FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Craig, NC Chen, YH van Besien, H Blake, TA AF Craig, Norman C. Chen, Yihui van Besien, Herman Blake, Thomas A. TI Analysis of the rotational structure in the high-resolution infrared spectra of trans-hexatriene-2-d(1) and-3-d(1) SO JOURNAL OF MOLECULAR SPECTROSCOPY LA English DT Article DE trans-Hexatriene-2-d(1) and-3-d(1); High-resolution infrared; Vibration wavenumbers; Rotational analysis; Rotational constants; C-type bands ID SEMIEXPERIMENTAL EQUILIBRIUM STRUCTURE; ELECTRON DELOCALIZATION; C-6 BACKBONE; HEXATRIENE AB The 2-d(1) and 3-d(1) isotopologues of trans-hexatriene have been synthesized, and their high-resolution (0.0015 cm(-1)) IR spectra have been recorded. For each of the isotopologues the rotational structure in four C-type bands for out-of-plane vibrational modes has been analyzed, and the ground state combination differences (GSCDs) have been pooled. Ground state rotational constants have been fitted to the GSCDs. For the 2-d species, A(0), B-0, and C-0 values of 0.7837254(5), 0.0442806(3), and 0.0419299(2) cm(-1) were fitted to 2450 GSCDs. For the 3-d species, A(0), B-0, and C-0 values of 0.7952226(8), 0.0446149(7), and 0.0422661(4) cm(-1) were fitted to 2234 GSCDs. For the eleven out-of-plane modes of the two isotopologues, predictions of wavenumbers corrected for anharmonicity and harmonic intensities have been computed and compared with experiment where possible. (C) 2014 Elsevier Inc. All rights reserved. C1 [Craig, Norman C.; Chen, Yihui; van Besien, Herman] Oberlin Coll, Dept Chem & Biochem, Oberlin, OH 44074 USA. [Blake, Thomas A.] Pacific Northwest Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Craig, NC (reprint author), Oberlin Coll, Dept Chem & Biochem, Oberlin, OH 44074 USA. EM norm.craig@oberlin.edu FU Dreyfus Senior Scholar Mentor Grant; National Science Foundation [0420717]; US Department of Energy [DE-AC05-76RLO 1830] FX Part of the work was supported by a Dreyfus Senior Scholar Mentor Grant. National Science Foundation Grant 0420717 provided for the purchase and technical support of the Beowulf computer cluster at Oberlin College. We are grateful to Oberlin College for continuing support of this research and to Hendrik Eberhardt for his exploratory work on the synthesis of tHTE-3-d, which was suggested by Professor Albert R. Matlin. PNNL is operated for the US Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RLO 1830. NR 16 TC 1 Z9 1 U1 0 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-2852 EI 1096-083X J9 J MOL SPECTROSC JI J. Mol. Spectrosc. PD SEP PY 2014 VL 303 BP 26 EP 35 DI 10.1016/j.jms.2014.07.001 PG 10 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA AO4CR UT WOS:000341284300005 ER PT J AU Benedict, JJ Maloney, ED Sobel, AH Frierson, DMW AF Benedict, James J. Maloney, Eric D. Sobel, Adam H. Frierson, Dargan M. W. TI Gross Moist Stability and MJO Simulation Skill in Three Full-Physics GCMs SO JOURNAL OF THE ATMOSPHERIC SCIENCES LA English DT Article ID MADDEN-JULIAN OSCILLATION; TEMPERATURE-GRADIENT APPROXIMATION; TROPICAL INTRASEASONAL VARIABILITY; COMMUNITY ATMOSPHERE MODEL; GENERAL-CIRCULATION MODEL; STATIC ENERGY BUDGET; CUMULUS PARAMETERIZATION; SUBSEASONAL VARIABILITY; CONVECTION FEEDBACKS; ARAKAWA-SCHUBERT AB Previous studies have demonstrated a link between gross moist stability (GMS) and intraseasonal variability in theoretical and reduced-complexity models. In such simplified models, MJO-like moisture modes - convectively coupled tropical disturbances akin to the MJO whose formation and dynamics are linked to moisture perturbations-develop only when GMS is either negative or "effectively" negative when considering additional sources of moist entropy. These simplified models typically use a prescribed, time-independent GMS value. Limited work has been done to assess GMS and its connection to intraseasonal variability in full-physics general circulation models (GCMs). The time-mean and intraseasonal behavior of normalized GMS (NGMS) are examined in three pairs of GCMs to elucidate the possible importance of NGMS for the MJO. In each GCM pair, one member produces weak intraseasonal variability, while the other produces robust MJOs because of a change in the treatment of deep convection. A strong linear correlation between time-mean NGMS and MJO simulation skill is observed, such that GCMs with less positive NGMS produce improved MJO eastward propagation. The reduction in time-mean NGMS is primarily due to a sharp drop to negative values in the NGMS component related to vertical advection, while the horizontal advection component has a less clear relationship with MJO simulations. Intraseasonal fluctuations of anomalous NGMS modulate the magnitude of background NGMS but generally do not change the sign of background NGMS. NGMS declines ahead of peak MJO rainfall and increases during and after heaviest precipitation. Total NGMS fluctuates during MJO passage but remains positive, suggesting that other sources of moist entropy are required to generate an effectively negative NGMS. C1 [Benedict, James J.; Maloney, Eric D.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Sobel, Adam H.] Columbia Univ, Dept Appl Math, New York, NY USA. [Sobel, Adam H.] Columbia Univ, Dept Earth & Environm Sci, New York, NY USA. [Sobel, Adam H.] Columbia Univ, Lamont Doherty Earth Observ, New York, NY USA. [Frierson, Dargan M. W.] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. RP Benedict, JJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS 74-0171, Berkeley, CA 94720 USA. EM jjbenedict@lbl.gov RI Maloney, Eric/A-9327-2008; Sobel, Adam/K-4014-2015; Frierson, Dargan/F-1763-2010; Benedict, James/M-5824-2013 OI Maloney, Eric/0000-0002-2660-2611; Sobel, Adam/0000-0003-3602-0567; Frierson, Dargan/0000-0001-8952-5644; Benedict, James/0000-0001-5115-5131 FU National Oceanic and Atmospheric Administration [NA08OAR4320893, NA12OAR4310077, NA08OAR4320912]; U.S. Department of Commerce; Climate and Large-Scale Dynamics Program of the National Science Foundation [AGS-1025584, AGS-1062161, AGS-1347738] FX We thank two anonymous reviewers for their constructive and insightful comments. We also thank David Raymond and the WGNE MJO Task Force for their scientific advice and motivation of this work. This work was supported by Awards NA08OAR4320893, NA12OAR4310077 (JJB, EDM) and NA08OAR4320912 (AHS) from the National Oceanic and Atmospheric Administration, U.S. Department of Commerce, and by the Climate and Large-Scale Dynamics Program of the National Science Foundation under Grants AGS-1025584, AGS-1062161, and AGS-1347738 (EDM). The statements, findings, conclusions, and recommendations do not necessarily reflect the views of NSF, NOAA, or the U.S. Department of Commerce. NR 75 TC 26 Z9 26 U1 1 U2 13 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0022-4928 EI 1520-0469 J9 J ATMOS SCI JI J. Atmos. Sci. PD SEP PY 2014 VL 71 IS 9 BP 3327 EP 3349 DI 10.1175/JAS-D-13-0240.1 PG 23 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AO3KC UT WOS:000341227100012 ER PT J AU Pyon, S Kudo, K Matsumura, J Ishii, H Matsuo, G Nohara, M Hojo, H Oka, K Azuma, M Garlea, VO Kodama, K Shamoto, S AF Pyon, Sunseng Kudo, Kazutaka Matsumura, Jun-ichi Ishii, Hiroyuki Matsuo, Genta Nohara, Minoru Hojo, Hajime Oka, Kengo Azuma, Masaki Garlea, V. Ovidiu Kodama, Katsuaki Shamoto, Shin-ichi TI Superconductivity in Noncentrosymmetric Iridium Silicide Li2IrSi3 SO JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN LA English DT Article ID HIGH-PRESSURE SYNTHESIS; UPPER CRITICAL-FIELD; DENSITY; PHASE AB The effects of lithium absorption on the crystal structure and electronic properties of IrSi3, a binary silicide with a noncentrosymmetric crystal structure, were studied. X-ray and neutron diffraction experiments revealed that hexagonal IrSi3 (space group P6(3)mc) transforms into trigonal Li2IrSi3 (space group P31c) upon lithium absorption. The structure of Li2IrSi3 is found to consist of a planar kagome network of silicon atoms with Li and Ir spaced at unequal distances between the kagome layers, resulting in a polar structure along the c-axis. Li2IrSi3 exhibited type-II superconductivity with a transition temperature T-c of 3.8 K, displaying a structure type that no previous superconductors have been reported to have. C1 [Pyon, Sunseng; Kudo, Kazutaka; Matsumura, Jun-ichi; Ishii, Hiroyuki; Matsuo, Genta; Nohara, Minoru] Okayama Univ, Dept Phys, Okayama 7008530, Japan. [Pyon, Sunseng; Kudo, Kazutaka; Matsumura, Jun-ichi; Ishii, Hiroyuki; Matsuo, Genta; Nohara, Minoru] Okayama Univ, Res Ctr New Funct Mat Energy Prod Storage & Trans, Okayama 7008530, Japan. [Hojo, Hajime; Oka, Kengo; Azuma, Masaki] Tokyo Inst Technol, Mat & Struct Lab, Yokohama, Kanagawa 2268503, Japan. [Garlea, V. Ovidiu] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Kodama, Katsuaki; Shamoto, Shin-ichi] Japan Atom Energy Agcy, Quantum Beam Sci Ctr, Sect Nucl Sci Res, Mat Sci Res Unit, Tokai, Ibaraki 3191195, Japan. RP Pyon, S (reprint author), Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan. EM nohara@science.okayama-u.ac.jp RI KUDO, Kazutaka/B-1468-2011; NOHARA, Minoru/B-1476-2011; Hojo, Hajime/C-5275-2012; Azuma, Masaki/C-2945-2009; Oka, Kengo/A-8753-2010; Garlea, Vasile/A-4994-2016 OI Azuma, Masaki/0000-0002-8378-321X; Oka, Kengo/0000-0002-1800-8575; Garlea, Vasile/0000-0002-5322-7271 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; U.S.-Japan Collaborative Program on Neutron Scattering; Japan Society for the Promotion of Science (JSPS) [24740238, 26820291, 26800180, 26106507, 25287094, 26287082, 25400372]; Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST Program) from JSPS FX Part of this work was performed at the Advanced Science Research Center, Okayama University. The synchrotron radiation experiments were performed at SPring-8 with the approval of the Japan Synchrotron Radiation Research Institute (2012A1665). Research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This work was partially supported by the U.S.-Japan Collaborative Program on Neutron Scattering, Grants-in-Aid for Young Scientists (B) (24740238, 26820291, and 26800180), Creative Scientific Research (26106507), Scientific Research (B) (25287094 and 26287082), and (C) (25400372) from the Japan Society for the Promotion of Science (JSPS), and the Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST Program) from JSPS. NR 33 TC 8 Z9 8 U1 4 U2 23 PU PHYSICAL SOC JAPAN PI TOKYO PA YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN SN 0031-9015 J9 J PHYS SOC JPN JI J. Phys. Soc. Jpn. PD SEP PY 2014 VL 83 IS 9 AR 093706 DI 10.7566/JPSJ.83.093706 PG 5 WC Physics, Multidisciplinary SC Physics GA AN8AI UT WOS:000340822100008 ER PT J AU Chen, SY Huang, JP Qian, Y Ge, JM Su, J AF Chen Si-yu Huang Jian-ping Qian Yun Ge Jin-ming Su Jing TI EFFECTS OF AEROSOLS ON AUTUMN PRECIPITATION OVER MID-EASTERN CHINA SO JOURNAL OF TROPICAL METEOROLOGY LA English DT Article DE aerosol; autumn precipitation; atmospheric stability; cloud microphysical properties ID DUST AEROSOL; SATELLITE MEASUREMENTS; HYDROLOGICAL CYCLE; TAKLIMAKAN DUST; CLIMATE; VISIBILITY; ASIA; CERES AB Long-term observational data indicated a decreasing trend for the amount of autumn precipitation (i.e. 54.3 mm per decade) over Mid-Eastern China, especially after the 1980s (similar to 5.6% per decade). To examine the cause of the decreasing trend, the mechanisms associated with the change of autumn precipitation were investigated from the perspective of water vapor transportation, atmospheric stability and cloud microphysics. Results show that the decrease of convective available potential energy (i.e. 12.81 J kg(-1)/ decade) and change of cloud microphysics, which were closely related to the increase of aerosol loading during the past twenty years, were the two primary factors responsible for the decrease of autumn precipitation. Our results showed that increased aerosol could enhance the atmospheric stability thus weaken the convection. Meanwhile, more aerosols also led to a significant decline of raindrop concentration and to a delay of raindrop formation because of smaller size of cloud droplets. Thus, increased aerosols produced by air pollution could be one of the major reasons for the decrease of autumn precipitation. Furthermore, we found that the aerosol effects on precipitation in autumn was more significant than in other seasons, partly due to relatively more stable synoptic systems in autumn. The impact of large-scale circulation dominant in autumn and the dynamic influence on precipitation was more important than the thermodynamic activity. C1 [Chen Si-yu; Huang Jian-ping; Ge Jin-ming; Su Jing] Lanzhou Univ, Minist Educ, Key Lab Semiarid Climate Change, Lanzhou 730000, Peoples R China. [Qian Yun] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Huang, JP (reprint author), Lanzhou Univ, Minist Educ, Key Lab Semiarid Climate Change, Lanzhou 730000, Peoples R China. EM hjp@lzu.edu.cn RI qian, yun/E-1845-2011; chen, siyu/D-3855-2016 OI chen, siyu/0000-0003-2532-6050 FU National Basic Research Program of China [2012CB955301] FX National Basic Research Program of China (2012CB955301) NR 46 TC 5 Z9 6 U1 1 U2 14 PU JOURNAL OF TROPICAL METEOROLOGICAL PRESS PI GUANGZHOU PA 6 FU JIN RD, GUANGZHOU, 510080, PEOPLES R CHINA SN 1006-8775 J9 J TROP METEOROL JI J. Trop. Meteorol. PD SEP PY 2014 VL 20 IS 3 BP 242 EP 250 PG 9 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AO2QL UT WOS:000341170200007 ER PT J AU Nkolola, JP Bricault, CA Cheung, A Shields, J Perry, J Kovacs, JM Giorgi, E van Winsen, M Apetri, A Brinkman-van der Linden, ECM Chen, B Korber, B Seaman, MS Barouch, DH AF Nkolola, Joseph P. Bricault, Christine A. Cheung, Ann Shields, Jennifer Perry, James Kovacs, James M. Giorgi, Elena van Winsen, Margot Apetri, Adrian Brinkman-van der Linden, Els C. M. Chen, Bing Korber, Bette Seaman, Michael S. Barouch, Dan H. TI Characterization and Immunogenicity of a Novel Mosaic M HIV-1 gp140 Trimer SO JOURNAL OF VIROLOGY LA English DT Article ID IMMUNODEFICIENCY-VIRUS TYPE-1; NEUTRALIZING ANTIBODY-RESPONSES; HUMAN MONOCLONAL-ANTIBODIES; T-LYMPHOCYTE RESPONSES; RHESUS-MONKEYS; ENVELOPE GLYCOPROTEIN; PROTECTIVE EFFICACY; IMMUNE-RESPONSES; SUBTYPE-C; VACCINE AB The extraordinary diversity of the human immunodeficiency virus type 1 (HIV-1) envelope (Env) glycoprotein poses a major challenge for the development of an HIV-1 vaccine. One strategy to circumvent this problem utilizes bioinformatically optimized mosaic antigens. However, mosaic Env proteins expressed as trimers have not been previously evaluated for their stability, antigenicity, and immunogenicity. Here, we report the production and characterization of a stable HIV-1 mosaic M gp140 Env trimer. The mosaic M trimer bound CD4 as well as multiple broadly neutralizing monoclonal antibodies, and biophysical characterization suggested substantial stability. The mosaic M trimer elicited higher neutralizing antibody (nAb) titers against clade B viruses than a previously described clade C (C97ZA.012) gp140 trimer in guinea pigs, whereas the clade C trimer elicited higher nAb titers than the mosaic M trimer against clade A and C viruses. A mixture of the clade C and mosaic M trimers elicited nAb responses that were comparable to the better component of the mixture for each virus tested. These data suggest that combinations of relatively small numbers of immunologically complementary Env trimers may improve nAb responses. IMPORTANCE The development of an HIV-1 vaccine remains a formidable challenge due to multiple circulating strains of HIV-1 worldwide. This study describes a candidate HIV-1 Env protein vaccine whose sequence has been designed by computational methods to address HIV-1 diversity. The characteristics and immunogenicity of this Env protein, both alone and mixed together with a clade C Env protein vaccine, are described. C1 [Nkolola, Joseph P.; Bricault, Christine A.; Cheung, Ann; Shields, Jennifer; Perry, James; Seaman, Michael S.; Barouch, Dan H.] Beth Israel Deaconess Med Ctr, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. [Kovacs, James M.; Chen, Bing] Harvard Univ, Sch Med, Childrens Hosp, Div Mol Med, Boston, MA USA. [Kovacs, James M.; Chen, Bing] Harvard Univ, Sch Med, Dept Pediat, Boston, MA 02115 USA. [Giorgi, Elena; Korber, Bette] Los Alamos Natl Lab, Los Alamos, NM USA. [Giorgi, Elena; Korber, Bette] New Mexico Consortium, Los Alamos, NM USA. [van Winsen, Margot; Apetri, Adrian; Brinkman-van der Linden, Els C. M.] Crucell Vaccine Inst, Leiden, Netherlands. [Barouch, Dan H.] MIT & Harvard, Ragon Inst MGH, Boston, MA USA. RP Barouch, DH (reprint author), Beth Israel Deaconess Med Ctr, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. EM dbarouch@bidmc.harvard.edu OI Korber, Bette/0000-0002-2026-5757 FU NIAID [AI078526, AI084794, AI096040]; Bill and Melinda Gates Foundation [OPP1033091, OPP1040741]; Ragon Institute of MGH, MIT, and Harvard FX We acknowledge support from NIAID grants AI078526, AI084794, and AI096040, Bill and Melinda Gates Foundation grants OPP1033091 and OPP1040741, and the Ragon Institute of MGH, MIT, and Harvard. NR 45 TC 12 Z9 13 U1 0 U2 1 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0022-538X EI 1098-5514 J9 J VIROL JI J. Virol. PD SEP PY 2014 VL 88 IS 17 BP 9538 EP 9552 DI 10.1128/JVI.01739-14 PG 15 WC Virology SC Virology GA AO3LW UT WOS:000341232300006 PM 24965452 ER PT J AU Patterson, BM Henderson, KC Gibbs, PJ Imhoff, SD Clarke, AJ AF Patterson, B. M. Henderson, K. C. Gibbs, P. J. Imhoff, S. D. Clarke, A. J. TI Laboratory micro- and nanoscale X-ray tomographic investigation of Al-7 at.%Cu solidification structures SO MATERIALS CHARACTERIZATION LA English DT Article DE X-ray tomography; Solidification; Aluminum; Copper; Eutectic ID IN-SITU; RESOLUTION; MICROTOMOGRAPHY; DAMAGE; ALLOY; FOAMS; QUANTIFICATION; POLYURETHANE; DEFORMATION; TEMPERATURE AB X-ray computed tomography across multiple length scales provides an opportunity to non-destructively visualize and quantify the micro- to nano-scale microstructural features of solidification structures in three dimensions. Aluminum-7 at.%copper samples were directionally solidified at three cooling rates (0.44, 0.67, and 1.33 C/s), resulting in systematic changes in the as-solidified microstructure, which are difficult to quantify using traditional microscopic techniques. The cooling rate of a material affects its ultimate microstructure, and characterizing that microstructure is key to predicting and understanding its bulk properties. Here, two different laboratory X-ray computed tomography instruments were used to characterize as-solidified microstructures, including micro-scale computed tomography with approximately 1 mm field-of-view, similar to 1.7 mu m resolution, and nano-scale X-ray computed tomography -65 mu m FOV, 150 nm resolution. Micro-scale X-ray radiography and computed tomography enabled a quantitative investigation of changes in the primary dendritic solidification structure with increasing cooling rate. Nano-scale absorption contrast X-ray computed tomography resolved the distinct phases of the lamellar eutectic structure and three dimensional measurements of the -1 mu m interlamellar spacing. It is found that the lamella eutectic structure thickness is inversely proportional to the cooling rate. Nano-scale Zernike phase contrast was also used to image voids at eutectic colony boundaries. The application and resolution of these two instruments are discussed with respect to the resolvable features of the solidification structures. (C) 2014 Elsevier Inc. All rights reserved. C1 [Patterson, B. M.; Henderson, K. C.; Gibbs, P. J.; Imhoff, S. D.; Clarke, A. J.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Patterson, BM (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, POB 1663, Los Alamos, NM 87545 USA. EM bpatterson@lanl.gov OI Patterson, Brian/0000-0001-9244-7376 FU AJC's Early Career Award from the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Los Alamos National Laboratory; US Department of Energy [DE-AC52-06NA25396] FX The authors acknowledge T.J. Tucker, T.V. Beard, R.W. Hudson, B.S. Folks, and D.A. Aragon for their help in preparing experimental hardware. B.R. Randolph is acknowledged for machining the samples. J.C. Cooley, M.R. Katz, and K.D. Clarke are thanked for their assistance with sample preparation. We gratefully acknowledge support from AJC's Early Career Award from the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering and Los Alamos National Laboratory, operated by Los Alamos National Security LLC under contract number DE-AC52-06NA25396 for the US Department of Energy. NR 34 TC 6 Z9 6 U1 3 U2 33 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1044-5803 EI 1873-4189 J9 MATER CHARACT JI Mater. Charact. PD SEP PY 2014 VL 95 BP 18 EP 26 DI 10.1016/j.matchar.2014.06.004 PG 9 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Materials Science, Characterization & Testing SC Materials Science; Metallurgy & Metallurgical Engineering GA AO0HO UT WOS:000340989900003 ER PT J AU Sadat, ME Patel, R Sookoor, J Bud'ko, SL Ewing, RC Zhang, JM Xu, H Wang, YL Pauletti, GM Mast, DB Shi, DL AF Sadat, M. E. Patel, Ronak Sookoor, Jason Bud'ko, Sergey L. Ewing, Rodney C. Zhang, Jiaming Xu, Hong Wang, Yilong Pauletti, Giovanni M. Mast, David B. Shi, Donglu TI Effect of spatial confinement on magnetic hyperthermia via dipolar interactions in Fe3O4 nanoparticles for biomedical applications SO MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS LA English DT Article DE Fe3O4 nanoparticles; Magnetic anisotropy; Dipole interaction; Superparamagnetism; Neel relaxation ID IRON-OXIDE NANOPARTICLES; FLUID HYPERTHERMIA; ILLITE; FIELD; SIZE; RELAXATION; RATES; XRD AB In this work, the effect of nanoparticle confinement on the magnetic relaxation of iron oxide (Fe3O4) nanoparticles (NP) was investigated by measuring the hyperthermia heating behavior in high frequency alternating magnetic field. Three different Fe3O4 nanoparticle systems having distinct nanoparticle configurations were studied in terms of magnetic hyperthermia heating rate and DC magnetization, All magnetic nanoparticle (MNP) systems were constructed using equivalent similar to 10 nm diameter NP that were structured differently in terms of configuration, physical confinement, and interparticle spacing. The spatial confinement was achieved by embedding the Fe3O4 nanoparticles in the matrices of the polystyrene spheres of 100 nm, while the unconfined was the free Fe3O4 nanoparticles well-dispersed in the liquid via PAA surface coating. Assuming the identical core MNPs in each system, the heating behavior was analyzed in terms of particle freedom (or confinement), interparticle spacing, and magnetic coupling (or dipole-dipole interaction). DC magnetization data were correlated to the heating behavior with different material properties. Analysis of DC magnetization measurements showed deviation from classical Langevin behavior near saturation due to dipole interaction modification of the MNPs resulting in a high magnetic anisotropy. It was found that the Specific Absorption Rate (SAR) of the unconfined nanoparticle systems were significantly higher than those of confined (the MNPs embedded in the polystyrene matrix). This increase of SAR was found to be attributable to high Neel relaxation rate and hysteresis loss of the unconfined MNPs. It was also found that the dipole-dipole interactions can significantly reduce the global magnetic response of the MNPs and thereby decrease the SAR of the nanoparticle systems. (C) 2014 Elsevier B.V. All rights reserved. C1 [Sadat, M. E.; Mast, David B.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Patel, Ronak; Shi, Donglu] Univ Cincinnati, Coll Engn & Appl Sci, Dept Mech & Mat Engn, Mat Sci & Engn Program, Cincinnati, OH 45221 USA. [Sookoor, Jason] Univ Cincinnati, Dept Neurosci, Cincinnati, OH 45221 USA. [Bud'ko, Sergey L.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Bud'ko, Sergey L.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Ewing, Rodney C.; Zhang, Jiaming] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. [Xu, Hong; Shi, Donglu] Shanghai Jiao Tong Univ, Med X Inst, Shanghai 200030, Peoples R China. [Wang, Yilong; Shi, Donglu] Tongji Univ, Shanghai East Hosp, Sch Med, Inst Biomed Engn & Nano Sci, Shanghai 200120, Peoples R China. [Pauletti, Giovanni M.] Univ Cincinnati, James L Winkle Coll Pharm, Cincinnati, OH 45267 USA. RP Mast, DB (reprint author), Univ Cincinnati, Coll Engn & Appl Sci, 493 Rhodes Hall,ML72, Cincinnati, OH 45221 USA. EM donglu.shi@uc.edu RI Wang, Yilong/E-3536-2015; Pauletti, Giovanni M./I-5468-2015 OI Wang, Yilong/0000-0003-0677-8385; Pauletti, Giovanni M./0000-0002-0053-4964 FU Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; Shanghai Nanotechnology Promotion Center [11 nm0506100, 12nm0501201]; National Natural Science Foundation of China [51173135]; National Science Foundation [EEC-1343568] FX Work at the Ames Laboratory was supported by the Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. The work at Tongji University was supported by grants from Shanghai Nanotechnology Promotion Center (grant No. 11 nm0506100, 12nm0501201) and the National Natural Science Foundation of China (51173135). Research at the University of Cincinnati was partially supported by a grant from the National Science Foundation under contract No. EEC-1343568. The authors would like to thank Dr. Barry Maynard, Professor, Department of Geology, University of Cincinnati for the X-ray diffraction of the analyzed samples. NR 43 TC 30 Z9 30 U1 5 U2 52 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0928-4931 EI 1873-0191 J9 MAT SCI ENG C-MATER JI Mater. Sci. Eng. C-Mater. Biol. Appl. PD SEP 1 PY 2014 VL 42 BP 52 EP 63 DI 10.1016/j.msec.2014.04.064 PG 12 WC Materials Science, Biomaterials SC Materials Science GA AN6EJ UT WOS:000340687400009 PM 25063092 ER PT J AU Berezovski, A Tang, WX Wan, WS AF Berezovski, Arkadi Tang, Wen-Xin Wan, Weishi TI Elastic wave Talbot effect in solids with inclusions SO MECHANICS RESEARCH COMMUNICATIONS LA English DT Article DE Elastic waves; Talbot effect; Periodic grating; Numerical simulations ID THERMOELASTIC WAVE; PROPAGATION; INTERFEROMETRY; SYSTEMS; FRONT AB The numerical simulation of elastic wave propagation through a grating in a homogeneous medium shows the characteristic Talbot self-imaging effect. The size of the imaging and patterns can be controlled by changing the periodicity of grating and wavelength, respectively. It provides a novel route to modulate elastic wave distributions in solids with inclusions. Time dependent simulation suggests a long-distance elastic-wave-based interconnection in solids. An interferometer based on the elastic wave Talbot effect is discussed. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Berezovski, Arkadi] Tallinn Univ Technol, Ctr Nonlinear Studies, Inst Cybernet, EE-12618 Tallinn, Estonia. [Tang, Wen-Xin] Chongqing Univ, Coll Mat Sci & Engn, Chongqing 400030, Peoples R China. [Tang, Wen-Xin] Monash Univ, Sch Phys, Clayton, Vic 3800, Australia. [Wan, Weishi] Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Berezovski, A (reprint author), Tallinn Univ Technol, Ctr Nonlinear Studies, Inst Cybernet, Akad Tee 21, EE-12618 Tallinn, Estonia. EM Arkadi.Berezovski@cs.ioc.ee; wenxintang@cqu.edu.cn; wwan@lbl.gov RI Berezovski, Arkadi/C-8816-2009; Tang, Wen Xin/F-9929-2010 OI Berezovski, Arkadi/0000-0002-6574-9771; FU EU through European Regional Development Fund; Estonian Science Foundation [8702]; NSFC in China [11227802/A04] FX The research was supported by the EU through the European Regional Development Fund and by the Estonian Science Foundation (grant No. 8702) (AB). WXT and WW thank for the support by the NSFC (grant No. 11227802/A04) in China. WXT thanks David Paganin for useful discussions. NR 24 TC 2 Z9 2 U1 0 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0093-6413 J9 MECH RES COMMUN JI Mech. Res. Commun. PD SEP PY 2014 VL 60 BP 21 EP 26 DI 10.1016/j.mechrescom.2014.05.004 PG 6 WC Mechanics SC Mechanics GA AO0DV UT WOS:000340980200004 ER PT J AU Lee, Y Rivera, JGL Liao, JC AF Lee, Yun Rivera, Jimmy G. Lafontaine Liao, James C. TI Ensemble Modeling for Robustness Analysis in engineering non-native metabolic pathways SO METABOLIC ENGINEERING LA English DT Article DE Metabolic engineering; Synthetic biology; Ensemble Modeling; Robustness ID ESCHERICHIA-COLI; PHOSPHOROLYTIC CLEAVAGE; EXPANDING METABOLISM; MICROBIAL-PRODUCTION; NETWORKS; CHEMICALS; FUELS; FRUCTOSE-6-PHOSPHATE; PHOSPHOKETOLASE; BIOSYNTHESIS AB Metabolic pathways in cells must be sufficiently robust to tolerate fluctuations in expression levels and changes in environmental conditions. Perturbations in expression levels may lead to system failure due to the disappearance of a stable steady state. Increasing evidence has suggested that biological networks have evolved such that they are intrinsically robust in their network structure. In this article, we presented Ensemble Modeling for Robustness Analysis (EMRA), which combines a continuation method with the Ensemble Modeling approach, for investigating the robustness issue of non-native pathways. EMRA investigates a large ensemble of reference models with different parameters, and determines the effects of parameter drifting until a bifurcation point, beyond which a stable steady state disappears and system failure occurs. A pathway is considered to have high bifurcational robustness if the probability of system failure is low in the ensemble. To demonstrate the utility of EMRA, we investigate the bifurcational robustness of two synthetic central metabolic pathways that achieve carbon conservation: non-oxidative glycolysis and reverse glyoxylate cycle. With EMRA, we determined the probability of system failure of each design and demonstrated that alternative designs of these pathways indeed display varying degrees of bifurcational robustness. Furthermore, we demonstrated that target selection for flux improvement should consider the trade-offs between robustness and performance. (C) 2014 The Authors. Published by Elsevier Inc. On behalf of International Metabolic Engineering Society. C1 [Lee, Yun; Rivera, Jimmy G. Lafontaine; Liao, James C.] Univ Calif Los Angeles, Dept Chem & Biomol Engn, Los Angeles, CA 90095 USA. [Liao, James C.] Univ Calif Los Angeles, UCLA DOE Inst Genom & Proteom, Los Angeles, CA 90095 USA. RP Liao, JC (reprint author), Univ Calif Los Angeles, Dept Chem & Biomol Engn, 5531-G Boelter Hall, Los Angeles, CA 90095 USA. EM liaoj@ucla.edu FU National Science Foundation [MCB-1139318]; UCLA-DOE Institute for Genomics and Proteomics; Office of Science (BER), U.S. Department of Energy [DE-SC0008744, DE-SC0006698] FX This work was supported by National Science Foundation (MCB-1139318), UCLA-DOE Institute for Genomics and Proteomics, and the Office of Science (BER), U.S. Department of Energy (DE-SC0008744 and DE-SC0006698). NR 39 TC 15 Z9 16 U1 3 U2 39 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7176 EI 1096-7184 J9 METAB ENG JI Metab. Eng. PD SEP PY 2014 VL 25 BP 63 EP 71 DI 10.1016/j.ymben.2014.06.006 PG 9 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AO4ME UT WOS:000341312200007 PM 24972370 ER PT J AU Bormann, S Baer, ZC Sreekumar, S Kuchenreuther, JM Toste, FD Blanch, HW Clark, DS AF Bormann, Sebastian Baer, Zachary C. Sreekumar, Sanil Kuchenreuther, Jon M. Toste, F. Dean Blanch, Harvey W. Clark, Douglas S. TI Engineering Clostridium acetobutylicum for production of kerosene and diesel blendstock precursors SO METABOLIC ENGINEERING LA English DT Article DE Clostridium acetobutylicum; Biodiesel; Solvent tolerance; Heterogeneous catalysis; Butanol; Metabolic engineering ID MICROBIAL-PRODUCTION; ESCHERICHIA-COLI; BUTANOL; FERMENTATION; MOLECULES; STRAINS; PROTEIN; STRESS; FUELS; GENE AB Processes for the biotechnological production of kerosene and diesel blendstocks are often economically unattractive due to low yields and product titers. Recently, Clostridium acetobutylicutn fermentation products acetone, butane!, and ethanol (ABE) were shown to senie as precursors for catalytic upgrading to higher chainlength molecules that can be used as fuel substitutes. To produce suitable kerosene and diesel blendstocks, the butanokacetone ratio of fermentation products needs to be increased to 2-25:1, while ethanol production is minimized. Here we show that the overexpression of selected proteins changes the ratio of ABE products relative to the wild type ATCC 824 strain. Overexpression of the native alcohol/aldehyde dehydrogenase (AAD) has been reported to primarily increase ethanol formation in C acetobutylicum. We found that overexpression of the AAD'G variant increased ethanol titers by 294%. Catalytic upgrading of the 824(uud'"G) ABE products resulted in a blend with nearly 50 wt% < C9 products, which are unsuitable for diesel. To selectively increase butanol production, C beijerinckii aldehyde dehydrogenase and C ljungdhalii butanol dehydrogenase were co-expressed (strain designate 824(Cb old-CI bdh)), which increased butanol titers by 27% to 16.9 g while acetone and ethanol titers remained essentially unaffected. The solvent ratio from 824(Cb aid-Cl bdh) resulted in more than 80 wt% of catalysis products having a carbon chain length C11 which amounts to 9.8 g L-1 of products suitable as kerosene or diesel blendstock based on fermentation volume. To tiwther increase solvent production, we investigated expression of both native and heterologous chaperones in C acetobutylicum. Expression of a heat shock protein (HSP33) from Bacillus psychrosaccharolyticus increased the total solvent titer by 22%. Co-expression of HSP33 and alclehydelbutanol dehydrogenases further increased ABE formation as well as acetone and butanol yields. HSP33 was identified as the first heterologous chaperone that significantly increases solvent titers above wild type C acetobutylicurn levels, which can be combined with metabolic engineering to further increase solvent production. (C) 2014 International Metabolic Engineering Society. Published by Elsevier Inc. All rights reserved. C1 [Bormann, Sebastian; Baer, Zachary C.; Sreekumar, Sanil; Kuchenreuther, Jon M.; Toste, F. Dean; Blanch, Harvey W.; Clark, Douglas S.] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94720 USA. [Baer, Zachary C.; Kuchenreuther, Jon M.; Blanch, Harvey W.; Clark, Douglas S.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Sreekumar, Sanil; Toste, F. Dean] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Toste, F. Dean] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Toste, FD (reprint author), Univ Calif Berkeley, Dept Chem, 419 Latimer Hall, Berkeley, CA 94720 USA. EM fdtoste@berkeley.edu; blanch@berkeley.edu; clark@berkeley.edu FU Energy Biosciences Institute; PROMOS scholarship from DAAD FX Funding for this work was provided by the Energy Biosciences Institute to D.S.C., H.W.B. and F.D.T. S.B. was supported by a PROMOS scholarship from DAAD. NR 18 TC 12 Z9 13 U1 4 U2 42 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7176 EI 1096-7184 J9 METAB ENG JI Metab. Eng. PD SEP PY 2014 VL 25 BP 124 EP 130 DI 10.1016/j.ymben.2014.07.003 PG 7 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AO4ME UT WOS:000341312200013 PM 25046159 ER PT J AU Faney, T Wirth, BD AF Faney, T. Wirth, B. D. TI Spatially dependent cluster dynamics modeling of microstructure evolution in low energy helium irradiated tungsten SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE tungsten; helium; THDS; cluster dynamics; molecular dynamics ID IMPLANTATION; SIMULATION; RETENTION; DEFECTS; KRYPTON; METALS; HE AB In fusion reactors, plasma facing components (PFC) and in particular the divertor will be irradiated with high fluxes of low energy (similar to 100 eV) helium and hydrogen ions. Tungsten is one of the leading candidate divertor materials for ITER and DEMO fusion reactors. However, the behavior of tungsten under high dose, coupled helium/hydrogen exposure remains to be fully understood. The PFC response and performance changes are intimately related to microstructural changes, such as the formation of point defect clusters, helium and hydrogen bubbles or dislocation loops. Computational materials modeling has been used to investigate the mechanisms controlling microstructural evolution in tungsten following high dose, high temperature helium exposure. The aim of this study is to understand and predict helium implantation, primary defect production and defect diffusion, helium-defect clustering and interactions below a tungsten surface exposed to low energy helium irradiation. The important defects include interstitial clusters, vacancy clusters, helium interstitials and helium-vacancy clusters. We report results from a one-dimensional, spatially dependent cluster dynamics model based on the continuum reaction-diffusion rate theory to describe the evolution in space and time of all these defects. The key parameter inputs to the model (diffusion coefficients, migration and binding energies, initial defect production) are determined from a combination of atomistic materials modeling and available experimental data. C1 [Faney, T.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Wirth, B. D.] Univ Tennessee, Knoxville, TN USA. [Wirth, B. D.] Oak Ridge Natl Lab, Knoxville, TN USA. RP Faney, T (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. EM tibo@berkeley.edu RI Wirth, Brian/O-4878-2015 OI Wirth, Brian/0000-0002-0395-0285 FU US Department of Energy, Office of Fusion Energy Sciences [DE-SC00-02060]; Scientific Discovery through Advanced Computing program on Plasma Surface Interactions - US DOE, Office of Science, Advanced Scientific Computing Research and Fusion Energy Science FX The authors thank Dr Sergei Krasheninnikov (UCSD) for useful comments on the modeling work presented here, in addition to collaborative interactions with the PSI Plasma Science Center and the PSI SciDAC project. Financial support has been provided by the US Department of Energy, Office of Fusion Energy Sciences through grant DE-SC00-02060 and the Scientific Discovery through Advanced Computing program on Plasma Surface Interactions, funded by US DOE, Office of Science, Advanced Scientific Computing Research and Fusion Energy Science. NR 25 TC 9 Z9 9 U1 4 U2 39 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD SEP PY 2014 VL 22 IS 6 AR 065010 DI 10.1088/0965-0393/22/6/065010 PG 17 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AO3LO UT WOS:000341230900010 ER PT J AU Hu, XX Xu, DH Byun, TS Wirth, BD AF Hu, Xunxiang Xu, Donghua Byun, Thak Sang Wirth, Brian D. TI Modeling of irradiation hardening of iron after low-dose and low-temperature neutron irradiation SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE irradiation hardening; cluster dynamics model; dispersed barrier hardening model ID COPPER SINGLE-CRYSTALS; MOLECULAR-DYNAMICS SIMULATIONS; POINT-DEFECT CLUSTERS; MECHANICAL-PROPERTIES; TENSILE PROPERTIES; YIELD STRENGTH; FUSION POWER; ALPHA-IRON; BCC IRON; MICROSTRUCTURE AB Irradiation hardening is a prominent low-temperature degradation phenomena in materials, and is characterized both by an irradiation-induced increase in yield strength along with the loss of ductility. In this paper, a reaction-diffusion cluster dynamics model is used to predict the distribution of vacancy and interstitial clusters in iron following low-temperature (<373 K) and low-dose (<0.1 dpa) neutron irradiation. The predicted microstructure evolutions of high-purity iron samples are compared to published experimental data (positron annihilation spectroscopy and transmission electron microscopy) and show good agreement for neutron irradiation in this regime. The defect cluster distributions are then coupled to a dispersed barrier hardening model that assumes a strength factor, a, which varies with cluster type and size to compute the yield strength increase; the results of which agree reasonably well with tensile tests performed in previous studies. The modeling results presented here compare quite well to the experimental observations in the low-dose regime, and provide insight into the underlying microstructure-property relationships and the need for spatially dependent modeling to accurately predict the saturation behavior of yield strength changes observed experimentally at higher dose levels. C1 [Hu, Xunxiang; Xu, Donghua; Wirth, Brian D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Hu, Xunxiang; Byun, Thak Sang] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Hu, XX (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. EM hux1@ornl.gov RI Wirth, Brian/O-4878-2015; Hu, Xunxiang/N-3267-2016 OI Wirth, Brian/0000-0002-0395-0285; Hu, Xunxiang/0000-0002-4271-2327 FU US Department of Energy, Office of Fusion Energy Sciences [DE-FG02-04GR54750]; US Department of Energy, Office of Nuclear Energy's Nuclear Energy University Programs (NEUP) FX The aid and technical insight of Drs Kurt A Terrani and Yutai Katoh at ORNL is gratefully acknowledged, as is financial support from the US Department of Energy, Office of Fusion Energy Sciences under grant DE-FG02-04GR54750 and the US Department of Energy, Office of Nuclear Energy's Nuclear Energy University Programs (NEUP). NR 71 TC 6 Z9 6 U1 6 U2 33 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD SEP PY 2014 VL 22 IS 6 AR 065002 DI 10.1088/0965-0393/22/6/065002 PG 27 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AO3LO UT WOS:000341230900002 ER PT J AU Wilson, SR Mendelev, MI AF Wilson, S. R. Mendelev, M. I. TI Dependence of solid-liquid interface free energy on liquid structure SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE molecular dynamics simulation; solid-liquid interface; semi-empirical potentials ID INTERATOMIC POTENTIALS APPROPRIATE; RADIAL-DISTRIBUTION FUNCTION; VAPOR INTERFACE; MELTING-POINT; AL; MODEL; METALS; SOLIDIFICATION; SEGREGATION; SIMULATION AB The Turnbull relation is widely believed to enable prediction of solid-liquid interface (SLI) free energies from measurements of the latent heat and the solid density. Ewing proposed an additional contribution to the SLI free energy to account for variations in liquid structure near the interface. In the present study, molecular dynamics (MD) simulations were performed to investigate whether SLI free energy depends on liquid structure. Analysis of the MD simulation data for 11 fcc metals demonstrated that the Turnbull relation is only a rough approximation for highly ordered liquids, whereas much better agreement is observed with Ewing's theory. A modification to Ewing's relation is proposed in this study that was found to provide excellent agreement with MD simulation data. C1 [Wilson, S. R.; Mendelev, M. I.] Ames Lab, Div Engn & Mat Sci, Ames, IA 50011 USA. RP Wilson, SR (reprint author), Ames Lab, Div Engn & Mat Sci, Ames, IA 50011 USA. EM mendelev@ameslab.gov FU US Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; US Department of Energy [DE-AC02-07CH11358] FX The authors gratefully acknowledge very useful discussions with J J Hoyt who drew their attention to Ewing's original work. This work was supported by the US Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. The research was performed at the Ames Laboratory. Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No DE-AC02-07CH11358. NR 32 TC 2 Z9 2 U1 6 U2 41 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD SEP PY 2014 VL 22 IS 6 AR 065004 DI 10.1088/0965-0393/22/6/065004 PG 12 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AO3LO UT WOS:000341230900004 ER PT J AU Yang, L Ye, YT Fan, KM Shen, HH Peng, SM Long, XG Zhou, XS Zu, XT Gao, F AF Yang, L. Ye, Y. T. Fan, K. M. Shen, H. H. Peng, S. M. Long, X. G. Zhou, X. S. Zu, X. T. Gao, F. TI An ab initio-based Er-He interatomic potential in hcp Er SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE potential; helium; hcp Er; ab initio calculation ID AUGMENTED-WAVE METHOD; HELIUM; ERBIUM; SYSTEM; FILMS; IRON; CLUSTERS AB We have developed an empirical erbium-helium (Er-He) potential by fitting to the results calculated from the ab initio method. Based on the electronic hybridization between Er and He atoms, an s-band model, along with a repulsive pair potential, has been derived to describe the Er-He interaction. The atomic configurations and the formation energies of single He defects, small He interstitial clusters (He-n) and He-vacancy (HenV) clusters obtained by ab initio calculations are used as the fitting database. The binding energies and relative stabilities of the HnVm clusters are studied by the present potential and compared with the ab initio calculations. The Er-He potential is also applied to study the migration of He in hcp Er at different temperatures, and He clustering is found to occur at 600K in hcp Er crystal, which may be due to the anisotropic migration behavior of He interstitials. C1 [Yang, L.; Ye, Y. T.; Fan, K. M.; Shen, H. H.; Zu, X. T.; Gao, F.] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. [Fan, K. M.] Sichuan Univ Arts & Sci, Dept Phys & Engn Technol, Dazhou 635000, Peoples R China. [Peng, S. M.; Long, X. G.; Zhou, X. S.] China Acad Engn Phys, Inst Nucl Phys & Chem, Mianyang 621900, Peoples R China. [Gao, F.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Yang, L (reprint author), Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. EM yanglildk@uestc.edu.cn OI Shen, Huahai/0000-0002-0086-2714 FU National Natural Science Foundation of China-NSAF [10976007]; US Department of Fusion Energy Science [DE-AC06-76RLO 1830] FX L Yang and X T Zu are grateful for the support of the National Natural Science Foundation of China-NSAF (grant No 10976007). F Gao is grateful for the support of the US Department of Fusion Energy Science under Contract DE-AC06-76RLO 1830. NR 29 TC 4 Z9 4 U1 4 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD SEP PY 2014 VL 22 IS 6 AR 065009 DI 10.1088/0965-0393/22/6/065009 PG 13 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AO3LO UT WOS:000341230900009 ER PT J AU Mueller, RC Balasch, MM Kuske, CR AF Mueller, Rebecca C. Balasch, Monica M. Kuske, Cheryl R. TI Contrasting soil fungal community responses to experimental nitrogen addition using the large subunit rRNA taxonomic marker and cellobiohydrolase I functional marker SO MOLECULAR ECOLOGY LA English DT Article DE cellulose decomposition; fungi; nitrogen deposition; pine forest ID ELEVATED ATMOSPHERIC CO2; EXTRACELLULAR ENZYME-ACTIVITIES; MICROBIAL DIVERSITY; PHYLOGENETIC INFERENCE; TERRESTRIAL ECOSYSTEMS; ECTOMYCORRHIZAL FUNGI; LITTER DECOMPOSITION; ORGANIC-MATTER; FOREST SOIL; PINE FOREST AB Human activities have resulted in increased nitrogen inputs into terrestrial ecosystems, but the impact of nitrogen on ecosystem function, such as nutrient cycling, will depend at least in part on the response of soil fungal communities. We examined the response of soil fungi to experimental nitrogen addition in a loblolly pine forest (North Carolina, USA) using a taxonomic marker (large subunit rDNA, LSU) and a functional marker involved in a critical step of cellulose degradation (cellobiohydrolase, cbhI) at five time points that spanned fourteen months. Sampling date had no impact on fungal community richness or composition for either gene. Based on the LSU, nitrogen addition led to increased fungal community richness, reduced relative abundance of fungi in the phylum Basidiomycota and altered community composition; however, similar shifts were not observed with cbhI. Fungal community dissimilarity of the LSU and cbhI genes was significantly correlated in the ambient plots, but not in nitrogen-amended plots, suggesting either functional redundancy of fungi with the cbhI gene or shifts in other functional groups in response to nitrogen addition. To determine whether sequence similarity of cbhI could be predicted based on taxonomic relatedness of fungi, we conducted a phylogenetic analysis of publically available cbhI sequences from known isolates and found that for a subset of isolates, similar cbhI genes were found within distantly related fungal taxa. Together, these findings suggest that taxonomic shifts in the total fungal community do not necessarily result in changes in the functional diversity of fungi. C1 [Mueller, Rebecca C.; Balasch, Monica M.; Kuske, Cheryl R.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Kuske, CR (reprint author), Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87545 USA. EM Kuske@lanl.gov FU U.S. Department of energy (DOE), Biological and Environmental Science Division, through a Science Focus Area grant [2009LANLF260] FX This study was supported by the U.S. Department of energy (DOE), Biological and Environmental Science Division, through a Science Focus Area grant to CRK (2009LANLF260). Sanger DNA sequencing was conducted at Los Alamos National Laboratory, by the DOE Joint Genome Institute (JGI). The authors gratefully acknowledge the excellent technical expertise of Carolyn Weber and La Verne Gallegos-Graves and wish to thank Rytas Vilgalys, Robert B. Jackson, Charles 'Will' Cook, Terri M. Porter, Greg Bonito and several dedicated undergraduate students and postdocs for assistance with sample collection, storage and shipping. We acknowledge the DOE Terrestrial Carbon Processes Program and the Duke forest for operation of the FACE research site within the Duke forest. This is LANL unclassified report LA-UR-13-26783. NR 73 TC 5 Z9 5 U1 5 U2 51 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0962-1083 EI 1365-294X J9 MOL ECOL JI Mol. Ecol. PD SEP PY 2014 VL 23 IS 17 BP 4406 EP 4417 DI 10.1111/mec.12858 PG 12 WC Biochemistry & Molecular Biology; Ecology; Evolutionary Biology SC Biochemistry & Molecular Biology; Environmental Sciences & Ecology; Evolutionary Biology GA AO2SN UT WOS:000341176200019 PM 25039479 ER PT J AU Richter, H Peter, J Collis, S AF Richter, Harald Peter, Justin Collis, Scott TI Analysis of a Destructive Wind Storm on 16 November 2008 in Brisbane, Australia SO MONTHLY WEATHER REVIEW LA English DT Article ID SEVERE THUNDERSTORM EVENTS; POLARIMETRIC MEASUREMENTS; SUPERCELL THUNDERSTORM; PROXIMITY SOUNDINGS; UNITED-STATES; ENVIRONMENTS; MODEL; DEPOLARIZATION; PRECIPITATION; EVAPORATION AB During the late afternoon on 16 November 2008 the Brisbane (Queensland, Australia) suburb of "The Gap" experienced extensive wind damage caused by an intense local thunderstorm. The CP2 research radar nearby detected near-surface radial velocities exceeding 43 ms(-1) above The Gap while hail size reports did not exceed golf ball size, and no tornadoes were reported. The storm environment was characterized by a layer of very moist near-surface air and strong storm-relative low-level flow, whereas the storm-relative winds aloft were weak. While the thermodynamic storm environment contained a range of downdraft-promoting ingredients such as a similar to 4-km-high melting level above a similar to 2-km-deep layer with nearly dry-adiabatic lapse rates mostly collocated with dry ambient air, a similar to 1-km-deep stable layer near the ground would generally lower expectations of destructive surface winds based on the downburst mechanism. Once observed reflectivities exceed 70 dBZ, downdraft cooling due to hail melting and downdraft acceleration based on hail loading are found to likely become nonnegligible forcing mechanisms. The event featured the close proximity of a hydrostatically and dynamically driven mesobigh at the base of the downdraft to a dynamically driven mesolow associated with a low-level circulation. This proximity was instrumental in the anisotropic horizontal acceleration of the near-ground outflow and the ultimate strength of the Gap storm surface winds. Weak storm-relative midlevel winds are speculated to have allowed the downdraft to descend close to the low-level circulation, which set up this strong horizontal perturbation pressure gradient. C1 [Richter, Harald; Peter, Justin] Bur Meteorol, Ctr Australian Weather & Climate Res, Melbourne, Vic 3001, Australia. [Collis, Scott] Argonne Natl Lab, Div Environm Sci, Downers Grove Township, IL USA. RP Richter, H (reprint author), Bur Meteorol, Ctr Australian Weather & Climate Res, GPO Box 1289K, Melbourne, Vic 3001, Australia. EM h.richter@bom.gov.au OI Peter, Justin/0000-0002-6054-4873 FU Weather and Environmental Prediction (WEP) program as part of the Centre for Australian Weather and Climate Research (CAWCR); U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-06CH11357]; Office of Biological and Environmental Research (OBER) of the U.S. Department of Energy (DOE) as part of the ARM Program FX This study was supported by funding from the Weather and Environmental Prediction (WEP) program as part of the Centre for Australian Weather and Climate Research (CAWCR). In particular, the authors applaud Dr. Peter May for his continuous prodding and consequential advancement of the manuscript. The lead author would also like to thank various members of the VORTEX-2 team for discussions on wind storms with weak storm-relative midlevel winds. We also thank Matt Kumjian, Michael Coniglio, and an anonymous reviewer for substantially strengthening the initial manuscript.; Argonne National Laboratory's work was supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, under Contract DE-AC02-06CH11357. This work has been supported by the Office of Biological and Environmental Research (OBER) of the U.S. Department of Energy (DOE) as part of the ARM Program. NR 48 TC 6 Z9 6 U1 1 U2 10 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0027-0644 EI 1520-0493 J9 MON WEATHER REV JI Mon. Weather Rev. PD SEP PY 2014 VL 142 IS 9 BP 3038 EP 3060 DI 10.1175/MWR-D-13-00405.1 PG 23 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AO2QU UT WOS:000341171100002 ER PT J AU Chen, Y Lin, Y Zhang, YX Wang, SW Su, D Yang, ZB Han, MF Chen, FL AF Chen, Yu Lin, Ye Zhang, Yanxiang Wang, Siwei Su, Dong Yang, Zhibin Han, Minfang Chen, Fanglin TI Low temperature solid oxide fuel cells with hierarchically porous cathode nano-network SO NANO ENERGY LA English DT Article DE Low temperature solid oxide fuel cell; Freeze-drying combustion; Freeze-drying tape-casting; Nano-network ID HIGH-PERFORMANCE; COMBUSTION SYNTHESIS; ELECTRICAL-CONDUCTIVITY; MICROSTRUCTURE; POLARIZATION; SOFCS; CERIA; MODEL AB Cost and reliability of solid oxide fuel cell (SOFC) system resulting from high operating temperature severely hinders its wide-spread commercialization. In this study, high performance low temperature SOFCs with hierarchically porous nano cathode network (Sm0.5Sr0.5CoO3-Gd0.1Ce0.9O2-delta, SSC-GDC) have been fabricated by vacuum-free infiltration and subsequent freeze-drying combustion. The straight open GDC cathode skeleton and NiO-GDC anode substrate prepared by freeze-drying tape-casting facilitate mass transport while the nano cathode catalyst promotes the electrochemical reactions. The cell with straight open electrodes and hierarchically porous cathode network demonstrates a maximum power density of 0.65 W cm(-2) at 500 degrees C and impressive stability for more than 500 h at 400 degrees C using H-2 as fuel and ambient air as oxidant. The simple and cost-effective fabrication process is expected to significantly impact the SOFC operability and accelerate its commercialization. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Chen, Yu; Lin, Ye; Zhang, Yanxiang; Wang, Siwei; Chen, Fanglin] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. [Zhang, Yanxiang] Harbin Inst Technol, Sch Mat Sci & Engn, Harbin 150001, Heilongjiang, Peoples R China. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Yang, Zhibin; Han, Minfang] China Univ Min & Technol, Sch Chem & Environm Engn, Beijing 100083, Peoples R China. RP Han, MF (reprint author), China Univ Min & Technol, Sch Chem & Environm Engn, Beijing 100083, Peoples R China. EM hanminfang@sina.com; chenfa@cec.sc.edu RI 杨, 志宾/B-2311-2015; Chen, Fanglin/K-1039-2012; Liu, Tong/N-7904-2013; Zhang, Yan Xiang/A-7604-2013; Su, Dong/A-8233-2013; OI 杨, 志宾/0000-0003-3845-1133; Chen, Fanglin/0000-0001-9942-8872; Liu, Tong/0000-0001-5311-9687; Zhang, Yan Xiang/0000-0002-9318-0324; Su, Dong/0000-0002-1921-6683; Lin, Ye/0000-0003-4289-894X FU U.S. National Science Foundation [DMR-1210792]; National Basic Research Program of China (973 Program) [2012CB215400]; NSFC-NSF China-US International Cooperation Project [51261120378]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We are grateful to the financial support from the U.S. National Science Foundation (DMR-1210792), National Basic Research Program of China (973 Program, 2012CB215400) and NSFC-NSF China-US International Cooperation Project (51261120378). TEM work has been carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract no. DE-AC02-98CH10886. NR 31 TC 39 Z9 39 U1 14 U2 114 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 J9 NANO ENERGY JI Nano Energy PD SEP PY 2014 VL 8 BP 25 EP 33 DI 10.1016/j.nanoen.2014.05.010 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AO0EK UT WOS:000340981700004 ER PT J AU Wang, HY Qian, F Li, Y AF Wang, Hanyu Qian, Fang Li, Yat TI Solar-assisted microbial fuel cells for bioelectricity and chemical fuel generation SO NANO ENERGY LA English DT Review DE Microbial fuel cell; Microbial electrogenesis; Bioelectricity; Hydrogen; Wastewater treatment; Energy recovery ID WASTE-WATER TREATMENT; ELECTRICITY-GENERATION; ELECTROLYSIS CELLS; HYDROGEN-PRODUCTION; ENERGY-CONVERSION; CATHODE MATERIALS; HALF CELL; PERFORMANCE; ELECTRODES; GEOBACTER AB Microbial fuel cell (MFC) is an electrochemical device that uses electrogenic bacteria as biocatalysts to decompose organic matter while simultaneously generating bioelectricity. Besides electricity, the bio-electrons generated in the microbial electrogenesis process at the anode can also be used to produce chemical fuels, such as hydrogen gas. However, microbial electrohydrogenesis process does not occur spontaneously due to the thermodynamic barrier for the conversion from protons to hydrogen gas, and therefore an electrical bias has to be supplied to supplement the energy required for the proton reduction. The requirement of external bias adds to the complexity and cost for hydrogen production, making microbial electrohydrogenesis less attractive as a cost-effective energy solution. Alternatively, the energy required to overcome the barrier can be provided by a renewable energy source such as solar light, which is a promising approach that could fundamentally address this issue. Recently, a number of solar-assisted microbial fuel cells have been demonstrated by coupling the conventional MFC with photosynthetic bacteria, semiconductor photoelectrodes, solar cell or photoelectrochemical cell. In these devices, solar energy was utilized to facilitate bioelectricity or hydrogen generation. The demonstration of these new solar-assisted MFC devices opens up new opportunities in the recovery of chemical energy in wastewater for chemical fuel production. This article highlights the recent accomplishments in the solar-assisted MFC technology and discusses the current challenges and future opportunities in the field. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Wang, Hanyu; Li, Yat] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. [Qian, Fang] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Li, Y (reprint author), Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. EM yli@chemistry.ucsc.edu OI Li, Yat/0000-0002-8058-2084 FU US. NSF [CBET103 4222]; LDRD of the U.S. Department of Energy by Lawrence Livermore National Laboratory [11 LW-054, DEAC52-07NA27344] FX Y.L. acknowledges financial support from US. NSF (CBET103 4222). F.Q. acknowledges support from LDRD Project 11 LW-054, performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DEAC52-07NA27344. NR 77 TC 8 Z9 9 U1 18 U2 126 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 EI 2211-3282 J9 NANO ENERGY JI Nano Energy PD SEP PY 2014 VL 8 BP 264 EP 273 DI 10.1016/j.nanoen.2014.06.004 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AO0EK UT WOS:000340981700032 ER PT J AU Lee, JH Luo, G Tung, IC Chang, SH Luo, Z Malshe, M Gadre, M Bhattacharya, A Nakhmanson, SM Eastman, JA Hong, H Jellinek, J Morgan, D Fong, DD Freeland, JW AF Lee, J. H. Luo, G. Tung, I. C. Chang, S. H. Luo, Z. Malshe, M. Gadre, M. Bhattacharya, A. Nakhmanson, S. M. Eastman, J. A. Hong, H. Jellinek, J. Morgan, D. Fong, D. D. Freeland, J. W. TI Dynamic layer rearrangement during growth of layered oxide films by molecular beam epitaxy SO NATURE MATERIALS LA English DT Article ID RUDDLESDEN-POPPER COMPOUNDS; TOTAL-ENERGY CALCULATIONS; TITANIUM-OXYGEN SYSTEM; WAVE BASIS-SET; THIN-FILMS; DEPOSITION; FERROELECTRICITY; HETEROSTRUCTURES; PEROVSKITES; INTERFACES AB The A(n+1)B(n)O(3n+1) Ruddlesden-Popper homologous series offers a wide variety of functionalities including dielectric, ferroelectric, magnetic and catalytic properties. Unfortunately, the synthesis of such layered oxides has been a major challenge owing to the occurrence of growth defects that result in poor materials behaviour in the higher-order members. To understand the fundamental physics of layered oxide growth, we have developed an oxide molecular beam epitaxy system with in situ synchrotron X-ray scattering capability. We present results demonstrating that layered oxide films can dynamically rearrange during growth, leading to structures that are highly unexpected on the basis of the intended layer sequencing. Theoretical calculations indicate that rearrangement can occur in many layered oxide systems and suggest a general approach that may be essential for the construction of metastable Ruddlesden-Popper phases. We demonstrate the utility of the new-found growth strategy by performing the first atomically controlled synthesis of single-crystalline La3Ni2O7. C1 [Lee, J. H.; Tung, I. C.; Hong, H.; Freeland, J. W.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Luo, G.; Gadre, M.; Morgan, D.] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Tung, I. C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Chang, S. H.; Luo, Z.; Bhattacharya, A.; Eastman, J. A.; Fong, D. D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Luo, Z.] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China. [Malshe, M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Bhattacharya, A.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Nakhmanson, S. M.] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Nakhmanson, S. M.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. RP Lee, JH (reprint author), Korea Atom Energy Res Inst, Div Neutron Sci, Taejon 305600, South Korea. EM ddmorgan@wisc.edu; freeland@anl.gov RI Bhattacharya, Anand/G-1645-2011; luo, zhenlin/G-2662-2013; Luo, Guangfu/E-3119-2012; OI Bhattacharya, Anand/0000-0002-6839-6860; Eastman, Jeff/0000-0002-0847-4265 FU US. Department of Energy, Office of Science, Materials Sciences and Engineering Division; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; DOE; University of Wisconsin Materials Research Science and Engineering Center [DMR-1121288]; [CNM29783]; [CNM35702] FX The authors acknowledge discussions with D. G. Schlom, K. Lee and Y. Nie, and support at the APS from H. Zhou and C. Schleputz. S.H.C., J.A.E., A.B. and D.D.F. were supported by the US. Department of Energy, Office of Science, Materials Sciences and Engineering Division. Work performed at Argonne National Laboratory, including the Advanced Photon Source, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. The calculations were carried out on the Fusion Cluster of Argonne's Laboratory Computing Resource Center, at NERSC (supported by DOE), and on Argonne's Carbon Cluster under award CNM29783 and CNM35702. D.M. and G.L. were partially supported by University of Wisconsin Materials Research Science and Engineering Center (DMR-1121288). NR 33 TC 45 Z9 45 U1 11 U2 125 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD SEP PY 2014 VL 13 IS 9 BP 879 EP 883 DI 10.1038/NMAT4039 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AO4XA UT WOS:000341343500019 PM 25087067 ER PT J AU Mitchell, E Gupta, RK Mensah-Darkwa, K Kumar, D Ramasamy, K Gupta, BK Kahol, P AF Mitchell, Elias Gupta, Ram K. Mensah-Darkwa, Kwadwo Kumar, Dhananjay Ramasamy, Karthik Gupta, Bipin K. Kahol, Pawan TI Facile synthesis and morphogenesis of superparamagnetic iron oxide nanoparticles for high-performance supercapacitor applications SO NEW JOURNAL OF CHEMISTRY LA English DT Article ID LITHIUM-ION BATTERIES; FE3O4 NANOPARTICLES; ELECTRODE MATERIALS; ELECTROCHEMICAL CAPACITORS; HYDROTHERMAL SYNTHESIS; MAGNETIC-PROPERTIES; ENERGY-STORAGE; ULTRACAPACITORS; NANOCOMPOSITE; FABRICATION AB A facile method has been developed for the synthesis of nearly mono-dispersed iron oxide nanocrystals. The structural analysis of the synthesized iron oxide nanocrystals reveals the magnetite phase of Fe3O4. The average particle size of the iron oxide was estimated to be 8 +/- 2 nm. The observed particle size is in good correlation with the particle size estimated by magnetic measurements. Furthermore, these nanocrystals showed bi-functional ferromagnetic and superparamagnetic behavior below and above the blocking temperature, respectively. The potential use of these nanocrystals as an electrode for supercapacitors was examined by investigating the electrochemical behavior of iron oxide using cyclic voltammetry (CV) and galvanostatic charge-discharge tests. The CV characteristics of the iron oxide electrode showed a typical pseudocapacitive behavior in 3 M KOH solution. Moreover, the specific capacitance of 185 F g(-1) at the current of 1 mA was observed with excellent cyclic stability, which is much higher than the reported value for iron oxide. The higher specific capacitance is due to the uniform nano-size of iron oxide. This work provides an ultimate facile method to synthesize nanostructured iron oxide for application in next generation energy storage materials. C1 [Mitchell, Elias; Gupta, Ram K.] Pittsburg State Univ, Dept Chem, Pittsburg, KS 66762 USA. [Mensah-Darkwa, Kwadwo] Kwame Nkrumah Univ Sci & Technol, Dept Mat Engn, Pmb Kumasi, Ghana. [Kumar, Dhananjay] North Carolina A&T State Univ, Dept Mech Engn, Greensboro, NC 27411 USA. [Ramasamy, Karthik] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Gupta, Bipin K.] Natl Phys Lab CSIR, New Delhi 110012, India. [Kahol, Pawan] Pittsburg State Univ, Dept Phys, Pittsburg, KS 66762 USA. RP Gupta, RK (reprint author), Pittsburg State Univ, Dept Chem, 1701 S Broadway, Pittsburg, KS 66762 USA. EM ramguptamsu@gmail.com NR 41 TC 23 Z9 23 U1 8 U2 98 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1144-0546 EI 1369-9261 J9 NEW J CHEM JI New J. Chem. PD SEP PY 2014 VL 38 IS 9 BP 4344 EP 4350 DI 10.1039/c4nj00741g PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA AO1IM UT WOS:000341065800038 ER PT J AU Andrews, MT Goorley, JT Corcoran, EC Kelly, DG AF Andrews, M. T. Goorley, J. T. Corcoran, E. C. Kelly, D. G. TI MODELING THE DETECTION OF DELAYED NEUTRON SIGNATURES IN MCNP6 AND COMPARISONS WITH MEASUREMENTS OF U-233, U-235, AND (PU)-P-239 SO NUCLEAR TECHNOLOGY LA English DT Article DE MCNP6; delayed neutron; nuclear instrumentation AB Study of the magnitude and temporal behavior of delayed neutrons (DNs) enables the identification of fissile isotopes and a determination of their relative quantities. Thus, the ability to model accurately these neutrons and the methods of their detection is of relevance to nuclear forensics and counterterrorism. The capability of MCNP6 to model these emissions was examined and compared to measurements of the DNs produced by U-233, U-235, and Pu-239 after neutron-induced fission. Fissile samples were irradiated in a SLOWPOKE-2 research reactor for 60 s and were then conveyed via pneumatic tubing to an array of six(3)He detectors embedded in a paraffin moderator. Several MCNP6 input files were created to reproduce irradiation conditions, temporal DN emission, and the detection arrangement. Nuclear reactions and other effects within the He-3 detectors were reproduced by MCNP6, and detection efficiencies of this modeled arrangement determined by MCNP6 were in agreement with experimental measurements. Finally, the library and model DN emission options in the MCNP6v1 release were evaluated and compared to the measured magnitudes and temporal behavior of U-233, U-235, and Pu-239. Significant discrepancies observed between the DN model option and measurements for count times >100 s are discussed. C1 [Andrews, M. T.; Corcoran, E. C.; Kelly, D. G.] Royal Mil Coll Canada, Kingston, ON K7K 7B4, Canada. [Andrews, M. T.; Goorley, J. T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Andrews, MT (reprint author), Royal Mil Coll Canada, POB 17000 Stn Forces, Kingston, ON K7K 7B4, Canada. EM jgoorley@lanl.gov FU Advanced Simulation and Computing program at Los Alamos National Laboratory; Director General of Environment and Nuclear Safety; Natural Sciences and Engineering Research Council of Canada FX Funding was provided by the Advanced Simulation and Computing program at Los Alamos National Laboratory, the Director General of Environment and Nuclear Safety, and the Natural Sciences and Engineering Research Council of Canada. The authors would like to thank K. Nielsen and D. Ferguson for assisting in experimentation for this project. Also, the technical work of S. White, J. Shaw, M. Mackay, and C. McEwen is greatly appreciated. Finally, the authors appreciate the feedback and input from both reviewers of this paper. NR 20 TC 2 Z9 2 U1 0 U2 3 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD SEP PY 2014 VL 187 IS 3 BP 235 EP 242 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AO1LY UT WOS:000341074800002 ER PT J AU Harp, DR Stauffer, PH Mishra, PK Levitt, DG Robinson, BA AF Harp, Dylan R. Stauffer, Philip H. Mishra, Phoolendra K. Levitt, Daniel G. Robinson, Bruce A. TI THERMAL MODELING OF HIGH-LEVEL NUCLEAR WASTE DISPOSAL IN A SALT REPOSITORY SO NUCLEAR TECHNOLOGY LA English DT Article DE salt; waste; thermal AB Salt formations have received recent attention for geologic disposal of heat-generating, high-level nuclear waste (HLW). Existing investigations are summarized and expanded upon using analytical and numerical models to investigate simulated temperatures in the salt after emplacement of HLW. Analytical modeling suggests that temperature variations near canisters will be smooth, indicating that the system can be approximated by a coarsely discretized numerical model. Two multidimensional parameter studies explore canister configuration using characteristics from (a) defense HLW and (b) spent nuclear fuel (SNF) waste. Numerical modeling was conducted for a disposal concept consisting of emplacement of waste canisters on the floor of drifts and covering each with salt backfill. Results indicate that waste forms with U.S. Department of Energy (DOE) waste characteristics can be easily configured to maintain simulated temperatures far below 200 degrees C at spacings as close as 0.3 m (similar to 1 ft), the minimum feasible spacing that could practically be achieved. For SNF waste packaged into canisters with heat loads of 1500 or 1000 W with canister spacing of 6 m (similar to 20 ft) and 3 m (similar to 10 ft), respectively, simulated temperatures can be maintained below 200 degrees C; much higher maximum temperatures would result for designs with higher canister heat loads and smaller spacings. These results indicate that from a thermal loading perspective, in-drift disposal of HLW in salt deposits is feasible for DOE-managed waste as long as the maximum temperature is managed through proper selection of canister heat loads and spacings. The results will aid in the design of potential future field tests to confirm this conclusion. C1 [Harp, Dylan R.; Stauffer, Philip H.; Mishra, Phoolendra K.; Levitt, Daniel G.; Robinson, Bruce A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Harp, DR (reprint author), Los Alamos Natl Lab, POB 1663,MS T003, Los Alamos, NM 87545 USA. EM dharp@lanl.gov OI Harp, Dylan/0000-0001-9777-8000; Stauffer, Philip/0000-0002-6976-221X FU Used Fuel Disposition Campaign, Office of Nuclear Energy, of the DOE FX Funding for this work was provided by the Used Fuel Disposition Campaign, Office of Nuclear Energy, of the DOE. NR 15 TC 0 Z9 0 U1 0 U2 4 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD SEP PY 2014 VL 187 IS 3 BP 294 EP 307 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AO1LY UT WOS:000341074800007 ER PT J AU Unruh, T Chase, B Rempe, J Nigg, D Imel, G Harris, J Sherman, T Villard, JF AF Unruh, Troy Chase, Benjamin Rempe, Joy Nigg, David Imel, George Harris, Jason Sherman, Todd Villard, Jean-Francois TI IN-CORE FLUX SENSOR EVALUATIONS AT THE ATR CRITICAL FACILITY SO NUCLEAR TECHNOLOGY LA English DT Article DE in-core instrumentation; flux detector; self-powered neutron detector ID REACTOR AB As part of an Idaho State University (ISU)-led Advanced Test Reactor (ATR) National Scientific User Facility (NSUF) collaborative project that includes Idaho National Laboratory (INL) and the French Alternative Energies and Atomic Energy Commission (CEA), flux detector evaluations were completed to compare their accuracy, response time, and long-duration performance. Special fixturing, developed by INL, allows real-time flux detectors to be inserted into various Advanced Test Reactor Critical Facility (ATRC) core positions to perform lobe power measurements, axial flux profile measurements, and detector cross-calibrations. Detectors initially evaluated in this program included miniature fission chambers, specialized self-powered neutron detectors (SPNDs), and specially developed commercial SPNDs. Results from this program provide important insights related to flux detector accuracy and resolution for subsequent ATR and CEA experiments and yield new flux data required for benchmarking models in the ATR Life Extension Program (LEP) Modeling Update Project. C1 [Unruh, Troy; Chase, Benjamin; Rempe, Joy; Nigg, David] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Imel, George; Harris, Jason; Sherman, Todd] Idaho State Univ, Pocatello, ID 83209 USA. [Villard, Jean-Francois] CEA, DEN, DER, Instrumentat Sensors & Dosimetry Lab, Cadarache, France. RP Unruh, T (reprint author), Idaho Natl Lab, POB 1625,MS 3531, Idaho Falls, ID 83415 USA. EM Troy.Unruh@inl.gov OI Rempe, Joy/0000-0001-5527-3549 FU U.S. Department of Energy, Office of Nuclear Energy, Science, and Technology, under DOE-NE Idaho Operations Office [DE AC07 05ID14517] FX This work is supported by the U.S. Department of Energy, Office of Nuclear Energy, Science, and Technology, under DOE-NE Idaho Operations Office contract DE AC07 05ID14517. NR 8 TC 1 Z9 1 U1 0 U2 5 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD SEP PY 2014 VL 187 IS 3 BP 308 EP 315 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AO1LY UT WOS:000341074800008 ER PT J AU Gatta, GD Morgenroth, W Dera, P Petitgirard, S Liermann, HP AF Gatta, G. D. Morgenroth, W. Dera, P. Petitgirard, S. Liermann, H. -P. TI Elastic behavior and pressure-induced structure evolution of topaz up to 45 GPa SO PHYSICS AND CHEMISTRY OF MINERALS LA English DT Article DE Topaz; High pressure; Single-crystal synchrotron X-ray diffraction; Compressibility; Structure refinement ID NEUTRON POWDER DIFFRACTION; OH-RICH TOPAZ; CRYSTAL-STRUCTURE; THERMODYNAMIC PROPERTIES; EASTERN CHINA; PHASE EGG; STABILITY; AL2SIO4(OH)2; REFINEMENT; DEPENDENCE AB The behavior of a natural topaz, Al2.00Si1.05O4.00(OH0.26F1.75), has been investigated by means of in situ single-crystal synchrotron X-ray diffraction up to 45 GPa. No phase transition or change in the compressional regime has been observed within the pressure-range investigated. The compressional behavior was described with a third-order Birch-Murnaghan equation of state (III-BM-EoS). The III-BM-EoS parameters, simultaneously refined using the data weighted by the uncertainties in P and V, are as follows: K (V) = 158(4) GPa and K (V) ' = 3.3(3). The confidence ellipse at 68.3 % (Delta chi(2) = 2.30, 1 sigma) was calculated starting from the variance-covariance matrix of K (V) and K' obtained from the III-BM-EoS least-square procedure. The ellipse is elongated with a negative slope, indicating a negative correlation of the parameters K (V) and K (V) ', with K (V) = 158 +/- A 6 GPa and K (V) ' = 3.3 +/- A 4. A linearized III-BM-EoS was used to obtain the axial-EoS parameters (at room-P), yielding: K(a) = 146(5) GPa [beta (a) = 1/(3K(a)) = 0.00228(6) GPa(-1)] and K'(a) = 4.6(3) for the a-axis; K(b) = 220(4) GPa [beta (b) = 0.00152(4) GPa(-1)] and K'(b) = 2.6(3) for the b-axis; K(c) = 132(4) GPa [beta (c) = 0.00252(7) GPa(-1)] and K'(c) = 3.3(3) for the c-axis. The elastic anisotropy of topaz at room-P can be expressed as: K(a):K(b):K(c) = 1.10:1.67:1.00 (beta (a):beta (b):beta (c) = 1.50:1.00:1.66). A series of structure refinements have been performed based on the intensity data collected at high pressure, showing that the P-induced structure evolution at the atomic scale is mainly represented by polyhedral compression along with inter-polyhedral tilting. A comparative analysis of the elastic behavior and P/T-stability of topaz polymorphs and "phase egg" (i.e., AlSiO3OH) is carried out. C1 [Gatta, G. D.] Univ Milan, Dipartimento Sci Terra, I-20133 Milan, Italy. [Gatta, G. D.] CNR, Ist Cristallog, I-70126 Bari, Italy. [Morgenroth, W.] Goethe Univ Frankfurt, Inst Geowissensch, Abt Kristallog, D-60438 Frankfurt, Germany. [Dera, P.] Univ Chicago, Argonne Natl Lab, Ctr Adv Radiat Sources, Argonne, IL USA. [Petitgirard, S.; Liermann, H. -P.] