Energy [DE-AC02-05CH11231]; National Natural Science Foundation of China [11227902] FX This work is supported by key project of Natural Science Foundation of China (No. 51232008). The authors would like to thank Robin Cours, Sebastien Joulie , Sebastien Moyano, Frederic Neumayer and Nicolas Ratel-Ramond from technical Poles of CEMES Lab for support during the experimental measurements. The Advanced Light Source at the Lawrence Berkeley National Laboratory is supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the US Department of Energy under contract No. DE-AC02-05CH11231. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the U. S. Department of Energy, Office of Basic Energy Sciences. Z.L. acknowledges the support of National Natural Science Foundation of China under Contract No. 11227902. NR 38 TC 13 Z9 14 U1 5 U2 49 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 13 PY 2014 VL 4 AR 4941 DI 10.1038/srep04941 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG9FP UT WOS:000335725100003 PM 24820819 ER PT J AU Chen, WNW Hudspeth, MC Claus, B Parab, ND Black, JT Fezzaa, K Luo, SN AF Chen, Weinong W. Hudspeth, Matthew C. Claus, Ben Parab, Niranjan D. Black, John T. Fezzaa, Kamel Luo, S. N. TI In situ damage assessment using synchrotron X-rays in materials loaded by a Hopkinson bar SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Article DE Hopkinson bar; synchrotron radiation; X-ray; phase contract imaging; granular materials; dynamic response ID PHASE-CONTRAST; DYNAMIC FRICTION; HIGH-PRESSURE; KOLSKY BAR; COMPRESSION; TENSION; IMPACT; SAND AB Split Hopkinson or Kolsky bars are common high-rate characterization tools for dynamic mechanical behaviour of materials. Stress-strain responses averaged over specimen volume are obtained as a function of strain rate. Specimen deformation histories can be monitored by high-speed imaging on the surface. It has not been possible to track the damage initiation and evolution during the dynamic deformation inside specimens except for a few transparent materials. In this study, we integrated Hopkinson compression/tension bars with high-speed X-ray imaging capabilities. The damage history in a dynamically deforming specimen was monitored in situ using synchrotron radiation via X-ray phase contrast imaging. The effectiveness of the novel union between these two powerful techniques, which opens a new angle for data acquisition in dynamic experiments, is demonstrated by a series of dynamic experiments on a variety of material systems, including particle interaction in granular materials, glass impact cracking, single crystal silicon tensile failure and ligament-bone junction damage. C1 [Chen, Weinong W.] Purdue Univ, Sch Mat Sci, W Lafayette, IN 47907 USA. [Chen, Weinong W.; Hudspeth, Matthew C.; Claus, Ben; Parab, Niranjan D.; Black, John T.] Purdue Univ, Sch Aeronaut & Astronaut, W Lafayette, IN 47907 USA. [Fezzaa, Kamel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Luo, S. N.] Sichuan Univ, Peac Inst Multiscale Sci, Chengdu 610064, Peoples R China. RP Chen, WNW (reprint author), Purdue Univ, Sch Mat Sci, W Lafayette, IN 47907 USA. EM wchen@purdue.edu RI Luo, Sheng-Nian /D-2257-2010 OI Luo, Sheng-Nian /0000-0002-7538-0541 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; US Army TARDEC; PEO Soldiers; Office of Naval Research; Defence Threat Reduction Agency FX The authors acknowledge professional help from A. Deriy (ANL) with technical and safety aspects of the experiments at 32ID. Use of the APS was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. Purdue University researchers were partially supported by research grants and contracts from US Army TARDEC, PEO Soldiers, Office of Naval Research and Defence Threat Reduction Agency. NR 38 TC 9 Z9 9 U1 4 U2 27 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-503X EI 1471-2962 J9 PHILOS T R SOC A JI Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci. PD MAY 13 PY 2014 VL 372 IS 2015 SI SI AR 20130191 DI 10.1098/rsta.2013.0191 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AE9TZ UT WOS:000334354500003 PM 24711489 ER PT J AU Jiang, CL Rehm, KE Back, BB Esbensen, H Janssens, RVF Stefanini, AM Montagnoli, G AF Jiang, C. L. Rehm, K. E. Back, B. B. Esbensen, H. Janssens, R. V. F. Stefanini, A. M. Montagnoli, G. TI Influence of heavy-ion transfer on fusion reactions SO PHYSICAL REVIEW C LA English DT Article ID MULTINUCLEON TRANSFER-REACTIONS; SUBBARRIER FUSION; TRANSFER COUPLINGS; COULOMB BARRIER; CROSS-SECTIONS; NEAR-BARRIER; NEUTRON; CA-40+ZR-90,ZR-96; COLLISIONS; HINDRANCE AB The influence of inelastic excitations on heavy-ion fusion is well established and can be quantitativly described by coupled-channels calculations. The influence of transfer channels, however, is still under debate. We have analyzed a large set of heavy-ion-induced fusion excitation functions involving nuclei with similar structures and show that there is a universal correlation between the shape (and enhancement) of the excitation function and the strength of the total neutron-transfer cross sections for systems ranging from light to heavy masses. C1 [Jiang, C. L.; Rehm, K. E.; Back, B. B.; Esbensen, H.; Janssens, R. V. F.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Stefanini, A. M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, IT-35020 Legnaro, Italy. [Montagnoli, G.] Univ Padua, Dipartimento Fis & Astron, IT-35131 Padua, Italy. [Montagnoli, G.] Ist Nazl Fis Nucl, Sez Padova, IT-35131 Padua, Italy. RP Jiang, CL (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. FU U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; European Union [262010-ENSAR] FX The authors thank Z. Kohley, J. J. Kolata and F. Scarlassara for providing us with their experimental fusion data. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. A.M.S. and G.M. acknowledge receiving funding from the European Union Seventh Framework Program FP7/2007-2013 under Grant Agreement No. 262010-ENSAR. NR 46 TC 18 Z9 18 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 12 PY 2014 VL 89 IS 5 AR 051603 DI 10.1103/PhysRevC.89.051603 PG 4 WC Physics, Nuclear SC Physics GA AH1XQ UT WOS:000335915500001 ER PT J AU Das, S Chaudhuri, SK Bhattacharya, RN Mandal, KC AF Das, Sandip Chaudhuri, Sandeep K. Bhattacharya, Raghu N. Mandal, Krishna C. TI Defect levels in Cu2ZnSn(SxSe1-x)(4) solar cells probed by current-mode deep level transient spectroscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID PHASE-EQUILIBRIA; CU2ZNSNS4; EFFICIENCY; SYSTEM; FILMS AB Defect levels in kesterite Cu2ZnSn(S,Se)(4) (CZTSSe) solar cells have been investigated by current-mode deep level transient spectroscopy. Experiments were carried out on two CZTSSe cells with photoconversion efficiencies of 4.1% and 7.1% measured under AM 1.5 illumination. The absorber layer of the 4.1% efficiency cell was prepared by annealing evaporated ZnS/Cu/Sn stacked precursor under S/Se vapor, while the absorber of the 7.1% efficiency cell was prepared by co-evaporation of the constituent elements. The 4.1% efficiency CZTSSe cell with a S/(S+Se) ratio of 0.58 exhibited two dominant deep acceptor levels at E-v+0.12 eV, and E-v+0.32 eV identified as Cu-Zn(-/0) and Cu-Sn(2-/-) antisite defects, respectively. The 7.1% efficiency cell with purely Se composition S/(S+Se) 0 showed only one shallow level at E-v+0.03 eV corresponding to Cu-vacancy (V-Cu). Our results revealed that V-Cu is the primary defect center in the high-efficiency kesterite solar cell in contrast to the detrimental Cu-Zn and Cu-Sn antisites found in the low efficiency CZTSSe cells limiting the device performance. (C) 2014 AIP Publishing LLC. C1 [Das, Sandip; Chaudhuri, Sandeep K.; Mandal, Krishna C.] Univ S Carolina, Dept Elect Engn, Columbia, SC 29208 USA. [Bhattacharya, Raghu N.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Mandal, KC (reprint author), Univ S Carolina, Dept Elect Engn, Columbia, SC 29208 USA. EM mandalk@cec.sc.edu OI Das, Sandip/0000-0002-7336-9568 FU Alliance for Sustainable Energy, LLC [DE-AC36-08GO28308]; U.S. Department of Energy (LDRD program) FX We would like to thank Ingrid Repins (NREL) for providing us with physical vapor deposited CZTSe sample. One of the authors (R. N. Bhattacharya, NREL) would like to acknowledge partial financial support from "Alliance for Sustainable Energy, LLC," under Contract No. DE-AC36-08GO28308 with the U.S. Department of Energy (LDRD program). NR 25 TC 7 Z9 7 U1 3 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 12 PY 2014 VL 104 IS 19 AR 192106 DI 10.1063/1.4876925 PG 4 WC Physics, Applied SC Physics GA AI5ON UT WOS:000336918600032 ER PT J AU Lo, CC Simmons, S Lo Nardo, R Weis, CD Tyryshkin, AM Meijer, J Rogalla, D Lyon, SA Bokor, J Schenkel, T Morton, JJL AF Lo, C. C. Simmons, S. Lo Nardo, R. Weis, C. D. Tyryshkin, A. M. Meijer, J. Rogalla, D. Lyon, S. A. Bokor, J. Schenkel, T. Morton, J. J. L. TI Stark shift and field ionization of arsenic donors in Si-28-silicon-on-insulator structures SO APPLIED PHYSICS LETTERS LA English DT Article ID ELECTRON-SPIN; SILICON; READOUT; QUBIT AB We develop an efficient back gate for silicon-on-insulator (SOI) devices operating at cryogenic temperatures and measure the quadratic hyperfine Stark shift parameter of arsenic donors in isotopically purified Si-28-SOI layers using such structures. The back gate is implemented using MeV ion implantation through the SOI layer forming a metallic electrode in the handle wafer, enabling large and uniform electric fields up to 2V/mu m to be applied across the SOI layer. Utilizing this structure, we measure the Stark shift parameters of arsenic donors embedded in the Si-28-SOI layer and find a contact hyperfine Stark parameter of eta(a) = -1.9 +/- 0.7 x 10(-3) mu m(2)/V-2. We also demonstrate electric-field driven dopant ionization in the SOI device layer, measured by electron spin resonance. (C) 2014 AIP Publishing LLC. C1 [Lo, C. C.; Lo Nardo, R.; Morton, J. J. L.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Lo, C. C.; Morton, J. J. L.] UCL, Dept Elect & Elect Engn, London WC1E 7JE, England. [Simmons, S.; Lo Nardo, R.] Univ Oxford, Dept Mat, Oxford OX1 3PH, England. [Weis, C. D.; Schenkel, T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. [Tyryshkin, A. M.; Lyon, S. A.] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA. [Meijer, J.; Rogalla, D.] Ruhr Univ Bochum, RUBION, Bochum, Germany. [Bokor, J.] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Lo, CC (reprint author), UCL, London Ctr Nanotechnol, London WC1H 0AH, England. EM cheuk.lo@ucl.ac.uk; jjl.morton@ucl.ac.uk RI Morton, John/I-3515-2013; Foundry, Molecular/G-9968-2014 FU EPSRC through the Materials World Network [EP/I035536/1]; CAESR [EP/D048559/1]; European Research Council under the European Community/ERC [279781]; NSF through Materials World Network [DMR-1107606]; Princeton MRSEC [DMR-0819860]; U.S. National Security Agency [100000080295]; U.S. Department of Energy [DE-AC02-05CH11231]; Royal Commission for the Exhibition of 1851; Violette and Samuel Glasstone Fund; St. John's College Oxford; Royal Society FX This research was supported by the EPSRC through the Materials World Network (EP/I035536/1) and CAESR (EP/D048559/1) as well as by the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC Grant Agreement No. 279781. Work at Princeton was supported by NSF through Materials World Network (DMR-1107606) and through the Princeton MRSEC (DMR-0819860). Work at LBNL was supported by the U.S. National Security Agency (No. 100000080295) and by the U.S. Department of Energy (DE-AC02-05CH11231, LBNL). C.C.L. is supported by the Royal Commission for the Exhibition of 1851. S.S. is supported by the Violette and Samuel Glasstone Fund and St. John's College Oxford. J.J.L.M. is supported by the Royal Society. NR 21 TC 9 Z9 9 U1 1 U2 18 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 12 PY 2014 VL 104 IS 19 AR 193502 DI 10.1063/1.4876175 PG 4 WC Physics, Applied SC Physics GA AI5ON UT WOS:000336918600066 ER PT J AU Rouleau, CM Shih, CY Wu, C Zhigilei, LV Puretzky, AA Geohegan, DB AF Rouleau, C. M. Shih, C-Y Wu, C. Zhigilei, L. V. Puretzky, A. A. Geohegan, D. B. TI Nanoparticle generation and transport resulting from femtosecond laser ablation of ultrathin metal films: Time-resolved measurements and molecular dynamics simulations SO APPLIED PHYSICS LETTERS LA English DT Article ID MICROSCOPIC MECHANISMS; SPALLATION AB The synthesis of metal nanoparticles by ultrafast laser ablation of nanometers-thick metal films has been studied experimentally and computationally. Near-threshold backside laser ablation of 2-20 nm-thick Pt films deposited on fused silica substrates was found to produce nanoparticles with size distributions that were bimodal for the thicker films, but collapsed into a single mode distribution for the thinnest film. Time-resolved imaging of blackbody emission from the Pt nanoparticles was used to reveal the nanoparticle propagation dynamics and estimate their temperatures. The observed nanoparticle plume was compact and highly forward-directed with a well-defined collective velocity that permitted multiple rebounds with substrates to be revealed. Large-scale molecular dynamics simulations were used to understand the evolution of compressive and tensile stresses in the thicker melted liquid films that lead to their breakup and ejection of two groups of nanoparticles with different velocity and size distributions. Ultrafast laser irradiation of ultrathin (few nm) metal films avoids the splitting of the film and appears to be a method wellsuited to cleanly synthesize and deposit nanoparticles from semitransparent thin film targets in highly directed beams. (C) 2014 AIP Publishing LLC. C1 [Rouleau, C. M.; Puretzky, A. A.; Geohegan, D. B.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Shih, C-Y; Wu, C.; Zhigilei, L. V.] Univ Virginia, Dept Mat Sci & Engn, Charlottesville, VA 22904 USA. RP Rouleau, CM (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM rouleaucm@ornl.gov RI Wu, Chengping/H-8741-2013; Rouleau, Christopher/Q-2737-2015; Puretzky, Alexander/B-5567-2016; Zhigilei, Leonid/E-2167-2012; Geohegan, David/D-3599-2013 OI Wu, Chengping/0000-0002-8337-9807; Rouleau, Christopher/0000-0002-5488-3537; Puretzky, Alexander/0000-0002-9996-4429; Geohegan, David/0000-0003-0273-3139 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; Oak Ridge National Laboratory by the Scientific User Facilities Division, U.S. Department of Energy; National Science Foundation [DMR-0907247, CMMI-1301298]; Air Force Office of Scientific Research [FA9550-10-1-0541]; NSF through the Extreme Science and Engineering Discovery Environment [TG-DMR110090]; Oak Ridge Leadership Computing Facility [MAT048] FX Research was sponsored by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy (synthesis science). A portion of this research was conducted as a user project at the Center for Nanophase Materials Sciences user facility, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, U.S. Department of Energy. Computational studies were funded by the National Science Foundation through Grants DMR-0907247 and CMMI-1301298, and the Air Force Office of Scientific Research through Grant FA9550-10-1-0541. Computational support was provided by NSF through the Extreme Science and Engineering Discovery Environment (Project TG-DMR110090) and by the Oak Ridge Leadership Computing Facility (Project MAT048). NR 30 TC 12 Z9 12 U1 1 U2 39 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 12 PY 2014 VL 104 IS 19 AR 193106 DI 10.1063/1.4876601 PG 5 WC Physics, Applied SC Physics GA AI5ON UT WOS:000336918600050 ER PT J AU Ye, Y Ye, ZL Gharghi, M Zhu, HY Zhao, M Wang, Y Yin, XB Zhang, X AF Ye, Yu Ye, Ziliang Gharghi, Majid Zhu, Hanyu Zhao, Mervin Wang, Yuan Yin, Xiaobo Zhang, Xiang TI Exciton-dominant electroluminescence from a diode of monolayer MoS2 SO APPLIED PHYSICS LETTERS LA English DT Article ID VALLEY POLARIZATION; LAYER MOS2; CONTACTS AB In two-dimensional monolayer MoS2, excitons dominate the absorption and emission properties. However, the low electroluminescent efficiency and signal-to-noise ratio limit our understanding of the excitonic behavior of electroluminescence. Here, we study the microscopic origin of the electroluminescence from a diode of monolayer MoS2 fabricated on a heavily p-type doped silicon substrate. Direct and bound-exciton related recombination processes are identified from the electroluminescence. At a high electron-hole pair injection rate, Auger recombination of the exciton-exciton annihilation of the bound exciton emission is observed at room temperature. Moreover, the efficient electrical injection demonstrated here allows for the observation of a higher energy exciton peak of 2.255 eV in the monolayer MoS2 diode, attributed to the excited exciton state of a direct-exciton transition. (C) 2014 AIP Publishing LLC. C1 [Ye, Yu; Ye, Ziliang; Gharghi, Majid; Zhu, Hanyu; Zhao, Mervin; Wang, Yuan; Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Zhao, Mervin; Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, 3112 Etcheverry Hall, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Wang, Yuan/F-7211-2011; Zhang, Xiang/F-6905-2011; Ye, Ziliang/A-2104-2011; Yin, Xiaobo/A-4142-2011 FU U.S. Air Force Office of Scientific Research; Multidisciplinary University Research Initiative program [FA9550-12-1-0024]; U.S. Department of Energy [DE-AC02-05CH11231] FX This research was supported by the U.S. Air Force Office of Scientific Research, Multidisciplinary University Research Initiative program under grant FA9550-12-1-0024 and the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 22 TC 25 Z9 25 U1 1 U2 66 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 12 PY 2014 VL 104 IS 19 AR 193508 DI 10.1063/1.4875959 PG 4 WC Physics, Applied SC Physics GA AI5ON UT WOS:000336918600072 ER PT J AU Macal, CM North, MJ Collier, N Dukic, VM Wegener, DT David, MZ Daum, RS Schumm, P Evans, JA Wilder, JR Miller, LG Eells, SJ Lauderdale, DS AF Macal, Charles M. North, Michael J. Collier, Nicholson Dukic, Vanja M. Wegener, Duane T. David, Michael Z. Daum, Robert S. Schumm, Philip Evans, James A. Wilder, Jocelyn R. Miller, Loren G. Eells, Samantha J. Lauderdale, Diane S. TI Modeling the transmission of community-associated methicillin-resistant Staphylococcus aureus: a dynamic agent-based simulation SO JOURNAL OF TRANSLATIONAL MEDICINE LA English DT Article DE MRSA; Agent-based model; Infectious disease model ID SOFT-TISSUE INFECTIONS; INTENSIVE-CARE-UNIT; RISK-FACTORS; COLONIZATION; SKIN; HOSPITALS; PREVALENCE; CALIFORNIA; PATHOGENS; EPIDEMIC AB Background: Methicillin-resistant Staphylococcus aureus (MRSA) has been a deadly pathogen in healthcare settings since the 1960s, but MRSA epidemiology changed since 1990 with new genetically distinct strain types circulating among previously healthy people outside healthcare settings. Community-associated (CA) MRSA strains primarily cause skin and soft tissue infections, but may also cause life-threatening invasive infections. First seen in Australia and the U.S., it is a growing problem around the world. The U.S. has had the most widespread CA-MRSA epidemic, with strain type USA300 causing the great majority of infections. Individuals with either asymptomatic colonization or infection may transmit CA-MRSA to others, largely by skin-to-skin contact. Control measures have focused on hospital transmission. Limited public health education has focused on care for skin infections. Methods: We developed a fine-grained agent-based model for Chicago to identify where to target interventions to reduce CA-MRSA transmission. An agent-based model allows us to represent heterogeneity in population behavior, locations and contact patterns that are highly relevant for CA-MRSA transmission and control. Drawing on nationally representative survey data, the model represents variation in sociodemographics, locations, behaviors, and physical contact patterns. Transmission probabilities are based on a comprehensive literature review. Results: Over multiple 10-year runs with one-hour ticks, our model generates temporal and geographic trends in CA-MRSA incidence similar to Chicago from 2001 to 2010. On average, a majority of transmission events occurred in households, and colonized rather than infected agents were the source of the great majority (over 95%) of transmission events. The key findings are that infected people are not the primary source of spread. Rather, the far greater number of colonized individuals must be targeted to reduce transmission. Conclusions: Our findings suggest that current paradigms in MRSA control in the United States cannot be very effective in reducing the incidence of CA-MRSA infections. Furthermore, the control measures that have focused on hospitals are unlikely to have much population-wide impact on CA-MRSA rates. New strategies need to be developed, as the incidence of CA-MRSA is likely to continue to grow around the world. C1 [Macal, Charles M.; North, Michael J.; Collier, Nicholson] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. [Macal, Charles M.; North, Michael J.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Dukic, Vanja M.] Univ Colorado Boulder, Boulder, CO 80309 USA. [Wegener, Duane T.] Ohio State Univ, Columbus, OH 43210 USA. [David, Michael Z.] Univ Chicago, Dept Med, Chicago, IL 60637 USA. [David, Michael Z.; Daum, Robert S.; Schumm, Philip; Evans, James A.; Wilder, Jocelyn R.; Lauderdale, Diane S.] Univ Chicago, Chicago, IL 60637 USA. [Miller, Loren G.; Eells, Samantha J.] Harbor UCLA Med Ctr, Div Infect Dis, Torrance, CA 90509 USA. RP Macal, CM (reprint author), Argonne Natl Lab, Decis & Informat Sci Div, 9700 S Cass Ave,Bldg 221, Argonne, IL 60439 USA. EM macal@anl.gov OI Wegener, Duane/0000-0001-7639-4251 FU National Institute of General Medical Sciences, Models of Infectious Disease Agent Study (MIDAS) [U01GM087729]; U.S. Department of Energy [DE-AC02-06CH11357]; Time-sharing Experiments for the Social Sciences, NSF [0818839] FX This work is supported by the National Institute of General Medical Sciences, Models of Infectious Disease Agent Study (MIDAS), grant number U01GM087729, the U.S. Department of Energy under contract number DE-AC02-06CH11357 and Time-sharing Experiments for the Social Sciences, NSF Grant 0818839. John Murphy provided computing support. Roberta Davidson provided data support. NR 40 TC 15 Z9 15 U1 1 U2 21 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1479-5876 J9 J TRANSL MED JI J. Transl. Med. PD MAY 12 PY 2014 VL 12 AR 124 DI 10.1186/1479-5876-12-124 PG 12 WC Medicine, Research & Experimental SC Research & Experimental Medicine GA AI5TY UT WOS:000336933300001 PM 24886400 ER PT J AU Weiss, CJ Egbert, JD Chen, ST Helm, ML Bullock, RM Mock, MT AF Weiss, Charles J. Egbert, Jonathan D. Chen, Shentan Helm, Monte L. Bullock, R. Morris Mock, Michael T. TI Protonation Studies of a Tungsten Dinitrogen Complex Supported by a Diphosphine Ligand Containing a Pendant Amine SO ORGANOMETALLICS LA English DT Article ID SYNTHETIC NITROGEN-FIXATION; N-2 REDUCTION; MOLECULAR-STRUCTURE; AMMONIA-SYNTHESIS; REACTION PATHWAY; BASICITY SCALE; MOLYBDENUM; MECHANISM; METAL; IRON AB Treatment of trans-[W(N-2)(2)(dppe)-((PNPEt)-N-Et-P-Me)](dppe = Ph2PCH2CH2PPh2; (PNPEt)-N-Et-P-Me = Et2PCH2N(Me)CH2PEt2) with 3 equiv of tetrafluoroboric acid (HBF4 center dot Et2O) at -78 degrees C generated the seven-coordinate tungsten hydride trans-[W(N-2)(2)(H)(dppe)(P(Et)N(Me)p(Et))][BF4]. At higher temperatures, protonation of a pendant amine is also observed, affording trans-[W(N-2)(2)(H)(dppe)((PNMe)-N-Et(H)P-Et)][BF4](2), with formation of the hydrazido complex [W(NNH2)(dppe)((PNMe)-N-Et(H)P-Et)][BF4](2) as a minor product. A similar product mixture was obtained using triflic acid (HOTf). The protonated products are thermally sensitive and do not persist at ambient temperature. Upon acid addition to the carbonyl analogue cis-[W(CO)(2)(dppe) (p(Et)N(Me)p(Et))] the seven-coordinate carbonyl hydride complex trans-[W(CO)(2)(H)(dppe)((PNMe)-N-Et(H)P-Et)][OTf](2) was generated. A mixed diphosphine complex without the pendant amine in the ligand backbone, trans-[W(N-2)(2)(dppe)(depp)] (depp = Et2P(CH2)(3)PEt2), was synthesized and treated with HOTf, selectively generating a hydrazido complex, [W(NNH2)(OTf)(dppe)(depp)][OTf]. Computational analysis probed the proton affinity of three sites of protonation in these complexes: the metal, pendant amine, and N2 ligand. Room-temperature reactions with 100 equiv of HOTf produced NH4+ from reduction of the N-2 ligand (electrons come from W). The addition of 100 equiv of HOTf to trans-[W(N-2)(2)(dppe)((PNPEt)-N-Et-P-Me)] afforded 0.81 equiv of NH4+, while 0.40 equiv of NH4+ was formed upon treatment of trans-[W(N-2)(2)(dppe)(depp)] with HOTf, showing that the complexes containing proton relays produce more products of reduction of N-2. C1 [Weiss, Charles J.; Egbert, Jonathan D.; Chen, Shentan; Helm, Monte L.; Bullock, R. Morris; Mock, Michael T.] Pacific NW Natl Lab, Div Phys Sci, Ctr Mol Electrocatalysis, Richland, WA 99352 USA. RP Mock, MT (reprint author), Pacific NW Natl Lab, Div Phys Sci, Ctr Mol Electrocatalysis, Richland, WA 99352 USA. EM Michael.Mock@pnnl.gov RI Bullock, R. Morris/L-6802-2016 OI Bullock, R. Morris/0000-0001-6306-4851 FU Center for Molecular Electrocatalysis, an Energy Frontier Research Center - U.S. Department of Energy Office of Science, Office of Basic Energy Sciences FX This work was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences. Computational resources were provided by the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory. Pacific Northwest National Laboratory is operated by Battelle for the DOE. We also thank Dr. Molly O'Hagan and Dr. Elliott B. Hulley for their assistance with NMR experiments. We thank Dr. Daniel L. DuBois and Dr. Roger Rousseau for helpful discussions. NR 82 TC 7 Z9 7 U1 3 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD MAY 12 PY 2014 VL 33 IS 9 BP 2189 EP 2200 DI 10.1021/om401127v PG 12 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA AH2GQ UT WOS:000335939900010 ER PT J AU Galan, BR Wiedner, ES Helm, ML Linehan, JC Appel, AM AF Galan, Brandon R. Wiedner, Eric S. Helm, Monte L. Linehan, John C. Appel, Aaron M. TI Effects of Phosphine-Carbene Substitutions on the Electrochemical and Thermodynamic Properties of Nickel Complexes SO ORGANOMETALLICS LA English DT Article ID N-HETEROCYCLIC-CARBENE; HYDRIDE DONOR ABILITIES; ELECTRONIC-PROPERTIES; COORDINATION CHEMISTRY; CATALYTIC-ACTIVITY; IRIDIUM COMPLEXES; METAL-HYDRIDES; BOND-ENERGIES; NHC LIGANDS; RHODIUM AB Nickel(II) complexes containing chelating N-heterocyclic carbene-phosphine ligands ([NiL2] (BPh4)(2), for which L = [MeIm(CH2)(2)PR2], MeIm = 1-methylimidizolylidene, and R = Ph or Et) have been synthesized for the purpose of studying how this class of ligand affects the electrochemical and thermodynamic properties compared to the nickel bis-diphosphine analogues. The nickel complexes were synthesized and then characterized by X-ray crystallography, electrochemical methods, and thermodynamic studies, including DFT calculations. On the basis of the reduction potentials (E degrees), substitution of an NHC for one of the phosphines in a diphoshine ligand resulted in negative shifts in potential by 0.6 to 1.2 V relative to the corresponding nickel bis-diphosphine complexes. From computational studies of the nickel hydride complex of the phenyl-substituted phosphine carbene ligand, the hydride donor ability was determined to improve by 32 kcal/mol relative to the estimated hydride donor ability for the analogous nickel complex of the chelating diphosphine ligand 1,3-bis(diphenylphosphino)propane. The free energy for addition of H-2 is presented, and the implications for catalysis are discussed. These quantitative results highlight the substantial effect that NHC ligands can have on the electronic properties of the metal complexes. C1 [Galan, Brandon R.; Wiedner, Eric S.; Helm, Monte L.; Linehan, John C.; Appel, Aaron M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Appel, AM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM aaron.appel@pnnl.gov OI Wiedner, Eric/0000-0002-7202-9676; Appel, Aaron/0000-0002-5604-1253 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Center for Molecular Electrocatalysis, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX B.R.G., E.S.W., J.C.L., and A.M.A. were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. M.L.H. was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for the DOE by Battelle. Computational resources were provided at the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory. NR 62 TC 9 Z9 9 U1 1 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD MAY 12 PY 2014 VL 33 IS 9 BP 2287 EP 2294 DI 10.1021/om500206e PG 8 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA AH2GQ UT WOS:000335939900019 ER PT J AU Barber, JL Barnes, CW Sandberg, RL Sheffield, RL AF Barber, John L. Barnes, Cris W. Sandberg, Richard L. Sheffield, Richard L. TI Diffractive imaging at large Fresnel number: Challenge of dynamic mesoscale imaging with hard x rays SO PHYSICAL REVIEW B LA English DT Article ID PHASE RETRIEVAL; RECONSTRUCTION; MICROSCOPY; OBJECT; LASER; BEAM AB Real materials have structure at both the atomic or crystalline scale as well as at interfaces and defects at the larger scale of grains. There is a need for the study of materials at the "mesoscale," the scale at which subgranular physical processes and intergranular organization couple to determine microstructure, crucially impacting constitutive response at the engineering macroscale. Diffractive imaging using photons that can penetrate multiple grains of material would be a transformative technique for the study of the performance of materials in dynamic extremes. Thicker samples imply higher energy photons of shorter wavelength, and imaging of multiple grains implies bigger spot sizes. Such imaging requires the use of future planned and proposed hard x-ray free electron lasers (such as the European XFEL) to provide both the spatial coherence transverse to the large spots and the peak brilliance to provide the short illumination times. The result is that the Fresnel number of the system becomes large and is no longer in the Fraunhofer far-field limit. The interrelated issues of diffractive imaging at large Fresnel number are analyzed, including proof that diffractive imaging is possible in this limit and estimates of the signal-to-noise possible. In addition, derivation of the heating rates for brilliant pulses of x rays are presented. The potential and limitations on multiple dynamic images are derived. This paper will present a study of x-ray interactions with materials in this new regime of spatially coherent but relatively large mesoscale spots at very hard energies. It should provide the theory and design background for the experiments and facilities required to control materials in extreme environments, in particular for the next generation of very-hard-x-ray free electron lasers. C1 [Barber, John L.; Barnes, Cris W.; Sandberg, Richard L.; Sheffield, Richard L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Barber, JL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM jlbarber@lanl.gov; cbarnes@lanl.gov; sandberg@lanl.gov; sheff@lanl.gov OI Barnes, Cris/0000-0002-3347-0741; Sandberg, Richard/0000-0001-9719-8188 NR 40 TC 1 Z9 1 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 12 PY 2014 VL 89 IS 18 AR 184105 DI 10.1103/PhysRevB.89.184105 PG 13 WC Physics, Condensed Matter SC Physics GA AH1WM UT WOS:000335912400003 ER PT J AU Clay, RC Mcminis, J McMahon, JM Pierleoni, C Ceperley, DM Morales, MA AF Clay, Raymond C., III Mcminis, Jeremy McMahon, Jeffrey M. Pierleoni, Carlo Ceperley, David M. Morales, Miguel A. TI Benchmarking exchange-correlation functionals for hydrogen at high pressures using quantum Monte Carlo SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; METALLIC HYDROGEN; DENSITY; TRANSITION; APPROXIMATION; FLUID AB The ab initio phase diagram of dense hydrogen is very sensitive to errors in the treatment of electronic correlation. Recently, it has been shown that the choice of the density functional has a large effect on the predicted location of both the liquid-liquid phase transition and the solid insulator-to-metal transition in dense hydrogen. To identify the most accurate functional for dense hydrogen applications, we systematically benchmark some of the most commonly used functionals using quantum Monte Carlo. By considering several measures of functional accuracy, we conclude that the van der Waals and hybrid functionals significantly outperform local density approximation and Perdew-Burke-Ernzerhof. We support these conclusions by analyzing the impact of functional choice on structural optimization in the molecular solid, and on the location of the liquid-liquid phase transition. C1 [Clay, Raymond C., III; McMahon, Jeffrey M.; Ceperley, David M.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Mcminis, Jeremy; Morales, Miguel A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Pierleoni, Carlo] Univ Aquila, Dept Phys & Chem Sci, I-67010 Laquila, Italy. [Pierleoni, Carlo] CNISM UdR Aquila, I-67010 Laquila, Italy. RP Clay, RC (reprint author), Univ Illinois, Dept Phys, Urbana, IL 61801 USA. EM rcclay2@illinois.edu RI Pierleoni, Carlo/D-5519-2016 OI Pierleoni, Carlo/0000-0001-9188-3846 FU U.S. Department of Energy at the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Basic Energy Science (BES); DOE [DE-NA0001789]; Italian Institute of Technology (IIT) under the SEED project [259 SIMBEDD]; PRACE [2011050781] FX M.A.M. and J.M. were supported by the U.S. Department of Energy at the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. M.A.M., J.B.M., R.C., and D.M.C. were supported through the Predictive Theory and Modeling for Materials and Chemical Science program by the Basic Energy Science (BES), DOE. R.C., J.M.M., and D.M.C. were also supported by DOE Grant No. DE-NA0001789. C.P. was supported by the Italian Institute of Technology (IIT) under the SEED project Grant No. 259 SIMBEDD. Computer time was provided by the U.S. DOE INCITE program, Lawrence Livermore National Laboratory through the 7th Institutional Unclassified Computing Grand Challenge program, and PRACE Project No. 2011050781. NR 39 TC 21 Z9 21 U1 1 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 12 PY 2014 VL 89 IS 18 AR 184106 DI 10.1103/PhysRevB.89.184106 PG 11 WC Physics, Condensed Matter SC Physics GA AH1WM UT WOS:000335912400004 ER PT J AU Thomas, JC Millunchick, JM Van der Ven, A Modine, NA AF Thomas, John C. Millunchick, Joanna Mirecki Van der Ven, Anton Modine, Normand A. TI Phase stability analysis of the InAs/GaAs (001) wetting layer from first principles SO PHYSICAL REVIEW B LA English DT Article ID MOLECULAR-BEAM EPITAXY; SURFACE RECONSTRUCTIONS; INGAAS ALLOYS; GAAS(001); GROWTH; INAS; HETEROEPITAXY; SEGREGATION; EVOLUTION; SYSTEMS AB The large atomic-size mismatch between In and Ga and the large lattice-mismatch strain between InAs and GaAs make the InAs/GaAs (001) growth interface a complex alloy system, the understanding of which can enhance control of device synthesis and nanostructure self-assembly. We present a detailed first-principles analysis of the full progression of surface reconstructions observed on the InAs/GaAs(001) wetting layer during early stages of In deposition. We use systematic techniques to identify the most likely surface reconstruction prototypes of the InAs wetting layer on GaAs(001) using density functional theory (DFT) and then develop several cluster expansion Hamiltonians in order to thoroughly explore surface alloy disorder due to species substitution of In, Ga, and As at the surface. We use these results to construct a first principles 0-K surface phase diagram of the InAs wetting layer on GaAs(001) and test the sensitivity of our predicted phase diagram to DFT approximations and convergence errors. We find two alloy configurations of the (4 x 3) structural prototype that are likely ground-state surface reconstructions, and simulated scanning tunneling micrographs (STM) of these reconstructions indicate that they can explain prominent features of experimentally obtained STM of the InAs/GaAs (4 Chi 3) surface. C1 [Thomas, John C.; Millunchick, Joanna Mirecki; Van der Ven, Anton] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. [Van der Ven, Anton] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Modine, Normand A.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Thomas, JC (reprint author), Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. EM johnct@umich.edu; joannamm@umich.edu; avdv@engineering.ucsb.edu; namodin@sandia.gov RI Thomas, John/A-2764-2009 OI Thomas, John/0000-0002-3162-0152 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSF through a CAREER [DMR-0748516]; Department of Defense, Army Research Office [W911NF-12-1-0338] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. A. Van der Ven gratefully acknowledges financial support from NSF through a CAREER award, No. DMR-0748516. J.M. Millunchick gratefully acknowledges Chakrapani Varanasi and the support of the Department of Defense, Army Research Office via the Grant No. W911NF-12-1-0338. NR 43 TC 1 Z9 1 U1 2 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 12 PY 2014 VL 89 IS 20 AR 205306 DI 10.1103/PhysRevB.89.205306 PG 9 WC Physics, Condensed Matter SC Physics GA AH1XM UT WOS:000335915100008 ER PT J AU Yang, SX Haase, P Terletska, H Meng, ZY Pruschke, T Moreno, J Jarrell, M AF Yang, S. -X. Haase, P. Terletska, H. Meng, Z. Y. Pruschke, T. Moreno, J. Jarrell, M. TI Dual-fermion approach to interacting disordered fermion systems SO PHYSICAL REVIEW B LA English DT Article ID OFF-DIAGONAL DISORDER; COHERENT POTENTIAL APPROXIMATION; RANDOM SUBSTITUTIONAL ALLOYS; CORRELATED ELECTRON-SYSTEMS; DIMENSIONS; LATTICE AB We generalize the recently introduced dual-fermion (DF) formalism for disordered fermion systems by including the effect of interactions. For an interacting disordered system the contributions to the full vertex function have to be separated into crossing-asymmetric and crossing-symmetric scattering processes, and addressed differently when constructing the DF diagrams. By applying our approach to the Anderson-Falicov-Kimball model and systematically restoring the nonlocal correlations in the DF lattice calculation, we show a significant improvement over the dynamical mean-field theory and the coherent potential approximation for both one-particle and two-particle quantities. C1 [Yang, S. -X.; Terletska, H.; Meng, Z. Y.; Moreno, J.; Jarrell, M.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Yang, S. -X.; Meng, Z. Y.; Moreno, J.; Jarrell, M.] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Haase, P.; Pruschke, T.] Univ Gottingen, Dept Phys, D-37077 Gottingen, Germany. [Terletska, H.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. RP Yang, SX (reprint author), Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. EM yangphysics@gmail.com RI Meng, Zi Yang/F-5212-2012; Moreno, Juana/D-5882-2012 OI Meng, Zi Yang/0000-0001-9771-7494; FU DOE SciDAC Grant [DE-FC02-10ER25916]; BES CMCSN Grant [DE-AC02-98CH10886]; NSF EPSCoR [EPS-1003897]; NSF [OISE-0952300]; DFG [FOR 1807]; NSF Extreme Science and Engineering Discovery Environment (XSEDE) [DMR100007]; Louisiana Optical Network Initiative; HPC@LSU computing; Gesellschaft fur wissenschaftliche Datenverarbeitung Gottingen (GWDG); GoeGrid project FX This work is supported by DOE SciDAC Grant DE-FC02-10ER25916 (S.Y. and M.J.) and BES CMCSN Grant DE-AC02-98CH10886 (H. T.). Additional support was provided by NSF EPSCoR Cooperative Agreement No. EPS-1003897 (S.Y., H. T., Z.Y.), NSF OISE-0952300 (S.Y., J.M.), and by DFG through research unit FOR 1807 (T. P. and P. H.). Computer support is provided by the NSF Extreme Science and Engineering Discovery Environment (XSEDE) under Grant No. DMR100007, the Louisiana Optical Network Initiative, and HPC@LSU computing, and by the Gesellschaft fur wissenschaftliche Datenverarbeitung Gottingen (GWDG) and the GoeGrid project. NR 43 TC 2 Z9 2 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 12 PY 2014 VL 89 IS 19 AR 195116 DI 10.1103/PhysRevB.89.195116 PG 15 WC Physics, Condensed Matter SC Physics GA AH1XA UT WOS:000335913900002 ER PT J AU Mikaelian, KO AF Mikaelian, Karnig O. TI Solution to Rayleigh-Taylor instabilities: Bubbles, spikes, and their scalings SO PHYSICAL REVIEW E LA English DT Article ID RICHTMYER-MESHKOV INSTABILITIES; NUMERICAL SIMULATIONS; ACCELERATION AB When a fluid pushes on and accelerates a heavier fluid, small perturbations at their interface grow with time and lead to turbulent mixing. The same instability, known as the Rayleigh-Taylor instability, operates when a heavy fluid is supported by a lighter fluid in a gravitational field. It has a particularly deleterious effect on inertial-confinement-fusion implosions and is known to operate over 18 orders of magnitude in dimension. We propose analytic expressions for the bubble and spike amplitudes and mixing widths in the linear, nonlinear, and turbulent regimes. They cover arbitrary density ratios and accelerations that are constant or changing relatively slowly with time. We discuss their scalings and compare them with simulations and experiments. C1 Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Mikaelian, KO (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank G. Dimonte for supplying the experimental data on alphab and alphas. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 27 TC 8 Z9 8 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD MAY 12 PY 2014 VL 89 IS 5 AR 053009 DI 10.1103/PhysRevE.89.053009 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AH1YJ UT WOS:000335917500019 PM 25353882 ER PT J AU Adamson, P Anghel, I Aurisano, A Barr, G Bishai, M Blake, A Bock, GJ Bogert, D Cao, SV Castromonte, CM Cherdack, D Childress, S Coelho, JAB Corwin, L Cronin-Hennessy, D de Jong, JK Devan, AV Devenish, NE Diwan, MV Escobar, CO Evans, JJ Falk, E Feldman, GJ Frohne, MV Gallagher, HR Gomes, RA Goodman, MC Gouffon, P Graf, N Gran, R Grzelak, K Habig, A Hahn, SR Hartnell, J Hatcher, R Himmel, A Holin, A Huang, J Hylen, J Irwin, GM Isvan, Z James, C Jensen, D Kafka, T Kasahara, SMS Koizumi, G Kordosky, M Kreymer, A Lang, K Ling, J Litchfield, PJ Lucas, P Mann, WA Marshak, ML Mayer, N McGivern, C Medeiros, MM Mehdiyev, R Meier, JR Messier, MD Michael, DG Miller, WH Mishra, SR Sher, SM Moore, CD Mualem, L Musser, J Naples, D Nelson, JK Newman, HB Nichol, RJ Nowak, JA O'Connor, J Orchanian, M Pahlka, RB Paley, J Patterson, RB Pawloski, G Perch, A Phan-Budd, S Plunkett, RK Poonthottathil, N Qiu, X Radovic, A Rebel, B Rosenfeld, C Rubin, HA Sanchez, MC Schneps, J Schreckenberger, A Schreiner, P Sharma, R Sousa, A Tagg, N Talaga, RL Thomas, J Thomson, MA Tian, X Timmons, A Tognini, SC Toner, R Torretta, D Tzanakos, G Urheim, J Vahle, P Viren, B Weber, A Webb, RC White, C Whitehead, L Whitehead, LH Wojcicki, SG Zwaska, R AF Adamson, P. Anghel, I. Aurisano, A. Barr, G. Bishai, M. Blake, A. Bock, G. J. Bogert, D. Cao, S. V. Castromonte, C. M. Cherdack, D. Childress, S. Coelho, J. A. B. Corwin, L. Cronin-Hennessy, D. de Jong, J. K. Devan, A. V. Devenish, N. E. Diwan, M. V. Escobar, C. O. Evans, J. J. Falk, E. Feldman, G. J. Frohne, M. V. Gallagher, H. R. Gomes, R. A. Goodman, M. C. Gouffon, P. Graf, N. Gran, R. Grzelak, K. Habig, A. Hahn, S. R. Hartnell, J. Hatcher, R. Himmel, A. Holin, A. Huang, J. Hylen, J. Irwin, G. M. Isvan, Z. James, C. Jensen, D. Kafka, T. Kasahara, S. M. S. Koizumi, G. Kordosky, M. Kreymer, A. Lang, K. Ling, J. Litchfield, P. J. Lucas, P. Mann, W. A. Marshak, M. L. Mayer, N. McGivern, C. Medeiros, M. M. Mehdiyev, R. Meier, J. R. Messier, M. D. Michael, D. G. Miller, W. H. Mishra, S. R. Sher, S. Moed Moore, C. D. Mualem, L. Musser, J. Naples, D. Nelson, J. K. Newman, H. B. Nichol, R. J. Nowak, J. A. O'Connor, J. Orchanian, M. Pahlka, R. B. Paley, J. Patterson, R. B. Pawloski, G. Perch, A. Phan-Budd, S. Plunkett, R. K. Poonthottathil, N. Qiu, X. Radovic, A. Rebel, B. Rosenfeld, C. Rubin, H. A. Sanchez, M. C. Schneps, J. Schreckenberger, A. Schreiner, P. Sharma, R. Sousa, A. Tagg, N. Talaga, R. L. Thomas, J. Thomson, M. A. Tian, X. Timmons, A. Tognini, S. C. Toner, R. Torretta, D. Tzanakos, G. Urheim, J. Vahle, P. Viren, B. Weber, A. Webb, R. C. White, C. Whitehead, L. Whitehead, L. H. Wojcicki, S. G. Zwaska, R. CA MINOS Collaboration TI Combined Analysis of nu(mu) Disappearance and nu(mu) -> nu(e) Appearance in MINOS Using Accelerator and Atmospheric Neutrinos SO PHYSICAL REVIEW LETTERS LA English DT Article ID MASS HIERARCHY; OSCILLATIONS; MATTER; MODEL AB We report on a new analysis of neutrino oscillations in MINOS using the complete set of accelerator and atmospheric data. The analysis combines the nu(mu) disappearance and nu(e) appearance data using the three-flavor formalism. We measure vertical bar Delta m(32)(2)vertical bar = [2.28-2.46] x 10(-3) eV(2) (68% C.L.) and sin(2)theta(23) = 0.35-0.65 (90% C.L.) in the normal hierarchy, and vertical bar Delta m(32)(2)vertical bar = [2.32-2.53] x 10(-3) eV(2) (68% C.L.) and sin(2)theta(23) = 0.34-0.67 (90% C.L.) in the inverted hierarchy. The data also constrain delta(CP), the theta(23) octant degeneracy and the mass hierarchy; we disfavor 36% (11%) of this three-parameter space at 68% (90%) C.L. C1 [Anghel, I.; Goodman, M. C.; Phan-Budd, S.; Sanchez, M. C.; Schreiner, P.; Talaga, R. L.] Argonne Natl Lab, Argonne, IL 60439 USA. [Tzanakos, G.] Univ Athens, Dept Phys, GR-15771 Athens, Greece. [Bishai, M.; Diwan, M. V.; Isvan, Z.; Ling, J.; Viren, B.; Whitehead, L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Himmel, A.; Michael, D. G.; Mualem, L.; Newman, H. B.; Orchanian, M.; Patterson, R. B.] CALTECH, Lauritsen Lab, Pasadena, CA 91125 USA. [Blake, A.; Thomson, M. A.; Toner, R.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Coelho, J. A. B.; Escobar, C. O.] Univ Estadual Campinas, IFGW UNICAMP, BR-13083970 Campinas, SP, Brazil. [Aurisano, A.; Sousa, A.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Adamson, P.; Bock, G. J.; Bogert, D.; Cherdack, D.; Childress, S.; Hahn, S. R.; Hylen, J.; James, C.; Jensen, D.; Koizumi, G.; Kreymer, A.; Lucas, P.; Sher, S. Moed; Moore, C. D.; Pahlka, R. B.; Plunkett, R. K.; Poonthottathil, N.; Rebel, B.; Sharma, R.; Torretta, D.; Zwaska, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Castromonte, C. M.; Gomes, R. A.; Medeiros, M. M.; Tognini, S. C.] Univ Fed Goias, Inst Fis, BR-74001970 Goiania, Go, Brazil. [Feldman, G. J.; Sousa, A.; Toner, R.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Frohne, M. V.] Coll Holy Cross, Notre Dame, IN 46556 USA. [Whitehead, L.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Graf, N.; Rubin, H. A.; White, C.] IIT, Dept Phys, Chicago, IL 60616 USA. [Corwin, L.; Mayer, N.; Messier, M. D.; Musser, J.; Urheim, J.] Indiana Univ, Bloomington, IN 47405 USA. [Anghel, I.; Sanchez, M. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Holin, A.; Nichol, R. J.; O'Connor, J.; Perch, A.; Radovic, A.; Thomas, J.; Toner, R.; Whitehead, L. H.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Evans, J. J.; Timmons, A.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Cronin-Hennessy, D.; Kasahara, S. M. S.; Litchfield, P. J.; Marshak, M. L.; Meier, J. R.; Miller, W. H.; Nowak, J. A.; Pawloski, G.; Schreckenberger, A.] Univ Minnesota, Minneapolis, MN 55455 USA. [Gran, R.; Habig, A.] Univ Minnesota, Dept Phys, Duluth, MN 55812 USA. [Tagg, N.] Otterbein Coll, Westerville, OH 43081 USA. [Barr, G.; de Jong, J. K.; Weber, A.] Univ Oxford, Subdept Particle Phys, Oxford OX1 3RH, England. [Graf, N.; Isvan, Z.; McGivern, C.; Naples, D.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Litchfield, P. J.; Weber, A.] Sci & Technol Facil Council, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Gouffon, P.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. [Mishra, S. R.; Rosenfeld, C.; Tian, X.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Irwin, G. M.; Pawloski, G.; Qiu, X.; Wojcicki, S. G.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Devenish, N. E.; Falk, E.; Hartnell, J.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Webb, R. C.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Cao, S. V.; Huang, J.; Lang, K.; Mehdiyev, R.; Schreckenberger, A.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Cherdack, D.; Coelho, J. A. B.; Gallagher, H. R.; Kafka, T.; Mann, W. A.; Mayer, N.; Schneps, J.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Grzelak, K.] Univ Warsaw, Dept Phys, PL-00681 Warsaw, Poland. [Devan, A. V.; Kordosky, M.; Nelson, J. K.; Radovic, A.; Vahle, P.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. RP Adamson, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RI Gomes, Ricardo/B-6899-2008; Coelho, Joao/D-3546-2013; Castromonte Flores, Cesar Manuel/O-6177-2014; Evans, Justin/P-4981-2014; Gouffon, Philippe/I-4549-2012; Nowak, Jaroslaw/P-2502-2016; Ling, Jiajie/I-9173-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Gomes, Ricardo/0000-0003-0278-4876; Castromonte Flores, Cesar Manuel/0000-0002-9559-3704; Evans, Justin/0000-0003-4697-3337; Gouffon, Philippe/0000-0001-7511-4115; Nowak, Jaroslaw/0000-0001-8637-5433; Ling, Jiajie/0000-0003-2982-0670; FU U.S. DOE; United Kingdom STFC; U.S. NSF; State and University of Minnesota; Brazil FAPESP; Brazil CNPq; Brazil CAPES FX This work was supported by the U.S. DOE, the United Kingdom STFC, the U.S. NSF, the State and University of Minnesota, Brazil's FAPESP, CNPq and CAPES. We are grateful to the Minnesota Department of Natural Resources and the personnel of the Soudan Laboratory and Fermilab for their contributions to the experiment. We thank the Texas Advanced Computing Center at The University of Texas at Austin for the provision of computing resources. NR 36 TC 71 Z9 71 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 12 PY 2014 VL 112 IS 19 AR 191801 DI 10.1103/PhysRevLett.112.191801 PG 6 WC Physics, Multidisciplinary SC Physics GA AH1YX UT WOS:000335918900004 PM 24877929 ER PT J AU Dodelson, S AF Dodelson, Scott TI How Much Can We Learn about the Physics of Inflation? SO PHYSICAL REVIEW LETTERS LA English DT Article ID GRAVITY-WAVES; UNIVERSE; POLARIZATION; COSMOLOGY; SPECTRUM; FLATNESS; HORIZON AB The recent BICEP2 measurement of B modes in the polarization of the cosmic microwave background suggests that inflation was driven by a field at an energy scale of 2 x 10(16) GeV. I explore the potential of upcoming cosmic microwave radiation polarization experiments to further constrain the physics underlying inflation. If the signal is confirmed, then two sets of experiments covering a large area will shed light on inflation. Low-resolution measurements can pin down the tensor to scalar ratio at the percent level, thereby distinguishing models from one another. A high angular resolution experiment will be necessary to measure the tilt of the tensor spectrum, testing the consistency relation that relates the tilt to the amplitude. C1 [Dodelson, Scott] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Dodelson, Scott] Univ Chicago, Enrico Fermi Inst, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Dodelson, Scott] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. RP Dodelson, S (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. FU U.S. Department of Energy [DE-FG02-95ER40896] FX I am grateful to Tom Crawford, Matthew Dodelson, Eiichiro Komatsu, Marilena Loverde, Chris Sheehy, and Anze Slosar for useful suggestions and conversations. This work is supported by the U.S. Department of Energy, including Grant No. DE-FG02-95ER40896. NR 37 TC 24 Z9 24 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 12 PY 2014 VL 112 IS 19 AR 191301 DI 10.1103/PhysRevLett.112.191301 PG 4 WC Physics, Multidisciplinary SC Physics GA AH1YX UT WOS:000335918900002 PM 24877925 ER PT J AU Rygg, JR Jones, OS Field, JE Barrios, MA Benedetti, LR Collins, GW Eder, DC Edwards, MJ Kline, JL Kroll, JJ Landen, OL Ma, T Pak, A Peterson, JL Raman, K Town, RPJ Bradley, DK AF Rygg, J. R. Jones, O. S. Field, J. E. Barrios, M. A. Benedetti, L. R. Collins, G. W. Eder, D. C. Edwards, M. J. Kline, J. L. Kroll, J. J. Landen, O. L. Ma, T. Pak, A. Peterson, J. L. Raman, K. Town, R. P. J. Bradley, D. K. TI 2D X-Ray Radiography of Imploding Capsules at the National Ignition Facility SO PHYSICAL REVIEW LETTERS LA English DT Article ID INERTIAL CONFINEMENT FUSION; NOVA HOHLRAUMS; TARGETS; SYMMETRY; DRIVE AB First measurements of the in-flight shape of imploding inertial confinement fusion (ICF) capsules at the National Ignition Facility (NIF) were obtained by using two-dimensional x-ray radiography. The sequence of area-backlit, time-gated pinhole images is analyzed for implosion velocity, low-mode shape and density asymmetries, and the absolute offset and center-of-mass velocity of the capsule shell. The in-flight shell is often observed to be asymmetric even when the concomitant core self-emission is round. A similar to 15 mu m shell asymmetry amplitude of the Y-40 spherical harmonic mode was observed for standard NIF ICF hohlraums at a shell radius of similar to 200 mu m (capsule at similar to 5x radial compression). This asymmetry is mitigated by a similar to 10% increase in the hohlraum length. C1 [Rygg, J. R.; Jones, O. S.; Field, J. E.; Barrios, M. A.; Benedetti, L. R.; Collins, G. W.; Eder, D. C.; Edwards, M. J.; Kroll, J. J.; Landen, O. L.; Ma, T.; Pak, A.; Peterson, J. L.; Raman, K.; Town, R. P. J.; Bradley, D. K.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Kline, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Rygg, JR (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RI Ma, Tammy/F-3133-2013; OI Ma, Tammy/0000-0002-6657-9604; Kline, John/0000-0002-2271-9919 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors thank the engineering, target fabrication, and operations teams at the National Ignition Facility who made these experiments possible. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 25 TC 55 Z9 55 U1 5 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 12 PY 2014 VL 112 IS 19 AR 195001 DI 10.1103/PhysRevLett.112.195001 PG 5 WC Physics, Multidisciplinary SC Physics GA AH1YX UT WOS:000335918900006 PM 24877944 ER PT J AU Wu, C Cheng, Q Wu, KB Wu, G Li, Q AF Wu, Can Cheng, Qin Wu, Kangbing Wu, Gang Li, Qing TI Graphene prepared by one-pot solvent exfoliation as a highly sensitive platform for electrochemical sensing SO ANALYTICA CHIMICA ACTA LA English DT Article DE Graphene; Solvent exfoliation; Electrochemical sensing; Analytical platform ID GLASSY-CARBON ELECTRODE; LIQUID-PHASE EXFOLIATION; OXIDE MODIFIED ELECTRODE; FILM-MODIFIED ELECTRODE; URIC-ACID; ASCORBIC-ACID; SUNSET YELLOW; BISPHENOL-A; PASTE ELECTRODE; VOLTAMMETRIC SENSOR AB Graphene was easily obtained via one-step ultrasonic exfoliation of graphite powder in N-methyl-2-pyrrolidone. Scanning electron microscopy, transmission electron microscopy, Raman and particle size measurements indicated that the exfoliation efficiency and the amount of produced graphene increased with ultrasonic time. The electrochemical properties and analytical applications of the resulting graphene were systematically studied. Compared with the predominantly-used reduced graphene oxides, the obtained graphene by one-step solvent exfoliation greatly enhanced the oxidation signals of various analytes, such as ascorbic acid (AA), dopamine (DA), uric acid (UA), xanthine (XA), hypoxanthine (HXA), bisphenol A (BPA), ponceau 4R, and sunset yellow. The detection limits of AA, DA, UA, XA, HXA, BPA, ponceau 4R, and sunset yellow were evaluated to be 0.8 mu M, 7.5 nM, 2.5 nM, 4 nM, 10 nM, 20 nM, 2 nM, and 1 nM, which are much lower than the reported values. Thus, the prepared graphene via solvent exfoliation strategy displays strong signal amplification ability and holds great promise in constructing a universal and sensitive electrochemical sensing platform. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wu, Can; Cheng, Qin; Wu, Kangbing] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Key Lab Large Format Battery Mat & Syst, Minist Educ, Wuhan 430074, Peoples R China. [Wu, Gang; Li, Qing] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Wu, KB (reprint author), Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Key Lab Large Format Battery Mat & Syst, Minist Educ, Wuhan 430074, Peoples R China. EM kbwu@hust.edu.cn; qing_li_2@brown.edu RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X FU National Natural Science Foundation of China [21375041, 61071052]; National Basic Research Program of China [2009CB320300]; Program for New Century Excellent Talents in University [NCET-11-0187] FX This work was supported by the National Natural Science Foundation of China (Nos. 21375041 and 61071052), the National Basic Research Program of China (973 Program, No. 2009CB320300), and the Program for New Century Excellent Talents in University (NCET-11-0187). The Center of Analysis and Testing of Huazhong University of Science and Technology was acknowledged for its help in the Raman and particle size measurements. The Center for Nanoscale Characterization and Devices of Wuhan National Laboratory for Optoelectronics (WNLO) was also thanked for its help in the SEM and TEM observation. NR 53 TC 23 Z9 24 U1 13 U2 153 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0003-2670 EI 1873-4324 J9 ANAL CHIM ACTA JI Anal. Chim. Acta PD MAY 12 PY 2014 VL 825 BP 26 EP 33 DI 10.1016/j.aca.2014.03.036 PG 8 WC Chemistry, Analytical SC Chemistry GA AG5ES UT WOS:000335442700002 PM 24767147 ER PT J AU Heikoop, JM Johnson, TM Birdsell, KH Longmire, P Hickmott, DD Jacobs, EP Broxton, DE Katzman, D Vesselinov, VV Ding, M Vaniman, DT Reneau, SL Goering, TJ Glessner, J Basu, A AF Heikoop, Jeffrey M. Johnson, Thomas M. Birdsell, Kay H. Longmire, Patrick Hickmott, Donald D. Jacobs, Elaine P. Broxton, David E. Katzman, Danny Vesselinov, Velimir V. Ding, Mei Vaniman, David T. Reneau, Steven L. Goering, Tim J. Glessner, Justin Basu, Anirban TI Isotopic evidence for reduction of anthropogenic hexavalent chromium in Los Alamos National Laboratory groundwater SO CHEMICAL GEOLOGY LA English DT Article DE Chromium; Contamination; Chromium isotopes; Reduction; Groundwater ID MASS-DEPENDENT FRACTIONATION; CR STABLE-ISOTOPES; CR(VI) REDUCTION; PAJARITO PLATEAU; MOJAVE DESERT; NEW-MEXICO; TRANSPORT; FATE; ENVIRONMENTS; REMEDIATION AB Reduction of toxic Cr(VI) to less toxic Cr(III) is an important process for attenuating Cr(VI) transport in groundwater. This process results in immobilization of chromium as Cr(III) and effectively decreases the overall mobility of the chromium inventory. During both abiotic and biotic reduction of Cr(VI) to Cr(III), a kinetic isotope effect occurs in which the lighter isotope, Cr-52, reacts preferentially, leaving the remaining dissolved Cr(VI) enriched in the heavier isotope, Cr-53. Cr isotopes have proven to be a useful tool for estimating the magnitude of Cr(VI) reduction and for determining where in a hydrologic system reduction is occurring. In this paper, we discuss patterns of reduction in perched-intermediate and regional aquifer systems contaminated with Cr(VI) related to historical use of potassium dichromate as an anticorrosion agent in cooling towers at a power plant at the Los Alamos National Laboratory in northern New Mexico. We utilize Cr isotopes to assess the relative effects of mixing and reduction on measured delta Cr-53 in groundwater, with an emphasis on where in the system reduction occurs. Chromium isotope measurements provide strong evidence for reduction of Cr(VI) in vadose zone basalts. (C) 2014 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY-NC-ND license C1 [Heikoop, Jeffrey M.; Birdsell, Kay H.; Longmire, Patrick; Hickmott, Donald D.; Jacobs, Elaine P.; Broxton, David E.; Vesselinov, Velimir V.; Ding, Mei; Vaniman, David T.; Reneau, Steven L.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Johnson, Thomas M.; Glessner, Justin; Basu, Anirban] Univ Illinois, Dept Geol, Environm Isotope Geochem Grp, Urbana, IL 61801 USA. [Katzman, Danny; Goering, Tim J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Heikoop, JM (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. EM jheikoop@lanl.gov RI Heikoop, Jeffrey/C-1163-2011; Vesselinov, Velimir/P-4724-2016; Basu, Anirban/P-5048-2016; OI Vesselinov, Velimir/0000-0002-6222-0530; Basu, Anirban/0000-0002-4905-9156; Heikoop, Jeffrey/0000-0001-7648-3385 FU U.S. Department of Energy's investigation of legacy contamination at Los Alamos National Laboratory FX This work was funded as part of the U. S. Department of Energy's investigation of legacy contamination at Los Alamos National Laboratory. This manuscript benefited significantly from the input of two anonymous reviewers. NR 38 TC 4 Z9 4 U1 3 U2 50 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD MAY 12 PY 2014 VL 373 BP 1 EP 9 DI 10.1016/j.chemgeo.2014.02.022 PG 9 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AF5EQ UT WOS:000334737200001 ER PT J AU Xiong, YL AF Xiong, Yongliang TI A Pitzer model for the Na-Al(OH)(4)-Cl-OH system and solubility of boehmite (AlOOH) to high ionic strength and to 250 degrees C SO CHEMICAL GEOLOGY LA English DT Article DE Bayer process; Aluminum speciation at elevated temperatures; Nuclear waste management; Borosilicates; Bentonite; Sodalite ID HIGH-TEMPERATURE SOLUBILITY; SODIUM ALUMINATE SOLUTIONS; IN-SITU MEASUREMENTS; THERMODYNAMIC PROPERTIES; HYDROTHERMAL SOLUTIONS; DEGREES-C; ACTINIDE COMPLEXATION; ELEVATED-TEMPERATURES; OSMOTIC COEFFICIENTS; CHLORIDE SOLUTIONS AB In this study, a Pitzer model for the Na-Cl-OH-Al(OH) 4 system, and solubility of boehmite (AlOOH) to high ionic strengths, and to high temperatures up to 250 C, has been developed by evaluating equilibrium quotients concerning boehmite in NaCl solutions to 5.0 mol . kg-(1), and boehmite solubility data in NaOH solutions to similar to 13 mol. kg(-1). This model is validated by comparing model-predicted solubilities with solubility data of boehmite in NaOH solutions that are independent from the model development. This model is of value to many fields, including accurate modeling geochemical behavior of aluminum in hydrothermal solutions with high ionic strengths at high temperatures up to 250 C, extraction of aluminum via the Bayer process from various ores, stability of borosilicate glass, aluminum silicate materials as waste forms for long-lived radio nuclides, and bentonite as engineered barrier, in geological repositories. Based on the model developed in this work, solubility of boehmite can be potentially used as a pH(m) (hydrogen ion concentration on molal scale) sensor/buffer in hydrothermal experiments under neutral to alkaline conditions in NaCl solutions in the absence of silica. This pHm sensor/buffer would enable experimentalists to conduct hydrothermal experiments in a wide range ionic strength under well-controlled pHm conditions. (C) 2014 Elsevier B.V. ll rights reserved. C1 Sandia Natl Labs, Carlsbad Programs Grp, Carlsbad, NM 88220 USA. RP Xiong, YL (reprint author), Sandia Natl Labs, Carlsbad Programs Grp, 4100 Natl Parks Highway, Carlsbad, NM 88220 USA. EM yxiong@sandia.gov FU Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation [DE-AC0494AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U. S. Department of Energy's National Nuclear Security Administration under contract DE-AC0494AL85000. The author would like to thank the journal reviewers, Dr. Dave Wesolowski, and Dr. Pascale Benezeth, for their detailed and insightful reviews, and to thank the journal Editor, Dr. Jeremy Fein, for his review and editorial efforts. NR 59 TC 3 Z9 4 U1 4 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD MAY 12 PY 2014 VL 373 BP 37 EP 49 DI 10.1016/j.chemgeo.2014.02.018 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AF5EQ UT WOS:000334737200004 ER PT J AU Filiz, S Bediz, B Romero, LA Ozdoganlar, OB AF Filiz, Sinan Bediz, Bekir Romero, L. A. Ozdoganlar, O. Burak TI Three dimensional dynamics of pretwisted beams: A spectral-Tchebychev solution SO JOURNAL OF SOUND AND VIBRATION LA English DT Article ID TIMOSHENKO BEAM; NATURAL FREQUENCIES; VIBRATION ANALYSIS; AXIAL VIBRATIONS; MODEL; LOADS; STABILITY; TORSION; DRILLS; TWIST AB This paper presents the application of the spectral-Tchebychev (ST) technique for solution of three-dimensional dynamics of unconstrained pretwisted beams with general cross-section (including both straight and curved cross-sections). In general, the dynamic response of pretwisted beams presents three-dimensional (3D) motions, including coupled bending-bending-torsional-axial motions. As such, accurately solving pretwisted beam dynamics requires a 3D solution approach. In this work, the integral boundary value problem based on the 3D linear elasticity equations is solved numerically using the 3D-ST approach. To simplify evaluation of the volume integrals, the boundaries are simplified by applying two coordinate transformations to render the pretwisted beam with curved cross-section into an equivalent straight beam with rectangular cross-section. Three sample pretwisted beam problems with rectangular, curved, and airfoil cross-sections at different twist rates are solved using the presented approach. In each case, the convergence of the solution is analyzed, and non-dimensional natural frequencies and mode shapes are compared to those from a finite-element (FE) solution. Furthermore, cross-sectional stress and displacements are obtained from the 3D-ST solution. Lastly, the non-dimensional natural frequencies from the 3D-ST and a 1D/2D solutions are compared. It is concluded that the 3D-ST solution can capture the three-dimensional dynamic behavior of pretwisted beam as accurately as an FE solution, but for a fraction of the computational cost. Furthermore, it is shown that 1D/2D solution can lead to significant errors at high twist rates, and thus, the 3D-ST solution should be preferred. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Filiz, Sinan; Bediz, Bekir; Ozdoganlar, O. Burak] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. [Romero, L. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ozdoganlar, OB (reprint author), Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. EM ozdoganlar@cmu.edu OI Bediz, Bekir/0000-0002-7925-8228 FU National Science Foundation Award [CMMI-0928393]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported in part by the National Science Foundation Award No. CMMI-0928393 (Ozdoganlar). The authors would like to acknowledge Sandia National Laboratories for allowing the authors to use the Matlab-based tensor toolbox. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 46 TC 3 Z9 3 U1 3 U2 16 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-460X EI 1095-8568 J9 J SOUND VIB JI J. Sound Vibr. PD MAY 12 PY 2014 VL 333 IS 10 BP 2823 EP 2839 DI 10.1016/j.jsv.2014.01.010 PG 17 WC Acoustics; Engineering, Mechanical; Mechanics SC Acoustics; Engineering; Mechanics GA AD8GM UT WOS:000333504500008 ER PT J AU McChesney, JL Reininger, R Ramanathan, M Benson, C Srajer, G Abbamonte, P Campuzano, JC AF McChesney, J. L. Reininger, R. Ramanathan, M. Benson, C. Srajer, G. Abbamonte, P. Campuzano, J. C. TI The intermediate energy X-ray beamline at the APS SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Beamline; Soft X-ray; VLS-PGM; Electromagnetic quasiperiodic undulator ID SYNCHROTRON-RADIATION; HIGH-RESOLUTION; MONOCHROMATOR; SCATTERING; SYSTEMS; OPTICS AB The optical design of the Intermediate Energy X-ray (IEX) beamline at the APS has been optimized to study emergent phenomena via angle-resolved photoemission spectroscopy (ARPES) and resonant soft X-ray scattering (RSXS). Driven by the scientific requirements of these two techniques the beamline consists of two separate branchlines sharing the same source, heat absorbing optics and monochromator, but each having its own refocusing optics. The ARPES branch is optimized for a very high "resolving power" and a small spot at the sample; whereas, the RSXS branch is designed for high flux and a low beam divergence at the sample. The very high "resolving power" in the ARPES branch is achieved by using a monochromator which consists of a plane mirror and a variable line spacing grating that focuses the beam at all photon energies. A flux higher than 1010 photons/s at a "resolving power" better than 5 x 104 will be available at the sample position of the ARPES beamline on a spot size (FWHM) smaller than 21 x 4 mu m(2) (hor. x ver.) for photon energies between 250 and 1660 eV. A second grating will increase the flux by more than a factor of 10 at a "resolving power" of 10(4). The flux expected at the RSXS branch for energies between 250 eV and 1900 eV is higher than 4 x 10112 photons/s at "resolving power" around 2.5 x 10(3). The expected spot in this branch is sub-millimeter and the beam divergence is less than 0.3 mrad (FWHM). (c) 2014 Elsevier B.V. All rights reserved. C1 [McChesney, J. L.; Reininger, R.; Ramanathan, M.; Benson, C.; Srajer, G.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Abbamonte, P.] Univ Illinois, Dept Phys, Urbana, IL USA. [Campuzano, J. C.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Campuzano, J. C.] Univ Illinois, Dept Phys, Chicago, IL 60680 USA. RP McChesney, JL (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM jmcchesn@aps.anl.gov FU National Science Foundation [DMR-0703406]; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; DOE Materials Sciences and Engineering Division [DE-FG02-06ER46285] FX This material is based upon work supported by National Science Foundation under Grant no. DMR-0703406. Work at Argonne National Laboratory is supported by the U.S. Department of Energy, Office of Science, under Contract no. DE-AC02-06CH11357. P.A.'s effort on this project was supported by the DOE Materials Sciences and Engineering Division Grant no. DE-FG02-06ER46285. We thank Y. Jaski for the FEA calculations. NR 28 TC 0 Z9 0 U1 3 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 11 PY 2014 VL 746 BP 98 EP 105 DI 10.1016/j.nima.2014.01.068 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AE6BS UT WOS:000334073900013 ER PT J AU Sheridan, LB Yates, VM Benson, DM Stickney, JL Robinson, DB AF Sheridan, Leah B. Yates, Veronica M. Benson, David M. Stickney, John L. Robinson, David B. TI Hydrogen sorption properties of bare and Rh-modified Pd nanofilms grown via surface limited redox replacement reactions SO ELECTROCHIMICA ACTA LA English DT Article; Proceedings Paper CT 13th Topical Meeting of the International-Society-of-Electrochemistry (ISE) - Advances in Electrochemical Materials Science and Manufacturing CY APR 07-11, 2013 CL Council Sci & Ind Res, Pretoria, SOUTH AFRICA SP Univ Western, Dept Sci & Technol, Hydrogen S Africa, Maccor Inc, Natl Res Fdn, Technol Innovat Agcy, DropSens S L, Elsevier, Electrochem Soc, Sasol, Amer Elements, Metrohm Autolab B V, MinTEK, Rhodes Univ HO Council Sci & Ind Res DE E-ALD; SLRR; Palladium; electrodeposition; Rhodium ID ATOMIC LAYER DEPOSITION; ELECTROCHEMICAL-BEHAVIOR; E-ALD; ABSORPTION REACTION; ELECTRODE SURFACES; CYCLIC VOLTAMMETRY; THIN-FILMS; EC-ALE; PALLADIUM; RHODIUM AB Pd nanofilms were grown using electrochemical atomic layer deposition (E-ALD) and used as a platform for investigations into changes in hydrogen absorption/desorption kinetics as a function of the coverage of Rh. Surface limited redox replacement (SLRR) reactions were used to form Pd atomic layers. That is, Pd atomic layers were grown on polycrystalline Au by first depositing a sacrificial Cu atomic layer using underpotential deposition (UPD), and then exchanging it for PdCl42- ions at open circuit potential (OCP). That cycle was then repeated 15 times to form one of the Pd nanofilms used in this study. Rh was deposited on the 15 cycle Pd films from a RhCl63- solution at constant potential or using an E-ALD procedure, similar to that employed to form the Pd nanofilms. Cyclic voltammetry (CV) of the Pd films modified with various coverages of Rh were compared with unmodified Pd nanofilms. The resulting CVs indicated that the presence of Rh enhanced the rates of hydrogen absorption and desorption into and out of the underlying Pd nanofilm. Rh overlayers formed at 0 V for 60s produced the greatest kinetic enhancement. Two possible explanations for the observed behavior are proposed and discussed. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Sheridan, Leah B.; Yates, Veronica M.; Benson, David M.; Stickney, John L.] Univ Georgia, Dept Chem, Athens, GA 30602 USA. [Robinson, David B.] Sandia Natl Labs, Energy Nanomat Dept, Livermore, CA 94550 USA. RP Stickney, JL (reprint author), Univ Georgia, Dept Chem, Athens, GA 30602 USA. EM Stickney@uga.edu NR 58 TC 7 Z9 7 U1 4 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD MAY 10 PY 2014 VL 128 SI SI BP 400 EP 405 DI 10.1016/j.electacta.2013.10.096 PG 6 WC Electrochemistry SC Electrochemistry GA AH5RC UT WOS:000336187600050 ER PT J AU Griest, K Cieplak, AM Lehner, MJ AF Griest, Kim Cieplak, Agnieszka M. Lehner, Matthew J. TI EXPERIMENTAL LIMITS ON PRIMORDIAL BLACK HOLE DARK MATTER FROM THE FIRST 2 YR OF KEPLER DATA SO ASTROPHYSICAL JOURNAL LA English DT Article DE dark matter; gravitational lensing: micro; stars: black holes ID MACHO PROJECT LIMITS; GALACTIC HALO; MICROLENSING EVENTS; MAGELLANIC CLOUDS; PARTICLE; SCIENCE; MISSION; SEARCH; STARS AB We present our analysis on new limits of the dark matter (DM) halo consisting of primordial black holes (PBHs) or massive compact halo objects. We present a search of the first two yr of publicly available Kepler mission data for potential signatures of gravitational microlensing caused by these objects as well as an extensive analysis of the astrophysical sources of background error. These include variable stars, flare events, and comets or asteroids that are moving through the Kepler field. We discuss the potential of detecting comets using the Kepler light curves, presenting measurements of two known comets and one unidentified object, most likely an asteroid or comet. After removing the background events with statistical cuts, we find no microlensing candidates. We therefore present our Monte Carlo efficiency calculation in order to constrain the PBH DM with masses in the range of 2 x 10(-9)M(circle dot) to 10(-7)M(circle dot). We find that PBHs in this mass range cannot make up the entirety of the DM, thus closing a full order of magnitude in the allowed mass range for PBH DM. C1 [Griest, Kim; Cieplak, Agnieszka M.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Cieplak, Agnieszka M.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Lehner, Matthew J.] Acad Sinica, Inst Astron & Astrophys, Taipei 106, Taiwan. [Lehner, Matthew J.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. RP Griest, K (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. OI Lehner, Matthew/0000-0003-4077-0985 FU US Department of Energy [DE-FG03-97ER40546, DESC0009919]; National Science Foundation Graduate Research Fellowship [DGE0707423]; NASA [NAS5-26555]; NASA Office of Space Science [NNX09AF08G] FX K.G. and A.M.C. were supported in part by the US Department of Energy under grants DE-FG03-97ER40546 and DESC0009919. A.M.C. was supported in part by the National Science Foundation Graduate Research Fellowship under grant number DGE0707423. Some of the data presented in this paper were obtained from the Multimission Archive at the Space Telescope Science Institute (MAST). STScI is operated by the Association of Universities for Research in Astronomy, Inc., under NASA contract NAS5-26555. Support for MAST for non-HST data is provided by the NASA Office of Space Science via grant NNX09AF08G and by other grants and contracts. NR 40 TC 6 Z9 7 U1 1 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2014 VL 786 IS 2 AR 158 DI 10.1088/0004-637X/786/2/158 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH1MI UT WOS:000335884500081 ER PT J AU Kaspi, VM Archibald, RF Bhalerao, V Dufour, F Gotthelf, EV An, HJ Bachetti, M Beloborodov, AM Boggs, SE Christensen, FE Craig, WW Grefenstette, BW Hailey, CJ Harrison, FA Kennea, JA Kouveliotou, C Madsen, KK Mori, K Markwardt, CB Stern, D Vogel, JK Zhang, WW AF Kaspi, Victoria M. Archibald, Robert F. Bhalerao, Varun Dufour, Francois Gotthelf, Eric V. An, Hongjun Bachetti, Matteo Beloborodov, Andrei M. Boggs, Steven E. Christensen, Finn E. Craig, William W. Grefenstette, Brian W. Hailey, Charles J. Harrison, Fiona A. Kennea, Jamie A. Kouveliotou, Chryssa Madsen, Kristin K. Mori, Kaya Markwardt, Craig B. Stern, Daniel Vogel, Julia K. Zhang, William W. TI TIMING AND FLUX EVOLUTION OF THE GALACTIC CENTER MAGNETAR SGR J1745-2900 SO ASTROPHYSICAL JOURNAL LA English DT Article DE Galaxy: center; pulsars: general; stars: magnetic field; stars: neutron; X-rays: stars ID SOFT GAMMA REPEATER; RAY PULSAR 1E-1048.1-5937; LARGE TORQUE VARIATIONS; SAGITTARIUS A-ASTERISK; X-RAY; NEUTRON-STARS; 2002 OUTBURST; VORTEX CREEP; VELA PULSAR; 1E 2259+586 AB We present the X-ray timing and spectral evolution of the Galactic Center magnetar SGR J1745-2900 for the first similar to 4 months post-discovery using data obtained with the Nuclear Spectroscopic Telescope Array and Swift observatories. Our timing analysis reveals a large increase in the magnetar spin-down rate by a factor of 2.60 +/- 0.07 over our data span. We further show that the change in spin evolution was likely coincident with a bright X-ray burst observed in 2013 June by Swift, and if so, there was no accompanying discontinuity in the frequency. We find that the source 3-10 keV flux has declined monotonically by a factor of similar to 2 over an 80 day period post-outburst accompanied by a similar to 20% decrease in the source's blackbody temperature, although there is evidence for both flux and kT having leveled off. We argue that the torque variations are likely to be magnetospheric in nature and will dominate over any dynamical signatures of orbital motion around Sgr A*. C1 [Kaspi, Victoria M.; Archibald, Robert F.; Dufour, Francois; An, Hongjun] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Bhalerao, Varun] Interuniv Ctr Astron & Astrophys, Pune 411007, Maharashtra, India. [Gotthelf, Eric V.; Beloborodov, Andrei M.; Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Bachetti, Matteo] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Bachetti, Matteo] CNRS, Inst Rech Astrophys & Planetol, F-31028 Toulouse 4, France. [Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William W.; Vogel, Julia K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grefenstette, Brian W.; Harrison, Fiona A.; Madsen, Kristin K.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Kennea, Jamie A.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Kouveliotou, Chryssa] NASA, Marshall Space Flight Ctr, Astrophys Off, Huntsville, AL 35812 USA. [Markwardt, Craig B.; Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP Kaspi, VM (reprint author), McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. EM vkaspi@physics.mcgill.ca RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bhalerao, Varun/0000-0002-6112-7609; Bachetti, Matteo/0000-0002-4576-9337; An, Hongjun/0000-0002-6389-9012; Madsen, Kristin/0000-0003-1252-4891 FU NASA [NNG08FD60C, NNX-10-AI72G, NNX-13-AI34G, NAS5-00136]; National Aeronautics and Space Administration; NSERC Discovery Grant FX This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software ( NuSTARDAS) jointly developed by the ASI Science Data Center ( ASDC, Italy) and the California Institute of Technology (USA). We acknowledge the use of public data from the Swift data archive. This research has made use of the XRT Data Analysis Software (XRTDAS) developed under the responsibility of the ASI Science Data Center (ASDC), Italy. We thank the Swift SOT team for their work in scheduling. V.M.K. receives support from an NSERC Discovery Grant and Accelerator Supplement, from the Centre de Recherche en Astrophysique du Quebec, an R. Howard Webster Foundation Fellowship from the Canadian Institute forAdvanced Study, the Canada Research Chairs Program and the Lorne Trottier Chair in Astrophysics and Cosmology. R.F.A. receives support from a Walter C. Sumner Memorial Fellowship. A.M.B. was supported by NASA grants NNX-10-AI72G and NNX-13-AI34G. J.A.K. was supported by supported by NASA contract NAS5-00136. J.K.V.'s work was performed under the auspices of the U. S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 51 TC 33 Z9 34 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2014 VL 786 IS 2 AR 84 DI 10.1088/0004-637X/786/2/84 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH1MI UT WOS:000335884500008 ER PT J AU McCully, C Jha, SW Foley, RJ Chornock, R Holtzman, JA Balam, DD Branch, D Filippenko, AV Frieman, J Fynbo, J Galbany, L Ganeshalingam, M Garnavich, PM Graham, ML Hsiao, EY Leloudas, G Leonard, DC Li, WD Riess, AG Sako, M Schneider, DP Silverman, JM Sollerman, J Steele, TN Thomas, RC Wheeler, JC Zheng, C AF McCully, Curtis Jha, Saurabh W. Foley, Ryan J. Chornock, Ryan Holtzman, Jon A. Balam, David D. Branch, David Filippenko, Alexei V. Frieman, Joshua Fynbo, Johan Galbany, Lluis Ganeshalingam, Mohan Garnavich, Peter M. Graham, Melissa L. Hsiao, Eric Y. Leloudas, Giorgos Leonard, Douglas C. Li, Weidong Riess, Adam G. Sako, Masao Schneider, Donald P. Silverman, Jeffrey M. Sollerman, Jesper Steele, Thea N. Thomas, Rollin C. Wheeler, J. Craig Zheng, Chen TI HUBBLE SPACE TELESCOPE AND GROUND-BASED OBSERVATIONS OF THE TYPE Iax SUPERNOVAE SN 2005hk AND SN 2008A SO ASTROPHYSICAL JOURNAL LA English DT Article DE supernovae: general; supernovae: individual (SN 2002cx, SN 2005hk, SN 2008A) ID DELAYED-DETONATION MODEL; LATE-TIME SPECTRA; MASS WHITE-DWARF; LIGHT CURVES; DARK ENERGY; FAINT TYPE; THERMONUCLEAR SUPERNOVAE; FACTORY OBSERVATIONS; NEBULAR SPECTRA; HIPASS CATALOG AB We present Hubble Space Telescope (HST) and ground-based optical and near-infrared observations of SN 2005hk and SN 2008A, typical members of the Type Iax class of supernovae (SNe). Here we focus on late-time observations, where these objects deviate most dramatically from all other SN types. Instead of the dominant nebular emission lines that are observed in other SNe at late phases, spectra of SNe 2005hk and 2008A show lines of Fe II, Ca II, and Fe I more than a year past maximum light, along with narrow [ Fe II] and [ Ca II] emission. We use spectral features to constrain the temperature and density of the ejecta, and find high densities at late times, with n(e) greater than or similar to 10(9) cm(-3). Such high densities should yield enhanced cooling of the ejecta, making these objects good candidates to observe the expected "infrared catastrophe," a generic feature of SN Ia models. However, our HST photometry of SN 2008A does not match the predictions of an infrared catastrophe. Moreover, our HST observations rule out a "complete deflagration" that fully disrupts the white dwarf for these peculiar SNe, showing no evidence for unburned material at late times. Deflagration explosion models that leave behind a bound remnant can match some of the observed properties of SNe Iax, but no published model is consistent with all of our observations of SNe 2005hk and 2008A. C1 [McCully, Curtis; Jha, Saurabh W.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Foley, Ryan J.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Foley, Ryan J.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Chornock, Ryan] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Holtzman, Jon A.] New Mexico State Univ, Dept Astron, Las Cruces, NM 88003 USA. [Balam, David D.] Herzberg Inst Astrophys, Dominion Astrophys Observ, Victoria, BC V9E 2E7, Canada. [Branch, David] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Filippenko, Alexei V.; Silverman, Jeffrey M.; Steele, Thea N.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Frieman, Joshua] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Frieman, Joshua] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Frieman, Joshua] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Fynbo, Johan; Leloudas, Giorgos; Sollerman, Jesper] Univ Copenhagen, Niels Bohr Inst, Dark Cosmol Ctr, DK-2100 Copenhagen O, Denmark. [Galbany, Lluis] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Bellaterra, Barcelona, Spain. [Galbany, Lluis] Inst Super Tecn, Ctr Multidisciplinar Astrofis, P-1049001 Lisbon, Portugal. [Ganeshalingam, Mohan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Garnavich, Peter M.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Graham, Melissa L.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. [Graham, Melissa L.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Graham, Melissa L.; Hsiao, Eric Y.] Las Campanas Observ, Carnegie Observ, Atacama, Chile. [Leloudas, Giorgos] Stockholm Univ, Oskar Klein Ctr, Dept Phys, SE-10691 Stockholm, Sweden. [Leonard, Douglas C.] San Diego State Univ, Dept Astron, San Diego, CA 92182 USA. [Riess, Adam G.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Sako, Masao] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Silverman, Jeffrey M.; Wheeler, J. Craig] Univ Texas Austin, Dept Astron, Austin, TX 78712 USA. [Sollerman, Jesper] Stockholm Univ, Dept Astron, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Thomas, Rollin C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Zheng, Chen] Kavli Inst Particle Astrophys & Cosmol, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Zheng, Chen] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. RP McCully, C (reprint author), Rutgers State Univ, Dept Phys & Astron, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA. EM cmccully@physics.rutgers.edu RI Galbany, Lluis/A-8963-2017; OI Galbany, Lluis/0000-0002-1296-6887; Sollerman, Jesper/0000-0003-1546-6615; McCully, Curtis/0000-0001-5807-7893 FU Rutgers University through NASA/HST [GO-11133.01, GO-11590.01]; NSF Astronomy and Astrophysics Postdoctoral Fellowship [AST-1302771]; NSF [AST-1109801, AST-1211916]; Swedish Research Council [623-2011-7117]; Gary and Cynthia Bengier; Richard and Rhoda Goldman Fund; TABASGO Foundation; NASA/HST [GO-10877, AR-12623]; Space Telescope Science Institute; NASA; Alfred P. Sloan Foundation; Participating Institutions; NSF; U.S. Department of Energy; Japanese Monbukagakusho; Max Planck Society; Higher Education Funding Council for England FX This research at Rutgers University was supported through NASA/HST grants GO-11133.01 and GO-11590.01, along with U. S. Department of Energy (DOE) grant DE-FG02-08ER41562, and National Science Foundation (NSF) CAREER award AST-0847157 to S.W.J., and a G Lambda Lambda NN Fellowship to C.M.J. M. S. is supported by an NSF Astronomy and Astrophysics Postdoctoral Fellowship under award AST-1302771. The research of J.C.W. is supported in part by NSF Grant AST-1109801. G. L. is supported by the Swedish Research Council through grant No. 623-2011-7117. A.V.F. and his group at UC Berkeley are funded by Gary and Cynthia Bengier, the Richard and Rhoda Goldman Fund, NSF grant AST-1211916, the TABASGO Foundation, and NASA/HST grants GO-10877 and AR-12623.; Support for HST programs GO-10877, GO-11133, GO-11590, and AR-12623 was provided by NASA through a grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555.; Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the University of California, the California Institute of Technology, and NASA, made possible by the generous financial support of the W. M. Keck Foundation. The authors recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community, and we are most privileged to have the opportunity to explore the universe from this mountain.; Funding for the SDSS and SDSS-II has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the NSF, the U.S. Department of Energy, NASA, the Japanese Monbukagakusho, the Max Planck Society, and the Higher Education Funding Council for England. The SDSS Web site is http://www.sdss.org/. The SDSS is managed by the Astrophysical Research Consortium for the Participating Institutions. The Participating Institutions are the American Museum of Natural History, Astrophysical Institute Potsdam, University of Basel, University of Cambridge, Case Western Reserve University, University of Chicago, Drexel University, Fermilab, the Institute for Advanced Study, the Japan Participation Group, Johns Hopkins University, the Joint Institute for Nuclear Astrophysics, the Kavli Institute for Particle Astrophysics and Cosmology, the Korean Scientist Group, the Chinese Academy of Sciences (LAMOST), Los Alamos National Laboratory, the Max- Planck-Institute for Astronomy (MPIA), the Max- Planck- Institute for Astrophysics (MPA), New Mexico State University, Ohio State University, University of Pittsburgh, University of Portsmouth, Princeton University, the United States Naval Observatory, and the University of Washington. NR 116 TC 17 Z9 17 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2014 VL 786 IS 2 AR 134 DI 10.1088/0004-637X/786/2/134 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AH1MI UT WOS:000335884500057 ER PT J AU Dreher, A Aranson, IS Kruse, K AF Dreher, A. Aranson, I. S. Kruse, K. TI Spiral actin-polymerization waves can generate amoeboidal cell crawling SO NEW JOURNAL OF PHYSICS LA English DT Article DE cell motility; phase-field approach; actin-polymerization waves ID DIRECTIONAL MOTILITY; SELF-POLARIZATION; CHEMOTAXIS; FRAGMENTS; POLARITY; MODEL; CYTOSKELETON; NEUTROPHILS; MICROSCOPY; PERSISTENT AB Amoeboidal cell crawling on solid substrates is characterized by protrusions that seemingly appear randomly along the cell periphery and drive the cell forward. For many cell types, it is known that the protrusions result from polymerization of the actin cytoskeleton. However, little is known about how the formation of protrusions is triggered and whether the appearance of subsequent protrusions is coordinated. Recently, the spontaneous formation of actin-polymerization waves was observed. These waves have been proposed to orchestrate the cytoskeletal dynamics during cell crawling. Here, we study the impact of cytoskeletal polymerization waves on cell migration using a phase-field approach. In addition to directionally moving cells, we find states reminiscent of amoeboidal cell crawling. In this framework, new protrusions are seen to emerge from a nucleation process, generating spiral actin waves in the cell interior. Nucleation of new spirals does not require noise, but occurs in a state that is apparently displaying spatio-temporal chaos. C1 [Dreher, A.; Kruse, K.] Univ Saarland, D-66041 Saarbrucken, Germany. [Aranson, I. S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Dreher, A (reprint author), Univ Saarland, Postfach 151150, D-66041 Saarbrucken, Germany. EM k.kruse@physik.uni-saarland.de FU US DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering; DFG [KR3430/1]; Graduate School 1276; [SFB 1027] FX AD and KK thank the Materials Theory Institute of Argonne National Laboratory, and ISA and KK thank the Isaac Newton Institute, Cambridge, UK, where part of the work was accomplished, for the kind hospitality. The research of ISA was supported by the US DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering. The work of KK and AD was funded by the DFG through KR3430/1, the Graduate School 1276, and SFB 1027. NR 52 TC 8 Z9 8 U1 0 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 9 PY 2014 VL 16 AR 055007 DI 10.1088/1367-2630/16/5/055007 PG 18 WC Physics, Multidisciplinary SC Physics GA AL0VD UT WOS:000338844100001 ER PT J AU Brierley, RT Littlewood, PB AF Brierley, R. T. Littlewood, P. B. TI Domain wall fluctuations in ferroelectrics coupled to strain SO PHYSICAL REVIEW B LA English DT Article ID PEROVSKITES; MARTENSITES; BOUNDARIES; 1ST-ORDER; DYNAMICS AB Using a Ginzburg-Landau-Devonshire model that includes the coupling of polarization to strain, we calculate the fluctuation spectra of ferroelectric domain walls. The influence of the strain coupling differs between 180 degrees. and 90 degrees. walls due to the different strain profiles of the two configurations. The finite speed of acoustic phonons, vs, retards the response of the strain to polarization fluctuations, and the results depend on v(s). For v(s) -> infinity, the strain mediates an instantaneous electrostrictive interaction, which is long-range in the 90 degrees. wall case. For finite v(s), acoustic phonons damp the wall excitations, producing a continuum in the spectral function. As v(s) -> 0, a gapped mode emerges, which corresponds to the polarization oscillating in a fixed strain potential. C1 [Brierley, R. T.] Univ Cambridge, Cavendish Lab, TCM, Cambridge CB3 0HE, England. [Littlewood, P. B.] Argonne Natl Lab, Phys Sci & Engn Div, Argonne, IL 60439 USA. [Littlewood, P. B.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Littlewood, P. B.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. RP Brierley, RT (reprint author), Yale Univ, Dept Phys, New Haven, CT 06520 USA. FU Basic Energy Sciences, Office of Science, US Department of Energy [DE-AC02-06CH11357]; Homerton College, Cambridge FX We acknowledge helpful discussions with A. Saxena, T. Lookman, and J. F. Scott. Work at Argonne was supported by Basic Energy Sciences, Office of Science, US Department of Energy, under Contract No. DE-AC02-06CH11357. R.T.B. is supported by Homerton College, Cambridge. NR 33 TC 3 Z9 3 U1 3 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 9 PY 2014 VL 89 IS 18 AR 184104 DI 10.1103/PhysRevB.89.184104 PG 7 WC Physics, Condensed Matter SC Physics GA AH3CV UT WOS:000335999800002 ER PT J AU Kemei, MC Moffitt, SL Darago, LE Seshadri, R Suchomel, MR Shoemaker, DP Page, K Siewenie, J AF Kemei, Moureen C. Moffitt, Stephanie L. Darago, Lucy E. Seshadri, Ram Suchomel, Matthew R. Shoemaker, Daniel P. Page, Katharine Siewenie, Joan TI Structural ground states of (A, A ') Cr2O4(A= Mg, Zn; A ' = Co,Cu) spinel solid solutions: Spin-Jahn-Teller and Jahn-Teller effects SO PHYSICAL REVIEW B LA English DT Article ID CHROMITE; ZNCR2O4; PHASE AB We examine the effect of small amounts of magnetic substituents in the A sites of the frustrated spinels MgCr2O4 and ZnCr2O4. Specifically, we look for the effects of spin and lattice disorder on structural changes accompanying magnetic ordering in these compounds. Substitution of Co2+ on the nonmagnetic Zn2+ site in Zn1-x Co-x Cr2O4 where 0 < x <= 0.2 completely suppresses the spin-Jahn-Teller distortion of ZnCr2O4 although these systems remain frustrated, and magnetic ordering occurs at very low temperatures of T < 20 K. On the other hand, the substitution of Jahn-Teller active Cu2+ for Mg2+ and Zn2+ in Mg1-x Cu-x Cr2O4 and Zn1-x Cu-x Cr2O4 where 0< x <= 0.2 induce Jahn-Teller ordering at temperatures well above the Neel temperatures of these solid solutions, and yet spin interactions remain frustrated with long-range magnetic ordering occurring below 20 K without any further lattice distortion. The Jahn-Teller distorted solid solutions Mg1-x Cu-x Cr2O4 and Zn1-x Cu-x Cr2O4 adopt the orthorhombic Fddd structure of ferrimagnetic CuCr2O4. Total neutron scattering studies of Zn1-x Cu-x Cr2O4 suggest that there are local AO(4) distortions in these Cu2+- containing solid solutions at room temperature and that these distortions become cooperative when average structure distortions occur. Magnetism evolves from compensated antiferromagnetism in MgCr2O4 and ZnCr2O4 to uncompensated antiferromagnetism with substitution of magnetic cations on the nonmagnetic cation sites of these frustrated compounds. The sharp heat capacity anomalies associated with the first-order spin-Jahn-Teller transitions of MgCr2O4 and ZnCr2O4 become broad in Mg1-x Cu-x Cr2O4, Zn1-x Co-x Cr2O4, and Zn1- x Cu (x) Cr2O4 whenx > 0. We present a temperature-composition phase diagram summarizing the structural ground states and magnetic properties of the studied spinel solid solutions. C1 [Kemei, Moureen C.; Moffitt, Stephanie L.; Darago, Lucy E.; Seshadri, Ram] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Kemei, Moureen C.; Moffitt, Stephanie L.; Darago, Lucy E.; Seshadri, Ram] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. [Suchomel, Matthew R.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Shoemaker, Daniel P.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Page, Katharine; Siewenie, Joan] Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA. RP Kemei, MC (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. EM kemei@mrl.ucsb.edu; seshadri@mrl.ucsb.edu; suchomel@aps.anl.gov; dpshoema@illinois.edu; kpage@lanl.gov; siewenie@lanl.gov RI Seshadri, Ram/C-4205-2013; Page, Katharine/C-9726-2009; OI Seshadri, Ram/0000-0001-5858-4027; Page, Katharine/0000-0002-9071-3383; SUCHOMEL, Matthew/0000-0002-9500-5079; Darago, Lucy/0000-0001-7515-5558 FU NSF [DMR 1105301]; Schlumberger Foundation Faculty for the Future fellowship FX This project was supported by the NSF through the Grant No. DMR 1105301. M.C.K. is supported by the Schlumberger Foundation Faculty for the Future fellowship. We acknowledge the use of shared experimental facilities of the Materials Research Laboratory: an NSF MRSEC, supported by NSF Grant No. DMR 1121053. The 11-BM beamline at the Advanced Photon Source is supported by the DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC0206CH11357. This work benefited from the use of NPDF at the Los Alamos Neutron Scattering Center at Los Alamos National Laboratory, funded by DOE Office of Basic Energy Sciences; LANL is operated by Los Alamos National Security LLC under DE-AC52-06NA25396. M. C. K. acknowledges helpful discussions with J.E. Douglas and B. C. Melot. NR 37 TC 10 Z9 10 U1 3 U2 57 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 9 PY 2014 VL 89 IS 17 AR 174410 DI 10.1103/PhysRevB.89.174410 PG 15 WC Physics, Condensed Matter SC Physics GA AH3CQ UT WOS:000335999300002 ER PT J AU Zhou, YZ Haller, EE Chrzan, DC AF Zhou, Yuzhi Haller, E. E. Chrzan, D. C. TI Theoretical Prediction of Magnetism in C-doped TIBr SO PHYSICAL REVIEW B LA English DT Article ID TRANSPORT-PROPERTIES; TLBR; SEMICONDUCTORS; DEFECT AB We predict that C, N, and O dopants in TIBr can display large, localized magnetic moments. Density functional theory based electronic structure calculations show that the moments arise from partial filling of the crystal-field-split localized p states of the dopant atoms. A simple model is introduced to explain the magnitude of the moments. C1 [Zhou, Yuzhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Zhou, YZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. FU U.S. Department of Homeland Security [2009-DN-077-ARI- 026-04]; Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Homeland Security under Grant Award No. 2009-DN-077-ARI- 026-04 and by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 22 TC 0 Z9 0 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 9 PY 2014 VL 89 IS 19 AR 195201 DI 10.1103/PhysRevB.89.195201 PG 5 WC Physics, Condensed Matter SC Physics GA AH3DB UT WOS:000336000400005 ER PT J AU Fobes, D Zaliznyak, IA Xu, ZJ Zhong, RD Gu, GD Tranquada, JM Harriger, L Singh, D Garlea, VO Lumsden, M Winn, B AF Fobes, David Zaliznyak, Igor A. Xu, Zhijun Zhong, Ruidan Gu, Genda Tranquada, John M. Harriger, Leland Singh, Deepak Garlea, V. Ovidiu Lumsden, Mark Winn, Barry TI Ferro-Orbital Ordering Transition in Iron Telluride Fe1+yTe SO PHYSICAL REVIEW LETTERS LA English DT Article ID SUPERCONDUCTIVITY AB Fe1+yTe with y less than or similar to 0.05 exhibits a first-order phase transition on cooling to a state with a lowered structural symmetry, bicollinear antiferromagnetic order, and metallic conductivity, dp/dT > 0. Here, we study samples with y = 0.09(1), where the frustration effects of the interstitial Fe decouple different orders, leading to a sequence of transitions. While the lattice distortion is closely followed by incommensurate magnetic order, the development of bicollinear order and metallic electronic coherence is uniquely associated with a separate hysteretic first-order transition, at a markedly lower temperature, to a phase with dramatically enhanced bond-order wave (BOW) order. The BOW state suggests ferro-orbital ordering, where electronic delocalization in ferromagnetic zigzag chains decreases local spin and results in metallic transport. C1 [Fobes, David; Zaliznyak, Igor A.; Xu, Zhijun; Zhong, Ruidan; Gu, Genda; Tranquada, John M.] Brookhaven Natl Lab, CMPMSD, Upton, NY 11973 USA. [Harriger, Leland; Singh, Deepak] NIST, NCNR, Gaithersburg, MD 20899 USA. [Garlea, V. Ovidiu; Lumsden, Mark; Winn, Barry] Oak Ridge Natl Lab, QCMD, Oak Ridge, TN 37831 USA. RP Fobes, D (reprint author), Brookhaven Natl Lab, CMPMSD, Upton, NY 11973 USA. EM dfobes@bnl.gov; zaliznyak@bnl.gov RI Fobes, David/E-8526-2014; xu, zhijun/A-3264-2013; Tranquada, John/A-9832-2009; Zhong, Ruidan/D-5296-2013; Winn, Barry/A-5065-2016; Garlea, Vasile/A-4994-2016; Lumsden, Mark/F-5366-2012 OI Fobes, David/0000-0001-8252-2061; xu, zhijun/0000-0001-7486-2015; Tranquada, John/0000-0003-4984-8857; Zhong, Ruidan/0000-0003-1652-9454; Winn, Barry/0000-0001-6383-4318; Garlea, Vasile/0000-0002-5322-7271; Lumsden, Mark/0000-0002-5472-9660 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. DOE [DE-AC02-98CH10886] FX Work at BNL was supported by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. DOE under Contract No. DE-AC02-98CH10886. Research conducted at ORNL's High Flux Isotope Reactor and Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. We acknowledge the support of NIST, U.S. Department of Commerce, in providing the neutron research facilities used in this work. NR 42 TC 15 Z9 15 U1 2 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 9 PY 2014 VL 112 IS 18 AR 187202 DI 10.1103/PhysRevLett.112.187202 PG 5 WC Physics, Multidisciplinary SC Physics GA AH1GI UT WOS:000335867400007 PM 24856717 ER PT J AU Lin, SZ Batista, CD Reichhardt, C Saxena, A AF Lin, Shi-Zeng Batista, Cristian D. Reichhardt, Charles Saxena, Avadh TI ac Current Generation in Chiral Magnetic Insulators and Skyrmion Motion induced by the Spin Seebeck Effect SO PHYSICAL REVIEW LETTERS LA English DT Article ID ANISOTROPIC SUPEREXCHANGE INTERACTION; WEAK FERROMAGNETISM; TEMPERATURE; CRYSTALS; STATES AB We show that a temperature gradient induces an ac electric current in multiferroic insulators when the sample is embedded in a circuit. We also show that a thermal gradient can be used to move magnetic Skyrmions in insulating chiral magnets: the induced magnon flow from the hot to the cold region drives the Skyrmions in the opposite direction via a magnonic spin transfer torque. Both results are combined to compute the effect of Skyrmion motion on the ac current generation and demonstrate that Skyrmions in insulators are a promising route for spin caloritronics applications. C1 [Lin, Shi-Zeng; Batista, Cristian D.; Reichhardt, Charles; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, SZ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008; Batista, Cristian/J-8008-2016 OI Lin, Shi-Zeng/0000-0002-4368-5244; FU NNSA of the U.S. DOE at LANL [DE-AC52-06NA25396]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX Computer resources for numerical calculations were supported by the Institutional Computing Program at LANL. This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396, and was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 47 TC 33 Z9 33 U1 7 U2 78 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 9 PY 2014 VL 112 IS 18 AR 187203 DI 10.1103/PhysRevLett.112.187203 PG 5 WC Physics, Multidisciplinary SC Physics GA AH1GI UT WOS:000335867400008 PM 24856718 ER PT J AU Agakishiev, G Balanda, A Belver, D Belyaev, A Berger-Chen, JC Blanco, A Bohmer, M Boyard, JL Cabanelas, P Chernenko, S Dybczak, A Epple, E Fabbietti, L Fateev, O Finocchiaro, P Fonte, P Friese, J Frohlich, I Galatyuk, T Garzon, JA Gernhauser, R Gobel, K Golubeva, M Gonzalez-Diaz, D Guber, F Gumberidze, M Heinz, T Hennino, T Holzmann, R Ierusalimov, A Iori, I Ivashkin, A Jurkovic, M Kampfer, B Karavicheva, T Koenig, I Koenig, W Kolb, BW Kornakov, G Kotte, R Krasa, A Krizek, F Krucken, R Kuc, H Kuhn, W Kugler, A Kurepin, A Ladygin, V Lalik, R Lang, S Lapidus, K Lebedev, A Liu, T Lopes, L Lorenz, M Maier, L Mangiarotti, A Markert, J Metag, V Michalska, B Michel, J Muntz, C Naumann, L Pachmayer, YC Palka, M Parpottas, Y Pechenov, V Pechenova, O Pietraszko, J Przygoda, W Ramstein, B Reshetin, A Rustamov, A Sadovsky, A Salabura, P Schmah, A Schwab, E Siebenson, J Sobolev, YG Spataro, S Spruck, B Strobele, H Stroth, J Sturm, C Tarantola, A Teilab, K Tlusty, P Traxler, M Trebacz, R Tsertos, H Vasiliev, T Wagner, V Weber, M Wendisch, C Wustenfeld, J Yurevich, S Zanevsky, Y AF Agakishiev, G. Balanda, A. Belver, D. Belyaev, A. Berger-Chen, J. C. Blanco, A. Boehmer, M. Boyard, J. L. Cabanelas, P. Chernenko, S. Dybczak, A. Epple, E. Fabbietti, L. Fateev, O. Finocchiaro, P. Fonte, P. Friese, J. Froehlich, I. Galatyuk, T. Garzon, J. A. Gernhaeuser, R. Goebel, K. Golubeva, M. Gonzalez-Diaz, D. Guber, F. Gumberidze, M. Heinz, T. Hennino, T. Holzmann, R. Ierusalimov, A. Iori, I. Ivashkin, A. Jurkovic, M. Kaempfer, B. Karavicheva, T. Koenig, I. Koenig, W. Kolb, B. W. Kornakov, G. Kotte, R. Krasa, A. Krizek, F. Kruecken, R. Kuc, H. Kuehn, W. Kugler, A. Kurepin, A. Ladygin, V. Lalik, R. Lang, S. Lapidus, K. Lebedev, A. Liu, T. Lopes, L. Lorenz, M. Maier, L. Mangiarotti, A. Markert, J. Metag, V. Michalska, B. Michel, J. Muentz, C. Naumann, L. Pachmayer, Y. C. Palka, M. Parpottas, Y. Pechenov, V. Pechenova, O. Pietraszko, J. Przygoda, W. Ramstein, B. Reshetin, A. Rustamov, A. Sadovsky, A. Salabura, P. Schmah, A. Schwab, E. Siebenson, J. Sobolev, Yu. G. Spataro, S. Spruck, B. Stroebele, H. Stroth, J. Sturm, C. Tarantola, A. Teilab, K. Tlusty, P. Traxler, M. Trebacz, R. Tsertos, H. Vasiliev, T. Wagner, V. Weber, M. Wendisch, C. Wuestenfeld, J. Yurevich, S. Zanevsky, Y. TI Baryon resonance production and dielectron decays in proton-proton collisions at 3.5 GeV SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID HEAVY-ION COLLISIONS; DILEPTON PRODUCTION; NUCLEAR-MATTER; BEAM ENERGIES; SIS ENERGIES; FORM-FACTORS; RHO-MESON; RADIATION; PION AB We report on baryon resonance production and decay in proton-proton collisions at a kinetic energy of 3.5 GeV based on data measured with HADES. The exclusive channels pp -> np pi(+) and pp -> pp pi(0) as well as pp -> ppe(+)e(-) are studied simultaneously for the first time. The invariant masses and angular distributions of the pion-nucleon systems were studied and compared to simulations based on a resonance model ansatz assuming saturation of the pion production by an incoherent sum of baryonic resonances (R) with masses < 2 GeV/c(2). A very good description of the one-pion production is achieved allowing for an estimate of individual baryon resonance production cross sections which are used as input to calculate the dielectron yields from R -> pe(+)e(-) decays. Two models of the resonance decays into dielectrons are examined assuming a point-like RN gamma* coupling and the dominance of the rho meson. The results of model calculations are compared to data from the exclusive ppe(+)e(-) channel by means of the dielectron and pe(+)e(-) invariant mass distributions. C1 [Finocchiaro, P.] Ist Nazl Fis Nucl, Lab Nazl Sud, I-95125 Catania, Italy. [Blanco, A.; Fonte, P.; Lopes, L.; Mangiarotti, A.] LIP Lab Instrumentacao & Fis Expt Particulas, P-3004516 Coimbra, Portugal. [Balanda, A.; Dybczak, A.; Kuc, H.; Michalska, B.; Palka, M.; Przygoda, W.; Salabura, P.; Trebacz, R.] Jagiellonian Univ, Smoluchowski Inst Phys, PL-30059 Krakow, Poland. [Heinz, T.; Holzmann, R.; Koenig, I.; Koenig, W.; Kolb, B. W.; Lang, S.; Pechenov, V.; Pietraszko, J.; Schwab, E.; Stroth, J.; Sturm, C.; Traxler, M.; Yurevich, S.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Galatyuk, T.; Gonzalez-Diaz, D.; Gumberidze, M.; Kornakov, G.] Tech Univ Darmstadt, D-64289 Darmstadt, Germany. [Kaempfer, B.; Kotte, R.; Naumann, L.; Wendisch, C.; Wuestenfeld, J.] Helmholtz Zentrum Dresden Rossendorf, Inst Strahlenphys, D-01314 Dresden, Germany. [Agakishiev, G.; Belyaev, A.; Chernenko, S.; Fateev, O.; Ierusalimov, A.; Ladygin, V.; Vasiliev, T.; Zanevsky, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Froehlich, I.; Goebel, K.; Lorenz, M.; Markert, J.; Michel, J.; Muentz, C.; Pachmayer, Y. C.; Pechenova, O.; Rustamov, A.; Stroebele, H.; Stroth, J.; Tarantola, A.; Teilab, K.] Goethe Univ Frankfurt, Inst Kernphys, D-60438 Frankfurt, Germany. [Berger-Chen, J. C.; Epple, E.; Fabbietti, L.; Lalik, R.; Lapidus, K.; Siebenson, J.] Excellence Cluster Origin & Struct Universe, D-85748 Garching, Germany. [Boehmer, M.; Friese, J.; Gernhaeuser, R.; Jurkovic, M.; Kruecken, R.; Maier, L.; Weber, M.] Tech Univ Munich, Phys Dept E12, D-85748 Garching, Germany. [Kuehn, W.; Metag, V.; Spruck, B.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Iori, I.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Golubeva, M.; Guber, F.; Ivashkin, A.; Karavicheva, T.; Kurepin, A.; Reshetin, A.; Sadovsky, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Lebedev, A.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Parpottas, Y.; Tsertos, H.] Univ Cyprus, Dept Phys, CY-1678 Nicosia, Cyprus. [Boyard, J. L.; Hennino, T.; Kuc, H.; Liu, T.; Ramstein, B.] Univ Paris 11, CNRS, IN2P3, Inst Phys Nucl,UMR 8608, F-91406 Orsay, France. [Krasa, A.; Krizek, F.; Kugler, A.; Sobolev, Yu. G.; Tlusty, P.; Wagner, V.] Acad Sci Czech Republic, Inst Nucl Phys, CZ-25068 Rez, Czech Republic. [Belver, D.; Cabanelas, P.; Garzon, J. A.] Univ Santiago de Compostela, LabCAF F Fis, Santiago De Compostela 15706, Spain. [Fonte, P.] ISEC Coimbra, Coimbra, Portugal. [Galatyuk, T.; Gumberidze, M.; Lorenz, M.] ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Iori, I.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Kaempfer, B.; Wendisch, C.] Tech Univ Dresden, D-01062 Dresden, Germany. [Parpottas, Y.] Frederick Univ, CY-1036 Nicosia, Cyprus. [Schmah, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Spataro, S.] Univ Torino, Dipartimento Fis Gen, I-10125 Turin, Italy. [Spataro, S.] Univ Torino, INFN, I-10125 Turin, Italy. RP Agakishiev, G (reprint author), Joint Inst Nucl Res, Dubna 141980, Russia. EM witold.przygoda@uj.edu.pl RI Wagner, Vladimir/G-5650-2014; Krizek, Filip/G-8967-2014; Mangiarotti, Alessio/I-1072-2012; Gonzalez Diaz, Diego/K-7265-2014; Blanco, Alberto/L-2520-2014; Guber, Fedor/I-4271-2013; Cabanelas, Pablo/B-2034-2016; Gobel, Kathrin/B-8531-2016; Kurepin, Alexey/H-4852-2013; Kruecken, Reiner/A-1640-2013; Fonte, Paulo/B-1842-2008 OI Tsertos, Charalambos/0000-0001-5966-343X; Finocchiaro, Paolo/0000-0001-7502-2229; Lopes, Luis/0000-0001-8571-0033; Mangiarotti, Alessio/0000-0001-7837-6057; Gonzalez Diaz, Diego/0000-0002-6809-5996; Guber, Fedor/0000-0001-8790-3218; Cabanelas, Pablo/0000-0002-5416-4647; Gobel, Kathrin/0000-0003-2832-8465; Kurepin, Alexey/0000-0002-1851-4136; Kruecken, Reiner/0000-0002-2755-8042; Fonte, Paulo/0000-0002-2275-9099 NR 46 TC 13 Z9 13 U1 2 U2 22 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD MAY 9 PY 2014 VL 50 IS 5 AR 82 DI 10.1140/epja/i2014-14082-1 PG 16 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AG9JP UT WOS:000335735700002 ER PT J AU Fujita, K Kim, CK Lee, I Lee, J Hamidian, MH Firmo, IA Mukhopadhyay, S Eisaki, H Uchida, S Lawler, MJ Kim, EA Davis, JC AF Fujita, K. Kim, Chung Koo Lee, Inhee Lee, Jinho Hamidian, M. H. Firmo, I. A. Mukhopadhyay, S. Eisaki, H. Uchida, S. Lawler, M. J. Kim, E. -A. Davis, J. C. TI Simultaneous Transitions in Cuprate Momentum-Space Topology and Electronic Symmetry Breaking SO SCIENCE LA English DT Article ID HIGH-T-C; COPPER-OXIDE SUPERCONDUCTORS; PHASE-TRANSITIONS; MOTT INSULATOR; PSEUDOGAP; ORDER; BI2SR2CACU2O8+DELTA; NEMATICITY; DIAGRAM; STATE AB The existence of electronic symmetry breaking in the underdoped cuprates and its disappearance with increased hole density p are now widely reported. However, the relation between this transition and the momentum-space ((k) over right arrow -space) electronic structure underpinning the superconductivity has not yet been established. Here, we visualize the (Q) over right arrow =0 (intra-unit-cell) and (Q) over right arrow not equal 0 (density-wave) broken-symmetry states, simultaneously with the coherent. (k) over right arrow -space topology, for Bi2Sr2CaCu2O8+delta samples spanning the phase diagram 0.06 <= p <= 0.23. We show that the electronic symmetry-breaking tendencies weaken with increasing p and disappear close to a critical doping p(c) = 0.19. Concomitantly, the coherent. (k) over right arrow -space topology undergoes an abrupt transition, from arcs to closed contours, at the same p(c). These data reveal that the (k) over right arrow -space topology transformation in cuprates is linked intimately with the disappearance of the electronic symmetry breaking at a concealed critical point. C1 [Fujita, K.; Kim, Chung Koo; Lee, Inhee; Lee, Jinho; Hamidian, M. H.; Davis, J. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Fujita, K.; Hamidian, M. H.; Firmo, I. A.; Mukhopadhyay, S.; Lawler, M. J.; Kim, E. -A.; Davis, J. C.] Cornell Univ, Dept Phys, Lab Atom & Solid State Phys, Ithaca, NY 14853 USA. [Fujita, K.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan. [Lee, Jinho] Inst for Basic Sci, Seoul 151747, South Korea. [Lee, Jinho] Seoul Natl Univ, Dept Phys & Astron, Seoul 151747, South Korea. [Mukhopadhyay, S.] Cornell Univ, Cornell Ctr Mat Res, Ithaca, NY 14853 USA. [Eisaki, H.] Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. [Lawler, M. J.] SUNY Binghamton, Dept Phys & Astron, Binghamton, NY 13902 USA. [Davis, J. C.] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Davis, J. C.] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Davis, JC (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM jcseamusdavis@gmail.com RI Lawler, Michael/K-6770-2012; OI Lawler, Michael/0000-0002-2319-2274; KIM, CHUNG KOO/0000-0002-2463-197X FU U.S. Department of Energy [DE-2009-BNL-PM015]; Ministry of Science and Education (Japan); Global Centers of Excellence Program for Japan Society for the Promotion of Science; FlucTeam program at BNL [DE-AC02-98CH10886]; Institute for Basic Science, Korea; Fundacao para a Ciencia e a Tecnologia, Portugal [SFRH/BD/60952/2009]; NSF [DMR-1120296, DMR-0955822] FX We are particularly grateful to S. Billinge, J. E. Hoffman, S. A. Kivelson, D.-H. Lee, and A. P. Mackenzie for key scientific advice. We thank K. Efetov, E. Fradkin, P. D. Johnson, J. W. Orenstein, C. Pepin, S. Sachdev, and K. M. Shen for helpful discussions and communications. Experimental studies were supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center, headquartered at Brookhaven National Laboratory (BNL) and funded by the U.S. Department of Energy under grant DE-2009-BNL-PM015, as well as by a Grant-in-Aid for Scientific Research from the Ministry of Science and Education (Japan) and the Global Centers of Excellence Program for Japan Society for the Promotion of Science. C. K. K. acknowledges support from the FlucTeam program at BNL under contract DE-AC02-98CH10886. J.L. acknowledges support from the Institute for Basic Science, Korea. I.A.F. acknowledges support from Fundacao para a Ciencia e a Tecnologia, Portugal, under fellowship number SFRH/BD/60952/2009. S.M. acknowledges support from NSF grant DMR-1120296 to the Cornell Center for Materials Research. Theoretical studies at Cornell University were supported by NSF grant DMR-1120296 to Cornell Center for Materials Research and by NSF grant DMR-0955822. The original data are archived by Davis Group, BNL, and Cornell University. NR 39 TC 66 Z9 67 U1 10 U2 71 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 9 PY 2014 VL 344 IS 6184 BP 612 EP 616 DI 10.1126/science.1248783 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG6OD UT WOS:000335537400038 PM 24812397 ER PT J AU Brunecky, R Alahuhta, M Xu, Q Donohoe, BS Crowley, MF Kataeva, IA Yang, SJ Resch, MG Adams, MWW Lunin, VV Himmel, ME Bomble, YJ AF Brunecky, Roman Alahuhta, Markus Xu, Qi Donohoe, Bryon S. Crowley, Michael F. Kataeva, Irina A. Yang, Sung-Jae Resch, Michael G. Adams, Michael W. W. Lunin, Vladimir V. Himmel, Michael E. Bomble, Yannick J. TI Response to Comment on "Revealing Nature's Cellulase Diversity: The Digestion Mechanism of Caldicellulosiruptor bescii CelA" SO SCIENCE LA English DT Editorial Material ID MIXTURES C1 [Brunecky, Roman; Alahuhta, Markus; Xu, Qi; Donohoe, Bryon S.; Crowley, Michael F.; Resch, Michael G.; Lunin, Vladimir V.; Himmel, Michael E.; Bomble, Yannick J.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Kataeva, Irina A.; Yang, Sung-Jae; Adams, Michael W. W.] Univ Georgia, Dept Biochem & Mol Biol, Athens, GA 30602 USA. RP Bomble, YJ (reprint author), Natl Renewable Energy Lab, Biosci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM yannick.bomble@nrel.gov NR 8 TC 0 Z9 0 U1 6 U2 39 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 9 PY 2014 VL 344 IS 6184 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG6OD UT WOS:000335537400024 ER PT J AU Shao, HS Ma, YQ Wang, K Chao, KT AF Shao, Hua-Sheng Ma, Yan-Qing Wang, Kai Chao, Kuang-Ta TI Polarizations of chi(c1) and chi(c2) in Prompt Production at the LHC SO PHYSICAL REVIEW LETTERS LA English DT Article ID ROOT S=1.8 TEV; HEAVY-QUARKONIUM; P(P)OVER-BAR COLLISIONS; PP COLLISIONS; J/PSI; RATIO AB Prompt chi(c) production at hadron colliders may provide a unique test for the color-octet mechanism in nonrelativistic QCD. We present an analysis for the polarization observables of chi(c1) and chi(c2) at next-to-leading order in alpha(S) and propose to measure them at the LHC, which is expected to be important for testing the validity of nonrelativistic QCD. C1 [Shao, Hua-Sheng; Wang, Kai; Chao, Kuang-Ta] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Shao, Hua-Sheng; Wang, Kai; Chao, Kuang-Ta] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Ma, Yan-Qing] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Chao, Kuang-Ta] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Chao, Kuang-Ta] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China. RP Shao, HS (reprint author), Peking Univ, Sch Phys, Beijing 100871, Peoples R China. FU National Natural Science Foundation of China [11021092, 11075002]; U.S. Department of Energy [DE-AC02-98CH10886] FX We are grateful to C. Meng, Y. J. Zhang, and H. Han for helpful discussions. This work was supported in part by the National Natural Science Foundation of China (No. 11021092 and No. 11075002). Y.-Q. M is supported by the U.S. Department of Energy, Contract No. DE-AC02-98CH10886. NR 26 TC 20 Z9 20 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 8 PY 2014 VL 112 IS 18 AR 182003 DI 10.1103/PhysRevLett.112.182003 PG 5 WC Physics, Multidisciplinary SC Physics GA AM1SU UT WOS:000339629400006 PM 24856690 ER PT J AU Smalyuk, VA Casey, DT Clark, DS Edwards, MJ Haan, SW Hamza, A Hoover, DE Hsing, WW Hurricane, O Kilkenny, JD Kroll, J Landen, OL Moore, A Nikroo, A Peterson, L Raman, K Remington, BA Robey, HF Weber, SV Widmann, K AF Smalyuk, V. A. Casey, D. T. Clark, D. S. Edwards, M. J. Haan, S. W. Hamza, A. Hoover, D. E. Hsing, W. W. Hurricane, O. Kilkenny, J. D. Kroll, J. Landen, O. L. Moore, A. Nikroo, A. Peterson, L. Raman, K. Remington, B. A. Robey, H. F. Weber, S. V. Widmann, K. TI First Measurements of Hydrodynamic Instability Growth in Indirectly Driven Implosions at Ignition-Relevant Conditions on the National Ignition Facility SO PHYSICAL REVIEW LETTERS LA English DT Article AB Ignition experiments have shown an anomalous susceptibility to hydrodynamic instability growth. To help understand these results, the first hydrodynamic instability growth measurements in indirectly driven implosions on the National Ignition Facility were performed at ignition conditions with peak radiation temperatures up to similar to 300 eV. Plastic capsules with two-dimensional preimposed, sinusoidal outer surface modulations of initial wavelengths of 240 (corresponding to a Legendre mode number of 30), 120 (mode 60), and 80 mu m (mode 90) were imploded by using actual low-adiabat ignition laser pulses. The measured growth was in excellent agreement, validating 2D HYDRA simulations for the most dangerous modes in the acceleration phase. These results reinforce confidence in the predictive capability of calculations that are paramount to illuminating the path toward ignition. C1 [Smalyuk, V. A.; Casey, D. T.; Clark, D. S.; Edwards, M. J.; Haan, S. W.; Hamza, A.; Hsing, W. W.; Hurricane, O.; Kroll, J.; Landen, O. L.; Peterson, L.; Raman, K.; Remington, B. A.; Robey, H. F.; Weber, S. V.; Widmann, K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hoover, D. E.; Kilkenny, J. D.; Nikroo, A.] Gen Atom Co, San Diego, CA 92121 USA. [Moore, A.] AWE Aldermaston, Reading RG7 4PR, Berks, England. RP Smalyuk, VA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 30 TC 41 Z9 42 U1 0 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 8 PY 2014 VL 112 IS 18 AR 185003 DI 10.1103/PhysRevLett.112.185003 PG 5 WC Physics, Multidisciplinary SC Physics GA AM1SU UT WOS:000339629400011 PM 24856703 ER PT J AU Wang, HQ Xu, GS Wan, BN Ding, SY Guo, HY Shao, LM Liu, SC Xu, XQ Wang, E Yan, N Naulin, V Nielsen, AH Rasmussen, JJ Candy, J Bravenec, R Sun, YW Shi, TH Liang, YF Chen, R Zhang, W Wang, L Chen, L Zhao, N Li, YL Liu, YL Hu, GH Gong, XZ AF Wang, H. Q. Xu, G. S. Wan, B. N. Ding, S. Y. Guo, H. Y. Shao, L. M. Liu, S. C. Xu, X. Q. Wang, E. Yan, N. Naulin, V. Nielsen, A. H. Rasmussen, J. Juul Candy, J. Bravenec, R. Sun, Y. W. Shi, T. H. Liang, Y. F. Chen, R. Zhang, W. Wang, L. Chen, L. Zhao, N. Li, Y. L. Liu, Y. L. Hu, G. H. Gong, X. Z. TI New Edge Coherent Mode Providing Continuous Transport in Long-Pulse H-mode Plasmas SO PHYSICAL REVIEW LETTERS LA English DT Article ID ALCATOR C-MOD; PARTICLE LOSSES; TOKAMAK; TURBULENCE; REGIME AB An electrostatic coherent mode near the electron diamagnetic frequency (20-90 kHz) is observed in the steep-gradient pedestal region of long pulse H-mode plasmas in the Experimental Advanced Superconducting Tokamak, using a newly developed dual gas-puff-imaging system and diamond-coated reciprocating probes. The mode propagates in the electron diamagnetic direction in the plasma frame with poloidal wavelength of similar to 8 cm. The mode drives a significant outflow of particles and heat as measured directly with the probes, thus greatly facilitating long pulse H-mode sustainment. This mode shows the nature of dissipative trapped electron mode, as evidenced by gyrokinetic turbulence simulations. C1 [Wang, H. Q.; Xu, G. S.; Wan, B. N.; Ding, S. Y.; Guo, H. Y.; Shao, L. M.; Liu, S. C.; Sun, Y. W.; Shi, T. H.; Liang, Y. F.; Chen, R.; Zhang, W.; Wang, L.; Chen, L.; Zhao, N.; Li, Y. L.; Liu, Y. L.; Hu, G. H.; Gong, X. Z.] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China. [Guo, H. Y.; Candy, J.] Gen Atom Co, San Diego, CA 92186 USA. [Xu, X. Q.; Wang, E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Yan, N.; Naulin, V.; Nielsen, A. H.; Rasmussen, J. Juul] Assoc EURATOM DTU, Dept Phys, DK-2800 Lyngby, Denmark. [Bravenec, R.] Fourth State Res, Austin, TX 78704 USA. RP Wang, HQ (reprint author), Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China. EM gsxu@ipp.ac.cn RI Nielsen, Anders/A-3973-2012; Naulin , Volker/A-2419-2012; Sun, Youwen/B-3553-2012; Rasmussen, Jens Juul/A-2757-2012 OI Nielsen, Anders/0000-0003-3642-3905; Naulin , Volker/0000-0001-5452-9215; Sun, Youwen/0000-0002-9934-1328; Rasmussen, Jens Juul/0000-0002-3543-690X FU National Magnetic Confinement Fusion Science Program of China [2011GB107001, 2011GB101000, 2013GB106000, 2013GB107003, 2010GB104001]; National Natural Science Foundation of China [10990212, 11321092, 11075181]; Thousand Talent Plan of China; Sino Danish Center for Education and Research FX This work was supported by National Magnetic Confinement Fusion Science Program of China under Contracts No. 2011GB107001, No. 2011GB101000, No. 2013GB106000, No. 2013GB107003, and No. 2010GB104001, National Natural Science Foundation of China under Contracts No. 10990212, No. 11321092, No. 11075181, the Thousand Talent Plan of China, and the Sino Danish Center for Education and Research. We would like to thank S. J. Zweben, J. Q. Dong, J. Q. Li, and Linjin Zheng for useful discussions. NR 24 TC 18 Z9 19 U1 14 U2 69 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 8 PY 2014 VL 112 IS 18 AR 185004 DI 10.1103/PhysRevLett.112.185004 PG 5 WC Physics, Multidisciplinary SC Physics GA AM1SU UT WOS:000339629400012 PM 24856704 ER PT J AU Gardeux, V Arslan, AD Achour, I Ho, TT Beck, WT Lussier, YA AF Gardeux, Vincent Arslan, Ahmet D. Achour, Ikbel Ho, Tsui-Ting Beck, William T. Lussier, Yves A. TI Concordance of deregulated mechanisms unveiled in underpowered experiments: PTBP1 knockdown case study SO BMC MEDICAL GENOMICS LA English DT Article; Proceedings Paper CT 3rd Annual Translational Bioinformatics Conference (TBC) / ISCB-Asia CY OCT 02-04, 2013 CL Seoul, SOUTH KOREA SP ISCB Asia ID INFORMATION-THEORY; GENE ONTOLOGY; RNA-SEQ; CANCER; GENOME; PREDICTION; BIOLOGY; KEGG; TOOL AB Background: Genome-wide transcriptome profiling generated by microarray and RNA-Seq often provides deregulated genes or pathways applicable only to larger cohort. On the other hand, individualized interpretation of transcriptomes is increasely pursued to improve diagnosis, prognosis, and patient treatment processes. Yet, robust and accurate methods based on a single paired-sample remain an unmet challenge. Methods: "N-of-1-pathways" translates gene expression data profiles into mechanism-level profiles on single pairs of samples (one p-value per geneset). It relies on three principles: i) statistical universe is a single paired sample, which serves as its own control; ii) statistics can be derived from multiple gene expression measures that share common biological mechanisms assimilated to genesets; iii) semantic similarity metric takes into account inter-mechanisms' relationships to better assess commonality and differences, within and cross study-samples (e. g. patients, cell-lines, tissues, etc.), which helps the interpretation of the underpinning biology. Results: In the context of underpowered experiments, N-of-1-pathways predictions perform better or comparable to those of GSEA and Differentially Expressed Genes enrichment (DEG enrichment), within-and cross-datasets. N-of-1-pathways uncovered concordant PTBP1-dependent mechanisms across datasets (Odds-Ratios >= 13, p-values <= 1 x 10(-5)), such as RNA splicing and cell cycle. In addition, it unveils tissue-specific mechanisms of alternatively transcribed PTBP1-dependent genesets. Furthermore, we demonstrate that GSEA and DEG Enrichment preclude accurate analysis on single paired samples. Conclusions: N-of-1-pathways enables robust and biologically relevant mechanism-level classifiers with small cohorts and one single paired samples that surpasses conventional methods. Further, it identifies unique sample/patient mechanisms, a requirement for precision medicine. C1 [Gardeux, Vincent; Achour, Ikbel; Lussier, Yves A.] Univ Illinois, Inst Translat Hlth Informat, Chicago, IL 60680 USA. [Gardeux, Vincent; Achour, Ikbel; Lussier, Yves A.] Univ Illinois, Dept Med, Chicago, IL 60680 USA. [Gardeux, Vincent] EISTI, Sch Engn, Dept Informat, Cergy, France. [Arslan, Ahmet D.; Ho, Tsui-Ting; Beck, William T.; Lussier, Yves A.] Univ Illinois, Coll Pharm, Dept Biopharmaceut Sci, Chicago, IL 60680 USA. [Arslan, Ahmet D.] Northwestern Univ, Robert H Lurie Comprehens Canc Ctr, Chicago, IL 60611 USA. [Ho, Tsui-Ting] Univ Mississippi, Med Ctr, Inst Canc, Jackson, MI USA. [Lussier, Yves A.] Univ Illinois, Dept Bioengn, Chicago, IL 60680 USA. [Lussier, Yves A.] Argonne Natl Lab, Computat Inst, Argonne, IL 60439 USA. [Lussier, Yves A.] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Lussier, Yves A.] Univ Chicago, Chicago, IL 60637 USA. [Lussier, Yves A.] Univ Illinois, Inst Personalized Resp Med, Chicago, IL 60680 USA. [Beck, William T.; Lussier, Yves A.] Univ Illinois, Ctr Canc, Chicago, IL 60680 USA. [Gardeux, Vincent; Achour, Ikbel; Lussier, Yves A.] Univ Arizona, Clin & Translat Sci Inst, Inst BIO5, Ctr Canc, Tucson, AZ 85721 USA. RP Beck, WT (reprint author), Univ Illinois, Inst Translat Hlth Informat, Chicago, IL 60680 USA. EM wtbeck@uic.edu; lussier.y@gmail.com RI Gardeux, Vincent/O-9653-2016; OI Gardeux, Vincent/0000-0001-8954-2161; Lussier, Yves/0000-0001-9854-1005 FU NLM NIH HHS [K22 LM008308] NR 28 TC 5 Z9 5 U1 0 U2 6 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1755-8794 J9 BMC MED GENOMICS JI BMC Med. Genomics PD MAY 8 PY 2014 VL 7 SU 1 AR S1 DI 10.1186/1755-8794-7-S1-S1 PG 13 WC Genetics & Heredity SC Genetics & Heredity GA AJ2EE UT WOS:000337467400002 PM 25079003 ER PT J AU Yang, XN Huang, Y Lee, Y Gardeux, V Achour, I Regan, K Rebman, E Li, HQ Lussier, YA AF Yang, Xinan Huang, Yong Lee, Younghee Gardeux, Vincent Achour, Ikbel Regan, Kelly Rebman, Ellen Li, Haiquan Lussier, Yves A. TI In Silico cancer cell versus stroma cellularity index computed from species-specific human and mouse transcriptome of xenograft models: towards accurate stroma targeting therapy assessment SO BMC MEDICAL GENOMICS LA English DT Article; Proceedings Paper CT 3rd Annual Translational Bioinformatics Conference (TBC) / ISCB-Asia CY OCT 02-04, 2013 CL Seoul, SOUTH KOREA SP ISCB Asia ID LASER CAPTURE MICRODISSECTION; GENE-EXPRESSION; TUMOR MICROENVIRONMENT; BREAST-CANCER; MATRIX METALLOPROTEINASES; PROGRESSION; AMPLIFICATION; FIBROBLASTS; MICROARRAY; RESISTANCE AB Background: The current state of the art for measuring stromal response to targeted therapy requires burdensome and rate limiting quantitative histology. Transcriptome measures are increasingly affordable and provide an opportunity for developing a stromal versus cancer ratio in xenograft models. In these models, human cancer cells are transplanted into mouse host tissues (stroma) and together coevolve into a tumour microenvironment. However, profiling the mouse or human component separately remains problematic. Indeed, laser capture microdissection is labour intensive. Moreover, gene expression using commercial microarrays introduces significant and underreported cross-species hybridization errors that are commonly overlooked by biologists. Method: We developed a customized dual-species array, H&M array, and performed cross-species and species-specific hybridization measurements. We validated a new methodology for establishing the stroma vs cancer ratio using transcriptomic data. Results: In the biological validation of the H&M array, cross-species hybridization of human and mouse probes was significantly reduced (4.5 and 9.4 fold reduction, respectively; p < 2x10(-16) for both, Mann-Whitney test). We confirmed the capability of the H&M array to determine the stromal to cancer cells ratio based on the estimation of cellularity index of mouse/human mRNA content in vitro. This new metrics enable to investigate more efficiently the stroma-cancer cell interactions (e. g. cellularity) bypassing labour intensive requirement and biases of laser capture microdissection. Conclusion: These results provide the initial evidence of improved and cost-efficient analytics for the investigation of cancer cell microenvironment, using species-specificity arrays specifically designed for xenografts models. C1 [Yang, Xinan; Huang, Yong; Lee, Younghee; Lussier, Yves A.] Univ Chicago, Dept Med, Ctr Biom Info, Med Genet Sect, Chicago, IL 60637 USA. [Gardeux, Vincent; Achour, Ikbel; Regan, Kelly; Rebman, Ellen; Li, Haiquan; Lussier, Yves A.] Univ Illinois, Inst Translat Hlth Informat, Chicago, IL 60680 USA. [Gardeux, Vincent] EISTI Engn Sch, Dept Informat, Cergy, France. [Gardeux, Vincent; Achour, Ikbel; Regan, Kelly; Rebman, Ellen; Li, Haiquan; Lussier, Yves A.] Univ Illinois, Dept Med, Chicago, IL 60680 USA. [Lussier, Yves A.] Univ Chicago, Ctr Comprehens Canc, Chicago, IL 60637 USA. [Lussier, Yves A.] Univ Chicago, Ludwig Ctr Metastasis Res, Chicago, IL 60637 USA. [Yang, Xinan] Univ Chicago, Med Comer Childrens Hosp, Dept Pediat, Hematol Oncol Sect, Chicago, IL 60637 USA. [Lussier, Yves A.] Univ Illinois, Dept Bioengn, Chicago, IL 60680 USA. [Lussier, Yves A.] Univ Illinois, Dept Pharmaceut Sci, Chicago, IL 60680 USA. [Lussier, Yves A.] Argonne Natl Lab, Comp Inst, Argonne, IL 60439 USA. [Lussier, Yves A.] Argonne Natl Lab, Inst Genom & Syst Bio, Argonne, IL 60439 USA. [Lussier, Yves A.] Univ Chicago, Chicago, IL 60637 USA. [Lussier, Yves A.] Univ Illinois, Inst Personalized Resp Med, Chicago, IL 60680 USA. [Gardeux, Vincent; Achour, Ikbel; Li, Haiquan; Lussier, Yves A.] Univ Arizona, Ctr Canc, Inst BIO5, Clin & Translat Sci Inst, Tucson, AZ 85721 USA. RP Lussier, YA (reprint author), Univ Chicago, Dept Med, Ctr Biom Info, Med Genet Sect, Chicago, IL 60637 USA. EM lussier.y@gmail.com RI Gardeux, Vincent/O-9653-2016; OI Gardeux, Vincent/0000-0001-8954-2161; Li, Haiquan/0000-0002-8049-0278; Lussier, Yves/0000-0001-9854-1005 FU NCI NIH HHS [R21 CA167305]; NLM NIH HHS [T15 LM011270, K22 LM008308] NR 35 TC 1 Z9 1 U1 0 U2 1 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1755-8794 J9 BMC MED GENOMICS JI BMC Med. Genomics PD MAY 8 PY 2014 VL 7 SU 1 AR S2 DI 10.1186/1755-8794-7-S1-S2 PG 13 WC Genetics & Heredity SC Genetics & Heredity GA AJ2EE UT WOS:000337467400003 PM 25079962 ER PT J AU Haines, BM Grinstein, FF Fincke, JR AF Haines, Brian M. Grinstein, Fernando F. Fincke, James R. TI Three-dimensional simulation strategy to determine the effects of turbulent mixing on inertial-confinement-fusion capsule performance SO PHYSICAL REVIEW E LA English DT Article ID RICHTMYER-MESHKOV INSTABILITIES; DIRECT-DRIVE; TAYLOR INSTABILITY; RAYLEIGH-TAYLOR; PLASTIC-SHELL; OMEGA; COMPRESSION; IMPLOSIONS AB In this paper, we present and justify an effective strategy for performing three-dimensional (3D) inertial-confinement-fusion (ICF) capsule simulations. We have evaluated a frequently used strategy in which two-dimensional (2D) simulations are rotated to 3D once sufficient relevant 2D flow physics has been captured and fine resolution requirements can be restricted to relatively small regions. This addresses situations typical of ICF capsules which are otherwise prohibitively intensive computationally. We tested this approach for our previously reported fully 3D simulations of laser-driven reshock experiments where we can use the available 3D data as reference. Our studies indicate that simulations that begin as purely 2D lead to significant underprediction of mixing and turbulent kinetic energy production at later time when compared to the fully 3D simulations. If, however, additional suitable nonuniform perturbations are applied at the time of rotation to 3D, we show that one can obtain good agreement with the purely 3D simulation data, as measured by vorticity distributions as well as integrated mixing and turbulent kinetic energy measurements. Next, we present results of simulations of a simple OMEGA-type ICF capsule using the developed strategy. These simulations are in good agreement with available experimental data and suggest that the dominant mechanism for yield degradation in ICF implosions is hydrodynamic instability growth seeded by long-wavelength surface defects. This effect is compounded by drive asymmetries and amplified by repeated shock interactions with an increasingly distorted shell, which results in further yield reduction. Our simulations are performed with and without drive asymmetries in order to compare the importance of these effects to those of surface defects; our simulations indicate that long-wavelength surface defects degrade yield by approximately 60% and short-wavelength drive asymmetry degrades yield by a further 30%. C1 [Haines, Brian M.; Grinstein, Fernando F.; Fincke, James R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Haines, BM (reprint author), Los Alamos Natl Lab, MS T087, Los Alamos, NM 87545 USA. EM bmhaines@lanl.gov OI Haines, Brian/0000-0002-3889-7074 FU US Department of Energy NNSA [DE-AC52-06NA25396] FX The authors would like to thank M. Daniels and M. McKay for code debugging assistance as well as L. Welser-Sherrill for useful discussions. The authors would also like to thank P. Bradley for assistance in modeling OMEGA shot 65036. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the US Department of Energy NNSA under Contract No. DE-AC52-06NA25396. NR 44 TC 8 Z9 8 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 8 PY 2014 VL 89 IS 5 AR 053302 DI 10.1103/PhysRevE.89.053302 PG 14 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AI5LU UT WOS:000336909400012 PM 25353910 ER PT J AU Zhao, YX Zhu, K AF Zhao, Yixin Zhu, Kai TI CH3NH3Cl-Assisted One-Step Solution Growth of CH(3)NH(3)Pbl(3): Structure, Charge-Carrier Dynamics, and Photovoltaic Properties of Perovskite Solar Cells SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ORGANOLEAD HALIDE PEROVSKITE; HOLE CONDUCTOR; LOW-COST; EFFICIENT; TRANSPORT; IODIDE; RECOMBINATION; PERFORMANCE; CH3NH3PBI3; DEPOSITION AB We demonstrate a novel one-step solution approach to prepare perovskite CH3NH3PbI3 films by adding CH3NH3Cl (or MACl) to the standard CH(3)NH(3)Pbl(3) precursor (equimolar mixture of CH3NH3I and PbI2) solution. The use of MACl strongly affects the crystallization process of forming pure CH3NH3PbI3, leading not only to enhanced absorption of CH3NH3PbI3 but also to significantly improved coverage of CH3NH3PbI3 on a planar substrate. Compared to the standard one-step solution approach for CH3NH3PbI3, using MACI improves the performance of CH3NH3PbI3 solar cells from about 2% to 12% for the planar cell structure and from about 8% to 10% for the mesostructured device architecture. Although we find no significant effect of using MACl on charge transport and recombination in mesostructured perovskite cells, the recombination resistance for planar cells increases by 1-2 orders of magnitude by using MACl. These results suggest that this new one-step solution approach is promising for controlling CH3NH3PbI3 growth to achieve high-performance perovskite solar cells. C1 [Zhao, Yixin; Zhu, Kai] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. RP Zhu, K (reprint author), Natl Renewable Energy Lab, Chem & Mat Sci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Kai.Zhu@nrel.gov RI Zhao, Yixin/D-2949-2012 FU U.S. Department of Energy/National Renewable Energy Laboratory's Laboratory Directed Research and Development (LDRD) program [DE-AC36-08GO28308]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [AG36-08GO28308]; National Renewable Energy Laboratory FX We acknowledge the support by the U.S. Department of Energy/National Renewable Energy Laboratory's Laboratory Directed Research and Development (LDRD) program under Contract DE-AC36-08GO28308. K.Z. acknowledges the support on the charge transport and recombination studies by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract DE-AG36-08GO28308 with the National Renewable Energy Laboratory. NR 34 TC 196 Z9 201 U1 23 U2 417 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 8 PY 2014 VL 118 IS 18 BP 9412 EP 9418 DI 10.1021/jp502696w PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH1KL UT WOS:000335878900012 ER PT J AU Zhao, X Shu, Q Nguyen, MC Wang, YG Ji, M Xiang, HJ Ho, KM Gong, XG Wang, CZ AF Zhao, Xin Shu, Qiang Manh Cuong Nguyen Wang, Yangang Ji, Min Xiang, Hongjun Ho, Kai-Ming Gong, Xingao Wang, Cai-Zhuang TI Interface Structure Prediction from First-Principles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; AB-INITIO DATA; EFFECTIVE POTENTIALS; GENETIC ALGORITHM; GRAIN-BOUNDARIES; SYSTEMS; METALS; OXIDES AB Information about the atomic structures at solid-solid interfaces is crucial for understanding and predicting the performance of materials. Due to the complexity of the interfaces, it is very challenging to resolve their atomic structures using either experimental techniques or computer simulations. In this paper, we present an efficient first-principles computational method for interface structure prediction based on an adaptive genetic algorithm. This approach significantly reduces the computational cost, while retaining the accuracy of first-principles prediction. The method is applied to the investigation of both stoichiometric and nonstoichiometric SrTiO3 Sigma 3(112)[(1) over bar 10] grain boundaries with unit cell containing up to 200 atoms. Several novel low-energy structures are discovered, which provide fresh insights into the structure and stability of the grain boundaries. C1 [Shu, Qiang; Ji, Min; Xiang, Hongjun; Gong, Xingao] Fudan Univ, State Key Lab Surface Phys, Minist Educ, Key Lab Computat Phys Sci, Shanghai 200433, Peoples R China. [Shu, Qiang; Ji, Min; Xiang, Hongjun; Gong, Xingao] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Zhao, Xin; Manh Cuong Nguyen; Wang, Yangang; Ji, Min; Ho, Kai-Ming; Wang, Cai-Zhuang] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. [Zhao, Xin; Manh Cuong Nguyen; Wang, Yangang; Ji, Min; Ho, Kai-Ming; Wang, Cai-Zhuang] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Wang, Yangang] Chinese Acad Sci, Supercomp Ctr, Beijing 100190, Peoples R China. RP Gong, XG (reprint author), Fudan Univ, State Key Lab Surface Phys, Minist Educ, Key Lab Computat Phys Sci, Shanghai 200433, Peoples R China. EM xggong@fudan.edu.cn; wangcz@ameslab.gov RI Nguyen, Manh Cuong/G-2783-2015; Xiang, Hongjun/I-4305-2016; gong, xingao/D-6532-2011; OI Nguyen, Manh Cuong/0000-0001-8027-9029; Xiang, Hongjun/0000-0002-9396-3214; Zhao, Xin/0000-0002-3580-512X FU Special Funds for Major State Basic Research of China [2012CB921400]; National Science Foundation of China (NSFC); U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358]; Oak Ridge Leadership Computing Facility (OLCF) in Oak Ridge, TN FX Work at Fudan was partially supported by the Special Funds for Major State Basic Research of China (2012CB921400), National Science Foundation of China (NSFC). Work at Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Scientific Computing Center (NERSC) in Berkeley, CA and the Oak Ridge Leadership Computing Facility (OLCF) in Oak Ridge, TN. NR 31 TC 1 Z9 1 U1 6 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 8 PY 2014 VL 118 IS 18 BP 9524 EP 9530 DI 10.1021/jp5010852 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH1KL UT WOS:000335878900025 ER PT J AU Kim, B Li, ZJ Kay, BD Dohnalek, Z Kim, YK AF Kim, Boseong Li, Zhenjun Kay, Bruce D. Dohnalek, Zdenek Kim, Yu Kwon TI Low-Temperature Desorption of N2O from NO on Rutile TiO2(110)-1 x 1 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SELECTIVE CATALYTIC-REDUCTION; DISSOCIATIVE ADSORPTION; OXYGEN VACANCIES; BAND-GAP; SURFACE; NH3; SITES; CO; DECOMPOSITION; CEO2/TIO2 AB We find that NO dosed on ruffle TiO2(110)-1 X 1 at substrate temperatures as low as 50 K readily reacts to produce N2O, which desorbs promptly from the surface leaving an oxygen adatom behind. The desorption rate of N2O reaches a maximum value after 1-2 s at an NO flux of 1.2 x 10(14) NO/cm(2).sec and then decreases rapidly as the initially dean, reduced TiO2(110) surface with similar to 5% oxygen vacancies (V-O's) becomes covered with oxygen adatoms and unreacted NO. The maximum desorption rate is also found to increase as the substrate temperature is raised up to about 100 K Interestingly, the N2O desorption during the low-temperature (LT) NO dose is strongly suppressed when molecular oxygen is predosed, whereas it persists on the surface with V-O's passivated by surface hydroxyls. Our results show that the surface charge, not the V-O sites, plays a dominant role in the LT N2O desorption induced by a facile NO reduction at such low temperatures. C1 [Kim, Boseong; Kim, Yu Kwon] Ajou Univ, Dept Energy Syst Res, Suwon 443749, South Korea. [Kim, Boseong; Kim, Yu Kwon] Ajou Univ, Dept Chem, Suwon 443749, South Korea. [Li, Zhenjun; Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Chem & Mat Sci Div, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Kim, YK (reprint author), Ajou Univ, Dept Energy Syst Res, Suwon 443749, South Korea. EM yukwonkim@ajou.ac.kr FU U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; Department of Energy's Office of Biological and Environmental Research; U.S. DOE [DE-AC06-76RLO 1830]; Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education, Science and Technology [NRF-2012R1A1A2007641] FX Part of this work was supported by the U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, and performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the U.S. DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RLO 1830. Y.K.K. acknowledges financial support from the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (NRF-2012R1A1A2007641). NR 34 TC 3 Z9 3 U1 1 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 8 PY 2014 VL 118 IS 18 BP 9544 EP 9550 DI 10.1021/jp501179y PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH1KL UT WOS:000335878900028 ER PT J AU Cui, JF Fang, XW Schmidt-Rohr, K AF Cui, J-F Fang, X-W Schmidt-Rohr, K. TI Quantification of C=C and C=O Surface Carbons in Detonation Nanodiamond by NMR SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SOLID-STATE NMR; NUCLEAR-MAGNETIC-RESONANCE; DIAMOND; CHEMISTRY; SPECTROSCOPY; GRAPHITIZATION; REACTIVITY; CRYSTALS; SIZE AB The ability of solid-state C-13 NMR to detect and quantify small amounts of sp(2)-hybridized carbon on the surface of similar to 5 nm diameter nanodiamond particles is demonstrated. The C=C carbon fraction is only 1.1 +/- 0.4% in pristine purified detonation nanodiamond, while a full single-layer graphitic or "bucky diamond" shell would contain ca. 25% of all C in a 5 nm diameter particle. Instead of large aromatic patches repeatedly proposed in the recent literature, sp(3)-hybridized CH and COH carbons cover most of the nanodiamond particle surface, accounting for similar to 5% each. C=O and COO groups also seen in X-ray absorption near-edge structure spectroscopy (XANES) but not detected in previous NMR studies make up ca. 1.5% of all C. They are removed by heat treatment at 800 degrees C, which increases the aromatic fraction. C-13{H-1} NMR demonstrates that the various sp2-hybridized carbons are mostly not protonated, but cross-polarization shows that they are separated from H-1 by only a few bond lengths, which proves that they are near the protonated surface. Together, the observed C-H, C-OH, C=O, and C=C groups account for 12-14% of all C, which matches the surface fraction expected for bulk-terminated 5 nm diameter diamond particles. C1 [Schmidt-Rohr, K.] US DOE, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Schmidt-Rohr, K (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM srohr@iastate.edu FU U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358] FX K.S.R. would like to thank Y. Gogotsi and V. Mochalin for stimulating discussions. This work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. It was performed at the Ames Laboratory, which is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 48 TC 11 Z9 11 U1 6 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 8 PY 2014 VL 118 IS 18 BP 9621 EP 9627 DI 10.1021/jp503053r PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH1KL UT WOS:000335878900037 ER PT J AU Deshmukh, SA Kamath, G Pol, VG Sankaranarayanan, SKRS AF Deshmukh, Sanket A. Kamath, Ganesh Pol, Vilas G. Sankaranarayanan, Subramanian K. R. S. TI Kinetic Pathways To Control Hydrogen Evolution and Nanocarbon Allotrope Formation via Thermal Decomposition of Polyethylene SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RING STATISTICS; CARBON; WASTE; PYROLYSIS; PRESSURE; LIQUID; ORDER; PURE AB Polyethylene-based plastic materials are nonbiodegradable in nature and have a profound negative impact on our environment. Efficient disposal of plastic wastes in an efficient, environmental friendly fashion or chemical fixation of plastics into useful intermediates remains an outstanding problem. We employ temperature accelerated reactive molecular dynamics (TARMD) simulations to identify the kinetic pathways during thermal pyrolysis of polyethylene (PE). This allows for attainment of a dual objective viz. (1) clean fuel production via controlled hydrogen evolution and (2) formation of novel nanocarbon allotropes. Detailed atomistic picture of high temperature thermal decomposition that leads to partial or complete dehydrogenation of PE is presented. We identify the various reaction pathways for PE decomposition at high temperatures and demonstrate that a quenching-cooling strategy holds promise for tailoring the degree of graphitic order within the nanocarbon materials while simultaneously fine-tuning the evolution of clean fuel such as hydrogen gas. TARMD simulation trajectories elucidate the effect of simulated kinetic pathways on the reactive decomposition into hydrogen/flue gas/carbon, gas liquid solid phase separation of reaction products, interface dynamics, nucleation, and microstructural evolution of carbon particles. Depending on the quenching rate and the residual hydrogen content, we show that it is kinetically possible to control the reaction pathways and diffusion mechanisms and selectively produce a wide gamut of carbon allotropes (carbon onions, spheres, rods, graphene sheets to name a few). Suitable comparisons are made between simulation and our experimental results. Our simulations illustrate an environmental friendly strategy for controlled synthesis of nanocarbon materials and simultaneous clean energy production from nonbiodegradable products. C1 [Deshmukh, Sanket A.; Sankaranarayanan, Subramanian K. R. S.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Pol, Vilas G.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Kamath, Ganesh] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. RP Sankaranarayanan, SKRS (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM skrssank@anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Center for Electrical Energy Storage, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. V.G.P. was supported by the Center for Electrical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. Use of SEM facilities at the Center for Nanoscale Materials at Argonne National Laboratory is acknowledged. NR 30 TC 1 Z9 1 U1 2 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 8 PY 2014 VL 118 IS 18 BP 9706 EP 9714 DI 10.1021/jp4109317 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH1KL UT WOS:000335878900048 ER PT J AU Gamble, T Decker, K Plett, TS Pevarnik, M Pietschmann, JF Vlassiouk, I Aksimentiev, A Siwy, ZS AF Gamble, Trevor Decker, Karl Plett, Timothy S. Pevarnik, Matthew Pietschmann, Jan-Frederik Vlassiouk, Ivan Aksimentiev, Aleksei Siwy, Zuzanna S. TI Rectification of Ion Current in Nanopores Depends on the Type of Monovalent Cations: Experiments and Modeling SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SYNTHETIC CONICAL NANOPORES; AUREUS ALPHA-TOXIN; MOLECULAR-DYNAMICS; NANOFLUIDIC DIODE; SURFACE-CHARGE; LIPID BILAYERS; TRANSPORT; MEMBRANE; DEVICES; NANOPIPETTES AB Rectifying nanopores feature ion currents that are higher for voltages of one polarity compared to the currents recorded for corresponding voltages of the opposite polarity. Rectification of nanopores has been found to depend on the pore opening diameter and distribution of surface charges on the pore walls as well as pore geometry. Very little is known, however, on the dependence of ionic rectification on the type of transported ions of the same charge. We performed experiments with single conically shaped nanopores in a polymer film and recorded current-voltage curves in three electrolytes: LiCl, NaCl, and KCl. Rectification degrees of the pores, quantified as the ratio of currents recorded for voltages of opposite polarities, were the highest for KCl and the lowest for LiCl. The experimental observations could not be explained by a continuum modeling based on the Poisson-Nernst-Planck equations. All-atom molecular dynamics simulations revealed differential binding between Li+, Na+, and K+ ions and carboxyl groups on the pore walls, resulting in changes to both the effective surface charge of the nanopore and cation mobility within the pore. C1 [Gamble, Trevor; Plett, Timothy S.; Pevarnik, Matthew; Siwy, Zuzanna S.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Decker, Karl; Aksimentiev, Aleksei] Univ Illinois, Beckman Inst, Dept Phys, Urbana, IL 61820 USA. [Pietschmann, Jan-Frederik] Tech Univ Darmstadt, Darmstadt, Germany. [Vlassiouk, Ivan] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Siwy, Zuzanna S.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Siwy, Zuzanna S.] Univ Calif Irvine, Dept Biomed Engn, Irvine, CA 92697 USA. RP Aksimentiev, A (reprint author), Univ Illinois, Beckman Inst, Dept Phys, Urbana, IL 61820 USA. EM aksiment@illinois.edu; zsiwy@uci.edu RI Vlassiouk, Ivan/F-9587-2010; OI Vlassiouk, Ivan/0000-0002-5494-0386; Aksimentiev, Aleksei/0000-0002-6042-8442 FU Nanostructures for Electrical Energy Storage, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC0001160]; National Science Foundation [CHE-1306058, DMR-0955959]; National Institutes of Health [R01-HG007406]; XSEDE Allocation Grant [MCA05S028] FX Irradiation with swift heavy ions was performed at the GSI Helmholtzzentrum fur Schwerionenforschung GmbH, Darmstadt, Germany. T. Gamble, M. Pevarnik, and Z. Siwy were supported by the Nanostructures for Electrical Energy Storage, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences (Award DESC0001160), and the National Science Foundation (CHE-1306058). K. Decker and A. Aksimentiev were supported by grants from the National Science Foundation (DMR-0955959) and the National Institutes of Health (R01-HG007406). The authors gladly acknowledge supercomputer time provided through XSEDE Allocation Grant MCA05S028 and the Blue Waters petascale computing facility at the University of Illinois. The authors are very grateful for many discussions with Prof. Phillip Collins and Prof. Reginald Penner from the University of California, Irvine. NR 77 TC 19 Z9 19 U1 7 U2 71 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 8 PY 2014 VL 118 IS 18 BP 9809 EP 9819 DI 10.1021/jp501492g PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AH1KL UT WOS:000335878900058 PM 25678940 ER PT J AU Kadel, K Kumari, L Wang, XW Li, WZ Huang, JY Provencio, PP AF Kadel, Kamal Kumari, Latha Wang, Xuewen Li, Wenzhi Huang, Jian Yu Provencio, Paula Polyak TI Synthesis and structure of undoped and indium-doped thermoelectric lead telluride nanoparticles SO NANOSCALE RESEARCH LETTERS LA English DT Article DE Lead telluride; Nanostructure; Solvothermal/hydrothermal synthesis; First principle calculation ID SHAPE EVOLUTION; PBTE; NANOSTRUCTURES; SELENIDE; FIGURE; MERIT AB Undoped and indium (In)-doped lead telluride (PbTe) nanostructures were synthesized via solvothermal/hydrothermal route. The crystalline structure of the as-prepared undoped and In-doped PbTe samples was examined by X-ray diffraction (XRD) which indicated the formation of face-centered single-phase cubic crystal. A first principle calculation on indium doping shows that the indium atoms are more likely to replace lead (Pb) rather than to take the interstitial sites. Laser-induced breakdown spectroscopy (LIBS) analysis confirms that indium is incorporated into the PbTe matrix of the indium-doped PbTe samples. The effects of surfactant and synthesis temperature on the structure and morphology of the undoped PbTe were also investigated; it was found that PbTe nanostructures synthesized with the addition of surfactants exhibited uniform shapes and their size increased with the synthesis temperature. C1 [Kadel, Kamal; Kumari, Latha; Wang, Xuewen; Li, Wenzhi] Florida Int Univ, Dept Phys, Miami, FL 33199 USA. [Huang, Jian Yu; Provencio, Paula Polyak] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Wang, XW (reprint author), Florida Int Univ, Dept Phys, Miami, FL 33199 USA. EM sherwin@fiu.edu; Wenzhi.Li@fiu.edu RI Li, Wenzhi/J-6797-2016; OI Li, Wenzhi/0000-0001-8442-2232; Kumari, Latha/0000-0001-8820-6043 FU Florida International University under the Bridge [AWD000000001773]; American Chemical Society Petroleum Research Foundation [51766-ND10]; Center for Integrated Nanotechnologies at Sandia National Laboratories [U2009B032, C2011A1022] FX This work is supported by the Florida International University under the Bridge Grant AWD000000001773 and the American Chemical Society Petroleum Research Foundation under grant 51766-ND10. This work was performed, in part, at the Center for Integrated Nanotechnologies at Sandia National Laboratories under the user proposals U2009B032 and C2011A1022. NR 27 TC 5 Z9 5 U1 3 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1556-276X J9 NANOSCALE RES LETT JI Nanoscale Res. Lett. PD MAY 8 PY 2014 VL 9 AR 227 DI 10.1186/1556-276X-9-227 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA AH7SX UT WOS:000336335600001 PM 24872808 ER PT J AU Kathmann, SM Cho, H Chang, TM Schenter, GK Parab, K Autrey, T AF Kathmann, Shawn M. Cho, Herman Chang, Tsun-Mei Schenter, Gregory K. Parab, Kshitij Autrey, Tom TI Experimental and Theoretical Study of Molecular Response of Amine Bases in Organic Solvents SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID FRUSTRATED-LEWIS-PAIRS; QUADRUPOLE COUPLING-CONSTANTS; HYDROGEN ACTIVATION; CATALYTIC-HYDROGENATION; HYPERFINE-STRUCTURE; H-2 ACTIVATION; DYNAMICS; RELAXATION; LIQUIDS; TEMPERATURE AB Reorientational correlation times of various amine bases (namely, pyridine, 2,6-lutidine, 2,2,6,6-tetramethylpiperidine) and organic solvents (dichloromethane, toluene) were determined by solution-state NMR relaxation time measurements and compared with predictions from molecular dynamics (MD) simulations. The amine bases are reagents in complex reactions catalyzed by frustrated Lewis pairs (FLP), which display remarkable activity in metal-free H-2 scission. The comparison of measured and simulated correlation times is a key test of the ability of recent MD and quantum electronic structure calculations to elucidate the mechanism of FLP activity. Correlation times were found to be in the range of 1.4-3.4 (NMR) and 1.23-5.28 ps (MD) for the amines and 0.9-2.3 (NMR) and 0.2-1.7 ps (MD) for the solvent molecules. C1 [Kathmann, Shawn M.; Cho, Herman; Schenter, Gregory K.; Parab, Kshitij; Autrey, Tom] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Chang, Tsun-Mei] Univ Wisconsin Parkside, Dept Chem, Kenosha, WI 53141 USA. RP Kathmann, SM (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. EM shawn.kathmann@pnnl.gov RI Schenter, Gregory/I-7655-2014 OI Schenter, Gregory/0000-0001-5444-5484 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences FX This work benefited from discussions with Don Camaioni, Mark Bowden, Abhi Karkamkar, and Bojana Ginovska-Pangovska. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. NR 51 TC 9 Z9 9 U1 1 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 8 PY 2014 VL 118 IS 18 BP 4883 EP 4888 DI 10.1021/jp500821u PG 6 WC Chemistry, Physical SC Chemistry GA AH1KC UT WOS:000335878000018 PM 24694007 ER PT J AU Hauser, AJ Lucy, JM Gaultois, MW Ball, MR Soliz, JR Choi, Y Restrepo, OD Windl, W Freeland, JW Haskel, D Woodward, PM Yang, FY AF Hauser, Adam J. Lucy, Jeremy M. Gaultois, Michael W. Ball, Molly R. Soliz, Jennifer R. Choi, Yongseong Restrepo, Oscar D. Windl, Wolfgang Freeland, John W. Haskel, Daniel Woodward, Patrick M. Yang, Fengyuan TI Magnetic structure in epitaxially strained Sr2CrReO6 thin films by element-specific XAS and XMCD SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; ENERGY-LOSS SPECTROSCOPY; CIRCULAR-DICHROISM; TRANSITION-METALS; CURIE-TEMPERATURE; PEROVSKITES; OXIDES; CRO2 AB We have analyzed the magnetic configuration for highly ordered Sr2CrReO6 films as a function of epitaxial strain using magnetometry and x-ray magnetic circular dichroism (XMCD) measurements of Cr, Re, and O sites. The in-plane magnetic moments change significantly when tensile strain is applied. O K-edge XMCD indicates that O sites carry at least a portion of the bulk magnetization. Spin moment values measured for Cr match calculations incorporating spin-orbit effects, while both spin and orbital moments measured for Re sites are slightly higher than previously predicted. Finally, we discuss large changes in the x-ray absorption near-edge structure that are observed at the Cr and Re L edges due to epitaxial strain. C1 [Hauser, Adam J.] Univ Calif Santa Barbara, Calif Nanosyst Inst, Santa Barbara, CA 93106 USA. [Lucy, Jeremy M.; Yang, Fengyuan] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Gaultois, Michael W.] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. [Ball, Molly R.; Restrepo, Oscar D.; Windl, Wolfgang] Ohio State Univ, Dept Mat Sci & Engn, Columbus, OH 43210 USA. [Soliz, Jennifer R.; Woodward, Patrick M.] Ohio State Univ, Dept Chem, Columbus, OH 43210 USA. [Choi, Yongseong; Freeland, John W.; Haskel, Daniel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Hauser, AJ (reprint author), Univ Calif Santa Barbara, Calif Nanosyst Inst, Santa Barbara, CA 93106 USA. RI Hauser, Adam/G-2530-2012; Gaultois, Michael/D-2867-2009 OI Hauser, Adam/0000-0003-1752-0937; Gaultois, Michael/0000-0003-2172-2507 FU Center for Emergent Materials at The Ohio State University; NSF Materials Research Science and Engineering Center [DMR-0820414]; NanoSystems Laboratory at The Ohio State University; US Department of Energy, Office of Science [DE-AC02-06CH11357]; Elings Prize Fellowship; NSERC Postgraduate Scholarship; International Fulbright Science & Technology Award FX The authors gratefully acknowledge Richard Rosenberg for assistance in measurements at beamline 4-ID-C, Advanced Photon Source, Argonne National Laboratory. This work is supported by the Center for Emergent Materials at The Ohio State University, a NSF Materials Research Science and Engineering Center (Award No. DMR-0820414). Partial support is provided by the NanoSystems Laboratory at The Ohio State University. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. A.J.H. acknowledges support through an Elings Prize Fellowship of the California Nanosystems Institute at University of California, Santa Barbara. M.W.G. is supported by a NSERC Postgraduate Scholarship and an International Fulbright Science & Technology Award. NR 36 TC 3 Z9 3 U1 1 U2 41 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 8 PY 2014 VL 89 IS 18 AR 180402 DI 10.1103/PhysRevB.89.180402 PG 6 WC Physics, Condensed Matter SC Physics GA AG6NF UT WOS:000335534600001 ER PT J AU Ueland, BG Kreyssig, A Prokes, K Lynn, JW Harriger, LW Pratt, DK Singh, DK Heitmann, TW Sauerbrei, S Saunders, SM Mun, ED Bud'ko, SL McQueeney, RJ Canfield, PC Goldman, AI AF Ueland, B. G. Kreyssig, A. Prokes, K. Lynn, J. W. Harriger, L. W. Pratt, D. K. Singh, D. K. Heitmann, T. W. Sauerbrei, S. Saunders, S. M. Mun, E. D. Bud'ko, S. L. McQueeney, R. J. Canfield, P. C. Goldman, A. I. TI Fragile antiferromagnetism in the heavy-fermion compound YbBiPt SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM PHASE-TRANSITIONS; CRITICAL-POINT; MAGNETISM; TEMPERATURE; CRITICALITY; CECU6-XAUX; SURFACE; ELECTRON; BEHAVIOR; SYSTEMS AB We report results from neutron scattering experiments on single crystals of YbBiPt that demonstrate antiferromagnetic order characterized by a propagation vector, tau(AFM) = ( 1/2 1/2 1/2), and ordered moments that align along the [1 1 1] direction of the cubic unit cell. We describe the scattering in terms of a two-Gaussian peak fit, which consists of a narrower component that appears below T-N approximate to 0.4 K and corresponds to a magnetic correlation length of xi(n) approximate to 80 angstrom, and a broad component that persists up to T-* approximate to 0.7 K and corresponds to antiferromagnetic correlations extending over xi(b) approximate to 20 angstrom. Our results illustrate the fragile magnetic order present in YbBiPt and provide a path forward for microscopic investigations of the ground states and fluctuations associated with the purported quantum critical point in this heavy-fermion compound. C1 [Ueland, B. G.; Kreyssig, A.; Sauerbrei, S.; Saunders, S. M.; Mun, E. D.; Bud'ko, S. L.; McQueeney, R. J.; Canfield, P. C.; Goldman, A. I.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Ueland, B. G.; Kreyssig, A.; Sauerbrei, S.; Saunders, S. M.; Mun, E. D.; Bud'ko, S. L.; McQueeney, R. J.; Canfield, P. C.; Goldman, A. I.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Prokes, K.] Helmholtz Zentrum Berlin Mat & Energie, D-14109 Berlin, Germany. [Lynn, J. W.; Harriger, L. W.; Pratt, D. K.; Singh, D. K.] Natl Inst Stand & Technol, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Singh, D. K.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Heitmann, T. W.] Univ Missouri, Missouri Res Reactor, Columbia, MO 65211 USA. RP Ueland, BG (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RI Canfield, Paul/H-2698-2014; Ueland, Benjamin/B-2312-2008; McQueeney, Robert/A-2864-2016 OI Ueland, Benjamin/0000-0001-9784-6595; McQueeney, Robert/0000-0003-0718-5602 FU Department of Energy, Basic Energy Sciences, Division of Materials Sciences Engineering [DE-AC02-07CH11358] FX We thank R. Flint for useful discussions and gratefully acknowledge the Missouri University Research Reactor, Advanced Photon Source Argonne, Helmholtz-Zentrum Berlin fur Materialien und Energie, the National Institute of Standards and Technology, and the US Dept. of Commerce for the allocated beamtime and support during the experiments. Work at the Ames Laboratory was supported by the Department of Energy, Basic Energy Sciences, Division of Materials Sciences & Engineering, under Contract No. DE-AC02-07CH11358. NR 36 TC 5 Z9 5 U1 3 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 8 PY 2014 VL 89 IS 18 AR 180403 DI 10.1103/PhysRevB.89.180403 PG 5 WC Physics, Condensed Matter SC Physics GA AG6NF UT WOS:000335534600002 ER PT J AU Ejiri, H Elliott, SR AF Ejiri, H. Elliott, S. R. TI Charged current neutrino cross section for solar neutrinos, and background to beta beta(0 nu) experiments SO PHYSICAL REVIEW C LA English DT Article ID DOUBLE-BETA-DECAY; SPECTROSCOPY AB Solar neutrinos can interact with the source isotope in neutrinoless double-beta-decay experiments through charged-current and neutral-current interactions. The charged-current product nucleus will then beta decay with a Q value larger than the double-beta-decay Q value. As a result, this process can populate the region of interest and be a background to the double-beta-decay signal. We estimate the solar neutrino capture rates on three commonly used double-beta-decay isotopes, Ge-76, Te-130, and Xe-136. We then use the decay scheme of each product nucleus to estimate the possible background rates in those materials. As half-life sensitivities in future experiments approach 1 Chi 10(28) yr, this background will have to be considered although its rate will depend on detector design in addition to nuclear structure. C1 [Ejiri, H.] Osaka Univ, Res Ctr Nucl Phys, Osaka 5670047, Japan. [Elliott, S. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Ejiri, H (reprint author), Osaka Univ, Res Ctr Nucl Phys, Osaka 5670047, Japan. FU Office of Nuclear Physics in the Department of Energy, Office of Science; US Department of Energy through the LANL/LDRD Program FX We acknowledge support from the Office of Nuclear Physics in the Department of Energy, Office of Science. We gratefully acknowledge the support of the US Department of Energy through the LANL/LDRD Program. We thank D. Frekers and R.G.H. Robertson for valuable discussion. NR 27 TC 5 Z9 5 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 8 PY 2014 VL 89 IS 5 AR 055501 DI 10.1103/PhysRevC.89.055501 PG 7 WC Physics, Nuclear SC Physics GA AG6NU UT WOS:000335536200009 ER PT J AU Escher, JE Thompson, IJ Arbanas, G Elster, C Eremenko, V Hlophe, L Nunes, FM AF Escher, J. E. Thompson, I. J. Arbanas, G. Elster, Ch Eremenko, V. Hlophe, L. Nunes, F. M. CA TORUS Collaboration TI Reexamining surface-integral formulations for one-nucleon transfers to bound and resonance states SO PHYSICAL REVIEW C LA English DT Article ID DISTORTED-WAVE ANALYSIS; CHANNELS CALCULATIONS; DEUTERON; SCATTERING; MODELS AB One-nucleon transfer reactions, in particular (d, p) reactions, have played a central role in nuclear structure studies for many decades. Present theoretical descriptions of the underlying reaction mechanisms are insufficient for addressing the challenges and opportunities that are opening up with new radioactive beam facilities. We investigate a theoretical approach that was proposed recently to address shortcomings in the description of transfers to resonance states. The method builds on ideas from the very successful R-matrix theory; in particular, it uses a similar separation of the coordinate space into interior and exterior regions and introduces a parametrization that can be related to physical observables, which, in principle, makes it possible to extract meaningful spectroscopic information from experiments. We carry out calculations, for a selection of isotopes and energies, to test the usefulness of the new approach. C1 [Escher, J. E.; Thompson, I. J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Arbanas, G.] Oak Ridge Natl Lab, Reactor & Nucl Syst Div, Oak Ridge, TN 37831 USA. [Elster, Ch; Eremenko, V.; Hlophe, L.] Ohio Univ, Inst Nucl & Particle Phys, Athens, OH 45701 USA. [Elster, Ch; Eremenko, V.; Hlophe, L.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Eremenko, V.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. [Nunes, F. M.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Nunes, F. M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. RP Escher, JE (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM escher1@llnl.gov RI Elster, Charlotte/N-9845-2015 FU US Department of Energy's Topical Collaboration TORUS - auspices of the DOE by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Ohio University [DE-FG02-93ER40756, DE-SC0004087]; Michigan State University [DE-FG52-08NA28552, DE-SC0004084] FX This work is supported through the US Department of Energy's Topical Collaboration TORUS (www. reactiontheory. org). It is performed under the auspices of the DOE by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, by Ohio University under Contracts No. DE-FG02-93ER40756 and No. DE-SC0004087, and by Michigan State University under Contracts No. DE-FG52-08NA28552 and No. DE-SC0004084. Constructive input from Akram Mukhamdezhanov in the early stages of the project is acknowledged. NR 23 TC 2 Z9 2 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 8 PY 2014 VL 89 IS 5 AR 054605 DI 10.1103/PhysRevC.89.054605 PG 11 WC Physics, Nuclear SC Physics GA AG6NU UT WOS:000335536200007 ER PT J AU Davoudiasl, H Lee, HS Marciano, WJ AF Davoudiasl, Hooman Lee, Hye-Sung Marciano, William J. TI Muon g-2, rare kaon decays, and parity violation from dark bosons SO PHYSICAL REVIEW D LA English DT Article ID MOLLER SCATTERING ASYMMETRIES; ATOMIC CESIUM; RADIATIVE-CORRECTIONS; STANDARD MODEL; GAUGE BOSON; PHYSICS; SEARCH AB The muon g(mu) - 2 discrepancy between theory and experiment may be explained by a light vector boson Z(d) that couples to the electromagnetic current via kinetic mixing with the photon. We illustrate how the existing electron g(e) - 2, pion Dalitz decay, and other direct production data disfavor that explanation if the Z(d) mainly decays into e(+)e(-), mu(+)mu(-). Implications of a dominant invisible Z(d) decay channel, such as light dark matter, along with the resulting strong bounds from the rare K -> pi + missing energy decay are examined. The K decay constraints may be relaxed if destructive interference effects due to Z - Z(d) mass mixing are included. In that scenario, we show that accommodating the g(mu) - 2 data through relaxation of K decay constraints leads to interesting signals for dark parity violation. As an illustration, we examine the alteration of the weak mixing angle running at low Q(2), which can be potentially observable in polarized electron scattering or atomic physics experiments. C1 [Davoudiasl, Hooman; Marciano, William J.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Lee, Hye-Sung] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Lee, Hye-Sung] Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. RP Davoudiasl, H (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RI Lee, Hye-Sung/B-2208-2009 OI Lee, Hye-Sung/0000-0002-7333-3741 FU U.S. DOE [DE-AC02-98CH10886, DE-AC05-06OR23177]; NSF [PHY-1068008]; Gutenberg Research College FX We thank R. Essig for discussions. This work was supported in part by the U.S. DOE under Grants No. DE-AC02-98CH10886 and No. DE-AC05-06OR23177 and by the NSF under Grant No. PHY-1068008. W. M. acknowledges partial support as a Fellow in the Gutenberg Research College. H. L. appreciates hospitality during his visit to BNL. NR 88 TC 38 Z9 39 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 8 PY 2014 VL 89 IS 9 AR 095006 DI 10.1103/PhysRevD.89.095006 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AG6NX UT WOS:000335536500009 ER PT J AU Neufeld, RB Vitev, I Xing, HX AF Neufeld, R. B. Vitev, Ivan Xing, Hongxi TI Operator definition and derivation of collisional energy and momentum loss in relativistic plasmas SO PHYSICAL REVIEW D LA English DT Article ID QUARK-GLUON PLASMA; NUCLEAR-MATTER; P PLUS; LENGTH; LHC; JET; QCD AB We present an operator definition of the collisional energy and momentum loss suffered by an energetic charged particle in the presence of a medium. Our approach uses the energy-momentum tensor of the medium to evaluate the energy and momentum transfer rates. We apply this formalism to an energetic lepton or quark propagating in thermal electron-positron or quark-gluon plasmas, respectively. By using two different approaches to describe the energetic charged particle, an external current approach and a diagrammatic approach, we show explicitly that the operator method reproduces the known results for collisional energy loss from the scattering rate formalism. We further use our results to evaluate the collisional energy and momentum loss for the cases of heavy quark propagation through a quark-gluon plasma and energetic muon propagation in an electron-positron plasma produced in a high-intensity laser field. C1 [Neufeld, R. B.] Elect Magnet Applicat, Lakewood, CO 80226 USA. [Vitev, Ivan; Xing, Hongxi] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Xing, Hongxi] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. RP Neufeld, RB (reprint author), Elect Magnet Applicat, Lakewood, CO 80226 USA. EM bryon@ema3d.com; ivitev@lanl.gov; hxing@lanl.gov FU U.S. Department of Energy, Office of Science FX This work was supported in part by the U.S. Department of Energy, Office of Science. NR 60 TC 4 Z9 4 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 8 PY 2014 VL 89 IS 9 AR 096003 DI 10.1103/PhysRevD.89.096003 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AG6NX UT WOS:000335536500012 ER PT J AU Girlando, A Masino, M Schlueter, JA Drichko, N Kaiser, S Dressel, M AF Girlando, Alberto Masino, Matteo Schlueter, John A. Drichko, Natalia Kaiser, Stefan Dressel, Martin TI Charge-order fluctuations and superconductivity in two-dimensional organic metals SO PHYSICAL REVIEW B LA English DT Article ID BEDT-TTF; OPTICAL-PROPERTIES; BETA''-(ET)(2)SF5RSO3 R; PHYSICAL-PROPERTIES; CH2CF2; SPECTRA; CHFCF2; BIS(ETHYLENEDITHIO)TETRATHIAFULVALENE; COUNTERION; CONDUCTORS AB We report comprehensive Raman and infrared investigations of charge-order (CO) fluctuations in the organicmetal beta ''-(BEDT-TTF)(2)SF5CHFSO3 and superconductor beta ''-(BEDT-TTF)(2)SF5CH2CF2SO3. The chargesensitive vibrational bands are analyzed through an extension of the well-known Kubo model for the spectral signatures of an equilibrium between two states. At room temperature, both salts exhibit charge fluctuations between two differently charged molecular states with an exchange frequency of about 6 x 10(11) s(-1). The exchange rate of the metallic salt remains roughly constant down to 10 K, while in the superconductor, the exchange velocity starts to decrease below 200 K, and a "frozen" charge-ordered state emerges and coexists with the charge-order fluctuation state down to the superconducting temperature. These findings are confronted with other spectroscopic experiments, and a tentative phase diagram is proposed for the beta '' BEDT-TTF quarter-filled salts. C1 [Girlando, Alberto; Masino, Matteo] Univ Parma, Dipartimento Chim, I-43124 Parma, Italy. [Girlando, Alberto; Masino, Matteo] Univ Parma, INSTM UdR Parma, I-43124 Parma, Italy. [Schlueter, John A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Schlueter, John A.] Natl Sci Fdn, Div Mat Res, Arlington, VA 22230 USA. [Drichko, Natalia; Kaiser, Stefan; Dressel, Martin] Univ Stuttgart, Inst Phys 1, D-70550 Stuttgart, Germany. [Drichko, Natalia] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. RP Girlando, A (reprint author), Univ Parma, Dipartimento Chim, Parco Area Sci 17-a, I-43124 Parma, Italy. RI Dressel, Martin/D-3244-2012; Kaiser, Stefan/B-7788-2008; Masino, Matteo/O-5429-2015 OI Kaiser, Stefan/0000-0001-9862-2788; Masino, Matteo/0000-0002-5869-6800 FU Italian Ministry of University and Research (M.I.U.R.) under the project PRIN; Deutsche Forschungsgemeinschaft (DFG); Independent Research/Development program while serving at the National Science Foundation FX The work in Parma has been supported by the Italian Ministry of University and Research (M.I.U.R.) under the project PRIN-2010ERFKXL. We would like to thank the Deutsche Forschungsgemeinschaft (DFG) for financial support. N. Drichko acknowledges a support of Margarete von Wrangell Habilitationstipendium. J.A. Schlueter acknowledges support from the Independent Research/Development program while serving at the National Science Foundation. NR 37 TC 2 Z9 2 U1 1 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 8 PY 2014 VL 89 IS 17 AR 174503 DI 10.1103/PhysRevB.89.174503 PG 9 WC Physics, Condensed Matter SC Physics GA AG6MZ UT WOS:000335534000003 ER PT J AU Abdullah, M Albin, E DiFranzo, A Frate, M Pitcher, C Shimmin, C Upadhyay, S Walker, J Weatherly, P Fox, PJ Whiteson, D AF Abdullah, Mohammad Albin, Eric DiFranzo, Anthony Frate, Meghan Pitcher, Craig Shimmin, Chase Upadhyay, Suneet Walker, James Weatherly, Pierce Fox, Patrick J. Whiteson, Daniel TI Systematically searching for new resonances at the energy frontier using topological models SO PHYSICAL REVIEW D LA English DT Article ID COLLISIONS; TEV AB We propose a new strategy to systematically search for new physics processes in particle collisions at the energy frontier. An examination of all possible topologies which give identifiable resonant features in a specific final state leads to a tractable number of "topological models" per final state and gives specific guidance for their discovery. Using one specific final state, lljj, as an example, we find that the number of possibilities is reasonable and reveals simple, but as-yet-unexplored, topologies which contain significant discovery potential. We propose analysis techniques and estimate the sensitivity for pp collisions with root s = 14 TeV and L = 300 fb(-1) C1 [Abdullah, Mohammad; Albin, Eric; DiFranzo, Anthony; Frate, Meghan; Pitcher, Craig; Shimmin, Chase; Upadhyay, Suneet; Walker, James; Weatherly, Pierce; Whiteson, Daniel] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Fox, Patrick J.] Fermilab Natl Accelerator Lab, Batavia, IL 60615 USA. RP Abdullah, M (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. OI DiFranzo, Anthony/0000-0002-3151-9150 FU Department of Energy Office of Science; Alfred P. Sloan Foundation; Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy FX We acknowledge useful conversations with Tim Tait, Roni Harnik, and Bogdan Dobrescu. We are grateful to Felix Yu and Flip Tanedo for insightful commentary. D.W. is supported by grants from the Department of Energy Office of Science and by the Alfred P. Sloan Foundation. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 29 TC 2 Z9 2 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 7 PY 2014 VL 89 IS 9 AR 095002 DI 10.1103/PhysRevD.89.095002 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AP8SF UT WOS:000342348500004 ER PT J AU Koutroulakis, G Yasuoka, H Chudo, H Tobash, PH Mitchell, JN Bauer, ED Thompson, JD AF Koutroulakis, G. Yasuoka, H. Chudo, H. Tobash, P. H. Mitchell, J. N. Bauer, E. D. Thompson, J. D. TI Microscopic properties of the heavy-fermion superconductor PuCoIn5 explored by nuclear quadrupole resonance SO NEW JOURNAL OF PHYSICS LA English DT Article DE NQR; heavy-fermion; unconventional superconductivity; Pu-115s ID METALS; TEMPERATURE; RELAXATION; ELECTRONS; PUCOGA5; SPIN AB We report In-115 nuclear quadrupolar resonance (NQR) measurements on the heavy-fermion superconductor PuCoIn5, in the temperature range 0.29K <= T <= 75K. The NQR parameters for the two crystallographically inequivalent In sites are determined, and their temperature dependence is investigated. A linear shift of the quadrupolar frequency with lowering temperature below the critical value T-c is revealed, in agreement with the prediction for composite pairing. The nuclear spin-lattice relaxation rate T-1(-1) (T) clearly signals a superconducting (SC) phase transition at T-c similar or equal to 2.3 K, with strong spin fluctuations, mostly in-plane, dominating the relaxation process in the normal state near to T-c. Analysis of the T-1(-1) data in the SC state suggests that PuCoIn5 is a strong-coupling d-wave superconductor. C1 [Koutroulakis, G.; Yasuoka, H.; Chudo, H.; Tobash, P. H.; Mitchell, J. N.; Bauer, E. D.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Yasuoka, H.; Chudo, H.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. RP Koutroulakis, G (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM gkoutrou@lanl.gov RI Mitchell, Jeremy/E-2875-2010; OI Mitchell, Jeremy/0000-0001-7109-3505; Bauer, Eric/0000-0003-0017-1937 FU Glenn T Seaborg Institute; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Los Alamos Laboratory Directed Research and Development program FX We thank S E Brown for his insightful input, and R Flint, P Coleman and H Harima for helpful discussions. Work at Los Alamos National Laboratory was performed under the auspices of the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, and from the Los Alamos Laboratory Directed Research and Development program. G K and H Y acknowledge support from the Glenn T Seaborg Institute. NR 31 TC 6 Z9 6 U1 1 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 7 PY 2014 VL 16 AR 053019 DI 10.1088/1367-2630/16/5/053019 PG 12 WC Physics, Multidisciplinary SC Physics GA AL0VA UT WOS:000338843800010 ER PT J AU Ulman, K Bhaumik, D Wood, BC Narasimhan, S AF Ulman, Kanchan Bhaumik, Debarati Wood, Brandon C. Narasimhan, Shobhana TI Physical origins of weak H-2 binding on carbon nanostructures: Insight from ab initio studies of chemically functionalized graphene nanoribbons SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID HYDROGEN STORAGE; MOLECULAR SIMULATION; HALF-METALLICITY; CO2 ADSORPTION; DERIVATIVES; ADSORBENTS; NANOTUBE; SURFACE; EDGES; WATER AB We have performed ab initio density functional theory calculations, incorporating London dispersion corrections, to study the absorption of molecular hydrogen on zigzag graphene nanoribbons whose edges have been functionalized by OH, NH2, COOH, NO2, or H2PO3. We find that hydrogen molecules always preferentially bind at or near the functionalized edge, and display induced dipole moments. Binding is generally enhanced by the presence of polar functional groups. The largest gains are observed for groups with oxygen lone pairs that can facilitate local charge reorganization, with the biggest single enhancement in adsorption energy found for "strong functionalization" by H2PO3 (115 meV/H-2 versus 52 meV/H-2 on bare graphene). We show that for binding on the "outer edge" near the functional group, the presence of the group can introduce appreciable contributions from Debye interactions and higher-order multipole electrostatic terms, in addition to the dominant London dispersion interactions. For those functional groups that contain the OH moiety, the adsorption energy is linearly proportional to the number of lone pairs on oxygen atoms. Mixed functionalization with two different functional groups on a graphene edge can also have a synergistic effect, particularly when electron-donating and electron-withdrawing groups are combined. For binding on the "inner edge" somewhat farther from the functional group, most of the binding again arises from London interactions; however, there is also significant charge redistribution in the pi manifold, which directly reflects the electron donating or withdrawing capacity of the functional group. Our results offer insight into the specific origins of weak binding of gas molecules on graphene, and suggest that edge functionalization could perhaps be used in combination with other strategies to increase the uptake of hydrogen in graphene. They also have relevance for the storage of hydrogen in porous carbon materials, such as activated carbons. (C) 2014 AIP Publishing LLC. C1 [Ulman, Kanchan; Bhaumik, Debarati; Narasimhan, Shobhana] Jawaharlal Nehru Ctr Adv Sci Res, Theoret Sci Unit, Bangalore 560064, Karnataka, India. [Wood, Brandon C.] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. [Narasimhan, Shobhana] Jawaharlal Nehru Ctr Adv Sci Res, ICMS, Sheikh Saqr Lab, Bangalore 560064, Karnataka, India. RP Ulman, K (reprint author), Jawaharlal Nehru Ctr Adv Sci Res, Theoret Sci Unit, Bangalore 560064, Karnataka, India. FU BPCL India; CSIR India; DST Nanomission; JNCASR; (U.S.) Department of Energy (DOE) by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Helpful discussions with K. Ganapathy Ayappa are gratefully acknowledged. Funding was provided by BPCL India, CSIR India, DST Nanomission, and JNCASR. Computational facilities were provided by TUE-CMS, JNCASR. A portion of this work was performed under the auspices of the (U.S.) Department of Energy (DOE) by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 45 TC 5 Z9 5 U1 1 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2014 VL 140 IS 17 AR 174708 DI 10.1063/1.4873435 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AH3TI UT WOS:000336048000040 PM 24811656 ER PT J AU Yin, C Tyo, E Kuchta, K von Issendorff, B Vajda, S AF Yin, C. Tyo, E. Kuchta, K. von Issendorff, B. Vajda, S. TI Atomically precise (catalytic) particles synthesized by a novel cluster deposition instrument SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SIZE-SELECTED CLUSTERS; OXIDATIVE DEHYDROGENATION; HETEROGENEOUS CATALYSIS; ELECTRONIC-STRUCTURE; BEAM DEPOSITION; METAL-CLUSTERS; GOLD CLUSTERS; CO OXIDATION; SURFACES; TIO2 AB We report a new high vacuum instrument which is dedicated to the preparation of well-defined clusters supported on model and technologically relevant supports for catalytic and materials investigations. The instrument is based on deposition of size selected metallic cluster ions that are produced by a high flux magnetron cluster source. The throughput of the apparatus is maximized by collecting and focusing ions utilizing a conical octupole ion guide and a linear ion guide. The size selection is achieved by a quadrupole mass filter. The new design of the sample holder provides for the preparation of multiple samples on supports of various sizes and shapes in one session. After cluster deposition onto the support of interest, samples will be taken out of the chamber for a variety of testing and characterization. (C) 2014 AIP Publishing LLC. C1 [Yin, C.; Tyo, E.; Vajda, S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Kuchta, K.] Extrel CMS LLC, Pittsburgh, PA 15238 USA. [von Issendorff, B.] Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany. [Vajda, S.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. [Vajda, S.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Vajda, S.] Yale Univ, Sch Engn & Appl Sci, Dept Chem & Environm Engn, New Haven, CT 06520 USA. RP Vajda, S (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM vajda@anl.gov RI BM, MRCAT/G-7576-2011; von Issendorff, Bernd/B-1941-2015 OI von Issendorff, Bernd/0000-0002-4358-4494 FU U.S. Department of Energy, BES-Materials Sciences [DE-AC-02-06CH11357]; UChicago Argonne, LLC; U.S. Department of Energy, Scientific User Facilities [DE-AC-02-06CH11357] FX We would like to thank the following for technical assistance, Al Youngs (ANL), Steve Landers (ANL), and Jim Bulka (ANL) for their contributions at customizing and assembling vacuum and electrical components; Dr. Gihan Kwon for his assistance at assembly of the apparatus and technical drawings of the sample holder as well as its incorporation; and Dr. Sungsik Lee for developing the deposition monitoring software. The work at Argonne National Laboratory was supported by the U.S. Department of Energy, BES-Materials Sciences, under Contract No. DE-AC-02-06CH11357, with UChicago Argonne, LLC, the operator of Argonne National Laboratory. The work at the Advanced Photon Source was supported by the U.S. Department of Energy, Scientific User Facilities under Contract No. DE-AC-02-06CH11357 with UChicago Argonne LLC, the operator of Argonne National Laboratory. NR 47 TC 12 Z9 12 U1 7 U2 53 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2014 VL 140 IS 17 AR 174201 DI 10.1063/1.4871799 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AH3TI UT WOS:000336048000018 PM 24811634 ER PT J AU Gofryk, K Saparov, B Durakiewicz, T Chikina, A Danzenbacher, S Vyalikh, DV Graf, MJ Sefat, AS AF Gofryk, K. Saparov, B. Durakiewicz, T. Chikina, A. Danzenbaecher, S. Vyalikh, D. V. Graf, M. J. Sefat, A. S. TI Fermi-Surface Reconstruction and Complex Phase Equilibria in CaFe2As2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID SUPERCONDUCTIVITY AB Fermi-surface topology governs the relationship between magnetism and superconductivity in ironbased materials. Using low-temperature transport, angle-resolved photoemission, and x-ray diffraction, we show unambiguous evidence of large Fermi-surface reconstruction in CaFe2As2 at magnetic spin-densitywave and nonmagnetic collapsed-tetragonal (cT) transitions. For the cT transition, the change in the Fermisurface topology has a different character with no contribution from the hole part of the Fermi surface. In addition, the results suggest that the pressure effect in CaFe2As2 is mainly leading to a rigid-band-like change of the valence electronic structure. We discuss these results and their implications for magnetism and superconductivity in this material. C1 [Gofryk, K.; Saparov, B.; Sefat, A. S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Durakiewicz, T.; Graf, M. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Chikina, A.; Vyalikh, D. V.] St Petersburg State Univ, Dept Phys, St Petersburg 198504, Russia. [Chikina, A.; Danzenbaecher, S.; Vyalikh, D. V.] Tech Univ Dresden, Inst Solid State Phys, Dresden, Germany. RP Gofryk, K (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. RI Vyalikh, Denis/H-8044-2013; Chikina, Alla/M-4192-2015; Sefat, Athena/R-5457-2016; OI Vyalikh, Denis/0000-0001-9053-7511; Sefat, Athena/0000-0002-5596-3504; Gofryk, Krzysztof/0000-0002-8681-6857 FU U.S. Department of Energy; Basic Energy Sciences; Materials Sciences and Engineering Division; Department of Energy, Office of Basic Energy Sciences, and LANL LDRD programs; DFG [GRK1621, LA655/12-1] FX Work at ORNL was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. Department of Energy, Office of Basic Energy Sciences, and LANL LDRD programs supported work at LANL. A. C. and D. V. V. acknowledge the DFG grants GRK1621 and LA655/12-1. NR 42 TC 19 Z9 19 U1 3 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 7 PY 2014 VL 112 IS 18 AR 186401 DI 10.1103/PhysRevLett.112.186401 PG 5 WC Physics, Multidisciplinary SC Physics GA AH6NA UT WOS:000336246400005 PM 24856707 ER PT J AU Lovato, A Gandolfi, S Carlson, J Pieper, SC Schiavilla, R AF Lovato, A. Gandolfi, S. Carlson, J. Pieper, Steven C. Schiavilla, R. TI Neutral Weak Current Two-Body Contributions in Inclusive Scattering from C-12 SO PHYSICAL REVIEW LETTERS LA English DT Article ID MONTE-CARLO CALCULATIONS; FORM-FACTOR; NUCLEI; PROTON AB An ab initio calculation of the sum rules of the neutral weak response functions in C-12 is reported, based on a realistic Hamiltonian, including two-and three-nucleon potentials, and on realistic currents, consisting of one-and two-body terms. We find that the sum rules of the response functions associated with the longitudinal and transverse components of the (spacelike) neutral current are largest and that a significant portion (similar or equal to 30%) of the calculated strength is due to two-body terms. This fact may have implications for the MiniBooNE and other neutrino quasielastic scattering data on nuclei. C1 [Lovato, A.] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. [Lovato, A.; Pieper, Steven C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Gandolfi, S.; Carlson, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Schiavilla, R.] Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. [Schiavilla, R.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. RP Lovato, A (reprint author), Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. OI Lovato, Alessandro/0000-0002-2194-4954; Gandolfi, Stefano/0000-0002-0430-9035 FU U.S. Department of Energy [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357, DE-AC02-05CH11231, DE-AC0506OR23177]; NUCLEI SciDAC program; LANL LDRD program FX Under an award of computer time provided by the INCITE program, this research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. We also used resources provided by Los Alamos Open Supercomputing, by the National Energy Research Scientific Computing Center (NERSC), and by Argonne's LCRC. This research is supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contracts No. DE-AC02-06CH11357 (A. L. and S. C. P.), No. DE-AC02-05CH11231 (S. G. and J. C.), No. DE-AC0506OR23177 (R. S.), the NUCLEI SciDAC program, and by the LANL LDRD program. NR 49 TC 24 Z9 24 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 7 PY 2014 VL 112 IS 18 AR 182502 DI 10.1103/PhysRevLett.112.182502 PG 5 WC Physics, Multidisciplinary SC Physics GA AH6NA UT WOS:000336246400002 PM 24856692 ER PT J AU Nocek, B Starus, A Makowska-Grzyska, M Gutierrez, B Sanchez, S Jedrzejczak, R Mack, JC Olsen, KW Joachimiak, A Holz, RC AF Nocek, Boguslaw Starus, Anna Makowska-Grzyska, Magdalena Gutierrez, Blanca Sanchez, Stephen Jedrzejczak, Robert Mack, Jamey C. Olsen, Kenneth W. Joachimiak, Andrzej Holz, Richard C. TI The Dimerization Domain in DapE Enzymes Is required for Catalysis SO PLOS ONE LA English DT Article ID N-SUCCINYL-L,L-DIAMINOPIMELIC ACID DESUCCINYLASE; AEROMONAS-PROTEOLYTICA AMINOPEPTIDASE; HAEMOPHILUS-INFLUENZAE; LYSINE BIOSYNTHESIS; CRYSTAL-STRUCTURE; MACROMOLECULAR STRUCTURES; ANTIBIOTIC-RESISTANCE; SUBSTRATE-SPECIFICITY; MOLECULAR-DYNAMICS; SWISS-MODEL AB The emergence of antibiotic-resistant bacterial strains underscores the importance of identifying new drug targets and developing new antimicrobial compounds. Lysine and meso-diaminopimelic acid are essential for protein production and bacterial peptidoglycan cell wall remodeling and are synthesized in bacteria by enzymes encoded within dap operon. Therefore dap enzymes may serve as excellent targets for developing a new class of antimicrobial agents. The dapE-encoded N-succinyl-L, L-diaminopimelic acid desuccinylase (DapE) converts N-succinyl-L, L-diaminopimelic acid to L, L-diaminopimelic acid and succinate. The enzyme is composed of catalytic and dimerization domains, and belongs to the M20 peptidase family. To understand the specific role of each domain of the enzyme we engineered dimerization domain deletion mutants of DapEs from Haemophilus influenzae and Vibrio cholerae, and characterized these proteins structurally and biochemically. No activity was observed for all deletion mutants. Structural comparisons of wild-type, inactive monomeric DapE enzymes with other M20 peptidases suggest that the dimerization domain is essential for DapE enzymatic activity. Structural analysis and molecular dynamics simulations indicate that removal of the dimerization domain increased the flexibility of a conserved active site loop that may provide critical interactions with the substrate. C1 [Nocek, Boguslaw; Makowska-Grzyska, Magdalena; Joachimiak, Andrzej] Univ Chicago, Computat Inst, Ctr Struct Genom Infect Dis, Chicago, IL 60637 USA. [Starus, Anna; Gutierrez, Blanca; Sanchez, Stephen; Olsen, Kenneth W.] Loyola Univ, Dept Chem & Biochem, Chicago, IL 60611 USA. [Jedrzejczak, Robert; Mack, Jamey C.; Joachimiak, Andrzej] Argonne Natl Lab, Bioscie Div, Midwest Ctr Struct Genom, Lemont, IL USA. [Holz, Richard C.] Marquette Univ, Dept Chem, Milwaukee, WI 53233 USA. RP Joachimiak, A (reprint author), Univ Chicago, Computat Inst, Ctr Struct Genom Infect Dis, Chicago, IL 60637 USA. EM andrzejj@anl.gov; richard.holz@marquette.edu FU National Institutes of Health [R15 AI085559-01A1, GM094585, HHSN272200700058C, HHSN272201200026C]; National Science Foundation [CHE-1004430]; U.S. Department of Energy; Office of Biological and Environmental Research [DE-AC02-06CH11357] FX This research has been funded in part by grants from the National Institutes of Health R15 AI085559-01A1 (RCH), GM094585 (AJ), Contract HHSN272200700058C and HHSN272201200026C ( AJ), from the National Science Foundation CHE-1004430 (KWO), and by the U.S. Department of Energy, Office of Biological and Environmental Research, under Contract DE-AC02-06CH11357. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 41 TC 3 Z9 3 U1 0 U2 10 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 7 PY 2014 VL 9 IS 5 AR e93593 DI 10.1371/journal.pone.0093593 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG9HB UT WOS:000335728900006 PM 24806882 ER PT J AU Sizmur, T Lind, KR Benomar, S VanEvery, H Cademartiri, L AF Sizmur, Tom Lind, Kara R. Benomar, Saida VanEvery, Hannah Cademartiri, Ludovico TI A Simple and Versatile 2-Dimensional Platform to Study Plant Germination and Growth under Controlled Humidity SO PLOS ONE LA English DT Article ID ROOT ARCHITECTURE; ARABIDOPSIS; PAPER; SOIL; TOMOGRAPHY; BIOASSAYS; SYMBIOSIS; SYSTEM; YIELD; VIGOR AB We describe a simple, inexpensive, but remarkably versatile and controlled growth environment for the observation of plant germination and seedling root growth on a flat, horizontal surface over periods of weeks. The setup provides to each plant a controlled humidity (between 56% and 91% RH), and contact with both nutrients and atmosphere. The flat and horizontal geometry of the surface supporting the roots eliminates the gravitropic bias on their development and facilitates the imaging of the entire root system. Experiments can be setup under sterile conditions and then transferred to a non-sterile environment. The system can be assembled in 1-2 minutes, costs approximately 8.78$ per plant, is almost entirely reusable (0.43$ per experiment in disposables), and is easily scalable to a variety of plants. We demonstrate the performance of the system by germinating, growing, and imaging Wheat (Triticum aestivum), Corn (Zea mays), and Wisconsin Fast Plants (Brassica rapa). Germination rates were close to those expected for optimal conditions. C1 [Sizmur, Tom; Lind, Kara R.; Benomar, Saida; VanEvery, Hannah; Cademartiri, Ludovico] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Sizmur, Tom; Benomar, Saida; Cademartiri, Ludovico] Iowa State Univ, Ames Lab, US DOE, Ames, IA USA. [VanEvery, Hannah; Cademartiri, Ludovico] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA USA. RP Cademartiri, L (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM lcademar@iastate.edu RI Cademartiri, Ludovico/A-4142-2008; OI Cademartiri, Ludovico/0000-0001-8805-9434; Sizmur, Tom/0000-0001-9835-7195 FU Iowa State University FX This work was funded by Iowa State University through startup funds to LC. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 43 TC 2 Z9 2 U1 4 U2 43 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 7 PY 2014 VL 9 IS 5 AR e96730 DI 10.1371/journal.pone.0096730 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG9HB UT WOS:000335728900086 PM 24806462 ER PT J AU Van Essendelft, D Li, TW Nicoletti, P Jordan, T AF Van Essendelft, Dirk Li, Tingwen Nicoletti, Philip Jordan, Terry TI Advanced Chemistry Surrogate Model Development within C3M for CFD Modeling, Part 1: Methodology Development for Coal Pyrolysis SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID ENERGY CHAIN MODEL; ENTRAINED FLOW GASIFICATION; CHEMICAL PERCOLATION MODEL; DEVOLATILIZATION KINETICS; FLASHCHAIN THEORY; CONVERSION SUBMODELS; NUMERICAL-SIMULATION; OPERATING-CONDITIONS; DESIGN APPLICATIONS; ELEVATED PRESSURES AB A generalized method was developed to implement complex chemistry from third-party computational coal chemistry tools within multiphase, reacting computational fluid dynamic (CFD) codes. This method involves generating response surfaces that represent the computational coal chemistry tool output and using them to build a comprehensive surrogate model which can be easily incorporated into a CFD code. In this first part of a series of work, the method was applied to coal pyrolysis of Powder River Basin coal using PC Coal Lab (PCCL) and Carbonaceous Chemistry for Computational Modeling (C3M) to generate the series of response surfaces which form the basis of the surrogate model that can be implemented in CFD. This method has the benefit that local environmental variables (such as heating rate, final pyrolysis temperature, local pressure, and particle diameter) can be incorporated as part of the chemistry model in CFD on a cell by cell, time step by time step basis which creates the potential to significantly increase the accuracy of and reduce uncertainty in modeling coal chemistry within CFD. As demonstrated with this surrogate modeling method, the modeler is alleviated of the responsibility to predetermine a heating rate and reactor temperature for pyrolysis. This particular part of the work focuses on the theory and development of the surrogate model method. The methods used to generate the response surfaces, build them into a coherent surrogate model, and estimate the thermochemical properties of pseudocomponents are discussed. Future work and publication will focus on verification within CFD, validation against experimental data, multidimensional surrogate model development, and application of the surrogate model methodology to other reaction chemistry. C1 [Van Essendelft, Dirk; Li, Tingwen; Nicoletti, Philip; Jordan, Terry] Natl Energy Technol Lab, Morgantown, WV 26505 USA. [Li, Tingwen; Nicoletti, Philip] URS Corp, Morgantown, WV 26505 USA. RP Van Essendelft, D (reprint author), Natl Energy Technol Lab, Morgantown, WV 26505 USA. EM dirk.vanessendelft@netl.doe.gov RI madha nia, suci/K-9554-2014 OI madha nia, suci/0000-0001-7396-9945 FU agency of the United States Government FX This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference therein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed therein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 72 TC 3 Z9 3 U1 2 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAY 7 PY 2014 VL 53 IS 18 BP 7780 EP 7796 DI 10.1021/ie402678f PG 17 WC Engineering, Chemical SC Engineering GA AH1KJ UT WOS:000335878700049 ER PT J AU Uffalussy, KJ Miller, JB Howard, BH Stanko, DC Yin, CR Granite, EJ AF Uffalussy, Karen J. Miller, James B. Howard, Bret H. Stanko, Dennis C. Yin, Chunrong Granite, Evan J. TI Arsenic Adsorption on Copper-Palladium Alloy Films SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID FUEL GAS; MERCURY CAPTURE; GASIFICATION SYSTEMS; COMPOSITION SPREADS; METHANOL SYNTHESIS; CUXPD1-X ALLOYS; SORBENTS; REMOVAL; TEMPERATURE; CATALYSTS AB The adsorption of arsine by copper palladium alloys was studied using a high-throughput composition spread alloy film (CSAF) sample library. A CuxPd1-x, CSAF coupon that spanned the complete alloy composition space (x = 0-1) was prepared by an evaporative deposition technique. The coupon was exposed to AsH3 in a N-2 background at 288 degrees C in a small flow reactor. Arsenic uptake was characterized by scanning electron microscopy, energy-dispersive X-ray spectroscopy (SEM-EDX), and micro X-ray diffraction (mu-XRD). Pd- and Cu-rich alloy compositions exhibited large surface concentrations of As after exposure to AsH3. In the Cu-rich alloy, composition and structure measurements suggest the formation of a Cu3As phase. Arsenic uptake at Pd-rich alloy compositions is consistent with Pd2As or Pd8As3 phases; structural results suggest Pd2As with a hexagonal structure. In contrast, over a wide range of intermediate compositions (x(Cu) approximate to 0.20-0.75), little As uptake was observed. These results contribute to a basis for rational design of sorbents for the capture of arsenic from fluid streams, and to an understanding of the stability of palladium copper alloy membranes employed for hydrogen separation from coal-derived syngas. This work illustrates the application of high-throughput approaches based on CSAF sample libraries that can be applied to a wide variety of materials development and optimization challenges. C1 [Uffalussy, Karen J.; Howard, Bret H.; Stanko, Dennis C.; Granite, Evan J.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Miller, James B.; Yin, Chunrong] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Granite, Evan J.] Univ Pittsburgh, Chem & Petr Engn Dept, Pittsburgh, PA 15261 USA. RP Granite, EJ (reprint author), Natl Energy Technol Lab, POB 10940, Pittsburgh, PA 15236 USA. EM evan.granite@netl.doe.gov FU U.S. Department of Energy FX E.G. thanks Jenny Tennant and James Bennett (USDOE) for support of the research. Karen Uffalussy acknowledges the support of a postdoctoral fellowship at the U.S. Department of Energy, administered by Oak Ridge Institute for Science and Education (ORISE). NR 42 TC 6 Z9 6 U1 1 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAY 7 PY 2014 VL 53 IS 18 BP 7821 EP 7827 DI 10.1021/ie404447b PG 7 WC Engineering, Chemical SC Engineering GA AH1KJ UT WOS:000335878700052 ER PT J AU Bordonali, L Furukawa, Y Mariani, M Sabareesh, KPV Garlatti, E Carretta, S Lascialfari, A Timco, G Winpenny, REP Borsa, F AF Bordonali, L. Furukawa, Y. Mariani, M. Sabareesh, K. P. V. Garlatti, E. Carretta, S. Lascialfari, A. Timco, G. Winpenny, R. E. P. Borsa, F. TI Low temperature spin dynamics in Cr7Ni-Cu-Cr7Ni coupled molecular rings SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO AB Proton Nuclear Magnetic Resonance (NMR) relaxation measurements have been performed down to very low temperature (50 mK) to determine the effect of coupling two Cr7Ni molecular rings via a Cu2+ ion. No difference in the spin dynamics was found from nuclear spin lattice relaxation down to 1.5 K. At lower temperature, the H-1-NMR line broadens dramatically indicating spin freezing. From the plot of the line width vs. magnetization, it is found that the freezing temperature is higher (260 mK) in the coupled ring with respect to the single Cr7Ni ring (140 mK). (C) 2014 AIP Publishing LLC. C1 [Bordonali, L.; Mariani, M.; Sabareesh, K. P. V.; Lascialfari, A.; Borsa, F.] Univ Pavia, INSTM, I-27100 Pavia, Italy. [Bordonali, L.; Mariani, M.; Sabareesh, K. P. V.; Lascialfari, A.; Borsa, F.] Univ Pavia, Dept Phys, I-27100 Pavia, Italy. [Bordonali, L.; Furukawa, Y.; Borsa, F.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Bordonali, L.; Furukawa, Y.; Borsa, F.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Bordonali, L.] Univ Uniroma TRE, Dept Phys E Amaldi, Rome, Italy. [Garlatti, E.; Lascialfari, A.] Univ Milan, INSTM, I-20133 Milan, Italy. [Garlatti, E.; Lascialfari, A.] Univ Milan, Dept Phys, I-20133 Milan, Italy. [Garlatti, E.; Carretta, S.] Univ Parma, Dipartimento Fis, I-43100 Parma, Italy. [Carretta, S.; Lascialfari, A.] S3 CNR, Inst Nanosci, I-41125 Modena, Italy. [Timco, G.; Winpenny, R. E. P.] Univ Manchester, Lewis Magnetism Lab, Manchester M13 9PL, Lancs, England. RP Bordonali, L (reprint author), Univ Pavia, INSTM, Via Palestro 3, I-27100 Pavia, Italy. EM lorenzo.bordonali@unipv.it RI K. P. VELU, SABAREESH/E-4289-2016; OI K. P. VELU, SABAREESH/0000-0003-4793-3062; Garlatti, Elena/0000-0002-0370-0534 FU PRIN Italian Project, MIUR [2008PARRTS 001]; FIRB Italian Project "Futuro in Ricerca" [RBFR12RPD1] FX PRIN Italian Project No. 2008PARRTS 001 by MIUR and FIRB Italian Project "Futuro in Ricerca" No. RBFR12RPD1 were here credited for partly funding the present research. NR 8 TC 0 Z9 0 U1 0 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17E102 DI 10.1063/1.4853255 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700475 ER PT J AU Cadogan, JM Ryan, DH Mudryk, Y Pecharsky, VK Gschneidner, KA AF Cadogan, J. M. Ryan, D. H. Mudryk, Ya. Pecharsky, V. K. Gschneidner, K. A., Jr. TI On the magnetic order of Gd5Ge3 SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID NEUTRON POWDER DIFFRACTION AB We have investigated the magnetic structure of Gd5Ge3 by neutron powder diffraction down to 3.6 K. This compound presents three events in the heat capacity which we show are related to fundamental changes in the magnetic order. The primary antiferromagnetic ordering occurs at 82(2) K and produces a magnetic cell that is tripled with respect to the underlying orthorhombic crystal cell. The propagation vector is k(1) = [0 0 1/3]. At 74(2) K, the magnetic order becomes "anti-C" with a propagation vector k(2) = [1 0 0]. A third change in the magnetic order occurs at 40(2) K, and the new magnetic structure is essentially the "anti-C" structure but with the addition of a tripled magnetic component corresponding to a propagation vector k(3) = [1/3 0 0]. (C) 2014 AIP Publishing LLC. C1 [Cadogan, J. M.] Australian Def Force Acad, UNSW Canberra, Sch Phys Environm & Math Sci, Canberra, ACT 2610, Australia. [Ryan, D. H.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Ryan, D. H.] McGill Univ, Ctr Phys Mat, Montreal, PQ H3A 2T8, Canada. [Mudryk, Ya.; Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Mudryk, Ya.; Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Ryan, DH (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. EM dhryan@physics.mcgill.ca FU Natural Sciences and Engineering Research Council of Canada; Fonds Quebecois de la Recherche sur la Nature et les Technologies; University of New South Wales; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; Iowa State University FX Financial support for this work was provided by the Natural Sciences and Engineering Research Council of Canada, the Fonds Quebecois de la Recherche sur la Nature et les Technologies, and The University of New South Wales. Work at Ames Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358 with Iowa State University. NR 11 TC 2 Z9 2 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A901 DI 10.1063/1.4852055 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700145 ER PT J AU Cui, J Choi, JP Li, G Polikarpov, E Darsell, J Kramer, MJ Zarkevich, NA Wang, LL Johnson, DD Marinescu, M Huang, QZ Wu, H Vuong, NV Liu, JP AF Cui, J. Choi, J. P. Li, G. Polikarpov, E. Darsell, J. Kramer, M. J. Zarkevich, N. A. Wang, L. L. Johnson, D. D. Marinescu, M. Huang, Q. Z. Wu, H. Vuong, N. V. Liu, J. P. TI Development of MnBi permanent magnet: Neutron diffraction of MnBi powder SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID INTERMETALLIC COMPOUND; RAPID SOLIDIFICATION; PHASE AB MnBi attracts great attention in recent years for its great potential as permanent magnet materials. MnBi phase is difficult to obtain because of the rather drastic peritectic reaction between Mn and Bi. In this paper, we report our effort on synthesizing high purity MnBi compound using conventional powder metallurgical approaches. Neutron diffraction was carried out to investigate the crystal and nuclear structure of the obtained powder. The result shows that the purity of the obtained powder is about 91 wt. % at 300 K, and the magnetic moment of the Mn atom in MnBi lattice is 4.424 and 4.013 mu(B) at 50 K and 300 K, respectively. (C) 2014 AIP Publishing LLC. C1 [Cui, J.; Choi, J. P.; Li, G.; Polikarpov, E.; Darsell, J.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Kramer, M. J.; Zarkevich, N. A.; Wang, L. L.; Johnson, D. D.] Ames Lab, Mat Sci & Engn Div, Ames, IA 50011 USA. [Marinescu, M.] Electron Energy Corp, Landisville, PA 17538 USA. [Huang, Q. Z.; Wu, H.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Vuong, N. V.; Liu, J. P.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. RP Cui, J (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. EM jun.cui@pnnl.gov RI Wu, Hui/C-6505-2008; Zarkevich, Nikolai/A-3261-2013; OI Wu, Hui/0000-0003-0296-5204; Zarkevich, Nikolai/0000-0003-1919-0177; Johnson, Duane/0000-0003-0794-7283 FU U.S. Department of Energy's Advanced Research Projects Agency-Energy [11/CJ000/09/03] FX This research was supported by the U.S. Department of Energy's Advanced Research Projects Agency-Energy under Contract No. 11/CJ000/09/03. NR 13 TC 10 Z9 10 U1 5 U2 52 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A743 DI 10.1063/1.4867230 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700117 ER PT J AU Dattelbaum, DM Coe, JD Kiyanda, CB Gustavsen, RL Patterson, BM AF Dattelbaum, Dana M. Coe, Joshua D. Kiyanda, Charles B. Gustavsen, Richard L. Patterson, Brian M. TI Reactive, anomalous compression in shocked polyurethane foams SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID EQUATION-OF-STATE; P-ALPHA MODEL; POROUS MATERIALS; INTERFEROMETER; TOMOGRAPHY AB We present the results of plate impact experiments performed on 30%-75% porous, polymeric methylene diphenyl diisocyanate polyurethane foams. The combination of new data with those previously obtained on full-density material was used to calibrate complete equations-of-state under both inert and chemically reactive frameworks. Description of unreacted polyurethane was based on a combination of Hayes and P-alpha models, whereas its decomposition products were predicted via free energy minimization under the assumption of chemical and thermodynamic equilibrium. Correspondence of experiment and theory suggests that polyurethane at all densities decomposes when shocked above some threshold pressure, and that this threshold falls dramatically as a function of initial porosity. The shock locus of foams at 50% or less of theoretical maximum density was found "anomalous" in the sense that final volumes increased with pressure. We attribute this anomaly to chemical decomposition of the initial matrix to a mixture of small-molecule fluids and bulk carbon (graphite or diamond, depending on the initial density). (C) 2014 AIP Publishing LLC. C1 [Dattelbaum, Dana M.; Gustavsen, Richard L.; Patterson, Brian M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Coe, Joshua D.; Kiyanda, Charles B.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Dattelbaum, DM (reprint author), Los Alamos Natl Lab, MS P952, Los Alamos, NM 87545 USA. EM danadat@lanl.gov; jcoe@lanl.gov OI Gustavsen, Richard/0000-0002-2281-2742; Patterson, Brian/0000-0001-9244-7376 FU NNSA; United States Department of Energy [DE-AC52-06NA25396]; DOE/NNSA FX The authors thank David Stahl and Brian Bartram for target assembly, Lee Gibson, Adam Pacheco, and Ben Hollowell for help with firing the gas gun, Steve Sheffield and Sam Shaw for technical assistance, and Jeff Leiding for carefully reading the manuscript. J.D.C. and C. B. K. also thank the Magpie development group for interesting conversations. LANL is operated by Los Alamos National Security L. L. C. under the auspices of the NNSA and the United States Department of Energy, under Contract No. DE-AC52-06NA25396. Funding for this work was provided by DOE/NNSA. NR 49 TC 1 Z9 1 U1 5 U2 29 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 174908 DI 10.1063/1.4875478 PG 12 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700661 ER PT J AU Dong, S Li, W Huang, X Dagotto, E AF Dong, Shuai Li, Wei Huang, Xin Dagotto, Elbio TI First principles study of the magnetic properties of LaOMnAs SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID SUPERCONDUCTIVITY; MAGNETORESISTANCE AB Recent experiments reported giant magnetoresistance at room temperature in LaOMnAs. Here, a density functional theory calculation is performed to investigate magnetic properties of LaOMnAs. The ground state is found to be the G-type antiferromagnetic order within the ab plane but coupled ferromagnetically between planes, in agreement with recent neutron investigations. The electronic band structures suggest an insulating state which is driven by the particular G-type magnetic order, while a metallic state accompanies the ferromagnetic order. This relation between magnetism and conductance may be helpful to qualitatively understand the giant magnetoresistance effects. (C) 2014 AIP Publishing LLC. C1 [Dong, Shuai; Huang, Xin] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. [Dong, Shuai; Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Dong, Shuai; Dagotto, Elbio] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Li, Wei] Chinese Acad Sci, Inst Microsyst & Informat Technol, Shanghai Ctr Superconduct, Shanghai 200050, Peoples R China. [Li, Wei] Chinese Acad Sci, Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China. [Li, Wei] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. RP Dong, S (reprint author), Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. EM sdong@seu.edu.cn RI Dong (董), Shuai (帅)/A-5513-2008 OI Dong (董), Shuai (帅)/0000-0002-6910-6319 FU 973 Projects of China [2011CB922101]; NSFC [11274060, 51322206]; National Science Foundation [DMR-1104386] FX Work was supported by the 973 Projects of China (No. 2011CB922101) and NSFC (Nos. 11274060 and 51322206). E. D. was supported by the National Science Foundation Grant No. DMR-1104386. NR 22 TC 3 Z9 3 U1 1 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17D723 DI 10.1063/1.4867757 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700455 ER PT J AU Du, H Yan, F Young, M To, B Jiang, CS Dippo, P Kuciauskas, D Chi, ZH Lund, EA Hancock, C Hlaing, OOWM Scarpulla, MA Teeter, G AF Du, Hui Yan, Fei Young, Matthew To, Bobby Jiang, Chun-Sheng Dippo, Pat Kuciauskas, Darius Chi, Zhenhuan Lund, Elizabeth A. Hancock, Chris Hlaing, Win Maw O. O. Scarpulla, Mike A. Teeter, Glenn TI Investigation of combinatorial coevaporated thin film Cu2ZnSnS4. I. Temperature effect, crystalline phases, morphology, and photoluminescence SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID SOLAR-CELLS; HIGH-EFFICIENCY AB Cu2ZnSnS4 is a promising low-cost, nontoxic, earth-abundant absorber material for thin-film solar cell applications. In this study, combinatorial coevaporation was used to synthesize individual thin-film samples spanning a wide range of compositions at low (325 degrees C) and high (475 degrees C) temperatures. Film composition, grain morphology, crystalline-phase and photo-excitation information have been characterized by x-ray fluorescence, scanning electron microscopy, x-ray diffraction, Raman spectroscopy, and photoluminescence imaging and mapping. Highly textured columnar grain morphology is observed for film compositions along the ZnS-Cu2ZnSnS4-Cu2SnS3 tie line in the quasi-ternary Cu2S-ZnS-SnS2 phase system, and this effect is attributed to structural similarity between the Cu2ZnSnS4, Cu2SnS3, and ZnS crystalline phases. At 475 degrees C growth temperature, Sn-S phases cannot condense because of their high vapor pressures. As a result, regions that received excess Sn flux during growth produced compositions falling along the ZnS-Cu2ZnSnS4-Cu2SnS3 tie line. Room-temperature photoluminescence imaging reveals a strong correlation for these samples between film composition and photoluminescence intensity, where film regions with Cu/Sn ratios greater than similar to 2 show strong photoluminescence intensity, in comparison with much weaker photoluminescence in regions that received excess Sn flux during growth or subsequent processing. The observed photoluminescence quenching in regions that received excess Sn flux is attributed to the effects of Sn-related native point defects in Cu2ZnSnS4 on non-radiative recombination processes. Implications for processing and performance of Cu2ZnSnS4 solar cells are discussed. (C) 2014 AIP Publishing LLC. C1 [Du, Hui; Yan, Fei; Young, Matthew; To, Bobby; Jiang, Chun-Sheng; Dippo, Pat; Kuciauskas, Darius; Teeter, Glenn] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Chi, Zhenhuan] Renishaw Inc, Hoffman Estates, IL 60192 USA. [Lund, Elizabeth A.; Hancock, Chris; Hlaing, Win Maw O. O.; Scarpulla, Mike A.] Univ Utah, Dept Chem Engn, Salt Lake City, UT 84112 USA. [Lund, Elizabeth A.; Hancock, Chris; Hlaing, Win Maw O. O.; Scarpulla, Mike A.] Univ Utah, Dept Elect & Comp Engn, Salt Lake City, UT 84112 USA. [Lund, Elizabeth A.; Hancock, Chris; Hlaing, Win Maw O. O.; Scarpulla, Mike A.] Univ Utah, Dept Mat Sci & Engn, Salt Lake City, UT 84112 USA. RP Teeter, G (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy,MS3218, Golden, CO 80401 USA. EM glenn.teeter@nrel.gov RI jiang, chun-sheng/F-7839-2012 FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 28 TC 11 Z9 11 U1 4 U2 44 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 173502 DI 10.1063/1.4871664 PG 11 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700600 ER PT J AU Flint, CL Grutter, AJ Jenkins, CA Arenholz, E Suzuki, Y AF Flint, C. L. Grutter, A. J. Jenkins, C. A. Arenholz, E. Suzuki, Y. TI Magnetism in CaMnO3 thin films SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO AB Epitaxial CaMnO3 thin films on (001) LaAlO3, (LaAlO3)(0.3)(Sr2AlTaO6)(0.7), and SrTiO3 were synthesized in a range of strain states from coherently strained on LaAlO3 (1.6% strain) to fully relaxed on SrTiO3. We observed a magnetic ordering transition in CaMnO3 thin films suppressed from the Neel temperature of bulk CaMnO3 with the suppression increasing with increasing strain in the thin film. In contrast to bulk studies, our CaMnO3 films do not exhibit any sign of weak ferromagnetism according to field-dependent magnetization and x-ray magnetic circular dichroism measurements. Therefore, to within experimental resolution, all of our CaMnO3 films are antiferromagnetic with negligible oxygen off-stoichiometry. (C) 2014 AIP Publishing LLC. C1 [Flint, C. L.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Flint, C. L.; Grutter, A. J.; Suzuki, Y.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Grutter, A. J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Grutter, A. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Jenkins, C. A.; Arenholz, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Suzuki, Y.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. RP Flint, CL (reprint author), Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. EM cflint@stanford.edu FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-SC0008505, DE-AC02-05CH11231] FX This research was funded by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy (DE-SC0008505 and DE-AC02-05CH11231). The work at the Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy (DE-AC02-05CH11231). NR 14 TC 1 Z9 1 U1 4 U2 48 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17D712 DI 10.1063/1.4864044 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700444 ER PT J AU Fu, H Hadimani, RL Ma, Z Wang, MX Teng, BH Jiles, DC AF Fu, H. Hadimani, R. L. Ma, Z. Wang, M. X. Teng, B. H. Jiles, D. C. TI Magnetocaloric effect in GdCoxAl2-x system for (0.15 <= x <= 1) compositions SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO AB Structure and magnetic properties of the GdAl2-GdCo2 system including magnetocaloric effect have been investigated for various compositions. The as-cast GdCoxAl2-x alloys prepared by arc-melting crystallize in the dual-phase structure of cubic MgCu2-type and hexagonal MgZn2-type phases. All the as-cast dual-phase alloys exhibit only one magnetic phase transition near 77K even though two ferrimagnetic phases coexist. The magnetic transition was broadened by the continuous transitions of the component phases, which resulted in enhancement of relative cooling power at the expense of the magnetic entropy changes. (C) 2014 AIP Publishing LLC. C1 [Fu, H.; Ma, Z.; Wang, M. X.; Teng, B. H.] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. [Hadimani, R. L.; Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Hadimani, R. L.; Jiles, D. C.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Hadimani, RL (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. EM hadimani@iastate.edu FU National Natural Science Foundation of China [51271049]; Fundamental Research Funds for the Central Universities [ZYGX2010J050] FX This work was supported by the National Natural Science Foundation of China (No. 51271049) and the Fundamental Research Funds for the Central Universities (No. ZYGX2010J050). NR 7 TC 3 Z9 3 U1 3 U2 29 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A914 DI 10.1063/1.4863167 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700158 ER PT J AU Hadimani, RL Mudryk, Y Prost, TE Pecharsky, VK Gschneidner, KA Jiles, DC AF Hadimani, R. L. Mudryk, Y. Prost, T. E. Pecharsky, V. K. Gschneidner, K. A. Jiles, D. C. TI Growth and characterization of Pt-protected Gd5Si4 thin films SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID GD AB Successful growth and characterization of thin films of giant magnetocaloric Gd-5(SixGe1-x)(4) were reported in the literature with limited success. The inherent difficulty in producing this complex material makes it difficult to characterize all the phases present in the thin films of this material. Therefore, thin film of binary compound of Gd5Si4 was deposited by pulsed laser deposition. It was then covered with platinum on the top of the film to protect against any oxidation when the film was exposed to ambient conditions. The average film thickness was measured to be approximately 350 nm using a scanning electron microscopy, and the composition of the film was analyzed using energy dispersive spectroscopy. X-ray diffraction analysis indicates the presence of Gd5Si4 orthorhombic structure along with Gd5Si3 secondary phase. The transition temperature of the film was determined from magnetic moment vs. temperature measurement. The transition temperature was between 320 and 345 K which is close to the transition temperature of the bulk material. Magnetic moment vs. magnetic field measurement confirmed that the film was ferromagnetic below 342 K. (C) 2014 AIP Publishing LLC. C1 [Hadimani, R. L.; Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Mudryk, Y.; Prost, T. E.; Pecharsky, V. K.; Gschneidner, K. A.] US DOE, Mat & Engn Phys Program, Ames Lab, Ames, IA 50011 USA. [Pecharsky, V. K.; Gschneidner, K. A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Hadimani, RL (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. EM hadimani@iastate.edu FU DOE-Basic Energy Sciences [DE-AC02-07CH11358]; Barbara and James Palmer Endowment at the Department of Electrical and Computer Engineering of Iowa State Universit FX This work at the Ames Laboratory was supported by the DOE-Basic Energy Sciences under Contract No. DE-AC02-07CH11358 and Barbara and James Palmer Endowment at the Department of Electrical and Computer Engineering of Iowa State University. The authors acknowledge the contributions of A. H. Shaw and K. W. Dennis of Ames Laboratory, U. S. DOE for helping with the PLD and SQUID measurements, respectively. NR 8 TC 5 Z9 5 U1 1 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17C113 DI 10.1063/1.4865322 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700304 ER PT J AU Hoffmann, A AF Hoffmann, Axel TI Preface to Special Topic: Invited Papers of the 58th Annual Conference on Magnetism and Magnetic Materials, Denver, Colorado, USA, November 2013 SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO C1 Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Hoffmann, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM hoffmann@anl.gov RI Hoffmann, Axel/A-8152-2009 OI Hoffmann, Axel/0000-0002-1808-2767 NR 1 TC 0 Z9 0 U1 0 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 172501 DI 10.1063/1.4871338 PG 1 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700569 ER PT J AU Hoffmann, A AF Hoffmann, Axel TI Preface: Proceedings of the 58th Annual Conference on Magnetism and Magnetic Materials, Denver, Colorado, USA, November 2013 SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO C1 Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Hoffmann, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM hoffmann@anl.gov RI Hoffmann, Axel/A-8152-2009 OI Hoffmann, Axel/0000-0002-1808-2767 NR 0 TC 1 Z9 1 U1 1 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A101 DI 10.1063/1.4871439 PG 2 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700001 ER PT J AU Jiang, YF Al Mehedi, M Fu, EG Wang, YQ Wang, JP AF Jiang, Yanfeng Al Mehedi, Md Fu, Engang Wang, Yongqiang Wang, Jian-Ping TI FeN foils by nitrogen ion-implantation SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID SINGLE-CRYSTAL FE16N2; MOLECULAR-BEAM EPITAXY; FILMS; ALPHA-FE16N2; PHASE; IRON; TRANSFORMATION; MAGNETIZATION; THICKNESS AB Iron nitride samples in foil shape (free standing, 500 nm in thickness) were prepared by a nitrogen ion-implantation method. To facilitate phase transformation, the samples were bonded on the substrate followed by a post-annealing step. By using two different substrates, single crystal Si and GaAs, structural and magnetic properties of iron nitride foil samples prepared with different nitrogen ion fluences were characterized. alpha ''-Fe16N2 phase in iron nitride foil samples was obtained and confirmed by the proposed approach. A hard magnetic property with coercivity up to 780 Oe was achieved for the FeN foil samples bonded on Si substrate. The feasibility of using nitrogen ion implantation techniques to prepare FeN foil samples up to 500 nm thickness with a stable martensitic phase under high ion fluences has been demonstrated. A possible mechanism was proposed to explain this result. This proposed method could potentially be an alternative route to prepare rare-earth-free FeN bulk magnets by stacking and pressing multiple free-standing thick alpha ''-Fe16N2 foils together. (C) 2014 AIP Publishing LLC. C1 [Jiang, Yanfeng; Wang, Jian-Ping] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. [Al Mehedi, Md] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [Fu, Engang; Wang, Yongqiang] Los Alamos Natl Lab, Ion Beam Mat Lab, Los Alamos, NM 87545 USA. RP Wang, JP (reprint author), Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. EM jpwang@umn.edu FU ARPA-E (Advanced Research Projects Agency-Energy) project [0472-1595]; NSF MRSEC facility program; Center for Integrated Nanotechnologies (CINT) FX This work was supported in part by ARPA-E (Advanced Research Projects Agency-Energy) project under the Contract No. 0472-1595 and NSF MRSEC facility program. Ion implantation was supported by the Center for Integrated Nanotechnologies (CINT), a US Department of Energy nanoscience user facility jointly operated by Los Alamos and Sandia National Laboratories. NR 23 TC 4 Z9 4 U1 9 U2 37 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A753 DI 10.1063/1.4868492 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700127 ER PT J AU Jiang, YF Dabade, V Brady, MP Rios, O James, RD Wang, JP AF Jiang, Yanfeng Dabade, Vivekanand Brady, Michael P. Rios, Orlando James, Richard D. Wang, Jian-Ping TI 9 T high magnetic field annealing effects on FeN bulk sample SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID SINGLE-CRYSTAL FE16N2; MOLECULAR-BEAM EPITAXY; FILMS; ALPHA-FE16N2; TRANSFORMATION; ALLOYS; MOMENT; PHASE; IRON AB alpha ''-Fe16N2 has been suggested as a promising candidate for future rare-earth-free magnets. In this paper, we report to use high magnetic field (9 T) assisted post-annealing process to enhance the Fe16N2 phase formation in FeN bulk rod samples during the alpha' -> alpha '' phase transformation and thus improve its magnetic properties. It was found by X-ray Diffraction measurement that the volume ratio of Fe16N2 phase was increased up to 22%, which corresponds to an increase in the amount of transformation from alpha' -> alpha '' up to 78%. Also, the saturation magnetization (M-s) of the prepared FeN rod sample was increased to 227 emu/g with its coercivity up to 376 Oe at room temperature. A working mechanism for the high field assisted post-annealing process was presented. (C) 2014 AIP Publishing LLC. C1 [Jiang, Yanfeng; Wang, Jian-Ping] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. [Dabade, Vivekanand; James, Richard D.] Univ Minnesota, Dept Aerosp Engn & Mech, Minneapolis, MN 55455 USA. [Brady, Michael P.; Rios, Orlando] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Wang, JP (reprint author), Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. EM jpwang@umn.edu RI Brady, Michael/A-8122-2008; Rios, Orlando/E-6856-2017 OI Brady, Michael/0000-0003-1338-4747; Rios, Orlando/0000-0002-1814-7815 FU ARPA-E (Advanced Research Projects Agency. Energy) project [0472-1595]; NSF MRSEC facility program FX This work was supported in part by ARPA-E (Advanced Research Projects Agency. Energy) project under Contract No. 0472-1595 and NSF MRSEC facility program. NR 24 TC 4 Z9 4 U1 3 U2 37 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A758 DI 10.1063/1.4868493 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700132 ER PT J AU Lendinez, S Jain, S Novosad, V Fradin, FY Pearson, JE Tejada, J Bader, SD AF Lendinez, Sergi Jain, Shikha Novosad, Valentyn Fradin, Frank Y. Pearson, John E. Tejada, Javier Bader, Samuel D. TI Dynamic decay of a single vortex into vortex-antivortex pairs SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID CORE REVERSAL; CIRCULAR DOTS; PERMALLOY; MAGNETIZATION; EXCITATION; NANODISKS AB A variety of metastable states, including vortices, antivortices, and their combinations, is typical for magnetically soft, thin films and patterned structures. The physics of individual spin vortices in patterned structures has been rather extensively explored. In contrast, there are few studies of the vortex-antivortex-vortex (v-av-v) system, in part because the configuration is rather challenging to obtain experimentally. We demonstrate herein how a recently proposed resonant-spin-ordering technique can be used to induce the dynamic decay of a single vortex into v-av states in elongated elements. The approach is based on first driving the system from the linear regime of constant vortex gyrations to the non-linear regime of vortex-core reversals at a fixed excitation frequency, and then subsequently reducing the excitation field back to the linear regime. This procedure stabilizes the system into a v-av-v state that is completely decoupled from the initialization excitation frequency. The newly acquired state is stable in remanence. The dynamic response of this system is expected to demonstrate a number of collective modes, depending on the combination of the vortex core polarities, and/or the excitation field direction, and, hence, is of interest for future studies. (C) 2014 AIP Publishing LLC. C1 [Lendinez, Sergi; Jain, Shikha; Novosad, Valentyn; Fradin, Frank Y.; Pearson, John E.; Bader, Samuel D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Lendinez, Sergi; Tejada, Javier] Univ Barcelona, Dept Fis Fonamental, E-08028 Barcelona, Spain. [Bader, Samuel D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Novosad, V (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM novosad@anl.gov RI Novosad, Valentyn/C-2018-2014; Tejada, Javier/A-5832-2009; Novosad, V /J-4843-2015; OI Tejada, Javier/0000-0001-9246-5566; Lendinez, Sergi/0000-0002-7360-1857 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; FPU of Ministerio de Educacion, Cultura y Deporte of the Spanish Government FX Work at Argonne and use of the Center for Nanoscale Materials were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. S. L. acknowledges financial support from the FPU Program of Ministerio de Educacion, Cultura y Deporte of the Spanish Government. NR 32 TC 3 Z9 3 U1 1 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17D121 DI 10.1063/1.4862219 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700399 ER PT J AU Lin, SZ AF Lin, Shi-Zeng TI Mutual synchronization of two stacks of intrinsic Josephson junctions in cuprate superconductors SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID THZ RADIATION; PHASE-LOCKING; ARRAYS; PLASMA; EMISSION; EMITTERS; FLOW AB Certain high-T-c cuprate superconductors, which naturally realize a stack of Josephson junctions, thus can be used to generate electromagnetic waves in the terahertz region. A plate-like single crystal with 10(4) junctions without cavity resonance was proposed to achieve strong radiation. For this purpose, it is required to synchronize the Josephson plasma oscillation in all junctions. In this work, we propose to use two stacks of junctions shunted in parallel to achieve synchronization. The two stacks are mutually synchronized in the whole IV curve, and there is a phase shift between the plasma oscillation in the two stacks. The phase shift is nonzero when the number of junctions in different stacks is the same, while it can be arbitrary when the number of junctions is different. This phase shift can be tuned continuously by applying a magnetic field when all the junctions are connected by superconducting wires. (C) 2014 AIP Publishing LLC. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, SZ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008 OI Lin, Shi-Zeng/0000-0002-4368-5244 FU NNSA of the U.S. DOE at LANL [DE-AC52-06NA25396] FX We thank L. N. Bulaevskii for useful discussions. This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Award No. DE-AC52-06NA25396. NR 47 TC 6 Z9 6 U1 2 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 173901 DI 10.1063/1.4874677 PG 6 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700616 ER PT J AU Lin, SZ Reichhardt, C Batista, CD Saxena, A AF Lin, Shi-Zeng Reichhardt, Charles Batista, Cristian D. Saxena, Avadh TI Dynamics of skyrmions in chiral magnets: Dynamic phase transitions and equation of motion SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID LATTICE; CRYSTALS; STATES; MNSI AB We study the dynamics of skyrmions in a metallic chiral magnet. First, we show that skyrmions can be created dynamically by destabilizing the ferromagnetic background state through a spin polarized current. We then treat skyrmions as rigid particles and derive the corresponding equation of motion. The dynamics of skyrmions is dominated by the Magnus force, which accounts for the weak pinning of skyrmions observed in experiments. Finally, we discuss the quantum motion of skyrmions. (C) 2014 AIP Publishing LLC. C1 [Lin, Shi-Zeng; Reichhardt, Charles; Batista, Cristian D.; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, SZ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM szl@lanl.gov RI Lin, Shi-Zeng/B-2906-2008; Batista, Cristian/J-8008-2016 OI Lin, Shi-Zeng/0000-0002-4368-5244; FU Los Alamos Laboratory Directed Research and Development Program [20110181ER] FX Computer resources for numerical calculations were provided by the Institutional Computing Program in LANL. This publication was made possible by funding from the Los Alamos Laboratory Directed Research and Development Program, Project No. 20110181ER. NR 28 TC 4 Z9 4 U1 0 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17D109 DI 10.1063/1.4861576 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700387 ER PT J AU Liu, T Chang, HC Vlaminck, V Sun, YY Kabatek, M Hoffmann, A Deng, LJ Wu, MZ AF Liu, Tao Chang, Houchen Vlaminck, Vincent Sun, Yiyan Kabatek, Michael Hoffmann, Axel Deng, Longjiang Wu, Mingzhong TI Ferromagnetic resonance of sputtered yttrium iron garnet nanometer films SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID FERRITE THIN-FILMS; MAGNETIC-PROPERTIES; ULTRATHIN FILMS; LASER DEPOSITION; YIG; LINEWIDTH; INSULATOR; GROWTH AB Growth of nm-thick yttrium iron garnet (YIG) films by sputtering and ferromagnetic resonance (FMR) properties in the films were studied. The FMR linewidth of the YIG film decreased as the film thickness was increased from several nanometers to about 100 nm. For films with very smooth surfaces, the linewidth increased linearly with frequency. In contrast, for films with big grains on the surface, the linewidth-frequency response was strongly nonlinear. Films in the 7-26 nm thickness range showed a surface roughness between 0.1 nm and 0.4nm, a 9.48-GHz FMR linewidth in the 6-10Oe range, and a damping constant of about 0.001. (C) 2014 AIP Publishing LLC. C1 [Liu, Tao; Chang, Houchen; Sun, Yiyan; Kabatek, Michael; Wu, Mingzhong] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. [Liu, Tao; Deng, Longjiang] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Peoples R China. [Vlaminck, Vincent; Hoffmann, Axel] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Wu, MZ (reprint author), Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. EM mwu@lamar.colostate.edu RI Hoffmann, Axel/A-8152-2009 OI Hoffmann, Axel/0000-0002-1808-2767 FU U.S. Army Research Office [W911NF-12-1-0518, W911NF-11-C-0075]; U.S. National Science Foundation [ECCS-1231598]; U.S. National Institute of Standards and Technology [60NANB10D011]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported mainly by the U.S. Army Research Office (W911NF-12-1-0518). The work was also supported in part by the U.S. National Science Foundation (ECCS-1231598), the U.S. Army Research Office (W911NF-11-C-0075), the U.S. National Institute of Standards and Technology (60NANB10D011), and the U.S. Department of Energy, Office of Basic Energy Sciences (DE-AC02-06CH11357). NR 35 TC 40 Z9 40 U1 11 U2 92 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A501 DI 10.1063/1.4852135 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700046 ER PT J AU Lund, EA Du, H Oo, WMH Teeter, G Scarpulla, MA AF Lund, E. A. Du, H. Oo, W. M. Hlaing Teeter, G. Scarpulla, M. A. TI Investigation of combinatorial coevaporated thin film Cu2ZnSnS4 (II): Beneficial cation arrangement in Cu-rich growth SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID PHASE-FORMATION; SOLAR-CELLS; EFFICIENCY; SULFIDES; SNS AB Cu2ZnSn(S,Se)(4) (CZTSSe) is an earth-abundant semiconductor with potential for economical photovoltaic power generation at terawatt scales. In this work, we use Raman scattering to investigate phase coexistence in combinatorial CZTS thin films grown at 325 or 470 degrees C. The surface of the samples grown at 325 degrees C is rough except for a prominent specularly reflective band near and along the ZnS-Cu2SnS3 (CTS) tie line in the Cu-Zn-Sn-S quaternary phase diagram. All structurally incoherent secondary phases (SnS2, CuS) exist only as surface phases or are embedded as separate grains, whereas the structurally coherent secondary phase CTS coexists with CZTS in the dense underlying film. In films grown at 325 degrees C, which are kinetically trapped by the low growth temperature, a change is observed in Cu and Sn site occupancy, evidenced by the shift from cubic-CTS in the Cu-rich region (Cu/Sn > 2) to more tetragonal-CTS in the Sn-rich region (Cu/Sn < 2). For CZTS samples grown at 470 degrees C, CTS is not observed and regions grown under excess Sn flux are more disordered than Cu-rich regions evidenced by broader CZTS A mode peaks. Therefore, increasing Sn chemical potential results in more CZTS lattice disorder, suggesting, with other evidence, the formation of Sn antisite defects. In contrast, the CZTS A mode breadth is insensitive to Zn richness suggesting that excess Zn does not induce significant disorder within the CZTS lattice. We postulate that initially growing CZTS films Cu-rich (Cu/Sn > 2) results in higher cation ordering meaning fewer antisite defects. (C) 2014 AIP Publishing LLC. C1 [Lund, E. A.; Scarpulla, M. A.] Univ Utah, Dept Chem Engn, Salt Lake City, UT 84112 USA. [Du, H.] Sion Power Corp, Tucson, AZ 85756 USA. [Oo, W. M. Hlaing; Scarpulla, M. A.] Univ Utah, Dept Mat Sci & Engn, Salt Lake City, UT 84112 USA. [Teeter, G.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Scarpulla, M. A.] Univ Utah, Dept Elect & Comp Engn, Salt Lake City, UT 84112 USA. RP Scarpulla, MA (reprint author), Univ Utah, Dept Chem Engn, 50 S Cent Campus Dr Rm 3290, Salt Lake City, UT 84112 USA. EM scarpulla@eng.utah.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0001630]; U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX The research at the University of Utah was supported in whole by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-SC0001630. The work at NREL was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 35 TC 12 Z9 12 U1 5 U2 69 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 173503 DI 10.1063/1.4871665 PG 11 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700601 ER PT J AU Ma, YL Liu, XB Gandha, K Vuong, NV Yang, YB Yang, JB Poudyal, N Cui, J Liu, JP AF Ma, Y. L. Liu, X. B. Gandha, K. Vuong, N. V. Yang, Y. B. Yang, J. B. Poudyal, N. Cui, J. Liu, J. P. TI Preparation and magnetic properties of MnBi-based hard/soft composite magnets SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO AB Bulk anisotropic composite magnets based on MnBi/Co(Fe) exhibiting the different morphology of the soft magnetic phase were prepared by powder metallurgy processing. First, single-phase MnBi bulk magnets were produced with a maximum energy product [(BH)(m)] of 6.3 MGOe at room temperature. The nanoscale soft phase with the different morphology was then added to form a composite magnet. It was observed that addition of magnetic soft-phase nanoflakes causes a dramatic coercivity reduction. However, the addition of soft magnetic phase nanowires enhanced the composite magnetization without sacrificing the coercivity. Nevertheless, a kink was still observed on the demagnetization curves and the coercivity decreased when the soft-phase content was larger than 10 wt.%, which was caused by the agglomeration of the soft phase nanowires that also led to a decreased degree of texture. (C) 2014 AIP Publishing LLC. C1 [Ma, Y. L.; Liu, X. B.; Gandha, K.; Vuong, N. V.; Poudyal, N.; Liu, J. P.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Ma, Y. L.] Chongqing Univ Sci & Technol, Coll Met & Mat Engn, Chongqing 401331, Peoples R China. [Yang, Y. B.; Yang, J. B.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Cui, J.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Ma, YL (reprint author), Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. EM pliu@uta.edu RI Liu, Xubo/A-1883-2008; Yang, Yunbo/F-1458-2015 OI Liu, Xubo/0000-0002-2558-0959; Yang, Yunbo/0000-0001-7895-024X FU US DOE/ARPA-E; Center for Nanostructured Materials and Characterization Center for Materials and Biology at the University of Texas at Arlington FX This work was supported in part by US DOE/ARPA-E and the Center for Nanostructured Materials and Characterization Center for Materials and Biology at the University of Texas at Arlington. NR 15 TC 5 Z9 5 U1 9 U2 98 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A755 DI 10.1063/1.4868078 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700129 ER PT J AU Nlebedim, IC Jiles, DC AF Nlebedim, I. C. Jiles, D. C. TI Dependence of the magnetostrictive properties of cobalt ferrite on the initial powder particle size distribution SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID NANOCRYSTALLINE AB The dependence of the magnetostrictive properties of cobalt ferrite on the size distribution of the powder used in deriving the samples from traditional ceramic approach is presented. Sample obtained by combining the smallest and largest particle size distributions gave the highest magnetostriction and strain sensitivity (216 ppm and 1.34 nm/A, respectively), for measurement in parallel direction but the least (66 ppm and 0.38 nm/A respectively) in perpendicular direction. Sample derived from largest particle size distribution gave the least magnetostriction and strain sensitivity (147 ppm and 0.61 nm/A, respectively) in parallel direction but the highest (126 ppm and 0.5 nm/A, respectively) in the perpendicular direction. (C) 2014 AIP Publishing LLC. C1 [Nlebedim, I. C.; Jiles, D. C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Nlebedim, I. C.; Jiles, D. C.] Iowa State Univ, Elect & Comp Engn Dept, Ames, IA 50011 USA. RP Nlebedim, IC (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM nlebedim@iastate.edu FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE by Iowa State University [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under contract # DE-AC02-07CH11358. NR 6 TC 2 Z9 2 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A928 DI 10.1063/1.4867343 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700172 ER PT J AU Nlebedim, IC Dennis, KW McCallum, RW Jiles, DC AF Nlebedim, I. C. Dennis, K. W. McCallum, R. W. Jiles, D. C. TI Structural and magnetic properties of Ti4+/Co2+ co-substituted cobalt ferrite SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO AB The variations in the structural magnetic properties of cobalt ferrite due to Ti4+/Co2+ co-substitution for 2Fe(3+) are presented. The non-linear relation in the variation of the lattice parameter agrees with a previous study on cation distribution, which showed that the rate of substitution of cations into the A-sites and B-sites varies with Ti-concentration. Such variation in the rate of substitution into the cation sites was also observed in the magnetization, coercive field, and susceptibility data. The coercive field and differential susceptibility are inversely related. Although the coercive field of the Ti-substituted cobalt ferrite generally decreased compared to the un-substituted cobalt ferrite, magnetic susceptibility was higher at higher Ti-concentrations. (C) 2014 AIP Publishing LLC. C1 [Nlebedim, I. C.; Dennis, K. W.; McCallum, R. W.; Jiles, D. C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Nlebedim, I. C.; Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. RP Nlebedim, IC (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM nlebedim@iastate.edu FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE by Iowa State University [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under contract # DE-AC02-07CH11358. NR 7 TC 4 Z9 4 U1 0 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A519 DI 10.1063/1.4866230 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700064 ER PT J AU Pathak, AK Paudyal, D Gschneidner, KA Pecharsky, VK AF Pathak, Arjun K. Paudyal, D. Gschneidner, K. A., Jr. Pecharsky, V. K. TI Low temperature crystal structure and magnetic properties of RAl2 SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO AB Low temperature crystal structure and magnetic properties of RAl2 (R = Pr and Nd) have been studied using temperature dependent powder x-ray diffraction, magnetization, and heat capacity measurements. Unlike PrAl2, NdAl2 retains cubic MgCu2-type structure from room temperature down to 5K, which is also confirmed from first principles electronic structure calculations. The magnetization measurements show both PrAl2 and NdAl2 order ferromagnetically at T-C = 32K and 77 K, respectively. However, the magnetization measurements show the former is a hard ferromagnet compared to the latter which is a soft ferromagnetic material. The magnetic entropy change obtained from heat capacity measurements at Delta H 30 kOe for PrAl2 and NdAl2 are 3.15 J mol(-1) K-1 and 1.18 J mol(-1) K-1, respectively. (C) 2014 AIP Publishing LLC. C1 [Pathak, Arjun K.; Paudyal, D.; Gschneidner, K. A., Jr.; Pecharsky, V. K.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Gschneidner, K. A., Jr.; Pecharsky, V. K.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Pathak, AK (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM pathak138@ameslab.gov FU U.S. Department of Energy, Office of Basic Energy Science, Division of Material Sciences, and Engineering; U.S. Department of Energy [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Material Sciences, and Engineering. The research was performed at the Ames Laboratory. The Ames Laboratory is operated by Iowa State University for the U.S. Department of Energy under Contract No. DE-AC02-07CH11358. NR 10 TC 1 Z9 1 U1 1 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17E109 DI 10.1063/1.4859096 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700482 ER PT J AU Paudyal, D Pecharsky, VK Gschneidner, KA AF Paudyal, Durga Pecharsky, V. K. Gschneidner, K. A., Jr. TI Electronic structure, magnetic properties, and magnetostructural transformations in rare earth dialuminides SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID CEAL2; ERAL2 AB We report electronic structure, magnetic properties, and magnetostructural transformations of selected rare earth dialuminides calculated by using local spin density approximation (LSDA), including the Hubbard U parameter (LSDA+U) approach. Total energy calculations show that CeAl2 and EuAl2 adopt antiferromagnetic (AFM) ground states, while dialuminides formed by other magnetic lanthanides have ferromagnetic (FM) ground states. The comparison of theoretical and experimental magnetic moments of CeAl2 indicates that the 4f orbital moment of Ce in CeAl2 is quenched. Theoretical calculations confirm that Eu in EuAl2 and Yb in YbAl2 are divalent. PrAl2 exhibits a tetragonal distortion near FM transition. HoAl2 shows a first order magnetostructural transition while DyAl2 shows a second order transformation below magnetic transition. The dialuminides formed by Nd, Tb, and Er are simple ferromagnets without additional anomalies in the FM state. (C) 2014 AIP Publishing LLC. C1 [Paudyal, Durga; Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Paudyal, D (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM durga@ameslab.gov FU U.S. DOE, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. DOE by Iowa State University [DE-AC02-07CH11358] FX This work was supported by the U.S. DOE, Office of Basic Energy Science, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 16 TC 1 Z9 1 U1 4 U2 48 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17E127 DI 10.1063/1.4866389 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700500 ER PT J AU Perera, D Landau, DP Nicholson, DM Stocks, GM Eisenbach, M Yin, JQ Brown, G AF Perera, Dilina Landau, David P. Nicholson, Don M. Stocks, G. Malcolm Eisenbach, Markus Yin, Junqi Brown, Gregory TI Phonon-magnon interactions in body centered cubic iron: A combined molecular and spin dynamics study SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID SIMULATIONS; SYSTEMS AB Combining an atomistic many-body potential with a classical spin Hamiltonian parameterized by first principles calculations, molecular-spin dynamics computer simulations were performed to investigate phonon-magnon interactions in body centered cubic iron. Results obtained for spin-spin and density-density dynamic structure factors show that noticeable softening and damping of magnon modes occur due to the presence of lattice vibrations. Furthermore, as a result of the phonon-magnon coupling, additional longitudinal spin wave excitations are observed, with the same frequencies as the longitudinal phonon modes. (C) 2014 AIP Publishing LLC. C1 [Perera, Dilina; Landau, David P.] Univ Georgia, Ctr Simulat Phys, Athens, GA 30602 USA. [Nicholson, Don M.; Stocks, G. Malcolm; Eisenbach, Markus; Yin, Junqi] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Brown, Gregory] Florida State Univ, Tallahassee, FL 32306 USA. RP Perera, D (reprint author), Univ Georgia, Ctr Simulat Phys, Athens, GA 30602 USA. EM dilinanp@physast.uga.edu RI Yin, Junqi/F-6920-2014; Brown, Gregory/F-7274-2016; Stocks, George Malcollm/Q-1251-2016; OI Yin, Junqi/0000-0003-3843-5520; Brown, Gregory/0000-0002-7524-8962; Stocks, George Malcollm/0000-0002-9013-260X; Eisenbach, Markus/0000-0001-8805-8327 FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, "Center for Defect Physics," an Energy Frontier Research Center FX We are indebted to Shan-Ho Tsai and Stefan Schnabel for helpful discussions. This work was sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, "Center for Defect Physics," an Energy Frontier Research Center. We also acknowledge the computational resources provided by the Georgia Advanced Computing Resource Center. NR 15 TC 7 Z9 7 U1 0 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17D124 DI 10.1063/1.4863488 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700402 ER PT J AU Rahman, BMF Divan, R Zhang, HQ Rosenmann, D Peng, YJ Wang, XH Wang, GA AF Rahman, B. M. Farid Divan, Ralu Zhang, Hanqiao Rosenmann, Daniel Peng, Yujia Wang, Xuehe Wang, Guoan TI Direct current tunable noise suppressor using sub-micrometer patterned permalloy films SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID COPLANAR TRANSMISSION-LINE; THIN-FILMS AB A tunable noise suppressor at gigahertz frequency using sub-micrometer patterned Permalloy (Py) loaded coplanar waveguide transmission line is presented. The transmission line consists of 100 nm thick Py patterns on top of 0.9 mu m thick gold lines. Measured results show that the stop band frequency of the noise suppressor is changed from 4.8 GHz to 6 GHz depending on the aspect ratios of Py patterns. Variation of the gap in between Py patterns changed the stop band frequency from 4 GHz to 6 GHz. Furthermore, a novel way of tuning the stop band frequency of the noise suppressor by using an external direct current is reported. By applying 150 mA direct current along the transmission line, the frequency is changed from 6 GHz to 4.3 GHz. The measured results of 1.5% pass band loss, 2 degrees transmitted signal phase distortion, and 3 dB extra return loss of the designed noise suppressor are demonstrated. Noise suppression frequency and the magnitude of signal attenuation can be further improved by increasing the thickness of Py or using multi-layer Py. (C) 2014 AIP Publishing LLC. C1 [Rahman, B. M. Farid; Peng, Yujia; Wang, Xuehe; Wang, Guoan] Univ S Carolina, Dept Elect Engn, Microwave Applicat Grp, Columbia, SC 29208 USA. [Divan, Ralu; Rosenmann, Daniel] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. [Zhang, Hanqiao] Intel Corp, Columbia, SC 29210 USA. RP Wang, GA (reprint author), Univ S Carolina, Dept Elect Engn, Microwave Applicat Grp, Columbia, SC 29208 USA. EM gwang@cec.sc.edu FU NSF [1253929]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The work was supported by NSF under Award No. 1253929. Fabrication of device using Center for Nanoscale Materials, Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors would also like to thanks ANSYS for software support. NR 12 TC 7 Z9 7 U1 0 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17E515 DI 10.1063/1.4865769 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700536 ER PT J AU Rahman, BMF Divan, R Zhang, HQ Rosenmann, D Peng, YJ Wang, XH Wang, GA AF Rahman, B. M. Farid Divan, Ralu Zhang, Hanqiao Rosenmann, Daniel Peng, Yujia Wang, Xuehe Wang, Guoan TI High performance tunable slow wave elements enabled with nano-patterned permalloy thin film for compact radio frequency applications SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID SHAPE ANISOTROPY; LINES; FE AB Slow wave elements are promising structures to design compact RF (radio frequency) and mmwave components. This paper reports a comparative study on different types of coplanar wave-guide (CPW) slow wave structures (SWS). New techniques including the use of defected ground structure and the different signal conductor shape have been implemented to achieve higher slow wave effect with comparative loss. Results show that over 42% and 35% reduction in length is reported in the expense of only 0.3 dB and 0.1 dB insertion loss, respectively, which can end up with 66% and 58% area reduction for the design of a branch line coupler. Implementation of the sub micrometer patterned Permalloy (Py) thin film on top of the simple SWS has been demonstrated for the first time to increase the slow wave effect. Comparing with the traditional slow wave structure, with 100 nm thick Py patterns, the inductance per unit length of the SWS has been increased from 879 nH/m to 963 nH/m. The slow wave effect of the designed structure is also tunable by applied DC current. Measured results have shown that the phase shift can be changed from 94 degrees to 90.5 degrees by applying 150mA DC current. This provides a solution in designing RF passive components which can work in multiple frequency bands. (C) 2014 AIP Publishing LLC. C1 [Rahman, B. M. Farid; Peng, Yujia; Wang, Xuehe; Wang, Guoan] Univ S Carolina, Dept Elect Engn, Microwave Applicat Grp, Columbia, SC 29208 USA. [Divan, Ralu; Rosenmann, Daniel] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. [Zhang, Hanqiao] Intel Corp, Columbia, SC 29210 USA. RP Wang, GA (reprint author), Univ S Carolina, Dept Elect Engn, Microwave Applicat Grp, Columbia, SC 29208 USA. EM gwang@cec.sc.edu FU NSF [1253929]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The work was supported by NSF under Award No. 1253929. Fabrication of device using Center for Nanoscale Materials, Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors would also like to thanks ANSYS for softwre support. NR 19 TC 5 Z9 5 U1 1 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A508 DI 10.1063/1.4862847 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700053 ER PT J AU Shen, S DeGeorge, V Ohodnicki, PR Kernion, SJ Keylin, V Huth, JF McHenry, ME AF Shen, S. DeGeorge, V. Ohodnicki, P. R. Kernion, S. J. Keylin, V. Huth, J. F. McHenry, M. E. TI Induced anisotropy in FeCo-based nanocomposites: Early transition metal content dependence SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID SI-B ALLOYS; MAGNETIC-PROPERTIES; HIGH-FREQUENCY; CO; NB AB Soft magnetic nanocomposites variants of FeCo-based (HTX002) alloys (Fe65Co35)(81+x)B12Nb4-xSi2Cu1, exhibiting high inductions (up to 1.9 T), low losses, and high temperature stability are studied for high frequency inductors and current sensors. For alloys with x 0, 1, 1.5, 2, and 3, we report field induced anisotropy, K-U, after annealing at temperatures of 340-450 degrees C for 1 h in a 2 T transverse magnetic field. The anisotropy field, H-K, measured by AC permeametry on toroidal cores, and by first order reversal curves on square sections of ribbon, decreases with annealing temperature and saturates at high annealing temperatures suggesting a nanostructure related anisotropy mechanism in which the amorphous phase exhibits a higher H-K than the crystalline phase. A high saturation induction nanocrystalline phase and high H-K amorphous phase were achieved by low temperature annealing resulting in a value of K-U exceeding 14 X 10(3) erg/cm(3), more than twice that reported previously for Fe-rich amorphous and nanocomposite alloys. (C) 2014 AIP Publishing LLC. C1 [Shen, S.; DeGeorge, V.; Ohodnicki, P. R.; Kernion, S. J.; McHenry, M. E.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. [Ohodnicki, P. R.] NETL, Funct Mat Dev Div, Electrochem & Magnet Mat Team, Pittsburgh, PA 15236 USA. [Keylin, V.; Huth, J. F.] Magnetics, Pittsburgh, PA 15238 USA. RP Shen, S (reprint author), Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. EM shenshencd@gmail.com FU ARL [W911NF-08-2-0024]; ARPA-E [DE-FOA-0000474] FX This work was supported by the ARL through Grant No. W911NF-08-2-0024 and ARPA-E through Grant No. DE-FOA-0000474. NR 27 TC 4 Z9 4 U1 2 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A335 DI 10.1063/1.4867124 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700036 ER PT J AU Singh, NK Mudryk, Y Pecharsky, VK Gschneidner, KA AF Singh, Niraj K. Mudryk, Ya. Pecharsky, V. K. Gschneidner, K. A., Jr. TI In situ X-ray powder diffraction study of Ho5Ge4 SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID RARE-EARTH; MAGNETISM AB In Ho5Ge4 the magnetostructural transition (MST) from high temperature paramagnetic Sm5Ge4-type (O-II type) orthorhombic structure to a new low temperature antiferromagnetic (AFM) monoclinic structure (M beta-structure; the distortion occurs in the ac-plane) results in discontinuities of 400, 400, and 300 ppm along a, b, and c axes, respectively. During MST the unit cell volume exhibits discontinuity of 1000 ppm, and changes in both inter and intra slab bonds are less than 2%. In the AFM state the application of 35 kOe magnetic field leads to a partial reconstruction of the high temperature O-II structure, which is accompanied with a large magnetostriction. The strain energy associated with magnetostriction effects leads to an incomplete field driven MST in the magnetically ordered state. (C) 2014 AIP Publishing LLC. C1 [Singh, Niraj K.; Mudryk, Ya.; Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Mudryk, Y (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM slavkomk@ameslab.gov FU Department of Energy, Office of Basic Energy Sciences, Materials Sciences Division [DE-AC02-07CH11358] FX The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University of Science and Technology. This work was supported by the Department of Energy, Office of Basic Energy Sciences, Materials Sciences Division under Contract No. DE-AC02-07CH11358. NR 23 TC 1 Z9 1 U1 2 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17E105 DI 10.1063/1.4853215 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700478 ER PT J AU Sundararajan, JA Kaur, M Jiang, WL McCloy, JS Qiang, Y AF Sundararajan, Jennifer A. Kaur, Maninder Jiang, Weilin McCloy, John S. Qiang, You TI Oxide shell reduction and magnetic property changes in core-shell Fe nanoclusters under ion irradiation SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID IRON-OXIDES; NANOPARTICLES; NANOSTRUCTURES; NI AB Ion irradiation effects are studied on the Fe-based core-shell nanocluster (NC) films with core as Fe and shell as Fe3O4/Fe3N. These NC films were deposited on Si substrates to thickness of similar to 0.5 mu m using a NC deposition system. The films were irradiated at room temperature with 5.5 MeV Si2+ ions to ion fluences of 10(15) and 10(16) ions/cm(2). It is found that the irradiation induces grain growth, Fe valence reduction in the shell, and crystallization or growth of Fe3N. The film retained its Fe-core and its ferromagnetic properties after irradiation. The nature and mechanism of oxide shell reduction and composition dependence after irradiation were studied by synthesizing additional NC films of Fe3O4 and FeO + Fe3N and irradiating them under the same conditions. The presence of nanocrystalline Fe is found to be a major factor for the oxide shell reduction. The surface morphologies of these films show dramatic changes in the microstructures due to cluster growth and agglomeration as a result of ion irradiation. (C) 2014 AIP Publishing LLC. C1 [Sundararajan, Jennifer A.; Kaur, Maninder; Qiang, You] Univ Idaho, Dept Phys, Moscow, ID 83844 USA. [Jiang, Weilin] Pacific NW Natl Lab, Richland, WA 99352 USA. [McCloy, John S.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Qiang, Y (reprint author), Univ Idaho, Dept Phys, Moscow, ID 83844 USA. EM youqiang@uidaho.edu OI Jiang, Weilin/0000-0001-8302-8313 FU U.S. Department of Energy (DOE) [DE-FC07-08ID14926]; INL-LDRD under the DOE [DE-AC07-05ID14517]; LDRD at PNNL; Department of Energy's Office of Biological and Environmental Research; Pacific Northwest National Laboratory FX This work was supported by U.S. Department of Energy (DOE) under Contract No. DE-FC07-08ID14926, by the INL-LDRD administered by the Center for Advanced Energy Studies under the DOE Contract No. DE-AC07-05ID14517, and by an LDRD at PNNL. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 33 TC 3 Z9 3 U1 3 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17B507 DI 10.1063/1.4862520 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700199 ER PT J AU Tang, W Zhou, L Sun, KW Dennis, KW Kramer, MJ Anderson, IE McCallum, RW AF Tang, W. Zhou, L. Sun, K. W. Dennis, K. W. Kramer, M. J. Anderson, I. E. McCallum, R. W. TI Anisotropic hot deformed magnets prepared from Zn-coated MRE-Fe-B ribbon powder (MRE = Nd plus Y plus Dy) SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID PERMANENT-MAGNETS; COERCIVITY AB Milled melt-spun ribbon flake of MRE-Fe-B coated with Zn coating using a vapor transport technique was found to have significant increase in coercivity without degrading the magnetization when the Zn thickness and heat treatment were optimized. Magnetic measurements show that 0.5-1 wt.% Zn coating increases the coercivity about 1 kOe over the initial ribbon powder. After vacuum hot deformation (VHD), the VHD magnet with Zn coating of 0.5 wt.% results in a nearly 3 kOe higher coercivity than an un-coated alloy magnet. An optimized VHD magnet with 0.5 wt.% Zn coating obtains a coercivity of 11.2 kOe and (BH)(max) of 23.0 MGOe, respectively. SEM and TEM microstructures analysis demonstrates that the Zn coating on the surface of ribbon powder has diffused along the intergranular boundaries after the ribbon powder was annealed at 750 degrees C for 30 min or was hot deformed at 700-750 degrees C. (C) 2014 AIP Publishing LLC. C1 [Tang, W.; Zhou, L.; Sun, K. W.; Dennis, K. W.; Kramer, M. J.; Anderson, I. E.; McCallum, R. W.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RP Tang, W (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM weitang@ameslab.gov FU Propulsion Materials Programs at the Ames Laboratory [DE-AC02-07CH11358]; DOE-EERE-VT-PEEM FX This work was supported by DOE-EERE-VT-PEEM and Propulsion Materials Programs at the Ames Laboratory through Contract No. DE-AC02-07CH11358. NR 11 TC 2 Z9 2 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A725 DI 10.1063/1.4866086 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700099 ER PT J AU Wei, YJ Jana, S Brucas, R Pogoryelov, Y Ranjbar, M Dumas, RK Warnicke, P Akerman, J Arena, DA Karis, O Svedlindh, P AF Wei, Yajun Jana, Somnath Brucas, Rimantas Pogoryelov, Yevgen Ranjbar, Mojtaba Dumas, Randy K. Warnicke, Peter Akerman, Johan Arena, Dario A. Karis, Olof Svedlindh, Peter TI Magnetic coupling in asymmetric FeCoV/Ru/FeNi trilayers SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID BRILLOUIN LIGHT-SCATTERING AB We have investigated the magnetic anisotropy and interlayer coupling in trilayer films of permendur(100 angstrom)/Ru/permalloy(100 angstrom), with the thickness of the Ru spacer varying from 0 to 200 angstrom. While the permendur/permalloy sample exhibits a small in-plane uniaxial magnetic anisotropy with H-u = 27 Oe, all trilayers are magnetically isotropic in-plane. Results from hysteresis loop and ferromagnetic resonance measurements were fitted to a micromagnetic model, with the results indicating that all the films are ferromagnetically coupled except the one with 10 angstrom Ru spacer, which shows antiferromagnetic coupling. The trilayers with Ru spacer layer thickness larger than 20 angstrom exhibit only very weak ferromagnetic coupling. (C) 2014 AIP Publishing LLC. C1 [Wei, Yajun; Brucas, Rimantas; Svedlindh, Peter] Uppsala Univ, Dept Engn Sci, S-75121 Uppsala, Sweden. [Jana, Somnath; Pogoryelov, Yevgen; Karis, Olof] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Ranjbar, Mojtaba; Dumas, Randy K.; Akerman, Johan] Univ Gothenburg, Dept Phys, S-41296 Gothenburg, Sweden. [Warnicke, Peter] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Arena, Dario A.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Wei, YJ (reprint author), Uppsala Univ, Dept Engn Sci, S-75121 Uppsala, Sweden. EM peter.svedlindh@angstrom.uu.se RI Dumas, Randy/E-3077-2010; Pogoryelov, Yevgen/A-9693-2009; Akerman, Johan/B-5726-2008; Svedlindh, Peter/K-2702-2012; OI Dumas, Randy/0000-0001-5505-2172; Pogoryelov, Yevgen/0000-0001-5867-425X; Akerman, Johan/0000-0002-3513-6608; Karis, Olof/0000-0001-6406-217X; Warnicke, Peter/0000-0002-5252-6392 FU Swedish Research Council; Knut and Alice Wallenberg Foundation; Swedish Foundation for Strategic Research FX This work was supported by the Swedish Research Council, the Knut and Alice Wallenberg Foundation, and the Swedish Foundation for Strategic Research. NR 13 TC 2 Z9 2 U1 2 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17D129 DI 10.1063/1.4864743 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700407 ER PT J AU Wierer, JJ Montano, I Crawford, MH Allerman, AA AF Wierer, J. J., Jr. Montano, I. Crawford, M. H. Allerman, A. A. TI Effect of thickness and carrier density on the optical polarization of Al0.44Ga0.56N/Al0.55Ga0.45N quantum well layers SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID LIGHT-EMITTING-DIODES; GAN; GAIN; SEMICONDUCTORS; PARAMETERS; EMISSION; ALLOYS; LASERS AB The thickness and carrier density of AlGaN quantum well (QW) layers have a strong influence on the valence subband structure, and the resulting optical polarization and light extraction of ultraviolet light-emitting diodes. An ultraviolet-emitting (270-280 nm) multiple quantum well heterostructure consisting of 3 periods of Al0.44Ga0.56N/Al0.55Ga0.45N with individual layer thicknesses between 2-3.2 nm is studied both experimentally and theoretically. The optical polarization changes to preferentially polarized perpendicular to the QW plane as the QW thickness increases or the carrier density increases. Calculations show these trends are due to (a) a larger decrease in overlap of conduction band to light and heavy hole envelope functions compared to crystal-field split-off envelope functions, and (b) coupling between the valence subbands where higher heavy hole subbands couple to lower light hole and crystal-field split-off subbands. These changes in the valence band have a profound effect on the optical polarization, emission patterns, and eventual light extraction for ultraviolet emitters at these compositions and thicknesses, and need to be controlled to ensure high device efficiency. (C) 2014 AIP Publishing LLC. C1 [Wierer, J. J., Jr.; Montano, I.; Crawford, M. H.; Allerman, A. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Wierer, JJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jwierer@sandia.gov RI Wierer, Jonathan/G-1594-2013 OI Wierer, Jonathan/0000-0001-6971-4835 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank W. W. Chow and A. J. Fischer for useful discussions. The authors would also like to thank K. Cross for fabrication of the UVLEDs and Q. Li for the STEM images while employed at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 30 TC 13 Z9 13 U1 3 U2 32 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 174501 DI 10.1063/1.4874739 PG 10 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700647 ER PT J AU Xiong, J Matias, V Tao, BW Li, YR Jia, QX AF Xiong, J. Matias, V. Tao, B. W. Li, Y. R. Jia, Q. X. TI Ferroelectric and ferromagnetic properties of epitaxial BiFeO3-BiMnO3 films on ion-beam-assisted deposited TiN buffered flexible Hastelloy SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID THIN-FILMS; BIFEO3; ELECTRONICS AB Growth of multifunctional thin films on flexible substrates is of great technological significance since such a platform is needed for flexible electronics. In this study, we report the growth of biaxially aligned (BiFeO3)(0.5):(BiMnO3)(0.5) [BFO-BMO] films on polycrystalline Hastelloy by using a biaxially aligned TiN as a seed layer deposited by ion-beam-assisted deposited and a La0.7Sr0.3MnO3 (LSMO) as a buffer layer deposited by pulsed laser deposition. The LSMO is used not only as a buffer layer but also as the bottom electrode of the BFO-BMO films. X-ray diffraction showed that the BFO-BMO films are biaxially oriented along both in-plane and out-of-plane directions. The BFO-BMO films on flexible metal substrates showed a polarization of 22.9 mu C/cm(2). The magnetization of the BFO-BMO/LSMO is 62 emu/cc at room temperature. (C) 2014 AIP Publishing LLC. C1 [Xiong, J.; Tao, B. W.; Li, Y. R.] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Peoples R China. [Xiong, J.; Matias, V.; Jia, Q. X.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Div Mat Phys & Applicat, Los Alamos, NM 87545 USA. RP Xiong, J (reprint author), Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Peoples R China. EM jiexiong@uestc.edu.cn RI Jia, Q. X./C-5194-2008 FU LDRD program; U.S. Department of Energy through the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory FX The work at Los Alamos was supported by LDRD program and, in part, by the U.S. Department of Energy through the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy. NR 17 TC 3 Z9 3 U1 1 U2 50 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17D913 DI 10.1063/1.4869438 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700473 ER PT J AU Zhang, BM Sun, CJ Chen, JS Venkatesan, T Heald, SM Chow, GM AF Zhang, Bangmin Sun, Cheng-Jun Chen, Jing-Sheng Venkatesan, T. Heald, Steve M. Chow, Gan Moog TI Temperature dependent electronic structure of Pr0.67Sr0.33MnO3 film probed by X-ray absorption near edge structure SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID THIN-FILMS; MANGANITES; STRAIN; LAMNO3 AB The Mn K edge X-ray absorption near edge structures (XANES) of Pr0.67Sr0.33MnO3 film (100 nm) on (001) LaAlO3 substrate was measured at different temperatures to probe the MnO6 octahedron distortion and corresponding electronic structure. The absorption of high temperature paramagnetic-insulator phase differed from that of the low temperature ferromagnetic-metal phase. The temperature-dependent absorption intensity of Mn K edge XANES was correlated with the relaxation of distorted MnO6 octahedron, which changed the crystal field acting on the Mn site and the related electronic structure and properties. At low temperature, the splitting of Mn majority e(g) orbitals decreased and the density of states above the Fermi level increased in the relaxed MnO6 octahedron, as reflected by a wider separation between two sub-peaks in the pre-edge XANES spectra. (C) 2014 AIP Publishing LLC. C1 [Zhang, Bangmin; Sun, Cheng-Jun; Heald, Steve M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Zhang, Bangmin; Chen, Jing-Sheng; Chow, Gan Moog] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore. [Zhang, Bangmin; Venkatesan, T.] Natl Univ Singapore, NUSNNI Nanocore, Singapore 117411, Singapore. [Venkatesan, T.] Natl Univ Singapore, Dept Phys, Singapore 117542, Singapore. [Venkatesan, T.] Natl Univ Singapore, Dept Elect & Comp Engn, Singapore 117576, Singapore. RP Sun, CJ (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM cjsun@aps.anl.gov; msecgm@nus.edu.sg RI Venkatesan, Thirumalai/E-1667-2013 FU US Department of Energy-Basic Energy Sciences from NSERC; University of Washington; Canadian Light Source; Advanced Photon Source; U.S. DOE [DE-AC02-06CH11357]; Ministry of Education, Singapore [R-284-000-107-112]; A*STAR [R-284-000-082-305] FX The PNC/XSD facilities at the Advanced Photon Source, and research at these facilities, are supported by the US Department of Energy-Basic Energy Sciences, a Major Resources Support grant from NSERC, the University of Washington, the Canadian Light Source and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Work at National University of Singapore is supported by Ministry of Education, Singapore under Grant No. R-284-000-107-112, and A*STAR under Grant No. R-284-000-082-305. G. M. C. also thanks the PNC/XSD facilities for his sabbatical support. Authors thank Dr. D. B. Xu for his help of XANES measurement. NR 20 TC 0 Z9 0 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 DI 10.1063/1.4862092 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700489 ER PT J AU Zhang, XW Yang, MY Jiang, YF Allard, LF Wang, JP AF Zhang, Xiaowei Yang, Meiyin Jiang, Yanfeng Allard, Lawrence F. Wang, Jian-Ping TI Thermal stability of partially ordered Fe16N2 film on non-magnetic Ag under layer SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 58th Annual Conference on Magnetism and Magnetic Materials CY NOV 04-08, 2013 CL Denver, CO ID MAGNETIC-MOMENT AB Partially ordered Fe16N2 thin film with (001) texture is successfully grown on a Ag under layer using a facing target sputtering system. Fe16N2 phase is formed after post-annealing, which is detected by X-ray diffraction (XRD). High saturation magnetization (M-s) of Fe16N2 thin films is observed by vibrating sample magnetometry. It is found that Fe16N2 phase can be stable up to 225 degrees C, which is demonstrated by the Fe16N2 finger print peak (002) in XRD. After heating to 250 degrees C, the Fe16N2 phase decomposes, which leads to low Ms and soft magnetic behavior. To further study Fe16N2 decomposition, X-ray photoelectron spectroscopy is performed to detect the binding energy of nitrogen atoms. Differences of binding energy corresponding to before and after heat treatment show the variation of nitrogen atom in electronic state with surrounding Fe atoms, indicating nitrogen atomic migration during heat treatment. (C) 2014 AIP Publishing LLC. C1 [Zhang, Xiaowei; Yang, Meiyin; Jiang, Yanfeng; Wang, Jian-Ping] Univ Minnesota, Ctr Micromagnet & Informat Technol MINT, Minneapolis, MN 55455 USA. [Zhang, Xiaowei; Yang, Meiyin; Jiang, Yanfeng; Wang, Jian-Ping] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. [Zhang, Xiaowei; Wang, Jian-Ping] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Allard, Lawrence F.] Oak Ridge Natl Lab, High Temp Mat Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Wang, JP (reprint author), Univ Minnesota, Ctr Micromagnet & Informat Technol MINT, Minneapolis, MN 55455 USA. EM jpwang@umn.edu FU ARPA-E (Advanced Research Projects Agency-Energy) project, Seagate Technology and Western Digital [0472-1595] FX This work was partially supported by ARPA-E (Advanced Research Projects Agency-Energy) project under Contract No. 0472-1595, Seagate Technology and Western Digital. Parts of this work were carried out in the Characterization Facility through NSF MRSEC program at University of Minnesota. NR 10 TC 2 Z9 2 U1 4 U2 42 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2014 VL 115 IS 17 AR 17A767 DI 10.1063/1.4869065 PG 3 WC Physics, Applied SC Physics GA AG8BO UT WOS:000335643700141 ER PT J AU Michimasa, S Yanagisawa, Y Inafuku, K Aoi, N Elekes, Z Fulop, Z Ichikawa, Y Iwasa, N Kurita, K Kurokawa, M Machida, T Motobayashi, T Nakamura, T Nakabayashi, T Notani, M Ong, HJ Onishi, TK Otsu, H Sakurai, H Shinohara, M Sumikama, T Takeuchi, S Tanaka, K Togano, Y Yamada, K Yamaguchi, M Yoneda, K AF Michimasa, S. Yanagisawa, Y. Inafuku, K. Aoi, N. Elekes, Z. Fueloep, Zs. Ichikawa, Y. Iwasa, N. Kurita, K. Kurokawa, M. Machida, T. Motobayashi, T. Nakamura, T. Nakabayashi, T. Notani, M. Ong, H. J. Onishi, T. K. Otsu, H. Sakurai, H. Shinohara, M. Sumikama, T. Takeuchi, S. Tanaka, K. Togano, Y. Yamada, K. Yamaguchi, M. Yoneda, K. TI Quadrupole collectivity in island-of-inversion nuclei Ne-28,Ne-30 and Mg-34,Mg-36 SO PHYSICAL REVIEW C LA English DT Article ID PROTON INELASTIC-SCATTERING; N=8 SHELL CLOSURE; MAGIC NUMBER; BETA-DECAY; NEUTRON; ISOTOPES; BE-12; DEFORMATION; TRANSITION; MODEL AB The quadrupole collectivity of neutron-rich even-even neon and magnesium nuclei around N = 20, Ne-28,Ne-30, and Mg-32,Mg-34,Mg-36, was studied via proton inelastic scattering on a liquid hydrogen target by in-beam gamma-ray spectroscopy in inverse kinematics. The angle-integrated cross sections for the first 2(+) states of these nuclei were determined by measuring de-excitation gamma rays. The deformation lengths were extracted from the angle-integrated cross sections using distorted-wave calculations. The deformation length of 30Ne (delta(( p, p')) = 1.59(-0.09)(+ 0.08) fm) is smaller than that of Mg-32 ( 1.83(- 0.11)(+ 0.10) fm), which exhibits the largest quadrupole collectivity among the neutron-rich N = 20 isotones. Along the magnesium isotopic chain, the deformation lengths of Mg-34 and Mg-36 were deduced to be 2.30(- 0.10)(+ 0.09) fm and 1.90(- 0.17)(+ 0.16) fm, respectively. The evolution of quadrupole deformation in the vicinity of Mg-32 is discussed by comparing the present results with the theoretical calculations. C1 [Michimasa, S.] Univ Tokyo, Ctr Nucl Study, Wako, Saitama 3510198, Japan. [Yanagisawa, Y.; Ichikawa, Y.; Motobayashi, T.; Otsu, H.; Sakurai, H.; Takeuchi, S.; Tanaka, K.; Yamada, K.; Yamaguchi, M.; Yoneda, K.] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan. [Inafuku, K.; Iwasa, N.; Sumikama, T.] Tohoku Univ, Dept Phys, Aoba Ku, Sendai, Miyagi 9808578, Japan. [Aoi, N.; Ong, H. J.] Osaka Univ, Res Ctr Nucl Phys, Ibaraki, Osaka 5670047, Japan. [Elekes, Z.; Fueloep, Zs.] Inst Nucl Res ATOMKI, H-4001 Debrecen, Hungary. [Kurita, K.; Kurokawa, M.; Machida, T.] Rikkyo Univ, Dept Phys, Toshima Ku, Tokyo 1718501, Japan. [Nakamura, T.; Nakabayashi, T.; Shinohara, M.; Togano, Y.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Notani, M.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Onishi, T. K.; Sakurai, H.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan. RP Michimasa, S (reprint author), Univ Tokyo, Ctr Nucl Study, RIKEN Campus,2-1 Hirosawa, Wako, Saitama 3510198, Japan. EM mitimasa@cns.s.u-tokyo.ac.jp RI Fulop, Zsolt/B-2262-2008; SAKURAI, HIROYOSHI/G-5085-2014; Nakamura, Takashi/N-5390-2015; Takeuchi, Satoshi/O-1529-2016 OI Nakamura, Takashi/0000-0002-1838-9363; FU European Social Fund; European Union FX This research was partly realized in the framework of TAMOP 4.2.4.A/2-11-1-2012-0001" National Excellence Program-Elaborating and operating an inland student and researcher personal support system." The project was subsidized by European Union and co-financed by European Social Fund. NR 63 TC 7 Z9 7 U1 0 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 7 PY 2014 VL 89 IS 5 AR 054307 DI 10.1103/PhysRevC.89.054307 PG 9 WC Physics, Nuclear SC Physics GA AG6WY UT WOS:000335560800001 ER PT J AU Vlasenko, A Fuller, GM Cirigliano, V AF Vlasenko, Alexey Fuller, George M. Cirigliano, Vincenzo TI Neutrino quantum kinetics SO PHYSICAL REVIEW D LA English DT Article ID BIG-BANG NUCLEOSYNTHESIS; CORE-COLLAPSE SUPERNOVAE; EARLY UNIVERSE; STERILE NEUTRINOS; ELECTROWEAK BARYOGENESIS; OSCILLATING NEUTRINOS; TRANSPORT-EQUATIONS; EXPLOSION MECHANISM; BOLTZMANN-EQUATION; DRIVEN CONVECTION AB We present a formulation of the quantum kinetic equations (QKEs), which govern the evolution of neutrino flavor at high density and temperature. Here, the structure of the QKEs is derived from the ground up, using fundamental neutrino interactions and quantum field theory. We show that the resulting QKEs describe coherent flavor evolution with an effective mass when inelastic scattering is negligible. The QKEs also contain a collision term. This term can reduce to the collision term in the Boltzmann equation when scattering is dominant and the neutrino effective masses and density matrices become diagonal in the interaction basis. We also find that the QKEs include equations of motion for a new dynamical quantity related to neutrino spin. This quantity decouples from the equations of motion for the density matrices at low densities or in isotropic conditions. However, the spin equations of motion allow for the possibility of coherent transformation between neutrinos and antineutrinos at high densities and in the presence of anisotropy. Although the requisite conditions for this exist in the core collapse supernova and compact object merger environments, it is likely that only a self-consistent incorporation of the QKEs in a sufficiently realistic model could establish whether or not significant neutrino-antineutrino conversion occurs. C1 [Vlasenko, Alexey; Fuller, George M.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Vlasenko, Alexey; Fuller, George M.; Cirigliano, Vincenzo] New Mexico Consortium, Neutrino Engn Inst, Los Alamos, NM 87545 USA. [Cirigliano, Vincenzo] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Vlasenko, A (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. OI Cirigliano, Vincenzo/0000-0002-9056-754X FU NSF at UCSD [PHY-09-70064]; DOE Office of Science; LDRD Program at LANL; University of California Office of the President; UC HIPACC collaboration; DOE/LANL Topical Collaboration FX This work was supported in part by NSF Grant No. PHY-09-70064 at UCSD and by the DOE Office of Science and the LDRD Program at LANL and by the University of California Office of the President and the UC HIPACC collaboration. We would also like to acknowledge support from the DOE/LANL Topical Collaboration. We thank J. Carlson, J. F. Cherry, A. Friedland, K. Intriligator, B. Keister, C. Lee, A. Manohar, M. J. Ramsey-Musolf, S. Reddy, M. Roberts, and S. Tulin for useful discussions. NR 137 TC 36 Z9 36 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 7 PY 2014 VL 89 IS 10 AR 105004 DI 10.1103/PhysRevD.89.105004 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AG6XC UT WOS:000335561300005 ER PT J AU Saremi, O AF Saremi, Omid TI Disorder in gauge/gravity duality, pole spectrum statistics and random matrix theory SO CLASSICAL AND QUANTUM GRAVITY LA English DT Article DE AdS/CFT correspondence; disordered systems; condensed-matter physics; Anderson model; gravitation ID METAL-INSULATOR-TRANSITION; SYSTEMS AB In condensed-matter, level statistics has long been used to characterize the phases of a disordered system. We provide evidence within the context of a simple model that in a disordered large-N gauge theorywith a gravity dual, there exist phases where the nearest neighbor spacing distribution of the unfolded pole spectra of generic two-point correlators is Poisson. This closely resembles the localized phase of the Anderson Hamiltonian. We perform two tests on our statistical hypothesis. One is based on a statistic defined in the context of random matrix theory, the so-called (Delta(3)) over bar, or spectral rigidity, proposed by Dyson and Mehta. The second is a chi-squared test. In our model, the results of both tests are consistent with the hypothesis that the pole spectra of two-point functions can be at least in two distinct phases; first a regular sequence and second a completely uncorrelated sequence with a Poisson nearest neighbor spacing distribution. C1 [Saremi, Omid] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Saremi, Omid] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Saremi, Omid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Saremi, O (reprint author), Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. EM omid@phas.ubc.ca FU Berkeley Center for Theoretical Physics, department of physics at UC Berkeley [DE-AC02-05CH11231] FX OS is grateful to Allan Adams for fruitful discussions, comments and collaboration on related topics. Special thanks to Sean Hartnoll for useful discussions, suggestions and comments. OS would like to thank Dionysios Anninos, Mohammad Edalati, Tarun Grover and John McGreevy for comments and Alex Dahlen, Shannon McCurdy, Valadimir Rosenhaus and Kevin Schaeffer for helping with the paper. OS is supported by the Berkeley Center for Theoretical Physics, department of physics at UC Berkeley and in part by DOE, under contract DE-AC02-05CH11231. NR 26 TC 4 Z9 4 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0264-9381 EI 1361-6382 J9 CLASSICAL QUANT GRAV JI Class. Quantum Gravity PD MAY 7 PY 2014 VL 31 IS 9 DI 10.1088/0264-9381/31/9/095014 PG 9 WC Astronomy & Astrophysics; Physics, Multidisciplinary; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AF4HF UT WOS:000334671900015 ER PT J AU Simon, E Palotas, K Ujfalussy, B Deak, A Stocks, GM Szunyogh, L AF Simon, E. Palotas, K. Ujfalussy, B. Deak, A. Stocks, G. M. Szunyogh, L. TI Spin-correlations and magnetic structure in an Fe monolayer on 5d transition metal surfaces SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE spin-correlations; spin-dynamics; magnetic ground state; Fe monolayer; 5d substrates; DFT ID ACCURATE; ENERGY AB We present a detailed first principles study on the magnetic structure of an Fe monolayer on different surfaces of 5d transition metals. We use the spin-cluster expansion technique to obtain parameters of a spin model, and predict the possible magnetic ground state of the studied systems by employing the mean field approach and, in certain cases, by spin dynamics calculations. We point out that the number of shells considered for the isotropic exchange interactions plays a crucial role in the determination of the magnetic ground state. In the case of Ta substrate we demonstrate that the out-of-plane relaxation of the Fe monolayer causes a transition from ferromagnetic to antiferromagnetic ground state. We examine the relative magnitude of nearest neighbour Dzyaloshinskii-Moriya (D) and isotropic (J) exchange interactions in order to get insight into the nature of magnetic pattern formations. For the Fe/Os(0 0 0 1) system we calculate a very large D/J ratio, correspondingly, a spin spiral ground state. We find that, mainly through the leading isotropic exchange and Dzyaloshinskii-Moriya interactions, the inward layer relaxation substantially influences the magnetic ordering of the Fe monolayer. For the Fe/Re(0 0 0 1) system characterized by large antiferromagnetic interactions we also determine the chirality of the 120 degrees Neel-type ground state. C1 [Simon, E.; Palotas, K.; Deak, A.; Szunyogh, L.] Budapest Univ Technol & Econ, Dept Theoret Phys, H-1111 Budapest, Hungary. [Ujfalussy, B.] Hungarian Acad Sci, Wigner Res Ctr Phys, Inst Solid State Phys & Opt, H-1525 Budapest, Hungary. [Stocks, G. M.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Szunyogh, L.] Budapest Univ Technol & Econ, Hungarian Acad Sci, Condensed Matter Res Grp, H-1111 Budapest, Hungary. RP Simon, E (reprint author), Budapest Univ Technol & Econ, Dept Theoret Phys, Budafoki Ut 8, H-1111 Budapest, Hungary. EM esimon@phy.bme.hu RI Palotas, Krisztian/C-5338-2009; Simon, Eszter/D-1252-2012; Ujfalussy, Balazs/A-8155-2013; Deak, Andras/H-4170-2012; Stocks, George Malcollm/Q-1251-2016 OI Palotas, Krisztian/0000-0002-1914-2901; Ujfalussy, Balazs/0000-0003-3338-4699; Deak, Andras/0000-0002-3210-2947; Stocks, George Malcollm/0000-0002-9013-260X FU Hungarian Scientific Research Fund [K77771, PD83353, K84078, K91219]; Hungarian Academy of Sciences; European Union; European Social Fund [TAMOP 4.2.4.A/2-11-1-2012-0001]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE), under its Vehicle Technologies Program, through the Ames Laboratory; Iowa State University [DE-AC02-07CH11358] FX This work was supported by the Hungarian Scientific Research Fund projects K77771, PD83353, K84078, and K91219. KP acknowledges the Bolyai Research Grant of the Hungarian Academy of Sciences. The work of LS was supported by the European Union, co-financed by the European Social Fund, in the framework of TAMOP 4.2.4.A/2-11-1-2012-0001 National Excellence Program. Support for the work of GMS was provided by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE), under its Vehicle Technologies Program, through the Ames Laboratory. Ames Laboratory is operated by Iowa State University under contract DE-AC02-07CH11358. Partial support of the work of BU was from the same source. NR 34 TC 6 Z9 6 U1 0 U2 25 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 7 PY 2014 VL 26 IS 18 AR 186001 DI 10.1088/0953-8984/26/18/186001 PG 8 WC Physics, Condensed Matter SC Physics GA AF7YG UT WOS:000334930900015 PM 24759288 ER PT J AU Zavala, VM AF Zavala, Victor M. TI Stochastic optimal control model for natural gas networks SO COMPUTERS & CHEMICAL ENGINEERING LA English DT Article DE Stochastic optimization; Natural gas; Real-time; Optimal control ID PREDICTIVE CONTROL; OPTIMIZATION; STRATEGIES; ALGORITHM; IMPLEMENTATION AB We present a stochastic optimal control model to optimize gas network inventories in the face of system uncertainties. The model captures detailed network dynamics and operational constraints and uses a weighted risk-mean objective. We perform a degrees-of-freedom analysis to assess operational flexibility and to determine conditions for model consistency. We compare the control policies obtained with the stochastic model against those of deterministic and robust counterparts. We demonstrate that the use of risk metrics can help operators to systematically mitigate system volatility. Moreover, we discuss computational scalability issues and effects of discretization resolution on economic performance. (C) 2014 Elsevier Ltd. All rights reserved. C1 Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Zavala, VM (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. FU DOE Office of Science Early Career award; U.S. Department of Energy [DE-AC02-06CH11357] FX The author acknowledges support from the DOE Office of Science Early Career award. The author would also like to thank Drew Kouri for pointing him to existing work on stochastic optimization of natural gas networks. This work was supported by the U.S. Department of Energy, under contract no. DE-AC02-06CH11357. NR 29 TC 14 Z9 15 U1 4 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0098-1354 EI 1873-4375 J9 COMPUT CHEM ENG JI Comput. Chem. Eng. PD MAY 7 PY 2014 VL 64 BP 103 EP 113 DI 10.1016/j.compchemeng.2014.02.002 PG 11 WC Computer Science, Interdisciplinary Applications; Engineering, Chemical SC Computer Science; Engineering GA AE2MB UT WOS:000333806000010 ER PT J AU Xiao, PH Sheppard, D Rogal, J Henkelman, G AF Xiao, Penghao Sheppard, Daniel Rogal, Jutta Henkelman, Graeme TI Solid-state dimer method for calculating solid-solid phase transitions SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID FINDING SADDLE-POINTS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; ELASTIC BAND METHOD; AB-INITIO; BASIS-SET; TRANSFORMATIONS; METASTABILITY; SYSTEMS; PATHS AB The dimer method is a minimum mode following algorithm for finding saddle points on a potential energy surface of atomic systems. Here, the dimer method is extended to include the cell degrees of freedom for periodic solid-state systems. Using this method, reaction pathways of solid-solid phase transitions can be determined without having to specify the final state structure or reaction mechanism. Example calculations include concerted phase transitions between CdSe polymorphs and a nucleation and growth mechanism for the A15 to BCC transition in Mo. (C) 2014 AIP Publishing LLC. C1 [Xiao, Penghao; Henkelman, Graeme] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. [Xiao, Penghao; Henkelman, Graeme] Univ Texas Austin, Inst Computat & Engn Sci, Austin, TX 78712 USA. [Sheppard, Daniel] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Rogal, Jutta] Ruhr Univ Bochum, Interdisciplinary Ctr Adv Mat Simulat, D-44780 Bochum, Germany. RP Xiao, PH (reprint author), Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. EM henkelman@cm.utexas.edu OI Xiao, Penghao/0000-0002-5846-6343 FU National Science Foundation [CHE-1152342]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-5C0001091]; Welch Foundation [F-1841] FX The method development work was supported by the National Science Foundation under Grant No. CHE-1152342, and the calculations were supported as part of the program "Understanding Charge Separation and Transfer at Interfaces in Energy Materials (EFRC:CST)" an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-5C0001091, and the Welch Foundation under Grant No. F-1841. Calculations were done with resources from the National Energy Research Scientific Computing Center and the Texas Advanced Computing Center. We would like to thank Rye Terrell, An Harjunmaa, and Ralf Drautz for helpful discussions and related research on the A15 to BCC phase transition. NR 33 TC 2 Z9 2 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2014 VL 140 IS 17 AR 174104 DI 10.1063/1.4873437 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AH3TI UT WOS:000336048000006 ER PT J AU Landau, SM Frosch, MP AF Landau, Susan M. Frosch, Matthew P. TI Tracking the earliest pathologic changes in Alzheimer disease SO NEUROLOGY LA English DT Editorial Material ID AMYLOID-BETA DEPOSITION; HYPOTHETICAL MODEL; DYNAMIC BIOMARKERS AB A current challenge in Alzheimer disease (AD) research is to identify the sequence of pathologic changes that occurs during preclinical stages of disease in advance of cognitive decline. The timing of appearance of the 2 pathologic hallmarks of ADamyloid deposition and tau-mediated neurodegenerationis a particular topic of debate, with researchers drawing on a broad range of genetic, neuroimaging, fluid biomarker, animal, and autopsy studies to piece together the series of events ultimately leading to the plaques, neurofibrillary tangles, and cognitive deficits that define AD. C1 [Landau, Susan M.] Univ Calif, Helen Wills Neurosci Inst, Berkeley, CA 94704 USA. Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Frosch, Matthew P.] Harvard Univ, Sch Med, Massachusetts Gen Hosp, Mass Gen Inst Neurodegenerat Dis, Charlestown, MA USA. [Frosch, Matthew P.] Harvard Univ, Sch Med, Massachusetts Gen Hosp, CS Kubik Lab Neuropathol, Charlestown, MA USA. RP Landau, SM (reprint author), Univ Calif, Helen Wills Neurosci Inst, Berkeley, CA 94704 USA. EM slandau@berkeley.edu NR 8 TC 4 Z9 5 U1 0 U2 2 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA SN 0028-3878 EI 1526-632X J9 NEUROLOGY JI Neurology PD MAY 6 PY 2014 VL 82 IS 18 BP 1576 EP 1577 DI 10.1212/WNL.0000000000000392 PG 2 WC Clinical Neurology SC Neurosciences & Neurology GA AH9XB UT WOS:000336497400005 PM 24706009 ER PT J AU Schaef, HT Horner, JA Owen, AT Thompson, CJ Loring, JS McGrail, BP AF Schaef, Herbert T. Horner, Jake A. Owen, Antoinette T. Thompson, Chris J. Loring, John S. McGrail, Bernard P. TI Mineralization of Basalts in the CO2-H2O-SO2-O-2 System SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SUPERCRITICAL CARBON-DIOXIDE; CO-SEQUESTRATION; JAROSITE; SULFATE; MINERALS; ALUNITE; SO2; INJECTION; PURE AB Sequestering carbon dioxide (CO2) containing minor amounts of co-contaminants in geologic formations was investigated in the laboratory through the use of high pressure static experiments. Five different basalt samples were immersed in water equilibrated with supercritical CO2 containing 1 wt % sulfur dioxide (SO2) and 1 wt % oxygen (O-2) at reservoir conditions (similar to 100 bar, 90 degrees C) for 48 and 98 days. Gypsum (CaSO4) was a common precipitate, occurred early as elongated blades with striations, and served as substrates for other mineral products. In addition to gypsum, bimodal pulses of water released during dehydroxylation were key indicators, along with X-ray diffraction, for verifying the presence of jarosite-alunite group minerals. Well-developed pseudocubic jarosite crystals formed surface coatings, and in some instances, mixtures of natrojarosite and natroalunite aggregated into spherically shaped structures measuring 100 mu m in diameter. Reaction products were also characterized using infrared spectroscopy, which indicated OH and Fe-O stretching modes. The presences of jarosite-alunite group minerals were found in the lower wavenumber region from 700 to 400 cm(-1). A strong preferential incorporation of Fe(III) into natrojarosite was attributed to the oxidation potential of O-2. Evidence of CO2 was detected during thermal decomposition of precipitates, suggesting the onset of mineral carbonation. C1 [Schaef, Herbert T.; Horner, Jake A.; Owen, Antoinette T.; Thompson, Chris J.; Loring, John S.; McGrail, Bernard P.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Schaef, HT (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM todd.schaef@pnnl.gov FU U.S. Department of Energy, Office of Fossil Energy; DOE [DE-AC06-76RLO-1830] FX This work was supported by the U.S. Department of Energy, Office of Fossil Energy. Part of this work was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility at PNNL that is managed by the DOE's office of Biological and Environmental Research. PNNL is operated for the DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RLO-1830. NR 40 TC 6 Z9 6 U1 9 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 6 PY 2014 VL 48 IS 9 BP 5298 EP 5305 DI 10.1021/es404964j PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AG9DY UT WOS:000335720100079 PM 24669947 ER PT J AU Wang, T Salazar, A Zabotina, OA Hong, M AF Wang, Tuo Salazar, Andre Zabotina, Olga A. Hong, Mei TI Structure and Dynamics of Brachypodium Primary Cell Wall Polysaccharides from Two-Dimensional C-13 Solid-State Nuclear Magnetic Resonance Spectroscopy SO BIOCHEMISTRY LA English DT Article ID ULTRASOUND-ASSISTED EXTRACTION; NEUTRON FIBER DIFFRACTION; HYDROGEN-BONDING SYSTEM; ANGLE-SPINNING NMR; SYNCHROTRON X-RAY; PECTIC POLYSACCHARIDES; CRYSTAL-STRUCTURE; CHEMICAL-SHIFT; MAS NMR; CELLULOSE AB The polysaccharide structure and dynamics in the primary cell wall of the model grass Brachypodium distachyon are investigated for the first time using solid-state nuclear magnetic resonance (NMR). While both grass and non-grass cell walls contain cellulose as the main structural scaffold, the former contains xylan with arabinose and glucuronic acid substitutions as the main hemicellulose, with a small amount of xyloglucan (XyG) and pectins, while the latter contains XyG as the main hemicellulose and significant amounts of pectins. We labeled the Brachypodium cell wall with C-13 to allow two-dimensional (2D) C-13 correlation NMR experiments under magic-angle spinning. Well-resolved 2D spectra are obtained in which the C-13 signals of cellulose, glucuronoarabinoxylan (GAX), and other matrix polysaccharides can be assigned. The assigned C-13 chemical shifts indicate that there are a large number of arabinose and xylose linkages in the wall, and GAX is significantly branched at the developmental stage of 2 weeks. 2D C-13-C-13 correlation spectra measured with long spin diffusion mixing times indicate that the branched GAX approaches cellulose microfibrils on the nanometer scale, contrary to the conventional model in which only unbranched GAX can bind cellulose. The GAX chains are highly dynamic, with average order parameters of similar to 0.4. Biexponential C-13 T-1 and H-1 T-1 rho relaxation indicates that there are two dynamically distinct domains in GAX: the more rigid domain may be responsible for cross-linking cellulose microfibrils, while the more mobile domain may fill the interfibrillar space. This dynamic heterogeneity is more pronounced than that of the non-grass hemicellulose, XyG, suggesting that GAX adopts the mixed characteristics of XyG and pectins. Moderate differences in cellulose rigidity are observed between the Brachypodium and Arabidopsis cell walls, suggesting different effects of the matrix polysaccharides on cellulose. These data provide the first molecular-level structural information about the three-dimensional organization of the polysaccharides in the grass primary wall. C1 [Wang, Tuo; Hong, Mei] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Wang, Tuo; Hong, Mei] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Salazar, Andre; Zabotina, Olga A.] Iowa State Univ, Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. RP Hong, M (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM mhong@iastate.edu FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; National Science Foundation [1121163]; DOE [DE-FG02-93ER-20097] FX This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract DE-AC02-07CH11358 (to M.H.) and by National Science Foundation Grant 1121163 (to O.A.Z.). Linkage composition was performed at CCRC Analytical services supported by the DOE-funded Center for Plant and Microbial Complex Carbohydrates under Contract DE-FG02-93ER-20097. NR 69 TC 16 Z9 16 U1 5 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 6 PY 2014 VL 53 IS 17 BP 2840 EP 2854 DI 10.1021/bi500231b PG 15 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AG9EC UT WOS:000335720500010 PM 24720372 ER PT J AU Liu, SX Chistol, G Bustamante, C AF Liu, Shixin Chistol, Gheorghe Bustamante, Carlos TI Mechanical Operation and Intersubunit Coordination of Ring-Shaped Molecular Motors: Insights from Single-Molecule Studies SO BIOPHYSICAL JOURNAL LA English DT Review ID DNA PACKAGING MOTOR; REPLICATIVE HEXAMERIC HELICASE; ATOMIC-FORCE MICROSCOPY; ATP SYNTHASE; CHROMOSOME-TRANSLOCATION; PHOSPHATE RELEASE; MAGNETIC TWEEZERS; BACILLUS-SUBTILIS; TORQUE GENERATION; OPTICAL TWEEZERS AB Ring NTPases represent a large and diverse group of proteins that couple their nucleotide hydrolysis activity to a mechanical task involving force generation and some type of transport process in the cell. Because of their shape, these enzymes often operate as gates that separate distinct cellular compartments to control and regulate the passage of chemical species across them. In this manner, ions and small molecules are moved across membranes, biopolymer substrates are segregated between cells or moved into confined spaces, double-stranded nucleic acids are separated into single strands to provide access to the genetic information, and polypeptides are unfolded and processed for recycling. Here we review the recent advances in the characterization of these motors using single-molecule manipulation and detection approaches. We describe the various mechanisms by which ring motors convert chemical energy to mechanical force or torque and coordinate the activities of individual subunits that constitute the ring. We also examine how single-molecule studies have contributed to a better understanding of the structural elements involved in motor-substrate interaction, mechanochemical coupling, and intersubunit coordination. Finally, we discuss how these molecular motors tailor their operation-often through regulation by other cofactors-to suit their unique biological functions. C1 [Liu, Shixin; Chistol, Gheorghe; Bustamante, Carlos] Univ Calif Berkeley, Jason L Choy Lab Single Mol Biophys, Berkeley, CA 94720 USA. [Liu, Shixin; Bustamante, Carlos] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Chistol, Gheorghe; Bustamante, Carlos] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bustamante, Carlos] Univ Calif Berkeley, Howard Hughes Med Inst, Dept Chem, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bustamante, C (reprint author), Univ Calif Berkeley, Jason L Choy Lab Single Mol Biophys, Berkeley, CA 94720 USA. EM carlosjbustamante@gmail.com FU National Institutes of Health [R01-GM071552]; Department of Energy [DE-AC02-05CH11231]; NIH Pathway to Independence [K99-GM107365]; Howard Hughes Medical Institute FX This work was supported by the National Institutes of Health under grant No. R01-GM071552, the Department of Energy under contract No. DE-AC02-05CH11231, and the Howard Hughes Medical Institute (to C.B.). S.L. acknowledges support from the NIH Pathway to Independence Award No. K99-GM107365. NR 128 TC 9 Z9 9 U1 3 U2 40 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD MAY 6 PY 2014 VL 106 IS 9 BP 1844 EP 1858 DI 10.1016/j.bpj.2014.03.029 PG 15 WC Biophysics SC Biophysics GA AG7PM UT WOS:000335610100006 PM 24806916 ER PT J AU Clausen, CH Brooks, MD Li, TD Grob, P Kemalyan, G Nogales, E Niyogi, KK Fletcher, DA AF Clausen, Casper H. Brooks, Matthew D. Li, Tai-De Grob, Patricia Kemalyan, Gigi Nogales, Eva Niyogi, Krishna K. Fletcher, Daniel A. TI Dynamic Mechanical Responses of Arabidopsis Thylakoid Membranes during PSII-Specific Illumination SO BIOPHYSICAL JOURNAL LA English DT Article ID ATOMIC-FORCE MICROSCOPY; PHOTOSYSTEM-II; CHLOROPLAST MEMBRANES; STATE TRANSITIONS; PHOTOSYNTHETIC MEMBRANES; GRANA MEMBRANES; LIGHT; SPINACH; ORGANIZATION; PHOTOPROTECTION AB Remodeling of thylakoid membranes in response to illumination is an important process for the regulation of photosynthesis. We investigated the thylakoid network from Arabidopsis thaliana using atomic force microscopy to capture dynamic changes in height, elasticity, and viscosity of isolated thylakoid membranes caused by changes in illumination. We also correlated the mechanical response of the thylakoid network with membrane ultrastructure using electron microscopy. We find that the elasticity of the thylakoid membranes increases immediately upon PSII-specific illumination, followed by a delayed height change. Direct visualization by electron microscopy confirms that there is a significant change in the packing repeat distance of the membrane stacks in response to illumination. Although experiments with Gramicidin show that the change in elasticity depends primarily on the transmembrane pH gradient, the height change requires both the pH gradient and STN7-kinase-dependent phosphorylation of LHCII. Our studies indicate that lumen expansion in response to illumination is not simply a result of the influx of water, and we propose a dynamic model in which protein interactions within the lumen drive these changes. C1 [Clausen, Casper H.; Li, Tai-De; Fletcher, Daniel A.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Brooks, Matthew D.; Niyogi, Krishna K.] Univ Calif Berkeley, Dept Plant & Microbial Sci, Berkeley, CA 94720 USA. [Nogales, Eva; Niyogi, Krishna K.; Fletcher, Daniel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Nogales, Eva] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Brooks, Matthew D.; Grob, Patricia; Kemalyan, Gigi; Nogales, Eva; Niyogi, Krishna K.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. RP Fletcher, DA (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. EM fletch@berkeley.edu FU Division of Chemical Sciences, Geosciences, and Biosciences; Office of Basic Energy Sciences; Office of Science; U.S. Department of Energy, FWP [SISGRKN]; Howard Hughes Medical Institute; Gordon and Betty Moore Foundation [GBMF3070]; Villum Kann Rasmussen foundation [495289] FX This research was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy, FWP No. SISGRKN. K.K.N. was funded by the Howard Hughes Medical Institute and the Gordon and Betty Moore Foundation (through grant GBMF3070). C.H.C. was funded by the Villum Kann Rasmussen foundation (grant 495289). NR 34 TC 3 Z9 3 U1 1 U2 20 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD MAY 6 PY 2014 VL 106 IS 9 BP 1864 EP 1870 DI 10.1016/j.bpj.2014.03.016 PG 7 WC Biophysics SC Biophysics GA AG7PM UT WOS:000335610100008 PM 24806918 ER PT J AU Gilmore, SF Sasaki, DY Parikh, AN AF Gilmore, Sean F. Sasaki, Darryl Y. Parikh, Atul N. TI Thermal Annealing Triggers Collapse of Biphasic Supported Lipid Bilayers into Multilayer Islands SO LANGMUIR LA English DT Article ID ATOMIC-FORCE MICROSCOPY; LANGMUIR-BLODGETT-FILMS; AIR-WATER-INTERFACE; PHOSPHOLIPID-BILAYERS; SURFACTANT MONOLAYERS; PHASE-TRANSITIONS; SP-B; MEMBRANES; ADSORPTION; ELLIPSOMETRY AB The collapse of phase-separating single, supported lipid bilayers, consisting of mixtures of a zwitterionic phospholipid (POPC) and an anionic lipid (DPPA) upon thermal annealing in the presence of ions is examined using a combination of scanning probe, epifluorescence, and ellipsometric microscopies. We find that thermal annealing in the presence of ions in the bathing medium induces an irreversible transition from domain-textured, single supported bilayers to one comprising islands of multibilayer stacks, whose lateral area decays with lamellarity, producing pyramidal staircase "mesa" topography. The higher order lamellae are almost invariably localized above the anionic-lipid rich, gel-phase domains in the parent bilayer and depends on the ions in the bathing medium. The collapse mechanism appears to involve synergistic influences of two independent mechanisms: (1) stabilization of the incipient headgroup-headgroup interface in the emergent multibilayer configuration facilitated by ions in the bath and (2) domain-boundary templated folding. This collapse mechanism is consistent with previous theoretical predictions of topography-induced rippling instability in collapsing lipid monolayers and suggests the role of the mismatch in height and/or spontaneous curvature at domain boundaries in the collapse of phase-separated single supported bilayers. C1 [Gilmore, Sean F.] Univ Calif Davis, Appl Sci Grad Grp, Davis, CA 95616 USA. [Parikh, Atul N.] Univ Calif Davis, Dept Biomed Engn, Davis, CA 95616 USA. [Parikh, Atul N.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Sasaki, Darryl Y.] Sandia Natl Labs, Biosci Grp, Livermore, CA 94550 USA. RP Parikh, AN (reprint author), 3001 Ghausi Hall,1 Shields Ave, Davis, CA 95616 USA. EM anparikh@ucdavis.edu RI PARIKH, ATUL/D-2243-2014 OI PARIKH, ATUL/0000-0002-5927-4968 FU The U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-FG02-04ER46173]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work is supported by a grant from The U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under the Award # DE-FG02-04ER46173. D.Y.S. is at Sandia National Laboratory. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 51 TC 1 Z9 1 U1 0 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 6 PY 2014 VL 30 IS 17 BP 4962 EP 4969 DI 10.1021/la5005424 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AG9ED UT WOS:000335720600011 PM 24708440 ER PT J AU Gamza, MB Tomczak, JM Brown, C Puri, A Kotliar, G Aronson, MC AF Gamza, M. B. Tomczak, J. M. Brown, C. Puri, A. Kotliar, G. Aronson, M. C. TI Electronic correlations in FeGa3 and the effect of hole doping on its magnetic properties SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR-TRANSITION; LOW-TEMPERATURE TRANSPORT; KONDO INSULATOR; SI-P; ANTIFERROMAGNETIC SYSTEMS; THERMOELECTRIC PROPERTIES; INTERMETALLIC COMPOUNDS; DOPED SILICON; SEMICONDUCTOR; FESI AB We investigate signatures of electronic correlations in the narrow-gap semiconductor FeGa3 by means of electrical resistivity and thermodynamic measurements performed on single crystals of FeGa3, Fe1-xMnxGa3, and FeGa3-yZny, complemented by a study of the 4d analog material RuGa3. We find that the inclusion of sizable amounts of Mn and Zn dopants into FeGa3 does not induce an insulator-to-metal transition. Our study indicates that both substitution of Zn onto the Ga site and replacement of Fe by Mn introduces states into the semiconducting gap that remain localized even at highest doping levels. Most importantly, using neutron powder diffraction measurements, we establish that FeGa3 orders magnetically above room temperature in a complex structure, which is almost unaffected by the doping with Mn and Zn. Using realistic many-body calculations within the framework of dynamical mean field theory (DMFT), we argue that while the iron atoms in FeGa3 are dominantly in an S = 1 state, there are strong charge and spin fluctuations on short-time scales, which are independent of temperature. Further, the low magnitude of local contributions to the spin susceptibility advocates an itinerant mechanism for the spin response in FeGa3. Our joint experimental and theoretical investigations classify FeGa3 as a correlated band insulator with only small dynamical correlation effects, in which nonlocal exchange interactions are responsible for the spin gap of 0.4 eV and the antiferromagnetic order. We show that hole doping of FeGa3 leads, within DMFT, to a notable strengthening of many-body renormalizations. C1 [Gamza, M. B.; Puri, A.; Aronson, M. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Tomczak, J. M.; Kotliar, G.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Brown, C.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Brown, C.] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19716 USA. [Puri, A.; Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Gamza, MB (reprint author), Univ London, Dept Phys, Egham TW20 0EX, Surrey, England. RI Tomczak, Jan/A-9729-2012; Brown, Craig/B-5430-2009 OI Tomczak, Jan/0000-0003-1581-8799; Brown, Craig/0000-0002-9637-9355 FU US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH1886]; Department of Defense National Security Science and Engineering Faculty Fellowship via the Air Force Office of Scientific Research; NSF [DMR 1308141] FX Work at Brookhaven National Laboratory (M.G., A.P., and M.C.A.) was carried out under the auspices of the US Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH1886. Research at Rutgers University (J.M.T. and G.K.) was sponsored by the Department of Defense National Security Science and Engineering Faculty Fellowship via the Air Force Office of Scientific Research. J.M.T. and G.K. were further supported by the NSF Grant No. DMR 1308141. NR 100 TC 7 Z9 7 U1 4 U2 41 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 6 PY 2014 VL 89 IS 19 AR 195102 DI 10.1103/PhysRevB.89.195102 PG 19 WC Physics, Condensed Matter SC Physics GA AG6LM UT WOS:000335530100001 ER PT J AU Bhattacharya, T Cohen, SD Gupta, R Joseph, A Lin, HW Yoon, B AF Bhattacharya, Tanmoy Cohen, Saul D. Gupta, Rajan Joseph, Anosh Lin, Huey-Wen Yoon, Boram CA PNDME Collaboration TI Nucleon charges and electromagnetic form factors from 2+1+1-flavor lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID ELECTRIC-DIPOLE MOMENTS; QUANTUM CHROMODYNAMICS; ULTRACOLD NEUTRONS; STAGGERED QUARKS; PRECISION; MASS AB We present lattice-QCD results on the nucleon isovector axial, scalar and tensor charges, the isovector electromagnetic Dirac and Pauli form factors, and the connected parts of the isoscalar charges. The calculations have been done using two ensembles of highly improved staggered quarks lattices generated by the MILC collaboration with 2 + 1 + 1 dynamical flavors at a lattice spacing of 0.12 fm and with light-quark masses corresponding to pions with masses 310 and 220 MeV. We perform a systematic study including excited-state degrees of freedom and examine the dependence of the extracted nucleon matrix elements on source-sink separation. This study demonstrates with high-statistics data that including excited-state contributions and generating data at multiple separations is necessary to remove contamination that would otherwise lead to systematic error. We also determine the renormalization constants of the associated quark bilinear operators in the RI-sMOM scheme and make comparisons of our renormalized results with previous dynamical-lattice calculations. C1 [Bhattacharya, Tanmoy; Gupta, Rajan; Joseph, Anosh; Yoon, Boram] Los Alamos Natl Lab, Theoret Div T2, Los Alamos, NM 87545 USA. [Cohen, Saul D.; Lin, Huey-Wen] Univ Washington, Dept Phys, Seattle, WA 98195 USA. RP Bhattacharya, T (reprint author), Los Alamos Natl Lab, Theoret Div T2, Los Alamos, NM 87545 USA. RI Bhattacharya, Tanmoy/J-8956-2013; Joseph, Anosh/F-9283-2012; OI Bhattacharya, Tanmoy/0000-0002-1060-652X; Joseph, Anosh/0000-0003-4288-8207; Gupta, Rajan/0000-0003-1784-3058 FU Office of Science of the U.S. Department of Energy; Extreme Science and Engineering Discovery Environment (XSEDE); National Science Foundation [OCI-1053575]; DOE [DE-KA-1401020, DE-FG02-97ER4014]; Institutional Computing at LANL FX We thank the MILC collaboration for providing the 2 + 1 + 1 flavor HISQ lattices used in our calculations. Simulations were carried out on computer facilities of the USQCD collaboration, which are funded by the Office of Science of the U.S. Department of Energy, and by the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant No. OCI-1053575. The calculations used the Chroma software suite [33]. T. B., R. G., A.J. and B.Y. are supported in part by DOE Grant No. DE-KA-1401020. The work of H. W. L. and S. D. C. is supported by DOE Grant No. DE-FG02-97ER4014. We also thank Vincenzo Cirigliano, Alejandro Garcia and Martin Gonzalez-Alonso for comments and discussions, and Jeremy Green for the updated LHPC numbers. We acknowledge Institutional Computing at LANL for support of this project. NR 71 TC 35 Z9 35 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 6 PY 2014 VL 89 IS 9 AR 094502 DI 10.1103/PhysRevD.89.094502 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AG6MJ UT WOS:000335532400002 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Miyashita, TS Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Sciolla, G Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Piredda, G Bunger, C Dittrich, S Grunberg, O Hartmann, T Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Anulli, F Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Lewis, P Lindemann, D Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wisniewski, WJ Wulsin, HW Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu I. Solodov, E. P. Todyshev, K. Yu Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Piredda, G. Buenger, C. Dittrich, S. Gruenberg, O. Hartmann, T. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Anulli, F. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Lewis, P. Lindemann, D. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Albert, J. Banerjee, Sw Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BaBar Collaboration TI Cross sections for the reactions e_e-. K0 SK0 L, K0 SK0 Lp_p-, K0 SK0 Sp_p-, and K0 SK0 SK_K- from events with initial- state radiation SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR; TAGGED PHOTONS AB We study the processes e_e-. K0 SK0 L., K0 SK0 Lp_p-., K0 SK0 Sp_p-., and K0 SK0 SK_K-., where the photon is radiated from the initial state, providing cross section measurements for the hadronic states over a continuum of center- of- mass energies. The results are based on 469 fb- 1 of data collected with the BABAR detector at SLAC. We observe the.d1020_ resonance in the K0 SK0 L final state and measure the product of its electronic width and branching fraction with about 3% uncertainty. We present a measurement of the e_e-. K0 SK0 L cross section in the energy range from 1.06 to 2.2 GeV and observe the production of a resonance at 1.67 GeV. We present the first measurements of the e_e-. K0 SK0 Lp_p-, K0 SK0 Sp_p-, and K0 SK0 SK_K- cross sections and study the intermediate resonance structures. We obtain the first observations of J=. decay to the K0 SK0 Lp_p-, K0 SK0 Sp_p-, and K0 SK0 SK_K- final states. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Koch, H.; Schroeder, T.] Ruhr Univ Bochum, Inst Expt Phys, D-44780 Bochum, Germany. [Hearty, C.; Mattison, T. S.; McKenna, J. A.; So, R. Y.] Univ British Columbia, Vancouver, BC V6T 1Z1, Canada. [Khan, A.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Blinov, V. E.; Buzykaev, A. R.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skovpen, Yu I.; Solodov, E. P.; Todyshev, K. Yu] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Serednyakov, S. I.; Skovpen, Yu I.; Solodov, E. P.; Todyshev, K. Yu] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Blinov, V. E.; Onuchin, A. P.] Novosibirsk State Tech Univ, Novosibirsk 630092, Russia. [Lankford, A. J.; Mandelkern, M.] Univ Calif Irvine, Irvine, CA 92697 USA. [Dey, B.; Gary, J. W.; Long, O.] Univ Calif Riverside, Riverside, CA 92521 USA. [Campagnari, C.; Sevilla, M. Franco; Hong, T. M.; Kovalskyi, D.; Richman, J. D.; West, C. A.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Eisner, A. M.; Lockman, W. S.; Vazquez, W. Panduro; Schumm, B. 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[De Nardo, G.; Onorato, G.; Sciacca, C.] Univ Naples Federico II, Dipartimento Sci Fis, I-80126 Naples, Italy. [Martinelli, M.; Raven, G.] Natl Inst Nucl Phys & High Energy Phys, NIKHEF, NL-1009 DB Amsterdam, Netherlands. [Jessop, C. P.; LoSecco, J. M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Honscheid, K.; Kass, R.] Ohio State Univ, Columbus, OH 43210 USA. [Feltresi, E.; Margoni, M.; Morandin, M.; Posocco, M.; Rotondo, M.; Simi, G.; Simonetto, F.; Stroili, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Feltresi, E.; Margoni, M.; Simi, G.; Simonetto, F.; Stroili, R.] Univ Padua, Dipartimento Fis, I-35131 Padua, Italy. [Akar, S.; Ben-Haim, E.; Bomben, M.; Bonneaud, G. R.; Briand, H.; Calderini, G.; Chauveau, J.; Leruste, Ph; Marchiori, G.; Ocariz, J.] Univ Paris 07, Univ Paris 06, CNRS, Lab Phys Nucl & Hautes Energies,IN2P3, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Pacetti, S.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Biasini, M.; Pacetti, S.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Perez, A.; Rizzo, G.; Walsh, J. J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Dittrich, S.; Gruenberg, O.; Hartmann, T.; Hess, M.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; Vasseur, G.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wisniewski, W. J.; Wulsin, H. W.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Peruzzi, I. M.] Univ Tabuk, Tabuk 71491, Saudi Arabia. [Ayad, R.] Univ Perugia, Dipartimento Fis, I-06100 Perugia, Italy. [Malaescu, B.] CNRS, IN2P3, Lab Phys Nucl & Hautes Energies, Paris, France. [Barlow, R. J.] Univ Huddersfield, Huddersfield HD1 3DH, W Yorkshire, England. [Godang, R.] Univ S Alabama, Mobile, AL 36688 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. [Anulli, F.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [White, R. M.] Univ Tecn Federico Santa Maria, Valparaiso 2390123, Chile. RP Lees, JP (reprint author), Univ Savoie, LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. RI Calcaterra, Alessandro/P-5260-2015; Lusiani, Alberto/A-3329-2016; Morandin, Mauro/A-3308-2016; Di Lodovico, Francesca/L-9109-2016; Patrignani, Claudia/C-5223-2009; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Monge, Maria Roberta/G-9127-2012; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015 OI Calcaterra, Alessandro/0000-0003-2670-4826; Lusiani, Alberto/0000-0002-6876-3288; Morandin, Mauro/0000-0003-4708-4240; Di Lodovico, Francesca/0000-0003-3952-2175; Patrignani, Claudia/0000-0002-5882-1747; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Monge, Maria Roberta/0000-0003-1633-3195; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975 NR 35 TC 11 Z9 11 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 6 PY 2014 VL 89 IS 9 AR 092002 DI 10.1103/PhysRevD.89.092002 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AG6MJ UT WOS:000335532400001 ER PT J AU Hong, S Tong, S Park, WI Hiranaga, Y Cho, YS Roelofs, A AF Hong, Seungbum Tong, Sheng Park, Woon Ik Hiranaga, Yoshiomi Cho, Yasuo Roelofs, Andreas TI Charge gradient microscopy SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE screen charge; atomic force microscopy; piezoresponse; charge scraping ID OPTICAL COHERENCE TOMOGRAPHY; FORCE MICROSCOPY; 180-DEGREES; INTEGRATION AB Here we present a simple and fast method to reliably image polarization charges using charge gradient microscopy (CGM). We collected the current from the grounded CGM probe while scanning a periodically poled lithium niobate single crystal and single-crystal LiTaO3 thin film on the Cr electrode. We observed current signals at the domains and domain walls originating from the displacement current and the relocation or removal of surface charges, which enabled us to visualize the ferroelectric domains at a scan frequency above 78 Hz over 10 mu m. We envision that CGM can be used in high-speed ferroelectric domain imaging and piezoelectric energy-harvesting devices. C1 [Hong, Seungbum; Park, Woon Ik] Argonne Natl Lab, Mat Sci Div, Lemont, IL 60439 USA. [Hong, Seungbum; Tong, Sheng; Park, Woon Ik; Roelofs, Andreas] Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA. [Hiranaga, Yoshiomi; Cho, Yasuo] Tohoku Univ, Res Inst Elect Commun, Sendai, Miyagi 9808577, Japan. RP Hong, S (reprint author), Argonne Natl Lab, Mat Sci Div, Lemont, IL 60439 USA. EM hong@anl.gov; roelofs@anl.gov RI Tong, Sheng/A-2129-2011; Hong, Seungbum/B-7708-2009; Roelofs, Andreas/H-1742-2011; OI Tong, Sheng/0000-0003-0355-7368; Hong, Seungbum/0000-0002-2667-1983; Roelofs, Andreas/0000-0003-4141-3082; Park, Woon Ik/0000-0002-2577-477X FU US Department of Energy, Office of Science, Materials Sciences and Engineering Division; Center for Nanoscale Materials, a US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facilities [DE-AC02-06CH11357] FX The authors acknowledge stimulating discussions with S. Hruszkewycz at Argonne National Laboratory, S. H. Baek at Korea Institute of Science and Technology, Korea, and B. Rodriguez at Trinity College, Ireland. The work was supported by the US Department of Energy, Office of Science, Materials Sciences and Engineering Division and by the Center for Nanoscale Materials, a US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facilities under Contract DE-AC02-06CH11357. The CGM and PFM in the main text and CGM/PFM/EFM/C-AFM in ambient condition in the SI Appendix were performed at Materials Science Division and the vacuum PFM and CGM and SEM (S. H., S. T., and W. I. P.) in the SI Appendix were performed at the Center for Nanoscale Materials and Electron Microscopy Center. We acknowledge Y.-Y. Choi and J. R. Guest at Argonne National Laboratory for their support in CGM experiments. NR 29 TC 10 Z9 10 U1 3 U2 34 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 6 PY 2014 VL 111 IS 18 BP 6566 EP 6569 DI 10.1073/pnas.1324178111 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG5RX UT WOS:000335477300028 PM 24760831 ER PT J AU Hochstrasser, ML Taylor, DW Bhat, P Guegler, CK Sternberg, SH Nogales, E Doudna, JA AF Hochstrasser, Megan L. Taylor, David W. Bhat, Prashant Guegler, Chantal K. Sternberg, Samuel H. Nogales, Eva Doudna, Jennifer A. TI CasA mediates Cas3-catalyzed target degradation during CRISPR RNA-guided interference SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID BACTERIAL IMMUNE-SYSTEM; IN-VITRO RECONSTITUTION; ELECTRON-MICROSCOPY; NEW-GENERATION; COMPLEX; DNA; CASCADE; DEFENSE; THERMOPHILUS; PROKARYOTES AB In bacteria, the clustered regularly interspaced short palindromic repeats (CRISPR)-associated (Cas) DNA-targeting complex Cascade (CRISPR-associated complex for antiviral defense) uses CRISPR RNA (crRNA) guides to bind complementary DNA targets at sites adjacent to a trinucleotide signature sequence called the protospacer adjacent motif (PAM). The Cascade complex then recruits Cas3, a nuclease-helicase that catalyzes unwinding and cleavage of foreign double-stranded DNA (dsDNA) bearing a sequence matching that of the crRNA. Cascade comprises the CasA-E proteins and one crRNA, forming a structure that binds and unwinds dsDNA to form an R loop in which the target strand of the DNA base pairs with the 32-nt RNA guide sequence. Single-particle electron microscopy reconstructions of dsDNA-bound Cascade with and without Cas3 reveal that Cascade positions the PAM-proximal end of the DNA duplex at the CasA subunit and near the site of Cas3 association. The finding that the DNA target and Cas3 colocalize with CasA implicates this subunit in a key target-validation step during DNA interference. We show biochemically that base pairing of the PAM region is unnecessary for target binding but critical for Cas3-mediated degradation. In addition, the L1 loop of CasA, previously implicated in PAM recognition, is essential for Cas3 activation following target binding by Cascade. Together, these data show that the CasA subunit of Cascade functions as an essential partner of Cas3 by recognizing DNA target sites and positioning Cas3 adjacent to the PAM to ensure cleavage. C1 [Hochstrasser, Megan L.; Bhat, Prashant; Nogales, Eva; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Taylor, David W.; Nogales, Eva; Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Taylor, David W.; Nogales, Eva; Doudna, Jennifer A.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Guegler, Chantal K.; Sternberg, Samuel H.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Nogales, E (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM enogales@lbl.gov; doudna@berkeley.edu OI Taylor, David/0000-0002-6198-1194 FU US National Science Foundation (NSF) [1244557] FX We thank G. Lander, P. Grob, Y. He, and T. Houweling for expert EM and image-processing assistance; K. Zhou and K. Condon for technical assistance; J. van der Oost, H.-W. Wang, B. Wiedenheft, and members of the E.N. and J. A. D. laboratories for helpful discussions. This project was funded by US National Science Foundation (NSF) Grant 1244557 (to J. A. D.). S. H. S. is an NSF and National Defense Science and Engineering Graduate Research Fellow. E.N. and J. A. D. are Howard Hughes Medical Institute Investigators. NR 36 TC 51 Z9 53 U1 3 U2 19 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 6 PY 2014 VL 111 IS 18 BP 6618 EP 6623 DI 10.1073/pnas.1405079111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG5RX UT WOS:000335477300037 PM 24748111 ER PT J AU Trastoy, B Lomino, JV Pierce, BG Carter, LG Gunther, S Giddens, JP Snyder, GA Weiss, TM Weng, ZP Wang, LX Sundberg, EJ AF Trastoy, Beatriz Lomino, Joseph V. Pierce, Brian G. Carter, Lester G. Guenther, Sebastian Giddens, John P. Snyder, Greg A. Weiss, Thomas M. Weng, Zhiping Wang, Lai-Xi Sundberg, Eric J. TI Crystal structure of Streptococcus pyogenes EndoS, an immunomodulatory endoglycosidase specific for human IgG antibodies SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID BETA-N-ACETYLGLUCOSAMINIDASE; GLYCAN HYDROLYSIS; HUMAN-IMMUNOGLOBULINS; GLYCOSYLATION; GLYCOFORMS; SUBSTRATE; PROTEIN; ENZYME; SPEB; TRANSGLYCOSYLATION AB To evade host immune mechanisms, many bacteria secrete immuno-modulatory enzymes. Streptococcus pyogenes, one of the most common human pathogens, secretes a large endoglycosidase, EndoS, which removes carbohydrates in a highly specific manner from IgG antibodies. This modification renders antibodies incapable of eliciting host effector functions through either complement or Fc. receptors, providing the bacteria with a survival advantage. On account of this antibody-specific modifying activity, EndoS is being developed as a promising injectable therapeutic for autoimmune diseases that rely on autoantibodies. Additionally, EndoS is a key enzyme used in the chemoenzymatic synthesis of homogenously glycosylated antibodies with tailored Fc. receptor-mediated effector functions. Despite the tremendous utility of this enzyme, the molecular basis of EndoS specificity for, and processing of, IgG antibodies has remained poorly understood. Here, we report the X-ray crystal structure of EndoS and provide a model of its encounter complex with its substrate, the IgG1 Fc domain. We show that EndoS is composed of five distinct protein domains, including glycosidase, leucine-rich repeat, hybrid Ig, carbohydrate binding module, and three-helix bundle domains, arranged in a distinctive V-shaped conformation. Our data suggest that the substrate enters the concave interior of the enzyme structure, is held in place by the carbohydrate binding module, and that concerted conformational changes in both enzyme and substrate are required for subsequent antibody deglycosylation. The EndoS structure presented here provides a framework from which novel endoglycosidases could be engineered for additional clinical and biotechnological applications. C1 [Trastoy, Beatriz; Lomino, Joseph V.; Guenther, Sebastian; Giddens, John P.; Snyder, Greg A.; Wang, Lai-Xi; Sundberg, Eric J.] Univ Maryland, Sch Med, Inst Human Virol, Baltimore, MD 21201 USA. [Lomino, Joseph V.; Giddens, John P.; Wang, Lai-Xi] Univ Maryland, Sch Med, Dept Biochem & Mol Biol, Baltimore, MD 21201 USA. [Snyder, Greg A.; Sundberg, Eric J.] Univ Maryland, Sch Med, Dept Med, Baltimore, MD 21201 USA. [Sundberg, Eric J.] Univ Maryland, Sch Med, Dept Microbiol & Immunol, Baltimore, MD 21201 USA. [Pierce, Brian G.; Weng, Zhiping] Univ Massachusetts, Sch Med, Program Bioinformat & Integrat Biol, Worcester, MA 01655 USA. [Pierce, Brian G.; Weng, Zhiping] Univ Massachusetts, Sch Med, Dept Biochem & Mol Pharmacol, Worcester, MA 01655 USA. [Carter, Lester G.; Weiss, Thomas M.] Stanford Linear Accelerator Ctr, Natl Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. RP Sundberg, EJ (reprint author), Univ Maryland, Sch Med, Inst Human Virol, Baltimore, MD 21201 USA. EM esundberg@ihv.umaryland.edu RI Carter, Lester/G-6561-2014; Trastoy , Beatriz/F-3692-2016; OI Trastoy , Beatriz/0000-0002-2178-732X; Pierce, Brian/0000-0003-4821-0368; Gunther, Sebastian/0000-0002-7329-6653 FU National Institutes of Health [R01AI090866, R01 GM080374]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Department of Energy, Office of Biological and Environmental Research; National Institutes of Health, National Center for Research Resources, Biomedical Technology Program FX We thank the beamline scientists at 23-ID-D and 23-ID-B, Advanced Photon Source (APS) and at 11-1, Stanford Synchrotron Radiation Lightsource (SSRL). These studies were supported by National Institutes of Health Grants R01AI090866 (to E.J.S.) and R01 GM080374 (to L.-X. W.). Use of APS is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. Portions of this research were carried out at SSRL, a national user facility operated by Stanford University on behalf of the US Department of Energy, Office of Basic Energy Sciences. The SSRL Structural Molecular Biology Program is supported by the Department of Energy, Office of Biological and Environmental Research, and by the National Institutes of Health, National Center for Research Resources, Biomedical Technology Program. NR 38 TC 7 Z9 7 U1 7 U2 22 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 6 PY 2014 VL 111 IS 18 BP 6714 EP 6719 DI 10.1073/pnas.1322908111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG5RX UT WOS:000335477300053 PM 24753590 ER PT J AU Anderson, JC Wan, Y Kim, YM Pasa-Tolic, L Metz, TO Peck, SC AF Anderson, Jeffrey C. Wan, Ying Kim, Young-Mo Pasa-Tolic, Ljiljana Metz, Thomas O. Peck, Scott C. TI Decreased abundance of type III secretion system-inducing signals in Arabidopsis mkp1 enhances resistance against Pseudomonas syringae SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID PV. TOMATO DC3000; GENE-EXPRESSION; INNATE IMMUNITY; PLANT; PATHOGENICITY; TRANSLOCATION; BACTERIA; BIOSYNTHESIS; METABOLOMICS; PHASEOLICOLA AB Genes encoding the virulence-promoting type III secretion system (T3SS) in phytopathogenic bacteria are induced at the start of infection, indicating that recognition of signals from the host plant initiates this response. However, the precise nature of these signals and whether their concentrations can be altered to affect the biological outcome of host-pathogen interactions remain speculative. Here we use a metabolomic comparison of resistant and susceptible genotypes to identify plant-derivedmetabolites that induce T3SS genes in Pseudomonas syringae pv tomato DC3000 and report that mapk phosphatase 1 (mkp1), an Arabidopsis mutant that is more resistant to bacterial infection, produces decreased levels of these bioactive compounds. Consistent with these observations, T3SS effector expression and delivery by DC3000 was impaired when infecting the mkp1 mutant. The addition of bioactive metabolites fully restored T3SS effector delivery and suppressed the enhanced resistance in the mkp1 mutant. Pretreatment of plants with pathogen-associated molecular patterns (PAMPs) to induce PAMP-triggered immunity (PTI) also restricts T3SS effector delivery and enhances resistance by unknown mechanisms, and the addition of the bioactive metabolites similarly suppressed both aspects of PTI. Together, these results demonstrate that DC3000 perceives multiple signals derived from plants to initiate its T3SS and that the level of these host-derived signals impacts bacterial pathogenesis. C1 [Anderson, Jeffrey C.; Wan, Ying; Peck, Scott C.] Univ Missouri, Div Biochem, Columbia, MO 65211 USA. [Anderson, Jeffrey C.; Wan, Ying; Peck, Scott C.] Univ Missouri, Christopher S Bond Life Sci Ctr, Columbia, MO 65211 USA. [Anderson, Jeffrey C.; Wan, Ying; Peck, Scott C.] Univ Missouri, Interdisciplinary Plant Grp, Columbia, MO 65211 USA. [Kim, Young-Mo; Metz, Thomas O.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99354 USA. [Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. RP Anderson, JC (reprint author), Univ Missouri, Div Biochem, Columbia, MO 65211 USA. EM andersonjef@missouri.edu; pecks@missouri.edu RI Kim, Young-Mo/D-3282-2009; OI Kim, Young-Mo/0000-0002-8972-7593; Metz, Tom/0000-0001-6049-3968 FU National Science Foundation [IOS 1051286]; Department of Energy's Office of Biological and Environmental Research; DOE Office of Biological and Environmental Research Genome Sciences Program FX We thank Dr. Greg Martin for comments and for providing the DC3000 hrcC- strain, avrPto-CyaA plasmid, and anti-AvrPto antibody. This work was supported by National Science Foundation Grant IOS 1051286 (to S. C. P.). A portion of the research was performed at the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated by Battelle for the Department of Energy (DOE) under Contract DE-AC05-76RLO 1830. Portions of this research were enabled by capabilities developed by the PNNL Pan-omics Program under support from the DOE Office of Biological and Environmental Research Genome Sciences Program. NR 42 TC 11 Z9 11 U1 1 U2 37 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 6 PY 2014 VL 111 IS 18 BP 6846 EP 6851 DI 10.1073/pnas.1403248111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG5RX UT WOS:000335477300075 PM 24753604 ER PT J AU Wang, CY Zhu, YW Caceres, TB Liu, L Peng, JH Wang, JC Chen, JJ Chen, XW Zhang, ZY Zuo, XB Gong, QG Teng, MK Hevel, JM Wu, JH Shi, YY AF Wang, Chongyuan Zhu, Yuwei Caceres, Tamar B. Liu, Lei Peng, Junhui Wang, Junchen Chen, Jiajing Chen, Xuwen Zhang, Zhiyong Zuo, Xiaobing Gong, Qingguo Teng, Maikun Hevel, Joan M. Wu, Jihui Shi, Yunyu TI Structural Determinants for the Strict Monomethylation Activity by Trypanosoma brucei Protein Arginine Methyltransferase 7 SO STRUCTURE LA English DT Article ID SCATTERING DATA-ANALYSIS; SYMMETRIC DIMETHYLATION; CRYSTAL-STRUCTURE; PROGRAM PACKAGE; METHYLATION; PRMT7; INSIGHTS; COMPLEX; BINDING; SYSTEM AB Trypanosoma brucei protein arginine methyltransferase 7 (TbPRMT7) exclusively generates monomethylarginine (MMA), which directs biological consequences distinct from that of symmetric dimethylarginine (SDMA) and asymmetric dimethylarginine (ADMA). However, determinants controlling the strict monomethylation activity are unknown. We present the crystal structure of the TbPRMT7 active core in complex with S-adenosyl-L-homocysteine (AdoHcy) and a histone H4 peptide substrate. In the active site, residues E172, E181, and Q329 hydrogen bond the guanidino group of the target arginine and align the terminal guanidino nitrogen in a position suitable for nucleophilic attack on the methyl group of S-adenosyl-L-methionine (AdoMet). Structural comparisons and isothermal titration calorimetry data suggest that the TbPRMT7 active site is narrower than those of protein arginine dimethyltransferases, making it unsuitable to bind MMA in a manner that would support a second turnover, thus abolishing the production of SDMA and ADMA. Our results present the structural interpretations for the monomethylation activity of TbPRMT7. C1 [Wang, Chongyuan; Zhu, Yuwei; Liu, Lei; Peng, Junhui; Wang, Junchen; Chen, Jiajing; Chen, Xuwen; Zhang, Zhiyong; Gong, Qingguo; Teng, Maikun; Wu, Jihui; Shi, Yunyu] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale & Sch Life Sci, Hefei 230027, Anhui, Peoples R China. [Caceres, Tamar B.; Hevel, Joan M.] Utah State Univ, Dept Chem & Biochem, Logan, UT 84322 USA. [Zuo, Xiaobing] Argonne Natl Lab, Adv Photon Source, Chicago, IL 60437 USA. RP Wu, JH (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale & Sch Life Sci, Hefei 230027, Anhui, Peoples R China. EM wujihui@ustc.edu.cn; yyshi@ustc.edu.cn FU National Basic Research Program of China [2011CB966302, 2012CB917201, 2011CB911104, 2013CB910200]; Chinese Academy of Sciences [XDB08010100]; Chinese National Natural Science Foundation [31270760, 31170693, 31330018]; Chinese Academy of Science [KJZD-EW-L05]; Anhui Nature Science Foundation [1208085MC38]; Herman Frasch Foundation [657-HF07]; National Science Foundation [0920776] FX We thank Dr. Shilai Bao (Institute of Genetics and Developmental Biology, Chinese Academy of Sciences) for providing the gene of CePRMT5 and staff members of Beamline BL17U at SSRF for the assistance in data collection. Financial support for this project was provided by the National Basic Research Program of China (973 Program grants 2011CB966302, 2012CB917201, 2011CB911104, and 2013CB910200), the Strategic Priority Research Program of the Chinese Academy of Sciences (grant XDB08010100), the Chinese National Natural Science Foundation (grants 31270760, 31170693, and 31330018), the Chinese Academy of Science (grant KJZD-EW-L05), the Anhui Nature Science Foundation (grant 1208085MC38), the Herman Frasch Foundation (award 657-HF07), and the National Science Foundation (award 0920776). NR 46 TC 17 Z9 17 U1 3 U2 30 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD MAY 6 PY 2014 VL 22 IS 5 BP 756 EP 768 DI 10.1016/j.str.2014.03.003 PG 13 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA AG5FB UT WOS:000335443700013 PM 24726341 ER PT J AU Martin, G Sinclair, CW Lebensohn, RA AF Martin, Guilhem Sinclair, Chad W. Lebensohn, Ricardo A. TI Microscale plastic strain heterogeneity in slip dominated deformation of magnesium alloy containing rare earth SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Magnesium polycrystals; Digital image correlation; EBSD; Strain heterogeneities; Crystal plasticity ID ROOM-TEMPERATURE; SINGLE-CRYSTALS; AZ31B SHEET; MG ALLOYS; DUPLEX STEELS; NONBASAL SLIP; SHEAR BANDS; MECHANISMS; TEXTURE; BEHAVIOR AB The propensity for the magnesium alloy ZEK100 to develop large microscale plistic strain heterogeneity has been quantified and correlated to microstructure using a combination of experiments and simulations. Conditions were specifically selected where deformation is dominated by slip rather than twinning. Digital image correlation measurements of intragranular plastic strain heterogeneity have revealed plastic strains as large as 5 times the macroscopic tensile strain. This strain amplification was found to be neither spatially correlated nor correlated with crystal orientation. Large local strains were, however, found to be statistically linked to proximity to grain boundaries. This suggests the importance of interactions between neighboring grains. To investigate this further full-field viscoplastic Fast Fourier Transform (VPFFT) crystal plasticity simulations were performed on synthetic microstructures representative of the material studied experimentally. It was found that both the macroscopic stress-strain response as well as the local plastic strain distribution could be well reproduced when the anisotropy in 'hardness' of the basal and non-basal slip systems was sufficiently high. Strain amplification was found to occur, in this case, to slip in regions of high basal slip activity adjacent to regions of high non-basal slip activity. (C) 2014 Elsevier B.V. All rights reserved. C1 [Martin, Guilhem; Sinclair, Chad W.] Univ British Columbia, Dept Mat Engn, Vancouver, BC V6T 1Z4, Canada. [Martin, Guilhem] Grp GPM2, Lab Sci & Ingn Mat & Proc SIMaP, F-38402 St Martin Dheres, France. [Lebensohn, Ricardo A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87544 USA. RP Martin, G (reprint author), Grp GPM2, Lab Sci & Ingn Mat & Proc SIMaP, Domaine Univ,101 Rue Phys, F-38402 St Martin Dheres, France. EM guilhem.martin@simap.grenoble-inp.fr RI Lebensohn, Ricardo/A-2494-2008; Sinclair, Chad/O-5744-2016 OI Lebensohn, Ricardo/0000-0002-3152-9105; Sinclair, Chad/0000-0002-6465-6952 FU NSREC-Canada FX The authors wish to express their gratitude to NSREC-Canada for the financial support of this work through the MAgNET Strategic Research Network. General Motors Canada is acknowledged for providing the materials. Michel Bornert is gratefully acknowledged for providing the software for the strain mapping analysis (CMV) and for his assistance with this tool. References NR 71 TC 20 Z9 20 U1 6 U2 34 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAY 6 PY 2014 VL 603 BP 37 EP 51 DI 10.1016/j.msea.2014.01.102 PG 15 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AG0KO UT WOS:000335104600005 ER PT J AU Ji, YD Zhang, Y Gao, M Yuan, Z Xia, YD Jin, CQ Tao, BW Chen, CL Jia, QX Lin, Y AF Ji, Yanda Zhang, Yin Gao, Min Yuan, Zhen Xia, Yudong Jin, Changqing Tao, Bowan Chen, Chonglin Jia, Quanxi Lin, Yuan TI Role of microstructures on the M1-M2 phase transition in epitaxial VO2 thin films SO SCIENTIFIC REPORTS LA English DT Article ID METAL-INSULATOR TRANSITIONS; VANADIUM DIOXIDE; DIELECTRIC-PROPERTIES; SINGLE-CRYSTAL; STRESS AB Vanadium dioxide (VO2) with its unique sharp resistivity change at the metal-insulator transition (MIT) has been extensively considered for the near-future terahertz/infrared devices and energy harvesting systems. Controlling the epitaxial quality and microstructures of vanadium dioxide thin films and understanding the metal-insulator transition behaviors are therefore critical to novel device development. The metal-insulator transition behaviors of the epitaxial vanadium dioxide thin films deposited on Al2O3 (0001) substrates were systematically studied by characterizing the temperature dependency of both Raman spectrum and Fourier transform infrared spectroscopy. Our findings on the correlation between the nucleation dynamics of intermediate monoclinic (M2) phase with microstructures will open a new avenue for the design and integration of advanced heterostructures with controllable multifunctionalities for sensing and imaging system applications. C1 [Ji, Yanda; Zhang, Yin; Gao, Min; Xia, Yudong; Tao, Bowan; Lin, Yuan] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Sichuan, Peoples R China. [Yuan, Zhen; Jin, Changqing] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Chen, Chonglin] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Lin, Y (reprint author), Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Sichuan, Peoples R China. EM linyuan@uestc.edu.cn RI Jia, Q. X./C-5194-2008; Ji, Yanda/C-9366-2013; lin, yuan/B-9955-2013; gao, min/F-4825-2015 OI Ji, Yanda/0000-0001-9979-6982; FU National Basic Research Program of China (973 Program) [2011CB301705]; National Natural Science Foundation of China [11329402, 51172036]; Ministry of Education, P. R. China; U.S. Department of Energy through the Center for Integrated Nanotechnologies; U.S. Department of Energy, Office of Basic Energy Sciences; U.S. Department of Energy [DE-AC52-06NA25396] FX This work was supported by the National Basic Research Program of China (973 Program, No. 2011CB301705), the National Natural Science Foundation of China (Nos. 11329402 and 51172036). Y. D. Ji acknowledges the support from the Scholarship Award for Excellent Doctoral Student granted by Ministry of Education, P. R. China. The work at Los Alamos was supported, in part, by the U.S. Department of Energy through the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 29 TC 24 Z9 24 U1 12 U2 191 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 6 PY 2014 VL 4 AR 4854 DI 10.1038/srep04854 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG4ET UT WOS:000335372800001 PM 24798056 ER PT J AU Rashkow, JT Patel, SC Tappero, R Sitharaman, B AF Rashkow, Jason T. Patel, Sunny C. Tappero, Ryan Sitharaman, Balaji TI Quantification of single-cell nanoparticle concentrations and the distribution of these concentrations in cell population SO JOURNAL OF THE ROYAL SOCIETY INTERFACE LA English DT Article DE nanoparticles; single cell; concentration; quantification; distribution; X-ray fluorescence ID X-RAY-FLUORESCENCE; CARBON NANOTUBES; MICROSCOPY; BIOLOGY AB Quantification of nanoparticle uptake into cells is necessary for numerous applications in cellular imaging and therapy. Herein, synchrotron X-ray fluorescence (SXRF) microscopy, a promising tool to quantify elements in plant and animal cells, was employed to quantify and characterize the distribution of titanium dioxide (TiO2) nanosphere uptake in a population of single cells. These results were compared with average nanoparticle concentrations per cell obtained by widely used inductively coupled plasma mass spectrometry (ICP-MS). The results show that nanoparticle concentrations per cell quantified by SXRF were of one to two orders of magnitude greater compared with ICP-MS. The SXRF results also indicate a Gaussian distribution of the nanoparticle concentration per cell. The results suggest that issues relevant to the field of single-cell analysis, the limitation of methods to determine physical parameters from large population averages leading to potentially misleading information and the lack of any information about the cellular heterogeneity are equally relevant for quantification of nanoparticles in cell populations. C1 [Rashkow, Jason T.; Patel, Sunny C.; Sitharaman, Balaji] SUNY Stony Brook, Dept Biomed Engn, Stony Brook, NY 11794 USA. [Tappero, Ryan] Brookhaven Natl Lab, Natl Synchrotron Light Source, Dept Photon Sci, Upton, NY 11973 USA. RP Sitharaman, B (reprint author), SUNY Stony Brook, Dept Biomed Engn, Stony Brook, NY 11794 USA. EM balaji.sitharaman@stonybrook.edu OI Sitharaman, Balaji/0000-0001-8391-8076 FU U.S. Department of Energy (DOE)-Geosciences [DE-FG02-92ER14244]; DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; National Institutes of Health [1DP2OD007394-01] FX X27A is supported in part by the U.S. Department of Energy (DOE)-Geosciences (DE-FG02-92ER14244 to The University of Chicago, CARS). Use of the NSLS was supported by the DOE, Office of Science, Office of Basic Energy Sciences, under Contract no. DE-AC02-98CH10886. This work was supported by the National Institutes of Health (grant no. 1DP2OD007394-01). NR 20 TC 6 Z9 6 U1 5 U2 49 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1742-5689 EI 1742-5662 J9 J R SOC INTERFACE JI J. R. Soc. Interface PD MAY 6 PY 2014 VL 11 IS 94 AR 20131152 DI 10.1098/rsif.2013.1152 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AD4BT UT WOS:000333191800008 PM 24554576 ER PT J AU Batell, B Wagner, CEM Wang, LT AF Batell, Brian Wagner, Carlos E. M. Wang, Lian-Tao TI Constraints on a very light sbottom SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology; Hadronic Colliders ID SUPERSYMMETRIC STANDARD MODEL; EVEN HIGGS BOSONS; E(+)E(-) COLLISIONS; E+E-ANNIHILATION; BOTTOM SQUARKS; SCALAR QUARKS; MASS; MSSM; SEARCH; LHC AB We investigate the phenomenological viability of a very light bottom squark, with a mass less than half of the Z boson mass. The decays of the Z and Higgs bosons to light sbottom pairs are, in a fairly model independent manner, strongly constrained by the precision electroweak data and Higgs signal strength measurements, respectively. These constraints are complementary to direct collider searches, which depend in detail on assumptions regarding the superpartner spectrum and decays of the sbottom. In particular, if the lightest sbottom has a mass below about 15 GeV, compatibility with these measurements is possible only in a special region of parameter space in which the couplings of the lightest sbottom to the Z and Higgs are suppressed. In this region, the second sbottom is predicted to be lighter than about 300 GeV and can also be searched for directly at the LHC. We also survey relevant collider searches for canonical scenarios with a bino, gravitino, or singlino LSP in the compressed and stealth kinematic regimes and provide suggestions to cover remaining open regions of parameter space. C1 [Batell, Brian; Wagner, Carlos E. M.; Wang, Lian-Tao] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Batell, Brian; Wagner, Carlos E. M.; Wang, Lian-Tao] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Wagner, Carlos E. M.] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. [Wagner, Carlos E. M.; Wang, Lian-Tao] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Batell, B (reprint author), Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. EM batell@uchicago.edu; cwagner@hep.anl.gov; liantaow@uchicago.edu FU U.S. Department of Energy [DE-AC02-06CH11357]; NSF [PHY-0756966]; DOE Early Career Award [DE-SC0003930]; National Science Foundation [PHYS-1066293] FX We are grateful to Patrick Janot for helpful discussions. Work at ANL is supported in part by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. L.T.W. and B.B. are supported by the NSF under grant PHY-0756966 and the DOE Early Career Award under grant DE-SC0003930. This work was supported in part by the National Science Foundation under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. NR 76 TC 6 Z9 6 U1 0 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 5 PY 2014 IS 5 AR 002 DI 10.1007/JHEP05(2014)002 PG 32 WC Physics, Particles & Fields SC Physics GA AY9BZ UT WOS:000347845900002 ER PT J AU Cybart, SA Wong, TJ Cho, EY Beeman, JW Yung, CS Moeckly, BH Dynes, RC AF Cybart, Shane A. Wong, T. J. Cho, E. Y. Beeman, J. W. Yung, C. S. Moeckly, B. H. Dynes, R. C. TI Large scale two-dimensional arrays of magnesium diboride superconducting quantum interference devices SO APPLIED PHYSICS LETTERS LA English DT Article ID JOSEPHSON-JUNCTION PAIRS; ION DAMAGE; THIN-FILMS; YBA2CU3O7-DELTA; BEAM; NANOLITHOGRAPHY; SQUIDS AB Magnetic field sensors based on two-dimensional arrays of superconducting quantum interference devices were constructed from magnesium diboride thin films. Each array contained over 30 000 Josephson junctions fabricated by ion damage of 30 nm weak links through an implant mask defined by nano-lithography. Current-biased devices exhibited very large voltage modulation as a function of magnetic field, with amplitudes as high as 8 mV. (C) 2014 AIP Publishing LLC. C1 [Cybart, Shane A.; Wong, T. J.; Cho, E. Y.; Dynes, R. C.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Cybart, Shane A.; Beeman, J. W.; Dynes, R. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Yung, C. S.; Moeckly, B. H.] Superconductor Technol Inc, Santa Barbara, CA 93111 USA. RP Cybart, SA (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM scybart@ucsd.edu RI Foundry, Molecular/G-9968-2014 FU AFOSR [FA9550-12-C-0050]; ONR [N00014-11-1-0049]; Office of Science and Office of Basic Energy Sciences of the U.S. Department of Energy [DEAC02 05CH11231] FX This work was supported by AFOSR Grant No. FA9550-12-C-0050, ONR Grant No. N00014-11-1-0049, and the Office of Science and Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DEAC02 05CH11231. We gratefully acknowledge B. D. Harteneck of the Molecular Foundry for electron-beam lithography and processing advice. NR 27 TC 5 Z9 5 U1 1 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 5 PY 2014 VL 104 IS 18 AR 182604 DI 10.1063/1.4876129 PG 4 WC Physics, Applied SC Physics GA AH6OF UT WOS:000336249600039 ER PT J AU Luo, ZL Huang, H Zhou, H Chen, ZH Yang, Y Wu, L Zhu, C Wang, H Yang, M Hu, S Wen, H Zhang, X Zhang, Z Chen, L Fong, DD Gao, C AF Luo, Z. L. Huang, H. Zhou, H. Chen, Z. H. Yang, Y. Wu, L. Zhu, C. Wang, H. Yang, M. Hu, S. Wen, H. Zhang, X. Zhang, Z. Chen, L. Fong, D. D. Gao, C. TI Probing the domain structure of BiFeO3 epitaxial films with three-dimensional reciprocal space mapping SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILMS; PHASE; STRAIN AB High-resolution 3-Dimensional Reciprocal Space Mapping (3D-RSM) has been performed on mixed-phase BiFeO3 (BFO) epitaxial films on (001)-oriented LaAlO3 substrates. Our results demonstrate that 3D-RSM is an effective way to present a structural overview of the different BFO polymorphs, domain variants, and even the interfacial regions between coexisting triclinic phases. The dislocation-free boundaries between the triclinic phases revealed by these 3D-RSMs are believed to be responsible for the large electromechanical response found in mixed-phase BFO films. This study demonstrates the unique merits of the 3D-RSM technique for the structural characterization of ferroic films with complicated domain structures. (C) 2014 AIP Publishing LLC. C1 [Luo, Z. L.; Huang, H.; Yang, Y.; Wu, L.; Wang, H.; Yang, M.; Hu, S.; Gao, C.] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China. [Zhou, H.; Wen, H.; Zhang, X.; Zhang, Z.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Chen, Z. H.; Chen, L.] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore. [Zhu, C.; Fong, D. D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Zhu, C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Chen, L.] South Univ Sci & Technol China, Dept Phys, Shenzhen 518055, Guangdong, Peoples R China. RP Luo, ZL (reprint author), Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China. EM zlluo@ustc.edu.cn; cgao@ustc.edu.cn RI CHEN, LANG/A-2251-2011; luo, zhenlin/G-2662-2013; Chen, Zuhuang/E-7131-2011; yang, yuanjun/K-2494-2013 OI Chen, Zuhuang/0000-0003-1912-6490; yang, yuanjun/0000-0002-6976-7416 FU SSRF; National Basic Research Program of China [2010CB934501, 2012CB922004]; Natural Science Foundation of China; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We thank Xin Zhao for discussions on Matlab, and Xiaolong Li and Wen Wen for support at the SSRF. This work was supported by the National Basic Research Program of China (2010CB934501, 2012CB922004) and the Natural Science Foundation of China. D. D. F. was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. The authors thank the staff at beamline BL14B of SSRF and beamline 33-ID-D of APS for their support. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 26 TC 4 Z9 4 U1 4 U2 101 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 5 PY 2014 VL 104 IS 18 AR 182901 DI 10.1063/1.4875579 PG 4 WC Physics, Applied SC Physics GA AH6OF UT WOS:000336249600040 ER PT J AU Lee, TG Wong, CY AF Lee, Teck-Ghee Wong, Cheuk-Yin TI Extended Glauber model of antiproton-nucleus annihilation for all energies and mass numbers SO PHYSICAL REVIEW C LA English DT Article ID VERY-LOW ENERGY; HEAVY-ION COLLISIONS; CROSS-SECTION; MOMENTUM RANGE; 600 MEV/C; SCATTERING; ABSORPTION AB Previous analytical formulas in the Glauber model for high-energy nucleus-nucleus collisions developed by Wong are utilized and extended to study antiproton-nucleus annihilations for both high and low energies, after taking into account the effects of Coulomb and nuclear interactions, and the change of the antiproton momentum inside a nucleus. The extended analytical formulas capture the main features of the experimental antiproton-nucleus annihilation cross sections for all energies and mass numbers. At high antiproton energies, they exhibit the granular property for the lightest nuclei and the black-disk limit for the heavy nuclei. At low antiproton energies, they display the effect of antiproton momentum increase due to the nuclear interaction for light nuclei, and the effect of magnification due to the attractive Coulomb interaction for heavy nuclei. C1 [Lee, Teck-Ghee] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Wong, Cheuk-Yin] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Lee, TG (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RI Lee, Teck Ghee/D-5037-2012; OI Lee, Teck Ghee/0000-0001-9472-3194; Wong, Cheuk-Yin/0000-0001-8223-0659 FU Division of Nuclear Physics, US Department of Energy FX This research was supported in part by the Division of Nuclear Physics, US Department of Energy. NR 40 TC 3 Z9 3 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. 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CA CDF Collaborat TI Invariant-mass distribution of jet pairs produced in association with a W boson in p(p)over-bar collisions at root s=1.96 TeV using the full CDF Run II data set SO PHYSICAL REVIEW D LA English DT Article AB We report on a study of the dijet invariant-mass distribution in events with one identified lepton, a significant imbalance in the total event transverse momentum, and two jets. This distribution is sensitive to the possible production of a new particle in association with a W boson, where the boson decays leptonically. We use the full data set of proton-antiproton collisions at 1.96 TeV center-of-mass energy collected by the Collider Detector at the Fermilab Tevatron, corresponding to an integrated luminosity of 8.9 fb(-1). The data are found to be consistent with standard model expectations, and a 95% confidence level upper limit is set on the production cross section of a W boson in association with a new particle decaying into two jets. C1 [Chen, Y. 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[Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Martinez, Mario /I-3549-2015; vilar, rocio/P-8480-2014; Chiarelli, Giorgio/E-8953-2012; Cavalli-Sforza, Matteo/H-7102-2015; Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Lysak, Roman/H-2995-2014; Liu, Qiuguang/I-8258-2014; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014 OI Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Chiarelli, Giorgio/0000-0001-9851-4816; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155 FU U.S. Department of Energy and National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A.P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, UK; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; Slovak RD Agency; the Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, UK; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); the EU community Marie Curie Fellowship Contract No. 302103. NR 27 TC 5 Z9 5 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 5 PY 2014 VL 89 IS 9 AR 092001 DI 10.1103/PhysRevD.89.092001 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH4MJ UT WOS:000336102000001 ER PT J AU Irsic, V Slosar, A AF Irsic, Vid Slosar, Anze TI Background power subtraction in Ly alpha forest SO PHYSICAL REVIEW D LA English DT Article ID OSCILLATION SPECTROSCOPIC SURVEY; SDSS-III; SPECTRUM; BOSS AB When measuring the one-dimensional (1D) power spectrum of the Lyman-alpha (Ly alpha) forest, it is common to measure the power spectrum in the flux fluctuations redward of the Ly alpha emission of quasars, and to subtract this power from the measurements of the Ly alpha flux power spectrum. This removes the excess power present in the Ly alpha forest, which is believed to be dominated by metal absorption of low-redshift metals uncorrelated with the neutral hydrogen absorbtion in Ly alpha. In this paper we note that, assuming the contaminants are additive in the optical depth, the correction contains a second-order term. We estimate the magnitude of this term for two currently published measurements of the 1D Ly alpha flux power spectrum and show that it is negligible for the current generation of measurements. However, future measurements must take this effect into account when the error bars improve by a factor of 2 or more. C1 [Irsic, Vid] Abdus Salam Int Ctr Theoret Phys, I-34151 Trieste, Italy. [Slosar, Anze] Brookhaven Natl Lab, Upton, NY 11375 USA. RP Irsic, V (reprint author), Abdus Salam Int Ctr Theoret Phys, Str Costiera 11, I-34151 Trieste, Italy. EM virsic@ictp.it; anze@bnl.gov OI Irsic, Vid/0000-0002-5445-461X NR 9 TC 0 Z9 0 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. 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CA CMS Collaboration TI Measurements of t(t)over-bar Spin Correlations and Top-Quark Polarization Using Dilepton Final States in pp Collisions at root s=7 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID PAIR PRODUCTION AB Spin correlations and polarization in the top quark-antiquark system are measured using dilepton final states produced in pp collisions at the LHC at root s = 7 TeV. The data correspond to an integrated luminosity of 5.0 fb(-1) collected with the CMS detector. The measurements are performed using events with two oppositely charged leptons (electrons or muons), a significant imbalance in transverse momentum, and two or more jets, where at least one of the jets is identified as originating from a b quark. The spin correlations and polarization are measured through asymmetries in angular distributions of the two selected leptons, unfolded to the parton level. All measurements are found to be in agreement with predictions of the standard model. 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J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Florent, A.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Bloch, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.; Chamizo Llatas, M.] Univ Strasbourg, Univ Haute Alsace Mulhouse, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Alvarez, J. D. Ruiz; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Inst Phys A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Inst Phys B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Geiser, A.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kraemer, M.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. Oe.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Schroeder, M.; Stein, M.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.; Abdulsalam, A.] DESY, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Goerner, M.; Gosselink, M.; Haller, J.; Heine, K.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, C.; Ntomari, E.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Choudhury, S.; Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Swain, S. K.; Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, EHEP, Bombay 400005, Maharashtra, India. [Banerjee, S.; Guchait, M.; Dugad, S.] Tata Inst Fundamental Res, HECR, Bombay 400005, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Benucci, L.; Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, Milan, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.; Dermenev, A.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Savrin, V.; Tsirova, N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Marinov, A.; Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] CIEMAT, Ctr Invest Energet Medioambient & Tecnol, E-28040 Madrid, Spain. [Albajar, C.; De Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Sharma, A.; Mohanty, A. K.; Giordano, F.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; Pelliccioni, M.; Cossutti, F.; Seixas, J.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. 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Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Abdulsalam, A.; Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Adair, A.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Abdulsalam, A.; Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Abdulsalam, A.; Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. 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RI Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Gonzalez Caballero, Isidro/E-7350-2010; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; Novaes, Sergio/D-3532-2012; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Moon, Chang-Seong/J-3619-2014; de la Cruz, Begona/K-7552-2014; Gregores, Eduardo/F-8702-2012; Cerrada, Marcos/J-6934-2014; Scodellaro, Luca/K-9091-2014; Torassa, Ezio/I-1788-2012; Venturi, Andrea/J-1877-2012; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011 OI Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Novaes, Sergio/0000-0003-0471-8549; Montanari, Alessandro/0000-0003-2748-6373; Moon, Chang-Seong/0000-0001-8229-7829; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812 FU BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP (Brazil); MES (Bulgaria) FX We would like to thank Professor W. Bernreuther and Professor Z.-G. Si for calculating the theoretical predictions of Fig. 1 and Table II for this Letter. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staff at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP ( Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS, and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR, and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (U. S.). NR 40 TC 34 Z9 34 U1 6 U2 71 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 5 PY 2014 VL 112 IS 18 AR 182001 DI 10.1103/PhysRevLett.112.182001 PG 16 WC Physics, Multidisciplinary SC Physics GA AH4LS UT WOS:000336099800004 PM 24856688 ER PT J AU Huber, GM Blok, HP Butuceanu, C Gaskell, D Horn, T Mack, DJ Abbott, D Aniol, K Anklin, H Armstrong, C Arrington, J Assamagan, K Avery, S Baker, OK Barrett, B Beise, EJ Bochna, C Boeglin, W Brash, EJ Breuer, H Chang, CC Chant, N Christy, ME Dunne, J Eden, T Ent, R Fenker, H Gibson, EF Gilman, R Gustafsson, K Hinton, W Holt, RJ Jackson, H Jin, S Jones, MK Keppel, CE Kim, PH Kim, W King, PM Klein, A Koltenuk, D Kovaltchouk, V Liang, M Liu, J Lolos, GJ Lung, A Margaziotis, DJ Markowitz, P Matsumura, A McKee, D Meekins, D Mitchell, J Miyoshi, T Mkrtchyan, H Mueller, B Niculescu, G Niculescu, I Okayasu, Y Pentchev, L Perdrisat, C Pitz, D Potterveld, D Punjabi, V Qin, LM Reimer, PE Reinhold, J Roche, J Roos, PG Sarty, A Shin, IK Smith, GR Stepanyan, S Tang, LG Tadevosyan, V Tvaskis, V van der Meer, RLJ Vansyoc, K Van Westrum, D Vidakovic, S Volmer, J Vulcan, W Warren, G Wood, SA Xu, C Yan, C Zhao, WX Zheng, X Zihlmann, B AF Huber, G. M. Blok, H. P. Butuceanu, C. Gaskell, D. Horn, T. Mack, D. J. Abbott, D. Aniol, K. Anklin, H. Armstrong, C. Arrington, J. Assamagan, K. Avery, S. Baker, O. K. Barrett, B. Beise, E. J. Bochna, C. Boeglin, W. Brash, E. J. Breuer, H. Chang, C. C. Chant, N. Christy, M. E. Dunne, J. Eden, T. Ent, R. Fenker, H. Gibson, E. F. Gilman, R. Gustafsson, K. Hinton, W. Holt, R. J. Jackson, H. Jin, S. Jones, M. K. Keppel, C. E. Kim, P. H. Kim, W. King, P. M. Klein, A. Koltenuk, D. Kovaltchouk, V. Liang, M. Liu, J. Lolos, G. J. Lung, A. Margaziotis, D. J. Markowitz, P. Matsumura, A. McKee, D. Meekins, D. Mitchell, J. Miyoshi, T. Mkrtchyan, H. Mueller, B. Niculescu, G. Niculescu, I. Okayasu, Y. Pentchev, L. Perdrisat, C. Pitz, D. Potterveld, D. Punjabi, V. Qin, L. M. Reimer, P. E. Reinhold, J. Roche, J. Roos, P. G. Sarty, A. Shin, I. K. Smith, G. R. Stepanyan, S. Tang, L. G. Tadevosyan, V. Tvaskis, V. van der Meer, R. L. J. Vansyoc, K. Van Westrum, D. Vidakovic, S. Volmer, J. Vulcan, W. Warren, G. Wood, S. A. Xu, C. Yan, C. Zhao, W. -X. Zheng, X. Zihlmann, B. CA Jefferson Lab Collaboration TI Separated Response Function Ratios in Exclusive, Forward pi(+/-) Electroproduction SO PHYSICAL REVIEW LETTERS LA English DT Article ID RESONANCE REGION; FORM-FACTOR; PHOTOPRODUCTION; PION; DEUTERIUM AB The study of exclusive pi(+/-) electroproduction on the nucleon, including separation of the various structure functions, is of interest for a number of reasons. The ratio R-L=sigma(pi-)(L) / sigma(pi+)(L) is sensitive to isoscalar contamination to the dominant isovector pion exchange amplitude, which is the basis for the determination of the charged pion form factor from electroproduction data. A change in the value of R-T=sigma(pi-)(L) / sigma(pi+)(L) from unity at small -t, to 1/4 at large -t, would suggest a transition from coupling to a (virtual) pion to coupling to individual quarks. Furthermore, the mentioned ratios may show an earlier approach to perturbative QCD than the individual cross sections. We have performed the first complete separation of the four unpolarized electromagnetic structure functions above the dominant resonances in forward, exclusive p pi(+/-) electroproduction on the deuteron at central Q(2) values of 0.6, 1.0, 1.6 GeV2 at W=1.95 GeV, and Q(2)=2.45 GeV2 at W=2.22 GeV. Here, we present the L and T cross sections, with emphasis on R-L and R-T, and compare them with theoretical calculations. Results for the separated ratio R-L indicate dominance of the pion-pole diagram at low -t, while results for R-T are consistent with a transition between pion knockout and quark knockout mechanisms. C1 [Huber, G. M.; Butuceanu, C.; Brash, E. J.; Kovaltchouk, V.; Lolos, G. J.; van der Meer, R. L. J.; Vidakovic, S.; Xu, C.] Univ Regina, Regina, SK S4S 0A2, Canada. [Blok, H. P.; Tvaskis, V.; Volmer, J.] Vrije Univ Amsterdam, NL-1081 HV Amsterdam, Netherlands. [Blok, H. P.; Tvaskis, V.] NIKHEF, NL-1009 DB Amsterdam, Netherlands. [Gaskell, D.; Mack, D. J.; Abbott, D.; Anklin, H.; Baker, O. K.; Dunne, J.; Eden, T.; Ent, R.; Fenker, H.; Gilman, R.; Keppel, C. E.; Liang, M.; Lung, A.; Meekins, D.; Mitchell, J.; Roche, J.; Smith, G. R.; Tang, L. G.; Vulcan, W.; Warren, G.; Wood, S. A.; Yan, C.; Zihlmann, B.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Horn, T.] Catholic Univ Amer, Washington, DC 20064 USA. [Aniol, K.; Margaziotis, D. J.] Calif State Univ Los Angeles, Los Angeles, CA 90032 USA. [Anklin, H.; Boeglin, W.; Markowitz, P.; Reinhold, J.] Florida Int Univ, Miami, FL 33119 USA. [Armstrong, C.; Jones, M. K.; Pentchev, L.; Perdrisat, C.] Coll William & Mary, Williamsburg, VA 23187 USA. [Arrington, J.; Holt, R. J.; Jackson, H.; Mueller, B.; Potterveld, D.; Reimer, P. E.; Zheng, X.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Assamagan, K.; Avery, S.; Baker, O. K.; Christy, M. E.; Hinton, W.; Keppel, C. E.; Tang, L. G.] Hampton Univ, Hampton, VA 23668 USA. [Barrett, B.; Sarty, A.] St Marys Univ, Halifax, NS B3H 3C3, Canada. [Beise, E. J.; Breuer, H.; Chang, C. C.; Chant, N.; Gustafsson, K.; King, P. M.; Liu, J.; Roos, P. G.] Univ Maryland, College Pk, MD 20742 USA. [Bochna, C.] Univ Illinois, Champaign, IL 61801 USA. [Eden, T.; Punjabi, V.] Norfolk State Univ, Norfolk, VA 23504 USA. [Gibson, E. F.] Calif State Univ Sacramento, Sacramento, CA 95819 USA. [Gilman, R.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Jin, S.; Kim, P. H.; Kim, W.; Shin, I. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Klein, A.; Qin, L. M.; Vansyoc, K.] Old Dominion Univ, Norfolk, VA 23529 USA. [Koltenuk, D.] Univ Penn, Philadelphia, PA 19104 USA. [Matsumura, A.; Miyoshi, T.; Okayasu, Y.] Tohoku Univ, Sendai, Miyagi 980, Japan. [McKee, D.] New Mexico State Univ, Las Cruces, NM 88003 USA. [Mkrtchyan, H.; Stepanyan, S.; Tadevosyan, V.] AI Alikhanyan Natl Sci Lab, Yerevan 0036, Armenia. [Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Pitz, D.] CEA Saclay, DAPNIA SPhN, F-91191 Gif Sur Yvette, France. [Van Westrum, D.] Univ Colorado, Boulder, CO 80309 USA. [Volmer, J.] DESY, Hamburg, Germany. [Zhao, W. -X.] MIT, Cambridge, MA 02139 USA. [Zihlmann, B.] Univ Virginia, Charlottesville, VA 22901 USA. RP Huber, GM (reprint author), Univ Regina, Regina, SK S4S 0A2, Canada. RI Arrington, John/D-1116-2012 OI Arrington, John/0000-0002-0702-1328 FU DOE and NSF (USA); NSERC (Canada); FOM (Netherlands); NATO; NRF (Rep. of Korea); Jefferson Science Associates; University of Regina; United States Department of Energy [DE-AC05-84150] FX The authors thank Dr. Goloskokov and Dr. Kroll for the unpublished model calculations at the kinematics of our experiment, and Dr. Guidal, Dr. Laget, and Dr. Vanderhaeghen for modifying their computer program for our needs. This work is supported by DOE and NSF (USA), NSERC (Canada), FOM (Netherlands), NATO, and NRF (Rep. of Korea). Additional support from Jefferson Science Associates and the University of Regina is gratefully acknowledged. At the time these data were taken, the Southeastern Universities Research Association (SURA) operated the Thomas Jefferson National Accelerator Facility for the United States Department of Energy under Contract No. DE-AC05-84150. NR 22 TC 2 Z9 2 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 5 PY 2014 VL 112 IS 18 AR 182501 DI 10.1103/PhysRevLett.112.182501 PG 6 WC Physics, Multidisciplinary SC Physics GA AH4LS UT WOS:000336099800006 PM 24856691 ER PT J AU Rosenberg, MJ Rinderknecht, HG Hoffman, NM Amendt, PA Atzeni, S Zylstra, AB Li, CK Seguin, FH Sio, H Johnson, MG Frenje, JA Petrasso, RD Glebov, VY Stoeckl, C Seka, W Marshall, FJ Delettrez, JA Sangster, TC Betti, R Goncharov, VN Meyerhofer, DD Skupsky, S Bellei, C Pino, J Wilks, SC Kagan, G Molvig, K Nikroo, A AF Rosenberg, M. J. Rinderknecht, H. G. Hoffman, N. M. Amendt, P. A. Atzeni, S. Zylstra, A. B. Li, C. K. Seguin, F. H. Sio, H. Johnson, M. Gatu Frenje, J. A. Petrasso, R. D. Glebov, V. Yu. Stoeckl, C. Seka, W. Marshall, F. J. Delettrez, J. A. Sangster, T. C. Betti, R. Goncharov, V. N. Meyerhofer, D. D. Skupsky, S. Bellei, C. Pino, J. Wilks, S. C. Kagan, G. Molvig, K. Nikroo, A. TI Exploration of the Transition from the Hydrodynamiclike to the Strongly Kinetic Regime in Shock-Driven Implosions SO PHYSICAL REVIEW LETTERS LA English DT Article ID INERTIAL-CONFINEMENT-FUSION; NATIONAL-IGNITION-FACILITY; LASER FUSION; PHYSICS BASIS; TARGETS; OMEGA; TRANSPORT; PLASMAS AB Clear evidence of the transition from hydrodynamiclike to strongly kinetic shock-driven implosions is, for the first time, revealed and quantitatively assessed. Implosions with a range of initial equimolar (DHe)-He-3 gas densities show that as the density is decreased, hydrodynamic simulations strongly diverge from and increasingly overpredict the observed nuclear yields, from a factor of similar to 2 at 3.1 mg/cm(3) to a factor of 100 at 0.14 mg/cm(3). (The corresponding Knudsen number, the ratio of ion mean-free path to minimum shell radius, varied from 0.3 to 9; similarly, the ratio of fusion burn duration to ion diffusion time, another figure of merit of kinetic effects, varied from 0.3 to 14.) This result is shown to be unrelated to the effects of hydrodynamic mix. As a first step to garner insight into this transition, a reduced ion kinetic (RIK) model that includes gradient-diffusion and loss-term approximations to several transport processes was implemented within the framework of a one-dimensional radiation-transport code. After empirical calibration, the RIK simulations reproduce the observed yield trends, largely as a result of ion diffusion and the depletion of the reacting tail ions. C1 [Rosenberg, M. J.; Rinderknecht, H. G.; Zylstra, A. B.; Li, C. K.; Seguin, F. H.; Sio, H.; Johnson, M. Gatu; Frenje, J. A.; Petrasso, R. D.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Hoffman, N. M.; Kagan, G.; Molvig, K.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Amendt, P. A.; Bellei, C.; Pino, J.; Wilks, S. C.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Atzeni, S.] Univ Roma La Sapienza, Dipartimento SBAI, I-00161 Rome, Italy. [Glebov, V. Yu.; Stoeckl, C.; Seka, W.; Marshall, F. J.; Delettrez, J. A.; Sangster, T. C.; Betti, R.; Goncharov, V. N.; Meyerhofer, D. D.; Skupsky, S.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Nikroo, A.] Gen Atom Co, San Diego, CA 92186 USA. RP Rosenberg, MJ (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM mrosenbe@mit.edu RI Atzeni, Stefano/F-5538-2012; OI Atzeni, Stefano/0000-0002-4339-2994; /0000-0003-4969-5571 FU US DOE [DE-NA0001857, DE-FC52-08NA28752]; FSC [5-24431]; NLUF [DE-NA0002035]; LLE [415935-G]; LLNL [B597367]; Italian Grants [PRIN 2009FCC9MS, Sapienza 2012 C26A12CZH2] FX The authors thank R. Frankel and E. Doeg for contributing to the processing of the CR-39 data used in this work as well as the OMEGA operations crew for their help in executing these experiments. This work is supported in part by US DOE ( Grants No. DE-NA0001857 and No. DE-FC52-08NA28752), FSC (No. 5-24431), NLUF (No. DE-NA0002035), LLE (No. 415935-G), and LLNL (No. B597367). S.A. is supported by Italian Grants No. PRIN 2009FCC9MS and No. Sapienza 2012 C26A12CZH2. NR 36 TC 22 Z9 22 U1 2 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 5 PY 2014 VL 112 IS 18 AR 185001 DI 10.1103/PhysRevLett.112.185001 PG 6 WC Physics, Multidisciplinary SC Physics GA AH4LS UT WOS:000336099800008 PM 24856701 ER PT J AU Zhou, YY Smith, SJ Elvidge, CD Zhao, KG Thomson, A Imhoff, M AF Zhou, Yuyu Smith, Steven J. Elvidge, Christopher D. Zhao, Kaiguang Thomson, Allison Imhoff, Marc TI A cluster-based method to map urban area from DMSP/OLS nightlights SO REMOTE SENSING OF ENVIRONMENT LA English DT Article DE DMSP/OLS; Nightlights; Urban area; Threshold; Cities; Segmentation; Land cover and land use change ID NIGHTTIME SATELLITE IMAGERY; REMOTELY-SENSED DATA; IMPERVIOUS SURFACES; CITY LIGHTS; LAND-USE; CHINA; URBANIZATION; SEGMENTATION; POPULATION; DATABASE AB Accurate information on urban areas at regional and global scales is important for both the science and policy-making communities. The Defense Meteorological Satellite Program/Operational Linescan System (DMSP/OLS) nighttime stable light data (NTL) provide a potential way to map the extent and dynamics of urban areas in an economic and timely manner. In this study, we developed a cluster-based method to estimate optimal thresholds and map urban extent from the DMSP/OLS Nil data in five major steps, including data preprocessing, urban cluster segmentation, logistic model development, threshold estimation, and urban extent delineation. In our method the optimal thresholds vary by clusters and are estimated based on cluster size and overall nightlight magnitude. The United States and China, two large countries with different urbanization patterns, were selected to test the proposed method. Our results indicate that the urbanized area occupies about 2% of total land area in the US, ranging from lower than 0.5% to higher than 10% at the state level, and less than 1% in China, ranging from lower than 0.1% to about 5% at the province level with some municipalities as high as 10%. The derived thresholds and urban extent were evaluated using a validation sub-sample of high-resolution land cover data at the cluster and regional levels. It was found that our method can map urban areas in both countries efficiently and accurately. The sensitivity analysis indicates that the derived optimal thresholds are not highly sensitive to the parameter choices in the logistic model. Our method reduces the over- and under-estimation issues often associated with previous fixed-threshold techniques when mapping urban extent over a large area. More importantly, our method shows potential to map global urban extent and temporal dynamics using the DMSP/OLS NTL data in a timely, cost-effective way. (C) 2014 Elsevier Inc. All rights reserved. C1 [Zhou, Yuyu; Smith, Steven J.; Thomson, Allison; Imhoff, Marc] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Elvidge, Christopher D.] NOAA, Natl Geophys Data Ctr, Earth Observat Grp, Boulder, CO 80303 USA. [Zhao, Kaiguang] Ohio State Univ, Sch Environm & Nat Resources, Wooster, OH 44691 USA. RP Zhou, YY (reprint author), Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. EM Yuyu.zhou@pnnl.gov RI Thomson, Allison/B-1254-2010; Zhao, Kaiguang/D-1172-2010; Elvidge, Christopher/C-3012-2009 FU NASA ROSES Land-Cover/Land-Use Change Program [NNH11ZDA001N-LCLUC]; Global Technology Strategy Project FX We acknowledge funding support from the NASA ROSES Land-Cover/Land-Use Change Program (NNH11ZDA001N-LCLUC) with additional support for Steven J. Smith from the Global Technology Strategy Project. We would like to thank Dr. Benjamin Bond-Lamberty and the anonymous reviewers for their constructive comments and suggestions, and the many colleagues and organizations that shared the data used in this project. NR 54 TC 39 Z9 43 U1 9 U2 77 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0034-4257 EI 1879-0704 J9 REMOTE SENS ENVIRON JI Remote Sens. Environ. PD MAY 5 PY 2014 VL 147 BP 173 EP 185 DI 10.1016/j.rse.2014.03.004 PG 13 WC Environmental Sciences; Remote Sensing; Imaging Science & Photographic Technology SC Environmental Sciences & Ecology; Remote Sensing; Imaging Science & Photographic Technology GA AH5QR UT WOS:000336186400015 ER PT J AU Intravaia, F Behunin, RO Dalvit, DAR AF Intravaia, F. Behunin, R. O. Dalvit, D. A. R. TI Quantum friction and fluctuation theorems SO PHYSICAL REVIEW A LA English DT Article ID IRREVERSIBLE-PROCESSES; DISSIPATION THEOREM; SYSTEMS; FORCE; APPROXIMATION; MOLECULES; SURFACE AB We use general concepts of statistical mechanics to compute the quantum frictional force on an atom moving at constant velocity above a planar surface. We derive the zero-temperature frictional force using a nonequilibrium fluctuation-dissipation relation, and we show that in the large-time, steady-state regime, quantum friction scales as the cubic power of the atom's velocity. We also discuss how approaches based on Wigner-Weisskopf and quantum regression approximations fail to predict the correct steady-state zero-temperature frictional force, mainly due to the low-frequency nature of quantum friction. C1 [Intravaia, F.; Behunin, R. O.; Dalvit, D. A. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Intravaia, F.] Max Born Inst, D-12489 Berlin, Germany. [Behunin, R. O.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Behunin, R. O.] Yale Univ, Dept Appl Phys, New Haven, CT 06511 USA. RP Intravaia, F (reprint author), Los Alamos Natl Lab, Div Theoret, MS B213, Los Alamos, NM 87545 USA. RI Intravaia, Francesco/E-6500-2010 OI Intravaia, Francesco/0000-0001-7993-4698 FU Alexander von Humboldt Foundation; LANL LDRD program FX We are grateful to G. Barton, S. Buhmann, L. Cugliandolo, J. P. Garrahan, C. Henkel, and S. Scheel for insightful discussions, and to the Alexander von Humboldt Foundation and the LANL LDRD program for financial support. NR 40 TC 25 Z9 25 U1 1 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAY 5 PY 2014 VL 89 IS 5 AR 050101 DI 10.1103/PhysRevA.89.050101 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AH4LY UT WOS:000336100500001 ER PT J AU Ticknor, C AF Ticknor, Christopher TI Dispersion relation and excitation character of a two-component Bose-Einstein condensate SO PHYSICAL REVIEW A LA English DT Article ID OPTICAL LATTICE; COLD ATOMS; SEPARATION; PHASE; GASES AB We present a study for the dispersion relation and character of the excitations of a single- and two-component Bose-Einstein condensate (BEC). We study the single- component dispersion for a finite BEC system and look at examples of quasiparticles to understand and characterize the dispersion relation. Next we present the dispersion relation for a two-component BEC in both the miscible and immiscible parameter regimes. Then we present examples of the quasiparticles for both regimes. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ticknor, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Ticknor, Christopher/B-8651-2014; OI Ticknor, Christopher/0000-0001-9972-4524 FU LDRD ECR; LANL; US Department of Energy [DE-AC52-06NA25396] FX The author is pleased to acknowledge excellent discussions and suggestions from R. N. Bisset and E. Chisolm. The author gratefully acknowledges support from LDRD ECR and LANL, which is operated by LANS, LLC for the NNSA of the US Department of Energy under Contract No. DE-AC52-06NA25396. NR 52 TC 9 Z9 9 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAY 5 PY 2014 VL 89 IS 5 AR 053601 DI 10.1103/PhysRevA.89.053601 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AH4LY UT WOS:000336100500004 ER PT J AU Wang, Z Kamenskyi, D Cepas, O Schmidt, M Quintero-Castro, DL Islam, ATMN Lake, B Aczel, AA Dabkowska, HA Dabkowski, AB Luke, GM Wan, Y Loidl, A Ozerov, M Wosnitza, J Zvyagin, SA Deisenhofer, J AF Wang, Zhe Kamenskyi, D. Cepas, O. Schmidt, M. Quintero-Castro, D. L. Islam, A. T. M. N. Lake, B. Aczel, A. A. Dabkowska, H. A. Dabkowski, A. B. Luke, G. M. Wan, Yuan Loidl, A. Ozerov, M. Wosnitza, J. Zvyagin, S. A. Deisenhofer, J. TI High-field electron spin resonance spectroscopy of singlet-triplet transitions in the spin-dimer systems Sr3Cr2O8 and Ba3Cr2O8 SO PHYSICAL REVIEW B LA English DT Article ID CRYSTAL; CUGEO3; GROWTH; WAVES; ESR AB Magnetic excitations in the isostructural spin-dimer systems Sr3Cr2O8 and Ba3Cr2O8 are probed by means of high-field electron spin resonance at subterahertz frequencies. Three types of magnetic modes were observed. One mode is gapless and corresponds to transitions within excited states, while two other sets of modes are gapped and correspond to transitions from the ground to the first excited states. The selection rules of the gapped modes are analyzed in terms of a dynamical Dzyaloshinskii-Moriya interaction, suggesting the presence of phonon-assisted effects in the low-temperature spin dynamics of Sr3Cr2O8 and Ba3Cr2O8. C1 [Wang, Zhe; Schmidt, M.; Loidl, A.; Deisenhofer, J.] Univ Augsburg, Inst Phys, Ctr Elect Correlat & Magnetism, D-86135 Augsburg, Germany. [Kamenskyi, D.; Ozerov, M.; Wosnitza, J.; Zvyagin, S. A.] Helmholtz Zentrum Dresden Rossendorf, Dresden High Magnet Field Lab HLD, D-01328 Dresden, Germany. [Cepas, O.] CNRS, Inst Neel, F-38042 Grenoble 9, France. [Cepas, O.] Univ Grenoble 1, F-38042 Grenoble 9, France. [Quintero-Castro, D. L.; Islam, A. T. M. N.; Lake, B.] Helmholtz Zentrum Berlin Mat & Energie, D-14109 Berlin, Germany. [Lake, B.] Tech Univ Berlin, Inst Festkorperphys, D-10623 Berlin, Germany. [Aczel, A. A.; Luke, G. M.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Aczel, A. A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Dabkowska, H. A.; Dabkowski, A. B.] McMaster Univ, Brockhouse Inst Mat Res, Hamilton, ON L8S 4M1, Canada. [Wan, Yuan] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Wosnitza, J.] Tech Univ Dresden, Inst Festkorperphys, D-01068 Dresden, Germany. RP Wang, Z (reprint author), Univ Augsburg, Inst Phys, Ctr Elect Correlat & Magnetism, D-86135 Augsburg, Germany. EM zhe.wang@physik.uni-augsburg.de RI Deisenhofer, Joachim/G-8937-2011; Zvyagin, Sergei/H-8389-2014; Kamenskyi, Dmytro/J-8530-2014; Luke, Graeme/A-9094-2010; Aczel, Adam/A-6247-2016; Loidl, Alois/L-8199-2015; OI Deisenhofer, Joachim/0000-0002-7645-9390; Aczel, Adam/0000-0003-1964-1943; Loidl, Alois/0000-0002-5579-0746; Lake, Bella/0000-0003-0034-0964 FU Deutsche Forschungsgemeinschaft [TRR 80, DE 1762/2-1, ZV 6/2-1] FX We thank V. Tsurkan for help with sample preparation. We acknowledge partial support by the Deutsche Forschungsgemeinschaft via TRR 80 (Augsburg-Munich), Projects No. DE 1762/2-1 and No. ZV 6/2-1, and also the support of the HLD at HZDR, member of the European Magnetic Field Laboratory. NR 37 TC 4 Z9 4 U1 0 U2 54 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 5 PY 2014 VL 89 IS 17 AR 174406 DI 10.1103/PhysRevB.89.174406 PG 6 WC Physics, Condensed Matter SC Physics GA AH4MA UT WOS:000336100800003 ER PT J AU Metzker, G Lopes, PP da Silva, ACH da Silva, SC Franco, DW AF Metzker, Gustavo Lopes, Pietro P. da Silva, Augusto C. H. da Silva, Sebastiao C. Franco, Douglas W. TI Unexpected NO Transfer Reaction between trans-[Ru-II(NO+)(NH3)(4)(L)](3+) and Fe(III) Species: Observation of a Heterobimetallic NO-Bridged Intermediate SO INORGANIC CHEMISTRY LA English DT Article ID EFFECTIVE CORE POTENTIALS; NITRIC-OXIDE NO; RUTHENIUM NITROSYL COMPLEXES; MOLECULAR CALCULATIONS; IRON(III) PORPHYRINS; BIOLOGICAL-ACTIVITY; AQUEOUS-SOLUTION; HEME-PROTEINS; LIGANDS; COORDINATION AB The reaction between trans-[Ru-II(NO+)(NH3)(4)(L)](3+), L = ImN, IsN, Nic, P(OMe)(3), P(OEt)(3), and P(OH)(OEt)(2), and the Fe(III) species [Fe-III(TPPS)], metmyoglobin, and hemoglobin was monitored by UV-vis, EPR, and electrochemical techniques (DPV, CV). No reaction was observed when L = ImN, IsN, Nic, and P(OH)(OEt)(2). However, when L = P(OMe)(3) and P(OEt)(3), the reaction was quantitative and the products were trans-[Ru-III(H2O)(NH3)(4)(P(OR)(3))](3+) and [Fe-II(NO+)] species. Reaction kinetics data and DFT calculations suggest a two-step reaction mechanism with the initial formation of a bridged [Ru-(mu NO)-Fe] intermediate, which was confirmed through electrochemical techniques (E-0' = -0.47 V vs NHE). The calculated specific rate constant values for the reaction were in the ranges k(1) =1.1 to 7.7 L mol(-1) s(-1) and k(2) = 2.4 x 10(-3) to 11.4 x 10(-3) s(-1) for L = P(OMe)(3) and P(OEt)(3). The oxidation of the ruthenium center (Ru(II) to Ru(III)) containing the nitrosonium ligand suggests that NO can act as an electron transfer bridge between the two metal centers. C1 [Metzker, Gustavo; Lopes, Pietro P.; da Silva, Augusto C. H.; Franco, Douglas W.] Univ Sao Paulo, Inst Quim Sao Carlos, Sao Carlos, SP, Brazil. [Lopes, Pietro P.] Argonne Natl Lab, Lemont, IL USA. [da Silva, Sebastiao C.] Univ Fed Mato Grosso, Cuiaba, MS, Brazil. RP Franco, DW (reprint author), Univ Sao Paulo, Inst Quim Sao Carlos, Ave Trab Sao Carlense 400, Sao Carlos, SP, Brazil. EM douglas@iqsc.usp.br RI Lopes, Pietro/E-2724-2013 OI Lopes, Pietro/0000-0003-3211-470X FU FAPESP; CNPq [2012/2365-4, 475631/2011-0] FX The authors acknowledge FAPESP and CNPq (grant numbers 2012/2365-4 and 475631/2011-0, respectively) for the financial support. The authors are also indebted to A.B.P. Lever (York University), Bruce R. King (University of Georgia), and Edward I. Solomon (Stanford University) for helpful discussions during the preparation of the manuscript. NR 50 TC 4 Z9 4 U1 1 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 5 PY 2014 VL 53 IS 9 BP 4475 EP 4481 DI 10.1021/ic500122b PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AG6RZ UT WOS:000335547400026 PM 24738470 ER PT J AU Ponou, S Lidin, S Zhang, YM Miller, GJ AF Ponou, Simeon Lidin, Sven Zhang, Yuemei Miller, Gordon J. TI Valence State Driven Site Preference in the Quaternary Compound Ca5MgAgGe5: An Electron-Deficient Phase with Optimized Bonding SO INORGANIC CHEMISTRY LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CRYSTAL-STRUCTURES; COLORING PROBLEM; ZINTL PHASES; BASIS-SET; INTERGROWTH; METALS; CHEMISTRY; BA7GA4SB9 AB The quaternary phase Ca5Mg0.95Ag1.05(1)Ge5 (3) was synthesized by high-temperature solid-state techniques, and its crystal structure was determined by single-crystal diffraction methods in the orthorhombic space group Pnma - Wyckoff sequence c(12) with a = 23.1481(4) angstrom, b = 4.4736(1) angstrom, c = 11.0128(2) angstrom, V = 1140.43(4) angstrom(3), Z = 4. The crystal structure can be described as linear intergrowths of slabs cut from the CaGe (CrB-type) and the CaMGe (TiNiSi-type; M = Mg, Ag) structures. Hence, 3 is a hettotype of the hitherto missing n = 3 member of the structure series with the general formula R2+nT2X2+n, previously described with n = 1, 2, and 4. The member with n = 3 was predicted in the space group Cmcm - Wyckoff sequence f(s)c(2). The experimental space group Pnma (in the nonstandard setting Pmcn) corresponds to a klassengleiche symmetry reduction of index two of the predicted space group Cmcm. This transition originates from the switching of one Ge and one Ag position in the TiNiSi-related slab, a process that triggers an uncoupling of each of the five 8f sites in Cmcm into two 4c sites in Pnma. The Mg/Ag site preference was investigated using VASP calculations and revealed a remarkable example of an intermetallic compound for which the electrostatic valency principle is a critical structure-directing force. The compound is deficient by one valence electron according to the Zintl concept, but LMTO electronic structure calculations indicate electronic stabilization and overall bonding optimization in the polyanionic network. Other stability factors beyond the Zintl concept that may account for the electronic stabilization are discussed. C1 [Ponou, Simeon; Lidin, Sven] Lund Univ, Dept Chem, Ctr Anal & Synth, SE-22100 Lund, Sweden. [Zhang, Yuemei; Miller, Gordon J.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Zhang, Yuemei; Miller, Gordon J.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Ponou, S (reprint author), Lund Univ, Dept Chem, Ctr Anal & Synth, Getingevagen 60,Box 124, SE-22100 Lund, Sweden. EM simeon.ponou@chem.lu.se; gmiller@iastate.edu RI Zhang, Yuemei/H-7370-2012; OI Lidin, Sven/0000-0001-9057-8233 FU Swedish National Science Council (VR); National Science Foundation [NSF DMR 10-05765, 12-09135] FX This work was financially supported by the Swedish National Science Council (VR). The authors also thank the National Science Foundation (NSF DMR 10-05765 and 12-09135) for generous financial support. NR 52 TC 6 Z9 6 U1 2 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 5 PY 2014 VL 53 IS 9 BP 4724 EP 4732 DI 10.1021/ic500449d PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AG6RZ UT WOS:000335547400053 PM 24745932 ER PT J AU Burdet, N Morrison, GR Huang, XJ Shi, XW Clark, JN Zhang, FC Civita, M Harder, R Robinson, IK AF Burdet, Nicolas Morrison, Graeme R. Huang, Xiaojing Shi, Xiaowen Clark, Jesse N. Zhang, Fucai Civita, Maria Harder, Ross Robinson, Ian K. TI Observations of artefacts in the x-ray ptychography method SO OPTICS EXPRESS LA English DT Article ID PHASE RETRIEVAL; ILLUMINATION AB X-ray ptychography, a scanning coherent diffraction imaging method, was used to reconstruct images of a "Siemens star" test pattern with amplitude and phase contrast. While studying how the use of illumination with an increased bandwidth results in clear improvements in the quality of image reconstructions, we found that an artificial change in the overall distance scale factor of the algorithm leads to a systematic response in the image, which is reproduced with an incorrect number of spokes. This pathology is explained by the conflict between the length scales set by the scan and by the diffraction patterns on the detector. (C) 2014 Optical Society of America C1 [Burdet, Nicolas; Morrison, Graeme R.; Clark, Jesse N.; Zhang, Fucai; Civita, Maria; Robinson, Ian K.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Burdet, Nicolas; Morrison, Graeme R.; Clark, Jesse N.; Zhang, Fucai; Civita, Maria; Robinson, Ian K.] Res Complex Harwell, Oxford OX11 0QF, England. [Huang, Xiaojing] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Shi, Xiaowen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Burdet, N (reprint author), UCL, London Ctr Nanotechnol, London WC1H 0AH, England. EM nicolas.burdet.10@ucl.ac.uk RI Huang, Xiaojing/K-3075-2012 OI Huang, Xiaojing/0000-0001-6034-5893 FU U.S. DOE [DE-AC02-06CH11357]; National Science Foundation [DMR-9724294]; UK Engineering and Physical Sciences Research Council (EPSRC) [EP/G068437/1, EP/I022562/1] FX Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Beamline 34-ID-C was built with a grant from the National Science Foundation DMR-9724294. This research was carried out under grants EP/G068437/1 and EP/I022562/1 from the UK Engineering and Physical Sciences Research Council (EPSRC). NR 21 TC 4 Z9 4 U1 1 U2 12 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 5 PY 2014 VL 22 IS 9 BP 10294 EP 10303 DI 10.1364/OE.22.010294 PG 10 WC Optics SC Optics GA AH1TZ UT WOS:000335905300060 PM 24921732 ER PT J AU Boyson, TK Rittman, DR Spence, TG Calzada, ME Kallapur, AG Petersen, IR Kirkbride, KP Moore, DS Harb, CC AF Boyson, Toby K. Rittman, Dylan R. Spence, Thomas G. Calzada, Maria E. Kallapur, Abhijit G. Petersen, Ian R. Kirkbride, K. Paul Moore, David S. Harb, Charles C. TI Pulsed quantum cascade laser based hypertemporal real-time headspace measurements SO OPTICS EXPRESS LA English DT Article ID CAVITY RINGDOWN SPECTROSCOPY; EXPLOSIVE-RELATED-COMPOUNDS; MOLECULAR-DETECTION; COMPOUND; TNT AB Optical cavity enhancement is a highly desirable process to make sensitive direct-absorption spectroscopic measurements of unknown substances, such as explosives, illicit material, or other species of interest. This paper reports advancements in the development of real-time cavity ringdown spectroscopy over a wide-bandwidth, with the aim to make headspace measurements of molecules at trace levels. We report results of two pulsed quantum cascade systems operating between (1200 to 1320) cm(-1) and (1316 to 1613) cm(-1) that measure the headspace of nitromethane, acetonitrile, acetone, and nitroglycerin, where the spectra are obtained in less than four seconds and contain at least 150,000 spectral wavelength datapoints. (C) 2014 Optical Society of America C1 [Boyson, Toby K.; Kallapur, Abhijit G.; Petersen, Ian R.; Harb, Charles C.] UNSW Australia, Sch Engn & Informat Technol, Canberra, ACT 2600, Australia. [Rittman, Dylan R.; Moore, David S.] Los Alamos Natl Lab, Shock & Detonat Phys Grp, Los Alamos, NM 87545 USA. [Spence, Thomas G.; Calzada, Maria E.] Loyola Univ, Dept Chem, New Orleans, LA 70118 USA. [Kirkbride, K. Paul] Flinders Univ S Australia, Sch Chem & Phys Sci, Adelaide, SA 5001, Australia. RP Harb, CC (reprint author), UNSW Australia, Sch Engn & Informat Technol, Canberra, ACT 2600, Australia. EM c.harb@adfa.edu.au OI Kirkbride, Kenneth/0000-0001-7666-4039 FU Australian Research Council; Australian Federal Police; ANU Connect Ventures FX We would like to thank Prof. Chris Lennard, University of Canberra, Chris Armacost and Sam Crevillo, Daylight Solutions, and Will Lohnstar, LohnStar Optics Inc., for their help during this work. This work was supported in part by the Australian Research Council, the Australian Federal Police, and ANU Connect Ventures. NR 22 TC 4 Z9 4 U1 0 U2 21 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 5 PY 2014 VL 22 IS 9 BP 10519 EP 10534 DI 10.1364/OE.22.010519 PG 16 WC Optics SC Optics GA AH1TZ UT WOS:000335905300082 PM 24921754 ER PT J AU Kim, J Li, TC Wang, Y Zhang, X AF Kim, Jeongmin Li, Tongcang Wang, Yuan Zhang, Xiang TI Vectorial point spread function and optical transfer function in oblique plane imaging SO OPTICS EXPRESS LA English DT Article ID CONVERGING ELECTROMAGNETIC-WAVES; HIGH-APERTURE SYSTEMS; INTEGRAL-REPRESENTATION; PUPIL FUNCTIONS; MICROSCOPY; FIELD; DIFFRACTION; ABERRATION; SHIFTS AB Oblique plane imaging, using remote focusing with a tilted mirror, enables direct two-dimensional (2D) imaging of any inclined plane of interest in three-dimensional (3D) specimens. It can image real-time dynamics of a living sample that changes rapidly or evolves its structure along arbitrary orientations. It also allows direct observations of any tilted target plane in an object of which orientational information is inaccessible during sample preparation. In this work, we study the optical resolution of this innovative wide-field imaging method. Using the vectorial diffraction theory, we formulate the vectorial point spread function (PSF) of direct oblique plane imaging. The anisotropic lateral resolving power caused by light clipping from the tilted mirror is theoretically analyzed for all oblique angles. We show that the 2D PSF in oblique plane imaging is conceptually different from the inclined 2D slice of the 3D PSF in conventional lateral imaging. Vectorial optical transfer function (OTF) of oblique plane imaging is also calculated by the fast Fourier transform (FFT) method to study effects of oblique angles on frequency responses. (C) 2014 Optical Society of America C1 [Kim, Jeongmin; Zhang, Xiang] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Li, Tongcang; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Kim, Jeongmin; Li, Tongcang; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Wang, Yuan/F-7211-2011; Zhang, Xiang/F-6905-2011 FU Gordon and Betty Moore Foundation FX This work was supported by the Gordon and Betty Moore Foundation. NR 25 TC 5 Z9 5 U1 3 U2 13 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 5 PY 2014 VL 22 IS 9 BP 11140 EP 11151 DI 10.1364/OE.22.011140 PG 12 WC Optics SC Optics GA AH1TZ UT WOS:000335905300140 PM 24921812 ER PT J AU Cox, JA Lentine, AL Trotter, DC Starbuck, AL AF Cox, Jonathan A. Lentine, Anthony L. Trotter, Douglas C. Starbuck, Andrew L. TI Control of integrated micro-resonator wavelength via balanced homodyne locking SO OPTICS EXPRESS LA English DT Article ID SILICON CHIP; MODULATORS; SWITCH AB We describe and experimentally demonstrate a method for active control of resonant modulators and filters in an integrated photonics platform. Variations in resonance frequency due to manufacturing processes and thermal fluctuations are corrected by way of balanced homodyne locking. The method is compact, insensitive to intensity fluctuations, minimally disturbs the micro-resonator, and does not require an arbitrary reference to lock. We demonstrate long-term stable locking of an integrated filter to a laser swept over 1.25 THz. In addition, we show locking of a modulator with low bit error rate while the chip temperature is varied from 5 to 60 degrees C. (C) 2014 Optical Society of America C1 [Cox, Jonathan A.; Lentine, Anthony L.; Trotter, Douglas C.; Starbuck, Andrew L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Cox, JA (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM joncox@alum.mit.edu FU Sandia's Laboratory Directed Research and Development (LDRD) program; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors wish to acknowledge helpful discussions with W. A. Zortman and C. T. DeRose regarding the design of sub-components used in this photonic circuit. Funding for this work was provided by Sandia's Laboratory Directed Research and Development (LDRD) program. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. SAND #: 2014-0787 J NR 26 TC 26 Z9 26 U1 2 U2 12 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 5 PY 2014 VL 22 IS 9 BP 11279 EP 11289 DI 10.1364/OE.22.011279 PG 11 WC Optics SC Optics GA AH1TZ UT WOS:000335905300153 PM 24921825 ER PT J AU AlZayed, NS Kityk, IV Soltan, S Wojciechowski, A Fedorchuk, AO Lakshminarayana, G Shahabuddin, M AF AlZayed, N. S. Kityk, I. V. Soltan, S. Wojciechowski, A. Fedorchuk, A. O. Lakshminarayana, G. Shahabuddin, M. TI Laser stimulated kinetics effects on the phase transition of the ferromagnetic/superconducting MgB2/(CrO2) bilayer thin films SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Optical materials; Thin films; Photoinduced properties ID 2ND-HARMONIC GENERATION; SUPERCONDUCTING FILMS; MAGNESIUM DIBORIDE; ELECTROOPTICS AB Using bicolor laser treatment by Nd:YAG 20 ns laser (1064-532 nm) and 180 ns CO2 laser beams (10.6-5.3 mu m) it was shown a possibility of critical temperature enhancement in ferromagnetic superconducting MgB2/CrO2 bilayer films. The role of the phonon sub-system effectively interacting with 3d Cr originating localized trapping levels is discussed. The pump-probe laser kinetics for the probing second harmonic generation at 1064 nm is explored in details to show principal role of the localized trapping levels. The relaxation of the processes after the switching off the photo inducing beams show the disappearance of the enhanced superconductivity after the 20-30 s. The temperature dependence of the resistance show nonlinear dependence versus the pumping power and different optimal fundamental to writing power density beams ratio. (C) 2014 Elsevier B.V. All rights reserved. C1 [AlZayed, N. S.; Shahabuddin, M.] King Saud Univ, Coll Sci, Dept Phys & Astron, Riyadh 11451, Saudi Arabia. [Kityk, I. V.; Wojciechowski, A.] Czestochowa Tech Univ, Fac Elect Engn, PL-42201 Czestochowa, Poland. [Soltan, S.] Max Planck Inst, D-70569 Stuttgart, Germany. [Soltan, S.] Helwan Univ, Fac Sci, Dept Phys, Cairo 11798, Egypt. [Fedorchuk, A. O.] Lviv Natl Univ Vet Med & Biotechnol, Dept Inorgan & Organ Chem, UA-79010 Lvov, Ukraine. [Lakshminarayana, G.] Los Alamos Natl Lab, Mat Sci & Technol Div MST 7, Los Alamos, NM 87545 USA. RP Kityk, IV (reprint author), Czestochowa Tech Univ, Fac Elect Engn, Armii Krajowej 17, PL-42201 Czestochowa, Poland. EM ikityk@el.pcz.czest.pl RI Soltan, Soltan/K-3400-2013; Soltan, Soltan/F-3300-2014; Kityk, Iwan/M-4032-2015 OI Soltan, Soltan/0000-0003-0440-4726; FU King Abdulaziz City for Science & Technology, Saudi Arabia under National Plan for Science and Technology Project [10-NAN1171-02] FX This work has been funded by King Abdulaziz City for Science & Technology, Saudi Arabia under National Plan for Science and Technology Project No. (10-NAN1171-02). NR 26 TC 5 Z9 5 U1 0 U2 43 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD MAY 5 PY 2014 VL 594 BP 60 EP 64 DI 10.1016/j.jallcom.2014.01.035 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AB3XI UT WOS:000331723100011 ER PT J AU Lazpita, P Barandiaran, JM Chernenko, VA Garcia, BV Tajada, ED Lograsso, T Schlagel, DL AF Lazpita, P. Barandiaran, J. M. Chernenko, V. A. Valle Garcia, B. Diaz Tajada, E. Lograsso, T. Schlagel, D. L. TI Magnetic properties of Ni40+xMn39-xSn21 (x=0, 2, 4, 6 and 8 at.%) Heusler alloys SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Ni-Mn-Sn; Metamagnetic shape memory alloys; Electron concentration; Magnetic moment ID SHAPE-MEMORY ALLOYS; MARTENSITIC-TRANSFORMATION; FIELD; CRYSTALS; NI2MNGA; PHASE; ORDER AB The low electron concentration region (e/a < 7.75) of the magnetic phase diagram of the off-stoichiometric Ni-Mn-Sn Heusler alloys was investigated in detail by DSC and magnetization measurements of the Ni40+xMn39-xSn21(x = 0, 2, 4, 6 and 8 at.%) alloys. The alloys show a stable austenitic phase without any martensitic transformation down to 5 K even after heat treatment. The Curie temperature exhibits a broad maximum over a large composition range. The evolution of the magnetic moment with the electron concentration fits the data of previous studies and confirms the peak-like dependence in the extended range of e/a values predicted by ab initio calculations. The explored part of the moment versus e/a curve can be explained in terms of a localized magnetic moment model and full atomic order in the alloys. (C) 2014 Elsevier B.V. All rights reserved. C1 [Lazpita, P.; Barandiaran, J. M.; Chernenko, V. A.] BCMaterials, Bilbao, Spain. [Lazpita, P.; Barandiaran, J. M.; Chernenko, V. A.] Univ Basque Country, Leioa 48940, Spain. [Chernenko, V. A.] Basque Fdn Sci, Ikerbasque, Bilbao, Spain. [Valle Garcia, B.] Univ Basque Country, EUITI Bilbao, Dpto Ing Min Met & Ciencia Mat, Bilbao 48940, Spain. [Diaz Tajada, E.] Univ Basque Country, ETS Naut & Maquinas Navales, Dpto Ing Min Met & Ciencia Mat, Portugalete, Spain. [Lograsso, T.; Schlagel, D. L.] Ames Lab, Div Mat Sci & Engn, Ames, IA USA. [Lograsso, T.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA USA. RP Lazpita, P (reprint author), Univ Basque Country, Dept Elect & Elect, B Sarriena S-N, Leioa 48940, Spain. EM patricia.lazpita@ehu.es RI Lazpita, Patricia/K-9887-2014; chernenko, volodymyr/K-8211-2014; Diaz, Esperanza/D-8380-2016; OI Lazpita, Patricia/0000-0002-8898-7713; chernenko, volodymyr/0000-0002-0933-9372; Diaz, Esperanza/0000-0001-6483-6593; Barandiaran Garcia, Jose Manuel/0000-0002-5402-9314 FU Spanish Ministry of Science and Innovation [MAT2011-28217-C02-02]; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division; U.S. Department of Energy [DE-AC02-07CH11358] FX This work has been carried out with the financial support of the Project No. MAT2011-28217-C02-02, by the Spanish Ministry of Science and Innovation. Technical and human support provided by SGIker is gratefully acknowledged. DLS and TAL acknowledge support by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 24 TC 0 Z9 0 U1 0 U2 63 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD MAY 5 PY 2014 VL 594 BP 171 EP 174 DI 10.1016/j.jallcom.2014.01.142 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AB3XI UT WOS:000331723100029 ER PT J AU de Prado, ML Foreman, MD AF de Prado, Marcos Lopez Foreman, Matthew D. TI A mixture of Gaussians approach to mathematical portfolio oversight: the EF3M algorithm SO QUANTITATIVE FINANCE LA English DT Article DE Skewness; Kurtosis; Mixture of Gaussians; Moment matching; Maximum likelihood; EM algorithm; C13; C15; C16; C44 ID EM ALGORITHM; DISTRIBUTIONS AB An analogue can be made between: (a) the slow pace at which species adapt to an environment, which often results in the emergence of a new distinct species out of a once homogeneous genetic pool and (b) the slow changes that take place over time within a fund, mutating its investment style. A fund's track record provides a sort of genetic marker, which we can use to identify mutations. This has motivated our use of a biometric procedure to detect the emergence of a new investment style within a fund's track record. In doing so, we answer the question: What is the probability that a particular PM's performance is departing from the reference distribution used to allocate her capital? The EF3M algorithm, inspired by evolutionary biology, may help detect early stages of an evolutionary divergence in an investment style and trigger a decision to review a fund's capital allocation. C1 [de Prado, Marcos Lopez] Hess Energy Trading Co, Quantitat Trading, New York, NY 10036 USA. [de Prado, Marcos Lopez] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Foreman, Matthew D.] Univ Calif Irvine, Irvine, CA USA. RP de Prado, ML (reprint author), Hess Energy Trading Co, Quantitat Trading, New York, NY 10036 USA. EM lopezdeprado@lbl.gov NR 27 TC 0 Z9 0 U1 1 U2 1 PU ROUTLEDGE JOURNALS, TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXFORDSHIRE, ENGLAND SN 1469-7688 EI 1469-7696 J9 QUANT FINANC JI Quant. Financ. PD MAY 4 PY 2014 VL 14 IS 5 BP 913 EP 930 DI 10.1080/14697688.2013.861075 PG 18 WC Business, Finance; Economics; Mathematics, Interdisciplinary Applications; Social Sciences, Mathematical Methods SC Business & Economics; Mathematics; Mathematical Methods In Social Sciences GA AE9NO UT WOS:000334334700012 ER PT J AU Elhadj, S Matthews, MJ Yang, ST AF Elhadj, Selim Matthews, Manyalibo J. Yang, Steven T. TI Combined Infrared Thermal Imaging and Laser Heating for the Study of Materials Thermophysical and Processing Properties at High Temperatures SO CRITICAL REVIEWS IN SOLID STATE AND MATERIALS SCIENCES LA English DT Review DE laser; infrared; pyrometry; thermophysical; thermography; thermal; rheology; model; temperature; heating; imaging ID CHEMICAL-VAPOR-DEPOSITION; FUSED-SILICA; STRUCTURAL RELAXATION; BLACKBODY RADIATION; ABLATION PARAMETERS; FEMTOSECOND LASER; REFRACTIVE-INDEX; ROOM-TEMPERATURE; GAS-PHASE; ICP-MS AB Focused laser irradiation can easily drive materials to extreme temperatures with very high precision and control. In combination with infrared imaging and material characterization techniques, the resulting thermal load can be assessed to derive meaningful thermophysical properties avoiding interferences that would normally occur with direct contact measurements of temperature. In this focused article we first address technical challenges with the experimental implementation involved in obtaining laser-induced temperature field data from infrared imaging. We then discuss suitable heat transport models for analysis of thermal data and, finally, describe specific examples of thermophysical material parameters derived from combined infrared imaging and laser heating. The aim is to illustrate general principles of this combined laser-based heating and IR thermal imaging approach that are useful for experimentation under extreme conditions, which often remain out of reach of conventional methods. C1 [Elhadj, Selim; Matthews, Manyalibo J.; Yang, Steven T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Elhadj, S (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM Elhadj2@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors would like to thank the following for contributing to the studies reviewed here: Dr. Nan Shen, Dr. Ted Laurence, Dr. Rajesh Raman, Dr. Isaac Bass, Gabe Guss, Dr. Michael Feit, and Dr. Jeff Bude for useful discussions on silica IR emissivity measurements. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 119 TC 5 Z9 5 U1 4 U2 45 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1040-8436 EI 1547-6561 J9 CRIT REV SOLID STATE JI Crit. Rev. Solid State Mat. Sci. PD MAY 4 PY 2014 VL 39 IS 3 BP 175 EP 196 DI 10.1080/10408436.2013.789962 PG 22 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA AE5XH UT WOS:000334062100001 ER PT J AU Yin, HF Chen, CJ Yang, J Weston, DJ Chen, JG Muchero, W Ye, N Tschaplinski, TJ Wullschleger, SD Cheng, ZM Tuskan, GA Yang, XH AF Yin, Hengfu Chen, Chun Ju Yang, Jun Weston, David J. Chen, Jin-Gui Muchero, Wellington Ye, Ning Tschaplinski, Timothy J. Wullschleger, Stan D. Cheng, Zong-Ming (Max) Tuskan, Gerald A. Yang, Xiaohan TI Functional Genomics of Drought Tolerance in Bioenergy Crops SO CRITICAL REVIEWS IN PLANT SCIENCES LA English DT Review DE bioenergy crops; proteomics; Populus; transcriptome; genomics; drought; Panicum; epigenetics ID E3 UBIQUITIN LIGASE; TRANSGENIC ARABIDOPSIS PLANTS; TRANSCRIPTION FACTOR GENE; STRESS-RESPONSIVE MICRORNAS; ALFALFA MEDICAGO-SATIVA; CHELATASE H-SUBUNIT; RICE ORYZA-SATIVA; JATROPHA-CURCAS L; MAIZE ZEA-MAYS; ABSCISIC-ACID AB With predicted global changes in temperature and precipitation, drought will increasingly impose a challenge to biomass production. Most of the bioenergy crops have some degree of drought susceptibility as revealed for example through measures of low water-use efficiency (WUE). It is imperative to improve drought tolerance and WUE in bioenergy crops for sustainable biomass production in arid and semi-arid regions. Genetics and functional genomics can play critical roles in generating knowledge to inform and aid genetic improvement for drought tolerance in bioenergy crops. The molecular aspects of drought response have been extensively investigated in model plants like Arabidopsis, yet our understanding of the molecular mechanisms underlying drought tolerance in bioenergy crops is limited. Plants in general exhibit various responses to drought stress depending on species and genotype. A rational strategy for studying drought tolerance in bioenergy crops is to translate the knowledge from model plants relative to the unique features associated with individual bioenergy species and genotypes. In this review, we summarize the general knowledge concerning drought responsive pathways, with a focus on the identification of commonality and specialty in drought responsive mechanisms among alternate species and genotypes. We describe the genomic resources developed for bioenergy crops and discuss genetic and epigenetic regulation of drought responses. We also examine comparative and evolutionary genomics as a means to leverage the ever-increasing genomics resources and provide new insights beyond what is known from studies on individual species. Finally, we outline future opportunities for studying drought tolerance using the emerging technologies. C1 [Yin, Hengfu; Chen, Chun Ju; Yang, Jun; Weston, David J.; Chen, Jin-Gui; Muchero, Wellington; Ye, Ning; Tschaplinski, Timothy J.; Tuskan, Gerald A.; Yang, Xiaohan] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Weston, David J.; Chen, Jin-Gui; Muchero, Wellington; Tschaplinski, Timothy J.; Tuskan, Gerald A.; Yang, Xiaohan] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Wullschleger, Stan D.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Cheng, Zong-Ming (Max)] Univ Tennessee, Dept Plant Sci, Knoxville, TN 37996 USA. RP Yang, XH (reprint author), Oak Ridge Natl Lab, Biosci Div, POB 2008 MS-6422, Oak Ridge, TN 37831 USA. EM yangx@ornl.gov RI Chen, Jin-Gui/A-4773-2011; Ye, Ning/O-3246-2015; Wullschleger, Stan/B-8297-2012; Tuskan, Gerald/A-6225-2011; Yin, Hengfu/H-1695-2012; Yang, Xiaohan/A-6975-2011; OI Chen, Jin-Gui/0000-0002-1752-4201; Cheng, Zong-Ming/0000-0002-1811-591X; Ye, Ning/0000-0001-7249-8352; Wullschleger, Stan/0000-0002-9869-0446; Tuskan, Gerald/0000-0003-0106-1289; Yin, Hengfu/0000-0002-0720-5311; Yang, Xiaohan/0000-0001-5207-4210; Tschaplinski, Timothy/0000-0002-9540-6622 FU Department of Energy, Office of Science, Genomic Science Program [DE-SC0008834]; U.S. DOE BioEnergy Science Center; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Office of Biological and Environmental Research in the DOE Office of Science; U.S. Department of Energy [DE-AC05-00OR22725] FX This material is based in part upon work supported by the Department of Energy, Office of Science, Genomic Science Program under Award Number DE-SC0008834, the U.S. DOE BioEnergy Science Center and the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory. The BioEnergy Science Center is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. The Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract Number DE-AC05-00OR22725. NR 276 TC 6 Z9 6 U1 4 U2 143 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 520 CHESTNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0735-2689 EI 1549-7836 J9 CRIT REV PLANT SCI JI Crit. Rev. Plant Sci. PD MAY 4 PY 2014 VL 33 IS 2-3 SI SI BP 205 EP 224 DI 10.1080/07352689.2014.870417 PG 20 WC Plant Sciences SC Plant Sciences GA AE4DJ UT WOS:000333930500007 ER PT J AU Hubbard, JA Salazar, KC Crown, KK Servantes, BL AF Hubbard, Joshua A. Salazar, Keiko C. Crown, Kevin K. Servantes, Brandon L. TI High-Volume Aerosol Filtration and Mitigation of Inertial Particle Rebound SO AEROSOL SCIENCE AND TECHNOLOGY LA English DT Article ID SMALL LATEX SPHERES; REYNOLDS-NUMBERS; FIBROUS FILTERS; BOUNCE; CAPTURE; FLOW; COLLECTION; EFFICIENCY; VELOCITY; DENSITY AB The performance of electrostatically charged blown microfiber filter media was characterized for high-volume sampling applications. Pressure drop and aerosol collection efficiency were measured at air pressures of 55.2 and 88.7 kilopascals (kPa) and filter face velocities ranging from 2.5 to 11.25 meters per second (m/s). Particle penetration was significant for particles above 0.5 micrometers (mu m) in aerodynamic diameter where the onset of particle rebound was observed as low as 200 nanometers (nm). Particle retention was enhanced by treating filters in an aqueous solution of glycerol. Adding this retention agent eliminated electrostatic capture mechanisms but mitigated inertial rebound. Untreated filters had higher nanoparticle collection efficiencies at lower filter face velocities where electrostatic capture was still significant. At higher filter face velocities, nanoparticle collection efficiencies were higher for treated filters where inertial capture was dominant and particle rebound was mitigated. Significant improvements to microparticle collection efficiency were observed for treated filters at all air flow conditions. At high air pressure, filter efficiency was greater than 95% for particles less than 5 mu m. At low air pressure, performance enhancements were not as significant since air velocities were significantly higher through the fiber mat. Measured single fiber efficiencies were normalized by the theoretical single fiber efficiency to calculate adhesion probability. The small fiber diameter (1.77 mu m) of this particular filter gave large Stokes numbers and interception parameters forcing the single fiber efficiency to its maximum theoretical value. The adhesion probability was plotted as a function of the ratio of Stokes and interception parameter similar to the works of others. Single fiber efficiencies for inertial nanoparticle collection were compared to existing theories and correlations. Copyright 2014 American Association for Aerosol Research C1 [Hubbard, Joshua A.; Salazar, Keiko C.; Crown, Kevin K.; Servantes, Brandon L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Hubbard, JA (reprint author), Sandia Natl Labs, POB 5800 MS 1148, Albuquerque, NM 87185 USA. EM jahubba@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 27 TC 1 Z9 1 U1 4 U2 14 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0278-6826 EI 1521-7388 J9 AEROSOL SCI TECH JI Aerosol Sci. Technol. PD MAY 4 PY 2014 VL 48 IS 5 BP 530 EP 540 DI 10.1080/02786826.2014.897681 PG 11 WC Engineering, Chemical; Engineering, Mechanical; Environmental Sciences; Meteorology & Atmospheric Sciences SC Engineering; Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA AE3MO UT WOS:000333880800008 ER PT J AU Damit, B Wu, CY Cheng, MD AF Damit, Brian Wu, Chang-Yu Cheng, Meng-Dawn TI On the Validity of the Poisson Assumption in Sampling Nanometer-Sized Aerosols SO AEROSOL SCIENCE AND TECHNOLOGY LA English DT Article ID SPATIAL-DISTRIBUTION; PARTICLES; NANOPARTICLES; ENVIRONMENT; CLOUDS AB For a constant aerosol concentration, it is traditionally assumed that a Poisson process describes the behavior of particle detections during sampling and consequently fluctuations in the measured concentration. Recent studies, however, have shown that sampling of micrometer-sized aerosols has non-Poissonian behavior with positive correlations. The validity of the Poisson assumption for nanometer-sized aerosols has not been established and thus was tested in this study. Its validity was tested for four particle sizes-10nm, 25nm, 50nm, and 100nm-by sampling from indoor air with a differential mobility analyzer-condensation particle counter (DMA-CPC) setup to obtain a time series of particle counts. Five metrics were calculated from the data: pair-correlation function (PCF), scaled clustering index (SCI), coefficient of variation, probability of measuring a concentration at least 25% greater than average, and posterior distributions from Bayesian inference. To identify departures from Poissonian behavior, these metrics were also calculated for 1000 computer-generated Poisson time series with the same mean as the experimental data. For most comparisons, the experimental data fell within the range of 80% of the Poisson-simulation values. Essentially, the metrics for the experimental data were mostly indistinguishable from a simulated Poisson process. The greater influence of Brownian motion for nanometer-sized aerosols may explain the Poissonian behavior observed for smaller aerosols. Although the Poisson assumption was found to be reasonable in this study it must be carefully applied, as the results here do not definitively prove applicability in all sampling situations. Copyright 2014 American Association for Aerosol Research C1 [Damit, Brian; Wu, Chang-Yu] Univ Florida, Dept Environm Engn Sci, Gainesville, FL 32611 USA. [Cheng, Meng-Dawn] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Damit, B (reprint author), Univ Florida, Dept Environm Engn Sci, 405 Black Hall, Gainesville, FL 32611 USA. EM bdamit@ufl.edu RI Cheng, Meng-Dawn/C-1098-2012; OI Cheng, Meng-Dawn/0000-0003-1407-9576 FU National Science Foundation Graduate Research Fellowship (NSF GRF) [DGE-0802270]; U.S. Department of Energy [DE-AC05-00OR22725] FX Brian Damit was supported by the National Science Foundation Graduate Research Fellowship (NSF GRF) under grant DGE-0802270. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. NR 21 TC 2 Z9 2 U1 1 U2 7 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 520 CHESTNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0278-6826 EI 1521-7388 J9 AEROSOL SCI TECH JI Aerosol Sci. Technol. PD MAY 4 PY 2014 VL 48 IS 5 BP 562 EP 570 DI 10.1080/02786826.2014.899682 PG 9 WC Engineering, Chemical; Engineering, Mechanical; Environmental Sciences; Meteorology & Atmospheric Sciences SC Engineering; Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA AE3MO UT WOS:000333880800011 ER PT J AU Nouidui, TS Wetter, M Zuo, WD AF Nouidui, Thierry Stephane Wetter, Michael Zuo, Wangda TI Functional mock-up unit for co-simulation import in EnergyPlus SO JOURNAL OF BUILDING PERFORMANCE SIMULATION LA English DT Article DE functional mock-up interface; functional mock-up unit; co-simulation; building simulation ID BUILDING ENERGY; PERFORMANCE AB This article describes the development and implementation of the functional mock-up unit (FMU) for co-simulation import interface in EnergyPlus. This new capability allows EnergyPlus to conduct co-simulation with various simulation programs that are packaged as FMUs. For example, one can model an innovative Heating, Ventilation, and Air Conditioning (HVAC) system and its controls in Modelica, export the HVAC system and the control algorithm as an FMU, and link it to a model of the building envelope in EnergyPlus for run-time data exchange. The formal of FMUs is specified in the functional mock-up interface (FMI) standard, an open standard designed to enable links between disparate simulation programs. An FMU may contain models, model description, source code, and executable programs for multiple platforms. A master simulator - in this case, EnergyPlus - imports and simulates the FMUs, controlling simulation time and coordinating the exchange of data between the different FMUs. This article describes the mathematical basis of the FMI standard, discusses its application to EnergyPlus, and describes the architecture of the EnergyPlus implementation. It then presents a typical workflow, including pre-processing and co-simulation. The article concludes by presenting two use cases in which models of a ventilation system and a shading controller are imported in EnergyPlus as an FMU. C1 [Nouidui, Thierry Stephane; Wetter, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Zuo, Wangda] Univ Miami, Dept Civil Architectural & Environm Engn, Miami, FL USA. RP Nouidui, TS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM TSNouidui@lbl.gov FU Office of Building Technologies of the US Department of Energy [DE-AC02-05CH11231] FX This research was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technologies of the US Department of Energy, under Contract No. DE-AC02-05CH11231. NR 28 TC 9 Z9 9 U1 3 U2 27 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1940-1493 EI 1940-1507 J9 J BUILD PERFORM SIMU JI J. Build. Perf. Simul. PD MAY 4 PY 2014 VL 7 IS 3 BP 192 EP 202 DI 10.1080/19401493.2013.808265 PG 11 WC Construction & Building Technology SC Construction & Building Technology GA 272ML UT WOS:000328464700003 ER PT J AU Zhang, LW Deshusses, M AF Zhang, Liwei Deshusses, Marc TI Application of the finite difference method to model pH and substrate concentration in a double-chamber microbial fuel cell SO ENVIRONMENTAL TECHNOLOGY LA English DT Article ID WASTE-WATER TREATMENT; ELECTRICITY-GENERATION; PERFORMANCE; TECHNOLOGY; MEMBRANE; ANODES C1 [Zhang, Liwei] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Deshusses, Marc] Duke Univ, Dept Civil & Environm Engn, Durham, NC 27708 USA. RP Zhang, LW (reprint author), Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM zlwe88@gmail.com NR 26 TC 2 Z9 2 U1 2 U2 65 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0959-3330 EI 1479-487X J9 ENVIRON TECHNOL JI Environ. Technol. PD MAY 3 PY 2014 VL 35 IS 9 BP 1064 EP 1076 PG 13 WC Environmental Sciences SC Environmental Sciences & Ecology GA AA2OG UT WOS:000330933300002 PM 24701902 ER PT J AU Gwon, GH Jo, A Baek, K Jin, KS Fu, Y Lee, JB Kim, Y Cho, Y AF Gwon, Gwang Hyeon Jo, Aera Baek, Kyuwon Jin, Kyeong Sik Fu, Yaoyao Lee, Jong-Bong Kim, YoungChang Cho, Yunje TI Crystal structures of the structure-selective nuclease Mus81-Eme1 bound to flap DNA substrates SO EMBO JOURNAL LA English DT Article DE crystal structure; flap DNA; homologous recombination; interstrand cross-link repair; Mus81 ID HOLLIDAY JUNCTION RESOLUTION; SACCHAROMYCES-CEREVISIAE MUS81-MMS4; HUMAN-CELLS; REPLICATION FORKS; ENDONUCLEASE; CLEAVAGE; RESOLVASE; COMPLEX; REPAIR; RECOGNITION AB The Mus81-Eme1 complex is a structure-selective endonuclease with a critical role in the resolution of recombination intermediates during DNA repair after interstrand cross-links, replication fork collapse, or double-strand breaks. To explain the molecular basis of 3 ' flap substrate recognition and cleavage mechanism by Mus81-Eme1, we determined crystal structures of human Mus81-Eme1 bound to various flap DNA substrates. Mus81-Eme1 undergoes gross substrate-induced conformational changes that reveal two key features: (i) a hydrophobic wedge of Mus81 that separates pre- and post-nick duplex DNA and (ii) a 5 ' end binding pocket that hosts the 5 ' nicked end of post-nick DNA. These features are crucial for comprehensive protein-DNA interaction, sharp bending of the 3 ' flap DNA substrate, and incision strand placement at the active site. While Mus81-Eme1 unexpectedly shares several common features with members of the 5 ' flap nuclease family, the combined structural, biochemical, and biophysical analyses explain why Mus81-Eme1 preferentially cleaves 3 ' flap DNA substrates with 5 ' nicked ends. C1 [Gwon, Gwang Hyeon; Jo, Aera; Baek, Kyuwon; Fu, Yaoyao; Cho, Yunje] Pohang Univ Sci & Technol, Dept Life Sci, Pohang, South Korea. [Jin, Kyeong Sik] Pohang Univ Sci & Technol, Pohang Accelerator Lab, Pohang, South Korea. [Lee, Jong-Bong] Pohang Univ Sci & Technol, Dept Phys, Pohang, South Korea. [Kim, YoungChang] Argonne Natl Lab, Struct Biol Ctr, Biosci Div, Argonne, IL 60439 USA. RP Cho, Y (reprint author), Pohang Univ Sci & Technol, Dept Life Sci, Pohang, South Korea. EM yunje@postech.ac.kr FU National R&D Program for Cancer Control, Ministry for Health and Welfare [1020280]; National Research Foundation of Korea (NRF) - Korea government (MEST) [2012004028, 2012-054226, 20120008833]; BK21 program (Ministry of Education) FX We thank Phil Jeffrey, Sang UK Kim and Chang II Ban for helpful discussion. We also thank G-One Ahn for critical reading. We also thank Wolf-Dietrich Heyer for sharing unpublished results (The Mus81-Mms4 structure-selective endonuclease requires nicked DNA junctions to undergo conformational changes and bend its DNA substrates for cleavage, Mukherjee et al, Nucleic Acids Res. In press). This work was supported by grants from the National R&D Program for Cancer Control, Ministry for Health and Welfare (1020280), National Research Foundation of Korea (NRF) grant funded by the Korea government (MEST, No. 2012004028, No. 2012-054226, and No. 20120008833), a rising star program (POSTECH), and the BK21 program (Ministry of Education). The authors declare that none of the authors have a financial interest related to this work. Coordinates and structure factors have been deposited to RCSB (4P0P for the 2.8 A complex, 4 P0Q for the 2.85 A metal-free complex, 4P0R for the 6.5 A complex, 4P0S for the 6.0 A complex). NR 51 TC 6 Z9 6 U1 1 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0261-4189 EI 1460-2075 J9 EMBO J JI Embo J. PD MAY 2 PY 2014 VL 33 IS 9 BP 1061 EP 1072 DI 10.1002/embj.201487820 PG 12 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA AH9WJ UT WOS:000336495500011 PM 24733841 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C Du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA PerezTomei, T Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Donckt, MV 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CA CMS Collaborat TI Search for Flavor-Changing Neutral Currents in Top-Quark Decays t -> Zq in pp Collisions at root s=8 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article AB A search for flavor-changing neutral currents in top-quark decays t -> Zq is performed in events produced from the decay chain (tt) over bar -> Zq + Wb, where both vector bosons decay leptonically, producing a final state with three leptons (electrons or muons). A data set collected with the CMS detector at the LHC is used, corresponding to an integrated luminosity of 19.7 fb(-1) of proton-proton collisions at a center-of-mass energy of 8 TeV. No excess is seen in the observed number of events relative to the standard model prediction; thus, no evidence for flavor-changing neutral currents in top-quark decays is found. A combination with a previous search at 7 TeV excludes a t. Zq branching fraction greater than 0.05% at the 95% confidence level. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. 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[Krammer, M.; Meyer, A.; Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Geiser, A.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. O.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Schroeder, M.; Stein, M.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.; Shepherd-Themistocleous, C. H.] Deutsch Elekt Synchrotron, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Goerner, M.; Gosselink, M.; Haller, J.; Heine, K.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Schlein, P.] Univ Hamburg, Hamburg, Germany. [Muentel, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Topsis-giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Swain, S. K.; Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Banerjee, S.; Guchait, M.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Potenza, R.; Tricomi, A.; Tuve, C.; Costa, M.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Rinkevicius, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, I-56010 Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. 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[Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.; De La Cruz, B.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. 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[Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Savoy-Navarro, A.; Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] ADeceased bAlso,Vienna Univ Technol,Vienna,Austri, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Sharma, A.; Mohanty, A. K.; Giordano, F.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; Pelliccioni, M.; Cossutti, F.; Seixas, J.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tauscher, L.; Theofilatos, K.; Treille, D.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Cosa, A.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76706 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL 35487 USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado Boulder, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY 14853 USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06824 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL 32611 USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA 52242 USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA 94720 USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN 55455 USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL 60208 USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR 00680 USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX 77251 USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN 37996 USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX 77843 USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA 22901 USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI 48202 USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. 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[Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Pioppi, M.] Univ Perugia, Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. 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KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Della Ricca, Giuseppe/B-6826-2013; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Ligabue, Franco/F-3432-2014; Lazzizzera, Ignazio/E-9678-2015; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015 OI Calvo Alamillo, Enrique/0000-0002-1100-2963; Cerrada, Marcos/0000-0003-0112-1691; Russ, James/0000-0001-9856-9155; Ragazzi, Stefano/0000-0001-8219-2074; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Scodellaro, Luca/0000-0002-4974-8330; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Novaes, Sergio/0000-0003-0471-8549; Montanari, Alessandro/0000-0003-2748-6373; Moon, Chang-Seong/0000-0001-8229-7829; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Sogut, Kenan/0000-0002-9682-2855; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Della Ricca, Giuseppe/0000-0003-2831-6982; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Lazzizzera, Ignazio/0000-0001-5092-7531; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350 FU BMWF; FWF (Austria); FNRS; FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/ IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAEandDST(India); IPM(Iran); SFI (Ireland); INFN(Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP- FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RASandRFBR(Russia); MESTD(Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 41 TC 44 Z9 44 U1 6 U2 64 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 2 PY 2014 VL 112 IS 17 AR 171802 DI 10.1103/PhysRevLett.112.171802 PG 16 WC Physics, Multidisciplinary SC Physics GA AH4LR UT WOS:000336099500003 PM 24836238 ER PT J AU Xu, TT Ripp, S Sayler, GS Close, DM AF Xu, Tingting Ripp, Steven Sayler, Gary S. Close, Dan M. TI Expression of a Humanized Viral 2A-Mediated lux Operon Efficiently Generates Autonomous Bioluminescence in Human Cells SO PLOS ONE LA English DT Article ID BACTERIAL LUCIFERASE; REPORTER; VECTORS; ASSAY; LINE; PCR AB Background: Expression of autonomous bioluminescence from human cells was previously reported to be impossible, suggesting that all bioluminescent-based mammalian reporter systems must therefore require application of a potentially influential chemical substrate. While this was disproven when the bacterial luciferase (lux) cassette was demonstrated to function in a human cell, its expression required multiple genetic constructs, was functional in only a single cell type, and generated a significantly reduced signal compared to substrate-requiring systems. Here we investigate the use of a humanized, viral 2A-linked lux genetic architecture for the efficient introduction of an autobioluminescent phenotype across a variety of human cell lines. Methodology/Principal Findings: The lux cassette was codon optimized and assembled into a synthetic human expression operon using viral 2A elements as linker regions. Human kidney, breast cancer, and colorectal cancer cell lines were both transiently and stably transfected with the humanized operon and the resulting autobioluminescent phenotype was evaluated using common imaging instrumentation. Autobioluminescent cells were screened for cytotoxic effects resulting from lux expression and their utility as bioreporters was evaluated through the demonstration of repeated monitoring of single populations over a prolonged period using both a modified E-SCREEN assay for estrogen detection and a classical cytotoxic compound detection assay for the antibiotic Zeocin. Furthermore, the use of self-directed bioluminescent initiation in response to target detection was assessed to determine its amenability towards deployment as fully autonomous sensors. In all cases, bioluminescent measurements were supported with traditional genetic and transcriptomic evaluations. Conclusions/Significance: Our results demonstrate that the viral 2A-linked, humanized lux genetic architecture successfully produced autobioluminescent phenotypes in all cell lines tested without the induction of cytotoxicity. This autobioluminescent phenotype allowed for repeated interrogation of populations and self-directed control of bioluminescent activation with detection limits and EC50 values similar to traditional reporter systems, making the autobioluminescent cells amenable to automated monitoring and significantly reducing the time and cost required to perform bioluminescent workflows. C1 [Xu, Tingting; Sayler, Gary S.] Oak Ridge Natl Lab, Joint Inst Biol Sci, Oak Ridge, TN USA. [Ripp, Steven; Close, Dan M.] 490 BioTech Inc, Knoxville, TN USA. RP Close, DM (reprint author), 490 BioTech Inc, Knoxville, TN USA. EM dan.close@490BioTech.com RI Ripp, Steven/B-2305-2008; Close, Dan/A-4417-2012 OI Ripp, Steven/0000-0002-6836-1764; FU NIH SBIR program [1R43ES022567-01]; National Institutes of Health, National Cancer Institute, Cancer Imaging Program [CA127745-01]; National Science Foundation Division of Chemical, Bioengineering, Environmental, and Transport Systems (CBET) [CBET-0853780]; Alternative Research & Development Foundation; Army Defense University Research Instrumentation Program FX This work was supported by the NIH SBIR program, award number 1R43ES022567-01, the National Institutes of Health, National Cancer Institute, Cancer Imaging Program, award number CA127745-01, the National Science Foundation Division of Chemical, Bioengineering, Environmental, and Transport Systems (CBET), award number CBET-0853780, the Alternative Research & Development Foundation, and the Army Defense University Research Instrumentation Program. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 33 TC 6 Z9 6 U1 4 U2 34 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 2 PY 2014 VL 9 IS 5 AR e96347 DI 10.1371/journal.pone.0096347 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI1ZS UT WOS:000336655700078 PM 24788811 ER PT J AU Knapik, JJ Steelman, RA Hoedebecke, SS Farina, EK Austin, KG Lieberman, HR AF Knapik, Joseph J. Steelman, Ryan A. Hoedebecke, Sally S. Farina, Emily K. Austin, Krista G. Lieberman, Harris R. TI A systematic review and meta-analysis on the prevalence of dietary supplement use by military personnel SO BMC COMPLEMENTARY AND ALTERNATIVE MEDICINE LA English DT Article DE Vitamins; Minerals; Multivitamins; Vitamin C; Vitamin E; Calcium; Iron; Protein; Creatine; Sport drink ID HEALTH INTERVIEW SURVEY; UNITED-STATES; ENERGY DRINKS; NATIONAL-HEALTH; CREATINE SUPPLEMENTATION; CARDIOVASCULAR-DISEASE; MINERAL SUPPLEMENTS; ARMY SOLDIERS; MULTIMINERAL SUPPLEMENTATION; NUTRITIONAL SUPPLEMENTS AB Background: Although a number of studies have been conducted on the prevalence of dietary supplement (DS) use in military personnel, these investigations have not been previously summarized. This article provides a systematic literature review of this topic. Methods: Literature databases, reference lists, and other sources were searched to find studies that quantitatively examined the prevalence of DS use in uniformed military groups. Prevalence data were summarized by gender and military service. Where there were at least two investigations, meta-analysis was performed using a random model and homogeneity of the prevalence values was assessed. Results: The prevalence of any DS use for Army, Navy, Air Force, and Marine Corps men was 55%, 60%, 60%, and 61%, respectively; for women corresponding values were 65%, 71%, 76%, and 71%, respectively. Prevalence of multivitamin and/or multimineral (MVM) use for Army, Navy, Air Force, and Marine Corps men was 32%, 46%, 47%, and 41%, respectively; for women corresponding values were 40%, 55%, 63%, and 53%, respectively. Use prevalence of any individual vitamin or mineral supplement for Army, Navy, Air Force, and Marine Corps men was 18%, 27%, 25%, and 24%, respectively; for women corresponding values were 29%, 36%, 40%, and 33%, respectively. Men in elite military groups (Navy Special Operations, Army Rangers, and Army Special Forces) had a use prevalence of 76% for any DS and 37% for MVM, although individual studies were not homogenous. Among Army men, Army women, and elite military men, use prevalence of Vitamin C was 15% for all three groups; for Vitamin E, use prevalence was 8%, 7%, and 9%, respectively; for sport drinks, use prevalence was 22%, 25% and 39%, respectively. Use prevalence of herbal supplements was generally low compared to vitamins, minerals, and sport drinks, <= 5% in most investigations. Conclusions: Compared to men, military women had a higher use prevalence of any DS and MVM. Army men and women tended to use DSs and MVM less than other service members. Elite military men appeared to use DSs and sport drinks more than other service members. C1 [Knapik, Joseph J.; Farina, Emily K.; Austin, Krista G.; Lieberman, Harris R.] US Army Res Inst Environm Med, Natick, MA 01760 USA. [Knapik, Joseph J.; Steelman, Ryan A.] US Army Inst Publ Hlth, Aberdeen Proving Ground, MD USA. [Hoedebecke, Sally S.] Seren Hill Nutr, Bethesda, MD USA. [Knapik, Joseph J.; Steelman, Ryan A.; Austin, Krista G.] Oak Ridge Inst Sci & Educ, Belcamp, MD USA. [Knapik, Joseph J.] USARIEM, Natick, KS USA. RP Knapik, JJ (reprint author), US Army Res Inst Environm Med, Natick, MA 01760 USA. EM joseph.j.knapik.ctr@mail.mil FU US Army Research Institute of Environmental Medicine (USARIEM); Army Institute of Public Health (AIPH); Department of Defense Center; Medical Research and Development Command FX We would like to thank Claudia Coleman and Dr Wayne Askew who assisted us in obtaining references. This research was supported in part by an appointment to the Knowledge Preservation Program at the US Army Research Institute of Environmental Medicine (USARIEM) and the Army Institute of Public Health (AIPH) administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and USARIEM. Funding was also provided by the Department of Defense Center for Dietary Supplement Research and the Medical Research and Development Command. NR 113 TC 13 Z9 14 U1 4 U2 12 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1472-6882 J9 BMC COMPLEM ALTERN M JI BMC Complement. Altern. Med. PD MAY 2 PY 2014 VL 14 AR 143 DI 10.1186/1472-6882-14-143 PG 19 WC Integrative & Complementary Medicine SC Integrative & Complementary Medicine GA AH3WV UT WOS:000336057800001 PM 24884570 ER PT J AU Tan, KM Chhor, G Binkowski, TA Jedrzejczak, RP Makowska-Grzyska, M Joachimiak, A AF Tan, Kemin Chhor, Gekleng Binkowski, T. Andrew Jedrzejczak, Robert P. Makowska-Grzyska, Magdalena Joachimiak, Andrzej TI Sensor Domain of Histidine Kinase KinB of Pseudomonas A HELIX- SWAPPED DIMER SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Bacterial Signal Transduction; Biosensors; Histidine Kinases; Protein Conformation; Protein Structure; Alginate Biosynthesis; Helix-swapped Dimer; Sensor Domain; Two-component System ID LIGAND-BINDING DOMAIN; CRYSTAL-STRUCTURE; SIGNAL-TRANSDUCTION; STRUCTURAL-ANALYSIS; LIGHT-SCATTERING; AERUGINOSA; PROTEINS; MECHANISM; VIRULENCE; RECEPTOR AB Background: The sensor domain (SD) of histidine kinase (HK) KinB (KinB-SD) receives signals from the environment and induces a transduction cascade. Results: Structures of the KinB-SD were obtained in ligand-free, phosphate-bound, and mutant forms. Conclusion: The unique helix-swapped KinB-SD structure forms a ligand-binding cavity on the dimer interface. Significance: KinB-SD studies provide insights into the signal transduction and identity of potential signaling molecules. The overproduction of polysaccharide alginate is responsible for the formation of mucus in the lungs of cystic fibrosis patients. Histidine kinase KinB of the KinB-AlgB two-component system in Pseudomonas aeruginosa acts as a negative regulator of alginate biosynthesis. The modular architecture of KinB is similar to other histidine kinases. However, its periplasmic signal sensor domain is unique and is found only in the Pseudomonas genus. Here, we present the first crystal structures of the KinB sensor domain. The domain is a dimer in solution, and in the crystal it shows an atypical dimer of a helix-swapped four-helix bundle. A positively charged cavity is formed on the dimer interface and involves several strictly conserved residues, including Arg-60. A phosphate anion is bound asymmetrically in one of the structures. In silico docking identified several monophosphorylated sugars, including -d-fructose 6-phosphate and -d-mannose 6-phosphate, a precursor and an intermediate of alginate synthesis, respectively, as potential KinB ligands. Ligand binding was confirmed experimentally. Conformational transition from a symmetric to an asymmetric structure and decreasing dimer stability caused by ligand binding may be a part of the signal transduction mechanism of the KinB-AlgB two-component system. C1 [Tan, Kemin; Chhor, Gekleng; Binkowski, T. Andrew; Jedrzejczak, Robert P.; Joachimiak, Andrzej] Argonne Natl Lab, Midwest Ctr Struct Genom, Argonne, IL 60439 USA. [Tan, Kemin; Joachimiak, Andrzej] Argonne Natl Lab, Struct Biol Ctr, Argonne, IL 60439 USA. [Tan, Kemin; Makowska-Grzyska, Magdalena; Joachimiak, Andrzej] Univ Chicago, Ctr Struct Genom Infect Dis, Chicago, IL 60637 USA. RP Joachimiak, A (reprint author), Argonne Natl Lab, Midwest Ctr Struct Genom, 9700 S Cass Ave, Argonne, IL 60439 USA. EM andrzejj@anl.gov FU Office of Science of the United States Department of Energy [DE-AC02-06CH11357] FX We thank members of the Structural Biology Center at Argonne National Laboratory for their help with data collection at the 19-ID beamline and Kimberly S. Buck for help with cloning. This research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the United States Department of Energy under Contract DE-AC02-06CH11357. NR 59 TC 2 Z9 2 U1 0 U2 2 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 2 PY 2014 VL 289 IS 18 BP 12232 EP 12244 DI 10.1074/jbc.M113.514836 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AG7ER UT WOS:000335581400005 PM 24573685 ER PT J AU Wycoff, DE Gott, MD DeGraffenreid, AJ Morrow, RP Sisay, N Embree, MF Ballard, B Fassbender, ME Cutler, CS Ketring, AR Jurisson, SS AF Wycoff, Donald E. Gott, Matthew D. DeGraffenreid, Anthony J. Morrow, Ryan P. Sisay, Nebiat Embree, Mary F. Ballard, Beau Fassbender, Michael E. Cutler, Cathy S. Ketring, Alan R. Jurisson, Silvia S. TI Chromatographic separation of selenium and arsenic: A potential Se-72/As-72 generator SO JOURNAL OF CHROMATOGRAPHY A LA English DT Article DE As-72; Se-72; Radionuclide generator; Ion exchange ID ISOTOPES; PET; RADIONUCLIDES; EXTRACTION; GERMANIUM; I-124; SE-72 AB An anion exchange method was developed to separate selenium and arsenic for potential utility in a Se-72/As-72 generator. The separation of the daughter As-72 from the Se-72 parent is based on the relative acid-base behavior of the two oxo-anions in their highest oxidation states. At pH 1.5, selenate is retained on strongly basic anion exchange resin as HSeO4- and SeO42-, while neutral arsenic acid, H3AsO4, is eluted. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wycoff, Donald E.; Gott, Matthew D.; DeGraffenreid, Anthony J.; Morrow, Ryan P.; Sisay, Nebiat; Jurisson, Silvia S.] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Embree, Mary F.; Cutler, Cathy S.; Ketring, Alan R.] Univ Missouri, Res Reactor Ctr, Columbia, MO 65211 USA. [Ballard, Beau; Fassbender, Michael E.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. RP Jurisson, SS (reprint author), Univ Missouri, Dept Chem, Columbia, MO 65211 USA. EM jurissons@missouri.edu RI Ballard, Beau/E-2925-2017; OI Ballard, Beau/0000-0003-1206-9358; Gott, Merryn/0000-0003-4399-962X FU Department of Energy, Office of Basic Energy Sciences, Isotope Research program [DE-SC0003851]; National Science Foundation under IGERT [DGE-0965983]; NIBIB Training Grant [NIBIB 5 T32 EB004822]; United States Department of Energy, Office of Science via from the Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics FX The authors acknowledge support from the Department of Energy, Office of Basic Energy Sciences, Isotope Research program under Grant No. DE-SC0003851, and trainee support from the National Science Foundation under IGERT award DGE-0965983 (M.D. Gott) and NIBIB Training Grant NIBIB 5 T32 EB004822 (A.J. DeGraffenreid). The 72Se production was funded by the United States Department of Energy, Office of Science via an award from the Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics. NR 27 TC 3 Z9 3 U1 1 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0021-9673 EI 1873-3778 J9 J CHROMATOGR A JI J. Chromatogr. A PD MAY 2 PY 2014 VL 1340 BP 109 EP 114 DI 10.1016/j.chroma.2014.03.033 PG 6 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA AH0JE UT WOS:000335804400012 PM 24679827 ER PT J AU Blaizot, JP Satow, D AF Blaizot, Jean-Paul Satow, Daisuke TI Ultrasoft fermionic excitation at finite chemical potential SO PHYSICAL REVIEW D LA English DT Article ID QUARK-GLUON PLASMA; HARD THERMAL LOOPS; ABELIAN GAUGE-FIELDS; HOT QED PLASMAS; HIGH-TEMPERATURE; QUASI-PARTICLES; COLLECTIVE EXCITATIONS; SUPERSYMMETRY BREAKING; GOLDSTONE FERMION; LANGEVIN EQUATION AB It has been suggested previously that an ultrasoft fermionic excitation develops, albeit with a small spectral weight, in a system of massless fermions and scalar bosons with Yukawa interaction at high temperature T. In this paper we study how this excitation is modified at finite chemical potential mu. We relate the existence of the ultrasoft mode to symmetries, in particular charge conjugation, and a supersymmetry of the free system which is spontaneously broken by finite temperature and finite density effects, as argued earlier by Lebedev and Smilga. A nonvanishing chemical potential breaks both symmetries explicitly and maximally at zero temperature where the mode ceases to exist. A detailed calculation indicates that the ultrasoft excitation persists as long as T >= 0.71 mu. C1 [Blaizot, Jean-Paul] CEA Saclay, CNRS, URA 2306, Inst Phys Theor, F-91191 Gif Sur Yvette, France. [Satow, Daisuke] RIKEN, Theoret Res Div, Nishina Ctr, Wako, Saitama 3510198, Japan. [Satow, Daisuke] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Blaizot, JP (reprint author), CEA Saclay, CNRS, URA 2306, Inst Phys Theor, F-91191 Gif Sur Yvette, France. EM jean-paul.blaizot@cea.fr; daisuke.sato@riken.jp FU JSPS KAKENHI [24.56384]; Universality and Emergence" from the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan; JSPS Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation [R2411]; European Research Council; Advanced Investigator [ERC-AD-267258] FX D. S. thanks Y. Hidaka for fruitful discussions and comments. D. S. was supported by JSPS KAKENHI Grant No. 24.56384, the Grant-in-Aid for the Global COE Program "The Next Generation of Physics, Spun from Universality and Emergence" from the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan, and JSPS Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation (No. R2411). The research of J. P. B. is supported by the European Research Council under the Advanced Investigator Grant No. ERC-AD-267258. NR 70 TC 7 Z9 7 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 2 PY 2014 VL 89 IS 9 AR 096001 DI 10.1103/PhysRevD.89.096001 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AH4MG UT WOS:000336101600003 ER PT J AU Ilan, R Bardarson, JH Sim, HS Moore, JE AF Ilan, Roni Bardarson, Jens H. Sim, H-S Moore, Joel E. TI Detecting perfect transmission in Josephson junctions on the surface of three dimensional topological insulators SO NEW JOURNAL OF PHYSICS LA English DT Article DE topological insulators; transport in nanowires; Majorana fermions; Josephson junctions; topological superconductivity; perfect transmission ID MAJORANA FERMIONS; SUPERCONDUCTORS; STATES; NANORIBBONS; NANOWIRES AB We consider Josephson junctions on surfaces of three dimensional topological insulator nanowires. We find that in the presence of a parallel magnetic field, short junctions on nanowires show signatures of a perfectly transmitted mode capable of supporting Majorana fermions. Such signatures appear in the current-phase relation in the presence or absence of the fermion parity anomaly, and are most striking when considering the critical current as a function of flux Phi, which exhibits a peak at Phi = h/2e. The peak sharpens in the presence of disorder at low but finite chemical potentials, and can be easily disentangled from weak-anti-localization effects. The peak also survives at small but finite temperatures, and represents a realistic and robust hallmark for perfect transmission and the emergence of Majorana physics inside the wire. C1 [Ilan, Roni] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ilan, Roni; Bardarson, Jens H.; Moore, Joel E.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Sim, H-S] Korea Adv Inst Sci & Technol, Dept Phys, Taejon 305701, South Korea. [Moore, Joel E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Ilan, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM rilan@berkeley.edu RI Sim, Heung-Sun/C-1624-2011; Moore, Joel/O-4959-2016 OI Moore, Joel/0000-0002-4294-5761 FU Weizmann Institute of Science-National Postdoctoral Award Program for Advancing Women in Science; AFOSR; DARPA; Korea NRF [2012S1A2A1A01030312] FX The authors thank Kathryn Moler, Ilya Sochnikov, Katja Nowack, David Goldhaber-Gordon and Gil Refael for useful discussions. RI is an Awardee of the Weizmann Institute of Science-National Postdoctoral Award Program for Advancing Women in Science. The authors acknowledges support from AFOSR (RI) and DARPA (JHB, H-SS, and JEM). H-SS is supported by Korea NRF (grant No. 2012S1A2A1A01030312). NR 55 TC 6 Z9 6 U1 5 U2 30 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 2 PY 2014 VL 16 AR 053007 DI 10.1088/1367-2630/16/5/053007 PG 13 WC Physics, Multidisciplinary SC Physics GA AG4IV UT WOS:000335384100001 ER PT J AU Turner, JA AF Turner, John A. TI Shining a Light on Solar Water Splitting Response SO SCIENCE LA English DT Letter ID HYDROGEN-PRODUCTION C1 Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Turner, JA (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM John.Turner@nrel.gov NR 12 TC 0 Z9 0 U1 6 U2 41 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 2 PY 2014 VL 344 IS 6183 BP 468 EP 469 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG1EK UT WOS:000335157700020 ER PT J AU Stephenson, B AF Stephenson, Brian TI Advanced Photon Source Upgrade Benefits All SO SCIENCE LA English DT Letter C1 [Stephenson, Brian] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Stephenson, Brian] Argonne Natl Lab, Argonne, IL 60439 USA. RP Stephenson, B (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM aps-director@aps.an.gov NR 0 TC 0 Z9 0 U1 0 U2 2 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 2 PY 2014 VL 344 IS 6183 BP 469 EP 469 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG1EK UT WOS:000335157700021 ER PT J AU Yin, XB Ye, ZL Chenet, DA Ye, Y O'Brien, K Hone, JC Zhang, X AF Yin, Xiaobo Ye, Ziliang Chenet, Daniel A. Ye, Yu O'Brien, Kevin Hone, James C. Zhang, Xiang TI Edge Nonlinear Optics on a MoS2 Atomic Monolayer SO SCIENCE LA English DT Article ID POLYCRYSTALLINE GRAPHENE; MOLYBDENUM-DISULFIDE; VALLEY POLARIZATION; GRAIN-BOUNDARIES; GENERATION; TRANSPORT; STATES AB The translational symmetry breaking of a crystal at its surface may form two-dimensional (2D) electronic states. We observed one-dimensional nonlinear optical edge states of a single atomic membrane of molybdenum disulfide (MoS2), a transition metal dichalcogenide. The electronic structure changes at the edges of the 2D crystal result in strong resonant nonlinear optical susceptibilities, allowing direct optical imaging of the atomic edges and boundaries of a 2D material. Using the symmetry of the nonlinear optical responses, we developed a nonlinear optical imaging technique that allows rapid and all-optical determination of the crystal orientations of the 2D material at a large scale. Our technique provides a route toward understanding and making use of the emerging 2D materials and devices. C1 [Yin, Xiaobo; Ye, Ziliang; Ye, Yu; O'Brien, Kevin; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Chenet, Daniel A.; Hone, James C.] Columbia Univ, Dept Mech Engn, New York, NY 10027 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Hone, James/E-1879-2011; Zhang, Xiang/F-6905-2011; Ye, Ziliang/A-2104-2011; Yin, Xiaobo/A-4142-2011 OI Hone, James/0000-0002-8084-3301; FU U.S. Air Force Office of Scientific Research, Multidisciplinary University Research Initiative program [FA9550-12-1-0024]; Center for Re-Defining Photovoltaic Efficiency Through Molecular-Scale Control, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001085] FX Supported by the U.S. Air Force Office of Scientific Research, Multidisciplinary University Research Initiative program, under grant FA9550-12-1-0024. The synthesis of the material was supported by the Center for Re-Defining Photovoltaic Efficiency Through Molecular-Scale Control, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under award DE-SC0001085 (D.A.C. and J.C.H.). NR 30 TC 142 Z9 143 U1 44 U2 405 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 2 PY 2014 VL 344 IS 6183 BP 488 EP 490 DI 10.1126/science.1250564 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AG1EK UT WOS:000335157700035 PM 24786072 ER PT J AU Lin, J Sinitsyn, NA AF Lin, J. Sinitsyn, N. A. TI The model of a level crossing with a Coulomb band: exact probabilities of nonadiabatic transitions SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE Landau-Zener; nonadiabatic transitions; exactly solvable model ID LANDAU-ZENER MODEL; SURVIVAL PROBABILITY AB We derive an exact solution of an explicitly time-dependent multichannel model of quantum mechanical nonadiabatic transitions. Our model corresponds to the case of a single linear diabatic energy level interacting with a band of an arbitrary N states, for which the diabatic energies decay with time according to the Coulomb law. We show that the time-dependent Schrodinger equation for this system can be solved in terms of Meijer functions whose asymptotics at a large time can be compactly written in terms of elementary functions that depend on the roots of an Nth order characteristic polynomial. Our model can be considered a generalization of the Demkov-Osherov model. In comparison to the latter, our model allows one to explore the role of curvature of the band levels and diabatic avoided crossings. C1 [Lin, J.] Princeton Univ, Dept Math, Princeton, NJ 08544 USA. [Lin, J.; Sinitsyn, N. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, J (reprint author), Princeton Univ, Dept Math, Princeton, NJ 08544 USA. EM jeffminl@princeton.edu; nsinitsyn@lanl.gov NR 20 TC 1 Z9 1 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD MAY 2 PY 2014 VL 47 IS 17 AR 175301 DI 10.1088/1751-8113/47/17/175301 PG 16 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA AF3IC UT WOS:000334604300005 ER PT J AU Ramirez, G Oezer, D Rivera, M Rodil, SE Sanjines, R AF Ramirez, G. Oezer, D. Rivera, M. Rodil, S. E. Sanjines, R. TI TaSiN nanocomposite thin films: Correlation between structure, chemical composition, and physical properties SO THIN SOLID FILMS LA English DT Article DE Tantalum nitride; Silicon nitride; Thin films; Optical properties; Electrical properties; Nanocomposites ID N DIFFUSION-BARRIERS; ELECTRICAL-RESISTIVITY; SPUTTER-DEPOSITION; CU METALLIZATION; TANTALUM NITRIDE; MAGNETRON; TA; MECHANISM; COATINGS; MEMORY AB The structural and electronic properties of fcc-TaN/SiNx nanocomposite thin films deposited by reactive magnetron sputtering have been investigated as function of the N and Si contents. Our studies have been mainly focused on three different types of nanocomposite TaxSiyNz films based on: nitrogen deficient fcc-TaN0.88, nearly stoichiometric fcc-TaN, and over-stoichiometric fcc-TaN1.2 with the Si contents in the range from 0 to about 15 at.%. The optical properties were investigated by ellipsometric measurements, while the DC. electrical resistivity was measured using the van der Pauw configuration at 300 K. The optical measurements were interpreted using the standard Drude-Lorentz model. The results showed that the electronic properties are closely correlated with both the compositional and the structural modifications of the TaxSiyNz films induced by the addition of Si atoms, and also depending on the stoichiometry of the starting fcc-TaN system. Thus, depending on both the nitrogen and the silicon contents, the fcc-TaxSiyNz films can exhibit room temperature resistivity values ranging from 10(2) mu Omega cm to about 6 x 10(4) mu Omega cm. Published by Elsevier B.V. C1 [Ramirez, G.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Ramirez, G.; Rodil, S. E.] Univ Nacl Autonoma Mexico, Inst Invest Mat, Mexico City 04510, DF, Mexico. [Oezer, D.; Sanjines, R.] Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland. [Rivera, M.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 04510, DF, Mexico. RP Ramirez, G (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jramirez@anl.gov RI RODIL, SANDRA ELIZABETH/A-5196-2008; EPFL, Physics/O-6514-2016; OI RODIL, SANDRA ELIZABETH/0000-0002-0275-4418; RAMIREZ, GIOVANNI/0000-0003-0985-1605 FU Swiss National Science Foundation; PAPIIT-UNAM [103910]; CONACYT FX The authors are grateful to the Swiss National Science Foundation and PAPIIT-UNAM 103910 for the financial support; G. Ramirez acknowledges the support of CONACYT for scholarship during his PhD studies. S. E. Rodil thanks the technical support from H. Zarco for the electronic maintenance, A. Tejeda for the XRD support and L. Huerta for the XPS analysis. NR 40 TC 5 Z9 6 U1 2 U2 25 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAY 2 PY 2014 VL 558 BP 104 EP 111 DI 10.1016/j.tsf.2014.02.079 PG 8 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA AE9GL UT WOS:000334314100015 ER PT J AU Jeanne, P Guglielmi, Y Cappa, F Rinaldi, AP Rutqvist, J AF Jeanne, Pierre Guglielmi, Yves Cappa, Frederic Rinaldi, Antonio P. Rutqvist, Jonny TI The effects of lateral property variations on fault-zone reactivation by fluid pressurization: Application to CO2 pressurization effects within major and undetected fault zones SO JOURNAL OF STRUCTURAL GEOLOGY LA English DT Article DE Fault zone architecture; Damage zone continuity; Coupled hydromechanical processes; Fault reactivation ID STRIKE-SLIP FAULTS; DAMAGE ZONE; STRUCTURAL EVOLUTION; EMPIRICAL RELATIONS; CARBONATE ROCKS; SE UTAH; PERMEABILITY; INJECTION; DISPLACEMENT; DEFORMATION AB In this study, we performed in situ multidisciplinary analyses of two different fault zones in carbonate formations. One is a seismically active fault zone several kilometers long (the Roccasseira Fault Zone); the other is a small fault zone a few hundred meters long (the GAS Fault Zone). The smaller, "immature" fault zone displays a discontinuous damage zone, because tectonic deformations have been accommodated differently according to the initial properties of the host rock. The larger, "mature" fault zone displays a continuous damage zone caused by the presence of secondary fault cores embedded in a heavily fractured area inside the damage zone. These markedly different fault-zone architectures were reflected in two hydraulic and geomechanical fault models, both generated from a coupled fluid-flow and geomechanical simulator, to examine the impact of hydromechanical property distribution on fault stability when the faults are reactivated by CO2 injection. In the smaller fault zone, marked differences in hydromechanical properties (Young's modulus and permeability) favor fluid accumulation, inducing high pressurization in parts of the damage zone, potentially resulting in small seismic events. On the other hand in the mature fault zone, fluid flows more easily and thus fluid-induced earthquakes may not readily occur, because the fault-zone pressurization is much lower, insufficient for triggering a seismic event. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Jeanne, Pierre; Rinaldi, Antonio P.; Rutqvist, Jonny] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Cappa, Frederic] Univ Nice Sophia Antipolis, Cote Azur Observ, Geoazur, F-06550 Sophia Antipolis, France. [Guglielmi, Yves] Aix Marseille Univ, CEREGE, F-13331 Marseille, France. RP Jeanne, P (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM pjeanne@lbl.gov RI Rinaldi, Antonio Pio/N-3284-2013; Rutqvist, Jonny/F-4957-2015; Jeanne, Pierre/I-2996-2015; Cappa, Frederic/B-4014-2017 OI Rinaldi, Antonio Pio/0000-0001-7052-8618; Rutqvist, Jonny/0000-0002-7949-9785; Jeanne, Pierre/0000-0003-1487-8378; Cappa, Frederic/0000-0003-4859-8024 FU ANR "Captage de CO2" through the "HPPP-CO2" project; PACA county; LSBB through the "PETRO-PRO" project; Assistant Secretary for Fossil Energy, Office of Natural Gas and Petroleum Technology, through the National Energy technology laboratory, under the U.S Department of Energy [DE-AC02-05CH11231] FX We thank the Low Noise Underground Laboratory (LSBB) engineering team (http://www.lsbb.eu) for the human and technical support during our field work, and their amazing hospitality. This work has been funded by the ANR "Captage de CO2" through the "HPPP-CO2" project, by the PACA county and by the LSBB through the "PETRO-PRO" project. This work was also supported by the Assistant Secretary for Fossil Energy, Office of Natural Gas and Petroleum Technology, through the National Energy technology laboratory, under the U.S Department of Energy Contract No. DE-AC02-05CH11231. We are grateful for the constructive comments and recommendations of the two reviewers Atilla Aydin and Tom Mitchell, which substantially improved this paper. NR 60 TC 5 Z9 7 U1 2 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0191-8141 J9 J STRUCT GEOL JI J. Struct. Geol. PD MAY PY 2014 VL 62 BP 97 EP 108 DI 10.1016/j.jsg.2014.01.017 PG 12 WC Geosciences, Multidisciplinary SC Geology GA CD7DP UT WOS:000351251300008 ER PT J AU Lin, H Hurt, RA Johs, A Parks, JM Morrell-Falvey, JL Liang, LY Elias, DA Gu, BH AF Lin, Hui Hurt, Richard A., Jr. Johs, Alexander Parks, Jerry M. Morrell-Falvey, Jennifer L. Liang, Liyuan Elias, Dwayne A. Gu, Baohua TI Unexpected Effects of Gene Deletion on Interactions of Mercury with the Methylation-Deficient Mutant Delta hgcAB SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS LA English DT Article ID NATURAL ORGANIC-MATTER; DISSOLVED ELEMENTAL MERCURY; DISULFIDE BOND FORMATION; GEOBACTER-SULFURREDUCENS; REDUCING BACTERIA; PRINCIPAL METHYLATORS; ANOXIC ENVIRONMENTS; ANAEROBIC-BACTERIA; REDUCTION; OXIDATION AB The hgcA and hgcB gene pair is essential for mercury (Hg) methylation by certain anaerobic bacteria, but little is known about how deletion of hgcAB affects the cell surface interactions and intracellular uptake of Hg. Here, we compare Delta hgcAB mutants with the wild-type (WT) strains of both Geobacter sulfurreducens PCA and Desulfovibrio desulfuricans ND132 and observe differences in Hg redox transformations, adsorption, and uptake in laboratory incubation studies. In both strains, deletion of hgcAB increased the rate of reduction of Hg(II) but decreased the rate of oxidation of Hg(0) under anaerobic conditions. The measured cellular thiol content in Delta hgcAB mutants was lower than that in the WT, accounting for the decreased rates of adsorption and uptake of Hg. Despite the lack of methylation activity, uptake of Hg by the Delta hgcAB mutant continued, albeit at a rate slower than that of the WT. These findings demonstrate that deletion of the hgcAB gene pair not only eliminates Hg methylation but also alters cell physiology, resulting in changes to Hg redox reactions, sorption, and uptake by cells. C1 [Lin, Hui; Johs, Alexander; Liang, Liyuan; Gu, Baohua] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Hurt, Richard A., Jr.; Parks, Jerry M.; Morrell-Falvey, Jennifer L.; Elias, Dwayne A.