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany. [Petitgirard, S.] Univ Bayreuth, Bayer GeoInst BGI, D-95444 Bayreuth, Germany. RP Gatta, GD (reprint author), Univ Milan, Dipartimento Sci Terra, Via Botticelli 23, I-20133 Milan, Italy. EM diego.gatta@unimi.it OI Gatta, G. Diego/0000-0001-8348-7181; Morgenroth, Wolfgang/0000-0001-8921-0052 FU National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-Geosciences [DE-FG02-94ER14466]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Italian MIUR [2008SPZ743]; BMBF [05KS7RF1, 05K10RFA, 05K13RF1] FX This work was performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (EAR-1128799) and Department of Energy-Geosciences (DE-FG02-94ER14466). Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. GDG acknowledges the Italian MIUR Grant No. 2008SPZ743. WM acknowledges support by BMBF projects 05KS7RF1, 05K10RFA, and 05K13RF1. Milan Rieder and two anonymous reviewers are thanked. NR 38 TC 2 Z9 2 U1 1 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0342-1791 EI 1432-2021 J9 PHYS CHEM MINER JI Phys. Chem. Miner. PD SEP PY 2014 VL 41 IS 8 BP 569 EP 577 DI 10.1007/s00269-014-0670-4 PG 9 WC Materials Science, Multidisciplinary; Mineralogy SC Materials Science; Mineralogy GA AN8XQ UT WOS:000340889700001 ER PT J AU El Mehdawi, AF Reynolds, RJB Prins, CN Lindblom, SD Cappa, JJ Fakra, SC Pilon-Smits, EAH AF El Mehdawi, Ali F. Reynolds, Ray Jason B. Prins, Christine N. Lindblom, Stormy D. Cappa, Jennifer J. Fakra, Sirine C. Pilon-Smits, Elizabeth A. H. TI Analysis of selenium accumulation, speciation and tolerance of potential selenium hyperaccumulator Symphyotrichum ericoides SO PHYSIOLOGIA PLANTARUM LA English DT Article ID PRAIRIE DOG HERBIVORY; STANLEYA-PINNATA; HIGHER-PLANTS; ASTRAGALUS-BISULCATUS; PROTECTS PLANTS; INDIAN MUSTARD; TOXICITY; SULFUR; ARABIDOPSIS; NONACCUMULATORS AB Symphyotrichum ericoides was shown earlier to contain hyperaccumulator levels of selenium (Se) in the field (>1000 mg kg(-1) dry weight (DW)), but only when growing next to other Se hyperaccumulators. It was also twofold larger next to hyperaccumulators and suffered less herbivory. This raised two questions: whether S. ericoides is capable of hyperaccumulation without neighbor assistance, and whether its Se-derived benefit is merely ecological or also physiological. Here, in a comparative greenhouse study, Se accumulation and tolerance of S. ericoides were analyzed in parallel with hyperaccumulator Astragalus bisulcatus, Se accumulator Brassica juncea and related Asteraceae Machaeranthera tanacetifolia. Symphyotrichum ericoides and M. tanacetifolia accumulated Se up to 3000 and 1500 mg Se kg-1 DW, respectively. They were completely tolerant to these Se levels and even grew 1.5- to 2.5-fold larger with Se. Symphyotrichum ericoides showed very high leaf Se/sulfur (S) and shoot/root Se concentration ratios, similar to A. bisulcatus and higher than M. tanacetifolia and B. juncea. Se X-ray absorption near-edge structure spectroscopy showed that S. ericoides accumulated Se predominantly (86%) as C-Se-C compounds indistinguishable from methyl-selenocysteine, which may explain its Se tolerance. Machaeranthera tanacetifolia accumulated 55% of its Se as C-Se-C compounds; the remainder was inorganic Se. Thus, in this greenhouse study S. ericoides displayed all of the characteristics of a hyperaccumulator. The larger size of S. ericoides when growing next to hyperaccumulators may be explained by a physiological benefit, in addition to the ecological benefit demonstrated earlier. C1 [El Mehdawi, Ali F.; Reynolds, Ray Jason B.; Prins, Christine N.; Lindblom, Stormy D.; Cappa, Jennifer J.; Pilon-Smits, Elizabeth A. H.] Colorado State Univ, Dept Biol, Ft Collins, CO 80523 USA. [Fakra, Sirine C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Pilon-Smits, EAH (reprint author), Colorado State Univ, Dept Biol, Ft Collins, CO 80523 USA. EM epsmits@lamar.colostate.edu FU National Science Foundation [IOS-0817748]; Libyan government; Office of Science, Basic Energy Sciences, and Division of Materials Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Funding for these studies was provided by National Science Foundation grant # IOS-0817748 to E. A. H. P.-S. and a graduate fellowship from the Libyan government to A. F. E. M. The Advanced Light Source is supported by the Office of Science, Basic Energy Sciences, and Division of Materials Science of the U.S. Department of Energy (DE-AC02-05CH11231). NR 43 TC 4 Z9 4 U1 3 U2 35 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0031-9317 EI 1399-3054 J9 PHYSIOL PLANTARUM JI Physiol. Plant. PD SEP PY 2014 VL 152 IS 1 BP 70 EP 83 DI 10.1111/ppl.12149 PG 14 WC Plant Sciences SC Plant Sciences GA AN6CU UT WOS:000340682100006 PM 24423113 ER PT J AU Holmes, HR DeRouin, A Wright, S Riedemann, TM Lograsso, TA Rajachar, RM Ong, KG AF Holmes, Hal R. DeRouin, Andrew Wright, Samantha Riedemann, Travor M. Lograsso, Thomas A. Rajachar, Rupak M. Ong, Keat Ghee TI Biodegradation and biocompatibility of mechanically active magnetoelastic materials SO SMART MATERIALS AND STRUCTURES LA English DT Article DE magnetoelastic; implant; degradation ID FLUID-FLOW VELOCITY; THICK-FILM SENSORS; VISCOSITY; BIOMATERIALS; TEMPERATURE; TOXICITY; PRESSURE; DENSITY AB Magnetoelastic (ME) materials have many advantages for use as sensors and actuators due to their wireless, passive nature. This paper describes the application of ME materials as biodegradable implants with controllable degradation rates. Experiments have been conducted to show that degradation rates of ME materials are dependent on the material compositions. In addition, it was shown that the degradation rates of the ME materials can be controlled remotely by applying a magnetic field, which causes the ME materials to generate low-magnitude vibrations that hasten their degradation rates. Another concern of ME materials for medical applications is biocompatibility. Indirect cytotoxicity analyses were performed on two types of ME materials: Metglas (TM) 2826 MB (FeNiMoB) and iron-gallium alloy. While results indicate Metglas is not biocompatible, the degradation products of iron-gallium materials have shown no adverse effects on cell viability. Overall, these results present the possibility of using ME materials as biodegradable, magnetically-controlled active implants. C1 [Holmes, Hal R.; DeRouin, Andrew; Wright, Samantha; Rajachar, Rupak M.; Ong, Keat Ghee] Michigan Technol Univ, Dept Biomed Engn, Houghton, MI 49931 USA. [Riedemann, Travor M.; Lograsso, Thomas A.] US DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA. [Lograsso, Thomas A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Holmes, HR (reprint author), Michigan Technol Univ, Dept Biomed Engn, Houghton, MI 49931 USA. EM kgong@mtu.edu FU DOE Office of Science, Basic Sciences, Materials Sciences and Engineering Division [DE-AC07CH11358] FX The authors of this work would like to recognize Dr Megan Frost (MTU) for the use of her equipment during the degradation study. TRM and TAL acknowledge the support of DOE Office of Science, Basic Sciences, Materials Sciences and Engineering Division under Contract No. DE-AC07CH11358. NR 19 TC 4 Z9 4 U1 3 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0964-1726 EI 1361-665X J9 SMART MATER STRUCT JI Smart Mater. Struct. PD SEP PY 2014 VL 23 IS 9 AR 095036 DI 10.1088/0964-1726/23/9/095036 PG 5 WC Instruments & Instrumentation; Materials Science, Multidisciplinary SC Instruments & Instrumentation; Materials Science GA AO1MX UT WOS:000341077700051 ER PT J AU Yue, DJ You, FQ Darling, SB AF Yue, Dajun You, Fengqi Darling, Seth B. TI Domestic and overseas manufacturing scenarios of silicon-based photovoltaics: Life cycle energy and environmental comparative analysis (vol 105, pg 669, 2014) SO SOLAR ENERGY LA English DT Correction C1 [Yue, Dajun; You, Fengqi] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. [Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Darling, Seth B.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. RP You, FQ (reprint author), Northwestern Univ, Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM you@northwestern.edu RI You, Fengqi/B-5040-2011 OI You, Fengqi/0000-0001-9609-4299 NR 1 TC 3 Z9 3 U1 1 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-092X J9 SOL ENERGY JI Sol. Energy PD SEP PY 2014 VL 107 BP 380 EP 380 DI 10.1016/j.solener.2014.06.001 PG 1 WC Energy & Fuels SC Energy & Fuels GA AN0WL UT WOS:000340304600038 ER PT J AU Haberkorn, N Kim, J Maiorov, B Usov, I Chen, GF Yu, W Civale, L AF Haberkorn, N. Kim, Jeehoon Maiorov, B. Usov, I. Chen, G. F. Yu, W. Civale, L. TI Increment of the collective pinning energy in Na1-xCaxFe2As2 single crystals with random point defects introduced by proton irradiation SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article DE iron pnictides; vortex dynamics; proton irradiation ID HIGH-TEMPERATURE SUPERCONDUCTORS; CU-O CRYSTALS; FLUX-CREEP; CURRENT-DENSITY; MAGNETIZATION; YBA2CU3O7-X; FILMS AB We study the influence of random point defects introduced by 3 MeV proton irradiation (doses 1 x 10(16) and 2 x 10(16) cm(2)) on the vortex dynamics of NaxCa1 - xFe2As2 (x = 0.5 and x = 0.75) single crystals. Our results indicate that the irradiation produces an enhancement of the critical current density and a reduction of the creep rate in vortex relaxation. The plateau in the temperature dependence of vortex creep rate initially present in as-grown single crystals disappears after irradiation. This fact can be associated with a large increment of the collective pinning energy (from <100 to 350-400 K). On the other hand, Maley analysis indicates that after irradiation both samples present a glassy exponent close to the one expected in the so-called large bundle regime (mu approximate to 7/9) for random point defects. C1 [Haberkorn, N.] Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Kim, Jeehoon] POSTECH, Inst Basic Sci, Ctr Artificial Low Dimens Elect Syst, Pohang 790784, South Korea. [Kim, Jeehoon] POSTECH, Dept Phys, Pohang 790784, South Korea. [Maiorov, B.; Civale, L.] Los Alamos Natl Lab, MPA CMMS, Los Alamos, NM 87545 USA. [Usov, I.] Los Alamos Natl Lab, MST 7, Los Alamos, NM 87545 USA. [Chen, G. F.; Yu, W.] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. RP Haberkorn, N (reprint author), Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. EM nhaberk@cab.cnea.gov.ar RI Yu, Weiqiang/E-9722-2012; OI Maiorov, Boris/0000-0003-1885-0436; Civale, Leonardo/0000-0003-0806-3113 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; NSFC [10974254, 11074304]; National Basic Research Program of China [2010CB923000, 2011CBA00100] FX Research at LANL was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (magnetometry, proton irradiation, data analysis, manuscript preparation). Work by G F C and W Y (fabrication of samples) was supported by the NSFC under Grants No. 10974254 and No. 11074304, and by the National Basic Research Program of China under Grants No. 2010CB923000 and No. 2011CBA00100. N H is member of CONICET (Argentina). NR 40 TC 3 Z9 3 U1 4 U2 26 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD SEP PY 2014 VL 27 IS 9 AR 095004 DI 10.1088/0953-2048/27/9/095004 PG 7 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AO3OY UT WOS:000341243500005 ER PT J AU Ning, SA AF Ning, S. Andrew TI A simple solution method for the blade element momentum equations with guaranteed convergence SO WIND ENERGY LA English DT Article DE blade element momentum equations; robust solution methodology; guaranteed convergence AB The blade element momentum (BEM) equations, though conceptually simple, can be challenging to solve reliably and efficiently with high precision. These requirements are particularly important for efficient rotor blade optimization that utilizes gradient-based algorithms. Many solution approaches exist for numerically converging the axial and tangential induction factors. These methods all generally suffer from a lack of robustness in some regions of the rotor blade design space, or require significantly increased complexity to promote convergence. The approach described here allows for the BEM equations to be parameterized by one variable-the local inflow angle. This reduction is mathematically equivalent, but greatly simplifies the solution approach. Namely, it allows for the use of one-dimensional root-finding algorithms for which very robust and efficient algorithms exist. This paper also discusses an appropriate arrangement of the equation and corresponding bounds for the one-dimensional search-intervals that bracket the solution and over which the function is well behaved. The result is a methodology for solving the BEM equations with guaranteed convergence and at a superlinear rate. Copyright (C) 2013 John Wiley & Sons, Ltd. C1 NREL, Golden, CO 80401 USA. RP Ning, SA (reprint author), NREL, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM andrew.ning@nrel.gov OI Ning, Andrew/0000-0003-2190-823X NR 22 TC 7 Z9 7 U1 0 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD SEP PY 2014 VL 17 IS 9 BP 1327 EP 1345 DI 10.1002/we.1636 PG 19 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA AN4IO UT WOS:000340551300003 ER PT J AU Heo, TW Chen, LQ AF Heo, Tae Wook Chen, Long-Qing TI Phase-field modeling of displacive phase transformations in elastically anisotropic and inhomogeneous polycrystals SO ACTA MATERIALIA LA English DT Article DE Displacive phase transformation; Inhomogeneous elasticity; Elastic anisotropy; Polycrystals; Phase-field model ID TETRAGONAL MARTENSITIC-TRANSFORMATION; MICROSTRUCTURE EVOLUTION; COMPUTER-SIMULATION; GRAIN-BOUNDARY; ORTHORHOMBIC TRANSFORMATION; STAINLESS-STEELS; ALLOYS; NUCLEATION; SYSTEM; GROWTH AB We integrate the inhomogeneous elasticity model and the phase-field equations for displacive phase transformations in polycrystalline materials. The relaxation of the misfit strain between parent and transformed product phases or among different structural variants of transformed product phases near grain boundaries is taken into account. It is applied to the fcc to bcc martensitic transformation described by a Bain strain in a polycrystalline Fe-31 at.%Ni metallic alloy. The focus is on the effect of grain boundaries on the displacive transformation behaviors. We first study nucleation of the bcc product phase at a grain boundary of a bicrystal. The predicted microstructures through nucleation near grain boundaries are compared to existing experimental observations in literature. The effects of grain boundary characteristics such as the degree and range of the misfit strain relaxation at the grain boundary and grain boundary curvature on the phase behaviors near a grain boundary are then examined for both a flat or a curved grain boundary. The model is also applied to polycrystals containing multiple grains. The effects of the misfit strain relaxation at grain boundaries, elastic anisotropy, and applied stress on the kinetics and the microstructures of displacive transformations are discussed. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Heo, Tae Wook] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. [Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Heo, TW (reprint author), Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. EM heo1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [12-ERD-053]; Center for Computational Materials Design (CCMD); National Science Foundation (NSF) Industry/University Cooperative Research Center at Penn State [IIP-1034965]; Georgia Tech [IIP-1034968]; National Science Foundation [DMR-0710483] FX The work of T.W. Heo was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344. This work was funded by the Laboratory Directed Research and Development Program at LLNL under project tracking code 12-ERD-053. The work of L.Q. Chen was supported by the Center for Computational Materials Design (CCMD), a joint National Science Foundation (NSF) Industry/University Cooperative Research Center at Penn State (IIP-1034965) and Georgia Tech (IIP-1034968) and by the National Science Foundation under the grant number DMR-0710483. Helpful discussions with Dr. S. Bhattacharyya (at Indian Institute of Technology Hyderabad), Dr. B.C. Wood (at LLNL), Y.M. Wang (at LLNL), and Mr. Y. An (at LLNL) are acknowledged. NR 80 TC 15 Z9 15 U1 1 U2 46 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD SEP 1 PY 2014 VL 76 BP 68 EP 81 DI 10.1016/j.actamat.2014.05.014 PG 14 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AN1GJ UT WOS:000340330400006 ER PT J AU Lind, J Li, SF Pokharel, R Lienert, U Rollett, AD Suter, RM AF Lind, J. Li, S. F. Pokharel, R. Lienert, U. Rollett, A. D. Suter, R. M. TI Tensile twin nucleation events coupled to neighboring slip observed in three dimensions SO ACTA MATERIALIA LA English DT Article DE Zirconium; Tensile behavior; Deformation twinning; 3-D characterization; nf-HEDM ID ENERGY DIFFRACTION MICROSCOPY; X-RAY-DIFFRACTION; NUMERICAL-METHOD; MAGNESIUM ALLOY; DEFORMATION; STRAIN; MICROSTRUCTURE; GRAIN; ORIENTATION; BEHAVIOR AB Low-symmetry crystals and polycrystals have anisotropic mechanical properties which, given better understanding of their deformation modes, could lead to development of next generation materials. Understanding how grains in a bulk polycrystal interact will guide and improve material modeling. Here, we show that tensile twins, in hexagonal close-packed metals, form where the macroscopic stress does not generate appropriate shear stress and vice versa. We use non-destructive high-energy X-ray diffraction microscopy to map local crystal orientations in three dimensions in a series of tensile strain states in a zirconium polycrystal. Twins and intragranular orientation variations are observed and it is found that deformation-induced rotations in neighboring grains are spatially correlated with many twins. We conclude that deformation twinning involves complex multigrain interactions which must be included in polycrystal plasticity models. Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Lind, J.; Li, S. F.; Suter, R. M.] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [Pokharel, R.; Rollett, A. D.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15232 USA. [Lienert, U.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Lind, J.; Li, S. F.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Pokharel, R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lienert, U.] DESY, Hamburg, Germany. RP Lind, J (reprint author), Carnegie Mellon Univ, Dept Phys, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. EM jlind@andrew.cmu.edu RI Suter, Robert/P-2541-2014; Rollett, Anthony/A-4096-2012 OI Suter, Robert/0000-0002-0651-0437; Rollett, Anthony/0000-0003-4445-2191 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DESC0002001]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Science Foundation [DMR080072]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This research was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under award DESC0002001. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. Research was also supported in part by the National Science Foundation through XSEDE resources provided by Texas Advanced Computing Center under Grant No. DMR080072. This work was partly performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The authors are grateful to Dr. R. Lebensohn of the Los Alamos National Laboratory for the use of the elastic full-field FFT code and the viscoplastic full-field FFT code. NR 38 TC 23 Z9 23 U1 6 U2 46 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD SEP 1 PY 2014 VL 76 BP 213 EP 220 DI 10.1016/j.actamat.2014.04.050 PG 8 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AN1GJ UT WOS:000340330400019 ER PT J AU Fu, B Yang, WY Wang, YD Li, LF Sun, ZQ Ren, Y AF Fu, B. Yang, W. Y. Wang, Y. D. Li, L. F. Sun, Z. Q. Ren, Y. TI Micromechanical behavior of TRIP-assisted multiphase steels studied with in situ high-energy X-ray diffraction SO ACTA MATERIALIA LA English DT Article DE High-energy X-ray diffraction; Micromechanical behavior; Constitutive model; TRIP-assisted multiphase steels ID TRANSFORMATION-INDUCED PLASTICITY; HIGH-STRENGTH STEELS; RETAINED AUSTENITE; NEUTRON-DIFFRACTION; MECHANICAL-PROPERTIES; DUAL-PHASE; STAINLESS-STEEL; MICROSTRUCTURE; STABILITY; STRESS AB The stress partitions among multiple phases for two cold-rolled transformation-induced-plasticity (TRIP)-assisted C-Mn-Al-Si steels, with different carbon content levels of 0.1% and 0.2% (mass fractions), were investigated using in situ high-energy X-ray diffraction at ambient and low temperatures (-40 degrees C) under uniaxial tensile loading. Based on the evolution of stresses for various phases during plastic deformation, a modified constitutive model was established for describing the micromechanical behavior of TRIP-assisted multiphase steels, based on a Gladman-type mixture law (GTML) embedded with the Mecking-Kocks work-hardening formula. The index n, an important parameter in the GTML for characterizing the accommodation of loading stresses among different phases, was determined to be severely affected by the transformation kinetics of retained austenite. The quantitative relationship between n and the transformation rate of retained austenite was also clearly revealed in the investigated alloys. The modified model thus correlates the mismatch of stresses for multiple phases with the transformation kinetics of metastable phases during plastic deformation and is suitable for all advanced steels with multi-scale microstructures. This model forms the basis for microstructure-based numerical simulations of micromechanical behavior and greatly benefits the design of a new type of high-strength and high-plasticity steel. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Fu, B.; Yang, W. Y.] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. [Wang, Y. D.; Li, L. F.; Sun, Z. Q.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Wang, Y. D.; Li, L. F.] Univ Sci & Technol Beijing, Innovat Ctr Adv Steel Technol, Beijing 100083, Peoples R China. [Ren, Y.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Yang, WY (reprint author), Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. EM wyyang@ustb.edu.cn RI wang, yandong/G-9404-2013 FU National Science Foundation of China (NSFC) [51231002]; Fundamental Research Funds for the Central Universities [06111020]; NPL [2012BA02]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors would like to acknowledge financial support by the State Key Laboratory for Advanced Metals and Materials, affiliated with University of Science and Technology Beijing, China. This work is also supported by the National Science Foundation of China (NSFC) under contract No. 51231002 and the Fundamental Research Funds for the Central Universities (Grant No. 06111020). In addition, the support from NPL under contract No. 2012BA02 is acknowledged. The use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 42 TC 6 Z9 6 U1 7 U2 42 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD SEP 1 PY 2014 VL 76 BP 342 EP 354 DI 10.1016/j.actamat.2014.05.029 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AN1GJ UT WOS:000340330400030 ER PT J AU Li, MM Wang, LY Almer, JD AF Li, Meimei Wang, Leyun Almer, Jonathan D. TI Dislocation evolution during tensile deformation in ferritic-martensitic steels revealed by high-energy X-rays SO ACTA MATERIALIA LA English DT Article DE Ferritic steels; Dislocation density; Deformation; In situ tension test; High-energy X-ray diffraction ID PCT CR STEELS; POLYCRYSTALLINE ALPHA-FE; STRESS-STRAIN BEHAVIOR; DYNAMIC RECOVERY; CUBIC-CRYSTALS; CREEP STRENGTH; LINE-PROFILES; THIN FILMS; DENSITIES; MODEL AB Deformation processes in Grade 91 (Fe-9%Cr-1%Mo-V,Nb) and Grade 92 (Fe-9%Cr-0.5%Mo-2%W-V,Nb) ferritic-martensitic steels were investigated at temperatures between 20 and 650 C using high-energy synchrotron X-ray diffraction with in situ thermal-mechanical loading. The change of the dislocation density with strain was quantified by X-ray diffraction line profile analysis complemented by transmission electron microscopy measurements. The relationship between dislocation density and strain during uniform deformation was described by a dislocation model, and two critical materials parameters, namely dislocation mean free path and dynamic recovery coefficient, were determined as a function of temperature. Effects of alloy chemistry, thermal mechanical treatment and temperature on the tensile deformation process in Grade 91 and Grade 92 steels can be well understood by the dislocation evolution behavior. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Li, Meimei; Wang, Leyun] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Almer, Jonathan D.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Li, MM (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mli@anl.gov FU US Department of Energy (DOE), Office of Nuclear Energy [DE-AC02-06CH11357]; US DOE, Office of Science, Office of Basic Energy Sciences [W-31-109-ENG-38]; UChicago Argonne, LLC [DE-AC02-06CH11357] FX Materials were provided by Oak Ridge National Laboratory. Work was supported by the US Department of Energy (DOE), Office of Nuclear Energy under Contract DE-AC02-06CH11357. Use of the APS was supported by the US DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. W-31-109-ENG-38. The electron microscopy was accomplished at the Electron Microscopy Center at Argonne National Laboratory, a USDOE Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 51 TC 18 Z9 18 U1 6 U2 53 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD SEP 1 PY 2014 VL 76 BP 381 EP 393 DI 10.1016/j.actamat.2014.05.026 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AN1GJ UT WOS:000340330400033 ER PT J AU Spear, AD Li, SF Lind, JF Suter, RM Ingraffea, AR AF Spear, Ashley D. Li, Shiu Fai Lind, Jonathan F. Suter, Robert M. Ingraffea, Anthony R. TI Three-dimensional characterization of microstructurally small fatigue-crack evolution using quantitative fractography combined with post-mortem X-ray tomography and high-energy X-ray diffraction microscopy SO ACTA MATERIALIA LA English DT Article DE Three-dimensional imaging; Synchrotron radiation; Fatigue crack initiation; Fracture surface; Al 6061-T6 ID ZN-MG-CU; MONTE-CARLO SIMULATIONS; FACET CRYSTALLOGRAPHY; ENVIRONMENTAL FATIGUE; GRAIN-BOUNDARIES; ALUMINUM-ALLOYS; GROWTH; INITIATION; PROPAGATION; POLYCRYSTAL AB An experimental methodology based on post-mortem measurements is proposed to quantify rates of propagation and crack-surface crystallography of a 3-D, naturally nucleated, microstructurally small fatigue crack (MSFC) in a polycrystalline aluminum alloy (Al-Mg-Si). The post-mortem characterization involves: scanning electron microscopy-based fractography to measure crack-front projections (marker bands) at known cycle counts during the load history, X-ray computed tomography to provide high-resolution reconstructions of the 3-D crack-surface morphology, and near-field high-energy X-ray diffraction microscopy to provide 3-D grain geometries and orientations adjacent to fatigue-crack surfaces. Local MSFC-propagation rates are measured by accounting for the 3-D crack-surface morphology and varied by two orders of magnitude in the Al-Mg-Si specimen. Both intergranular and transgranular MSFC evolution were observed, with the latter occurring along a wide range of crystallographic planes. The findings demonstrate: (i) the complexity and variability of 3-D MSFC evolution in the Al-Mg-Si alloy; and (ii) the viability of the post-mortem characterization approach for quantifying 3-D MSFC evolution in polycrystalline alloys. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Spear, Ashley D.; Ingraffea, Anthony R.] Cornell Univ, Sch Civil & Environm Engn, Ithaca, NY 14853 USA. [Li, Shiu Fai] Lawrence Livermore Natl Lab, Livermore, CA USA. [Lind, Jonathan F.; Suter, Robert M.] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. RP Spear, AD (reprint author), Cornell Univ, 640 Rhodes Hall, Ithaca, NY 14853 USA. EM ads259@comell.edu RI Suter, Robert/P-2541-2014 OI Suter, Robert/0000-0002-0651-0437 FU National Science Foundation Graduate Research Fellowship Program [DGE-0707428]; US Department of Energy (DOE); Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Carnegie Mellon University [DESC0002001]; US DOE [DE-AC02-06CH11357]; National Science Foundation [OCI-1053575] FX Gratitude is expressed to Drs. Robert Piascik, Stephen Smith, and Edward Glaessgen of NASA Langley Research Center for providing valuable discussions and support for specimen machining, mechanical testing and SEM-based imaging. The authors also wish to thank Dr. Peter Kenesei of Argonne National Laboratory for assisting with X-ray tomography reconstructions. This work is supported by the National Science Foundation Graduate Research Fellowship Program under Grant No. DGE-0707428; under the auspices of the US Department of Energy (DOE) by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344; and by grant DESC0002001 at Carnegie Mellon University. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US DOE Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. HEDM reconstruction was performed using allocation TG-MSS110031 through the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by the National Science Foundation Grant No. OCI-1053575. NR 58 TC 9 Z9 10 U1 5 U2 52 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD SEP 1 PY 2014 VL 76 BP 413 EP 424 DI 10.1016/j.actamat.2014.05.021 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AN1GJ UT WOS:000340330400036 ER PT J AU Zhou, SH Wang, Y Chen, LQ Liu, ZK Napolitano, RE AF Zhou, S. H. Wang, Y. Chen, L. -Q. Liu, Z. -K. Napolitano, R. E. TI Solution-based thermodynamic modeling of the Ni-Al-Mo system using first-principles calculations SO CALPHAD-COMPUTER COUPLING OF PHASE DIAGRAMS AND THERMOCHEMISTRY LA English DT Article DE CALPHAD; First-principles calculation; Ni-Al-Mo phase diagram; ATAT ID ELEVATED-TEMPERATURE STABILITY; PHASE-EQUILIBRIA; ALUMINUM-MOLYBDENUM; RICH ALLOYS; TA SYSTEM; DIAGRAM; CONSTITUTION; SUPERALLOYS; EUTECTICS; ELEMENTS AB A solution-based thermodynamic description of the ternary Ni-Al-Mo system is developed here, incorporating first-principles calculations and reported modeling of the binary Ni-Al, Ni-Mo and Al-Mo systems. To search for the configurations with the lowest energies of the N phase, the Alloy Theoretic Automated Toolkit (ATAT) was employed and combined with VASP. The liquid, bcc and gamma-fcc phases are modeled as random atomic solutions, and the gamma'-Ni3Al phase is modeled by describing the ordering within the fcc structure using two sublattices, summarized as (ALMo,Ni)(0.75)(Al,Mo,Ni)(0.25). Thus, gamma-fcc and gamma'-Ni3Al are modeled with a single Gibbs free energy function with appropriate treatment of the chemical ordering contribution. In addition, notable improvements are the following: first, the ternary effects of Mo and Al in the B2-NiAl and D0(a)-Ni3Mo phases, respectively, are considered; second, the N-NiAl8Mo3 phase is described as a solid solution using a three-sublattice model; third, the X-Ni14Al75Mo11 phase is treated as a stoichiometric compound. Model parameters are evaluated using first-principles calculations of zero-Kelvin formation enthalpies and reported experimental data. In comparison with the enthalpies of formation for the compounds psi-AlMo, theta-Al8Mo3 and B-2-NiAl, the first-principles results indicate that the N-NiAl8Mo3 phase, which is stable at high temperatures, decomposes into other phases at low temperature. Resulting phase equilibria are summarized in the form of isothermal sections and liquidus projections. To clearly identify the relationship between the gamma-fcc and gamma'-Ni3Al phases in the ternary Ni-Al-Mo system, the specific gamma-fcc and gamma'-Ni3Al phase fields are plotted in x(Al)-x(Mo)-T space for a temperature range 1200-1800 K. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Zhou, S. H.; Wang, Y.; Chen, L. -Q.; Liu, Z. -K.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Zhou, S. H.; Napolitano, R. E.] US DOE, Ames Lab, Mat & Engn Phys Program, Washington, DC 20585 USA. [Napolitano, R. E.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Zhou, SH (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RI Wang, Yi/D-1032-2013; Liu, Zi-Kui/A-8196-2009 OI Liu, Zi-Kui/0000-0003-3346-3696 FU NSF [DMR-9983532, DMR-0122638, DMR-0205232]; Pennsylvania State University FX This work was supported by the Pennsylvania State University by the NSF Grants (DMR-9983532, DMR-0122638, and DMR-0205232). First-principles calculations were carried out on the LION clusters at the Pennsylvania State University supported in part by the NSF Grants (DMR-9983532, DMR-0122638, and DMR-0205232). NR 48 TC 3 Z9 3 U1 6 U2 76 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0364-5916 EI 1873-2984 J9 CALPHAD JI Calphad-Comput. Coupling Ph. Diagrams Thermochem. PD SEP PY 2014 VL 46 BP 124 EP 133 DI 10.1016/j.calphad.2014.03.002 PG 10 WC Thermodynamics; Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Thermodynamics; Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AN1EO UT WOS:000340325700014 ER PT J AU Sun, WC Mota, A AF Sun, WaiChing Mota, Alejandro TI A multiscale overlapped coupling formulation for large-deformation strain localization SO COMPUTATIONAL MECHANICS LA English DT Article DE Domain coupling; Variational principle; Energy based coupling method; Multiscale modeling ID FINITE-ELEMENT-METHOD; ARLEQUIN METHOD; CONTINUUM MODELS; MULTIPLIERS; PARTICLE AB We generalize the multiscale overlapped domain framework to couple multiple rate-independent standard dissipative material models in the finite deformation regime across different length scales. We show that a fully coupled multiscale incremental boundary-value problem can be recast as the stationary point that optimizes the partitioned incremental work of a three-field energy functional. We also establish inf-sup tests to examine the numerical stability issues that arise from enforcing weak compatibility in the three-field formulation. We also devise a new block solver for the domain coupling problem and demonstrate the performance of the formulation with one-dimensional numerical examples. These simulations indicate that it is sufficient to introduce a localization limiter in a confined region of interest to regularize the partial differential equation if loss of ellipticity occurs. C1 [Sun, WaiChing] Columbia Univ City New York, Dept Civil Engn & Engn Mech, New York, NY 10027 USA. [Mota, Alejandro] Sandia Natl Labs, Mech Mat Dept, Livermore, CA 94550 USA. RP Sun, WC (reprint author), Columbia Univ City New York, Dept Civil Engn & Engn Mech, New York, NY 10027 USA. EM wsun@columbia.edu RI Sun, WaiChing/A-2638-2009 OI Sun, WaiChing/0000-0002-3078-5086 FU U.S. Department of Energy's Advanced Simulation and Computing (ASC) Program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We thank James W. Foulk III for providing us with the analytical solution of the singular bar problem. Thanks are also due to Micheal L. Parks for suggesting the one-dimensional patch test. Support for this work was received through the U.S. Department of Energy's Advanced Simulation and Computing (ASC) Program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 38 TC 4 Z9 4 U1 1 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0178-7675 EI 1432-0924 J9 COMPUT MECH JI Comput. Mech. PD SEP PY 2014 VL 54 IS 3 BP 803 EP 820 DI 10.1007/s00466-014-1034-0 PG 18 WC Mathematics, Interdisciplinary Applications; Mechanics SC Mathematics; Mechanics GA AN4CO UT WOS:000340535400014 ER PT J AU Rabeling, C Love, CN Lance, SL Jones, KL Pierce, NE Bacci, M AF Rabeling, Christian Love, Cara N. Lance, Stacey L. Jones, Kenneth L. Pierce, Naomi E. Bacci, Mauricio, Jr. TI Development of twenty-one polymorphic microsatellite markers for the fungus-growing ant, Mycocepurus goeldii (Formicidae: Attini), using Illumina paired-end genomic sequencing SO CONSERVATION GENETICS RESOURCES LA English DT Article DE Polygyny; Polyandry; Social parasitism; Inquilinism; PAL_FINDER; SSR ID HYMENOPTERA-FORMICIDAE; SOCIAL PARASITISM AB Obligate social parasites, or inquilines, exploit the colonies of free-living social species and evolved at least 80 times in ants alone. Most species of the highly specialized inquiline social parasites are rare, only known from one or very few, geographically isolated populations, and the sexual offspring of most inquiline species mates inside the maternal colony. Therefore, inquiline populations are believed to be small and genetically homogeneous due to inbreeding. To comparatively study the genetic diversity of the socially parasitic fungus-growing ant, Mycocepurus castrator, and its only known host species, Mycocepurus goeldii, and to infer the parasite's conservation status, we developed 21 microsatellite markers for the host species, M. goeldii, and evaluated whether these markers cross-amplify in the social parasite, M. castrator. We isolated and characterized a total of 21 microsatellite loci for M. goeldii. The loci were screened for 24 individuals from geographically distant and genetically divergent populations in Brazil. The number of alleles per locus ranged from 18 to 4, the observed heterozygosity ranged from 0.25 to 0.636, and the probability of identity values ranged from 0.011 to 0.146. Preliminary analyses show that these markers cross amplify in the closely related social parasite species M. castrator. These newly developed loci provide tools for studying the genetic diversity and the evolution of social parasitism in the Mycocepurus host-parasite system. C1 [Rabeling, Christian; Pierce, Naomi E.] Harvard Univ, Museum Comparat Zool, Cambridge, MA 02138 USA. [Love, Cara N.; Lance, Stacey L.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Jones, Kenneth L.] Univ Colorado, Dept Biochem & Mol Genet, Sch Med, Aurora, CO 80045 USA. [Bacci, Mauricio, Jr.] UNESP Univ Estadual Paulista, Inst Biociencias, Ctr Estudos Insetos Sociais, BR-13506900 Rio Claro, SP, Brazil. RP Rabeling, C (reprint author), Univ Rochester, Dept Biol, Rochester, NY 14627 USA. EM crabeling@gmail.com RI Lance, Stacey/K-9203-2013 OI Lance, Stacey/0000-0003-2686-1733 FU Harvard Society; William F. Milton Fund; FAPESP [2011/50226-0]; PROPE-UNESP fund; NSF [SES-0750480]; DOE [DE-FC09-07SR22506] FX We thank the Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq) and the Instituto Brasileiro do Meio Ambiente e dos Recursos Naturais Renovaveis (IBAMA) for permission to conduct fieldwork in Brazil. A Junior Fellowship from the Harvard Society of Fellows and the William F. Milton Fund financially supported CR's research. MB's and CR's field research was support by FAPESP Grant 2011/50226-0 and by the PROPE-UNESP fund. NEP was supported by NSF SES-0750480. Manuscript preparation was partially supported by the DOE under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation. NR 5 TC 0 Z9 0 U1 0 U2 8 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1877-7252 EI 1877-7260 J9 CONSERV GENET RESOUR JI Conserv. Genet. Resour. PD SEP PY 2014 VL 6 IS 3 BP 739 EP 741 DI 10.1007/s12686-014-0204-x PG 3 WC Biodiversity Conservation; Genetics & Heredity SC Biodiversity & Conservation; Genetics & Heredity GA AN2HJ UT WOS:000340404900066 ER PT J AU Beasley, RR Lance, SL Jones, KL Berry, RB Johnson, JA AF Beasley, Rochelle R. Lance, Stacey L. Jones, Kenneth L. Berry, Robert B. Johnson, Jeff A. TI Development of polymorphic microsatellite markers for the orange-breasted falcon (Falco deiroleucus) SO CONSERVATION GENETICS RESOURCES LA English DT Article DE Falco deiroleucus; Orange-breasted falcon; Microsatellite; SSR ID POPULATION AB We isolated and characterized a total of 24 microsatellite loci from the orange-breasted falcon (Falco deiroleucus). Loci were screened in 32 individuals currently maintained as a captive population: 13 wild-caught individuals from Panama and four from Belize, and the remaining 15 were first generation F1 offspring. The number of alleles per locus ranged from 2 to 9, observed heterozygosity ranged from 0.000 to 0.938, and the probability of identity values ranged from 0.075 to 0.604. These new loci will provide tools for identifying relatedness values among sampled individuals currently in captivity and for exploring genetic diversity levels and connectivity between populations in Central America. C1 [Beasley, Rochelle R.; Lance, Stacey L.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Jones, Kenneth L.] Univ Colorado, Dept Biochem & Mol Genet, Sch Med, Aurora, CO 80045 USA. [Berry, Robert B.] Peregrine Fund, Boise, ID 83709 USA. [Johnson, Jeff A.] Univ N Texas, Inst Appl Sci, Dept Biol Sci, Denton, TX 76203 USA. RP Johnson, JA (reprint author), Univ N Texas, Inst Appl Sci, Dept Biol Sci, Denton, TX 76203 USA. EM jajohnson@unt.edu RI Lance, Stacey/K-9203-2013; Beasley, Rochelle/M-1396-2015 OI Lance, Stacey/0000-0003-2686-1733; Beasley, Rochelle/0000-0001-7325-4085 FU Wolf Creek Charitable Foundation; DOE [DE-FC09-07SR22506] FX The authors acknowledge the financial support of Wolf Creek Charitable Foundation and the DOE under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation. Biostatistics/Bioinformatics Shared Resource of the University of Colorado Cancer Center (5P30CA046934) provided bioinformatics support. Samples were collected under permits issued by the Belize Agricultural Health Authority and the Forest Department, and Ministry of Forestry, Fisheries and Sustainable Development. NR 5 TC 0 Z9 0 U1 1 U2 8 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1877-7252 EI 1877-7260 J9 CONSERV GENET RESOUR JI Conserv. Genet. Resour. PD SEP PY 2014 VL 6 IS 3 BP 743 EP 745 DI 10.1007/s12686-014-0205-9 PG 3 WC Biodiversity Conservation; Genetics & Heredity SC Biodiversity & Conservation; Genetics & Heredity GA AN2HJ UT WOS:000340404900067 ER PT J AU D'Elia, G Beasley, RR Lance, SL Jones, KL Bacigalupe, LD AF D'Elia, Guillermo Beasley, Rochelle R. Lance, Stacey L. Jones, Kenneth L. Bacigalupe, Leonardo D. TI Development of polymorphic microsatellite markers for the Pleuroderma thaul SO CONSERVATION GENETICS RESOURCES LA English DT Article DE Leptodactylidae; Pleuroderma thaul; Illumina; Microsatellite; PAL_FINDER; PCR primers; SSR AB Pleurodema thaul (Leptodactylidae) is a small frog from Chile and Argentina with a distributional range that spans more than 2,500 km. We isolated and characterized a total of 23 microsatellite loci from 24 individuals. The number of alleles per locus ranged from 7 to 22, observed heterozygosity ranged from 0.417 to 0.958, and the probability of identity values ranged from 0.0064 to 0.21. C1 [D'Elia, Guillermo; Bacigalupe, Leonardo D.] Univ Austral Chile, Inst Ciencias Ambientales & Evolut, Fac Ciencias, Valdivia, Chile. [Beasley, Rochelle R.; Lance, Stacey L.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Jones, Kenneth L.] Univ Colorado, Dept Biochem & Mol Genet, Sch Med, Aurora, CO 80045 USA. RP Bacigalupe, LD (reprint author), Univ Austral Chile, Inst Ciencias Ambientales & Evolut, Fac Ciencias, Casilla 567, Valdivia, Chile. EM lbacigal@gmail.com RI Lance, Stacey/K-9203-2013; Beasley, Rochelle/M-1396-2015; D'Elia, Guillermo/G-2253-2011 OI Lance, Stacey/0000-0003-2686-1733; Beasley, Rochelle/0000-0001-7325-4085; D'Elia, Guillermo/0000-0001-7173-2709 FU FONDECYT [1120461]; DOE [DE-FC09-07SR22506] FX Financial support was granted by FONDECYT 1120461. Manuscript preparation was partially supported by the DOE under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation. NR 6 TC 1 Z9 1 U1 1 U2 8 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1877-7252 EI 1877-7260 J9 CONSERV GENET RESOUR JI Conserv. Genet. Resour. PD SEP PY 2014 VL 6 IS 3 BP 747 EP 749 DI 10.1007/s12686-014-0206-8 PG 3 WC Biodiversity Conservation; Genetics & Heredity SC Biodiversity & Conservation; Genetics & Heredity GA AN2HJ UT WOS:000340404900068 ER PT J AU Ahmed, M Sultan, M Wahr, J Yan, E AF Ahmed, Mohamed Sultan, Mohamed Wahr, John Yan, Eugene TI The use of GRACE data to monitor natural and anthropogenic induced variations in water availability across Africa SO EARTH-SCIENCE REVIEWS LA English DT Article DE GRACE; TWS; Africa; Water availability; Climate change; Anthropogenic effects ID NORTH-ATLANTIC OSCILLATION; CLIMATE EXPERIMENT GRACE; SATELLITE GRAVITY MEASUREMENTS; DROUGHT SEVERITY INDEX; GROUNDWATER DEPLETION; RIVER-BASIN; GLOBAL PRECIPITATION; CANADIAN PRAIRIE; UNITED-STATES; INDIAN-OCEAN AB Inter-annual trends in terrestrial water storage (TWS) were extracted from monthly (01/2003-09/2012) Gravity Recovery and Climate Experiment (GRACE) data acquired over Africa and correlated (in a geographic information system [GIS] environment) with relevant temporal remote sensing, geologic, and hydrologic datasets. Findings include the following: (1) large sectors of Africa are undergoing statistically significant TWS variations (+44 mm/yr to -15 mm/yr) due to natural and anthropogenic causes; (2) warming of the tropical Atlantic Ocean apparently intensified Atlantic monsoons and increased precipitation and TWS over western and central Africa; (3) warming in the central Indian Ocean decreased precipitation and TWS over eastern Africa; (4) the high frequency of flooding events increased TWS over the Zambezi and Okavango basins; (5) extraction of fossil groundwater decreased TWS over the Saharan aquifers; (6) deforestation decreased TWS in three subbasins (Ubangi, Congo, and Sangha) of the Congo River Basin; and (7) the construction of dams increased TWS in the Blue Nile and Atbara subbasins. Given the 10 years of monthly GRACE data acquired on the subbasin scale across the globe, as well as the plans underway for deployment of a GRACE-FO and GRACE-II, using GRACE-derived TWS data should be considered an alternative, viable index for measuring temporal and spatial variations in water availability. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ahmed, Mohamed; Sultan, Mohamed] Western Michigan Univ, Dept Geosci, Kalamazoo, MI 49008 USA. [Ahmed, Mohamed] Suez Canal Univ, Fac Sci, Dept Geol, Ismailia 41522, Egypt. [Wahr, John] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Yan, Eugene] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. RP Sultan, M (reprint author), Western Michigan Univ, Dept Geosci, 1903 West Michigan Ave, Kalamazoo, MI 49008 USA. EM mohamed.sultan@wmich.edu FU National Aeronautics and Space Administration [NNX08AJ85G, NNX12AJ94G] FX Funding was provided by the National Aeronautics and Space Administration grants NNX08AJ85G and NNX12AJ94G to Western Michigan University. We thank the Editor and the anonymous Reviewers of the Earth-Sciences Reviews for their instructive comments and suggestions. NR 112 TC 16 Z9 16 U1 5 U2 58 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0012-8252 EI 1872-6828 J9 EARTH-SCI REV JI Earth-Sci. Rev. PD SEP PY 2014 VL 136 BP 289 EP 300 DI 10.1016/j.earscirev.2014.05.009 PG 12 WC Geosciences, Multidisciplinary SC Geology GA AN0WD UT WOS:000340303800012 ER PT J AU Doscher, H Geisz, JF Deutsch, TG Turner, JA AF Doescher, H. Geisz, J. F. Deutsch, T. G. Turner, J. A. TI Sunlight absorption in water - efficiency and design implications for photoelectrochemical devices SO ENERGY & ENVIRONMENTAL SCIENCE LA English DT Article ID HYDROGEN-PRODUCTION; SOLAR-CELLS; PHOTOLYSIS AB Sunlight absorption in water has a critical impact on solar fuel generation by direct photoelectrolysis because devices are commonly illuminated through the aqueous electrolyte. We show the relevant reference spectra, calculate fundamental solar-to-hydrogen efficiency prospects, and discuss the design implications for unassisted solar water-splitting devices. C1 [Doescher, H.; Geisz, J. F.; Deutsch, T. G.; Turner, J. A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Doescher, H.] Tech Univ Ilmenau, D-98693 Ilmenau, Germany. RP Doscher, H (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM doscher@nrel.gov OI Deutsch, Todd/0000-0001-6577-1226 FU EU Marie Curie fellowship (IOF) [300971]; U. S. Department of Energy (DOE) [DEAC36-08-GO28308]; National Renewable Energy Laboratory FX H. D. appreciates financial support by a EU Marie Curie fellowship (IOF no. 300971). This work was supported by the U. S. Department of Energy (DOE) under contract no. DEAC36-08-GO28308 with the National Renewable Energy Laboratory. NR 19 TC 49 Z9 49 U1 7 U2 70 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1754-5692 EI 1754-5706 J9 ENERG ENVIRON SCI JI Energy Environ. Sci. PD SEP PY 2014 VL 7 IS 9 BP 2951 EP 2956 DI 10.1039/c4ee01753f PG 6 WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical; Environmental Sciences SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology GA AN2XU UT WOS:000340450100010 ER PT J AU Lin, F Nordlund, D Markus, IM Weng, TC Xin, HL Doeff, MM AF Lin, Feng Nordlund, Dennis Markus, Isaac M. Weng, Tsu-Chien Xin, Huolin L. Doeff, Marca M. TI Profiling the nanoscale gradient in stoichiometric layered cathode particles for lithium-ion batteries SO ENERGY & ENVIRONMENTAL SCIENCE LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; CHARGE COMPENSATION; ELECTRONIC-STRUCTURE; COMPOSITE CATHODE; STORAGE MECHANISM; NICKEL-OXIDE; IN-SITU; SURFACE; SOFT; PHASE AB Chemical and structural evolution in battery materials influences properties relevant to ionic and electronic transport and ultimately impacts the battery performance. Although chemical and structural gradients have been observed in several cathode materials, the origin(s) of these phenomena are poorly understood. Via high-throughput core-level spectroscopies {i.e., X-ray absorption spectroscopy (XAS), depth-profiled X-ray photoelectron spectroscopy (XPS) and electron energy loss spectroscopy (EELS)}, as well as scanning transmission electron microscopy (STEM), the present study seeks to achieve mechanistic understanding for these phenomena in a stoichiometric R (3) over barm layered cathode material (e.g., LiNixMnxCo1-2xO2, NMC). We observed that the surfaces of particles in the composite electrode are complicated by the presence of a surface reaction layer resulting from electrolyte decomposition. In large particle ensembles, the global nickel oxidation state switches between Ni2+ and Ni2+x (x = 1-2) during charging/discharging processes, and hole states are also created at the O2p level due to the TM3d-O2p hybridization states. In primary particles, the surface is less oxidized than the bulk counterpart of the same particle whenever the particle has been cycled. This is partially attributed to the reconstruction from an R (3) over barm structure to an Fm (3) over barm structure at the surfaces of NMC particles. This work provides a unique insight into correlating crystal structures with charge compensation mechanisms and performance fading in stoichiometric layered cathode materials. C1 [Lin, Feng; Markus, Isaac M.; Doeff, Marca M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Nordlund, Dennis; Weng, Tsu-Chien] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Markus, Isaac M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Xin, Huolin L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Lin, F (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM flin@lbl.gov; hxin@bnl.gov; mmdoeff@lbl.gov RI Nordlund, Dennis/A-8902-2008; Foundry, Molecular/G-9968-2014; Xin, Huolin/E-2747-2010; OI Nordlund, Dennis/0000-0001-9524-6908; Xin, Huolin/0000-0002-6521-868X; Doeff, Marca/0000-0002-2148-8047 FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02- 05CH11231]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; National Center for Electron Microscopy (NCEM) of the Lawrence Berkeley National Laboratory (LBNL); U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract no. DE-AC02- 05CH11231 under the Batteries for Advanced Transportation Technologies (BATT) Program. The synchrotron X-ray portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. STEM-EELS experiments were performed at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract no. DE-AC02-98CH10886, and at National Center for Electron Microscopy (NCEM) of the Lawrence Berkeley National Laboratory (LBNL), which is supported by the U.S. Department of Energy (DOE) under Contract no. DE-AC02-05CH11231. F.L., I. M. M. and M.M.D. would like to acknowledge the discussions with Prof. Mark Asta, Dr Tanghong Yi, Lei Cheng, Dr Guoying Chen and Dr Thomas Richardson. F.L., D.N. and T.-C.W. thank Dr Jun-Sik Lee and Glen Kerr for the help at SSRL Beam Line 8-2. H.L.X. would like to acknowledge Dr Haimei Zheng for her advice on the project. NR 35 TC 23 Z9 23 U1 7 U2 78 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1754-5692 EI 1754-5706 J9 ENERG ENVIRON SCI JI Energy Environ. Sci. PD SEP PY 2014 VL 7 IS 9 BP 3077 EP 3085 DI 10.1039/c4ee01400f PG 9 WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical; Environmental Sciences SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology GA AN2XU UT WOS:000340450100026 ER PT J AU Kosnicki, E Sefick, SA Paller, MH Jarrell, MS Prusha, BA Sterrett, SC Tuberville, TD Feminella, JW AF Kosnicki, Ely Sefick, Stephen A. Paller, Michael H. Jarrell, Miller S. Prusha, Blair A. Sterrett, Sean C. Tuberville, Tracey D. Feminella, Jack W. TI Defining the Reference Condition for Wadeable Streams in the Sand Hills Subdivision of the Southeastern Plains Ecoregion, USA SO ENVIRONMENTAL MANAGEMENT LA English DT Article DE Reference condition; Sand Hills ecoregion; Stream management; Historical land use; Macroinvertebrates; Stressors ID WATER-QUALITY; BENTHIC MACROINVERTEBRATES; LAND-USE; ASSEMBLAGES; ASSESSMENTS; RICHNESS; GRADIENT; ROADS; SCALE AB The Sand Hills subdivision of the Southeastern Plains ecoregion has been impacted by historical land uses over the past two centuries and, with the additive effects of contemporary land use, determining reference condition for streams in this region is a challenge. We identified reference condition based on the combined use of 3 independent selection methods. Method 1 involved use of a multivariate disturbance gradient derived from several stressors, method 2 was based on variation in channel morphology, and method 3 was based on passing 6 of 7 environmental criteria. Sites selected as reference from all 3 methods were considered primary reference, whereas those selected by 2 or 1 methods were considered secondary or tertiary reference, respectively. Sites not selected by any of the methods were considered non-reference. In addition, best professional judgment (BPJ) was used to exclude some sites from any reference class, and comparisons were made to examine the utility of BPJ. Non-metric multidimensional scaling indicated that use of BPJ may help designate non-reference sites when unidentified stressors are present. The macroinvertebrate community measures Ephemeroptera, Plecoptera, Trichoptera richness and North Carolina Biotic Index showed no differences between primary and secondary reference sites when BPJ was ignored. However, there was no significant difference among primary, secondary, and tertiary reference sites when BPJ was used. We underscore the importance of classifying reference conditions, especially in regions that have endured significant anthropogenic activity. We suggest that the use of secondary reference sites may enable construction of models that target a broader set of management interests. C1 [Kosnicki, Ely; Sefick, Stephen A.; Jarrell, Miller S.; Feminella, Jack W.] Auburn Univ, Dept Biol Sci, Auburn, AL 36849 USA. [Paller, Michael H.; Tuberville, Tracey D.] Savannah River Natl Lab, Aiken, SC 29802 USA. [Prusha, Blair A.] Midwest Biodivers Inst, Hilliard, OH 43235 USA. [Sterrett, Sean C.] Univ Georgia, Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. RP Kosnicki, E (reprint author), Auburn Univ, Dept Biol Sci, 331 Funchess Hall, Auburn, AL 36849 USA. EM ekosnick@brockport.edu FU Strategic Research and Development Program Project [RC-1694]; Department of Energy [DE-FC09-07SR22506] FX We thank Hugh Westbury (Fort Benning, Natural Resources Branch), Chuck Bryan (Fort Bragg, Endangered Species Branch), Michael Juhan (Fort Gordon, Natural Resources Branch), Harvey Belser (Manchester State Forest), Michele Brossett (Georgia Department of Natural Resources), Michael Walters (North Carolina Biological Assessment Unit), George Williams (Osage of Virginia, Inc.), Nancy Jordan (Sandhills National Wildlife Refuge), Brian Davis (Sand Hills State Forest), Michele Elmore and Geoff Sorrell (The Nature Conservancy), and special thanks to Brady Beck (Sandhills Gamelands). We also thank Brian Helms at the Auburn Museum of Natural History for field assistance and Andrew Grosse and Bess Harris at Savannah River Ecology Lab for help with GIS analysis. This project was funded by the Strategic Research and Development Program Project RC-1694. Support was provided in part by Award Number DE-FC09-07SR22506 from Department of Energy to the University of Georgia Research Foundation. NR 60 TC 3 Z9 3 U1 1 U2 10 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0364-152X EI 1432-1009 J9 ENVIRON MANAGE JI Environ. Manage. PD SEP PY 2014 VL 54 IS 3 BP 494 EP 504 DI 10.1007/s00267-014-0320-0 PG 11 WC Environmental Sciences SC Environmental Sciences & Ecology GA AN4DP UT WOS:000340538100009 PM 25011531 ER PT J AU Guo, Y Keller, J Parker, RG AF Guo, Yi Keller, Jonathan Parker, Robert G. TI Nonlinear dynamics and stability of wind turbine planetary gear sets under gravity effects SO EUROPEAN JOURNAL OF MECHANICS A-SOLIDS LA English DT Article DE Dynamics; Wind turbine; Planetary gear ID HARMONIC-BALANCE METHOD; ELEMENT/CONTACT MECHANICS MODEL; SYSTEM; STIFFNESS; MOTIONS AB This paper investigates the dynamics of wind turbine planetary gear sets under the effect of gravity using a modified harmonic balance method that includes simultaneous excitations. This modified method along with arc-length continuation and Floquet theory is applied to a lumped-parameter planetary gear model including gravity, fluctuating mesh stiffness, bearing clearance, and nonlinear tooth contact to obtain the dynamic response of the system. The calculated dynamic responses compare well with time domain-integrated mathematical models and experimental results. Gravity is a fundamental vibration source in wind turbine planetary gear sets and plays an important role in the system dynamic response compared to excitations from tooth meshing alone. Gravity causes nonlinear effects induced by tooth wedging and bearing-raceway contacts. Tooth wedging, also known as a tight mesh, occurs when a gear tooth comes into contact on the drive-side and back-side simultaneously and it is a source of planet-bearing failures. Clearance in carrier bearings decreases bearing stiffness and significantly reduces the lowest resonant frequencies of the translational modes. Gear tooth wedging can be prevented if the carrier-bearing clearance is less than the tooth backlash. (C) 2014 Elsevier Masson SAS. All rights reserved. C1 [Guo, Yi; Keller, Jonathan] Natl Wind Technol Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. [Parker, Robert G.] Virginia Tech, Dept Mech Engn, Blacksburg, VA USA. RP Guo, Y (reprint author), Natl Wind Technol Ctr, Natl Renewable Energy Lab, Mail Stop 3811,15013 Denver West Pkwy, Golden, CO 80401 USA. EM yi.guo@nrel.gov RI Parker, Robert/A-3792-2008 OI Parker, Robert/0000-0003-3320-8898 FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 37 TC 11 Z9 12 U1 2 U2 27 PU GAUTHIER-VILLARS/EDITIONS ELSEVIER PI PARIS PA 23 RUE LINOIS, 75015 PARIS, FRANCE SN 0997-7538 EI 1873-7285 J9 EUR J MECH A-SOLID JI Eur. J. Mech. A-Solids PD SEP-OCT PY 2014 VL 47 BP 45 EP 57 DI 10.1016/j.euromechsol.2014.02.013 PG 13 WC Mechanics SC Mechanics GA AN6FB UT WOS:000340689200004 ER PT J AU Sebastiani, M Korsunsky, AM Eberl, C Bemporad, E Pharr, GM AF Sebastiani, M. Korsunsky, A. M. Eberl, C. Bemporad, E. Pharr, G. M. TI Discussion on "Interfacial Residual Stress Analysis of Thermal Spray Coatings by Miniature Ring-Core Cutting Combined with DIC Method" by JG Zhu et al., Experimental Mechanics DOI:10.1007/s11340-012-9640-2 SO EXPERIMENTAL MECHANICS LA English DT Editorial Material C1 [Sebastiani, M.; Bemporad, E.] Univ Rome ROMA TRE, Dept Engn, I-00146 Rome, Italy. [Korsunsky, A. M.] Univ Oxford, Dept Engn Sci, Oxford OX1 3PJ, England. [Eberl, C.] Fraunhofer IWM, D-79108 Freiburg, Germany. [Eberl, C.] Johns Hopkins Univ, Dept Mech Engn, Baltimore, MD 21218 USA. [Pharr, G. M.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Pharr, G. M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Sebastiani, M (reprint author), Univ Rome ROMA TRE, Dept Engn, Via Vasca Navale 79, I-00146 Rome, Italy. EM Marco.sebastiani@uniroma3.it RI Sebastiani, Marco/D-4228-2012; Bemporad, Edoardo/D-4251-2012 OI Sebastiani, Marco/0000-0002-9574-1578; Bemporad, Edoardo/0000-0001-6282-1929 NR 5 TC 0 Z9 0 U1 2 U2 17 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0014-4851 EI 1741-2765 J9 EXP MECH JI Exp. Mech. PD SEP PY 2014 VL 54 IS 7 BP 1305 EP 1306 DI 10.1007/s11340-014-9912-0 PG 2 WC Materials Science, Multidisciplinary; Mechanics; Materials Science, Characterization & Testing SC Materials Science; Mechanics GA AN2NP UT WOS:000340422900015 ER PT J AU Kwicklis, E Farnham, I AF Kwicklis, Edward Farnham, Irene TI Testing the C-14 ages and conservative behavior of dissolved C-14 in a carbonate aquifer in Yucca Flat, Nevada (USA), using Cl-36 from groundwater and packrat middens SO HYDROGEOLOGY JOURNAL LA English DT Article DE Groundwater age; Radioactive isotopes; Carbonate rocks; Solute transport; USA ID ARID SYSTEM HYDRODYNAMICS; SOUTHERN GREAT-BASIN; CAL KYR BP; UNITED-STATES; WATER; RADIOCARBON; DESERT; CALIBRATION; DIFFUSION; TRANSPORT AB Corrected groundwater C-14 ages from the carbonate aquifer in Yucca Flat at the former Nevada Test Site (now the Nevada National Security Site), USA, were evaluated by comparing temporal variations of groundwater Cl-36/Cl estimated with these C-14 ages with published records of meteoric Cl-36/Cl variations preserved in packrat middens (piles of plant fragments, fecal matter and urine). Good agreement between these records indicates that the groundwater C-14 ages are reasonable and that C-14 is moving with chloride without sorbing to the carbonate rock matrix or fracture coatings, despite opposing evidence from laboratory experiments. The groundwater C-14 ages are consistent with other hydrologic evidence that indicates significant basin infiltration ceased 8,000 to 10,000 years ago, and that recharge to the carbonate aquifer is from paleowater draining through overlying tuff confining units along major faults. This interpretation is supported by the relative age differences as well as hydraulic head differences between the alluvial and volcanic aquifers and the carbonate aquifer. The carbonate aquifer C-14 ages suggest that groundwater velocities throughout much of Yucca Flat are about 2 m/yr, consistent with the long-held conceptual model that blocking ridges of low-permeability rock hydrologically isolate the carbonate aquifer in Yucca Flat from the outlying regional carbonate flow system. C1 [Kwicklis, Edward] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Farnham, Irene] Navarro Intera LLC, North Las Vegas, NV 89030 USA. RP Kwicklis, E (reprint author), Los Alamos Natl Lab, POB 1163Drop Pt 19U,MS T003, Los Alamos, NM 87545 USA. EM kwicklis@lanl.gov FU US Department of Energy Nevada Field Office FX The authors would like to thank Bill Wilborn, Underground Test Area (UGTA) Project Manager, and the US Department of Energy Nevada Field Office for funding this study. NR 54 TC 1 Z9 1 U1 2 U2 16 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1431-2174 EI 1435-0157 J9 HYDROGEOL J JI Hydrogeol. J. PD SEP PY 2014 VL 22 IS 6 BP 1359 EP 1381 DI 10.1007/s10040-014-1131-3 PG 23 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA AN3OX UT WOS:000340498900010 ER PT J AU Berryman, JG AF Berryman, James G. TI Influence of crack density on geomechanical behavior of granular composites with porous grains and fluid-saturated pores SO INTERNATIONAL JOURNAL FOR NUMERICAL AND ANALYTICAL METHODS IN GEOMECHANICS LA English DT Article DE cracked grains; poroelastic response; orthotropic anisotropy ID EFFECTIVE ELASTIC-MODULI; LONG-WAVELENGTH PROPAGATION; HASHIN-SHTRIKMAN BOUNDS; TETRAGONAL SYMMETRIES; POLYCRYSTALS; CONSTANTS; CRYSTALS; MEDIA; INCLUSIONS; ROCKS AB The analysis of geomechanical behavior for granular systems including fluid-filled pores depends strongly on the crack density present within the system being studied. Effective overall bulk and shear moduli are both significantly influenced by these crack system parameters. Present effort concentrates on the geomechanical analyses needed to treat anisotropic (specifically orthotropic) poroelastic grains jumbled together to form an overall isotropic polycrystalline poroelastic material. As predicted, poroelastic effects induced by fluids in the cracks are observed to be significant for the effective bulk modulus, but simple pore fluids do not affect the magnitude of effective overall shear modulus. These results are also shown to depend in a quantitatively predictable way on crack density values. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Berryman, JG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd MS74R316C, Berkeley, CA 94720 USA. EM JGBerryman@lbl.gov FU US Department of Energy, at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Geosciences Research Program of the DOE Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences FX Work performed under the auspices of the US Department of Energy, at the Lawrence Berkeley National Laboratory under contract no. DE-AC02-05CH11231. Support was provided specifically by the Geosciences Research Program of the DOE Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. NR 49 TC 0 Z9 0 U1 0 U2 18 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0363-9061 EI 1096-9853 J9 INT J NUMER ANAL MET JI Int. J. Numer. Anal. Methods Geomech. PD SEP PY 2014 VL 38 IS 13 BP 1381 EP 1396 DI 10.1002/nag.2263 PG 16 WC Engineering, Geological; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA AN5AX UT WOS:000340602500004 ER PT J AU Abusnina, M Moutinho, H Al-Jassim, M Dehart, C Matin, M AF Abusnina, Mohamed Moutinho, Helio Al-Jassim, Mowafak Dehart, Clay Matin, Mohammed TI Fabrication and Characterization of CZTS Thin Films Prepared by the Sulfurization of RF-Sputtered Stacked Metal Precursors SO JOURNAL OF ELECTRONIC MATERIALS LA English DT Article DE Thin films; CZTS; sulfurization; stacked metal precursor ID OPTICAL-PROPERTIES; CU2ZNSNS4 AB In this work, Cu2ZnSnS4 (CZTS) thin films were prepared by the sulfurization of metal precursors deposited sequentially via radio frequency magnetron sputtering on Mo-coated soda-lime glass. The stack order of the precursors was Mo/Zn/Sn/Cu. Sputtered precursors were annealed in sulfur atmosphere with nine different conditions to study the impact of sulfurization time and substrate temperature on the structural, morphological, and optical properties of the final CZTS films. X-ray fluorescence was used to determine the elemental composition ratio of the metal precursors. Final CZTS films were characterized by x-ray diffraction (XRD), scanning electron microscopy (SEM), and energy-dispersive spectroscopy (EDS). XRD and EDS were combined to investigate the films' structure and to identify the presence of secondary phases. XRD analysis indicated an improvement in film crystallinity with an increase of the substrate temperature and annealing times. Also indicated was the minimization and/or elimination of secondary phases when the films experienced longer annealing time. EDS revealed slight Sn loss in films sulfurized at 550A degrees C; however, an increase of the sulfurization temperature to 600A degrees C did not confirm these results. SEM study showed that films treated with higher temperatures exhibited dense morphology, indicating the completion of the sulfurization process. The estimated absorption coefficient was on the order of 10(4) cm(-1) for all CZTS films, and the values obtained for the optical bandgap energy of the films were between 1.33 eV and 1.52 eV. C1 [Abusnina, Mohamed; Matin, Mohammed] Univ Denver, Elect & Comp Engn Dept, Daniel Felix Ritchie Sch Engn & Comp Sci, Denver, CO 80208 USA. [Abusnina, Mohamed; Moutinho, Helio; Al-Jassim, Mowafak; Dehart, Clay] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Abusnina, M (reprint author), Univ Denver, Elect & Comp Engn Dept, Daniel Felix Ritchie Sch Engn & Comp Sci, Denver, CO 80208 USA. EM mohamed.abusnina@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308] FX This work was performed under U.S. Department of Energy Contract No. DE-AC36-08GO28308 to the National Renewable Energy Laboratory. The authors would like to thank Jeff Alleman for the technical support. NR 31 TC 3 Z9 3 U1 2 U2 43 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0361-5235 EI 1543-186X J9 J ELECTRON MATER JI J. Electron. Mater. PD SEP PY 2014 VL 43 IS 9 BP 3145 EP 3154 DI 10.1007/s11664-014-3259-2 PG 10 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied SC Engineering; Materials Science; Physics GA AN1SJ UT WOS:000340363600012 ER PT J AU Saha, NR Ota, T Litman, GW Hansen, J Parra, Z Hsu, E Buonocore, F Canapa, A Cheng, JF Amemiya, CT AF Saha, Nil Ratan Ota, Tatsuya Litman, Gary W. Hansen, John Parra, Zuly Hsu, Ellen Buonocore, Francesco Canapa, Adriana Cheng, Jan-Fang Amemiya, Chris T. TI Genome complexity in the coelacanth is reflected in its adaptive immune system SO JOURNAL OF EXPERIMENTAL ZOOLOGY PART B-MOLECULAR AND DEVELOPMENTAL EVOLUTION LA English DT Article ID IMMUNOGLOBULIN HEAVY-CHAIN; MAJOR HISTOCOMPATIBILITY COMPLEX; CLASS SWITCH RECOMBINATION; TROUT ONCORHYNCHUS-MYKISS; VARIABLE REGION GENE; TAKIFUGU-RUBRIPES; MOLECULAR CHARACTERIZATION; LATIMERIA-MENADOENSIS; INDONESIAN COELACANTH; EXPRESSION ANALYSIS AB We have analyzed the available genome and transcriptome resources from the coelacanth in order to characterize genes involved in adaptive immunity. Two highly distinctive IgW-encoding loci have been identified that exhibit a unique genomic organization, including a multiplicity of tandemly repeated constant region exons. The overall organization of the IgW loci precludes typical heavy chain class switching. A locus encoding IgM could not be identified either computationally or by using several different experimental strategies. Four distinct sets of genes encoding Ig light chains were identified. This includes a variant sigma-type Ig light chain previously identified only in cartilaginous fishes and which is now provisionally denoted sigma-2. Genes encoding / and / T-cell receptors, and CD3, CD4, and CD8 co-receptors also were characterized. Ig heavy chain variable region genes and TCR components are interspersed within the TCR / locus; this organization previously was reported only in tetrapods and raises questions regarding evolution and functional cooption of genes encoding variable regions. The composition, organization and syntenic conservation of the major histocompatibility complex locus have been characterized. We also identified large numbers of genes encoding cytokines and their receptors, and other genes associated with adaptive immunity. In terms of sequence identity and organization, the adaptive immune genes of the coelacanth more closely resemble orthologous genes in tetrapods than those in teleost fishes, consistent with current phylogenomic interpretations. Overall, the work reported described herein highlights the complexity inherent in the coelacanth genome and provides a rich catalog of immune genes for future investigations. J. Exp. Zool. (Mol. Dev. Evol.) 322B: 438-463, 2014. (c) 2014 Wiley Periodicals, Inc. C1 [Saha, Nil Ratan; Amemiya, Chris T.] Benaroya Res Inst Virginia Mason, Mol Genet Program, Seattle, WA 98101 USA. [Ota, Tatsuya] Grad Univ Adv Studies, Dept Evolutionary Studies Biosyst, Hayama, Japan. [Litman, Gary W.] Univ S Florida, Coll Med, Dept Pediat, St Petersburg, FL 33701 USA. [Hansen, John] US Geol Survey, Western Fisheries Res Ctr, Seattle, WA USA. [Parra, Zuly] Univ New Mexico, Dept Biol, Ctr Evolutionary & Theoret Immunol, Albuquerque, NM 87131 USA. [Hsu, Ellen] SUNY Hlth Sci Ctr, Dept Physiol & Pharmacol, Brooklyn, NY USA. [Buonocore, Francesco] Univ Tuscia, Dept Innovat Biol Agrofood & Forest Syst, Viterbo, Italy. [Canapa, Adriana] Univ Politecn Marche, Dipartimento Sci Vita & Ambiente, Ancona, Italy. [Cheng, Jan-Fang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Amemiya, Chris T.] Univ Washington, Dept Biol, Seattle, WA 98195 USA. RP Saha, NR (reprint author), Benaroya Res Inst Virginia Mason, Mol Genet Program, 1201 Ninth Ave, Seattle, WA 98101 USA. EM nsaha@benaroyaresearch.org FU National Science Foundation [IOS-0321461, MCB-0719558]; National Institutes of Health [HL66728, AI23338, AI57559, RR14085, GM090049]; US Geological Survey Base Funds FX Grant sponsor: National Science Foundation (partial support); grant numbers: IOS-0321461, MCB-0719558; grant sponsor: National Institutes of Health; grant numbers: HL66728, AI23338, AI57559, RR14085, GM090049; grant sponsor: US Geological Survey Base Funds. NR 91 TC 6 Z9 6 U1 1 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1552-5007 EI 1552-5015 J9 J EXP ZOOL PART B JI J. Exp. Zool. Part B PD SEP PY 2014 VL 322 IS 6 SI SI BP 438 EP 463 DI 10.1002/jez.b.22558 PG 26 WC Evolutionary Biology; Developmental Biology; Zoology SC Evolutionary Biology; Developmental Biology; Zoology GA AN3JU UT WOS:000340484400011 PM 24464682 ER PT J AU Andrews, MJ Youngs, DL Livescu, D Wei, T AF Andrews, Malcolm J. Youngs, David L. Livescu, Daniel Wei, Tie TI Computational Studies of Two-Dimensional Rayleigh-Taylor Driven Mixing for a Tilted-Rig SO JOURNAL OF FLUIDS ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article ID NUMERICAL SIMULATIONS; INSTABILITY AB A time-dependent, incompressible, turbulent mixing problem, referred here to as the "tilted-rig," is defined, based results from an experiment that involved the introduction of a large-scale overturning motion, with a superposed localized Rayleigh-Taylor (RT) driven mixing. The problem serves to examine the development of RT turbulent mixing while being strained by a large-scale two-dimensional confined motion. Care is taken to define the problem in detail so others might use the definition, and the results, to help develop advanced models of buoyancy driven mixing in complex flows. Aside from a careful definition, the problem has been solved using two different implicit-large-Eddy-simulations (ILES) based codes, and with a direct numerical simulations (DNS) code. Two-dimensional and one-dimensional mix metrics are defined, and then used to examine the development of the mixing region, and the overall evolution of the flow. Comparison of simulations with experiment reveals that large-scale overturning can be well captured in all the simulations, similarly central mix widths, and spike/bubble sidewall penetrations are also in good agreement. A comparison between the different simulation methodologies, ILES and DNS, reveals an overall good agreement between mix metrics such as the amount of molecular mixing. The DNS simulations reveal a dependency on Reynolds number that merits further experimental work. C1 [Andrews, Malcolm J.; Livescu, Daniel] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Youngs, David L.] AWE, Aldermaston RG7 4PR, Berks, England. [Wei, Tie] New Mexico Inst Min & Technol, Dept Mech Engn, Socorro, NM 87801 USA. RP Andrews, MJ (reprint author), Los Alamos Natl Lab, MS F644, Los Alamos, NM 87544 USA. EM mandrews@lanl.gov; david.youngs@awe.co.uk; Livescu@lanl.gov; twei@nmt.edu OI Livescu, Daniel/0000-0003-2367-1547 FU United States Government FX The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for United States Government purposes. NR 19 TC 3 Z9 3 U1 0 U2 7 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0098-2202 EI 1528-901X J9 J FLUID ENG-T ASME JI J. Fluids Eng.-Trans. ASME PD SEP PY 2014 VL 136 IS 9 SI SI DI 10.1115/1.4027587 PG 14 WC Engineering, Mechanical SC Engineering GA AN1VU UT WOS:000340372900016 ER PT J AU Denissen, NA Rollin, B Reisner, JM Andrews, MJ AF Denissen, Nicholas A. Rollin, Bertrand Reisner, Jon M. Andrews, Malcolm J. TI The Tilted Rocket Rig: A Rayleigh-Taylor Test Case for RANS Models SO JOURNAL OF FLUIDS ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article ID RICHTMYER-MESHKOV; NUMERICAL SIMULATIONS; TURBULENCE MODEL; INSTABILITY; ACCELERATION; TRANSPORT AB Reynolds-Averaged Navier-Stokes (RANS) models remain the most common design tool in a wide variety of fluid mixing applications. This includes variable-density turbulent mixing as occurs in inertial confinement fusion. The present work extends validation of the BHR-2 RANS model for variable-density turbulence to a two-dimensional Rayleigh-Taylor test case, the "tilted-rig." The combined effects of bulk fluid motion and turbulence model behavior are discussed, and several quantities of interest are shown to demonstrate the capability of a four-equation turbulence model to describe this type of two-dimensional turbulent mixing. More generally, the tilted-rig test problem is shown to be a useful exercise for RANS model validation. C1 [Denissen, Nicholas A.; Rollin, Bertrand; Reisner, Jon M.; Andrews, Malcolm J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Denissen, NA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM denissen@lanl.gov FU U.S. Department of Energy by Los Alamos National Laboratory [DEAC52-06NA2-5396] FX This work was performed for the U.S. Department of Energy by Los Alamos National Laboratory under Contract No. DEAC52-06NA2-5396. The authors thank Tie Wei and Daniel Livescu for access to the DNS data. NR 61 TC 0 Z9 0 U1 1 U2 10 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0098-2202 EI 1528-901X J9 J FLUID ENG-T ASME JI J. Fluids Eng.-Trans. ASME PD SEP PY 2014 VL 136 IS 9 SI SI AR 091301 DI 10.1115/1.4027776 PG 13 WC Engineering, Mechanical SC Engineering GA AN1VU UT WOS:000340372900017 ER PT J AU Drikakis, D Youngs, DL Williams, RJR Schilling, O Dalziel, S AF Drikakis, Dimitris Youngs, David L. Williams, Robin J. R. Schilling, Oleg Dalziel, Stuart TI Special Issue on the 13th International Workshop on the Physics of Compressible Turbulent Mixing SO JOURNAL OF FLUIDS ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Editorial Material C1 [Drikakis, Dimitris] Cranfield Univ, Cranfield MK43 0AL, Beds, England. [Youngs, David L.; Williams, Robin J. R.] Atom Weap Estab, Aldermaston RG7 4PR, England. [Schilling, Oleg] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Dalziel, Stuart] Univ Cambridge, Cambridge CB3 0WA, England. RP Drikakis, D (reprint author), Cranfield Univ, Cranfield MK43 0AL, Beds, England. RI Williams, Robin/H-1637-2011 OI Williams, Robin/0000-0002-0486-0580 NR 0 TC 0 Z9 0 U1 0 U2 1 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0098-2202 EI 1528-901X J9 J FLUID ENG-T ASME JI J. Fluids Eng.-Trans. ASME PD SEP PY 2014 VL 136 IS 9 SI SI AR 090201 PG 1 WC Engineering, Mechanical SC Engineering GA AN1VU UT WOS:000340372900001 ER PT J AU Melvin, J Rao, P Kaufman, R Lim, H Yu, Y Glimm, J Sharp, DH AF Melvin, J. Rao, P. Kaufman, R. Lim, H. Yu, Y. Glimm, J. Sharp, D. H. TI Turbulent Transport at High Reynolds Numbers in an Inertial Confinement Fusion Context SO JOURNAL OF FLUIDS ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article DE computational fluid dynamics; hydrodynamics; large eddy simulation (LES); mixing; turbulence modeling; shocks ID MODEL AB Mix is a critical input to hydro simulations used in modeling chemical or nuclear reaction processes in fluids. It has been identified as a possible cause of performance degradation in inertial confinement fusion (ICF) targets. Mix contributes to numerical solution uncertainty through its dependence on turbulent transport coefficients, themselves uncertain and even controversial quantities. These coefficients are a central object of study in this paper, carried out in an Richtmyer-Meshkov unstable circular two-dimensional (2D) geometry suggested by an ICF design. We study a pre-turbulent regime and a fully developed regime. The former, at times between the first shock passage and reshock, is characterized by mixing in the form of interpenetrating but coherent fingers and the latter, at times after reshock, has fully developed turbulent structures. This paper focuses on the scaling of spatial averages of turbulence coefficients under mesh refinement and under variation of molecular viscosity [i.e., Reynolds number (Re)]. We find that the coefficients scale under mesh refinement with a power of spatial grid spacing derived from the Kolmogorov 2/3 law, especially after reshock. We document the dominance of turbulent over molecular transport and convergence of the turbulent transport coefficients in the infinite Re limit. The transport coefficients do not coincide for the pre- and post-reshock flow regimes, with significantly stronger transport coefficients after reshock. C1 [Melvin, J.; Rao, P.; Kaufman, R.; Lim, H.; Yu, Y.; Glimm, J.] SUNY Stony Brook, Dept Appl Math & Stat, Stony Brook, NY 11794 USA. [Sharp, D. H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Rao, P (reprint author), SUNY Stony Brook, Dept Appl Math & Stat, Stony Brook, NY 11794 USA. EM prao@ams.sunysb.edu; glimm@ams.sunysb.edu; dcso@lanl.gov FU Leland Stanford Junior University (DOE) [2175022040367A]; Army Research Office [W911NF0910306]; Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357] FX This work is supported in part by Leland Stanford Junior University 2175022040367A (subaward with DOE as prime sponsor), Army Research Office W911NF0910306. Computational resources were provided by the Stony Brook Galaxy cluster and the Stony Brook/BNL New York Blue Gene/L IBM machine. This research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-06CH11357. David H. Sharp, Fellow Los Alamos National Laboratory, retired. Los Alamos National Laboratory preprint LA-UR-13-20765. Stony Brook University preprint SUNYSB-AMS-13-02. NR 18 TC 3 Z9 3 U1 0 U2 3 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0098-2202 EI 1528-901X J9 J FLUID ENG-T ASME JI J. Fluids Eng.-Trans. ASME PD SEP PY 2014 VL 136 IS 9 SI SI AR 091206 DI 10.1115/1.4027382 PG 6 WC Engineering, Mechanical SC Engineering GA AN1VU UT WOS:000340372900010 ER PT J AU Wing, BJ Schaeffer, DA Hendricks, TR Bennett, D Chaum, E Simpson, JT AF Wing, B. J. Schaeffer, D. A. Hendricks, T. R. Bennett, D. Chaum, E. Simpson, J. T. TI Structural Manipulation of Microcone Arrays for Microsurgical Modification of Ophthalmic Tissues SO JOURNAL OF MEDICAL DEVICES-TRANSACTIONS OF THE ASME LA English DT Article; Proceedings Paper CT 13th Annual University-of-Minnesota Design of Medical Devices Conference CY APR 07-10, 2014 CL Minneapolis, MN ID TRANSDERMAL DRUG-DELIVERY; RECURRENT CORNEAL EROSION; ANTERIOR STROMAL PUNCTURE; MICRONEEDLES AB The purpose of this study was to utilize controllable fiber-drawing techniques in order to fabricate glass microcone arrays for use in office-based optical surgery instruments. The cone spacing is controlled via the drawing process while an etching process controls the cone height-to-base ratio. The device viability was tested by imprinting, and subsequent staining, of low-density polyethylene and porcine corneas, resulting in a consistent patterned structure of micronsized perforations. After imprint, the device was examined and no evidence of microcone fracture or overpenetration was present during the course of these experiments. This research promises to lead to advances in optical surgery for the treatment of recurrent corneal erosions, providing quicker, safer, and more cost-effective procedures with decreased risk of vision loss and scarring associated with current procedures such as anterior stromal puncture. The ease of procedure and micron-sized incisions could potentially replace current techniques and provide a viable treatment alternative for recurrent corneal erosions in the visual axis. C1 [Wing, B. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Schaeffer, D. A.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Hendricks, T. R.; Simpson, J. T.] Oak Ridge Natl Lab, Measurement Sci & Syst Engn Div, Oak Ridge, TN 37831 USA. [Bennett, D.; Chaum, E.] Univ Tennessee, Ctr Hlth Sci, Dept Ophthalmol, Memphis, TN 38163 USA. RP Schaeffer, DA (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. EM bwing1@utk.edu; schaefferda@ornl.gov; troy.r.hendricks@jci.com; bennettmon@gmail.com; echaum@uthsc.edu; simpsonjts@gmail.com FU Oak Ridge National Laboratory (ORNL); Research to Prevent Blindness, New York, NY; Plough Foundation, Memphis, TN; Office of Science; Oak Ridge Institute for Science and Education (ORISE) FX This research was supported by Oak Ridge National Laboratory (ORNL), managed by UT-Battelle, LLC for the U.S. Department of Energy, an unrestricted Departmental grant from Research to Prevent Blindness, New York, NY, the Plough Foundation, Memphis, TN, and the Office of Science and the Oak Ridge Institute for Science and Education (ORISE). The authors would also like to acknowledge Dr. Justin Wilkin for the image presented in Fig. 5. NR 21 TC 0 Z9 0 U1 0 U2 4 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 1932-6181 EI 1932-619X J9 J MED DEVICES JI J. Med. Devices PD SEP PY 2014 VL 8 IS 3 AR 034558 DI 10.1115/1.4026828 PG 4 WC Engineering, Biomedical SC Engineering GA AN2SC UT WOS:000340434600061 ER PT J AU Burger, S Boulyga, SF Penkin, MV Bostick, D Jovanovic, S Lindvall, R Rasmussen, G Riciputi, L AF Buerger, S. Boulyga, S. F. Penkin, M. V. Bostick, D. Jovanovic, S. Lindvall, R. Rasmussen, G. Riciputi, L. TI Quantifying multiple trace elements in uranium ore concentrates: an interlaboratory comparison SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT Biennial Symposium on Nuclear and Radiochemistry CY FEB 19-23, 2013 CL Jabalpur, INDIA DE Impurity analysis; Inductively coupled plasma mass spectrometry; Interlaboratory comparison; Reference material; Uranium ore concentrate ID RARE-EARTH-ELEMENTS; ICP-MS; SPECTROMETRIC DETERMINATION; BEARING MATERIALS; NUCLEAR-FUEL; IMPURITIES; PLASMA; MATRIX; SAMPLE; RESOLUTION AB An intercomparison was organized, with six laboratories tasked to quantify sixty-nine impurities in two uranium materials. The main technique employed for analysis was inductively coupled plasma mass spectrometry in combination with matrix-matched external calibration. The results presented highlight the current state-of-the-practice; lessons learned include previously unaccounted polyatomic interferences, issues related to sample dissolution, blank correction and calibration, and the challenge of estimating measurement uncertainties. The exercise yielded consensus values for the two analysed materials, suitable for use as laboratory standards to partially fill a gap in the availability of uranium reference materials characterized for impurities. C1 [Buerger, S.; Boulyga, S. F.; Penkin, M. V.] IAEA, Dept Safeguards, A-1400 Vienna, Austria. [Bostick, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jovanovic, S.] Canadian Nucl Safety Commiss Lab, Ottawa, ON K1V 1E1, Canada. [Lindvall, R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Rasmussen, G.] Inst Transuranium Elements, D-76125 Karlsruhe, Germany. [Riciputi, L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Penkin, MV (reprint author), IAEA, Dept Safeguards, POB 100, A-1400 Vienna, Austria. EM m.penkin@iaea.org NR 46 TC 6 Z9 6 U1 0 U2 20 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD SEP PY 2014 VL 301 IS 3 BP 711 EP 729 DI 10.1007/s10967-014-3224-9 PG 19 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA AN3MA UT WOS:000340491000010 ER PT J AU Tu, QC Yu, H He, ZL Deng, Y Wu, LY Van Nostrand, JD Zhou, AF Voordeckers, J Lee, YJ Qin, YJ Hemme, CL Shi, Z Xue, K Yuan, T Wang, AJ Zhou, JZ AF Tu, Qichao Yu, Hao He, Zhili Deng, Ye Wu, Liyou Van Nostrand, Joy D. Zhou, Aifen Voordeckers, James Lee, Yong-Jin Qin, Yujia Hemme, Christopher L. Shi, Zhou Xue, Kai Yuan, Tong Wang, Aijie Zhou, Jizhong TI GeoChip 4: a functional gene-array-based high-throughput environmental technology for microbial community analysis SO MOLECULAR ECOLOGY RESOURCES LA English DT Article DE environmental technology; functional gene array; GeoChip 4; microbial community analysis ID MICROARRAY-BASED ANALYSIS; PROBE DESIGN CRITERIA; METAGENOMIC ANALYSIS; ELEVATED CO2; HOST-RANGE; DEEP-SEA; SOIL; DIVERSITY; BACTERIA; VIRUSES AB Micro-organisms play critical roles in many important biogeochemical processes in the Earth's biosphere. However, understanding and characterizing the functional capacity of microbial communities are still difficult due to the extremely diverse and often uncultivable nature of most micro-organisms. In this study, we developed a new functional gene array, GeoChip 4, for analysing the functional diversity, composition, structure, metabolic potential/activity and dynamics of microbial communities. GeoChip 4 contained approximately 82 000 probes covering 141 995 coding sequences from 410 functional gene families related to microbial carbon (C), nitrogen (N), sulphur (S), and phosphorus (P) cycling, energy metabolism, antibiotic resistance, metal resistance/reduction, organic remediation, stress responses, bacteriophage and virulence. A total of 173 archaeal, 4138 bacterial, 404 eukaryotic and 252 viral strains were targeted, providing the ability to analyse targeted functional gene families of micro-organisms included in all four domains. Experimental assessment using different amounts of DNA suggested that as little as 500 ng environmental DNA was required for good hybridization, and the signal intensities detected were well correlated with the DNA amount used. GeoChip 4 was then applied to study the effect of long-term warming on soil microbial communities at a Central Oklahoma site, with results indicating that microbial communities respond to long-term warming by enriching carbon degradation, nutrient cycling (nitrogen and phosphorous) and stress response gene families. To the best of our knowledge, GeoChip 4 is the most comprehensive functional gene array for microbial community analysis. C1 [Tu, Qichao; Yu, Hao; He, Zhili; Deng, Ye; Wu, Liyou; Van Nostrand, Joy D.; Zhou, Aifen; Voordeckers, James; Lee, Yong-Jin; Qin, Yujia; Hemme, Christopher L.; Shi, Zhou; Xue, Kai; Yuan, Tong; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, IEG, Norman, OK 73019 USA. [Yu, Hao] Harbin Inst Technol, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China. [Yu, Hao] Liaoning Tech Univ, Sch Environm Sci & Engn, Fuxing 123000, Liaoning, Peoples R China. [Wang, Aijie] Chinese Acad Sci, Ecoenvironm Sci Res Ctr, Beijing 100085, Peoples R China. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Zhou, JZ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Biol, IEG, Norman, OK 73019 USA. EM jzhou@ou.edu RI Van Nostrand, Joy/F-1740-2016; OI Van Nostrand, Joy/0000-0001-9548-6450; ?, ?/0000-0002-7584-0632 FU Office of Science, Office of Biological and Environmental Research (OBER) of the U.S. Department of Energy [DE-AC02-05CH11231]; OBER Biological Systems Research on the Role of Microbial Communities in Carbon Cycling Program [DE-SC0004601]; U.S. National Science Foundation MacroSystems Biology programme [NSF EF-1065844]; Oklahoma Applied Research Support (OARS), Oklahoma Center for the Advancement of Science and Technology (OCAST), State of Oklahoma [AR062-034, AR11-035] FX This work was conducted by ENIGMA-Ecosystems and Networks Integrated with Genes and Molecular Assemblies (http://enigma.lbl.gov), a Scientific Focus Area Program at Lawrence Berkeley National Laboratory, was supported by the Office of Science, Office of Biological and Environmental Research (OBER), of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This study was also supported by the OBER Biological Systems Research on the Role of Microbial Communities in Carbon Cycling Program (DE-SC0004601), by the U.S. National Science Foundation MacroSystems Biology programme under the contract (NSF EF-1065844) and by Oklahoma Applied Research Support (OARS), Oklahoma Center for the Advancement of Science and Technology (OCAST) through the Projects AR062-034 and AR11-035, the State of Oklahoma. NR 105 TC 55 Z9 59 U1 23 U2 154 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1755-098X EI 1755-0998 J9 MOL ECOL RESOUR JI Mol. Ecol. Resour. PD SEP PY 2014 VL 14 IS 5 BP 914 EP 928 DI 10.1111/1755-0998.12239 PG 15 WC Biochemistry & Molecular Biology; Ecology; Evolutionary Biology SC Biochemistry & Molecular Biology; Environmental Sciences & Ecology; Evolutionary Biology GA AN2OL UT WOS:000340425100004 PM 24520909 ER PT J AU Baxter, HL Mazarei, M Labbe, N Kline, LM Cheng, QK Windham, MT Mann, DGJ Fu, CX Ziebell, A Sykes, RW Rodriguez, M Davis, MF Mielenz, JR Dixon, RA Wang, ZY Stewart, CN AF Baxter, Holly L. Mazarei, Mitra Labbe, Nicole Kline, Lindsey M. Cheng, Qunkang Windham, Mark T. Mann, David G. J. Fu, Chunxiang Ziebell, Angela Sykes, Robert W. Rodriguez, Miguel, Jr. Davis, Mark F. Mielenz, Jonathan R. Dixon, Richard A. Wang, Zeng-Yu Stewart, C. Neal, Jr. TI Two-year field analysis of reduced recalcitrance transgenic switchgrass SO PLANT BIOTECHNOLOGY JOURNAL LA English DT Article DE COMT; Field trial; lignocellulosic biofuel; switchgrass ID ACID-O-METHYLTRANSFERASE; LIGNIN BIOSYNTHESIS; PANICUM-VIRGATUM; CELL-WALL; BIOFUEL PRODUCTION; DOWN-REGULATION; LIGNOCELLULOSIC BIOMASS; ALTERED LIGNIFICATION; DISEASE RESISTANCE; PUCCINIA-EMACULATA AB Switchgrass (Panicum virgatum L.) is a leading candidate for a dedicated lignocellulosic biofuel feedstock owing to its high biomass production, wide adaptation and low agronomic input requirements. Lignin in cell walls of switchgrass, and other lignocellulosic feedstocks, severely limits the accessibility of cell wall carbohydrates to enzymatic breakdown into fermentable sugars and subsequently biofuels. Low-lignin transgenic switchgrass plants produced by the down-regulation of caffeic acid O-methyltransferase (COMT), a lignin biosynthetic enzyme, were analysed in the field for two growing seasons. COMT transcript abundance, lignin content and the syringyl/guaiacyl lignin monomer ratio were consistently lower in the COMT-down-regulated plants throughout the duration of the field trial. In general, analyses with fully established plants harvested during the second growing season produced results that were similar to those observed in previous greenhouse studies with these plants. Sugar release was improved by up to 34% and ethanol yield by up to 28% in the transgenic lines relative to controls. Additionally, these results were obtained using senesced plant material harvested at the end of the growing season, compared with the young, green tissue that was used in the greenhouse experiments. Another important finding was that transgenic plants were not more susceptible to rust (Puccinia emaculata). The results of this study suggest that lignin down-regulation in switchgrass can confer real-world improvements in biofuel yield without negative consequences to biomass yield or disease susceptibility. C1 [Baxter, Holly L.; Mazarei, Mitra; Mann, David G. J.; Stewart, C. Neal, Jr.] Univ Tennessee, Dept Plant Sci, Knoxville, TN 37996 USA. [Baxter, Holly L.; Mazarei, Mitra; Mann, David G. J.; Fu, Chunxiang; Ziebell, Angela; Sykes, Robert W.; Rodriguez, Miguel, Jr.; Davis, Mark F.; Mielenz, Jonathan R.; Dixon, Richard A.; Wang, Zeng-Yu; Stewart, C. Neal, Jr.] Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, Oak Ridge, TN 37831 USA. [Labbe, Nicole; Kline, Lindsey M.] Univ Tennessee, Ctr Renewable Carbon, Knoxville, TN 37996 USA. [Cheng, Qunkang; Windham, Mark T.] Univ Tennessee, Dept Entomol & Plant Pathol, Knoxville, TN 37996 USA. [Fu, Chunxiang; Wang, Zeng-Yu] Samuel Roberts Noble Fdn Inc, Ardmore, OK 73401 USA. [Ziebell, Angela; Sykes, Robert W.; Davis, Mark F.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Rodriguez, Miguel, Jr.; Mielenz, Jonathan R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Dixon, Richard A.] Univ N Texas, Dept Biol Sci, Denton, TX 76203 USA. RP Stewart, CN (reprint author), Univ Tennessee, Dept Plant Sci, Knoxville, TN 37996 USA. EM nealstewart@utk.edu OI davis, mark/0000-0003-4541-9852 FU Southeastern Sun Grant Center; BioEnergy Science Center; Office of Biological and Environmental Research in the DOE Office of Science FX We thank Crissa Doeppke, Geoff Turner, Steve Decker, Melvin Tucker and Kelsey Yee for their assistance with the cell wall and biofuel characterization. We also thank Ben Wolfe, Derek Green, Johnathan Branson and the UT field staff for general field maintenance, Arnold Saxton and Charlie Kwit for their assistance with the field design and statistical analyses and Susan Holladay for her assistance with data entry into LIMS. This work was supported by funding from the Southeastern Sun Grant Center and the BioEnergy Science Center. The BioEnergy Science Center is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. NR 52 TC 33 Z9 33 U1 8 U2 44 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1467-7644 EI 1467-7652 J9 PLANT BIOTECHNOL J JI Plant Biotechnol. J. PD SEP PY 2014 VL 12 IS 7 BP 914 EP 924 DI 10.1111/pbi.12195 PG 11 WC Biotechnology & Applied Microbiology; Plant Sciences SC Biotechnology & Applied Microbiology; Plant Sciences GA AN3ZS UT WOS:000340528000010 PM 24751162 ER PT J AU Flicker, J Kaplar, R Yang, B Marinella, M Granata, J AF Flicker, Jack Kaplar, Robert Yang, Benjamin Marinella, Matthew Granata, Jennifer TI Insulated gate bipolar transistor reliability testing protocol for PV inverter applications SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE IGBT; photovoltaic; power electronics; transistors; BOS; reliability ID SHORT-CIRCUIT CONDITIONS; SINGLE-CHIP IGBT; FAILURE MECHANISMS; OXIDE BREAKDOWN; MODULES; BEHAVIOR; DEVICES; STRESS; DEGRADATION; METHODOLOGY AB To decrease the cost of ownership of photovoltaic systems, less costly and more reliable photovoltaic inverters must be developed. Insulated gate bipolar transistors are a significant cause of inverter failures and system inefficiencies, so a thorough understanding of their strengths and weaknesses with regards to inverters is necessary. This paper summarizes the current state of experimentation surrounding the use of IGBTs in photovoltaic inverters and discusses their construction, use, lifetime, and reliability of IGBTs regularly used in photovoltaic inverters. Published 2013. This article is a U.S. Government work and is in the public domain in the USA. C1 [Flicker, Jack; Kaplar, Robert; Yang, Benjamin; Marinella, Matthew; Granata, Jennifer] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Flicker, J (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jdflick@sandia.gov FU DOE Office of Energy Efficiency and Renewable Energy; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the DOE Office of Energy Efficiency and Renewable Energy. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 96 TC 3 Z9 3 U1 0 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD SEP PY 2014 VL 22 IS 9 BP 970 EP 983 DI 10.1002/pip.2351 PG 14 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA AN4WL UT WOS:000340589800004 ER PT J AU Trumbo, BA Ahmann, ML Renholds, JF Brown, RS Colotelo, AH Deng, ZD AF Trumbo, Bradly A. Ahmann, Martin L. Renholds, Jon F. Brown, Richard S. Colotelo, Alison H. Deng, Z. D. TI Improving hydroturbine pressures to enhance salmon passage survival and recovery SO REVIEWS IN FISH BIOLOGY AND FISHERIES LA English DT Article DE Hydroturbine; Turbine passage; Turbine design; Salmon; Survival; Barotrauma ID JUVENILE CHINOOK SALMON; ACOUSTIC TELEMETRY SYSTEM; HYDRO-TURBINE PASSAGE; NEUTRALLY BUOYANT; TRANSMITTERS; BAROTRAUMA; SMOLTS; INSTRUMENTATION; MORTALITY; TRACKING AB Barotrauma caused by rapid decompression during hydroturbine (turbine) passage may occur as fish move through the low pressure region below the turbine runner. This scenario is of particular concern in North American rivers with populations of ESA-listed salmon. The US Army Corps of Engineers (USACE) and the Pacific Northwest National Laboratory released Sensor Fish into lower Snake and Columbia River turbines to determine the magnitude and rate of pressure change fish might experience. Recorded pressures were applied to simulated turbine passage (STP) in laboratory studies to determine the effect of rapid decompression on juvenile Chinook salmon. These STP studies have increased our understanding of how pressure effects fish passing through turbines and suggest that the ratio of pressure change [acclimation pressure (the depth upstream of the dam where fish are neutrally buoyant) divided by nadir pressure (lowest pressure)] is highly predictive in determining the effect on smolt survival. However, uncertainty remains in smolt acclimation depth prior to entering turbine intakes at hydroelectric facilities. The USACE continues to make progress on salmon survival and recovery efforts through continued research and by applying pressure study results to turbine design. Designing new turbines with higher nadir pressure criteria is likely to provide safer fish passage for all salmonid species experiencing turbine passage. C1 [Trumbo, Bradly A.; Ahmann, Martin L.; Renholds, Jon F.] US Army Corps Engineers, Walla Walla, WA 99362 USA. [Brown, Richard S.; Colotelo, Alison H.; Deng, Z. D.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Trumbo, BA (reprint author), US Army Corps Engineers, 201N Third Ave, Walla Walla, WA 99362 USA. EM bradly.a.trumbo@usace.army.mil RI Deng, Daniel/A-9536-2011 OI Deng, Daniel/0000-0002-8300-8766 NR 52 TC 7 Z9 7 U1 9 U2 45 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0960-3166 EI 1573-5184 J9 REV FISH BIOL FISHER JI Rev. Fish. Biol. Fish. PD SEP PY 2014 VL 24 IS 3 SI SI BP 955 EP 965 DI 10.1007/s11160-013-9340-8 PG 11 WC Fisheries; Marine & Freshwater Biology SC Fisheries; Marine & Freshwater Biology GA AN2ZS UT WOS:000340455200015 ER PT J AU Grant, SL Kim, M Lin, P Crist, KC Ghosh, S Kotamarthi, VR AF Grant, Shanique L. Kim, Myoungvvoo Lin, Peng Crist, Kevin C. Ghosh, Saikat Kotamarthi, V. Rao TI A simulation study of atmospheric mercury and its deposition in the Great Lakes SO ATMOSPHERIC ENVIRONMENT LA English DT Article DE Deposition; Integrated planning management; Reactive gaseous mercury; Chinese emissions ID WET DEPOSITION; ANTHROPOGENIC SOURCES; EMISSION INVENTORY; SPATIAL-PATTERNS; UNITED-STATES; CMAQ MODEL; REGION; TRENDS; CHINA AB The Great Lakes eco-region is one of the largest sources of fresh water in North America; however it is chronically exposed to heavy metal loadings such as mercury. In this study a comprehensive model evaluation was conducted to determine mercury loadings to the Great Lakes. The study also evaluated the relative impact of anthropogenic mercury emissions from China, regional and global sources on deposition to the Great Lakes. For the 2005 study period, CMAQ4.7.1 model estimated a total of 6.4 +/- 0.5 metric tons of mercury deposited in the Great Lakes. The total deposition breakdown showed a net loading for Lake Superior of 1906 +/- 246 kg/year which is the highest of all the lakes. Lake Michigan followed with 1645 +/- 203 kg/year and 1511 +/- 107 kg/year in Lake Huron. The lowest total deposition was seen in Lakes Erie and Ontario amassing annual totals of 837 +/- 107 kg and 506 +/- 63 kg, respectively. Wet and dry deposition of mercury were both significant pathways and exhibited strong seasonal variability with higher deposition occurring in the warmer months (June November) and the lowest in winter. Wet deposition of RGM significantly influenced the deposition proportions accounting for roughly 90% of all mercury deposited. Of the three emission sources (global background, integrated planning management (IPM) and Chinese), global background concentrations represented the maximum impact to deposition loading in the Great Lakes, except for Lake Erie and parts of Lake Michigan. There was minimal seasonality for the global background, but differences in percentage contribution between dry (28-97%) and wet deposition (43-98%) was predicted. The contributions were seen mainly in the northern sections of the Great Lakes further away from IPM point sources. These findings suggest strong localized impact of IPM sources on the southernmost lakes. Deposition as a result of emissions from China exhibited seasonality in both wet and dry deposition and showed significant contributions ranging from 0.2 to 9%. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Grant, Shanique L.; Kim, Myoungvvoo; Lin, Peng; Crist, Kevin C.; Ghosh, Saikat] Ohio Univ, Ctr Air Qual, Athens, OH 45701 USA. [Kotamarthi, V. Rao] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. RP Crist, KC (reprint author), Ohio Univ, Ctr Air Qual, Stocker 159, Athens, OH 45701 USA. EM cristk@ohio.edu FU Great Lakes Commission under Great Lakes Air Deposition (GLAD) program FX This project (Assessing Methods of Alleviating Impacts from Mercury on Human Health and Environment in the Great Lakes Basin) was funded by the Great Lakes Commission under the Great Lakes Air Deposition (GLAD) program. The authors thank Beth A. Drewniak for contributions to the global chemical model analyses and development. Also, we acknowledge Jozef M. Pacyna, Elisabeth G. Pacyna and David G. Streets for providing the global anthropogenic mercury emissions data that was incorporated in the global model. NR 41 TC 2 Z9 4 U1 5 U2 58 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1352-2310 EI 1873-2844 J9 ATMOS ENVIRON JI Atmos. Environ. PD SEP PY 2014 VL 94 BP 164 EP 172 DI 10.1016/j.atmosenv.2014.05.033 PG 9 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA AN1AY UT WOS:000340316300018 ER PT J AU Duncan, BN Prados, AI Lamsal, LN Liu, Y Streets, DG Gupta, P Hilsenrath, E Kahn, RA Nielsen, JE Beyersdorf, AJ Burton, SP Fiore, AM Fishman, J Henze, DK Hostetler, CA Krotkov, NA Lee, P Lin, MY Pawson, S Pfister, G Pickering, KE Pierce, RB Yoshida, Y Ziemba, LD AF Duncan, Bryan N. Prados, Ana I. Lamsal, Lok N. Liu, Yang Streets, David G. Gupta, Pawan Hilsenrath, Ernest Kahn, Ralph A. Nielsen, J. Eric Beyersdorf, Andreas J. Burton, Sharon P. Fiore, Arlene M. Fishman, Jack Henze, Daven K. Hostetler, Chris A. Krotkov, Nickolay A. Lee, Pius Lin, Meiyun Pawson, Steven Pfister, Gabriele Pickering, Kenneth E. Pierce, R. Bradley Yoshida, Yasuko Ziemba, Luke D. TI Satellite data of atmospheric pollution for US air quality applications: Examples of applications, summary of data end-user resources, answers to FAQs, and common mistakes to avoid SO ATMOSPHERIC ENVIRONMENT LA English DT Review DE Satellite data; Air quality; End-user resources; Remote sensing ID AEROSOL OPTICAL DEPTH; OZONE MONITORING EXPERIMENT; RETRIEVAL ALGORITHM; TROPOSPHERIC OZONE; ECONOMIC RECESSION; ISOPRENE EMISSIONS; NITROGEN-OXIDES; UNITED-STATES; NOX EMISSIONS; MEXICO-CITY AB Satellite data of atmospheric pollutants are becoming more widely used in the decision-making and environmental management activities of public, private sector and non-profit organizations. They are employed for estimating emissions, tracking pollutant plumes, supporting air quality forecasting activities, providing evidence for "exceptional event" declarations, monitoring regional long-term trends, and evaluating air quality model output. However, many air quality managers are not taking full advantage of the data for these applications nor has the full potential of satellite data for air quality applications been realized. A key barrier is the inherent difficulties associated with accessing, processing, and properly interpreting observational data. A degree of technical skill is required on the part of the data end-user, which is often problematic for air quality agencies with limited resources. Therefore, we 1) review the primary uses of satellite data for air quality applications, 2) provide some background information on satellite capabilities for measuring pollutants, 3) discuss the-many resources available to the end-user for accessing, processing, and visualizing the data, and 4) provide answers to common questions in plain language. Published by Elsevier Ltd. C1 [Duncan, Bryan N.; Prados, Ana I.; Lamsal, Lok N.; Gupta, Pawan; Kahn, Ralph A.; Krotkov, Nickolay A.; Pawson, Steven; Pickering, Kenneth E.; Yoshida, Yasuko] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Prados, Ana I.; Hilsenrath, Ernest] Univ Maryland, Joint Ctr Earth Syst Technol, Baltimore, MD 21201 USA. [Lamsal, Lok N.; Gupta, Pawan] Univ Space Res Assoc, Goddard Earth Sci Technol & Res, Columbia, MD USA. [Liu, Yang] Emory Univ, Rollins Sch Publ Hlth, Atlanta, GA 30322 USA. [Streets, David G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Hilsenrath, Ernest] Sigma Space Corp, Lanham, MD USA. [Nielsen, J. Eric; Yoshida, Yasuko] Sci Syst & Applicat Inc, Lanham, MD USA. [Beyersdorf, Andreas J.; Burton, Sharon P.; Hostetler, Chris A.; Ziemba, Luke D.] NASA, Langley Res Ctr, Hampton, VA 23665 USA. [Fiore, Arlene M.] Columbia Univ, Dept Earth & Environm Sci, Palisades, NY USA. [Fiore, Arlene M.] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY USA. [Fishman, Jack] St Louis Univ, St Louis, MO 63103 USA. [Henze, Daven K.] Univ Colorado, Boulder, CO 80309 USA. [Lee, Pius] NOAA, College Pk, MD USA. [Lin, Meiyun] Princeton Univ, Princeton, NJ 08544 USA. [Lin, Meiyun] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Pfister, Gabriele] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Pierce, R. Bradley] NOAA, Madison, WI USA. RP Duncan, BN (reprint author), NASA, Goddard Space Flight Ctr, Code 614, Greenbelt, MD 20771 USA. EM Bryan.N.Duncan@nasa.gov RI Pickering, Kenneth/E-6274-2012; Pawson, Steven/I-1865-2014; Duncan, Bryan/A-5962-2011; Lin, Meiyun/D-6107-2013; Pierce, Robert Bradley/F-5609-2010; Krotkov, Nickolay/E-1541-2012; Lee, Pius/D-5201-2016 OI Pawson, Steven/0000-0003-0200-717X; Lin, Meiyun/0000-0003-3852-3491; Pierce, Robert Bradley/0000-0002-2767-1643; Krotkov, Nickolay/0000-0001-6170-6750; FU NASA Air Quality Applied Sciences Team (AQAST); Applied Remote SEnsing Training (ARSET) program, within NASA's Applied Sciences Program FX This work was funded by the NASA Air Quality Applied Sciences Team (AQAST) and the Applied Remote SEnsing Training (ARSET) program, within NASA's Applied Sciences Program. We thank Ginger Butcher, the NASA Aura Mission's education and public outreach lead, for her comments which greatly improved the readability of the article. NR 89 TC 29 Z9 29 U1 4 U2 71 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1352-2310 EI 1873-2844 J9 ATMOS ENVIRON JI Atmos. Environ. PD SEP PY 2014 VL 94 BP 647 EP 662 DI 10.1016/j.atmosenv.2014.05.061 PG 16 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA AN1AY UT WOS:000340316300069 ER PT J AU Albert, C Jameson, J Smith, P Harris, G AF Albert, Carolyne Jameson, John Smith, Peter Harris, Gerald TI Reduced diaphyseal strength associated with high intracortical vascular porosity within long bones of children with osteogenesis imperfecta SO BONE LA English DT Article DE Osteogenesis imperfecta; Pediatric bone; Flexural properties; Strength; Intracortical porosity ID OSTEOCYTE LACUNAR DENSITY; FEMORAL CORTICAL BONE; RADIATION MICRO-CT; MECHANICAL-PROPERTIES; COMPACT-BONE; ELASTIC PROPERTIES; CANCELLOUS BONE; MINERAL DENSITY; I COLLAGEN; ALENDRONATE TREATMENT AB Osteogenesis imperfecta is a genetic disorder resulting in bone fragility. The mechanisms behind this fragility are not well understood. In addition to characteristic bone mass deficiencies, research suggests that bone material properties are compromised in individuals with this disorder. However, little data exists regarding bone properties beyond the microstructural scale in individuals with this disorder. Specimens were obtained from long bone diaphyses of nine children with osteogenesis imperfecta during routine osteotomy procedures. Small rectangular beams, oriented longitudinally and transversely to the diaphyseal axis, were machined from these specimens and elastic modulus, yield strength, and maximum strength were measured in three-point bending. Intracortical vascular porosity, bone volume fraction, osteocyte lacuna density, and volumetric tissue mineral density were determined by synchrotron micro-computed tomography, and relationships among these mechanical properties and structural parameters were explored. Modulus and strength were on average 64-68% lower in the transverse vs. longitudinal beams (P < 0.001, linear mixed model). Vascular porosity ranged between 3 and 42% of total bone volume. Longitudinal properties were associated negatively with porosity (P <= 0.006, linear regressions). Mechanical properties, however, were not associated with osteocyte lacuna density or volumetric tissue mineral density (P >= 0.167). Bone properties and structural parameters were not associated significantly with donor age (P >= 0.225, linear mixed models). This study presents novel data regarding bone material strength in children with osteogenesis imperfecta. Results confirm that these properties are anisotropic. Elevated vascular porosity was observed in most specimens, and this parameter was associated with reduced bone material strength. These results offer insight toward understanding bone fragility and the role of intracortical porosity on the strength of bone tissue in children with osteogenesis imperfecta. (C) 2014 Elsevier Inc. All rights reserved. C1 [Albert, Carolyne; Smith, Peter; Harris, Gerald] Shriners Hosp Children, Chicago, IL USA. [Albert, Carolyne; Jameson, John; Harris, Gerald] Marquette Univ, OREC, Dept Biomed Engn, Milwaukee, WI 53201 USA. [Jameson, John] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Smith, Peter] Rush Univ, Med Ctr, Dept Orthoped Surg, Chicago, IL 60612 USA. RP Albert, C (reprint author), Marquette Univ, OREC, Dept Biomed Engn, 735 N 17th St,ASF Room 105, Milwaukee, WI 53201 USA. EM carolyne.albert@marquette.edu; john.jameson@marquette.edu; psmith@shrinenet.org; gerald.harris@marquette.edu FU U.S. Department of Education [H133P080005, H133E100007]; Clinical and Translational Science Award (CTSA) program of the National Center for Research Resources (NRCC) [UL1RR031973]; National Center for Advancing Translational Science (NCATS); Shriners Hospitals for Children as well as the ALS, a Division of the Lawrence Berkeley National Laboratory; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by NIDRR grants H133P080005 and H133E100007 from the U.S. Department of Education, and grant UL1RR031973 from the Clinical and Translational Science Award (CTSA) program of the National Center for Research Resources (NRCC) and the National Center for Advancing Translational Science (NCATS). These contents, however, do not necessarily represent the policy of the Department of Education, and endorsement by the Federal Government should not be assumed. Finally, the study was also supported by research fellowships from Shriners Hospitals for Children as well as the ALS, a Division of the Lawrence Berkeley National Laboratory. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 110 TC 4 Z9 4 U1 3 U2 9 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 8756-3282 EI 1873-2763 J9 BONE JI Bone PD SEP PY 2014 VL 66 BP 121 EP 130 DI 10.1016/j.bone.2014.05.022 PG 10 WC Endocrinology & Metabolism SC Endocrinology & Metabolism GA AM7DB UT WOS:000340023800016 PM 24928496 ER PT J AU Liu, B Xiao, HY Zhang, YW Aidhy, DS Weber, WJ AF Liu, Bin Xiao, Haiyan Zhang, Yanwen Aidhy, Dilpuneet S. Weber, William J. TI Investigation of oxygen point defects in cubic ZrO2 by density functional theory SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Cubic ZrO2; Nuclear materials; Point defects; Formation; Diffusion ID YTTRIA-STABILIZED ZIRCONIA; RADIATION-DAMAGE; DIFFUSION; VACANCIES; ENERGY AB The energetics of formation and migration of the oxygen vacancy and interstitial in cubic ZrO2 are investigated by density functional theory calculations. In an O-rich environment, the negatively charged oxygen interstitial is the most dominant defect whereas, the positively charged oxygen vacancy is the most dominant defect under O-poor conditions. Oxygen interstitial migration occurs by the interstitialcy and the direct interstitial mechanisms, with calculated migration energy barriers of 2.94 eV and 2.15 eV, respectively. For the oxygen vacancy, diffusion is preferred along the < 100 > direction, and the calculated energy barriers are 0.26 eV for V-o(2+), 0.27 eV for V-o(1+) and 0.54 eV for V-o(0). These results indicate that oxygen diffusivity is higher through the vacancy-migration mechanism. (C) 2014 Elsevier B.V. All rights reserved. C1 [Liu, Bin; Zhang, Yanwen; Aidhy, Dilpuneet S.; Weber, William J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Xiao, Haiyan; Zhang, Yanwen; Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Liu, B (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM liub2@ornl.gov; wjweber@utk.edu RI Weber, William/A-4177-2008; Liu, Bin/N-9955-2014 OI Weber, William/0000-0002-9017-7365; FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Office of Science, U.S. Department of Energy [DEAC02-05CH11231] FX This research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science, U.S. Department of Energy under Contract No. DEAC02-05CH11231. NR 44 TC 9 Z9 9 U1 5 U2 43 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD SEP PY 2014 VL 92 BP 22 EP 27 DI 10.1016/j.commatsci.2014.05.017 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA AM7LG UT WOS:000340048100004 ER PT J AU Barker, EI Choi, KS Sun, X Deda, E Allison, J Li, M Forsmark, J Zindel, J Godlewski, L AF Barker, E. I. Choi, K. S. Sun, X. Deda, E. Allison, J. Li, M. Forsmark, J. Zindel, J. Godlewski, L. TI Microstructure based modeling of beta phase influence on mechanical response of cast AM series Mg alloys SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Cast magnesium alloys; Microstructure; Plasticity; Eutectic phase; Volume fraction; Morphology ID MAGNESIUM ALLOY; PRESSURE; BEHAVIOR AB Understanding the impact of microstructural features on bulk response is key to improving the properties of AM series cast Mg alloys for more widespread use and for moving towards truly predicting modeling capabilities. This study focuses on modeling the volume fraction and morphology of beta phase within the microstructure of cast AM series Mg alloys and quantifying its impact on bulk performance. Finite element results are validated against experimental tensile tests of AM40 and AM70. Digital microstructures with fully connected beta phase morphologies are shown to increase hardening versus less connected, clumped morphologies. (C) 2014 Elsevier B.V. All rights reserved. C1 [Barker, E. I.; Choi, K. S.; Sun, X.] Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. [Deda, E.; Allison, J.] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. [Li, M.; Forsmark, J.; Zindel, J.; Godlewski, L.] Ford Motor Co, Ford Res & Adv Engn Lab, Dearborn, MI 48124 USA. RP Barker, EI (reprint author), Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. EM erin.barker@pnnl.gov FU Battelle Memorial Institute for the US Department of Energy [DE-AC05-76RL01830]; Department of Energy Vehicle Technologies Office under the Automotive Lightweighting Materials Program FX Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the US Department of Energy under Contract No. DE-AC05-76RL01830. This work was funded by the Department of Energy Vehicle Technologies Office under the Automotive Lightweighting Materials Program managed by William Joost. NR 25 TC 2 Z9 2 U1 2 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD SEP PY 2014 VL 92 BP 353 EP 361 DI 10.1016/j.commatsci.2014.03.010 PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA AM7LG UT WOS:000340048100046 ER PT J AU Huhn, WP Widom, M Gao, MC AF Huhn, William Paul Widom, Michael Gao, Michael C. TI First principles modeling of the temperature dependent ternary phase diagram for the Cu-Pd-S system SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Bulk sulfidization; Sulfidization threshholds; First principles calculations; Phase stability; Phase diagram; Pd16S7; Pd4S; CuPdS ID CRYSTAL-STRUCTURE; AB-INITIO; CHALCOCITE CU2S; X-RAY; ALLOYS; STABILITY; MEMBRANES; SULFIDE AB As an aid to the development of hydrogen separation membranes, we predict the temperature dependent phase diagrams using first principles calculations combined with thermodynamic principles. Our method models the phase diagram without empirical fitting parameters. By applying thermodynamic principles and solid solution models, temperature-dependent features of the Cu-Pd-S system can be explained, specifically solubility ranges for substitutions in select crystalline phases. Electronic densities of states calculations explain the relative favorability of certain chemical substitutions. In addition, we calculate sulfidization thresholds for the Pd-S-2 system and activities for the Cu-Pd binary in temperature regimes where the phase diagram contains multiple solid phases. (C) 2014 Elsevier B.V. All rights reserved. C1 [Huhn, William Paul; Widom, Michael] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [Gao, Michael C.] Natl Energy Technol Lab, Albany, OR 97321 USA. [Gao, Michael C.] URS Corp, Albany, OR 97321 USA. RP Huhn, WP (reprint author), Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. EM wph@andrew.cmu.edu; widom@andrew.cmu.edu RI Widom, Michael/P-2531-2014; OI Widom, Michael/0000-0001-5972-5696; Huhn, William/0000-0002-8815-4594 FU RES [DE-FE0004000] FX We are grateful to B. Gleeson, M. Mihalkovic., and J. Kitchin for useful discussion. This technical effort was performed in support of the Fuels Program of Strategic Center for Coal at DOE National Energy Technology Laboratory under the RES contract DE-FE0004000. NR 43 TC 1 Z9 1 U1 2 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD SEP PY 2014 VL 92 BP 377 EP 386 DI 10.1016/j.commatsci.2014.05.065 PG 10 WC Materials Science, Multidisciplinary SC Materials Science GA AM7LG UT WOS:000340048100049 ER PT J AU Modine, NA Wright, AF Lee, SR AF Modine, N. A. Wright, A. F. Lee, S. R. TI Bounds on the range of density-functional-theory point-defect levels in semiconductors and insulators SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Density functional theory; Defects; Semiconductors ID 1ST-PRINCIPLES CALCULATIONS; ELECTRONIC-STRUCTURE; AB-INITIO; ENERGY; GAAS; DEPENDENCE; STATE; ZNSE; GAS AB Defects in semiconductors and insulators are characterized by their levels, which are defined as the values of the Fermi level at which the charge state of the defect changes. Kohn-Sham density functional theory calculations for charged defects have been widely and successfully used to predict defect levels. Due to their lower computational cost and demonstrated ability to predict levels spanning the measured band gap, semilocal exchange-correlation functionals are widely used in these calculations. However, there is a potential pitfall in using semilocal functionals: although they often predict accurate energies for adding or removing electrons from states that are localized near the defect, the famous band gap error results in overly small energies for adding or removing electrons from extended band edge states. As a result, electrons (or holes) that should occupy localized states may become partially or fully delocalized. In order to help detect and analyze such cases, we introduce bounds on the defect levels that can be obtained using a given functional, supercell, and Brillouin zone sampling. Since these bounds correspond to the charge transition levels of the corresponding defect-free supercell, comparison with the bounds reveals when a calculated level is behaving in a bulk-like rather than defect-like manner. We find that the bounds depend significantly on supercell size due to band-filling effects that arise from the finite charge density created when one electron is added to or removed from a finite-sized supercell, and this size dependence helps explain the success of defect level calculations using semilocal functionals. (C) 2014 Elsevier B.V. All rights reserved. C1 [Modine, N. A.; Wright, A. F.; Lee, S. R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Modine, NA (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM namodin@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 42 TC 8 Z9 8 U1 1 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD SEP PY 2014 VL 92 BP 431 EP 438 DI 10.1016/j.commatsci.2014.05.032 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA AM7LG UT WOS:000340048100055 ER PT J AU Cowart, J Raynes, M Hamilton, L Prak, DL Mehl, M Pitz, W AF Cowart, Jim Raynes, Michael Hamilton, Len Prak, Dianne Luning Mehl, Marco Pitz, William TI An Experimental and Modeling Study Into Using Normal and Isocetane Fuel Blends as a Surrogate for a Hydroprocessed Renewable Diesel Fuel SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID THERMOPHYSICAL PROPERTIES; PHYSICOCHEMICAL AUTHENTICITY; ORGANIC LIQUIDS; SURFACE-TENSION; N-HEXADECANE; KEROSENE; DENSITY; MIXTURE; PREDICTION; BIODIESEL AB A new hydroprocessed renewable diesel (HRD) fuel comprised both straight chain and branched alkane fuel components. In an effort to find a research surrogate for this fuel, single cylinder engine testing was performed with various blends of n-hexadecane (cetane) and isocetane in order to find a binary surrogate mixture with similar performance characteristics to that of the HRD. A blend of approximately two-thirds n-hexadecane with one-third isocetane showed the most similar behavior based on conventional combustion metrics. Companion combustion modeling was then pursued using a combined detailed chemical kinetic mechanism for both n-hexadecane and isocetane. These modeling results show both the importance of isocetane in lengthening ignition delay (IGD), as well as the overall importance of chemical ignition delay as the dominating effect in the overall ignition delay of these binary blend fuels. C1 [Cowart, Jim; Raynes, Michael; Hamilton, Len; Prak, Dianne Luning] US Naval Acad, Annapolis, MD 21402 USA. [Mehl, Marco; Pitz, William] LLNL, Livermore, CA 94550 USA. RP Cowart, J (reprint author), US Naval Acad, Annapolis, MD 21402 USA. RI Mehl, Marco/A-8506-2009 OI Mehl, Marco/0000-0002-2227-5035 FU Office of Naval Research; U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX The authors would like to thank Dr. Sharon Beerman-Curtain and the Office of Naval Research for their support of this work. The LLNL portion of this work was performed under the auspices of the U.S. Department of Energy by LLNL under Contract No. DE-AC52-07NA27344. NR 37 TC 2 Z9 2 U1 0 U2 9 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD SEP PY 2014 VL 136 IS 3 AR 032202 DI 10.1115/1.4027408 PG 9 WC Energy & Fuels SC Energy & Fuels GA AN0RW UT WOS:000340292700008 ER PT J AU Krishnaswamy, R Kaneko, TK Mazumdar, BM Rozelle, P Sridhar, S Kuhlman, JM AF Krishnaswamy, Ramalakshmi Kaneko, Tetsuya Kenneth Mazumdar, Bishal Madhab Rozelle, Peter Sridhar, Seetharaman Kuhlman, John M. TI Infiltration Velocity and Thickness of Flowing Slag Film on Porous Refractory of Slagging Gasifiers SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID OXYGEN PARTIAL-PRESSURE; COAL GASIFIERS; GASIFICATION; VISCOSITY; AL2O3; CHARS; OXIDE AB Two analytical formulations that describe the fluid interactions of slag with the porous refractory linings of gasification reactors have been derived. The first formulation considers the infiltration velocity of molten slag into the porous microstructure of the refractory material that possesses an inherent temperature gradient in the direction of infiltration. Capillary pressures are assumed to be the primary driving force for the infiltration. Considering that the geometry of the pores provides a substantially shorter length scale in the radial direction as compared with the penetration direction, a lubrication approximation was employed to simplify the equation of motion. The assumption of a fully developed flow in the pores is justified based on the extremely small Reynolds numbers of the infiltration slag flow. The second formulation describes the thickness of the slag film that flows down the perimeter of the refractory lining. The thickness of the film was approximated by equating the volumetric slag production rate of the gasification reactor to the integration of the velocity profile with respect to the lateral flow cross-sectional area of the film. These two models demonstrate that both the infiltration velocity into the refractory and the thickness of the film that forms at the refractory surface were sensitive to the viscosity of the fluid slag. The slag thickness model has been applied to predict film thicknesses in a generic slagging gasifier with assumed axial temperature distributions, using slag viscosity from the literature, both for the case of a constant slag volumetric flow rate down the gasifier wall, and for the case of a constant flyash flux distributed uniformly over the entire gasifier wall. C1 [Krishnaswamy, Ramalakshmi; Kuhlman, John M.] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [Kaneko, Tetsuya Kenneth] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. [Mazumdar, Bishal Madhab] Ctr Study Sci Technol & Policy CSTEP, Bangalore 560001, Karnataka, India. [Rozelle, Peter] US DOE, Off Clean Energy Syst, Washington, DC 20585 USA. [Sridhar, Seetharaman] Univ Warwick, Warwick Mfg Grp, Coventry CV4 7AL, W Midlands, England. RP Krishnaswamy, R (reprint author), W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. NR 26 TC 0 Z9 0 U1 2 U2 13 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD SEP PY 2014 VL 136 IS 3 AR 032203 DI 10.1115/1.4026918 PG 9 WC Energy & Fuels SC Energy & Fuels GA AN0RW UT WOS:000340292700009 ER PT J AU Bates, CR Pies, C Kempf, S Gastaldo, L Fleischmann, A Enss, C Friedrich, S AF Bates, C. R. Pies, C. Kempf, S. Gastaldo, L. Fleischmann, A. Enss, C. Friedrich, S. TI Development of MMC Gamma Detectors for Nuclear Analysis SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE MMC; Gamma ray; Low-temperature detectors; Metallic magnetic calorimeters; Nuclear safeguards ID ENERGY RESOLUTION AB Non-destructive assay (NDA) of nuclear materials would benefit from gamma detectors with improved energy resolution in cases where line overlap in current Ge detectors limits NDA accuracy. We are developing metallic magnetic calorimeter gamma-detectors for this purpose by electroplating 150 m thick Au absorbers into microfabricated molds on top of Au:Er sensors. Initial tests under non-optimized conditions show an energy resolution of 200 eV FWHM at 60 keV. Monte Carlo simulations illustrate that this resolution is starting to be sufficient for direct detection of Pu in plutonium separated from spent nuclear fuel. C1 [Bates, C. R.; Friedrich, S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Pies, C.; Kempf, S.; Gastaldo, L.; Fleischmann, A.; Enss, C.] Heidelberg Univ, Kirchhoff Inst Phys, D-69120 Heidelberg, Germany. RP Bates, CR (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave L-188, Livermore, CA 94550 USA. EM bates26@llnl.gov RI Kempf, Sebastian/P-7612-2016 OI Kempf, Sebastian/0000-0002-3303-128X FU US Department of Energy Office on Non-proliferation Research [NA-22, LL12-MagMicro-PD2Ja]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was funded by the US Department of Energy Office on Non-proliferation Research NA-22 under Grant LL12-MagMicro-PD2Ja. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 12 TC 2 Z9 2 U1 0 U2 6 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 631 EP 636 DI 10.1007/s10909-013-1063-7 PG 6 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400003 ER PT J AU Suzuki, A Arnold, K Edwards, J Engargiola, G Holzapfel, W Keating, B Lee, AT Meng, XF Myers, MJ O'Brient, R Quealy, E Rebeiz, G Richards, PL Rosen, D Siritanasak, P AF Suzuki, A. Arnold, K. Edwards, J. Engargiola, G. Holzapfel, W. Keating, B. Lee, A. T. Meng, X. F. Myers, M. J. O'Brient, R. Quealy, E. Rebeiz, G. Richards, P. L. Rosen, D. Siritanasak, P. TI Multi-Chroic Dual-Polarization Bolometric Detectors for Studies of the Cosmic Microwave Background SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Cosmic Microwave Background; B-mode; Broadband; Multichroic; Polarization; Anti-Reflectoin Coating ID ANTENNAS; LENSES AB We are developing multi-chroic antenna-coupled Transition Edge Sensor (TES) bolometer detectors for Cosmic Microwave Background (CMB) polarimetry. Multi-chroic detectors increase focal plane area efficiency, and thus the mapping speed per focal plane area, and provide greater discrimination against polarized galactic foregrounds with no increase in weight or cryogenic cost. In each pixel, a silicon lens-coupled dual-polarized sinuous antenna collects photons over a two-octave frequency band. The antenna couples the broadband millimeter wave signal into microstrip transmission lines, and on-chip filter banks split the broadband signal into multiple frequency bands. Separate TES bolometers detect the power in each frequency band and linear polarization state. We will describe the design and performance of these devices and present optical data taken. Our measurements of dual-polarization pixels in multiple frequency bands show beams with percent-level ellipticity, and percent-level cross-polarization leakage. We will also describe the development of large arrays of these multi-chroic pixels. Finally, we will describe kilo-pixel arrays of these detectors planned for the future CMB experiments that will achieve unprecedented mapping speed. C1 [Suzuki, A.; Holzapfel, W.; Lee, A. T.; Myers, M. J.; Quealy, E.; Richards, P. L.; Rosen, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Arnold, K.; Keating, B.; Siritanasak, P.