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Lin, H (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. EM linh1@ornl.gov; gub1@ornl.gov RI Parks, Jerry/B-7488-2009; Morrell-Falvey, Jennifer/A-6615-2011; Gu, Baohua/B-9511-2012 OI Parks, Jerry/0000-0002-3103-9333; Morrell-Falvey, Jennifer/0000-0002-9362-7528; Gu, Baohua/0000-0002-7299-2956 FU Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy (DOE) as part of the Mercury Science Focus Area at Oak Ridge National Laboratory; DOE [DE-AC05-00OR22725] FX We thank Xiangping Yin and Yun Qian for technical assistance during methylmercury analysis. This research was sponsored by the Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy (DOE) as part of the Mercury Science Focus Area at Oak Ridge National Laboratory, which is managed by UT-Battelle LLC for the DOE under Contract DE-AC05-00OR22725. NR 32 TC 10 Z9 10 U1 2 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2328-8930 J9 ENVIRON SCI TECH LET JI Environ. Sci. Technol. Lett. PD MAY PY 2014 VL 1 IS 5 BP 271 EP 276 DI 10.1021/ez500107r PG 6 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CD1JL UT WOS:000350831100006 ER PT J AU Paskaleva, BS Godoy, SE Jang, WY Bender, SC Krishna, S Hayat, MM AF Paskaleva, Biliana S. Godoy, Sebastian E. Jang, Woo-Yong Bender, Steven C. Krishna, Sanjay Hayat, Majeed M. TI Model-Based Edge Detector for Spectral Imagery Using Sparse Spatiospectral Masks SO IEEE TRANSACTIONS ON IMAGE PROCESSING LA English DT Article DE Edge detection; isoluminant edge; classification; multicolor edge detection; spatio-spectral mask; spectral ratios ID MULTISPECTRAL IMAGES; CLASSIFICATION; SEGMENTATION; GRADIENT AB Two model-based algorithms for edge detection in spectral imagery are developed that specifically target capturing intrinsic features such as isoluminant edges that are characterized by a jump in color but not in intensity. Given prior knowledge of the classes of reflectance or emittance spectra associated with candidate objects in a scene, a small set of spectral-band ratios, which most profoundly identify the edge between each pair of materials, are selected to define a edge signature. The bands that form the edge signature are fed into a spatial mask, producing a sparse joint spatiospectral nonlinear operator. The first algorithm achieves edge detection for every material pair by matching the response of the operator at every pixel with the edge signature for the pair of materials. The second algorithm is a classifier-enhanced extension of the first algorithm that adaptively accentuates distinctive features before applying the spatiospectral operator. Both algorithms are extensively verified using spectral imagery from the airborne hyperspectral imager and from a dots-in-a-well midinfrared imager. In both cases, the multicolor gradient (MCG) and the hyperspectral/spatial detection of edges (HySPADE) edge detectors are used as a benchmark for comparison. The results demonstrate that the proposed algorithms outperform the MCG and HySPADE edge detectors in accuracy, especially when isoluminant edges are present. By requiring only a few bands as input to the spatiospectral operator, the algorithms enable significant levels of data compression in band selection. In the presented examples, the required operations per pixel are reduced by a factor of 71 with respect to those required by the MCG edge detector. C1 [Paskaleva, Biliana S.; Godoy, Sebastian E.; Bender, Steven C.; Krishna, Sanjay; Hayat, Majeed M.] Univ New Mexico, Dept Elect & Comp Engn, Ctr High Technol Mat, Albuquerque, NM 87131 USA. [Jang, Woo-Yong] US Air Force, Res Lab, Wright Patterson AFB, OH 45433 USA. RP Paskaleva, BS (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. EM bspaska@sandia.gov; sgodoy@unm.edu; jangusc@gmail.com; sbender@lanl.gov; skrishna@chtm.unm.edu; hayat@chtm.unm.edu RI Godoy, Sebastian/J-7148-2015 OI Godoy, Sebastian/0000-0001-8692-5749 FU National Consortium for MASINT Research Partnership Project through the Los Alamos National Laboratory [57461-001-07]; National Science Foundation [ECS-0401154, IIS-0434102, ECCS-0925757]; Korea Research Institute of Standards and Science; Nanostructures Far-IR/terahertz Detectors for Next Generation Imaging Technology Phase II Project; AFOSR Optoelectronic Research Center; New Mexico Cancer Nanoscience and Microsystems Training Center, University of New Mexico; CONICYT, Chile; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX Manuscript received July 14, 2013; revised December 20, 2013 and February 27, 2014; accepted March 16, 2014. Date of publication April 1, 2014; date of current version April 22, 2014. This work was supported in part by the National Consortium for MASINT Research Partnership Project through the Los Alamos National Laboratory under Grant 57461-001-07, in part by the National Science Foundation under Grant ECS-0401154 and Grant IIS-0434102, in part by the Korea Research Institute of Standards and Science, in part by Nanostructures Far-IR/terahertz Detectors for Next Generation Imaging Technology Phase II Project, in part by the National Science Foundation under Grant ECCS-0925757, and in part by AFOSR Optoelectronic Research Center Grant. The work of S. E. Godoy was supported in part by the New Mexico Cancer Nanoscience and Microsystems Training Center, University of New Mexico, and in part by CONICYT, Chile. Sandia National Laboratories is a MultiProgram Laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, through the U.S. Department of Energy National Nuclear Security Administration under Contract DE-AC04-94AL85000. The associate editor coordinating the review of this manuscript and approving it for publication was Dr. Debargha Mukherjee. NR 40 TC 1 Z9 1 U1 1 U2 7 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1057-7149 EI 1941-0042 J9 IEEE T IMAGE PROCESS JI IEEE Trans. Image Process. PD MAY PY 2014 VL 23 IS 5 BP 2315 EP 2327 DI 10.1109/TIP.2014.2315154 PG 13 WC Computer Science, Artificial Intelligence; Engineering, Electrical & Electronic SC Computer Science; Engineering GA CC3XK UT WOS:000350284400002 PM 24710830 ER PT J AU Hansen, N Skeen, SA Michelsen, HA Wilson, KR Kohse-Hoinghaus, K AF Hansen, Nils Skeen, Scott A. Michelsen, Hope A. Wilson, Kevin R. Kohse-Hoeinghaus, Katharina TI Flame Experiments at the Advanced Light Source: New Insights into Soot Formation Processes SO Jove-Journal of Visualized Experiments LA English DT Article DE Physics; Issue 87; Combustion; Flame; Energy Conversion; Mass Spectrometry; Photoionization; Synchrotron; Hydrocarbon; Soot; Aerosol; Isomer ID PHOTOIONIZATION MASS-SPECTROMETRY; FUEL-RICH FLAMES; COMBUSTION CHEMISTRY; AIR-POLLUTION; SYNCHROTRON; ISOMERS; IDENTIFICATION; MECHANISMS; EMISSIONS; CANCER AB The following experimental protocols and the accompanying video are concerned with the flame experiments that are performed at the Chemical Dynamics Beamline of the Advanced Light Source (ALS) of the Lawrence Berkeley National Laboratory(1-4). This video demonstrates how the complex chemical structures of laboratory-based model flames are analyzed using flame-sampling mass spectrometry with tunable synchrotron-generated vacuum-ultraviolet (VUV) radiation. This experimental approach combines isomer-resolving capabilities with high sensitivity and a large dynamic range(5,6). The first part of the video describes experiments involving burner-stabilized, reduced-pressure (20-80 mbar) laminar premixed flames. A small hydrocarbon fuel was used for the selected flame to demonstrate the general experimental approach. It is shown how species' profiles are acquired as a function of distance from the burner surface and how the tunability of the VUV photon energy is used advantageously to identify many combustion intermediates based on their ionization energies. For example, this technique has been used to study gas-phase aspects of the soot-formation processes, and the video shows how the resonance-stabilized radicals, such as C3H3, C3H5, and i-C4H5, are identified as important intermediates(7). The work has been focused on soot formation processes, and, from the chemical point of view, this process is very intriguing because chemical structures containing millions of carbon atoms are assembled from a fuel molecule possessing only a few carbon atoms in just milliseconds. The second part of the video highlights a new experiment, in which an opposed-flow diffusion flame and synchrotron-based aerosol mass spectrometry are used to study the chemical composition of the combustion-generated soot particles(4). The experimental results indicate that the widely accepted H-abstraction-C2H2-addition (HACA) mechanism is not the sole molecular growth process responsible for the formation of the observed large polycyclic aromatic hydrocarbons (PAHs). C1 [Hansen, Nils; Skeen, Scott A.; Michelsen, Hope A.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. [Wilson, Kevin R.] Lawrence Berkeley Natl Lab, Chem Sci Div, Adv Light Source, Berkeley, CA USA. [Kohse-Hoeinghaus, Katharina] Univ Bielefeld, Bielefeld, Germany. RP Hansen, N (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. EM nhansen@sandia.gov RI Kohse-Hoinghaus, Katharina/A-3867-2012; Hansen, Nils/G-3572-2012 FU National Nuclear Security Administration [DE-AC04-94-AL85000]; U.S. Department of Energy, Office of Basic Energy Sciences under the Single Investigator Small Group Research project [DE-SC0002619]; Department of Energy, Office of Science, Early Career Research Program under U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; DFG [KO 1363/18-3] FX Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000. The work was also supported by the U.S. Department of Energy, Office of Basic Energy Sciences under the Single Investigator Small Group Research project (Grant No. DE-SC0002619) of Prof. Violi (University of Michigan, Ann Arbor). KRW is supported by the Department of Energy, Office of Science, Early Career Research Program under U.S. Department of Energy Contract No. DE-AC02-05CH11231. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. KKH acknowledges continuing support of part of this research by the DFG under contract KO 1363/18-3. NR 28 TC 0 Z9 0 U1 3 U2 26 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD MAY PY 2014 IS 87 AR e51369 DI 10.3791/51369 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA4VV UT WOS:000348905400040 ER PT J AU Mitra, PP Loque, D AF Mitra, Prajakta Pradhan Loque, Dominique TI Histochemical Staining of Arabidopsis thaliana Secondary Cell Wall Elements SO Jove-Journal of Visualized Experiments LA English DT Article DE Cellular Biology; Issue 87; Xylem; Fibers; Lignin; polysaccharides; Plant cell wall; Maule staining; Phloroglucinol; Congo red; Toluidine blue O; Calcofluor white; Cell wall staining methods ID LIGNIN BIOSYNTHESIS; DEPOSITION; POLYSACCHARIDES; SPECIFICITY; BRIGHTENER; MUTANTS; PLANTS; ROOTS AB Arabidopsis thaliana is a model organism commonly used to understand and manipulate various cellular processes in plants, and it has been used extensively in the study of secondary cell wall formation. Secondary cell wall deposition occurs after the primary cell wall is laid down, a process carried out exclusively by specialized cells such as those forming vessel and fiber tissues. Most secondary cell walls are composed of cellulose (40-50%), hemicellulose (25-30%), and lignin (20-30%). Several mutations affecting secondary cell wall biosynthesis have been isolated, and the corresponding mutants may or may not exhibit obvious biochemical composition changes or visual phenotypes since these mutations could be masked by compensatory responses. Staining procedures have historically been used to show differences on a cellular basis. These methods are exclusively visual means of analysis; nevertheless their role in rapid and critical analysis is of great importance. Congo red and calcofluor white are stains used to detect polysaccharides, whereas Maule and phloroglucinol are commonly used to determine differences in lignin, and toluidine blue O is used to differentially stain polysaccharides and lignin. The seemingly simple techniques of sectioning, staining, and imaging can be a challenge for beginners. Starting with sample preparation using the A. thaliana model, this study details the protocols of a variety of staining methodologies that can be easily implemented for observation of cell and tissue organization in secondary cell walls of plants. C1 [Mitra, Prajakta Pradhan; Loque, Dominique] Joint Bioenergy Inst, Feedstocks Div, Emeryville, CA USA. [Mitra, Prajakta Pradhan; Loque, Dominique] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA USA. RP Loque, D (reprint author), Joint Bioenergy Inst, Feedstocks Div, Emeryville, CA USA. EM dloque@lbl.gov RI Loque, Dominique/A-8153-2008 FU U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX We are thankful to Sabin Russell for editing assistance. This work was part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. NR 22 TC 2 Z9 2 U1 1 U2 25 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD MAY PY 2014 IS 87 AR e51381 DI 10.3791/51381 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA4VV UT WOS:000348905400041 ER PT J AU Balibrea, J Mendoza, E Cano-Ott, D Guerrero, C Berthoumieux, E Altstadt, S Andrzejewski, J Audouin, L Barbagallo, M Becares, V Becvar, F Belloni, F Billowes, J Boccone, V Bosnar, D Brugger, M Calviani, M Calvino, F Carrapico, C Cerutti, F Chiaveri, E Chin, M Colonna, N Cortes, G Cortes-Giraldo, MA Diakaki, M Domingo-Pardo, C Duran, I Dressler, R Dzysiuk, N Eleftheriadis, C Ferrari, A Fraval, K Ganesan, S Garcia, AR Giubrone, G Gomez-Hornillos, MB Goncalves, IF Gonzalez-Romero, E Griesmayer, E Gunsing, F Gurusamy, P Jenkins, DG Jericha, E Kadi, Y Kappeler, F Karadimos, D Kawano, T Kivel, N Koehler, P Kokkoris, M Korschinek, G Krticka, M Kroll, J Langer, C Lampoudis, C Lederer, C Leeb, H Leong, LS Losito, R Manousos, A Marganiec, J Martinez, T Mastinu, PF Mastromarco, M Massimi, C Meaze, M Mengoni, A Milazzo, PM Mingrone, F Mirea, M Mondelaers, W Paradela, C Pavlik, A Perkowski, J Pignatari, M Plompen, A Praena, J Quesada, JM Rauscher, T Reifarth, R Riego, A Roman, F Rubbia, C Sarmento, R Schillebeeckx, P Schmidt, S Schumann, D Stetcu, I Sabate, M Tagliente, G Tain, JL Tarrio, D Tassan-Got, L Tsinganis, A Valenta, S Vannini, G Variale, V Vaz, P Ventura, A Versaci, R Vermeulen, MJ Vlachoudis, V Vlastou, R Wallner, A Ware, T Weigand, M Weiss, C Wright, TJ Zugec, P AF Balibrea, J. Mendoza, E. Cano-Ott, D. Guerrero, C. Berthoumieux, E. Altstadt, S. Andrzejewski, J. Audouin, L. Barbagallo, M. Becares, V. Becvar, F. Belloni, F. Billowes, J. Boccone, V. Bosnar, D. Brugger, M. Calviani, M. Calvino, F. Carrapico, C. Cerutti, F. Chiaveri, E. Chin, M. Colonna, N. Cortes, G. Cortes-Giraldo, M. A. Diakaki, M. Domingo-Pardo, C. Duran, I. Dressler, R. Dzysiuk, N. Eleftheriadis, C. Ferrari, A. Fraval, K. Ganesan, S. Garcia, A. R. Giubrone, G. Gomez-Hornillos, M. B. Goncalves, I. F. Gonzalez-Romero, E. Griesmayer, E. Gunsing, F. Gurusamy, P. Jenkins, D. G. Jericha, E. Kadi, Y. Kaeppeler, F. Karadimos, D. Kawano, T. Kivel, N. Koehler, P. Kokkoris, M. Korschinek, G. Krticka, M. Kroll, J. Langer, C. Lampoudis, C. Lederer, C. Leeb, H. Leong, L. S. Losito, R. Manousos, A. Marganiec, J. Martinez, T. Mastinu, P. F. Mastromarco, M. Massimi, C. Meaze, M. Mengoni, A. Milazzo, P. M. Mingrone, F. Mirea, M. Mondelaers, W. Paradela, C. Pavlik, A. Perkowski, J. Pignatari, M. Plompen, A. Praena, J. Quesada, J. M. Rauscher, T. Reifarth, R. Riego, A. Roman, F. Rubbia, C. Sarmento, R. Schillebeeckx, P. Schmidt, S. Schumann, D. Stetcu, I. Sabate, M. Tagliente, G. Tain, J. L. Tarrio, D. Tassan-Got, L. Tsinganis, A. Valenta, S. Vannini, G. Variale, V. Vaz, P. Ventura, A. Versaci, R. Vermeulen, M. J. Vlachoudis, V. Vlastou, R. Wallner, A. Ware, T. Weigand, M. Weiss, C. Wright, T. J. Zugec, P. TI Measurement of the Neutron Capture Cross Section of the Fissile Isotope U-235 with the CERN n_TOF Total Absorption Calorimeter and a Fission Tagging Based on Micromegas Detectors SO NUCLEAR DATA SHEETS LA English DT Article AB Current and future nuclear technologies require more accurate nuclear data on (n,gamma) cross sections and the alpha-ratios of fissile isotopes. Their measurement presents several difficulties, mainly related to the strong fission gamma-ray background competing with the weaker gamma- ray cascades used as the experimental signature of the (n,gamma) process. A specific setup was used at the CERN n_TOF facility in 2012 for the measurement of the (n,alpha) cross section and alpha-ratios of fissile isotopes and used for the case of the U-235 isotope. The setup consists of a set of micromegas fission detectors surrounding the U-235 samples all placed inside a segmented BaF2 Total Absorption Calorimeter. C1 [Balibrea, J.; Mendoza, E.; Cano-Ott, D.; Becares, V.; Garcia, A. R.; Gonzalez-Romero, E.; Martinez, T.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Guerrero, C.; Belloni, F.; Boccone, V.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Ferrari, A.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Tsinganis, A.; Versaci, R.; Vlachoudis, V.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Berthoumieux, E.; Belloni, F.; Chiaveri, E.; Fraval, K.; Gunsing, F.; Lampoudis, C.] CEA Saclay Irfu, Gif Sur Yvette, France. [Altstadt, S.; Langer, C.; Lederer, C.; Reifarth, R.; Schmidt, S.; Weigand, M.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Andrzejewski, J.; Marganiec, J.; Perkowski, J.] Uniwersytet Lodzki, Lodz, Poland. [Audouin, L.; Leong, L. S.; Tassan-Got, L.] CNRS, IN2P3, IPN, F-91405 Orsay, France. [Barbagallo, M.; Colonna, N.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Becvar, F.; Krticka, M.; Kroll, J.; Valenta, S.] Charles Univ Prague, Prague, Czech Republic. [Billowes, J.; Ware, T.; Wright, T. J.] Univ Manchester, Manchester, Lancs, England. [Bosnar, D.; Zugec, P.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia. [Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, Barcelona, Spain. [Carrapico, C.; Goncalves, I. F.; Sarmento, R.; Vaz, P.] Univ Tecn Lisboa, Inst Super Tecn, Inst Tecnol & Nucl, P-1096 Lisbon, Portugal. [Cortes-Giraldo, M. A.; Praena, J.; Quesada, J. M.; Sabate, M.] Univ Seville, Seville, Spain. [Diakaki, M.; Karadimos, D.; Kokkoris, M.; Vlastou, R.] Natl Tech Univ Athens, GR-10682 Athens, Greece. [Domingo-Pardo, C.; Giubrone, G.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain. [Duran, I.; Paradela, C.; Tarrio, D.] Univ Santiago de Compostela, Santiago De Compostela, Spain. [Dressler, R.; Kivel, N.; Schumann, D.] Paul Scherrer Inst, Villigen, Switzerland. [Dzysiuk, N.; Mastinu, P. F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Eleftheriadis, C.; Manousos, A.] Aristotle Univ Thessaloniki, Thessaloniki, Greece. [Ganesan, S.; Gurusamy, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Griesmayer, E.; Jericha, E.; Leeb, H.; Weiss, C.] Vienna Univ Technol, Atominst, Vienna, Austria. [Jenkins, D. G.; Vermeulen, M. J.] Univ York, York YO10 5DD, N Yorkshire, England. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Kawano, T.; Stetcu, I.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Koehler, P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Korschinek, G.] Tech Univ Munich, D-80290 Munich, Germany. [Lederer, C.; Pavlik, A.; Wallner, A.] Univ Vienna, Fac Phys, Vienna, Austria. [Massimi, C.; Mingrone, F.; Vannini, G.] Univ Bologna, Dept Fis, I-40126 Bologna, Italy. [Massimi, C.; Mingrone, F.; Vannini, G.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Mengoni, A.; Ventura, A.] Agenzia Nazl Nuove Tecnol, Energia Sviluppo Econ Sostenibile ENEA, Bologna, Italy. [Milazzo, P. M.] Ist Nazl Fis Nucl, Trieste, Italy. [Mirea, M.; Roman, F.] Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HH, Bucharest, Magurele, Romania. [Mondelaers, W.; Plompen, A.; Schillebeeckx, P.] European Commiss JRC, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Pignatari, M.; Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rubbia, C.] Lab Nazl Gran Sasso INFN, Assergi, AQ, Italy. RP Cano-Ott, D (reprint author), Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. EM daniel.cano@ciemat.es RI Calvino, Francisco/K-5743-2014; Langer, Christoph/L-3422-2016; Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012; Becares, Vicente/K-4514-2014; Vaz, Pedro/K-2464-2013; Martinez, Trinitario/K-6785-2014; Rauscher, Thomas/D-2086-2009; Mirea, Mihail/C-2297-2011; Cano Ott, Daniel/K-4945-2014; Gonzalez Romero, Enrique/L-7561-2014; Duran, Ignacio/H-7254-2015; Massimi, Cristian/K-2008-2015; Paradela, Carlos/J-1492-2012; Chin, Mary Pik Wai/B-6644-2012; Mendoza Cembranos, Emilio/K-5789-2014 OI Calvino, Francisco/0000-0002-7198-4639; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038; Tarrio, Diego/0000-0002-9858-3341; Becares, Vicente/0000-0003-3434-9086; Vaz, Pedro/0000-0002-7186-2359; Martinez, Trinitario/0000-0002-0683-5506; Rauscher, Thomas/0000-0002-1266-0642; Mirea, Mihail/0000-0002-9333-6595; Cano Ott, Daniel/0000-0002-9568-7508; Gonzalez Romero, Enrique/0000-0003-2376-8920; Massimi, Cristian/0000-0003-2499-5586; Chin, Mary Pik Wai/0000-0001-5176-9723; Mendoza Cembranos, Emilio/0000-0002-2843-1801 FU Spanish Plan Nacional [FPA2008-04972-C03-01, FPA2011-28770-C03-01] FX This work was supported in part by the Spanish national company for radioactive waste management ENRESA, through the CIEMAT ENRESA agreements on "Transmutacioon de residuos radiactivos de alta actividad" the Spanish Plan Nacional de I + D + i de Fisica de Particulas (project FPA2008-04972-C03-01 and FPA2011-28770-C03-01), the Spanish Ministerio de Ciencia e Innovacion through the CONSOLIDER CSD 200700042 project. The analysis of this measurement has been proposed for the "solving CHAllenges in Nuclear DAta" - CHANDA project of the 7th Framework Programme, currently under negotiation. NR 12 TC 2 Z9 2 U1 3 U2 15 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 10 EP 13 DI 10.1016/j.nds.2014.08.005 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200121 ER PT J AU Ullmann, JL Mosby, S Bredeweg, TA Couture, AJ Haight, RC Jandel, M Kawano, T O'Donnell, JM Rundberg, RS Vieira, DJ Wilhelmy, JB Wu, CY Becker, JA Chyzh, A Baramsai, B Mitchell, GE Krticka, M AF Ullmann, J. L. Mosby, S. Bredeweg, T. A. Couture, A. J. Haight, R. C. Jandel, M. Kawano, T. O'Donnell, J. M. Rundberg, R. S. Vieira, D. J. Wilhelmy, J. B. Wu, C. -Y. Becker, J. A. Chyzh, A. Baramsai, B. Mitchell, G. E. Krticka, M. TI Neutron Capture Cross Sections and Gamma Emission Spectra from Neutron Capture on U-234,U-236,U-238 Measured with DANCE SO NUCLEAR DATA SHEETS LA English DT Article ID NUCLEI; STRENGTH; U-236 AB A new measurement of the U-238(n, gamma) cross section using a thin 48 mg/cm(2) target was made using the DANCE detector at LANSCE over the energy range from 10 eV to 500 keV. The results confirm earlier measurements. Measurements of the gamma- ray emission spectra were also made for U-238(n, gamma) as well as U-234,U-236(n, gamma). These measurements help to constrain the radiative strength function used in the cross- section calculations. C1 [Ullmann, J. L.; Mosby, S.; Bredeweg, T. A.; Couture, A. J.; Haight, R. C.; Jandel, M.; Kawano, T.; O'Donnell, J. M.; Rundberg, R. S.; Vieira, D. J.; Wilhelmy, J. B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Wu, C. -Y.; Becker, J. A.; Chyzh, A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Baramsai, B.; Mitchell, G. E.] N Carolina State Univ, Raleigh, NC 27695 USA. [Krticka, M.] Charles Univ Prague, Prague, Czech Republic. RP Ullmann, JL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM ullmann@lanl.gov FU U.S. Department of Energy, National Nuclear Security Administration, by Los Alamos National Security, LLC, [DE-AC52-06NA25396]; Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]; Ministry of Education of the Czech Republic [MSM 0021620859]; Czech Science Foundation [13-07117S] FX This work benefitted from the use of the LANSCE Facility and the Manuel J. Lujan, Jr. Neutron Scattering Center. This work was performed under the auspices of the U.S. Department of Energy, National Nuclear Security Administration, by Los Alamos National Security, LLC, under contract DE-AC52-06NA25396, and by Lawrence Livermore National Security, LLC, under contract DE-AC52-07NA27344. Dr. Krticka's work was supported by plan MSM 0021620859 of the Ministry of Education of the Czech Republic and by the Czech Science Foundation under Grant No. 13-07117S. Substantial support for graduate students and post-docs was provided by the Stockpile Stewardship Academic Alliance of the NNSA. NR 19 TC 0 Z9 0 U1 1 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 22 EP 25 DI 10.1016/j.nds.2014.08.008 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200124 ER PT J AU Wright, T Guerrero, C Billowes, J Ware, T Cano-Ott, D Mendoza, E Massimi, C Mingrone, F Gunsing, F Berthoumieux, E Lampoudis, C Altstadt, S Andrzejewski, J Audouin, L Barbagallo, M Becares, V Becvar, F Belloni, F Boccone, V Bosnar, D Brugger, M Calviani, M Calvino, F Carrapico, C Cerutti, F Chiaveri, E Chin, M Colonna, N Cortes, G Cortes-Giraldo, MA Diakaki, M Domingo-Pardo, C Duran, I Dressler, R Dzysiuk, N Eleftheriadis, C Ferrari, A Fraval, K Ganesan, S Garcia, AR Gomez-Hornillos, MB Goncalves, IF Gonzalez-Romero, E Griesmayer, E Giubrone, G Gurusamy, P Jenkins, DG Jericha, E Kadi, Y Kappeler, F Karadimos, D Kivel, N Koehler, P Kokkoris, M Korschinek, G Krticka, M Kroll, J Langer, C Lederer, C Leeb, H Leong, LS Losito, R Manousos, A Marganiec, J Martinez, T Mastinu, PF Mastromarco, M Meaze, M Mengoni, A Milazzo, PM Mirea, M Mondelaers, W Paradela, C Pavlik, A Perkowski, J Pignatari, M Plompen, A Praena, J Quesada, JM Rauscher, T Reifarth, R Riego, A Roman, F Rubbia, C Sarmento, R Schillebeeckx, P Schmidt, S Schumann, D Tagliente, G Tain, JL Tarrio, D Tassan-Got, L Tsinganis, A Valenta, S Vannini, G Variale, V Vaz, P Ventura, A Versaci, R Vermeulen, MJ Vlachoudis, V Vlastou, R Wallner, A Weigand, M Weiss, C Zugec, P AF Wright, T. Guerrero, C. Billowes, J. Ware, T. Cano-Ott, D. Mendoza, E. Massimi, C. Mingrone, F. Gunsing, F. Berthoumieux, E. Lampoudis, C. Altstadt, S. Andrzejewski, J. Audouin, L. Barbagallo, M. Becares, V. Becvar, F. Belloni, F. Boccone, V. Bosnar, D. Brugger, M. Calviani, M. Calvino, F. Carrapico, C. Cerutti, F. Chiaveri, E. Chin, M. Colonna, N. Cortes, G. Cortes-Giraldo, M. A. Diakaki, M. Domingo-Pardo, C. Duran, I. Dressler, R. Dzysiuk, N. Eleftheriadis, C. Ferrari, A. Fraval, K. Ganesan, S. Garcia, A. R. Gomez-Hornillos, M. B. Goncalves, I. F. Gonzalez-Romero, E. Griesmayer, E. Giubrone, G. Gurusamy, P. Jenkins, D. G. Jericha, E. Kadi, Y. Kaeppeler, F. Karadimos, D. Kivel, N. Koehler, P. Kokkoris, M. Korschinek, G. Krticka, M. Kroll, J. Langer, C. Lederer, C. Leeb, H. Leong, L. S. Losito, R. Manousos, A. Marganiec, J. Martinez, T. Mastinu, P. F. Mastromarco, M. Meaze, M. Mengoni, A. Milazzo, P. M. Mirea, M. Mondelaers, W. Paradela, C. Pavlik, A. Perkowski, J. Pignatari, M. Plompen, A. Praena, J. Quesada, J. M. Rauscher, T. Reifarth, R. Riego, A. Roman, F. Rubbia, C. Sarmento, R. Schillebeeckx, P. Schmidt, S. Schumann, D. Tagliente, G. Tain, J. L. Tarrio, D. Tassan-Got, L. Tsinganis, A. Valenta, S. Vannini, G. Variale, V. Vaz, P. Ventura, A. Versaci, R. Vermeulen, M. J. Vlachoudis, V. Vlastou, R. Wallner, A. Weigand, M. Weiss, C. Zugec, P. TI High-precision Measurement of the U-238(n,gamma) Cross Section with the Total Absorption Calorimeter (TAC) at n_TOF, CERN SO NUCLEAR DATA SHEETS LA English DT Article AB The neutron capture cross section of U-238 is fundamental to the design and operation of current reactors and future fast nuclear reactors, and thus must be measured to a high level of accuracy. An experiment has been performed at the CERN n TOF facility using a 4 pi Total Absorption Calorimeter (TAC) to measure the capture cross section in the resolved resonance region between 1 eV and 25 keV. A preliminary analysis of the TAC data is presented with particular emphasis to the experimental background in this energy region of interest. C1 [Wright, T.; Guerrero, C.; Billowes, J.; Ware, T.] Univ Manchester, Manchester, Lancs, England. [Guerrero, C.; Belloni, F.; Boccone, V.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Ferrari, A.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Tsinganis, A.; Versaci, R.; Vlachoudis, V.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Cano-Ott, D.; Mendoza, E.; Becares, V.; Garcia, A. R.; Gonzalez-Romero, E.; Martinez, T.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Massimi, C.; Mingrone, F.; Vannini, G.] Univ Bologna, Dipartmento Fis, Bologna, Italy. [Massimi, C.; Mingrone, F.; Vannini, G.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Gunsing, F.; Berthoumieux, E.; Belloni, F.; Chiaveri, E.; Fraval, K.] CEA Saclay Irfu, Gif Sur Yvette, France. [Lampoudis, C.] CEA, Grenoble, France. [Altstadt, S.; Langer, C.; Reifarth, R.; Schmidt, S.; Weigand, M.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Andrzejewski, J.; Marganiec, J.; Perkowski, J.] Uniwersytet Lodzki, Lodz, Poland. [Audouin, L.; Leong, L. S.; Tassan-Got, L.] CNRS, IN2P3, IPN, Orsay, France. [Barbagallo, M.; Colonna, N.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Becvar, F.; Krticka, M.; Kroll, J.; Valenta, S.] Charles Univ Prague, Prague, Czech Republic. [Bosnar, D.; Zugec, P.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia. [Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, Barcelona, Spain. [Carrapico, C.; Goncalves, I. F.; Sarmento, R.; Vaz, P.] Univ Tecn Lisboa, Inst Super Tecn, Inst Tecnol & Nucl, P-1096 Lisbon, Portugal. [Cortes-Giraldo, M. A.; Praena, J.; Quesada, J. M.] Univ Seville, Seville, Spain. [Diakaki, M.; Karadimos, D.; Kokkoris, M.; Vlastou, R.] Natl Tech Univ Athens, GR-10682 Athens, Greece. [Domingo-Pardo, C.; Giubrone, G.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46003 Valencia, Spain. [Duran, I.; Paradela, C.; Tarrio, D.] Univ Santiago de Compostela, Santiago De Compostela, Spain. [Dressler, R.; Kivel, N.; Schumann, D.] Paul Scherrer Inst, Villigen, Switzerland. [Dzysiuk, N.; Mastinu, P. F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Eleftheriadis, C.; Manousos, A.] Aristotle Univ Thessaloniki, Thessaloniki, Greece. [Ganesan, S.; Gurusamy, P.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Griesmayer, E.; Jericha, E.; Leeb, H.; Weiss, C.] Vienna Univ Technol, Atominst, Vienna, Austria. [Jenkins, D. G.; Vermeulen, M. J.] Univ York, York YO10 5DD, N Yorkshire, England. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Koehler, P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Korschinek, G.] Tech Univ Munich, D-80290 Munich, Germany. [Lederer, C.; Pavlik, A.; Wallner, A.] Univ Vienna, Fac Phys, Vienna, Austria. [Mengoni, A.; Ventura, A.] Agenzia Nazl Nuove Tecnol, Energia Sviluppo Econ Sostenibile ENEA, Bologna, Italy. [Milazzo, P. M.] Ist Nazl Fis Nucl, Trieste, Italy. [Mirea, M.; Roman, F.] Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HH, Bucharest, Magurele, Romania. [Mondelaers, W.; Plompen, A.; Schillebeeckx, P.] European Commiss JRC, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Pignatari, M.; Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rubbia, C.] Lab Nazl Gran Sasso INFN, Assergi, AQ, Italy. RP Wright, T (reprint author), Univ Manchester, Oxford Rd, Manchester, Lancs, England. EM tobias.wright@postgrad.manchester.ac.uk RI Paradela, Carlos/J-1492-2012; Chin, Mary Pik Wai/B-6644-2012; Mendoza Cembranos, Emilio/K-5789-2014; Becares, Vicente/K-4514-2014; Martinez, Trinitario/K-6785-2014; Vaz, Pedro/K-2464-2013; Rauscher, Thomas/D-2086-2009; Mirea, Mihail/C-2297-2011; Cano Ott, Daniel/K-4945-2014; Gonzalez Romero, Enrique/L-7561-2014; Duran, Ignacio/H-7254-2015; Massimi, Cristian/K-2008-2015; Calvino, Francisco/K-5743-2014; Langer, Christoph/L-3422-2016; Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012 OI Chin, Mary Pik Wai/0000-0001-5176-9723; Mendoza Cembranos, Emilio/0000-0002-2843-1801; Becares, Vicente/0000-0003-3434-9086; Martinez, Trinitario/0000-0002-0683-5506; Vaz, Pedro/0000-0002-7186-2359; Rauscher, Thomas/0000-0002-1266-0642; Mirea, Mihail/0000-0002-9333-6595; Cano Ott, Daniel/0000-0002-9568-7508; Gonzalez Romero, Enrique/0000-0003-2376-8920; Massimi, Cristian/0000-0003-2499-5586; Calvino, Francisco/0000-0002-7198-4639; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038 FU UK Nuclear Decommissioning Authority (NDA); EPSRC; CERN; EC-FP7 ANDES project [FP7-249671]; ENRESA under the CIEMAT-ENRESA agreement; Spanish Ministry of Science and Innovation [FPA2005-06918-C03-01] FX The authors acknowledge financial support from the UK Nuclear Decommissioning Authority (NDA), EPSRC, CERN, the EC-FP7 ANDES (FP7-249671) project, ENRESA under the CIEMAT-ENRESA agreement and the Spanish Ministry of Science and Innovation (FPA2005-06918-C03-01). NR 14 TC 7 Z9 7 U1 1 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 26 EP 30 DI 10.1016/j.nds.2014.08.009 PG 5 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200125 ER PT J AU Mosby, S Arnold, C Bredeweg, TA Chyzh, A Couture, A Henderson, R Jandel, M Kwan, E O'Donnell, JM Rusev, G Ullmann, L Wu, CY AF Mosby, S. Arnold, C. Bredeweg, T. A. Chyzh, A. Couture, A. Henderson, R. Jandel, M. Kwan, E. O'Donnell, J. M. Rusev, G. Ullmann, L. Wu, C. Y. TI Neutron Capture Cross Section of Pu-239 SO NUCLEAR DATA SHEETS LA English DT Article ID NUCLEAR-DATA; DANCE; DETECTOR AB The Detector for Advanced Neutron Capture Experiments (DANCE) has been used to measure the Pu-239(n,gamma) cross section from 10 eV to the keV region. Three experimental run conditions were used to characterize the prompt fission gamma-ray spectrum across the entire energy regime, measure the cross section in the resolved resonance region, and obtain necessary count rate well into the keV region. The preliminary cross sections are in good agreement with current evaluations from 10 eV to 80 keV. C1 [Mosby, S.; Arnold, C.; Bredeweg, T. A.; Couture, A.; Jandel, M.; O'Donnell, J. M.; Rusev, G.; Ullmann, L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Chyzh, A.; Henderson, R.; Kwan, E.; Wu, C. Y.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Mosby, S (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM smosby@lanl.gov FU US Department of Energy by Los Alamos National Security, LLC [DE-AC52-06NA25396]; US Department of Energy by Lawrence Livermore National Security, LLC [DE-AC52- 07NA27344] FX This work benefited from the use of the LANSCE accelerator facility. Work was performed under the auspices of the US Department of Energy by Los Alamos National Security, LLC under contract DE-AC52-06NA25396 and by Lawrence Livermore National Security, LLC under contract DE-AC52- 07NA27344. NR 19 TC 0 Z9 0 U1 2 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 31 EP 34 DI 10.1016/j.nds.2014.08.010 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200126 ER PT J AU Tarrio, D Leong, LS Audouin, L Duran, I Paradela, C Tassan-Got, L Altstadt, S Andrzejewski, J Barbagallo, M Becares, V Becvar, F Belloni, F Berthoumieux, E Billowes, J Boccone, V Bosnar, D Brugger, M Calviani, M Calvino, F Cano-Ott, D Carrapico, C Cerutti, F Chiaveri, E Chin, M Colonna, N Cortes, G Cortes-Giraldo, MA Diakaki, M Domingo-Pardo, C Dzysiuk, N Eleftheriadis, C Ferrari, A Fraval, K Ganesan, S Garcia, AR Giubrone, G Gomez-Hornillos, MB Goncalves, IF Gonzalez-Romero, E Griesmayer, E Guerrero, C Gunsing, F Gurusamy, P Jenkins, DG Jericha, E Kadi, Y Kappeler, F Karadimos, D Koehler, P Kokkoris, M Krticka, M Kroll, J Langer, C Lederer, C Leeb, H Losito, R Manousos, A Marganiec, J Martinez, T Massimi, C Mastinu, PF Mastromarco, M Meaze, M Mendoza, E Mengoni, A Milazzo, PM Mingrone, F Mirea, M Mondalaers, W Pavlik, A Perkowski, J Plompen, A Praena, J Quesada, JM Rauscher, T Reifarth, R Riego, A Roman, F Rubbia, C Sarmento, R Schillebeeckx, P Schmidt, S Tagliente, G Tain, JL Tsinganis, A Valenta, S Vannini, G Variale, V Vaz, P Ventura, A Versaci, R Vermeulen, MJ Vlachoudis, V Vlastou, R Wallner, A Ware, T Weigand, M Weiss, C Wright, TJ Zugec, P AF Tarrio, D. Leong, L. S. Audouin, L. Duran, I. Paradela, C. Tassan-Got, L. Altstadt, S. Andrzejewski, J. Barbagallo, M. Becares, V. Becvar, F. Belloni, F. Berthoumieux, E. Billowes, J. Boccone, V. Bosnar, D. Brugger, M. Calviani, M. Calvino, F. Cano-Ott, D. Carrapico, C. Cerutti, F. Chiaveri, E. Chin, M. Colonna, N. Cortes, G. Cortes-Giraldo, M. A. Diakaki, M. Domingo-Pardo, C. Dzysiuk, N. Eleftheriadis, C. Ferrari, A. Fraval, K. Ganesan, S. Garcia, A. R. Giubrone, G. Gomez-Hornillos, M. B. Goncalves, I. F. Gonzalez-Romero, E. Griesmayer, E. Guerrero, C. Gunsing, F. Gurusamy, P. Jenkins, D. G. Jericha, E. Kadi, Y. Kaeppeler, F. Karadimos, D. Koehler, P. Kokkoris, M. Krticka, M. Kroll, J. Langer, C. Lederer, C. Leeb, H. Losito, R. Manousos, A. Marganiec, J. Martinez, T. Massimi, C. Mastinu, P. F. Mastromarco, M. Meaze, M. Mendoza, E. Mengoni, A. Milazzo, P. M. Mingrone, F. Mirea, M. Mondalaers, W. Pavlik, A. Perkowski, J. Plompen, A. Praena, J. Quesada, J. M. Rauscher, T. Reifarth, R. Riego, A. Roman, F. Rubbia, C. Sarmento, R. Schillebeeckx, P. Schmidt, S. Tagliente, G. Tain, J. L. Tsinganis, A. Valenta, S. Vannini, G. Variale, V. Vaz, P. Ventura, A. Versaci, R. Vermeulen, M. J. Vlachoudis, V. Vlastou, R. Wallner, A. Ware, T. Weigand, M. Weiss, C. Wright, T. J. Zugec, P. CA N TOF Collaboration TI Fission Fragment Angular Distribution of Th-232(n,f) at the CERN n_TOF Facility SO NUCLEAR DATA SHEETS LA English DT Article AB The angular distribution of fragments emitted in neutron-induced fission of Th-232 was measured in the white spectrum neutron beam at the n_TOF facility at CERN. A reaction chamber based on Parallel Plate Avalanche Counters (PPAC) was used, where the detectors and the targets have been tilted 45 degrees with respect to the neutron beam direction in order to cover the full angular range of the fission fragments. A GEANT4 simulation has been developed to study the setup efficiency. The data analysis and the preliminary results obtained for the Th-232(n,f) between fission threshold and 100 MeV are presented here. C1 Univ Santiago de Compostela, Santiago De Compostela, Spain. [Leong, L. S.; Audouin, L.; Tassan-Got, L.; Lederer, C.] IPN, CNRS, IN2P3, Orsay, France. [Altstadt, S.; Langer, C.; Lederer, C.; Reifarth, R.; Schmidt, S.; Weigand, M.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Andrzejewski, J.; Marganiec, J.; Perkowski, J.] Univ Lodz, PL-90131 Lodz, Poland. [Barbagallo, M.; Colonna, N.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Becares, V.; Cano-Ott, D.; Garcia, A. R.; Gonzalez-Romero, E.; Martinez, T.; Mendoza, E.] CIEMAT, E-28040 Madrid, Spain. [Becvar, F.; Krticka, M.; Kroll, J.; Valenta, S.] Charles Univ Prague, Prague, Czech Republic. [Belloni, F.; Berthoumieux, E.; Bosnar, D.; Chiaveri, E.; Fraval, K.; Gunsing, F.] CEA Saclay, Irfu, F-91191 Gif Sur Yvette, France. [Berthoumieux, E.; Boccone, V.; Bosnar, D.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Ferrari, A.; Guerrero, C.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Tsinganis, A.; Versaci, R.; Vlachoudis, V.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Billowes, J.; Ware, T.; Wright, T. J.] Univ Manchester, Manchester, Lancs, England. [Zugec, P.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia. [Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, Barcelona, Spain. [Carrapico, C.; Goncalves, I. F.; Sarmento, R.; Vaz, P.] Univ Tecn Lisboa, Inst Super Tecn, Inst Tecnol Nucl, P-1096 Lisbon, Portugal. [Cortes-Giraldo, M. A.; Praena, J.; Quesada, J. M.] Univ Seville, Seville, Spain. [Diakaki, M.; Karadimos, D.; Kokkoris, M.; Vlastou, R.] Natl Tech Univ Athens, GR-10682 Athens, Greece. [Domingo-Pardo, C.; Giubrone, G.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46003 Valencia, Spain. [Dzysiuk, N.; Mastinu, P. F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Eleftheriadis, C.; Manousos, A.] Aristotle Univ Thessaloniki, GR-54006 Thessaloniki, Greece. [Ganesan, S.; Gurusamy, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Griesmayer, E.; Jericha, E.; Leeb, H.; Weiss, C.] Vienna Univ Technol, Inst Atom, Vienna, Austria. [Jenkins, D. G.; Vermeulen, M. J.] Univ York, York YO10 5DD, N Yorkshire, England. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Koehler, P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Lederer, C.; Pavlik, A.; Wallner, A.] Univ Vienna, Fac Phys, A-1010 Vienna, Austria. [Massimi, C.; Mingrone, F.; Vannini, G.] Univ Bologna, Dipartimento Fis, I-40126 Bologna, Italy. [Massimi, C.; Mingrone, F.; Vannini, G.] Sez INFN Bologna, Bologna, Italy. [Mengoni, A.; Ventura, A.] Agenzia Nazl Nuove Tecnol, Eenergia & Sviluppo Econ Sostenibile ENEA, Bologna, Italy. [Milazzo, P. M.] Ist Nazl Fis Nucl, Trieste, Italy. [Mirea, M.; Roman, F.] Horia Hulubei Natl Inst Phys & Nucl Engn, IFIN HH, Bucharest, Romania. [Mondalaers, W.; Plompen, A.; Schillebeeckx, P.] European Commiss JRC, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rubbia, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. RP Tarrio, D (reprint author), Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. EM dtarriov@gmail.com RI Calvino, Francisco/K-5743-2014; Rauscher, Thomas/D-2086-2009; Mirea, Mihail/C-2297-2011; Cano Ott, Daniel/K-4945-2014; Gonzalez Romero, Enrique/L-7561-2014; Duran, Ignacio/H-7254-2015; Massimi, Cristian/K-2008-2015; Paradela, Carlos/J-1492-2012; Chin, Mary Pik Wai/B-6644-2012; Mendoza Cembranos, Emilio/K-5789-2014; Becares, Vicente/K-4514-2014; Martinez, Trinitario/K-6785-2014; Langer, Christoph/L-3422-2016; Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012; OI Calvino, Francisco/0000-0002-7198-4639; Rauscher, Thomas/0000-0002-1266-0642; Mirea, Mihail/0000-0002-9333-6595; Cano Ott, Daniel/0000-0002-9568-7508; Gonzalez Romero, Enrique/0000-0003-2376-8920; Massimi, Cristian/0000-0003-2499-5586; Chin, Mary Pik Wai/0000-0001-5176-9723; Mendoza Cembranos, Emilio/0000-0002-2843-1801; Becares, Vicente/0000-0003-3434-9086; Martinez, Trinitario/0000-0002-0683-5506; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038; Tarrio, Diego/0000-0002-9858-3341; Garcia Rios, Aczel Regino/0000-0002-7955-1475 NR 8 TC 8 Z9 8 U1 3 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 35 EP 37 DI 10.1016/j.nds.2014.08.011 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200127 ER PT J AU Leal-Cidoncha, E Duran, I Paradela, C Tarrio, D Leong, LS Audouin, L Tassan-Got, L Praena, J Berthier, B Ferrant, L Isaev, S Le Naour, C Stephan, C Trubert, D Abbondanno, U Aerts, G Alvarez, H Alvarez-Velarde, F Andriamonje, S Andrzejewski, J Badurek, G Baumann, P Becvar, F Berthoumieux, E Calvino, F Calviani, M Cano-Ott, D Capote, R Carrapico, C Cennini, P Chepel, V Chiaveri, E Colonna, N Cortes, G Couture, A Cox, J Dahlfors, M David, S Dillmann, I Domingo-Pardo, C Dridi, W Eleftheriadis, C Embid-Segura, M Ferrari, A Ferreira-Marques, R Fujii, K Furman, W Goncalves, I Gonzalez-Romero, E Gramegna, F Guerrero, C Gunsing, F Haas, B Haight, R Heil, M Herrera-Martinez, A Igashira, M Jericha, E Kadi, Y Kappeler, F Karadimos, D Kerveno, M Koehler, P Kossionides, E Krticka, M Lampoudis, C Leeb, H Lindote, A Lopes, I Lozano, M Lukic, S Marganiec, J Marrone, S Martinez, T Massimi, C Mastinu, P Mengoni, A Milazzo, PM Moreau, C Mosconi, M Neves, F Oberhummer, H O'Brien, S Oshima, M Pancin, J Papadopoulos, C Pavlik, A Pavlopoulos, P Perrot, L Pigni, MT Plag, R Plompen, A Plukis, A Poch, A Pretel, C Quesada, J Rauscher, T Reifarth, R Rubbia, C Rudolf, G Rullhusen, P Salgado, J Santos, C Sarchiapone, L Savvidis, I Tagliente, G Tain, JL Tavora, L Terlizzi, R Vannini, G Vaz, P Ventura, A Villamarin, D Vincente, MC Vlachoudis, V Vlastou, R Voss, F Walter, S Wiescher, M Wisshak, K AF Leal-Cidoncha, E. Duran, I. Paradela, C. Tarrio, D. Leong, L. S. Audouin, L. Tassan-Got, L. Praena, J. Berthier, B. Ferrant, L. Isaev, S. Le Naour, C. Stephan, C. Trubert, D. Abbondanno, U. Aerts, G. Alvarez, H. Alvarez-Velarde, F. Andriamonje, S. Andrzejewski, J. Badurek, G. Baumann, P. Becvar, F. Berthoumieux, E. Calvino, F. Calviani, M. Cano-Ott, D. Capote, R. Carrapico, C. Cennini, P. Chepel, V. Chiaveri, E. Colonna, N. Cortes, G. Couture, A. Cox, J. Dahlfors, M. David, S. Dillmann, I. Domingo-Pardo, C. Dridi, W. Eleftheriadis, C. Embid-Segura, M. Ferrari, A. Ferreira-Marques, R. Fujii, K. Furman, W. Goncalves, I. Gonzalez-Romero, E. Gramegna, F. Guerrero, C. Gunsing, F. Haas, B. Haight, R. Heil, M. Herrera-Martinez, A. Igashira, M. Jericha, E. Kadi, Y. Kappeler, F. Karadimos, D. Kerveno, M. Koehler, P. Kossionides, E. Krticka, M. Lampoudis, C. Leeb, H. Lindote, A. Lopes, I. Lozano, M. Lukic, S. Marganiec, J. Marrone, S. Martinez, T. Massimi, C. Mastinu, P. Mengoni, A. Milazzo, P. M. Moreau, C. Mosconi, M. Neves, F. Oberhummer, H. O'Brien, S. Oshima, M. Pancin, J. Papadopoulos, C. Pavlik, A. Pavlopoulos, P. Perrot, L. Pigni, M. T. Plag, R. Plompen, A. Plukis, A. Poch, A. Pretel, C. Quesada, J. Rauscher, T. Reifarth, R. Rubbia, C. Rudolf, G. Rullhusen, P. Salgado, J. Santos, C. Sarchiapone, L. Savvidis, I. Tagliente, G. Tain, J. L. Tavora, L. Terlizzi, R. Vannini, G. Vaz, P. Ventura, A. Villamarin, D. Vincente, M. C. Vlachoudis, V. Vlastou, R. Voss, F. Walter, S. Wiescher, M. Wisshak, K. TI Study of U-234(n,f) Resonances Measured at the CERN n_TOF Facility SO NUCLEAR DATA SHEETS LA English DT Article ID CROSS-SECTIONS; NUCLEAR-DATA AB We present the analysis of the resolved resonance region for the U-234(n,f) cross section data measured at the CERN n_TOF facility. The resonance parameters in the energy range from 1 eV to 1500 eV have been obtained with the SAMMY code by using as initial parameters for the fit the resonance parameters of the JENDL-3.3 evaluation. In addition, the statistical analysis has been accomplished, partly with the SAMDIST code, in order to study the level spacing and the Mehta-Dyson correlation. C1 [Leal-Cidoncha, E.; Duran, I.; Paradela, C.; Tarrio, D.; Alvarez, H.] Univ Santiago de Compostela, Santiago De Compostela, Spain. [Leong, L. S.; Audouin, L.; Tassan-Got, L.; Berthier, B.; Ferrant, L.; Isaev, S.; Le Naour, C.; Stephan, C.; Trubert, D.; Dillmann, I.] IPN, CNRS, IN2P3, Orsay, France. [Praena, J.; Capote, R.; Lozano, M.; Quesada, J.] Univ Seville, Seville, Spain. [Abbondanno, U.; Fujii, K.; Milazzo, P. M.; Moreau, C.] Ist Nazl Fis Nucl, Trieste, Italy. [Aerts, G.] CEA Saclay, IRFU, F-91191 Gif Sur Yvette, France. [Alvarez-Velarde, F.; Cano-Ott, D.; Embid-Segura, M.; Gonzalez-Romero, E.; Guerrero, C.; Martinez, T.; Villamarin, D.; Vincente, M. C.] Ctr Invest Energet Medioambientales & Tecnol, Madrid, Spain. [Andriamonje, S.; Berthoumieux, E.; Carrapico, C.; Eleftheriadis, C.; Gunsing, F.; Pancin, J.; Perrot, L.; Plukis, A.] CEA Saclay, DSM, DAPNIA, F-91191 Gif Sur Yvette, France. [Andrzejewski, J.; Marganiec, J.] Univ Lodz, PL-90131 Lodz, Poland. [Badurek, G.; Jericha, E.; Leeb, H.; Oberhummer, H.; Pigni, M. T.] Vienna Univ Technol, Atominst Osterreich Univ, Vienna, Austria. [Baumann, P.; Kerveno, M.; Lukic, S.; Rudolf, G.] CNRS, IN2P3, IReS, Strasbourg, France. [Becvar, F.; Krticka, M.] Charles Univ Prague, Prague, Czech Republic. [Calvino, F.; Cortes, G.; Poch, A.; Pretel, C.] Univ Politecn Cataluna, Barcelona, Spain. [Calviani, M.; Gramegna, F.; Mastinu, P.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Calviani, M.] Univ Padua, Dipartimento Fis, I-35100 Padua, Italy. [Capote, R.; Mengoni, A.] IAEA, Nucl Data Sect, A-1400 Vienna, Austria. [Carrapico, C.; Goncalves, I.; Salgado, J.; Santos, C.; Tavora, L.; Vaz, P.] Inst Tecnol Nucl, Lisbon, Portugal. [Chepel, V.; Ferreira-Marques, R.; Lindote, A.; Lopes, I.; Neves, F.] CERN, Geneva, Switzerland. [Chepel, V.; Ferreira-Marques, R.; Lindote, A.; Lopes, I.; Neves, F.] Univ Coimbra, LIP Coimbra, P-3000 Coimbra, Portugal. [Chepel, V.; Ferreira-Marques, R.; Lindote, A.; Lopes, I.; Neves, F.] Univ Coimbra, Dept Fis, P-3000 Coimbra, Portugal. [Colonna, N.; Marrone, S.; Tagliente, G.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Couture, A.; Cox, J.; Dahlfors, M.; O'Brien, S.; Wiescher, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Domingo-Pardo, C.; Heil, M.; Kappeler, F.; Mosconi, M.; Plag, R.; Voss, F.; Walter, S.; Wisshak, K.] Forschungszentrum Karlsruhe GmbH FZK, Inst Kernphys, Karlsruhe, Germany. [Dridi, W.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46003 Valencia, Spain. [Lampoudis, C.; Savvidis, I.] Aristotle Univ Thessaloniki, Thessaloniki, Greece. [Furman, W.] Joint Inst Nucl Res, Frank Lab Neutron Phys, Dubna, Russia. [Haas, B.] CNRS, IN2P3, CENBG, Bordeaux, France. [Haight, R.; Reifarth, R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Igashira, M.] Tokyo Inst Technol, Tokyo 152, Japan. [Karadimos, D.; Papadopoulos, C.; Vlastou, R.] Natl Tech Univ Athens, GR-10682 Athens, Greece. [Koehler, P.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Kossionides, E.] NCSR, Athens, Greece. [Massimi, C.; Vannini, G.] Univ Bologna, Dipartimento Fis, I-40126 Bologna, Italy. [Massimi, C.; Pavlik, A.; Vannini, G.] Sez INFN Bologna, Bologna, Italy. [Oshima, M.; Pavlik, A.] Japan Atom Energy Res Inst, Tokai, Ibaraki 31911, Japan. [Pavlik, A.] Univ Vienna, Fac Phys, A-1010 Vienna, Austria. [Plompen, A.; Rullhusen, P.] CEC JRC IRMM, Geel, Belgium. RP Leal-Cidoncha, E (reprint author), Univ Santiago de Compostela, Santiago De Compostela, Spain. EM esther.leal@rai.usc.es RI Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012; Paradela, Carlos/J-1492-2012; Capote Noy, Roberto/M-1245-2014; Martinez, Trinitario/K-6785-2014; Calvino, Francisco/K-5743-2014; Vaz, Pedro/K-2464-2013; Rauscher, Thomas/D-2086-2009; Cano Ott, Daniel/K-4945-2014; Gonzalez Romero, Enrique/L-7561-2014; Duran, Ignacio/H-7254-2015; Alvarez Pol, Hector/F-1930-2011; Massimi, Cristian/K-2008-2015 OI Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038; Pavlik, Andreas/0000-0001-7526-3372; Tarrio, Diego/0000-0002-9858-3341; Capote Noy, Roberto/0000-0002-1799-3438; Martinez, Trinitario/0000-0002-0683-5506; Calvino, Francisco/0000-0002-7198-4639; Vaz, Pedro/0000-0002-7186-2359; Rauscher, Thomas/0000-0002-1266-0642; Cano Ott, Daniel/0000-0002-9568-7508; Gonzalez Romero, Enrique/0000-0003-2376-8920; Alvarez Pol, Hector/0000-0001-9643-6252; Massimi, Cristian/0000-0003-2499-5586 NR 9 TC 3 Z9 3 U1 4 U2 12 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 42 EP 44 DI 10.1016/j.nds.2014.08.013 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200129 ER PT J AU Mendoza, E Cano-Ott, D Guerrero, C Altstadt, S Andrzejewski, J Audouin, L Barbagallo, M Becares, V Becvar, F Belloni, F Berthoumieux, E Billowes, J Boccone, V Bosnar, D Brugger, M Calviani, M Calvino, F Carrapico, C Cerutti, F Chiaveri, E Chin, M Colonna, N Cortes, G Cortes-Giraldo, MA Diakaki, M Domingo-Pardo, C Duran, I Dressler, R Dzysiuk, N Eleftheriadis, C Ferrari, A Fraval, K Ganesan, S Garcia, AR Giubrone, G Gomez-Hornillos, MB Goncalves, IF Gonzalez-Romero, E Griesmayer, E Gunsing, F Gurusamy, P Jenkins, DG Jericha, E Kadi, Y Kappeler, F Karadimos, D Kivel, N Koehler, P Kokkoris, M Korschinek, G Krticka, M Kroll, J Langer, C Lederer, C Leeb, H Leong, LS Losito, R Manousos, A Marganiec, J Martinez, T Mastinu, PF Mastromarco, M Massimi, C Meaze, M Mengoni, A Milazzo, PM Mingrone, F Mirea, M Mondelaers, W Paradela, C Pavlik, A Perkowski, J Pignatari, M Plompen, A Praena, J Quesada, JM Rauscher, T Reifarth, R Riego, A Roman, F Rubbia, C Sarmento, R Schillebeeckx, P Schmidt, S Schumann, D Tagliente, G Tain, JL Tarrio, D Tassan-Got, L Tsinganis, A Valenta, S Vannini, G Variale, V Vaz, P Ventura, A Versaci, R Vermeulen, MJ Vlachoudis, V Vlastou, R Wallner, A Ware, T Weigand, M Weiss, C Wright, TJ Zugec, P AF Mendoza, E. Cano-Ott, D. Guerrero, C. Altstadt, S. Andrzejewski, J. Audouin, L. Barbagallo, M. Becares, V. Becvar, F. Belloni, F. Berthoumieux, E. Billowes, J. Boccone, V. Bosnar, D. Brugger, M. Calviani, M. Calvino, F. Carrapico, C. Cerutti, F. Chiaveri, E. Chin, M. Colonna, N. Cortes, G. Cortes-Giraldo, M. A. Diakaki, M. Domingo-Pardo, C. Duran, I. Dressler, R. Dzysiuk, N. Eleftheriadis, C. Ferrari, A. Fraval, K. Ganesan, S. Garcia, A. R. Giubrone, G. Gomez-Hornillos, M. B. Goncalves, I. F. Gonzalez-Romero, E. Griesmayer, E. Gunsing, F. Gurusamy, P. Jenkins, D. G. Jericha, E. Kadi, Y. Kaeppeler, F. Karadimos, D. Kivel, N. Koehler, P. Kokkoris, M. Korschinek, G. Krticka, M. Kroll, J. Langer, C. Lederer, C. Leeb, H. Leong, L. S. Losito, R. Manousos, A. Marganiec, J. Martinez, T. Mastinu, P. F. Mastromarco, M. Massimi, C. Meaze, M. Mengoni, A. Milazzo, P. M. Mingrone, F. Mirea, M. Mondelaers, W. Paradela, C. Pavlik, A. Perkowski, J. Pignatari, M. Plompen, A. Praena, J. Quesada, J. M. Rauscher, T. Reifarth, R. Riego, A. Roman, F. Rubbia, C. Sarmento, R. Schillebeeckx, P. Schmidt, S. Schumann, D. Tagliente, G. Tain, J. L. Tarrio, D. Tassan-Got, L. Tsinganis, A. Valenta, S. Vannini, G. Variale, V. Vaz, P. Ventura, A. Versaci, R. Vermeulen, M. J. Vlachoudis, V. Vlastou, R. Wallner, A. Ware, T. Weigand, M. Weiss, C. Wright, T. J. Zugec, P. TI Measurement of the Am-241 and the Am-243 Neutron Capture Cross Sections at the n_TOF Facility at CERN SO NUCLEAR DATA SHEETS LA English DT Article ID NUCLEAR-DATA LIBRARY; TOTAL ABSORPTION CALORIMETER; SCIENCE; TECHNOLOGY AB The capture cross sections of Am-241 and Am-243 were measured at the n_TOF facility at CERN in the epithermal energy range with a BaF2 Total Absorption Calorimeter. A preliminary analysis of the Am-241 and a complete analysis of the Am-243 measurement, including the data reduction and the resonance analysis, have been performed. C1 [Mendoza, E.; Cano-Ott, D.; Becares, V.; Garcia, A. R.; Gonzalez-Romero, E.; Martinez, T.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Guerrero, C.; Berthoumieux, E.; Boccone, V.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Ferrari, A.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Tsinganis, A.; Versaci, R.; Vlachoudis, V.] European Org Nucl Res CERN, Geneva, Switzerland. [Altstadt, S.; Langer, C.; Lederer, C.; Reifarth, R.; Schmidt, S.; Weigand, M.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Andrzejewski, J.; Marganiec, J.; Perkowski, J.] Uniwersytet Lodzki, Lodz, Poland. [Audouin, L.; Leong, L. S.; Tassan-Got, L.] IPN, IN2P3, Ctr Natl Rech Sci, Orsay, France. [Barbagallo, M.; Colonna, N.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Becvar, F.; Krticka, M.; Kroll, J.; Valenta, S.] Charles Univ Prague, Prague, Czech Republic. [Belloni, F.; Berthoumieux, E.; Chiaveri, E.; Fraval, K.; Gunsing, F.] Commissariat Energie Atom CEA Saclay Irfu, Gif Sur Yvette, France. [Billowes, J.; Ware, T.; Wright, T. J.] Univ Manchester, Manchester, Lancs, England. [Bosnar, D.; Zugec, P.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia. [Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, Barcelona, Spain. [Carrapico, C.; Goncalves, I. F.; Sarmento, R.; Vaz, P.] Univ Tecn Lisboa, Inst Super Tecn, Inst Tecnol & Nucl, P-1096 Lisbon, Portugal. [Cortes-Giraldo, M. A.; Praena, J.; Quesada, J. M.] Univ Seville, Seville, Spain. [Diakaki, M.; Karadimos, D.; Kokkoris, M.; Vlastou, R.] Natl Tech Univ Athens, GR-10682 Athens, Greece. [Domingo-Pardo, C.; Giubrone, G.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46003 Valencia, Spain. [Duran, I.; Paradela, C.; Tarrio, D.] Univ Santiago de Compostela, Santiago De Compostela, Spain. [Dressler, R.; Kivel, N.; Schumann, D.] Paul Scherrer Inst, Villigen, Switzerland. [Dzysiuk, N.; Mastinu, P. F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Eleftheriadis, C.; Manousos, A.] Aristotle Univ Thessaloniki, GR-54006 Thessaloniki, Greece. [Ganesan, S.; Gurusamy, P.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Griesmayer, E.; Jericha, E.; Leeb, H.; Weiss, C.] Vienna Univ Technol, Atominst, Vienna, Austria. [Jenkins, D. G.; Vermeulen, M. J.] Univ York, York YO10 5DD, N Yorkshire, England. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Koehler, P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Korschinek, G.] Tech Univ Munich, D-80290 Munich, Germany. [Lederer, C.; Pavlik, A.; Wallner, A.] Univ Vienna, Fac Phys, Vienna, Austria. [Massimi, C.; Mingrone, F.; Vannini, G.] Univ Bologna, Dipartimento Fis, I-40126 Bologna, Italy. [Massimi, C.; Mingrone, F.; Vannini, G.] Sez INFN Bologna, Bologna, Italy. [Mengoni, A.; Ventura, A.] Agenzia Nazl Nuove Tecnol, Energia Sviluppo Econ Sostenibile ENEA, Bologna, Italy. [Milazzo, P. M.] Ist Nazl Fis Nucl, Trieste, Italy. [Mirea, M.; Roman, F.] Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HH, Bucharest, Romania. [Mondelaers, W.; Plompen, A.; Schillebeeckx, P.] European Commiss JRC, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Pignatari, M.; Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rubbia, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. RP Mendoza, E (reprint author), Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. EM emilio.mendoza@ciemat.es RI Calvino, Francisco/K-5743-2014; Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012; Langer, Christoph/L-3422-2016; Rauscher, Thomas/D-2086-2009; Mirea, Mihail/C-2297-2011; Cano Ott, Daniel/K-4945-2014; Gonzalez Romero, Enrique/L-7561-2014; Duran, Ignacio/H-7254-2015; Massimi, Cristian/K-2008-2015; Paradela, Carlos/J-1492-2012; Chin, Mary Pik Wai/B-6644-2012; Mendoza Cembranos, Emilio/K-5789-2014; Becares, Vicente/K-4514-2014; Martinez, Trinitario/K-6785-2014 OI Calvino, Francisco/0000-0002-7198-4639; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038; Tarrio, Diego/0000-0002-9858-3341; Rauscher, Thomas/0000-0002-1266-0642; Mirea, Mihail/0000-0002-9333-6595; Cano Ott, Daniel/0000-0002-9568-7508; Gonzalez Romero, Enrique/0000-0003-2376-8920; Massimi, Cristian/0000-0003-2499-5586; Chin, Mary Pik Wai/0000-0001-5176-9723; Mendoza Cembranos, Emilio/0000-0002-2843-1801; Becares, Vicente/0000-0003-3434-9086; Martinez, Trinitario/0000-0002-0683-5506 FU ENRESA under the CIEMAT-ENRESA agreement on "Transmutation of high level radioactive waste"; Spanish Plan on Nuclear and Particle Physics of the Spanish Ministry of Science and Innovation [FPA2005-06918-C03-01]; European Commission 6th Framework Programme project IP-EUROTRANS [F16W-CT-2004-516520]; CONSOLIDER-INGENIO project [CSD-2007-00042] FX This work has been supported by ENRESA under the CIEMAT-ENRESA agreement on "Transmutation of high level radioactive waste", by the Spanish Plan on Nuclear and Particle Physics of the Spanish Ministry of Science and Innovation (project FPA2005-06918-C03-01), the European Commission 6th Framework Programme project IP-EUROTRANS (F16W-CT-2004-516520) and the CONSOLIDER-INGENIO project CSD-2007-00042. NR 20 TC 4 Z9 4 U1 2 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 65 EP 68 DI 10.1016/j.nds.2014.08.020 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200136 ER PT J AU Firestone, RB Abusaleem, K Basunia, MS Becvar, F Belgya, T Bernstein, LA Choi, HD Escher, JE Genreith, C Hurst, AM Krticka, M Renne, PR Revay, Z Rogers, AM Rossbach, M Siem, S Sleaford, B Summers, NC Szentmiklosi, L van Bibber, K Wiedeking, M AF Firestone, R. B. Abusaleem, K. Basunia, M. S. Becvar, F. Belgya, T. Bernstein, L. A. Choi, H. D. Escher, J. E. Genreith, C. Hurst, A. M. Krticka, M. Renne, P. R. Revay, Zs. Rogers, A. M. Rossbach, M. Siem, S. Sleaford, B. Summers, N. C. Szentmiklosi, L. van Bibber, K. Wiedeking, M. TI EGAF: Measurement and Analysis of Gamma-ray Cross Sections SO NUCLEAR DATA SHEETS LA English DT Article ID RESONANCE INTEGRALS; NEUTRON; CAPTURE; PROBABILITY; DIFFUSION; GRAPHITE; ELEMENTS; K-42 AB The Evaluated Gamma-ray Activation File (EGAF) is the result of a 2000-2007 IAEA Coordinated Research Project to develop a database of thermal, prompt gamma-ray cross sections, sigma(gamma), for all elemental and selected radioactive targets. No previous database of this kind had existed. EGAF was originally based on measurements using guided neutron beams from the Budapest Reactor on all elemental targets from Z=1-82, 90 and 92, except for He and Pm. The EGAF sigma(gamma) data were published in the Database of Prompt Gamma Rays from Slow Neutron Capture for Elemental Analysis [1]. An international collaboration has formed to continue the EGAF measurements with isotopically enriched targets, derive total radiative thermal neutron cross sections, sigma(0), extend the sigma(gamma) data from thermal to 20 MeV neutrons, compile a completed activation data file, improve sections of the Reference Input Parameter Library (RIPL) with more complete and up to date level and gamma-ray data, evaluate statistical gamma-ray data from reaction studies, and determine recommended neutron separations energies, S-n, for atomic mass evaluations. A new guided neutron beam facility has become available at the Garching (Munich) FRM II Reactor, and high energy neutron experimental facilities are being developed by a Berkeley area collaboration where 5-33 MeV neutron beams are available at the LBNL 88" cyclotron, 2.5 and 14 MeV beams at the University of California, Berkeley neutron generator laboratory, and high flux, 10(27-33) n.cm(-2).s(-1), neutron pulses available from the LLNL National Ignition Facility (NIF). C1 [Firestone, R. B.; Basunia, M. S.; Hurst, A. M.; Rogers, A. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Abusaleem, K.] Univ Jordan, Jordan Atom Energy Commiss, Amman 11942, Jordan. [Abusaleem, K.] Univ Jordan, Dept Phys, Amman 11942, Jordan. [Becvar, F.; Krticka, M.] Charles Univ Prague, CZ-18000 Prague 8, Czech Republic. [Belgya, T.; Szentmiklosi, L.] Hungarian Acad Sci, Energy Res Ctr, H-1525 Budapest, Hungary. [Bernstein, L. A.; Escher, J. E.; Sleaford, B.; Summers, N. C.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Choi, H. D.] Seoul Natl Univ, Seoul 151744, South Korea. [Genreith, C.; Rossbach, M.] Forschungszentrum Julich, Inst Energy & Climate Res Nucl Waste Management &, D-52425 Julich, Germany. [Renne, P. R.] Berkeley Geochronol Ctr, Berkeley, CA 94709 USA. [Revay, Zs.] Tech Univ Munich, Forsch Neutronenquelle Heinz Maier Leibnitz FRM 2, D-80290 Munich, Germany. [Siem, S.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. [van Bibber, K.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Wiedeking, M.] iThemba LABS, ZA-7129 Somerset West, South Africa. RP Firestone, RB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM rbfirestone@lbl.gov RI Szentmiklosi, Laszlo/F-5362-2015; OI Szentmiklosi, Laszlo/0000-0001-7747-8545; Rossbach, Matthias/0000-0002-4342-743X FU U. S. Department of Energy [DE-AC52-07NA27344, DE-AC02-05CH11231]; University of California Office of the President (U.C.-Berkeley); Ministry of Education of the Czech Republic [MSM 0021620859]; Czech Science Foundation [13-07117S]; NAP-VENEUS of Hungary [OMFB-001842006]; National Research Foundation of South Africa FX This work was performed under the auspices of the U. S. Department of Energy Contracts DE-AC52-07NA27344 (Lawrence Livermore National Laboratory), DE-AC02-05CH11231 (Lawrence Berkeley National Laboratory) and the University of California Office of the President (U.C.-Berkeley). Additional support was provided by the research plan MSM 0021620859 of the Ministry of Education of the Czech Republic, by the Czech Science Foundation under Grant No. 13-07117S, by NAP-VENEUS Contract No. OMFB-001842006 of Hungary, and by the National Research Foundation of South Africa. NR 42 TC 0 Z9 0 U1 2 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 79 EP 87 DI 10.1016/j.nds.2014.08.024 PG 9 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200140 ER PT J AU Basunia, MS Firestone, RB Revay, Z Choi, HD Belgya, T Escher, JE Hurst, AM Krticka, M Szentmiklosi, L Sleaford, B Summers, NC AF Basunia, M. S. Firestone, R. B. Revay, Zs. Choi, H. D. Belgya, T. Escher, J. E. Hurst, A. M. Krticka, M. Szentmiklosi, L. Sleaford, B. Summers, N. C. TI Determination of the Eu-151(n,gamma) Eu-152m1,Eu-g and Eu-153(n,gamma) Eu-154 Reaction Cross Sections at Thermal Neutron Energy SO NUCLEAR DATA SHEETS LA English DT Article ID ACTIVATION AB We have measured partial gamma-ray cross sections following neutron capture in enriched Eu-151 and Eu-153 targets at the cold-neutron-beam facility of the Budapest Research Reactor. The cross sections were standardized using a stoichiometric (EuCl3)-Eu-nat target with the well-known 1951-keV gamma-ray cross section from the Cl-35(n,gamma) Cl-36 reaction at the cold-neutron-beam facility of the Garching Research Reactor. The gamma-ray cross sections were corrected for effective g-factors. These data were combined with the structural information of Eu-152 and Eu-154 given in the Evaluated Nuclear Structure Data File to produce capture gamma-ray level schemes. The total radiative capture cross sections of the Eu-151(n,gamma) Eu-152m1,Eu- g and Eu-153(n,gamma) 154 Eu reactions were determined by summing the experimental transition intensities from known levels with simulated intensities of transitions from higher excitations to the ground- or metastable-state. The individual Eu-151(n,gamma) Eu-152m1 and Eu-151(n,gamma) Eu-152g reaction cross sections disagree with values in the literature. However, the total cross section of the Eu-151(n,gamma) Eu-152 reaction does agree with those values. Also, our deduced cross section for the Eu-153(n,gamma) Eu-154 reaction closely follows the data in the literature. These results are supported by an earlier standardization experiment done at the Budapest Research Reactor using a target of Eu2O3 solution in H2SO4. C1 [Basunia, M. S.; Firestone, R. B.; Hurst, A. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Revay, Zs.] Tech Univ Munich, D-80290 Munich, Germany. [Choi, H. D.] Seoul Natl Univ, Seoul 151, South Korea. [Belgya, T.; Szentmiklosi, L.] HAS, Energy Res Ctr, Budapest, Hungary. [Escher, J. E.; Sleaford, B.; Summers, N. C.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Krticka, M.] Charles Univ Prague, Prague, Czech Republic. RP Basunia, MS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM SBasunia@lbl.gov RI Szentmiklosi, Laszlo/F-5362-2015 OI Szentmiklosi, Laszlo/0000-0001-7747-8545 FU U.S. Department of Energy of Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; NAP VENEUS OMFB [00184/2006]; plan MSM of the Ministry of Education of the Czech Republic [0021620859]; Czech Science Foundation [13-07117S] FX We wish to thank Dr. E. Browne for enlightening discussions during this work and for reading the manuscript. This work was performed under the auspices of the U.S. Department of Energy of Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231, and for Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, supported by NAP VENEUS OMFB 00184/2006, by the plan MSM 0021620859 of the Ministry of Education of the Czech Republic and by the Czech Science Foundation under Grant No. 13-07117S. NR 16 TC 2 Z9 2 U1 2 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 88 EP 90 DI 10.1016/j.nds.2014.08.025 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200141 ER PT J AU Hurst, AM Firestone, RB Szentmiklosi, L Revay, Z Basunia, MS Belgya, T Escher, JE Krticka, M Summers, NC Sleaford, BW AF Hurst, A. M. Firestone, R. B. Szentmiklosi, L. Revay, Zs. Basunia, M. S. Belgya, T. Escher, J. E. Krticka, M. Summers, N. C. Sleaford, B. W. TI New Measurement of the Thermal-capture Cross Section for the Minor Isotope W-180 SO NUCLEAR DATA SHEETS LA English DT Article ID GAMMA ACTIVATION-ANALYSIS; NUCLEAR-DATA AB Tungsten occurs naturally in five isotopic forms; four of them, 182,183,184,186 W, contribute significantly to the overall elemental abundance (with each contribution between 14 and 30 %), whereas 180 W only occurs at the 0.12 % level and is a minor isotope. Given its very low abundance, a precise measurement of the thermal neutron-capture cross section is extremely challenging. This work reports a new value of the thermal neutron-capture cross section from a direct W-180(n,gamma) measurement using a guided-thermal beam at the Budapest Research Reactor, incident upon an 11.35 % enriched sample to induce prompt gamma-ray activation within the sample. The thermal-capture cross section was determined as the sum of experimentally observed partial neutron-capture gamma-ray cross sections feeding the ground state directly, and, the modeled contribution from the (unobserved) ground-state feeding predicted from statistical-model calculations using the Monte Carlo program DICEBOX. The preliminary value of the W-180(n,gamma) thermal neutron-capture cross section is 20.5(42) b. C1 [Hurst, A. M.; Firestone, R. B.; Basunia, M. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Szentmiklosi, L.; Belgya, T.] Hungarian Acad Sci, Energy Res Ctr, H-1525 Budapest, Hungary. [Revay, Zs.] Tech Univ Munich, Forschunsneutronenquelle Heinz Maier Leibnitz FRM, Garching, Germany. [Escher, J. E.; Summers, N. C.; Sleaford, B. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Krticka, M.] Charles Univ Prague, Fac Math & Phys, CZ-18000 Prague, Czech Republic. RP Hurst, AM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM AMHurst@lbl.gov RI Szentmiklosi, Laszlo/F-5362-2015 OI Szentmiklosi, Laszlo/0000-0001-7747-8545 FU Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; U. S. Department of Energy by Lawrence Livermore National Laboratory [AC52-07NA27344]; NAP [VENEUS08, OMFB-00184/2006]; Ministry of Education of the Czech Republic [MSM 0021620859]; [13-07117S] FX This work was performed under the auspices of the University of California, supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy at Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231, the U. S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Access to the Budapest PGAA facility was supported by the NAP VENEUS08 grant under Contract OMFB-00184/2006. This work was also supported by the research plan MSM 0021620859 of the Ministry of Education of the Czech Republic and by the Czech Science Foundation under Grant No. 13-07117S. NR 23 TC 0 Z9 0 U1 1 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 91 EP 93 DI 10.1016/j.nds.2014.08.026 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200142 ER PT J AU Schillebeeckx, P Becker, B Capote, R Emiliani, F Guber, K Heyse, J Kauwenberghs, K Kopecky, S Lampoudis, C Massimi, C Mondelaers, W Moxon, M Noguere, G Plompen, AJM Pronyaev, V Siegler, P Sirakov, I Trkov, A Volev, K Zerovnik, G AF Schillebeeckx, P. Becker, B. Capote, R. Emiliani, F. Guber, K. Heyse, J. Kauwenberghs, K. Kopecky, S. Lampoudis, C. Massimi, C. Mondelaers, W. Moxon, M. Noguere, G. Plompen, A. J. M. Pronyaev, V. Siegler, P. Sirakov, I. Trkov, A. Volev, K. Zerovnik, G. TI Evaluation of Neutron Resonance Cross Section Data at GELINA SO NUCLEAR DATA SHEETS LA English DT Article ID NUCLEAR-DATA; COVARIANCES; LIBRARY; SCIENCE; REGION AB Over the last decade, the EC-JRC-IRMM, in collaboration with other institutes such as INRNE Sofia (BG), INFN Bologna (IT), ORNL (USA), CEA Cadarache (FR) and CEA Saclay (FR), has made an intense effort to improve the quality of neutron-induced cross section data in the resonance region. These improvements relate to both the infrastructure of the facility and the measurement setup, and the data reduction and analysis procedures. As a result total and reaction cross section data in the resonance region with uncertainties better than 0.5 % and 2 %, respectively, can be produced together with evaluated data files for both the resolved and unresolved resonance region. The methodology to produce full ENDF compatible files, including covariances, is illustrated by the production of resolved resonance parameter files for Am-241, Cd and W and an evaluation for Au-197 in the unresolved resonance region. C1 [Schillebeeckx, P.; Becker, B.; Emiliani, F.; Heyse, J.; Kauwenberghs, K.; Kopecky, S.; Lampoudis, C.; Mondelaers, W.; Plompen, A. J. M.; Siegler, P.; Sirakov, I.; Volev, K.; Zerovnik, G.] EC JRC IRMM, B-2440 Geel, Belgium. [Capote, R.] IAEA, A-1400 Vienna, Austria. [Guber, K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Massimi, C.] Univ Bologna, I-40126 Bologna, Italy. [Massimi, C.] Sez INFN Bologna, I-40126 Bologna, Italy. [Moxon, M.] Hyde Copse 3, Marcham, Oxon, England. [Noguere, G.] CEN Cadarache, DEN, F-13108 St Paul Les Durance, France. [Pronyaev, V.] Inst Phys & Power Engn, Obninsk 249033, Russia. [Sirakov, I.; Volev, K.] Inst Nucl Energy Res, Sofia, Bulgaria. [Trkov, A.; Zerovnik, G.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. RP Schillebeeckx, P (reprint author), EC JRC IRMM, Retieseweg 111, B-2440 Geel, Belgium. EM peter.schillebeeckx@ec.europa.eu RI Massimi, Cristian/K-2008-2015; Capote Noy, Roberto/M-1245-2014; OI Massimi, Cristian/0000-0003-2499-5586; Capote Noy, Roberto/0000-0002-1799-3438; Becker, Bjorn/0000-0001-6821-1873 FU Nuclear Energy Agency of the OECD; European Commission through the EUFRAT project [FP7-21499] FX We are grateful to the Nuclear Energy Agency of the OECD for their interest and support to our work. The work program at GELINA was partly supported by the European Commission through the EUFRAT project (FP7-21499). The authors are grateful to the GELINA technical staff. NR 24 TC 5 Z9 5 U1 2 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 94 EP 97 DI 10.1016/j.nds.2014.08.027 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200143 ER PT J AU Massey, TN Ralston, J Grimes, SM Haight, RC AF Massey, T. N. Ralston, J. Grimes, S. M. Haight, R. C. TI B-10(n, Z) Measurements in the Energy Range 0.7 to 5.0 MeV SO NUCLEAR DATA SHEETS LA English DT Article ID CROSS-SECTION; B-10(N,ALPHA)LI-7 REACTION; NEUTRONS; STATES; B-11 AB Four Delta E E telescopes were used at the WNR (n,Z) station to investigate the production of charged particles from B-10. The telescope consisted of a gas proportional detector and a silicon surface barrier detector. The flux was determined using a U-235 fission chamber. A clear separation of the ground state alpha group and first excited state was not achieved due to the target thickness. Proton emission was also observed. The proton branch was up to an order of magnitude larger than predicted in ENDF/B-VII. A simple R-matrix analysis has been performed on the available data. C1 [Massey, T. N.; Ralston, J.; Grimes, S. M.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Haight, R. C.] Los Alamos Neutron Sci Ctr, Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Massey, TN (reprint author), Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. EM massey@ohio.edu OI Massey, Thomas/0000-0002-5578-5357 FU US Department of Energy by Los Alamos National Security, LLC [DE-AC52-06NA25396] FX This work benefited from the use of the LANSCE accelerator facility and was performed under the auspices of the US Department of Energy by Los Alamos National Security, LLC under contract DE-AC52-06NA25396. NR 14 TC 1 Z9 1 U1 2 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 107 EP 109 DI 10.1016/j.nds.2014.08.030 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200146 ER PT J AU Guber, K Kopecky, S Schillebeeckx, P Kauwenberghs, K Siegler, P AF Guber, K. Kopecky, S. Schillebeeckx, P. Kauwenberghs, K. Siegler, P. TI Neutron-induced Cross Section Measurements of Calcium SO NUCLEAR DATA SHEETS LA English DT Article ID CAPTURE AB To support the US Department of Energy Nuclear Criticality Safety Program, neutron-induced cross section experiments were performed at the Geel Electron Linear Accelerator of the Institute for Reference Material and Measurements of the Joint Research Centers, European Union. Neutron capture and transmission measurements were carried out using a metallic calcium sample. The measured data will be used for a new calcium evaluation, which will be submitted with covariances to the ENDF/B nuclear data library. C1 [Guber, K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Kopecky, S.; Schillebeeckx, P.; Kauwenberghs, K.; Siegler, P.] EC JRC IRMM, Nucl Phys Unit, B-2440 Geel, Belgium. RP Guber, K (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM guberkh@ornl.gov FU U.S. Department of Energy [DE-AC05-00OR22725]; U.S. Department of Energy Nuclear Criticality Safety Program FX This manuscript has been authored by the Oak Ridge National Laboratory, managed by UT-Battelle LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The U.S. Department of Energy Nuclear Criticality Safety Program sponsored the work that is presented in this paper. NR 7 TC 0 Z9 0 U1 0 U2 1 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 113 EP 116 DI 10.1016/j.nds.2014.08.032 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200148 ER PT J AU Giubrone, G Domingo-Pardo, C Tain, JL Lederer, C Altstadt, S Andrzejewski, J Audouin, L Barbagallo, M Becares, V Becvar, F Belloni, F Berthoumieux, E Billowes, J Boccone, V Bosnar, D Brugger, M Calviani, M Calvino, F Cano-Ott, D Carrapico, C Cerutti, F Chiaveri, E Chin, M Colonna, N Cortes, G Cortes-Giraldo, MA Diakaki, M Duran, I Dressler, R Dzysiuk, N Eleftheriadis, C Ferrari, A Fraval, K Ganesan, S Garcia, AR Gomez-Hornillos, MB Goncalves, IF Gonzalez-Romero, E Griesmayer, E Guerrero, C Gunsing, F Gurusamy, P Jenkins, DG Jericha, E Kadi, Y Kappeler, F Karadimos, D Kivel, N Koehler, P Kokkoris, M Korschinek, G Krticka, M Kroll, J Langer, C Leeb, H Leong, LS Losito, R Manousos, A Massimi, C Marganiec, J Martinez, T Mastinu, PF Mastromarco, M Meaze, M Mendoza, E Mengoni, A Milazzo, PM Mingrone, F Mirea, M Mondelaers, W Paradela, C Pavlik, A Perkowski, J Pignatari, M Plompen, A Praena, J Quesada, JM Rauscher, T Reifhart, R Riego, A Roman, F Rubbia, C Sarmento, R Schillebeeckx, P Schmidt, S Schumann, D Tagliente, G Tarrio, D Tassan-Got, L Tsinganis, A Valenta, S Vannini, G Variale, V Vaz, P Ventura, A Versaci, R Vermeulen, MJ Vlachoudis, V Vlastou, R Wallner, A Ware, T Weigand, M Weiss, C Wright, T Zugec, P AF Giubrone, G. Domingo-Pardo, C. Tain, J. L. Lederer, C. Altstadt, S. Andrzejewski, J. Audouin, L. Barbagallo, M. Becares, V. Becvar, F. Belloni, F. Berthoumieux, E. Billowes, J. Boccone, V. Bosnar, D. Brugger, M. Calviani, M. Calvino, F. Cano-Ott, D. Carrapico, C. Cerutti, F. Chiaveri, E. Chin, M. Colonna, N. Cortes, G. Cortes-Giraldo, M. A. Diakaki, M. Duran, I. Dressler, R. Dzysiuk, N. Eleftheriadis, C. Ferrari, A. Fraval, K. Ganesan, S. Garcia, A. R. Gomez-Hornillos, M. B. Goncalves, I. F. Gonzalez-Romero, E. Griesmayer, E. Guerrero, C. Gunsing, F. Gurusamy, P. Jenkins, D. G. Jericha, E. Kadi, Y. Kaeppeler, F. Karadimos, D. Kivel, N. Koehler, P. Kokkoris, M. Korschinek, G. Krticka, M. Kroll, J. Langer, C. Leeb, H. Leong, L. S. Losito, R. Manousos, A. Massimi, C. Marganiec, J. Martinez, T. Mastinu, P. F. Mastromarco, M. Meaze, M. Mendoza, E. Mengoni, A. Milazzo, P. M. Mingrone, F. Mirea, M. Mondelaers, W. Paradela, C. Pavlik, A. Perkowski, J. Pignatari, M. Plompen, A. Praena, J. Quesada, J. M. Rauscher, T. Reifhart, R. Riego, A. Roman, F. Rubbia, C. Sarmento, R. Schillebeeckx, P. Schmidt, S. Schumann, D. Tagliente, G. Tarrio, D. Tassan-Got, L. Tsinganis, A. Valenta, S. Vannini, G. Variale, V. Vaz, P. Ventura, A. Versaci, R. Vermeulen, M. J. Vlachoudis, V. Vlastou, R. Wallner, A. Ware, T. Weigand, M. Weiss, C. Wright, T. Zugec, P. TI Measurement of the Fe-54,Fe-57(n,gamma) Cross Section in the Resolved Resonance Region at CERN n_TOF SO NUCLEAR DATA SHEETS LA English DT Article ID CAPTURE AB Fe-54 and Fe-57 are stable iron isotopes, which play an important role in the nucleosynthesis of the slow neutron capture process (s process). In addition, these nuclei are present in many structural materials, and therefore, the knowledge of their neutron capture cross sections is of importance for reactor design studies. This contribution summarizes the results of the (n,gamma) cross sections of these two isotopes in the resolved resonance region. The experiment was carried out at the CERN n_TOF facility using the Pulse-Height Weighting Technique in combination with an experimental set-up optmized for reducing neutron induced backgrounds. C1 [Giubrone, G.; Domingo-Pardo, C.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, IFIC, E-46003 Valencia, Spain. [Lederer, C.; Altstadt, S.; Langer, C.; Reifhart, R.; Schmidt, S.; Weigand, M.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Lederer, C.; Pavlik, A.; Wallner, A.; Weiss, C.] Univ Vienna, Fac Phys, Vienna, Austria. [Andrzejewski, J.; Marganiec, J.; Perkowski, J.] Univ Lodz, PL-90131 Lodz, Poland. [Audouin, L.; Leong, L. S.; Tassan-Got, L.] IPN, CNRS, IN2P3, Orsay, France. [Barbagallo, M.; Colonna, N.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Becares, V.; Cano-Ott, D.; Garcia, A. R.; Gonzalez-Romero, E.; Martinez, T.; Mendoza, E.] CIEMAT, E-28040 Madrid, Spain. [Becvar, F.; Krticka, M.; Kroll, J.; Valenta, S.] Charles Univ Prague, Prague, Czech Republic. [Belloni, F.; Chiaveri, E.; Fraval, K.; Gunsing, F.] CEA Saclay, Irfu, F-91191 Gif Sur Yvette, France. [Berthoumieux, E.; Boccone, V.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Ferrari, A.; Guerrero, C.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Tsinganis, A.; Versaci, R.; Vlachoudis, V.; Ware, T.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Billowes, J.; Wright, T.] Univ Manchester, Manchester, Lancs, England. [Bosnar, D.; Zugec, P.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia. [Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, Barcelona, Spain. [Carrapico, C.; Goncalves, I. F.; Sarmento, R.; Vaz, P.] Univ Tecn Lisboa, Inst Super Tecn, Inst Tecnol & Nucl, P-1096 Lisbon, Portugal. [Cortes-Giraldo, M. A.; Praena, J.; Quesada, J. M.] Univ Seville, Seville, Spain. [Diakaki, M.; Karadimos, D.; Kokkoris, M.; Vlastou, R.] Natl Tech Univ Athens, GR-10682 Athens, Greece. [Duran, I.; Paradela, C.; Tarrio, D.] Univ Santiago de Compostela, Santiago De Compostela, Spain. [Dressler, R.; Kivel, N.; Schumann, D.] Paul Scherrer Inst, Villigen, Switzerland. [Dzysiuk, N.; Mastinu, P. F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Eleftheriadis, C.; Manousos, A.] Aristotle Univ Thessaloniki, GR-54006 Thessaloniki, Greece. [Ganesan, S.; Gurusamy, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Griesmayer, E.; Jericha, E.; Leeb, H.] Vienna Univ Technol, Inst Atom, Vienna, Austria. [Jenkins, D. G.; Vermeulen, M. J.] Univ York, York YO10 5DD, N Yorkshire, England. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Koehler, P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Korschinek, G.] Tech Univ Munich, D-80290 Munich, Germany. [Massimi, C.; Mingrone, F.; Vannini, G.] Univ Bologna, Dipartimento Fis, I-40126 Bologna, Italy. [Massimi, C.; Mingrone, F.; Vannini, G.] Sez INFN Bologna, Bologna, Italy. Agenzia Nazl Nuove Tecnol, Energia Sviluppo Econ Sostenibile ENEA, Bologna, Italy. [Milazzo, P. M.] Ist Nazl Fis Nucl, Trieste, Italy. [Mirea, M.; Roman, F.] Horia Hulubei Natl Inst Phys & Nucl Engn, IFIN HH, Bucharest, Romania. [Mondelaers, W.; Plompen, A.; Schillebeeckx, P.] European Commiss JRC, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Pignatari, M.; Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rubbia, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. RP Giubrone, G (reprint author), Univ Valencia, CSIC, Inst Fis Corpuscular, IFIC, E-46003 Valencia, Spain. EM giubrone@ific.uv.es RI Rauscher, Thomas/D-2086-2009; Mirea, Mihail/C-2297-2011; Cano Ott, Daniel/K-4945-2014; Gonzalez Romero, Enrique/L-7561-2014; Duran, Ignacio/H-7254-2015; Massimi, Cristian/K-2008-2015; Paradela, Carlos/J-1492-2012; Chin, Mary Pik Wai/B-6644-2012; Mendoza Cembranos, Emilio/K-5789-2014; Becares, Vicente/K-4514-2014; Martinez, Trinitario/K-6785-2014; Calvino, Francisco/K-5743-2014; Langer, Christoph/L-3422-2016; Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012 OI Rauscher, Thomas/0000-0002-1266-0642; Mirea, Mihail/0000-0002-9333-6595; Cano Ott, Daniel/0000-0002-9568-7508; Gonzalez Romero, Enrique/0000-0003-2376-8920; Massimi, Cristian/0000-0003-2499-5586; Chin, Mary Pik Wai/0000-0001-5176-9723; Mendoza Cembranos, Emilio/0000-0002-2843-1801; Becares, Vicente/0000-0003-3434-9086; Martinez, Trinitario/0000-0002-0683-5506; Calvino, Francisco/0000-0002-7198-4639; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038 NR 10 TC 2 Z9 2 U1 2 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 117 EP 120 DI 10.1016/j.nds.2014.08.033 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200149 ER PT J AU Fotiades, N Devlin, M Haight, RC Kawano, T Kunieda, S Nelson, RO AF Fotiades, N. Devlin, M. Haight, R. C. Kawano, T. Kunieda, S. Nelson, R. O. TI Measurements of Partial gamma-ray Cross Sections in Ni-60(n, xnypz alpha gamma) Reactions SO NUCLEAR DATA SHEETS LA English DT Article ID NUCLEAR-DATA SHEETS AB Absolute partial cross sections for production of discrete gamma-rays using Ni-60(n, xnypz alpha gamma) reactions with x <= 3, y <= 2 and z <= 4 in a total of 20 reaction channels were measured. The data were taken using the GEANIE spectrometer comprised of 20 high-purity Ge detectors with BGO escapesuppression shields. The broad-spectrum pulsed neutron beam of the Los Alamos Neutron Science Center's (LANSCE) WNR facility provided neutrons in the energy range from 0.2 to 300 MeV. The time-of-flight technique was used to determine the incident neutron energies. Partial gamma-ray cross sections have been measured for a total of 59 transitions and for neutron energies 1 MeV< E-n <300 MeV. Hauser-Feshbach theoretical calculations with an improved cluster emission model in the pre-equilibrium process were performed up to E-n = 30 MeV and are compared to the experimental results. C1 [Fotiades, N.; Devlin, M.; Haight, R. C.; Kawano, T.; Kunieda, S.; Nelson, R. O.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Fotiades, N (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM fotia@lanl.gov RI Devlin, Matthew/B-5089-2013; OI Devlin, Matthew/0000-0002-6948-2154; Fotiadis, Nikolaos/0000-0003-1410-3871 FU U.S. Department of Energy (DOE) [DE-AC52-06NA25396]; DOE [DE-AC52-06NA25396] FX This work was performed under the auspices of the U.S. Department of Energy (DOE) under Contract No. DE-AC52-06NA25396. This work has benefitted from use of the LANSCE accelerator facility supported under DOE Contract No. DE-AC52-06NA25396. NR 18 TC 1 Z9 1 U1 0 U2 0 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 124 EP 127 DI 10.1016/j.nds.2014.08.035 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200151 ER PT J AU Kroll, J Agvaanluvsan, U Baramsai, B Becker, JA Becvar, F Bredeweg, TA Chyzh, A Couture, A Dashdorj, D Haight, RC Jandel, M Keksis, AL Krticka, M Mitchell, GE O'Donnell, JM Parker, W Rundberg, RS Ullmann, JL Valenta, S Vieira, DJ Walker, CL Wilhelmy, JB Wouters, JM Wu, CY AF Kroll, J. Agvaanluvsan, U. Baramsai, B. Becker, J. A. Becvar, F. Bredeweg, T. A. Chyzh, A. Couture, A. Dashdorj, D. Haight, R. C. Jandel, M. Keksis, A. L. Krticka, M. Mitchell, G. E. O'Donnell, J. M. Parker, W. Rundberg, R. S. Ullmann, J. L. Valenta, S. Vieira, D. J. Walker, C. L. Wilhelmy, J. B. Wouters, J. M. Wu, C. Y. TI Systematics of Scissors Mode in Gd Nuclei from Experiments with the DANCE Detector SO NUCLEAR DATA SHEETS LA English DT Article ID LEVEL DENSITY; EXCITATION MODE; STRENGTH; DEFORMATION; SCATTERING; GD-156; ARRAY AB Multi-step cascade gamma-ray spectra from neutron capture at isolated resonances of Gd-152,Gd-154-158 nuclei were measured at the LANSCE/DANCE time-of-flight facility in Los Alamos National Laboratory. The main objective of these experiments was to obtain new information on photon strength functions with emphasis on the role of the M1 scissors mode vibration. An analysis of the data obtained shows that the scissors mode plays a significant role in the ground state transitions, as well as in the transitions populating all excited states of the studied nuclei. The estimates of the scissors mode strength indicate that for Gd-157,Gd-159 this strength is significantly higher than in neighboring even-even nuclei Gd-156,Gd-158. The results are compared with the (gamma,gamma ') data for the ground-state scissors mode and the results from He-3-induced reactions. C1 [Kroll, J.; Becvar, F.; Krticka, M.; Valenta, S.] Charles Univ Prague, CZ-18000 Prague 8, Czech Republic. [Agvaanluvsan, U.] MonAme Sci Res Ctr, Ulaanbaatar, Mongol Peo Rep. [Baramsai, B.; Mitchell, G. E.; Walker, C. L.] N Carolina State Univ, Raleigh, NC 27695 USA. [Baramsai, B.; Mitchell, G. E.; Walker, C. L.] Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Becker, J. A.; Becvar, F.; Dashdorj, D.; Parker, W.; Wu, C. Y.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Bredeweg, T. A.; Couture, A.; Haight, R. C.; Jandel, M.; Keksis, A. L.; O'Donnell, J. M.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wouters, J. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Kroll, J (reprint author), Charles Univ Prague, CZ-18000 Prague 8, Czech Republic. EM kroll@ipnp.troja.mff.cuni.cz FU U.S. Department of Energy (DOE) [DE-NA0001784, DE-FG02-97-ER41042]; U.S. DOE at LANL by the Los Alamos National Security, LLC [DE-AC52-06NA25396]; U.S. DOE at LLNL by the Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]; Ministry of Education of the Czech Republic [MSM 0021620859, LG13031]; Czech Science Foundation [13-07117S] FX This work was supported in part by U.S. Department of Energy (DOE) Grants No. DE-NA0001784 and No. DE-FG02-97-ER41042. It benefited from the use of the LANSCE accelerator and was performed under the auspices of the U.S. DOE at LANL by the Los Alamos National Security, LLC under Contract No. DE-AC52-06NA25396 and at LLNL by the Lawrence Livermore National Security, LLC under Contract No. DE-AC52-07NA27344. It was also supported by the research plans MSM 0021620859 and LG13031 of the Ministry of Education of the Czech Republic, and grant 13-07117S of the Czech Science Foundation. NR 37 TC 0 Z9 0 U1 2 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 158 EP 161 DI 10.1016/j.nds.2014.08.044 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200160 ER PT J AU Roig, O Theroine, C Ebran, A Meot, V Bond, EM Bredeweg, TA Couture, A Haight, RC Jandel, M Nortier, FM O'Donnell, JM Rundberg, RS Taylor, WA Ullmann, JL Vieira, DJ AF Roig, O. Theroine, C. Ebran, A. Meot, V. Bond, E. M. Bredeweg, T. A. Couture, A. Haight, R. C. Jandel, M. Nortier, F. M. O'Donnell, J. M. Rundberg, R. S. Taylor, W. A. Ullmann, J. L. Vieira, D. J. TI Measurement of Lu-173(n,gamma) Cross Sections at DANCE SO NUCLEAR DATA SHEETS LA English DT Article AB A highly gamma-radioactive target, 3.7 GBq, of Lu-173 isotope was placed inside the DANCE array (Detector for Advanced Neutron Capture Experiments) at Los Alamos to study the radiative neutron capture on an unstable isotope. The Lu-173 element was produced by Hf-natural(p,xn) reactions following by beta-decays at the Isotope Production Facility (IPF). Measurements of radiative neutron capture cross section on Lu-173 were achieved at the Los Alamos Neutron Science Center (LANSCE) spallation neutron source facility over the neutron energy range from thermal up to 1 keV. A special configuration was necessary to perform the experiment using the DANCE [1] array due to the high gamma activity of the target. We will report on the target production, the experiment and the results obtained for the radiative neutron capture on Lu-173. The radiative capture cross section was obtained for the first time on this unstable nucleus. Some resonances have been characterized. A comparison with a recent data evaluation is presented. C1 [Roig, O.; Theroine, C.; Ebran, A.; Meot, V.] CEA, DAM, F-91297 Arpajon, France. [Bond, E. M.; Bredeweg, T. A.; Couture, A.; Haight, R. C.; Jandel, M.; Nortier, F. M.; O'Donnell, J. M.; Rundberg, R. S.; Taylor, W. A.; Ullmann, J. L.; Vieira, D. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Roig, O (reprint author), CEA, DAM, F-91297 Arpajon, France. EM olivier.roig@cea.fr FU DOE Office of Basic Energy Sciences; Department of Energy [W-7405-ENG-36] FX The authors are indebted to Dr. P. Romain (CEA/DAM) for the constant help for TALYS evaluation and Dr. F. Gunsing (CEA/IRFU) and Dr. P. Koehler (ORNL) for useful suggestions on SAMMY. This work has benefited from the use of the Lujan Center at the Los Alamos Neutron Science Center, funded by the DOE Office of Basic Energy Sciences and Los Alamos National Laboratory funded by the Department of Energy under contract W-7405-ENG-36. NR 16 TC 0 Z9 0 U1 2 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 165 EP 168 DI 10.1016/j.nds.2014.08.046 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200162 ER PT J AU Youinou, G Vondrasek, R Veselka, H Salvatores, M Paul, M Pardo, R Palmiotti, G Palchan, T Nusair, O Nimmagadda, J Nair, C Murray, P Maddock, T Kondrashev, S Kondev, FG Jones, W Imel, G Glass, C Fonnesbeck, J Berg, J Bauder, W AF Youinou, G. Vondrasek, R. Veselka, H. Salvatores, M. Paul, M. Pardo, R. Palmiotti, G. Palchan, T. Nusair, O. Nimmagadda, J. Nair, C. Murray, P. Maddock, T. Kondrashev, S. Kondev, F. G. Jones, W. Imel, G. Glass, C. Fonnesbeck, J. Berg, J. Bauder, W. TI MANTRA: An Integral Reactor Physics Experiment to Infer the Neutron Capture Cross Sections of Actinides and Fission Products in Fast and Epithermal Spectra SO NUCLEAR DATA SHEETS LA English DT Article AB This paper presents an update of an on-going collaborative INL-ANL-ISU integral reactor physics experiment whose objective is to infer the effective neutron capture cross sections for most of the actinides of importance for reactor physics and fuel cycle studies in both fast and epithermal spectra. Some fission products are also being considered. The principle of the experiment is to irradiate very pure actinide samples in the Advanced Test Reactor at INL and, after a given time, determine the amount of the different transmutation products. The determination of the nuclide densities before and after neutron irradiation together with the neutron fluence will allow inference of effective neutron capture cross-sections in different neutron spectra. C1 [Youinou, G.; Veselka, H.; Salvatores, M.; Palmiotti, G.; Murray, P.; Maddock, T.; Jones, W.; Glass, C.; Fonnesbeck, J.; Berg, J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Vondrasek, R.; Paul, M.; Pardo, R.; Palchan, T.; Nusair, O.; Nair, C.; Kondrashev, S.; Kondev, F. G.; Bauder, W.] Argonne Natl Lab, Argonne, IL 60439 USA. [Salvatores, M.] CEN Cadarache, F-13108 St Paul Les Durance, France. [Nimmagadda, J.; Imel, G.] Idaho State Univ, Pocatello, ID 83209 USA. RP Youinou, G (reprint author), Idaho Natl Lab, 2525 Fremont Ave, Idaho Falls, ID 83415 USA. EM gilles.youinou@inl.gov FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under DOE Idaho Operations Office [DE-AC07-05ID14517]; ANL [DE-AC02-06CH11357]; ATR National Scientific User Facility FX This work is supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under DOE Idaho Operations Office Contract DE-AC07-05ID14517 as well as by the ANL Contract DE-AC02-06CH11357 and by the ATR National Scientific User Facility. NR 4 TC 1 Z9 1 U1 0 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 169 EP 172 DI 10.1016/j.nds.2014.08.047 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200163 ER PT J AU Bhatia, C Gooden, ME Tornow, W Tonchev, AP AF Bhatia, C. Gooden, M. E. Tornow, W. Tonchev, A. P. TI Measurements of the (n,2n) Reaction Cross Section of Ta-181 from 8 to 15 MeV SO NUCLEAR DATA SHEETS LA English DT Article ID EXCITATION FUNCTIONS; NEUTRONS; SCATTERING; NUCLEI; DECAY AB The cross section for the reaction Ta-181(n,2n) Ta-180(g) was measured from 8 to 15 MeV in small energy steps to resolve inconsistencies in the existing databases. The activation technique was used, and the 93.4 keV gamma-ray from the decay of the Ta-180(g) ground state was recorded with a HPGe detector. In addition, the gamma-rays from the monitor reactions Al-27(n,alpha)Na-24 and Au-197(n,2n) Au-196 were measured for neutron fluence determination. As a cross check, a calibrated neutron detector was also used. The ENDF/B-VII. 1 and TENDL-2011 evaluations are in considerable disagreement with the present data, which in turn agree very well with the majority of the existing data in the 14 MeV energy region. C1 [Bhatia, C.; Tornow, W.] Duke Univ, Dept Phys, TUNL, Durham, NC 27708 USA. [Gooden, M. E.] N Carolina State Univ, Dept Phys, TUNL, Raleigh, NC 27695 USA. [Tonchev, A. P.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. RP Bhatia, C (reprint author), McMaster Univ, 1280 Main St W, Hamilton, ON L8S 4K1, Canada. EM chitra@tunl.duke.edu FU National Nuclear Security Administration under the Stewardship Science Academic Alliance Program through the US Department of Energy [DE-FG52-09NA29465] FX The authors acknowledge valuable contributions from M. Bhike, S.W. Finch, C.R. Howell, J.H. Kelley, J.B. Wilhelmy and D.J. Vieira. Fruitful discussions with S. Goriely are gratefully acknowledged. This work was supported in part by the National Nuclear Security Administration under the Stewardship Science Academic Alliance Program through the US Department of Energy Grant No. DE-FG52-09NA29465. NR 24 TC 0 Z9 0 U1 1 U2 1 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 176 EP 178 DI 10.1016/j.nds.2014.08.049 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200165 ER PT J AU Bacquias, A Dessagne, P Kerveno, M Rudolf, G Plompen, AJM Drohe, JC Rouki, C Nankov, N Nyman, M Borcea, C Negret, A Archier, P De Saint Jean, C Noguere, G Vaglio-Gaudard, C Koning, A Domula, A Zuber, K Leal, LC AF Bacquias, A. Dessagne, Ph. Kerveno, M. Rudolf, G. Plompen, A. J. M. Drohe, J. C. Rouki, C. Nankov, N. Nyman, M. Borcea, C. Negret, A. Archier, P. De Saint Jean, C. Noguere, G. Vaglio-Gaudard, C. Koning, A. Domula, A. Zuber, K. Leal, L. C. TI Neutron Inelastic Scattering Measurements for Na, Ge, Zr, Mo and U SO NUCLEAR DATA SHEETS LA English DT Article ID CROSS-SECTIONS; REACTORS; SYSTEM AB Studies for advanced reactor systems such as sodium-cooled fast reactors designed for recycling of high level waste, accelerator driven systems for transmutation, and systems envisioning the use of the Th/U fuel cycle impose tight requirements on nuclear data for accurate predictions of their operation and safety characteristics. Among the identified needs established by sensitivity studies, neutron inelastic scattering on the main structural materials and actinides and some (n,xn) cross sections for actinides feature prominently. Prompt-gamma spectroscopy and time-of-flight techniques were used to measure (n, xn gamma) cross-sections of interest. Experiments were performed at the GELINA neutron time-of-flight facility of IRMM. Results for U-235 and Na-23 are briefly recalled; pertaining theoretical discussions are mentioned to explain observations concerning U-238. The status of studies on Ge-76, Zr and Mo is also reported. C1 [Bacquias, A.; Dessagne, Ph.; Kerveno, M.; Rudolf, G.] Univ Strasbourg, IPHC, CNRS, UMR7178, F-67037 Strasbourg, France. [Plompen, A. J. M.; Drohe, J. C.; Rouki, C.; Nankov, N.; Nyman, M.] Commiss European Communities, Joint Res Ctr, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Borcea, C.; Negret, A.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Archier, P.; De Saint Jean, C.; Noguere, G.; Vaglio-Gaudard, C.] CEA, DEN, F-13108 St Paul Les Durance, France. [Koning, A.] NRG, NL-1755 ZG Petten, Netherlands. [Domula, A.; Zuber, K.] Tech Univ Dresden, D-01069 Dresden, Germany. [Leal, L. C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Bacquias, A (reprint author), Univ Strasbourg, IPHC, CNRS, UMR7178, 23 Rue Loess, F-67037 Strasbourg, France. EM antoine.bacquias@iphc.cnrs.fr RI De Saint Jean, Cyrille/E-8853-2011 FU PACEN/GEDEPEON; European Commission within the Sixth Framework Programme through I3-EFNUDAT (EURATOM) [036434]; NUDAME [FP6-516487]; Seventh Framework Programme through EUFRAT (EURATOM) [FP7-211499]; ANDES (EURATOM) [FP7-249671] FX The authors wish to thank the team of the GELINA facility for the preparation of the neutron beam and for their constant support. This work was partly supported by PACEN/GEDEPEON and by the European Commission within the Sixth Framework Programme through I3-EFNUDAT (EURATOM contract no. 036434) and NUDAME (Contract FP6-516487), and within the Seventh Framework Programme through EUFRAT (EURATOM contract no. FP7-211499) and through ANDES (EURATOM contract no. FP7-249671). NR 26 TC 3 Z9 3 U1 2 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 186 EP 189 DI 10.1016/j.nds.2014.08.052 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200168 ER PT J AU Bevilacqua, R Pomp, S Jansson, K Gustavsson, C Osterlund, M Simutkin, V Hayashi, M Hirayama, S Naitou, Y Watanabe, Y Hjalmarsson, A Prokofiev, A Tippawan, U Lecolley, FR Marie, N Leray, S David, JC Mashnik, S AF Bevilacqua, R. Pomp, S. Jansson, K. Gustavsson, C. Osterlund, M. Simutkin, V. Hayashi, M. Hirayama, S. Naitou, Y. Watanabe, Y. Hjalmarsson, A. Prokofiev, A. Tippawan, U. Lecolley, F. -R. Marie, N. Leray, S. David, J. -C. Mashnik, S. TI Light-ion Production from O, Si, Fe and Bi Induced by 175 MeV Quasi-monoenergetic Neutrons SO NUCLEAR DATA SHEETS LA English DT Article ID MEDLEY AB We have measured double-differential cross sections in the interaction of 175 MeV quasimonoenergetic neutrons with O, Si, Fe and Bi. We have compared these results with model calculations with INCL4.5-Abla07, MCNP6 and TALYS-1.2. We have also compared our data with PHITS calculations, where the pre-equilibrium stage of the reaction was accounted respectively using the JENDL/HE-2007 evaluated data library, the quantum molecular dynamics model (QMD) and a modified version of QMD (MQMD) to include a surface coalescence model. The most crucial aspect is the formation and emission of composite particles in the pre-equilibrium stage. C1 [Bevilacqua, R.; Pomp, S.; Jansson, K.; Gustavsson, C.; Osterlund, M.; Simutkin, V.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Hayashi, M.; Hirayama, S.; Naitou, Y.; Watanabe, Y.] Kyushu Univ, Dept Adv Energy Engn Sci, Fukuoka 8168580, Japan. [Hjalmarsson, A.; Prokofiev, A.] Uppsala Univ, Svedberg Lab, S-75121 Uppsala, Sweden. [Tippawan, U.] Chiang Mai Univ, Chiang Mai 50200, Thailand. [Lecolley, F. -R.; Marie, N.] Univ Caen, LPC, F-14050 Caen, France. [Leray, S.; David, J. -C.] CEA, Ctr Saclay, Irfu SPhN, F-91191 Gif Sur Yvette, France. [Mashnik, S.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Bevilacqua, R (reprint author), Commiss European Communities, Joint Res Ctr, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. EM Riccardo.BEVILACQUA@ec.europa.eu RI U-ID, Kyushu/C-5291-2016; Leray, Sylvie/A-3924-2012 OI Leray, Sylvie/0000-0002-1942-2911 FU ENEN Association; Uppsala University; Thailand Research Fund (TRF) [MGR5280165] FX R.B. is grateful to the ENEN Association and to Uppsala University for the financial support to participate in the ND2013 Conference. U.T. expresses his gratitude to the Thailand Research Fund (TRF) for financial support under Project No. MGR5280165. NR 13 TC 1 Z9 1 U1 0 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 190 EP 193 DI 10.1016/j.nds.2014.08.053 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200169 ER PT J AU Haight, RC Lee, HY Taddeucci, TN O'Donnell, JM Perdue, BA Fotiades, N Devlin, M Ullmann, JL Laptev, A Bredeweg, T Jandel, M Nelson, RO Wender, SA White, MC Wu, CY Kwan, E Chyzh, A Henderson, R Gostic, J AF Haight, R. C. Lee, H. Y. Taddeucci, T. N. O'Donnell, J. M. Perdue, B. A. Fotiades, N. Devlin, M. Ullmann, J. L. Laptev, A. Bredeweg, T. Jandel, M. Nelson, R. O. Wender, S. A. White, M. C. Wu, C. Y. Kwan, E. Chyzh, A. Henderson, R. Gostic, J. TI The Prompt Fission Neutron Spectrum (PFNS) Measurement Program at LANSCE SO NUCLEAR DATA SHEETS LA English DT Article AB The prompt neutron spectrum from neutron-induced fission needs to be known in designing new fast reactors, predicting criticality for safety analyses, and developing techniques for global security application. A program to measure this spectrum for neutron-induced fission of Pu-239 is underway at the Los Alamos Neutron Science Center. The goal is to obtain data on the shape of the spectrum with a small uncertainty over the emitted neutron energy range of 100 keV to 12 MeV with additional data below and above this range. The incident neutron energy range will be from 0.5 to 30 MeV. The status of this program including results of initial experimental measurements is described here. C1 [Haight, R. C.; Lee, H. Y.; Taddeucci, T. N.; O'Donnell, J. M.; Perdue, B. A.; Fotiades, N.; Devlin, M.; Ullmann, J. L.; Laptev, A.; Bredeweg, T.; Jandel, M.; Nelson, R. O.; Wender, S. A.; White, M. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Wu, C. Y.; Kwan, E.; Chyzh, A.; Henderson, R.; Gostic, J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Haight, RC (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM haight@lanl.gov RI Laptev, Alexander/D-4686-2009; Devlin, Matthew/B-5089-2013; OI Laptev, Alexander/0000-0002-9759-9907; Devlin, Matthew/0000-0002-6948-2154; Fotiadis, Nikolaos/0000-0003-1410-3871; White, Morgan/0000-0003-3876-421X; Wender, Stephen/0000-0002-2446-5115 FU US Department of Energy by Los Alamos National Security, LLC [DE-AC52-06NA25396]; Lawrence Livermore National Security, LLC [DE-AC52-07NA27344] FX This work benefitted from the use of the LANSCE accelerator facility and was performed under the auspices of the US Department of Energy by Los Alamos National Security, LLC under contract DE-AC52-06NA25396 and by Lawrence Livermore National Security, LLC under contract DE-AC52-07NA27344. NR 14 TC 2 Z9 2 U1 0 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 205 EP 208 DI 10.1016/j.nds.2014.08.057 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200173 ER PT J AU Kwan, E Wu, CY Haight, RC Lee, HY Bredeweg, TA Chyzh, A Devlin, M Fotiades, N Gostic, JM Henderson, RA Jandel, M Laptev, A Nelson, RO O'Donnell, JM Perdue, BA Taddeucci, TN Ullmann, JL Wender, SA AF Kwan, E. Wu, C. Y. Haight, R. C. Lee, H. Y. Bredeweg, T. A. Chyzh, A. Devlin, M. Fotiades, N. Gostic, J. M. Henderson, R. A. Jandel, M. Laptev, A. Nelson, R. O. O'Donnell, J. M. Perdue, B. A. Taddeucci, T. N. Ullmann, J. L. Wender, S. A. TI Prompt Fission gamma-rays Measured Using Liquid Scintillators SO NUCLEAR DATA SHEETS LA English DT Article AB The prompt.-ray spectra from U-235(n,f) at incident energies of 1 to 20 MeV and for Cf-235(s.f.) were measured up to 4 MeV in coincidence with two parallel plate avalanche counters and the liquid scintillator array FIGARO. The unfolded gamma-ray spectra from 1-4 MeV using the single value decomposition and iterative Bayesian techniques for the incident neutron energy regions corresponding to the first, second and third chance fissions were found to nearly identical and similar to the distribution from the spontaneous fission of Cf-252. General agreement with the gamma-ray distributions from fission was also found with previous measurements. C1 [Kwan, E.; Wu, C. Y.; Chyzh, A.; Gostic, J. M.; Henderson, R. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Haight, R. C.; Lee, H. Y.; Bredeweg, T. A.; Devlin, M.; Fotiades, N.; Jandel, M.; Laptev, A.; Nelson, R. O.; O'Donnell, J. M.; Perdue, B. A.; Taddeucci, T. N.; Ullmann, J. L.; Wender, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Kwan, E (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. EM kwan@nscl.msu.edu RI Laptev, Alexander/D-4686-2009; Devlin, Matthew/B-5089-2013; OI Laptev, Alexander/0000-0002-9759-9907; Devlin, Matthew/0000-0002-6948-2154; Fotiadis, Nikolaos/0000-0003-1410-3871; Wender, Stephen/0000-0002-2446-5115 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work benefited from the use of the LANSCE accelerator facility and was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and Los Alamos National Laboratory under Contract DE-AC52-06NA25396. NR 16 TC 0 Z9 0 U1 1 U2 1 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 221 EP 224 DI 10.1016/j.nds.2014.08.061 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200177 ER PT J AU Wiedeking, M Bernstein, LA Allmond, JM Basunia, MS Bleuel, DL Burke, JT Fallon, P Firestone, RB Goldblum, BL Hatarik, R Krticka, M Lake, PT Larsen, AC Lee, IY Lesher, SR Paschalis, S Petri, M Phair, L Scielzo, ND AF Wiedeking, M. Bernstein, L. A. Allmond, J. M. Basunia, M. S. Bleuel, D. L. Burke, J. T. Fallon, P. Firestone, R. B. Goldblum, B. L. Hatarik, R. Krticka, M. Lake, P. T. Larsen, A. C. Lee, I-Y. Lesher, S. R. Paschalis, S. Petri, M. Phair, L. Scielzo, N. D. TI Photon Strength Function at Low Energies in Mo-95 SO NUCLEAR DATA SHEETS LA English DT Article AB A new and model-independent experimental method has been developed to determine the energy dependence of the photon strength function. It is designed to study statistical feeding from the quasi continuum to individual low-lying discrete levels. This new technique is presented and results for Mo-95 are compared to data from the University of Oslo. In particular, questions regarding the existence of the low-energy enhancement in the photon strength function are addressed. C1 [Wiedeking, M.] iThemba LABS, ZA-7129 Somerset West, South Africa. [Wiedeking, M.; Bernstein, L. A.; Bleuel, D. L.; Burke, J. T.; Hatarik, R.; Lesher, S. R.; Scielzo, N. D.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. [Allmond, J. M.] Univ Richmond, Dept Phys, Richmond, VA 23173 USA. [Allmond, J. M.] Oak Ridge Natl Lab, Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. [Basunia, M. S.; Fallon, P.; Firestone, R. B.; Lake, P. T.; Lee, I-Y.; Paschalis, S.; Petri, M.; Phair, L.] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Goldblum, B. L.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Krticka, M.] Charles Univ Prague, Fac Math & Phys, Prague 8, Czech Republic. [Larsen, A. C.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. RP Wiedeking, M (reprint author), iThemba LABS, POB 722, ZA-7129 Somerset West, South Africa. EM wiedeking@tlabs.ac.za RI Burke, Jason/I-4580-2012; Larsen, Ann-Cecilie/C-8742-2014; Petri, Marina/H-4630-2016; Paschalis, Stefanos/H-8758-2016; OI Larsen, Ann-Cecilie/0000-0002-2188-3709; Petri, Marina/0000-0002-3740-6106; Paschalis, Stefanos/0000-0002-9113-3778; Allmond, James Mitchell/0000-0001-6533-8721 FU National Research Foundation of South Africa; U.S. Department of Energy Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; University of Richmond [DE-FG52-06NA26206, DE-FG02-05ER41379]; Director, Office of Science, Office of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; Ministry of Education of the Czech Republic [MSM 0021620859]; Research Council of Norway [205528] FX This work is based on research supported by the National Research Foundation of South Africa and on work performed under the auspices of the U.S. Department of Energy Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 and University of Richmond under DE-FG52-06NA26206 and DE-FG02-05ER41379. For Lawrence Berkeley National Laboratory, this work was supported by the Director, Office of Science, Office of Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. MK acknowledges support from the research plan MSM 0021620859 of the Ministry of Education of the Czech Republic and from the Czech Science Foundation under Grant No. 13-07117S. ACL acknowledges support from the Research Council of Norway, project grant no. 205528. NR 14 TC 0 Z9 0 U1 3 U2 13 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 258 EP 260 DI 10.1016/j.nds.2014.08.071 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200187 ER PT J AU Bhatia, C Fallin, B Howell, C Tornow, W Gooden, M Kelley, J Arnold, C Bond, E Bredeweg, T Fowler, M Moody, W Rundberg, R Rusev, G Vieira, D Wilhelmy, J Becker, J Macri, R Ryan, C Sheets, S Stoyer, M Tonchev, A AF Bhatia, C. Fallin, B. Howell, C. Tornow, W. Gooden, M. Kelley, J. Arnold, C. Bond, E. Bredeweg, T. Fowler, M. Moody, W. Rundberg, R. Rusev, G. Vieira, D. Wilhelmy, J. Becker, J. Macri, R. Ryan, C. Sheets, S. Stoyer, M. Tonchev, A. TI Fission Product Yield Study of U-235, U-238 and Pu-239 Using Dual-Fission Ionization Chambers SO NUCLEAR DATA SHEETS LA English DT Article AB To resolve long-standing differences between LANL and LLNL regarding the correct fission basis for analysis of nuclear test data [1, 2], a collaboration between TUNL/LANL/LLNL has been established to perform high-precision measurements of neutron induced fission product yields. The main goal is to make a definitive statement about the energy dependence of the fission yields to an accuracy better than 2-3% between 1 and 15 MeV, where experimental data are very scarce. At TUNL, we have completed the design, fabrication and testing of three dual-fission chambers dedicated to U-235, U-238, and Pu-239. The dual-fission chambers were used to make measurements of the fission product activity relative to the total fission rate, as well as for high-precision absolute fission yield measurements. The activation method was employed, utilizing the mono-energetic neutron beams available at TUNL. Neutrons of 4.6, 9.0, and 14.5 MeV were produced via the H-2(d, n)(3) He reaction, and for neutrons at 14.8 MeV, the H-3(d, n)(4) He reaction was used. After activation, the induced gamma-ray activity of the fission products was measured for two months using high-resolution HPGe detectors in a low-background environment. Results for the yield of seven fission fragments of U-235, U-238, and Pu-239 and a comparison to available data at other energies are reported. For the first time results are available for neutron energies between 2 and 14 MeV. C1 [Bhatia, C.; Fallin, B.; Howell, C.; Tornow, W.] Duke Univ, TUNL, Durham, NC 27708 USA. [Gooden, M.; Kelley, J.] N Carolina State Univ, TUNL, Raleigh, NC 27695 USA. [Arnold, C.; Bond, E.; Bredeweg, T.; Fowler, M.; Moody, W.; Rundberg, R.; Rusev, G.; Vieira, D.; Wilhelmy, J.] Los Alamos Natl Lab, Los Alamos, NM USA. [Becker, J.; Macri, R.; Ryan, C.; Sheets, S.; Stoyer, M.; Tonchev, A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Bhatia, C (reprint author), McMaster Univ, 1280 Main St West, Hamilton, ON L8S 4K1, Canada. EM chitra@tunl.duke.edu FU U.S. Department of Energy by Triangle Universities Nuclear Laboratory through the Stewardship Science Academic Alliances Program [DE-FG52-09NA29465]; Los Alamos National Security and LLC [DE-AC52-06NA25396]; Lawrence Livermore National Security, LLC [DE-AC52-07NA27344] FX We would like to thank and acknowledge Mark Chadwick for his help and advocacy in undertaking these measurements. Work was performed under the auspices of the U.S. Department of Energy by Triangle Universities Nuclear Laboratory through the Stewardship Science Academic Alliances Program (grant DE-FG52-09NA29465), Los Alamos National Security and LLC (contract DE-AC52-06NA25396) Lawrence Livermore National Security, LLC (contract DE-AC52-07NA27344). NR 5 TC 0 Z9 0 U1 1 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 324 EP 327 DI 10.1016/j.nds.2014.08.089 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200205 ER PT J AU Belloni, F Andriamonje, S Berthoumieux, E Calviani, M Chiaveri, E Colonna, N Giomataris, Y Guerrero, C Gunsing, F Iguaz, FJ Kebbiri, M Pancin, J Papaevangelou, T Tsinganis, A Vlachoudis, V Altstadt, S Andrzejewski, J Audouin, L Barbagallo, M Becares, V Becvar, F Billowes, J Boccone, V Bosnar, D Brugger, M Calvino, F Cano-Ott, D Carrapico, C Cerutti, F Chiaveri, E Chin, M Cortes, G Corte-Giraldo, MA Diakaki, M Domingo-Pardo, C Duran, I Dzysiuk, N Eleftheriadis, C Ferrari, A Fraval, K Ganesan, S Garcia, AR Giubrone, G Gomez-Hornillos, MB Goncalves, IF Gonzalez-Romero, E Griesmayer, E Gurusamy, P Jenkins, DG Jericha, E Kadi, Y Kappeler, F Karadimos, D Koehler, P Kokkoris, M Krticka, M Kroll, J Langer, C Lederer, C Leeb, H Leong, LS Losito, R Manousos, A Marganiec, J Maritnez, T Massimi, C Mastinu, PF Mastromarco, M Meaze, M Mendoza, E Mengoni, A Milazzo, PM Mingrone, F Mirea, M Mondalaers, W Paradela, C Pavlik, A Perkowski, J Plompen, AJM Praena, J Quesada, JM Rauscher, T Reifarth, R Riego, A Roman, F Rubbia, C Sarmento, R Schillebeeckx, P Schmidt, S Tagliente, G Tain, JL Tarrio, D Tassan-Got, L Valenta, S Vannini, G Variale, V Vaz, P Ventura, A Versaci, R Vermeulen, MJ Vlastou, R Wallner, A Ware, T Weigand, M Weiss, C Wright, TJ Zugec, P AF Belloni, F. Andriamonje, S. Berthoumieux, E. Calviani, M. Chiaveri, E. Colonna, N. Giomataris, Y. Guerrero, C. Gunsing, F. Iguaz, F. J. Kebbiri, M. Pancin, J. Papaevangelou, T. Tsinganis, A. Vlachoudis, V. Altstadt, S. Andrzejewski, J. Audouin, L. Barbagallo, M. Becares, V. Becvar, F. Billowes, J. Boccone, V. Bosnar, D. Brugger, M. Calvino, F. Cano-Ott, D. Carrapico, C. Cerutti, F. Chiaveri, E. Chin, M. Cortes, G. Corte-Giraldo, M. A. Diakaki, M. Domingo-Pardo, C. Duran, I. Dzysiuk, N. Eleftheriadis, C. Ferrari, A. Fraval, K. Ganesan, S. Garcia, A. R. Giubrone, G. Gomez-Hornillos, M. B. Goncalves, I. F. Gonzalez-Romero, E. Griesmayer, E. Gurusamy, P. Jenkins, D. G. Jericha, E. Kadi, Y. Kaeppeler, F. Karadimos, D. Koehler, P. Kokkoris, M. Krticka, M. Kroll, J. Langer, C. Lederer, C. Leeb, H. Leong, L. S. Losito, R. Manousos, A. Marganiec, J. Maritnez, T. Massimi, C. Mastinu, P. F. Mastromarco, M. Meaze, M. Mendoza, E. Mengoni, A. Milazzo, P. M. Mingrone, F. Mirea, M. Mondalaers, W. Paradela, C. Pavlik, A. Perkowski, J. Plompen, A. J. M. Praena, J. Quesada, J. M. Rauscher, T. Reifarth, R. Riego, A. Roman, F. Rubbia, C. Sarmento, R. Schillebeeckx, P. Schmidt, S. Tagliente, G. Tain, J. L. Tarrio, D. Tassan-Got, L. Valenta, S. Vannini, G. Variale, V. Vaz, P. Ventura, A. Versaci, R. Vermeulen, M. J. Vlastou, R. Wallner, A. Ware, T. Weigand, M. Weiss, C. Wright, T. J. Zugec, P. TI A Micromegas Detector for Neutron Beam Imaging at the n_TOF Facility at CERN SO NUCLEAR DATA SHEETS LA English DT Article AB Micromegas (Micro-MEsh Gaseous Structure) detectors are gas detectors consisting of a stack of one ionization and one proportional chamber. A micromesh separates the two communicating regions, where two different electric fields establish respectively a charge drift and a charge multiplication regime. The n_TOF facility at CERN provides a white neutron beam (from thermal up to GeV neutrons) for neutron induced cross section measurements. These measurements need a perfect knowlodge of the incident neutron beam, in particular regarding its spatial profile. A position sensitive micromegas detector equipped with a B-10 based neutron/charged particle converter has been extensively used at the n_TOF facility for characterizing the neutron beam profile and extracting the beam interception factor for samples of different size. The boron converter allowed to scan the energy region of interest for neutron induced capture reactions as a function of the neutron energy, determined by the time of flight. Experimental results will be presented and compared to simulations, performed by means of the FLUKA code. C1 [Belloni, F.; Berthoumieux, E.; Giomataris, Y.; Gunsing, F.; Iguaz, F. J.; Kebbiri, M.; Pancin, J.; Papaevangelou, T.; Chiaveri, E.; Fraval, K.] CEA Saclay, Irfu, F-91191 Gif Sur Yvette, France. [Andriamonje, S.; Calviani, M.; Chiaveri, E.; Guerrero, C.; Tsinganis, A.; Vlachoudis, V.; Boccone, V.; Brugger, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Ferrari, A.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Versaci, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Colonna, N.; Barbagallo, M.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Tsinganis, A.; Diakaki, M.; Karadimos, D.; Kokkoris, M.; Vlastou, R.] Natl Tech Univ Athens, Athens, Greece. [Altstadt, S.; Langer, C.; Lederer, C.; Reifarth, R.; Schmidt, S.; Weigand, M.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Andrzejewski, J.; Marganiec, J.; Perkowski, J.] Univ Lodz, PL-90131 Lodz, Poland. [Audouin, L.; Leong, L. S.; Tassan-Got, L.] IPN, CNRS, IN2P3, Orsay, France. [Becares, V.; Cano-Ott, D.; Garcia, A. R.; Gonzalez-Romero, E.; Maritnez, T.; Mendoza, E.] CIEMAT, E-28040 Madrid, Spain. [Becvar, F.; Krticka, M.; Kroll, J.; Valenta, S.] Charles Univ Prague, Prague, Czech Republic. [Billowes, J.; Ware, T.; Wright, T. J.] Univ Manchester, Manchester, Lancs, England. [Bosnar, D.; Zugec, P.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia. [Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, Barcelona, Spain. [Carrapico, C.; Goncalves, I. F.; Sarmento, R.; Vaz, P.] Univ Tecn Lisboa, Inst Super Tecn, Inst Tecnol & Nucl, P-1096 Lisbon, Portugal. [Corte-Giraldo, M. A.; Praena, J.; Quesada, J. M.] Univ Seville, Seville, Spain. [Domingo-Pardo, C.; Giubrone, G.; Tain, J. L.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46003 Valencia, Spain. [Duran, I.; Paradela, C.; Tarrio, D.] Univ Santiago de Compostela, Santiago, Spain. [Dzysiuk, N.; Mastinu, P. F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Milan, Italy. [Eleftheriadis, C.; Manousos, A.] Aristotle Univ Thessaloniki, GR-54006 Thessaloniki, Greece. [Ganesan, S.; Gurusamy, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Griesmayer, E.; Jericha, E.; Leeb, H.; Weiss, C.] Vienna Univ Technol, Inst Atom, Vienna, Austria. [Jenkins, D. G.; Vermeulen, M. J.] Univ York, York YO10 5DD, N Yorkshire, England. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Koehler, P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Lederer, C.; Pavlik, A.; Wallner, A.] Univ Vienna, Fac Phys, A-1010 Vienna, Austria. [Massimi, C.; Mingrone, F.; Vannini, G.] Univ Bologna, Dipartimento Fis, I-40126 Bologna, Italy. [Massimi, C.; Mingrone, F.; Vannini, G.] Sez INFN Bologna, Bologna, Italy. [Mengoni, A.; Ventura, A.] Agenzia Nazl Nuove Tecnol, Energia Sviluppo Econ Sostenibile ENEA, Bologna, Italy. [Milazzo, P. M.] Ist Nazl Fis Nucl, Trieste, Italy. [Mirea, M.; Roman, F.] Horia Hulubei Natl Inst Phys & Nucl Engn, IFIN HH, Bucharest, Romania. [Mondalaers, W.; Plompen, A. J. M.; Schillebeeckx, P.] European Commiss JRC, Inst Reference Mat & Measurements, B-2440 Geel, Belgium. [Rauscher, T.] Univ Basel, Basel, Switzerland. [Rubbia, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. RP Belloni, F (reprint author), CEA Saclay, Irfu, F-91191 Gif Sur Yvette, France. EM francesca.belloni@cea.fr RI Mendoza Cembranos, Emilio/K-5789-2014; Becares, Vicente/K-4514-2014; Papaevangelou, Thomas/G-2482-2016; Vaz, Pedro/K-2464-2013; Rauscher, Thomas/D-2086-2009; Mirea, Mihail/C-2297-2011; Cano Ott, Daniel/K-4945-2014; Gonzalez Romero, Enrique/L-7561-2014; Duran, Ignacio/H-7254-2015; Massimi, Cristian/K-2008-2015; Paradela, Carlos/J-1492-2012; Chin, Mary Pik Wai/B-6644-2012; Calvino, Francisco/K-5743-2014; Langer, Christoph/L-3422-2016; Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012; OI Mendoza Cembranos, Emilio/0000-0002-2843-1801; Becares, Vicente/0000-0003-3434-9086; Papaevangelou, Thomas/0000-0003-2829-9158; Vaz, Pedro/0000-0002-7186-2359; Rauscher, Thomas/0000-0002-1266-0642; Mirea, Mihail/0000-0002-9333-6595; Cano Ott, Daniel/0000-0002-9568-7508; Gonzalez Romero, Enrique/0000-0003-2376-8920; Massimi, Cristian/0000-0003-2499-5586; Chin, Mary Pik Wai/0000-0001-5176-9723; Calvino, Francisco/0000-0002-7198-4639; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038; Paradela Dobarro, Carlos/0000-0003-0175-8334; Iguaz Gutierrez, Francisco Jose/0000-0001-6327-9369; Koehler, Paul/0000-0002-6717-0771; Garcia Rios, Aczel Regino/0000-0002-7955-1475 NR 5 TC 0 Z9 0 U1 4 U2 11 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 365 EP 367 DI 10.1016/j.nds.2014.08.100 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200216 ER PT J AU Perdue, BA Taddeucci, TN Haight, RC Bredeweg, T Devlin, M Fotiades, N Jandel, M Laptev, A Lee, HY Nelson, RO O'Donnell, JM Ullmann, JL Wender, SA Wu, CY Kwan, E Chyzh, A Henderson, RA Gostic, JM AF Perdue, B. A. Taddeucci, T. N. Haight, R. C. Bredeweg, T. Devlin, M. Fotiades, N. Jandel, M. Laptev, A. Lee, H. Y. Nelson, R. O. O'Donnell, J. M. Ullmann, J. L. Wender, S. A. Wu, C. Y. Kwan, E. Chyzh, A. Henderson, R. A. Gostic, J. M. TI Development of an Array of Liquid Scintillators to Measure the Prompt Fission Neutron Spectrum at LANSCE SO NUCLEAR DATA SHEETS LA English DT Article ID DETECTION EFFICIENCY AB Higher quality measurements of outgoing prompt neutron spectra from neutron-induced fission as a function of the incoming neutron energy are needed. These data can be used in designing new fast reactors, predicting criticality for safety analyses, and developing techniques for global security applications. As part of the program to measure the prompt fission neutron spectra (PFNS) from the fission of Pu-239 at the Los Alamos Neutron Science Center, we are developing a new array of liquid-scintillator detectors. This array will be used to measure the PFNS over a range of outgoing neutron energies from approximately 600 keV to 12 MeV and incident neutron energies from 0.5 to 30 MeV. A complete characterization of the detectors and the array as a whole will be carried out, targeted at understanding the light-output curves, efficiencies, and the neutron multiple-scattering backgrounds. C1 [Perdue, B. A.; Taddeucci, T. N.; Haight, R. C.; Bredeweg, T.; Devlin, M.; Fotiades, N.; Jandel, M.; Laptev, A.; Lee, H. Y.; Nelson, R. O.; O'Donnell, J. M.; Ullmann, J. L.; Wender, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Wu, C. Y.; Kwan, E.; Chyzh, A.; Henderson, R. A.; Gostic, J. M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Perdue, BA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM perdue@lanl.gov RI Laptev, Alexander/D-4686-2009; Devlin, Matthew/B-5089-2013; OI Laptev, Alexander/0000-0002-9759-9907; Devlin, Matthew/0000-0002-6948-2154; Fotiadis, Nikolaos/0000-0003-1410-3871; Wender, Stephen/0000-0002-2446-5115 FU U.S. Department of Energy (LANL) [DEAC5206NA25396]; U.S. Department of Energy (LLNL) [DEAC5207NA27344] FX This work benefits from the LANSCE accelerator facility and is supported by the U.S. Department of Energy under contracts DEAC5206NA25396 (LANL) and DEAC5207NA27344 (LLNL). NR 4 TC 2 Z9 2 U1 0 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 371 EP 372 DI 10.1016/j.nds.2014.08.102 PG 2 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200218 ER PT J AU Meharchand, R Asner, DM Baker, RG Bundgaard, J Burgett, E Cunningham, M Deaven, J Duke, DL Greife, U Grimes, S Heffner, M Hill, T Isenhower, D Klay, JL Kleinrath, V Kornilov, N Laptev, AB Loveland, W Massey, TN Qu, H Ruz, J Sangiorgio, S Seilhan, B Snyder, L Stave, S Tatishvili, G Thornton, RT Tovesson, F Towell, D Towell, RS Watson, S Wendt, B Wood, L AF Meharchand, R. Asner, D. M. Baker, R. G. Bundgaard, J. Burgett, E. Cunningham, M. Deaven, J. Duke, D. L. Greife, U. Grimes, S. Heffner, M. Hill, T. Isenhower, D. Klay, J. L. Kleinrath, V. Kornilov, N. Laptev, A. B. Loveland, W. Massey, T. N. Qu, H. Ruz, J. Sangiorgio, S. Seilhan, B. Snyder, L. Stave, S. Tatishvili, G. Thornton, R. T. Tovesson, F. Towell, D. Towell, R. S. Watson, S. Wendt, B. Wood, L. TI Commissioning the NIFFTE Time Projection Chamber: Towards the U-238/U-235 (n,f) Cross-section Ratio SO NUCLEAR DATA SHEETS LA English DT Article AB The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration is developing a Time Projection Chamber (TPC) to measure neutron-induced fission cross sections with unprecedented accuracy. Modifying TPC technology for nuclear physics applications is a challenging endeavor, and frequent testing and evaluation is required to ensure that all components are behaving as expected. In-beam tests of the NIFFTE TPC at the Los Alamos Neutron Science Center (LANSCE) commenced in 2010. An overview of the NIFFTE TPC experiments performed at LANSCE will be presented, along with preliminary performance results. C1 [Meharchand, R.; Laptev, A. B.; Tovesson, F.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Asner, D. M.; Stave, S.; Tatishvili, G.; Wood, L.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Baker, R. G.; Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Bundgaard, J.; Duke, D. L.; Greife, U.] Colorado Sch Mines, Golden, CO 80401 USA. [Burgett, E.; Deaven, J.; Kleinrath, V.; Wendt, B.] Idaho State Univ, Pocatello, ID 83209 USA. [Cunningham, M.; Heffner, M.; Ruz, J.; Sangiorgio, S.; Seilhan, B.; Snyder, L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grimes, S.; Kornilov, N.; Massey, T. N.] Ohio Univ, Athens, OH 45701 USA. [Hill, T.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Isenhower, D.; Qu, H.; Thornton, R. T.; Towell, D.; Towell, R. S.; Watson, S.] Abilene Christian Univ, Abilene, TX 79699 USA. [Loveland, W.] Oregon State Univ, Corvallis, OR 97331 USA. RP Meharchand, R (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM meharchand@lanl.gov RI Laptev, Alexander/D-4686-2009; OI Laptev, Alexander/0000-0002-9759-9907; Geppert-Kleinrath, Verena/0000-0002-6869-5772 FU U.S. Department of Energy by Los Alamos National Security, LLC [DE-AC52-06NA25396]; U.S. Department of Energy by Lawrence Livermore National Security, LLC [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Los Alamos National Security, LLC under contract DE-AC52-06NA25396 and by Lawrence Livermore National Security, LLC under contract DE-AC52-07NA27344. NR 6 TC 0 Z9 0 U1 0 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 373 EP 376 DI 10.1016/j.nds.2014.08.103 PG 4 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200219 ER PT J AU Wood, L Asner, DM Baker, RG Bundgaard, J Burgett, E Cunningham, M Deaven, J Duke, DL Greife, U Grimes, S Heffner, M Hill, T Isenhower, D Klay, JL Kleinrath, V Kornilov, N Laptev, AB Loveland, W Massey, TN Meharchand, R Qu, H Ruz, J Sangiorgio, S Seilhan, B Snyder, L Stave, S Tatishvili, G Thornton, RT Tovesson, F Towell, D Towell, RS Watson, S Wendt, B AF Wood, L. Asner, D. M. Baker, R. G. Bundgaard, J. Burgett, E. Cunningham, M. Deaven, J. Duke, D. L. Greife, U. Grimes, S. Heffner, M. Hill, T. Isenhower, D. Klay, J. L. Kleinrath, V. Kornilov, N. Laptev, A. B. Loveland, W. Massey, T. N. Meharchand, R. Qu, H. Ruz, J. Sangiorgio, S. Seilhan, B. Snyder, L. Stave, S. Tatishvili, G. Thornton, R. T. Tovesson, F. Towell, D. Towell, R. S. Watson, S. Wendt, B. TI An Ethernet-based Data Acquisition System for the NIFFTE Time Projection Chamber SO NUCLEAR DATA SHEETS LA English DT Article AB When fully instrumented, the NIFFTE Time Projection Chamber will consist of nearly 6000 channels, each of which requires a preamplifier, ADC, and digital readout. To minimize channel cost and size, the EtherDAQ data acquisition system utilizes off-the-shelf FPGA and Ethernet fiber technology. This application of commercially-available components made it possible to meet the requirements of the DAQ system with considerably less development cost and time than the a customized ASIC solution, and provides considerable flexibility in the final design. The detailed design and current status of the preamplifier and EtherDAQ boards will be discussed. C1 [Wood, L.; Asner, D. M.; Stave, S.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Baker, R. G.; Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Bundgaard, J.; Duke, D. L.; Greife, U.] Colorado Sch Mines, Golden, CO 80401 USA. [Burgett, E.; Deaven, J.; Kleinrath, V.; Wendt, B.] Idaho State Univ, Pocatello, ID 83209 USA. [Cunningham, M.; Heffner, M.; Ruz, J.; Sangiorgio, S.; Seilhan, B.; Snyder, L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grimes, S.; Kornilov, N.; Massey, T. N.] Ohio Univ, Athens, OH 45701 USA. [Hill, T.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Isenhower, D.; Qu, H.; Thornton, R. T.; Towell, D.; Towell, R. S.; Watson, S.] Abilene Christian Univ, Abilene, TX 79699 USA. [Laptev, A. B.; Meharchand, R.; Tovesson, F.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Loveland, W.] Oregon State Univ, Corvallis, OR 97331 USA. RP Wood, L (reprint author), Pacific NW Natl Lab, Richland, WA 99354 USA. EM lynn.wood@pnnl.gov RI Laptev, Alexander/D-4686-2009; OI Laptev, Alexander/0000-0002-9759-9907; Geppert-Kleinrath, Verena/0000-0002-6869-5772 FU US Department of Energy, Office of Nuclear Energy FX This work was funded in part by the US Department of Energy, Office of Nuclear Energy. NR 2 TC 1 Z9 1 U1 0 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 377 EP 379 DI 10.1016/j.nds.2014.08.104 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200220 ER PT J AU Stave, S Asner, DM Baker, RG Bundgaard, J Burgett, E Cunningham, M Deaven, J Duke, DL Greife, U Grimes, S Heffner, M Hill, T Isenhower, D Klay, JL Kleinrath, V Kornilov, N Laptev, AB Loveland, W Massey, TN Meharchand, R Qu, H Ruz, J Sangiorgio, S Seilhan, B Snyder, L Tatishvili, G Thornton, RT Tovesson, F Towell, D Towell, RS Watson, S Wendt, B Wood, L AF Stave, S. Asner, D. M. Baker, R. G. Bundgaard, J. Burgett, E. Cunningham, M. Deaven, J. Duke, D. L. Greife, U. Grimes, S. Heffner, M. Hill, T. Isenhower, D. Klay, J. L. Kleinrath, V. Kornilov, N. Laptev, A. B. Loveland, W. Massey, T. N. Meharchand, R. Qu, H. Ruz, J. Sangiorgio, S. Seilhan, B. Snyder, L. Tatishvili, G. Thornton, R. T. Tovesson, F. Towell, D. Towell, R. S. Watson, S. Wendt, B. Wood, L. TI The Data Analysis Framework for the NIFFTE Fission Time Projection Chamber SO NUCLEAR DATA SHEETS LA English DT Article AB The NIFFTE collaboration has developed a time projection chamber to study neutron-induced fission events in actinide targets by tracking and identifying fission fragments in three dimensions as they traverse a gas volume. This paper will provide an overview of the analysis software that has been developed by the NIFFTE collaboration, as well as examples of its success in analyzing data. C1 [Stave, S.; Asner, D. M.; Tatishvili, G.; Wood, L.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Baker, R. G.; Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Bundgaard, J.; Duke, D. L.; Greife, U.] Colorado Sch Mines, Golden, CO 80401 USA. [Burgett, E.; Deaven, J.; Kleinrath, V.; Wendt, B.] Idaho State Univ, Pocatello, ID 83209 USA. [Cunningham, M.; Heffner, M.; Ruz, J.; Sangiorgio, S.; Seilhan, B.; Snyder, L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grimes, S.; Kornilov, N.; Massey, T. N.] Ohio Univ, Athens, OH 45701 USA. [Hill, T.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Isenhower, D.; Qu, H.; Thornton, R. T.; Towell, D.; Towell, R. S.; Watson, S.] Abilene Christian Univ, Abilene, TX 79699 USA. [Laptev, A. B.; Meharchand, R.; Tovesson, F.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Loveland, W.] Oregon State Univ, Corvallis, OR 97331 USA. RP Stave, S (reprint author), Pacific NW Natl Lab, Richland, WA 99354 USA. EM sean.stave@pnnl.gov RI Laptev, Alexander/D-4686-2009; OI Laptev, Alexander/0000-0002-9759-9907; Geppert-Kleinrath, Verena/0000-0002-6869-5772 FU US Department of Energy, Office of Nuclear Energy FX This work was funded in part by the US Department of Energy, Office of Nuclear Energy. NR 11 TC 1 Z9 1 U1 0 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 380 EP 382 DI 10.1016/j.nds.2014.08.105 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200221 ER PT J AU Loveland, W Yao, L Asner, DM Baker, RG Bundgaard, J Burgett, E Cunningham, M Deaven, J Duke, DL Greife, U Grimes, S Heffner, M Hill, T Isenhower, D Klay, JL Kleinrath, V Kornilov, N Laptev, AB Massey, TN Meharchand, R Qu, H Ruz, J Sangiorgio, S Selhan, B Snyder, L Stave, S Tatishvili, G Thornton, RT Tovesson, F Towell, D Towell, RS Watson, S Wendt, B Wood, L AF Loveland, W. Yao, L. Asner, D. M. Baker, R. G. Bundgaard, J. Burgett, E. Cunningham, M. Deaven, J. Duke, D. L. Greife, U. Grimes, S. Heffner, M. Hill, T. Isenhower, D. Klay, J. L. Kleinrath, V. Kornilov, N. Laptev, A. B. Massey, T. N. Meharchand, R. Qu, H. Ruz, J. Sangiorgio, S. Selhan, B. Snyder, L. Stave, S. Tatishvili, G. Thornton, R. T. Tovesson, F. Towell, D. Towell, R. S. Watson, S. Wendt, B. Wood, L. TI Targets for Precision Measurements SO NUCLEAR DATA SHEETS LA English DT Article ID NUCLEAR TARGETS; FISSION; FILMS AB The general properties needed in targets (sources) for high precision, high accuracy measurements are reviewed. The application of these principles to the problem of developing targets for the Fission TPC is described. Longer term issues, such as the availability of actinide materials, improved knowledge of energy losses and straggling and the stability of targets during irradiation are also discussed. C1 [Loveland, W.; Yao, L.] Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA. [Asner, D. M.; Stave, S.; Tatishvili, G.; Wood, L.] Pacific NW Natl Lab, Richland, WA 99351 USA. [Baker, R. G.; Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Bundgaard, J.; Duke, D. L.; Greife, U.] Colorado Sch Mines, Golden, CO 80401 USA. [Burgett, E.; Deaven, J.; Kleinrath, V.; Wendt, B.] Idaho State Univ, Pocatello, ID 83209 USA. [Cunningham, M.; Heffner, M.; Ruz, J.; Sangiorgio, S.; Selhan, B.; Snyder, L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grimes, S.; Kornilov, N.; Massey, T. N.] Ohio Univ, Athens, OH 45701 USA. [Hill, T.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Isenhower, D.; Qu, H.; Thornton, R. T.; Towell, D.; Towell, R. S.; Watson, S.] Abilene Christian Univ, Abilene, TX 79699 USA. [Laptev, A. B.; Meharchand, R.; Tovesson, F.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Loveland, W (reprint author), Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA. EM lovelanw@onid.orst.edu RI Laptev, Alexander/D-4686-2009; OI Laptev, Alexander/0000-0002-9759-9907; Geppert-Kleinrath, Verena/0000-0002-6869-5772 FU Office of Nuclear Physics, Office of Science of the U.S. Department of Energy [DE-FG06-97ER41026] FX The authors are indebted to Dr. John D. Baker (deceased) who participated in developing many of the ideas used preparing targets for the Fission TPC, and Dr. Chris McGrath who purified the 235UF4 for use in this project. This work was funded by the Office of Nuclear Physics, Office of Science of the U.S. Department of Energy, under Contract No. DE-FG06-97ER41026. NR 13 TC 1 Z9 1 U1 2 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 383 EP 385 DI 10.1016/j.nds.2014.08.106 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200222 ER PT J AU Snyder, L Asner, DM Baker, RG Bundgaard, J Burgett, E Cunningham, M Deaven, J Duke, DL Greife, U Grimes, S Heffner, M Hill, T Isenhower, D Klay, JL Kleinrath, V Kornilov, N Laptev, AB Loveland, W Massey, TN Meharchand, R Qu, H Ruz, J Sangiorgio, S Seilhan, B Stave, S Tatishvili, G Thornton, RT Tovesson, F Towell, D Towell, RS Watson, S Wendt, B Wood, L AF Snyder, L. Asner, D. M. Baker, R. G. Bundgaard, J. Burgett, E. Cunningham, M. Deaven, J. Duke, D. L. Greife, U. Grimes, S. Heffner, M. Hill, T. Isenhower, D. Klay, J. L. Kleinrath, V. Kornilov, N. Laptev, A. B. Loveland, W. Massey, T. N. Meharchand, R. Qu, H. Ruz, J. Sangiorgio, S. Seilhan, B. Stave, S. Tatishvili, G. Thornton, R. T. Tovesson, F. Towell, D. Towell, R. S. Watson, S. Wendt, B. Wood, L. CA NIFFTE Collaboration TI Measuring the alpha/SF Branching Ratio of Cf-252 with the NIFFTE TPC SO NUCLEAR DATA SHEETS LA English DT Article ID THICK URANIUM-OXIDE; SCATTERING CORRECTION; FISSION FRAGMENTS; PARTICLE SOURCES; BACKSCATTERING AB A fission TPC is being developed to measure the energy-dependent neutron induced fission cross sections of the major and minor actinides to an accuracy of better than 1%. Achieving such an accuracy will depend in part, on the ability of the TPC to provide precise tracking and identification of charged particles. A measurement of the a-decay to spontaneous fission branching ratio of Cf-252 used to benchmark the performance of the TPC will be discussed. C1 [Snyder, L.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Asner, D. M.; Stave, S.; Tatishvili, G.; Wood, L.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Baker, R. G.; Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Bundgaard, J.; Duke, D. L.; Greife, U.] Colorado Sch Mines, Golden, CO 80401 USA. [Burgett, E.; Deaven, J.; Kleinrath, V.; Wendt, B.] Idaho State Univ, Pocatello, ID 83209 USA. [Cunningham, M.; Heffner, M.; Ruz, J.; Sangiorgio, S.; Seilhan, B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grimes, S.; Kornilov, N.; Massey, T. N.] Ohio Univ, Athens, OH 45701 USA. [Hill, T.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Isenhower, D.; Qu, H.; Thornton, R. T.; Towell, D.; Towell, R. S.; Watson, S.] Abilene Christian Univ, Abilene, TX 79699 USA. [Laptev, A. B.; Meharchand, R.; Tovesson, F.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Loveland, W.] Oregon State Univ, Corvallis, OR 97331 USA. RP Snyder, L (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM snyder35@llnl.gov RI Laptev, Alexander/D-4686-2009 OI Laptev, Alexander/0000-0002-9759-9907 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 13 TC 0 Z9 0 U1 0 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 386 EP 388 DI 10.1016/j.nds.2014.08.107 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200223 ER PT J AU Meierbachtol, K Tovesson, F Arnold, CW Laptev, AB Bredeweg, TA Jandel, M Nelson, RO White, MC AF Meierbachtol, K. Tovesson, F. Arnold, C. W. Laptev, A. B. Bredeweg, T. A. Jandel, M. Nelson, R. O. White, M. C. TI Development of an Ionization Chamber for the SPIDER Fission Fragment Detector SO NUCLEAR DATA SHEETS LA English DT Article AB The ionization chamber component of the SPIDER detector has been designed to measure energy loss and kinetic energy of fragments produced through neutron-induced fission with energy resolutions of <1% and a time-dependent signal collection. Important design elements implemented are an axial configuration of the electrodes for improved energy loss and measurement and a thin silicon nitride entrance window to minimize both energy loss and energy straggling of the incoming fragments. High energy resolution and improved charge resolution from the ionization chamber are combined with the high precision of the upstream time-of-flight component of SPIDER to achieve resolutions in mass and nuclear charge of 1 AMU and Z=1. A discussion of the present resolution capabilities of the ionization chamber will be presented. C1 [Meierbachtol, K.; Tovesson, F.; Laptev, A. B.; Nelson, R. O.] Los Alamos Natl Lab, LANSCE NS, Los Alamos, NM 87545 USA. [Arnold, C. W.; Bredeweg, T. A.; Jandel, M.; White, M. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Meierbachtol, K (reprint author), Los Alamos Natl Lab, LANSCE NS, Los Alamos, NM 87545 USA. EM meierbachtol@lanl.gov RI Laptev, Alexander/D-4686-2009; OI Laptev, Alexander/0000-0002-9759-9907; White, Morgan/0000-0003-3876-421X FU US Department of Energy, Los Alamos National Security, LLC [DE-AC52-06NA25396]; LDRD Project [20110037DR.LA-UR-13-21662] FX This work was performed under the auspices of the US Department of Energy by Los Alamos National Security, LLC under contract DE-AC52-06NA25396 and grants for LDRD Project 20110037DR.LA-UR-13-21662. NR 2 TC 2 Z9 2 U1 0 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 389 EP 391 DI 10.1016/j.nds.2014.08.108 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200224 ER PT J AU Arnold, CW Tovesson, F Meierbachtol, KC Laptev, AB Bredeweg, TA Jandel, M Nelson, RO White, MC AF Arnold, C. W. Tovesson, F. Meierbachtol, K. C. Laptev, A. B. Bredeweg, T. A. Jandel, M. Nelson, R. O. White, M. C. TI Precision Velocity Measurements of Fission Fragments Using the SPIDER Detector SO NUCLEAR DATA SHEETS LA English DT Article AB The SPectrometer for Ion DEtermination in fission Research (SPIDER) measures both position and time-of-flight (TOF) of charged particles using a system of thin carbon foils, electrostatic mirrors, microchannel plates, delay-line anodes, and a fast TDC. Tests have been conducted using Th-229 and the alpha emitters in its decay chain. To date, timing resolution of 200 ps (FWHM) has been achieved corresponding to roughly 0.5% uncertainty in velocity measurements of fission fragments over a flight path of 52.1 cm. This velocity resolution, in combination with demonstrated fragment energy resolution is sufficient for 1 amu resolution of light mass fragments. C1 [Arnold, C. W.; Bredeweg, T. A.; Jandel, M.; White, M. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Tovesson, F.; Meierbachtol, K. C.; Laptev, A. B.; Nelson, R. O.] Los Alamos Natl Lab, LANSCE NS, Los Alamos, NM 87545 USA. RP Arnold, CW (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM arnold@lanl.gov RI Laptev, Alexander/D-4686-2009; OI Laptev, Alexander/0000-0002-9759-9907; White, Morgan/0000-0003-3876-421X FU U.S. Department of Energy, Los Alamos National Security, LLC [DE-AC52-06NA25396]; LDRD Project [20110037DR] FX This work has been performed under the auspices of the U.S. Department of Energy by Los Alamos National Security, LLC (contract DE-AC52-06NA25396 and grants for LDRD Project 20110037DR). NR 1 TC 1 Z9 1 U1 0 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 392 EP 394 DI 10.1016/j.nds.2014.08.109 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200225 ER PT J AU Kornilov, NV Grimes, SM Massey, TN Brient, CE Carter, DE O'Donnell, JE Bateman, FB Carlson, AD Haight, RC Boukharouba, N AF Kornilov, N. V. Grimes, S. M. Massey, T. N. Brient, C. E. Carter, D. E. O'Donnell, J. E. Bateman, F. B. Carlson, A. D. Haight, R. C. Boukharouba, N. TI Development of a New Method for Measurement of Neutron Detector Efficiency up to 20 MeV SO NUCLEAR DATA SHEETS LA English DT Article ID CALIBRATION; ENERGY AB A new approach to neutron detector efficiency detemination has been taken. A neutron detector has been calibrated with a Cf-252 source at low energy. The calibration can be extended to energies above 8 MeV with accelerator-based neutron sources. This techniques uses the fact that the cross section for a symmetric reaction with nucleus of atomic number A yielding a final nucleus with atomic number (2A - 1) and a neutron A + A --> (2A - 1) + n. This reaction must be symmetric about 90 degrees in the center-of-mass system. The laboratory energies for the neutrons at the paired energies differ substantially. Thus, an efficiency known at one of the two angles can be used to determine the efficiency to higher energies or, for a negative Q, to lower neutron energies. C1 [Kornilov, N. V.; Grimes, S. M.; Massey, T. N.; Brient, C. E.; Carter, D. E.; O'Donnell, J. E.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Bateman, F. B.; Carlson, A. D.] NIST, Gaithersburg, MD 20899 USA. [Haight, R. C.] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA. [Boukharouba, N.] Univ Guelma, Dept Phys, Guelma 24000, Algeria. RP Massey, TN (reprint author), Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. EM massey@ohio.edu NR 23 TC 1 Z9 1 U1 1 U2 1 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAY PY 2014 VL 119 BP 413 EP 415 DI 10.1016/j.nds.2014.08.116 PG 3 WC Physics, Nuclear SC Physics GA AY6XN UT WOS:000347706200232 ER PT J AU Sharma, S Mulder, ML Sack, A Schroeder, K Hammack, R AF Sharma, Shikha Mulder, Michon L. Sack, Andrea Schroeder, Karl Hammack, Richard TI Isotope Approach to Assess Hydrologic Connections During Marcellus Shale Drilling SO GROUNDWATER LA English DT Article ID DISSOLVED INORGANIC CARBON; FRESH-WATER ENVIRONMENTS; SALINE FORMATION WATERS; ACID-MINE DRAINAGE; NATURAL-GAS; STABLE-ISOTOPES; BIOGENIC METHANE; MICHIGAN BASIN; CO2 REDUCTION; ORIGIN AB Water and gas samples were collected from (1) nine shallow groundwater aquifers overlying Marcellus Shale in north-central West Virginia before active shale gas drilling, (2) wells producing gas from Upper Devonian sands and Middle Devonian Marcellus Shale in southwestern Pennsylvania, (3) coal-mine water discharges in southwestern Pennsylvania, and (4) streams in southwestern Pennsylvania and north-central West Virginia. Our preliminary results demonstrate that the oxygen and hydrogen isotope composition of water, carbon isotope composition of dissolved inorganic carbon, and carbon and hydrogen isotope compositions of methane in Upper Devonian sands and Marcellus Shale are very different compared with shallow groundwater aquifers, coal-mine waters, and stream waters of the region. Therefore, spatiotemporal stable isotope monitoring of the different sources of water before, during, and after hydraulic fracturing can be used to identify migrations of fluids and gas from deep formations that are coincident with shale gas drilling. C1 [Sharma, Shikha; Mulder, Michon L.; Sack, Andrea] W Virginia Univ, Dept Geol & Geog, Morgantown, WV 26506 USA. [Sharma, Shikha; Sack, Andrea] Natl Technol Lab Reg Univ Alliance, Berkeley, CA USA. [Schroeder, Karl; Hammack, Richard] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Sharma, S (reprint author), W Virginia Univ, Dept Geol & Geog, Morgantown, WV 26506 USA. EM shikha.sharma@mail.wvu.edu FU USGS 104b grant through the West Virginia Water Research Institute; collaborative initiative of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA) under the RES [DE-FE0004000] FX The groundwater sampling was supported by USGS 104b grant to S. Sharma through the West Virginia Water Research Institute. The sampling from gas producing wells in Upper Devonian sands and Marcellus Shale was supported by a collaborative initiative of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA) under the RES contract DE-FE0004000. Dr. Jennifer Weidhaas is thanked for the q-PCR analysis of the produced water sample. Lindsey Bowman and Adam Pelak are also thanked for their help in the field and laboratory. All groundwater and surface water sampling in north-central West Virginia was done in collaboration with Douglas Chambers, Jeremy White, and Katherine Paybins of the USGS West Virginia Water Science Center. Their prior understanding of dissolved methane in the area, cooperation in field sampling and site access aided this research invaluably. Comments and suggestions from Drs Stotler, Schwartz, and two anonymous reviewers greatly helped in revising this manuscript. NR 74 TC 8 Z9 8 U1 1 U2 25 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0017-467X EI 1745-6584 J9 GROUNDWATER JI Groundwater PD MAY-JUN PY 2014 VL 52 IS 3 BP 424 EP 433 DI 10.1111/gwat.12083 PG 10 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA AZ1CY UT WOS:000347979100013 PM 23772970 ER PT J AU Langhorst, B Lillo, TM Chu, HS AF Langhorst, Benjamin Lillo, Thomas M. Chu, Henry S. TI A Residual Mass Ballistic Testing Method to Compare Armor Materials or Components (Residual Mass Ballistic Testing Method) SO JOURNAL OF TESTING AND EVALUATION LA English DT Article DE ballistic testing; perforation; statistics; armor; penetration ID LONG-ROD PENETRATION; IMPACT; PROJECTILE; MECHANICS; TARGETS; PLATES; MODEL AB A statistics based ballistic test method is presented for use when comparing multiple groups of test articles of unknown relative ballistic perforation resistance. The method is intended to be more efficient than many traditional methods for research and development testing. To establish the validity of the method, it is employed in this study to compare test groups of known relative ballistic performance. Multiple groups of test articles were perforated using consistent projectiles and impact conditions. Test groups were made of rolled homogeneous armor (RHA) plates and differed in thickness. After perforation, each residual projectile was captured behind the target and its mass was measured. The residual masses measured for each test group were analyzed to provide ballistic performance rankings with associated confidence levels. When compared to traditional V50 methods, the residual mass (RM) method was found to require fewer test events and be more tolerant of variations in impact conditions. C1 [Langhorst, Benjamin; Lillo, Thomas M.; Chu, Henry S.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Langhorst, B (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM Benjamin.Langhorst@inl.gov; Thomas.Lillo@inl.gov; Henry.Chu@inl.gov RI Lilllo, Thomas/S-5031-2016 OI Lilllo, Thomas/0000-0002-7572-7883 FU Laboratory Directed Research and Development program at Idaho National Laboratory [12-017]; U.S. Department of Energy [DE-AC07-05ID14517] FX This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. This work was funded by the Laboratory Directed Research and Development program at Idaho National Laboratory [12-017]. The writers thank Jeffrey M. Lacy of Idaho National Laboratory for stimulating and thoughtful discussion and feedback regarding this study. NR 27 TC 0 Z9 0 U1 1 U2 4 PU AMER SOC TESTING MATERIALS PI W CONSHOHOCKEN PA 100 BARR HARBOR DR, W CONSHOHOCKEN, PA 19428-2959 USA SN 0090-3973 EI 1945-7553 J9 J TEST EVAL JI J. Test. Eval. PD MAY PY 2014 VL 42 IS 3 BP 740 EP 748 DI 10.1520/JTE20130092 PG 9 WC Materials Science, Characterization & Testing SC Materials Science GA AU5JU UT WOS:000345643800020 ER PT J AU Afrin, S Kumar, V Bharathan, D Glatzmaier, GC Ma, ZW AF Afrin, Samia Kumar, Vinod Bharathan, Desikan Glatzmaier, Greg C. Ma, Zhiwen TI Computational Analysis of a Pipe Flow Distributor for a Thermocline Based Thermal Energy Storage System SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article AB The overall efficiency of a concentrating solar power (CSP) plant depends on the effectiveness of thermal energy storage (TES) system (Kearney and Herrmann, 2002, "Assessment of a Molten Salt Heat Transfer Fluid," ASME). A single tank TES system consists of a thermocline region which produces the temperature gradient between hot and cold storage fluid by density difference (Energy Efficiency and Renewable Energy, http://www.eere.energy.gov/basics/renewable_energy/thermal_storage.html). Preservation of this thermocline region in the tank during charging and discharging cycles depends on the uniformity of the velocity profile at any horizontal plane. Our objective is to maximize the uniformity of the velocity distribution using a pipe-network distributor by varying the number of holes, distance between the holes, position of the holes and number of distributor pipes. For simplicity, we consider that the diameter of the inlet, main pipe, the distributor pipes and the height and the width of the tank are constant. We use Hitec(R) molten salt as the storage medium and the commercial software Gambit 2.4.6 and Fluent 6.3 for the computational analysis. We analyze the standard deviation in the velocity field and compare the deviations at different positions of the tank height for different configurations. Since the distance of the holes from the inlet and their respective arrangements affects the flow distribution throughout the tank; we investigate the impacts of rearranging the holes position on flow distribution. Impact of the number of holes and distributor pipes are also analyzed. We analyze our findings to determine a configuration for the best case scenario. C1 [Afrin, Samia; Kumar, Vinod; Bharathan, Desikan] Univ Texas El Paso, Dept Mech Engn, El Paso, TX 79968 USA. [Glatzmaier, Greg C.; Ma, Zhiwen] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Afrin, S (reprint author), Univ Texas El Paso, Dept Mech Engn, El Paso, TX 79968 USA. EM safrin@miners.utep.edu; vkumar@utep.edu; desikan.bharathan@nrel.gov; greg.glatzmair@nrel.gov; zhiwen.ma@nrel.com NR 16 TC 0 Z9 0 U1 1 U2 7 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0199-6231 EI 1528-8986 J9 J SOL ENERG-T ASME JI J. Sol. Energy Eng. Trans.-ASME PD MAY PY 2014 VL 136 IS 2 AR 021010 DI 10.1115/1.4024927 PG 6 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA AS8SM UT WOS:000344518400010 ER PT J AU Shabgard, H Faghri, A Bergman, TL Andraka, CE AF Shabgard, Hamidreza Faghri, Amir Bergman, Theodore L. Andraka, Charles E. TI Numerical Simulation of Heat Pipe-Assisted Latent Heat Thermal Energy Storage Unit for Dish-Stirling Systems SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article DE dish-Stirling systems; latent heat thermal energy storage; heat pipe ID PHASE-CHANGE MATERIAL; NATURAL-CONVECTION; ENHANCEMENT AB A two-dimensional numerical model is developed to simulate the transient response of a heat pipe-assisted latent heat thermal energy storage (LHTES) unit integrated with dish-Stirling solar power generation systems. The unit consists of a container which houses a phase change material (PCM) and two sets of interlaced input and output heat pipes (HPs) embedded in the PCM. The LHTES unit is exposed to time-varying concentrated solar irradiance. A three-stage operating scenario is investigated that includes: (i) charging only, (ii) simultaneous charging and discharging, and (iii) discharging only. In general, it was found that the PCM damps the temporal variations of the input solar irradiance, and provides relatively smooth thermal power to the engine over a time period that can extend to after-sunset hours. Heat pipe spacing was identified as a key parameter to control the dynamic response of the unit. The system with the greatest (smallest) heat pipe spacing was found to have the greatest (smallest) temperature drops across the LHTES, as well as the maximum (minimum) amount of PCM melting and solidification. Exergy analyses were also performed, and it was found that the exergy efficiencies of all the systems considered were greater than 97%, with the maximum exergy efficiency associated with the system having the minimum heat pipe spacing. C1 [Shabgard, Hamidreza; Faghri, Amir] Univ Connecticut, Dept Mech Engn, Storrs, CT 06269 USA. [Bergman, Theodore L.] Univ Kansas, Dept Mech Engn, Lawrence, KS 66045 USA. [Andraka, Charles E.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Faghri, A (reprint author), Univ Connecticut, Dept Mech Engn, AB Bronwell Bldg Room 123, Storrs, CT 06269 USA. EM h.shabgard@engr.uconn.edu; faghri@engr.uconn.edu; tlbergman@ku.edu; ceandra@sandia.gov NR 33 TC 10 Z9 10 U1 3 U2 22 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0199-6231 EI 1528-8986 J9 J SOL ENERG-T ASME JI J. Sol. Energy Eng. Trans.-ASME PD MAY PY 2014 VL 136 IS 2 AR 021025 DI 10.1115/1.4025973 PG 12 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA AS8SM UT WOS:000344518400025 ER PT J AU Logan, J Kim, SW Pareto, D Telang, F Wang, GJ Fowler, JS Biegon, A AF Logan, Jean Kim, Sung Won Pareto, Deborah Telang, Frank Wang, Gene-Jack Fowler, Joanna S. Biegon, Anat TI Kinetic Analysis of [C-11]Vorozole Binding in the Human Brain with Positron Emission Tomography SO MOLECULAR IMAGING LA English DT Article ID MONOAMINE-OXIDASE-A; IN-VIVO; AROMATASE INHIBITOR; PET; BOLUS; CYTOCHROME-P450; INFUSION; SMOKING; POTENT; RAT AB Using positron emission tomography, we investigated the kinetics of [C-11]vorozole ([C-11]VOR), a radiotracer for the enzyme aromatase that catalyzes the last step in estrogen biosynthesis. Six subjects were scanned under baseline conditions followed by retest 2 weeks later. The retest was followed by a blocking study with 2.5 mg of the aromatase inhibitor letrozole. The binding potential (BPNDA) was estimated from a Lassen plot using the total tissue distribution volume (V-T) for baseline and blocked. BPNDA for the thalamus was found to be 15 times higher than that for the cerebellum. From the letrozole studies, we found that [C-11]VOR exhibits a slow binding compartment (small k(4)) that has a nonspecific and a blockable component. Because of the sensitivity of V-T to variations in k(4), a common value was used for the four highest binding regions. We also considered the tissue uptake to plasma ratio for 60 to 90 minutes as an outcome measure. Using the ratio method, the difference between the highest and lowest was 2.4 compared to 3.5 for the V-T. The ratio method underestimates the high regions but is less variable and may be more suitable for patient studies. Because of its kinetics and distribution, this tracer is not a candidate for a bolus infusion or reference tissue methods. C1 [Logan, Jean] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. NIAAA, Bethesda, MD USA. Hosp Valle De Hebron, Magnet Resonance Unit, Barcelona, Spain. CIBER BBN, Zaragoza, Spain. Mt Sinai Sch Med, Dept Psychiat, New York, NY USA. SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. SUNY Stony Brook, Sch Med, Dept Neurol, Stony Brook, NY 11794 USA. RP Logan, J (reprint author), Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. EM jean.logan@nyumc.org FU [1R21EB012707] FX Financial disclosure of authors: This study was supported by grant 1R21EB012707 (Anat Biegon PI). NR 41 TC 0 Z9 0 U1 1 U2 2 PU B C DECKER INC PI HAMILTON PA 69 JOHN STREET SOUTH, STE 310, HAMILTON, ONTARIO L8N 2B9, CANADA SN 1535-3508 EI 1536-0121 J9 MOL IMAGING JI Mol. Imaging PD MAY PY 2014 VL 13 IS 3 DI 10.2310/7290.2014.00004 PG 12 WC Biochemical Research Methods; Radiology, Nuclear Medicine & Medical Imaging SC Biochemistry & Molecular Biology; Radiology, Nuclear Medicine & Medical Imaging GA AS4AF UT WOS:000344215300003 ER PT J AU Pryor, JM Walker, WC AF Pryor, Jeff M. Walker, William C. TI PCMT Error Pressure Change Measurement Leak Testing Errors SO MATERIALS EVALUATION LA English DT Article C1 [Pryor, Jeff M.; Walker, William C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Pryor, JM (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM pryorjm@ornl.gov; walkerwc@ornl.gov NR 2 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC NONDESTRUCTIVE TEST PI COLUMBUS PA 1711 ARLINGATE LANE PO BOX 28518, COLUMBUS, OH 43228-0518 USA SN 0025-5327 J9 MATER EVAL JI Mater. Eval. PD MAY PY 2014 VL 72 IS 5 BP 544 EP 553 PG 10 WC Materials Science, Characterization & Testing SC Materials Science GA AR1HD UT WOS:000343335400001 ER PT J AU Pokharel, M Zhao, HZ Modic, KA Ren, ZF Opeil, C AF Pokharel, Mani Zhao, Huaizhou Modic, Kimberly A. Ren, Zhifeng Opeil, Cyril TI Magnetic Properties of Hot-Pressed FeSb2 SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article DE Hall effect; hysterisis; iron doantimonide; magnetization AB We report on the magnetic properties of a hot-pressed FeSb2 sample. We find a significant increase in the magnetic susceptibility in our sample when compared with the values previously reported for the polycrystalline sample. The pronounced Curie tail at low temperature corresponds to 0.2% of Fe2+ impurities per mole. In the intrinsic conductivity region, the susceptibility due to free carriers shows thermally activated behavior and is consistent with the data reported for single crystal FeSb2. Based on our data and analysis, while the enhanced magnetic susceptibility in our sample comes mainly from a small amount of unreacted Fe, the contribution from the enhanced carrier density due to lattice and strain defects arising from the ball milling process is also significant. Existence of an unreacted Fe phase is evidenced by small coercivity values of similar to 100 Oe observed at 50 and 300 K. C1 [Pokharel, Mani; Opeil, Cyril] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Zhao, Huaizhou; Ren, Zhifeng] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Zhao, Huaizhou; Ren, Zhifeng] Univ Houston, TcSUH, Houston, TX 77204 USA. [Modic, Kimberly A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Pokharel, M (reprint author), Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. EM pokharem@bc.edu FU Department of Defense, U.S. Air Force Office of Scientific Research MURI Program [FA9550-10-1-0533] FX This work was supported by the Department of Defense, U.S. Air Force Office of Scientific Research MURI Program under Contract FA9550-10-1-0533. C. Opeil would like to thank J. C. Lashley for technical assistance and T. Hoeler for a careful review of the manuscript. NR 15 TC 1 Z9 1 U1 5 U2 17 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD MAY PY 2014 VL 50 IS 5 AR 2400304 DI 10.1109/TMAG.2013.2292607 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA AQ7XL UT WOS:000343033500003 ER PT J AU Ho, CK AF Ho, Clifford K. TI Computational fluid dynamics for concentrating solar power systems SO WILEY INTERDISCIPLINARY REVIEWS-ENERGY AND ENVIRONMENT LA English DT Article ID THERMAL-ENERGY STORAGE; WIND LOADS; PHOTOVOLTAIC TRACKERS; HELIOSTAT; FLOW; SIMULATION; RECEIVER; MODEL; CFD AB Computational fluid dynamics (CFD) can be used to better understand complex processes and to improve designs and system performance in concentrating solar power (CSP) applications. Applications presented in this paper include CFD simulations for collectors, thermal receivers, and thermal storage technologies. CFD simulations of wind flow around collectors such as parabolic troughs and heliostats have been used to determine wind loads, which impact the design and requirements of the support structure. Simulations of the heat transfer and heat loss in solar thermal receivers have been performed to identify designs that optimize thermal efficiency, and to better understand radiative, convective, and conductive heat losses. CFD models have also been developed to understand processes in thermal storage systems, including mixing in thermoclines, heat transfer in solid media, and melting and solidification processes in phase-change materials. Researchers have generally concluded that CFD modeling is a useful and cost-effective tool to understand processes and improve designs for CSP systems. (C) 2013 John Wiley & Sons, Ltd. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ho, CK (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM ckho@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 52 TC 0 Z9 0 U1 4 U2 19 PU WILEY PERIODICALS, INC PI SAN FRANCISCO PA ONE MONTGOMERY ST, SUITE 1200, SAN FRANCISCO, CA 94104 USA SN 2041-8396 EI 2041-840X J9 WIRES ENERGY ENVIRON JI Wiley Interdiscip. Rev. Energy Environ. PD MAY-JUN PY 2014 VL 3 IS 3 BP 290 EP 300 DI 10.1002/wene.90 PG 11 WC Energy & Fuels SC Energy & Fuels GA AQ9WO UT WOS:000343208900004 ER PT J AU Arnold, R Augier, C Barabash, AS Basharina-Freshville, A Blondel, S Blot, S Bongrand, M Brudanin, V Busto, J Caffrey, AJ Cermak, P Cerna, C Chapon, A Chauveau, E Dragounova, L Duchesneau, D Durand, D Egorov, V Eurin, G Evans, JJ Flack, R Garrido, X Gomez, H Guillon, B Guzowski, P Hodak, R Hubert, P Hugon, C Hulka, J Jullian, S Klimenko, A Kochetov, O Konovalov, SI Kovalenko, V Lalanne, D Lang, K Lemiere, Y Liptak, Z Loaiza, P Lutter, G Mamedov, F Marquet, C Mauger, F Morgan, B Mott, J Nemchenok, I Nomachi, M Nova, F Nowacki, F Ohsumi, H Pahlka, RB Perrot, F Piquemal, F Povinec, P Ramachers, YA Remoto, A Reyss, JL Richards, B Riddle, CL Rukhadze, E Rukhadze, N Saakyan, R Sarazin, X Shitov, Y Simard, L Simkovic, F Smetana, A Smolek, K Smolnikov, A Soldner-Rembold, S Soule, B Stekl, I Suhonen, J Sutton, CS Szklarz, G Thomas, J Timkin, V Torre, S Tretyak, VI Tretyak, VI Umatov, V Vilela, C Vorobel, V Warot, G Waters, D Zukauskas, A AF Arnold, R. Augier, C. Barabash, A. S. Basharina-Freshville, A. Blondel, S. Blot, S. Bongrand, M. Brudanin, V. Busto, J. Caffrey, A. J. Cermak, P. Cerna, C. Chapon, A. Chauveau, E. Dragounova, L. Duchesneau, D. Durand, D. Egorov, V. Eurin, G. Evans, J. J. Flack, R. Garrido, X. Gomez, H. Guillon, B. Guzowski, P. Hodak, R. Hubert, P. Hugon, C. Hulka, J. Jullian, S. Klimenko, A. Kochetov, O. Konovalov, S. I. Kovalenko, V. Lalanne, D. Lang, K. Lemiere, Y. Liptak, Z. Loaiza, P. Lutter, G. Mamedov, F. Marquet, C. Mauger, F. Morgan, B. Mott, J. Nemchenok, I. Nomachi, M. Nova, F. Nowacki, F. Ohsumi, H. Pahlka, R. B. Perrot, F. Piquemal, F. Povinec, P. Ramachers, Y. A. Remoto, A. Reyss, J. L. Richards, B. Riddle, C. L. Rukhadze, E. Rukhadze, N. Saakyan, R. Sarazin, X. Shitov, Yu. Simard, L. Simkovic, F. Smetana, A. Smolek, K. Smolnikov, A. Soeldner-Rembold, S. Soule, B. Stekl, I. Suhonen, J. Sutton, C. S. Szklarz, G. Thomas, J. Timkin, V. Torre, S. Tretyak, V. I. Tretyak, Vl. I. Umatov, V. Vilela, C. Vorobel, V. Warot, G. Waters, D. Zukauskas, A. CA NEMO-3 Collaboration TI Investigation of double beta decay of Mo-100 to excited states of Ru-100 SO NUCLEAR PHYSICS A LA English DT Article DE Double beta decay; Mo-100; Excited states ID SOLAR-NEUTRINO OBSERVATIONS; FINAL-STATES; STATISTICS; OSCILLATION; VIOLATION; PHYSICS; GALLEX; MASS AB Double beta decay of Mo-100 to the excited states of daughter nuclei has been studied using a 600 cm(3) low-background HPGe detector and an external source consisting of 2588 g of 97.5% enriched metallic (100)mo, which was formerly inside the NEMO-3 detector and used for the NEMO-3 measurements of Mo-100. The half-life for the two-neutrino double beta decay of Mo-100 to the excited 0(1)(+) state in Ru-100 is measured to be T-1/2 = [7.5 +/- 0.6(stat) +/- 0.6(syst)] . 10(20) yr. For other (0 nu + 2 nu) transitions to the 2(1)(+), 2(2)(+), 0(2)(+), 2(3)(+) and 0(3)(+) levels in Ru-100, limits are obtained at the level of similar to(0.25-1.1) . 10(22) yr. (C) 2014 Elsevier B.V. All rights reserved. C1 [Arnold, R.; Nowacki, F.] UPL, IPHC, CNRS, IN2P3, F-67037 Strasbourg, France. [Augier, C.; Blondel, S.; Bongrand, M.; Eurin, G.; Garrido, X.; Gomez, H.; Jullian, S.; Lalanne, D.; Sarazin, X.; Simard, L.; Szklarz, G.] Univ Paris 11, LAL, CNRS, IN2P3, F-91405 Orsay, France. [Barabash, A. S.; Konovalov, S. I.; Umatov, V.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Basharina-Freshville, A.; Eurin, G.; Flack, R.; Mott, J.; Richards, B.; Saakyan, R.; Thomas, J.; Torre, S.; Vilela, C.; Waters, D.] UCL, London WC1E 6BT, England. [Blot, S.; Chauveau, E.; Evans, J. J.; Guzowski, P.; Soeldner-Rembold, S.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Brudanin, V.; Egorov, V.; Klimenko, A.; Kochetov, O.; Kovalenko, V.; Nemchenok, I.; Rukhadze, N.; Shitov, Yu.; Smolnikov, A.; Timkin, V.; Tretyak, V. I.] Joint Inst Nucl Res, Dubna 141980, Russia. [Busto, J.] Univ Marseille, CPPM, CNRS, IN2P3, F-13288 Marseille, France. [Caffrey, A. J.; Riddle, C. L.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Cermak, P.; Hodak, R.; Mamedov, F.; Rukhadze, E.; Smetana, A.; Smolek, K.; Stekl, I.] Czech Tech Univ, IEAP, CZ-12800 Prague, Czech Republic. [Cerna, C.; Hubert, P.; Hugon, C.; Lutter, G.; Marquet, C.; Perrot, F.; Soule, B.] Univ Bordeaux, CENBG, CNRS, IN2P3, F-33175 Gradignan, France. [Chapon, A.; Durand, D.; Guillon, B.; Lemiere, Y.; Mauger, F.] Univ Caen, CNRS, IN2P3, LPC Caen,ENSICAEN, F-14050 Caen, France. [Dragounova, L.; Hulka, J.] Natl Radiat Protect Inst, CZ-14000 Prague, Czech Republic. [Duchesneau, D.; Remoto, A.] Univ Savoie, LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. [Lang, K.; Liptak, Z.; Nova, F.; Pahlka, R. B.] Univ Texas Austin, Austin, TX 78712 USA. [Garrido, X.; Loaiza, P.; Piquemal, F.; Warot, G.] CNRS CEA, Lab Souterrain Modane, F-73500 Modane, France. [Morgan, B.; Ramachers, Y. A.] Univ Warwick, Coventry CV4 7AL, W Midlands, England. [Nomachi, M.] Osaka Univ, Osaka 5600043, Japan. [Ohsumi, H.] Saga Univ, Saga 8408502, Japan. [Povinec, P.; Simkovic, F.] Comenius Univ, FMFI, SK-84248 Bratislava, Slovakia. [Reyss, J. L.] CNRS, LSCE, F-91190 Gif Sur Yvette, France. [Shitov, Yu.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Simard, L.] Inst Univ France, F-75005 Paris, France. [Suhonen, J.] Univ Jyvaskyla, FIN-40351 Jyvaskyla, Finland. [Sutton, C. S.] MHC, S Hadley, MA 01075 USA. [Tretyak, Vl. I.] Ukrainian Acad Sci, Inst Nucl Res, UA-252028 Kiev, Ukraine. [Vorobel, V.; Zukauskas, A.] Charles Univ Prague, Fac Math & Phys, CZ-12116 Prague, Czech Republic. RP Barabash, AS (reprint author), Inst Theoret & Expt Phys, Moscow 117218, Russia. RI Nemchenok, Igor/F-9715-2014; Evans, Justin/P-4981-2014; Hodak, Rastislav/O-4243-2016; Barabash, Alexander/S-8851-2016; OI Evans, Justin/0000-0003-4697-3337; Hodak, Rastislav/0000-0001-7640-5643; Tretyak, Vladimir/0000-0002-2369-0679; Povinec, Pavel/0000-0003-0275-794X; Remoto, Alberto/0000-0001-9413-0356; Torre, Stefano/0000-0002-7565-0118 FU RFBR [12-02-12112, 13-02-93107]; MEYS, Czech Republic [LG11030, LM2011027] FX The authors would like to thank the Modane Underground Laboratory staff for their technical assistance in running the experiment. Portions of this work were supported by grants from RFBR (Nos. 12-02-12112 and 13-02-93107) and by grants LG11030 and LM2011027 (MEYS, Czech Republic). NR 75 TC 9 Z9 9 U1 2 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9474 EI 1873-1554 J9 NUCL PHYS A JI Nucl. Phys. A PD MAY PY 2014 VL 925 BP 25 EP 36 DI 10.1016/j.nuclphysa.2014.01.008 PG 12 WC Physics, Nuclear SC Physics GA AO4XV UT WOS:000341345600003 ER PT J AU Thomas, T Regis, JM Jolie, J Heinze, S Albers, M Bernards, C Fransen, C Radeck, D AF Thomas, T. Regis, J. -M. Jolie, J. Heinze, S. Albers, M. Bernards, C. Fransen, C. Radeck, D. TI Bose-Fermi symmetry in the odd-even gold isotopes SO NUCLEAR PHYSICS A LA English DT Article DE NUCLEAR REACTIONS Pt-196(p, 2n); E=14 MeV; Measured E gamma, I gamma, gamma gamma-coin; gamma(theta) using HORUS spectrometer Au-195 deduced levels; J, pi, branching and mixing ratios; B(E2). Comparison with IBFM calculations ID NUCLEAR-DATA SHEETS; DYNAMICAL SUPERSYMMETRY; ATOMIC-NUCLEI; MODEL; AU-197; HG-195M; STATES; DECAY; COEXISTENCE; REGION AB In this work the results of an in-beam experiment on Au-195 are presented, yielding new spins, multipole mixing ratios, and new low-lying states essential for the understanding of this nucleus. The positive-parity states from this work together with compiled data from the available literature for Au185-199 are compared to Interacting Boson Fermion Model calculations employing the Spin(6) Bose Fermi symmetry. The evolution of the parameters for the tau splitting and the J splitting reveals a smooth behavior. Thereby, a common description based on the Bose Fermi symmetry is found for Au189-199. Furthermore, the calculated E2 transition strengths are compared to experimental values with fixed effective boson and fermion charges for all odd even gold isotopes, emphasizing that the Spin(6) Bose-Fermi symmetry is valid for the gold isotopes. (C) 2014 Elsevier B.V. All rights reserved. C1 [Thomas, T.; Regis, J. -M.; Jolie, J.; Heinze, S.; Albers, M.; Bernards, C.; Fransen, C.; Radeck, D.] Univ Cologne, Inst Nucl Phys, D-50937 Cologne, Germany. [Albers, M.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Bernards, C.] Yale Univ, WNSL, New Haven, CT 06520 USA. RP Thomas, T (reprint author), Univ Cologne, Inst Nucl Phys, Zulpicher Str 77, D-50937 Cologne, Germany. RI Bernards, Christian/C-4879-2013 OI Bernards, Christian/0000-0001-5346-1415 FU DFG [JO391/2-1, JO391/3-2] FX We thank our coworkers and the Tandem accelerator staff at the IKP Koln for their help during the experiment. We thank R.V. Jobs for fruitful discussions concerning this work. Part of this work was supported by DFG under grant JO391/2-1 and JO391/3-2. NR 49 TC 0 Z9 0 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9474 EI 1873-1554 J9 NUCL PHYS A JI Nucl. Phys. A PD MAY PY 2014 VL 925 BP 96 EP 111 DI 10.1016/j.nuclphysa.2014.02.002 PG 16 WC Physics, Nuclear SC Physics GA AO4XV UT WOS:000341345600006 ER PT J AU Grygoryev, D Dan, C Gauny, S Eckelmann, B Ohlrich, AP Connolly, M Lasarev, M Grossi, G Kronenberg, A Turker, MS AF Grygoryev, Dmytro Dan, Cristian Gauny, Stacey Eckelmann, Bradley Ohlrich, Anna P. Connolly, Marissa Lasarev, Michael Grossi, Gianfranco Kronenberg, Amy Turker, Mitchell S. TI Autosomal Mutants of Proton-Exposed Kidney Cells Display Frequent Loss of Heterozygosity on Nonselected Chromosomes SO RADIATION RESEARCH LA English DT Article ID INDUCED GENOMIC INSTABILITY; IONIZING-RADIATION; IN-VIVO; SOLID TISSUES; MITOTIC RECOMBINATION; OXIDATIVE STRESS; MAMMALIAN-CELLS; ALPHA-PARTICLES; DEFICIENT MICE; BONE-MARROW AB High-energy protons found in the space environment can induce mutations and cancer, which are inextricably linked. We hypothesized that some mutants isolated from proton-exposed kidneys arose through a genome-wide incident that causes loss of heterozygosity (LOH)-generating mutations on multiple chromosomes (termed here genomic LOH). To test this hypothesis, we examined 11 pairs of nonselected chromosomes for LOH events in mutant cells isolated from the kidneys of mice exposed to 4 or 5 Gy of 1 GeV protons. The mutant kidney cells were selected for loss of expression of the chromosome 8-encoded Aprt gene. Genomic LOH events were also assessed in Aprt mutants isolated from isogenic cultured kidney epithelial cells exposed to 5 Gy of protons in vitro. Control groups were spontaneous Aprt mutants and clones isolated without selection from the proton-exposed kidneys or cultures. The in vivo results showed significant increases in genomic LOH events in the Aprt mutants from proton-exposed kidneys when compared with spontaneous Aprt mutants and when compared with nonmutant (i.e., nonselected) clones from the proton-exposed kidneys. A bias for LOH events affecting chromosome 14 was observed in the proton-induced Aprt mutants, though LOH for this chromosome did not confer increased radiation resistance. Genomic LOH events were observed in Aprt mutants isolated from proton-exposed cultured kidney cells; however the incidence was fivefold lower than in Aprt mutants isolated from exposed intact kidneys, suggesting a more permissive environment in the intact organ and/or the evolution of kidney clones prior to their isolation from the tissue. We conclude that proton exposure creates a subset of viable cells with LOH events on multiple chromosomes, that these cells form and persist in vivo, and that they can be isolated from an intact tissue by selection for a mutation on a single chromosome. (C) 2014 by Radiation Research Society C1 [Grygoryev, Dmytro; Dan, Cristian; Eckelmann, Bradley; Ohlrich, Anna P.; Connolly, Marissa; Lasarev, Michael; Turker, Mitchell S.] Oregon Hlth & Sci Univ, Ctr Res Occupat & Environm Toxicol, Portland, OR 97239 USA. [Gauny, Stacey; Kronenberg, Amy] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Grossi, Gianfranco] Univ Naples Federico II, Dept Phys, I-80126 Naples, Italy. [Grossi, Gianfranco] Univ Naples Federico II, Ctr Radioprotect & Hlth Phys, I-80126 Naples, Italy. [Turker, Mitchell S.] Oregon Hlth & Sci Univ, Dept Mol & Med Genet, Portland, OR 97239 USA. RP Kronenberg, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,Bldg 977, Berkeley, CA 94720 USA. EM a_kronenberg@lbl.gov; turkerm@ohsu.edu OI Lasarev, Michael R/0000-0002-1896-2705 FU NASA [NNJ07HC721, NNJ12HB88I, NNX10AC12G]; INFN (Italy); CROET FX The authors thank Adam Rusek, Peter Guida, Paul Wilson, Mary Ann Petry and their colleagues for help provided for the experiments at Brookhaven National Laboratory. This work was supported by NASA grants NNJ07HC721, NNJ12HB88I and NNX10AC12G, the INFN (Italy) and CROET summer fellowships to Marissa Connolly and Bradley Eckelmann. NR 68 TC 1 Z9 1 U1 1 U2 3 PU RADIATION RESEARCH SOC PI LAWRENCE PA 810 E TENTH STREET, LAWRENCE, KS 66044 USA SN 0033-7587 EI 1938-5404 J9 RADIAT RES JI Radiat. Res. PD MAY PY 2014 VL 181 IS 5 BP 452 EP 463 DI 10.1667/RR13654.1 PG 12 WC Biology; Biophysics; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Biophysics; Radiology, Nuclear Medicine & Medical Imaging GA AO4KZ UT WOS:000341308100002 PM 24758577 ER PT J AU Mishra, U Riley, WJ AF Mishra, Umakant Riley, William J. TI Active-Layer Thickness across Alaska: Comparing Observation-Based Estimates with CMIP5 Earth System Model Predictions SO SOIL SCIENCE SOCIETY OF AMERICA JOURNAL LA English DT Article ID LAND-SURFACE SCHEME; CLIMATE-CHANGE; PERMAFROST CARBON; NORTHERN ALASKA; CYCLE; THAW; GCM; VULNERABILITY; SENSITIVITY; SIMULATION AB Predicted active-layer (AL) thicknesses of permafrost-affected soils influence earth system model predictions of C-climate feedbacks; yet, only a few observation-based studies have estimated AL thicknesses across large regions and at the spatial scale at which they vary. We used spatially referenced soil profile description data (n = 153) and environmental variables (topography, climate, and land cover) in a geographically weighted regression approach to predict the spatial variability of AL thickness across Alaska at a 60-m spatial resolution. The predicted AL thickness across Alaska ranged from 0.14 to 0.93 m, with a spatial average of 0.46 m and a coefficient of variation of 30%. The average prediction error and ratio of performance to deviation were 0.11 m and 1.8, respectively. Our study showed mean annual surface air temperature, land cover type, and slope gradient were primary controllers of AL thickness spatial variability. We compared our estimates with Coupled Model Intercomparison Project Phase 5 (CMIP5) earth system model predictions; those predictions showed large interquartile ranges in predicted AL thicknesses (0.35-4.4 m) indicating substantial overestimate of current AL thickness in Alaska, which might result in higher positive permafrost C feedback under future warming scenarios. The CMIP5 predictions of AL thicknesses spatial heterogeneity were unrealistic when compared with observations, and prediction errors were several times larger in comparison to errors from our observation-based approach. The coefficient of variability of AL thickness was substantially lower in CMIP5 predictions compared to our estimates when gridded at similar spatial resolutions. These results indicate the need for better process representations and representation of natural spatial heterogeneity due to local environment (topography, vegetation, and soil properties) in earth system models to generate a realistic variation of regional scale AL thickness, which could reduce the existing uncertainty in predicting permafrost C-climate feedbacks. C1 [Mishra, Umakant] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. [Riley, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Mishra, U (reprint author), Argonne Natl Lab, Div Environm Sci, 9700 S Cass Ave 240-6143, Argonne, IL 60439 USA. EM umishra@anl.gov RI Riley, William/D-3345-2015 OI Riley, William/0000-0002-4615-2304 FU Office of Science, Office of Biological and Environmental Research, U.S. Department of Energy under Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Office of Science, Office of Biological and Environmental Research, U.S. Department of Energy under Argonne National Laboratory [DE-AC02-06CH11357] FX This study was jointly supported by two grants from the Director, Office of Science, Office of Biological and Environmental Research, U.S. Department of Energy under Lawrence Berkeley National Laboratory contract no. DE-AC02-05CH11231 and under Argonne National Laboratory contract no. DE-AC02-06CH11357. We appreciate help from Charlie Koven who provided the calculation of active-layer thickness from the CMIP5 models across Alaska. NR 55 TC 6 Z9 6 U1 0 U2 24 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 0361-5995 EI 1435-0661 J9 SOIL SCI SOC AM J JI Soil Sci. Soc. Am. J. PD MAY-JUN PY 2014 VL 78 IS 3 BP 894 EP 902 DI 10.2136/sssaj2013.11.0484 PG 9 WC Soil Science SC Agriculture GA AO7WU UT WOS:000341564100022 ER PT J AU Perumalla, KS Park, AJ Tipparaju, V AF Perumalla, Kalyan S. Park, Alfred J. Tipparaju, Vinod TI Discrete Event Execution with One-Sided and Two-Sided GVT Algorithms on 216,000 Processor Cores SO ACM TRANSACTIONS ON MODELING AND COMPUTER SIMULATION LA English DT Article DE Parallel discrete event simulation; time warp; global virtual time; one-sided communication; asynchrony ID VIRTUAL TIME; SIMULATIONS AB Global Virtual Time (GVT) computation is a key determinant of the efficiency and runtime dynamics of Parallel Discrete Event Simulations (PDES), especially on large-scale parallel platforms. Here, three execution modes of a generalized GVT computation algorithm are studied on high-performance parallel computing systems: (1) a synchronous GVT algorithm that affords ease of implementation, (2) an asynchronous GVT algorithm that is more complex to implement but can relieve blocking latencies, and (3) a variant of the asynchronous GVT algorithm to exploit one-sided communication in extant supercomputing platforms. Performance results are presented of implementations of these algorithms on up to 216,000 cores of a Cray XT5 system, exercised on a range of parameters: optimistic and conservative synchronization, fine- to medium-grained event computation, synthetic and nonsynthetic applications, and different lookahead values. Detailed PDES-specific runtime metrics are presented to further the understanding of tightly coupled discrete event dynamics on massively parallel platforms. C1 [Perumalla, Kalyan S.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Park, Alfred J.] Microsoft Corp, Redmond, WA 98052 USA. [Tipparaju, Vinod] Adv Micro Devices Inc, Sunnyvale, CA 94088 USA. RP Perumalla, KS (reprint author), 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM perumallaks@ornl.gov; alfpark@outlook.com; tipparajuv@gmail.com OI Perumalla, Kalyan/0000-0002-7458-0832 FU U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; Early Career Research Program of the DOE Office of Science, Advanced Scientific Computing Research; DOE Office of Science FX This paper has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the U.S. Department of Energy (DOE). Accordingly, the United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. This research was supported by the Early Career Research Program of the DOE Office of Science, Advanced Scientific Computing Research. The research used resources of the National Center for Computational Sciences (NCCS) at Oak Ridge National Laboratory, which is supported by the DOE Office of Science. NR 42 TC 0 Z9 0 U1 0 U2 4 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 1049-3301 EI 1558-1195 J9 ACM T MODEL COMPUT S JI ACM Trans. Model. Comput. Simul. PD MAY PY 2014 VL 24 IS 3 AR 16 DI 10.1145/2611561 PG 25 WC Computer Science, Interdisciplinary Applications; Mathematics, Applied SC Computer Science; Mathematics GA AO1LM UT WOS:000341073600004 ER PT J AU Armengaud, E Avignone, FT Betz, M Brax, P Brun, P Cantatore, G Carmona, JM Carosi, GP Caspers, F Caspi, S Cetin, SA Chelouche, D Christensen, FE Dael, A Dafni, T Davenport, M Derbin, AV Desch, K Diago, A Dobrich, B Dratchnev, I Dudarev, A Eleftheriadis, C Fanourakis, G Ferrer-Ribas, E Galan, J Garcia, JA Garza, JG Geralis, T Gimeno, B Giomataris, I Gninenko, S Gomez, H Gonzalez-Diaz, D Guendelman, E Hailey, CJ Hiramatsu, T Hoffmann, DHH Horns, D Iguaz, FJ Irastorza, IG Isern, J Imai, K Jakobsen, AC Jaeckel, J Jakovcic, K Kaminski, J Kawasaki, M Karuza, M Krcmar, M Kousouris, K Krieger, C Lakic, B Limousin, O Lindner, A Liolios, A Luzon, G Matsuki, S Muratova, VN Nones, C Ortega, I Papaevangelou, T Pivovaroff, MJ Raffelt, G Redondo, J Ringwald, A Russenschuck, S Ruz, J Saikawa, K Savvidis, I Sekiguchi, T Semertzidis, YK Shilon, I Sikivie, P Silva, H ten Kate, H Tomas, A Troitsky, S Vafeiadis, T van Bibber, K Vedrine, P Villar, JA Vogel, JK Walckiers, L Weltman, A Wester, W Yildiz, SC Zioutas, K AF Armengaud, E. Avignone, F. T. Betz, M. Brax, P. Brun, P. Cantatore, G. Carmona, J. M. Carosi, G. P. Caspers, F. Caspi, S. Cetin, S. A. Chelouche, D. Christensen, F. E. Dael, A. Dafni, T. Davenport, M. Derbin, A. V. Desch, K. Diago, A. Doebrich, B. Dratchnev, I. Dudarev, A. Eleftheriadis, C. Fanourakis, G. Ferrer-Ribas, E. Galan, J. Garcia, J. A. Garza, J. G. Geralis, T. Gimeno, B. Giomataris, I. Gninenko, S. Gomez, H. Gonzalez-Diaz, D. Guendelman, E. Hailey, C. J. Hiramatsu, T. Hoffmann, D. H. H. Horns, D. Iguaz, F. J. Irastorza, I. G. Isern, J. Imai, K. Jakobsen, A. C. Jaeckel, J. Jakovcic, K. Kaminski, J. Kawasaki, M. Karuza, M. Krcmar, M. Kousouris, K. Krieger, C. Lakic, B. Limousin, O. Lindner, A. Liolios, A. Luzon, G. Matsuki, S. Muratova, V. N. Nones, C. Ortega, I. Papaevangelou, T. Pivovaroff, M. J. Raffelt, G. Redondo, J. Ringwald, A. Russenschuck, S. Ruz, J. Saikawa, K. Savvidis, I. Sekiguchi, T. Semertzidis, Y. K. Shilon, I. Sikivie, P. Silva, H. ten Kate, H. Tomas, A. Troitsky, S. Vafeiadis, T. van Bibber, K. Vedrine, P. Villar, J. A. Vogel, J. K. Walckiers, L. Weltman, A. Wester, W. Yildiz, S. C. Zioutas, K. TI Conceptual design of the International Axion Observatory (IAXO) SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Dark Matter detectors (WIMPs, axions, etc.); Large detector systems for particle and astroparticle physics; X-ray detectors; Micropattern gaseous detectors (MSGC, GEM, THGEM, RETHGEM, MHSP, MICROPIC, MICROMEGAS, In Grid; etc) ID X-RAY TELESCOPE; SOLAR AXIONS; COHERENT CONVERSION; CP CONSERVATION; MAGNETIC-FIELD; DIRECT SEARCH; MICROMEGAS; PARTICLES; DETECTOR; READOUT AB The International Axion Observatory (IAXO) will be a forth generation axion helioscope. As its primary physics goal, TAX will look for axions or axion-like particles (ALPs) originating in the Sun via the Primakoff conversion of the solar plasma photons. In terms of signalto-noise ratio, TAX will be about 4-5 orders of magnitude more sensitive than CAST, currently the most powerful axion helioscope, reaching sensitivity to axion-photon couplings down to a few x 10-12 GeV-1 and thus probing a large fraction of the currently unexplored axion and ALP parameter space. TAX will also be sensitive to solar axions produced by mechanisms mediated by the axion-electron coupling ga, with sensitivity for the first time to values of ga, not previously excluded by astrophysics. With several other possible physics cases, TAX has the potential to serve as a multi-purpose facility for generic axion and ALP research in the next decade. In this paper we present the conceptual design of IAXO, which follows the layout of an enhanced axion helioscope, based on a purpose-built 20 m-long 8-coils toroidal superconducting magnet. All the eight 60cm-diameter magnet bores are equipped with focusing x-ray optics, able to focus the signal photons into similar to 0.2 cm(2) spots that are imaged by ultra-low-background Micromegas x-ray detectors. The magnet is built into a structure with elevation and azimuth drives that will allow for solar tracking for similar to 12 h each day. C1 [Armengaud, E.; Brun, P.; Dael, A.; Ferrer-Ribas, E.; Galan, J.; Giomataris, I.; Limousin, O.; Nones, C.; Papaevangelou, T.; Vedrine, P.] CEA Irfu, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Avignone, F. T.] Univ S Carolina, Dept Phys, Columbia, SC 29208 USA. [Betz, M.; Caspers, F.; Davenport, M.; Dudarev, A.; Kousouris, K.; Russenschuck, S.; Shilon, I.; Silva, H.; ten Kate, H.; Vafeiadis, T.; Walckiers, L.] European Org Nucl Res CERN, Geneva, Switzerland. [Brax, P.] Ctr Etud Saclay CEA Saclay, IPHT, Gif Sur Yvette, France. [Cantatore, G.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Cantatore, G.] Univ Trieste, Trieste, Italy. [Carmona, J. M.; Dafni, T.; Diago, A.; Garcia, J. A.; Garza, J. G.; Gomez, H.; Gonzalez-Diaz, D.; Iguaz, F. J.; Irastorza, I. G.; Luzon, G.; Ortega, I.; Tomas, A.; Villar, J. A.] Univ Zaragoza, Lab Fis Nucl & Altas Energias, Zaragoza, Spain. [Carosi, G. P.; Pivovaroff, M. J.; Ruz, J.; Vogel, J. K.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Caspi, S.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Cetin, S. A.; Yildiz, S. C.] Dogus Univ, Istanbul, Turkey. [Chelouche, D.] Univ Haifa, Dept Phys, IL-31905 Haifa, Israel. [Christensen, F. E.; Jakobsen, A. C.] Tech Univ Denmark, DTU Space, Lyngby, Denmark. [Derbin, A. V.; Dratchnev, I.; Muratova, V. N.] St Petersburg Nucl Phys Inst, St Petersburg, Russia. [Desch, K.; Kaminski, J.; Krieger, C.] Univ Bonn, Inst Phys, Bonn, Germany. [Doebrich, B.; Lindner, A.; Ringwald, A.] Deutsch Elektronen Synchrotron DESY, Hamburg, Germany. [Eleftheriadis, C.; Liolios, A.; Savvidis, I.] Aristotle Univ Thessaloniki, GR-54006 Thessaloniki, Greece. [Fanourakis, G.; Geralis, T.] Demokritos Natl Ctr Sci Res, GR-15310 Athens, Greece. [Gimeno, B.] Univ Valencia, Inst Ciencias Mat, Valencia, Spain. [Gninenko, S.; Troitsky, S.] Russian Acad Sci, INR, Moscow, Russia. [Guendelman, E.] Ben Gurion Univ Negev, Dept Phys, IL-84105 Beer Sheva, Israel. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Hiramatsu, T.] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 606, Japan. [Hoffmann, D. H. H.] Tech Univ Darmstadt, IKP, Darmstadt, Germany. [Horns, D.] Univ Hamburg, Inst Expt Phys, D-22761 Hamburg, Germany. [Isern, J.] Inst Ciencies Espai CSIC IEEC, Fac Ciencies, Bellaterra, Spain. [Imai, K.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki, Japan. [Jaeckel, J.] Heidelberg Univ, Inst Theoret Phys, D-69120 Heidelberg, Germany. [Jakovcic, K.; Krcmar, M.; Lakic, B.] Rudjer Boskovic Inst, Zagreb, Croatia. [Kawasaki, M.; Sekiguchi, T.] Univ Tokyo, Inst Cosm Ray Res, Tokyo, Japan. [Karuza, M.] Univ Rijeka, Rijeka, Croatia. [Matsuki, S.] Kyoto Univ, Res Ctr Low Temp & Mat Sci, Kyoto 6068502, Japan. [Raffelt, G.; Redondo, J.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Saikawa, K.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Semertzidis, Y. K.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Sikivie, P.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [van Bibber, K.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Weltman, A.] Univ Cape Town, ZA-7700 Rondebosch, South Africa. [Wester, W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Zioutas, K.] Univ Patras, Dept Phys, GR-26110 Patras, Greece. RP Irastorza, IG (reprint author), Univ Zaragoza, Lab Fis Nucl & Altas Energias, Zaragoza, Spain. EM Igor.Irastorza@cern.ch RI Papaevangelou, Thomas/G-2482-2016; Iguaz Gutierrez, Francisco Jose/F-4117-2016; Troitsky, Sergey/C-1377-2014; Villar, Jose Angel/K-6630-2014; Gonzalez Diaz, Diego/K-7265-2014; Irastorza, Igor/B-2085-2012; Pivovaroff, Michael/M-7998-2014; Isern, Jordi/B-1844-2015; Carmona, Jose/H-3732-2015; Redondo, Javier/H-9362-2015; Gracia Garza, Javier/F-5713-2016; Dafni, Theopisti/J-9646-2012; OI Papaevangelou, Thomas/0000-0003-2829-9158; Iguaz Gutierrez, Francisco Jose/0000-0001-6327-9369; Troitsky, Sergey/0000-0001-6917-6600; Villar, Jose Angel/0000-0003-0228-7589; Gonzalez Diaz, Diego/0000-0002-6809-5996; Irastorza, Igor/0000-0003-1163-1687; Pivovaroff, Michael/0000-0001-6780-6816; Isern, Jordi/0000-0002-0819-9574; Carmona, Jose/0000-0003-2264-2306; Redondo, Javier/0000-0002-1044-8197; Gracia Garza, Javier/0000-0003-0800-1588; Drachnev, Ilia/0000-0002-4064-8093; Limousin, Olivier/0000-0002-8794-5853; Dafni, Theopisti/0000-0002-8921-910X; Karuza, Marin/0000-0002-2646-9427; Derbin, Alexander/0000-0002-4351-2255; Luzon Marco, Gloria/0000-0002-5352-1884 FU Spanish Ministry of Science and Innovation (MICINN) [FPA2008-03456, FPA2011-24058]; CPAN project from the Consolider-Ingenio program of the MICINN [CSD2007-00042]; European Regional Development Fund (ERDF/FEDER); European Commission under the European Research Council T-REX Starting Grant of the IDEAS program of the EU [ERC-2009-StG-240054]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LDRD program [10-SI-015]; CAST; CERN, Physics Department; ATLAS; Deutsche Forschungsgemeinschaft (Germany) [EXC-153]; MSES of Croatia; Russian Foundation for Basic Research (RFBR); Eurotalents program FX We acknowledge support from the Spanish Ministry of Science and Innovation (MICINN) under contract FPA2008-03456 and FPA2011-24058, as well as under the CPAN project CSD2007-00042 from the Consolider-Ingenio2010 program of the MICINN. Part of these grants are funded by the European Regional Development Fund (ERDF/FEDER). We also acknowledge support from the European Commission under the European Research Council T-REX Starting Grant ERC-2009-StG-240054 of the IDEAS program of the 7th EU Framework Program. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 with support from the LDRD program through grant 10-SI-015. We also acknowledge support from the CAST collaboration. The design work on the magnet system was supported by CERN, Physics Department as well as the ATLAS Collaboration. Partial support by the Deutsche Forschungsgemeinschaft (Germany) under grant EXC-153, by the MSES of Croatia and the Russian Foundation for Basic Research (RFBR) is also acknowledged. F. I. acknowledges the support from the Eurotalents program. NR 83 TC 34 Z9 34 U1 2 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAY PY 2014 VL 9 AR T05002 DI 10.1088/1748-0221/9/05/T05002 PG 46 WC Instruments & Instrumentation SC Instruments & Instrumentation GA AM7HJ UT WOS:000340036100077 ER PT J AU Baller, B Bromberg, C Buchanan, N Cavanna, F Chen, H Church, E Gehman, V Greenlee, H Guardincerri, E Jones, B Junk, T Katori, T Kirby, M Lang, K Loer, B Marchionni, A Maruyama, T Mauger, C Menegolli, A Montanari, D Mufson, S Norris, B Pordes, S Raaf, J Rebel, B Sanders, R Soderberga, M St John, J Strauss, T Szelc, A Tope, T Touramanis, C Thorn, C Urheim, J Van de Water, R Wang, H Yu, B Zuckerbrot, M AF Baller, B. Bromberg, C. Buchanan, N. Cavanna, F. Chen, H. Church, E. Gehman, V. Greenlee, H. Guardincerri, E. Jones, B. Junk, T. Katori, T. Kirby, M. Lang, K. Loer, B. Marchionni, A. Maruyama, T. Mauger, C. Menegolli, A. Montanari, D. Mufson, S. Norris, B. Pordes, S. Raaf, J. Rebel, B. Sanders, R. Soderberg, M. St John, J. Strauss, T. Szelc, A. Tope, T. Touramanis, C. Thorn, C. Urheim, J. Van de Water, R. Wang, H. Yu, B. Zuckerbrot, M. TI Liquid Argon Time Projection Chamber research and development in the United States SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Time projection Chambers (TPC); Noble liquid detectors (scintillation, ionization, double-phase); Neutrino detectors; Dark Matter detectors (WIMPs, axions, etc.) ID ELECTRONICS; DETECTOR; TPC AB A workshop was held at Fermilab on March 20-21, 2013 to discuss the development of liquid argon time projection chambers (LArTPCs) in the United States. The workshop was organized under the auspices of the Coordinating Panel for Advanced Detectors, a body that was initiated by the American Physical Society Division of Particles and Fields. All presentations at the workshop were made in seven topical plenary sessions: i) Argon Purity, ii) Cryogenics, iii) TPC and High Voltage, iv) Electronics, Data Acquisition and Triggering, v) Scintillation Light Detection, vi) Calibration and Test Beams, and vii) Software. This document summarizes the current efforts in each of these areas. It also highlights areas in LArTPC research and development that are common between neutrino experiments and dark matter experiments. C1 [Baller, B.; Greenlee, H.; Junk, T.; Kirby, M.; Loer, B.; Marchionni, A.; Montanari, D.; Norris, B.; Pordes, S.; Raaf, J.; Rebel, B.; Sanders, R.; Soderberg, M.; Tope, T.; Zuckerbrot, M.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Bromberg, C.] Michigan State Univ, E Lansing, MI 48824 USA. [Buchanan, N.] Colorado State Univ, Ft Collins, CO 80523 USA. [Cavanna, F.; Church, E.; Szelc, A.] Yale Univ, New Haven, CT 06520 USA. [Chen, H.; Thorn, C.; Yu, B.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Gehman, V.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Guardincerri, E.; Mauger, C.; Van de Water, R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Jones, B.; Katori, T.] MIT, Cambridge, MA 02139 USA. [Lang, K.] Univ Texas Austin, Austin, TX 78712 USA. [Maruyama, T.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 3050801, Japan. [Menegolli, A.] Ist Nazl Fis Nucl, I-27100 Pavia, Italy. [Mufson, S.; Urheim, J.] Indiana Univ, Bloomington, IN 47405 USA. [Soderberg, M.] Syracuse Univ, Syracuse, NY 13210 USA. [St John, J.] Univ Cincinnati, Cincinnati, OH 45220 USA. [Strauss, T.] Univ Bern, CH-3012 Bern, Switzerland. [Touramanis, C.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Wang, H.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. RP Baller, B (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. OI Raaf, Jennifer/0000-0002-4533-929X; Van de Water, Richard/0000-0002-1573-327X; Marchionni, Alberto/0000-0003-3039-9537; Katori, Teppei/0000-0002-9429-9482; Cavanna, Flavio/0000-0002-5586-9964 FU U.S. Department of Energy Office of Science [DE-FG02-91ER40661]; LBNE project from Brookhaven National Laboratory [BNL 240296]; U.S. Department of Energy Office of Science; National Science Foundation; LDRD program FX We thank the ICARUS collaboration for sharing their experiences and lessons learned in building and operating the first large LArTPC. The High Energy Astrophysics Group at Indiana University is supported by the U.S. Department of Energy Office of Science with grant DE-FG02-91ER40661 to Indiana University and LBNE project funding from Brookhaven National Laboratory with grant BNL 240296 to Indiana University. The LArIAT collaboration is supported by the U.S. Department of Energy Office of Science and the National Science Foundation. The CAPTAIN detector has been designed and is being built by the Physics and the Theory divisions of Los Alamos National Laboratory under the auspices of the LDRD program. T. Strauss spoke on behalf of the Albert Einstein Center. Laboratory of High Energy Physics of the University of Bern. The MicroBooNE and LBNE collaborations have participated in the development of cold electronics as supported by the U.S. Department of Energy Office of Science. NR 36 TC 5 Z9 5 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAY PY 2014 VL 9 AR T05005 DI 10.1088/1748-0221/9/05/T05005 PG 53 WC Instruments & Instrumentation SC Instruments & Instrumentation GA AM7HJ UT WOS:000340036100080 ER PT J AU Bergmann, B Nelson, RO O'Donnell, JM Pospisil, S Solc, J Takai, H Vykydal, Z AF Bergmann, B. Nelson, R. O. O'Donnell, J. M. Pospisil, S. Solc, J. Takai, H. Vykydal, Z. TI Time-of-flight measurement of fast neutrons with Timepix detectors SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Solid state detectors; Interaction of radiation with matter; Hybrid detectors; Neutron detectors (cold, thermal, fast neutrons) ID RADIATION AB Timepix pixel detectors have been used to study the response of silicon hybrid pixel detectors to fast neutrons from a pulsed neutron beam at WNR FP30R, a 14m long flight path, in the Los Alamos Neutron Science Center. Neutrons with kinetic energies up to 600 MeV were available. In order to enhance the conversion of neutrons to energetic charged particles, several converter foils and filters were attached to the 300 mu m thick silicon sensor, i.e. polyethylene, polyethylene with aluminum, (LiF)-Li-6, (LiF)-Li-6 with aluminum, aluminum. The Time-of-Arrival mode of the Timepix detectors has permitted the application of the Time-of-Flight (TOF) technique for the assignment of the detected interactions in the form of clusters (groups of adjacent pixels) in the pixel matrix, to the kinetic energies of the incident neutrons. It was found that, for lower neutron energies (similar to MeV range) the cluster rates below the polyethylene and the polyethylene and aluminum region, produced by recoil protons, are a good measure for the mean kinetic energies of neutrons. For energies above 50 MeV nuclear reactions in the silicon dominate the detector response. In this energy range the shape of the clusters indicates the neutron kinetic energy. C1 [Bergmann, B.; Pospisil, S.; Solc, J.; Vykydal, Z.] Czech Tech Univ, Inst Expt & Appl Phys, Prague 12800 2, Czech Republic. [Nelson, R. O.; O'Donnell, J. M.] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA. [Takai, H.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Bergmann, B (reprint author), Czech Tech Univ, Inst Expt & Appl Phys, Horska 3a-22, Prague 12800 2, Czech Republic. EM Benedikt.Bergmann@utef.cvut.cz RI Vykydal, Zdenek/H-6426-2016 OI Vykydal, Zdenek/0000-0003-2329-0672 FU Marie Curie Early Initial Training Network Fellowship of the European Community [PITN-GA-2011-289198-ARDENT]; Ministry of Education, Youth and Sports of the Czech Republic [LG13031, LG13009]; U.S. Department of Energy [DE-AC52-06NA25396] FX This research project has been supported by a Marie Curie Early Initial Training Network Fellowship of the European Community's Seventh Framework Programme under contract number (PITN-GA-2011-289198-ARDENT) and Ministry of Education, Youth and Sports of the Czech Republic under INGO II projects number LG13031 and LG13009. The work has been done in the frame of the Medipix collaboration. This work has benefited from the use of the Los Alamos Neutron Science Center at LANL. This facility is funded by the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 15 TC 3 Z9 3 U1 4 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAY PY 2014 VL 9 AR C05048 DI 10.1088/1748-0221/9/05/C05048 PG 10 WC Instruments & Instrumentation SC Instruments & Instrumentation GA AM7HJ UT WOS:000340036100048 ER PT J AU Miucci, A Gonella, L Hemperek, T Hugging, F Kruger, H Obermann, T Wermes, N Garcia-Sciveres, M Backhaus, M Capeans, M Feigl, S Nessi, M Pernegger, H Ristic, B Gonzalez-Sevilla, S Ferrere, D Iacobucci, G La Rosa, A Muenstermann, D George, M Grosse-Knetter, J Quadt, A Rieger, J Weingarten, J Bates, R Blue, A Buttar, C Hynds, D Kreidl, C Peric, I Breugnon, P Pangaud, P Godiot-Basolo, S Fougeron, D Bompard, F Clemens, JC Liu, J Barbero, M Rozanov, A AF Miucci, A. Gonella, L. Hemperek, T. Huegging, F. Krueger, H. Obermann, T. Wermes, N. Garcia-Sciveres, M. Backhaus, M. Capeans, M. Feigl, S. Nessi, M. Pernegger, H. Ristic, B. Gonzalez-Sevilla, S. Ferrere, D. Iacobucci, G. La Rosa, A. Muenstermann, D. George, M. Grosse-Knetter, J. Quadt, A. Rieger, J. Weingarten, J. Bates, R. Blue, A. Buttar, C. Hynds, D. Kreidl, C. Peric, I. Breugnon, P. Pangaud, P. Godiot-Basolo, S. Fougeron, D. Bompard, F. Clemens, J. C. Liu, J. Barbero, M. Rozanov, A. CA HV-CMOS Collaboration TI Radiation-hard Active Pixel Sensors for HL-LHC Detector Upgrades based on HV-CMOS Technology SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Particle tracking detectors; Particle tracking detectors (Solid-state detectors) AB Luminosity upgrades are discussed for the LHC (HL-LHC) which would make updates to the detectors necessary, requiring in particular new, even more radiation-hard and granular, sensors for the inner detector region. A proposal for the next generation of inner detectors is based on HV-CMOS: a new family of silicon sensors based on commercial high-voltage CMOS technology, which enables the fabrication of part of the pixel electronics inside the silicon substrate itself. The main advantages of this technology with respect to the standard silicon sensor technology are: low material budget, fast charge collection time, high radiation tolerance, low cost and operation at room temperature. A traditional readout chip is still needed to receive and organize the data from the active sensor and to handle high-level functionality such as trigger management. HV-CMOS has been designed to be compatible with both pixel and strip readout. In this paper an overview of HV2FEI4, a HV-CMOS prototype in 180 nm AMS technology, will be given. Preliminary results after neutron and X-ray irradiation are shown. C1 [Miucci, A.; Gonzalez-Sevilla, S.; Ferrere, D.; Iacobucci, G.; La Rosa, A.; Muenstermann, D.] Univ Geneva, Geneva, Switzerland. [Gonella, L.; Hemperek, T.; Huegging, F.; Krueger, H.; Obermann, T.; Wermes, N.] Univ Bonn, Inst Phys, Bonn, Germany. [Garcia-Sciveres, M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Backhaus, M.; Capeans, M.; Feigl, S.; Nessi, M.; Pernegger, H.; Ristic, B.] CERN, PH DT Dept, Geneva, Switzerland. [George, M.; Grosse-Knetter, J.; Quadt, A.; Rieger, J.; Weingarten, J.] Univ Gottingen, Inst Phys, D-37073 Gottingen, Germany. [Bates, R.; Blue, A.; Buttar, C.; Hynds, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Kreidl, C.; Peric, I.] Heidelberg Univ, Inst Comp Sci, D-68131 Mannheim, Germany. [Breugnon, P.; Pangaud, P.; Godiot-Basolo, S.; Fougeron, D.; Bompard, F.; Clemens, J. C.; Liu, J.; Barbero, M.; Rozanov, A.] Ctr Phys Particules Marseille, Marseille, France. RP Miucci, A (reprint author), Univ Geneva, Quai Ernest Anserment 24, Geneva, Switzerland. EM antonio.miucci@cern.com RI Buttar, Craig/D-3706-2011; Blue, Andrew/C-9882-2016 OI Blue, Andrew/0000-0002-7716-5626 NR 6 TC 1 Z9 1 U1 2 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAY PY 2014 VL 9 AR C05064 DI 10.1088/1748-0221/9/05/C05064 PG 8 WC Instruments & Instrumentation SC Instruments & Instrumentation GA AM7HJ UT WOS:000340036100064 ER PT J AU Twining, BS Nodder, SD King, AL Hutchins, DA LeCleir, GR DeBruyn, JM Maas, EW Vogt, S Wilhelm, SW Boyd, PW AF Twining, Benjamin S. Nodder, Scott D. King, Andrew L. Hutchins, David A. LeCleir, Gary R. DeBruyn, Jennifer M. Maas, Elizabeth W. Vogt, Stefan Wilhelm, Steven W. Boyd, Philip W. TI Differential remineralization of major and trace elements in sinking diatoms SO LIMNOLOGY AND OCEANOGRAPHY LA English DT Article ID DISSOLVED IRON CONCENTRATIONS; PARTICULATE ORGANIC-MATTER; MARINE-PHYTOPLANKTON; ATLANTIC-OCEAN; NORTH PACIFIC; WORLD OCEAN; THALASSIOSIRA-PSEUDONANA; BIOGENIC SILICA; SOUTHERN-OCEAN; RELEASE RATES AB Macronutrients in sinking phytoplankton are typically remineralized at different rates, but less is known about the fate of micronutrient metals associated with sinking cells. Scavenging, the presence of co-occurring abiotic particles, and inadvertent contamination limit the utility of bulk analytical approaches to study remineralization of trace metals in sinking phytoplankton. We used synchrotron x-ray fluorescence mapping to measure macronutrients (P, S, and Si) and trace metals (Fe, Ni, and Zn) in individual cells of the diatom Asterionellopsis glacialis during a spring bloom in subtropical waters off New Zealand. P, S, Zn, and Ni were released significantly faster than Fe and Si from sinking cells in the upper 200 m. Bulk particulate element fluxes to sediment traps indicated similar trends, but biogenic silica flux was attenuated much faster than Si was lost from intact sinking cells collected in the traps. The metals were spatially co-located with P and S in upper ocean cells, but this association with P and S (based on a spatial resolution of 450 nm) was largely absent in sinking cells. In contrast, Fe retained a weak spatial association with Si, suggesting that remineralized Fe may be re-scavenged onto cell surfaces. As a result, dissolved Fe : macronutrient stoichiometries in the water column likely underestimate stoichiometries in sinking cells. We propose linkages between the selective loss of diatom cellular components (e.g., ribosomes or phospholipid membranes, Zn-finger proteins, and urease) and the observed recycling of specific elements (P, Zn, and Ni, respectively), which set the stoichiometry of macro-and micronutrient supply to surface waters. C1 [Twining, Benjamin S.] Bigelow Lab Ocean Sci, East Boothbay, ME 04544 USA. [Nodder, Scott D.; Maas, Elizabeth W.; Boyd, Philip W.] Natl Inst Water & Atmospher Res NIWA Ltd, Wellington, New Zealand. [King, Andrew L.; Hutchins, David A.] Univ So Calif, Dept Biol Sci, Los Angeles, CA 90089 USA. [LeCleir, Gary R.; Wilhelm, Steven W.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [LeCleir, Gary R.; Wilhelm, Steven W.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37932 USA. [DeBruyn, Jennifer M.] Univ Tennessee, Dept Biosyst Engn & Soil Sci, Knoxville, TN USA. [Vogt, Stefan] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Boyd, Philip W.] Univ Otago, NIWA Ctr Chem & Phys Oceanog, Dunedin, New Zealand. RP Twining, BS (reprint author), Bigelow Lab Ocean Sci, East Boothbay, ME 04544 USA. EM btwining@bigelow.org RI Boyd, Philip/J-7624-2014; Wilhelm, Steven/B-8963-2008; DeBruyn, Jennifer/A-8813-2010; Vogt, Stefan/B-9547-2009; Vogt, Stefan/J-7937-2013; OI Boyd, Philip/0000-0001-7850-1911; Wilhelm, Steven/0000-0001-6283-8077; DeBruyn, Jennifer/0000-0002-2993-4144; Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513; Twining, Benjamin/0000-0002-1365-9192 FU New Zealand Ministry of Science Innovation [CO1X0501]; U.S. National Science Foundation [OCE 0825379/0825405/0825319]; U.S. DOE [DE-AC02-06CH11357] FX The FeCycle II project was supported by New Zealand Ministry of Science & Innovation funding to the Coasts and Oceans OBI program (PWB, SDN, EWM, CO1X0501) and by a grant from the U.S. National Science Foundation (OCE 0825379/0825405/0825319) to BST, SWW, and DAH. R. Frew, S. Searson, and L. Northcote assisted with sediment trap cleaning, deployment, and sample processing, respectively. F. Hoe Chang (National Institute of Water and Atmospheric Research) provided phytoplankton identification and counts. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. We thank two anonymous reviewers for comments that improved the paper. NR 65 TC 22 Z9 23 U1 5 U2 57 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0024-3590 EI 1939-5590 J9 LIMNOL OCEANOGR JI Limnol. Oceanogr. PD MAY PY 2014 VL 59 IS 3 BP 689 EP 704 DI 10.4319/lo.2014.59.3.0689 PG 16 WC Limnology; Oceanography SC Marine & Freshwater Biology; Oceanography GA AM5MQ UT WOS:000339904300005 ER PT J AU Shehabi, A Walker, B Masanet, E AF Shehabi, Arman Walker, Ben Masanet, Eric TI The energy and greenhouse-gas implications of internet video streaming in the United States SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE life-cycle assessment; energy; greenhouse gases; data center; cloud computing; streaming video ID TECHNOLOGIES; NETWORKS; INFORMATION; COMMERCE; DELIVERY; IMPACTS AB The rapid growth of streaming video entertainment has recently received attention as a possibly less energy intensive alternative to the manufacturing and transportation of digital video discs (DVDs). This study utilizes a life-cycle assessment approach to estimate the primary energy use and greenhouse-gas emissions associated with video viewing through both traditional DVD methods and online video streaming. Base-case estimates for 2011 video viewing energy and CO2(e) emission intensities indicate video streaming can be more efficient than DVDs, depending on DVD viewing method. Video streaming benefits from relatively more efficient end-user devices than DVD viewing, though much of that savings is lost when accounting for the additional energy from network data transmission. Video streaming appears distinctly favorable when compared against any DVD viewing that includes consumer driving, which significantly increases the energy and CO2(e) emissions per viewing hour. Total US 2011 video viewing required about 192 PJ of primary energy and emitted about 10.5 billion kg of CO2(e). Shifting all 2011 DVD viewing to video streaming reduces the total primary energy use to about 162 PJ and the CO2(e) emissions to about 8.6 billion kg, representing a savings equivalent to the primary energy used to meet the electricity demand of nearly 200 000 US households each year. Sensitivity analysis indicates that results are most influenced by the end-user DVD player power demand, data transmission energy, and consumer travel for store DVDs. Data center energy use-both operational and embodied within the IT equipment-account for <1% of the total video streaming energy use. Results from this study indicate that designers and policy makers should focus on the efficiency of end-user devices and network transmission energy to curb future increases in energy use from the proliferation of video streaming. C1 [Shehabi, Arman] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Walker, Ben; Masanet, Eric] Northwestern Univ, McCormick Sch Engn, Evanston, IL 60208 USA. RP Shehabi, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM ashehabi@lbl.gov RI Masanet, Eric /I-5649-2012 FU Google; Office of Science of the United States Department of Energy; [DE-AC02-05CH11231] FX This material is based upon work conducted by Lawrence Berkeley National Laboratory with support from Google. Lawrence Berkeley National Laboratory is supported by the Office of Science of the United States Department of Energy and operated under Contract Grant No. DE-AC02-05CH11231. NR 57 TC 4 Z9 4 U1 1 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD MAY PY 2014 VL 9 IS 5 AR 054007 DI 10.1088/1748-9326/9/5/054007 PG 11 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA AM5GM UT WOS:000339885100008 ER PT J AU Oliveira-Neto, F Pontes, P Wichmann, B AF Oliveira-Neto, Francisco Pontes, Paulo Wichmann, Bruno TI A Benchmarking Analysis of the Brazilian Airport Infrastructure SO JOURNAL OF TRANSPORT ECONOMICS AND POLICY LA English DT Article ID NONPARAMETRIC FRONTIER ESTIMATION; DATA ENVELOPMENT ANALYSIS; COMMERCIAL AIRPORTS; EFFICIENCY SCORES; PRODUCTIVITY; DEA AB This paper assesses the technical efficiency (TE) of the infrastructure of sixty-three major airports in Brazil. We use the order-m approach in which airports are benchmarked against an expected minimum input frontier. Despite being a non-parametric estimator, the order-m is robust to noise in the data, outliers, and extreme values. In addition, the approach is able to rank airports successfully even in a small sample, a characteristic unusual for traditional non-parametric estimators. We find that international airports are more efficient than domestic ones. We also find evidence that order-m TB estimation of domestic and international airports must be done separately. C1 [Wichmann, Bruno] Univ Alberta, Dept Resource Econ & Environm Sociol, Edmonton, AB, Canada. [Oliveira-Neto, Francisco] Oak Ridge Natl Lab, Ctr Transportat Anal, Knoxville, TN USA. [Pontes, Paulo] Inst Pesquisa & Estrategia Econ Ceara, Fortaleza, Ceara, Brazil. RP Wichmann, B (reprint author), Univ Alberta, Dept Resource Econ & Environm Sociol, 503 Gen Serv Bldg, Edmonton, AB, Canada. EM bwichmann@ualberta.ca NR 27 TC 0 Z9 0 U1 1 U2 9 PU UNIV BATH PI BATH PA JRNL OF TRANSPORT ECON & POL CLAVERTON DOWN, BATH BA2 7AY, AVON, ENGLAND SN 0022-5258 EI 1754-5951 J9 J TRANSP ECON POLICY JI J. Transp. Econ. Policy PD MAY PY 2014 VL 48 BP 297 EP 313 PN 2 PG 17 WC Economics; Transportation SC Business & Economics; Transportation GA AM5WK UT WOS:000339931500007 ER PT J AU Hu, PG Zhang, J Yoon, MN Qiao, XF Zhang, X Feng, W Tan, PH Zheng, W Liu, JJ Wang, XN Idrobo, JC Geohegan, DB Xiao, K AF Hu, Pingan Zhang, Jia Yoon, Mina Qiao, Xiao-Fen Zhang, Xin Feng, Wei Tan, Pingheng Zheng, Wei Liu, Jingjing Wang, Xiaona Idrobo, Juan C. Geohegan, David B. Xiao, Kai TI Highly sensitive phototransistors based on two-dimensional GaTe nanosheets with direct bandgap SO NANO RESEARCH LA English DT Article DE photodetector; gallium telluride; two-dimensional; semiconductor; nanosheet ID ULTRAFAST GRAPHENE PHOTODETECTOR; METAL DICHALCOGENIDE NANOSHEETS; CONTROLLED GROWTH; MONOLAYER MOS2; CRYSTALS; GAS; FABRICATION; FILMS AB Highly sensitive phototransistors based on two-dimensional (2D) GaTe nanosheet have been demonstrated. The performance (photoresponsivity, detectivity) of the GaTe nanosheet phototransistor can be efficiently adjusted by using the applied gate voltage. The devices exhibit an ultrahigh photoresponsivity of 274.3 AW(-1). The detectivity of 2D GaTe devices is similar to 10(12) Jones, which surpasses that of currently-exploited InGaAs photodetectors (10(11)-10(12) Jones). To reveal the origin of the enhanced photocurrent in GaTe nanosheets, theoretical modeling of the electronic structures was performed to show that GaTe nanosheets also have a direct bandgap structure, which contributes to the promotion of photon absorption and generation of excitons. This work shows that GaTe nanosheets are promising materials for high performance photodetectors. C1 [Hu, Pingan; Zhang, Jia; Feng, Wei; Zheng, Wei; Liu, Jingjing; Wang, Xiaona] Harbin Inst Technol, Key Lab Microsyst & Microstruct, Minist Educ, Harbin 150080, Peoples R China. [Yoon, Mina; Idrobo, Juan C.; Geohegan, David B.; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Qiao, Xiao-Fen; Zhang, Xin; Tan, Pingheng] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China. RP Hu, PG (reprint author), Harbin Inst Technol, Key Lab Microsyst & Microstruct, Minist Educ, 2 Yikuang St, Harbin 150080, Peoples R China. EM hupa@hit.edu.cn; phtan@semi.ac.cn; xiaok@ornl.gov RI Feng, Wei/J-5913-2014; TAN, Ping-Heng/D-1137-2009; zhang, xin/C-4163-2014; Idrobo, Juan/H-4896-2015; Yoon, Mina/A-1965-2016; Zhang, Jia/C-9453-2016; Geohegan, David/D-3599-2013; Hu, Ping'an/C-1289-2013 OI TAN, Ping-Heng/0000-0001-6575-1516; zhang, xin/0000-0002-1450-2525; Idrobo, Juan/0000-0001-7483-9034; Yoon, Mina/0000-0002-1317-3301; Geohegan, David/0000-0003-0273-3139; FU National Natural Science Foundation of China (NSFC) [61172001, 21373068, 11225421, 10934007]; National Basic Research Program of China [2013CB632900, 2009CB929301]; Scientific User Facility Division, Office of Basic Energy Sciences, U.S. Department of Energy; Laboratory Directed Research and Development award from Oak Ridge National Laboratory (ORNL); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors gratefully acknowledge financial support from National Natural Science Foundation of China (NSFC, Nos. 61172001, 21373068, 11225421, and 10934007), and the National Basic Research Program of China (Nos. 2013CB632900 and 2009CB929301). Part of the research was conducted at the Center for Nanophase Materials Sciences, which are sponsored at Oak Ridge National Laboratory by the Scientific User Facility Division, Office of Basic Energy Sciences, U.S. Department of Energy. K. X. and M. Y. acknowledge support provided by a Laboratory Directed Research and Development award from Oak Ridge National Laboratory (ORNL). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 38 Z9 38 U1 12 U2 94 PU TSINGHUA UNIV PRESS PI BEIJING PA TSINGHUA UNIV, RM A703, XUEYAN BLDG, BEIJING, 10084, PEOPLES R CHINA SN 1998-0124 EI 1998-0000 J9 NANO RES JI Nano Res. PD MAY PY 2014 VL 7 IS 5 BP 694 EP 703 DI 10.1007/s12274-014-0430-2 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AM5IS UT WOS:000339891400006 ER PT J AU Ashby, MLN Stanford, SA Brodwin, M Gonzalez, AH Martinez-Manso, J Bartlett, JG Benson, BA Bleem, LE Crawford, TM Dey, A Dressler, A Eisenhardt, PRM Galametz, A Jannuzi, BT Marrone, DP Mei, S Muzzin, A Pacaud, F Pierre, M Stern, D Vieira, JD AF Ashby, M. L. N. Stanford, S. A. Brodwin, M. Gonzalez, A. H. Martinez-Manso, J. Bartlett, J. G. Benson, B. A. Bleem, L. E. Crawford, T. M. Dey, A. Dressler, A. Eisenhardt, P. R. M. Galametz, A. Jannuzi, B. T. Marrone, D. P. Mei, S. Muzzin, A. Pacaud, F. Pierre, M. Stern, D. Vieira, J. D. TI THE SPITZER SOUTH POLE TELESCOPE DEEP FIELD: SURVEY DESIGN AND INFRARED ARRAY CAMERA CATALOGS (vol 209, 16, 2013) SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Correction C1 [Ashby, M. L. N.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Stanford, S. A.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Stanford, S. A.] Lawrence Livermore Natl Lab, Inst Geophys & Planetary Phys, Livermore, CA 94551 USA. [Brodwin, M.] Univ Missouri, Dept Phys & Astron, Kansas City, MO 64110 USA. [Gonzalez, A. H.; Martinez-Manso, J.] Univ Florida, Dept Astron, Gainesville, FL 32611 USA. [Bartlett, J. G.] Univ Paris Diderot, CEA IRFU, Observ Paris, Sorbonne Paris Cite,CNRS IN2P3, F-75205 Paris 13, France. [Benson, B. A.; Bleem, L. E.; Crawford, T. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Benson, B. A.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Bleem, L. E.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Crawford, T. M.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Dey, A.] Natl Opt Astron Observ, Tucson, AZ 85719 USA. [Dressler, A.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Eisenhardt, P. R. M.; Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Galametz, A.] INAF Osservatorio Roma, I-00040 Monte Porzio Catone, Italy. [Jannuzi, B. T.; Marrone, D. P.] Univ Arizona, Dept Astron, Tucson, AZ 85719 USA. [Jannuzi, B. T.; Marrone, D. P.] Univ Arizona, Steward Observ, Tucson, AZ 85719 USA. [Mei, S.] Observ Paris, GEPI, Sect Meudon, F-92190 Meudon, France. [Mei, S.] Univ Paris Denis Diderot, F-75205 Paris 13, France. [Mei, S.] Infrared Proc & Anal Ctr, Pasadena, CA 91125 USA. [Muzzin, A.] Leiden Univ, Leiden Observ, NL-9513 RA Leiden, Netherlands. [Pacaud, F.] Argelander Inst Astron, D-53121 Bonn, Germany. [Pierre, M.] AIM IRFU DSM CEA, Serv Astrophys, F-91190 Gif Sur Yvette, France. [Vieira, J. D.] CALTECH, Pasadena, CA 91125 USA. RP Ashby, MLN (reprint author), Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. EM mashby@cfa.harvard.edu NR 1 TC 2 Z9 2 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 EI 1538-4365 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD MAY PY 2014 VL 212 IS 1 AR 16 DI 10.1088/0067-0049/212/1/16 PG 2 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AL6HG UT WOS:000339232600016 ER PT J AU Mandelbaum, R Rowe, B Bosch, J Chang, C Courbin, F Gill, M Jarvis, M Kannawadi, A Kacprzak, T Lackner, C Leauthaud, A Miyatake, H Nakajima, R Rhodes, J Simet, M Zuntz, J Armstrong, B Bridle, S Coupon, J Dietrich, JP Gentile, M Heymans, C Jurling, AS Kent, SM Kirkby, D Margala, D Massey, R Melchior, P Peterson, J Roodman, A Schrabback, T AF Mandelbaum, Rachel Rowe, Barnaby Bosch, James Chang, Chihway Courbin, Frederic Gill, Mandeep Jarvis, Mike Kannawadi, Arun Kacprzak, Tomasz Lackner, Claire Leauthaud, Alexie Miyatake, Hironao Nakajima, Reiko Rhodes, Jason Simet, Melanie Zuntz, Joe Armstrong, Bob Bridle, Sarah Coupon, Jean Dietrich, Jorg P. Gentile, Marc Heymans, Catherine Jurling, Alden S. Kent, Stephen M. Kirkby, David Margala, Daniel Massey, Richard Melchior, Peter Peterson, John Roodman, Aaron Schrabback, Tim TI THE THIRD GRAVITATIONAL LENSING ACCURACY TESTING (GREAT3) CHALLENGE HANDBOOK SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Article DE gravitational lensing: weak; methods: data analysis; methods: statistical; techniques: image processing ID HUBBLE-SPACE-TELESCOPE; DIGITAL SKY SURVEY; IMAGE-ANALYSIS COMPETITION; COSMIC SHEAR MEASUREMENT; POINT-SPREAD FUNCTION; ATMOSPHERIC-TURBULENCE; ADVANCED CAMERA; DARK-MATTER; SHAPE MEASUREMENTS; POLAR SHAPELETS AB The GRavitational lEnsing Accuracy Testing 3 (GREAT3) challenge is the third in a series of image analysis challenges, with a goal of testing and facilitating the development of methods for analyzing astronomical images that will be used to measure weak gravitational lensing. This measurement requires extremely precise estimation of very small galaxy shape distortions, in the presence of far larger intrinsic galaxy shapes and distortions due to the blurring kernel caused by the atmosphere, telescope optics, and instrumental effects. The GREAT3 challenge is posed to the astronomy, machine learning, and statistics communities, and includes tests of three specific effects that are of immediate relevance to upcoming weak lensing surveys, two of which have never been tested in a community challenge before. These effects include many novel aspects including realistically complex galaxy models based on high-resolution imaging from space; a spatially varying, physically motivated blurring kernel; and a combination of multiple different exposures. To facilitate entry by people new to the field, and for use as a diagnostic tool, the simulation software for the challenge is publicly available, though the exact parameters used for the challenge are blinded. Sample scripts to analyze the challenge data using existing methods will also be provided. C1 [Mandelbaum, Rachel; Kannawadi, Arun; Simet, Melanie] Carnegie Mellon Univ, McWilliams Ctr Cosmol, Pittsburgh, PA 15213 USA. [Rowe, Barnaby; Kacprzak, Tomasz] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Rowe, Barnaby; Rhodes, Jason] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Bosch, James; Miyatake, Hironao] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Chang, Chihway; Gill, Mandeep; Roodman, Aaron] Stanford Univ, KIPAC, Stanford, CA 94309 USA. [Courbin, Frederic; Gentile, Marc] EPFL, Astrophys Lab, Observ Sauverny, CH-1290 Versoix, Switzerland. [Jarvis, Mike; Armstrong, Bob] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Lackner, Claire; Leauthaud, Alexie] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba, Japan. [Nakajima, Reiko; Schrabback, Tim] Univ Bonn, Argelander Inst Astron, D-53121 Bonn, Germany. [Rhodes, Jason] CALTECH, Pasadena, CA 91125 USA. [Zuntz, Joe; Bridle, Sarah] Univ Manchester, Jodrell Bank Ctr Astrophys, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Coupon, Jean] Acad Sinica, Inst Astron & Astrophys, Taipei 10617, Taiwan. [Dietrich, Jorg P.] Univ Sternwarte Munchen, D-81679 Munich, Germany. [Dietrich, Jorg P.] Excellence Cluster Universe, D-85748 Munich, Germany. [Heymans, Catherine] Univ Edinburgh, Scottish Univ Phys Alliance, Inst Astron, Royal Observ, Edinburgh EH9 3HJ, Midlothian, Scotland. [Jurling, Alden S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Jurling, Alden S.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14618 USA. [Kent, Stephen M.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Kirkby, David; Margala, Daniel] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Massey, Richard] Univ Durham, Inst Computat Cosmol, Durham DH1 3LE, England. [Melchior, Peter] Ohio State Univ, Ctr Cosmol & Astro Particle Phys, Columbus, OH 43210 USA. [Melchior, Peter] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Peterson, John] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. RP Mandelbaum, R (reprint author), Carnegie Mellon Univ, McWilliams Ctr Cosmol, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. RI Mandelbaum, Rachel/N-8955-2014; Simet, Melanie/A-3415-2016; EPFL, Physics/O-6514-2016; OI Mandelbaum, Rachel/0000-0003-2271-1527; Simet, Melanie/0000-0001-8823-8926; Kirkby, David/0000-0002-8828-5463; Dietrich, Jorg/0000-0002-8134-9591; Rowe, Barnaby/0000-0002-7042-9174; Massey, Richard/0000-0002-6085-3780 FU National Science Foundation [PHYS-1066293]; NASA via the Strategic University Research Partnership (SURP) Program of the Jet Propulsion Laboratory, California Institute of Technology; IST Programme of the European Community under the PASCAL2 Network of Excellence [IST-2007-216886]; NASA through Space Telescope Science Institute; NASA [NAS5-26555]; European Research Council [240672, 240185]; JSPS Postdoctoral Fellowships for Research Abroad; Swiss National Science Foundation (SNSF); LLC [De-AC02-07CH11359]; United States Department of Energy; [HST-AR-12857.01-A] FX The authors of this work benefited greatly from discussions with Christopher Hirata, Gary Bernstein, Lance Miller, and Erin Sheldon; the WFIRST project office, including David Content; the Euclid Consortium; and the LSST imSim team, including En-Hsin Peng; and Peter Freeman. We thank the PASCAL-2 network for its sponsorship of the challenge. This work was supported in part by the National Science Foundation under grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics.; This project was supported in part by NASA via the Strategic University Research Partnership (SURP) Program of the Jet Propulsion Laboratory, California Institute of Technology; and by the IST Programme of the European Community, under the PASCAL2 Network of Excellence, IST-2007-216886. This article only reflects the authors' views.; R.M. was supported in part by program HST-AR-12857.01-A, provided by NASA through a grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555. B.R. and S.B. acknowledge support from the European Research Council in the form of a Starting Grant with number 240672. H.M. acknowledges support from JSPS Postdoctoral Fellowships for Research Abroad. C.H. acknowledges support from the European Research Council under the EC FP7 grant number 240185. F.C. and M.G. are supported by the Swiss National Science Foundation (SNSF).; Center for Particle Astrophysics, Fermi National Accelerator Laboratory is operated by Fermi Research Alliance, LLC under contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 100 TC 37 Z9 37 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 EI 1538-4365 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD MAY PY 2014 VL 212 IS 1 AR 5 DI 10.1088/0067-0049/212/1/5 PG 28 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AL6HG UT WOS:000339232600005 ER PT J AU Cho, SY Briscoe, JL Hansen, IA Smith, JK Chang, YM Brener, I AF Cho, Sang-Yeon Briscoe, Jayson L. Hansen, Immo A. Smith, Jesse K. Chang, Yoomi Brener, Igal TI Label-Free Plasmonic Immunosensing for Plasmodium in a Whole Blood Lysate SO IEEE SENSORS JOURNAL LA English DT Article DE Biosensors; malaria; nanohole array; optical sensor; surface plasmon polaritons; whole blood sensing ID OF-CARE DIAGNOSTICS; POLYMER BRUSHES; REAL-TIME; SURFACE; RESONANCE; TRANSMISSION; BINDING; FILMS; BIOSENSOR; MALARIA AB In this paper, we report an experimental demonstration of malaria pathogen detection in a whole blood lysate using plasmonic nanostructures. The plasmon sensor utilizes extraordinary optical transmission through a nanostructure to directly probe antibody-antigen interactions. The measured refractive index sensitivity of the nanostructured sensor is 378 nm per refractive index unit in the visible range. The surface chemistry reported here provides highly site directed and stable antibody immobilization. To validate the observed response of the optical sensor, positive and negative control tests were performed. Results confirm that a refractive index change induced by the interaction between immobilized antibodies and malaria parasites is successfully detected by the fabricated sensor. The demonstrated plasmonic sensor is a compact, highly sensitive, cost effective, selective diagnostic tool for many portable biosensing applications, such as point-of-care diagnostics. C1 [Cho, Sang-Yeon; Briscoe, Jayson L.] New Mexico State Univ, Dept Elect Engn, Klipsch Sch, Las Cruces, NM 88003 USA. [Hansen, Immo A.; Smith, Jesse K.] New Mexico State Univ, Dept Biol & Inst Appl Biosci, Las Cruces, NM 88003 USA. [Chang, Yoomi] New Mexico State Univ, Dept Chem & Biochem, Las Cruces, NM 88003 USA. [Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Cho, SY (reprint author), New Mexico State Univ, Dept Elect Engn, Klipsch Sch, Las Cruces, NM 88003 USA. EM sangycho@nmsu.edu; briscojl@nmsu.edu; immoh@nmsu.edu; jksmith@nmsu.edu; changy@nmsu.edu; ibrener@sandia.gov RI Cho, Sang-Yeon/C-3075-2008 OI Cho, Sang-Yeon/0000-0002-4721-4087 FU Bill and Melinda Gates Foundation through the Grand Challenges Exploration Initiative; U.S. Department of Energy, Center for Integrated Nanotechnologies, Sandia National Laboratories [DE-AC04-94AL85000] FX This work was supported in part by the Bill and Melinda Gates Foundation through the Grand Challenges Exploration Initiative and in part by the U.S. Department of Energy, Center for Integrated Nanotechnologies, Sandia National Laboratories under Contract DE-AC04-94AL85000. An earlier version of this paper was presented at the IEEE Sensors Conference in 2013 and was published in its Proceedings. The associate editor coordinating the review of this paper and approving it for publication was Prof. Julian C. C. Chan. NR 35 TC 6 Z9 6 U1 4 U2 21 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1530-437X EI 1558-1748 J9 IEEE SENS J JI IEEE Sens. J. PD MAY PY 2014 VL 14 IS 5 BP 1399 EP 1404 DI 10.1109/JSEN.2013.2295714 PG 6 WC Engineering, Electrical & Electronic; Instruments & Instrumentation; Physics, Applied SC Engineering; Instruments & Instrumentation; Physics GA AM1QX UT WOS:000339624000007 ER PT J AU Benuzzi-Mounaix, A Mazevet, S Ravasio, A Vinci, T Denoeud, A Koenig, M Amadou, N Brambrink, E Festa, F Levy, A Harmand, M Brygoo, S Huser, G Recoules, V Bouchet, J Morard, G Guyot, F de Resseguier, T Myanishi, K Ozaki, N Dorchies, F Gaudin, J Leguay, PM Peyrusse, O Henry, O Raffestin, D Le Pape, S Smith, R Musella, R AF Benuzzi-Mounaix, Alessandra Mazevet, Stephane Ravasio, Alessandra Vinci, Tommaso Denoeud, Adrien Koenig, Michel Amadou, Nourou Brambrink, Erik Festa, Floriane Levy, Anna Harmand, Marion Brygoo, Stephanie Huser, Gael Recoules, Vanina Bouchet, Johan Morard, Guillaume Guyot, Francois de Resseguier, Thibaut Myanishi, Kohei Ozaki, Norimasa Dorchies, Fabien Gaudin, Jerome Leguay, Pierre Marie Peyrusse, Olivier Henry, Olivier Raffestin, Didier Le Pape, Sebastien Smith, Ray Musella, Riccardo TI Progress in warm dense matter study with applications to planetology SO PHYSICA SCRIPTA LA English DT Article; Proceedings Paper CT International Conference on Research and Applications of Plasmas (PLASMA) CY SEP 02-06, 2013 CL Inst Plasma Phys & Laser Microfus, Warsaw, POLAND SP Polish Phys Soc HO Inst Plasma Phys & Laser Microfus DE laser compression; ab initio calculations; strongly coupled plasma ID EARTHS CORE; IRON; EXOPLANETS; STATE; EQUATION AB We present an overview of some recent theoretical and experimental results obtained on the properties of iron and silica at conditions encountered in planetary interiors. The first part is concerned with the development of x-ray absorption near edge spectroscopy in dynamical experiments using high-energy lasers as a tool to investigate phase transitions and structural changes at extreme pressure-temperature conditions for these two key constituents. The second part focuses on the development of a quasi-isentropic compression technique to achieve the pressure-temperature conditions anticipated in planetary interiors (3-10 Mbar, 5000-8000 K). The experiments were performed using the LULI, LLNL and LIL high-energy lasers' facilities. The experimental results are analyzed using first-principle simulations based on density functional theory. C1 [Benuzzi-Mounaix, Alessandra; Ravasio, Alessandra; Vinci, Tommaso; Denoeud, Adrien; Koenig, Michel; Amadou, Nourou; Brambrink, Erik; Festa, Floriane; Levy, Anna; Harmand, Marion] UPMC, CEA, CNRS, LULI,Ecole Polytech, F-91128 Palaiseau, France. [Benuzzi-Mounaix, Alessandra; Mazevet, Stephane; Musella, Riccardo] Univ Paris Diderot, CNRS, Observ Paris, LUTH, F-92195 Meudon, France. [Mazevet, Stephane; Brygoo, Stephanie; Huser, Gael; Recoules, Vanina; Bouchet, Johan] CEA, DAM, DIF, F-91297 Arpajon, France. [Morard, Guillaume; Guyot, Francois] Univ Paris 06, CNRS, IMPMC Univ Paris Diderot, IPGP, Paris, France. [de Resseguier, Thibaut] Univ Poitiers, ENSMA, CNRS, Inst P, Poitiers, France. [Myanishi, Kohei; Ozaki, Norimasa] Osaka Univ, Grad Sch Engn, Suita, Osaka 5650871, Japan. [Dorchies, Fabien; Gaudin, Jerome; Leguay, Pierre Marie; Peyrusse, Olivier] Univ Bordeaux CNRS CEA, Ctr Lasers Intenses & Applicat CELIA, F-33405 Talence, France. [Henry, Olivier; Raffestin, Didier] CEA, CESTA, DAM, F-33114 Le Barp, France. [Le Pape, Sebastien; Smith, Ray] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Benuzzi-Mounaix, A (reprint author), UPMC, CEA, CNRS, LULI,Ecole Polytech, Route Saclay, F-91128 Palaiseau, France. EM alessandra.benuzzi-mounaix@polytechnique.fr RI lepape, sebastien/J-3010-2015; GUYOT, Francois/C-3824-2016; IMPMC, Geobio/F-8819-2016; harmand, marion/Q-1248-2016 OI GUYOT, Francois/0000-0003-4622-2218; harmand, marion/0000-0003-0713-5824 FU [ANR-07-BLANC-0239 SECHEL]; [ANR-12-BS04-0015-04 PLANETLAB] FX We wish to warmly thank the LIL and LULI technical staff and ANR-07-BLANC-0239 SECHEL and ANR-12-BS04-0015-04 PLANETLAB for the support. NR 38 TC 4 Z9 4 U1 1 U2 23 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 EI 1402-4896 J9 PHYS SCRIPTA JI Phys. Scr. PD MAY PY 2014 VL T161 AR 014060 DI 10.1088/0031-8949/2014/T161/014060 PG 8 WC Physics, Multidisciplinary SC Physics GA AM1PP UT WOS:000339620200061 ER PT J AU Lorkiewicz, J Nietubyc, R Barlak, M Mirowski, R Bartnik, A Kostecki, J Sekutowicz, J Malinowska, A Kneisel, P Witkowski, J AF Lorkiewicz, Jerzy Nietubyc, Robert Barlak, Marek Mirowski, Robert Bartnik, Andrzej Kostecki, Jerzy Sekutowicz, Jacek Malinowska, Aneta Kneisel, Peter Witkowski, Jan TI Deposition and optimization of thin lead layers for superconducting accelerator photocathodes SO PHYSICA SCRIPTA LA English DT Article; Proceedings Paper CT International Conference on Research and Applications of Plasmas (PLASMA) CY SEP 02-06, 2013 CL Inst Plasma Phys & Laser Microfus, Warsaw, POLAND SP Polish Phys Soc HO Inst Plasma Phys & Laser Microfus DE superconducting electron photoinjector; photocathode; UHV arc deposition; rod plasma injector AB A combination of a ultra high vacuum arc deposition system and a recrystallization method was used to optimize the smoothness and thickness of thin-layer lead cathodes for superconducting niobium electron injectors. A non-filtered arc system was chosen to deposit Pb films on niobium. The films then underwent melting and recrystallization by treating them with pulsed argon ion beams in a rod plasma injector. C1 [Lorkiewicz, Jerzy; Nietubyc, Robert; Barlak, Marek; Mirowski, Robert; Malinowska, Aneta; Witkowski, Jan] Natl Ctr Nucl Res NCBJ, PL-05400 Otwock, Poland. [Bartnik, Andrzej; Kostecki, Jerzy] Mil Univ Technol IOE MUT, Inst Optoelect, PL-00908 Warsaw, Poland. [Sekutowicz, Jacek] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany. [Kneisel, Peter] TJNAF, Newport News, VA USA. RP Lorkiewicz, J (reprint author), Natl Ctr Nucl Res NCBJ, 7 Andrzeja Soltana, PL-05400 Otwock, Poland. EM jerzy.lorkiewicz@ncbj.gov.pl FU European Coordination in Accelerator Research and Development, a part of FP7 FX Investigations were supported with European Coordination in Accelerator Research and Development, a part of FP7. NR 11 TC 1 Z9 1 U1 2 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 EI 1402-4896 J9 PHYS SCRIPTA JI Phys. Scr. PD MAY PY 2014 VL T161 AR 014071 DI 10.1088/0031-8949/2014/T161/014071 PG 5 WC Physics, Multidisciplinary SC Physics GA AM1PP UT WOS:000339620200072 ER PT J AU Rhee, M Liu, P Meagher, RJ Light, YK Singh, AK AF Rhee, Minsoung Liu, Peng Meagher, Robert J. Light, Yooli K. Singh, Anup K. TI Versatile on-demand droplet generation for controlled encapsulation SO BIOMICROFLUIDICS LA English DT Article ID MICROFLUIDIC PLATFORM; SOFT LITHOGRAPHY; FLOW; MANIPULATION; SYSTEMS; ARRAYS AB We present a droplet-based microfluidic system for performing bioassays requiring controlled analyte encapsulation by employing highly flexible on-demand droplet generation. On-demand droplet generation and encapsulation are achieved pneumatically using a microdispensing pump connected to a constant pressure source. The system generates single droplets to the collection route only when the pump is actuated with a designated pressure level and produces two-phase parallel flow to the waste route during the stand-by state. We analyzed the effect of actuation pressure on the stability and size of droplets and optimized conditions for generation of stable droplets over a wide pressure range. By increasing the duration of pump actuation, we could either trigger a short train of identical size droplets or generate a single larger droplet. We also investigated the methodology to control droplet contents by fine-tuning flow rates or implementing a resistance bridge between the pump and main channels. We demonstrated the integrated chip for on-demand mixing between two aqueous phases in droplets and on-demand encapsulation of Escherichia coli cells. Our unique on-demand feature for selective encapsulation is particularly appropriate for bioassays with extremely dilute samples, such as pathogens in a clinical sample, since it can significantly reduce the number of empty droplets that impede droplet collection and subsequent data analysis. (C) 2014 AIP Publishing LLC. C1 [Rhee, Minsoung; Liu, Peng; Meagher, Robert J.; Light, Yooli K.; Singh, Anup K.] Sandia Natl Labs, Livermore, CA 94550 USA. [Singh, Anup K.