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92092 USA. [Edwards, J.; Rebeiz, G.] Univ Calif San Diego, Dept Elect & Comp Engn, La Jolla, CA 92092 USA. [Engargiola, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Meng, X. F.] Univ Calif Berkeley, Dept Elect Engn, Berkeley, CA 94720 USA. [O'Brient, R.] CALTECH, Dept Phys, Pasadena, CA 91125 USA. RP Suzuki, A (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM asuzuki@berkeley.edu RI Holzapfel, William/I-4836-2015 FU NASA; NASA [NNG06GJ08G]; Royal Thai Government FX We acknowledge support from the NASA, NASA grant NNG06GJ08G. Detectors were fabricated at Berkeley nanofabrication laboratory. Praween Siritanasak is supported by the Royal Thai Government fellowship. NR 9 TC 9 Z9 9 U1 0 U2 1 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 650 EP 656 DI 10.1007/s10909-013-1049-5 PG 7 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400006 ER PT J AU Suzuki, A Ade, P Akiba, Y Aleman, C Arnold, K Atlas, M Barron, D Borrill, J Chapman, S Chinone, Y Cukierman, A Dobbs, M Elleflot, T Errard, J Fabbian, G Feng, G Gilbert, A Grainger, W Halverson, N Hasegawa, M Hattori, K Hazumi, M Holzapfel, W Hori, Y Inoue, Y Jaehnig, G Katayama, N Keating, B Kermish, Z Keskitalo, R Kisner, T Lee, A Matsuda, F Matsumura, T Morii, H Moyerman, S Myers, M Navaroli, M Nishino, H Okamura, T Reichart, C Richards, P Ross, C Rotermund, K Sholl, M Siritanasak, P Smecher, G Stebor, N Stompor, R Suzuki, J Takada, S Takakura, S Tomaru, T Wilson, B Yamaguchi, H Zahn, O AF Suzuki, A. Ade, P. Akiba, Y. Aleman, C. Arnold, K. Atlas, M. Barron, D. Borrill, J. Chapman, S. Chinone, Y. Cukierman, A. Dobbs, M. Elleflot, T. Errard, J. Fabbian, G. Feng, G. Gilbert, A. Grainger, W. Halverson, N. Hasegawa, M. Hattori, K. Hazumi, M. Holzapfel, W. Hori, Y. Inoue, Y. Jaehnig, G. Katayama, N. Keating, B. Kermish, Z. Keskitalo, R. Kisner, T. Lee, A. Matsuda, F. Matsumura, T. Morii, H. Moyerman, S. Myers, M. Navaroli, M. Nishino, H. Okamura, T. Reichart, C. Richards, P. Ross, C. Rotermund, K. Sholl, M. Siritanasak, P. Smecher, G. Stebor, N. Stompor, R. Suzuki, J. Takada, S. Takakura, S. Tomaru, T. Wilson, B. Yamaguchi, H. Zahn, O. TI The POLARBEAR-2 Experiment SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Cosmic microwave background; Inflation; Lensing; Polarization; B-mode ID POLARIZATION AB We present an overview of the design and development of the POLARBEAR-2 experiment. The POLARBEAR-2 experiment is a cosmic microwave background polarimetry experiment, which aims to characterize the small angular scale B-mode signal due to gravitational lensing and search for the large angular scale B-mode signal from inflationary gravitational waves. The experiment will have a 365 mm diameter multi-chroic focal plane filled with 7,588 polarization sensitive antenna-coupled Transition Edge Sensor bolometers and will observe at 95 and 150 GHz. The focal plane is cooled to 250 mK. The bolometers will be read-out by SQUIDs with frequency domain multiplexing. The experiment will utilize high purity alumina lenses and thermal filters to achieve the required high optical throughput. A continuously rotating, cooled half-wave plate will be used to give stringent control over systematic errors. The experiment is designed to achieve a noise equivalent temperature of 5.7 K, and this allows us to constrain the signal from the inflationary primordial gravitational corresponding to a tensor-to-scalar ratio of (). POLARBEAR-2 will also be able to put a constraint on the sum of neutrino masses to 90 meV () with POLARBEAR-2 data alone and 65 meV () when combined with the Planck satellite. We plan to start observations in 2014 in the Atacama Desert in Chile. C1 [Suzuki, A.; Cukierman, A.; Holzapfel, W.; Lee, A.; Myers, M.; Reichart, C.; Richards, P.; Zahn, O.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ade, P.; Grainger, W.] Cardiff Univ, Sch Phys & Astron, Cardiff CF10 3AX, S Glam, Wales. [Akiba, Y.; Chinone, Y.; Hasegawa, M.; Hattori, K.; Hazumi, M.; Hori, Y.; Inoue, Y.; Matsumura, T.; Morii, H.; Okamura, T.; Suzuki, J.; Tomaru, T.; Yamaguchi, H.] High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Aleman, C.; Arnold, K.; Atlas, M.; Barron, D.; Elleflot, T.; Feng, G.; Keating, B.; Matsuda, F.; Moyerman, S.; Navaroli, M.; Siritanasak, P.; Stebor, N.; Stompor, R.; Wilson, B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Borrill, J.; Errard, J.; Keskitalo, R.; Kisner, T.; Sholl, M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Chapman, S.; Ross, C.; Rotermund, K.] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS, Canada. [Dobbs, M.; Gilbert, A.; Smecher, G.] McGill Univ, Montreal, PQ, Canada. [Fabbian, G.] Lab Astroparticule & Cosmol, Paris, France. [Halverson, N.; Jaehnig, G.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Katayama, N.; Nishino, H.] Kavli Inst Phys & Math Universe, Kashiwa, Chiba, Japan. [Kermish, Z.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Takada, S.] Natl Inst Nat Sci, Natl Inst Fus Sci, Toki, Gifu 5095292, Japan. [Takakura, S.] Osaka Univ, Dept Phys, Osaka, Japan. RP Suzuki, A (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM asuzuki@berkeley.edu RI Holzapfel, William/I-4836-2015; OI Fabbian, Giulio/0000-0002-3255-4695; Chinone, Yuji/0000-0002-3266-857X FU MEXT Kahenhi grant [21111002]; NSF [AST-0618398]; NASA [NNG06GJ08G]; Simons Foundation; Natural Sciences and Engineering Research Council; Canadian Institute for Advanced Research; CONICYT FX We acknowledge support from the MEXT Kahenhi grant 21111002, NSF grant AST-0618398, NASA grant NNG06GJ08G, The Simons Foundation, Natural Sciences and Engineering Research Council, Canadian Institute for Advanced Research and the CONICYT. Detectors were fabricated at Berkeley nanofabrication laboratory. NR 16 TC 6 Z9 6 U1 6 U2 11 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 719 EP 725 DI 10.1007/s10909-014-1112-x PG 7 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400016 ER PT J AU Barron, D Ade, P Anthony, A Arnold, K Boettger, D Borrill, J Chapman, S Chinone, Y Dobbs, M Edwards, J Errard, J Fabbian, G Flanigan, D Fuller, G Ghribi, A Grainger, W Halverson, N Hasegawa, M Hattori, K Hazumi, M Holzapfel, W Howard, J Hyland, P Jaehnig, G Jaffe, A Keating, B Kermish, Z Keskitalo, R Kisner, T Lee, AT Le Jeune, M Linder, E Lungu, M Matsuda, F Matsumura, T Meng, X Miller, NJ Morii, H Moyerman, S Myers, M Nishino, H Paar, H Peloton, J Quealy, E Rebeiz, G Reichardt, CL Richards, PL Ross, C Shimizu, A Shimmin, C Shimon, M Sholl, M Siritanasak, P Spieler, H Stebor, N Steinbach, B Stompor, R Suzuki, A Tomaru, T Tucker, C Yadav, A Zahn, O AF Barron, D. Ade, P. Anthony, A. Arnold, K. Boettger, D. Borrill, J. Chapman, S. Chinone, Y. Dobbs, M. Edwards, J. Errard, J. Fabbian, G. Flanigan, D. Fuller, G. Ghribi, A. Grainger, W. Halverson, N. Hasegawa, M. Hattori, K. Hazumi, M. Holzapfel, W. Howard, J. Hyland, P. Jaehnig, G. Jaffe, A. Keating, B. Kermish, Z. Keskitalo, R. Kisner, T. Lee, A. T. Le Jeune, M. Linder, E. Lungu, M. Matsuda, F. Matsumura, T. Meng, X. Miller, N. J. Morii, H. Moyerman, S. Myers, M. Nishino, H. Paar, H. Peloton, J. Quealy, E. Rebeiz, G. Reichardt, C. L. Richards, P. L. Ross, C. Shimizu, A. Shimmin, C. Shimon, M. Sholl, M. Siritanasak, P. Spieler, H. Stebor, N. Steinbach, B. Stompor, R. Suzuki, A. Tomaru, T. Tucker, C. Yadav, A. Zahn, O. TI The POLARBEAR Cosmic Microwave Background Polarization Experiment SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Cosmic microwave background; CMB polarization; Millimeter-wave AB The polarbear cosmic microwave background (CMB) polarization experiment has been observing since early 2012 from its 5,200 m site in the Atacama Desert in Northern Chile. polarbear's measurements will characterize the expected CMB polarization due to gravitational lensing by large scale structure, and search for the possible B-mode polarization signature of inflationary gravitational waves. polarbear's 250 mK focal plane detector array consists of 1,274 polarization-sensitive antenna-coupled bolometers, each with an associated lithographed band-defining filter and contacting dielectric lenslet, an architecture unique in current CMB experiments. The status of the polarbear instrument, its focal plane, and the analysis of its measurements are presented. C1 [Barron, D.; Arnold, K.; Boettger, D.; Edwards, J.; Fuller, G.; Keating, B.; Matsuda, F.; Meng, X.; Moyerman, S.; Paar, H.; Rebeiz, G.; Siritanasak, P.; Stebor, N.; Yadav, A.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Ade, P.; Tucker, C.] Cardiff Univ, Sch Phys & Astron, Cardiff CF10 3AX, S Glam, Wales. [Anthony, A.; Halverson, N.; Jaehnig, G.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80309 USA. [Borrill, J.; Errard, J.; Keskitalo, R.; Kisner, T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Borrill, J.; Richards, P. L.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Chapman, S.; Ross, C.] Dalhousie Univ, Dept Phys, Halifax, NS B3H 3J5, Canada. [Chinone, Y.; Hasegawa, M.; Hattori, K.; Hazumi, M.; Matsumura, T.; Morii, H.; Shimizu, A.; Tomaru, T.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki, Japan. [Dobbs, M.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Fabbian, G.; Le Jeune, M.; Peloton, J.; Stompor, R.] Univ Paris 07, Lab Astroparticule & Cosmol APC, Paris, France. [Flanigan, D.; Ghribi, A.; Holzapfel, W.; Howard, J.; Lee, A. T.; Lungu, M.; Myers, M.; Quealy, E.; Reichardt, C. L.; Richards, P. L.; Shimmin, C.; Steinbach, B.; Suzuki, A.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Grainger, W.] STFC, Rutherford Appleton Lab, Didcot, Oxon, England. [Hyland, P.] Austin Coll, Dept Phys, Sherman, TX 75090 USA. [Jaffe, A.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London, England. [Kermish, Z.] Princeton Univ, Princeton, NJ 08544 USA. [Linder, E.; Sholl, M.; Spieler, H.; Zahn, O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Miller, N. J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Nishino, H.] Univ Tokyo, Kavli Inst Phys & Math Universe, Kashiwa, Chiba, Japan. [Shimon, M.] Tel Aviv Univ, IL-69978 Tel Aviv, Israel. [Zahn, O.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys BCCP, Berkeley, CA 94720 USA. RP Barron, D (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM dbarron@physics.ucsd.edu RI Holzapfel, William/I-4836-2015; OI Fabbian, Giulio/0000-0002-3255-4695; Reichardt, Christian/0000-0003-2226-9169; Tucker, Carole/0000-0002-1851-3918; Chinone, Yuji/0000-0002-3266-857X FU National Science Foundation [AST-0618398]; NASA [NNG06GJ08G]; Natural Sciences and Engineering Research Council; Canadian Institute for Advanced Research; MEXT KAKENHI [21111002]; Simons Foundation FX POLARBEAR is funded by the National Science Foundation under Grant AST-0618398. Antenna-coupled bolometer development at Berkeley is funded by NASA under Grant NNG06GJ08G. The McGill authors acknowledge funding from the Natural Sciences and Engineering Research Council and Canadian Institute for Advanced Research. The KEK authors are supported by MEXT KAKENHI Grant Number 21111002. The Chilean site is located in the Parque Astronomico Atacama in agreement with the Comision Nacional de Investigacion Cientifica y Tecnologica de Chile. The Simons Array is funded by the Simons Foundation. NR 14 TC 0 Z9 0 U1 3 U2 5 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 726 EP 732 DI 10.1007/s10909-013-1065-5 PG 7 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400017 ER PT J AU Matsumura, T Akiba, Y Borrill, J Chinone, Y Dobbs, M Fuke, H Ghribi, A Hasegawa, M Hattori, K Hattori, M Hazumi, M Holzapfel, W Inoue, Y Ishidoshiro, K Ishino, H Ishitsuka, H Karatsu, K Katayama, N Kawano, I Kibayashi, A Kibe, Y Kimura, K Kimura, N Koga, K Kozu, M Komatsu, E Lee, A Matsuhara, H Mima, S Mitsuda, K Mizukami, K Morii, H Morishima, T Murayama, S Nagai, M Nagata, R Nakamura, S Naruse, M Natsume, K Nishibori, T Nishino, H Noda, A Noguchi, T Ogawa, H Oguri, S Ohta, I Otani, C Richards, P Sakai, S Sato, N Sato, Y Sekimoto, Y Shimizu, A Shinozaki, K Sugita, H Suzuki, T Suzuki, A Tajima, O Takada, S Takakura, S Takei, Y Tomaru, T Uzawa, Y Wada, T Watanabe, H Yoshida, M Yamasaki, N Yoshida, T Yotsumoto, K AF Matsumura, T. Akiba, Y. Borrill, J. Chinone, Y. Dobbs, M. Fuke, H. Ghribi, A. Hasegawa, M. Hattori, K. Hattori, M. Hazumi, M. Holzapfel, W. Inoue, Y. Ishidoshiro, K. Ishino, H. Ishitsuka, H. Karatsu, K. Katayama, N. Kawano, I. Kibayashi, A. Kibe, Y. Kimura, K. Kimura, N. Koga, K. Kozu, M. Komatsu, E. Lee, A. Matsuhara, H. Mima, S. Mitsuda, K. Mizukami, K. Morii, H. Morishima, T. Murayama, S. Nagai, M. Nagata, R. Nakamura, S. Naruse, M. Natsume, K. Nishibori, T. Nishino, H. Noda, A. Noguchi, T. Ogawa, H. Oguri, S. Ohta, I. Otani, C. Richards, P. Sakai, S. Sato, N. Sato, Y. Sekimoto, Y. Shimizu, A. Shinozaki, K. Sugita, H. Suzuki, T. Suzuki, A. Tajima, O. Takada, S. Takakura, S. Takei, Y. Tomaru, T. Uzawa, Y. Wada, T. Watanabe, H. Yoshida, M. Yamasaki, N. Yoshida, T. Yotsumoto, K. TI Mission Design of LiteBIRD SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Cosmic microwave background radiation; B-mode polarization; Inflation; Transition edge sensor bolometer for space application AB LiteBIRD is a next-generation satellite mission to measure the polarization of the cosmic microwave background (CMB) radiation. On large angular scales the B-mode polarization of the CMB carries the imprint of primordial gravitational waves, and its precise measurement would provide a powerful probe of the epoch of inflation. The goal of LiteBIRD is to achieve a measurement of the characterizing tensor to scalar ratio to an uncertainty of . In order to achieve this goal we will employ a kilo-pixel superconducting detector array on a cryogenically cooled sub-Kelvin focal plane with an optical system at a temperature of 4 K. We are currently considering two detector array options; transition edge sensor (TES) bolometers and microwave kinetic inductance detectors. In this paper we give an overview of LiteBIRD and describe a TES-based polarimeter designed to achieve the target sensitivity of 2 K arcmin over the frequency range 50-320 GHz. C1 [Matsumura, T.; Chinone, Y.; Hasegawa, M.; Hattori, K.; Hazumi, M.; Kimura, K.; Kimura, N.; Morii, H.; Nagata, R.; Oguri, S.; Sato, N.; Suzuki, T.; Tajima, O.; Tomaru, T.; Yoshida, M.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki, Japan. [Akiba, Y.; Inoue, Y.; Ishitsuka, H.; Shimizu, A.; Watanabe, H.] Grad Univ Adv Studies SOKENDAI, Hayama, Kanagawa, Japan. [Borrill, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Dobbs, M.] McGill Univ, Montreal, PQ, Canada. [Fuke, H.; Kawano, I.; Matsuhara, H.; Mitsuda, K.; Nishibori, T.; Noda, A.; Sakai, S.; Sato, Y.; Shinozaki, K.; Sugita, H.; Takei, Y.; Wada, T.; Yamasaki, N.; Yoshida, T.; Yotsumoto, K.] Japan Aerosp Explorat Agcy JAXA, Sagamihara, Kanagawa, Japan. [Ghribi, A.; Holzapfel, W.; Lee, A.; Richards, P.; Suzuki, A.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Hattori, M.; Ishidoshiro, K.; Morishima, T.] Tohoku Univ, Sendai, Miyagi 980, Japan. [Ishino, H.; Kibayashi, A.; Kibe, Y.] Okayama Univ, Okayama, Japan. [Karatsu, K.; Noguchi, T.; Sekimoto, Y.; Uzawa, Y.] Natl Astron Observ Japan NAOJ, Mitaka, Tokyo, Japan. [Katayama, N.; Nishino, H.] Univ Tokyo, Kavli Inst Phys & Math Universe IPMU, Kashiwa, Chiba, Japan. [Koga, K.; Mima, S.; Otani, C.] RIKEN, Terahertz Wave Res Grp, Sendai, Miyagi, Japan. [Komatsu, E.] Max Planck Inst Astrophys, D-85741 Garching, Germany. [Mizukami, K.; Murayama, S.; Nakamura, S.; Natsume, K.] Yokohama Natl Univ, Yokohama, Kanagawa 240, Japan. [Nagai, M.; Takada, S.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Naruse, M.] Saitama Univ, Saitama 3388570, Japan. [Kozu, M.; Ogawa, H.] Osaka Prefecture Univ, Osaka, Japan. [Ohta, I.] Kinki Univ, Higashiosaka, Osaka 577, Japan. [Takakura, S.] Osaka Univ, Osaka, Japan. RP Matsumura, T (reprint author), High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki, Japan. EM tomotake.matsumura@kek.jp RI Mitsuda, Kazuhisa/C-2649-2008; Yamasaki, Noriko/C-2252-2008; NAKAMURA, Shogo/M-5177-2014; Ishino, Hirokazu/C-1994-2015; Holzapfel, William/I-4836-2015; Otani, Chiko/A-6510-2016; Kibayashi, Atsuko/K-7327-2015; NAKAMURA, Shogo/L-3303-2016; OI NAKAMURA, Shogo/0000-0003-2921-7046; Ishino, Hirokazu/0000-0002-8623-4080; NAKAMURA, Shogo/0000-0003-2921-7046; Chinone, Yuji/0000-0002-3266-857X FU Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan under KAKENHI [21111002, 21111003, 24111715, 24740182] FX This work is supported by the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan under KAKENHI Grant Numbers 21111002, 21111003, 24111715, 24740182. NR 18 TC 53 Z9 53 U1 0 U2 6 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 733 EP 740 DI 10.1007/s10909-013-0996-1 PG 8 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400018 ER PT J AU Canonica, L Biassoni, M Brofferio, C Bucci, C Calvano, S Di Vacri, ML Goett, J Gorla, P Pavan, M Yeh, M AF Canonica, L. Biassoni, M. Brofferio, C. Bucci, C. Calvano, S. Di Vacri, M. L. Goett, J. Gorla, P. Pavan, M. Yeh, M. TI Rejection of Surface Background in Thermal Detectors SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Thermal detectors; Rare events searches; Scintillation; Surface background ID ELECTRODES; SEARCH AB A challenging aspect of the next generation detector for rare events searches (i.e. neutrinoless double beta decay and dark matter searches) is the reduction of the background in the region of interest that can mimic the expected signals. In the field of thermal detectors, which have a leading role in rare events searches thanks to their excellent energy resolution and to the wide choice of absorber materials, the background coming from surface contaminations is frequently dominant. A background surface rejection detector is a scintillation-based approach for tagging this type of background. We discuss the innovative application of this technique in non-scintillating thermal detectors. We will report on the performances of the prototype bolometric detector, realized to prove the feasibility of this new technique. C1 [Canonica, L.; Bucci, C.; Calvano, S.; Di Vacri, M. L.; Gorla, P.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. [Biassoni, M.; Brofferio, C.; Pavan, M.] Univ Milano Bicocca, Milan, Italy. [Biassoni, M.; Brofferio, C.; Pavan, M.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Goett, J.] Los Alamos Natl Lab, Los Alamos, NM USA. [Yeh, M.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Canonica, L (reprint author), Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. EM lucia.canonica@lngs.infn.it OI Canonica, Lucia/0000-0001-8734-206X; Goett, Johnny/0000-0002-3685-2227; pavan, maura/0000-0002-9723-7834 FU 5th Commission of the Istituto Nazionale di Fisica Nucleare (INFN) FX We would like to thank M. Pedretti and W. Seidel for useful discussions and S. Pirro and L. Cardani for constructive help in various stages of this experiment. This work was supported by the 5th Commission of the Istituto Nazionale di Fisica Nucleare (INFN). NR 19 TC 0 Z9 0 U1 0 U2 3 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 898 EP 904 DI 10.1007/s10909-014-1152-2 PG 7 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400040 ER PT J AU Canonica, L Artusa, DR Avignone, FT Azzolini, O Balata, M Banks, TI Bari, G Beeman, J Bellini, F Bersani, A Biassoni, M Bloxham, T Brofferio, C Bucci, C Cai, XZ Camacho, A Cao, X Capelli, S Carbone, L Cardani, L Carrettoni, M Casali, N Chiesa, D Chott, N Clemenza, M Cosmelli, C Cremonesi, O Creswick, RJ Dafinei, I Dally, A Datskov, V De Biasi, A Deninno, MM Di Domizio, S di Vacri, ML Ejzak, L Faccini, R Fang, DQ Farach, HA Faverzani, M Fernandes, G Ferri, E Ferroni, F Fiorini, E Franceschi, MA Freedman, SJ Fujikawa, BK Giachero, A Gironi, L Giuliani, A Goett, J Gorla, P Gotti, C Gutierrez, TD Haller, EE Han, K Heeger, KM Huang, HZ Kadel, R Kazkaz, K Keppel, G Kogler, L Kolomensky, YG Lenz, D Li, YL Ligi, C Liu, X Ma, YG Maiano, C Maino, M Martinez, M Maruyama, RH Mei, Y Moggi, N Morganti, S Napolitano, T Newman, S Nisi, S Nones, C Norman, EB Nucciotti, A O'Donnell, T Orio, F Orlandi, D Ouellet, JL Pallavicini, M Palmieri, V Pattavina, L Pavan, M Pedretti, M Pessina, G Piperno, G Pira, C Pirro, S Previtali, E Rampazzo, V Rimondi, F Rosenfeld, C Rusconi, C Sala, E Sangiorgio, S Scielzo, ND Sisti, M Smith, AR Taffarello, L Tenconi, M Terranova, F Tian, WD Tomei, C Trentalange, S Ventura, G Vignati, M Wang, BS Wang, HW Wielgus, L Wilson, J Wise, T Woodcraft, A Zanotti, L Zarra, C Zhu, BX Zucchelli, S AF Canonica, L. Artusa, D. R. Avignone, F. T., III Azzolini, O. Balata, M. Banks, T. I. Bari, G. Beeman, J. Bellini, F. Bersani, A. Biassoni, M. Bloxham, T. Brofferio, C. Bucci, C. Cai, X. Z. Camacho, A. Cao, X. Capelli, S. Carbone, L. Cardani, L. Carrettoni, M. Casali, N. Chiesa, D. Chott, N. Clemenza, M. Cosmelli, C. Cremonesi, O. Creswick, R. J. Dafinei, I. Dally, A. Datskov, V. De Biasi, A. Deninno, M. M. Di Domizio, S. di Vacri, M. L. Ejzak, L. Faccini, R. Fang, D. Q. Farach, H. A. Faverzani, M. Fernandes, G. Ferri, E. Ferroni, F. Fiorini, E. Franceschi, M. A. Freedman, S. J. Fujikawa, B. K. Giachero, A. Gironi, L. Giuliani, A. Goett, J. Gorla, P. Gotti, C. Gutierrez, T. D. Haller, E. E. Han, K. Heeger, K. M. Huang, H. Z. Kadel, R. Kazkaz, K. Keppel, G. Kogler, L. Kolomensky, Yu G. Lenz, D. Li, Y. L. Ligi, C. Liu, X. Ma, Y. G. Maiano, C. Maino, M. Martinez, M. Maruyama, R. H. Mei, Y. Moggi, N. Morganti, S. Napolitano, T. Newman, S. Nisi, S. Nones, C. Norman, E. B. Nucciotti, A. O'Donnell, T. Orio, F. Orlandi, D. Ouellet, J. L. Pallavicini, M. Palmieri, V. Pattavina, L. Pavan, M. Pedretti, M. Pessina, G. Piperno, G. Pira, C. Pirro, S. Previtali, E. Rampazzo, V. Rimondi, F. Rosenfeld, C. Rusconi, C. Sala, E. Sangiorgio, S. Scielzo, N. D. Sisti, M. Smith, A. R. Taffarello, L. Tenconi, M. Terranova, F. Tian, W. D. Tomei, C. Trentalange, S. Ventura, G. Vignati, M. Wang, B. S. Wang, H. W. Wielgus, L. Wilson, J. Wise, T. Woodcraft, A. Zanotti, L. Zarra, C. Zhu, B. X. Zucchelli, S. TI First CUORE-0 Performance Results and Status of CUORE Experiment SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Neutrinoless double beta decay; Neutrino mass; Majorana particle; Bolometer ID CONTAMINATION; VALIDATION AB The CUORE (Cryogenic Underground Observatory for Rare Events) experiment will search for neutrinoless double beta decay in Te. Observation of the process would unambiguously establish that neutrinos are Majorana particles as well as provide information about the absolute neutrino mass scale and mass hierarchy.The CUORE setup will consist of an array of 988 tellurium dioxide crystals (containing 206 kg of Te in total), operated as bolometers at a temperature of 10 mK. The experiment is now under construction at the Gran Sasso National Laboratory in Italy. As a first step towards CUORE, a tower (CUORE-0) has been assembled and is taking data. Here a detailed description of the CUORE-0 tower and its performance is reported. The status of the CUORE experiment and its expected sensitivity will then be discussed. C1 [Canonica, L.; Artusa, D. R.; Balata, M.; Banks, T. I.; Bucci, C.; Casali, N.; di Vacri, M. L.; Goett, J.; Gorla, P.; Newman, S.; Nisi, S.; Orlandi, D.; Pattavina, L.; Zarra, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. [Artusa, D. R.; Avignone, F. T., III; Chott, N.; Creswick, R. J.; Farach, H. A.; Newman, S.; Rosenfeld, C.; Wilson, J.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Azzolini, O.; Camacho, A.; De Biasi, A.; Keppel, G.; Palmieri, V.; Pira, C.; Rampazzo, V.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Banks, T. I.; Freedman, S. J.; Kogler, L.; Kolomensky, Yu G.; O'Donnell, T.; Ouellet, J. L.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Banks, T. I.; Bloxham, T.; Freedman, S. J.; Fujikawa, B. K.; Han, K.; Kogler, L.; Mei, Y.; Ouellet, J. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bari, G.; Deninno, M. M.; Moggi, N.; Rimondi, F.; Zucchelli, S.] Ist Nazl Fis Nucl, Sez Bologna, I-40127 Bologna, Italy. [Beeman, J.; Haller, E. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bellini, F.; Cardani, L.; Cosmelli, C.; Faccini, R.; Ferroni, F.; Piperno, G.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Bellini, F.; Cardani, L.; Cosmelli, C.; Dafinei, I.; Faccini, R.; Ferroni, F.; Morganti, S.; Orio, F.; Piperno, G.; Tomei, C.; Vignati, M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Bersani, A.; Di Domizio, S.; Fernandes, G.; Pallavicini, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carrettoni, M.; Chiesa, D.; Clemenza, M.; Faverzani, M.; Ferri, E.; Fiorini, E.; Giachero, A.; Gironi, L.; Gotti, C.; Maiano, C.; Maino, M.; Nucciotti, A.; Pavan, M.; Sala, E.; Sisti, M.; Zanotti, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carbone, L.; Carrettoni, M.; Chiesa, D.; Clemenza, M.; Cremonesi, O.; Datskov, V.; Faverzani, M.; Ferri, E.; Fiorini, E.; Giachero, A.; Gironi, L.; Gotti, C.; Maiano, C.; Maino, M.; Nucciotti, A.; Pavan, M.; Pessina, G.; Pirro, S.; Previtali, E.; Rusconi, C.; Sala, E.; Sisti, M.; Terranova, F.; Zanotti, L.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy. [Cai, X. Z.; Cao, X.; Fang, D. Q.; Li, Y. L.; Ma, Y. G.; Tian, W. D.; Wang, H. W.] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Dally, A.; Ejzak, L.; Heeger, K. M.; Lenz, D.; Maruyama, R. H.; Wielgus, L.; Wise, T.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Di Domizio, S.; Fernandes, G.; Pallavicini, M.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Franceschi, M. A.; Ligi, C.; Napolitano, T.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Rome, Italy. [Giuliani, A.; Tenconi, M.] Ctr Spectrometrie Nucl & Spectrometrie Masse, F-91405 Orsay, France. [Gutierrez, T. D.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 93407 USA. [Haller, E. E.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Huang, H. Z.; Liu, X.; Trentalange, S.; Zhu, B. X.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Kadel, R.; Kolomensky, Yu G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley, CA 94720 USA. [Kazkaz, K.; Norman, E. B.; Pedretti, M.; Sangiorgio, S.; Scielzo, N. D.; Wang, B. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Martinez, M.] Univ Zaragoza, Lab Fis Nucl & Astroparticulas, E-50009 Zaragoza, Spain. [Nones, C.] CEA Saclay, Serv Phys Particules, F-91191 Gif Sur Yvette, France. [Norman, E. B.; Wang, B. S.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Rimondi, F.; Zucchelli, S.] Univ Bologna, Dipartimento Fis, I-40127 Bologna, Italy. [Smith, A. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, EH&S Div, Berkeley, CA 94720 USA. [Taffarello, L.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Ventura, G.] Univ Florence, Dipartimento Fis, I-50125 Florence, Italy. [Ventura, G.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Woodcraft, A.] Univ Edinburgh, Inst Astron, SUPA, Edinburgh EH9 3HJ, Midlothian, Scotland. RP Canonica, L (reprint author), Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. EM lucia.canonica@lngs.infn.it RI Bellini, Fabio/D-1055-2009; Kolomensky, Yury/I-3510-2015; Pattavina, Luca/I-7498-2015; Pallavicini, Marco/G-5500-2012; Sisti, Monica/B-7550-2013; Giachero, Andrea/I-1081-2013; Nucciotti, Angelo/I-8888-2012; Chiesa, Davide/H-7240-2014; Vignati, Marco/H-1684-2013; Martinez, Maria/K-4827-2012; Di Domizio, Sergio/L-6378-2014; Ferri, Elena/L-8531-2014; Faverzani, Marco/K-3865-2016; Ligi, Carlo/M-4007-2016; Gironi, Luca/P-2860-2016; capelli, silvia/G-5168-2012; Ma, Yu-Gang/M-8122-2013; Casali, Nicola/C-9475-2017; Sangiorgio, Samuele/F-4389-2014; OI Bellini, Fabio/0000-0002-2936-660X; Kolomensky, Yury/0000-0001-8496-9975; Pattavina, Luca/0000-0003-4192-849X; Pallavicini, Marco/0000-0001-7309-3023; Sisti, Monica/0000-0003-2517-1909; Giachero, Andrea/0000-0003-0493-695X; Nucciotti, Angelo/0000-0002-8458-1556; Chiesa, Davide/0000-0003-1978-1727; Vignati, Marco/0000-0002-8945-1128; Martinez, Maria/0000-0002-9043-4691; Di Domizio, Sergio/0000-0003-2863-5895; Ferri, Elena/0000-0003-1425-3669; Faverzani, Marco/0000-0001-8119-2953; Goett, Johnny/0000-0002-3685-2227; Faccini, Riccardo/0000-0003-2613-5141; Bersani, Andrea/0000-0003-3276-5713; azzolini, oscar/0000-0003-3951-0537; Keppel, Giorgio/0000-0003-4579-3342; Clemenza, Massimiliano/0000-0002-8064-8936; pavan, maura/0000-0002-9723-7834; Gotti, Claudio/0000-0003-2501-9608; Pessina, Gianluigi Ezio/0000-0003-3700-9757; Ligi, Carlo/0000-0001-7943-7704; Gironi, Luca/0000-0003-2019-0967; capelli, silvia/0000-0002-0300-2752; Ma, Yu-Gang/0000-0002-0233-9900; Casali, Nicola/0000-0003-3669-8247; Sangiorgio, Samuele/0000-0002-4792-7802; Camacho, Andrea/0000-0002-1916-0130; Pira, Cristian/0000-0002-5893-1567; Gutierrez, Thomas/0000-0002-0330-6414; Canonica, Lucia/0000-0001-8734-206X FU Istituto Nazionale di Fisica Nucleare (INFN); Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231, DE-AC52-07NA27344]; DOE Office of Nuclear Physics [DE-FG02-08ER41551, DEFG03-00ER41138]; National Science Foundation [NSF-PHY-0605119, NSF-PHY-0500337, NSF-PHY-0855314, NSF-PHY-0902171]; Alfred P. Sloan Foundation; University of Wisconsin Foundation FX The CUORE Collaboration thanks the Directors and Staff of the Laboratori Nazionali del Gran Sasso and the technical staff of our Laboratories. This work was supported by the Istituto Nazionale di Fisica Nucleare (INFN); the Director, Office of Science, of the U.S. Department of Energy under Contract Nos. DE-AC02-05CH11231 and DE-AC52-07NA27344; the DOE Office of Nuclear Physics under Contract Nos. DE-FG02-08ER41551 and DEFG03-00ER41138; the National Science Foundation under Grant Nos. NSF-PHY-0605119, NSF-PHY-0500337, NSF-PHY-0855314, and NSF-PHY-0902171; the Alfred P. Sloan Foundation; and the University of Wisconsin Foundation. NR 9 TC 2 Z9 2 U1 1 U2 19 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 986 EP 994 DI 10.1007/s10909-014-1094-8 PG 9 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400053 ER PT J AU Croce, MP Bond, EM Hoover, AS Kunde, GJ Moody, WA Rabin, MW Bennett, DA Hayes-Wehle, J Kotsubo, V Schmidt, DR Ullom, JN AF Croce, M. P. Bond, E. M. Hoover, A. S. Kunde, G. J. Moody, W. A. Rabin, M. W. Bennett, D. A. Hayes-Wehle, J. Kotsubo, V. Schmidt, D. R. Ullom, J. N. TI Integration of Radioactive Material with Microcalorimeter Detectors SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Transition-edge sensor microcalorimeter; Nuclear forensics; Neutrino mass AB Microcalorimeter detectors with embedded radioactive material offer many possibilities for new types of measurements and applications. We will discuss the designs and methods that we are developing for precise deposition of radioactive material and its encapsulation in the absorber of transition-edge sensor (TES) microcalorimeter detectors for two specific applications. The first application is total nuclear reaction energy (Q) spectroscopy for nuclear forensics measurements of trace actinide samples, where the goal is determination of ratios of isotopes with Q values in the range of 5-7 MeV. Simplified, rapid sample preparation and detector assembly is necessary for practical measurements, while maintaining good energy resolution. The second application is electron capture spectroscopy of isotopes with low Q values, such as Ho, for measurement of neutrino mass. Detectors for electron capture spectroscopy are designed for measuring energies up to approximately 6 keV. Their smaller heat capacity and physical size present unique challenges. Both applications require precise deposition of radioactive material and encapsulation in an absorber with optimized thermal properties and coupling to the TES. We have made detectors for both applications with a variety of designs and assembly methods, and will present their development. C1 [Croce, M. P.; Bond, E. M.; Hoover, A. S.; Kunde, G. J.; Moody, W. A.; Rabin, M. W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Bennett, D. A.; Hayes-Wehle, J.; Kotsubo, V.; Schmidt, D. R.; Ullom, J. N.] NIST, Boulder, CO USA. RP Croce, MP (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM mpcroce@lanl.gov OI Bennett, Douglas/0000-0003-3011-3690; Bond, Evelyn/0000-0001-7335-4086 NR 11 TC 9 Z9 9 U1 1 U2 6 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD SEP PY 2014 VL 176 IS 5-6 BP 1009 EP 1014 DI 10.1007/s10909-013-1045-9 PG 6 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AM5DE UT WOS:000339875400056 ER PT J AU Hanson, DE Roland, CM AF Hanson, David E. Roland, C. M. TI Theoretical Implications of the Elastic Modulus Discontinuity in Rubber Networks (vol 48, pg 1795, 2010) SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Correction C1 [Hanson, David E.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Roland, C. M.] Naval Res Lab, Div Chem, Washington, DC 20375 USA. RP Hanson, DE (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. NR 5 TC 0 Z9 0 U1 1 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD SEP 1 PY 2014 VL 52 IS 17 BP 1178 EP 1178 DI 10.1002/polb.23542 PG 1 WC Polymer Science SC Polymer Science GA AM6FJ UT WOS:000339958500005 ER PT J AU Cao, Y Zhu, KJ Wu, QL Gu, QL Qiu, JH AF Cao, Yang Zhu, Kongjun Wu, Qingliu Gu, Qilin Qiu, Jinhao TI Hydrothermally synthesized barium titanate nanostructures from K2Ti4O9 precursors: Morphology evolution and its growth mechanism SO MATERIALS RESEARCH BULLETIN LA English DT Article DE Layered compounds; Microstructure; Transmission electron microscopy (TEM); Crystal structure ID ION-EXCHANGE REACTION; SOFT CHEMICAL-PROCESS; STRONTIUM-TITANATE; NANOTUBES; BATIO3; SHAPE; NANORODS; NANOWIRES; TRANSFORMATION AB A morphology-controlled synthesis of barium titanate (BaTiO3) nanostructures from nano-whiskers to nanoparticles, were prepared via a hydrothermal strategy by manipulating the alkalinity and reaction temperature. Initially, the K2Ti4O9 precursors almost remain unchanged in the temperature of 80-160 degrees C at 0.1 M. By increasing the alkalinity and temperature, the BaTiO3 nanostructures initially undergoes ion exchange with precursors while retaining the morphology at the self-sacrifice of K2Ti4O9 nano-whiskers, followed by the formation of BaTiO3 nano-maces. Finally, recrystallization occurs and converts into nanoparticles at 120-220 degrees C at 0.8 M. Also, time-dependent experiment was conducted to probe the ion exchange process. The formation mechanism involves the generation of chemical site inducing the ion exchange process and the dissolution-precipitation reaction. By investigating the synthesis and morphology evolution of one-dimensional BaTiO3 nanostructures, this work may be of great significance for fabrication of other perovskite-type MTiO3 (M = Ca, Sr, Pb). (C) 2014 Elsevier Ltd. All rights reserved. C1 [Cao, Yang; Zhu, Kongjun; Gu, Qilin; Qiu, Jinhao] Nanjing Univ Aeronaut & Astronaut, Coll Aerosp Engn, State Key Lab Mech & Control Mech Struct, Nanjing 210016, Jiangsu, Peoples R China. [Cao, Yang] Tohoku Univ, Frontier Res Inst Interdisciplinary Sci, Sendai, Miyagi 9808578, Japan. [Wu, Qingliu] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Zhu, KJ (reprint author), Nanjing Univ Aeronaut & Astronaut, Coll Aerosp Engn, State Key Lab Mech & Control Mech Struct, Nanjing 210016, Jiangsu, Peoples R China. EM kjzhu@nuaa.edu.cn RI Cao, Yang/E-9169-2014; Gu, Qilin/H-6399-2011 OI Gu, Qilin/0000-0003-4951-0207 FU National Nature Science Foundation of China (NSFC) [51372114]; NUAA Fundamental Research Funds [NP2013301]; Priority Academic Program Development of Jiangsu Higher Education Institutions FX We would like to express our gratitude for the college of Materials Science & Technology at Nanjing University of Aeronautics and Astronautics for its technical assistance. We greatly appreciate the financial support from National Nature Science Foundation of China (NSFC No. 51372114), the NUAA Fundamental Research Funds (No. NP2013301), and a Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions. NR 28 TC 10 Z9 10 U1 2 U2 52 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0025-5408 EI 1873-4227 J9 MATER RES BULL JI Mater. Res. Bull. PD SEP PY 2014 VL 57 BP 162 EP 169 DI 10.1016/j.materresbull.2014.05.043 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA AN0ZV UT WOS:000340313400028 ER PT J AU Mandadapu, KK Jones, RE Zimmerman, JA AF Mandadapu, Kranthi K. Jones, Reese E. Zimmerman, Jonathan A. TI On the microscopic definitions of the dislocation density tensor SO MATHEMATICS AND MECHANICS OF SOLIDS LA English DT Article DE Dislocations; plasticity; dislocation density tensor; Burgers vector; Burger circuit ID GRADIENT THEORY; PLASTICITY; INCOMPATIBILITY; LENGTH AB The dislocation density tensor at the macroscale may be obtained by using two seemingly disparate definitions given by Nye and Arsenlis and Parks. Nye's definition depends on counting the dislocations crossing a Burgers circuit of infinitesimal area at the macroscale, where as Arsenlis and Parks's definition is defined as an integrated property of dislocations within an infinitesimal volume. In this paper, it is shown that Arsenlis and Parks' and Nye's definitions for the dislocation density tensor are equivalent when conditions on the length scales of the spacing and curvature of the dislocation lines are obeyed. It is also shown that the definition by Arsenlis and Parks, which can be easily employed in microscopic dislocation dynamics simulations, follows the fundamental extensive property of the Burgers vector, namely, the total Burgers vector of a Burgers circuit is the sum of Burgers vectors of individual dislocation lines intersecting the circuit. C1 [Mandadapu, Kranthi K.; Jones, Reese E.; Zimmerman, Jonathan A.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Jones, RE (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM rjones@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 22 TC 0 Z9 0 U1 2 U2 13 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1081-2865 EI 1741-3028 J9 MATH MECH SOLIDS JI Math. Mech. Solids PD SEP PY 2014 VL 19 IS 7 BP 744 EP 757 DI 10.1177/1081286513486792 PG 14 WC Materials Science, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Materials Science; Mathematics; Mechanics GA AM8HU UT WOS:000340114900002 ER PT J AU Sandim, HRZ Bolmaro, RE Renzetti, RA Sandim, MJR Hartwig, KT Vogel, SC Raabe, D AF Sandim, H. R. Z. Bolmaro, R. E. Renzetti, R. A. Sandim, M. J. R. Hartwig, K. T. Vogel, S. C. Raabe, D. TI Texture Evolution as Determined by In situ Neutron Diffraction During Annealing of Iron Deformed by Equal Channel Angular Pressing SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article ID LOW-CARBON-STEEL; ELECTRON BACKSCATTER DIFFRACTION; SEVERE PLASTIC-DEFORMATION; INTERSTITIAL-FREE STEEL; GRAIN-REFINEMENT; SIMPLE SHEAR; MECHANICAL-PROPERTIES; PHASE-TRANSFORMATION; TOF DIFFRACTOMETER; INITIAL TEXTURE AB In situ neutron diffraction experiments were performed to follow the annealing behavior of iron deformed by equal-channel angular pressing at room temperature using route B (c) to a total von Mises strain of epsilon (vM) = 9.2. The temperature was varied from room temperature to 1223 K (950 A degrees C), while neutron diffraction data for quantitative texture analysis were collected at a given temperature when holding for 5 minutes. Pole figures and orientation distribution function maps from neutron diffraction and electron backscatter diffraction measurements were used to follow the changes in crystallographic texture and grain size during annealing. In situ neutron diffraction experiments allowed understanding and identifying texture-related changes that occur during recrystallization, grain growth, and phase transformation in iron. C1 [Sandim, H. R. Z.; Renzetti, R. A.; Sandim, M. J. R.] Univ Sao Paulo, Escola Engn Lorena, BR-12600970 Lorena, Brazil. [Bolmaro, R. E.] CONICET UNR, Inst Fis Rosario, RA-2000 Rosario, Santa Fe, Argentina. [Hartwig, K. T.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Vogel, S. C.] LANSCE LANL, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA. [Raabe, D.] MPIE, D-40237 Dusseldorf, Germany. RP Sandim, HRZ (reprint author), Univ Sao Paulo, Escola Engn Lorena, BR-12600970 Lorena, Brazil. EM hsandim@demar.eel.usp.br RI Raabe, Dierk/A-6470-2009; Bolmaro, Raul/H-6520-2016; Sandim, Maria /Q-9682-2016; Sandim, Hugo/F-2778-2013; OI Raabe, Dierk/0000-0003-0194-6124; Bolmaro, Raul/0000-0002-8218-6958; Sandim, Hugo/0000-0003-4522-6639; Vogel, Sven C./0000-0003-2049-0361 FU U.S. Department of Energy's Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396] FX Authors acknowledge the kind assistance of R. Barber (Texas A&M University) for ECAP processing. Authors are also grateful to Prof. P. R. Rios (UFF, Brazil) for supplying the material for this study. The kind assistance of K. Angenendt (MPIE) in EBSD measurements is also deeply acknowledged. This work has benefited from Lujan Neutron Scattering Center at LANSCE, which is funded by the U.S. Department of Energy's Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE contract DE-AC52-06NA25396. NR 65 TC 1 Z9 1 U1 2 U2 18 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD SEP PY 2014 VL 45A IS 10 BP 4235 EP 4246 DI 10.1007/s11661-014-2401-3 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AM5HP UT WOS:000339888100009 ER PT J AU Agarwal, B Dalla Vecchia, C Johnson, JL Khochfar, S Paardekooper, JP AF Agarwal, Bhaskar Dalla Vecchia, Claudio Johnson, Jarrett L. Khochfar, Sadegh Paardekooper, Jan-Pieter TI The First Billion Years project: birthplaces of direct collapse black holes SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: high-redshift; quasars: supermassive black holes; dark ages; reionization; first stars; early Universe ID POPULATION III STARS; DARK-MATTER HALOES; METAL-FREE STARS; VIRIAL TEMPERATURES; HYDRODYNAMICAL SIMULATIONS; SUPERMASSIVE STARS; GALAXY FORMATION; EARLY UNIVERSE; 10(4) K; EVOLUTION AB We investigate the environment in which direct-collapse black holes may form by analysing a cosmological, hydrodynamical simulation that is part of the First Billion Years project. This simulation includes the most relevant physical processes leading to direct collapse of haloes, most importantly, molecular hydrogen depletion by dissociation of H-2 and H- from the evolving Lyman-Werner radiation field. We selected a sample of pristine atomic-cooling haloes that have never formed stars in their past, have not been polluted with heavy elements and are cooling predominantly via atomic hydrogen lines. Amongst them we identified six haloes that could potentially harbour massive seed black holes formed via direct collapse (with masses in the range of 10(4-6) M-aS (TM)). These potential hosts of direct-collapse black holes form as satellites are found within 15 physical kpc of protogalaxies, with stellar masses in the range a parts per thousand 10(5-7) M-aS (TM) and maximal star formation rates of a parts per thousand 0.1 M-aS (TM) yr(-1) over the past 5 Myr, and are exposed to the highest flux of Lyman-Werner radiation emitted from the neighbouring galaxies. It is the proximity to these protogalaxies that differentiates these haloes from rest of the sample. C1 [Agarwal, Bhaskar; Dalla Vecchia, Claudio; Johnson, Jarrett L.; Khochfar, Sadegh; Paardekooper, Jan-Pieter] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Dalla Vecchia, Claudio] Inst Astrofis Canarias, Tenerife 38205, Spain. [Dalla Vecchia, Claudio] Univ La Laguna, Dept Astrofis, Tenerife 38205, Spain. [Johnson, Jarrett L.] Los Alamos Natl Lab, Theoret Div 10, Los Alamos, NM 87545 USA. [Khochfar, Sadegh] Univ Edinburgh, Inst Astron, Royal Observ, Edinburgh EH9 3HJ, Midlothian, Scotland. RP Agarwal, B (reprint author), Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. EM agarwalb@mpe.mpg.de OI Dalla Vecchia, Claudio/0000-0002-2620-7056; Agarwal, Bhaskar/0000-0003-1390-6170 FU Marie Curie Reintegration Grant [PERG06-GA-2009-256573]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX The simulation was run on the facilities of the Max-Planck Rechenzentrum Garching. BA would like to thank Andrew Davis for his extremely useful inputs during the early stages of the study. BA would also like to thank Jonny Elliott and Alessia Longobardi for their comments during the preparation of the manuscript. CDV acknowledges support by Marie Curie Reintegration Grant PERG06-GA-2009-256573. Work at LANL was done under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 61 TC 33 Z9 33 U1 0 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD SEP 1 PY 2014 VL 443 IS 1 BP 648 EP 657 DI 10.1093/mnras/stu1112 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM5UR UT WOS:000339927000049 ER PT J AU Gorbikov, E Gal-Yam, A Ofek, EO Vreeswijk, PM Nugent, PE Chotard, N Kulkarni, SR Cao, Y De Cia, A Yaron, O Tal, D Arcavi, I Kasliwal, MM Cenko, SB Sullivan, M Chen, JC AF Gorbikov, Evgeny Gal-Yam, Avishay Ofek, Eran O. Vreeswijk, Paul M. Nugent, Peter E. Chotard, Nicolas Kulkarni, Shrinivas R. Cao, Yi De Cia, Annalisa Yaron, Ofer Tal, David Arcavi, Iair Kasliwal, Mansi M. Cenko, S. Bradley Sullivan, Mark Chen, Juncheng TI iPTF13beo: the double-peaked light curve of a Type Ibn supernova discovered shortly after explosion SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE supernovae: general; supernovae: individual: iPTF13beo; stars: winds, outflows; stars: Wolf-Rayet ID RICH CIRCUMSTELLAR MEDIUM; SN 2009IP; SHOCK BREAKOUT; DUST FORMATION; CORE-COLLAPSE; MASSIVE STAR; 2006JC; EMISSION; OUTBURST; SPECTROSCOPY AB We present optical photometric and spectroscopic observations of the Type Ibn (SN 2006jc-like) supernova (SN) iPTF13beo. Detected by the intermediate Palomar Transient Factory similar to 3 h after the estimated first light, iPTF13beo is the youngest and the most distant (similar to 430 Mpc) Type Ibn event ever observed. The iPTF13beo light curve is consistent with light curves of other Type Ibn SNe and with light curves of fast Type Ic events, but with a slightly faster rise-time of two days. In addition, the iPTF13beo R-band light curve exhibits a double-peak structure separated by similar to 9 d, not observed before in any Type Ibn SN. A low-resolution spectrum taken during the iPTF13beo rising stage is featureless, while a late-time spectrum obtained during the declining stage exhibits narrow and intermediate-width He i and Si ii features with full width at half-maximum a parts per thousand 2000-5000 km s(-1) and is remarkably similar to the prototypical SN Ibn 2006jc spectrum. We suggest that our observations support a model of a massive star exploding in a dense He-rich circumstellar medium (CSM). A shock breakout in a CSM model requires an eruption releasing a total mass of similar to 0.1 MaS (TM) over a time-scale of couple of weeks prior to the SN explosion. C1 [Gorbikov, Evgeny; Gal-Yam, Avishay; Ofek, Eran O.; Vreeswijk, Paul M.; De Cia, Annalisa; Yaron, Ofer; Tal, David; Arcavi, Iair] Weizmann Inst Sci, Fac Phys, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Nugent, Peter E.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Nugent, Peter E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Chotard, Nicolas] Univ Lyon, F-69622 Lyon, France. [Chotard, Nicolas] Univ Lyon 1, F-69622 Villeurbanne, France. [Chotard, Nicolas] CNRS, IN2P3, Inst Phys Nucl Lyon, F-75700 Paris, France. [Kulkarni, Shrinivas R.; Cao, Yi] CALTECH, Dept Astron, Pasadena, CA 91125 USA. [Kasliwal, Mansi M.] Carnegie Inst Sci, Pasadena, CA 91101 USA. [Cenko, S. Bradley] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Cenko, S. Bradley] Univ Maryland, Joint Space Sci Inst, College Pk, MD 20742 USA. [Sullivan, Mark] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Chen, Juncheng] Tsinghua Univ, Tsinghua Ctr Astrophys, Beijing 100084, Peoples R China. RP Gorbikov, E (reprint author), Weizmann Inst Sci, Fac Phys, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. EM mrmagnate@mail.ru OI Sullivan, Mark/0000-0001-9053-4820 FU W. M. Keck Foundation; Israeli Ministry of Science; I-CORE Programme of the Planning and Budgeting Committee; Israel Science Foundation [1829/12]; EU/FP7 via ERC grant [307260]; ISF grant; BSF grant; Minerva grant; GIF grant; ISF; Israeli Planning and Budgeting Committee; Kimmel award; Lyon Institute of Origins [ANR-10-LABX-66] FX This paper is based on observations obtained with the Samuel Oschin Telescope as part of the Palomar Transient Factory project, a scientific collaboration between the California Institute of Technology, Columbia University, Las Cumbres Observatory, the Lawrence Berkeley National Laboratory, the National Energy Research Scientific Computing Center, the University of Oxford, and the Weizmann Institute of Science. Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and NASA; the Observatory was made possible by the generous financial support of the W. M. Keck Foundation. We are grateful for excellent staff assistance at Palomar, Lick, and Keck Observatories. EOO is incumbent of the Arye Dissentshik career development chair and is grateful to support by a grant from the Israeli Ministry of Science and the I-CORE Programme of the Planning and Budgeting Committee and The Israel Science Foundation (grant no. 1829/12).; AG-Y acknowledges support by the EU/FP7 via ERC grant no. 307260, ISF, BSF, Minerva and GIF grants, the 'Quantum Universe' I-Core programme funded by the ISF and the Israeli Planning and Budgeting Committee, and the Kimmel award.; NC acknowledges support from the Lyon Institute of Origins under grant ANR-10-LABX-66. NR 45 TC 17 Z9 18 U1 0 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD SEP 1 PY 2014 VL 443 IS 1 BP 671 EP 677 DI 10.1093/mnras/stu1184 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM5UR UT WOS:000339927000052 ER PT J AU Zhang, HX Ren, F Wang, YQ Hong, MQ Xiao, XH Liu, D Qin, WJ Zheng, XD Liu, YC Jiang, CZ AF Zhang, Hongxiu Ren, Feng Wang, Yongqiang Hong, Mengqing Xiao, Xiangheng Liu, Dan Qin, Wenjing Zheng, Xudong Liu, Yichao Jiang, Changzhong TI Enhanced radiation tolerance of nanochannel V films through defects release SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Nanochannel film; Radiation tolerance; TEM; Hardening ID HELIUM ION-IRRADIATION; GRAIN-BOUNDARIES; DISPLACEMENT CASCADES; MECHANICAL-PROPERTIES; ELECTRON-MICROSCOPY; INDUCED DIFFUSION; BUBBLE FORMATION; POINT-DEFECTS; PHASE-DIAGRAM; NANOPOROUS AU AB Since surfaces are perfect sinks for defects, nanochannel material with a high surface to volume ratio has the potential to be extremely radiation tolerant. Nanochannel V films deposited at 500 degrees C and 600 degrees C, Ag and V/Ag multilayer films deposited at room temperature and bulk V, were subjected to He irradiation. TEM images show larger bubbles appeared in the Ag film and the V/Ag multilayer under He+ ion irradiation to a fluence of 5 x 10(16) ions/cm(2). While few small He bubbles formed in the irradiated nanochannel V film and a high density of small bubbles appeared in the irradiated bulk V when the fluence of He+ ions reaches 1 x 10(17) ions/cm(2), which is two times higher than the fluences on the Ag and multilayer films. Radiation-induced defects can quickly diffuse to the free surfaces of the nanochannels, which greatly reduces the concentration of defects in material and increases the radiation tolerance. Radiation hardening is observed in all specimens. The irradiation-induced hardening in the V nanochannel films is around one third to one fourth of that in the bulk V. (C) 2014 Elsevier B.V. All rights reserved. C1 [Zhang, Hongxiu; Ren, Feng; Hong, Mengqing; Xiao, Xiangheng; Liu, Dan; Qin, Wenjing; Zheng, Xudong; Liu, Yichao; Jiang, Changzhong] Wuhan Univ, Ctr Ion Beam Applicat, Sch Phys & Technol, Wuhan 430072, Peoples R China. [Zhang, Hongxiu; Ren, Feng; Hong, Mengqing; Xiao, Xiangheng; Liu, Dan; Qin, Wenjing; Zheng, Xudong; Liu, Yichao; Jiang, Changzhong] Wuhan Univ, Ctr Electron Microscopy, Wuhan 430072, Peoples R China. [Wang, Yongqiang] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Ren, F (reprint author), Wuhan Univ, Ctr Ion Beam Applicat, Sch Phys & Technol, Wuhan 430072, Peoples R China. EM fren@whu.edu.cn RI Ren, Feng/F-9778-2014; Jiang, Changzhong/O-6273-2014; OI Ren, Feng/0000-0002-9557-5995; xiao, xiangheng/0000-0001-9111-1619 FU Natural Science Foundation of China [91026014, 11175133, U1260102]; Foundations from Chinese Ministry of Education [20100014112004, 311002, NCET-13-0438]; Hubei Provincial Natural Science Foundation [2012FFA042]; Center for Integrated Nanotechnologies (CINT), a US Department of Energy FX The author thanks the Natural Science Foundation of China (91026014, 11175133, U1260102), the Foundations from Chinese Ministry of Education (20100014112004, 311002, NCET-13-0438), and the Hubei Provincial Natural Science Foundation (2012FFA042) for financial support. Partial support for Y.Q. Wang was provided by the Center for Integrated Nanotechnologies (CINT), a US Department of Energy nanoscience user center jointly operated by Los Alamos and Sandia National Laboratories. NR 63 TC 3 Z9 3 U1 0 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD SEP 1 PY 2014 VL 334 BP 1 EP 7 DI 10.1016/j.nimb.2014.05.003 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AN1JT UT WOS:000340339300001 ER PT J AU Khadilkar, A Rozelle, PL Pisupati, SV AF Khadilkar, Aditi Rozelle, Peter L. Pisupati, Sarma V. TI Models of agglomerate growth in fluidized bed reactors: Critical review, status and applications SO POWDER TECHNOLOGY LA English DT Review DE Agglomeration; Fluidization; Combustion; Gasification; Granulation; Population balance ID MELT GRANULATION; WET GRANULATION; COAL ASH; COLLISION; TEMPERATURES; COMBUSTION; MECHANISMS; PARTICLES; SPHERES AB Agglomeration, which leads to growth in particle size over time, is an important phenomenon in several applications that use fluidized bed technologies. Understanding, predicting and controlling this phenomenon are important to avoid operational problems, reduced efficiencies, reactor down-time and thereby monetary losses. Operating conditions, material properties and particle hydrodynamics can simultaneously affect the extent of agglomeration. This makes accurate prediction with mere experimentation difficult. Theoretical models to predict agglomeration based on particle collision dynamics have been evolving. They will enable easier predictions with quick estimates for any changes in parameters. In general, the models use certain criteria to determine the outcome of two-particle collisions, and a technique to estimate the kinetics of agglomerate growth. In addition, they may also include a method to account for the hydrodynamics of the discrete and continuous phases. This paper provides a critical review of the development of such theoretical models and analyzes their suitability to different applications. Several avenues for further development of mathematical models to predict agglomeration are identified. Published by Elsevier B.V. C1 [Khadilkar, Aditi; Pisupati, Sarma V.] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. [Khadilkar, Aditi; Pisupati, Sarma V.] Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA. [Rozelle, Peter L.] US DOE, Off Fossil Energy, Washington, DC 20585 USA. [Khadilkar, Aditi; Pisupati, Sarma V.] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Rozelle, PL (reprint author), 1000 Independence Ave NW, Washington, DC 20585 USA. EM peter.rozelle@hq.doe.gov RI Pisupati, Sarma/A-9861-2009 OI Pisupati, Sarma/0000-0002-2098-3302 NR 65 TC 12 Z9 12 U1 6 U2 44 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0032-5910 EI 1873-328X J9 POWDER TECHNOL JI Powder Technol. PD SEP PY 2014 VL 264 BP 216 EP 228 DI 10.1016/j.powtec.2014.04.063 PG 13 WC Engineering, Chemical SC Engineering GA AM9PR UT WOS:000340214000026 ER PT J AU Riding, R Fralick, P Liang, LY AF Riding, Robert Fralick, Philip Liang, Liyuan TI Identification of an Archean marine oxygen oasis SO PRECAMBRIAN RESEARCH LA English DT Article DE Archean; 2800 Ma; Oxygenation; Carbonate platform; Superior Province; Canada ID BILLION YEARS AGO; STEEP ROCK GROUP; SOUTH-AFRICA; TRANSVAAL SUPERGROUP; CARBONATE PRECIPITATION; PRECAMBRIAN CARBONATES; PONGOLA SUPERGROUP; ISOTOPE EVIDENCE; PHOTOSYNTHESIS; GEOCHEMISTRY AB The early Earth was essentially anoxic. A number of indicators suggest the presence of oxygenic photosynthesis similar to 2700-3000 million years (Ma) ago, but direct evidence for molecular oxygen (O-2) in seawater has remained elusive. Here we report rare earth element (REE) analyses of similar to 2800 million year old shallow-marine limestones and deep-water iron-rich sediments at Steep Rock Lake, Canada. These show that the seawater from which extensive shallow-water limestones precipitated was oxygenated, whereas the adjacent deeper waters where iron-rich sediments formed were not. We propose that oxygen promoted limestone precipitation by oxidative removal of dissolved ferrous iron species, Fe(II), to insoluble Fe(III) oxyhydroxide, and estimate that at least 10.25 mu M oxygen concentration in seawater was required to accomplish this at Steep Rock. This agrees with the hypothesis that an ample supply of dissolved Fe(II) in Archean oceans would have hindered limestone formation. There is no direct evidence for the oxygen source at Steep Rock, but organic carbon isotope values and diverse stromatolites in the limestones suggest the presence of cyanobacteria. Our findings support the view that during the Archean significant oxygen levels first developed in protected nutrient-rich shallow marine habitats. They indicate that these environments were spatially restricted, transient, and promoted limestone precipitation. If Archean marine limestones in general reflect localized oxygenic removal of dissolved iron at the margins of otherwise anoxic iron-rich seas, then early oxygen oases are less elusive than has been assumed. (C) 2014 Elsevier B.V. All rights reserved. C1 [Riding, Robert] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. [Fralick, Philip] Lakehead Univ, Dept Geol, Thunder Bay, ON P7B 5E1, Canada. [Liang, Liyuan] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Riding, R (reprint author), Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. EM rriding@utk.edu RI Liang, Liyuan/O-7213-2014 OI Liang, Liyuan/0000-0003-1338-0324 FU Natural Science and Engineering Research Council of Canada Discovery Grant; Lakehead University Research Chair; DOE [DE-AC05-00OR22725] FX This work was partly supported by a Natural Science and Engineering Research Council of Canada Discovery Grant and a Lakehead University Research Chair to PF. The U.S. Department of Energy (DOE), Office of Science, supports LL at Oak Ridge National Laboratory (ORNL) which is managed by UT Battelle, LLC for the DOE under contract DE-AC05-00OR22725. We are very grateful to Tobias Himmler for running LA-ICP-MS analyses at the University of Bremen. Sam Spivik and Fabio Tosti assisted in figure preparation. We thank an anonymous reviewer for helpful comments, and Balz Kamber for critical suggestions regarding Ce-anomaly interpretation that improved the article. Chris Fedo and Guochun Zhao provided expert editorial guidance. NR 47 TC 12 Z9 18 U1 3 U2 45 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-9268 EI 1872-7433 J9 PRECAMBRIAN RES JI Precambrian Res. PD SEP PY 2014 VL 251 BP 232 EP 237 DI 10.1016/j.precamres.2014.06.017 PG 6 WC Geosciences, Multidisciplinary SC Geology GA AM9TX UT WOS:000340225000014 ER PT J AU Czumaj, A Goldreich, O Ron, D Seshadhri, C Shapira, A Sohler, C AF Czumaj, Artur Goldreich, Oded Ron, Dana Seshadhri, C. Shapira, Asaf Sohler, Christian TI Finding Cycles and Trees in Sublinear Time SO RANDOM STRUCTURES & ALGORITHMS LA English DT Article DE sublinear-time algorithms; property testing; bounded-degree graphs; one-sided versus two-sided error probability ID GRAPHS; PROPERTY; BIPARTITENESS AB We present sublinear-time (randomized) algorithms for finding simple cycles of length at least k3 and tree-minors in bounded-degree graphs. The complexity of these algorithms is related to the distance of the graph from being C-k-minor free (resp., free from having the corresponding tree-minor). In particular, if the graph is (1)-far from being cycle-free (i.e., a constant fraction of the edges must be deleted to make the graph cycle-free), then the algorithm finds a cycle of polylogarithmic length in time O(N), where N denotes the number of vertices. This time complexity is optimal up to polylogarithmic factors. The foregoing results are the outcome of our study of the complexity of one-sided error property testing algorithms in the bounded-degree graphs model. For example, we show that cycle-freeness of N-vertex graphs can be tested with one-sided error within time complexity O(poly(1/E)N), where denotes the proximity parameter. This matches the known (N) query lower bound for one-sided error cycle-freeness testing, and contrasts with the fact that any minor-free property admits a two-sided error tester of query complexity that only depends on . We show that the same upper bound holds for testing whether the input graph has a simple cycle of length at least k, for any k3. On the other hand, for any fixed tree T, we show that T-minor freeness has a one-sided error tester of query complexity that only depends on the proximity parameter . Our algorithm for finding cycles in bounded-degree graphs extends to general graphs, where distances are measured with respect to the actual number of edges. Such an extension is not possible with respect to finding tree-minors in o(N) complexity. (c) 2012 Wiley Periodicals, Inc. Random Struct. Alg., 45, 139-184, 2014 C1 [Czumaj, Artur] Univ Warwick, Dept Comp Sci, Ctr Discrete Math & Its Applicat DIMAP, Coventry CV4 7AL, W Midlands, England. [Goldreich, Oded] Weizmann Inst Sci, Dept Comp Sci, IL-76100 Rehovot, Israel. [Ron, Dana] Tel Aviv Univ, Sch Elect Engn, IL-69978 Tel Aviv, Israel. [Seshadhri, C.] Sandia Natl Labs, Livermore, CA USA. [Shapira, Asaf] Tel Aviv Univ, Sch Math, IL-69978 Tel Aviv, Israel. [Shapira, Asaf] Georgia Inst Technol, Sch Math, Atlanta, GA 30332 USA. [Shapira, Asaf] Georgia Inst Technol, Sch Comp Sci, Atlanta, GA 30332 USA. [Sohler, Christian] TU Dortmund Univ, Dept Comp Sci, Dortmund, Germany. RP Goldreich, O (reprint author), Weizmann Inst Sci, Dept Comp Sci, IL-76100 Rehovot, Israel. EM oded.goldreich@weizmann.ac.il FU EPSRC [EP/G064679/1, EP/D063191/1]; Israel Science Foundation [1041/08, 246/08]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSF Grant [DMS-0901355]; ISF Grant [224/11]; Marie-Curie CIG Grant [303320]; DFG grant [So 514/3-2] FX Research partially supported by EPSRC awards EP/G064679/1 and EP/D063191/1.; Supported by the Israel Science Foundation (grant No. 1041/08).; Supported by the Israel Science Foundation (grant No. 246/08).; Employee of Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000.; Supported in part by NSF Grant DMS-0901355, ISF Grant 224/11, and a Marie-Curie CIG Grant 303320.; Supported by DFG grant So 514/3-2. NR 22 TC 1 Z9 1 U1 1 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1042-9832 EI 1098-2418 J9 RANDOM STRUCT ALGOR JI Random Struct. Algorithms PD SEP PY 2014 VL 45 IS 2 BP 139 EP 184 DI 10.1002/rsa.20462 PG 46 WC Computer Science, Software Engineering; Mathematics, Applied; Mathematics SC Computer Science; Mathematics GA AN0MM UT WOS:000340278700001 ER PT J AU Popovic, ZV Lazarevic, N Bogdanovic, S Radonjic, MM Tanaskovic, D Hu, RW Lei, HC Petrovic, C AF Popovic, Z. V. Lazarevic, N. Bogdanovic, S. Radonjic, M. M. Tanaskovic, D. Hu, Rongwei Lei, Hechang Petrovic, C. TI Signatures of the spin-phonon coupling in Fe1+yTe1-xSex alloys SO SOLID STATE COMMUNICATIONS LA English DT Article DE Magnetically ordered materials; Crystal structure and symmetry; Phonos; Inelastic light scattering ID 1ST-PRINCIPLES CALCULATIONS; SUPERCONDUCTIVITY AB Raman scattering spectra of Fe1+yTe1-xSex (x=0, y=0.07; x=0.1, y=0.05 and x=0.4, y=0.02) alloys are measured in a temperature range between 20 K and 300 K. The A(1g) and B-1g Raman active modes have been experimentally observed at energies 156 and 198 cm(-1), which is in rather good agreement with the lattice dynamics calculation. The antiferromagnetic spin ordering below 70 K in Fe1.07Te leaves a fingerprint only in the B-1g phonon mode linewidth and energy, whose temperature dependence follows the normalized magnetic susceptibility, indicating the presence of the spin-phonon coupling. The frequency and the linewidth of the A(1g) mode assume a conventional anharmonic temperature dependence in all measured samples, which is also the case for the B-1g mode in the Se doped samples. The linewidth (energy) of the A(1g) mode decreases (increases) with doping, whereas the opposite is seen for the B-1g mode. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Popovic, Z. V.; Lazarevic, N.; Bogdanovic, S.] Univ Belgrade, Inst Phys Belgrade, Ctr Solid State Phys & New Mat, Belgrade 11080, Serbia. [Radonjic, M. M.; Tanaskovic, D.] Univ Belgrade, Inst Phys Belgrade, Comp Sci Lab, Belgrade 11080, Serbia. [Hu, Rongwei; Lei, Hechang; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Popovic, ZV (reprint author), Univ Belgrade, Inst Phys Belgrade, Ctr Solid State Phys & New Mat, Pregrevica 118, Belgrade 11080, Serbia. RI Petrovic, Cedomir/A-8789-2009; Radonjic, Milos/M-1890-2015; LEI, Hechang/H-3278-2016 OI Petrovic, Cedomir/0000-0001-6063-1881; FU Serbian Ministry of Education, Science and Technological Development [ON171032, ON171017, III45018]; US DOE [DE-AC02-98CH10886]; Center for Emergent Superconductivity, an Energy Frontier Research Center - US DOE, Office for Basic Energy Science; FP7 project EGI-InSPIRE; FP7 project PRACE-3IP FX This work was supported by the Serbian Ministry of Education, Science and Technological Development under Projects ON171032, ON171017 and III45018. Work at Brookhaven was supported by the US DOE under Contract No. DE-AC02-98CH10886 and in part by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US DOE, Office for Basic Energy Science (H.L. and C.P.). Numerical simulations were run on the AEGIS e-Infrastructure, supported in part by FP7 projects EGI-InSPIRE, and PRACE-3IP. NR 36 TC 2 Z9 2 U1 0 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-1098 EI 1879-2766 J9 SOLID STATE COMMUN JI Solid State Commun. PD SEP PY 2014 VL 193 BP 51 EP 55 DI 10.1016/j.ssc.2014.05.025 PG 5 WC Physics, Condensed Matter SC Physics GA AN1KL UT WOS:000340341100012 ER PT J AU Comoglio, Y Levitz, J Kienzler, MA Isacoff, EY Sandoz, G AF Comoglio, Y. Levitz, J. Kienzler, M. A. Isacoff, E. Y. Sandoz, G. TI Optophamacological study of TREK channel physiology SO FEBS JOURNAL LA English DT Meeting Abstract CT FEBS EMBO 2014 Conference CY AUG 30-SEP 04, 2014 CL Paris, FRANCE SP FEBS, EMBO DE TREK channels; optopharmacology; hippocampal neurons; excitability; signaling C1 [Comoglio, Y.; Sandoz, G.] Univ Nice Sophia Antipolis, iBV, UMR7277, F-06100 Nice, France. [Comoglio, Y.; Sandoz, G.] CNRS, UMR7277, iBV, F-06100 Nice, France. [Comoglio, Y.; Sandoz, G.] INSERM, U1091, iBV, F-06100 Nice, France. [Comoglio, Y.; Sandoz, G.] Labs Excellence Ion Channel Sci & Therapeut Nice, Nice, France. [Levitz, J.; Kienzler, M. A.; Isacoff, E. Y.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Levitz, J.; Kienzler, M. A.; Isacoff, E. Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Life Sci Addit 271, Berkeley, CA 94720 USA. [Levitz, J.; Isacoff, E. Y.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Isacoff, E. Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1742-464X EI 1742-4658 J9 FEBS J JI FEBS J. PD SEP PY 2014 VL 281 SU 1 SI SI MA CS-I-4-3 BP 14 EP 14 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP1WE UT WOS:000359666800041 ER PT J AU Tyagi, S Vandelinder, V Banterle, N Fuertes, G Milles, S Agez, M Lemke, EA AF Tyagi, S. Vandelinder, V. Banterle, N. Fuertes, G. Milles, S. Agez, M. Lemke, E. A. TI Continuous throughput and long-term observation of single-molecule FRET without immobilization for studying protein dynamics SO FEBS JOURNAL LA English DT Meeting Abstract CT FEBS EMBO 2014 Conference CY AUG 30-SEP 04, 2014 CL Paris, FRANCE SP FEBS, EMBO C1 [Tyagi, S.; Banterle, N.; Fuertes, G.; Milles, S.; Agez, M.; Lemke, E. A.] EMBL, SCB UNIT, Heidelberg, Germany. [Vandelinder, V.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Livermore, CA 94550 USA. NR 1 TC 0 Z9 0 U1 2 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1742-464X EI 1742-4658 J9 FEBS J JI FEBS J. PD SEP PY 2014 VL 281 SU 1 SI SI MA CS III-1-3 BP 27 EP 28 PG 2 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP1WE UT WOS:000359666800086 ER PT J AU Osterwalder, M Speziale, D Shoukry, M Mohan, R Ivanek, R Kohler, M Beisel, C Christoffels, V Visel, A Zeller, R Lopez-Rios, J AF Osterwalder, M. Speziale, D. Shoukry, M. Mohan, R. Ivanek, R. Kohler, M. Beisel, C. Christoffels, V. Visel, A. Zeller, R. Lopez-Rios, J. TI HAND2 regulates the transcriptional circuits that compartmentalize the early mouse limb bud SO FEBS JOURNAL LA English DT Meeting Abstract CT FEBS EMBO 2014 Conference CY AUG 30-SEP 04, 2014 CL Paris, FRANCE SP FEBS, EMBO DE ChIP-seq; Hand2; limb bud C1 [Osterwalder, M.; Speziale, D.; Ivanek, R.; Zeller, R.; Lopez-Rios, J.] Univ Basel, Dept Biomed, Basel, Switzerland. [Shoukry, M.; Visel, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Mohan, R.; Christoffels, V.] Univ Amsterdam, Acad Med Ctr, NL-1105 AZ Amsterdam, Netherlands. [Kohler, M.; Beisel, C.] ETHZ Dept Biosyst Sci & Engn, Basel, Switzerland. NR 0 TC 0 Z9 0 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1742-464X EI 1742-4658 J9 FEBS J JI FEBS J. PD SEP PY 2014 VL 281 SU 1 SI SI MA MON-230 BP 326 EP 326 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP1WE UT WOS:000359666802210 ER PT J AU Macho, AP Schwessinger, B Ntoukakis, V Brutus, A Segonzac, C Roy, S Kadota, Y Oh, MH Sklenar, J Derbyshire, P Lozano-Duran, R Malinovsky, FG Monaghan, J Menke, FL Huber, SC He, SY Zipfel, C AF Macho, A. P. Schwessinger, B. Ntoukakis, V. Brutus, A. Segonzac, C. Roy, S. Kadota, Y. Oh, M. -H. Sklenar, J. Derbyshire, P. Lozano-Duran, R. Malinovsky, F. Gro Monaghan, J. Menke, F. L. Huber, S. C. He, S. Yang Zipfel, C. TI A bacterial tyrosine phosphatase inhibits plant pattern recognition receptor activation SO FEBS JOURNAL LA English DT Meeting Abstract CT FEBS EMBO 2014 Conference CY AUG 30-SEP 04, 2014 CL Paris, FRANCE SP FEBS, EMBO C1 [Macho, A. P.; Schwessinger, B.; Ntoukakis, V.; Segonzac, C.; Roy, S.; Kadota, Y.; Lozano-Duran, R.; Malinovsky, F. Gro; Monaghan, J.; Menke, F. L.; Zipfel, C.] Sainsbury Lab, Norwich, Norfolk, England. [Brutus, A.; He, S. Yang] Michigan State Univ, DOE Plant Res Lab, E Lansing, MI 48824 USA. [He, S. Yang] Michigan State Univ, Howard Hughes Med Inst, E Lansing, MI 48824 USA. [Oh, M. -H.; Huber, S. C.] Univ Illinois, USDA ARS, Urbana, IL 61801 USA. [Oh, M. -H.; Huber, S. C.] Univ Illinois, Dept Plant Biol, Urbana, IL 61801 USA. [Oh, M. -H.] Chungnam Natl Univ, Dept Biol Sci, Taejon 305764, South Korea. RI Kadota, Yasuhiro/A-9406-2011 OI Kadota, Yasuhiro/0000-0002-4782-1418 NR 0 TC 0 Z9 0 U1 1 U2 9 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1742-464X EI 1742-4658 J9 FEBS J JI FEBS J. PD SEP PY 2014 VL 281 SU 1 SI SI MA WED-324 BP 726 EP 726 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP1WE UT WOS:000359666804297 ER PT J AU Nguyen, VV Poudyal, N Liu, XB Liu, JP Sun, K Kramer, MJ Cui, J AF Nguyen, V. Vuong Poudyal, N. Liu, X. B. Liu, J. Ping Sun, K. Kramer, M. J. Cui, J. TI Novel processing of high-performance MnBi magnets SO MATERIALS RESEARCH EXPRESS LA English DT Article DE rare-earth-free magnets; MnBi magnets; LTP MnBi phase AB Rare-earth-free MnBi magnets have attracted much attention recently due to their positive temperature coefficient of coercivity. In this work, the preparation, microstructure and magnetic properties of bulk MnBi magnets have been investigated. A low-temperature (-120 degrees C), low-energy ball-milling (LTLEBM) process has been adopted in the initial MnBi powder preparation that reduces the particle size to 1-5 mu m from the 35-75 mu m size of raw material powders of the MnBi low-temperature phase (LTP) (similar to 97 wt%) made by melting and annealing. The LTLEBM process has significantly suspended the decomposition of the LTP MnBi that occurs excessively during ordinary room-temperature ball milling. After the LTLEBM, the coercivity H-i(c) of the MnBi powder was increased from 1 kOe to 12 kOe while the LTP content in the powder was retained as high as 95 wt%. The as-milled powders were then aligned in an 18 kOe field and warm-compacted into a dense bulk magnet at 300 degrees C for 10 min to reach a mass density of similar to 8.4 g cm(-3). The bulk magnets have a maximum energy product of 7.8 MGOe and coercivity of 6.5 kOe at room temperature. When the temperature is increased to 475 K, the coercivity is increased to 23 kOe. C1 [Nguyen, V. Vuong; Poudyal, N.; Liu, X. B.; Liu, J. Ping] Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. [Sun, K.; Kramer, M. J.] Iowa State Univ, Dept Energy, Ames Lab US, Ames, IA 50011 USA. [Cui, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Nguyen, VV (reprint author), Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. EM pliu@uta.edu RI Liu, Xubo/A-1883-2008 OI Liu, Xubo/0000-0002-2558-0959 FU US DOE/ARPA-E [REACT 0472-1526]; Center for Nanostructured Materials and Characterization Center for Materials and Biology at the University of Texas at Arlington; US DOE [DE-AC02-07CH11358] FX This work was supported in part by US DOE/ARPA-E (REACT 0472-1526) and the Center for Nanostructured Materials and Characterization Center for Materials and Biology at the University of Texas at Arlington. The TEM characterization and magnetometry (MJK and KS) was performed at Ames Laboratory. Ames Laboratory is operated for the US DOE by Iowa State University under contract DE-AC02-07CH11358. NR 9 TC 5 Z9 5 U1 6 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2053-1591 J9 MATER RES EXPRESS JI Mater. Res. Express PD SEP PY 2014 VL 1 IS 3 AR 036108 DI 10.1088/2053-1591/1/3/036108 PG 10 WC Materials Science, Multidisciplinary SC Materials Science GA V43ER UT WOS:000209665200085 ER PT J AU Velisavljevic, N Jacobsen, MK Vohra, YK AF Velisavljevic, Nenad Jacobsen, Matthew K. Vohra, Yogesh K. TI Structural phase stability in nanocrystalline titanium to 161 GPa SO MATERIALS RESEARCH EXPRESS LA English DT Article DE high pressure; diamond anvil cell; titanium; electrical resistance AB Nanocrystalline titanium (nc-Ti) metal was investigated up to 161 GPa at room temperature using a diamond anvil cell. X-ray diffraction and electrical resistance techniques were used to investigate the compressibility and structural phase stability. nc-Ti is observed to undergo three structural phase transitions at high pressures, starting with alpha -> omega at 10 GPa and followed by omega -> gamma at 127 GPa and gamma -> delta at 140 GPa. The observed structural phase transitions, as well as compressibility, are consistent with previously reported values for coarse grained Ti (c-Ti). The high pressure experiments on nc-Ti samples do no show any significant variation of the alpha -> omega transition pressure under varying non-hydrostatic conditions. This is in sharp contrast to c-Ti, where a significant decrease in the alpha -> omega transition pressure is observed under increasing non-hydrostatic conditions. This would indicate that the decrease in grain size in nano grained titanium makes the alpha -> omega phase transition less sensitive to shear stresses as compared to bulk or c-Ti. C1 [Velisavljevic, Nenad; Jacobsen, Matthew K.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. [Vohra, Yogesh K.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. RP Velisavljevic, N (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. EM nenad@lanl.gov FU DOE-NNSA [DE-AC52-06NA25396, DE-NA0001974, DE-NA0002014]; LANL Science Campaign 1; LANL Science Campaign 2; DOE-BES [DE-FG02-99ER45775, DE-AC02-06CH11357]; NSF; US DOE [DE-AC02-06CH11357]; NSFNIH/National Institute of General Medical Sciences under NSF award [DMR-0225180] FX Los Alamos National Laboratory (LANL) is operated by LANS, LLC for the DOE-NNSA under contract no. DE-AC52-06NA25396. NV and MKJ acknowledge funding support from LANL Science Campaigns 1 and 2. YKV is supported by the DOE/NNSA under Award No. DE-NA0002014. Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. APS is supported by DOE-BES, under Contract No. DE-AC02-06CH11357. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. Part of the work was also performed at the B2 beamline at the Cornell High Energy Synchrotron Source (CHESS), which is supported by the NSF and the NIH/National Institute of General Medical Sciences under NSF award DMR-0225180. The authors would also like to thank Dr ST Weir (LLNL) for his work on the designer diamond anvil project and Drs Yuntian T Zhu (LANL) and George T Gray, III (LANL) for providing nc-Ti and high-purity c-Ti sample, respectively. We also thank HPCAT and CHESS beamline staff for their assistance. NR 32 TC 2 Z9 2 U1 2 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2053-1591 J9 MATER RES EXPRESS JI Mater. Res. Express PD SEP PY 2014 VL 1 IS 3 AR 035044 DI 10.1088/2053-1591/1/3/035044 PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA V43ER UT WOS:000209665200047 ER PT J AU Lopez-Velarde, A Vasquez, PD AF Lopez-Velarde, Alejandro Vasquez, Philip D. TI Historic Break with the Past: The New Foreign Investment Possibilities in the Mexican Oil and Gas Industry SO NATURAL RESOURCES JOURNAL LA English DT Article AB One of the missing oil and gas jurisdictions in the world for private participation was finally opened when the Mexican government reformed its constitution and congressional laws last December 2013 and August 2014. Now, the private sector will be able to participate in the exploration, extraction, refining, transportation, storage, distribution, and commercialization of petroleum and its by-products through (i) contracts to be granted by the National Hydrocarbons Commission, and/or (ii) permits to be granted by the Ministry of Energy or the Regulatory Energy Commission. These are important modifications not only for the Mexican oil and gas industry, but also for the local and foreign private industry. These modifications will be analyzed throughout this article with the purpose of explaining the (i) background of petroleum regulation in Mexico; (ii) modifications made to the Mexican Constitution and the legal protection to be provided to foreign participants; (iii) the new legal system applicable to the private sector in each phase of the industry and the potential for foreign investment; and (iv) the new status and role of the national oil company, "Petroleos Mexicanos," and its potential joint ventures with private companies. C1 [Lopez-Velarde, Alejandro] Univ Nacl Autonoma Mexico, Law Energy, Mexico City, DF, Mexico. [Lopez-Velarde, Alejandro] Lo6pez Velarde Wilson Hernandez & Barhem SC, Energy Practice Grp, Mexico City Off, Mexico City, DF, Mexico. [Vasquez, Philip D.] US DOE, Oil & Gas Dept, Washington, DC 20585 USA. RP Lopez-Velarde, A (reprint author), Univ Nacl Autonoma Mexico, Law Energy, Mexico City, DF, Mexico. EM alopezv@lvwhb.com; pdvasquez@gmail.com NR 24 TC 0 Z9 0 U1 3 U2 3 PU UNIV NEW MEXICO, SCH LAW PI ALBUQUERQUE PA MSC11-6070, 1 UNIVERSITY NEW MEXICO, ALBUQUERQUE, NM 87131 USA SN 0028-0739 J9 NAT RESOUR J JI Nat. Resour. J. PD FAL PY 2014 VL 55 IS 1 BP 153 EP 179 PG 27 WC Environmental Studies; Law SC Environmental Sciences & Ecology; Government & Law GA V41YG UT WOS:000209580900005 ER PT J AU Lincoln, D Nord, B AF Lincoln, Don Nord, Brian TI The Expanding Universe: Dark Energy SO PHYSICS TEACHER LA English DT Editorial Material C1 [Lincoln, Don; Nord, Brian] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Lincoln, D (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM lincoln@fnal.gov; nord@fnal.gov OI Nord, Brian/0000-0001-6706-8972 NR 12 TC 0 Z9 0 U1 0 U2 2 PU AMER ASSN PHYSICS TEACHERS PI COLLEGE PK PA 5110 ROANOKE PLACE SUITE 101, COLLEGE PK, MD 20740 USA SN 0031-921X J9 PHYS TEACH JI Phys. Teach. PD SEP PY 2014 VL 52 IS 6 BP 337 EP 343 DI 10.1119/1.4893086 PG 7 WC Physics, Multidisciplinary SC Physics GA CX5YA UT WOS:000365777200007 ER PT J AU Sun, KY Yan, D Hong, TZ Guo, SY AF Sun, Kaiyu Yan, Da Hong, Tianzhen Guo, Siyue TI Stochastic modeling of overtime occupancy and its application in building energy simulation and calibration SO BUILDING AND ENVIRONMENT LA English DT Article DE Building energy use; Building simulation; Model calibration; Occupant behavior; Overtime occupancy; Stochastic modeling ID OFFICE BUILDINGS; PERFORMANCE; WORK AB Overtime is a common phenomenon around the world. Overtime drives both internal heat gains from occupants, lighting and plug-loads, and HVAC operation during overtime periods. Overtime leads to longer occupancy hours and extended operation of building services systems beyond normal working hours, thus overtime impacts total building energy use. Current literature lacks methods to model overtime occupancy because overtime is stochastic in nature and varies by individual occupants and by time. To address this gap in the literature, this study aims to develop a new stochastic model based on the statistical analysis of measured overtime occupancy data from an office building. A binomial distribution is used to represent the total number of occupants working overtime, while an exponential distribution is used to represent the duration of overtime periods. The overtime model is used to generate overtime occupancy schedules as an input to the energy model of a second office building. The measured and simulated cooling energy use during the overtime period is compared in order to validate the overtime model. A hybrid approach to energy model calibration is proposed and tested, which combines ASHRAE Guideline 14 for the calibration of the energy model during normal working hours, and a proposed KS test for the calibration of the energy model during overtime. The developed stochastic overtime model and the hybrid calibration approach can be used in building energy simulations to improve the accuracy of results, and better understand the characteristics of overtime in office buildings. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Sun, Kaiyu; Yan, Da; Guo, Siyue] Tsinghua Univ, Sch Architecture, Dept Bldg Sci, Beijing 100084, Peoples R China. [Hong, Tianzhen] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Hong, TZ (reprint author), Lawrence Berkeley Natl Lab, Environm Energy Technol Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM sky07@mails.tsinghua.edu.cn; yanda@tsinghua.edu.cn; thong@lbl.gov; guo-cy12@mails.tsinghua.edu.cn OI Hong, Tianzhen/0000-0003-1886-9137 FU U.S. Department of Energy [DE-AC02-05CH11231]; Ministry of Science & Technology under the U.S.-China Clean Energy Research Center for Building Energy Efficiency [2010DFA72740-02]; China Project "Research on a framework to support energy efficiency technologies in buildings" [2012BAJ12B00]; China Ministry of Housing and Urban - Rural Development FX This work was sponsored by the U.S. Department of Energy(Contract No. DE-AC02-05CH11231) and the China Ministry of Housing and Urban - Rural Development and the Ministry of Science & Technology (Grant No. 2010DFA72740-02) under the U.S.-China Clean Energy Research Center for Building Energy Efficiency. It was co-sponsored by the China Project "Research on a framework to support energy efficiency technologies in buildings" (Grant No. 2012BAJ12B00). NR 35 TC 26 Z9 26 U1 3 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 EI 1873-684X J9 BUILD ENVIRON JI Build. Environ. PD SEP PY 2014 VL 79 BP 1 EP 12 DI 10.1016/j.buildenv.2014.04.030 PG 12 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA AM2QS UT WOS:000339696500001 ER PT J AU Shin, HM McKone, TE Bennett, DH AF Shin, Hyeong-Moo McKone, Thomas E. Bennett, Deborah H. TI Attributing population-scale human exposure to various source categories: Merging exposure models and biomonitoring data SO ENVIRONMENT INTERNATIONAL LA English DT Article DE Biomarker; Environmental modeling; Exposure routes; Generalized sensitivity analysis; Total production volume ID POLYCYCLIC AROMATIC-HYDROCARBON; GENERALIZED SENSITIVITY-ANALYSIS; POLYBROMINATED DIPHENYL ETHERS; PERSONAL CARE PRODUCTS; DIETARY EXPOSURE; RISK-ASSESSMENT; DECABROMODIPHENYL ETHER; PHTHALATE DIESTERS; FLAME RETARDANTS; INTAKE FRACTION AB Information about the distribution of chemical-production mass with respect to use and release is a major and unavailable input for calculating population-scale exposure estimates. Based on exposure models and biomonitoring data, this study evaluates the distribution of total production volumes (and environmental releases if applicable) for a suite of organic compounds. We used Bayesian approaches that take the total intake from our exposure models as the prior intake distribution and the intake inferred from measured biomarker concentrations in the NHANES survey as the basis for updating. By carrying out a generalized sensitivity analysis, we separated the input parameters for which the modeled range of the total intake is within a factor of 2 of the intake inferred from biomonitoring data and those that result in a range greater than a factor of 2 of the intake. This analysis allows us to find the most sensitive (or important) parameters and the likelihood of emission rates for various source emission categories. Pie charts of contribution from each exposure pathway indicate that chemical properties are a primary determinant of the relative contribution of each exposure pathway within a given class of compounds. For compounds with relatively high octanol-water partition coefficients (K-ow) such as di-2-ethylhexyl phthalate (DEHP), pyrene, 2,2',4,4'-tetrabromodiphenyl ether (PBDE-47), and 2,2',4,4',5,5'-hexabromodiphenyl ether (PBDE-153), more than 80% of exposure derives from outdoor food ingestion and/or indoor dust ingestion. In contrast, for diethyl phthalate (DEP), di-iso-butyl phthalate (DiBP), di-n-butyl phthalate (DnBP), butylbenzyl phthalate (BBP), and naphthalene, all relatively volatile compounds, either inhalation (indoor and outdoor) or dermal uptake from direct consumer use is the dominant exposure pathway. The approach of this study provides insights on confronting data gaps to improve population-scale exposure estimates used for high-throughput chemical prioritization. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Shin, Hyeong-Moo; Bennett, Deborah H.] Univ Calif Davis, Dept Publ Hlth Sci, Davis, CA 95616 USA. [McKone, Thomas E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [McKone, Thomas E.] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA. RP Shin, HM (reprint author), Univ Calif Davis, One Shields Ave,MS1-C, Davis, CA 95616 USA. EM hmshin@ucdavis.edu FU American Chemistry Council [3-DBACC01] FX This research is funded by the American Chemistry Council (Grant#: 3-DBACC01). NR 82 TC 2 Z9 2 U1 5 U2 55 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0160-4120 EI 1873-6750 J9 ENVIRON INT JI Environ. Int. PD SEP PY 2014 VL 70 BP 183 EP 191 DI 10.1016/j.envint.2014.05.020 PG 9 WC Environmental Sciences SC Environmental Sciences & Ecology GA AM2PL UT WOS:000339693200018 PM 24934857 ER PT J AU Petrov, PV Newman, GA AF Petrov, Petr V. Newman, Gregory A. TI Three-dimensional inverse modelling of damped elastic wave propagation in the Fourier domain SO GEOPHYSICAL JOURNAL INTERNATIONAL LA English DT Article DE Numerical solutions; Inverse theory; Seismic tomography; Computational seismology; Wave propagation ID SEISMIC-REFLECTION DATA; FORM INVERSION; FINITE-DIFFERENCE; FREQUENCY-DOMAIN; ELECTROMAGNETIC INVERSION; CONJUGATE GRADIENTS; BOUNDARY-CONDITION; GAUSS-NEWTON; VELOCITY; STRATEGY AB 3-D full waveform inversion (FWI) of seismic wavefields is routinely implemented with explicit time-stepping simulators. A clear advantage of explicit time stepping is the avoidance of solving large-scale implicit linear systems that arise with frequency domain formulations. However, FWI using explicit time stepping may require a very fine time step and (as a consequence) significant computational resources and run times. If the computational challenges of wavefield simulation can be effectively handled, an FWI scheme implemented within the frequency domain utilizing only a few frequencies, offers a cost effective alternative to FWI in the time domain. We have therefore implemented a 3-D FWI scheme for elastic wave propagation in the Fourier domain. To overcome the computational bottleneck in wavefield simulation, we have exploited an efficient Krylov iterative solver for the elastic wave equations approximated with second and fourth order finite differences. The solver does not exploit multilevel preconditioning for wavefield simulation, but is coupled efficiently to the inversion iteration workflow to reduce computational cost. The workflow is best described as a series of sequential inversion experiments, where in the case of seismic reflection acquisition geometries, the data has been laddered such that we first image highly damped data, followed by data where damping is systemically reduced. The key to our modelling approach is its ability to take advantage of solver efficiency when the elastic wavefields are damped. As the inversion experiment progresses, damping is significantly reduced, effectively simulating non-damped wavefields in the Fourier domain. While the cost of the forward simulation increases as damping is reduced, this is counterbalanced by the cost of the outer inversion iteration, which is reduced because of a better starting model obtained from the larger damped wavefield used in the previous inversion experiment. For cross-well data, it is also possible to launch a successful inversion experiment without laddering the damping constants. With this type of acquisition geometry, the solver is still quite effective using a small fixed damping constant. To avoid cycle skipping, we also employ a multiscale imaging approach, in which frequency content of the data is also laddered (with the data now including both reflection and cross-well data acquisition geometries). Thus the inversion process is launched using low frequency data to first recover the long spatial wavelength of the image. With this image as a new starting model, adding higher frequency data refines and enhances the resolution of the image. FWI using laddered frequencies with an efficient damping schemed enables reconstructing elastic attributes of the subsurface at a resolution that approaches half the smallest wavelength utilized to image the subsurface. We show the possibility of effectively carrying out such reconstructions using two to six frequencies, depending upon the application. Using the proposed FWI scheme, massively parallel computing resources are essential for reasonable execution times. C1 [Petrov, Petr V.; Newman, Gregory A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Petrov, PV (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, One Cyclotron Rd,MS 74R-0120, Berkeley, CA 94720 USA. EM pvpetrov@lbl.gov RI Petrov, Petr/G-2486-2015; Newman, Gregory/G-2813-2015 FU U.S. Department of Energy Office of Science and Geothermal Program Office [DE-AC02-05CH11231, GT-480010-19823-10] FX This work was carried out at Lawrence Berkeley National Laboratory with funding provided by the U.S. Department of Energy Office of Science and Geothermal Program Office under respective contract numbers DE-AC02-05CH11231 and GT-480010-19823-10. Computational resources were provided by the National Energy Research Scientific Computing (NERSC) Center. NR 55 TC 2 Z9 2 U1 1 U2 14 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0956-540X EI 1365-246X J9 GEOPHYS J INT JI Geophys. J. Int. PD SEP PY 2014 VL 198 IS 3 BP 1599 EP 1617 DI 10.1093/gji/ggu222 PG 19 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AM6EN UT WOS:000339955900025 ER PT J AU Parsons, N Levin, DA Walker, AC Moore, CH Goldstein, DB Varghese, PL Trafton, L AF Parsons, Neal Levin, Deborah A. Walker, Andrew C. Moore, Chris H. Goldstein, David B. Varghese, Philip L. Trafton, Laurence TI Influence of ab initio chemistry models on simulations of the Ionian atmosphere SO ICARUS LA English DT Article DE Io; Atmospheres, structure; Jupiter, satellites ID IOS ATMOSPHERE; VOLCANIC PLUMES; PLASMA AB There is significant scientific interest in simulating the unique atmospheric conditions on the Jovian moon Io that range from cold surface temperatures to hyperthermal interactions which possibly supply the Jovian plasma torus. The Direct Simulation Monte Carlo (DSMC) method is well suited to model the rarefied, predominantly SO2, Ionian atmosphere. High speed collisions between SO2 and the hypervelocity O atoms and ions that compose the plasma torus are a significant mechanism in determining the composition of the atmosphere; therefore, high-fidelity modeling of their interactions is crucial to the accuracy of such simulations. Typically, the Total Collision Energy (TCE) model is used to determine molecular dissociation probabilities and the Variable Hard Sphere (VHS) model is used to determine collision cross sections. However, the parameters for each of these baseline models are based on low-temperature experimental data and thus have unknown reliability for the hyperthermal conditions in the Ionian atmosphere. Recently, Molecular Dynamics/Quasi-Classical Trajectory (MD/QCT) studies have been conducted to generate accurate collision and chemistry models for the SO2-O collision pair in order to replace the baseline models. However, the influence of MD/QCT models on Ionian simulations compared to the previously used models is not well understood. In this work, 1D simulations are conducted using both the MD/QCT-based and baseline models in order to determine the effect of MD/QCT models on Ionian simulations. It is found that atmospheric structure predictions are highly sensitive to the chemistry and collision models. Specifically, the MD/QCT model predicts approximately half the SO2 atmospheric dissociation due to O and O+ bombardment compared to TCE models, and also predicts a temperature rise due to plasma heating further from the Ionian surface than the existing baseline methodologies. These findings indicate that the accurate MD/QCT chemistry and collision models provide a significant improvement over the baseline models for DSMC simulations of the Ionian atmosphere. (C) 2014 Elsevier Inc. All rights reserved. C1 [Parsons, Neal; Levin, Deborah A.] Penn State Univ, Dept Aerosp Engn, University Pk, PA 16802 USA. [Walker, Andrew C.] Los Alamos Natl Lab, Intelligence & Space Res Div, Los Alamos, NM 87545 USA. [Moore, Chris H.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Goldstein, David B.; Varghese, Philip L.; Trafton, Laurence] Univ Texas Austin, Dept Aerosp Engn & Engn Mech, Austin, TX 78712 USA. RP Parsons, N (reprint author), Penn State Univ, Dept Aerosp Engn, 229 Hammond Bldg, University Pk, PA 16802 USA. EM nsp5088@psu.edu OI Walker, Andrew/0000-0002-7890-1779 FU NASA [NNG05G083G] FX This research was supported by NASA Grant NNG05G083G. NR 31 TC 2 Z9 2 U1 0 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD SEP 1 PY 2014 VL 239 BP 32 EP 38 DI 10.1016/j.icarus.2014.05.041 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM3WE UT WOS:000339782700004 ER PT J AU Lim, H Carroll, JD Battaile, CC Buchheit, TE Boyce, BL Weinberger, CR AF Lim, H. Carroll, J. D. Battaile, C. C. Buchheit, T. E. Boyce, B. L. Weinberger, C. R. TI Grain-scale experimental validation of crystal plasticity finite element simulations of tantalum oligocrystals SO INTERNATIONAL JOURNAL OF PLASTICITY LA English DT Article DE Crystal plasticity; Finite elements; Digital image correlation; Electron microscopy; Microstructures ID CENTERED-CUBIC METALS; CONSTRAINED SURFACE MICROSTRUCTURE; STRAIN-RATE DEPENDENCE; HIGH-PURITY NIOBIUM; SINGLE-CRYSTALS; ANOMALOUS SLIP; FLOW-STRESS; CRYSTALLOGRAPHIC TEXTURE; SCREW DISLOCATIONS; LATTICE FRICTION AB In this work, the grain-scale elastoplastic deformation behavior of coarse-grained body centered cubic (BCC) tantalum was simulated using a crystal plasticity finite element method (CP-FEM) and compared to experimental measurements of intragranular strain and rotation fields. To mitigate the effects of unknown subsurface microstructure, tantalum tensile specimens with millimeter-sized grains provided nearly constant microstructure through the thickness of the tensile bar. Experimental validation was performed in three ways: (1) electron backscatter diffraction (EBSD) to map intragranular rotation, (2) high-resolution digital image correlation (HR-DIC) to map the surface strain field, and (3) surface profilometry to map the out-of-plane topographic distortion. To ensure a direct apples-to-apples comparison to experiments, the details of the initial microstructure and boundary conditions were carefully replicated in the model. The deformation predictions using this novel BCC CP-FEM model for tantalum agree reasonably well with the experimental measurements. In addition, the model successfully predicted the failure location of a specimen subjected to large plastic strains. Several model parameters were explored that influence the BCC CP-FEM predictions such as the mesh dependence, the choice of active slip planes in BCC metals and the assignment of initial crystal orientations. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Lim, H.; Battaile, C. C.; Buchheit, T. E.] Sandia Natl Labs, Dept Computat Mat & Data Sci, Albuquerque, NM 87185 USA. [Carroll, J. D.; Boyce, B. L.] Sandia Natl Labs, Dept Met & Mat Joining, Albuquerque, NM 87185 USA. [Weinberger, C. R.] Drexel Univ, Dept Mech Engn & Mech, Philadelphia, PA 19104 USA. RP Lim, H (reprint author), Sandia Natl Labs, Dept Computat Mat & Data Sci, Albuquerque, NM 87185 USA. EM hnlim@sandia.gov RI Carroll, Jay/K-2720-2012 OI Carroll, Jay/0000-0002-5818-4709 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 85 TC 32 Z9 32 U1 8 U2 65 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0749-6419 EI 1879-2154 J9 INT J PLASTICITY JI Int. J. Plast. PD SEP PY 2014 VL 60 BP 1 EP 18 DI 10.1016/j.ijplas.2014.05.004 PG 18 WC Engineering, Mechanical; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA AM2RI UT WOS:000339698100001 ER PT J AU Juan, PA Berbenni, S Barnett, MR Tome, CN Capolungo, L AF Juan, P. -A. Berbenni, S. Barnett, M. R. Tome, C. N. Capolungo, L. TI A double inclusion homogenization scheme for polycrystals with hierarchal topologies: application to twinning in Mg alloys SO INTERNATIONAL JOURNAL OF PLASTICITY LA English DT Article DE Twinning; Magnesium; Micromechanics ID VISCOPLASTIC HETEROGENEOUS MATERIALS; FINITE-ELEMENT MODEL; SELF-CONSISTENT; NONLINEAR COMPOSITES; NEUTRON-DIFFRACTION; TEXTURE DEVELOPMENT; DEFORMATION; PLASTICITY; BEHAVIOR; METALS AB The present work introduces a double inclusion elasto-plastic self-consistent (DI-EPSC) scheme for topologies in which crystals can contain subdomains (i.e. twins, etc.). The approach yields a direct coupling between the mechanical response of grains and their subdomains via a concentration relationship on mean fields derived from both the Eshelby and the Tanaka-Mod properties. The latent effect caused by twinning on the mechanical response is observed on both initially extruded and non-textured Mg alloys. For twinned grains, it is shown that deformation system activities and plastic strain distributions within twins drastically depend on the interaction with parent domains. Moreover, a quantitative study on the coupled influence of secondary slip activities on the material response is proposed. (C) 2014 Published by Elsevier Ltd. C1 [Juan, P. -A.; Capolungo, L.] Georgia Inst Technol, GW Woodruff Sch Mech Engn, UMI GT CNRS 2958, Metz, France. [Juan, P. -A.; Berbenni, S.] Univ Lorraine, UMR CNRS 7239, LEM3, Metz, France. [Barnett, M. R.] Deakin Univ, CMFI, ARC Ctr Excellence Design Light Met, Geelong, Vic 3217, Australia. [Tome, C. N.] Los Alamos Natl Lab, MST 8, Los Alamos, NM 87545 USA. RP Capolungo, L (reprint author), Georgia Inst Technol, GW Woodruff Sch Mech Engn, UMI GT CNRS 2958, Metz, France. EM laurent.capolungo@me.gatech.edu RI Tome, Carlos/D-5058-2013 FU French State through the National Research Agency (ANR) [ANR-11-LABX-0008-01]; project MAGTWIN [ANR-12-BS09-0010-02]; Office of basic Energy Science [FWP 06SCPE401] FX P.-A. Juan and S. Berbenni would like to thank the support of the French State through the National Research Agency (ANR) under the program "Investment in the future" (Labex DAMAS referenced as ANR-11-LABX-0008-01) and the project MAGTWIN (referenced as ANR-12-BS09-0010-02) for its support. C. Tome and L. Capolungo were fully supported by Office of basic Energy Science, Project FWP 06SCPE401. NR 47 TC 15 Z9 15 U1 4 U2 33 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0749-6419 EI 1879-2154 J9 INT J PLASTICITY JI Int. J. Plast. PD SEP PY 2014 VL 60 BP 182 EP 196 DI 10.1016/j.ijplas.2014.04.001 PG 15 WC Engineering, Mechanical; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA AM2RI UT WOS:000339698100011 ER PT J AU Lopez-Yglesias, X Schrader, PE Michelsen, HA AF Lopez-Yglesias, Xerxes Schrader, Paul E. Michelsen, Hope A. TI Soot maturity and absorption cross sections SO JOURNAL OF AEROSOL SCIENCE LA English DT Article DE Soot; Thermal accommodation; Absorption; Cross section; Flame; LII ID LASER-INDUCED INCANDESCENCE; TURBULENT-DIFFUSION FLAMES; PRIMARY PARTICLE-SIZE; PREMIXED FLAT FLAME; LOW-FLUENCE LII; BLACK CARBON; LIGHT-ABSORPTION; VOLUME FRACTION; ACCOMMODATION COEFFICIENTS; WAVELENGTH DEPENDENCE AB We used time-resolved laser-induced incandescence (LID to compare optical and physical properties of soot at the edge and in the center of two co-flow diffusion flames in common use for soot optical-diagnostics development. We made these measurements over a wide range of laser fluences using a laser wavelength of either 532 or 1064 nm. Our results, combined with the previous results, suggest that the 532:1064 nm absorption cross-section ratio is <= 1.8 for mature soot and increases with increasing hydrogen content and decreasing soot maturity. The absolute absorption cross sections at 532 and 1064 nm, on the other hand, increase with soot maturity. Differences in the signal decay rates between center and edge regions further suggest that the thermal-accommodation coefficient decreases with increasing soot maturity. These results were analyzed using an energy- and mass-balance model that accounts for the effects of soot maturity on the absorption cross section, thermal-accommodation coefficient, and particle density. Given the sensitivity of LII to these parameters, it may be possible to use a combination of in situ measurements of pulsed LII fluence curves and temporal profiles to gain information about soot maturity. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Lopez-Yglesias, Xerxes; Schrader, Paul E.; Michelsen, Hope A.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Michelsen, HA (reprint author), Sandia Natl Labs, POB 969,MS 9055, Livermore, CA 94551 USA. EM hamiche@sandia.gov FU National Nuclear Security Administration [DE-AC04-94-AL85000]; Division of Chemical Sciences, Geosciences, and Biosciences; Office of Basic Energy Sciences; U.S. Department of Energy FX We thank Daniel Strong for the rendition of the experimental setup shown in Fig. 1 and Pascale Desgroux and Salma Bejaoui for helpful suggestions. This work was funded by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under Contract DE-AC04-94-AL85000. NR 103 TC 22 Z9 23 U1 6 U2 27 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0021-8502 EI 1879-1964 J9 J AEROSOL SCI JI J. Aerosol. Sci. PD SEP PY 2014 VL 75 BP 43 EP 64 DI 10.1016/j.jaerosci.2014.04.011 PG 22 WC Engineering, Chemical; Engineering, Mechanical; Environmental Sciences; Meteorology & Atmospheric Sciences SC Engineering; Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA AM2TN UT WOS:000339703800006 ER PT J AU Lloyd, JT Clayton, JD Austin, RA McDowell, DL AF Lloyd, J. T. Clayton, J. D. Austin, R. A. McDowell, D. L. TI Plane wave simulation of elastic-viscoplastic single crystals SO JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS LA English DT Article DE Single crystal; Micromechanics; High rate deformation; Viscoplasticity; Dislocations ID LITHIUM FLUORIDE CRYSTALS; HIGH-STRAIN RATES; CONSTITUTIVE MODEL; SHOCK-WAVE; DISLOCATION DENSITIES; ALUMINUM; PLASTICITY; DYNAMICS; METALS; COPPER AB Despite the large amount of research that has been performed to quantify the high strain rate response of Aluminum, few studies have addressed effects of crystal orientation and subsequent crystal-level microstructure evolution on its high strain rate response. To study orientation effects in single crystal Al, both a constitutive model and novel numerical method have been developed. A plane wave formulation is developed so that materials undergoing anisotropic viscoplastic deformation can be modeled in a thermodynamically consistent framework. Then, a recently developed high strain rate viscoplastic model is extended to include single crystal effects by incorporating higher order crystal-based thermoelasticity, anisotropic plasticity kinetics, and distinguishing influences of forest and parallel dislocation densities. Steady propagating shock waves are simulated for [100], [110], and [111] oriented single crystals and compared to existing experimental wave profile and strength measurements. Finally, influences of initial orientation and peak pressure ranging from 0 to 30 GPa are quantified. Results indicate that orientation plays a significant role in dictating the high rate response of both the wave profile and the resultant microstructure evolution of Al. The plane wave formulation can be used to evaluate microstructure-sensitive constitutive relations in a computationally efficient framework. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Lloyd, J. T.; McDowell, D. L.] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Lloyd, J. T.; Clayton, J. D.] US Army, Res Lab, Impact Phys Branch, RDRL WMP C, Aberdeen Proving Ground, MD 21005 USA. [Austin, R. A.] Lawrence Livermore Natl Lab, Mat Modeling & Simulat Grp, Livermore, CA 94550 USA. [McDowell, D. L.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. RP Lloyd, JT (reprint author), US Army, Res Lab, Impact Phys Branch, RDRL WMP C, Aberdeen Proving Ground, MD 21005 USA. EM jeff.lloyd@gatech.edu; john.d.clayton1.civ@mail.mil; austin28@llnl.gov; david.mcdowell@me.gatech.edu RI Austin, Ryan/J-9003-2014; Clayton, John/C-7760-2009 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Carter N. Paden, Jr. Distinguished Chair in Metals Processing FX This work performed, in part, under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. DLM gratefully acknowledges support of the Carter N. Paden, Jr. Distinguished Chair in Metals Processing. NR 70 TC 10 Z9 10 U1 1 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-5096 EI 1873-4782 J9 J MECH PHYS SOLIDS JI J. Mech. Phys. Solids PD SEP PY 2014 VL 69 BP 14 EP 32 DI 10.1016/j.jmps.2014.04.009 PG 19 WC Materials Science, Multidisciplinary; Mechanics; Physics, Condensed Matter SC Materials Science; Mechanics; Physics GA AM2RU UT WOS:000339699300004 ER PT J AU Reina, C Marian, J AF Reina, Celia Marian, Jaime TI Slip-induced conservation laws for dislocation structures in the finite kinematic framework SO JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS LA English DT Article DE Dislocation dynamics; Cross slip; Partial dislocations; Conservation laws; Large deformations ID MOLECULAR-DYNAMICS SIMULATIONS; DEFECTS; CRYSTALS; PLASTICITY; GEOMETRY AB In the present paper we develop a general framework that captures topological, geometric, and energetic aspects of slip surfaces to provide conservation laws for dislocation structures. In this work, dislocations act as the boundary of active slip regions that support a finite displacement jump, while treating the material outside the slip regions with a continuum mechanic framework in the setting of large deformations. Within this semicontinuous description, it is shown that the condition of slip imposes an important restriction on the shape of the slip surfaces regardless of the material structure. This catalog of shapes for the slip surfaces can be further restricted for crystalline materials, providing a simple geometric description of common dislocation processes such as cross slip or dislocation loop glide. In this setting, the classical Kirchhoff-type rule for the conservation of the Burgers vector emanates directly from the formulation, while recent conservation laws designed for partial dislocations in face centered cubic crystals are also naturally captured. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Reina, Celia; Marian, Jaime] Lawrence Livermore Natl Lab, Sci & Technol Principal Directorate, Livermore, CA 94551 USA. [Reina, Celia] Univ Penn, Dept Mech Engn & Appl Mech, Philadelphia, PA 19104 USA. RP Reina, C (reprint author), Univ Penn, Dept Mech Engn & Appl Mech, Philadelphia, PA 19104 USA. EM creina@seas.upenn.edu; marian1@llnl.gov FU Lawrence Fellowship program at Lawrence Livermore National Laboratory; DOE-OFES; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This paper feeds to a large degree from work and discussions with Pr. Sergio Conti regarding reference Reina and Conti (2014), which we gratefully acknowledge. C. Reina acknowledges support from the Lawrence Fellowship program at Lawrence Livermore National Laboratory. J. Marian acknowledges support from DOE-OFES Early Career Program. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 28 TC 1 Z9 1 U1 1 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-5096 EI 1873-4782 J9 J MECH PHYS SOLIDS JI J. Mech. Phys. Solids PD SEP PY 2014 VL 69 BP 123 EP 131 DI 10.1016/j.jmps.2014.04.013 PG 9 WC Materials Science, Multidisciplinary; Mechanics; Physics, Condensed Matter SC Materials Science; Mechanics; Physics GA AM2RU UT WOS:000339699300009 ER PT J AU Zhu, B Gutknecht, JLM Herman, DJ Keck, DC Firestone, MK Cheng, WX AF Zhu, Biao Gutknecht, Jessica L. M. Herman, Donald J. Keck, Daniel C. Firestone, Mary K. Cheng, Weixin TI Rhizosphere priming effects on soil carbon and nitrogen mineralization SO SOIL BIOLOGY & BIOCHEMISTRY LA English DT Article DE Rhizosphere priming effect; SOM decomposition; Gross nitrogen mineralization; Microbial biomass; Extracellular enzyme activity; Rhizosphere respiration ID ORGANIC-MATTER DECOMPOSITION; TEMPERATURE SENSITIVITY; ROOT EXUDATION; ELEVATED CO2; FOREST; RESPIRATION; FEEDBACKS; PLANT; RHIZODEPOSITION; AVAILABILITY AB Living roots and their rhizodeposits affect microbial activity and soil carbon (C) and nitrogen (N) mineralization. This so-called rhizosphere priming effect (RPE) has been increasingly recognized recently. However, the magnitude of the RPE and its driving mechanisms remain elusive. Here we investigated the RPE of two plant species (soybean and sunflower) grown in two soil types (a farm or a prairie soil) and sampled at two phenological stages (vegetative and mature stages) over an 88-day period in a greenhouse experiment. We measured soil C mineralization using a continuous C-13-labeling method, and quantified gross N mineralization with a N-15-pool dilution technique. We found that living roots significantly enhanced soil C mineralization, by 27-245%. This positive RPE on soil C mineralization did not vary between the two soils or the two phenological stages, but was significantly greater in sunflower compared to soybean. The magnitude of the RPE was positively correlated with rhizosphere respiration rate across all treatments, suggesting the variation of RPE among treatments was likely caused by variations in root activity and rhizodeposit quantity. Moreover, living roots stimulated gross N mineralization rate by 36-62% in five treatments, while they had no significant impact in the other three treatments. We also quantified soil microbial biomass and extracellular enzyme activity when plants were at the vegetative stage. Generally, living roots increased microbial biomass carbon by 0-28%, beta-glucosidase activity by 19-56%, and oxidative enzyme activity by 0-46%. These results are consistent with the positive rhizosphere effect on soil C (45-79%) and N (10-52%) mineralization measured at the same period. We also found significant positive relationships between beta-glucosidase activity and soil C mineralization rates and between oxidative enzyme activity and gross N mineralization rates across treatments. These relationships provide clear evidence for the microbial activation hypothesis of RPE. Our results demonstrate that root-soil-microbial interactions can stimulate soil C and N mineralization through rhizosphere effects. The relationships between the RPE and rhizosphere respiration rate and soil enzyme activity can be used for explicit representations of RPE in soil organic matter models. Published by Elsevier Ltd. C1 [Zhu, Biao; Gutknecht, Jessica L. M.; Keck, Daniel C.; Cheng, Weixin] Univ Calif Santa Cruz, Dept Environm Studies, Santa Cruz, CA 95064 USA. [Zhu, Biao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Gutknecht, Jessica L. M.] Univ Minnesota, Dept Soil Water & Climate, St Paul, MN 55108 USA. [Herman, Donald J.; Firestone, Mary K.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Keck, Daniel C.] Univ Calif Los Angeles, Environm Hlth & Safety Program, Los Angeles, CA 90095 USA. RP Zhu, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM biaozhu@gmail.com RI Cheng, Weixin/F-4968-2011; Zhu, Biao/F-8712-2010 OI Cheng, Weixin/0000-0003-2964-2376; Zhu, Biao/0000-0001-9858-7943 FU National Research Initiative of the U.S. Department of Agriculture's Cooperative State Research, Education and Extension Service [2006-35107-17225]; Division of Environmental Biology of the U.S. National Science Foundation [1354659] FX We thank Jowin Cheung and Ilya Yevdokimov for laboratory assistance, Joy Matthews and Dyke Andreasen for isotope analysis, and an anonymous reviewer for insightful comments on an earlier version of our manuscript. This study was supported by a grant from the National Research Initiative of the U.S. Department of Agriculture's Cooperative State Research, Education and Extension Service (#2006-35107-17225) and a grant from the Division of Environmental Biology of the U.S. National Science Foundation (#1354659). NR 56 TC 30 Z9 34 U1 31 U2 297 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-0717 J9 SOIL BIOL BIOCHEM JI Soil Biol. Biochem. PD SEP PY 2014 VL 76 BP 183 EP 192 DI 10.1016/j.soilbio.2014.04.033 PG 10 WC Soil Science SC Agriculture GA AM2QM UT WOS:000339695900023 ER PT J AU Dunbar, J Gallegos-Graves, L Steven, B Mueller, R Hesse, C Zak, DR Kuske, CR AF Dunbar, John Gallegos-Graves, La Verne Steven, Blaire Mueller, Rebecca Hesse, Cedar Zak, Donald R. Kuske, Cheryl R. TI Surface soil fungal and bacterial communities in aspen stands are resilient to eleven years of elevated CO2 and O-3 SO SOIL BIOLOGY & BIOCHEMISTRY LA English DT Article DE Elevated carbon dioxide; Ozone; Forest soil; Soil bacteria; Soil fungi; Metagenome ID ATMOSPHERIC CARBON-DIOXIDE; LONG-TERM EXPOSURE; TROPOSPHERIC O-3; TREMBLING ASPEN; FOREST SOIL; NORTHERN FORESTS; NITROGEN UPTAKE; PAPER BIRCH; PCR; PRODUCTIVITY AB Soil microbial community changes associated with altered carbon cycling dynamics were investigated in aspen (Populus tremuloides) stands exposed to elevated atmospheric CO2 (eCO(2)) and/or elevated ozone (eO(3)) for eleven years, at the Rhinelander Free Air CO2 Enrichment (FACE) experiment (Wisconsin, USA). The relative abundance and composition of fungal and bacterial communities in the 0-5 cm soil depth was evaluated using qPCR of fungal or bacterial rRNA genes, cloned 16S (bacterial) and LSU (fungal) rRNA gene sequencing, small subunit rRNA pyrosequencing, and soil shotgun metagenomes. Fungal or bacterial biomass, measured by qPCR, did not differ with treatment. Under eO(3), the ratio of Basidiomycota to Ascomycota significantly increased by two-fold (P < 0.04) relative to the ambient control, but no robust significant differences (P > 0.1) in the B diversity of fungal or bacterial communities were detected under eCO(2). The overall composition of fungal and bacterial communities was resilient despite substantial changes in plant productivity, plant genotype, root density, and rates of soil C and N cycling under eCO(2), documented in prior studies. Nonetheless, some candidate taxa (up to 20% of the total at the genus level) shifted in relative abundance in soils from eCO(2) plots, suggesting that although community composition was generally stable, it was not static. The eCO(2)-responsive taxa did not shift under eCO(2) plus eO(3) conditions, suggesting an interactive effect of eO(3) on the soil community. Our results show that the fungal and bacterial communities in the 0-5 cm depth mineral soil changed only in small ways after eleven years of eCO(2). This study reinforces the view that soil microbial community changes in ecosystems responding to global climate change drivers may be highly-localized in soil strata. Published by Elsevier Ltd. C1 [Dunbar, John; Gallegos-Graves, La Verne; Steven, Blaire; Mueller, Rebecca; Hesse, Cedar; Kuske, Cheryl R.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Zak, Donald R.] Univ Michigan, Sch Nat Resources & Environm, Ann Arbor, MI 48109 USA. [Zak, Donald R.] Univ Michigan, Dept Ecol & Evolutionary Biol, Ann Arbor, MI 48109 USA. RP Kuske, CR (reprint author), Los Alamos Natl Lab, Biosci Div, M888, Los Alamos, NM 87545 USA. EM kuske@lanl.gov FU U.S. Department of Energy (DOE); Office of Biological and Environmental Research (BER); Biological System Sciences Division [2009LANLF260]; BER Climate and Environmental Science Division FX This work was supported by the U.S. Department of Energy (DOE), Office of Biological and Environmental Research (BER), Biological System Sciences Division, through a Science Focus Area grant (2009LANLF260), as well as grants from the BER Climate and Environmental Science Division for infrastructure and science at the Rhinelander FACE Experiment. DNA sequencing for this study was provided by the DOE Joint Genome Institute and the Los Alamos National Laboratory LDRD program. NR 45 TC 4 Z9 5 U1 11 U2 99 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-0717 J9 SOIL BIOL BIOCHEM JI Soil Biol. Biochem. PD SEP PY 2014 VL 76 BP 227 EP 234 DI 10.1016/j.soilbio.2014.05.027 PG 8 WC Soil Science SC Agriculture GA AM2QM UT WOS:000339695900028 ER PT J AU Xu, YW Alexoff, DL Kunert, AT Qu, WC Kim, D Paven, M Babst, BA Ferrieri, RA Schueller, MJ Fowler, JS AF Xu, Youwen Alexoff, David L. Kunert, Anna T. Qu, Wenchao Kim, Dohyun Paven, Max Babst, Benjamin A. Ferrieri, Richard A. Schueller, Michael J. Fowler, Joanna S. TI Radiosynthesis of 3-indolyl[1-C-11]acetic acid for phyto-PET-imaging: An improved production procedure and formulation method SO APPLIED RADIATION AND ISOTOPES LA English DT Article DE 3-Indolyl[1-C-11]acetic acid; Phyto-PET-imaging; Formulation; Radiochemical yield; Specific activity ID AUXIN; C-11; TRANSPORT; CARBON; ROOTS; GROWTH AB An improved production procedure and formulation method for the carbon-11 radiolabeled phytohormone, 3-indolyl-[1-C-11]acetic acid ([C-11]IAA), was developed by modifying selected original reaction parameters. This updated procedure both doubled the yield (from 25.9 +/- 6.7% (n=12) to 61.0 +/- 0.3% (n=10)) and increased the concentration (0.2-0.4 GBq/0.15-0.3 mL), enabling us to provide the radiotracer [C-11]IAA suitable for in vivo phyto-PET-imaging studies. The specific activity was improved by more than a factor of three (26.7 +/- 5.6 GBq/mu mol to 82.5 +/- 36.1 GBq/mu mol). The total synthesis time for both production and formulation was 81.8 +/- 3.0 min (n=10). In addition, a streamlined semi-remote controlled production system, containing five processing modules, was designed and built for routine [C-11]IAA production. This integrated system facilitated routine high radiation level production of [C-11]IAA while minimizing radiation exposure to the production chemists. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Xu, Youwen; Alexoff, David L.; Kunert, Anna T.; Qu, Wenchao; Kim, Dohyun; Paven, Max; Babst, Benjamin A.; Ferrieri, Richard A.; Schueller, Michael J.; Fowler, Joanna S.] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. [Kunert, Anna T.; Paven, Max] Johannes Gutenberg Univ Mainz, Fachbereich Chem, D-55099 Mainz, Germany. RP Qu, WC (reprint author), Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. EM youwen@bnl.gov; alexoff@bnl.gov; akunert@students.uni-mainz.de; wqu@bnl.gov; dohkim@bnl.gov; m.paven@gmail.com; bbabst@bnl.gov; ferrieri@bnl.gov; mschueller@bnl.gov; fowler@bnl.gov FU Office of Biological and Environmental Research, U. S. Department of Energy [AC02-98CH10886]; German Academic Exchange Service (Deutscher Akademischer Austauschdienst, DAAD) Bonn FX This research was supported by the Office of Biological and Environmental Research, U. S. Department of Energy under Contract DE-AC02-98CH10886. Additional support was provided by the German Academic Exchange Service (Deutscher Akademischer Austauschdienst, DAAD) Bonn, which supported Anna T. Kunert and Max Paven. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States retains a non-exclusive, paid-up irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purpose. The authors thank Colleen Shea for editorial assistance. The authors also thanks to Colleen Shea, Lisa Muench, Carina Weber, and Sunny Kim for their helps in radiotracer production. NR 38 TC 3 Z9 3 U1 0 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD SEP PY 2014 VL 91 BP 155 EP 160 DI 10.1016/j.apradiso.2014.05.017 PG 6 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA AM0KA UT WOS:000339533300023 PM 24946093 ER PT J AU Reynaldo, G Biegalski, S Woods, V AF Reynaldo, Gomez Biegalski, Steven Woods, Vincent TI Aerosol sample inhomogeneity with debris from the Fukushima Daiichi accident SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Fukushima; Sample inhomogeneity; Aerosol sampling; Radionuclides; Cs-137; Cs-134 AB Radionuclide aerosol sampling is a vital component in the detection of nuclear explosions, nuclear accidents, and other radiation releases. This was proven by the detection and tracking of emissions from the Fukushima Daiichi incident across the globe by IMS stations. Two separate aerosol samplers were operated in Richland, WA following the event and debris from the accident were measured at levels well above detection limits. While the atmospheric activity concentration of radionuclides generally compared well between the two stations, they did not agree within uncertainties. This paper includes a detailed study of the aerosol sample homogeneity of Cs-134 and Cs-137, then relates it to the overall uncertainty of the original measurement. Our results show that sample inhomogeneity adds an additional 5 -10% uncertainty to each aerosol measurement and that this uncertainty is in the same range as the discrepancies between the two aerosol sample measurements from Richland, WA. Published by Elsevier Ltd. C1 [Reynaldo, Gomez; Biegalski, Steven] Univ Texas Austin, Nucl Engn Teaching Lab, Austin, TX 78712 USA. [Woods, Vincent] Pacific NW Natl Lab, Richland, WA USA. RP Reynaldo, G (reprint author), Univ Texas Austin, Nucl Engn Teaching Lab, 10100 Burnet Rd,Bldg 159, Austin, TX 78712 USA. EM gomez_rey09@yahoo.com; Biegalski@maiLutexas.edu; Vincent.woods@pnnl.gov NR 7 TC 0 Z9 0 U1 0 U2 6 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD SEP PY 2014 VL 135 BP 1 EP 5 DI 10.1016/j.jenvrad.2014.03.011 PG 5 WC Environmental Sciences SC Environmental Sciences & Ecology GA AM1JU UT WOS:000339603000001 ER PT J AU Eslinger, PW Napier, BA Anspaugh, LR AF Eslinger, Paul W. Napier, Bruce A. Anspaugh, Lynn R. TI Representative doses to members of the public from atmospheric releases of I-131 at the Mayak Production Association facilities from 1948 through 1972 SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Dose assessment; I-131; Airborne radioactivity; Population dose ID UNCERTAINTY AB Scoping epidemiology studies performed by researchers from the Southern Urals Biophysics Institute revealed an excess prevalence of thyroid nodules and an increased incidence of thyroid cancer among residents of Ozersk, Russia, who were born in the early 1950s. Ozersk is located about 5 km from the facilities where the Mayak Production Association produced nuclear materials for the Russian weapons program. Reactor operations began in June 1948 and chemical separation of plutonium from irradiated fuel began in February 1949. The U.S.-Russia Joint Coordinating Committee on Radiation Effects Research conducted a series of projects over a 10-year period to assess the radiation risks in the Southern Urals. This paper uses data collected under Committee projects to present examples of reconstructed time-dependent thyroid doses to reference individuals living in Ozersk from 1311 released to the atmosphere for all relevant exposure pathways. Between 3.22 x 10(16) and 4.31 x 10(16) Bq of I-131 may have been released during the 1948-1972 time period, and a best estimate is 3.76 x 10(16) Bq. In general, younger children incur greater thyroid doses from I-131 than adults. A child born in 1947 is estimated to have received a cumulative thyroid dose of 2.3 Gy for 1948-1972, with a 95% confidence interval of 0.51 -73 Gy. Annual doses were the highest in 1949 and a child who was 5 years old in 1949 is estimated to have a received an annual thyroid dose of 0.93 Gy with a 95% confidence interval of 0.19-3.5 Gy. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Eslinger, Paul W.; Napier, Bruce A.] Pacif NW Natl Lab, Richland, WA 99354 USA. [Anspaugh, Lynn R.] Univ Utah, Sch Med, Div Radiobiol, Salt Lake City, UT 84112 USA. RP Eslinger, PW (reprint author), Pacif NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99354 USA. EM paul.w.eslinger@pnnl.gov NR 21 TC 1 Z9 1 U1 1 U2 4 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD SEP PY 2014 VL 135 BP 44 EP 53 DI 10.1016/j.jenvrad.2014.04.003 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA AM1JU UT WOS:000339603000006 PM 24769389 ER PT J AU Atkinson, R Eddy, T Kuhne, W Jannik, T Brandl, A AF Atkinson, Robert Eddy, Teresa Kuhne, Wendy Jannik, Tim Brandl, Alexander TI Measurement of the tritium concentration in the fractionated distillate from environmental water samples SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Tritium analysis; Surface water samples; Vapor pressure isotope effect ID VAPOR-PRESSURES; EVAPORATION; EFFICIENCY; SYSTEMS; OXIDE AB Standard procedures for the measurement of tritium in water samples often require distillation of an appropriate sample aliquot. This distillation process may result in a fractionation of tritiated water and regular light water due to the vapor pressure isotope effect, introducing either a bias or an additional contribution to the total tritium measurement uncertainty. The current study investigates the relative change in vapor pressure isotope effect in the course of the distillation process, distinguishing it from and extending previously published measurements. The separation factor as a quantitative measure of the vapor pressure isotope effect is found to assume values of 1.04 +/- 0.036, 1.05 +/- 0.026, and 1.07 +/- 0.038, depending on the vigor of the boiling process during distillation of the sample. A lower heat setting in the experimental setup, and therefore a less vigorous boiling process, results in a larger value for the separation factor. For a tritium measurement in water samples where the first 5 mL are discarded, the tritium concentration could be underestimated by 4-7%. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Atkinson, Robert; Brandl, Alexander] Colorado State Univ, Environm & Radiol Hlth Sci, Ft Collins, CO 80523 USA. [Eddy, Teresa; Kuhne, Wendy; Jannik, Tim] Savannah River Nucl Solut, Savannah River Natl Lab, Aiken, SC 29808 USA. RP Brandl, A (reprint author), Colorado State Univ, Environm & Radiol Hlth Sci, 1618 Campus Delivery, Ft Collins, CO 80523 USA. EM Robert.Atkinson@wpafb.af.mil; Teresa.eddy@srni.doe.gov; Wendy.Kuhne@srni.doe.gov; Timjannik@srnl.doe.gov; Alexander.brandl@colostate.edu FU Savannah River Nuclear Solutions, LLC [DE-AC09-08SR22470]; U.S. Department of Energy FX This manuscript has been co-authored by Savannah River Nuclear Solutions, LLC under Contract No. DE-AC09-08SR22470 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting this article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for United States Government purposes. The work presented in this manuscript was prepared through the Savannah River National Laboratory's National Center for Radioecology (NCoRE). Neither the U.S. Government or its employees, nor any of its contractors, subcontractors or their employees, makes any express or implied: 1. warranty or assumes any legal liability for the accuracy, completeness, or for the use or results of such use of any information, product, or process disclosed; or 2. representation that such use or results of such use would not infringe privately owned rights; or 3. endorsement or recommendation of any specifically identified commercial product, process, or service. The opinions, findings, conclusions or recommendations expressed herein are those of the authors and do not necessarily represent the views of the Department of Energy, Savannah River National Laboratory or the key partners and member organizations of NCoRE. NR 19 TC 2 Z9 2 U1 3 U2 14 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD SEP PY 2014 VL 135 BP 113 EP 119 DI 10.1016/j.jenvrad.2014.04.012 PG 7 WC Environmental Sciences SC Environmental Sciences & Ecology GA AM1JU UT WOS:000339603000015 PM 24814721 ER PT J AU Yamaguchi, M Kitamura, A Oda, Y Onishi, Y AF Yamaguchi, Masaaki Kitamura, Akihiro Oda, Yoshihiro Onishi, Yasuo TI Predicting the long-term Cs-137 distribution in Fukushima after the Fukushima Dai-ichi nuclear power plant accident: a parameter sensitivity analysis SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Fukushima Dai-ichi nuclear power plant; Cs-137; Soil erosion; Transport ID SOIL-EROSION; SYSTEMS; MODEL AB Radioactive materials deposited on the land surface of Fukushima Prefecture from the Fukushima Daiichi Nuclear Power Plant explosion is a crucial issue for a number of reasons, including external and internal radiation exposure and impacts on agricultural environments and aquatic biota. Predicting the future distribution of radioactive materials and their fates is therefore indispensable for evaluation and comparison of the effectiveness of remediation options regarding human health and the environment. Cesium-137, the main radionuclide to be focused on, is well known to adsorb to clay-rich soils; therefore its primary transportation mechanism is in the form of soil erosion on the land surface and transport of sediment-sorbed contaminants in the water system. In this study, we applied the Soil and Cesium Transport model, which we have developed, to predict a long-term cesium distribution in the Fukushima area, based on the Universal Soil Loss Equation and simple sediment discharge formulas. The model consists of calculation schemes of soil erosion, transportation and deposition, as well as cesium transport and its future distribution. Since not all the actual data on parameters is available, a number of sensitivity analyses were conducted here to find the range of the output results due to the uncertainties of parameters. The preliminary calculation indicated that a large amount of total soil loss remained in slope, and the residual sediment was transported to rivers, deposited in rivers and lakes, or transported farther downstream to the river mouths. Most of the sediment deposited in rivers and lakes consists of sand. On the other hand, most of the silt and clay portions transported to river were transported downstream to the river mouths. The rate of sediment deposition in the Abukuma River basin was three times as high as those of the other 13 river basins. This may be due to the larger catchment area and more moderate channel slope of the Abukuma River basin than those of the other rivers. Annual sediment outflows from the Abukuma River and the total from the other 13 river basins were calculated as 3.2 x 10(4)-3.1 x 10(5) and 3.4 x 10(4)-2.1 x 10(5) t y(-1), respectively. The values vary between calculation cases because of the critical shear stress, the rainfall factor, and other differences. On the other hand, contributions of those parameters were relatively small for Cs-137 concentration within transported soil. This indicates that the total amount of Cs-137 outflow into the ocean would mainly be controlled by the amount of soil erosion and transport and the total amount of Cs-137 concentration remaining within the basin. Outflows of Cs-137 from the Abukuma River and the total from the other 13 river basins during the first year after the accident were calculated to be 2.3 x 10(11)-3.7 x 10(12) and 4.6 x 10(11)-.6.5 x 10(12) Bq y(-1), respectively. The former results were compared with the field investigation results, and the order of magnitude was matched between the two, but the value of the investigation result was beyond the upper limit of model prediction. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Yamaguchi, Masaaki; Kitamura, Akihiro; Oda, Yoshihiro] Japan Atom Energy Agcy, Radoact Waste Proc & Disposal Res Dept, Ibaraki 3191194, Japan. [Kitamura, Akihiro; Oda, Yoshihiro] Japan Atom Energy Agcy, Fukushima Environm Safety Ctr, Fukushima 9608034, Japan. [Onishi, Yasuo] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Yamaguchi, M (reprint author), Japan Atom Energy Agcy, Radoact Waste Proc & Disposal Res Dept, 4-33 Muramatsu Tokai mura, Ibaraki 3191194, Japan. EM yamaguchi.masaaki@jaea.go.jp NR 38 TC 13 Z9 13 U1 7 U2 63 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD SEP PY 2014 VL 135 BP 135 EP 146 DI 10.1016/j.jenvrad.2014.04.011 PG 12 WC Environmental Sciences SC Environmental Sciences & Ecology GA AM1JU UT WOS:000339603000018 PM 24836353 ER PT J AU Szecsody, JE Jansik, DP McKinley, JP Hess, NJ AF Szecsody, Jim E. Jansik, Danielle P. McKinley, James P. Hess, Nancy J. TI Influence of alkaline co-contaminants on technetium mobility in vadose zone sediments SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Technetium; Subsurface contamination; Alkaline dissolution/precipitation; Pertechnetate reduction ID X-RAY-ABSORPTION; TANK WASTE PLUMES; EXTRACTION TECHNIQUES; CONTAMINATED AQUIFER; SUBSURFACE SEDIMENTS; ESTUARINE SEDIMENTS; HIGHLY ALKALINE; FERROUS IRON; PERTECHNETATE; REDUCTION AB Pertechnetate was slowly reduced in a natural, untreated arid sediment under anaerobic conditions (0.02 nmol g(-1) h(-1)), which could occur in low permeability zones in the field, most of which was quickly oxidized. A small portion of the surface Tc may be incorporated into slowly dissolving surface phases, so was not readily oxidized/remobilized into pore water. In contrast, pertechnetate reduction in an anaerobic sediment containing adsorbed ferrous iron as the reductant was rapid (15-600 nmol g(-1) h(-1)), and nearly all (96-98%) was rapidly oxidized/remobilized (2.6-6.8 nmol g(-1) h(-1)) within hours. Tc reduction in an anaerobic sediment containing 0.5-10 mM sulfide showed a relatively slow reduction rate (0.01-0.03 nmol g(-1) h(-1)) that was similar to observations in the natural sediment. Pertechnetate infiltration into sediment with a highly alkaline water resulted in rapid reduction (0.07-0.2 nmol g h(-1)) from ferrous iron released during biotite or magnetite dissolution. Oxidation of NaOH-treated sediments resulted in slow Tc oxidation (similar to 0.05 nmol g(-1) h(-1)) of a small fraction of the surface Tc (13-23%). The Tc remaining on the surface was Tc-IV (by XANES), and autoradiography and elemental maps of Tc (by electron microprobe) showed Tc was present associated with specific minerals, rather than being evenly distributed on the surface. Dissolution of quartz, montmorillonite, muscovite, and kaolinite also occurred in the alkaline water, resulting in significant aqueous silica and aluminum. Over time, aluminosilicates, cancrinite, zeolite and sodalite were precipitating. These precipitates may be coating surface Tc(IV) phases, limiting reoxidation. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Szecsody, Jim E.; McKinley, James P.; Hess, Nancy J.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Jansik, Danielle P.] Washington State Dept Ecol, Yakima, WA USA. RP Szecsody, JE (reprint author), Pacific NW Natl Lab, POB 999,MSIN K3-61, Richland, WA 99354 USA. EM jim.szecsody@pnnl.gov; daja461@ecy.wa.gov; james.mckinley@pnnl.gov; nancy.hess@pnnl.gov OI Hess, Nancy/0000-0002-8930-9500 FU Subsurface Biogeochemical Remediation Program, U.S. Department of Energy; Deep Vadose Zone-Applied Field Research Initiative, Richland Operations Office, U.S. Department of Energy; U.S. Department of Energy [DE-AC06-76RLO 1830] FX This work was supported by the Subsurface Biogeochemical Remediation Program, U.S. Department of Energy and the Deep Vadose Zone-Applied Field Research Initiative, Richland Operations Office, U.S. Department of Energy. Micro-XAS data were collected at the Advanced Photon Source (APS), which is operated by the Department of Energy (DOE), Office of Basic Energy Sciences. The authors thank Dr. S.M. Heald for his assistance at the Advanced Photon Source (APS). Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy under Contract DE-AC06-76RLO 1830. NR 75 TC 5 Z9 5 U1 2 U2 26 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD SEP PY 2014 VL 135 BP 147 EP 160 DI 10.1016/j.jenvrad.2014.02.003 PG 14 WC Environmental Sciences SC Environmental Sciences & Ecology GA AM1JU UT WOS:000339603000019 PM 24814749 ER PT J AU Choi, J Um, W Choung, S AF Choi, Jongkwon Um, Wooyong Choung, Sungwook TI Development of iron phosphate ceramic waste form to immobilize radioactive waste solution SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID SALT WASTE; POTASSIUM; STABILIZATION/SOLIDIFICATION; FUEL AB The objective of this research was to develop an iron phosphate ceramic (IPC) waste form using converter slag obtained as a by-product of the steel industry as a source of iron instead of conventional iron oxide. Both synthetic off-gas scrubber solution containing technetium-99 (or Re as a surrogate) and LiCl-KCl eutectic salt, a final waste solution from pyrochemical processing of spent nuclear fuel, were used as radioactive waste streams. The IPC waste form was characterized for compressive strength, reduction capacity, chemical durability, and contaminant leachability. Compressive strengths of the IPC waste form prepared with different types of waste solutions were 16 MPa and 19 MPa for LiCl-KCl eutectic salt and the off-gas scrubber simulant, respectively, which meet the minimum compressive strength of 3.45 MPa (500 psi) for waste forms to be accepted into the radioactive waste repository. The reduction capacity of converter slag, a main dry ingredient used to prepare the IPC waste form, was 4136 meq/kg by the Ce(IV) method, which is much higher than those of the conventional Fe oxides used for the IPC waste form and the blast furnace slag materials. Average leachability indexes of Tc, Li, and K for the IPC waste form were higher than 6.0, and the IPC waste form demonstrated stable durability even after 63-day leaching. In addition, the Toxicity Characteristic Leach Procedure measurements of converter slag and the IPC waste form with LiCl-KCl eutectic salt met the universal treatment standard of the leachability limit for metals regulated by the Resource Conservation and Recovery Act. This study confirms the possibility of development of the IPC waste form using converter slag, showing its immobilization capability for radionuclides in both LiCl-KCl eutectic salt and off-gas scrubber solutions with significant cost savings. Published by Elsevier B.V. C1 [Choi, Jongkwon; Um, Wooyong; Choung, Sungwook] Pohang Univ Sci & Technol POSTECH, Div Adv Nucl Engn, Pohang, South Korea. [Um, Wooyong] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Um, W (reprint author), Pacific NW Natl Lab, POB 999,Mail Stop P7-54, Richland, WA 99354 USA. EM wooyong.um@pnnl.gov FU World Class University (WCU) Program through the National Research Foundation of Korea - Ministry of Education, Science and Technology [R31-30005]; BK21+ Program through the National Research Foundation of Korea (NRF) - Ministry of Education, Science and Technology FX This work was supported by World Class University (WCU) (R31-30005) and BK21+ Programs through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology. The authors appreciate the help of the Environmental Sciences Laboratory staffs at Pacific Northwest National Laboratory for conducting sample analysis and testing. NR 30 TC 1 Z9 2 U1 5 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 16 EP 23 DI 10.1016/j.jnucmat.2014.04.033 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200004 ER PT J AU Han, WZ Mara, NA Wang, YQ Misra, A Demkowicz, MJ AF Han, W. Z. Mara, N. A. Wang, Y. Q. Misra, A. Demkowicz, M. J. TI He implantation of bulk Cu-Nb nanocomposites fabricated by accumulated roll bonding SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID NANOLAYERED COMPOSITES; MULTILAYER COMPOSITES; HIGH-STRENGTH; INTERFACES; BUBBLE; MECHANISMS; REDUCTION; FILMS AB We perform room temperature and elevated temperature He implantation of bulk Cu-Nb nanocomposites synthesized by accumulated roll bonding (ARB). Transmission electron microscopy (TEM) reveals that nanoscale He precipitates form preferentially along Cu-Nb interfaces during implantation at 20 degrees C and 450 degrees C. Bubble-free zones may be identified near interfaces after implantation at 450 degrees C. He implantation at 480 degrees C results in large, faceted cavities in thick Cu layers and highly elongated cavities in thin Cu layers. Only nanoscale bubbles are seen in Nb layers after implantation at 480 degrees C. Similar to vapor deposited Cu-Nb multilayers, ARB Cu-Nb nanocomposites exhibit He precipitate morphologies that are highly sensitive to implantation temperature and layer thickness. (C) 2014 Elsevier B. V. All rights reserved. C1 [Han, W. Z.] Xi An Jiao Tong Univ, Ctr Adv Mat Performance Nanoscale, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. [Han, W. Z.; Mara, N. A.; Misra, A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Wang, Y. Q.