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. RP Singh, AK (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM aksingh@sandia.gov FU NIDCR - U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [R01 DE020891]; US DOE, Office of Science, Office of Biological and Environmental Research [DE-AC02-05 CH11231]; US DOE's Nuclear Security Administration [DE-AC04-94AL85000] FX We thank David Brekke for his support and guidance for experiments and David Heredia for consistent assistance with clean room use. We are also grateful to Matthew Piccini, Ben Schudel, Mais Jebrail, Junyu Mai, and Mary Bao Trang for helpful conversations and help with the laboratory work. We also acknowledge Victoria VanderNoot for valuable advice. Financial support for the work was provided by the grants: R01 DE020891, funded by the NIDCR; ENIGMA, a LBNL Scientific Focus Area Program supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research; and the DOE Joint BioEnergy Institute supported by the US DOE, Office of Science, Office of Biological and Environmental Research through Contract No. DE-AC02-05 CH11231 (LBNL). Sandia is a Multiprogram Laboratory operated by Sandia Corporation, a Lockheed Martin Company, for US DOE's Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 27 TC 3 Z9 3 U1 8 U2 52 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1932-1058 J9 BIOMICROFLUIDICS JI Biomicrofluidics PD MAY PY 2014 VL 8 IS 3 AR 034112 DI 10.1063/1.4874715 PG 12 WC Biochemical Research Methods; Biophysics; Nanoscience & Nanotechnology; Physics, Fluids & Plasmas SC Biochemistry & Molecular Biology; Biophysics; Science & Technology - Other Topics; Physics GA AL3DB UT WOS:000339004500012 PM 25379072 ER PT J AU Schmid, B Tomlinson, JM Hubbe, JM Comstock, JM Mei, F Chand, D Pekour, MS Kluzek, CD Andrews, E Biraud, SC Mcfarquhar, GM AF Schmid, B. Tomlinson, J. M. Hubbe, J. M. Comstock, J. M. Mei, F. Chand, D. Pekour, M. S. Kluzek, C. D. Andrews, E. Biraud, S. C. Mcfarquhar, G. M. TI THE DOE ARM AERIAL FACILITY SO BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY LA English DT Article ID SOUTHERN GREAT-PLAINS; AEROSOL OPTICAL-PROPERTIES; SPECTRAL-RESOLUTION LIDAR; IN-SITU MEASUREMENTS; SIZE DISTRIBUTION; CARBONACEOUS AEROSOL; ATMOSPHERIC RESEARCH; SPARTICUS CAMPAIGN; CENTRAL CALIFORNIA; UNITED-STATES AB The Department of Energy Atmospheric Radiation Measurement (ARM) program is a climate research user facility operating stationary ground sites that provide long-term measurements of climate-relevant properties, mobile ground- and ship-based facilities to conduct shorter field campaigns (6-12 months), and the ARM Aerial Facility (AAF). The airborne observations acquired by the AAF enhance the surface-based ARM measurements by providing high-resolution in situ measurements for process understanding, retrieval-algorithm development, and model evaluation that are not possible using surface- or satellite-based techniques. Several ARM aerial efforts were consolidated to form AAF in 2006. With the exception of a small aircraft used for routine measurements of aerosols and carbon cycle gases, AAF at the time had no dedicated aircraft and only a small number of instruments at its disposal. AAF successfully carried out several missions contracting with organizations and investigators who provided their research aircraft and instrumentation. In 2009, AAF started managing operations of the Battelle-owned Gulfstream I (G-1) large twin-turboprop research aircraft. Furthermore, the American Recovery and Reinvestment Act of 2009 provided funding for the procurement of over twenty new instruments to be used aboard the G-1 and AAF contracted aircraft. Depending on the requested scope, AAF now executes campaigns using the G-1 or contracted aircraft, producing freely available datasets for studying gas, aerosol, cloud, and radiative processes and their interactions in the atmosphere. AAF is also engaged in the maturation and testing of newly developed airborne sensors to help foster the next generation of airborne instruments. C1 [Schmid, B.; Tomlinson, J. M.; Hubbe, J. M.; Comstock, J. M.; Mei, F.; Chand, D.; Pekour, M. S.; Kluzek, C. D.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Andrews, E.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Biraud, S. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Mcfarquhar, G. M.] Univ Illinois, Urbana, IL USA. RP Schmid, B (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM beat.schmid@pnnl.gov RI Biraud, Sebastien/M-5267-2013; OI Biraud, Sebastien/0000-0001-7697-933X; Mei, Fan/0000-0003-4285-2749; McFarquhar, Greg/0000-0003-0950-0135 FU ARM; California Energy Commission FX The ARM Aerial Facility is an integral part of the Department of Energy (DOE) Office of Science Atmospheric Radiation Measurement (ARM) Program. Funding for the campaigns described here has been provided by ARM, with contributions from the DOE Atmospheric Systems Research Program, NASA, and the Canadian National Research Council. The CalWater campaign has been funded by the California Energy Commission. It is the dedication of lead scientists, instrument scientists, engineers, and technicians from many agencies, institutions, and research companies; pilots; ground crew; fixed base operators; contracting officers; administrative personnel; program managers; and many others that make the AAF successful NR 106 TC 10 Z9 10 U1 3 U2 20 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0003-0007 EI 1520-0477 J9 B AM METEOROL SOC JI Bull. Amer. Meteorol. Soc. PD MAY PY 2014 VL 95 IS 5 BP 723 EP + DI 10.1175/BAMS-D-13-00040.1 PG 21 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AL4GS UT WOS:000339091500009 ER PT J AU Hahn, SH Welander, AS Yoon, SW Bak, JG Eidietis, NW Han, HS Humphreys, DA Hyatt, A Jeon, YM Johnson, RD Kim, HS Kim, J Kolemen, E Mueller, D Penaflor, BG Piglowski, DA Shin, GW Walker, ML Woo, MH AF Hahn, Sang-hee Welander, A. S. Yoon, S. W. Bak, J. G. Eidietis, N. W. Han, H. S. Humphreys, D. A. Hyatt, A. Jeon, Y. M. Johnson, R. D. Kim, H. S. Kim, J. Kolemen, E. Mueller, D. Penaflor, B. G. Piglowski, D. A. Shin, G. W. Walker, M. L. Woo, M. H. TI Progress and improvement of KSTAR plasma control using model-based control simulators SO FUSION ENGINEERING AND DESIGN LA English DT Article; Proceedings Paper CT 9th IAEA Technical Meeting on Control, Data Acquisition and Remote Participation for Fusion Research CY MAY 06-10, 2013 CL Hefei, PEOPLES R CHINA DE Magnetic fusion; Tokamak; Simulator; KSTAR; Plasma control; Control design ID DIII-D; TOKAMAKS AB Superconducting tokamaks like KSTAR, EAST and ITER need elaborate magnetic controls mainly due to either the demanding experiment schedule or tighter hardware limitations caused by the superconducting coils. In order to reduce the operation runtime requirements, two types of plasma simulators for the KSTAR plasma control system (PCS) have been developed for improving axisymmetric magnetic controls. The first one is an open-loop type, which can reproduce the control done in an old shot by loading the corresponding diagnostics data and PCS setup. The other one, a closed-loop simulator based on a linear nonrigid plasma model, is designed to simulate dynamic responses of the plasma equilibrium and plasma current (I-p,) due to changes of the axisymmetric poloidal field (PF) coil currents, poloidal beta, and internal inductance. The closed-loop simulator is the one that actually can test and enable alteration of the feedback control setup for the next shot. The simulators have been used routinely in 2012 plasma campaign, and the experimental performances of the axisymmetric shape control algorithm are enhanced. Quality of the real-time EFIT has been enhanced by utilizations of the open-loop type. Using the closed-loop type, the decoupling scheme of the plasma current control and axisymmetric shape controls are verified through both the simulations and experiments. By combining with the relay feedback tuning algorithm, the improved controls helped to maintain the shape suitable for longer H-mode (10-16s) with the number of required commissioning shots largely reduced. (C) 2013 Elsevier B.V. All rights reserved. C1 [Hahn, Sang-hee; Yoon, S. W.; Bak, J. G.; Han, H. S.; Jeon, Y. M.; Kim, H. S.; Kim, J.; Woo, M. H.] Natl Fus Res Inst, Taejon, South Korea. [Welander, A. S.; Eidietis, N. W.; Humphreys, D. A.; Hyatt, A.; Johnson, R. D.; Penaflor, B. G.; Piglowski, D. A.; Walker, M. L.] Gen Atom Co, San Diego, CA USA. [Kolemen, E.; Mueller, D.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Shin, G. W.] Univ Sci & Technol, Taejon, South Korea. RP Hahn, SH (reprint author), Natl Fus Res Inst, 169-148 Gwahak Ro, Taejon, South Korea. EM hahn76@nfri.re.kr FU Ministry of Science, ICT and Future Planning; NRF FX This work was supported by the Ministry of Science, ICT and Future Planning under the KSTAR project, and the NRF A3 Foresight Program in field of Plasma Physics. NR 17 TC 1 Z9 1 U1 0 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0920-3796 EI 1873-7196 J9 FUSION ENG DES JI Fusion Eng. Des. PD MAY PY 2014 VL 89 IS 5 BP 542 EP 547 DI 10.1016/j.fusengdes.2013.12.040 PG 6 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AL4VT UT WOS:000339133600009 ER PT J AU Davis, WM Ko, MK Maqueda, RJ Roquemore, AL Scotti, F Zweben, SJ AF Davis, W. M. Ko, M. K. Maqueda, R. J. Roquemore, A. L. Scotti, F. Zweben, S. J. TI Fast 2-D camera control, data acquisition, and database techniques for edge studies on NSTX SO FUSION ENGINEERING AND DESIGN LA English DT Article; Proceedings Paper CT 9th IAEA Technical Meeting on Control, Data Acquisition and Remote Participation for Fusion Research CY MAY 06-10, 2013 CL Hefei, PEOPLES R CHINA DE Fast cameras; NSTX; Blobs ID ALCATOR C-MOD; SPHERICAL TORUS EXPERIMENT; SCRAPE-OFF-LAYER; TURBULENCE AB Fast 2-D cameras examine a variety of important aspects of the plasma edge and in-vessel components on the National Spherical Torus Experiment (NSTX). Four Phantom and two Miro visible-light cameras manufactured by Vision Research are used on NSTX for edge studies. Each camera can take several gigabytes (GBs) of data during each plasma pulse. Timely access to this amount of data can itself be a challenge, but analysing all these data using manual frame-by-frame examination is not practical. This paper describes image analysis, database techniques, and visualization methods used to organize the fast camera data and to facilitate physics insights from it. An example is presented of analysing and characterizing the size, movement and dynamics of coherent plasma structures (typically referred to as "blobs") near the plasma edge. Software tools that generate statistics of blob speed, shape, amplitude, size, and orientation are described. The characteristics of emitted blobs affect plasma confinement and heat loads on plasma facing components, and are thus of particular interest to future machines like ITER. (C) 2014 Elsevier B.V. All rights reserved. C1 [Davis, W. M.; Maqueda, R. J.; Roquemore, A. L.; Scotti, F.; Zweben, S. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Ko, M. K.] Princeton HS, Princeton, NJ 08540 USA. [Maqueda, R. J.] Nova Photon, Princeton, NJ 08543 USA. RP Davis, WM (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM bdavis@pppl.gov; matthewko@verizon.net; rmaqueda@pppl.gov; lroquemo@pppl.gov; fscotti@pppl.gov; szweben@pppl.gov OI Davis, William/0000-0003-0666-7247 FU DOE [DE-AC02-09CH11466] FX Many thanks to the NSTX team for operating NSTX and for providing plasma shot data. Special thanks goes to Steve Sabbagh for EFIT analysis and Jon Menard for LRDfit analysis used for plotting plasma edge positions. Thanks to Bin Cao, for handling the Lithium Scan experiments. We would also like to thank Jim Myra for many insights on blob physics and suggestions on what to look for in our data analysis. This work was supported by DOE Contract DE-AC02-09CH11466. NR 18 TC 2 Z9 2 U1 0 U2 11 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0920-3796 EI 1873-7196 J9 FUSION ENG DES JI Fusion Eng. Des. PD MAY PY 2014 VL 89 IS 5 BP 717 EP 720 DI 10.1016/j.fusengdes.2013.11.014 PG 4 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AL4VT UT WOS:000339133600044 ER PT J AU Schissel, DP Abla, G Flanagan, SM Greenwald, M Lee, X Romosan, A Shoshani, A Stillerman, J Wright, J AF Schissel, D. P. Abla, G. Flanagan, S. M. Greenwald, M. Lee, X. Romosan, A. Shoshani, A. Stillerman, J. Wright, J. TI Automated metadata, provenance cataloging and navigable interfaces: Ensuring the usefulness of extreme-scale data SO FUSION ENGINEERING AND DESIGN LA English DT Article; Proceedings Paper CT 9th IAEA Technical Meeting on Control, Data Acquisition and Remote Participation for Fusion Research CY MAY 06-10, 2013 CL Hefei, PEOPLES R CHINA DE Metadata; Workflow; Data management; Data provenance AB For scientific research, it is not the mere existence of experimental or simulation data that is important, but the ability to make use of it. This paper presents the results of research to create a data model, infrastructure, and a set of tools that support data tracking, cataloging, and integration across a broad scientific domain. The system is intended to document workflow and data provenance in the widest sense. Combining research on integrated metadata, provenance, and ontology information with research on user interfaces has allowed the construction of early prototype. While using fusion science as a test bed, the system's framework and data model is quite general. (C) 2014 Elsevier B.V. All rights reserved. C1 [Schissel, D. P.; Abla, G.; Flanagan, S. M.; Lee, X.] Gen Atom, San Diego, CA 92186 USA. [Greenwald, M.; Stillerman, J.; Wright, J.] MIT, Cambridge, MA 02139 USA. [Romosan, A.; Shoshani, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Schissel, DP (reprint author), Gen Atom, POB 85608, San Diego, CA 92186 USA. EM schissel@fusion.gat.com OI Stillerman, Joshua/0000-0003-0901-0806; Greenwald, Martin/0000-0002-4438-729X FU US DOE, Office of Advanced Scientific Computing Research and; Office of Fusion Energy Sciences [DE-SC0008697, DE-AC02-05CH11231, DE-SC0008736] FX This work was supported by the US DOE, Office of Advanced Scientific Computing Research and the Office of Fusion Energy Sciences under DE-SC0008697, DE-AC02-05CH11231, and DE-SC0008736. NR 5 TC 4 Z9 4 U1 0 U2 0 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0920-3796 EI 1873-7196 J9 FUSION ENG DES JI Fusion Eng. Des. PD MAY PY 2014 VL 89 IS 5 BP 745 EP 749 DI 10.1016/j.fusengdes.2014.01.053 PG 5 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AL4VT UT WOS:000339133600050 ER PT J AU Wright, JC Greenwald, M Stillerman, J Abla, G Chanthavong, B Flanagan, S Schissel, D Lee, X Romosan, A Shoshani, A AF Wright, John C. Greenwald, Martin Stillerman, Joshua Abla, Gheni Chanthavong, Bobby Flanagan, Sean Schissel, David Lee, Xia Romosan, Alex Shoshani, Arie TI The MPO API: A tool for recording scientific workflows SO FUSION ENGINEERING AND DESIGN LA English DT Article; Proceedings Paper CT 9th IAEA Technical Meeting on Control, Data Acquisition and Remote Participation for Fusion Research CY MAY 06-10, 2013 CL Hefei, PEOPLES R CHINA DE Metadata; Bigdata; Provenance; Workflow; Database ID METADATA AB Data from large-scale experiments and extreme-scale computing is expensive to produce and may be used for high-consequence applications. The Metadata, Provenance and Ontology (MPO) project builds on previous work [M. Greenwald, Fusion Eng. Des. 87 (2012) 2205-2208] and is focused on providing documentation of workflows, data provenance and the ability to data-mine large sets of results. While there are important design and development aspects to the data structures and user interfaces, we concern ourselves in this paper with the application programming interface (API) - the set of functions that interface with the data server. Our approach for the data server is to follow the Representational State Transfer (RESTful) software architecture style for client server communication. At its core, the API uses the POST and GET methods of the HTTP protocol to transfer workflow information in message bodies to targets specified in the URL to and from the database via a web server. Higher level API calls are built upon this core API. This design facilitates implementation on different platforms and in different languages and is robust to changes in the underlying technologies used. The command line client implementation can communicate with the data server from any machine with HTTP access. Published by Elsevier B.V. C1 [Wright, John C.; Greenwald, Martin; Stillerman, Joshua] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Abla, Gheni; Chanthavong, Bobby; Flanagan, Sean; Schissel, David; Lee, Xia] Gen Atom Co, San Diego, CA USA. [Romosan, Alex; Shoshani, Arie] Lawrence Berkeley Lab, Berkeley, CA USA. RP Wright, JC (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM jcwright@mit.edu OI Stillerman, Joshua/0000-0003-0901-0806; Greenwald, Martin/0000-0002-4438-729X FU US DOE, Office of Advanced Scientific Computing Research; Office of Fusion Energy Sciences [DE-SC0008697, DE-AC02-05CH11231, DE-SC0008736] FX This work was supported by the US DOE, Office of Advanced Scientific Computing Research and the Office of Fusion Energy Sciences under DE-SC0008697, DE-AC02-05CH11231, and DE-SC0008736. NR 8 TC 2 Z9 2 U1 0 U2 16 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0920-3796 EI 1873-7196 J9 FUSION ENG DES JI Fusion Eng. Des. PD MAY PY 2014 VL 89 IS 5 BP 754 EP 757 DI 10.1016/j.fusengdes.2014.02.011 PG 4 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AL4VT UT WOS:000339133600052 ER PT J AU Kuehl, JV Price, MN Ray, J Wetmore, KM Esquivel, Z Kazakov, AE Nguyen, M Kuehn, R Davis, RW Hazen, TC Arkin, AP Deutschbauer, A AF Kuehl, Jennifer V. Price, Morgan N. Ray, Jayashree Wetmore, Kelly M. Esquivel, Zuelma Kazakov, Alexey E. Nguyen, Michelle Kuehn, Raquel Davis, Ronald W. Hazen, Terry C. Arkin, Adam P. Deutschbauer, Adam TI Functional Genomics with a Comprehensive Library of Transposon Mutants for the Sulfate-Reducing Bacterium Desulfovibrio alaskensis G20 SO MBIO LA English DT Article ID DESULFURICANS G20; VULGARIS HILDENBOROUGH; SYNTROPHIC GROWTH; ELECTRON-TRANSFER; GENETIC-ANALYSIS; HUMAN FECES; ENZYME; BIOSYNTHESIS; REDUCTION; IDENTIFICATION AB The genomes of sulfate-reducing bacteria remain poorly characterized, largely due to a paucity of experimental data and genetic tools. To meet this challenge, we generated an archived library of 15,477 mapped transposon insertion mutants in the sulfate-reducing bacterium Desulfovibrio alaskensis G20. To demonstrate the utility of the individual mutants, we profiled gene expression in mutants of six regulatory genes and used these data, together with 1,313 high-confidence transcription start sites identified by tiling microarrays and transcriptome sequencing (5' RNA-Seq), to update the regulons of Fur and Rex and to confirm the predicted regulons of LysX, PhnF, PerR, and Dde_3000, a histidine kinase. In addition to enabling single mutant investigations, the D. alaskensis G20 transposon mutants also contain DNA bar codes, which enables the pooling and analysis of mutant fitness for thousands of strains simultaneously. Using two pools of mutants that represent insertions in 2,369 unique protein-coding genes, we demonstrate that the hypothetical gene Dde_3007 is required for methionine biosynthesis. Using comparative genomics, we propose that Dde_3007 performs a missing step in methionine biosynthesis by transferring a sulfur group to O-phosphohomoserine to form homocysteine. Additionally, we show that the entire choline utilization cluster is important for fitness in choline sulfate medium, which confirms that a functional microcompartment is required for choline oxidation. Finally, we demonstrate that Dde_3291, a MerR-like transcription factor, is a choline-dependent activator of the choline utilization cluster. Taken together, our data set and genetic resources provide a foundation for systems-level investigation of a poorly studied group of bacteria of environmental and industrial importance. IMPORTANCE Sulfate-reducing bacteria contribute to global nutrient cycles and are a nuisance for the petroleum industry. Despite their environmental and industrial significance, the genomes of sulfate-reducing bacteria remain poorly characterized. Here, we describe a genetic approach to fill gaps in our knowledge of sulfate-reducing bacteria. We generated a large collection of archived, transposon mutants in Desulfovibrio alaskensis G20 and used the phenotypes of these mutant strains to infer the function of genes involved in gene regulation, methionine biosynthesis, and choline utilization. Our findings and mutant resources will enable systematic investigations into gene function, energy generation, stress response, and metabolism for this important group of bacteria. C1 [Kuehl, Jennifer V.; Price, Morgan N.; Ray, Jayashree; Wetmore, Kelly M.; Esquivel, Zuelma; Kazakov, Alexey E.; Arkin, Adam P.; Deutschbauer, Adam] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Nguyen, Michelle; Kuehn, Raquel; Davis, Ronald W.] Stanford Univ, Stanford Genome Technol Ctr, Palo Alto, CA 94304 USA. [Hazen, Terry C.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN USA. [Hazen, Terry C.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP Deutschbauer, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM AMDeutschbauer@lbl.gov RI Arkin, Adam/A-6751-2008; Ray, Jayashree/F-9162-2016; Hazen, Terry/C-1076-2012 OI Arkin, Adam/0000-0002-4999-2931; Hazen, Terry/0000-0002-2536-9993 FU Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work conducted by ENIGMA was supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 66 TC 10 Z9 10 U1 4 U2 17 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2014 VL 5 IS 3 AR e01041-14 DI 10.1128/mBio.01041-14 PG 13 WC Microbiology SC Microbiology GA AL1HH UT WOS:000338875900036 PM 24865553 ER PT J AU Ladner, JT Beitzel, B Chain, PSG Davenport, MG Donaldson, EF Frieman, M Kugelman, JR Kuhn, JH O'Rear, J Sabeti, PC Wentworth, DE Wiley, MR Yu, GY Sozhamannan, S Bradburne, C Palacios, G AF Ladner, Jason T. Beitzel, Brett Chain, Patrick S. G. Davenport, Matthew G. Donaldson, Eric F. Frieman, Matthew Kugelman, Jeffrey R. Kuhn, Jens H. O'Rear, Jules Sabeti, Pardis C. Wentworth, David E. Wiley, Michael R. Yu, Guo-Yun Sozhamannan, Shanmuga Bradburne, Christopher Palacios, Gustavo CA Threat Characterization Consortium TI Standards for Sequencing Viral Genomes in the Era of High-Throughput Sequencing SO MBIO LA English DT Editorial Material ID DISCOVERY; VIRUSES; CORONAVIRUS; POPULATION; DIVERSITY; CHINA AB Thanks to high-throughput sequencing technologies, genome sequencing has become a common component in nearly all aspects of viral research; thus, we are experiencing an explosion in both the number of available genome sequences and the number of institutions producing such data. However, there are currently no common standards used to convey the quality, and therefore utility, of these various genome sequences. Here, we propose five "standard" categories that encompass all stages of viral genome finishing, and we define them using simple criteria that are agnostic to the technology used for sequencing. We also provide genome finishing recommendations for various downstream applications, keeping in mind the cost-benefit trade-offs associated with different levels of finishing. Our goal is to define a common vocabulary that will allow comparison of genome quality across different research groups, sequencing platforms, and assembly techniques. C1 [Ladner, Jason T.; Beitzel, Brett; Kugelman, Jeffrey R.; Wiley, Michael R.; Yu, Guo-Yun; Palacios, Gustavo] US Army, Med Res Inst Infect Dis, Ctr Genome Sci, Ft Detrick, MD 21702 USA. [Chain, Patrick S. G.] Los Alamos Natl Lab, Bioinformat & Analyt Team, Biosci Div, Los Alamos, NM USA. [Davenport, Matthew G.; Bradburne, Christopher] Johns Hopkins Univ, Appl Phys Lab, Natl Secur Syst Biol Ctr, Asymmetr Operat Sect, Laurel, MD USA. [Donaldson, Eric F.; O'Rear, Jules] US FDA, Silver Spring, MD USA. [Frieman, Matthew] Univ Maryland, Dept Microbiol & Immunol, Baltimore, MD 21201 USA. [Kuhn, Jens H.] NIAID, Integrated Res Facil Ft Detrick, NIH, Frederick, MD USA. [Sabeti, Pardis C.] Harvard Univ, Dept Organism & Evolutionary Biol, FAS Ctr Syst Biol, Cambridge, MA 02138 USA. [Sabeti, Pardis C.] Broad Inst, Cambridge, MA USA. [Wentworth, David E.] J Craig Venter Inst, Rockville, MD USA. [Threat Characterization Consortium] Def Threat Reduct Agcy, Threat Characterizat Consortium, Ft Belvoir, VA USA. [Sozhamannan, Shanmuga] GoldBelt Raven LLC, Frederick, MD USA. [Sozhamannan, Shanmuga] Joint Program Execut Off, Crit Reagents Program, Ft Detrick, MD USA. RP Ladner, JT (reprint author), US Army, Med Res Inst Infect Dis, Ctr Genome Sci, Ft Detrick, MD 21702 USA. EM jason.t.ladner.ctr@mail.mil; gustavo.f.palacios.ctr@mail.mil RI Kuhn, Jens H./B-7615-2011; Palacios, Gustavo/I-7773-2015; OI Kuhn, Jens H./0000-0002-7800-6045; Palacios, Gustavo/0000-0001-5062-1938; Wentworth, David/0000-0002-5190-980X; Chain, Patrick/0000-0003-3949-3634 FU NIAID NIH HHS [HHSN272200700016I]; PHS HHS [HHSN272200700016I] NR 23 TC 20 Z9 20 U1 0 U2 5 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2014 VL 5 IS 3 AR e01360-14 DI 10.1128/mBio.01360-14 PG 5 WC Microbiology SC Microbiology GA AL1HH UT WOS:000338875900037 PM 24939889 ER PT J AU Lennon, CW Lemmer, KC Irons, JL Sellman, MI Donohue, TJ Gourse, RL Ross, W AF Lennon, Christopher W. Lemmer, Kimberly C. Irons, Jessica L. Sellman, Max I. Donohue, Timothy J. Gourse, Richard L. Ross, Wilma TI A Rhodobacter sphaeroides Protein Mechanistically Similar to Escherichia coli DksA Regulates Photosynthetic Growth SO MBIO LA English DT Article ID TRANSCRIPTION FACTOR DKSA; COILED-COIL TIP; RNA-POLYMERASE; STRINGENT RESPONSE; SECONDARY CHANNEL; DNA-REPLICATION; RHODOPSEUDOMONAS-SPHEROIDES; CAULOBACTER-CRESCENTUS; GENE-EXPRESSION; TRIGGER LOOP AB DksA is a global regulatory protein that, together with the alarmone ppGpp, is required for the "stringent response" to nutrient starvation in the gammaproteobacterium Escherichia coli and for more moderate shifts between growth conditions. DksA modulates the expression of hundreds of genes, directly or indirectly. Mutants lacking a DksA homolog exhibit pleiotropic phenotypes in other gammaproteobacteria as well. Here we analyzed the DksA homolog RSP2654 in the more distantly related Rhodobacter sphaeroides, an alphaproteobacterium. RSP2654 is 42% identical and similar in length to E. coli DksA but lacks the Zn finger motif of the E. coli DksA globular domain. Deletion of the RSP2654 gene results in defects in photosynthetic growth, impaired utilization of amino acids, and an increase in fatty acid content. RSP2654 complements the growth and regulatory defects of an E. coli strain lacking the dksA gene and modulates transcription in vitro with E. coli RNA polymerase (RNAP) similarly to E. coli DksA. RSP2654 reduces RNAP-promoter complex stability in vitro with RNAPs from E. coli or R. sphaeroides, alone and synergistically with ppGpp, suggesting that even though it has limited sequence identity to E. coli DksA (DksA(Ec)), it functions in a mechanistically similar manner. We therefore designate the RSP2654 protein DksA(Rsp). Our work suggests that DksARsp has distinct and important physiological roles in alphaproteobacteria and will be useful for understanding structure-function relationships in DksA and the mechanism of synergy between DksA and ppGpp. IMPORTANCE The role of DksA has been analyzed primarily in the gammaproteobacteria, in which it is best understood for its role in control of the synthesis of the translation apparatus and amino acid biosynthesis. Our work suggests that DksA plays distinct and important physiological roles in alphaproteobacteria, including the control of photosynthesis in Rhodobacter sphaeroides. The study of DksA(Rsp), should be useful for understanding structure-function relationships in the protein, including those that play a role in the little-understood synergy between DksA and ppGpp. C1 [Lennon, Christopher W.; Irons, Jessica L.; Donohue, Timothy J.; Gourse, Richard L.; Ross, Wilma] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Lemmer, Kimberly C.; Sellman, Max I.; Donohue, Timothy J.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Wisconsin Energy Inst, Madison, WI USA. RP Gourse, RL (reprint author), Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. EM rgourse@bact.wisc.edu OI Donohue, Timothy/0000-0001-8738-2467 FU Public Health Service grant from NIGMS [R37 GM37048]; DOE Great Lakes Bioenergy Research Center grant (DOE Office of Science BER) [DE-FC02-07ER64494]; USDA NIFA [2011-67012-30702]; NIH [T32 GM008349]; NSF FX This work was supported by Public Health Service grant R37 GM37048 to R.L.G. from NIGMS, by DOE Great Lakes Bioenergy Research Center grant (DOE Office of Science BER DE-FC02-07ER64494) to T.J.D., and by a USDA NIFA fellowship, 2011-67012-30702, to K. C. L. C. W. L. was supported in part by a biotechnology predoctoral fellowship from the NIH (T32 GM008349), and J.L.I. was supported by a summer stipend from the NSF (Research Experience for Undergraduates). NR 68 TC 3 Z9 3 U1 1 U2 5 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2014 VL 5 IS 3 AR e01105-14 DI 10.1128/mBio.01105-14 PG 14 WC Microbiology SC Microbiology GA AL1HH UT WOS:000338875900039 PM 24781745 ER PT J AU Menachery, VD Eisfeld, AJ Schafer, A Josset, L Sims, AC Proll, S Fan, SF Li, CJ Neumann, G Tilton, SC Chang, J Gralinski, LE Long, C Green, R Williams, CM Weiss, J Matzke, MM Webb-Robertson, BJ Schepmoes, AA Shukla, AK Metz, TO Smith, RD Waters, KM Katze, MG Kawaoka, Y Baric, RS AF Menachery, Vineet D. Eisfeld, Amie J. Schaefer, Alexandra Josset, Laurence Sims, Amy C. Proll, Sean Fan, Shufang Li, Chengjun Neumann, Gabriele Tilton, Susan C. Chang, Jean Gralinski, Lisa E. Long, Casey Green, Richard Williams, Christopher M. Weiss, Jeffrey Matzke, Melissa M. Webb-Robertson, Bobbie-Jo Schepmoes, Athena A. Shukla, Anil K. Metz, Thomas O. Smith, Richard D. Waters, Katrina M. Katze, Michael G. Kawaoka, Yoshihiro Baric, Ralph S. TI Pathogenic Influenza Viruses and Coronaviruses Utilize Similar and Contrasting Approaches To Control Interferon-Stimulated Gene Responses SO MBIO LA English DT Article ID RESPIRATORY SYNDROME CORONAVIRUS; INNATE IMMUNE-RESPONSES; LENGTH INFECTIOUS CDNA; A VIRUS; I INTERFERON; NS1 PROTEIN; VIRULENCE DETERMINANTS; HISTONE MODIFICATIONS; REVERSE GENETICS; MESSENGER-RNAS AB The broad range and diversity of interferon-stimulated genes (ISGs) function to induce an antiviral state within the host, impeding viral pathogenesis. While successful respiratory viruses overcome individual ISG effectors, analysis of the global ISG response and subsequent viral antagonism has yet to be examined. Employing models of the human airway, transcriptomics and proteomics datasets were used to compare ISG response patterns following highly pathogenic H5N1 avian influenza (HPAI) A virus, 2009 pandemic H1N1, severe acute respiratory syndrome coronavirus (SARS-CoV), and Middle East respiratory syndrome CoV (MERS-CoV) infection. The results illustrated distinct approaches utilized by each virus to antagonize the global ISG response. In addition, the data revealed that highly virulent HPAI virus and MERS-CoV induce repressive histone modifications, which downregulate expression of ISG subsets. Notably, influenza A virus NS1 appears to play a central role in this histone-mediated downregulation in highly pathogenic influenza strains. Together, the work demonstrates the existence of unique and common viral strategies for controlling the global ISG response and provides a novel avenue for viral antagonism via altered histone modifications. IMPORTANCE This work combines systems biology and experimental validation to identify and confirm strategies used by viruses to control the immune response. Using a novel screening approach, specific comparison between highly pathogenic influenza viruses and coronaviruses revealed similarities and differences in strategies to control the interferon and innate immune response. These findings were subsequently confirmed and explored, revealing both a common pathway of antagonism via type I interferon (IFN) delay as well as a novel avenue for control by altered histone modification. Together, the data highlight how comparative systems biology analysis can be combined with experimental validation to derive novel insights into viral pathogenesis. C1 [Menachery, Vineet D.; Schaefer, Alexandra; Sims, Amy C.; Gralinski, Lisa E.; Long, Casey; Baric, Ralph S.] Univ N Carolina, Dept Epidemiol, Chapel Hill, NC 27515 USA. [Baric, Ralph S.] Univ N Carolina, Dept Microbiol & Immunol, Chapel Hill, NC USA. [Eisfeld, Amie J.; Fan, Shufang; Li, Chengjun; Neumann, Gabriele; Kawaoka, Yoshihiro] Univ Wisconsin, Sch Vet Med, Dept Pathobiol Sci, Influenza Res Inst, Madison, WI 53706 USA. [Josset, Laurence; Proll, Sean; Chang, Jean; Green, Richard; Williams, Christopher M.; Weiss, Jeffrey; Katze, Michael G.] Univ Washington, Sch Med, Dept Microbiol, Seattle, WA 98195 USA. [Tilton, Susan C.; Matzke, Melissa M.; Webb-Robertson, Bobbie-Jo; Schepmoes, Athena A.; Shukla, Anil K.; Metz, Thomas O.; Smith, Richard D.; Waters, Katrina M.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Katze, Michael G.] Univ Washington, Washington Natl Primate Res Ctr, Seattle, WA 98195 USA. [Kawaoka, Yoshihiro] Univ Tokyo, Inst Med Sci, Div Virol, Dept Microbiol & Immunol, Tokyo, Japan. [Kawaoka, Yoshihiro] Univ Tokyo, Inst Med Sci, Int Res Ctr Infect Dis, Dept Special Pathogens, Tokyo, Japan. [Kawaoka, Yoshihiro] ERATO Infect Induced Host Responses Project, Saitama, Japan. RP Baric, RS (reprint author), Univ N Carolina, Dept Epidemiol, Chapel Hill, NC 27515 USA. EM Rbaric@email.unc.edu RI Smith, Richard/J-3664-2012; Josset, Laurence/A-7960-2015; OI Smith, Richard/0000-0002-2381-2349; Josset, Laurence/0000-0002-7158-1186; Metz, Tom/0000-0001-6049-3968 FU NIAID of the NIH [U19AI100625, U19AI106772, F32AI102561]; DOE Office of Biological and Environmental Research; National Institute of General Medical Sciences [8 P41 GM103493-10]; DOE [DE AC05 76RLO1830]; [HHSN272200800060C] FX Research was supported by grants from NIAID of the NIH (U19AI100625 to R. S. B., U19AI106772 to Y.K., and F32AI102561 to V. D. M.) and under contract no. HHSN272200800060C (to M.G.K.).; The proteomics was performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research and located at PNNL and used capabilities developed under efforts supported by the National Institute of General Medical Sciences (8 P41 GM103493-10). PNNL is operated by Battelle Memorial Institute for the DOE under contract number DE AC05 76RLO1830. NR 54 TC 22 Z9 22 U1 1 U2 4 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2014 VL 5 IS 3 AR e01174-14 DI 10.1128/mBio.01174-14 PG 11 WC Microbiology SC Microbiology GA AL1HH UT WOS:000338875900044 PM 24846384 ER PT J AU Tian, C Deng, ZD Lu, J Xu, XY Zhao, W Xu, M AF Tian, Chuan Deng, Zhiqun Daniel Lu, Jun Xu, Xiaoyang Zhao, Wei Xu, Ming TI Evaluation of a Low-Cost and Accurate Ocean Temperature Logger on Subsurface Mooring Systems SO MARINE TECHNOLOGY SOCIETY JOURNAL LA English DT Article DE internal waves; ocean mixing; subsurface mooring systems; temperature loggers ID THERMISTORS; CALIBRATION; INSTRUMENT; NOISE AB Monitoring seawater temperature is important to understanding evolving ocean processes. To monitor internal waves or ocean mixing, a large number of temperature loggers are typically mounted on subsurface mooring systems to obtain high-resolution temperature data at different water depths. In this study, we redesigned and evaluated a compact, low-cost, self-contained, high-resolution and high-accuracy ocean temperature logger, the TC-1121. The newly designed TC-1121 logger is smaller and more robust, and its sampling interval can be automatically changed by indicated events. The loggers initial accuracy is +/- 0.002 degrees C, and its effective resolution is about 0.0001 degrees C. The drift error of all six TC-1121 temperature loggers during a 450-day experiment was less than +/- 0.002 degrees C. They are being widely used in many mooring systems to study internal wave and ocean mixing. The loggers fundamental design, noise analysis, calibration, and drift test are discussed. A long-term sea trial in the South China Sea was completed successfully and demonstrated the effectiveness of the logger. C1 [Tian, Chuan] Chinese Acad Sci, Inst Oceanol, Beijing 100864, Peoples R China. [Deng, Zhiqun Daniel; Lu, Jun] Pacific NW Natl Lab, Richland, WA 99352 USA. [Xu, Xiaoyang; Zhao, Wei; Xu, Ming] Ocean Univ China, Qingdao, Peoples R China. RP Deng, ZD (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM zhiqun.deng@pnnl.gov RI Deng, Daniel/A-9536-2011 OI Deng, Daniel/0000-0002-8300-8766 FU National Natural Science Foundation of China [41006005]; National High Technology Research and Development (863) Program of China [2013AA09A501, 2013AA09A502] FX This study was funded by the National Natural Science Foundation of China (41006005) and the National High Technology Research and Development (863) Program of China (2013AA09A501, 2013AA09A502). NR 28 TC 3 Z9 3 U1 2 U2 10 PU MARINE TECHNOLOGY SOC INC PI COLUMBIA PA 5565 STERRETT PLACE, STE 108, COLUMBIA, MD 21044 USA SN 0025-3324 EI 1948-1209 J9 MAR TECHNOL SOC J JI Mar. Technol. Soc. J. PD MAY-JUN PY 2014 VL 48 IS 3 BP 146 EP 154 PG 9 WC Engineering, Ocean; Oceanography SC Engineering; Oceanography GA AK9NR UT WOS:000338754300014 ER PT J AU Bushnell, PJ Tatum-Gibbs, R Mckee, JM Evansky, PA Higuchi, M MLin, MT Oshiro, WM Judson, R Hester, S Reif, D Morozova, T Mackay, TFC Boyes, WK AF Bushnell, P. J. Tatum-Gibbs, R. McKee, J. M. Evansky, P. A. Higuchi, M. MLin, M. T. Oshiro, W. M. Judson, R. Hester, S. Reif, D. Morozova, T. Mackay, T. F. C. Boyes, W. K. TI ToxiFly: Can fruit flies be used to identify toxicity pathways for airborne chemicals? SO NEUROTOXICOLOGY AND TERATOLOGY LA English DT Meeting Abstract CT 38th Annual Meeting of the Neurobehavioral-Teratology-Society CY JUN 28-JUL 02, 2014 CL Bellevue, WA SP Neurobehavioral Teratol Soc C1 [Bushnell, P. J.; McKee, J. M.; Evansky, P. A.; Higuchi, M.; Oshiro, W. M.; Boyes, W. K.] US EPA, Natl Hlth & Environm Effects Res Lab, Res Triangle Pk, NC USA. [Tatum-Gibbs, R.; MLin, M. T.; Hester, S.] Oak Ridge Inst Sci Educ, Oak Ridge, TN USA. [Judson, R.] US EPA, Natl Ctr Computat Toxicol, Res Triangle Pk, NC USA. [Reif, D.] N Carolina State Univ, Bioinformat Res Ctr, Raleigh, NC 27695 USA. [Morozova, T.; Mackay, T. F. C.] N Carolina State Univ, Dept Biol Sci, Raleigh, NC 27695 USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0892-0362 EI 1872-9738 J9 NEUROTOXICOL TERATOL JI Neurotoxicol. Teratol. PD MAY-JUN PY 2014 VL 43 MA NBTS 42 BP 89 EP 89 DI 10.1016/j.ntt.2014.04.045 PG 1 WC Neurosciences; Toxicology SC Neurosciences & Neurology; Toxicology GA AK7QC UT WOS:000338621800052 ER PT J AU Lopez-Plaza, EL Hernandez, S Barroso-Munoz, FO Segovia-Hernandez, JG Aceves, SM Martinez-Frias, J Saxena, S Dibble, R AF Luis Lopez-Plaza, Emilio Hernandez, Salvador Omar Barroso-Munoz, Fabricio Gabriel Segovia-Hernandez, Juan Aceves, Salvador M. Martinez-Frias, Joel Saxena, Samveg Dibble, Robert TI Experimental and Theoretical Study of the Energy Savings from Wet Ethanol Production and Utilization SO ENERGY TECHNOLOGY LA English DT Article DE biofuels; ethanol; distillation; moisture; engines ID EXTRACTIVE DISTILLATION; COLUMNS; SYSTEMS; FUEL AB As a result of the energy crisis in recent decades, biofuels have gained importance as an option to diminish the oil dependence of automotive industry. Ethanol is one of these biofuels for which demand around the world has increased in recent years. However, to be used as a fuel, the ethanol must be dehydrated to avoid problems in actual engines, and this step has a high energy cost. To overcome this drawback, some studies have demonstrated the use of wet ethanol in homogeneous charge compression ignition (HCCI) engines. In this work, the production of wet ethanol, using conventional distillation, was studied using rigorous simulation studies and experimental tests in a distillation column. The simulation analysis and experimental validation of the energy requirements to obtain wet ethanol were achieved. The results showed that wet ethanol can be produced by using a distillation column with a small number of stages and low reflux ratios, which results in energy savings. Also, the results indicated that for low purities of the distilled ethanol (wet ethanol), the ratios between the energy required during the distillation process and the energy produced by ethanol during the combustion were low. This result implies that the use of wet ethanol can be considered as realistic option in HCCI engines. C1 [Luis Lopez-Plaza, Emilio; Hernandez, Salvador; Omar Barroso-Munoz, Fabricio; Gabriel Segovia-Hernandez, Juan] Univ Guanajuato, DCNyE, Dept Ingn Quim, Guanajuato 36050, Gto, Mexico. [Aceves, Salvador M.; Martinez-Frias, Joel] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Saxena, Samveg; Dibble, Robert] Univ Calif Berkeley, Berkeley, CA 94704 USA. RP Hernandez, S (reprint author), Univ Guanajuato, DCNyE, Dept Ingn Quim, Campus Guanajuato,Noria Alta S-N, Guanajuato 36050, Gto, Mexico. EM hernasa@ugto.mx RI Barroso-Munoz, Fabricio Omar/I-9176-2016 FU SAGAR-PA-CONACYT; PROMEP (Mexico) FX We acknowledge the financial support provided by SAGAR-PA-CONACYT and PROMEP (Mexico). NR 19 TC 3 Z9 3 U1 1 U2 5 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 2194-4288 EI 2194-4296 J9 ENERGY TECHNOL-GER JI Energy Technol. PD MAY PY 2014 VL 2 IS 5 BP 440 EP 445 DI 10.1002/ente.201300180 PG 6 WC Energy & Fuels SC Energy & Fuels GA AK3VL UT WOS:000338353000003 ER PT J AU Um, ES Commer, M Newman, GA AF Um, Evan Schankee Commer, Michael Newman, Gregory A. TI A strategy for coupled 3D imaging of large-scale seismic and electromagnetic data sets: Application to subsalt imaging SO GEOPHYSICS LA English DT Article ID WAVE-FORM INVERSION; ABSORBING BOUNDARY-CONDITIONS; NEAR-SURFACE MATERIALS; JOINT INVERSION; LAPLACE-DOMAIN; STRUCTURAL CONSTRAINTS; DC RESISTIVITY; CSEM DATA; EXPLORATION; GRADIENT AB Offshore seismic and electromagnetic (EM) imaging for hydrocarbons can require up to tens of millions of parameters to describe the 3D distribution of complex seabed geology and relevant geophysical attributes. The imaging and data volumes for such problems are enormous. Descent-based methods are the only viable imaging approach, where it is often challenging to manage the convergence of stand-alone seismic and EM inversion experiments. When a joint seismic-EM inversion is implemented, convergence problems with descent-based methods are further aggravated. Moreover, resolution mismatches between seismic and EM pose another challenge for joint inversion. To overcome these problems, we evaluated a coupled seismic-EM inversion workflow and applied it to a set of full-wave-seismic, magnetotelluric (MT) and controlled-source electromagnetic (CSEM) data for subsalt imaging. In our workflow, we address disparate resolution properties between seismic and EM data by implementing the seismic inversion in the Laplace domain, where the wave equation is transformed into a diffusion equation. The resolution of seismic data thus becomes comparable to that of EM data. To mitigate the convergence problems, the full joint seismic-EM inverse problem is split into manageable components: separate seismic and EM inversions and an intermediate step that enforces structural coupling through a cross-gradient-only inversion and resistivity-velocity crossplots. In this workflow, stand-alone seismic and MT inversion are performed first. The cross-gradient-only inversion and the crossplots are used to precondition the resistivity and velocity models for subsequent stand-alone inversions. By repeating the sequence of the stand-alone seismic, MT, and cross-gradient-only inversions along with the crossplots, we introduce the seismic structural information into the resistivity model, and vice versa, significantly improving the salt geometry in both resistivity and velocity images. We conclude that the improved salt geometry can then be used to precondition a starting model for CSEM inversions, yielding significant improvement in the resistivity images of hydrocarbon reservoirs adjacent to the salt. C1 [Um, Evan Schankee; Commer, Michael; Newman, Gregory A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Um, ES (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM evanum@gmail.com; mcommer@lbl.gov; ganewman@lbl.gov RI Newman, Gregory/G-2813-2015; Commer, Michael/G-3350-2015; Um, Evan/E-9414-2015 OI Commer, Michael/0000-0003-0015-9217; FU U.S. Department of Energy Office of Science [DE-AC02-05CH11231] FX This work was carried out at Lawrence Berkeley Laboratory (LBL) with funding and computing access to the NERSC supercomputing center provided by the U.S. Department of Energy Office of Science, contract number DE-AC02-05CH11231. We thank associate editors M. Sacchi (University of Alberta) and A. Abubakar (Schlumberger) and reviewer N. Linde (University of Lausanne), M. Meju (Petronas), and the two anonymous reviewers for constructive comments that helped us to improve the paper. NR 55 TC 5 Z9 6 U1 4 U2 21 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 EI 1942-2156 J9 GEOPHYSICS JI Geophysics PD MAY-JUN PY 2014 VL 79 IS 3 BP ID1 EP ID13 DI 10.1190/GEO2013-0053.1 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AK3KP UT WOS:000338322900019 ER PT J AU Calyam, P Dovrolis, C Jorgenson, L Kettimuthu, R Tierney, B Zurawski, J AF Calyam, Prasad Dovrolis, Constantine Joergenson, Loki Kettimuthu, Raj Tierney, Brian Zurawski, Jason TI MONITORING AND TROUBLESHOOTING MULTI-DOMAIN NETWORKS USING MEASUREMENT FEDERATIONS: PART 2 SO IEEE COMMUNICATIONS MAGAZINE LA English DT Editorial Material C1 [Calyam, Prasad] Univ Missouri Columbia, Dept Comp Sci, Columbia, MO 65211 USA. [Dovrolis, Constantine] Georgia Inst Technol, Coll Comp, Atlanta, GA 30332 USA. [Joergenson, Loki] Lionsgate Technol, Vancouver, BC, Canada. [Kettimuthu, Raj] Univ Chicago, Computat Inst, Math & Comp Sci Div, Div Argonne Natl Lab, Chicago, IL 60637 USA. [Tierney, Brian] Lawrence Berkeley Natl Lab, ESnet Adv Network Technol Grp, Berkeley, CA USA. [Zurawski, Jason] LBNL, Comp Sci Directorate, Sci Networking Div, Energy Sci Network, Berkeley, CA USA. RP Calyam, P (reprint author), Univ Missouri Columbia, Dept Comp Sci, Columbia, MO 65211 USA. EM calyamp@missouri.edu; dovrolis@cc.gatech.edu; ljorgenson@ACM.org; kettimut@mcs.anl.gov; bltierney@es.net; zurawski@es.net NR 0 TC 0 Z9 0 U1 0 U2 1 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0163-6804 EI 1558-1896 J9 IEEE COMMUN MAG JI IEEE Commun. Mag. PD MAY PY 2014 VL 52 IS 5 BP 145 EP 146 PG 2 WC Engineering, Electrical & Electronic; Telecommunications SC Engineering; Telecommunications GA AJ9LM UT WOS:000338032200018 ER PT J AU Neumann, PG Peisert, S Schaefer, M AF Neumann, Peter G. Peisert, Sean Schaefer, Marvin TI The IEEE Symposium on Security and Privacy, in Retrospect SO IEEE SECURITY & PRIVACY LA English DT Editorial Material C1 [Neumann, Peter G.] SRI Int, Comp Sci Lab, Menlo Pk, CA 94025 USA. [Peisert, Sean] Lawrence Berkeley Natl Lab, Davis, CA USA. [Peisert, Sean] Univ Calif Davis, Davis, CA 95616 USA. RP Neumann, PG (reprint author), SRI Int, Comp Sci Lab, Menlo Pk, CA 94025 USA. EM Neumann@csl.sri.com; peisert@cs.ucdavis.edu; bwapast@verizon.net NR 1 TC 0 Z9 0 U1 3 U2 3 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1540-7993 EI 1558-4046 J9 IEEE SECUR PRIV JI IEEE Secur. Priv. PD MAY-JUN PY 2014 VL 12 IS 3 BP 15 EP 17 PG 3 WC Computer Science, Information Systems; Computer Science, Software Engineering SC Computer Science GA AK1RC UT WOS:000338192200003 ER PT J AU Bonebrake, C O'Neil, LR AF Bonebrake, Chris O'Neil, Lori Ross TI Attacks on GPS Time Reliability SO IEEE SECURITY & PRIVACY LA English DT Article C1 [Bonebrake, Chris; O'Neil, Lori Ross] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Bonebrake, C (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM bonebrake@pnnl.gov; lro@pnnl.gov NR 6 TC 6 Z9 6 U1 0 U2 4 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1540-7993 EI 1558-4046 J9 IEEE SECUR PRIV JI IEEE Secur. Priv. PD MAY-JUN PY 2014 VL 12 IS 3 BP 82 EP 84 PG 3 WC Computer Science, Information Systems; Computer Science, Software Engineering SC Computer Science GA AK1RC UT WOS:000338192200015 ER PT J AU Thompson, GL Roth, CC Dalzell, DR Kuipers, M Ibey, BL AF Thompson, Gary Lee Roth, Caleb C. Dalzell, Danielle R. Kuipers, Marjorie Ibey, Bennett L. TI Calcium influx affects intracellular transport and membrane repair following nanosecond pulsed electric field exposure SO JOURNAL OF BIOMEDICAL OPTICS LA English DT Article DE nanosecond pulsed electric fields; lysosomal exocytosis; cytoskeleton; FM1-43; nanopores ID MAMMALIAN-CELLS; LYSOSOMES; MICROTUBULES; EXOCYTOSIS; ULTRASHORT; ELECTROPORATION; TRANSLOCATION; CYTOSKELETON; FIBROBLASTS; INTEGRITY AB The cellular response to subtle membrane damage following exposure to nanosecond pulsed electric fields (nsPEF) is not well understood. Recent work has shown that when cells are exposed to nsPEF, ion permeable nanopores (<2 nm) are created in the plasma membrane in contrast to larger diameter pores (> 2 nm) created by longer micro- and millisecond duration pulses. Nanoporation of the plasma membrane by nsPEF has been shown to cause a transient increase in intracellular calcium concentration within milliseconds after exposure. Our research objective is to determine the impact of nsPEF on calcium-dependent structural and repair systems in mammalian cells. Chinese hamster ovary (CHO-K1) cells were exposed in the presence and absence of calcium ions in the outside buffer to either 1 or 20, 600-ns duration electrical pulses at 16.2 kV/cm, and pore size was determined using propidium iodide and calcium green. Membrane organization was observed with morphological changes and increases in FM1-43 fluorescence. Migration of lysosomes, implicated in membrane repair, was followed using confocal microscopy of red fluorescent protein-tagged LAMP1. Microtubule structure was imaged using mEmerald-tubulin. We found that at high 600-ns PEF dosage, calcium-induced membrane restructuring and microtubule depolymerization coincide with interruption of membrane repair via lysosomal exocytosis. (C) 2014 Society of Photo-Optical Instrumentation Engineers (SPIE) C1 [Thompson, Gary Lee] JBSA Ft Sam Houston, Oak Ridge Inst Sci & Educ, Ft Sam Houston, TX 78234 USA. [Roth, Caleb C.] Univ Texas Hlth Sci Ctr San Antonio, Dept Radiol Sci, San Antonio, TX 78229 USA. [Dalzell, Danielle R.; Kuipers, Marjorie; Ibey, Bennett L.] JBSA Ft Sam Houston, Ft Sam Houston, TX 78234 USA. RP Thompson, GL (reprint author), JBSA Ft Sam Houston, Oak Ridge Inst Sci & Educ, Ft Sam Houston, TX 78234 USA. EM gary.l.thompson205.ctr@mail.mil FU Air Force Office of Scientific Research [AFOSR-LRIR 13RH08COR] FX The authors would like to thank Dr. Xiao Shu from Old Dominion University for constructing the custom, variable pulse width, and high voltage pulsing system. We wish to thank the Oak Ridge Institute for Science & Education Postdoctoral Research Associateship program and the Air Force Research Laboratory for providing us with the opportunity to conduct this study. This study was supported by a grant from the Air Force Office of Scientific Research (Grant No. AFOSR-LRIR 13RH08COR). NR 78 TC 10 Z9 10 U1 1 U2 13 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1083-3668 EI 1560-2281 J9 J BIOMED OPT JI J. Biomed. Opt. PD MAY PY 2014 VL 19 IS 5 AR 055005 DI 10.1117/1.JBO.19.5.055005 PG 12 WC Biochemical Research Methods; Optics; Radiology, Nuclear Medicine & Medical Imaging SC Biochemistry & Molecular Biology; Optics; Radiology, Nuclear Medicine & Medical Imaging GA AK3OR UT WOS:000338334600017 PM 24825506 ER PT J AU Ivanshin, VA Litvinova, TO Ivanshin, NA Poppl, A Sokolov, DA Aronson, MC AF Ivanshin, V. A. Litvinova, T. O. Ivanshin, N. A. Poeppl, A. Sokolov, D. A. Aronson, M. C. TI Evolution of the 4f electron localization from YbRh2Si2 to YbRh2Pb studied by electron spin resonance SO JOURNAL OF EXPERIMENTAL AND THEORETICAL PHYSICS LA English DT Article ID HEAVY-FERMION COMPOUNDS; COMPOUND AB We report on electron spin resonance (ESR) experiments on the Heusler alloy YbRh2Pb and compare its spin dynamics with that of several other Yb-based intermetallics. A detailed analysis of the derived ESR parameters indicates the extremely weak hybridization, more localized distribution of the 4f states, and a smaller RKKY interaction in YbRh2Pb. These findings reveal the important interplay between hybridization effects, chemical substitution, and crystalline electric field interactions that determines the ground state properties of strongly correlated electron systems. C1 [Ivanshin, V. A.; Litvinova, T. O.] Kazan Fed Volga Reg Univ, MRS Lab, Kazan 420008, Russia. [Ivanshin, N. A.] Kazan State Univ Architecture & Engn, Kazan 420043, Russia. [Ivanshin, V. A.; Poeppl, A.] Univ Leipzig, Fac Phys & Earth Sci, D-04103 Leipzig, Germany. [Sokolov, D. A.] Univ Edinburgh, Sch Phys, Edinburgh EH 3JZ, Midlothian, Scotland. [Sokolov, D. A.] Univ Edinburgh, CSEC, Edinburgh EH 3JZ, Midlothian, Scotland. [Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Aronson, M. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Dept, Upton, NY 11973 USA. RP Ivanshin, VA (reprint author), Kazan Fed Volga Reg Univ, MRS Lab, Kazan 420008, Russia. EM Vladimir.Ivanshin@kpfu.ru RI Sokolov, D/G-7755-2011 FU US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH1886] FX The authors are grateful to J. Hoentsch for his assistance during the Q-band ESR measurements. One of the autors (V. A. I.) thanks the University of Leipzig for hospitality. Work at Brookhaven National Laboratory was carried out under the auspices of the US Department of Energy, Office of Basic Energy Sciences under Contract no. DE-AC02-98CH1886. NR 31 TC 1 Z9 1 U1 1 U2 12 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 1063-7761 EI 1090-6509 J9 J EXP THEOR PHYS+ JI J. Exp. Theor. Phys. PD MAY PY 2014 VL 118 IS 5 BP 760 EP 764 DI 10.1134/S1063776114050033 PG 5 WC Physics, Multidisciplinary SC Physics GA AK3QW UT WOS:000338340800009 ER PT J AU Fei, Q Guarnieri, MT Tao, L Laurens, LML Dowe, N Pienkos, PT AF Fei, Qiang Guarnieri, Michael T. Tao, Ling Laurens, Lieve M. L. Dowe, Nancy Pienkos, Philip T. TI Bioconversion of natural gas to liquid fuel: Opportunities and challenges SO BIOTECHNOLOGY ADVANCES LA English DT Review DE Bioconversion of natural gas into liquid fuels (Bio-GTL); Greenhouse gas; Renewable diesel fuel; Methanotrophic bacteria; Microbial lipids; Bioprocess optimization; Lipid extraction; Hydrotreating process; Techno-economic analysis ID METHYLOSINUS-TRICHOSPORIUM OB3B; SOLUBLE METHANE MONOOXYGENASE; METHYLOCOCCUS-CAPSULATUS BATH; METHYLOMICROBIUM-ALCALIPHILUM 20Z; POLY-BETA-HYDROXYBUTYRATE; INTRA-CYTOPLASMIC MEMBRANES; BRANCHED-CHAIN ALCOHOLS; GRAM-NEGATIVE BACTERIA; HIGH-MOLECULAR-WEIGHT; STIRRED-TANK REACTOR AB Natural gas is a mixture of low molecular weight hydrocarbon gases that can be generated from either fossil or anthropogenic resources. Although natural gas is used as a transportation fuel, constraints in storage, relatively low energy content (MJ/L), and delivery have limited widespread adoption. Advanced utilization of natural gas has been explored for biofuel production by microorganisms. In recent years, the aerobic bioconversion of natural gas (or primarily the methane content of natural gas) into liquid fuels (Bio-GTL) by biocatalysts (methanotrophs) has gained increasing attention as a promising alternative for drop-in biofuel production. Methanotrophic bacteria are capable of converting methane into microbial lipids, which can in turn be converted into renewable diesel via a hydrotreating process. In this paper, biodiversity, catalytic properties and key enzymes and pathways of these microbes are summarized. Bioprocess technologies are discussed based upon existing literature, including cultivation conditions, fermentation modes, bioreactor design, and lipid extraction and upgrading. This review also outlines the potential of Bio-GTL using methane as an alternative carbon source as well as the major challenges and future research needs of microbial lipid accumulation derived from methane, key performance index, and techno-economic analysis. An analysis of raw material costs suggests that methane-derived diesel fuel has the potential to be competitive with petroleum-derived diesel. (C) 2014 The Authors. Published by Elsevier Inc. C1 [Fei, Qiang; Guarnieri, Michael T.; Tao, Ling; Laurens, Lieve M. L.; Dowe, Nancy; Pienkos, Philip T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Pienkos, PT (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Philip.Pienkos@nrel.gov RI Fei, Qiang/M-8710-2014 FU Advanced Research Projects Agency - Energy (ARPA-E) [0670-5169]; U.S. Department of Energy (DOE) FX This work was supported by a funding (project number: 0670-5169) from Advanced Research Projects Agency - Energy (ARPA-E) and U.S. Department of Energy (DOE). NR 283 TC 43 Z9 43 U1 13 U2 112 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0734-9750 EI 1873-1899 J9 BIOTECHNOL ADV JI Biotechnol. Adv. PD MAY-JUN PY 2014 VL 32 IS 3 BP 596 EP 614 DI 10.1016/j.biotechadv.2014.03.011 PG 19 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AJ7CS UT WOS:000337855400005 PM 24726715 ER PT J AU Levin, T Thomas, VM AF Levin, Todd Thomas, Valerie M. TI Utility-maximizing financial contracts for distributed rural electrification SO ENERGY LA English DT Article DE Rural electrification; Distributed energy systems; Electricity subsidies; Energy micro-finance; Financial delivery mechanisms; International energy development ID DEVELOPING-COUNTRIES; CREDIT MARKETS; TECHNOLOGIES; ELECTRICITY; SYSTEMS; AFRICA; POLICY; AREAS; MODEL AB We develop a cost-benefit framework for extending electricity access in currently un-electrified regions. We first show that distributed technologies may be the lowest-cost electrification option in areas where electricity consumption is low and grid connection costs are high. We also show that some centralized electrification programs provide services with subsidized rates far below cost recovery. An economic model is developed to compare three financial mechanisms that can be used to make capital intensive, distributed electrification technologies more accessible to rural populations; direct subsidies, rental programs and microloans. These contracts are compared on their ability to increase consumer utility for a given cost to the providing agency. We show that a direct technology subsidy is generally preferred when the desired subsidization is high and that, under certain parameter combinations, microloan and rental programs can improve energy access for the poor while also making a profit for the providing agency. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Levin, Todd; Thomas, Valerie M.] Georgia Inst Technol, Sch Ind & Syst Engn, Atlanta, GA 30332 USA. [Thomas, Valerie M.] Georgia Inst Technol, Sch Publ Policy, Atlanta, GA 30332 USA. RP Levin, T (reprint author), Argonne Natl Lab, Decis & Informat Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM tlevin@anl.gov; valerie.thomas@isye.gatech.edu OI Thomas, Valerie/0000-0002-0968-8863 FU National Science Foundation FX Todd Levin is supported by a Graduate Research Fellowship from the National Science Foundation. We wish to thank Wisdom Ahiataku-Togobo, Gifty Tettey and Dennis Turkson of the Ghana Ministry of Energy for their assistance and cooperation. NR 44 TC 5 Z9 5 U1 4 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-5442 EI 1873-6785 J9 ENERGY JI Energy PD MAY 1 PY 2014 VL 69 SI SI BP 613 EP 621 DI 10.1016/j.energy.2014.03.057 PG 9 WC Thermodynamics; Energy & Fuels SC Thermodynamics; Energy & Fuels GA AJ7CZ UT WOS:000337856100058 ER PT J AU Larsen, MV Cosentino, S Lukjancenko, O Saputra, D Rasmussen, S Hasman, H Sicheritz-Ponten, T Aarestrup, FM Ussery, DW Lund, O AF Larsen, Mette V. Cosentino, Salvatore Lukjancenko, Oksana Saputra, Dhany Rasmussen, Simon Hasman, Henrik Sicheritz-Ponten, Thomas Aarestrup, Frank M. Ussery, David W. Lund, Ole TI Benchmarking of Methods for Genomic Taxonomy SO JOURNAL OF CLINICAL MICROBIOLOGY LA English DT Article ID SEQUENCING-BASED METHODS; BACILLUS-CEREUS GROUP; IN-SILICO ANALYSIS; ESCHERICHIA-COLI; PROTEIN FAMILIES; BACTERIA; IDENTIFICATION; DATABASE; TREE; ARB AB One of the first issues that emerges when a prokaryotic organism of interest is encountered is the question of what it is-that is, which species it is. The 16S rRNA gene formed the basis of the first method for sequence-based taxonomy and has had a tremendous impact on the field of microbiology. Nevertheless, the method has been found to have a number of shortcomings. In the current study, we trained and benchmarked five methods for whole-genome sequence-based prokaryotic species identification on a common data set of complete genomes: (i) SpeciesFinder, which is based on the complete 16S rRNA gene; (ii) Reads2Type that searches for species-specific 50-mers in either the 16S rRNA gene or the gyrB gene (for the Enterobacteraceae family); (iii) the ribosomal multilocus sequence typing (rMLST) method that samples up to 53 ribosomal genes; (iv) TaxonomyFinder, which is based on species-specific functional protein domain profiles; and finally (v) KmerFinder, which examines the number of cooc-curring k-mers (substrings of k nucleotides in DNA sequence data). The performances of the methods were subsequently evaluated on three data sets of short sequence reads or draft genomes from public databases. In total, the evaluation sets constituted sequence data from more than 11,000 isolates covering 159 genera and 243 species. Our results indicate that methods that sample only chromosomal, core genes have difficulties in distinguishing closely related species which only recently diverged. The KmerFinder method had the overall highest accuracy and correctly identified from 93% to 97% of the isolates in the evaluations sets. C1 [Larsen, Mette V.; Cosentino, Salvatore; Lukjancenko, Oksana; Saputra, Dhany; Rasmussen, Simon; Sicheritz-Ponten, Thomas; Ussery, David W.; Lund, Ole] Tech Univ Denmark, Ctr Biol Sequence Anal, Dept Syst Biol, DK-2800 Lyngby, Denmark. [Hasman, Henrik; Aarestrup, Frank M.] Tech Univ Denmark, Natl Food Inst, DK-2800 Lyngby, Denmark. [Ussery, David W.] Oak Ridge Natl Lab, Biosci Div, Comparat Genom Grp, Oak Ridge, TN USA. RP Larsen, MV (reprint author), Tech Univ Denmark, Ctr Biol Sequence Anal, Dept Syst Biol, DK-2800 Lyngby, Denmark. EM metteb@cbs.dtu.dk RI Lund, Ole/F-4437-2014; Rasmussen, Simon/G-6258-2016; OI Lund, Ole/0000-0003-1108-0491; Rasmussen, Simon/0000-0001-6323-9041; Ussery, David/0000-0003-3632-5512 FU Center for Genomic Epidemiology at the Technical University of Denmark - Danish Council for Strategic Research [09-067103/DSF] FX This work was supported by the Center for Genomic Epidemiology at the Technical University of Denmark and funded by grant 09-067103/DSF from the Danish Council for Strategic Research. NR 51 TC 20 Z9 20 U1 0 U2 20 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0095-1137 EI 1098-660X J9 J CLIN MICROBIOL JI J. Clin. Microbiol. PD MAY PY 2014 VL 52 IS 5 BP 1529 EP 1539 DI 10.1128/JCM.02981-13 PG 11 WC Microbiology SC Microbiology GA AJ7XV UT WOS:000337915700033 PM 24574292 ER PT J AU Raybourn, EM AF Raybourn, Elaine M. TI A new paradigm for serious games: Transmedia learning for more effective training and education SO JOURNAL OF COMPUTATIONAL SCIENCE LA English DT Article DE Transmedia learning; Serious games; Transmedia campaigns; Storytelling; Social media; Data mining; xAPI; MOOC AB Serious games present a relatively new approach to training and education for international organizations such as NATO (North Atlantic Treaty Organization), non-governmental organizations (NGOs), the U.S. Department of Defense (DOD) and the U.S. Department of Homeland Security (DHS). Although serious games are often deployed as stand-alone solutions, they can also serve as entry points into a comprehensive training pipeline in which content is delivered via different media to rapidly scale immersive training and education for mass audiences. The present paper introduces a new paradigm for more effective and scalable training and education called transmedia learning. Transmedia learning leverages several new media trends including the peer communications of social media, the scalability of massively openonline course (MOOCs), and the design of transmedia storytelling used by entertainment, advertising, and commercial game industries to sustain audience engagement. Transmedia learning is defined as the scalable system of messages representing a narrative or core experience that unfolds from the use of multiple media, emotionally engaging learners by involving them personally in the story. In the present paper, we introduce the transmedia learning paradigm as offering more effective use of serious games for training and education. This approach is consistent with the goals of international organizations implementing approaches similar to those described by the Army Learning Model (ALM) to deliver training and education to Soldiers across multiple media. We discuss why the human brain is wired for transmedia learning and demonstrate how the Simulation Experience Design Method can be used to create transmedia learning story worlds for serious games. We describe how social media interactions and MOOCs may be used in transmedia learning, and how data mining social media and experience tracking can inform the development of computational learner models for transmedia learning campaigns. Examples of how the U.S. Army has utilized transmedia campaigns for strategic communication and game-based training are provided. Finally, we provide strategies the reader can use today to incorporate transmedia storytelling elements such as Internet, serious games, video, social media, graphic novels, machinima, blogs, and alternate reality gaming into a new paradigm for training and education: transmedia learning. (c) 2013 Elsevier B.V. All rights reserved. C1 Sandia Natl Labs, Livermore, CA 94550 USA. RP Raybourn, EM (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM emraybo@sandia.gov NR 42 TC 7 Z9 7 U1 8 U2 91 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1877-7503 J9 J COMPUT SCI-NETH JI J. Comput. Sci. PD MAY PY 2014 VL 5 IS 3 BP 471 EP 481 DI 10.1016/j.jocs.2013.08.005 PG 11 WC Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA AJ7JT UT WOS:000337873700019 ER PT J AU Colman, SM Hemming, SR Stine, S Zimmerman, SRH AF Colman, S. M. Hemming, S. R. Stine, S. Zimmerman, S. R. H. TI The effects of recent uplift and volcanism on deposition in Mono Lake, California, from seismic-reflection (CHIRP) profiles SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article ID SEDIMENTATION; DROUGHT; CLIMATE; TAHOE; BASIN AB About 150 km of high-resolution, seismic reflection (Compressed High-Intensity Radar Pulse) profiles (approximately 20 m penetration) were collected in Mono Lake in order to define the uppermost sedimentary architecture of the basin, which has been heavily impacted by recent volcanic, tectonic, and climatic processes. The study also provides an important background for ongoing efforts to obtain paleoenvironmental records from sediment cores in the lake. The history of four seismic-stratigraphic units in the upper 20 m of section are inferred from the data, and the interpretations are generally consistent with previous interpretations of lake history for the past 2000 years, including a major lowstand at 1941 m. No shorelines below the previously documented major lowstand at 1941 m were found. A relatively steep slope segment, whose toe is at about 1918 m, and which occurs on the southern and western margins of the deep basin of the lake, is interpreted as the relict foreset slope of deposition from prograding western tributaries. This topography is unconformably overlain by a unit of interbedded tephra and lake sediments of variable lithology, which contains tephra of the North Mono (600-625 cal yr BP) eruption in its upper part. The tephra-rich unit is overlain by a mostly massive mudflow deposit that is locally more than 18m thick and that is distributed in a radial pattern around Paoha Island. The evidence suggests that within the past few hundred years, rapid uplift of Paoha Island through thick, preexisting lake deposits led to widespread slope failures, which created a terrain of disrupted, intact blocks near the island, and a thick, fluid mudflow beyond. As is common in mudflows, the mudflow moved up the depositional slope of the lake floor, terminating against the preexisting slopes, likely in multiple surges. Since about 1700 Common Era, fine-grained, well-laminated sediments have accumulated in the deep parts of the lake at anomalously rapid rates, probably driven by continued rapid, small-scale shedding of sediment from Paoha Island. C1 [Colman, S. M.] Univ Minnesota, Large Lakes Observ, Duluth, MN 55812 USA. [Hemming, S. R.] Columbia Univ, Dept Earth & Environm Sci, Palisades, NY USA. [Hemming, S. R.] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY USA. [Stine, S.] Calif State Univ Eastbay, Hayward, CA USA. [Zimmerman, S. R. H.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. RP Colman, SM (reprint author), Univ Minnesota, Large Lakes Observ, Duluth, MN 55812 USA. EM scolman@d.umn.edu RI Zimmerman, Susan/A-3351-2013 NR 26 TC 2 Z9 2 U1 2 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD MAY PY 2014 VL 119 IS 5 BP 3955 EP 3970 DI 10.1002/2013JB010726 PG 16 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AJ9EK UT WOS:000338009800002 ER PT J AU Takeda, M Hiratsuka, T Manaka, M Finsterle, S Ito, K AF Takeda, M. Hiratsuka, T. Manaka, M. Finsterle, S. Ito, K. TI Experimental examination of the relationships among chemico-osmotic, hydraulic, and diffusion parameters of Wakkanai mudstones SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article ID TRIPLE-LAYER MODEL; HORONOBE URL SITE; CLAY MEMBRANES; SEDIMENTARY BASINS; OSMOSIS EXPERIMENT; WATER TRANSPORT; OPALINUS CLAY; ROCK SAMPLE; EFFICIENCY; FLOW AB Sequential permeability and chemical osmosis experiments on Wakkanai mudstones were performed to explore the relationships between the semipermeability of clayey rocks and the hydraulic and diffusion parameters as well as the pore structure characteristics. The wide ranges in osmotic efficiency (0.0004-0.046) and intrinsic permeability (8.92 x 10(-20) to 1.24 x 10(-17) m(2)) reflect the variation in the pore size distributions of the Wakkanai mudstones. A regression analysis between osmotic efficiency and permeability shows that the osmotic efficiency is proportional to the inverse of permeability, suggesting that the permeability is indeed indicative of the degree of semipermeability. Osmotic efficiency was determined invariant with the effective diffusion coefficient for the Wakkanai mudstones (3.59-8.36 x 10(-11) m(2)/s) due to their small osmotic efficiencies (<= 0.046). The wide variation in osmotic efficiencies and pore structure characteristics of Wakkanai mudstones indicates that the nanoscale pores enable semipermeability in Wakkanai mudstones. However, the pressure evolution caused by chemical osmosis is limited by the connected wide pores that are the main conduits for water, thus dissipating the osmotic pressure buildup induced by the semipermeability of nanoscale pores. C1 [Takeda, M.; Hiratsuka, T.; Manaka, M.; Ito, K.] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki, Japan. [Finsterle, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Takeda, M (reprint author), Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki, Japan. EM mikio-takeda@aist.go.jp RI Finsterle, Stefan/A-8360-2009 OI Finsterle, Stefan/0000-0002-4446-9906 FU Secretariat of Nuclear Regulation Authority (Secretariat of NRA), Japan; U.S. Department of Energy [DE-AC02-05CH11231] FX The primary part of this research project has been conducted as regulatory-supporting research funded by the Secretariat of Nuclear Regulation Authority (Secretariat of NRA), Japan. The second-to-last author (Stefan Finsterle) was supported, in part, by the U.S. Department of Energy under contract DE-AC02-05CH11231. The data for this paper are available upon request. The authors wish to thank Masashi Nakayama and JAEA for providing the mudstone samples. The authors also wish to thank Tomochika Tokunaga (University of Tokyo) for the fruitful comments and discussions. Careful and very constructive comments on the manuscript by Ian Charles Bourg (LBNL) are gratefully acknowledged. Finally, the Associate Editor, one anonymous reviewer, and Julio Goncalves are gratefully appreciated for their constructive and valuable comments. NR 70 TC 2 Z9 3 U1 0 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD MAY PY 2014 VL 119 IS 5 BP 4178 EP 4201 DI 10.1002/2013JB010421 PG 24 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AJ9EK UT WOS:000338009800013 ER PT J AU Lin, WC Villez, KRE Garcia, HE AF Lin, Wen-Chiao Villez, Kris R. E. Garcia, Humberto E. TI Experimental validation of a resilient monitoring and control system SO JOURNAL OF PROCESS CONTROL LA English DT Article DE Resilient monitoring and control systems; Experimental validation; Cyber-physical attacks; Health condition assessment; Hardware-in-the-loop; Adaptive supervisory controls; Fault detection; Identification; Accommodation ID PROCESS FAULT-DETECTION; MATHEMATICAL-THEORY; ADAPTIVE-CONTROL; IDENTIFICATION; STRATEGIES; TRENDS; MODEL; PCA AB Complex, high performance, engineering systems have to be closely monitored and controlled to ensure safe operation and protect public from potential hazards. One of the main challenges in designing monitoring and control algorithms for these systems is that sensors and actuators may be malfunctioning due to malicious or natural causes. To address this challenge, this paper addresses a resilient monitoring and control (ReMAC) system by expanding previously developed resilient condition assessment monitoring systems and Kalman filter-based diagnostic methods and integrating them with a supervisory controller developed here. While the monitoring and diagnostic algorithms assess plant cyber and physical health conditions, the supervisory controller selects, from a set of candidates, the best controller based on the current plant health assessments. To experimentally demonstrate its enhanced performance, the developed ReMAC system is then used for monitoring and control of a chemical reactor with a water cooling system in a hardware-in-the-loop setting, where the reactor is computer simulated and the water cooling system is implemented by a machine condition monitoring testbed at Idaho National Laboratory. Results show that the ReMAC system is able to make correct plant health assessments despite sensor malfunctioning due to cyber attacks and make decisions that achieve best control actions despite possible actuator malfunctioning. Monitoring challenges caused by mismatches between assumed system component models and actual measurements are also identified for future work. Published by Elsevier Ltd. C1 [Lin, Wen-Chiao; Garcia, Humberto E.] Idaho Natl Lab, Dynam Syst Integrat Optimizat & Resilient Control, Idaho Falls, ID 83415 USA. [Villez, Kris R. E.] Eawag Proc Engn, CH-8600 Dubendorf, Switzerland. RP Garcia, HE (reprint author), Idaho Natl Lab, Dynam Syst Integrat Optimizat & Resilient Control, Idaho Falls, ID 83415 USA. FU Instrumentation, Control, and Intelligent Systems (ICIS) initiative at Idaho National Laboratory under U.S. Department of Energy [DE-AC07-05ID14517] FX The research reported here was supported by the Instrumentation, Control, and Intelligent Systems (ICIS) initiative at Idaho National Laboratory under U.S. Department of Energy contract DE-AC07-05ID14517. The authors would also like to thank Mr. Reed B. Carlson of the Idaho National Laboratory for his assistance in running the HiL experiments. NR 37 TC 3 Z9 3 U1 1 U2 12 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0959-1524 EI 1873-2771 J9 J PROCESS CONTR JI J. Process Control PD MAY PY 2014 VL 24 IS 5 BP 621 EP 639 DI 10.1016/j.jprocont.2014.03.006 PG 19 WC Automation & Control Systems; Engineering, Chemical SC Automation & Control Systems; Engineering GA AJ7BO UT WOS:000337852300015 ER PT J AU Aitken, ML Kosovic, B Mirocha, JD Lundquist, JK AF Aitken, Matthew L. Kosovic, Branko Mirocha, Jeffrey D. Lundquist, Julie K. TI Large eddy simulation of wind turbine wake dynamics in the stable boundary layer using the Weather Research and Forecasting Model SO JOURNAL OF RENEWABLE AND SUSTAINABLE ENERGY LA English DT Article ID LOW-LEVEL JET; REYNOLDS-NUMBER; TURBULENCE; FARM; FLOW AB Recently, an actuator disk parameterization was implemented in the Weather Research and Forecasting (WRF) Model for large eddy simulation (LES) of wind turbine wakes. To thoroughly verify this model, simulations of various types of turbines and atmospheric conditions must be evaluated against corresponding experimental data. In this work, numerical simulations are compared to nacelle-based scanning lidar measurements taken in stable atmospheric conditions during a field campaign conducted at a wind farm in the western United States. Using several wake characteristics-such as the velocity deficit, centerline location, and wake width-as metrics for model verification, the simulations show good agreement with the observations. Notable results include a high average velocity deficit, decreasing from 73% at a downwind distance x of 1.2 rotor diameters (D) to 25% at x=6.6D, resulting from a low average wind speed and therefore high average turbine thrust coefficient. Moreover, the wake width expands from 1.4D at x=1.2D to 2.3D at x=6.6D. Finally, new features-namely rotor tilt and drag from the nacelle and tower-are added to the existing actuator disk model in WRF-LES. Compared to the rotor, the effect of the tower and nacelle on the flow is relatively small but nevertheless important for an accurate representation of the entire turbine. Adding rotor tilt to the model causes the vertical location of the wake center to shift upward. Continued advancement of the actuator disk model in WRF-LES will help lead to optimized turbine siting and controls at wind farms. (C) 2014 AIP Publishing LLC. C1 [Aitken, Matthew L.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Kosovic, Branko] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Mirocha, Jeffrey D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Lundquist, Julie K.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. [Lundquist, Julie K.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Aitken, ML (reprint author), Univ Colorado, Dept Phys, 390 UCB, Boulder, CO 80309 USA. EM matthew.aitken@colorado.edu OI LUNDQUIST, JULIE/0000-0001-5490-2702 FU National Science Foundation [CNS-0821794]; University of Colorado Boulder; University of Colorado Denver; National Center for Atmospheric Research; National Renewable Energy Laboratory [UGA-0-41026-22, UGA-0-41026-65]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We wish to thank the wind farm operator for generously collecting and sharing the observational data and for providing the wind turbine specifications used in the actuator disk model. Many thanks also to Brian Vanderwende for innumerable helpful discussions on WRF and high performance computing. This work utilized the Janus supercomputer, which is supported by the National Science Foundation (Award No. CNS-0821794), the University of Colorado Boulder, the University of Colorado Denver, and the National Center for Atmospheric Research. The Janus supercomputer is operated by the University of Colorado Boulder. Parts of this research were supported by the National Renewable Energy Laboratory under Professor Lundquist's Joint Appointment, UGA-0-41026-22 and UGA-0-41026-65. Work by Dr. Mirocha was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 44 TC 12 Z9 12 U1 2 U2 34 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1941-7012 J9 J RENEW SUSTAIN ENER JI J. Renew. Sustain. Energy PD MAY PY 2014 VL 6 IS 3 AR 033137 DI 10.1063/1.4885111 PG 13 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA AJ9ZS UT WOS:000338072800039 ER PT J AU Liu, RQ Li, DY Wang, C Li, N Li, Q Lu, XJ Spendelow, JS Wu, G AF Liu, Ruiqing Li, Deyu Wang, Chen Li, Ning Li, Qing Lu, Xujie Spendelow, Jacob S. Wu, Gang TI Core-shell structured hollow SnO2-polypyrrole nanocomposite anodes with enhanced cyclic performance for lithium-ion batteries SO NANO ENERGY LA English DT Article DE SnO2 nanoparticles; Polypyrrole; Hollow morphology; Anodes; Lithium ion batteries ID COMPOSITE CATHODE MATERIALS; FACILE SYNTHESIS; MESOPOROUS SNO2; TIN; ELECTRODE; OXIDE; STABILITY; NANOTUBES; CAPACITY; HYBRID AB Core-shell structured hollow SnO2-polypyrrole (PPy) nanocomposites (SnO2 PPy) with excellent electrochemical performance were synthesized using a hydrothermal method followed by an in situ chemical-polymerization route. The thickness of the polymerized amorphous PPy coating covering on the hollow SnO2 microspheres is about 25 nm, demonstrated by microscopy images. As an anode in lithium ion batteries, the nanocomposite is capable of retaining a high capacity of 448.4 mAh g(-1) after 100 cycles with a coulomb efficiency above 97%. Compared to other reported SnO2 anodes, the enhanced cycling stability is attributed to the unique core-shell structure and a possible synergistic effect between the PPy coating layer and the hollow SnO2 spheres. The PPy coating not only prevents the possible pulverization of the hollow SnO2 spheres, but also prevents the SnO2/Sn spheres from aggregating. Furthermore, the hollow space within the SnO2 nanoparticles effectively mitigates the enormous volume change during charge-discharge cycling. Meanwhile, the Li+ diffusion coefficient in the hollow SnO2@PPy (21wt%) core-shell nanocomposite electrode is significantly improved compared to the hollow SnO2 microspheres electrode. Thus, these benefits from the PPy coating and the hollow SnO2 spheres are able to provide a robust architecture for lithium-ion battery anodes. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Liu, Ruiqing; Li, Deyu; Wang, Chen; Li, Ning] Harbin Inst Technol, Sch Chem Engn Technol, Harbin 150001, Peoples R China. [Li, Qing; Lu, Xujie; Spendelow, Jacob S.; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Li, N (reprint author), Harbin Inst Technol, Sch Chem Engn Technol, Harbin 150001, Peoples R China. EM lininghit@263.net; qinglilanl@gmail.com; wugang@lanl.gov RI Wu, Gang/E-8536-2010; Lu, Xujie/L-9672-2014; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Lu, Xujie/0000-0001-8402-7160; Li, Qing/0000-0003-4807-030X FU Los Alamos National Laboratory Early Career Laboratory-Directed Research and Development (LDRD) Program [20110483ER] FX Financial support from the Los Alamos National Laboratory Early Career Laboratory-Directed Research and Development (LDRD) Program (20110483ER) for this work is gratefully acknowledged. NR 41 TC 45 Z9 45 U1 29 U2 279 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 J9 NANO ENERGY JI Nano Energy PD MAY PY 2014 VL 6 BP 73 EP 81 DI 10.1016/j.nanoen.2014.03.010 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AJ8DH UT WOS:000337932400010 ER PT J AU Xia, T Zhang, W Wang, ZH Zhang, YL Song, XY Murowchick, J Battaglia, V Liu, G Chen, XB AF Xia, Ting Zhang, Wei Wang, Zhihui Zhang, Yuliang Song, Xiangyun Murowchick, James Battaglia, Vincent Liu, Gao Chen, Xiaobo TI Amorphous carbon-coated TiO2 nanocrystals for improved lithium-ion battery and photocatalytic performance SO NANO ENERGY LA English DT Article DE TiO2 nanocrystals; Amorphous carbon coating; Lithium ion battery; Photocatalytic performance ID ANATASE TIO2; NANOSTRUCTURED TIO2; ROOM-TEMPERATURE; SURFACE; HYDROGENATION; STORAGE; GROWTH AB 10-time lithium rate improvement and 4-time photocatalytic performance enhancement have been achieved with TiO2 nanocrystals when coated with a thin layer of amorphous carbon. The enhanced performances can be attributed to lower lithium ion diffusion and electronic conduction resistance across the carbon layer into the TiO2 electrode material and better surface adsorption of the dye molecules and ions. Thus, the current study may provide us an alternative approach in improving the performances of TiO2 nanocrystals in both lithium ion battery and photocatalysis applications. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Xia, Ting; Zhang, Yuliang; Chen, Xiaobo] Univ Missouri, Dept Chem, Kansas City, MO 64110 USA. [Zhang, Wei; Wang, Zhihui; Song, Xiangyun; Battaglia, Vincent; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Zhang, Yuliang] Shanghai Maritime Univ, Inst Mat Sci & Engn, Shanghai 201306, Peoples R China. [Murowchick, James] Univ Missouri, Dept Geosci, Kansas City, KS 64110 USA. RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM GLiu@lbl.gov; Chenxiaobo@umkc.edu FU Assistant Secretary for Energy Efficiency, Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC03-76SF00098]; College of Arts and Sciences, University of Missouri - Kansas City; University of Missouri Research Board; National Natural Science Foundation of China [21071096] FX G. L. thanks the fund by the Assistant Secretary for Energy Efficiency, Office of Vehicle Technologies of the U.S. Department of Energy under Contract no. DE-AC03-76SF00098. X. C. thanks the support from College of Arts and Sciences, University of Missouri - Kansas City, the University of Missouri Research Board, and the generous gift from Dow Kokam. Y. Z. thanks National Natural Science Foundation of China (No. 21071096) for its financial support. NR 51 TC 65 Z9 66 U1 27 U2 160 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 J9 NANO ENERGY JI Nano Energy PD MAY PY 2014 VL 6 BP 109 EP 118 DI 10.1016/j.nanoen.2014.03.012 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AJ8DH UT WOS:000337932400014 ER PT J AU Zeng, X Anitescu, M AF Zeng, X. Anitescu, M. TI Sequential Monte Carlo sampling in hidden Markov models of nonlinear dynamical systems SO APPLIED MATHEMATICS AND COMPUTATION LA English DT Article DE Hidden Markov model; Ordinary differential equation; Sequential Monte Carlo methods; Chemical process ID ENSEMBLE KALMAN FILTER; DATA ASSIMILATION; RECOGNITION; STATISTICS; SEPARATION AB We investigate the issue of which state functionals can have their uncertainty estimated efficiently in dynamical systems with uncertainty. Because of the high dimensionality and complexity of the problem, sequential Monte Carlo (SMC) methods are used. We investigate SMC methods where the proposal distribution is computed by maximum likelihood or by a linearization approach. We prove that the variance of the SMC method is bounded linearly in the number of time steps when the proposal distribution is truncated normal distribution. We also show that for a moderate large number of steps the error produced by approximation of dynamical systems linearly accumulates on the condition that the logarithm of the density function of noise is Lipschitz continuous. This finding is significant because the uncertainty in many dynamical systems, in particular, in chemical engineering systems, can be assumed to have this nature. We demonstrate our findings for a simple test case from chemical engineering. The theoretical findings provide a foundation for the parallel software SISTOS. (C) 2014 Elsevier Inc. All rights reserved. C1 [Zeng, X.] Shanghai Univ, Dept Math, Shanghai, Peoples R China. [Zeng, X.; Anitescu, M.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Anitescu, M (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 South Cass Ave,Bldg 240, Argonne, IL 60439 USA. EM anitescu@mcs.anl.gov FU U.S. Department of Energy [DE-AC02-06CH11357] FX We are grateful to the anonymous referee for comments that have improved the paper, particularly for the suggestion of describing differences with the bootstrap filter. We are grateful to Candido Pereira and John Krebs from the Chemical Sciences and Engineering Division at Argonne National Laboratory for comments and suggestions concerning applications in chemical engineering. This work was supported by the U.S. Department of Energy under contract DE-AC02-06CH11357. NR 35 TC 0 Z9 1 U1 1 U2 7 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0096-3003 EI 1873-5649 J9 APPL MATH COMPUT JI Appl. Math. Comput. PD MAY 1 PY 2014 VL 233 BP 507 EP 521 DI 10.1016/j.amc.2014.02.012 PG 15 WC Mathematics, Applied SC Mathematics GA AI9VH UT WOS:000337288900049 ER PT J AU Abdo, AA Abeysekara, AU Allen, BT Aune, T Barber, AS Berley, D Braun, J Chen, C Christopher, GE DeYoung, T Dingus, BL Ellsworth, RW Gonzalez, MM Goodman, JA Hays, E Hoffman, CM Huntemeyer, PH Imran, A Kolterman, BE Linnemann, JT McEnery, JE Morgan, T Mincer, AI Nemethy, P Pretz, J Ryan, JM Parkinson, PMS Schneider, M Shoup, A Sinnis, G Smith, AJ Vasileiou, V Walker, GP Williams, DA Yodh, GB AF Abdo, A. A. Abeysekara, A. U. Allen, B. T. Aune, T. Barber, A. S. Berley, D. Braun, J. Chen, C. Christopher, G. E. DeYoung, T. Dingus, B. L. Ellsworth, R. W. Gonzalez, M. M. Goodman, J. A. Hays, E. Hoffman, C. M. Huentemeyer, P. H. Imran, A. Kolterman, B. E. Linnemann, J. T. McEnery, J. E. Morgan, T. Mincer, A. I. Nemethy, P. Pretz, J. Ryan, J. M. Parkinson, P. M. Saz Schneider, M. Shoup, A. Sinnis, G. Smith, A. J. Vasileiou, V. Walker, G. P. Williams, D. A. Yodh, G. B. TI Milagro observations of potential TeV emitters SO ASTROPARTICLE PHYSICS LA English DT Article DE Astroparticle physics; Pulsars; Galaxies; Active galactic nuclei; Gamma-rays ID CYGNUS REGION; SPECTRUM; MARKARIAN-421; DISCOVERY; EMISSION; AREA AB This paper reports the results from three targeted searches of Milagro TeV sky maps: two extragalactic point source lists and one pulsar source list. The first extragalactic candidate list consists of 709 candidates selected from the Fermi-LAT 2FGL catalog. The second extragalactic candidate list contains 31 candidates selected from the TeVCat source catalog that have been detected by imaging atmospheric Cherenkov telescopes (IACTs). In both extragalactic candidate lists Mkn 421 was the only source detected by Milagro. This paper presents the Milagro TeV flux for Mkn 421 and flux limits for the brighter Fermi-LAT extragalactic sources and for all TeVCat candidates. The pulsar list extends a previously published Milagro targeted search for Galactic sources. With the 32 new gamma-ray pulsars identified in 2FGL, the number of pulsars that are studied by both Fermi-LAT and Milagro is increased to 52. In this sample, we find that the probability of Milagro detecting a TeV emission coincident with a pulsar increases with the GeV flux observed by the Fermi-LAT in the energy range from 0.1 GeV to 100 GeV. (C) 2014 Elsevier B.V. All rights reserved. C1 [Abdo, A. A.; Abeysekara, A. U.; Barber, A. S.; Linnemann, J. T.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Allen, B. T.; Chen, C.; Yodh, G. B.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Aune, T.; Parkinson, P. M. Saz; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Berley, D.; Braun, J.; Goodman, J. A.; Smith, A. J.; Vasileiou, V.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Christopher, G. E.; Kolterman, B. E.; Mincer, A. I.; Nemethy, P.] NYU, Dept Phys, New York, NY 10003 USA. [DeYoung, T.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Dingus, B. L.; Hoffman, C. M.; Imran, A.; Pretz, J.; Sinnis, G.; Walker, G. P.] Los Alamos Natl Lab, Grp P 23, Los Alamos, NM 87545 USA. [Ellsworth, R. W.] George Mason Univ, Dept Phys & Astron, Fairfax, VA 22030 USA. [Gonzalez, M. M.] Univ Nacl Autonoma Mexico, Inst Astron, Mexico City 04510, DF, Mexico. [Hays, E.; McEnery, J. E.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Huentemeyer, P. H.] Michigan Technol Univ, Dept Phys, Houghton, MI 49931 USA. [Morgan, T.; Ryan, J. M.] Univ New Hampshire, Dept Phys, Durham, NH 03824 USA. [Schneider, M.] Univ Calif Santa Cruz, Santa Cruz, CA 95064 USA. [Shoup, A.] Ohio State Univ, Lima, OH 45804 USA. [Parkinson, P. M. Saz] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. RP Abeysekara, AU (reprint author), Michigan State Univ, Dept Phys & Astron, BioMed Phys Sci Bldg, E Lansing, MI 48824 USA. EM udaraabeysekara@yahoo.com OI Mincer, Allen/0000-0002-6307-1418; Dingus, Brenda/0000-0001-8451-7450 NR 20 TC 1 Z9 1 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD MAY-JUN PY 2014 VL 57-58 BP 16 EP 25 DI 10.1016/j.astropartphys.2014.03.001 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AJ4MY UT WOS:000337651700004 ER PT J AU Wu, JY Zhou, Y Gao, Y Fu, JS Johnson, BA Huang, C Kim, YM Liu, Y AF Wu, Jianyong Zhou, Ying Gao, Yang Fu, Joshua S. Johnson, Brent A. Huang, Cheng Kim, Young-Min Liu, Yang TI The Time Trend Temperature-Mortality as a Factor of Uncertainty Analysis of Impacts of Future Heat Waves: Wu et al. Respond SO ENVIRONMENTAL HEALTH PERSPECTIVES LA English DT Letter C1 [Wu, Jianyong; Zhou, Ying; Kim, Young-Min; Liu, Yang] Emory Univ, Rollins Sch Publ Hlth, Dept Environm Hlth, Atlanta, GA 30322 USA. [Gao, Yang; Fu, Joshua S.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN USA. [Gao, Yang] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Johnson, Brent A.] Emory Univ, Rollins Sch Publ Hlth, Dept Biostat & Bioinformat, Atlanta, GA 30322 USA. [Huang, Cheng] George Washington Univ, Sch Publ Hlth & Hlth Serv, Dept Global Hlth, Washington, DC USA. RP Wu, JY (reprint author), Emory Univ, Rollins Sch Publ Hlth, Dept Environm Hlth, Atlanta, GA 30322 USA. EM yang.liu@emory.edu RI Wu, Jianyong/A-6854-2011 OI Wu, Jianyong/0000-0002-5864-3186 NR 7 TC 1 Z9 1 U1 2 U2 9 PU US DEPT HEALTH HUMAN SCIENCES PUBLIC HEALTH SCIENCE PI RES TRIANGLE PK PA NATL INST HEALTH, NATL INST ENVIRONMENTAL HEALTH SCIENCES, PO BOX 12233, RES TRIANGLE PK, NC 27709-2233 USA SN 0091-6765 EI 1552-9924 J9 ENVIRON HEALTH PERSP JI Environ. Health Perspect. PD MAY PY 2014 VL 122 IS 5 BP A118 EP A119 DI 10.1289/ehp.1308042R PG 2 WC Environmental Sciences; Public, Environmental & Occupational Health; Toxicology SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Toxicology GA AJ3ZC UT WOS:000337606300002 PM 24784327 ER PT J AU Walker, AP Hanson, PJ De Kauwe, MG Medlyn, BE Zaehle, S Asao, S Dietze, M Hickler, T Huntingford, C Iversen, CM Jain, A Lomas, M Luo, YQ McCarthy, H Parton, WJ Prentice, IC Thornton, PE Wang, SS Wang, YP Warlind, D Weng, ES Warren, JM Woodward, FI Oren, R Norby, RJ AF Walker, Anthony P. Hanson, Paul J. De Kauwe, Martin G. Medlyn, Belinda E. Zaehle, Soenke Asao, Shinichi Dietze, Michael Hickler, Thomas Huntingford, Chris Iversen, Colleen M. Jain, Atul Lomas, Mark Luo, Yiqi McCarthy, Heather Parton, William J. Prentice, I. Colin Thornton, Peter E. Wang, Shusen Wang, Ying-Ping Warlind, David Weng, Ensheng Warren, Jeffrey M. Woodward, F. Ian Oren, Ram Norby, Richard J. TI Comprehensive ecosystem model-data synthesis using multiple data sets at two temperate forest free-air CO2 enrichment experiments: Model performance at ambient CO2 concentration SO JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES LA English DT Article DE model structural analysis; model benchmarking; net primary production (NPP); leaf area index (LAI); sap flow; transpiration; FACE experiment ID ELEVATED ATMOSPHERIC CO2; GLOBAL VEGETATION MODELS; CARBON-DIOXIDE ENRICHMENT; NET PRIMARY PRODUCTIVITY; LONG-TERM RESPONSE; CANOPY LEAF-AREA; LAND-USE CHANGE; DECIDUOUS FOREST; TERRESTRIAL BIOSPHERE; NITROGEN AVAILABILITY AB Free-air CO2 enrichment (FACE) experiments provide a remarkable wealth of data which can be used to evaluate and improve terrestrial ecosystem models (TEMs). In the FACE model-data synthesis project, 11 TEMs were applied to two decadelong FACE experiments in temperate forests of the southeastern U.S.the evergreen Duke Forest and the deciduous Oak Ridge Forest. In this baseline paper, we demonstrate our approach to model-data synthesis by evaluating the models' ability to reproduce observed net primary productivity (NPP), transpiration, and leaf area index (LAI) in ambient CO2 treatments. Model outputs were compared against observations using a range of goodness-of-fit statistics. Many models simulated annual NPP and transpiration within observed uncertainty. We demonstrate, however, that high goodness-of-fit values do not necessarily indicate a successful model, because simulation accuracy may be achieved through compensating biases in component variables. For example, transpiration accuracy was sometimes achieved with compensating biases in leaf area index and transpiration per unit leaf area. Our approach to model-data synthesis therefore goes beyond goodness-of-fit to investigate the success of alternative representations of component processes. Here we demonstrate this approach by comparing competing model hypotheses determining peak LAI. Of three alternative hypotheses(1) optimization to maximize carbon export, (2) increasing specific leaf area with canopy depth, and (3) the pipe modelthe pipe model produced peak LAI closest to the observations. This example illustrates how data sets from intensive field experiments such as FACE can be used to reduce model uncertainty despite compensating biases by evaluating individual model assumptions. C1 [Walker, Anthony P.; Hanson, Paul J.; Iversen, Colleen M.; Thornton, Peter E.; Warren, Jeffrey M.; Norby, Richard J.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Walker, Anthony P.; Hanson, Paul J.; Iversen, Colleen M.; Thornton, Peter E.; Warren, Jeffrey M.; Norby, Richard J.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Walker, Anthony P.; Lomas, Mark; Woodward, F. Ian] Univ Sheffield, Dept Anim & Plant Sci, Sheffield S10 2TN, S Yorkshire, England. [De Kauwe, Martin G.; Medlyn, Belinda E.; Prentice, I. Colin] Macquarie Univ, Dept Biol Sci, Sydney, NSW 2109, Australia. [Zaehle, Soenke] Max Planck Inst Biogeochem, Biogeochem Integrat Dept, D-07745 Jena, Germany. [Asao, Shinichi; Parton, William J.] Colorado State Univ, Dept Ecosyst Sci & Sustainabil, Ft Collins, CO 80523 USA. [Dietze, Michael] Boston Univ, Dept Earth & Environm, Boston, MA 02215 USA. [Hickler, Thomas] Biodivers & Climate Res Ctr BiK F, Frankfurt, Germany. [Hickler, Thomas] Senckenberg Gesell Nat Forsch, Frankfurt, Germany. [Hickler, Thomas] Goethe Univ Frankfurt, Dept Phys Geog, D-60054 Frankfurt, Germany. [Huntingford, Chris] Ctr Ecol & Hydrol, Wallingford, Oxon, England. [Jain, Atul] Univ Illinois, Dept Atmospher Sci, Urbana, IL 61801 USA. [Luo, Yiqi; McCarthy, Heather] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Prentice, I. Colin] Univ London Imperial Coll Sci Technol & Med, Dept Life Sci, London, England. [Prentice, I. Colin] Univ London Imperial Coll Sci Technol & Med, Grantham Inst Climate Change, London, England. [Wang, Shusen] Nat Resources Canada, Canada Ctr Mapping & Earth Observat, Ottawa, ON, Canada. [Wang, Ying-Ping] CSIRO Marine & Atmospher Res, Aspendale, Vic, Australia. [Wang, Ying-Ping] Ctr Australian Weather & Climate Res, Aspendale, Vic, Australia. [Warlind, David] Lund Univ, Dept Phys Geog & Ecosyst Sci, Lund, Sweden. [Weng, Ensheng] Princeton Univ, Dept Ecol & Evolutionary Biol, Princeton, NJ 08544 USA. [Oren, Ram] Duke Univ, Nicholas Sch Environm, Div Environm Sci & Policy, Durham, NC 27708 USA. [Oren, Ram] Swedish Univ Agr Sci, Dept Forest Ecol & Management, S-90183 Umea, Sweden. RP Walker, AP (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. EM walkerap@ornl.gov RI Warren, Jeffrey/B-9375-2012; Asao, Shinichi/R-9514-2016; Hickler, Thomas/S-6287-2016; Huntingford, Chris/A-4307-2008; Weng, Ensheng/E-4390-2012; wang, yp/A-9765-2011; Walker, Anthony/G-2931-2016; Dietze, Michael/A-5834-2009; Warlind, David/A-5109-2015; Hanson, Paul J./D-8069-2011; Norby, Richard/C-1773-2012; Thornton, Peter/B-9145-2012; Jain, Atul/D-2851-2016; Zaehle, Sonke/C-9528-2017; OI Warren, Jeffrey/0000-0002-0680-4697; Asao, Shinichi/0000-0002-0334-5464; Hickler, Thomas/0000-0002-4668-7552; Weng, Ensheng/0000-0002-1858-4847; Walker, Anthony/0000-0003-0557-5594; Dietze, Michael/0000-0002-2324-2518; Hanson, Paul J./0000-0001-7293-3561; Norby, Richard/0000-0002-0238-9828; Thornton, Peter/0000-0002-4759-5158; Jain, Atul/0000-0002-4051-3228; Zaehle, Sonke/0000-0001-5602-7956; Medlyn, Belinda/0000-0001-5728-9827; Huntingford, Chris/0000-0002-5941-7770; Wang, Shusen/0000-0003-1860-899X FU National Center for Ecological Analysis and Synthesis (NCEAS) [EF-0553768]; U.S. Department of Energy (DOE) Office of Science's Biological and Environmental Research (BER); UK National Centre for Earth Observation (NCEO); ARC [DP1094791]; U.S. Department of Energy [DE-AC05-00OR22725] FX This effort was conducted by the "Benchmarking ecosystem response models with experimental data from long-term CO2 enrichment experiments" Working Group supported by National Center for Ecological Analysis and Synthesis (NCEAS; grant EF-0553768). The Oak Ridge and Duke FACE sites and additional synthesis were supported by the U.S. Department of Energy (DOE) Office of Science's Biological and Environmental Research (BER). Running the simulations was supported by funding available to the individual modeling groups. Additional support for A.P.W. was provided by a UK National Centre for Earth Observation (NCEO) sponsored PhD. M. D. K. was also supported by ARC Discovery grant DP1094791. Much of the data used in this model-data synthesis project can be found on the FACE Data Management System on the ORNL Carbon Dioxide Information Analysis Center (CDIAC) website (http://public.ornl.gov/face/), and the model data will be made available on that site in due course. Please contact the corresponding author for more information. This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 119 TC 24 Z9 24 U1 8 U2 62 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-8953 EI 2169-8961 J9 J GEOPHYS RES-BIOGEO JI J. Geophys. Res.-Biogeosci. PD MAY PY 2014 VL 119 IS 5 BP 937 EP 964 DI 10.1002/2013JG002553 PG 28 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA AJ3ZN UT WOS:000337607900016 ER PT J AU Rowan, AV Brocklehurst, SH Schultz, DM Plummer, MA Anderson, LS Glasser, NF AF Rowan, Ann V. Brocklehurst, Simon H. Schultz, David M. Plummer, Mitchell A. Anderson, Leif S. Glasser, Neil F. TI Late Quaternary glacier sensitivity to temperature and precipitation distribution in the Southern Alps of New Zealand SO JOURNAL OF GEOPHYSICAL RESEARCH-EARTH SURFACE LA English DT Article DE glacier climate; palaeoclimate; Otiran glaciation ID FRANZ JOSEF GLACIER; MASS-BALANCE; CLIMATE VARIABILITY; INTIMATE PROJECT; MAXIMUM CLIMATE; UINTA MOUNTAINS; ENERGY-BALANCE; ICE FLOW; EVOLUTION; HOLOCENE AB Glaciers respond to climate variations and leave geomorphic evidence that represents an important terrestrial paleoclimate record. However, the accuracy of paleoclimate reconstructions from glacial geology is limited by the challenge of representing mountain meteorology in numerical models. Precipitation is usually treated in a simple manner and yet represents difficult-to-characterize variables such as amount, distribution, and phase. Furthermore, precipitation distributions during a glacial probably differed from present-day interglacial patterns. We applied two models to investigate glacier sensitivity to temperature and precipitation in the eastern Southern Alps of New Zealand. A 2-D model was used to quantify variations in the length of the reconstructed glaciers resulting from plausible precipitation distributions compared to variations in length resulting from change in mean annual air temperature and precipitation amount. A 1-D model was used to quantify variations in length resulting from interannual climate variability. Assuming that present-day interglacial values represent precipitation distributions during the last glacial, a range of plausible present-day precipitation distributions resulted in uncertainty in the Last Glacial Maximum length of the Pukaki Glacier of 17.1km (24%) and the Rakaia Glacier of 9.3km (25%), corresponding to a 0.5 degrees C difference in temperature. Smaller changes in glacier length resulted from a 50% decrease in precipitation amount from present-day values (-14% and -18%) and from a 50% increase in precipitation amount (5% and 9%). Our results demonstrate that precipitation distribution can produce considerable variation in simulated glacier extents and that reconstructions of paleoglaciers should include this uncertainty. C1 [Rowan, Ann V.; Glasser, Neil F.] Aberystwyth Univ, Dept Geog & Earth Sci, Ctr Glaciol, Aberystwyth, Dyfed, Wales. [Brocklehurst, Simon H.; Schultz, David M.] Univ Manchester, Sch Earth Atmospher & Environm Sci, Manchester, Lancs, England. [Plummer, Mitchell A.] Idaho Natl Lab, Idaho Falls, ID USA. [Anderson, Leif S.] Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA. [Anderson, Leif S.] Univ Colorado, Dept Geol Sci, Boulder, CO 80309 USA. RP Rowan, AV (reprint author), British Geol Survey, Ctr Environm Sci, Nottingham NG12 5GG, England. EM annr@bgs.ac.uk RI Schultz, David M./A-3091-2010; OI Schultz, David M./0000-0003-1558-6975; Rowan, Ann/0000-0002-3715-5554; Glasser, Neil/0000-0002-8245-2670 FU Climate Change Consortium of Wales (C3W); Natural Environment Research Council (NERC) [NE/F008295/1]; University of Canterbury; NERC [NE/I026545/1]; National Science Foundation [DGE-1144083] FX A.V. Rowan was supported by a postdoctoral fellowship from the Climate Change Consortium of Wales (C3W), and some of this research was carried out under Natural Environment Research Council (NERC) studentship NE/F008295/1. S. H. Brocklehurst is partially supported by a University of Canterbury Visiting Erskine Fellowship. D. M. Schultz is partially supported by NERC grant NE/I026545/1 Precipitation Structures over Orography (PRESTO). L. S. Anderson is supported by National Science Foundation grant DGE-1144083 (GRFP). The National Institute of Water and Atmospheric Research (NIWA) Ltd. provided the gridded rainfall data used in some simulations. Land Information New Zealand (LINZ) provided the digital elevation model. Gerard Roe is thanked for his comments on the white noise experiments. We thank the Editor Alex Densmore and the Associate Editor Mike Bentley for their helpful suggestions. Comments from Jamie Shulmeister and two anonymous reviewers greatly improved this manuscript. NR 72 TC 5 Z9 5 U1 1 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9003 EI 2169-9011 J9 J GEOPHYS RES-EARTH JI J. Geophys. Res.-Earth Surf. PD MAY PY 2014 VL 119 IS 5 BP 1064 EP 1081 DI 10.1002/2013JF003009 PG 18 WC Geosciences, Multidisciplinary SC Geology GA AJ4DH UT WOS:000337620600006 ER PT J AU Zhang, XY Moldwin, MB Steinberg, JT Skoug, RM AF Zhang, X. -Y. Moldwin, M. B. Steinberg, J. T. Skoug, R. M. TI Alfven waves as a possible source of long-duration, large-amplitude, and geoeffective southward IMF SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE Alfven wave; IMF Bs; geomagnetic activity ID CORONAL MASS EJECTIONS; MAGNETIC-FLUX ROPES; SOLAR-WIND; FIELD; TURBULENCE; RECONNECTION; DYNAMICS; REGIONS; AU AB The southward component (Bs) of the interplanetary magnetic field (IMF) is a strong driver of geomagnetic activity. Well-defined solar wind structures such as magnetic clouds and corotating interaction regions are the main sources of long-duration, large-amplitude IMF Bs. Here we analyze IMF Bsevents (t> 1 h, Bz<-5nT) unrelated with any well-defined solar wind structure at 1 AU using ACE spacecraft observations from 1998 to 2004. We find that about one third of these Bs events show Alfvenic wave features; therefore, those Alfven waves in the solar wind are also an important source of long-duration, large-amplitude IMF southward component. We find that more than half of the Alfven wave (AW)-related Bs events occur in slow solar wind (Vsw < 400 km/s). One third of the AW-type Bsevents triggered geomagnetic storms, and half triggered substorms. C1 [Zhang, X. -Y.; Moldwin, M. B.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Steinberg, J. T.; Skoug, R. M.] Los Alamos Natl Lab, ISR Grp 1, Los Alamos, NM USA. RP Zhang, XY (reprint author), Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. EM zhangxy@umich.edu RI Moldwin, Mark/F-8785-2011; OI Moldwin, Mark/0000-0003-0954-1770; Steinberg, John/0000-0003-2491-1661 FU NASA NESSF [NNX13AM35H]; U.S. Department of Energy; NASA ACE program; Los Alamos Space Weather Summer School FX This work was supported by NASA NESSF grant NNX13AM35H. Work at Los Alamos was performed under the auspices of the U.S. Department of Energy, with support from the NASA ACE program and the Los Alamos Space Weather Summer School (2013). NR 37 TC 3 Z9 3 U1 0 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2014 VL 119 IS 5 BP 3259 EP 3266 DI 10.1002/2013JA019623 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ4DS UT WOS:000337622100004 ER PT J AU Xiao, FL Yang, C He, ZG Su, ZP Zhou, QH He, YH Kletzing, CA Kurth, WS Hospodarsky, GB Spence, HE Reeves, GD Funsten, HO Blake, JB Baker, DN Wygant, JR AF Xiao, Fuliang Yang, Chang He, Zhaoguo Su, Zhenpeng Zhou, Qinghua He, Yihua Kletzing, C. A. Kurth, W. S. Hospodarsky, G. B. Spence, H. E. Reeves, G. D. Funsten, H. O. Blake, J. B. Baker, D. N. Wygant, J. R. TI Chorus acceleration of radiation belt relativistic electrons during March 2013 geomagnetic storm SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE chorus waves; wave-particle interaction; relativistic electron acceleration; RBSP results ID QUASI-LINEAR DIFFUSION; MAGNETIC STORM; RESONANT DIFFUSION; PITCH-ANGLE; RING; MAGNETOSPHERE; PLASMASPHERE; COEFFICIENTS; MODEL AB The recent launching of Van Allen probes provides an unprecedent opportunity to investigate variations of the radiation belt relativistic electrons. During the 17-19 March 2013 storm, the Van Allen probes simultaneously detected strong chorus waves and substantial increases in fluxes of relativistic (2 - 4.5 MeV) electrons around L = 4.5. Chorus waves occurred within the lower band 0.1-0.5fce (the electron equatorial gyrofrequency), with a peak spectral density approximate to 10-4 nT2/Hz. Correspondingly, relativistic electron fluxes increased by a factor of 102-103 during the recovery phase compared to the main phase levels. By means of a Gaussian fit to the observed chorus spectra, the drift and bounce-averaged diffusion coefficients are calculated and then used to solve a 2-D Fokker-Planck diffusion equation. Numerical simulations demonstrate that the lower-band chorus waves indeed produce such huge enhancements in relativistic electron fluxes within 15 h, fitting well with the observation. C1 [Xiao, Fuliang; Yang, Chang; Zhou, Qinghua; He, Yihua] Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha, Hunan, Peoples R China. [He, Zhaoguo] Chinese Acad Sci, Ctr Space Sci & Appl Res, Beijing, Peoples R China. [Su, Zhenpeng] Univ Sci & Technol China, Dept Geophys & Planetary Sci, CAS Key Lab Geospace Environm, Hefei 230026, Peoples R China. [Kletzing, C. A.; Kurth, W. S.; Hospodarsky, G. B.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Funsten, H. O.] Los Alamos Natl Lab, ISR Div, Los Alamos, NM USA. [Blake, J. B.] Aerosp Corp, Los Angeles, CA 90009 USA. [Baker, D. N.] Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO USA. [Wygant, J. R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. RP Xiao, FL (reprint author), Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha, Hunan, Peoples R China. EM flxiao@126.com RI Xiao, Fuliang/B-9245-2011; Funsten, Herbert/A-5702-2015; Su, Zhenpeng/E-1641-2011; Reeves, Geoffrey/E-8101-2011; OI Xiao, Fuliang/0000-0003-1487-6620; Funsten, Herbert/0000-0002-6817-1039; Hospodarsky, George/0000-0001-9200-9878; Su, Zhenpeng/0000-0001-5577-4538; Reeves, Geoffrey/0000-0002-7985-8098; Kletzing, Craig/0000-0002-4136-3348; Kurth, William/0000-0002-5471-6202 FU JHU/APL under NASA [921647, 967399, NAS5-01072] FX This work was also supported from JHU/APL contract No. 921647 and 967399 under NASA Prime contract No. NAS5-01072. NR 36 TC 26 Z9 27 U1 0 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2014 VL 119 IS 5 BP 3325 EP 3332 DI 10.1002/2014JA019822 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ4DS UT WOS:000337622100009 ER PT J AU Schleyer, F Cairns, IH Kim, EH AF Schleyer, Fiona Cairns, Iver H. Kim, Eun-Hwa TI Linear mode conversion of Langmuir/z mode waves to radiation: Averaged energy conversion efficiencies, polarization, and applications to Earth's continuum radiation SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE linear mode conversion; plasma waves; radio emission; planetary continuum radiation; magnetopause; plasmapause ID TERRESTRIAL MYRIAMETRIC RADIATION; NONTHERMAL CONTINUUM; ELECTROMAGNETIC-RADIATION; GEOTAIL OBSERVATIONS; ELECTROSTATIC-WAVES; MAGNETIZED PLASMA; DENSITY PROFILE; RADIO EMISSIONS; O-MODE; MAGNETOSPHERE AB Linear mode conversion (LMC) is the linear transfer of energy from one wave mode to another in a density gradient. It is relevant to planetary continuum radiation, type II and III radio bursts, and ionospheric radio emissions. This paper analyzes LMC by calculating angle-averaged energy (epsilon) and power (epsilon p) conversion efficiencies in both 2-D and 3-D for Langmuir/z mode waves (including upper hybrid waves for perpendicular wave vectors) converting to free-space radiation in turbulent plasmas. The averages are over the distributions of the incoming Langmuir/z mode wave vectors k, density scale lengths L, and angles and , where is the angle between k and the background magnetic field B0 and is the angle between the density gradient delta N0 and B0. The results show that the averaged and unaveraged conversion efficiencies are dependent on , where is the adiabatic index and is related to the electron temperature Te by = Te/mec2. The averaged energy conversion efficiencies are proportional to in 2-D and to ()3/2 in 3-D, whereas the power conversion efficiencies are proportional to ()1/2 in 2-D and in 3-D. The special case of a perpendicular density gradient (approximate to 90 degrees) is considered and used to predict the conversion efficiencies of terrestrial continuum radiation (TCR) in three known source regions: the plasmapause, magnetopause, and the plasma sheet. The observed energy conversion efficiencies are estimated and are found to be consistent with the 2-D and 3-D predicted efficiencies; importantly, these results imply that LMC is a possible generation mechanism for TCR. The polarization of TCR is also predicted: TCR should be produced primarily in the o mode at the plasmapause and in both the o and x modes at the magnetopause and plasma sheet. These predictions are consistent with previous independent predictions and observations. C1 [Schleyer, Fiona; Cairns, Iver H.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Kim, Eun-Hwa] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Schleyer, F (reprint author), Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. EM fiona@physics.usyd.edu.au OI Cairns, Iver/0000-0001-6978-9765 FU Australian Research Council, the School of Physics at the University of Sydney; NASA [NNH09AM531, NNH09AK631, NNH11AQ461, NNH13AV37I]; NSF [ATM0902730]; DOE [DE-AC02-09CH11466] FX We acknowledge funding from the Australian Research Council, the School of Physics at the University of Sydney, NASA grants NNH09AM531, NNH09AK631, NNH11AQ461, and NNH13AV37I, NSF grant ATM0902730, and DOE contract DE-AC02-09CH11466. NR 62 TC 2 Z9 2 U1 1 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2014 VL 119 IS 5 BP 3392 EP 3410 DI 10.1002/2013JA019364 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ4DS UT WOS:000337622100015 ER PT J AU Birn, J Hesse, M AF Birn, J. Hesse, M. TI The substorm current wedge: Further insights from MHD simulations SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE substorm current wedge ID MAGNETOTAIL; ASSOCIATION; FLOWS; FIELD AB Using a recent magnetohydrodynamic simulation of magnetotail dynamics, we further investigate the buildup and evolution of the substorm current wedge (SCW), resulting from flow bursts generated by near-tail reconnection. Each flow burst generates an individual current wedge, which includes the reduction of cross-tail current and the diversion to region 1 (R1)-type field-aligned currents (earthward on the dawn and tailward on the duskside), connecting the tail with the ionosphere. Multiple flow bursts generate initially multiple SCW patterns, which at later times combine to a wider single SCW pattern. The standard SCW model is modified by the addition of several current loops, related to particular magnetic field changes: the increase of Bz in a local equatorial region (dipolarization), the decrease of |Bx|away from the equator (current disruption), and increases in |By|resulting from azimuthally deflected flows. The associated loop currents are found to be of similar magnitude, 0.1-0.3 MA. The combined effect requires the addition of region 2 (R2)-type currents closing in the near tail through dawnward currents but also connecting radially with the R1 currents. The current closure at the inner boundary, taken as a crude proxy of an idealized ionosphere, demonstrates westward currents as postulated in the original SCW picture as well as North-South currents connecting R1- and R2-type currents, which were larger than the westward currents by a factor of almost 2. However, this result should be applied with caution to the ionosphere because of our neglect of finite resistance and Hall effects. C1 [Birn, J.] Space Sci Inst, Boulder, CO 80301 USA. [Birn, J.] Los Alamos Natl Lab, Los Alamos, NM USA. [Hesse, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Birn, J (reprint author), Space Sci Inst, Boulder, CO 80301 USA. EM jbirn@spacescience.org RI NASA MMS, Science Team/J-5393-2013 OI NASA MMS, Science Team/0000-0002-9504-5214 FU NASA [NNX13AD10G, NNX13AD21G]; NSF [1203711] FX This work was performed mostly at Los Alamos National Laboratory under a Guest Scientist agreement, supported by NASA grants NNX13AD10G and NNX13AD21G and NSF grant 1203711. J.B. also acknowledges the hospitality and support of the International Space Science Institute, Bern, Switzerland, and fruitful discussions with Wolfgang Baumjohann and members of the ISSI team on the substorm current wedge. Data necessary to understand, evaluate, replicate, and build upon the reported research will be made available upon request. NR 23 TC 15 Z9 15 U1 0 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2014 VL 119 IS 5 BP 3503 EP 3513 DI 10.1002/2014JA019863 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ4DS UT WOS:000337622100022 ER PT J AU Birn, J Runov, A Hesse, M AF Birn, J. Runov, A. Hesse, M. TI Energetic electrons in dipolarization events: Spatial properties and anisotropy SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE electron acceleration; dipolarization fronts; injections ID TEST PARTICLE ORBITS; GEOSYNCHRONOUS OBSERVATIONS; MAGNETOTAIL; ACCELERATION; SUBSTORMS; SIMULATIONS; INJECTIONS; TRANSPORT; DISTRIBUTIONS; ENERGIZATION AB Using the electromagnetic fields of an MHD simulation of magnetotail reconnection, flow bursts, and dipolarization, we further investigate the acceleration of electrons to suprathermal energies. Particular emphasis is on spatial properties and anisotropies as functions of energy and time. The simulation results are compared with Time History of Events and Macroscale Interactions during Substorms observations. The test particle approach successfully reproduces several observed injection features and puts them into a context of spatial maps of the injection region(s): a dominance of perpendicular anisotropies farther down the tail and closer to the equatorial plane, an increasing importance of parallel anisotropy closer to Earth and at higher latitudes, a drop in energy fluxes at energies below approximate to 10keV, coinciding with the plasma density drop, together with increases at higher energy, a triple peak structure of flux increases near 0 degrees, 90 degrees, and 180 degrees, and a tendency of flux increases to extend to higher energy closer to Earth and at lower latitudes. We identified the plasma sheet boundary layers and adjacent lobes as a main source region for both increased and decreased energetic electron fluxes, related to the different effects of adiabatic acceleration at high and low energies. The simulated anisotropies tend to exceed the observed ones, particularly for perpendicular fluxes at high energies. The most plausible reason is that the MHD simulation lacks the effects of anisotropy-driven microinstabilities and waves, which would reduce anisotropies. C1 [Birn, J.] Space Sci Inst, Boulder, CO 80301 USA. [Birn, J.] Los Alamos Natl Lab, Los Alamos, NM USA. [Runov, A.] Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA USA. [Hesse, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Birn, J (reprint author), Space Sci Inst, Boulder, CO 80301 USA. EM jbirn@spacescience.org RI NASA MMS, Science Team/J-5393-2013 OI NASA MMS, Science Team/0000-0002-9504-5214 FU U.S. Department of Energy; NASA [NNX13AD10G, NNX13AD21G, NAS5-0299, NNX13AF81G]; NSF [1203711]; DLR [50 OC 0302]; International Space Science Institute Bern, Switzerland FX The simulation work was performed at Los Alamos under the auspices of the U.S. Department of Energy, supported by NASA grants NNX13AD10G and NNX13AD21G and NSF grant 1203711. THEMIS data analysis was supported by NASA grants NAS5-0299 and NNX13AF81G. We thank V. Angelopoulos for use of data from the THEMIS Mission, C. W. Carlson and J.P. McFadden for use of ESA data, D. Larson and R. P. Lin for use of SST data, D. L. Turner and P. Cruce for help with SST data calibration, and K.-H. Glassmeier, U. Auster, and W. Baumjohann for the use of FGM data provided with financial support through the DLR contract 50 OC 0302. We are grateful to the hospitality and support by the International Space Science Institute Bern, Switzerland, and the fruitful discussions with members of the ISSI working group. NR 37 TC 12 Z9 12 U1 0 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2014 VL 119 IS 5 BP 3604 EP 3616 DI 10.1002/2013JA019738 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ4DS UT WOS:000337622100029 ER PT J AU Shashurin, A Zhuang, T Teel, G Keidar, M Kundrapu, M Loverich, J Beilis, II Raitses, Y AF Shashurin, A. Zhuang, T. Teel, G. Keidar, M. Kundrapu, M. Loverich, J. Beilis, I. I. Raitses, Y. TI Laboratory Modeling of the Plasma Layer at Hypersonic Flight SO JOURNAL OF SPACECRAFT AND ROCKETS LA English DT Article ID ARC CATHODE SPOTS; ANODE VACUUM-ARC; ION FLUX AB A simple approach to modeling the plasma layer similar to that appearing in the vicinity of a hypersonic vehicle is demonstrated in a laboratory experiment. This approach is based on the use of a hypersonic jet from a cathodic arc plasma. Another critical element of this laboratory experiment is a blunt body made from a fairly thin foil of refractory material. In experiments, this blunt body is heated by the plasma jet to a temperature sufficiently high to ensure evaporation of surface deposits produced by the metallic plasma jet. This process mimics reflection of gas flow from the hypersonic vehicle in a real flight. Two-dimensional distributions of the hypersonic plasma flow around the blunt body were measured using electrostatic Langmuir probes. Measured plasma density was typically 10(12) cm(-3), which is close to the values measured for real hypersonic flight. The demonstrated laboratory experiment can be used to validate numerical codes for simulating hypersonic flight and to conduct ground-based tests for efficiency validation of various radio communication blackout mitigation techniques. C1 [Shashurin, A.; Zhuang, T.; Teel, G.; Keidar, M.] George Washington Univ, Dept Mech & Aerosp Engn, Washington, DC 20052 USA. [Kundrapu, M.; Loverich, J.] Tech X Corp, USim Dev Team, Boulder, CO 80303 USA. [Beilis, I. I.] Tel Aviv Univ, Dept Interdisciplinary Studies, IL-69978 Tel Aviv, Israel. [Raitses, Y.] Princeton Plasma Phys Lab, Plasma Technol & Off Site Res Program, Princeton, NJ 08543 USA. RP Shashurin, A (reprint author), George Washington Univ, Dept Mech & Aerosp Engn, Washington, DC 20052 USA. RI Kundrapu, Madhusudhan/D-3795-2015 FU U.S. Air Force Office of Scientific Research Small Business Technology Transfer (STTR) Phase II [FA9550-12-C-0039] FX This work was supported by the U.S. Air Force Office of Scientific Research Small Business Technology Transfer (STTR) Phase II award FA9550-12-C-0039. NR 36 TC 5 Z9 5 U1 0 U2 9 PU AMER INST AERONAUTICS ASTRONAUTICS PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0022-4650 EI 1533-6794 J9 J SPACECRAFT ROCKETS JI J. Spacecr. Rockets PD MAY-JUN PY 2014 VL 51 IS 3 BP 838 EP 846 DI 10.2514/1.A32771 PG 9 WC Engineering, Aerospace SC Engineering GA AJ2NV UT WOS:000337495500016 ER PT J AU Mehta, PM Walker, A McLaughlin, CA Koller, J AF Mehta, Piyush M. Walker, Andrew McLaughlin, Craig A. Koller, Josef TI Comparing Physical Drag Coefficients Computed Using Different Gas-Surface Interaction Models SO JOURNAL OF SPACECRAFT AND ROCKETS LA English DT Article ID ENERGY-ACCOMMODATION COEFFICIENTS; MONTE-CARLO METHOD; ATMOSPHERIC DENSITY; IMPLEMENTATION; FLOW AB Drag coefficient is a major source of uncertainty in calculating the aerodynamic forces on satellites in low Earth orbit. Closed-form solutions are available for simple geometries under the assumption of free molecular flow; however, most satellites have complex geometries, and a more sophisticated method of calculating the drag coefficient is needed. This work builds toward modeling physical drag coefficients using the direct simulation Monte Carlo method capable of accurately modeling flow shadowing and concave geometries. The direct simulation three-dimensional visual program and the direct simulation Monte Carlo analysis code are used to compare the effects of two separate gas surface interaction models: diffuse reflection with incomplete accommodation and quasi-specular Cercignani-Lampis-Lord models. Results show that the two gas surface interaction models compare well at altitudes below similar to 500 km during solar maximum conditions and below 400 km during solar minimum conditions. The difference in drag coefficient of a sphere at similar to 800 km calculated using the two gas-surface interaction models is similar to 6% during solar maximum and increases to similar to 10% during solar minimum. The difference in drag coefficient of the GRACE satellite computed using the two gas surface interaction models at similar to 500 km differs by similar to 15% during solar minimum conditions and by similar to 2-3% during solar maximum conditions. C1 [Mehta, Piyush M.; Walker, Andrew; Koller, Josef] Los Alamos Natl Lab, Intelligence & Space Res ISR 1, Los Alamos, NM 87544 USA. [McLaughlin, Craig A.] Univ Kansas, Dept Aerosp Engn, Lawrence, KS 66045 USA. RP Mehta, PM (reprint author), Los Alamos Natl Lab, Intelligence & Space Res ISR 1, POB 1663, Los Alamos, NM 87544 USA. OI Walker, Andrew/0000-0002-7890-1779 FU U.S. Department of Energy through the Los Alamos National Laboratory/Laboratory Directed Research and Development program as part of the Integrated Modeling of Perturbations in Atmospheres for Conjunction Tracking project; U.S. Department of Defense Experimental Program to Stimulate Competitive Research [FA9550-10-1-0038] FX Funding for this work was provided by the U.S. Department of Energy through the Los Alamos National Laboratory/Laboratory Directed Research and Development program as part of the Integrated Modeling of Perturbations in Atmospheres for Conjunction Tracking project. Part of the funding was provided by the U.S. Department of Defense Experimental Program to Stimulate Competitive Research grant FA9550-10-1-0038 administered by the U.S. Air Force Office of Scientific Research. The authors would like to thank Eric Sutton for providing the drag coefficient data for GRACE. The authors would also like to thank Vivek Ram, graduate student at the University of Kansas, for his help with developing the high-fidelity GRACE CAD model. NR 46 TC 9 Z9 9 U1 2 U2 13 PU AMER INST AERONAUTICS ASTRONAUTICS PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0022-4650 EI 1533-6794 J9 J SPACECRAFT ROCKETS JI J. Spacecr. Rockets PD MAY-JUN PY 2014 VL 51 IS 3 BP 873 EP 883 DI 10.2514/1.A32566 PG 11 WC Engineering, Aerospace SC Engineering GA AJ2NV UT WOS:000337495500019 ER PT J AU Avci, S Chmaissem, O Allred, JM Rosenkranz, S Eremin, I Chubukov, AV Bugaris, DE Chung, DY Kanatzidis, MG Castellan, JP Schlueter, JA Claus, H Khalyavin, DD Manuel, P Daoud-Aladine, A Osborn, R AF Avci, S. Chmaissem, O. Allred, J. M. Rosenkranz, S. Eremin, I. Chubukov, A. V. Bugaris, D. E. Chung, D. Y. Kanatzidis, M. G. Castellan, J. -P Schlueter, J. A. Claus, H. Khalyavin, D. D. Manuel, P. Daoud-Aladine, A. Osborn, R. TI Magnetically driven suppression of nematic order in an iron-based superconductor SO NATURE COMMUNICATIONS LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; TRANSITION AB A theory of superconductivity in the iron-based materials requires an understanding of the phase diagram of the normal state. In these compounds, superconductivity emerges when stripe spin density wave (SDW) order is suppressed by doping, pressure or atomic disorder. This magnetic order is often pre-empted by nematic order, whose origin is yet to be resolved. One scenario is that nematic order is driven by orbital ordering of the iron 3d electrons that triggers stripe SDW order. Another is that magnetic interactions produce a spin-nematic phase, which then induces orbital order. Here we report the observation by neutron powder diffraction of an additional fourfold-symmetric phase in Ba1-xNaxFe2As2 close to the suppression of SDW order, which is consistent with the predictions of magnetically driven models of nematic order. C1 [Avci, S.; Chmaissem, O.; Allred, J. M.; Rosenkranz, S.; Bugaris, D. E.; Chung, D. Y.; Kanatzidis, M. G.; Castellan, J. -P; Schlueter, J. A.; Claus, H.; Osborn, R.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Chmaissem, O.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Eremin, I.] Ruhr Univ Bochum, Inst Theoret Phys 3, D-44801 Bochum, Germany. [Chubukov, A. V.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kanatzidis, M. G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Khalyavin, D. D.; Manuel, P.; Daoud-Aladine, A.] Rutherford Appleton Lab, ISIS Pulsed Neutron & Muon Facil, Didcot OX11 0QX, Oxon, England. RP Osborn, R (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ROsborn@anl.gov RI Rosenkranz, Stephan/E-4672-2011; Allred, Jared/N-4719-2014; Eremin, Ilya /M-2079-2016; Khalyavin, Dmitry/E-4335-2017 OI Rosenkranz, Stephan/0000-0002-5659-0383; Allred, Jared/0000-0002-5953-300X; Eremin, Ilya /0000-0003-0557-8015; Khalyavin, Dmitry/0000-0002-6724-7695 FU U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division [DE-FG02-ER46900]; DFG [SPP 1458, ER 463/5]; German Academic Exchange Service (DAAD PPP USA) [57051534] FX We are thankful to J. Knolle, R. Fernandes, J. Schmalian, R. Moessner and V. Stanev for useful discussions. This work was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division (S.A., O.C., J.A., S.R., D.E.B., D.Y.C., M.G.K., J.-P.C., J.A.S., H.C., R.O.), which also supported A.V.C. under grant #DE-FG02-ER46900 (A.V.C.). I.E. acknowledges financial support from the DFG under priority programme SPP 1458 (ER 463/5) and the German Academic Exchange Service (DAAD PPP USA No. 57051534). NR 37 TC 53 Z9 53 U1 11 U2 78 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3845 DI 10.1038/ncomms4845 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0VE UT WOS:000337373500007 PM 24848521 ER PT J AU Collins, L Jesse, S Kilpatrick, JI Tselev, A Varenyk, O Okatan, MB Weber, SAL Kumar, A Balke, N Kalinin, SV Rodriguez, BJ AF Collins, Liam Jesse, Stephen Kilpatrick, Jason I. Tselev, Alexander Varenyk, Oleksandr Okatan, M. Baris Weber, Stefan A. L. Kumar, Amit Balke, Nina Kalinin, Sergei V. Rodriguez, Brian J. TI Probing charge screening dynamics and electrochemical processes at the solid-liquid interface with electrochemical force microscopy SO NATURE COMMUNICATIONS LA English DT Article ID AQUEOUS-SOLUTIONS; CORROSION C1 [Collins, Liam; Rodriguez, Brian J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Collins, Liam; Kilpatrick, Jason I.; Weber, Stefan A. L.; Rodriguez, Brian J.] Univ Coll Dublin, Conway Inst Biomol & Biomed Res, Dublin 4, Ireland. [Jesse, Stephen; Tselev, Alexander; Okatan, M. Baris; Kumar, Amit; Balke, Nina; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Varenyk, Oleksandr] Taras Shevchenko Natl Univ Kyiv, Radiophys Fac, UA-03022 Kiev, Ukraine. RP Rodriguez, BJ (reprint author), Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. EM brian.rodriguez@ucd.ie RI Tselev, Alexander/L-8579-2015; Kumar, Amit/C-9662-2012; Balke, Nina/Q-2505-2015; Collins, Liam/A-3833-2016; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; Okatan, M. Baris/E-1913-2016; Weber, Stefan/F-1508-2013 OI Kilpatrick, Jason/0000-0002-8675-4262; Tselev, Alexander/0000-0002-0098-6696; Kumar, Amit/0000-0002-1194-5531; Balke, Nina/0000-0001-5865-5892; Collins, Liam/0000-0003-4946-9195; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Okatan, M. Baris/0000-0002-9421-7846; Weber, Stefan/0000-0003-3052-326X FU Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy [CNMS2012-036, CNMS2013-339]; Alexander von Humboldt Foundation FX This publication has emanated from research conducted with the financial support of UCD Research and NANOREMEDIES, which is funded under the Programme for Research in Third Level Institutions Cycle 5 and co-funded by the European Regional Development Fund. This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy (CNMS2012-036 and CNMS2013-339). S. A. L. W. acknowledges support from the Alexander von Humboldt Foundation. B. J. R. is grateful to S. P. Jarvis for insightful discussions. NR 37 TC 19 Z9 19 U1 11 U2 86 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3871 DI 10.1038/ncomms4871 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2QL UT WOS:000337503800015 PM 24846328 ER PT J AU Gao, P Britson, J Nelson, CT Jokisaari, JR Duan, C Trassin, M Baek, SH Guo, H Li, LZ Wang, YR Chu, YH Minor, AM Eom, CB Ramesh, R Chen, LQ Pan, XQ AF Gao, Peng Britson, Jason Nelson, Christopher T. Jokisaari, Jacob R. Duan, Chen Trassin, Morgan Baek, Seung-Hyub Guo, Hua Li, Linze Wang, Yiran Chu, Ying-Hao Minor, Andrew M. Eom, Chang-Beom Ramesh, Ramamoorthy Chen, Long-Qing Pan, Xiaoqing TI Ferroelastic domain switching dynamics under electrical and mechanical excitations SO NATURE COMMUNICATIONS LA English DT Article ID FERROELECTRIC THIN-FILMS; 90-DEGREES DOMAINS; DISLOCATIONS; DISPLACEMENT; SIMULATIONS; RESOLUTION; STABILITY; TITANATE; STRAIN; WALLS AB In thin film ferroelectric devices, switching of ferroelastic domains can significantly enhance electromechanical response. Previous studies have shown disagreement regarding the mobility or immobility of ferroelastic domain walls, indicating that switching behaviour strongly depends on specific microstructures in ferroelectric systems. Here we study the switching dynamics of individual ferroelastic domains in thin Pb(Zr-0.2, Ti-0.8)O-3 films under electrical and mechanical excitations by using in situ transmission electron microscopy and phase-field modelling. We find that ferroelastic domains can be effectively and permanently stabilized by dislocations at the substrate interface while similar domains at free surfaces without pinning dislocations can be removed by either electric or stress fields. For both electrical and mechanical switching, ferroelastic switching is found to occur most readily at the highly active needle points in ferroelastic domains. Our results provide new insights into the understanding of polarization switching dynamics as well as the engineering of ferroelectric devices. C1 [Gao, Peng; Nelson, Christopher T.; Jokisaari, Jacob R.; Li, Linze; Wang, Yiran; Pan, Xiaoqing] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. [Britson, Jason; Duan, Chen; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Trassin, Morgan; Chu, Ying-Hao; Minor, Andrew M.; Ramesh, Ramamoorthy] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Eom, Chang-Beom] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Guo, Hua; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Pan, XQ (reprint author), Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. EM panx@umich.edu RI Eom, Chang-Beom/I-5567-2014; Gao, Peng/B-4675-2012; Foundry, Molecular/G-9968-2014; Ying-Hao, Chu/A-4204-2008 OI Ying-Hao, Chu/0000-0002-3435-9084 FU Department of Energy (DOE) [DE-FG02-07ER46416]; National Science Foundation [DMR-0820404, DMR/MRI-0723032]; Army Research Office [W911NF-10-1-0362]; DOE [DE-FG02-07ER46417]; NSF [DMR-0820404, DMR-1210588]; National Center for Electron Microscopy at Lawrence Berkeley National Laboratory under the DOE [DE-AC02-05CH11231] FX The work at the University of Michigan was supported by the Department of Energy (DOE) under the Grant DE-FG02-07ER46416 and partially by the National Science Foundation under Grants DMR-0820404 (J.R.J.) and DMR/MRI-0723032 (TEM instrument). The work at University of Wisconsin-Madison was supported by the Army Research Office under Grant number W911NF-10-1-0362. The work at Penn State University was supported by the DOE under the Grant DE-FG02-07ER46417 and partially by the NSF through Grants DMR-0820404 and DMR-1210588 (C.D.). We also acknowledge the National Center for Electron Microscopy at Lawrence Berkeley National Laboratory for their support under the DOE Grant DE-AC02-05CH11231 for user facilities. NR 42 TC 24 Z9 24 U1 10 U2 135 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3801 DI 10.1038/ncomms4801 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0US UT WOS:000337372200012 PM 24787035 ER PT J AU Hsieh, CH Ding, SD Erdem, OF Crouthers, DJ Liu, TB McCrory, CCL Lubitz, W Popescu, CV Reibenspies, JH Hall, MB Darensbourg, MY AF Hsieh, Chung-Hung Ding, Shengda Erdem, Oezlen F. Crouthers, Danielle J. Liu, Tianbiao McCrory, Charles C. L. Lubitz, Wolfgang Popescu, Codrina V. Reibenspies, Joseph H. Hall, Michael B. Darensbourg, Marcetta Y. TI Redox active iron nitrosyl units in proton reduction electrocatalysis SO NATURE COMMUNICATIONS LA English DT Article ID N-HETEROCYCLIC CARBENE; ELECTRONIC-STRUCTURE; H-CLUSTER; COMPLEXES; HYDROGENASE; SITE; FE; ACTIVATION; LIGANDS; SUBSITE AB Base metal, molecular catalysts for the fundamental process of conversion of protons and electrons to dihydrogen, remain a substantial synthetic goal related to a sustainable energy future. Here we report a diiron complex with bridging thiolates in the butterfly shape of the 2Fe2S core of the [FeFe]-hydrogenase active site but with nitrosyl rather than carbonyl or cyanide ligands. This binuclear [(NO)Fe(N2S2)Fe(NO)(2)](+) complex maintains structural integrity in two redox levels; it consists of a (N2S2)Fe(NO) complex (N2S2 = N,N'-bis(2-mercaptoethyl)-1,4-diazacycloheptane) that serves as redox active metallodithiolato bidentate ligand to a redox active dinitrosyl iron unit, Fe(NO)(2). Experimental and theoretical methods demonstrate the accommodation of redox levels in both components of the complex, each involving electronically versatile nitrosyl ligands. An interplay of orbital mixing between the Fe(NO) and Fe(NO)(2) sites and within the iron nitrosyl bonds in each moiety is revealed, accounting for the interactions that facilitate electron uptake, storage and proton reduction. C1 [Hsieh, Chung-Hung; Ding, Shengda; Crouthers, Danielle J.; Reibenspies, Joseph H.; Hall, Michael B.; Darensbourg, Marcetta Y.] Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA. [Erdem, Oezlen F.; Lubitz, Wolfgang] Max Planck Inst Chem Energy Convers, D-45470 Mulheim, Germany. [Liu, Tianbiao] Ctr Mol Electrocatalysis, Pacific NW Natl Lab, Richland, WA 99354 USA. [McCrory, Charles C. L.] CALTECH, Joint Ctr Artificial Photosynth, Pasadena, CA 91125 USA. [Popescu, Codrina V.] Ursinus Coll, Dept Chem, Collegeville, PA 19426 USA. RP Darensbourg, MY (reprint author), Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA. EM marcetta@mail.chem.tamu.edu RI Darensbourg, Marcetta/O-5093-2014; Liu, Tianbiao/A-3390-2011; OI Darensbourg, Marcetta/0000-0002-0070-2075; Hall, Michael B./0000-0003-3263-3219 FU National Science Foundation [CHE-1266097, CHE-0910552, CHE-0956779]; Welch Foundation [A-0924, A-0648]; EU/Energy Network Project SOLAR-H2 [212508]; Max Planck Society; DOE Innovation Hub through the Office of Science of the US Department of Energy [DE-SC0004993] FX We are grateful for financial support from the National Science Foundation (CHE-1266097 to M.Y.D., CHE-0910552 to M. B. H. and CHE-0956779 to C.V.P.) and the R.A. Welch Foundation (A-0924 to M.Y.D. and A-0648 to M.B.H.). We acknowledge Gudrun Klihm for EPR technical support and financial support from the EU/Energy Network Project SOLAR-H2 (FP7 contract 212508) and the Max Planck Society (to O.F.E. and W.L.). Bulk electrolysis measurements are based in part on work performed at the Joint Center for Artificial Photosynthesis, a DOE Innovation Hub, supported through the Office of Science of the US Department of Energy under Award Number DE-SC0004993. NR 45 TC 8 Z9 8 U1 4 U2 69 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3684 DI 10.1038/ncomms4684 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0RJ UT WOS:000337363100001 PM 24785411 ER PT J AU Jimenez-Martinez, R Kennedy, DJ Rosenbluh, M Donley, EA Knappe, S Seltzer, SJ Ring, HL Bajaj, VS Kitching, J AF Jimenez-Martinez, Ricardo Kennedy, Daniel J. Rosenbluh, Michael Donley, Elizabeth A. Knappe, Svenja Seltzer, Scott J. Ring, Hattie L. Bajaj, Vikram S. Kitching, John TI Optical hyperpolarization and NMR detection of Xe-129 on a microfluidic chip SO NATURE COMMUNICATIONS LA English DT Article ID NUCLEAR-MAGNETIC-RESONANCE; POLARIZED NOBLE-GASES; SPIN-EXCHANGE; REMOTE DETECTION; ATOMIC CLOCKS; MRI; RUBIDIUM; XENON AB Optically hyperpolarized Xe-129 gas has become a powerful contrast agent in nuclear magnetic resonance (NMR) spectroscopy and imaging, with applications ranging from studies of the human lung to the targeted detection of biomolecules. Equally attractive is its potential use to enhance the sensitivity of microfluidic NMR experiments, in which small sample volumes yield poor sensitivity. Unfortunately, most Xe-129 polarization systems are large and non-portable. Here we present a microfabricated chip that optically polarizes Xe-129 gas. We have achieved Xe-129 polarizations >0.5% at flow rates of several microlitres per second, compatible with typical microfluidic applications. We employ in situ optical magnetometry to sensitively detect and characterize the Xe-129 polarization at magnetic fields of 1 mu T. We construct the device using standard microfabrication techniques, which will facilitate its integration with existing microfluidic platforms. This device may enable the implementation of highly sensitive Xe-129 NMR in compact, low-cost, portable devices. C1 [Jimenez-Martinez, Ricardo; Donley, Elizabeth A.; Knappe, Svenja; Kitching, John] NIST, Boulder, CO 80305 USA. [Jimenez-Martinez, Ricardo] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Kennedy, Daniel J.; Seltzer, Scott J.; Ring, Hattie L.; Bajaj, Vikram S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Kennedy, Daniel J.; Seltzer, Scott J.; Ring, Hattie L.; Bajaj, Vikram S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Rosenbluh, Michael] Bar Ilan Univ, Jack & Pearl Resnick Inst Adv Technol, Dept Phys, IL-52900 Ramat Gan, Israel. RP Bajaj, VS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM vsbajaj@lbl.gov; john.kitching@nist.gov OI Kennedy, Daniel/0000-0001-7186-7443; Rosenbluh, Michael/0000-0002-9150-4129 FU National Institute of Standards and Technology (NIST); agency of the U.S. government; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-05CH11231]; Roberto Rocca Education Program FX We thank S. Schima for help with the fabrication of the device, E. Pratt and K. Stupic for useful comments on the manuscript, A. Pines for helpful discussions and L. Jimenez for help in the preparation of Fig. 1. This work is a contribution of the National Institute of Standards and Technology (NIST), an agency of the U.S. government, and is not subject to copyright. Research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under contract No. DE-AC02-05CH11231 (D.J.K., S.J.S., H.L.R. and V.S.B.). R.J.M. was supported in part by the Roberto Rocca Education Program. NR 31 TC 8 Z9 8 U1 4 U2 50 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3908 DI 10.1038/ncomms4908 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2QP UT WOS:000337504400004 PM 24844396 ER PT J AU Lee, Y Lo, SH Chen, CQ Sun, H Chung, DY Chasapis, TC Uher, C Dravid, VP Kanatzidis, MG AF Lee, Yeseul Lo, Shih-Han Chen, Changqiang Sun, Hui Chung, Duck-Young Chasapis, Thomas C. Uher, Ctirad Dravid, Vinayak P. Kanatzidis, Mercouri G. TI Contrasting role of antimony and bismuth dopants on the thermoelectric performance of lead selenide SO NATURE COMMUNICATIONS LA English DT Article ID P-TYPE PBSE; NANOSTRUCTURED THERMOELECTRICS; FIGURE; MERIT; EFFICIENCY; ELEMENTS; PBTE; CHALCOGENIDES; ENHANCEMENT; SYSTEMS AB Increasing the conversion efficiency of thermoelectric materials is a key scientific driver behind a worldwide effort to enable heat to electricity power generation at competitive cost. Here we report an increased performance for antimony-doped lead selenide with a thermoelectric figure of merit of similar to 1.5 at 800 K. This is in sharp contrast to bismuth doped lead selenide, which reaches a figure of merit of < 1. Substituting antimony or bismuth for lead achieves maximum power factors between similar to 23-27 mu Wcm(-1) K-2 at temperatures above 400 K. The addition of small amounts (similar to 0.25 mol%) of antimony generates extensive nanoscale precipitates, whereas comparable amounts of bismuth results in very few or no precipitates. The antimony-rich precipitates are endotaxial in lead selenide, and appear remarkably effective in reducing the lattice thermal conductivity. The corresponding bismuth-containing samples exhibit smaller reduction in lattice thermal conductivity. C1 [Lee, Yeseul; Chasapis, Thomas C.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Lo, Shih-Han; Chen, Changqiang; Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Sun, Hui; Uher, Ctirad] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Chung, Duck-Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Dravid, VP (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM v-dravid@northwestern.edu; m-kanatzidis@northwestern.edu RI Dravid, Vinayak/B-6688-2009; Sun, Hui/D-3411-2014 OI Sun, Hui/0000-0002-9745-3510 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [ED-SC 0001054]; U.S Department of Energy, Office of Science [DE-AC02-06CH11357]; NSF-NSEC; NSF-MRSEC; Keck Foundation; State of Illinois; Northwestern University FX This material is based upon work supported as part of the Revolutionary Materials for Solid State Energy Conversion, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. ED-SC 0001054. This work was also supported by the U.S Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. TEM work was performed in the EPIC/NIFTI/Keck-II facility of the NUANCE Center at Northwestern University. The NUANCE Center is supported by NSF-NSEC, NSF-MRSEC, Keck Foundation, the State of Illinois, and Northwestern University. NR 47 TC 15 Z9 15 U1 14 U2 117 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3640 DI 10.1038/ncomms4640 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0RD UT WOS:000337362400001 PM 24784991 ER PT J AU McCabe, RJ Beyerlein, IJ Carpenter, JS Mara, NA AF McCabe, Rodney J. Beyerlein, Irene J. Carpenter, John S. Mara, Nathan A. TI The critical role of grain orientation and applied stress in nanoscale twinning SO NATURE COMMUNICATIONS LA English DT Article ID NANOCRYSTALLINE AL; DEFORMATION TWINS; DISLOCATION NUCLEATION; FCC METALS; TEMPERATURE; MECHANISM; SLIP; DIFFRACTION; COMPOSITES; INTERFACES AB Numerous recent studies have focused on the effects of grain size on deformation twinning in nanocrystalline fcc metals. However, grain size alone cannot explain many observed twinning characteristics. Here we show that the propensity for twinning is dependent on the applied stress, grain orientation and stacking fault energy. The lone factor for twinning dependent on grain size is the stress necessary to nucleate partial dislocations from a boundary. We use bulk processing of controlled nanostructures coupled with unique orientation mapping at the nanoscale to show the profound effect of crystal orientation on deformation twinning. Our theoretical model reveals an orientation-dependent critical threshold stress for twinning, which is presented in the form of a generalized twinnability map. Our findings provide a newfound orientation-based explanation for the grain size effect: as grain size decreases the applied stress needed for further deformation increases, thereby allowing more orientations to reach the threshold stress for twinning. C1 [McCabe, Rodney J.; Carpenter, John S.; Mara, Nathan A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Mara, Nathan A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, MPA CINT Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP McCabe, RJ (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, MST 6 Mat Technol Met, Los Alamos, NM 87545 USA. EM rmccabe@lanl.gov RI Mara, Nathan/J-4509-2014; OI McCabe, Rodney /0000-0002-6684-7410; Carpenter, John/0000-0001-8821-043X FU Los Alamos National Laboratory Directed Research and Development (LDRD) Project [DR20110029]; Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; Los Alamos National Security LLC under DOE [DE-AC52-06NA25396] FX This work is supported by the Los Alamos National Laboratory Directed Research and Development (LDRD) Project DR20110029 and the Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number 2008LANL1026. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. Electron Microscopy was performed at the Los Alamos Electron Microscopy Laboratory. NR 40 TC 11 Z9 11 U1 1 U2 68 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3806 DI 10.1038/ncomms4806 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0US UT WOS:000337372200017 PM 24811868 ER PT J AU Wu, CH Arju, N Kelp, G Fan, JA Dominguez, J Gonzales, E Tutuc, E Brener, I Shvets, G AF Wu, Chihhui Arju, Nihal Kelp, Glen Fan, Jonathan A. Dominguez, Jason Gonzales, Edward Tutuc, Emanuel Brener, Igal Shvets, Gennady TI Spectrally selective chiral silicon metasurfaces based on infrared Fano resonances SO NATURE COMMUNICATIONS LA English DT Article ID PHOTONIC CRYSTALS; METAMATERIALS; GRAPHENE; LIGHT; ENHANCEMENT; MONOLAYERS; MOLECULES; INDEX AB Metamaterials and metasurfaces represent a remarkably versatile platform for light manipulation, biological and chemical sensing, and nonlinear optics. Many of these applications rely on the resonant nature of metamaterials, which is the basis for extreme spectrally selective concentration of optical energy in the near field. In addition, metamaterial-based optical devices lend themselves to considerable miniaturization because of their subwavelength features. This additional advantage sets metamaterials apart from their predecessors, photonic crystals, which achieve spectral selectivity through their long-range periodicity. Unfortunately, spectral selectivity of the overwhelming majority of metamaterials that are made of metals is severely limited by high plasmonic losses. Here we propose and demonstrate Fano-resonant all-dielectric metasurfaces supporting optical resonances with quality factors Q > 100 that are based on CMOS-compatible materials: silicon and its oxide. We also demonstrate that these infrared metasurfaces exhibit extreme planar chirality, opening exciting possibilities for efficient ultrathin circular polarizers and narrow-band thermal emitters of circularly polarized radiation. C1 [Wu, Chihhui; Arju, Nihal; Kelp, Glen; Shvets, Gennady] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Fan, Jonathan A.] Stanford Univ, Dept Elect Engn, Ginzton Lab, Stanford, CA 94305 USA. [Dominguez, Jason; Gonzales, Edward; Brener, Igal] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Gonzales, Edward] Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Tutuc, Emanuel] Univ Texas Austin, Dept Elect & Comp Engn, Austin, TX 78712 USA. RP Shvets, G (reprint author), Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. EM gena@physics.utexas.edu FU Office of Naval Research (ONR) Award [N00014-13-10837]; National Science Foundation (NSF) Award [DMR 1120923]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Office of Naval Research (ONR) Award N00014-13-10837 and by the National Science Foundation (NSF) Award DMR 1120923. This work was performed, in part, at the Center for Integrated Nanotechnologies, an US Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by the Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 69 TC 76 Z9 76 U1 35 U2 247 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3892 DI 10.1038/ncomms4892 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2QL UT WOS:000337503800036 PM 24861488 ER PT J AU Joshi, TH Sangiorgio, S Bernstein, A Foxe, M Hagmann, C Jovanovic, I Kazkaz, K Mozin, V Norman, EB Pereverzev, SV Rebassoo, F Sorensen, P AF Joshi, T. H. Sangiorgio, S. Bernstein, A. Foxe, M. Hagmann, C. Jovanovic, I. Kazkaz, K. Mozin, V. Norman, E. B. Pereverzev, S. V. Rebassoo, F. Sorensen, P. TI First Measurement of the Ionization Yield of Nuclear Recoils in Liquid Argon SO PHYSICAL REVIEW LETTERS LA English DT Article ID NEUTRAL-CURRENT; XENON; DETECTOR AB This Letter details a measurement of the ionization yield (Q(y)) of 6.7 keV Ar-40 atoms stopping in a liquid argon detector. The Q(y) of 3.6-6.3 detected e(-)/keV, for applied electric fields in the range 240-2130 V/cm, is encouraging for the use of this detector medium to search for the signals from hypothetical dark matter particle interactions and from coherent elastic neutrino-nucleus scattering. A significant dependence of Q(y) on the applied electric field is observed and explained in the context of ion recombination. C1 [Joshi, T. H.; Norman, E. B.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Joshi, T. H.; Sangiorgio, S.; Bernstein, A.; Foxe, M.; Hagmann, C.; Kazkaz, K.; Mozin, V.; Norman, E. B.; Pereverzev, S. V.; Rebassoo, F.; Sorensen, P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Foxe, M.; Jovanovic, I.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. RP Joshi, TH (reprint author), Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. EM thjoshi@berkeley.edu FU U.S. Department of Homeland Security, Domestic Nuclear Detection Office; U.S. Department of Defense, Defense Threat Reduction Agency; LDRD program [LDRD 13-FS-005]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We would like to thank G. Bench and T. Brown for assistance and support throughout the beam measurements and J. Coleman and K. Mavrokoridis for previous detector contributions. We would like to acknowledge the Lawrence Scholars Program and the Department of Homeland Security for funding T. H. J.'s research. A portion of M. F.'s research was performed under the Nuclear Forensics Graduate Fellowship Program, which is sponsored by the U.S. Department of Homeland Security, Domestic Nuclear Detection Office, and the U.S. Department of Defense, Defense Threat Reduction Agency. We gratefully acknowledge the LDRD program (LDRD 13-FS-005) at LLNL. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. LLNL-Article-766160. NR 22 TC 9 Z9 9 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 1 PY 2014 VL 112 IS 17 AR 171303 DI 10.1103/PhysRevLett.112.171303 PG 5 WC Physics, Multidisciplinary SC Physics GA AJ5AV UT WOS:000337693600002 PM 24836233 ER PT J AU Khuyagbaatar, J Yakushev, A Dullmann, CE Ackermann, D Andersson, LL Asai, M Block, M Boll, RA Brand, H Cox, DM Dasgupta, M Derkx, X Di Nitto, A Eberhardt, K Even, J Evers, M Fahlander, C Forsberg, U Gates, JM Gharibyan, N Golubev, P Gregorich, KE Hamilton, JH Hartmann, W Herzberg, RD Hessberger, FP Hinde, DJ Hoffmann, J Hollinger, R Hubner, A Jager, E Kindler, B Kratz, JV Krier, J Kurz, N Laatiaoui, M Lahiri, S Lang, R Lommel, B Maiti, M Miernik, K Minami, S Mistry, A Mokry, C Nitsche, H Omtvedt, JP Pang, GK Papadakis, P Renisch, D Roberto, J Rudolph, D Runke, J Rykaczewski, KP Sarmiento, LG Schadel, M Schausten, B Semchenkov, A Shaughnessy, DA Steinegger, P Steiner, J Tereshatov, EE Thorle-Pospiech, P Tinschert, K De Heidenreich, TT Trautmann, N Turler, A Uusitalo, J Ward, DE Wegrzecki, M Wiehl, N Van Cleve, SM Yakusheva, V AF Khuyagbaatar, J. Yakushev, A. Duellmann, Ch. E. Ackermann, D. Andersson, L. -L. Asai, M. Block, M. Boll, R. A. Brand, H. Cox, D. M. Dasgupta, M. Derkx, X. Di Nitto, A. Eberhardt, K. Even, J. Evers, M. Fahlander, C. Forsberg, U. Gates, J. M. Gharibyan, N. Golubev, P. Gregorich, K. E. Hamilton, J. H. Hartmann, W. Herzberg, R. -D. Hessberger, F. P. Hinde, D. J. Hoffmann, J. Hollinger, R. Huebner, A. Jaeger, E. Kindler, B. Kratz, J. V. Krier, J. Kurz, N. Laatiaoui, M. Lahiri, S. Lang, R. Lommel, B. Maiti, M. Miernik, K. Minami, S. Mistry, A. Mokry, C. Nitsche, H. Omtvedt, J. P. Pang, G. K. Papadakis, P. Renisch, D. Roberto, J. Rudolph, D. Runke, J. Rykaczewski, K. P. Sarmiento, L. G. Schaedel, M. Schausten, B. Semchenkov, A. Shaughnessy, D. A. Steinegger, P. Steiner, J. Tereshatov, E. E. Thoerle-Pospiech, P. Tinschert, K. De Heidenreich, T. Torres Trautmann, N. Tuerler, A. Uusitalo, J. Ward, D. E. Wegrzecki, M. Wiehl, N. Van Cleve, S. M. Yakusheva, V. TI Ca-48+Bk-249 Fusion Reaction Leading to Element Z=117: Long-Lived alpha-Decaying (270)Db and Discovery of Lr-266 SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVIEST ELEMENTS; CA-48-INDUCED REACTIONS; SUPERHEAVY NUCLEI; TASCA; SEPARATOR; GSI AB The superheavy element with atomic number Z = 117 was produced as an evaporation residue in the Ca-48 + Bk-249 fusion reaction at the gas-filled recoil separator TASCA at GSI Darmstadt, Germany. The radioactive decay of evaporation residues and their alpha-decay products was studied using a detection setup that allowed measuring decays of single atomic nuclei with half-lives between sub-mu s and a few days. Two decay chains comprising seven a decays and a spontaneous fission each were identified and are assigned to the isotope (294)117 and its decay products. A hitherto unknown alpha-decay branch in (270)Db (Z = 105) was observed, which populated the new isotope Lr-266 (Z = 103). The identification of the long-lived (T-1/2 = 1.0(-0.4)(+1.9) h) alpha-emitter (270)Db marks an important step towards the observation of even more long-lived nuclei of superheavy elements located on an "island of stability." C1 [Khuyagbaatar, J.; Duellmann, Ch. E.; Andersson, L. -L.; Derkx, X.; Eberhardt, K.; Even, J.; Hessberger, F. P.; Laatiaoui, M.; Mokry, C.; Thoerle-Pospiech, P.; Wiehl, N.; Yakusheva, V.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Khuyagbaatar, J.; Yakushev, A.; Duellmann, Ch. E.; Ackermann, D.; Block, M.; Brand, H.; Hartmann, W.; Hessberger, F. P.; Hoffmann, J.; Hollinger, R.; Huebner, A.; Jaeger, E.; Kindler, B.; Krier, J.; Kurz, N.; Lang, R.; Lommel, B.; Minami, S.; Runke, J.; Schaedel, M.; Schausten, B.; Steiner, J.; Tinschert, K.; De Heidenreich, T. Torres] GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. [Duellmann, Ch. E.; Derkx, X.; Di Nitto, A.; Eberhardt, K.; Kratz, J. V.; Mokry, C.; Renisch, D.; Thoerle-Pospiech, P.; Trautmann, N.; Wiehl, N.] Johannes Gutenberg Univ Mainz, D-55099 Mainz, Germany. [Asai, M.; Schaedel, M.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Boll, R. A.; Miernik, K.; Roberto, J.; Rykaczewski, K. P.; Van Cleve, S. M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Cox, D. M.; Herzberg, R. -D.; Mistry, A.; Papadakis, P.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Dasgupta, M.; Evers, M.; Hinde, D. J.] Australian Natl Univ, Canberra, ACT 0200, Australia. [Fahlander, C.; Forsberg, U.; Golubev, P.; Rudolph, D.; Sarmiento, L. G.; Ward, D. E.] Lund Univ, S-22100 Lund, Sweden. [Gates, J. M.; Gregorich, K. E.; Nitsche, H.; Pang, G. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Gharibyan, N.; Shaughnessy, D. A.; Tereshatov, E. E.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Hamilton, J. H.] Vanderbilt Univ, Nashville, TN 37235 USA. [Lahiri, S.; Maiti, M.] Saha Inst Nucl Phys, Kolkata 700064, India. [Omtvedt, J. P.; Semchenkov, A.] Univ Oslo, N-0315 Oslo, Norway. [Papadakis, P.; Uusitalo, J.] Univ Jyvaskyla, SF-40351 Jyvaskyla, Finland. [Steinegger, P.; Tuerler, A.] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Steinegger, P.; Tuerler, A.] Univ Bern, CH-3012 Bern, Switzerland. [Wegrzecki, M.] Inst Electr Mat Technol, PL-02668 Warsaw, Poland. RP Khuyagbaatar, J (reprint author), Helmholtz Inst Mainz, D-55099 Mainz, Germany. EM J.Khuyagbaatar@gsi.de RI Steinegger, Patrick/M-5531-2013; Rudolph, Dirk/D-4259-2009; Block, Michael/I-2782-2015; Hinde, David/D-5051-2013; Dasgupta, Mahananda/D-6951-2013; Evers, Maurits/B-3672-2011; Evers, Maurits/A-9985-2016; Boll, Rose/C-4138-2016; Even, Julia/K-1186-2016; Turler, Andreas/D-3913-2014; Laatiaoui, Mustapha/Q-6295-2016 OI Steinegger, Patrick/0000-0002-5054-0924; Rudolph, Dirk/0000-0003-1199-3055; Block, Michael/0000-0001-9282-8347; Hinde, David/0000-0002-4595-0742; Dasgupta, Mahananda/0000-0002-1677-9421; Evers, Maurits/0000-0003-1252-7603; Boll, Rose/0000-0003-2507-4834; Even, Julia/0000-0002-6314-9094; Turler, Andreas/0000-0002-4274-1056; Laatiaoui, Mustapha/0000-0003-0105-8303 FU German BMBF [05P12UMFNE]; Helmholtz association [VH-NG-723]; Australian Research Council; Swedish Research Council; U.S. Department of Energy by LLNL [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [11-ERD-011]; Helmholtz Institute Mainz; Office of Science, U.S. Department of Energy; U.S. DOE [DE-AC05-00OR22725]; Vanderbilt DOE [DE-FG05-88ER40407]; UK Science and Technology Funding Council (STFC); U.S. Department of Energy, Office of Science, Nuclear Physics, Low Energy Physics Program, through the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX We are grateful for GSI's ECR ion source and UNILAC staff, and the Experimental Electronics department for their continuous support of the experiment. This work was financially supported in part by the German BMBF (05P12UMFNE), the Helmholtz association (VH-NG-723), the Australian and Swedish Research Councils, the U.S. Department of Energy by LLNL (DE-AC52-07NA27344), the Laboratory Directed Research and Development Program at LLNL (11-ERD-011) and the Helmholtz Institute Mainz. This work was co-sponsored by the Office of Science, U.S. Department of Energy, and supported under U.S. DOE Grant No. DE-AC05-00OR22725, and at Vanderbilt DOE Grant No. DE-FG05-88ER40407, and the UK Science and Technology Funding Council (STFC). J. M. G., K. E. G., and H. N. were supported by the U.S. Department of Energy, Office of Science, Nuclear Physics, Low Energy Physics Program, through the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. NR 37 TC 68 Z9 69 U1 7 U2 51 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 1 PY 2014 VL 112 IS 17 AR 172501 DI 10.1103/PhysRevLett.112.172501 PG 5 WC Physics, Multidisciplinary SC Physics GA AJ5AV UT WOS:000337693600003 PM 24836239 ER PT J AU Hla, SW AF Hla, Saw Wai TI Atom-by-atom assembly SO REPORTS ON PROGRESS IN PHYSICS LA English DT Review DE STM; atom manipulation; atomic level assembly ID SCANNING TUNNELING MICROSCOPE; CONTROLLED LATERAL MANIPULATION; QUANTUM CORRALS; SINGLE-ATOM; METAL-SURFACES; ROOM-TEMPERATURE; STM MANIPULATION; VERTICAL MANIPULATION; ELECTRONIC-PROPERTIES; FORCE MICROSCOPY AB Atomic manipulation using a scanning tunneling microscope (STM) tip enables the construction of quantum structures on an atom-by-atom basis, as well as the investigation of the electronic and dynamical properties of individual atoms on a one-atom-at-a-time basis. An STM is not only an instrument that is used to 'see' individual atoms by means of imaging, but is also a tool that is used to 'touch' and 'take' the atoms, or to 'hear' their movements. Therefore, the STM can be considered as the 'eyes', 'hands' and 'ears' of the scientists, connecting our macroscopic world to the exciting atomic world. In this article, various STM atom manipulation schemes and their example applications are described. The future directions of atomic level assembly on surfaces using scanning probe tips are also discussed. C1 [Hla, Saw Wai] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60661 USA. [Hla, Saw Wai] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. RP Hla, SW (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Lemont, IL 60661 USA. FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-FG02-02ER46012, DE-AC02-06CH11357] FX We acknowledge financial support by the US Department of Energy, Office of Science, Office of Basic Energy Sciences grant, DE-FG02-02ER46012. Use of the Center for Nanoscale Materials was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract no DE-AC02-06CH11357. NR 160 TC 9 Z9 9 U1 17 U2 92 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0034-4885 EI 1361-6633 J9 REP PROG PHYS JI Rep. Prog. Phys. PD MAY PY 2014 VL 77 IS 5 AR 056502 DI 10.1088/0034-4885/77/5/056502 PG 16 WC Physics, Multidisciplinary SC Physics GA AJ0NS UT WOS:000337351800002 PM 24787453 ER PT J AU He, QP Chen, JH Keffer, DJ Joy, DC AF He, Qianping Chen, Jihua Keffer, David J. Joy, David C. TI Electron Beam Induced Radiation Damage in the Catalyst Layer of a Proton Exchange Membrane Fuel Cell SO SCANNING LA English DT Article DE STEM; EELS; radiation damage; catalyst layer; PEMFC ID PERFORMANCE; NAFION; MICROSTRUCTURE; PEMFC; TEM AB Electron microscopy is an essential tool for the evaluation of microstructure and properties of the catalyst layer (CL) of proton exchange membrane fuel cells (PEMFCs). However, electron microscopy has one unavoidable drawback, which is radiation damage. Samples suffer temporary or permanent change of the surface or bulk structure under radiation damage, which can cause ambiguity in the characterization of the sample. To better understand the mechanism of radiation damage of CL samples and to be able to separate the morphological features intrinsic to the material from the consequences of electron radiation damage, a series of experiments based on high-angle annular dark-field-scanning transmission scanning microscope (HAADF-STEM), energy filtering transmission scanning microscope (EFTEM), and electron energy loss spectrum (EELS) are conducted. It is observed that for thin samples (0.3-1 times l), increasing the incident beam energy can mitigate the radiation damage. Platinum nanoparticles in the CL sample facilitate the radiation damage. The radiation damage of the catalyst sample starts from the interface of Pt/C or defective thin edge and primarily occurs in the form of mass loss accompanied by atomic displacement and edge curl. These results provide important insights on the mechanism of CL radiation damage. Possible strategies of mitigating the radiation damage are provided. (C) 2013 Wiley Periodicals, Inc. C1 [He, Qianping] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Chen, Jihua; Joy, David C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Keffer, David J.; Joy, David C.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Joy, DC (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM djoy@utk.edu RI Chen, Jihua/F-1417-2011; OI Chen, Jihua/0000-0001-6879-5936; Keffer, David/0000-0002-6246-0286 FU National Science Foundation [DGE-0801470, OCI 07-11134.5] FX Contract grant sponsor: National Science Foundation; contract grant numbers: DGE-0801470, OCI 07-11134.5. NR 28 TC 0 Z9 0 U1 1 U2 18 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0161-0457 EI 1932-8745 J9 SCANNING JI Scanning PD MAY-JUN PY 2014 VL 36 IS 3 BP 338 EP 346 DI 10.1002/sca.21117 PG 9 WC Instruments & Instrumentation; Microscopy SC Instruments & Instrumentation; Microscopy GA AJ4YD UT WOS:000337685000009 PM 23897710 ER PT J AU Lo, WC Sposito, G Chu, HH AF Lo, Wei-Cheng Sposito, Garrison Chu, Hsiuhua TI Poroelastic Theory of Consolidation in Unsaturated Soils SO VADOSE ZONE JOURNAL LA English DT Article ID 2 IMMISCIBLE FLUIDS; ONE-DIMENSIONAL CONSOLIDATION; ELASTIC POROUS-MEDIA; HYDRAULIC CONDUCTIVITY; WAVE-PROPAGATION; EQUATION; CLAYS AB The theory of poroelastic behavior in a deformable porous medium containing two immiscible, viscous, compressible fluids was applied to the three-dimensional consolidation of unsaturated soils. Three coupled partial differential equations were developed that feature the displacement vector of the solid phase and the excess pore water and air pressures as dependent variables. These equations generalize the classic Biot consolidation model, which applies to saturated soils, with effective stress emerging naturally from a pure compliance formulation of the relation between stress and strain. Under uniaxial strain and constant total compaction stress, the equations simplify to two coupled diffusion equations for the excess pore water and air pressures. Analytical solutions describing the response to instantaneous compression under both permeable and semipermeable boundary drainage conditions were obtained using the Laplace transform. Numerical calculations of pore water pressure, effective stress, and total settlement were made for a soil with clay texture as a representative example. The results show that excess pore water pressure dissipates faster at higher initial water content, leading to higher effective stress. The loading efficiency also was found to be highly sensitive to initial water saturation. C1 [Lo, Wei-Cheng] Natl Cheng Kung Univ, Dept Hydraul & Ocean Engn, Tainan 701, Taiwan. [Sposito, Garrison] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Sposito, Garrison] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Chu, Hsiuhua] Ind Technol Res Inst, Cloud Serv Technol Ctr, Tainan 701, Taiwan. RP Lo, WC (reprint author), Natl Cheng Kung Univ, Dept Hydraul & Ocean Engn, Tainan 701, Taiwan. EM lowc@mail.ncku.edu.tw FU National Science Council, Taiwan [NSC 101-2625-M-006-007] FX Gratitude is expressed for financial support to the National Science Council, Taiwan, under Contract no. NSC 101-2625-M-006-007. NR 31 TC 3 Z9 3 U1 4 U2 24 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD MAY PY 2014 VL 13 IS 5 DI 10.2136/vzj2013.07.0117 PG 12 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA AJ0NL UT WOS:000337351000013 ER PT J AU Yang, GX Bowling, LC AF Yang, Guoxiang Bowling, Laura C. TI Detection of changes in hydrologic system memory associated with urbanization in the Great Lakes region SO WATER RESOURCES RESEARCH LA English DT Article ID UNITED-STATES; HURST PHENOMENON; ENERGY FLUXES; UPPER MIDWEST; TIME-SERIES; MODEL; SCALE; PRECIPITATION; VARIABILITY; SIMULATION AB The change of long memory with urbanization in a regional hydrologic system was investigated using both stochastic time series models and a physically based hydrologic model. Based on observed streamflow at five USGS gauge stations in the Great Lakes region, objective fractional autoregressive integrated moving average (FARIMA) model identification and estimation procedures were used for daily streamflow. The recently improved Variable Infiltration Capacity (VIC) model with urban representation was applied to simulate the water and energy response in 16 basins in the region with various degrees of urbanization. The VIC model was driven by different years' land use/cover maps, including a year 1992 base map, and year 2010 and 2030 maps projected by the Land Transformation Model. The ability of the VIC model to capture long memory of observed daily streamflow was evaluated before applying the FARIMA model to all 16 basins. Overall, the northern portion of the domain generally has larger long-term hydrologic dependence than the southern portion. Simulated streamflow statistics show that the long memory in the hydrologic system has decreased with urbanization. In order to interpret the long memory change with urbanization from a physical point of view, spectral analysis was conducted to examine the spectrum change of soil moisture content with urbanization. The decrease in simulated streamflow long memory relates to the decreased low-frequency power and amplitude of soil moisture in the deep soil layer. The long-term response of surface water systems to urbanization should be considered by water resources and urban planners. C1 [Yang, Guoxiang; Bowling, Laura C.] Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. RP Yang, GX (reprint author), US EPA, Oak Ridge Inst Sci & Educ Fellow, Water Supply & Water Resources Div, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA. EM yang.gavin@epa.gov RI Yang, Guoxiang/I-5619-2012; Bowling, Laura/B-6963-2013 OI Bowling, Laura/0000-0002-1439-3154 FU NASA [NNG06GC40G] FX We gratefully acknowledge the support of the NASA land cover land use change program (grant NNG06GC40G). We would like to thank Henning Rust, Salvatore Grimaldi, and three anonymous reviewers whose comments led to significant improvement of the manuscript. The land use/cover maps projected from the Land Transformation Model provided by Bryan C. Pijanowski's group at Purdue University are appreciated. NR 42 TC 4 Z9 6 U1 2 U2 27 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD MAY PY 2014 VL 50 IS 5 BP 3750 EP 3763 DI 10.1002/2014WR015339 PG 14 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA AJ4UN UT WOS:000337672900009 ER PT J AU Shi, XQ Ye, M Curtis, GP Miller, GL Meyer, PD Kohler, M Yabusaki, S Wu, JC AF Shi, Xiaoqing Ye, Ming Curtis, Gary P. Miller, Geoffery L. Meyer, Philip D. Kohler, Matthias Yabusaki, Steve Wu, Jichun TI Assessment of parametric uncertainty for groundwater reactive transport modeling SO WATER RESOURCES RESEARCH LA English DT Article ID MONTE-CARLO-SIMULATION; INVERSE PROBLEM; EQUILIBRIUM CALCULATIONS; DIFFERENTIAL EVOLUTION; GLOBAL OPTIMIZATION; FLOW; IDENTIFICATION; PROPAGATION; CALIBRATION; HYDROLOGY AB The validity of using Gaussian assumptions for model residuals in uncertainty quantification of a groundwater reactive transport model was evaluated in this study. Least squares regression methods explicitly assume Gaussian residuals, and the assumption leads to Gaussian likelihood functions, model parameters, and model predictions. While the Bayesian methods do not explicitly require the Gaussian assumption, Gaussian residuals are widely used. This paper shows that the residuals of the reactive transport model are non-Gaussian, heteroscedastic, and correlated in time; characterizing them requires using a generalized likelihood function such as the formal generalized likelihood function developed by Schoups and Vrugt (2010). For the surface complexation model considered in this study for simulating uranium reactive transport in groundwater, parametric uncertainty is quantified using the least squares regression methods and Bayesian methods with both Gaussian and formal generalized likelihood functions. While the least squares methods and Bayesian methods with Gaussian likelihood function produce similar Gaussian parameter distributions, the parameter distributions of Bayesian uncertainty quantification using the formal generalized likelihood function are non-Gaussian. In addition, predictive performance of formal generalized likelihood function is superior to that of least squares regression and Bayesian methods with Gaussian likelihood function. The Bayesian uncertainty quantification is conducted using the differential evolution adaptive metropolis (DREAM((ZS))) algorithm; as a Markov chain Monte Carlo (MCMC) method, it is a robust tool for quantifying uncertainty in groundwater reactive transport models. For the surface complexation model, the regression-based local sensitivity analysis and Morris-and DREAM((ZS))-based global sensitivity analysis yield almost identical ranking of parameter importance. The uncertainty analysis may help select appropriate likelihood functions, improve model calibration, and reduce predictive uncertainty in other groundwater reactive transport and environmental modeling. C1 [Shi, Xiaoqing; Wu, Jichun] Nanjing Univ, Sch Earth Sci & Engn, Minist Educ, Key Lab Surficial Geochem, Nanjing 210008, Jiangsu, Peoples R China. [Shi, Xiaoqing; Ye, Ming; Miller, Geoffery L.] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. [Curtis, Gary P.; Kohler, Matthias] US Geol Survey, Menlo Pk, CA 94025 USA. [Meyer, Philip D.; Yabusaki, Steve] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Ye, M (reprint author), Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. EM mye@fsu.edu RI Ye, Ming/A-5964-2008; Shi, Xiaoqing/G-4439-2010; OI Shi, Xiaoqing/0000-0002-5074-8856; Meyer, Philip/0000-0002-8714-4693 FU National Natural Science Foundation of China [51328902, 41172206, 41172207]; NSF-EAR [0911074]; DOE-SBR [DE-SC0002687, DE-SC0000801]; DOE Early Career Award [DE-SC0008272]; ORAU/ORNL High Performance Computing Grant FX This work was supported in part by National Natural Science Foundation of China grants 51328902, 41172206, and 41172207, NSF-EAR grant 0911074, DOE-SBR grants DE-SC0002687 and DE-SC0000801, DOE Early Career Award DE-SC0008272, and ORAU/ORNL High Performance Computing Grant. The first author was employed by the Florida State University when conducting part of this research. The authors thank Jasper Vrugt for providing the DREAM(zs) code, and Bruno Mendes, and David Draper for discussion on comparison of confidence and credible intervals. We also thank G.-H. Crystal Ng and the anonymous reviewers for improving the manuscript. NR 89 TC 16 Z9 18 U1 8 U2 48 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD MAY PY 2014 VL 50 IS 5 BP 4416 EP 4439 DI 10.1002/2013WR013755 PG 24 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA AJ4UN UT WOS:000337672900045 ER PT J AU Keitz, BK Yu, CJ Long, JR Ameloot, R AF Keitz, Benjamin K. Yu, Chung Jui Long, Jeffrey R. Ameloot, Rob TI Lithographic Deposition of Patterned Metal-Organic Framework Coatings Using a Photobase Generator SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE copper; metal-organic frameworks; photochemistry; thin films ID SELF-ASSEMBLED MONOLAYERS; THIN-FILMS; CHEMICAL-DETECTION; ORIENTED GROWTH; CRYSTALS; MOF; TETRAPHENYLBORATE; CU-3(BTC)(2); IRRADIATION; FABRICATION AB A photobase generator was used to induce metal-organic framework (MOF) nucleation upon UV irradiation. This method was further developed into a simple, one-step method for depositing patterned MOF films. Furthermore, the ability of our method to coat a single substrate with MOF films having different chemical compositions is illustrated. The method is an important step towards integrating MOF deposition with existing lithographic techniques and the incorporation of these materials into sensors and other electronic devices. C1 [Keitz, Benjamin K.; Yu, Chung Jui; Long, Jeffrey R.; Ameloot, Rob] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. RP Ameloot, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. EM rob.ameloot@biw.kuleuven.be RI Ameloot, Rob/C-9175-2013 OI Ameloot, Rob/0000-0003-3178-5480 FU Research Foundation Flanders (FWO Vlaanderen) FX We thank Dr. Bill Flounders and Dr. Sia Parsa from the UC Berkeley Marvell Nanofabrication Laboratory for helpful discussions and the use of photomasks. We are grateful to Miguel Gonzalez and Dr. Alan Yiu for assistance with photography, optical microscopy, and profilometry measurements. Nick Kornienko is acknowledged for assistance with electron microscopy and EDX analysis. R. A. thanks the Research Foundation Flanders (FWO Vlaanderen) for a post-doctoral fellowship. NR 37 TC 12 Z9 12 U1 11 U2 97 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAY PY 2014 VL 53 IS 22 BP 5561 EP 5565 DI 10.1002/anie.201400580 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA AI7DE UT WOS:000337041600008 PM 24719391 ER PT J AU Carver, JC Epperly, T AF Carver, Jeffrey C. Epperly, Tom TI Software Engineering for Computational Science and Engineering INTRODUCTION SO COMPUTING IN SCIENCE & ENGINEERING LA English DT Editorial Material ID INTERNATIONAL WORKSHOP C1 [Carver, Jeffrey C.] Univ Alabama, Dept Comp Sci, Tuscaloosa, AL 35487 USA. [Epperly, Tom] Lawrence Livermore Natl Lab, Comp Sci Grp, Ctr Appl Sci Comp, Livermore, CA USA. RP Carver, JC (reprint author), Univ Alabama, Dept Comp Sci, Tuscaloosa, AL 35487 USA. EM carver@cs.ua.edu; epperly2@llnl.gov NR 5 TC 1 Z9 1 U1 0 U2 1 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1521-9615 EI 1558-366X J9 COMPUT SCI ENG JI Comput. Sci. Eng. PD MAY-JUN PY 2014 VL 16 IS 3 BP 6 EP 9 PG 4 WC Computer Science, Interdisciplinary Applications SC Computer Science GA AI9PB UT WOS:000337263400001 ER PT J AU Nanthaamornphong, A Carver, JC Morris, K Michelsen, HA Rouson, DWI AF Nanthaamornphong, Aziz Carver, Jeffrey C. Morris, Karla Michelsen, Hope A. Rouson, Damian W. I. TI Building CLiiME via Test-Driven Development: A Case Study SO COMPUTING IN SCIENCE & ENGINEERING LA English DT Article ID SOFTWARE-DEVELOPMENT AB The Community Laser-Induced Incandescence Modeling Environment (CLiiME) project used the agile approaches of test-driven development and refactoring to implement a collaborative model infrastructure for its researchers to use, modify, and extend. As the project's results show, using agile methods can offer several benefits for software development in the CSE community. C1 [Nanthaamornphong, Aziz; Carver, Jeffrey C.] Univ Alabama, Dept Comp Sci, Tuscaloosa, AL 35487 USA. [Morris, Karla] Sandia Natl Labs, Livermore, CA 94550 USA. [Morris, Karla] Sandia Natl Labs, Reacting Flow Res Dept, Livermore, CA 94550 USA. [Michelsen, Hope A.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. [Rouson, Damian W. I.] Stanford Univ, Stanford, CA 94305 USA. RP Nanthaamornphong, A (reprint author), Univ Alabama, Dept Comp Sci, Tuscaloosa, AL 35487 USA. EM ananthaamornphong@crimson.ua.edu; carver@cs.ua.edu; knmorri@sandia.gov; hamiche@sandia.gov; sourcery@rouson.net FU US Department of Energy's Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences; National Nuclear Security Administration [DE-AC04-94-AL85000]; US National Science Foundation [124887] FX The US Department of Energy's Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, provided funding for this work. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000. Jeffrey Carver and Aziz Nanthaamornphong also acknowledge support from the US National Science Foundation under grant number 124887. NR 12 TC 1 Z9 1 U1 0 U2 6 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1521-9615 EI 1558-366X J9 COMPUT SCI ENG JI Comput. Sci. Eng. PD MAY-JUN PY 2014 VL 16 IS 3 BP 36 EP 46 PG 11 WC Computer Science, Interdisciplinary Applications SC Computer Science GA AI9PB UT WOS:000337263400005 ER PT J AU Guedj, J Yu, J Levi, M Li, B Kern, S Naoumov, NV Perelson, AS AF Guedj, Jeremie Yu, Jing Levi, Micha Li, Bin Kern, Steven Naoumov, Nikolai V. Perelson, Alan S. TI Modeling Viral Kinetics and Treatment Outcome During Alisporivir Interferon-Free Treatment in Hepatitis C Virus Genotype 2 and 3 Patients SO HEPATOLOGY LA English DT Article ID CYCLOPHILIN INHIBITORS; INFECTION; TELAPREVIR; RIBAVIRIN; RESISTANCE; DYNAMICS; THERAPY; AGENTS; RNA AB Alisporivir (ALV) is a cyclophilin inhibitor with pan-genotypic activity against hepatitis C virus (HCV). Here, we characterize the viral kinetics observed in 249 patients infected with HCV genotypes 2 or 3 and treated for 6 weeks with different doses of ALV with or without ribavirin (RBV). We use this model to predict the effects of treatment duration and different doses of ALV plus RBV on sustained virologic response (SVR). Continuous viral decline was observed in 214 (86%) patients that could be well described by the model. All doses led to a high level of antiviral effectiveness equal to 0.98, 0.96, and 0.90 in patients treated with 1,000, 800, and 600 mg of ALV once-daily, respectively. Patients that received RBV had a significantly faster rate of viral decline, which was attributed to an enhanced loss rate of infected cells, (mean =0.35 d(-1) vs. 0.21 d(-1) in patients +/- RBV, respectively; P=0.0001). The remaining 35 patients (14%) had a suboptimal response with flat or increasing levels of HCV RNA after 1 week of treatment, which was associated with ALV monotherapy, high body weight, and low RBV levels in patients that received ALV plus RBV. Assuming full compliance and the same proportion of suboptimal responders, the model predicted 71% and 79% SVR after ALV 400 mg with RBV 400 mg twice-daily for 24 and 36 weeks, respectively. The model predicted that response-guided treatment could allow a reduction in mean treatment duration to 25.3 weeks and attain a 78.6% SVR rate. Conclusion: ALV plus RBV may represent an effective IFN-free treatment that is predicted to achieve high SVR rates in patients with HCV genotype 2 or 3 infection. C1 [Guedj, Jeremie] INSERM, UMR 1137, IAME, F-75018 Paris, France. [Guedj, Jeremie; Perelson, Alan S.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Yu, Jing; Li, Bin] Novartis Inst Biomed Res, Cambridge, MA USA. [Levi, Micha] Novartis Pharmaceut, E Hanover, NJ USA. [Kern, Steven; Naoumov, Nikolai V.] Novartis Pharma AG, Basel, Switzerland. RP Perelson, AS (reprint author), Los Alamos Natl Lab, MS-K710,POB 1663, Los Alamos, NM 87545 USA. EM asp@lanl.gov RI Guedj, Jeremie/A-6842-2017 OI Guedj, Jeremie/0000-0002-5534-5482 FU Novartis; Roche FX Potential conflict of interest: J.G. has consulted for Gilead; A. S. P. has received research grants from Novartis and Roche and has consulted for Merck, Gilead, Achillion, Bristol-Myers Squibb, Progenics, and Santaris Pharmaceuticals; S. K. was employed by Novartis when this work was done (currently at the Bill and Melinda Gates Foundation); and J.Y., M. L., B. L., and N.V.N. are Novartis employees. NR 22 TC 13 Z9 13 U1 0 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0270-9139 EI 1527-3350 J9 HEPATOLOGY JI Hepatology PD MAY PY 2014 VL 59 IS 5 BP 1706 EP 1714 DI 10.1002/hep.26989 PG 9 WC Gastroenterology & Hepatology SC Gastroenterology & Hepatology GA AI9TA UT WOS:000337278400013 PM 24375768 ER PT J AU Branch, DW Wojciechowski, KE Olsson, RH AF Branch, Darren W. Wojciechowski, Kenneth E. Olsson, Roy H., III TI Elucidating the Origin of Spurious Modes in Aluminum Nitride Microresonators Using a 2-D Finite-Element Model SO IEEE TRANSACTIONS ON ULTRASONICS FERROELECTRICS AND FREQUENCY CONTROL LA English DT Article ID INTERDIGITAL TRANSDUCERS; EFFECTIVE PERMITTIVITY; WAVE-PROPAGATION; GREENS-FUNCTION; LAMB MODE; SAW; RESONATORS; MEDIA AB In this work, an approach has been developed to predict the location of large spurious modes in the resonant response of aluminum nitride (AlN) microelectromechanical systems (MEMS) resonators over a wide range of desired operating frequencies. This addresses significant challenges in the design of more complex AlN devices, namely the prediction and elimination of spurious modes in the resonance response. Using the finite element method (FEM), the dispersion curves at wavelengths ranging from 8 to 20 mu m were computed. It was determined that the velocities of symmetric Lamb (S0) and high-order antisymmetric (A) modes overlap at specific wavelengths. A 2-D FEM analysis showed that both the S0 and higher order A modes are mutually excited at a common operating wavelength. From this analysis, the coupling-of-modes (COM) parameters were extracted and used to compute the P-matrix and S-parameters using a 6-port transmission matrix. The P-matrix simulation was able to predict the electrical response of the S0 and nearby spurious modes. This work identified specific wavelength regions where COM has limited accuracy because of mode conversion. In these regions, the reflection (kappa(p)) and transduction (zeta(p)) parameters change rapidly. C1 [Branch, Darren W.] Sandia Natl Labs, Biosensors & Nanomat Dept, Albuquerque, NM 87185 USA. [Wojciechowski, Kenneth E.] Sandia Natl Labs, Adv Microelect & Radiat Effects Dept, Albuquerque, NM 87185 USA. [Wojciechowski, Kenneth E.; Olsson, Roy H., III] Sandia Natl Labs, Adv MEMS Dept, Albuquerque, NM 87185 USA. RP Branch, DW (reprint author), Sandia Natl Labs, Biosensors & Nanomat Dept, POB 5800, Albuquerque, NM 87185 USA. EM dwbranc@sandia.gov FU Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; US Department of Energy's National Nuclear Security Administration [DE-AC 04-94AL85000] FX This work was partially supported by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lock-heed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC 04-94AL85000. NR 24 TC 9 Z9 9 U1 0 U2 12 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-3010 EI 1525-8955 J9 IEEE T ULTRASON FERR JI IEEE Trans. Ultrason. Ferroelectr. Freq. Control PD MAY PY 2014 VL 61 IS 5 BP 729 EP 738 DI 10.1109/TUFFC.2014.2965 PG 10 WC Acoustics; Engineering, Electrical & Electronic SC Acoustics; Engineering GA AI8IY UT WOS:000337157700001 PM 24802295 ER PT J AU Bacmeister, JT Wehner, MF Neale, RB Gettelman, A Hannay, C Lauritzen, PH Caron, JM Truesdale, JE AF Bacmeister, Julio T. Wehner, Michael F. Neale, Richard B. Gettelman, Andrew Hannay, Cecile Lauritzen, Peter H. Caron, Julie M. Truesdale, John E. TI Exploratory High-Resolution Climate Simulations using the Community Atmosphere Model (CAM) SO JOURNAL OF CLIMATE LA English DT Article DE Climate models ID GENERAL-CIRCULATION MODEL; ATLANTIC HURRICANE ACTIVITY; WARM-SEASON PRECIPITATION; TROPICAL CYCLONE ACTIVITY; DYNAMICAL CORE; INTERANNUAL VARIABILITY; PART I; CONVECTION; DATASET; IMPACT AB Extended, high-resolution (0.23 degrees latitude x 0.31 degrees longitude) simulations with Community Atmosphere Model versions 4 and 5 (CAM4 and CAM5) are examined and compared with results from climate simulations conducted at a more typical resolution of 0.9 degrees latitude x 1.25 degrees longitude. Overall, the simulated climate of the high-resolution experiments is not dramatically better than that of their low-resolution counterparts. Improvements appear primarily where topographic effects may be playing a role, including a substantially improved summertime Indian monsoon simulation in CAM4 at high resolution. Significant sensitivity to resolution is found in simulated precipitation over the southeast United States during winter. Some aspects of the simulated seasonal mean precipitation deteriorate notably at high resolution. Prominent among these is an exacerbated Pacific double ITCZ bias in both models. Nevertheless, while large-scale seasonal means are not dramatically better at high resolution, realistic tropical cyclone (TC) distributions are obtained. Some skill in reproducing interannual variability in TC statistics also appears. C1 [Bacmeister, Julio T.; Neale, Richard B.; Gettelman, Andrew; Hannay, Cecile; Lauritzen, Peter H.; Caron, Julie M.; Truesdale, John E.] NCAR, Atmospher Modeling & Predict Sect, Boulder, CO 80301 USA. [Wehner, Michael F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bacmeister, JT (reprint author), NCAR, Atmospher Modeling & Predict Sect, Boulder, CO 80301 USA. EM juliob@ucar.edu FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research; Office of Science of the Department of Energy FX Partial support for this work was provided through the Scientific Discovery through Advanced Computing (SciDAC) program funded by U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research. This research used computing resources of the Oak Ridge Leadership Computing Facility and of the National Energy Research Scientific Computing Center, which are supported by the Office of Science of the Department of Energy. We would also like to thank David Williamson for useful discussions, and three anonymous reviewers for helpful questions and comments on the manuscript. NR 62 TC 50 Z9 51 U1 4 U2 30 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD MAY PY 2014 VL 27 IS 9 BP 3073 EP 3099 DI 10.1175/JCLI-D-13-00387.1 PG 27 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AI9RU UT WOS:000337272700001 ER PT J AU Geng, XL Davatzes, NC Soeder, DJ Torlapati, J Rodriguez, RS Boufadel, MC AF Geng, Xiaolong Davatzes, Nicholas C. Soeder, Daniel J. Torlapati, Jagadish Rodriguez, Rebecca S. Boufadel, Michel C. TI Migration of High-Pressure Air during Gas Well Drilling in the Appalachian Basin SO JOURNAL OF ENVIRONMENTAL ENGINEERING LA English DT Article DE Fractured aquifer; 3D numerical modeling; Air migration; TOUGH2; Air hammer drilling ID HYDRAULIC CONDUCTIVITY; NUMERICAL-SIMULATION; ROCK FRACTURE; NATURAL-GAS; FLUID-FLOW; MODEL; CONTAMINATION; PERMEABILITY; JOINTS; MEDIA AB We present the details of a numerical model simulating the migration of pressurized air used for pneumatic drilling of a well in an aquifer. We used an incident that occurred in West Virginia during June 2012 as a basis for making the simulations realistic. We developed a 3D conceptual model using the multipurpose model TOUGH2 to simulate the events during this incident. Input parameters for the model were obtained from field measurements, and a number of reasonable assumptions were made for other parameters. Our results showed that compressed air from a drilling well is capable of creating a high pressure gradient in groundwater at hundreds of meters from the drill hole, even if the air leakage from the drilling well occurs in a confined aquifer, and even if the leakage duration is only 2 h. Therefore, one way to prevent the pressure buildup in the surrounding aquifers is through emplacement of observation wells before drilling, which would alert the drillers to any unusual pressure buildup inside the confined aquifer. However, air leakage in unconfined aquifers seems to have a much smaller spatial extent (less than tens of meters). Sensitivity analysis revealed that air pressure, fracture permeability, and injection time are critical parameters for the propagation of air. (C) 2014 American Society of Civil Engineers. C1 [Geng, Xiaolong; Torlapati, Jagadish; Boufadel, Michel C.] New Jersey Inst Technol, Dept Civil & Environm Engn, Newark Coll Engn, Ctr Nat Resources Dev & Protect, Newark, NJ 07102 USA. [Davatzes, Nicholas C.] Temple Univ, Coll Sci & Technol, Philadelphia, PA 19122 USA. [Soeder, Daniel J.; Rodriguez, Rebecca S.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Boufadel, MC (reprint author), New Jersey Inst Technol, Dept Civil & Environm Engn, Newark Coll Engn, Ctr Nat Resources Dev & Protect, Newark, NJ 07102 USA. EM boufadel@gmail.com OI Soeder, Daniel/0000-0003-2248-6235 FU William Penn Foundation; Claneil Foundation FX This project was funded in part by the William Penn Foundation and the Claneil Foundation. However, no endorsement of the results by these organizations should be assumed. NR 47 TC 1 Z9 1 U1 2 U2 9 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 0733-9372 EI 1943-7870 J9 J ENVIRON ENG JI J. Environ. Eng.-ASCE PD MAY PY 2014 VL 140 IS 5 SI SI AR B4014002 DI 10.1061/(ASCE)EE.1943-7870.0000769 PG 10 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AI9FB UT WOS:000337234800005 ER PT J AU Ren, Y Ma, Z Dai, S AF Ren, Yu Ma, Zhen Dai, Sheng TI Nanosize Control on Porous beta-MnO2 and Their Catalytic Activity in CO Oxidation and N2O Decomposition SO MATERIALS LA English DT Article DE mesoporous; pyrolusite; CO oxidation; N2O decomposition; textural properties ID MESOPOROUS MOLECULAR-SIEVES; METAL-OXIDES; LITHIUM BATTERIES; SILICA; REPLICATION; FUNCTIONALIZATION; ADSORPTION; MECHANISM; CO3O4; SIZE AB A major challenge in the synthesis of porous metal oxides is the control of pore size and/or wall thickness that may affect the performance of these materials. Herein, nanoporous beta-MnO2 samples were prepared using different hard templates, e.g., ordered mesoporous silica SBA-15 and KIT-6, disordered mesoporous silica, and colloidal silica. These samples were characterized by Powder X-Ray Diffraction (PXRD), Transmission Electron Microscopy (TEM), and N-2 adsorption-desorption. The pore size distribution of beta-MnO2 was tuned by the different hard templates and their preparation details. Catalytic activities in CO oxidation and N2O decomposition were tested and the mesoporous beta-MnO2 samples demonstrated superior catalytic activities compared with their bulk counterpart. C1 [Ren, Yu] Natl Inst Clean & Low Carbon Energy, Beijing 102211, Peoples R China. [Ren, Yu] Univ St Andrews, Sch Chem, St Andrews KY16 9ST, Fife, Scotland. [Ren, Yu] Univ St Andrews, EaStChem, St Andrews KY16 9ST, Fife, Scotland. [Ma, Zhen] Fudan Univ, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Prev, Shanghai 200433, Peoples R China. [Ma, Zhen; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Ren, Y (reprint author), Natl Inst Clean & Low Carbon Energy, Beijing 102211, Peoples R China. EM renyu3@gmail.com; zhenma@fudan.edu.cn; dais@ornl.gov RI Ma, Zhen/F-1348-2010; Dai, Sheng/K-8411-2015 OI Ma, Zhen/0000-0002-2391-4943; Dai, Sheng/0000-0002-8046-3931 FU National Natural Science Foundation of China [21007011, 21177028]; PhD Programs Foundation of the Ministry of Education in China [20100071120012]; Overseas Returnees Start-Up Research Fund of the Ministry of Education in China; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy [De-AC05-00OR22725]; Oak Ridge National Laboratory FX Zhen Ma acknowledges the financial support by National Natural Science Foundation of China (Grant Nos. 21007011 and 21177028), the PhD Programs Foundation of the Ministry of Education in China (Grant No. 20100071120012), and the Overseas Returnees Start-Up Research Fund of the Ministry of Education in China. Sheng Dai acknowledges the financial support by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy, under contract No. De-AC05-00OR22725 with Oak Ridge National Laboratory managed and operated by UT-Batelle, Limited-Liability Company. NR 28 TC 4 Z9 4 U1 5 U2 73 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 1996-1944 J9 MATERIALS JI Materials PD MAY PY 2014 VL 7 IS 5 BP 3547 EP 3556 DI 10.3390/ma7053547 PG 10 WC Materials Science, Multidisciplinary SC Materials Science GA AI9KF UT WOS:000337250800015 ER PT J AU Ruan, GL Velasco, JI Valles, C Li, ZM Gloria, A Lin, WZ Liu, F AF Ruan, G. L. Velasco, J. I. Valles, C. Li, Z. M. Gloria, A. Lin, W. Z. Liu, F. TI Review: Frontiers of materials science and engineering SO MATERIALS RESEARCH INNOVATIONS LA English DT Editorial Material ID FIBER-REINFORCED POLYMER; MECHANICAL-PROPERTIES; MOLECULAR-DYNAMICS; COMPOSITES; MICROSTRUCTURE; FILM; ORIENTATION; TEMPERATURE; FABRICATION; DESIGN AB Materials science and engineering is one of the hot research topics in the world, which is changing the way we live daily. As a result of this, the 2nd Global Conference on Materials Science and Engineering was held on November 20-22, 2013. During this event, more than 200 attendees discussed the frontiers of materials science and engineering. This editorial highlights some of these papers that present the new frontiers of materials science research in 2013. C1 [Ruan, G. L.; Li, Z. M.] Hubei Univ Sci & Technol, Sch Elect & Informat Engn, Xianning, Peoples R China. [Velasco, J. I.] Tech Univ Catalonia, Dept Mat Sci & Met, Terrassa, Spain. [Valles, C.] Univ Manchester, Sch Mat, Manchester, Lancs, England. [Gloria, A.] Natl Res Council Italy, Inst Composite & Biomed Mat, Naples, Italy. [Lin, W. Z.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Liu, F.] Wuhan Univ, Int Sch Software, Wuhan 430072, Peoples R China. RP Ruan, GL (reprint author), Hubei Univ Sci & Technol, Sch Elect & Informat Engn, Xianning, Peoples R China. EM GLRuan@163.com; liufeng.whu@gmail.com RI Velasco, Jose Ignacio/C-5732-2011 OI Velasco, Jose Ignacio/0000-0003-0331-5270 NR 24 TC 0 Z9 0 U1 2 U2 25 PU MANEY PUBLISHING PI LEEDS PA STE 1C, JOSEPHS WELL, HANOVER WALK, LEEDS LS3 1AB, W YORKS, ENGLAND SN 1432-8917 EI 1433-075X J9 MATER RES INNOV JI Mater. Res. Innov. PD MAY PY 2014 VL 18 SU 2 BP 1 EP 4 DI 10.1179/1432891714Z.000000000633 PG 4 WC Materials Science, Multidisciplinary SC Materials Science GA AI8FZ UT WOS:000337146600001 ER PT J AU Cretnik, S Bernstein, A Shouakar-Stash, O Loffler, F Elsner, M AF Cretnik, Stefan Bernstein, Anat Shouakar-Stash, Orfan Loeffler, Frank Elsner, Martin TI Chlorine Isotope Effects from Isotope Ratio Mass Spectrometry Suggest Intramolecular C-Cl Bond Competition in Trichloroethene (TCE) Reductive Dehalogenation SO MOLECULES LA English DT Article DE reductive dehalogenation; chlorinated ethenes; trichloroethene; biodegradation; organohalide respiration; dechlorination mechanism; regioselectivity; vitamin B-12; reductive dehalogenase ID VINYL-CHLORIDE; DCE ISOMERS; DECHLORINATION; TETRACHLOROETHENE; TRANSFORMATION; FRACTIONATION; COMPLEXES; COBALAMIN; CARBON; IRON AB Chlorinated ethenes are prevalent groundwater contaminants. To better constrain (bio) chemical reaction mechanisms of reductive dechlorination, the position-specificity of reductive trichloroethene (TCE) dehalogenation was investigated. Selective biotransformation reactions (i) of tetrachloroethene (PCE) to TCE in cultures of Desulfitobacterium sp. strain Viet1; and (ii) of TCE to cis-1,2-dichloroethene (cis-DCE) in cultures of Geobacter lovleyi strain SZ were investigated. Compound-average carbon isotope effects were -19.0 parts per thousand +/- 0.9 parts per thousand (PCE) and -12.2 parts per thousand +/- 1.0 parts per thousand (TCE) (95% confidence intervals). Using instrumental advances in chlorine isotope analysis by continuous flow isotope ratio mass spectrometry, compound-average chorine isotope effects were measured for PCE (-5.0 parts per thousand +/- 0.1 parts per thousand) and TCE (-3.6 parts per thousand +/- 0.2 parts per thousand). In addition, position-specific kinetic chlorine isotope effects were determined from fits of reactant and product isotope ratios. In PCE biodegradation, primary chlorine isotope effects were substantially larger (by -16.3 parts per thousand +/- 1.4 parts per thousand (standard error)) than secondary. In TCE biodegradation, in contrast, the product cis-DCE reflected an average isotope effect of -2.4 parts per thousand +/- 0.3 parts per thousand and the product chloride an isotope effect of -6.5 parts per thousand +/- 2.5 parts per thousand, in the original positions of TCE from which the products were formed (95% confidence intervals). A greater difference would be expected for a position-specific reaction (chloride would exclusively reflect a primary isotope effect). These results therefore suggest that both vicinal chlorine substituents of TCE were reactive (intramolecular competition). This finding puts new constraints on mechanistic scenarios and favours either nucleophilic addition by Co(I) or single electron transfer as reductive dehalogenation mechanisms. C1 [Cretnik, Stefan; Bernstein, Anat; Elsner, Martin] Helmholtz Zentrum Munchen, Inst Groundwater Ecol, D-85764 Neuherberg, Germany. [Shouakar-Stash, Orfan] Univ Waterloo, Dept Earth & Environm Sci, Waterloo, ON N2L 3G1, Canada. [Loeffler, Frank] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Loeffler, Frank] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37996 USA. [Loeffler, Frank] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Loeffler, Frank] Oak Ridge Natl Lab, JIBS, Oak Ridge Natl Lab UT ORNL, Oak Ridge, TN 37831 USA. [Loeffler, Frank] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Elsner, M (reprint author), Helmholtz Zentrum Munchen, Inst Groundwater Ecol, Ingolstadter Landstr 1, D-85764 Neuherberg, Germany. EM one_fiftyone@hotmail.com; anatbern@bgu.ac.il; orfan@uwaterloo.ca; frank.loeffler@utk.edu; martin.elsner@helmholtz-muenchen.de RI Elsner, Martin/J-4637-2012; Bernstein, Anat/J-2612-2016 OI Elsner, Martin/0000-0003-4746-9052; FU German Research Foundation (DFG) [EL 266/3-1]; Initiative and Networking Fund of the Helmholtz Association; Minerva Foundation, Max-Planck-Gesellschaft FX We thank Kris McNeill from the ETH Zurich and Stefan Haderlein from University of Tubingen for helpful discussions and critical comments. We further thank Wolfgang zu Castell-Rudenhausen and Michael Hagen from the Institute of Bioinformatics, Helmholtz Zentrum Munich, for helpful initial discussions on alternative approaches to mathematical fitting. This work was supported by the German Research Foundation (DFG), EL 266/3-1, as well as by the Initiative and Networking Fund of the Helmholtz Association. A.B. was supported by a fellowship of the Minerva Foundation, Max-Planck-Gesellschaft. NR 40 TC 10 Z9 10 U1 6 U2 45 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 1420-3049 J9 MOLECULES JI Molecules PD MAY PY 2014 VL 19 IS 5 BP 6450 EP 6473 DI 10.3390/molecules19056450 PG 24 WC Chemistry, Organic SC Chemistry GA AI7WR UT WOS:000337113000063 PM 24853618 ER PT J AU Ethier-Majcher, G St-Jean, P Boso, G Tosi, A Klem, JF Francoeur, S AF Ethier-Majcher, G. St-Jean, P. Boso, G. Tosi, A. Klem, J. F. Francoeur, S. TI Complete quantum control of exciton qubits bound to isoelectronic centres SO NATURE COMMUNICATIONS LA English DT Article ID SINGLE-PHOTON; DOT SPIN; COHERENT CONTROL; ENTANGLEMENT; NITROGEN; STATE AB In recent years, impressive demonstrations related to quantum information processing have been realized. The scalability of quantum interactions between arbitrary qubits within an array remains however a significant hurdle to the practical realization of a quantum computer. Among the proposed ideas to achieve fully scalable quantum processing, the use of photons is appealing because they can mediate long-range quantum interactions and could serve as buses to build quantum networks. Quantum dots or nitrogen-vacancy centres in diamond can be coupled to light, but the former system lacks optical homogeneity while the latter suffers from a low dipole moment, rendering their large-scale interconnection challenging. Here, through the complete quantum control of exciton qubits, we demonstrate that nitrogen isoelectronic centres in GaAs combine both the uniformity and predictability of atomic defects and the dipole moment of semiconductor quantum dots. This establishes isoelectronic centres as a promising platform for quantum information processing. C1 [Ethier-Majcher, G.; St-Jean, P.; Francoeur, S.] Ecole Polytech, Dept Genie Phys, Montreal, PQ H3C 3A7, Canada. [Boso, G.; Tosi, A.] Politecn Milan, Dipartimento Elettron Informaz & Bioingn, I-20133 Milan, Italy. [Klem, J. F.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ethier-Majcher, G (reprint author), Ecole Polytech, Dept Genie Phys, 2900 Boul Edouard Montpetit, Montreal, PQ H3C 3A7, Canada. EM gabriel.ethier-majcher@polymtl.ca; sebastien.francoeur@polymtl.ca RI Tosi, Alberto/J-5275-2012; Francoeur, Sebastien/E-6614-2011 OI Tosi, Alberto/0000-0003-1210-2875; Francoeur, Sebastien/0000-0002-6129-7026 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We would like to thank N. Bertone for initiating contacts between Polytechnique Montreal and Politecnico di Milano. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 34 TC 6 Z9 6 U1 0 U2 16 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3980 DI 10.1038/ncomms4980 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ3BV UT WOS:000337541000001 PM 24875932 ER PT J AU Kis-Papo, T Weig, AR Riley, R Persoh, D Salamov, A Sun, H Lipzen, A Wasser, SP Rambold, G Grigoriev, IV Nevo, E AF Kis-Papo, Tamar Weig, Alfons R. Riley, Robert Persoh, Derek Salamov, Asaf Sun, Hui Lipzen, Anna Wasser, Solomon P. Rambold, Gerhard Grigoriev, Igor V. Nevo, Eviatar TI Genomic adaptations of the halophilic Dead Sea filamentous fungus Eurotium rubrum SO NATURE COMMUNICATIONS LA English DT Article ID PHYLOGENETIC ANALYSIS; PROTEIN FAMILIES; WATER ACTIVITY; TOOL; GENE; SALT; ANNOTATION; PREDICTION; STRESS; LIFE AB The Dead Sea is one of the most hypersaline habitats on Earth. The fungus Eurotium rubrum (Eurotiomycetes) is among the few species able to survive there. Here we highlight its adaptive strategies, based on genome analysis and transcriptome profiling. The 26.2 Mb genome of E. rubrum shows, for example, gains in gene families related to stress response and losses with regard to transport processes. Transcriptome analyses under different salt growth conditions revealed, among other things differentially expressed genes encoding ion and metabolite transporters. Our findings suggest that long-term adaptation to salinity requires cellular and metabolic responses that differ from short-term osmotic stress signalling. The transcriptional response indicates that halophilic E. rubrum actively counteracts the salinity stress. Many of its genes encode for proteins with a significantly higher proportion of acidic amino acid residues. This trait is characteristic of the halophilic prokaryotes as well, supporting the theory of convergent evolution under extreme hypersaline stress. C1 [Kis-Papo, Tamar; Wasser, Solomon P.; Nevo, Eviatar] Univ Haifa, Inst Evolut, IL-3498838 Haifa, Israel. [Weig, Alfons R.; Rambold, Gerhard] Univ Bayreuth, Div Biol, D-95447 Bayreuth, Germany. [Riley, Robert; Salamov, Asaf; Sun, Hui; Lipzen, Anna; Grigoriev, Igor V.] US Dept Energy Joint Genome Inst, Walnut Creek, CA 94598 USA. [Persoh, Derek; Rambold, Gerhard] Univ Bayreuth, Dept Mycol, D-95447 Bayreuth, Germany. [Wasser, Solomon P.] Natl Acad Sci Ukraine, MG Kholodny Inst Bot, UA-01601 Kiev, Ukraine. RP Rambold, G (reprint author), Univ Bayreuth, Div Biol, Univ Str 30, D-95447 Bayreuth, Germany. EM gerhard.rambold@uni-bayreuth.de; ivgrigoriev@lbl.gov; nevo@research.haifa.ac.il RI Persoh, Derek/G-4527-2010; Weig, Alfons/I-5359-2013 OI Persoh, Derek/0000-0001-5561-0189; FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Ancell Teicher Research Foundation for Genetics and Molecular Evolution FX We wish to thank Benjamin A. Horwitz for comments on the manuscript, and Ronald P. de Vries and his colleagues from CBS for their help with the classification of this fungus. The work conducted by the U.S. Department of Energy Joint Genome Institute is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The work conducted at the Institute of Evolution is supported by the Ancell Teicher Research Foundation for Genetics and Molecular Evolution. NR 56 TC 7 Z9 8 U1 4 U2 28 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3745 DI 10.1038/ncomms4745 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0SR UT WOS:000337366800001 PM 24811710 ER PT J AU O'Brien, L Erickson, MJ Spivak, D Ambaye, H Goyette, RJ Lauter, V Crowell, PA Leighton, C AF O'Brien, L. Erickson, M. J. Spivak, D. Ambaye, H. Goyette, R. J. Lauter, V. Crowell, P. A. Leighton, C. TI Kondo physics in non-local metallic spin transport devices SO NATURE COMMUNICATIONS LA English DT Article ID ROOM-TEMPERATURE; MAGNETIC MULTILAYERS; INJECTION; ACCUMULATION; VALVES; MAGNETORESISTANCE; FERROMAGNETISM; ENHANCEMENT; PRECESSION; RESISTANCE AB The non- local spin-valve is pivotal in spintronics, enabling separation of charge and spin currents, disruptive potential applications and the study of pressing problems in the physics of spin injection and relaxation. Primary among these problems is the perplexing non-monotonicity in the temperature-dependent spin accumulation in non-local ferromagnetic/non-magnetic metal structures, where the spin signal decreases at low temperatures. Here we show that this effect is strongly correlated with the ability of the ferromagnetic to form dilute local magnetic moments in the NM. This we achieve by studying a significantly expanded range of ferromagnetic/non-magnetic combinations. We argue that local moments, formed by ferromagnetic/non-magnetic interdiffusion, suppress the injected spin polarization and diffusion length via a manifestation of the Kondo effect, thus explaining all observations. We further show that this suppression can be completely quenched, even at interfaces that are highly susceptible to the effect, by insertion of a thin non-moment-supporting interlayer. C1 [O'Brien, L.; Leighton, C.] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [O'Brien, L.] Univ Cambridge, Cavendish Lab, Dept Phys, Cambridge CB3 0HE, England. [Erickson, M. J.; Spivak, D.; Crowell, P. A.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Ambaye, H.; Goyette, R. J.; Lauter, V.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Leighton, C (reprint author), Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. EM leighton@umn.edu RI O'Brien, Liam/H-1994-2012; Ambaye, Haile/D-1503-2016 OI O'Brien, Liam/0000-0002-0136-8603; Ambaye, Haile/0000-0002-8122-9952 FU NSF MRSEC [DMR-819885]; Marie Curie International Outgoing Fellowship within the 7th European Community Framework Programme [299376]; US Department of Energy [DE-AC05-00OR22725]; NSF through the MRSEC program; NSF through the NNIN program FX This project was funded by the NSF MRSEC under award DMR-819885 and a Marie Curie International Outgoing Fellowship within the 7th European Community Framework Programme (project no. 299376). Research at the ORNL Spallation Neutron Source ORNL was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. ORNL is managed by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy. Parts of this work were carried out in the Characterization Facility, University of Minnesota, which receives partial support from NSF through the MRSEC program. Parts of this work were carried out in the Minnesota Nano Center, which receives partial support from the NSF through the NNIN program. NR 55 TC 13 Z9 13 U1 6 U2 47 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3927 DI 10.1038/ncomms4927 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2QU UT WOS:000337505000001 PM 24873934 ER PT J AU Terrapon, N Li, C Robertson, HM Ji, L Meng, XH Booth, W Chen, ZS Childers, CP Glastad, KM Gokhale, K Gowin, J Gronenberg, W Hermansen, RA Hu, HF Hunt, BG Huylmans, AK Khalil, SMS Mitchell, RD Munoz-Torres, MC Mustard, JA Pan, HL Reese, JT Scharf, ME Sun, FM Vogel, H Xiao, J Yang, W Yang, ZK Yang, ZQ Zhou, JJ Zhu, JW Brent, CS Elsik, CG Goodisman, MAD Liberles, DA Roe, RM Vargo, EL Vilcinskas, A Wang, J Bornberg-Bauer, E Korb, J Zhang, GJ Liebig, J AF Terrapon, Nicolas Li, Cai Robertson, Hugh M. Ji, Lu Meng, Xuehong Booth, Warren Chen, Zhensheng Childers, Christopher P. Glastad, Karl M. Gokhale, Kaustubh Gowin, Johannes Gronenberg, Wulfila Hermansen, Russell A. Hu, Haofu Hunt, Brendan G. Huylmans, Ann Kathrin Khalil, Sayed M. S. Mitchell, Robert D. Munoz-Torres, Monica C. Mustard, Julie A. Pan, Hailin Reese, Justin T. Scharf, Michael E. Sun, Fengming Vogel, Heiko Xiao, Jin Yang, Wei Yang, Zhikai Yang, Zuoquan Zhou, Jiajian Zhu, Jiwei Brent, Colin S. Elsik, Christine G. Goodisman, Michael A. D. Liberles, David A. Roe, R. Michael Vargo, Edward L. Vilcinskas, Andreas Wang, Jun Bornberg-Bauer, Erich Korb, Judith Zhang, Guojie Liebig, Jurgen TI Molecular traces of alternative social organization in a termite genome SO NATURE COMMUNICATIONS LA English DT Article ID DNA METHYLATION; ZOOTERMOPSIS-ANGUSTICOLLIS; RETICULITERMES-FLAVIPES; PROTEASOME PATHWAY; SIAH-1 INTERACTS; GENE-EXPRESSION; APIS-MELLIFERA; DRAFT GENOME; HONEY-BEE; EVOLUTION AB Although eusociality evolved independently within several orders of insects, research into the molecular underpinnings of the transition towards social complexity has been confined primarily to Hymenoptera (for example, ants and bees). Here we sequence the genome and stage-specific transcriptomes of the dampwood termite Zootermopsis nevadensis (Blattodea) and compare them with similar data for eusocial Hymenoptera, to better identify commonalities and differences in achieving this significant transition. We show an expansion of genes related to male fertility, with upregulated gene expression in male reproductive individuals reflecting the profound differences in mating biology relative to the Hymenoptera. For several chemoreceptor families, we show divergent numbers of genes, which may correspond to the more claustral lifestyle of these termites. We also show similarities in the number and expression of genes related to caste determination mechanisms. Finally, patterns of DNA methylation and alternative splicing support a hypothesized epigenetic regulation of caste differentiation. C1 [Terrapon, Nicolas; Huylmans, Ann Kathrin; Bornberg-Bauer, Erich] Univ Munster, Inst Evolut & Biodivers, D-48149 Munster, Germany. [Li, Cai; Ji, Lu; Meng, Xuehong; Chen, Zhensheng; Hu, Haofu; Pan, Hailin; Sun, Fengming; Xiao, Jin; Yang, Wei; Yang, Zhikai; Yang, Zuoquan; Zhou, Jiajian; Wang, Jun; Zhang, Guojie] BGI Shenzhen, China Natl GeneBank, Shenzhen, Peoples R China. [Li, Cai] Univ Copenhagen, Nat Hist Museum Denmark, Ctr GeoGenet, DK-1350 Copenhagen, Denmark. [Robertson, Hugh M.] Univ Illinois, Dept Entomol, Urbana, IL 61801 USA. [Booth, Warren; Khalil, Sayed M. S.; Mitchell, Robert D.; Zhu, Jiwei; Roe, R. Michael; Vargo, Edward L.] N Carolina State Univ, Dept Entomol, Raleigh, NC 27695 USA. [Booth, Warren; Khalil, Sayed M. S.; Mitchell, Robert D.; Zhu, Jiwei; Roe, R. Michael; Vargo, Edward L.] N Carolina State Univ, WM Keck Ctr Behav Biol, Raleigh, NC 27695 USA. [Childers, Christopher P.; Reese, Justin T.; Elsik, Christine G.] Univ Missouri, Div Anim Sci, Columbia, MO 65211 USA. [Glastad, Karl M.; Hunt, Brendan G.; Goodisman, Michael A. D.] Georgia Inst Technol, Sch Biol, Atlanta, GA 30332 USA. [Gokhale, Kaustubh; Mustard, Julie A.; Liebig, Jurgen] Arizona State Univ, Sch Life Sci, Tempe, AZ 85287 USA. [Gowin, Johannes; Korb, Judith] Univ Osnabruck, D-49076 Osnabruck, Germany. [Gronenberg, Wulfila] Univ Arizona, Dept Neurosci, Tucson, AZ 85721 USA. [Hermansen, Russell A.; Liberles, David A.] Univ Wyoming, Dept Mol Biol, Laramie, WY 82071 USA. [Khalil, Sayed M. S.] Agr Genet Engn Res Inst, Dept Microbial Mol Biol, Giza 12619, Egypt. [Munoz-Torres, Monica C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Scharf, Michael E.] Purdue Univ, Dept Entomol, W Lafayette, IN 47907 USA. [Vogel, Heiko] Max Planck Inst Chem Ecol, Dept Entomol, D-07745 Jena, Germany. [Brent, Colin S.] USDA, Arid Land Agr Res Ctr, Maricopa, AZ 85138 USA. [Elsik, Christine G.] Univ Missouri, Div Plant Sci, Columbia, MO 65211 USA. [Vilcinskas, Andreas] Univ Giessen, Inst Phytopathol & Angew, D-35390 Giessen, Germany. [Wang, Jun] Univ Copenhagen, Dept Biol, DK-1165 Copenhagen, Denmark. [Wang, Jun] King Abdulaziz Univ, Princess Jawhara Ctr Excellence Res Hereditary Di, Jeddah 21589, Saudi Arabia. [Wang, Jun] Macau Univ Sci & Technol, Taipa 999078, Madhya Pradesh, Peoples R China. [Wang, Jun] Univ Hong Kong, Dept Med, Hong Kong, Hong Kong, Peoples R China. [Zhang, Guojie] Univ Copenhagen, Ctr Social Evolut, Dept Biol, DK-2100 Copenhagen, Denmark. RP Korb, J (reprint author), Univ Freiburg, D-79117 Freiburg, Germany. EM judith.korb@biologie.uni-freiburg.de; zhanggj@genomics.org.cn; jliebig@asu.edu RI Hunt, Brendan/B-9816-2009; Zhang, Guojie/B-6188-2014; Terrapon, Nicolas/O-3630-2014; Wang, Jun/C-8434-2016; Bornberg-Bauer, Erich/A-1563-2013; Elsik, Christine/C-4120-2017; Wang, Jun/B-9503-2016 OI Hu, Haofu/0000-0001-8145-3009; Childers, Chris/0000-0002-1253-5550; Hunt, Brendan/0000-0002-0030-9302; Zhang, Guojie/0000-0001-6860-1521; Terrapon, Nicolas/0000-0002-3693-6017; Wang, Jun/0000-0002-8540-8931; Bornberg-Bauer, Erich/0000-0002-1826-3576; Elsik, Christine/0000-0002-4248-7713; Huylmans, Ann Kathrin/0000-0001-8871-4961; Li, Cai/0000-0001-7843-2151; Wang, Jun/0000-0002-2113-5874 FU Agriculture and Food Research Initiative Competitive from the USDA National Institute of Food and Agriculture [2007-35302-18172]; Deutschen Forschungsgemeinschaft (DFG) [KO1895/6]; LOEWE Research Focus 'Insect Biotechnology' FX We thank the administrators of the Pebble Beach Company for permission to collect termites and Navdeep Mutti for initial help in RNA and DNA sampling. This work was supported by the Agriculture and Food Research Initiative Competitive Grant number 2007-35302-18172 from the USDA National Institute of Food and Agriculture to J.L. and C.S.B.; and a research grant from the Deutschen Forschungsgemeinschaft (DFG) to J.K. (KO1895/6) and LOEWE Research Focus 'Insect Biotechnology' to A.V. Mention of trade names or commercial products in this article is solely for the purpose of providing specific information and does not imply recommendation or endorsement by the US Department of Agriculture. USDA is an equal opportunity provider and employer. NR 70 TC 69 Z9 76 U1 9 U2 81 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3636 DI 10.1038/ncomms4636 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0RB UT WOS:000337362200001 PM 24845553 ER PT J AU Yan, ZJ Gray, SK Scherer, NF AF Yan, Zijie Gray, Stephen K. Scherer, Norbert F. TI Potential energy surfaces and reaction pathways for light-mediated self-organization of metal nanoparticle clusters SO NATURE COMMUNICATIONS LA English DT Article ID OPTICAL BINDING; SILVER NANOPARTICLES; MANIPULATION; NANOSTRUCTURES; SINGLE AB Potential energy surfaces are the central concept in understanding the assembly of molecules; atoms form molecules via covalent bonds with structures defined by the stationary points of the surfaces. Similarly, dispersion interactions give Lennard-Jones potentials that describe atomic clusters and liquids. The formation of molecules and clusters can follow various pathways depending on the initial conditions and the potentials. Here we show that analogous mechanistic effects occur in light-mediated self-organization of metal nanoparticles; atoms are replaced by silver nanoparticles that are arranged by electrodynamic (that is, optical trapping and optical binding) interactions. We demonstrate this concept using simple Gaussian optical fields and the formation of stable clusters with various two-dimensional (2D) and three-dimensional (3D) geometries. The formation of specific clusters is 'path-dependent'; the particle motions follow an electrodynamic potential energy surface. This work paves the way for rational design of photonic clusters with combinations of imposed beam shapes, gradients and optical binding interactions. C1 [Yan, Zijie; Scherer, Norbert F.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Yan, Zijie; Scherer, Norbert F.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Gray, Stephen K.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Scherer, NF (reprint author), Univ Chicago, James Franck Inst, 929 East 57th St, Chicago, IL 60637 USA. EM nfschere@uchicago.edu RI Yan, Zijie/C-5805-2009 OI Yan, Zijie/0000-0003-0726-7042 FU National Science Foundation [CHE-1059057]; Center for Nanoscale Materials; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX This work was supported by the National Science Foundation (CHE-1059057). This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. We thank Dr Matthew Pelton for helpful discussions. NR 38 TC 19 Z9 19 U1 4 U2 53 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2014 VL 5 AR 3751 DI 10.1038/ncomms4751 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0SY UT WOS:000337367500001 PM 24786197 ER PT J AU Ampleford, DJ Jones, B Jennings, CA Hansen, SB Cuneo, ME Harvey-Thompson, AJ Rochau, GA Coverdale, CA Laspe, AR Flanagan, TM Moore, NW Sinars, DB Lamppa, DC Harding, EC Thornhill, JW Giuliani, JL Chong, YK Apruzese, JP Velikovich, AL Dasgupta, A Ouart, N Sygar, WA Savage, ME Moore, JK Focia, R Wagoner, TC Killebrew, KL Edens, AD Dunham, GS Jones, MC Lake, PW Nielsen, DS Wu, M Carlson, AL Kernahan, MD Ball, CR Scharberg, RD Mulville, TD Breden, EW Speas, CS Olivas, G Sullivan, MA York, AJ Justus, DW Cisneros, JC Strizic, T Reneker, J Cleveland, M Vigil, MP Robertson, G Sandoval, D Cox, C Maurer, AJ Graham, DA Huynh, NB Toledo, S Molina, LP Lopez, MR Long, FW McKee, GR Porter, JL Herrmann, MC AF Ampleford, D. J. Jones, B. Jennings, C. A. Hansen, S. B. Cuneo, M. E. Harvey-Thompson, A. J. Rochau, G. A. Coverdale, C. A. Laspe, A. R. Flanagan, T. M. Moore, N. W. Sinars, D. B. Lamppa, D. C. Harding, E. C. Thornhill, J. W. Giuliani, J. L. Chong, Y. -K. Apruzese, J. P. Velikovich, A. L. Dasgupta, A. Ouart, N. Sygar, W. A. Savage, M. E. Moore, J. K. Focia, R. Wagoner, T. C. Killebrew, K. L. Edens, A. D. Dunham, G. S. Jones, M. C. Lake, P. W. Nielsen, D. S. Wu, M. Carlson, A. L. Kernahan, M. D. Ball, C. R. Scharberg, R. D. Mulville, T. D. Breden, E. W. Speas, C. S. Olivas, G. Sullivan, M. A. York, A. J. Justus, D. W. Cisneros, J. C. Strizic, T. Reneker, J. Cleveland, M. Vigil, M. P. Robertson, G. Sandoval, D. Cox, C. Maurer, A. J. Graham, D. A. Huynh, N. B. Toledo, S. Molina, L. P. Lopez, M. R. Long, F. W. McKee, G. R. Porter, J. L. Herrmann, M. C. TI Contrasting physics in wire array z pinch sources of 1-20 keV emission on the Z facility SO PHYSICS OF PLASMAS LA English DT Article; Proceedings Paper CT 55th Annual Meeting of the APS Division ofPlasma Physics CY NOV 11-14, 2013 CL Denver, CO ID K-SHELL RADIATION; X-RAY POWER; IMPLOSIONS; DYNAMICS; PLASMAS; MA AB a Imploding wire arrays on the 20 MA Z generator have recently provided some of the most powerful and energetic laboratory sources of multi-keV photons, including similar to 375 kJ of Al K-shell emission (h nu similar to 1-2 keV), similar to 80 kJ of stainless steel K-shell emission (h nu similar to 5-9 keV) and a kJ-level of Mo K-shell emission (h nu similar to 17 keV). While the global implosion dynamics of these different wire arrays are very similar, the physical process that dominates the emission from these x-ray sources fall into three broad categories. Al wire arrays produce a column of plasma with densities up to similar to 3 x 10(21) ions/cm(3), where opacity inhibits the escape of K-shell photons. Significant structure from instabilities can reduce the density and increase the surface area, therefore increase the K-shell emission. In contrast, stainless steel wire arrays operate in a regime where achieving a high pinch temperature (achieved by thermalizing a high implosion kinetic energy) is critical and, while opacity is present, it has less impact on the pinch emissivity. At higher photon energies, line emission associated with inner shell ionization due to energetic electrons becomes important. (C) 2014 AIP Publishing LLC. C1 [Ampleford, D. J.; Jones, B.; Jennings, C. A.; Hansen, S. B.; Cuneo, M. E.; Harvey-Thompson, A. J.; Rochau, G. A.; Coverdale, C. A.; Laspe, A. R.; Flanagan, T. M.; Moore, N. W.; Sinars, D. B.; Lamppa, D. C.; Harding, E. C.; Sygar, W. A.; Savage, M. E.; Moore, J. K.; Focia, R.; Wagoner, T. C.; Killebrew, K. L.; Edens, A. D.; Dunham, G. S.; Jones, M. C.; Lake, P. W.; Nielsen, D. S.; Wu, M.; Carlson, A. L.; Kernahan, M. D.; Ball, C. R.; Scharberg, R. D.; Mulville, T. D.; Breden, E. W.; Speas, C. S.; Olivas, G.; Sullivan, M. A.; York, A. J.; Justus, D. W.; Cisneros, J. C.; Strizic, T.; Reneker, J.; Cleveland, M.; Vigil, M. P.; Robertson, G.; Sandoval, D.; Cox, C.; Maurer, A. J.; Graham, D. A.; Huynh, N. B.; Toledo, S.; Molina, L. P.; Lopez, M. R.; Long, F. W.; McKee, G. R.; Porter, J. L.; Herrmann, M. C.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Thornhill, J. W.; Giuliani, J. L.; Chong, Y. -K.; Apruzese, J. P.; Velikovich, A. L.; Dasgupta, A.; Ouart, N.] Naval Res Lab, Washington, DC 20375 USA. RP Ampleford, DJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM damplef@sandia.gov FU Laboratory Directed Research and Development Project at Sandia National Laboratories [165733]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NNSA FX The authors gratefully acknowledge the many individuals who enabled these experiments at Z, including the Z Diagnostics group, the Z Center Section team, Load Hardware Designers, Hardware and Wire Array Assembly, Electrical Diagnostics the ZBL laser and Z Operations. The authors thank many colleagues for useful discussions, including J. P. Chittenden, N. Niasse, B. Appelbe (Imperial College), A. Safronova, V. Kantsyrev, R. Pressura (University of Nevada, Reno), and C. Deeney (NSTec). The authors would also like to thank M. K. Matzen, J. Lee, G. Heffelfinger, E. F. Hartman, J. W. Bryson, J. Lash, and C. J. Bourdon (Sandia) for programmatic support. Work on non-thermal emission from wire array z pinches performed under Laboratory Directed Research and Development Project No. 165733 at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. Work at Naval Research Laboratory is supported by NNSA. NR 39 TC 10 Z9 10 U1 2 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAY PY 2014 VL 21 IS 5 AR 056708 DI 10.1063/1.4876621 PG 10 WC Physics, Fluids & Plasmas SC Physics GA AI7UY UT WOS:000337107200137 ER PT J AU Awe, TJ Jennings, CA McBride, RD Cuneo, ME Lamppa, DC Martin, MR Rovang, DC Sinars, DB Slutz, SA Owen, AC Tomlinson, K Gomez, MR Hansen, SB Herrmann, MC Jones, MC McKenney, JL Robertson, GK Rochau, GA Savage, ME Schroen, DG Stygar, WA AF Awe, T. J. Jennings, C. A. McBride, R. D. Cuneo, M. E. Lamppa, D. C. Martin, M. R. Rovang, D. C. Sinars, D. B. Slutz, S. A. Owen, A. C. Tomlinson, K. Gomez, M. R. Hansen, S. B. Herrmann, M. C. Jones, M. C. McKenney, J. L. Robertson, G. K. Rochau, G. A. Savage, M. E. Schroen, D. G. Stygar, W. A. TI Modified helix-like instability structure on imploding z-pinch liners that are pre-imposed with a uniform axial magnetic field SO PHYSICS OF PLASMAS LA English DT Article; Proceedings Paper CT 55th Annual Meeting of the APS Division ofPlasma Physics CY NOV 11-14, 2013 CL Denver, CO ID FUSION AB Recent experiments at the Sandia National Laboratories Z Facility have, for the first time, studied the implosion dynamics of magnetized liner inertial fusion (MagLIF) style liners that were pre-imposed with a uniform axial magnetic field. As reported [T. J. Awe et al., Phys. Rev. Lett. 111, 235005 (2013)] when premagnetized with a 7 or 10 T axial field, these liners developed 3D-helix-like hydrodynamic instabilities; such instabilities starkly contrast with the azimuthally correlated magneto-Rayleigh-Taylor (MRT) instabilities that have been consistently observed in many earlier non-premagnetized experiments. The helical structure persisted throughout the implosion, even though the azimuthal drive field greatly exceeded the expected axial field at the liner's outer wall for all but the earliest stages of the experiment. Whether this modified instability structure has practical importance for magneto-inertial fusion concepts depends primarily on whether the modified instability structure is more stable than standard azimuthally correlated MRT instabilities. In this manuscript, we discuss the evolution of the helix-like instability observed on premagnetized liners. While a first principles explanation of this observation remains elusive, recent 3D simulations suggest that if a small amplitude helical perturbation can be seeded on the liner's outer surface, no further influence from the axial field is required for the instability to grow. (C) 2014 AIP Publishing LLC. C1 [Awe, T. J.; Jennings, C. A.; McBride, R. D.; Cuneo, M. E.; Lamppa, D. C.; Martin, M. R.; Rovang, D. C.; Sinars, D. B.; Slutz, S. A.; Owen, A. C.; Gomez, M. R.; Hansen, S. B.; Herrmann, M. C.; Jones, M. C.; McKenney, J. L.; Robertson, G. K.; Rochau, G. A.; Savage, M. E.; Stygar, W. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Tomlinson, K.; Schroen, D. G.] Gen Atom Co, San Diego, CA 92121 USA. RP Awe, TJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tjawe@sandia.gov FU Sandia's Laboratory Directed Research and Development Program [141537, 165736]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank the ABZ Team, the MagLIF Team, the Z Operations Team, the Z-Beamlet Operations Team, Center Section personnel, the Z Diagnostics Team, the Neutron Team, CMDAS personnel, Lab 101 personnel, the VISAR team, the Gas Fill Team, the Target Fabrication Team, J. Greenly, D. Johnson, R. Kamm, J. Moore, S. Radovich, G. Smith, and I. Smith. This project was funded in part by Sandia's Laboratory Directed Research and Development Program (Projects Nos. 141537 and 165736). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 19 TC 22 Z9 22 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAY PY 2014 VL 21 IS 5 AR 056303 DI 10.1063/1.4872331 PG 8 WC Physics, Fluids & Plasmas SC Physics GA AI7UY UT WOS:000337107200112 ER PT J AU Baalrud, SD Daligault, J AF Baalrud, Scott D. Daligault, Jerome TI Extending plasma transport theory to strong coupling through the concept of an effective interaction potential SO PHYSICS OF PLASMAS LA English DT Article; Proceedings Paper CT 55th Annual Meeting of the APS Division ofPlasma Physics CY NOV 11-14, 2013 CL Denver, CO ID KINETIC-EQUATION; IONIZED-GASES; COEFFICIENTS; APPROXIMATION AB A method for extending traditional plasma transport theories into the strong coupling regime is presented. Like traditional theories, this is based on a binary scattering approximation, but where physics associated with many body correlations is included through the use of an effective interaction potential. The latter is simply related to the pair-distribution function. Modeling many body effects in this manner can extend traditional plasma theory to orders of magnitude stronger coupling. Theoretical predictions are tested against molecular dynamics simulations for electron-ion temperature relaxation as well as diffusion in one component systems. Emphasis is placed on the connection with traditional plasma theory, where it is stressed that the effective potential concept has precedence through the manner in which screening is imposed. The extension to strong coupling requires accounting for correlations in addition to screening. Limitations of this approach in the presence of strong caging are also discussed. (C) 2014 AIP Publishing LLC. C1 [Baalrud, Scott D.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Daligault, Jerome] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Baalrud, SD (reprint author), Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. FU University of Iowa; National Nuclear Security Administration of the U.S. Department of Energy (DOE) at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Office of Fusion Sciences FX The work of S.D.B. was supported in part by the University of Iowa and in part under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy (DOE) at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The work of J.D. was supported by the DOE Office of Fusion Sciences. NR 45 TC 13 Z9 13 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAY PY 2014 VL 21 IS 5 AR 055707 DI 10.1063/1.4875282 PG 12 WC Physics, Fluids & Plasmas SC Physics GA AI7UY UT WOS:000337107200090 ER PT J AU Baumgaertel, JA Bradley, PA Hsu, SC Cobble, JA Hakel, P Tregillis, IL Krasheninnikova, NS Murphy, TJ Schmitt, MJ Shah, RC Obrey, KD Batha, S Johns, H Joshi, T Mayes, D Mancini, RC Nagayama, T AF Baumgaertel, J. A. Bradley, P. A. Hsu, S. C. Cobble, J. A. Hakel, P. Tregillis, I. L. Krasheninnikova, N. S. Murphy, T. J. Schmitt, M. J. Shah, R. C. Obrey, K. D. Batha, S. Johns, H. Joshi, T. Mayes, D. Mancini, R. C. Nagayama, T. TI Observation of early shell-dopant mix in OMEGA direct-drive implosions and comparisons with radiation-hydrodynamic simulations SO PHYSICS OF PLASMAS LA English DT Article ID NATIONAL-IGNITION-FACILITY; RAYLEIGH-TAYLOR GROWTH; PLANAR TARGETS AB Temporally, spatially, and spectrally resolved x-ray image data from direct-drive implosions on OMEGA were interpreted with the aid of radiation-hydrodynamic simulations. Neither clean calculations nor those using a turbulent mix model can explain fully the observed migration of shell-dopant material (titanium) into the core. Shell-dopant migration was observed via time-dependent, spatially integrated spectra, and spatially and spectrally resolved x-ray images of capsule implosions and resultant dopant emissions. The titanium emission was centrally peaked in narrowband x-ray images. In post-processed clean simulations, the peak titanium emission forms in a ring in self-emission images as the capsule implodes. Post-processed simulations with mix reproduce trends in time-dependent, spatially integrated spectra, as well having centrally peaked Ti emission in synthetic multiple monochromatic imager. However, mix simulations still do not transport Ti to the core as is observed in the experiment. This suggests that phenomena in addition to the turbulent mix must be responsible for the transport of Ti. Simple diffusion estimates are unable to explain the early Ti mix into the core. Mechanisms suggested for further study are capsule surface roughness, illumination non-uniformity, and shock entrainment. (C) 2014 AIP Publishing LLC. C1 [Baumgaertel, J. A.; Bradley, P. A.; Hsu, S. C.; Cobble, J. A.; Hakel, P.; Tregillis, I. L.; Krasheninnikova, N. S.; Murphy, T. J.; Schmitt, M. J.; Shah, R. C.; Obrey, K. D.; Batha, S.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Johns, H.; Joshi, T.; Mayes, D.; Mancini, R. C.; Nagayama, T.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. RP Baumgaertel, JA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RI Murphy, Thomas/F-3101-2014; OI Murphy, Thomas/0000-0002-6137-9873; Hakel, Peter/0000-0002-7936-4231; Schmitt, Mark/0000-0002-0197-9180; Bradley, Paul/0000-0001-6229-6677; Hsu, Scott/0000-0002-6737-4934; Joshi, Tirtha/0000-0003-2218-8190 FU U.S. Department of Energy by Los Alamos National Security, LLC [DE-AC52-06NA25396] FX The authors wish to especially thank the OMEGA operations team for executing the experiments. We also thank General Atomics for creating the capsules, and B. Yaakobi of LLE for providing the XRS data that were used to calibrate the SSCA. We gratefully acknowledge M. Marinak for his assistance with HYDRA. This work was performed under the auspices of the U.S. Department of Energy by Los Alamos National Security, LLC under Contract No. DE-AC52-06NA25396. NR 56 TC 7 Z9 7 U1 2 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAY PY 2014 VL 21 IS 5 AR 052706 DI 10.1063/1.4881463 PG 9 WC Physics, Fluids & Plasmas SC Physics GA AI7UY UT WOS:000337107200045 ER PT J AU Bellei, C Rinderknecht, H Zylstra, A Rosenberg, M Sio, H Li, CK Petrasso, R Wilks, SC Amendt, PA AF Bellei, C. Rinderknecht, H. Zylstra, A. Rosenberg, M. Sio, H. Li, C. K. Petrasso, R. Wilks, S. C. Amendt, P. A. TI Species separation and kinetic effects in collisional plasma shocks SO PHYSICS OF PLASMAS LA English DT Article; Proceedings Paper CT 55th Annual Meeting of the APS Division ofPlasma Physics CY NOV 11-14, 2013 CL Denver, CO ID WAVE; SIMULATIONS; IMPLOSIONS; CODE AB The properties of collisional shock waves propagating in uniform plasmas are studied with ion-kinetic calculations, in both slab and spherical geometry and for the case of one and two ion species. Despite the presence of an electric field at the shock front-and in contrast to the case where an interface is initially present [C. Bellei et al., Phys. Plasmas 20, 044702 (2013)]-essentially no ion reflection at the shock front is observed due to collisions, with a probability of reflection less than or similar to 10(-4) for the cases presented. A kinetic two-ion-species spherical convergent shock is studied in detail and compared against an average-species calculation, confirming effects of species separation and differential heating of the ion species at the shock front. The effect of different ion temperatures on the DT and (DHe)-He-3 fusion reactivity is discussed in the fluid limit and is estimated to be moderately important. (C) 2014 AIP Publishing LLC. C1 [Bellei, C.; Wilks, S. C.; Amendt, P. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Rinderknecht, H.; Zylstra, A.; Rosenberg, M.; Sio, H.; Li, C. K.; Petrasso, R.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. RP Bellei, C (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM bellei1@llnl.gov OI /0000-0003-4969-5571 FU U.S. Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; [LDRD-11-ERD-075] FX C. B. acknowledges useful discussions with B. Cohen and A. Dimits on the collision operator in particle-in-cell codes and with D. Ryutov on the fusion reactivity. Computing support for this work came from the Lawrence Livermore National Laboratory (LLNL) Institutional Computing Grand Challenge program. This work was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and supported by LDRD-11-ERD-075. NR 32 TC 8 Z9 8 U1 2 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAY PY 2014 VL 21 IS 5 AR 056310 DI 10.1063/1.4876614 PG 11 WC Physics, Fluids & Plasmas SC Physics GA AI7UY UT WOS:000337107200119 ER PT J AU Benedetti, C Schroeder, CB Esarey, E Leemans, WP AF Benedetti, C. Schroeder, C. B. Esarey, E. Leemans, W. P. TI Plasma wakefields driven by an incoherent combination of laser pulses: A path towards high-average power laser-plasma accelerators SO PHYSICS OF PLASMAS LA English DT Article; Proceedings Paper CT 55th Annual Meeting of the APS Division ofPlasma Physics CY NOV 11-14, 2013 CL Denver, CO ID ELECTRON-ACCELERATORS; FEMTOSECOND; INJECTION; FUTURE; PHASE AB The wakefield generated in a plasma by incoherently combining a large number of low energy laser pulses (i.e., without constraining the pulse phases) is studied analytically and by means of fully self-consistent particle-in-cell simulations. The structure of the wakefield has been characterized and its amplitude compared with the amplitude of the wake generated by a single (coherent) laser pulse. We show that, in spite of the incoherent nature of the wakefield within the volume occupied by the laser pulses, behind this region, the structure of the wakefield can be regular with an amplitude comparable or equal to that obtained from a single pulse with the same energy. Wake generation requires that the incoherent structures in the laser energy density produced by the combined pulses exist on a time scale short compared to the plasma period. Incoherent combination of multiple laser pulses may enable a technologically simpler path to high-repetition rate, high-average power laser-plasma accelerators, and associated applications. (C) 2014 AIP Publishing LLC. C1 [Benedetti, C.; Schroeder, C. B.; Esarey, E.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Benedetti, C (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. OI Schroeder, Carl/0000-0002-9610-0166 FU Office of Science, Office of High Energy Physics, of the U.S. DOE [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of High Energy Physics, of the U.S. DOE under Contract No. DE-AC02-05CH11231, and used the computational facilities (Hopper, Edison) at the National Energy Research Scientific Computing Center (NERSC). We would like to thank A. Galvanauskas for useful discussions. NR 34 TC 8 Z9 8 U1 0 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAY PY 2014 VL 21 IS 5 AR 056706 DI 10.1063/1.4878620 PG 12 WC Physics, Fluids & Plasmas SC Physics GA AI7UY UT WOS:000337107200135 ER EF