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Demkowicz, M. J.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP Han, WZ (reprint author), Xi An Jiao Tong Univ, Ctr Adv Mat Performance Nanoscale, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. EM wzhanmail@gmail.com RI Han, Weizhong/C-9963-2011; Misra, Amit/H-1087-2012; Mara, Nathan/J-4509-2014; xjtu, campnano/Q-1904-2015 FU Center for Materials in Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center (EFRC) - US Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; XJTU, China FX This work was supported by the Center for Materials in Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center (EFRC) funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. 2008LANL1026. WZH was partially supported by the new faculty start-up funding from XJTU, China. WZH also acknowledges I.J. Beyerlein for fruitful discussion as well as E. G. Fu and J. Zhang for their assistance with the He implantation. NR 29 TC 8 Z9 8 U1 3 U2 68 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 57 EP 60 DI 10.1016/j.jnucmat.2014.04.034 PG 4 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200011 ER PT J AU He, JC Wan, FR Sridharan, K Allen, TR Certain, A Wu, YQ AF He, Jianchao Wan, Farong Sridharan, Kumar Allen, Todd R. Certain, A. Wu, Y. Q. TI Response of 9Cr-ODS steel to proton irradiation at 400 degrees C SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID FERRITIC ALLOYS; ION-IRRADIATION; OXIDE PARTICLES; ATOM-PROBE; ODS STEEL; DISPERSION; STABILITY; NANOCLUSTERS; SEGREGATION; EVOLUTION AB The stability of Y-Ti-O nanoclusters, dislocation structure, and grain boundary segregation in 9Cr-ODS steels has been investigated following proton irradiation at 400 degrees C with damage levels up to 3.7 dpa. A slight coarsening and a decrease in number density of nanoclusters were observed as a result of irradiation. The composition of nanoclusters was also observed to change with a slight increase of Y and Cr concentration in the nanoclusters following irradiation. Size, density, and composition of the nanoclusters were investigated as a function of nanocluster size, specifically classified to three groups. In addition to the changes in nanoclusters, dislocation loops were observed after irradiation. Finally, radiation-induced enrichment of Cr and depletion of W were observed at grain boundaries after irradiation. (C) 2014 Elsevier B. V. All rights reserved. C1 [He, Jianchao; Wan, Farong] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. [He, Jianchao; Sridharan, Kumar; Allen, Todd R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Allen, Todd R.] EG&G Idaho Inc, Idaho Natl Engn Lab, Idaho Falls, ID 83401 USA. [Certain, A.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Wu, Y. Q.] Boise State Univ, Dept Mat Sci & Engn, Boise, ID 83725 USA. [Wu, Y. Q.] Ctr Adv Energy Studies, Idaho Falls, ID 83401 USA. RP He, JC (reprint author), Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. EM hjch1985@gmail.com OI Allen, Todd/0000-0002-2372-7259 FU DOE Office of Nuclear Energy's Nuclear Energy University Programs; National Magnetic Confinement Fusion Program of China [2011GB108002]; National Natural Science Foundation of China [50971030] FX Samples of APT prepared by FIB and APT analysis were performed at the Center for Advanced Energy Studies (CAES) in Idaho Falls, Idaho through the Advanced Test Reactor National Scientific User Facility (ATR NSUF). This work was performed in part using the NSF-supported shared facilities at the University of Wisconsin. This research was performed using funding from the DOE Office of Nuclear Energy's Nuclear Energy University Programs. Additional support was provided by the National Magnetic Confinement Fusion Program of China with Grant No. 2011GB108002 and the National Natural Science Foundation of China with Grant No. 50971030. NR 35 TC 7 Z9 7 U1 0 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 87 EP 94 DI 10.1016/j.jnucmat.2014.05.004 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200015 ER PT J AU Chakraborty, P Tonks, MR Pastore, G AF Chakraborty, Pritam Tonks, Michael R. Pastore, Giovanni TI Modeling the influence of bubble pressure on grain boundary separation and fission gas release SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID UO2 FUEL; FACE BUBBLES; LWR FUEL; DENSITY; STRESS; BURNUP; CRACK AB Grain boundary (GB) separation as a mechanism for fission gas release (FGR), complementary to gas bubble interlinkage, has been experimentally observed in irradiated light water reactor fuel. However there has been limited effort to develop physics-based models incorporating this mechanism for the analysis of FGR. In this work, a computational study is carried out to investigate GB separation in UO2 fuel under the effect of gas bubble pressure and hydrostatic stress. A non-dimensional stress intensity factor formula is obtained through 2D axisymmetric analyses considering lenticular bubbles and Mode-I crack growth. The obtained functional form can be used in higher length-scale models to estimate the contribution of GB separation to FGR. Published by Elsevier B.V. C1 [Chakraborty, Pritam; Tonks, Michael R.; Pastore, Giovanni] EG&G Idaho Inc, Idaho Natl Engn Lab, Idaho Falls, ID 83401 USA. RP Chakraborty, P (reprint author), EG&G Idaho Inc, Idaho Natl Engn Lab, 2525 Fremont Ave, Idaho Falls, ID 83401 USA. EM pritam.chakraborty@inl.gov OI Pastore, Giovanni/0000-0003-2812-506X FU DOE Nuclear Energy Advanced Modeling and Simulation Program FX This work was funded by the DOE Nuclear Energy Advanced Modeling and Simulation Program. NR 37 TC 4 Z9 4 U1 1 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 95 EP 101 DI 10.1016/j.jnucmat.2014.04.023 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200016 ER PT J AU Usov, IO Dickerson, RM Dickerson, PO Byler, DD McClellan, KJ AF Usov, I. O. Dickerson, R. M. Dickerson, P. O. Byler, D. D. McClellan, K. J. TI Uranium dioxide films with xenon filled bubbles for fission gas behavior studies SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID HIGH BURNUP UO2; TRANSMISSION ELECTRON-MICROSCOPY; THIN-FILMS; FUEL; GROWTH; XE; IRRADIATION; MECHANISMS; DEPOSITION; DIFFUSION AB Electron beam evaporation and ion beam assisted deposition (IBAD) methods were utilized to fabricate depleted UO2 films and UO2 films with embedded Xe atoms, respectively. The films were fabricated at elevated temperature of 700 degrees C and also subsequently annealed at 1000 degrees C to induce grain growth and Xe atom redistribution. The goal of this work was to synthesize reference UO2 samples with controlled microstructures and Xe-filled bubble morphologies, without the effects attendant to rector irradiation-induced fission. Transmission electron microscopy (TEM) microstructural characterization revealed that fine Xe-filled bubbles nucleated in the as grown films and subsequent annealing resulted in noticeable bubble size increase. Reported results demonstrate the great potential IBAD techniques and UO2 films have for various areas of nuclear materials studies. (C) 2014 Elsevier B.V. All rights reserved. C1 [Usov, I. O.; Dickerson, R. M.; Dickerson, P. O.; Byler, D. D.; McClellan, K. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Usov, IO (reprint author), Los Alamos Natl Lab, Mailstop E549, Los Alamos, NM 87545 USA. EM iusov@lanl.gov FU US Department of Energy Advanced Fuel Cycle Campaign and Fuel Cycle RD Program FX This work was supported by the US Department of Energy Advanced Fuel Cycle Campaign and Fuel Cycle R&D Program. TEM analysis was performed at the Electron Microscopy Laboratory (EML) at LANL. NR 32 TC 0 Z9 0 U1 1 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 173 EP 177 DI 10.1016/j.jnucmat.2014.04.050 PG 5 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200026 ER PT J AU Riley, BJ Schweiger, MJ Kim, DS Lukens, WW Williams, BD Iovin, C Rodriguez, CP Overman, NR Bowden, ME Dixon, DR Crum, JV McCloy, JS Kruger, AA AF Riley, Brian J. Schweiger, Michael J. Kim, Dong-Sang Lukens, Wayne W., Jr. Williams, Benjamin D. Iovin, Cristian Rodriguez, Carmen P. Overman, Nicole R. Bowden, Mark E. Dixon, Derek R. Crum, Jarrod V. McCloy, John S. Kruger, Albert A. TI Iodine solubility in a low-activity waste borosilicate glass at 1000 degrees C SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID RHENIUM; XANES; IMMOBILIZATION; SPECIATION; EXAFS AB The purpose of this study was to determine the solubility of iodine in a low-activity waste borosilicate glass when heated inside an evacuated and sealed fused quartz ampoule. The iodine was added to glass frit as KI in quantities of 99.4-24,005 ppm iodine (by mass). Each mixture was added to an ampoule, heated at 1000 degrees C for 2 h, and then air quenched. In samples with >= 11,999 ppm iodine, low viscosity salt phases were observed on the surface of the melts that solidified into a white coating upon cooling. These salts were identified by X-ray diffraction as mixtures of KI, NaI, and Na2SO4. Iodine concentrations in glass specimens were analyzed with inductively-coupled plasma mass spectrometry, and the overall iodine solubility was determined to be 10,000 ppm. Several crystalline inclusions of iodine sodalite, Na-8(AlSiO4)(6)I-2, were observed in the 24,005 ppm specimen. (C) 2014 Elsevier B.V. All rights reserved. C1 [Riley, Brian J.; Schweiger, Michael J.; Kim, Dong-Sang; Williams, Benjamin D.; Iovin, Cristian; Rodriguez, Carmen P.; Overman, Nicole R.; Bowden, Mark E.; Dixon, Derek R.; Crum, Jarrod V.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Lukens, Wayne W., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [McCloy, John S.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Kruger, Albert A.] US DOE, Off River Protect, Richland, WA 99352 USA. RP Riley, BJ (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM brian.riley@pnnl.gov OI Riley, Brian/0000-0002-7745-6730 FU U.S. Department of Energy's (DOE) Waste Treatment and Immobilization Plant Project of the Office of River Protection; DOE [DE-AC05-76RL01830]; DOE's Office of Biological and Environmental Research; Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy's (DOE) Waste Treatment and Immobilization Plant Project of the Office of River Protection. The authors thank Clyde Chamberlin and Shelley Carlson for helping prepare the specimens for analyses as well as David Pierce, Jesse Lang, and Steven Luksic for their optical microscopy documentation. Pacific Northwest National Laboratory (PNNL) is operated by Battelle Memorial Institute for the DOE under contract DE-AC05-76RL01830. A portion of the research was performed using capabilities in the William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. Portions of this work were performed at Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for DOE's Office of Science by Stanford University. NR 39 TC 7 Z9 7 U1 0 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 178 EP 188 DI 10.1016/j.jnucmat.2014.04.027 PG 11 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200027 ER PT J AU Zhang, YF Millett, PC Tonks, MR Bai, XM Biner, SB AF Zhang, Yongfeng Millett, Paul C. Tonks, Michael R. Bai, Xian-Ming Biner, S. Bulent TI Molecular dynamics simulations of intergranular fracture in UO2 with nine empirical interatomic potentials SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID SINTERED URANIUM-DIOXIDE; HIGH-TEMPERATURES; SURFACE-ENERGY; FUEL PELLETS; DEFORMATION; STRENGTH; MICROSTRUCTURE; CLUSTERS; METALS; FCC AB The intergranular fracture behavior of UO2 was studied using molecular dynamics simulations with a bicrystal model. The anisotropic fracture behavior due to the different grain boundary characters was investigated with the < 100 > symmetrical tilt Sigma 5 and the < 110 > symmetrical tilt Sigma 3 ({111} twin) grain boundaries. Nine interatomic potentials, seven rigid-ion plus two core-shell ones, were utilized to elucidate possible potential dependence. Initiating from a notch, crack propagation along grain boundaries was observed for most potentials. The Sigma 3 boundary was found to be more prone to fracture than the Sigma 5 one, indicated by a lower energy release rate associated with the former. However, some potential dependence was identified on the existence of transient plastic deformation at crack tips, and the results were discussed regarding the relevant material properties including the excess energies of metastable phases and the critical energy release rate for intergranular fracture. In general, local plasticity at crack tips was observed in fracture simulations with potentials that predict low excess energies for metastable phases and high critical energy release rates for intergranular fracture. (C) 2014 Elsevier B.V. All rights reserved. C1 [Zhang, Yongfeng; Tonks, Michael R.; Bai, Xian-Ming; Biner, S. Bulent] Idaho Natl Lab, Fuels Modeling & Simulat Dept, Idaho Falls, ID 83415 USA. [Millett, Paul C.] Univ Arkansas, Dept Mech Engn, Fayetteville, AR 72701 USA. RP Zhang, YF (reprint author), Idaho Natl Lab, Fuels Modeling & Simulat Dept, Idaho Falls, ID 83415 USA. EM yongfeng.zhang@inl.gov RI Bai, Xianming/E-2376-2017 OI Bai, Xianming/0000-0002-4609-6576 FU DOE Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program, under the Fuels Integrated Performance and Safety Code (IPSC) project [FTLA11MS0603]; Battelle Energy Alliance, LLC [DE-AC07-05ID14517]; U.S. Department of Energy FX The authors gratefully acknowledge the support of the DOE Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program, under the Fuels Integrated Performance and Safety Code (IPSC) project with work Package No. FTLA11MS0603. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 51 TC 4 Z9 4 U1 3 U2 32 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 296 EP 303 DI 10.1016/j.jnucmat.2014.05.034 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200043 ER PT J AU White, JT Nelson, AT Byler, DD Valdez, JA McClellan, KJ AF White, J. T. Nelson, A. T. Byler, D. D. Valdez, J. A. McClellan, K. J. TI Thermophysical properties of U3Si to 1150 K SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID THERMAL-CONDUCTIVITY; HEAT-CAPACITY; URANIUM SILICIDE; LOW-TEMPERATURES; FLASH METHOD; U-SI; ALLOYS; DIFFUSIVITY AB U3Si has the highest uranium density of the U-Si compounds, making it an attractive option for specialized reactor applications. Although the compound has been used in research and test reactors for nearly six decades, little data has been published in the literature which characterizes the thermophysical properties at elevated temperatures. A systematic study was conducted on U3Si to characterize thermal expansion, heat capacity, thermal diffusivity, and thermal conductivity as a function of temperature to 1150 K. Thermophysical properties were also tabulated for the high temperature delta'-U3Si phase as a function of temperature, which has not been reported previously. (C) 2014 Elsevier B.V. All rights reserved. C1 [White, J. T.; Nelson, A. T.; Byler, D. D.; Valdez, J. A.; McClellan, K. J.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP White, JT (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. EM jtwhite@lanl.gov FU U.S. Department of Energy, Office of Nuclear Energy Fuel Cycle Research and Development program; U.S. Department of Energy FX The support of the U.S. Department of Energy, Office of Nuclear Energy Fuel Cycle Research and Development program is gratefully acknowledged. This work was performed at Los Alamos National Laboratory under the auspices of the U.S. Department of Energy. NR 31 TC 9 Z9 10 U1 1 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 304 EP 310 DI 10.1016/j.jnucmat.2014.05.037 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200044 ER PT J AU Courty, O Motta, AT Hales, JD AF Courty, Olivier Motta, Arthur T. Hales, Jason D. TI Modeling and simulation of hydrogen behavior in Zircaloy-4 fuel cladding SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID MECHANICAL-PROPERTIES; TEMPERATURE GRADIENT; ZIRCONIUM ALLOYS; ALPHA-PHASE; SOLUBILITY; HYDRIDE; REDISTRIBUTION; DIFFUSION; TRANSPORT; HEAT AB As a result of corrosion during normal operation in nuclear reactors, hydrogen can enter the zirconium-alloy fuel cladding and precipitate as brittle hydride platelets, which can severely degrade the cladding ductility. Under a heterogeneous temperature distribution, hydrides tend to accumulate in the colder areas, creating local spots of degraded cladding that can favor crack initiation. Therefore, an estimation of the local hydride distribution is necessary to help predict the risk of cladding failure. The hydride distribution is governed by three competing phenomena. Hydrogen in solid solution diffuses under a concentration gradient due to Fick's law and under a temperature gradient due to the Soret effect. Precipitation of the hydride platelets occurs once the hydrogen solubility limit is reached. A model of these phenomena was implemented in the 3D fuel performance code BISON in order to calculate the hydrogen distribution for arbitrary geometries, such as a nuclear fuel rod, and is now available for BISON users. Simulations have been performed on simple geometries to validate the model and its implementation. The simulations predict that before precipitation occurs, hydrogen tends to accumulate in the colder spots due to the Soret effect. Once the solubility limit is reached, hydrogen precipitates and forms a rim close to the outer edge of the cladding. The simulations also predict that the reactor shut down has little effect on already precipitated hydrides but causes the remaining hydrogen to precipitate homogeneously into hydrides. (C) 2014 Published by Elsevier B.V. C1 [Courty, Olivier] Penn State Univ, F-75017 Paris, France. [Motta, Arthur T.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Hales, Jason D.] Idaho Natl Lab, Fuels Modeling & Simulat Dept, Idaho Falls, ID USA. RP Motta, AT (reprint author), Penn State Univ, Dept Mech & Nucl Engn, 227 Reber Bldg, University Pk, PA 16802 USA. EM o.courty@gmail.com; atm2@psu.edu; jason.hales@inl.gov OI Hales, Jason/0000-0003-0836-0476 FU DOE NEUP project of US Department of Energy [11-2987]; US Government [DE-AC07-05ID14517] FX This research was funded by DOE NEUP project 11-2987 of the US Department of Energy. This work is the result of collaborative project between Penn State University and the Idaho National Laboratory, which also includes Maria Avramova (PSU), Ian Davis (PSU), Kostadin Ivanov (PSU) and Richard Williamson (INL). We would like to thank Matthew Lindenberg for his help in configuring BISON. We would also like to thank Kevin Cass for his assistance in the analysis of the results during his Toshiba-Westinghouse Undergraduate Fellows program internship at Penn State.; The submitted manuscript has been authored by a contractor of the US Government under Contract DE-AC07-05ID14517. Accordingly, the US Government retains a non-exclusive, royalty free license to publish or reproduce the published form of this contribution, or allow others to do so, for US Government purposes. NR 38 TC 5 Z9 5 U1 3 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 311 EP 320 DI 10.1016/j.jnucmat.2014.05.013 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200045 ER PT J AU Chen, Y Jiao, L Sun, C Song, M Yu, KY Liu, Y Kirk, M Li, M Wang, H Zhang, X AF Chen, Y. Jiao, L. Sun, C. Song, M. Yu, K. Y. Liu, Y. Kirk, M. Li, M. Wang, H. Zhang, X. TI In situ studies of radiation induced crystallization in Fe/a-Y2O3 nanolayers SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID Y2O3 THIN-FILMS; ION IRRADIATION TOLERANCE; SWIFT HEAVY-IONS; HE ION; PHASE-TRANSFORMATION; FERRITIC/MARTENSITIC STEELS; DAMAGE PRODUCTION; MULTILAYERS; SIZE; COMPOSITES AB Oxide dispersion strengthened ferritic alloys have superior radiation tolerance and thus become appealing candidates as fuel cladding materials for next generation nuclear reactors. In this study we constructed a model system, Fe/Y2O3 nanolayers with individual layer thicknesses of 10 and 50 nm, in order to understand their radiation response and corresponding damage mitigation mechanisms. These nanolayers were subjected to in situ Kr ion irradiation at room temperature up to similar to 8 displacements-per-atom. As-deposited Y2O3 layers had primarily amorphous structure. Radiation induced prominent nanocrystallization and grain growth in 50 nm thick Y2O3 layers. Conversely, little crystallization occurred in 10 nm thick Y2O3 layers implying size dependent enhancement of radiation tolerance. In situ video also captured grain growth in both Fe and Y2O3 and outstanding morphological stability of layer interfaces against Kr ion irradiation. (C) 2014 Elsevier B.V. All rights reserved. C1 [Chen, Y.; Jiao, L.; Song, M.; Yu, K. Y.; Liu, Y.; Wang, H.; Zhang, X.] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Sun, C.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Kirk, M.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Li, M.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Wang, H.] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Zhang, X.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. RP Zhang, X (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. EM zhangx@tamu.edu RI Liu, Yue/H-4071-2014; Wang, Haiyan/P-3550-2014; Yu, Kaiyuan /B-8398-2014; Chen, Youxing/P-5006-2016 OI Liu, Yue/0000-0001-8518-5734; Wang, Haiyan/0000-0002-7397-1209; Yu, Kaiyuan /0000-0002-5442-2992; Chen, Youxing/0000-0003-1111-4495 FU NSF [DMR-1304101]; DOE-OBES FX We acknowledge financial support by NSF DMR-1304101. Accesses to DOE-Center for Integrated Nanotechnologies (CINT) at Los Alamos and Sandia National Laboratories and microscopy and imaging center (MIC) at Texas A&M University are also acknowledged. We also thank Edward A. Ryan and Peter M. Baldo at Argonne National Laboratory for their help during in situ experiments. The IVEM facility at Argonne National Laboratory is supported by DOE-OBES. NR 47 TC 17 Z9 17 U1 3 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 321 EP 327 DI 10.1016/j.jnucmat.2014.05.046 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200046 ER PT J AU Chen, TY Chen, D Sencer, BH Shao, L AF Chen, Tianyi Chen, Di Sencer, Bulent H. Shao, Lin TI Molecular dynamics simulations of grain boundary thermal resistance in UO2 SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID NONSTOICHIOMETRIC URANIUM-DIOXIDE; THERMOPHYSICAL PROPERTIES; NUCLEAR-FUELS; CONDUCTIVITY; POTENTIALS AB By means of molecular dynamics (MD) simulations, we have calculated Kaptiza resistance of UO2 with or without radiation damage. For coincident site lattice boundaries of different configurations, the boundary thermal resistance of unirradiated UO2 can be well described by a parameter-reduced formula by using boundary energies as variables. We extended the study to defect-loaded UO2 by introducing damage cascades in close vicinity to the boundaries. Following cascade annealing and defect migrations toward grain boundaries, the boundary energy increases and so does Kaptiza resistance. The correlations between these two still follow the same formula extracted from the unirradiated UO2. The finding will benefit multi-scale modeling of UO2 thermal properties under extreme radiation conditions by combining effects from boundary configurations and damage levels. (C) 2014 Elsevier B. V. All rights reserved. C1 [Chen, Tianyi; Chen, Di; Shao, Lin] Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. [Sencer, Bulent H.] Idaho Natl Lab, Mat & Nucl Fuels Dept, Idaho Falls, ID 83415 USA. RP Shao, L (reprint author), Texas A&M Univ, Dept Nucl Eng, 335 Zachry, College Stn, TX 77843 USA. EM lshao@tamu.edu OI Chen, Tianyi/0000-0003-2880-824X FU US Department of Energy under DOE-NE Idaho Operations Office [DE-AC07-05ID14517]; National Science Foundation (US) [CMMI-0846835] FX We acknowledge the Texas A&M Supercomputing Facility (http://sc.tamu.edu/) for providing computing resources useful in conducting the research reported in this paper. This work was supported by the US Department of Energy under DOE-NE Idaho Operations Office Contract DE-AC07-05ID14517. LS acknowledges the support from National Science Foundation (US) under Grant No. CMMI-0846835. NR 31 TC 8 Z9 8 U1 1 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 364 EP 369 DI 10.1016/j.jnucmat.2014.05.035 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200052 ER PT J AU McMurray, JW Shin, D Slone, BW Besmann, TM AF McMurray, J. W. Shin, D. Slone, B. W. Besmann, T. M. TI Thermodynamic reassessment of U-Gd-O system SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID RARE-EARTH-OXIDES; HEAT-CAPACITY MEASUREMENTS; TOTAL-ENERGY CALCULATIONS; OXYGEN PHASE-DIAGRAM; WAVE BASIS-SET; URANIUM-DIOXIDE; SOLID-SOLUTIONS; TEMPERATURE; UO2; NONSTOICHIOMETRY AB The CALPHAD approach is used to describe the thermodynamic properties and phase relations in the U-Gd-O system. A compound energy formalism (CEF) model is developed for the U1-yGdyO2 (+/-) (x) phase that includes the introduction of a U6+ cation to better reproduce the phase equilibria. The lattice stability for a fictive gadolinium oxide fluorite structure compound is calculated from density functional theory (DFT) for use in the model for U1-yGdyO2 (+/-) (x). A Gibbs function is proposed for the stoichiometric UGd6O12 compound and the partially ionic liquid sublattice model is used to represent the liquid phase. Reported experimental thermodynamic and phase equilibria data were then used in optimizations to develop representations of the phases in the system. These will be able to be extended to include other actinide and fission products to develop multi-component models within the CALPHAD framework. The models developed in this assessment well reproduce the reported phase relations for the U-Gd-O system. The computed oxygen potentials from the CEF for U1-yGdyO2 (+/- x) are in good agreement with experimentally determined values. (C) 2014 Elsevier B. V. All rights reserved. C1 [McMurray, J. W.; Shin, D.; Slone, B. W.; Besmann, T. M.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Besmann, TM (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM besmanntm@ornl.gov RI Shin, Dongwon/C-6519-2008; OI Shin, Dongwon/0000-0002-5797-3423; McMurray, Jacob/0000-0001-5111-3054 FU US Department of Energy, Office of Nuclear Energy Fuel Cycle Technology Program FX The authors would like to thank Stewart Voit and Dane Wilson for helpful comments. The work was supported by the US Department of Energy, Office of Nuclear Energy Fuel Cycle Technology Program. NR 63 TC 12 Z9 12 U1 3 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 397 EP 406 DI 10.1016/j.jnucmat.2014.04.047 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200057 ER PT J AU Field, KG Gussev, MN Busby, JT AF Field, Kevin G. Gussev, Maxim N. Busby, Jeremy T. TI Microstructural characterization of deformation localization at small strains in a neutron-irradiated 304 stainless steel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID AUSTENITIC STAINLESS-STEEL; CLEARED CHANNELS; PURE COPPER; MECHANISMS; ORIGIN; 316-STAINLESS-STEEL; TRANSFORMATION; PROPAGATION; NUCLEATION; BOUNDARIES AB A specific phenomenon - highly localized regions of deformation - was found and investigated at the free surface and near-surface layer of a neutron irradiated AISI 304 stainless steel bend specimen deformed to a maximum surface strain of 0.8%. It was shown that local plastic deformation near the surface might reach significant levels being localized at specific spots even when the maximum free surface strain remains below 1%. The effect was not observed in non-irradiated steel of the same composition at similar strain levels. Cross-sectional EBSD analysis demonstrated that the local misorientation level was highest near the free surface and diminished with increasing depth in these regions. (S)TEM indicated that the local density of dislocation channels might vary up to an order of magnitude. These channels may contain twins or may be twin free depending on grain orientation and local strain levels. BCC-phase (alpha-martensite) formation associated with channel-grain boundary intersection points was observed using EBSD and STEM in the near-surface layer. (C) 2014 Elsevier B. V. All rights reserved. C1 [Field, Kevin G.; Gussev, Maxim N.; Busby, Jeremy T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Field, KG (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, POB 2008, Oak Ridge, TN 37831 USA. EM fieldkg@ornl.gov; gussevmn@ornl.gov; busbyjt@ornl.gov RI Field, Kevin/K-1942-2013 OI Field, Kevin/0000-0002-3105-076X FU U.S. Department of Energy, Office of Nuclear Energy; Scientific User Facilities Division, Office of Basic Energy Sciences; U.S. Department of Energy; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was sponsored by the U.S. Department of Energy, Office of Nuclear Energy, for the Light Water Reactor Sustainability Research and Development Effort, and the SHaRE User Facility, sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, and the U.S. Department of Energy. The authors would like to thank Dr. C. M. Parish and Dr. T. S. Byun from Oak Ridge National Laboratory (ORNL) for their fruitful discussions on the results and D. P. Stevens (ORNL) for assisting in preparations of this manuscript.; This manuscript has been authored by the Oak Ridge National Laboratory, managed by UT-Battelle LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. NR 35 TC 3 Z9 3 U1 1 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 500 EP 508 DI 10.1016/j.jnucmat.2014.05.053 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200073 ER PT J AU Couet, A Motta, AT de Gabory, B Cai, ZH AF Couet, Adrien Motta, Arthur T. de Gabory, Benoit Cai, Zhonghou TI Microbeam X-ray Absorption Near-Edge Spectroscopy study of the oxidation of Fe and Nb in zirconium alloy oxide layers SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT Conference on Nuclear Materials (NuMat) CY OCT 22-25, 2012 CL Osaka, JAPAN ID HIGH-TEMPERATURE WATER; IN-REACTOR CORROSION; ZR-BASED ALLOYS; SYNCHROTRON-RADIATION; HYDROGEN UPTAKE; ZIRCALOY-4; IRON; SOLUBILITY; INTERFACE; EVOLUTION AB Alloy optimization of zirconium based alloys used for nuclear fuel cladding is key to increasing corrosion resistance and reducing hydrogen pickup. The mechanism by which alloying elements influence these processes is investigated by focusing on the chemical state evolution of two alloying elements, Fe and Nb, when incorporated into the growing oxide layers of various production zirconium alloys Zircaloy-4, ZIRLO (R) and Zr-2.5Nb - as well as a model alloy -Zr-0.4Fe-0.2Cr. X-ray Absorption Near-Edge Spectroscopy (XANES) measurements to determine the evolution of their oxidation states is performed using micro-beam synchrotron radiation on cross sectional oxide samples. A thin (similar to 12 mu m) cross-sectional sample of Zircaloy-4 oxide was also designed and fabricated to differentiate the signal coming from the Fe in solid solution from the signal coming from the Fe in precipitates. The XANES spectra were fitted using a combination of standards, to determine the evolution of the oxidized fractions of Fe and Nb in the oxide as function of distance from the oxide/metal interface. The results show that the oxidation of Fe and Nb in the oxide layer is delayed relative to that of Zr. Both the second phase precipitates and solid solution Fe atoms were initially incorporated in metallic form into the oxide layer, although it appears that Fe in solid solution oxidizes first. It is shown that after a given distance from the metal/oxide interface (which is alloy dependent), the alloying elements start to oxidize. Qualitative TEM examinations of precipitates embedded in zirconium oxide layers correlate well with the quantitative XANES results. These results allow a discussion of a qualitative oxidation model of Fe and Nb in Zr alloys. (C) 2014 Elsevier B.V. All rights reserved. C1 [Couet, Adrien; Motta, Arthur T.; de Gabory, Benoit] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Cai, Zhonghou] Argonne Natl Lab, Adv Photon Source, XFD B3194 401, Argonne, IL 60439 USA. RP Couet, A (reprint author), Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. EM adrien.couet@gmail.com NR 43 TC 8 Z9 8 U1 2 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 614 EP 627 DI 10.1016/j.jnucmat.2014.05.047 PG 14 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200086 ER PT J AU Thompson, AE Meredig, B Stan, M Wolverton, C AF Thompson, Alexander E. Meredig, Bryce Stan, Marius Wolverton, C. TI Interatomic potential for accurate phonons and defects in UO2 (vol 446, pg 155, 2014) SO JOURNAL OF NUCLEAR MATERIALS LA English DT Correction C1 [Thompson, Alexander E.; Meredig, Bryce; Wolverton, C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Stan, Marius] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Wolverton, C (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM c-wolverton@northwestern.edu RI Wolverton, Christopher/B-7542-2009 NR 1 TC 0 Z9 0 U1 0 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2014 VL 452 IS 1-3 BP 634 EP 634 DI 10.1016/j.jnucmat.2014.05.056 PG 1 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AM2CU UT WOS:000339657200089 ER PT J AU Inabinett, D Knight, T Adams, T Gray, J AF Inabinett, D. Knight, T. Adams, T. Gray, J. TI Study of XeF2 fluorination potential against Rh2O3, RuO2, ZrO2, and U3O8 for use in reactive gas recycle of used nuclear fuel SO PROGRESS IN NUCLEAR ENERGY LA English DT Article DE Xenon difluoride; TGA; Reactive gas recycle; Reprocessing; Fluorination; Used nuclear fuel ID SYSTEM AB Triuranium octoxide (U3O8) and stable surrogate oxides of selected fission product species representative of a Used Nuclear Fuel (UNF) matrix typical of Light Water Reactor (LWR) service were fluorinated using an alternate, solid-phase fluorinating agent, XeF2. This fluorination reaction formed volatile and non-volatile compounds and demonstrated the possibility of chemical and thermal separations of the UNF matrix based on this approach. A series of experiments was conducted at the milligram quantity scale using a Shimadzu DTG-60 TG/DTA for testing of all non-radioactive samples and a Netzsch STA 409 TGA for testing of all radioactive samples. The fluorination and subsequent volatilization potentials were analyzed by mixing excess fluorinating agent with an oxide form of the UNF material and then heating to elevated temperatures for analysis. Thermogravimetric and differential thermal analysis allowed reaction pathways to be analyzed and suggested windows both thermally and chemically for separations of these various components. The differences in thermophysical properties of these products can be utilized as a starting point to effectively separate, isolate, and collect product streams with different compositions for further processing. The study of these chemistries could be incorporated into advanced separations methods to provide another possible solution for the long-term sustainability of nuclear energy applications. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Inabinett, D.; Knight, T.] Univ S Carolina, Columbia, SC 29208 USA. [Adams, T.; Gray, J.] Savannah River Natl Lab, Aiken, SC USA. RP Knight, T (reprint author), Univ S Carolina, 300 Main St, Columbia, SC 29208 USA. EM inabined@gmail.com; twknight@sc.edu FU National Academy for Nuclear Training (NANT) FX Thanks are given to SRNL's internship program which allowed Dillon Inabinett to join the RGR research team and complete this research. The authors would also like to thank the National Academy for Nuclear Training (NANT) in providing a fellowship to fund Dillon Inabinett in his pursuit of a Master's Degree. NR 8 TC 2 Z9 2 U1 0 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0149-1970 J9 PROG NUCL ENERG JI Prog. Nucl. Energy PD SEP PY 2014 VL 76 BP 106 EP 111 DI 10.1016/j.pnucene.2014.05.012 PG 6 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AM1IQ UT WOS:000339600000011 ER PT J AU Perusquia, R Montes-Tadeo, JL Ortiz-Servin, JJ Oliver, A Perry, RT AF Perusquia, Raul Montes-Tadeo, Jose-Luis Jose Ortiz-Servin, Juan Oliver G, Alicia Perry, Robert T. TI Modified Bi-parametric Method for optimization of BWR fuel reload patterns SO PROGRESS IN NUCLEAR ENERGY LA English DT Article DE BWR reactor; Fuel reload pattern; Optimization ID BOILING WATER-REACTOR; EXPERT-SYSTEM; DESIGN; ALGORITHM AB In this paper, a Modified Bi-parametric Method for optimization of fuel reload patterns of the Laguna Verde Nuclear Power Plant BWR reactors is presented. This method is a modification of Bi-parametric Method developed by D.P. Burte and Vaidya. The BWR reactors of LVNPP operate under a reactivity control system that is not compatible with the original Bi-parametric Method. A computer code, MAPATES, was developed which utilized the Modified Bi-parametric Method. The MAPATES code is used to generate reload patterns for Cycle 4-Unit 1 of the LVNPP. The reload patterns were generated using reactor quarter core symmetry. Without varying neither number nor characteristic of reload fuel assemblies; the MAPATES code generated a reload pattern that extended the cycle length reference loading pattern by 16 full-power operation days. It was also made a comparison against two other approaches to solve the same reload pattern, MBM overcame these approaches. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Perusquia, Raul; Montes-Tadeo, Jose-Luis; Jose Ortiz-Servin, Juan] Inst Nacl Invest Nucl ININ, Ocoyoacac 52750, Edo De Mexico, Mexico. [Oliver G, Alicia] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 01000, DF, Mexico. [Perry, Robert T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Montes-Tadeo, JL (reprint author), Inst Nacl Invest Nucl ININ, Carr Mexico Toluca S-N,Km 36-5, Ocoyoacac 52750, Edo De Mexico, Mexico. EM raul.perusquia@inin.gob.mx; joseluis.montes@inin.gob.mx; juanjose.ortiz@inin.gob.mx; oliver@fisica.unam.mx; rtperry@lanl.gov FU Consejo Nacional de Ciencia y Tecnologia of Mexico [CB-2011-01-168722]; Instituto Nacional de Investigaciones Nucleares, Mexico [CA-215]; Departamento de Gestion de Combustible of the Comision Federal de Electricidad of Mexico FX The authors acknowledge the support given by Consejo Nacional de Ciencia y Tecnologia of Mexico through the research project CB-2011-01-168722, to Instituto Nacional de Investigaciones Nucleares, Mexico through the research project CA-215 and to Departamento de Gestion de Combustible of the Comision Federal de Electricidad of Mexico. NR 16 TC 2 Z9 2 U1 0 U2 1 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0149-1970 J9 PROG NUCL ENERG JI Prog. Nucl. Energy PD SEP PY 2014 VL 76 BP 255 EP 268 DI 10.1016/j.pnucene.2014.05.024 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AM1IQ UT WOS:000339600000023 ER PT J AU Fontes, CJ Zhang, HL AF Fontes, Christopher J. Zhang, Hong Lin TI Relativistic distorted-wave collision strengths for the 49 Delta n=0 optically allowed transitions with n=2 in the 67 N-like ions with 26 <= Z <= 92 SO ATOMIC DATA AND NUCLEAR DATA TABLES LA English DT Article DE Electron-impact excitation collision strengths; Relativistic distorted-wave theory; Nitrogen-like ions; Improved top-up method ID HIGHLY-CHARGED IONS; ELECTRON-IMPACT EXCITATION; B-LIKE IONS; POSSIBLE N=2-N=3 TRANSITIONS; C-LIKE IONS; OSCILLATOR-STRENGTHS; ATOMIC DATA; IRON PROJECT; 8-LESS-THAN-OR-EQUAL-TO-Z-LESS-THAN-OR-EQUAL-TO-92; INCLUSION AB Relativistic distorted-wave collision strengths have been calculated for the 49 Delta n = 0 optically allowed transitions with n = 2 in the 67 N-like ions with nuclear charge number Z in the range 26 <= Z <= 92. The calculations were made for the four final, or scattered, electron energies E' = 0.20, 0.42, 0.80, and 1.40, where E' is in units of Z(eff)(2) Ry with Z(eff) = Z - 5. In the present calculations, an improved "top-up" method, which employs relativistic plane waves, was used to obtain the high partial-wave contribution for each transition, in contrast to the partial-relativistic Coulomb-Bethe approximation used in the previous work by Zhang and Sampson [H.L. Zhang and D.H. Sampson, At. Data Nucl. Data Tables 72 (1999) 153]. In that earlier work, collision strengths were also provided for N-like ions, but for a more comprehensive data set consisting of all possible 105 Delta n = 0 transitions, six scattered energies and the 81 ions with Z in the range 12 <= Z <= 92. The collision strengths covered in the present work should be more accurate than the corresponding data given by Zhang and Sampson [H.L. Zhang,and D.H. Sampson, At. Data Nucl. Data Tables 72 (1999) 153] and are presented here to replace those earlier results. (C) 2014 Elsevier Inc. All rights reserved. C1 [Fontes, Christopher J.; Zhang, Hong Lin] Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. RP Fontes, CJ (reprint author), Los Alamos Natl Lab, Computat Phys Div, POB 1663, Los Alamos, NM 87545 USA. EM cjf@lanl.gov FU U.S. Department of Energy by Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work was performed under the auspices of the U.S. Department of Energy by Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 37 TC 4 Z9 4 U1 0 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0092-640X EI 1090-2090 J9 ATOM DATA NUCL DATA JI Atom. Data Nucl. Data Tables PD SEP PY 2014 VL 100 IS 5 BP 1292 EP 1321 DI 10.1016/j.adt.2014.02.002 PG 30 WC Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA AL9JX UT WOS:000339458500007 ER PT J AU Abughayada, C Dabrowski, B Avdeev, M Kolesnik, S Remsen, S Chmaissem, O AF Abughayada, C. Dabrowski, B. Avdeev, M. Kolesnik, S. Remsen, S. Chmaissem, O. TI Structural, magnetic, and oxygen storage properties of hexagonal Dy1-xYxMnO3+delta SO JOURNAL OF SOLID STATE CHEMISTRY LA English DT Article DE Hexagonal-manganites; Oxygen storage capacity; Structural properties; Magnetic properties ID CRYSTAL-STRUCTURE; PEROVSKITES; MANGANITES; OXIDES AB Single-phase polycrystalline samples of hexagonal Dy1-xYxMnO3+delta were synthesized over the full solubility range under reducing oxygen partial pressure conditions. Rietveld refinements using neutron powder diffraction data (NPD) confirmed the persistence of the parent hexagonal P(63)cm (Space group #185) structure for all the stoichiometric (delta=0) samples. The (Mn-O) bond lengths derived from NPD data were found to be consistent with non-degenerate Mn+3 high-spin state e"2 e'2 in trigonalbipyramidal coordination. Detailed thermogravimetric measurements show large reversible oxygen storage/release capabilities (within the range of oxygen content 3.0-3.3) at unusually low temperatures of 200-400 degrees C in air or oxygen atmospheres. A phase transition to a new hexagonal phase (Hexl) was observed to take place around 5-0.29 for the oxygen-loaded Dy-rich samples (x < 0.5). Analysis of x-ray and neutron diffraction data using Rietveld refinements demonstrate that the superstructure is formed by tripling the c-axis of the original P63cm unit cell. Modeling of the Hexl superstructure converged to a structural symmetry consistent with the noncentrosymmetric space group R3c (#161). In magnetization measurements, a ferrimagnetic order for DyMn03.0 was observed below 8 K. The dilution of Dy magnetism with nonmagnetic yttrium results in reducing both the transition temperature and the effective paramagnetic moment. (C) 2014 Elsevier Inc. All rights reserved. C1 [Abughayada, C.; Dabrowski, B.; Kolesnik, S.; Remsen, S.; Chmaissem, O.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Dabrowski, B.; Chmaissem, O.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Avdeev, M.] Australian Nucl Sci & Technol Org, Sydney, NSW, Australia. RP Abughayada, C (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. EM castro.gha@gmail.com FU Northern Illinois University FX This work was supported by the Great Journeys assistantship, Northern Illinois University. NR 30 TC 7 Z9 7 U1 1 U2 18 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-4596 EI 1095-726X J9 J SOLID STATE CHEM JI J. Solid State Chem. PD SEP PY 2014 VL 217 BP 127 EP 135 DI 10.1016/j.jssc.2014.05.017 PG 9 WC Chemistry, Inorganic & Nuclear; Chemistry, Physical SC Chemistry GA AL5BP UT WOS:000339148800018 ER PT J AU O'Malley, D Vesselinov, VV Cushman, JH AF O'Malley, D. Vesselinov, V. V. Cushman, J. H. TI A Method for Identifying Diffusive Trajectories with Stochastic Models SO JOURNAL OF STATISTICAL PHYSICS LA English DT Article DE Anomalous diffusion; Model identification; Polymer; E. coli; Gulf of Mexico ID PARTICLE TRACKING VELOCIMETRY; ANOMALOUS DIFFUSION; DYNAMICS; DISPERSION; MEDIA AB Single particle tracking is a tool that is being increasingly used to study diffusive or dispersive processes in many branches of natural science. Often the ability to collect these trajectories experimentally or produce them numerically outpaces the ability to understand them theoretically. On the other hand many stochastic models have been developed and continue to be developed capable of capturing complex diffusive behavior such as heavy tails, long-range correlations, nonstationarity, and combinations of these things. We describe a computational method for connecting particle trajectory data with stochastic models of diffusion. Several tests are performed to demonstrate the efficacy of the method, and the method is applied to polymer diffusion, RNA diffusion in E. coli, and RAFOS dispersion in the Gulf of Mexico. C1 [O'Malley, D.; Vesselinov, V. V.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Cushman, J. H.] Purdue Univ, Dept Earth Atmospher & Planetary Sci & Math, W Lafayette, IN 47907 USA. RP O'Malley, D (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM omalled@lanl.gov RI Vesselinov, Velimir/P-4724-2016; OI Vesselinov, Velimir/0000-0002-6222-0530; O'Malley, Daniel/0000-0003-0432-3088 FU NSF [EAR 1314828] FX The authors wish to thank two anonymous reviewers for feedback that substantially improved the manuscript. DO and VVV wish to acknowledge the Environmental Programs Directorate of the Los Alamos National Laboratory; the Advanced Simulation Capability for Environmental Management (ASCEM) project, Department of Energy, Environmental Management; and the Integrated Multifaceted Approach to Mathematics at the Interfaces of Data, Models, and Decisions (DiaMonD) project, Department of Energy, Office of Science. JHC wishes to acknowledge NSF Grant #EAR 1314828. The authors wish to thank Ido Golding and Edward C. Cox for the RNA data as well as BOEMRE for the Gulf of Mexico float data. NR 46 TC 5 Z9 5 U1 0 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-4715 EI 1572-9613 J9 J STAT PHYS JI J. Stat. Phys. PD SEP PY 2014 VL 156 IS 5 BP 896 EP 907 DI 10.1007/s10955-014-1035-6 PG 12 WC Physics, Mathematical SC Physics GA AL7UX UT WOS:000339342600004 ER PT J AU du Can, SD Leventis, G Phadke, A Gopal, A AF du Can, Stephane de la Rue Leventis, Greg Phadke, Amol Gopal, Anand TI Design of incentive programs for accelerating penetration of energy-efficient appliances SO ENERGY POLICY LA English DT Article DE Energy efficiency; Incentive; Program design; Energy saving obligations; DSM AB Incentives are policy tools that sway purchase, retail stocking, and production decisions toward energy-efficient products. Incentives complement mandatory standards and labeling policies by accelerating market penetration of products that are more energy efficient than required by existing standards and by preparing the market for more stringent future mandatory requirements. Incentives can be directed at different points in the appliance's supply chain; one point may be more effective than another depending on the technology's maturity and market penetration. This paper seeks to inform future policy and program design by categorizing the main elements of incentive programs from around the world. We identify advantages and disadvantages of program designs through a qualitative overview of incentive programs worldwide. We find that financial incentive programs have greater impact when they target highly efficient technologies with a small market share, and that program designs depend on the market barriers addressed, the target equipment, and the local market context. No program design is inherently superior to another. The key to successful program design and implementation is a thorough understanding of the market and identification of the most important local obstacles to the penetration of energy-efficient technologies. (C) 2014 The Authors. Published by Elsevier Ltd. C1 [du Can, Stephane de la Rue; Leventis, Greg; Phadke, Amol; Gopal, Anand] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Int Energy Studies Grp, Berkeley, CA 94720 USA. RP du Can, SD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Int Energy Studies Grp, 1 Cyclotron Rd,Mail Stop 90R2002, Berkeley, CA 94720 USA. EM sadelarueducan@lbl.gov FU Bureau of Oceans and International Environmental and Scientific Affairs, U.S. Department of State; U.S. Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank Gabrielle Dreyfus and Chad Gallinat of the U.S. Department of Energy as well as Matthew Wittenstein previously at the U.S. Department of Energy and now at the International Energy Agency for providing significant and thoughtful input during the period of this study. We would like to extend our gratitude to all the reviewers that provided insightful comments and input. This work was funded by the Bureau of Oceans and International Environmental and Scientific Affairs, U.S. Department of State, and administered by the U.S. Department of Energy in support of the Super-efficient Equipment and Appliance Deployment (SEAD) Initiative through the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Any errors or omissions are the authors' own. NR 84 TC 9 Z9 9 U1 1 U2 21 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD SEP PY 2014 VL 72 BP 56 EP 66 DI 10.1016/j.enpol.2014.04.035 PG 11 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA AL0LA UT WOS:000338817200006 ER PT J AU Bates, EA Driscoll, MJ Lester, RK Arnold, BW AF Bates, E. A. Driscoll, M. J. Lester, R. K. Arnold, B. W. TI Can deep boreholes solve America's nuclear waste problem? SO ENERGY POLICY LA English DT Article DE Deep borehole disposal; Nuclear waste policy; Geological repository ID DRILLING PROGRAM KTB; CONTINENTAL-CRUST; DISPOSAL; FLUIDS; BASEMENT; GEOLOGY; AGES AB The United States is in need of a new and more adaptive long-term strategy for spent nuclear fuel. In this communication, we outline the fundamental reasons why deep borehole disposal should receive more detailed investigation, alongside traditional shallow mined repositories. This potential solution is supported by advancing drilling technologies and an improving understanding of extremely long fluid residence times in deep bedrock. Radionuclide isolation is supported by verifiable and stable geologic barriers such as long transport distances to aquifers, low permeability, and reducing chemical conditions. The modular nature of implementing deep borehole disposal could offer unique programmatic and economic advantages. Experience with a pilot borehole program will be required to confirm the feasibility of drilling and emplacement operations, and key chemical and hydraulic conditions. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Bates, E. A.; Driscoll, M. J.; Lester, R. K.] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Arnold, B. W.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Bates, EA (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave,NW-12-220, Cambridge, MA 02139 USA. EM eabates@mit.edu FU DOE/Sandia National Laboratories; Nuclear Energy University Programs (NEUP) grant FX Work at MIT on this subject has been supported by DOE/Sandia National Laboratories, and most recently under a Nuclear Energy University Programs (NEUP) grant. NR 41 TC 4 Z9 4 U1 2 U2 30 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD SEP PY 2014 VL 72 BP 186 EP 189 DI 10.1016/j.enpol.2014.03.003 PG 4 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA AL0LA UT WOS:000338817200019 ER PT J AU Woo, CK Ho, T Shiu, A Cheng, YS Horowitz, I Wang, J AF Woo, C. K. Ho, T. Shiu, A. Cheng, Y. S. Horowitz, I. Wang, J. TI Residential outage cost estimation: Hong Kong SO ENERGY POLICY LA English DT Article DE Residential outage cost estimation; Electricity reliability in Hong Kong; Contingent valuation survey ID WILLINGNESS-TO-PAY; AVOID POWER OUTAGES; ELECTRICITY CONSUMPTION; SUPPLY SECURITY; STATUS-QUO; HOUSEHOLDS; CHOICE; GDP; RELIABILITY; CALIFORNIA AB Hong Kong has almost perfect electricity reliability, the result of substantial investments ultimately financed by electricity consumers who may be willing to accept lower reliability in exchange for lower bills. But consumers with high outage costs are likely to reject the reliability reduction. Our ordered-logit regression analysis of the responses by 1876 households to a telephone survey conducted in June 2013 indicates that Hong Kong residents exhibit a statistically-significant preference for their existing service reliability and rate. Moreover, the average residential cost estimate for a 1-h outage is US$45 (HK$350), topping the estimates reported in 10 of the 11 studies published in the last 10 years. The policy implication is that absent additional compelling evidence, Hong Kong should not reduce its service reliability. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Woo, C. K.; Ho, T.; Cheng, Y. S.] Hong Kong Baptist Univ, Dept Econ, Hong Kong, Hong Kong, Peoples R China. [Shiu, A.] Hong Kong Polytech Univ, Sch Accounting & Finance, Hong Kong, Hong Kong, Peoples R China. [Horowitz, I.] Univ Florida, Warrington Coll Business, Gainesville, FL 32611 USA. [Wang, J.] Argonne Natl Lab, Ctr Energy Environm & Econ Syst, Argonne, IL 60439 USA. RP Woo, CK (reprint author), Hong Kong Baptist Univ, Dept Econ, Hong Kong, Hong Kong, Peoples R China. EM ck@ethree.com; hstony1@hotmail.com; afshiu@polyu.edu.hk; ycheng@hkbu.edu.hk; ira.horowitz@warrington.ufl.edu; jianhui.wang@anl.gov RI Shiu, Alice/A-3457-2015; OI Shiu, Alice/0000-0002-1487-2534; Woo, Chi-keung/0000-0001-6366-0960; Cheng, Yuk-shing/0000-0002-6420-4411 FU Hong Kong Baptist University's Business School; Hong Kong Polytechnic University's School of Accounting and Finance FX Major funding of this research is provided by the Hong Kong Baptist University's Business School. Additional funding is provided by the Hong Kong Polytechnic University's School of Accounting and Finance. Opinions expressed in this paper are those of the authors and do not represent the stance of the two funding universities. We thank J. Lam for her help in preparing the initial English version of the questionnaire, A. Law for her help in preparing the final Cantonese version used in the telephone survey, C.W. Tso for his timely reply to our information request, and three referees for their very helpful and constructive comments. Without implication, all errors are ours. NR 52 TC 3 Z9 3 U1 1 U2 8 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD SEP PY 2014 VL 72 BP 204 EP 210 DI 10.1016/j.enpol.2014.05.002 PG 7 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA AL0LA UT WOS:000338817200021 ER PT J AU Roege, PE Collier, ZA Mancillas, J McDonagh, JA Linkov, I AF Roege, Paul E. Collier, Zachary A. Mancillas, James McDonagh, John A. Linkov, Igor TI Metrics for energy resilience SO ENERGY POLICY LA English DT Article DE Resilience; Energy security; Energy-informed; Risk ID SYSTEMS AB Energy lies at the backbone of any advanced society and constitutes an essential prerequisite for economic growth, social order and national defense. However there is an Achilles heel to today's energy and technology relationship; namely a precarious intimacy between energy and the fiscal, social, and technical systems it supports. Recently, widespread and persistent disruptions in energy systems have highlighted the extent of this dependence and the vulnerability of increasingly optimized systems to changing conditions. Resilience is an emerging concept that offers to reconcile considerations of performance under dynamic environments and across multiple time frames by supplementing traditionally static system performance measures to consider behaviors under changing conditions and complex interactions among physical, information and human domains. This paper identifies metrics useful to implement guidance for energy-related planning, design, investment, and operation. Recommendations are presented using a matrix format to provide a structured and comprehensive framework of metrics relevant to a system's energy resilience. The study synthesizes previously proposed metrics and emergent resilience literature to provide a multidimensional model intended for use by leaders and practitioners as they transform our energy posture from one of stasis and reaction to one that is proactive and which fosters sustainable growth. Published by Elsevier Ltd. C1 [Roege, Paul E.] Idaho Natl Lab, Idaho Falls, ID 83402 USA. [Collier, Zachary A.; Linkov, Igor] US Army Engineer Res & Dev Ctr, Concord, MA 01742 USA. [Mancillas, James; McDonagh, John A.] US Army Environm Command, Ft Sam Houston, TX 78234 USA. RP Linkov, I (reprint author), US Army Engineer Res & Dev Ctr, 696 Virginia Rd, Concord, MA 01742 USA. EM paul.roege@alum.mit.edu; Zachary.A.Collier@usace.army.mil; james.w.mancillas.civ@mail.mil; john.a.mcdonagh2.civ@mail.mil; Igor.Linkov@usace.army.mil NR 30 TC 13 Z9 17 U1 1 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD SEP PY 2014 VL 72 BP 249 EP 256 DI 10.1016/j.enpol.2014.04.012 PG 8 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA AL0LA UT WOS:000338817200025 ER PT J AU Zhao, WH France, DM Yu, WH Kim, T Singh, D AF Zhao, Weihuan France, David M. Yu, Wenhua Kim, Taeil Singh, Dileep TI Phase change material with graphite foam for applications in high-temperature latent heat storage systems of concentrated solar power plants SO RENEWABLE ENERGY LA English DT Article DE Concentrated solar power; Graphite foam-MgCl2 combination; Latent heat thermal energy storage; Three-dimensional heat transfer simulation; Exergy efficiency ID THERMAL-ENERGY STORAGE; FRONT-TRACKING ALGORITHM; EXERGY ANALYSIS; SOLIDIFICATION PROBLEMS; OPTIMIZATION; CONVECTION AB A high-temperature latent heat thermal energy storage (LHTES) system was analyzed for applications to concentrated solar power (CSP) plants (utilizing steam at similar to 610 degrees C) for large-scale electricity generation. Magnesium chloride was selected as the phase change material (PCM) for the latent heat storage because of its high melting point (714 degrees C). Because the thermal conductivities of most salt materials are very low, usually less than 1 W/m K, graphite foam was applied as an additive to considerably enhance the overall thermal conductivity of the resulting graphite foam PCM combination in the LHTES system. The heat transfer performance and the exergy efficiency in the graphite foam-MgCl2 LHTES system were considered for the design and optimization of the storage system. Three-dimensional (3-D) heat transfer simulations were conducted for the storage system using commercial software COMSOL Three groups of analyses were performed for an LHTES system: using PCM alone without graphite foam, using average material properties for graphite foam PCM combination, and using anisotropic thermal conductivity and temperature-dependent material properties for graphite foam PCM. Results presented show that the graphite foam can help to significantly improve the heat transfer performance as well as the exergy efficiency in the LHTES system. They also show the effects of the anisotropic thermal conductivity and indicate capital cost savings for a CSP electric power plant by reducing the number of heat transfer fluid (HTF) pipes in the LHTES tank by a factor of eight. (C) 2014 Published by Elsevier Ltd. C1 [Zhao, Weihuan; Yu, Wenhua; Kim, Taeil] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [France, David M.] Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA. [Singh, Dileep] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Singh, D (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM dsingh@anl.gov FU Solar Energy Technologies Program (Sunshot Initiative) of the U.S. Department of Energy at Argonne National Laboratory [DE-AC02-06CH11357] FX This work was sponsored by the Solar Energy Technologies Program (Sunshot Initiative) of the U.S. Department of Energy under contract number DE-AC02-06CH11357 at Argonne National Laboratory, managed by UChicago Argonne LLC. Authors are grateful for helpful insights from Joseph Stekli and Levi Irwin of DOE. NR 31 TC 21 Z9 22 U1 5 U2 81 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-1481 J9 RENEW ENERG JI Renew. Energy PD SEP PY 2014 VL 69 BP 134 EP 146 DI 10.1016/j.renene.2014.03.031 PG 13 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA AL0FI UT WOS:000338802400016 ER PT J AU Nozaki, H Harada, M Ohta, S Watanabe, I Miyake, Y Ikedo, Y Jalarvo, NH Mamontov, E Sugiyama, J AF Nozaki, Hiroshi Harada, Masashi Ohta, Shingo Watanabe, Isao Miyake, Yasuhiro Ikedo, Yutaka Jalarvo, Niina H. Mamontov, Eugene Sugiyama, Jun TI Li diffusive behavior of garnet-type oxides studied by muon-spin relaxation and QENS SO SOLID STATE IONICS LA English DT Article; Proceedings Paper CT 19th International Conference on Solid State Ionics (SSI) CY JUN 02-07, 2013 CL Kyoto, JAPAN SP Solid State Ion Soc Japan, Int Soc Solid State Ion, Japan Soc Promot Sci, Commemorat Org Japan World Exposit, Kyushu Univ, Int Inst Carbon Neutral Energy Res, Electrochem Soc Japan, Comm Battery Technol, Murata Sci Fdn, Electrochem Soc Japan, Kansai Branch, Japan Soc Appl Phys, Phys Soc Japan, Electrochem Soc Japan, Soc Polymer Sci, Iron & Steel Inst Japan, Ceram Soc Japan, Chem Soc Japan, Japan Inst Met DE Muon-spin relaxation; Quasi-elastic neutron scattering; Lithium battery; Solid electrolyte AB A diffusive behavior of Li+ ion in a garnet-type oxide, Li(5 + x)La(3)Zr(x)Nb(2 - x)0(12) with x = 0-2, has been investigated by both a positive muon-spin relaxation (mu+SR) and quasi-elastic neutron scattering (QENS) technique using powder samples. The mu+SR results revealed that Li+ ions start to diffuse above similar to 150 K for the whole samples measured. The activation energy of Li diffusion (E-a) estimated from the mu+SR data was in good agreement with E-a obtained by the QENS measurements. However, both E(a)s were about a half of E-a of ionic conductivity of Li+ (sigma(Li)), which was evaluated by AC-impedance measurements on sintered pellets. This indicated the serious effect of grain boundary and/or surface on E-a. Furthermore, since the diffusion coefficient of Li+ estimated by mu+SR is roughly independent of x, the number of mobile Li+ in the garnet lattice was found to be the predominant parameter to determine sigma(Li). (C) 2013 Elsevier B.V. All rights reserved. C1 [Nozaki, Hiroshi; Harada, Masashi; Ohta, Shingo; Sugiyama, Jun] Toyota Cent Res & Dev Labs Inc, Nagakute, Aichi 4801192, Japan. [Watanabe, Isao] RIKEN, Adv Meson Sci Lab, Wako, Saitama 3510198, Japan. [Miyake, Yasuhiro; Ikedo, Yutaka] KEK, Inst Mat Struct Sci, Muon Sci Lab, Tsukuba, Ibaraki 3050801, Japan. [Jalarvo, Niina H.; Mamontov, Eugene] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Nozaki, H (reprint author), Toyota Cent Res & Dev Labs Inc, 41-1 Yokomichi, Nagakute, Aichi 4801192, Japan. EM h-nozaki@mosk.tytlabs.co.jp RI Sugiyama, Jun/M-6535-2015; Mamontov, Eugene/Q-1003-2015; Jalarvo, Niina/Q-1320-2015 OI Sugiyama, Jun/0000-0002-0916-5333; Mamontov, Eugene/0000-0002-5684-2675; Jalarvo, Niina/0000-0003-0644-6866 NR 16 TC 4 Z9 4 U1 3 U2 43 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD SEP 1 PY 2014 VL 262 SI SI BP 585 EP 588 DI 10.1016/j.ssi.2013.10.014 PG 4 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA AL0IL UT WOS:000338810500128 ER PT J AU Wang, YY Fan, F Agapov, AL Yu, X Hong, KL Mays, J Sokolov, AP AF Wang, Yangyang Fan, Fei Agapov, Alexander L. Yu, Xiang Hong, Kunlun Mays, Jimmy Sokolov, Alexei P. TI Design of superionic polymers-New insights from Walden plot analysis SO SOLID STATE IONICS LA English DT Article; Proceedings Paper CT 19th International Conference on Solid State Ionics (SSI) CY JUN 02-07, 2013 CL Kyoto, JAPAN SP Solid State Ion Soc Japan, Int Soc Solid State Ion, Japan Soc Promot Sci, Commemorat Org Japan World Exposit, Kyushu Univ, Int Inst Carbon Neutral Energy Res, Electrochem Soc Japan, Comm Battery Technol, Murata Sci Fdn, Electrochem Soc Japan, Kansai Branch, Japan Soc Appl Phys, Phys Soc Japan, Electrochem Soc Japan, Soc Polymer Sci, Iron & Steel Inst Japan, Ceram Soc Japan, Chem Soc Japan, Japan Inst Met DE Polymer electrolytes; Decoupling; Walden plot; Superionic ID IONIC-CONDUCTIVITY; ELECTROLYTES; GLASSES; RELAXATION; TRANSPORT AB Using a modified Walden plot analysis, we demonstrate that polyether-based solid electrolytes have intrinsic limitations for ionic transport at ambient and low temperatures, due to strongly coupled segmental and ion dynamics. On the other hand, rigid polymers can exhibit ionic conductivity that is highly decoupled from segmental relaxation, thus providing a significant advantage over traditional polyether electrolytes. Our analysis emphasizes that decoupling of ionic transport from segmental dynamics is the key for macromolecular design of "superionic" polymers. (C) 2013 Elsevier B.V. All rights reserved. C1 [Wang, Yangyang; Yu, Xiang; Mays, Jimmy; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Fan, Fei; Agapov, Alexander L.; Mays, Jimmy; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Wang, YY (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM wangy@ornl.gov RI Hong, Kunlun/E-9787-2015; Wang, Yangyang/A-5925-2010 OI Hong, Kunlun/0000-0002-2852-5111; Wang, Yangyang/0000-0001-7042-9804 NR 25 TC 7 Z9 7 U1 1 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD SEP 1 PY 2014 VL 262 SI SI BP 782 EP 784 DI 10.1016/j.ssi.2013.09.026 PG 3 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA AL0IL UT WOS:000338810500170 ER PT J AU Hanson, DT Collins, AM Jones, HDT Roesgen, J Lopez-Nieves, S Timlin, JA AF Hanson, David T. Collins, Aaron M. Jones, Howland D. T. Roesgen, John Lopez-Nieves, Samuel Timlin, Jerilyn A. TI On-line stable isotope gas exchange reveals an inducible but leaky carbon concentrating mechanism in Nannochloropsis salina SO PHOTOSYNTHESIS RESEARCH LA English DT Article DE Nannochloropsis; CO2 concentrating mechanism; (CO2)-C-13; Tunable diode laser; Lipid; Leakiness to CO2 ID INORGANIC-CARBON; CHLAMYDOMONAS-REINHARDTII; CHLOROPHYLL FLUORESCENCE; CO2; ALGAE; MICROALGAE; DIOXIDE; GROWTH; ACQUISITION; TRANSPORT AB Carbon concentrating mechanisms (CCMs) are common among microalgae, but their regulation and even existence in some of the most promising biofuel production strains is poorly understood. This is partly because screening for new strains does not commonly include assessment of CCM function or regulation despite its fundamental role in primary carbon metabolism. In addition, the inducible nature of many microalgal CCMs means that environmental conditions should be considered when assessing CCM function and its potential impact on biofuels. In this study, we address the effect of environmental conditions by combining novel, high frequency, on-line (CO2)-C-13 gas exchange screen with microscope-based lipid characterization to assess CCM function in Nannochloropsis salina and its interaction with lipid production. Regulation of CCM function was explored by changing the concentration of CO2 provided to continuous cultures in airlift bioreactors where cell density was kept constant across conditions by controlling the rate of media supply. Our isotopic gas exchange results were consistent with N. salina having an inducible "pump-leak" style CCM similar to that of Nannochloropsis gaditana. Though cells grew faster at high CO2 and had higher rates of net CO2 uptake, we did not observe significant differences in lipid content between conditions. Since the rate of CO2 supply was much higher for the high CO2 conditions, we calculated that growing cells bubbled with low CO2 is about 40 % more efficient for carbon capture than bubbling with high CO2. We attribute this higher efficiency to the activity of a CCM under low CO2 conditions. C1 [Hanson, David T.; Roesgen, John; Lopez-Nieves, Samuel] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. [Collins, Aaron M.; Jones, Howland D. T.; Timlin, Jerilyn A.] Sandia Natl Labs, Dept Bioenergy & Def Technol, Albuquerque, NM 87185 USA. RP Hanson, DT (reprint author), Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. EM dthanson@unm.edu RI Hanson, David/J-8034-2012; OI Timlin, Jerilyn/0000-0003-2953-1721 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; National Science Foundation Award [IOS 0719118]; EPSCoR (New Mexico) [IIA-1301346]; U.S. Department of Energy [DE-AC04-94AL85000]; Laboratory Directed Research and Development Program at Sandia National Laboratories FX The authors are grateful to Dr. Michael B. Sinclair for the use and maintenance of the hyperspectral confocal fluorescence microscope and Dr. Bryan D. Carson for the use of the flow cytometer. Majority support for this research was from the Laboratory Directed Research and Development Program at Sandia National Laboratories (JAT, AMC, HDTJ, JR and DTH). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was also partially supported by the National Science Foundation Award # IOS 0719118 (SLN, DTH) and the EPSCoR Program under Award # IIA-1301346 (New Mexico). Any opinions, findings, and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the National Science Foundation. This manuscript has been authored by Sandia Corporation under Contract No. DE-AC04-94AL85000 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 63 TC 1 Z9 1 U1 2 U2 25 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0166-8595 EI 1573-5079 J9 PHOTOSYNTH RES JI Photosynth. Res. PD SEP PY 2014 VL 121 IS 2-3 SI SI BP 311 EP 322 DI 10.1007/s11120-014-0001-0 PG 12 WC Plant Sciences SC Plant Sciences GA AK9RD UT WOS:000338763500019 PM 24844569 ER PT J AU Beaubrun, JJG Ewing, L Jarvis, K Dudley, K Grim, C Gopinath, G Flamer, ML Auguste, W Jayaram, A Elmore, J Lamont, M McGrath, T Hanes, DE AF Beaubrun, J. Jean-Gilles Ewing, L. Jarvis, K. Dudley, K. Grim, C. Gopinath, G. Flamer, M. -L. Auguste, W. Jayaram, A. Elmore, J. Lamont, M. McGrath, T. Hanes, D. E. TI Comparison of a PCR serotyping assay, Check&Trace assay for Salmonella, and Luminex Salmonella serotyping assay for the characterization of Salmonella enterica identified from fresh and naturally contaminated cilantro SO FOOD MICROBIOLOGY LA English DT Article DE Salmonella spp.; Molecular serotyping; Cilantro ID REAL-TIME PCR; MULTIPLEX PCR AB Salmonella enterica isolated from fresh cilantro samples collected through the USDA/AMS Microbiological Data Program (MDP) were used to compare a PCR serotyping assay against the Check&Trace assay and the Luminex (BioPlex) Salmonella serotyping assay. The study was conducted to evaluate the effectiveness of the three methods for serotyping Salmonella from both enrichment broth cultures and pure Salmonella cultures. In this investigation, Salmonella spp. serotyping was conducted using 24 h enrichment broth cultures and pure Salmonella cultures from cilantro samples, with the PCR serotyping assay. Conversely, the Check&Trace and Luminex for Salmonella assays required pure cultures for Salmonella serotyping. The cilantro samples contained S. enterica serovar Montevideo, Newport, Saintpaul, and Tennessee, identified by the PCR serotyping assay and Check&Trace for Salmonella, but the Luminex assay only identified two of the four serotypes of the cilantro samples. The anticipated impact from this study is that the PCR serotyping assay provides a time- and cost-effective means for screening, identifying and serotyping Salmonella using DNA extracted from 24 h enrichment cilantro samples. Published by Elsevier Ltd. C1 [Beaubrun, J. Jean-Gilles; Ewing, L.; Jarvis, K.; Dudley, K.; Grim, C.; Gopinath, G.; Flamer, M. -L.; Auguste, W.; Jayaram, A.; Elmore, J.; Hanes, D. E.] US FDA, Laurel, MD 20708 USA. [Grim, C.] Oak Ridge Inst Sci & Technol, Oak Ridge, TN USA. [Lamont, M.] USDA AMS Microbiol Data Program MDP, Manassas, VA 20110 USA. [McGrath, T.] ORA DFS FERN, Rockville, MD 20857 USA. [Flamer, M. -L.] Univ Maryland, UMCP JIFSAN Program, College Pk, MD 20742 USA. [Auguste, W.] Frostburg State Univ, Frostburg, MD 21532 USA. [Jayaram, A.] Richard Montgomery High Sch, Rockville, MD 20852 USA. [Elmore, J.] Howard Univ, Washington, DC 20059 USA. RP Beaubrun, JJG (reprint author), US FDA, MOD Facil 1, Virulence Mech Branch,Ctr Food Safety & Appl Nutr, Div Virulence Assessment,Off Appl Res & Safety As, HFS 025,8301 Muirkirk Rd, Laurel, MD 20708 USA. EM junia.jean-gillesbeaubrun@fda.hhs.gov NR 9 TC 2 Z9 2 U1 1 U2 13 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0740-0020 EI 1095-9998 J9 FOOD MICROBIOL JI Food Microbiol. PD SEP PY 2014 VL 42 BP 181 EP 187 DI 10.1016/j.fm.2014.02.008 PG 7 WC Biotechnology & Applied Microbiology; Food Science & Technology; Microbiology SC Biotechnology & Applied Microbiology; Food Science & Technology; Microbiology GA AK7GQ UT WOS:000338597100027 ER PT J AU Sanna, A Hutter, C Kenning, DBR Karayiannis, TG Sefiane, K Nelson, RA AF Sanna, A. Hutter, C. Kenning, D. B. R. Karayiannis, T. G. Sefiane, K. Nelson, R. A. TI Numerical investigation of nucleate boiling heat transfer on thin substrates SO INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER LA English DT Article DE Nucleate boiling; Heat transfer; Single bubble; Multi bubble sites; Coalescence ID BUBBLE-GROWTH; VAPOR BUBBLES; LIQUID; SURFACE; PREDICTION; DYNAMICS; FC-72; SITE AB The objective of this paper is to define the guidelines for the design of new boiling test sections with a large number of artificial nucleation sites during nucleate boiling for thin substrates horizontally immersed in a saturated liquid with artificial cavities located on the upper surface. The findings of numerical simulations of pool boiling heat transfer for a single bubble and for a large number of nucleation sites based on the analysis of experimental cases were analysed. Dedicated test sections were used in experiments for the study of boiling mechanisms and interactions between active sites so that the numerical models representing the physics of the problem could be improved. The hybrid nature of the code used in this study, combining the complete solution of the three-dimensional time-dependent energy equation in the solid substrate with semi-empirical models representing the physical phenomena occurring in the liquid side, in a simplified way, allows a large number of simulations in a reasonable computational time. The present paper focuses in the first part on the capability of the model to reproduce the experimental results for various conditions, while in the second part, the results for a large number of nucleation sites are analysed. Regarding the single bubble growth, two series of simulations will be presented in this paper: the first one analyses the mechanisms of nucleate boiling on a silicon substrate immersed in the dielectric fluid FC-72. The second series studies the behaviour of bubbles on metallic substrates, platinum and titanium, in saturated water. In the last section, the effect of the position of a site during simulations of a large population of sites (of the order of 100) on the waiting time, growth time, type and occurrence of coalescence and the thermal characteristics is presented. (C) 2014 The Authors. Published by Elsevier Ltd. C1 [Sanna, A.; Kenning, D. B. R.; Karayiannis, T. G.] Brunel Univ, Sch Engn & Design, Uxbridge UB8 3PH, Middx, England. [Hutter, C.; Sefiane, K.] Univ Edinburgh, Sch Engn, Edinburgh EH9 3JL, Midlothian, Scotland. [Nelson, R. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Karayiannis, TG (reprint author), Brunel Univ, Sch Engn & Design, Uxbridge UB8 3PH, Middx, England. EM tassos.karayiannis@brunel.ac.uk FU UK Engineering and Physical Sciences Research Council (EPSRC) [EP/C532813/1] FX This work was funded by the UK Engineering and Physical Sciences Research Council (EPSRC) by grant EP/C532813/1. NR 37 TC 6 Z9 7 U1 3 U2 40 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0017-9310 EI 1879-2189 J9 INT J HEAT MASS TRAN JI Int. J. Heat Mass Transf. PD SEP PY 2014 VL 76 BP 45 EP 64 DI 10.1016/j.ijheatmasstransfer.2014.04.026 PG 20 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA AK4IJ UT WOS:000338387800004 ER PT J AU Chen, L Kang, QJ Mu, YT He, YL Tao, WQ AF Chen, Li Kang, Qinjun Mu, Yutong He, Ya-Ling Tao, Wen-Quan TI A critical review of the pseudopotential multiphase lattice Boltzmann model: Methods and applications SO INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER LA English DT Review DE Pseudopotential model; Lattice Boltzmann method; Multiphase flow; Porous media; Slip phenomenon; Multiple physicochemical processes ID MEMBRANE FUEL-CELL; LIQUID WATER TRANSPORT; GAS-DIFFUSION LAYER; POROUS-MEDIA; NONIDEAL GASES; EQUATION MODEL; NUMERICAL-SIMULATION; PHASE-TRANSITIONS; IMMISCIBLE FLUIDS; FLOW SIMULATION AB This article presents a critical review of the theory and applications of a multiphase model in the community of the lattice Boltzmann method (LBM), the pseudopotential model proposed by Shan and Chen (1993) [4], which has been successfully applied to a wide range of multiphase flow problems during the past two decades. The first part of the review begins with a description of the LBM and the original pseudopotential model. The distinct features and the limitations of the original model are described in detail. Then various enhancements necessary to improve the pseudopotential model in terms of decreasing the spurious currents, obtaining high density/viscosity ratio, reducing thermodynamic inconsistency, unraveling the coupling between surface tension and equations of state (EOS), and unraveling the coupling between viscosity and surface tension, are reviewed. Then the fluid-solid interactions are presented and schemes to obtain different contact angles are discussed. The final section of this part focuses on the multi-component multiphase pseudopotential model. The second part of this review describes fruitful applications of this model to various multiphase flows. Coupling of this model with other models for more complicated multiple physicochemical processes are also introduced in this part. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Chen, Li; Mu, Yutong; He, Ya-Ling; Tao, Wen-Quan] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Thermofluid Sci & Engn MOE, Xian 710049, Shaanxi, Peoples R China. [Chen, Li; Kang, Qinjun] Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM 87544 USA. RP Kang, QJ (reprint author), Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM 87544 USA. EM lichennht@gmail.com; qkang@lanl.gov; muyutong@stu.xjtu.edu.cn; yalinghe@mail.xjtu.edu.cn; wqtao@mail.xjtu.edu.cn RI Chen, Li/P-4886-2014; Kang, Qinjun/A-2585-2010 OI Chen, Li/0000-0001-7956-3532; Kang, Qinjun/0000-0002-4754-2240 FU National Nature Science Foundation of China [51136004]; LANL LDRD Program; UC Lab Fees Research Program FX Financial support of this work was provided by the National Nature Science Foundation of China (No. 51136004), the LANL LDRD Program, and the UC Lab Fees Research Program. We thank Dr. Xiaowen Shan for the insightful comments, which have greatly improved the quality of this paper. We also appreciate the useful discussions with Prof. Haibo Huang from University of Science and Technology of China, Research Engineer Jie Bao from Pacific Northwest National Laboratory, Dr. Zhao Yu from the Dow Chemical Company, Dr. Qing Li from University of Southampton, and Prof. M. Sbragaglia from University of Tor Vergata. NR 152 TC 73 Z9 79 U1 33 U2 181 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0017-9310 EI 1879-2189 J9 INT J HEAT MASS TRAN JI Int. J. Heat Mass Transf. PD SEP PY 2014 VL 76 BP 210 EP 236 DI 10.1016/j.ijheatmasstransfer.2014.04.032 PG 27 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA AK4IJ UT WOS:000338387800018 ER PT J AU Konomi, BA Sang, HY Mallick, BK AF Konomi, Bledar A. Sang, Huiyan Mallick, Bani K. TI Adaptive Bayesian Nonstationary Modeling for Large Spatial Datasets Using Covariance Approximations SO JOURNAL OF COMPUTATIONAL AND GRAPHICAL STATISTICS LA English DT Article DE Bayesian treed Gaussian process; Full-scale approximation; Kernel Convolution; Markov chain Monte Carlo; Reversible-jump Markov chain Monte Carlo ID PROCESS-CONVOLUTION APPROACH; DATA SETS; INTERPOLATION; DEFORMATIONS; OZONE; PLANE AB Gaussian process models have been widely used in spatial statistics but face tremendous modeling and computational challenges for very large nonstationary spatial datasets. To address these challenges, we develop a Bayesian modeling approach using a nonstationary covariance function constructed based on adaptively selected partitions. The partitioned nonstationary class allows one to knit together local covariance parameters into a valid global nonstationary covariance for prediction, where the local covariance parameters are allowed to be estimated within each partition to reduce computational cost. To further facilitate the computations in local covariance estimation and global prediction, we use the full-scale covariance approximation (FSA) approach for the Bayesian inference of our model. One of our contributions is to model the partitions stochastically by embedding a modified treed partitioning process into the hierarchical models that leads to automated partitioning and substantial computational benefits. We illustrate the utility of our method with simulation studies and the global Total Ozone Matrix Spectrometer (TOMS) data. Supplementary materials for this article are available online. C1 [Konomi, Bledar A.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Sang, Huiyan; Mallick, Bani K.] Texas A&M Univ, Dept Stat, College Stn, TX 77843 USA. RP Konomi, BA (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM bledar.konomi@pnnl.gov; huiyan@stat.tamu.edu; bmallick@stat.tamu.edu FU National Science Foundation [DMS-1007618]; NSF [DMS 0914951]; King Abdullah University of Science and Technology [KUS-CI-016-04] FX The research of Huiyan Sang was partially sponsored by National Science Foundation grant DMS-1007618 and the research of Bani Mallick was partially supported by NSF DMS 0914951. Bani Mallick and Huiyan Sang were also partially supported by award KUS-CI-016-04, made by King Abdullah University of Science and Technology. The authors thank the referees and the editors for valuable comments. NR 39 TC 4 Z9 4 U1 0 U2 8 PU AMER STATISTICAL ASSOC PI ALEXANDRIA PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA SN 1061-8600 EI 1537-2715 J9 J COMPUT GRAPH STAT JI J. Comput. Graph. Stat. PD SEP PY 2014 VL 23 IS 3 BP 802 EP 829 DI 10.1080/10618600.2013.812872 PG 28 WC Statistics & Probability SC Mathematics GA AK1VJ UT WOS:000338205400011 ER PT J AU Pratola, MT Chipman, HA Gattiker, JR Higdon, DM McCulloch, R Rust, WN AF Pratola, Matthew T. Chipman, Hugh A. Gattiker, James R. Higdon, David M. McCulloch, Robert Rust, William N. TI Parallel Bayesian Additive Regression Trees SO JOURNAL OF COMPUTATIONAL AND GRAPHICAL STATISTICS LA English DT Article DE Big Data; Markov chain Monte Carlo; Nonlinear; Scalable; Statistical computing ID COMPUTER-MODEL CALIBRATION; CLUSTERS AB Bayesian additive regression trees (BART) is a Bayesian approach to flexible nonlinear regression which has been shown to be competitive with the best modern predictive methods such as those based on bagging and boosting. BART offers some advantages. For example, the stochastic search Markov chain Monte Carlo (MCMC) algorithm can provide a more complete search of the model space and variation across MCMC draws can capture the level of uncertainty in the usual Bayesian way. The BART prior is robust in that reasonable results are typically obtained with a default prior specification. However, the publicly available implementation of the BART algorithm in the R package BayesTree is not fast enough to be considered interactive with over a thousand observations, and is unlikely to even run with 50,000 to 100,000 observations. In this article we show how the BART algorithm may be modified and then computed using single program, multiple data (SPMD) parallel computation implemented using the Message Passing Interface (MPI) library. The approach scales nearly linearly in the number of processor cores, enabling the practitioner to perform statistical inference on massive datasets. Our approach can also handle datasets too massive to fit on any single data repository. C1 [Pratola, Matthew T.] Ohio State Univ, Dept Stat, Columbus, OH 43210 USA. [Chipman, Hugh A.] Acadia Univ, Dept Math & Stat, Wolfville, NS B4P 2R6, Canada. [Gattiker, James R.; Higdon, David M.; Rust, William N.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA. [McCulloch, Robert] Univ Chicago, Booth Sch Business, Chicago, IL 60637 USA. RP Pratola, MT (reprint author), Ohio State Univ, Dept Stat, 1958 Neil Ave,404 Cockins Hall, Columbus, OH 43210 USA. EM mpratola@stat.osu.edu; hugh.chipman@acadiau.ca; gatt@lanl.gov; dhigdon@lanl.gov; robert.mcculloch@chicagobooth.edu; wnr@lanl.gov FU U.S. Department of Energy Office of Science, Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program FX This work was supported in part by the U.S. Department of Energy Office of Science, Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program. NR 28 TC 6 Z9 6 U1 0 U2 7 PU AMER STATISTICAL ASSOC PI ALEXANDRIA PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA SN 1061-8600 EI 1537-2715 J9 J COMPUT GRAPH STAT JI J. Comput. Graph. Stat. PD SEP PY 2014 VL 23 IS 3 BP 830 EP 852 DI 10.1080/10618600.2013.841584 PG 23 WC Statistics & Probability SC Mathematics GA AK1VJ UT WOS:000338205400012 ER PT J AU Samulon, EC Gundiah, G Gascon, M Khodyuk, IV Derenzo, SE Bizarri, GA Bourret-Courchesne, ED AF Samulon, E. C. Gundiah, G. Gascon, M. Khodyuk, I. V. Derenzo, S. E. Bizarri, G. A. Bourret-Courchesne, E. D. TI Luminescence and scintillation properties of Ce3+-activated Cs2NaGdCl6, Cs3GdCl6, Cs2NaGdBr6 and Cs3GdBr6 SO JOURNAL OF LUMINESCENCE LA English DT Article DE Scintillator; gamma-ray detector; Non-proportionality; Elpasolite ID SINGLE-CRYSTAL; CE3+; ELPASOLITES; LANTHANIDE AB We report on the structure, scintillation and luminescence properties of Cs2BGdX6:Ce (where B=Na, Cs; X=Cl, Br). Single crystals were obtained for four different compounds with both cubic and monoclinic structures. gamma-ray spectroscopy measurements revealed light yields of 27,000 ph/MeV, 24,500 ph/MeV, 48,000 ph/MeV and 47,000 ph/MeV and energy resolutions of 4.0%, 4.5%, 3.3%, and 4.0% for Cs2NaGdCl6:Ce, Cs3GdCl6:Ce, Cs2NaGdBr6:Ce and Cs3GdBr6:Ce, respectively. X-ray emission and optical emission measurements of the samples exhibited both the characteristic Ce3+ 5d-4f emission and the Gd3+ 4f-4f emission. The optimal concentration of Ce3+ for these compounds was also determined from X-ray excited luminescence decay measurements of polycrystalline forms of these materials. Published by Elsevier B.V. C1 [Samulon, E. C.; Gundiah, G.; Gascon, M.; Khodyuk, I. V.; Derenzo, S. E.; Bizarri, G. A.; Bourret-Courchesne, E. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Samulon, EC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM ESamulon@lbl.gov RI Gascon, Martin/C-9440-2011 OI Gascon, Martin/0000-0002-2065-009X FU US Department of Homeland Security/DNDO; US Department of Energy/NNSA/NA22; Lawrence Berkeley National Laboratory [AC02-05CH11231] FX The authors would like to thank Kathleen Brennan for assistance with powder synthesis, Guang Wu for performing X-ray diffraction measurements, Stephen Hanrahan for measurements and Christopher Ramsey, David Wilson and James Powell for their technical and engineering expertise. This work was supported by the US Department of Homeland Security/DNDO and the US Department of Energy/NNSA/NA22 and carried out at Lawrence Berkeley National Laboratory under Contract no. AC02-05CH11231. This work does not constitute an express or implied endorsement on the part of the government. NR 20 TC 3 Z9 5 U1 4 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-2313 EI 1872-7883 J9 J LUMIN JI J. Lumines. PD SEP PY 2014 VL 153 BP 64 EP 72 DI 10.1016/j.jlumin.2014.02.021 PG 9 WC Optics SC Optics GA AK4KC UT WOS:000338392600010 ER PT J AU Jacobsen, MK Liu, W Li, B AF Jacobsen, M. K. Liu, W. Li, B. TI Enhancement of thermoelectric performance with pressure in Ce0.8Fe3CoSb12.1 SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article DE Chalcogenides; Semiconductors; High pressure; Transport properties ID FILLED SKUTTERUDITES CEFE4SB12; ELASTIC-CONSTANTS; KONDO INSULATORS; X-RAY; CERIUM; TEMPERATURE; MOLYBDENUM; TRANSITION; CRYSTALS; ENERGY AB Transport properties (resistivity, thermal conductivity, and Seebeck coefficient) and sound velocities have been determined for the skutterudite Ce0.8Fe3CoSb12.1 with pressure up to 14 GPa. From these measurements, high pressure anomalous features were found in all transport properties. By correlating these with results from previous x-ray work, it has been determined that there is likely an electronic topological transition in this material induced by pressure. This is possibly due to the known pressure variation of valence in the void-filling Ce atom and has been found to induce an improved figure of merit at higher pressures, which shows a nearly two-fold increase with applied pressure. At higher pressures, it was determined that this anomalous behavior is suppressed and is possibly induced by insertion of Sb from the cage into the remaining central voids of the structure, similar to that seen in the CoSb3 parent compound. Published by Elsevier Ltd. C1 [Jacobsen, M. K.; Liu, W.; Li, B.] SUNY Stony Brook, Inst Mineral Phys, Dept Geosci, Stony Brook, NY 11794 USA. RP Jacobsen, MK (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. EM mjacobsen@lanl.gov OI Jacobsen, Matthew/0000-0002-0326-2562 FU Department of Energy, National Nuclear Security Administration (NNSA) [DE-FG5209NA29458]; National Science foundation [EAR-1045630] FX This research is supported by a grant from the Department of Energy, National Nuclear Security Administration (NNSA) under contract number DE-FG5209NA29458 to BL. WL is also supported by the National Science foundation (EAR-1045630). NR 46 TC 3 Z9 3 U1 0 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 EI 1879-2553 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD SEP PY 2014 VL 75 IS 9 BP 1017 EP 1023 DI 10.1016/j.jpcs.2014.04.012 PG 7 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA AK4QY UT WOS:000338410400002 ER PT J AU Bhatia, C Fallin, B Gooden, ME Howell, CR Kelley, JH Tornow, W Arnold, CW Bond, EM Bredeweg, TA Fowler, MM Moody, WA Rundberg, RS Rusev, G Vieira, DJ Wilhelmy, JB Becker, JA Macri, R Ryan, C Sheets, SA Stoyer, MA Tonchev, AP AF Bhatia, C. Fallin, B. Gooden, M. E. Howell, C. R. Kelley, J. H. Tornow, W. Arnold, C. W. Bond, E. M. Bredeweg, T. A. Fowler, M. M. Moody, W. A. Rundberg, R. S. Rusev, G. Vieira, D. J. Wilhelmy, J. B. Becker, J. A. Macri, R. Ryan, C. Sheets, S. A. Stoyer, M. A. Tonchev, A. P. TI Dual-fission chamber and neutron beam characterization for fission product yield measurements using monoenergetic neutrons SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Fission product yields; Dual-fission chamber; Neutron production; Beam characterization ID THERMAL-NEUTRONS; SPECTRUM; PU-239; U-238 AB A program has been initiated to measure the energy dependence of selected high-yield fission products used in the analysis of nuclear test data. We present out initial work of neutron activation using a dual-fission chamber with quasi-monoenergetic neutrons and gamma-counting method. Quasi-monoenergetic neutrons of energies from 0.5 to 15 MeV using the TUNL 10 MV FM tandem to provide high-precision and self-consistent measurements of fission product yields (FPY). The final FPY results will be coupled with theoretical analysis to provide a more fundamental understanding of the fission process. To accomplish this goal, we have developed and tested a set of dual-fission ionization chambers to provide an accurate determination of the number of fissions occurring in a thick target located in the middle plane of the chamber assembly. Details of the fission chamber and its performance are presented along with neutron beam production and characterization. Also presented are studies on the background issues associated with room-return and off-energy neutron production. We show that the off-energy neutron contribution can be significant, but correctable, while room-return neutron background levels contribute less than < 1% to the fission signal. (C) 2014 Elsevier B.V. All rights reserved, C1 [Bhatia, C.; Fallin, B.; Howell, C. R.; Tornow, W.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Bhatia, C.; Fallin, B.; Gooden, M. E.; Howell, C. R.; Kelley, J. H.; Tornow, W.] Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Gooden, M. E.; Kelley, J. H.] N Carolina State Univ, Dept Phys, Raleigh, NC 27605 USA. [Arnold, C. W.; Bond, E. M.; Bredeweg, T. A.; Fowler, M. M.; Moody, W. A.; Rundberg, R. S.; Rusev, G.; Vieira, D. J.; Wilhelmy, J. B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Becker, J. A.; Macri, R.; Ryan, C.; Sheets, S. A.; Stoyer, M. A.; Tonchev, A. P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Gooden, ME (reprint author), N Carolina State Univ, Dept Phys, Raleigh, NC 27605 USA. EM megooden@tunl.duke.edu OI Rusev, Gencho/0000-0001-7563-1518; Bond, Evelyn/0000-0001-7335-4086 FU U.S. Department of Energy at Triangle Universities Nuclear Laboratory through NNSA; Stewardship Science Academic Alliances Program [DE-FG52-09NA29465, DE-FG52-09NA29448, DE-NA0001839, DE-NA0001784]; Los Alamos National Security, LLC [DE-AC52 06NA25396]; Lawrence Livermore National Security, LLC [DE-AC52-07NA27344] FX This work was performed under the auspices of U.S. Department of Energy at Triangle Universities Nuclear Laboratory through NNSA, Stewardship Science Academic Alliances Program under Contract nos. DE-FG52-09NA29465, DE-FG52-09NA29448, DE-NA0001839 and DE-NA0001784. At Los Alamos National Laboratory operated by the Los Alamos National Security, LLC under Contract no. DE-AC52 06NA25396 and at Lawrence Livermore National Laboratory operated by the Lawrence Livermore National Security, LLC under Contract no. DE-AC52-07NA27344. NR 14 TC 6 Z9 6 U1 3 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2014 VL 757 BP 7 EP 19 DI 10.1016/j.nima.2014.03.022 PG 13 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AK3TR UT WOS:000338348100002 ER PT J AU Kaplan, AC Henzl, V Menlove, HO Swinhoe, MT Belian, AP Flaska, M Pozzi, SA AF Kaplan, Alexis C. Henzl, Vladimir Menlove, Howard O. Swinhoe, Martyn T. Belian, Anthony P. Flaska, Marek Pozzi, Sara A. TI Determination of spent nuclear fuel assembly multiplication with the differential die-away self-interrogation instrument SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Safeguards; Nondestructive assay; Spent fuel; Rossi-alpha distribution AB We present a novel method for determining the multiplication of a spent nuclear fuel assembly with a Differential Die-Away Self-Interrogation (DDSI) instrument. The signal, which is primarily created by thermal neutrons, is measured with four He-3 detector banks surrounding a spent fuel assembly. The Rossi-alpha distribution (RAD) at early times reflects coincident events from single fissions as well as fission chains. Because of this fact, the early time domain contains information about both the fissile material and spontaneous fission material in the assembly being measured. A single exponential function fit to the early time domain of the RAD has a die-away time proportional to the spent fuel assembly (SFA) multiplication. This correlation was tested by simulating assay of 44 different SFAs with the DDSI instrument. The SFA multiplication was determined with a variance of 0.7%. (C) Published by Elsevier B.V. C1 [Kaplan, Alexis C.; Henzl, Vladimir; Menlove, Howard O.; Swinhoe, Martyn T.; Belian, Anthony P.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Kaplan, Alexis C.; Flaska, Marek; Pozzi, Sara A.] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. RP Kaplan, AC (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. FU U.S. Department of Homeland Security [2012-DN-130-NF0001-02]; Next Generation Safeguards Initiative (NGSI); Office of Nonproliferation and International Security (NIS); National Nuclear Security Administration (NNSA) FX This material is partially based upon work supported by the U.S. Department of Homeland Security under Grant Award Number, 2012-DN-130-NF0001-02. The authors also would like to acknowledge the support of the Next Generation Safeguards Initiative (NGSI), Office of Nonproliferation and International Security (NIS), National Nuclear Security Administration (NNSA). The views and conclusions contained in this document are those of the authors and should not be interpreted as necessarily representing the official policies, either expressed or implied, of the U.S. Department of Homeland Security or the National Nuclear Security Administration, LA-UR-13-29465, NR 19 TC 2 Z9 2 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2014 VL 757 BP 20 EP 27 DI 10.1016/j.nima.2014.04.023 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AK3TR UT WOS:000338348100003 ER PT J AU Quinn, SJ Spyrou, A Simon, A Battaglia, A Bowers, M Bucher, B Casarella, C Couder, M DeYoung, PA Dombos, AC Greene, JP Gorres, J Kontos, A Li, Q Long, A Moran, M Paul, N Pereira, J Robertson, D Smith, K Smith, MK Stech, E Talwar, R Tan, WP Wiescher, M AF Quinn, S. J. Spyrou, A. Simon, A. Battaglia, A. Bowers, M. Bucher, B. Casarella, C. Couder, M. DeYoung, P. A. Dombos, A. C. Greene, J. P. Gorres, J. Kontos, A. Li, Q. Long, A. Moran, M. Paul, N. Pereira, J. Robertson, D. Smith, K. Smith, M. K. Stech, E. Talwar, R. Tan, W. P. Wiescher, M. TI First application of the gamma-summing technique in inverse kinematics SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Summing technique; Capture reaction; Resonance strength; Inverse kinematics ID RADIATIVE PROTON CAPTURE; RECOIL SEPARATOR; NUCLEAR ASTROPHYSICS; ELEMENTS; DESIGN; ENERGY; NI-58; RATES; STARS AB The gamma-summing technique was successfully implemented for the first Lime in inverse kinematics using the NSCL Summing NaI(Tl) detector at the Nuclear Science Laboratory of the University of Notre Dame. This new method offers a way to measure (p,gamma) and (alpha,gamma) reactions on unstable nuclei, which are critical for an improved understanding of nucleosynthesis. As a proof of principle, the well-known resonances at E-c.m. = 956 key in the p(Al-27,gamma)Si-28 reaction and at E-c.m. = 1400 keV in the p(Ni-58,gamma)Cu-59 reaction were measured and their resonance strengths were deduced. The values of the present work agree well with the reported literature values, demonstrating the viability of the technique. (C) 2014 Elsevier B.V. All rights reserved. C1 [Quinn, S. J.; Spyrou, A.; Simon, A.; Dombos, A. C.; Kontos, A.; Pereira, J.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 43824 USA. [Quinn, S. J.; Spyrou, A.; Dombos, A. C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 43324 USA. [Quinn, S. J.; Spyrou, A.; Dombos, A. C.; Kontos, A.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 43324 USA. [Battaglia, A.; Bowers, M.; Bucher, B.; Casarella, C.; Couder, M.; Gorres, J.; Kontos, A.; Li, Q.; Long, A.; Moran, M.; Paul, N.; Robertson, D.; Smith, K.; Smith, M. K.; Stech, E.; Talwar, R.; Tan, W. P.; Wiescher, M.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Battaglia, A.; Bowers, M.; Bucher, B.; Casarella, C.; Couder, M.; Gorres, J.; Kontos, A.; Li, Q.; Long, A.; Moran, M.; Paul, N.; Robertson, D.; Smith, K.; Smith, M. K.; Stech, E.; Talwar, R.; Tan, W. P.; Wiescher, M.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [DeYoung, P. A.] Hope Coll, Dept Phys, Holland, MI 49423 USA. [Greene, J. P.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Quinn, SJ (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 43824 USA. EM quinn@nscl.msu.edu RI Couder, Manoel/B-1439-2009; Tan, Wanpeng/A-4687-2008 OI Couder, Manoel/0000-0002-0636-744X; Tan, Wanpeng/0000-0002-5930-1823 FU National Science Foundation [PHY 1102511, PHY 0822648, PHY 0969058, PHY 0319523] FX The authors would like to thank the staff at HIBAL for the characterization of the target and the operations staff at the University of Notre Dame for their assistance in the measurements. This work was supported by the National Science Foundation under Grant nos. PHY 1102511, PHY 0822648 (Joint Institute for Nuclear Astrophysics), PHY 0969058, and PHY 0319523, NR 33 TC 2 Z9 2 U1 2 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2014 VL 757 BP 62 EP 66 DI 10.1016/j.nima.2014.05.020 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AK3TR UT WOS:000338348100009 ER PT J AU Mosby, S Tovesson, F Couture, A Duke, DL Kleinrath, V Meharchand, R Meierbachtol, K O'Donnell, JM Perdue, B Richman, D Shields, D AF Mosby, S. Tovesson, F. Couture, A. Duke, D. L. Kleinrath, V. Meharchand, R. Meierbachtol, K. O'Donnell, J. M. Perdue, B. Richman, D. Shields, D. TI A fission fragment detector for correlated fission output studies SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Fission; Ionization chamber; Digital data acquisition AB A digital data acquisition system has been combined with a double Frisch gridded ionization chamber for use at both moderated and unmoderated neutron sources at the Los Alamos Neutron Science (LANSCE) facility. The high efficiency of the instrument combined with intense LANSCE beams and new acquisition system permits fission output measurements across 11 orders of magnitude incident neutron energy. The acquisition and analysis system is presented along with the first in beam performance tests of the setup. (C) 2014 Elsevier B.V. All rights reserved. C1 [Mosby, S.; Tovesson, F.; Couture, A.; Duke, D. L.; Kleinrath, V.; Meharchand, R.; Meierbachtol, K.; O'Donnell, J. M.; Perdue, B.; Richman, D.; Shields, D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Duke, D. L.; Shields, D.] Colorado Sch Mines, Golden, CO 80401 USA. [Kleinrath, V.] Idaho State Univ, Pocatello, ID 83201 USA. RP Mosby, S (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM smosby@lanl.gov OI Geppert-Kleinrath, Verena/0000-0002-6869-5772 FU US Department of Energy by Los Alamos National Security, LLC [DE-AC52-06NA25396] FX This work benefited from the use of the LANSCE accelerator facility. Work was performed under the auspices of the US Department of Energy by Los Alamos National Security, LLC under contract DE-AC52-06NA25396. We are indebted to F.-J. Hambsch for the construction of the ionization chamber used for this experiment, and W. Loveland for the preparation of the 235U samples that made the experiment possible. NR 23 TC 3 Z9 3 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2014 VL 757 BP 75 EP 81 DI 10.1016/j.nima.2014.04.066 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AK3TR UT WOS:000338348100011 ER PT J AU Hunt, RD Collins, JL AF Hunt, R. D. Collins, J. L. TI Recommended dispersing conditions for broths used in the preparation of uranium microspheres with carbon SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Internal gelation; Uranium oxide microspheres; Carbon black ID INTERNAL-GELATION AB Early preparations of uranium fuel kernels with carbon demonstrated the need for better dispersion of the carbon black in the aqueous feed solutions and in the subsequent microspheres. Therefore, the dispersing conditions for various carbon blacks were evaluated. A rheometer has proven to be a very useful tool in evaluation of dispersion conditions for carbon blacks (Black Pearl L and Raven 1000) with Tamol SN in the uranium and hexamethylenetetramine-urea feed solutions. The recommended dispersion conditions for Tamol SN were then used to make uranium microspheres with two carbon blacks. Optical images of these microspheres confirmed that the carbon was adequately dispersed, which supports the use of the viscosity measurements to determine appropriate carbon dispersion conditions. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Hunt, R. D.; Collins, J. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Hunt, RD (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM huntrd@ornl.gov FU Oak Ridge National Laboratory - UT-Battelle LLC - U.S. Department of Energy [DE-AC05-000R22725] FX This manuscript has been authored by the Oak Ridge National Laboratory, managed by UT-Battelle LLC under Contract No. DE-AC05-000R22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 13 TC 1 Z9 1 U1 1 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD SEP PY 2014 VL 71 BP 1 EP 5 DI 10.1016/j.anucene.2014.03.025 PG 5 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AJ8VH UT WOS:000337985500001 ER PT J AU Choung, S Um, W Choi, S Francis, AJ Kim, S Park, JB Kim, SH AF Choung, Sungwook Um, Wooyong Choi, Seho Francis, Arokiasamy J. Kim, Sungpyo Park, Jin Beak Kim, Suk-Hoon TI Biogeochemical changes at early stage after the closure of radioactive waste geological repository in South Korea SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Geological repository; Radionuclide; Gas generation; Microbial activities; Organic waste ID DISPOSAL AB Permanent disposal of low- and intermediate-level radioactive wastes in the subterranean environment has been the preferred method of many countries, including Korea. A safety issue after the closure of a geological repository is that biodegradation of organic materials due to microbial activities generates gases that lead to overpressure of the waste containers in the repository and its disintegration with the release of radionuclides. As part of an ongoing large-scale in situ experiment using organic wastes and groundwater to simulate geological radioactive waste repository conditions, we investigated the geo-chemical alteration and microbial activities at an early stage (similar to 63 days) intended to be representative of the initial period after repository closure. The increased numbers of both aerobes and facultative anaerobes in waste effluents indicate that oxygen content could be the most significant parameter to control biogeochemical conditions at very early periods of reaction (<35 days). Accordingly, the values of dissolved oxygen and redox potential were decreased. The activation of anaerobes after 35 days was supported by the increased concentration to similar to 50 mg L-1 of ethanol. These results suggest that the biogeochemical conditions were rapidly altered to more reducing and anaerobic conditions within the initial 2 months after repository closure. Although no gases were detected during the study, activated anaerobic microbes will play more important role in gas generation over the long term. Published by Elsevier Ltd. C1 [Choung, Sungwook; Um, Wooyong; Choi, Seho; Francis, Arokiasamy J.] Pohang Univ Sci & Technol POSTECH, Div Adv Nucl Engn, Pohang 790784, South Korea. [Um, Wooyong] PNNL, Energy & Environm Directorate, Richland, WA 99354 USA. [Francis, Arokiasamy J.] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. [Kim, Sungpyo] Korea Univ, Dept Environm Engn, Sejong 339700, South Korea. [Park, Jin Beak] Korea Radioact Waste Agcy KORAD, Taejon 305353, South Korea. [Kim, Suk-Hoon] Seoul Natl Univ, FNC Technol Co, Seoul 110799, South Korea. RP Um, W (reprint author), PNNL, Energy & Environm Directorate, 902 Battelle Blvd,P7-54, Richland, WA 99354 USA. EM Wooyong.um@pnnl.gov FU BK21+ program through the National Research Foundation of Korea - Ministry of Education, Science, and Technology; Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Ministry of Knowledge Economy [2009T10 0100500]; Korea Ministry of Environment as Global Top Project [GT-11-B-01-005-1] FX The authors specially appreciate anonymous reviewers for their valuable advice. This research project was carried out at the Division of Advanced Nuclear Engineering, POSTECH supported by BK21+ program through the National Research Foundation of Korea funded by the Ministry of Education, Science, and Technology. This research project was financially supported by the Korea Institute of Energy Technology Evaluation and Planning (KETEP) funded by the Ministry of Knowledge Economy (Grant No. 2009T10 0100500), and partially supported by Korea Ministry of Environment as Global Top Project (GT-11-B-01-005-1). NR 15 TC 1 Z9 1 U1 1 U2 17 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD SEP PY 2014 VL 71 BP 6 EP 10 DI 10.1016/j.anucene.2014.03.021 PG 5 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AJ8VH UT WOS:000337985500002 ER PT J AU Hales, JD Novascone, SR Spencer, BW Williamson, RL Pastore, G Perez, DM AF Hales, J. D. Novascone, S. R. Spencer, B. W. Williamson, R. L. Pastore, G. Perez, D. M. TI Verification of the BISON fuel performance code SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Nuclear fuel performance modeling; Verification; Validation ID MULTIDIMENSIONAL MULTIPHYSICS SIMULATION; VALIDATION AB Complex multiphysics simulations such as those used in nuclear fuel performance analysis are composed of many submodels used to describe specific phenomena. These phenomena include, for example, mechanical material constitutive behavior, heat transfer across a gas gap, and mechanical contact. These submodels work in concert to simulate real-world events, like the behavior of a fuel rod in a reactor. If a simulation tool is able to represent real-world behavior, the tool is said to be validated. While much emphasis is rightly placed on validation, model verification is equally important. Verification involves showing that a submodel computes results consistent with its mathematical description. This paper reviews the differences between verification, validation, and calibration as well as their dependencies on one another. Verification problems specific to nuclear fuel analysis are presented. Other verification problems suitable to assess the correctness of a finite element-based nuclear fuel application such as BISON (written to be applicable to many fuel forms and arbitrary geometry) are also presented. BISON calculates the correct solution to each of the verification tests, laying the foundation for subsequent validation. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Hales, J. D.; Novascone, S. R.; Spencer, B. W.; Williamson, R. L.; Pastore, G.; Perez, D. M.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Hales, JD (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM Jason.Hales@inl.gov OI Hales, Jason/0000-0003-0836-0476; Williamson, Richard/0000-0001-7734-3632; Pastore, Giovanni/0000-0003-2812-506X FU U.S. Government [DE-AC07-05ID14517] FX The submitted manuscript has been authored by a contractor of the U.S. Government under Contract DE-AC07-05ID14517. Accordingly, the U.S. Government retains a non-exclusive, royalty free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. NR 29 TC 6 Z9 6 U1 0 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD SEP PY 2014 VL 71 BP 81 EP 90 DI 10.1016/j.anucene.2014.03.027 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AJ8VH UT WOS:000337985500009 ER PT J AU Siefert, NS Chang, BY Litster, S AF Siefert, Nicholas S. Chang, Brian Y. Litster, Shawn TI Exergy and economic analysis of a CaO-looping gasifier for IGFC-CCS and IGCC-CCS SO APPLIED ENERGY LA English DT Article DE Coal gasification; CO2 capture; Solid oxide fuel cell; Thermo-economic analysis; Exergy; Levelized cost of electricity ID OXIDE FUEL-CELLS; CATALYTIC COAL-GASIFICATION; POWER-PLANTS; CO2 CAPTURE; ELEMENTAL MERCURY; HYDROGEN-SULFIDE; CARBON FORMATION; H2S REMOVAL; NATURAL-GAS; REGENERATION AB We present exergy and economic analyses for two potential advanced coal-based power plants with CO2 capture and sequestration. Each system generates three products: electricity, carbon dioxide compressed to 15 MPa, and pre-calcined feedstock for cement kilns. First, we analyzed a system that integrates a CaO-looping gasifier with a solid oxide fuel cell (SOFC), labeled here as IGFC-CCS. The SOFC is modeled based on a commercial pressurized SOFC system. Second, we analyzed a system that integrates a CaO-looping gasifier with a Brayton-Rankine combined cycle, labeled here as IGCC-CCS. The exergy analyses evaluated both the power generation/consumption and the exergy destruction in each of the major sub-systems within the power plant. The economic analyses evaluated the internal rate of return on investment (IRR), including the upfront construction costs and the yearly net revenue. Using recent capital cost estimates, we performed a parametric study of this IGFC-CCS system to determine the effect on the IRR on the four key SOFC parameters: current density, air pressure, fuel utilization, and air stoichiometric ratio. For this IGFC-CCS configuration, the calculated exergetic efficiency was 60% at the parameters values that maximized the IRR. For the IGCC-CCS system with same gasifier specifications, the efficiency was 46%; although, this configuration often achieved a higher value of IRR than the IGFC-CCS configuration, depending on the assumptions made on gas turbine and fuel cell equipment costs. We conducted a sensitivity analysis to determine how the IRR was affected by assumptions, such as capital costs and the sale price of CO2. Most importantly, we analyzed the effect of the coal gasification kinetic rate and CaO capture degradation rate on the IRR so that experimental researchers have goal posts as far as required rates for this CaO-looping process. From our sensitivity analysis, we conclude that the addition of alkali catalysts to CaO-looping gasification process can increase the IRR compared with a CaO-looping process without the addition of alkali catalysts, such as KOH. Published by Elsevier Ltd. C1 [Siefert, Nicholas S.; Chang, Brian Y.] Natl Energy Technol Lab, Dept Energy, Pittsburgh, PA 15236 USA. [Siefert, Nicholas S.; Chang, Brian Y.; Litster, Shawn] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. RP Siefert, NS (reprint author), Natl Energy Technol Lab, Dept Energy, Pittsburgh, PA 15236 USA. EM nicholas.siefert@netl.doe.gov FU National Energy Technology Laboratory FX We thank Taneasha Bledsoe for her assistance in building the AD-SOFC model. We thank Sweta Agarwal, Jay Apt, Kirk Gerdes, Melanie Jasper, Thomas Kalapos, Hunaid Nulwala, Allen Robinson, Edward Rubin, and Dushyant Shekhawat for their assistance in reviewing this manuscript. We thank the National Energy Technology Laboratory for their financial support of this research. It should be noted that the statements in this report represent the view of the authors and do not reflect an official position of the Department of Energy. Also, this paper includes forward-looking statements that should not be construed investment advice. NR 67 TC 6 Z9 6 U1 2 U2 46 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD SEP 1 PY 2014 VL 128 BP 230 EP 245 DI 10.1016/j.apenergy.2014.04.065 PG 16 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AJ6CE UT WOS:000337776500022 ER PT J AU Sanstad, AH McMenamin, S Sukenik, A Barbose, GL Goldman, CA AF Sanstad, Alan H. McMenamin, Stuart Sukenik, Andrew Barbose, Galen L. Goldman, Charles A. TI Modeling an aggressive energy-efficiency scenario in long-range load forecasting for electric power transmission planning SO APPLIED ENERGY LA English DT Article DE Load forecasting; Energy efficiency; Transmission planning AB Improving the representation of end-use energy efficiency, and of the effects of policies and programs to promote it, is an emergent priority for electricity load forecasting models and methods. This paper describes a "hybrid" load forecasting approach combining econometric and technological elements that is designed to meet this need, in a novel application to long-run electric power transmission planning in the western United States. A twenty-year load forecast incorporating significant increases in energy-efficiency programs and policies across multiple locations was developed in order to assess the potential of efficiency to reduce load growth and requirements for expanded transmission capacity. Load forecasting and transmission planning background is summarized, the theoretical and empirical aspects of the hybrid methodology described, and the assumptions, structure, data development, and results of the aggressive efficiency scenario are presented. The analysis shows that substantial electricity savings are possible in this scenario in most residential and commercial end-uses, and in the industrial sector, with magnitudes depending upon the specific end-use as well as upon the geographic location of the utility or other entity providing the electricity. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Sanstad, Alan H.; Barbose, Galen L.; Goldman, Charles A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [McMenamin, Stuart; Sukenik, Andrew] Itron Inc, Liberty Lake, WA USA. RP Sanstad, AH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mailstop 90-2002,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM ahsanstad@lbl.gov FU U.S. Department of Energy's Office of Electricity Delivery and Energy Reliability [DE-AC02-05CH11231] FX The work described in this report was supported by the U.S. Department of Energy's Office of Electricity Delivery and Energy Reliability under Contract No. DE-AC02-05CH11231. We would like to thank three anonymous referees for their invaluable comments. NR 34 TC 8 Z9 8 U1 1 U2 17 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD SEP 1 PY 2014 VL 128 BP 265 EP 276 DI 10.1016/j.apenergy.2014.04.096 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AJ6CE UT WOS:000337776500025 ER PT J AU Golari, M Fan, N Wang, JH AF Golari, Mehdi Fan, Neng Wang, Jianhui TI Two-stage stochastic optimal islanding operations under severe multiple contingencies in power grids SO ELECTRIC POWER SYSTEMS RESEARCH LA English DT Article DE Grid islanding; Cascading blackout; Stochastic mixed integer programming; Contingency ID OF-STEP RELAY; SPLITTING STRATEGIES; SYSTEM; NETWORKS; GENERATION AB Due to the catastrophic consequences of rolling blackouts, there is an increasing concern with the security and stability of modern power grids. Power grid islanding, as an emergency control operation method, can divide power grids into several self-sufficient islands and can then avoid wide-area blackouts. In this paper, we present a two-stage stochastic programming model to divide the power grids into self-sufficient islands before any multiple failures happen, and optimize islanding operations plan under severe multiple contingencies that lead to extreme situations where rolling blackouts may occur. Line switching and controlled load shedding are main tools for islanding, and the expected penalty for load shedding cost is minimized in consideration of contingencies with certain probabilities to happen. The presented model can give the system operator an efficient and optimal way to properly respond to outages. Several numerical experiments are performed on IEEE test cases to show the effectiveness of the proposed islanding operations method. (C) 2014 Elsevier B.V. All rights reserved. C1 [Golari, Mehdi; Fan, Neng] Univ Arizona, Dept Syst & Ind Engn, Tucson, AZ 85721 USA. [Wang, Jianhui] Argonne Natl Lab, Ctr Energy Environm & Econ Syst Anal, Argonne, IL 60439 USA. RP Fan, N (reprint author), Univ Arizona, Dept Syst & Ind Engn, Tucson, AZ 85721 USA. EM nfan@email.arizona.edu FU U.S. Department of Energy's Office of Electricity Delivery and Energy Reliability FX J. Wang's work is sponsored by the U.S. Department of Energy's Office of Electricity Delivery and Energy Reliability. NR 35 TC 2 Z9 2 U1 1 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7796 EI 1873-2046 J9 ELECTR POW SYST RES JI Electr. Power Syst. Res. PD SEP PY 2014 VL 114 BP 68 EP 77 DI 10.1016/j.epsr.2014.04.007 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA AJ8XS UT WOS:000337992000008 ER PT J AU Ao, T Harding, EC Bailey, JE Loisel, G Patel, S Sinars, DB Mix, LP Wenger, DF AF Ao, T. Harding, E. C. Bailey, J. E. Loisel, G. Patel, S. Sinars, D. B. Mix, L. P. Wenger, D. F. TI Relative x-ray collection efficiency, spatial resolution, and spectral resolution of spherically-bent quartz, mica, germanium, and pyrolytic graphite crystals SO JOURNAL OF QUANTITATIVE SPECTROSCOPY & RADIATIVE TRANSFER LA English DT Article DE X-ray scattering; Spherically-bent crystals; Imaging spectrometer ID VON-HAMOS SPECTROMETER; THOMSON SCATTERING; GIANT PLANETS; LASER SYSTEM; DENSE MATTER; Z-BEAMLET; K-ALPHA; RADIATION; PLASMAS; SPECTROSCOPY AB The relative x-ray collection efficiency, spatial resolution, and spectral resolution of spherically-bent quartz, mica, and germanium crystals were compared with cylindrically and spherically-bent highly oriented pyrolytic graphite (HOPG) and spherically-bent highly annealed pyrolytic graphite (HAPG) mosaic crystals. The crystals were characterized using Mn-K-alpha(1) (5898.8 eV) and Mn-K-alpha(2) (5887.6 eV) x-rays generated from a Manson x-ray source. The HOPG and HAPG crystals had about (10-100) x higher x-ray collection efficiency than the quartz, mica, and germanium crystals. However, good spatial resolutions were obtained with the quartz (49 mu m), mica (61 mu m), and germanium (275 mu m) crystals, while the HOPG and HAPG crystals provided no useful spatial resolving power. Deconvolution of the spectral broadening due to the Mn-K-alpha(1) intrinsic width (2.33 eV), source size (320 mu m), and image plate detector resolution (63 mu m) demonstrated the spectral resolutions (E/Delta E) of the quartz (3800-6600), mica (4600), and germanium (3400-4500) crystals to be considerably higher than that of the HOPG (1200-2400) and HAPG (2500) crystals. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Ao, T.; Harding, E. C.; Bailey, J. E.; Loisel, G.; Sinars, D. B.; Mix, L. P.; Wenger, D. F.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Patel, S.] Univ Michigan, Ann Arbor, MI 48109 USA. RP Ao, T (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tao@sandia.gov FU U.S. Department of Energy's National Nuclear Securities Administration [DE-AC04-94AL85000]; LDRD program at Sandia [141540] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Securities Administration under Contract No. DE-AC04-94AL85000. Funding of this work was through the LDRD program at Sandia (Project 141540). NR 68 TC 6 Z9 6 U1 2 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-4073 EI 1879-1352 J9 J QUANT SPECTROSC RA JI J. Quant. Spectrosc. Radiat. Transf. PD SEP PY 2014 VL 144 BP 92 EP 107 DI 10.1016/j.jqsrt.2014.03.023 PG 16 WC Optics; Spectroscopy SC Optics; Spectroscopy GA AJ9AS UT WOS:000337999800008 ER PT J AU Schoeppner, RL Bahr, DF Jin, H Goeke, RS Moody, NR Prasad, SV AF Schoeppner, R. L. Bahr, D. F. Jin, H. Goeke, R. S. Moody, N. R. Prasad, S. V. TI Wear behavior of Au-ZnO nanocomposite films for electrical contacts SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID GRAIN-SIZE STABILIZATION; NANOCRYSTALLINE MATERIALS; PLASTIC ZONE; STRAIN-RATE; THIN-FILMS; GROWTH; STRESS; GOLD; DEFORMATION; SIMULATIONS AB Electrical contact switches require low contact resistance for efficient passage of signals, while withstanding repetitive cycling. Hard gold with alloy additions of Ni, Co, or Ag can increase the wear resistance of Au films, however, this causes a significant decrease in conductivity and alloying elements can segregate during long-term aging leading to property evolution. The current work demonstrates that Au-zinc oxide (ZnO) nanocomposites can create a hard Au coating with a uniform, stable structure under frictional loading. Addition of ZnO particles decreases the grain size and texture of the film by 35 and 40-75 %, respectively, indicating a change in growth behavior of the film. The nanoindentation hardness increased directly with increasing ZnO concentration. Atomic force microscopy examination of wear-tested films demonstrated morphological stability after frictional contact and thus showed the potential for these films to replace current hard Au used on contact terminals. C1 [Schoeppner, R. L.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Schoeppner, R. L.; Bahr, D. F.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Jin, H.; Moody, N. R.] Sandia Natl Labs, Livermore, CA USA. [Goeke, R. S.; Prasad, S. V.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Bahr, DF (reprint author), Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. EM dfbahr@purdue.edu RI Bahr, David/A-6521-2012 OI Bahr, David/0000-0003-2893-967X FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 42 TC 4 Z9 4 U1 4 U2 56 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD SEP PY 2014 VL 49 IS 17 BP 6039 EP 6047 DI 10.1007/s10853-014-8326-9 PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA AJ2RI UT WOS:000337507100024 ER PT J AU Williams, PT AF Williams, Paul T. TI Significantly greater reduction in breast cancer mortality from post-diagnosis running than walking SO INTERNATIONAL JOURNAL OF CANCER LA English DT Article DE running; walking; prevention ID CORONARY-HEART-DISEASE; PHYSICAL-ACTIVITY; POSTMENOPAUSAL WOMEN; PROSPECTIVE COHORT; RISK-FACTORS; LIFE-STYLE; SURVIVAL; RUNNERS; HEALTH; DISTANCE AB The purpose of these analyses is to test prospectively whether post-diagnosis running and walking differ significantly in their association with breast cancer mortality. Cox proportional hazard analyses were used to compare breast cancer mortality to baseline exercise energy expenditure (METs, 1 MET-hour congruent to 1 km run) in 272 runners and 714 walkers previously diagnosed with breast cancer from the National Runners' and Walkers' Health Studies when adjusted for age, race, menopause, family history, breastfeeding and oral contraceptive use. Diagnosis occurred (mean +/- SD) 7.9 +/- 7.3 years before baseline. Forty-six women (13 runners and 33 walkers) died from breast cancer during 9.1-year mortality surveillance. For the 986 runners and walkers combined, breast cancer mortality decreased an average of 23.9% MET-hours/day [95% confidence interval (CI): 7.9-38.3%; p = 0.004]. There was a significantly greater decrease in risk for running than walking (risk per MET-hours/day run vs. walked: p = 0.03). For the 272 runners analyzed separately, breast cancer mortality decreased an average of 40.9% per MET-hours/day run (95% CI: 19.3-60.0%, p = 0.0004). When analyzed by categories of running energy expenditure, breast cancer mortality was 87.4% lower for the 1.8-3.6 MET-hours/day category (95% CI: 41.3-98.2% lower, p = 0.008) and 95.4% lower for the >= 3.6 MET-hours/day category (95% CI: 71.9-100% lower, p = 0.0004) compared to the <1.07 MET-hours/day category. In contrast, the 714 walkers showed a nonsignificant 4.6% decrease in breast cancer mortality per MET-hours/day walked (95% CI: 27.3% decreased risk to 21.3% increased risk, p = 0.71). These results suggest that post-diagnosis running is associated with significantly lower breast cancer mortality than post-diagnosis walking. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Williams, PT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Donner 464,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM ptwilliams@lbl.gov FU National Heart, Lung, and Blood Institute [HL094717] FX Grant sponsor: National Heart, Lung, and Blood Institute; Grant number: HL094717 NR 47 TC 9 Z9 9 U1 0 U2 26 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0020-7136 EI 1097-0215 J9 INT J CANCER JI Int. J. Cancer PD SEP 1 PY 2014 VL 135 IS 5 BP 1195 EP 1202 DI 10.1002/ijc.28740 PG 8 WC Oncology SC Oncology GA AJ3ZQ UT WOS:000337608300020 PM 24470442 ER PT J AU Zhu, TL Lin, Y Yang, ZB Su, D Ma, SG Han, MF Chen, FL AF Zhu, Tenglong Lin, Ye Yang, Zhibin Su, Dong Ma, Shuguo Han, Minfang Chen, Fanglin TI Evaluation of Li2O as an efficient sintering aid for gadolinia-doped ceria electrolyte for solid oxide fuel cells SO JOURNAL OF POWER SOURCES LA English DT Article DE Gadolinia-doped ceria; Sintering aid; Conductivity; Electrolyte; Solid oxide fuel cell ID ELECTRICAL-PROPERTIES; GRAIN-BOUNDARIES; TEMPERATURE; CONDUCTIVITY; PERFORMANCE; FABRICATION; CERAMICS; ZIRCONIA; SOFCS AB Li2O has been evaluated as a sintering aid for Gd0.1Ce0.9O2-delta(GDC). Using 2.5 mol% ratio of Li2O to GDC (5LiGDC), dense samples with relative density of 993% were achieved at sintering temperature as low as 900 degrees C. A high total conductivity of 0.059 S cm(-1) at 600 degrees C was obtained for the 5LiGDC samples sintered at 1000 degrees C (5LiGDC1000), while 5LiGDC samples sintered at 1400 degrees C showed a lower conductivity of 0.017 S cm(-1) at 600 degrees C. It has been found that Li2O has the tendency to accumulate in the grain boundary region to form Li-Gd-Ce-O phases when the 5LiGDC sintering temperature is at 1000 degrees C or below, leading to an increase in the grain boundary conductivity. Increasing the 5LiGDC sintering temperature above 1000 degrees C will accelerate the vaporization of Li2O, association of the oxygen vacancy and formation of additional pores in the bulk, resulting in a decrease of both the grain boundary and grain interior conductivity. Secondary ion mass spectrometry (SIMS) results have confirmed the existence of Li ions for the 5LiGDC samples sintered at or below 1000 degrees C, while most of Li species has vaporized for the 5LiGDC samples sintered above 1000 degrees C. (c) 2014 Elsevier B.V. All rights reserved. C1 [Zhu, Tenglong; Yang, Zhibin; Han, Minfang] China Univ Min & Technol, Union Res Ctr Fuel Cell, Beijing 100083, Peoples R China. [Lin, Ye; Chen, Fanglin] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Ma, Shuguo] Univ S Carolina, Coll Engn & Comp, Columbia, SC 29208 USA. RP Han, MF (reprint author), China Univ Min & Technol, Union Res Ctr Fuel Cell, Beijing 100083, Peoples R China. EM hanminfang@sina.com; chenfa@cec.sc.edu RI 杨, 志宾/B-2311-2015; Chen, Fanglin/K-1039-2012; Liu, Tong/N-7904-2013; Su, Dong/A-8233-2013 OI Lin, Ye/0000-0003-4289-894X; 杨, 志宾/0000-0003-3845-1133; Chen, Fanglin/0000-0001-9942-8872; Liu, Tong/0000-0001-5311-9687; Su, Dong/0000-0002-1921-6683 FU US National Science Foundation [DMR-1210792]; National Basic Research Program of China (973 Program) [2012CB215400]; NSFC-NSF China-US international Cooperation Project [51261120378]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-ACO2-98CH10886] FX We're grateful to the financial support from the US National Science Foundation (DMR-1210792), National Basic Research Program of China (973 Program, 2012CB215400) and NSFC-NSF China-US international Cooperation Project (51261120378). TEM work has been carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-ACO2-98CH10886. NR 30 TC 13 Z9 13 U1 4 U2 45 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD SEP 1 PY 2014 VL 261 BP 255 EP 263 DI 10.1016/j.jpowsour.2014.03.010 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AI6BF UT WOS:000336954100033 ER PT J AU Das, PK Weber, AZ Bender, G Manak, A Bittinat, D Herring, AM Ulsh, M AF Das, Prodip K. Weber, Adam Z. Bender, Guido Manak, Austin Bittinat, Daniel Herring, Andrew M. Ulsh, Michael TI Rapid detection of defects in fuel-cell electrodes using infrared reactive-flow-through technique SO JOURNAL OF POWER SOURCES LA English DT Article DE Catalyst layer; Defect detection; Infrared thermography; Fuel cells; Manufacturing ID LAYER-THICKNESS; TRANSPORT AB As fuel cells become more prominent, new manufacturing and production methods will need to be developed to deal efficiently and effectively with increased demand. One necessary component of this industrial growth is the accurate measurement of the variability in the manufacturing process. In this study, we present a diagnostic system that combines infrared thermography with a reactive-flow-through technique to detect catalyst-loading defects in fuel-cell gas-diffusion electrodes accurately with high spatial and temporal resolutions. Experimental results are compared with model predictions of thermal response with good agreement. Data analysis, operating-condition impacts, and detection limits are explored using both experiments and simulation. Overall, the results demonstrate the potential of this technique to measure defects on the millimeter length scale with temporal resolutions appropriate for use on a web-line. Thus we present the first development stage of a next-generation non-destructive diagnostic tool, which may be amenable to eventual use on roll-to-roll manufacturing lines. (C) 2014 Elsevier B.V. All rights reserved. C1 [Das, Prodip K.; Weber, Adam Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Bender, Guido; Manak, Austin; Bittinat, Daniel; Ulsh, Michael] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. RP Ulsh, M (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM michael.ulsh@nrel.gov OI Weber, Adam/0000-0002-7749-1624; Das, Prodip/0000-0001-9096-3721; Herring, Andrew/0000-0001-7318-5999 FU Fuel Cell Technologies Office, of the U. S. Department of Energy, Energy Efficiency and Renewable Energy [DE-AC36-08-GO28308 (NREL), DE-AC02-05CH11231 (LBNL)] FX The authors acknowledge funding for this work provided by the Fuel Cell Technologies Office, of the U. S. Department of Energy, Energy Efficiency and Renewable Energy under contract numbers DE-AC36-08-GO28308 (NREL) and DE-AC02-05CH11231 (LBNL). NR 19 TC 6 Z9 6 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD SEP 1 PY 2014 VL 261 BP 401 EP 411 DI 10.1016/j.jpowsour.2013.11.124 PG 11 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AI6BF UT WOS:000336954100051 ER PT J AU Hauck, C Sun, Y Timofeyev, I AF Hauck, Cory Sun, Yi Timofeyev, Ilya TI On cellular automata models of traffic flow with look-ahead potential SO STOCHASTICS AND DYNAMICS LA English DT Article DE Traffic flow; cellular automata model; look-ahead potential; coarse-grained PDE model ID SYSTEMS; FILTER AB We study the statistical properties of a cellular automata model of traffic flow with the look-ahead potential. The model defines stochastic rules for the movement of cars on a lattice. We analyze the underlying statistical assumptions needed for the derivation of the coarse-grained model and demonstrate that it is possible to relax some of them to obtain an improved coarse-grained ODE model. We also demonstrate that spatial correlations play a crucial role in the presence of the look-ahead potential and propose a simple empirical correction to account for the spatial dependence between neighboring cells. C1 [Hauck, Cory] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Sun, Yi] Univ S Carolina, Dept Math, Columbia, SC 29208 USA. [Timofeyev, Ilya] Univ Houston, Dept Math, Houston, TX 77204 USA. RP Timofeyev, I (reprint author), Univ Houston, Dept Math, Houston, TX 77204 USA. EM hauckc@ornl.gov; yisun@math.sc.edu; ilya@math.uh.edu FU NSF [DMS-1109582]; Office of Advanced Scientific Computing Research; USC; SC EPSCoR GEAR Award; [DE-AC05-00OR22725] FX The work presented in this paper emerged as a result of discussions in a working group at the NSF funded Statistical and Applied Mathematical Sciences Institute. I.T. also acknowledges support from SAMSI as a long-term visitor in the Fall of 2010 and the Fall of 2011. C. H. was sponsored by the Office of Advanced Scientific Computing Research and performed at the Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725. I. T. was supported in part by the NSF Grant DMS-1109582. Y.S. was partially supported by a USC startup fund and a SC EPSCoR GEAR Award. NR 24 TC 4 Z9 5 U1 2 U2 22 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0219-4937 EI 1793-6799 J9 STOCH DYNAM JI Stoch. Dyn. PD SEP PY 2014 VL 14 IS 3 AR 1350022 DI 10.1142/S0219493713500226 PG 21 WC Statistics & Probability SC Mathematics GA AI6CC UT WOS:000336956400005 ER PT J AU Bamgbade, BA Wu, Y Baled, HO Enick, RM Burgess, WA Tapriyal, D McHugh, MA AF Bamgbade, Babatunde A. Wu, Yue Baled, Hseen O. Enick, Robert M. Burgess, Ward A. Tapriyal, Deepak McHugh, Mark A. TI Experimental density measurements of bis(2-ethylhexyl) phthalate at elevated temperatures and pressures (vol 63, pg 102, 2013) SO JOURNAL OF CHEMICAL THERMODYNAMICS LA English DT Correction C1 [Bamgbade, Babatunde A.; Wu, Yue; Baled, Hseen O.; Enick, Robert M.; Burgess, Ward A.; Tapriyal, Deepak; McHugh, Mark A.] Natl Energy Technol Lab, Dept Energy, Off Res & Dev, Pittsburgh, PA 15236 USA. [Bamgbade, Babatunde A.; Wu, Yue; McHugh, Mark A.] Virginia Commonwealth Univ, Chem & Life Sci Engn Dept, Richmond, VA 23284 USA. [Baled, Hseen O.; Enick, Robert M.] Univ Pittsburgh, Swanson Sch Engn, Chem & Petr Engn Dept, Pittsburgh, PA 15261 USA. [Tapriyal, Deepak] URS, Pittsburgh, PA USA. RP Bamgbade, BA (reprint author), Virginia Commonwealth Univ, Chem & Life Sci Engn Dept, 601 West Main St, Richmond, VA 23284 USA. EM bamgbadeba@vcu.edu NR 1 TC 0 Z9 0 U1 2 U2 8 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0021-9614 EI 1096-3626 J9 J CHEM THERMODYN JI J. Chem. Thermodyn. PD SEP PY 2014 VL 76 BP 172 EP 172 DI 10.1016/j.jct.2014.02.011 PG 1 WC Thermodynamics; Chemistry, Physical SC Thermodynamics; Chemistry GA AI0QG UT WOS:000336552100019 ER PT J AU Chou, CS Shu, CW Xing, YL AF Chou, Ching-Shan Shu, Chi-Wang Xing, Yulong TI Optimal energy conserving local discontinuous Galerkin methods for second-order wave equation in heterogeneous media SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Wave propagation; Local discontinuous Galerkin method; Energy conservation; Optimal error estimate; Heterogeneous media ID FINITE-ELEMENT-METHOD; ONE SPACE DIMENSION; CONSERVATION-LAWS; HYPERBOLIC-EQUATIONS; NUMERICAL-SOLUTION; ORDER METHODS; SYSTEMS; SUPERCONVERGENCE; PROPAGATION; SCHEMES AB Solving wave propagation problems within heterogeneous media has been of great interest and has a wide range of applications in physics and engineering. The design of numerical methods for such general wave propagation problems is challenging because the energy conserving property has to be incorporated in the numerical algorithms in order to minimize the phase or shape errors after long time integration. In this paper, we focus on multi-dimensional wave problems and consider linear second-order wave equation in heterogeneous media. We develop and analyze an LDG method, in which numerical fluxes are carefully designed to maintain the energy conserving property and accuracy. Compatible high order energy conserving time integrators are also proposed. The optimal error estimates and the energy conserving property are proved for the semi-discrete methods. Our numerical experiments demonstrate optimal rates of convergence, and show that the errors of the numerical solutions do not grow significantly in time due to the energy conserving property. (C) 2014 Elsevier Inc. All rights reserved. C1 [Chou, Ching-Shan] Ohio State Univ, Dept Math, Columbus, OH 43221 USA. [Shu, Chi-Wang] Brown Univ, Div Appl Math, Providence, RI 02912 USA. [Xing, Yulong] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Xing, Yulong] Univ Tennessee, Dept Math, Knoxville, TN 37996 USA. RP Xing, YL (reprint author), Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. EM chou@math.ohio-state.edu; shu@dam.brown.edu; xingy@math.utk.edu FU NSF [DMS-1020625, DMS-1253481, DMS-1112700, DMS-1216454]; DOE [DE-FG02-08ER25863]; ORNL; U.S. Department of Energy, Office of Advanced Scientific Computing Research; UT-Battelle, LLC [DE-AC05-00OR22725] FX Research is supported by NSF grants DMS-1020625 and DMS-1253481.; Research is supported by DOE grant DE-FG02-08ER25863 and NSF grant DMS-1112700.; Research is sponsored by NSF grant DMS-1216454, ORNL and the U.S. Department of Energy, Office of Advanced Scientific Computing Research. The work was partially performed at ORNL, which is managed by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725. NR 46 TC 9 Z9 9 U1 1 U2 13 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD SEP 1 PY 2014 VL 272 BP 88 EP 107 DI 10.1016/j.jcp.2014.04.009 PG 20 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AI1OP UT WOS:000336620900005 ER PT J AU Kylasa, SB Aktulga, HM Grama, AY AF Kylasa, S. B. Aktulga, H. M. Grama, A. Y. TI PuReMD-GPU: A reactive molecular dynamics simulation package for GPUs SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE GPUs; GPU-enabled applications; Reactive molecular dynamics; Performance optimizations ID FORCE-FIELD; HYDROCARBONS; REAXFF; ALGORITHMS; SYSTEMS AB We present an efficient and highly accurate GP-GPU implementation of our community code, PuReMD, for reactive molecular dynamics simulations using the ReaxFF force field. PuReMD and its incorporation into LAMMPS (Reax/C) is used by a large number of research groups worldwide for simulating diverse systems ranging from biomembranes to explosives (RDX) at atomistic level of detail. The sub-femtosecond time-steps associated with ReaxFF strongly motivate significant improvements to per-timestep simulation time through effective use of GPUs. This paper presents, in detail, the design and implementation of PuReMD-GPU, which enables ReaxFF simulations on GPUs, as well as various performance optimization techniques we developed to obtain high performance on state-of-the-art hardware. Comprehensive experiments on model systems (bulk water and amorphous silica) are presented to quantify the performance improvements achieved by PuReMD-GPU and to verify its accuracy. In particular, our experiments show up to 16 x improvement in runtime compared to our highly optimized CPU-only single-core ReaxFF implementation. PuReMD-GPU is a unique production code, and is currently available on request from the authors. (C) 2014 Elsevier Inc. All rights reserved. C1 [Kylasa, S. B.] Purdue Univ, Dept Elec & Comp Eng, W Lafayette, IN 47907 USA. [Grama, A. Y.] Purdue Univ, Dept Comp Sci, W Lafayette, IN 47907 USA. [Aktulga, H. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Kylasa, SB (reprint author), Purdue Univ, Dept Elec & Comp Eng, W Lafayette, IN 47907 USA. EM skylasa@purdue.edu; hmaktulga@lbl.gov; ayg@cs.purdue.edu NR 33 TC 10 Z9 11 U1 6 U2 54 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD SEP 1 PY 2014 VL 272 BP 343 EP 359 DI 10.1016/j.jcp.2014.04.035 PG 17 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AI1OP UT WOS:000336620900018 ER PT J AU Lipnikov, K Manzini, G AF Lipnikov, K. Manzini, G. TI A high-order mimetic method on unstructured polyhedral meshes for the diffusion equation SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE High-order method; Unstructured polyhedral mesh; Mimetic finite difference method; Diffusion problem ID FINITE-DIFFERENCE METHOD; ELLIPTIC PROBLEMS; LINEAR ELASTICITY; POLYGONAL MESHES; ERROR ESTIMATOR; STOKES PROBLEM; DISCRETIZATION; ELEMENTS; CONVERGENCE; PRINCIPLES AB We present a new family of mimetic finite difference schemes for solving elliptic partial differential equations in the primal form on unstructured polyhedral meshes. These mimetic discretizations are built to satisfy local consistency and stability conditions. The consistency condition is an exactness property, i.e., the mimetic schemes are exact when the solution is a polynomial of an assigned degree. The stability condition ensures the well-posedness of the method. The degrees of freedom are the solution moments on mesh faces and inside mesh cells. Higher order schemes are built using higher order moments. The developed schemes are verified numerically on diffusion problems with constant and spatially variable (possibly, discontinuous) tensorial coefficients. Published by Elsevier Inc. C1 [Lipnikov, K.; Manzini, G.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Manzini, G.] IMATI CNR, I-27100 Pavia, Italy. [Manzini, G.] Ctr Simulaz Numer Avanzata CeSNA IUSS Pavia, I-27100 Pavia, Italy. RP Manzini, G (reprint author), Los Alamos Natl Lab, Div Theoret, Grp T-5,MS B284, Los Alamos, NM 87545 USA. OI Manzini, Gianmarco/0000-0003-3626-3112 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics FX The authors gratefully thank the anonymous reviewers for many useful suggestions on how to improve the presentation of this paper. This work was partially supported by the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and the DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics. NR 40 TC 10 Z9 10 U1 0 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD SEP 1 PY 2014 VL 272 BP 360 EP 385 DI 10.1016/j.jcp.2014.04.021 PG 26 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AI1OP UT WOS:000336620900019 ER PT J AU Kedia, KS Safta, C Ray, J Najm, HN Ghoniem, AF AF Kedia, Kushal S. Safta, Cosmin Ray, Jaideep Najm, Habib N. Ghoniem, Ahmed F. TI A second-order coupled immersed boundary-SAMR construction for chemically reacting flow over a heat-conducting Cartesian grid-conforming solid SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Reacting flow; Conjugate heat exchange; Cartesian solid; Immersed boundary; Adaptive mesh refinement; Operator-split projection ID DIRECT NUMERICAL-SIMULATION; ADAPTIVE MESH REFINEMENT; NAVIER-STOKES EQUATIONS; FLAME-WALL INTERACTION; UNSTEADY-FLOW; COMPLEX FLOW; PLATE; MECHANISMS; CHEMISTRY; MOTION AB In this paper, we present a second-order numerical method for simulations of reacting flow around heat-conducting immersed solid objects. The method is coupled with a block-structured adaptive mesh refinement (SAMR) framework and a low-Mach number operator-split projection algorithm. A "buffer zone" methodology is introduced to impose the solid-fluid boundary conditions such that the solver uses symmetric derivatives and interpolation stencils throughout the interior of the numerical domain; irrespective of whether it describes fluid or solid cells. Solid cells are tracked using a binary marker function. The no-slip velocity boundary condition at the immersed wall is imposed using the staggered mesh. Near the immersed solid boundary, single-sided buffer zones (inside the solid) are created to resolve the species discontinuities, and dual buffer zones (inside and outside the solid) are created to capture the temperature gradient discontinuities. The development discussed in this paper is limited to a two-dimensional Cartesian grid-conforming solid. We validate the code using benchmark simulations documented in the literature. We also demonstrate the overall second-order convergence of our numerical method. To demonstrate its capability, a reacting flow simulation of a methane/air premixed flame stabilized on a channel-confined bluff-body using a detailed chemical kinetics model is discussed. (C) 2014 Elsevier Inc. All rights reserved. C1 [Kedia, Kushal S.; Ghoniem, Ahmed F.] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Safta, Cosmin; Ray, Jaideep; Najm, Habib N.] Sandia Natl Labs, Livermore, CA USA. RP Ghoniem, AF (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. FU King Abdullah University of Science and Technology (KAUST) [KUS-11-010-01]; U.S. Department of Energy (DOE), Office of Basic Energy Sciences (BES) Division of Chemical Sciences, Geosciences, and Biosciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94-AL85000] FX This work was supported by King Abdullah University of Science and Technology (KAUST) award number KUS-11-010-01. This work was also supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences (BES) Division of Chemical Sciences, Geosciences, and Biosciences. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94-AL85000. NR 44 TC 6 Z9 6 U1 2 U2 12 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD SEP 1 PY 2014 VL 272 BP 408 EP 428 DI 10.1016/j.jcp.2014.04.019 PG 21 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AI1OP UT WOS:000336620900021 ER PT J AU Chacon, L del-Castillo-Negrete, D Hauck, CD AF Chacon, L. del-Castillo-Negrete, D. Hauck, C. D. TI An asymptotic-preserving semi-Lagrangian algorithm for the time-dependent anisotropic heat transport equation SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Asymptotic preserving methods; Anisotropic transport; Parallel transport; Operator-splitting ID DEFERRED CORRECTION METHODS; MAGNETIZED PLASMAS; DIFFUSION-EQUATIONS; OPTICALLY THICK; FINITE-ELEMENT; DYNAMICS; REGIMES; SCHEME; FLOW AB We propose a semi-Lagrangian numerical algorithm for a time-dependent, anisotropic temperature transport equation in magnetized plasmas in regimes with negligible variation of the magnitude of the magnetic field B along field lines. The approach is based on a formal integral solution of the parallel (i.e., along the magnetic field) transport equation with sources. While this study focuses on a Braginskii (local) heat flux closure, the approach is able to accommodate nonlocal parallel heat flux closures as well. The numerical implementation is based on an operator-split formulation, with two straightforward steps: a perpendicular transport step (including sources), and a Lagrangian (field-line integral) parallel transport step. Algorithmically, the first step is amenable to the use of modern iterative methods, while the second step has a fixed cost per degree of freedom (and is therefore algorithmically scalable). Accuracy-wise, the approach is free from the numerical pollution introduced by the discrete parallel transport term when the perpendicular to parallel transport coefficient ratio chi perpendicular to/chi parallel to becomes arbitrarily small, and is shown to capture the correct limiting solution when is an element of = chi perpendicular to L-parallel to(2)/chi parallel to L-perpendicular to(2)-> 0 (with L-parallel to, L (perpendicular to)the parallel and perpendicular diffusion length scales, respectively). Therefore, the approach is asymptotic-preserving. We demonstrate the performance of the scheme with several numerical experiments with varying magnetic field complexity in two dimensions, including the case of heat transport across a magnetic island in cylindrical geometry in the presence of a large guide field. Published by Elsevier Inc. C1 [Chacon, L.; del-Castillo-Negrete, D.; Hauck, C. D.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Chacon, L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Hauck, C. D.] Univ Tennessee, Knoxville, TN 37996 USA. RP Chacon, L (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM chacon@lanl.gov OI Chacon, Luis/0000-0002-4566-8763; del-Castillo-Negrete, Diego/0000-0001-7183-801X FU Office of Applied Scientific Computing Research; Office of Fusion Energy Sciences of the US Department of Energy; US Department of Energy at Oak Ridge National Laboratory [DE-AC05-000R22725]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX L.C. would like to thank N. Krasheninnikova for providing the fourth-order spatial discretization of the perpendicular transport equation. This work was sponsored by the Office of Applied Scientific Computing Research and the Office of Fusion Energy Sciences of the US Department of Energy. This work was performed under the auspices of the US Department of Energy at Oak Ridge National Laboratory, managed by UT-Battelle, LLC under contract DE-AC05-000R22725, and the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory, managed by LANS, LLC under contract DE-AC52-06NA25396. NR 44 TC 4 Z9 4 U1 4 U2 12 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD SEP 1 PY 2014 VL 272 BP 719 EP 746 DI 10.1016/j.jcp.2014.04.049 PG 28 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AI1OP UT WOS:000336620900039 ER PT J AU Phillips, CL AF Phillips, Carolyn L. TI A learning heuristic for space mapping and searching self-organizing systems using adaptive mesh refinement SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Self-assembly; Optimization; Adaptive mesh refinement ID ALGORITHMS; COMPLEX; GRIDS AB In a complex self-organizing system, small changes in the interactions between the system's components can result in different emergent macrostructures or macrobehavior. In chemical engineering and material science, such spontaneously self-assembling systems, using polymers, nanoscale or colloidal-scale particles, DNA, or other precursors, are an attractive way to create materials that are precisely engineered at a fine scale. Changes to the interactions can often be described by a set of parameters. Different contiguous regions in this parameter space correspond to different ordered states. Since these ordered states are emergent, often experiment, not analysis, is necessary to create a diagram of ordered states over the parameter space. By issuing queries to points in the parameter space (e.g., performing a computational or physical experiment), ordered states can be discovered and mapped. Queries can be costly in terms of resources or time, however. In general, one would like to learn the most information using the fewest queries. Here we introduce a learning heuristic for issuing queries to map and search a two-dimensional parameter space. Using a method inspired by adaptive mesh refinement, the heuristic iteratively issues batches of queries to be executed in parallel based on past information. By adjusting the search criteria, different types of searches (for example, a uniform search, exploring boundaries, sampling all regions equally) can be flexibly implemented. We show that this method will densely search the space, while preferentially targeting certain features. Using numerical examples, including a study simulating the self-assembly of complex crystals, we show how this heuristic can discover new regions and map boundaries more accurately than a uniformly distributed set of queries. (C) 2014 Elsevier Inc. All rights reserved. C1 Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Phillips, CL (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. FU Office of Naval Research; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; Office of the Director through the Named Postdoctoral Fellowship Program (Aneesur Rahman Postdoctoral Fellowship); Argonne National Laboratory FX This research was supported in part by a grant from the Office of Naval Research and in part by the U.S. Department of Energy, Office of Science, under Contract DE-AC02-06CH11357. C.L.P. was funded by the Office of the Director through the Named Postdoctoral Fellowship Program (Aneesur Rahman Postdoctoral Fellowship), Argonne National Laboratory. We acknowledge numerous useful discussions with Todd Munson, Tim Tautges, and Stefan Wild. We thank Michael Engel for providing the Injavis software package and Aaron Keys for the SMAC software package. Both the k-nearest-neighbor classifier and the support vector machine used software from the scikit-learn open source package [25]. NR 24 TC 0 Z9 0 U1 2 U2 14 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD SEP 1 PY 2014 VL 272 BP 799 EP 813 DI 10.1016/j.jcp.2014.05.001 PG 15 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AI1OP UT WOS:000336620900042 ER PT J AU Caballero, FG Miller, MK Garcia-Mateo, C AF Caballero, F. G. Miller, M. K. Garcia-Mateo, C. TI Opening previously impossible avenues for phase transformation in innovative steels by atom probe tomography SO MATERIALS SCIENCE AND TECHNOLOGY LA English DT Article DE Phase transformations; Bainite; Steels; Atom probe tomography (APT) ID BAINITE TRANSFORMATION; CARBIDE PRECIPITATION; SILICON STEEL; MARTENSITE; ACCOMMODATION; DISLOCATIONS; MICROSCOPY AB After decades of debate on the mechanism for the formation of bainite, it is accepted that bainite grows via a displacive mechanism, i.e. as plate shaped transformation products exhibiting an invariant plane strain surface relief effect. But there is still much discussion on the diffusion or diffusionless nature of bainite. The purpose of this atom probe tomography study was to track the atom distributions during the bainite reaction in steels with different carbon and silicon contents. The steels were transformed over a wide range of temperatures (200-525 degrees C) to elucidate the role of reaction rate and diffusion in the formation of bainite with and without cementite precipitation. C1 [Caballero, F. G.; Garcia-Mateo, C.] Natl Ctr Met Res CENIM CSIC, E-28040 Madrid, Spain. [Miller, M. K.] ORNL, Oak Ridge, TN 37831 USA. RP Caballero, FG (reprint author), Natl Ctr Met Res CENIM CSIC, Avda Gregorio del Amo 8, E-28040 Madrid, Spain. EM fgc@cenim.csic.es RI Garcia-Mateo, Carlos/A-7752-2008; CABALLERO, FRANCISCA/A-4292-2008; OI Garcia-Mateo, Carlos/0000-0002-4773-5077; Caballero, Francisca/0000-0002-5548-7659 FU ORNL's Shared Research Equipment User Facility - Office of Basic Energy Sciences, Scientific User Facilities Division, US Department of Energy; Spanish Ministry of Science and Innovation [MAT2010-15330] FX Research was supported by ORNL's Shared Research Equipment User Facility, which is sponsored by the Office of Basic Energy Sciences, Scientific User Facilities Division, US Department of Energy. The authors also gratefully acknowledge the support of the Spanish Ministry of Science and Innovation for funding this research under the contract MAT2010-15330 respectively. NR 32 TC 9 Z9 9 U1 1 U2 20 PU MANEY PUBLISHING PI LEEDS PA STE 1C, JOSEPHS WELL, HANOVER WALK, LEEDS LS3 1AB, W YORKS, ENGLAND SN 0267-0836 EI 1743-2847 J9 MATER SCI TECH-LOND JI Mater. Sci. Technol. PD SEP PY 2014 VL 30 IS 9 BP 1034 EP 1039 DI 10.1179/1743284714Y.0000000512 PG 6 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AI3DC UT WOS:000336738200006 ER PT J AU Capdevila, C Miller, MK AF Capdevila, C. Miller, M. K. TI Simultaneous Cr rich and Ti rich nanoprecipitation in ferritic steel designed for use in extreme environments of future energy generation systems SO MATERIALS SCIENCE AND TECHNOLOGY LA English DT Article DE Phase separation; Ferrous alloy; Mechanical alloying; Tomography; Thermoelectric power; Spinodal decomposition ID ATOM-PROBE; PHASE-SEPARATION; ALLOY; PRECIPITATION; DECOMPOSITION; KINETICS; DIFFUSION; LEVEL AB The temporal evolution of the microstructure resulting from phase separation into Fe rich (alpha), Cr rich (alpha'), and Fe(Ti,Al) (beta') phases of an oxide dispersion strengthened ferritic steel has been analysed by thermoelectric power measurements. The early stages of decomposition and the evolution of the threedimensional microstructure have been characterised by atom probe tomography. The roles of Cr, Al, and Ti during the decomposition process have been investigated in terms of solute partitioning between the phases. Analysis of proximity histograms revealed that significant Al and Ti partitioning occurs, which is consistent with theoretical calculations. The results indicate that both nanoscale precipitation processes occurs simultaneously, with an earlier completion time for beta' precipitation than alpha-alpha' phase separation. Finally, a value of activation energy for alpha-alpha' phase separation of 264 kJ mol(-1) was obtained from the analysis of thermoelectric power measurements data, which is consistent with a value of 248 kJ mol 21 for self-diffusion of Cr in alpha-Fe. C1 [Capdevila, C.] Ctr Nacl Invest Met CENIM CSIC, E-28040 Madrid, Spain. [Miller, M. K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Capdevila, C (reprint author), Ctr Nacl Invest Met CENIM CSIC, Avda Gregorio del Amo 8, E-28040 Madrid, Spain. EM ccm@cenim.csic.es RI Capdevila, Carlos/B-6970-2015 OI Capdevila, Carlos/0000-0002-1869-4085 FU Spanish Ministerio de Ciencia e Innovacion through in the form of a Coordinate Project in the Energy Area of Plan Nacional [ENE2009-13766-C04-01]; ORNL's Center for Nanophase Materials Sciences (CNMS) - Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX PM 2000 is a trademark of Plansee GmbH. LEAP is a registered trademark of Cameca Instruments. CC acknowledges financial support to Spanish Ministerio de Ciencia e Innovacion through in the form of a Coordinate Project in the Energy Area of Plan Nacional 2009 (ENE2009-13766-C04-01). Atom probe tomography and MKM were sponsored through a user project supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy NR 22 TC 0 Z9 0 U1 0 U2 16 PU MANEY PUBLISHING PI LEEDS PA STE 1C, JOSEPHS WELL, HANOVER WALK, LEEDS LS3 1AB, W YORKS, ENGLAND SN 0267-0836 EI 1743-2847 J9 MATER SCI TECH-LOND JI Mater. Sci. Technol. PD SEP PY 2014 VL 30 IS 9 BP 1079 EP 1085 DI 10.1179/1743284714Y.0000000531 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AI3DC UT WOS:000336738200013 ER PT J AU Johansson, T Pakhare, D Haynes, D Abdelsayed, V Shekhawat, D Spivey, J AF Johansson, Ted Pakhare, Devendra Haynes, Daniel Abdelsayed, Victor Shekhawat, Dushyant Spivey, James TI Characterization of LaRhO3 perovskites for dry (CO2) reforming of methane (DRM) SO CHEMICAL PAPERS LA English DT Article DE perovskite; LaRhO3; dry reforming of methane; temperature programmed reduction; temperature programmed surface reaction ID SYNTHESIS GAS; CATALYSTS; SUBSTITUTION; PERFORMANCE; REDUCTION; OXIDATION; CH4 AB This work reports on the characterization of LaRhO3 perovskite as a catalyst for dry reforming of methane. The catalyst was studied using CH4-temperature programmed reduction (TPR), H-2-TPR, and temperature programmed surface reaction (TPSR), and the changes in the crystal structure of the catalyst due to these treatments were studied by X-ray diffraction (XRD). XRD pattern of the freshly calcined perovskites showed the formation of highly crystalline LaRhO3 and La2O3 phases. H-2-TPR of the fresh calcined catalyst showed a shoulder at 342A degrees C and a broad peak at 448A degrees C, suggesting that the reduction of Rh in perovskite occurs in multiple steps. XRD pattern of the reduced catalyst suggests complete reduction of the LaRhO3 phase and the formation of metallic Rh and minor amounts of La(OH)(3). The CH4-TPR data show qualitatively similar results as H-2-TPR, with a shoulder and a broad peak in the same temperature range. Following the H-2-TPR up to 950A degrees C, the same batch of catalyst was oxidized by flowing 5 vol. % O-2/He up to 500A degrees C and a second H-2-TPR (also up to 950A degrees C) was conducted. This second H-2-TPR differed significantly from that of the fresh calcined catalyst. The single sharp peak at 163A degrees C in the second H-2-TPR suggests a significant change in the catalyst, probably causedby the transformation of about 90 % of the perovskite into Rh/La2O3. This was confirmed by the XRD studies of the catalyst reduced after the oxidation at 500A degrees C. TPSR of the dry reforming reaction on the fresh calcined catalyst showed CO and H-2 formation starting at 400A degrees C, with complete consumption of the reactants at 650A degrees C. The uneven consumption of reactants between 400A degrees C and 650A degrees C suggests that reactions other than DRM occur, including reverse water gas shift (RWGS) and the Boudouard reaction (BR), probably as a result of in-situ changes in the catalyst, consistent with the H-2-TPR results. TPSR, after a H-2-TPR up to 950A degrees C, showed that the dry reforming reaction did not light off until 570A degrees C, which is much higher temperature than the one observed using fresh calcined catalyst. This shows that the uniform sites produced during the 950A degrees C H-2-TPR are catalytically less active than those of the fresh calcined catalyst, and that no significant side reactions such as RWGS or the Boudouard reaction occur. This suggests that reduction leads to the formation of a single type of sites which do not catalyze simultaneous side reactions. C1 [Johansson, Ted] Royal Inst Technol, Sch Chem Sci & Engn, SE-10044 Stockholm, Sweden. [Pakhare, Devendra; Spivey, James] Louisiana State Univ, Dept Chem Engn, Baton Rouge, LA 70803 USA. [Haynes, Daniel; Abdelsayed, Victor; Shekhawat, Dushyant] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Spivey, J (reprint author), Louisiana State Univ, Dept Chem Engn, Baton Rouge, LA 70803 USA. EM jjspivey@lsu.edu FU Center for Atomic Level Catalyst Design, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001058] FX This paper is based upon a work supported as a part of the Center for Atomic Level Catalyst Design, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001058. This work was performed as a part of the ongoing CHUST program between LSU and KTH, Stockholm. NR 22 TC 4 Z9 4 U1 1 U2 59 PU DE GRUYTER OPEN LTD PI WARSAW PA SOLIPSKA 14A-1, 02-482 WARSAW, POLAND SN 0366-6352 EI 1336-9075 J9 CHEM PAP JI Chem. Pap. PD SEP PY 2014 VL 68 IS 9 BP 1240 EP 1247 DI 10.2478/s11696-014-0566-2 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA AH9EE UT WOS:000336443400011 ER PT J AU Dietrich, PJ Sollberger, FG Akatay, MC Stach, EA Delgass, WN Miller, JT Ribeiro, FH AF Dietrich, Paul J. Sollberger, Fred G. Akatay, M. Cem Stach, Eric A. Delgass, W. Nicholas Miller, Jeffrey T. Ribeiro, Fabio H. TI Structural and catalytic differences in the effect of Co and Mo as promoters for Pt-based aqueous phase reforming catalysts SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE Aqueous phase reforming; Pt bimetallic catalyst; Operand X-ray absorption spectroscopy; Hydrogen production from biomass ID SUPPORTED PLATINUM CATALYSTS; DENSITY-FUNCTIONAL THEORY; GAS SHIFT REACTION; ETHYLENE-GLYCOL; OXYGENATED HYDROCARBONS; ELECTRONIC-STRUCTURE; BIMETALLIC SURFACES; RHENIUM CATALYSTS; CARBON NANOTUBES; METAL-CATALYSTS AB Reaction rates (site time yields, normalized to CO chemisorption sites) and product selectivity were determined for PtCo, PtMo, and Pt supported on multi-walled carbon nanotubes for aqueous phase reforming of glycerol. The bimetallic PtCo and PtMo catalysts had 4.6x and 5.4x higher glycerol consumption rates than Pt, and 3.9x and 0.6x rates in H-2 formation compared to Pt. Hydrogen generation selectivity was similar on Pt and PtCo, but PtMo had an increase in selectivity to C-O cleavage products, which reduced H-2 yield at conversions over 60% (85-90% hydrogen yield for Pt and PtCo, 65% for PtMo). X-ray absorption spectroscopy and scanning transmission electron microscopy results indicate that PtCo adopts multiple mono- and bimetallic structures (Pt shell/Co core, well-mixed alloy, Pt only), which maintain surface Pt sites that are selective to hydrogen generation while adding a promotional metal that increases reaction rates. This is in contrast to a previously characterized PtMo catalyst which introduced surface sites capable of deoxygenation reactions (in the form of Pt Mo metallic or Pt MoO/OH acid pairs) which result in the observed decrease in selectivity. (C) 2014 Elsevier B.V. All rights reserved. C1 [Dietrich, Paul J.; Sollberger, Fred G.; Delgass, W. Nicholas; Ribeiro, Fabio H.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Akatay, M. Cem] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Akatay, M. Cem] Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Miller, Jeffrey T.] Argonne Natl Lab, Argonne, IL 60439 USA. [Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Ribeiro, FH (reprint author), Purdue Univ, Sch Chem Engn, 480 Stadium Mall Dr, W Lafayette, IN 47907 USA. EM fabio@purdue.edu RI BM, MRCAT/G-7576-2011; Stach, Eric/D-8545-2011; ID, MRCAT/G-7586-2011; OI Stach, Eric/0000-0002-3366-2153; Ribeiro, Fabio/0000-0001-7752-461X FU Atom-efficient Chemical Transformations (TACT); U.S. Department of Energy Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357, DE-AC02-98CH10886]; MRCAT member institutions FX This material is based upon work supported as part of the Institute for Atom-efficient Chemical Transformations (TACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. Scanning transmission electron microscopy was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The authors would like to thank Kaiwalya Sabnis and Yanran Cui for their assistance in collecting the water-gas shift reaction data. NR 46 TC 15 Z9 15 U1 3 U2 94 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD SEP PY 2014 VL 156 BP 236 EP 248 DI 10.1016/j.apcatb.2014.03.016 PG 13 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA AH3HB UT WOS:000336013200026 ER PT J AU Zhong, ZY Wang, W Wang, Q Zhang, WD Wang, Y Umar, A AF Zhong, Ziyi Wang, Wei Wang, Qiang Zhang, Wei-De Wang, Yu Umar, Ahmad TI A Special Section on Nanocatalysis and Their Applications SO JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY LA English DT Editorial Material C1 [Zhong, Ziyi] Inst Chem & Engn Sci, Singapore 627833, Singapore. [Wang, Wei] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Wang, Qiang] Beijing Forestry Univ, Coll Environm Sci & Engn, Beijing, Peoples R China. [Zhang, Wei-De] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou, Guangdong, Peoples R China. [Wang, Yu] Chongqing Univ, Sch Chem & Chem Engn, Chongqing, Peoples R China. [Umar, Ahmad] Najran Univ, Fac Sci & Arts, Dept Chem, PCSED, Najran, Saudi Arabia. RP Zhong, ZY (reprint author), Inst Chem & Engn Sci, 1 Pesek Rd, Singapore 627833, Singapore. RI Umar, Ahmad/H-9219-2012 OI Umar, Ahmad/0000-0002-8626-1564 NR 2 TC 1 Z9 1 U1 0 U2 21 PU AMER SCIENTIFIC PUBLISHERS PI VALENCIA PA 26650 THE OLD RD, STE 208, VALENCIA, CA 91381-0751 USA SN 1533-4880 EI 1533-4899 J9 J NANOSCI NANOTECHNO JI J. Nanosci. Nanotechnol. PD SEP PY 2014 VL 14 IS 9 BP 6789 EP 6791 DI 10.1166/jnn.2014.8919 PG 3 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH1IN UT WOS:000335873900041 PM 25924332 ER PT J AU Sharma, G Kodali, V Gaffrey, M Wang, W Minard, KR Karin, NJ Teeguarden, JG Thrall, BD AF Sharma, Gaurav Kodali, Vamsi Gaffrey, Matthew Wang, Wei Minard, Kevin R. Karin, Norman J. Teeguarden, Justin G. Thrall, Brian D. TI Iron oxide nanoparticle agglomeration influences dose rates and modulates oxidative stress-mediated dose-response profiles in vitro SO NANOTOXICOLOGY LA English DT Article DE nanotoxicology; agglomeration; iron oxide nanoparticles; oxidative stress; gene expression; dosimetry modelling ID PULMONARY INFLAMMATION; TOXICITY; PARTICLES; MODEL; SIZE; CELLS; VIVO; NANOTECHNOLOGY; SOLUBILITY; EXPRESSION AB Spontaneous agglomeration of engineered nanoparticles (ENPs) is a common problem in cell culture media which can confound interpretation of in vitro nanotoxicity studies. The authors created stable agglomerates of iron oxide nanoparticles (IONPs) in conventional culture medium, which varied in hydrodynamic size (276 nm-1.5 mu m) but were composed of identical primary particles with similar surface potentials and protein coatings. Studies using C10 lung epithelial cells show that the dose rate effects of agglomeration can be substantial, varying by over an order of magnitude difference in cellular dose in some cases. Quantification by magnetic particle detection showed that small agglomerates of carboxylated IONPs induced greater cytotoxicity and redox-regulated gene expression when compared with large agglomerates on an equivalent total cellular IONP mass dose basis, whereas agglomerates of amine-modified IONPs failed to induce cytotoxicity or redox-regulated gene expression despite delivery of similar cellular doses. Dosimetry modelling and experimental measurements reveal that on a delivered surface area basis, large and small agglomerates of carboxylated IONPs have similar inherent potency for the generation of ROS, induction of stress-related genes and eventual cytotoxicity. The results suggest that reactive moieties on the agglomerate surface are more efficient in catalysing cellular ROS production than molecules buried within the agglomerate core. Because of the dynamic, size and density-dependent nature of ENP delivery to cells in vitro, the biological consequences of agglomeration are not discernible from static measures of exposure concentration (mu g/ml) alone, highlighting the central importance of integrated physical characterisation and quantitative dosimetry for in vitro studies. The combined experimental and computational approach provides a quantitative framework for evaluating relationships between the biocompatibility of nanoparticles and their physical and chemical characteristics. C1 [Sharma, Gaurav] Battelle Mem Inst, Columbus, OH 43201 USA. [Sharma, Gaurav; Kodali, Vamsi; Gaffrey, Matthew; Minard, Kevin R.; Karin, Norman J.; Teeguarden, Justin G.; Thrall, Brian D.] Pacific NW Natl Lab, Div Biol Sci, Ctr Nanotoxicol, Richland, WA 99352 USA. [Wang, Wei] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Wang, Wei; Minard, Kevin R.; Karin, Norman J.; Teeguarden, Justin G.; Thrall, Brian D.] Battelle Ctr Fundamental & Appl Syst Toxicol, Richland, WA USA. RP Thrall, BD (reprint author), Pacific NW Natl Lab, Div Biol Sci, Ctr Nanotoxicol, Box 999,MS J4-02, Richland, WA 99352 USA. EM brian.thrall@pnnl.gov RI Wang, Wei/B-5924-2012; Kodali, Vamsi/D-2497-2009; Geracitano, Laura/E-6926-2013; OI Teeguarden, Justin/0000-0003-3817-4391; Kodali, Vamsi/0000-0001-6177-0568 FU Battelle Memorial Institute [PNNL 2119]; National Institutes of Health [U19 ES019544]; Battelle for the US Department of Energy [ACO6 76RLO 1830]; DOE FX Support for this research was provided by Battelle Memorial Institute under a cooperative research and development agreement (# PNNL 2119) and by the National Institutes of Health grant U19 ES019544. Pacific Northwest National Laboratory is operated by Battelle for the US Department of Energy under contract ACO6 76RLO 1830. The authors also thank Dr. Libor Kovarik for technical support with TEM images conducted at the Environmental Molecular Sciences Laboratory, a DOE-funded National User Facility at PNNL. NR 53 TC 33 Z9 33 U1 6 U2 210 PU INFORMA HEALTHCARE PI NEW YORK PA 52 VANDERBILT AVE, NEW YORK, NY 10017 USA SN 1743-5390 EI 1743-5404 J9 NANOTOXICOLOGY JI Nanotoxicology PD SEP PY 2014 VL 8 IS 6 BP 663 EP 675 DI 10.3109/17435390.2013.822115 PG 13 WC Nanoscience & Nanotechnology; Toxicology SC Science & Technology - Other Topics; Toxicology GA 267VY UT WOS:000328127600006 PM 23837572 ER PT J AU Mao, YG Damodaran, K AF Mao, Yougang Damodaran, Krishnan TI Ionization dynamics in ionic liquids probed via self-diffusion coefficient measurements SO CHEMICAL PHYSICS LA English DT Article DE Ionicity; Ion concentration; Thermodynamics; Non-Arrhenius behavior ID PHYSICOCHEMICAL PROPERTIES; CELLULOSE; SOLVENT; FUTURE; SYSTEM AB Ionic liquids contain ions and ion pairs with fast exchange between them. We propose a novel process to deduce the fraction of ions present in an ionic liquid and the equilibrium constants of ionization processes from measured ion self-diffusion coefficients using Pulsed Field Gradient (PFG) NMR. The enthalpy and entropy changes of ionization and ion self-diffusion processes are obtained for a series of ionic liquids using this method. These data were used to explain the interactions between cations and anions of ionic liquids. The interactions are also interpreted by the delocalization of the ion's charge densities. The self-diffusion coefficients of cations and anions for measured ionic liquids are discussed. (C) 2014 Elsevier B.V. All rights reserved. C1 [Damodaran, Krishnan] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. RP Damodaran, K (reprint author), Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM damodak@pitt.edu FU National Energy Technology Laboratory's (US-Department of Energy) under the RES [DE-FE0004000] FX This technical effort was performed in support of the National Energy Technology Laboratory's (US-Department of Energy) ongoing research in CO2 capture under the RES contract DE-FE0004000. NR 18 TC 6 Z9 6 U1 2 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD AUG 31 PY 2014 VL 440 BP 87 EP 93 DI 10.1016/j.chemphys.2014.06.014 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN4NP UT WOS:000340565000012 ER PT J AU Raman, RN Elhadj, S Laurence, TA Matthews, MJ AF Raman, R. N. Elhadj, S. Laurence, T. A. Matthews, M. J. TI The role of electronic defects and brittle microstructure in laser-driven material failure SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article DE fused silca; electronic defects; optical breakdown; thermal anneal; finite element model; crack healing; thermoelasticity ID FUSED-SILICA SURFACES; DAMAGE RESISTANCE; INDUCED BREAKDOWN; CRACKS; GLASS; NM; FRACTURE; TEMPERATURE; ABSORPTION; INTERFACE AB The microstructural thermal response of fused silica subjected to laser-induced breakdown was investigated. Rapid thermal annealing of laser modified material at the surface was achieved using a CO2 laser and the relaxation response of photoluminescence, infrared (IR) reflectance, electron and white light microscope images were recorded. Subsequent nanosecond-pulsed laser damage threshold measurements revealed thermally driven kinetics which were dominated by absorbing defect annealing at heat-treatment temperatures (T-HT) below similar to 1200K and material toughening at higher T-HT. A decrease in the peak photoluminescence lifetime with T-HT revealed two types of defects which were correlated with non-bridging IR vibrational modes. Near the glass transition temperature, a weakening of the laser modified material was observed and explained in terms of a residual compressive stress relaxation. A nonlinear absorption model was used to predict optical breakdown threshold and compared with critical fracture predictions based on crack tip annealing. Combined with a qualitative stress relaxation analysis, our model agrees well with the experimental data and yields insight to the rate-limiting contributions driving the onset of laser-induced breakdown in defective silica. C1 [Raman, R. N.; Elhadj, S.; Laurence, T. A.; Matthews, M. J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Raman, RN (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM raman4@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors acknowledge many useful and enlightening discussions with S G Demos, C W Carr, and J D Bude. The authors thank G Guss, D Cross, R Luthi, J Vickers, J Pryor, and W Hollingsworth for assistance with experiments. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 54 TC 1 Z9 1 U1 2 U2 23 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. 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Sarangi, T. Savin, A. Smith, W. H. Woods, N. CA CMS Collaboration TI Search for massive resonances in dijet systems containing jets tagged as W or Z boson decays in pp collisions at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jet substructure; Jets; Jet physics; Hadron-Hadron Scattering; Particle and resonance production ID PROTON-PROTON COLLISIONS; HADRON COLLIDERS; ATLAS DETECTOR; SPECTRUM; LEPTON AB A search is reported for massive resonances decaying into a quark and a vector boson (W or Z), or two vector bosons (WW, WZ, or ZZ). The analysis is performed on an inclusive sample of multijet events corresponding to an integrated luminosity of 19.7 fb(-1), collected in proton-proton collisions at a centre-of-mass energy of 8 TeV with the CMS detector at the LHC. The search uses novel jet-substructure identification techniques that provide sensitivity to the presence of highly boosted vector bosons decaying into a pair of quarks. Exclusion limits are set at a confidence level of 95% on the production of: (i) excited quark resonances q* decaying to qW and qZ for masses less than 3.2 TeV and 2.9 TeV, respectively, (ii) a Randall-Sundrum graviton G(RS) decaying into WW for masses below 1.2 TeV, and (iii) a heavy partner of the W boson W' decaying into WZ for masses less than 1.7 TeV. For the first time mass limits are set on W' -> WZ and G(RS) -> WW in the all-jets final state. The mass limits on q* -> qW, q* -> qZ, W' -> WZ, G(RS) -> WW are the most stringent to date. A model with a "bulk" graviton G(bulk) that decays into WW or ZZ bosons is also studied. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. 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Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Park, S.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Antunes, J. 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[Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; P. Fernandez Ramos, J.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; De Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Abdulsalam, A.; Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFCA, CSIC, E-39005 Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Mohanty, A. K.; Masetti, G.; Giordano, F.; Gori, V.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Di Guida, S.; Meola, S.; Paolucci, P.; Spiezia, A.; Palla, F.; Vernieri, C.; Micheli, F.; Argiro, S.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. 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Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Marrouche, J.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodoresc, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Richardson, C.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Dittmer, S.; Eggert, N.; Hopkins, W.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Fischer, R.; Acosta, D.; Avery, P.; Bourilkov, D.; Carver, M.; Cheng, T.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.; Xin, Y.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Malik, S.; Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Pearson, T.; Planer, M.; Ruchti, R.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Driga, O.; Elmer, P.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Mendez, H.; Vargas, JJ. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, MN USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Manganote, E. J. 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RI Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Montanari, Alessandro/J-2420-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Mundim, Luiz/A-1291-2012; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Scodellaro, Luca/K-9091-2014; Cerrada, Marcos/J-6934-2014; Dahms, Torsten/A-8453-2015; Ferguson, Thomas/O-3444-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Gonzalez Caballero, Isidro/E-7350-2010; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ragazzi, Stefano/D-2463-2009; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015 OI Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Heath, Helen/0000-0001-6576-9740; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476; Ferguson, Thomas/0000-0001-5822-3731; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ragazzi, Stefano/0000-0001-8219-2074; Codispoti, Giuseppe/0000-0003-0217-7021; FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COL-CIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COL-CIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 65 TC 48 Z9 48 U1 7 U2 78 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 29 PY 2014 IS 8 AR UNSP 173 DI 10.1007/JHEP08(2014)173 PG 37 WC Physics, Particles & Fields SC Physics GA AP0PC UT WOS:000341763300001 ER PT J AU Burgie, ES Wang, T Bussell, AN Walker, JM Li, HL Vierstra, RD AF Burgie, E. Sethe Wang, Tong Bussell, Adam N. Walker, Joseph M. Li, Huilin Vierstra, Richard D. TI Crystallographic and Electron Microscopic Analyses of a Bacterial Phytochrome Reveal Local and Global Rearrangements during Photoconversion SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Electron Microscopy (EM); Photomorphogenesis; Photoreceptor; Phototransduction; Plant Biochemistry; Protein Structure; X-ray Crystallography; Bilin; Photoconversion; Phytochrome ID PSEUDOMONAS-AERUGINOSA BACTERIOPHYTOCHROME; CHROMOPHORE-BINDING DOMAIN; CRYSTAL-STRUCTURE; GROUND-STATE; BILIVERDIN CHROMOPHORE; PLANT PHYTOCHROME; LIGHT; CYANOBACTERIOCHROMES; PHOTORECEPTORS; TRANSDUCTION AB Background: Phytochromes are dimeric bili-proteins central to photoperception by plants and microorganisms. Results: An informative perspective on photoconversion from the dark-adapted to the photoactivated state was provided by crystallographic and electron microscopic analyses of a bacterial version. Conclusion: Light-induced conformational changes in the bilin induce a large scale reorientation of the sister output modules. Significance: The structures offer a model for signal transmission by phytochromes. Phytochromes are multidomain photoswitches that drive light perception in plants and microorganisms by coupling photoreversible isomerization of their bilin chromophore to various signaling cascades. How changes in bilin conformation affect output by these photoreceptors remains poorly resolved and might include several species-specific routes. Here, we present detailed three-dimensional models of the photosensing module and a picture of an entire dimeric photoreceptor through structural analysis of the Deinococcus radiodurans phytochrome BphP assembled with biliverdin (BV). A 1.16- resolution crystal structure of the bilin-binding pocket in the dark-adapted red light-absorbing state illuminated the intricate network of bilin/protein/water interactions and confirmed the protonation and ZZZssa conformation of BV. Structural and spectroscopic comparisons with the photochemically compromised D207A mutant revealed that substitutions of Asp-207 allow inclusion of cyclic porphyrins in addition to BV. A crystal structure of the entire photosensing module showed a head-to-head, twisted dimeric arrangement with bowed helical spines and a hairpin protrusion connecting the cGMP phosphodiesterase/adenylyl cyclase/FhlA (GAF) and phytochrome-specific (PHY) domains. A key conserved hairpin feature is its anti-parallel, two -strand stem, which we show by mutagenesis to be critical for BphP photochemistry. Comparisons of single particle electron microscopic images of the full-length BphP dimer in the red light-absorbing state and the photoactivated far-red light-absorbing state revealed a large scale reorientation of the PHY domain relative to the GAF domain, which alters the position of the downstream histidine kinase output module. Together, our data support a toggle model whereby bilin photoisomerization alters GAF/PHY domain interactions through conformational modification of the hairpin, which regulates signaling by impacting the relationship between sister output modules. C1 [Burgie, E. Sethe; Bussell, Adam N.; Walker, Joseph M.; Vierstra, Richard D.] Univ Wisconsin, Dept Genet, Madison, WI 53706 USA. [Wang, Tong; Li, Huilin] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Li, Huilin] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. RP Vierstra, RD (reprint author), Univ Wisconsin, Dept Genet, 425-G Henry Mall, Madison, WI 53706 USA. EM vierstra@wisc.edu FU National Institutes of Health [R01 AI070285]; National Science Foundation [MCB-1329956]; Brookhaven National Laboratory Laboratory [10-16] FX This work was supported, in whole or in part, by National Institutes of Health Grant R01 AI070285 (to H. L.). This work was also supported by National Science Foundation Grant MCB-1329956 (to R. D. V.) and Brookhaven National Laboratory Laboratory-directed Research Project 10-16. NR 50 TC 20 Z9 20 U1 5 U2 27 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD AUG 29 PY 2014 VL 289 IS 35 BP 24573 EP 24587 DI 10.1074/jbc.M114.571661 PG 15 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AO7AY UT WOS:000341505600048 PM 25006244 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Homann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Roland, B Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Klein, B Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C Du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, TD Pol, ME Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Aleksandrov, A Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Mahmoud, MA Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Montoya, CAC De Oliveira, ACA Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Garcia, JG Geiser, A Gunnellini, P Hauk, J Hellwig, G Hempel, M Horton, D Jung, H Kasemann, M Katsas, P Kieseler, J Kleinwort, C Krucker, D Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Ron, E Sahin, MO Salfeld-Nebgen, J Saxena, P Schmidt, R Schoerner-Sadenius, T Schroder, M Spannagel, S Trevino, ADRV Walsh, R Wissing, C Martin, MA Blobel, V Vignali, MC Erfle, J Garutti, E Goebel, K Gorner, M Gosselink, M Haller, J Hoing, RS Kirschenmann, H Klanner, R Kogler, R Lange, J Lapsien, T Lenz, T Marchesini, I Ott, J Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Hartmann, F Hauth, T Husemann, U Katkov, I Kornmayer, A Kuznetsova, E 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Smith, W. H. Woods, N. CA CMS Collaboration TI Search for massive resonances decaying into pairs of boosted bosons in semi-leptonic final states at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Particle and resonance production; Jet substructure ID DYNAMICAL SYMMETRY-BREAKING; ATLAS DETECTOR; PP COLLISIONS; PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; HADRON-COLLISIONS; STANDARD MODEL; LHC; MASSES AB A search for new resonances decaying to WW, ZZ, or WZ is presented. Final states are considered in which one of the vector bosons decays leptonically and the other hadronically. Results are based on data corresponding to an integrated luminosity of 19.7 fb(-1) recorded in proton-proton collisions at root s= 8 TeV with the CMS detector at the CERN LHC. Techniques aiming at identifying jet substructures are used to analyze signal events in which the hadronization products from the decay of highly boosted W or Z bosons are contained within a single reconstructed jet. Upper limits on the production of generic WW, ZZ, or WZ resonances are set as a function of the resonance mass and width. We increase the sensitivity of the analysis by statistically combining the results of this search with a complementary study of the all-hadronic final state. Upper limits at 95% confidence level are set on the bulk graviton production cross section in the range from 700 to 10 fb for resonance masses between 600 and 2500 GeV, respectively. These limits on the bulk graviton model are the most stringent to date in the diboson final state. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoemann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Bansal, M.; Bansal, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Luyckx, S.; Ochesanu, S.; Roland, B.; Rougny, R.; Van De Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Daci, N.; Heracleous, N.; Kalogeropoulos, A.; Keaveney, J.; Kim, T. J.; Lowette, S.; Maes, M.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Dobur, D.; Favart, L.; Gay, A. P. R.; Grebenyuk, A.; Leonard, A.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Crucy, S.; Dildick, S.; Fagot, A.; Garcia, G.; Klein, B.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; Du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Komm, M.; Lemaitre, V.; Liao, J.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; Correa Martins Junior, M.; Dos Reis Martins, T.; Pol, M. E.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Alda Junior, W. L.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Malek, M.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santaolalla, J.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dias, F. A.; Fernandez Perez Tomei, T. R.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Genchev, V.; Iaydjiev, P.; Marinov, A.; Piperov, S.; Rodozov, M.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Du, R.; Jiang, C. H.; Liang, D.; Liang, S.; Plestina, R.; Tao, J.; Wang, X.; Wang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, Q.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Moreno, B. Gomez; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Elgammal, S.; Mahmoud, M. A.; Radi, A.] Acad Sci Res & Technol, Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, IRFU, DSM, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Charlot, C.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, CNRS IN2P3, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Montoya, C. A. Carrillo; De Oliveira, A. Carvalho Antunes; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, Univ Lyon, CNRS, IN2P3,Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Gunnellini, P.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Ron, E.; Sahin, M. Oe.; Salfeld-Nebgen, J.; Saxena, P.; Schmidt, R.; Schoerner-Sadenius, T.; Schroeder, M.; Spannagel, S.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] Deutsch Elekt Synchrotron, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Vignali, M. Centis; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Gosselink, M.; Haller, J.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kalsi, A. K.; Kaur, M.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] EHEP, Tata Inst Fundamental Res, Bombay, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dewanjee, R. K.; Dugad, S.] HECR, Tata Inst Fundamental Res, Bombay, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Grunewald, M.; Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Grunewald, M.; Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Biasotto, M.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Galanti, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Barone, L.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Foa, L.; Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Ligabue, F.; Barone, L.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Park, S.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrument Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Adzic, P.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia. [Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Contardo, D.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Silvestris, L.; Masetti, G.; Giordano, F.; Gori, V.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Di Guida, S.; Meola, S.; Paolucci, P.; Spiezia, A.; Palla, F.; Micheli, F.; Soffi, L.; Argiro, S.; Casasso, S.; Obertino, M. M.; Schizzi, A.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Wardle, N.; Woehri, H. K.; Zeuner, W. D.; Stickland, D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Tzeng, Y. M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Marrouche, J.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Richardson, C.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Kennedy, E.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Dittmer, S.; Eggert, N.; Hopkins, W.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Acosta, D.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Carver, M.; Cheng, T.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Pearson, T.; Planer, M.; Ruchti, R.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Driga, O.; Elmer, P.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Lucas, R.; Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. 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[Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A& M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calderon, Alicia/K-3658-2014; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Scodellaro, Luca/K-9091-2014; Cerrada, Marcos/J-6934-2014; Dahms, Torsten/A-8453-2015; Ferguson, Thomas/O-3444-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Montanari, Alessandro/J-2420-2012; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Gonzalez Caballero, Isidro/E-7350-2010; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016 OI Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Codispoti, Giuseppe/0000-0003-0217-7021; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476; Ferguson, Thomas/0000-0001-5822-3731; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Montanari, Alessandro/0000-0003-2748-6373; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Dudko, Lev/0000-0002-4462-3192; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626 FU Austrian Federal Ministry of Science and Research and the Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency(FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy and the Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR; Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion; Desarrollo e Innovacion and Programa Consolider-Ingenio, spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council and EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU; Regional Development Fund; Thalis and Aristeia programmes; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, co-financed by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 87 TC 41 Z9 41 U1 6 U2 73 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 29 PY 2014 IS 8 AR UNSP 174 DI 10.1007/JHEP08(2014)174 PG 59 WC Physics, Particles & Fields SC Physics GA AO8BW UT WOS:000341578500001 ER PT J AU Alna'Washi, GA Lu, M Habibi, M Esteves-Macaluso, D Wang, JC Phaneuf, RA Kilcoyne, ALD Cisneros, C McLaughlin, BM AF Alna'Washi, G. A. Lu, M. Habibi, M. Esteves-Macaluso, D. Wang, J. C. Phaneuf, R. A. Kilcoyne, A. L. D. Cisneros, C. McLaughlin, B. M. TI Valence-shell single photoionization of chlorine-like K2+ ions: Experiment and theory SO PHYSICAL REVIEW A LA English DT Article ID ATOMIC CHLORINE; CROSS-SECTIONS; OSCILLATOR-STRENGTHS; RR TELESCOPII; ENERGY-LEVELS; SPECTROSCOPY; SPECTRA; FORBIDDEN; LINES; 3S AB The absolute single-photoionization cross section was measured for Cl-like K2+ over the photon energy range from 44.2 to 69.7 eV at a constant energy resolution of 0.045 eV. The experiments were performed by merging an ion beam with a beam of synchrotron radiation from an undulator. The ground-state ionization threshold was measured at 0.004-eV energy resolution to be 45.717 +/- 0.030 eV. The measurements are rich in resonance structure due to multiple Rydberg series of transitions to autoionizing states. These series are assigned spectroscopically using the quantum defect method, guided by pseudorelativistic Hartree-Fock calculations for the energies and oscillator strengths of transitions to autoionizing states. The experimental results, which include significant contributions from K2+ ions initially in metastable states, are in satisfactory agreement with a linear superposition of semirelativistic R-matrix calculations of photoionization cross sections from these initial states. C1 [Alna'Washi, G. A.; Lu, M.; Habibi, M.; Esteves-Macaluso, D.; Wang, J. C.; Phaneuf, R. A.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. [Kilcoyne, A. L. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Cisneros, C.] Univ Nacl Autonoma Mexico, Inst Ciencias Fis, Cuernavaca 62210, Morelos, Mexico. [McLaughlin, B. M.] Inst Theoret Atom & Mol Phys, Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. RP Alna'Washi, GA (reprint author), Univ Nevada, Dept Phys, Reno, NV 89557 USA. EM alnawashi@hu.edu.jo RI Kilcoyne, David/I-1465-2013 FU Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy [DE-FG02-03ER15424, DE-AC03-76SF-00098]; PAPIT-UNAM, Mexico [IN107912-IN10261]; US National Science Foundation, under the visitors program; Queen's University Belfast; National Science Foundation [OCI-1053575]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX The Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy supported this research under Grant No. DE-FG02-03ER15424 and Contract No. DE-AC03-76SF-00098. C.C. acknowledges support from PAPIT-UNAM Grant No. IN107912-IN10261, Mexico. B.M.McL. acknowledges support by the US National Science Foundation, under the visitors program, through a grant to ITAMP at the Harvard-Smithsonian Center for Astrophysics, where this work was completed, and a visiting research fellowship from Queen's University Belfast. The computational work was performed at the National Energy Research Scientific Computing Center in Oakland, California, and on the Kraken XT5 facility at the National Institute for Computational Science (NICS) in Knoxville, Tennessee. The Kraken XT5 facility is a resource of the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant No. OCI-1053575. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 49 TC 0 Z9 1 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD AUG 29 PY 2014 VL 90 IS 2 AR 023417 DI 10.1103/PhysRevA.90.023417 PG 16 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AO0TV UT WOS:000341026200003 ER PT J AU Avila, ML Rogachev, GV Goldberg, VZ Johnson, ED Kemper, KW Tchuvil'sky, YM Volya, AS AF Avila, M. L. Rogachev, G. V. Goldberg, V. Z. Johnson, E. D. Kemper, K. W. Tchuvil'sky, Yu. M. Volya, A. S. TI alpha-cluster structure of O-18 SO PHYSICAL REVIEW C LA English DT Article ID INVERSE-KINEMATICS; ELASTIC-SCATTERING; UNSTABLE NUCLEI; LIGHT-NUCLEI; STATES; MODEL; ENERGY; NE-20; C-13(LI-6,P)O-18; RESONANCES AB Background: Clustering phenomena in N not equal Z nuclei provide an opportunity to understand the interplay between cluster and nucleon degrees of freedom. Purpose: To study resonances in the O-18 spectrum, populated in C-14 + alpha elastic scattering. Method: The thick target inverse kinematics technique was used to measure the excitation function for the C-14 + alpha elastic scattering. A 42-MeV C-14 beam was used to populate states of excitation energy up to 14.9 MeV in O-18. The analysis was performed using a multilevel, multichannel R-matrix approach. Results: Detailed spectroscopic information, including spin parities, partial alpha-and neutron-decay widths and dimensionless reduced widths, was obtained for excited states in O-18 between 8 and 14.9 MeV in excitation energy. Cluster-nucleon configuration interaction model calculations of the same quantities are performed and compared to the experimental results. Conclusions: Strong fragmentation of large a-cluster strengths is observed in the spectrum of O-18, making the a-cluster structure of O-18 quite different from the pattern of known quasirotational bands of alternating parity that are characteristic of N = Z, even-even nuclei like O-16 and Ne-20. C1 [Avila, M. L.; Johnson, E. D.; Kemper, K. W.; Volya, A. S.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Avila, M. L.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Rogachev, G. V.; Goldberg, V. Z.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Rogachev, G. V.; Goldberg, V. Z.] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA. [Tchuvil'sky, Yu. M.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. RP Avila, ML (reprint author), Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. EM mavila@anl.gov; rogachev@tamu.edu RI Rogachev, Grigory/J-2693-2015 FU National Science Foundation [PHY-456463]; U.S. Department of Energy [DE-SC0009883, DE-FG03-93ER40773] FX The authors would like to acknowledge the financial support provided by the National Science Foundation under Grant No. PHY-456463, the U.S. Department of Energy under Contracts No. DE-SC0009883 and No. DE-FG03-93ER40773. NR 69 TC 7 Z9 7 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 29 PY 2014 VL 90 IS 2 AR 024327 DI 10.1103/PhysRevC.90.024327 PG 19 WC Physics, Nuclear SC Physics GA AO0UL UT WOS:000341027800003 ER PT J AU McDonnell, JD Nazarewicz, W Sheikh, JA Staszczak, A Warda, M AF McDonnell, J. D. Nazarewicz, W. Sheikh, J. A. Staszczak, A. Warda, M. TI Excitation-energy dependence of fission in the mercury region SO PHYSICAL REVIEW C LA English DT Article ID ACTINIDE NUCLEI; ROTATING NUCLEI AB Background: Recent experiments on beta-delayed fission reported an asymmetric mass yield in the neutron-deficient nucleus Hg-180. Earlier experiments in the mass region A = 190-200 close to the beta-stability line, using the (p, f) and (alpha, f) reactions, observed a more symmetric distribution of fission fragments. While the beta-delayed fission of Hg-180 can be associated with relatively low excitation energy, this is not the case for light-ion reactions, which result in warm compound nuclei. The low-energy fission of Hg-180,Hg-198 has been successfully described by theory in terms of strong shell effects in pre-scission configurations associated with dinuclear structures. Purpose: To elucidate the roles of proton and neutron numbers and excitation energy in determining symmetric and asymmetric-fission yields, we compute and analyze the isentropic potential energy surfaces of Hg-174,Hg-180,Hg-198 and Po-196,Po-210. Methods: We use the finite-temperature superfluid nuclear density functional theory for excitation energies up to E* = 30 MeV and zero angular momentum. For our theoretical framework, we consider the Skyrme energy density functional SkM* and a density-dependent pairing interaction. Results: For Hg-174,Hg-180, we predict fission pathways consistent with asymmetric fission at low excitation energies, with the symmetric-fission pathway opening very gradually as excitation energy is increased. For Hg-198 and Po-196, we expect the nearly symmetric-fission channel to dominate. Po-210 shows a preference for a slightly asymmetric pathway at low energies, and a preference for a symmetric pathway at high energies. Conclusions: Our self-consistent theory suggests that excitation energy weakly affects the fission pattern of the nuclei considered. The transition from the asymmetric fission in the proton-rich nuclei to a more symmetric fission in the heavier isotopes is governed by the shell structure of pre-scission configurations. C1 [McDonnell, J. D.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94551 USA. [McDonnell, J. D.; Nazarewicz, W.; Sheikh, J. A.; Staszczak, A.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Nazarewicz, W.; Sheikh, J. A.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Nazarewicz, W.] Univ Warsaw, Inst Theoret Phys, PL-00681 Warsaw, Poland. [Sheikh, J. A.] Univ Kashmir, Dept Phys, Srinagar 190006, Jammu & Kashmir, India. [Staszczak, A.; Warda, M.] Marie Curie Sklodowska Univ, Dept Theoret Chem, PL-20031 Lublin, Poland. RP McDonnell, JD (reprint author), Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94551 USA. RI Warda, Michal/B-5619-2013 FU US Department of Energy [DE-FG02-96ER40963]; (University of Tennessee) [DE-NA0001820, DE-SC0008499]; Polish National Science Center [DEC-2011/01/B/ST2/03667]; NNSA SSGF Fellowship [DE-FC52-08NA28752]; US Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; nter for Computational Sciences (NCCS) FX Useful discussions with A. Andreyev and N. Schunck are gratefully acknowledged. This work was finalized during the Program INT-13-3 "Quantitative Large Amplitude Shape Dynamics: fission and heavy ion fusion" at the National Institute for Nuclear Theory in Seattle; it was supported by the US Department of Energy under Contracts No. DE-FG02-96ER40963 (University of Tennessee), No. DE-NA0001820 (the Stewardship Science Academic Alliances program), and No. DE-SC0008499 (NUCLEI SciDAC Collaboration). This work was partly supported by the Polish National Science Center Grant No. DEC-2011/01/B/ST2/03667. J.M. was funded by a NNSA SSGF Fellowship under Grant No. DE-FC52-08NA28752. This work was performed under the auspices of the US Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Computational resources were provided through an INCITE award " Computational Nuclear Structure" by the National Center for Computational Sciences (NCCS), and by the National Institute for Computational Sciences (NICS). NR 42 TC 16 Z9 16 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 29 PY 2014 VL 90 IS 2 AR 021302 DI 10.1103/PhysRevC.90.021302 PG 6 WC Physics, Nuclear SC Physics GA AO0UL UT WOS:000341027800001 ER PT J AU Prok, Y Bosted, P Kvaltine, N Adhikari, KP Adikaram, D Aghasyan, M Amaryan, MJ Anderson, MD Pereira, SA Avakian, H Baghdasaryan, H Ball, J Baltzell, NA Battaglieri, M Biselli, AS Bono, J Briscoe, WJ Brock, J Brooks, WK Bultmann, S Burkert, VD Carlin, C Carman, DS Celentano, A Chandavar, S Colaneri, L Cole, PL Contalbrigo, M Cortes, O Crabb, D Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Dodge, GE Doughty, D Dupre, R El Alaoui, A El Fassi, L Elouadrhiri, L Fedotov, G Fegan, S Fersch, R Fleming, JA Forest, TA Garcon, M Garillon, B Gevorgyan, N Ghandilyan, Y Gilfoyle, GP Girod, FX Giovanetti, KL Goetz, JT Gohn, W Gothe, RW Griffioen, KA Guegan, B Guler, N Hafidi, K Hanretty, C Harrison, N Hattawy, M Hicks, K Ho, D Holtrop, M Ilieva, Y Ireland, DG Ishkhanov, BS Isupov, EL Jawalkar, S Jiang, X Jo, HS Joo, K Kalantarians, N Keith, C Keller, D Khandaker, M Kim, A Kim, W Klein, A Klein, FJ Koirala, S Kubarovsky, V Kuhn, SE Kuleshov, SV Lenisa, P Livingston, K Lu, HY MacGregor, IJD Markov, N Mayer, M McKinnon, B Meekins, D Mineeva, T Mirazita, M Mokeev, V Montgomery, RA Moutarde, H Movsisyan, A Munevar, E Camacho, CM Nadel-Turonski, P Niccolai, S Niculescu, G Niculescu, I Osipenko, M Ostrovidov, AI Pappalardo, LL Paremuzyan, R Park, K Peng, P Phillips, JJ Pierce, J Pisano, S Pogorelko, O Pozdniakov, S Price, JW Procureur, S Protopopescu, D Puckett, AJR Raue, BA Rimal, D Ripani, M Rizzo, A Rosner, G Rossi, P Roy, P Sabatie, F Saini, MS Salgado, C Schott, D Schumacher, RA Seder, E Sharabian, YG Simonyan, A Smith, C Smith, G Sober, DI Sokhan, D Stepanyan, SS Stepanyan, S Strakovsky, II Strauch, S Sytnik, V Taiuti, M Tang, W Tkachenko, S Ungaro, M Vernarsky, B Vlassov, AV Voskanyan, H Voutier, E Walford, NK Watts, DP Weinstein, LB Zachariou, N Zana, L Zhang, J Zhao, B Zhao, ZW Zonta, I AF Prok, Y. Bosted, P. Kvaltine, N. Adhikari, K. P. Adikaram, D. Aghasyan, M. Amaryan, M. J. Anderson, M. D. Pereira, S. Anefalos Avakian, H. Baghdasaryan, H. Ball, J. Baltzell, N. A. Battaglieri, M. Biselli, A. S. Bono, J. Briscoe, W. J. Brock, J. Brooks, W. K. Bultmann, S. Burkert, V. D. Carlin, C. Carman, D. S. Celentano, A. Chandavar, S. Colaneri, L. Cole, P. L. Contalbrigo, M. Cortes, O. Crabb, D. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Dodge, G. E. Doughty, D. Dupre, R. El Alaoui, A. El Fassi, L. Elouadrhiri, L. Fedotov, G. Fegan, S. Fersch, R. Fleming, J. A. Forest, T. A. Garcon, M. Garillon, B. Gevorgyan, N. Ghandilyan, Y. Gilfoyle, G. P. Girod, F. X. Giovanetti, K. L. Goetz, J. T. Gohn, W. Gothe, R. W. Griffioen, K. A. Guegan, B. Guler, N. Hafidi, K. Hanretty, C. Harrison, N. Hattawy, M. Hicks, K. Ho, D. Holtrop, M. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Isupov, E. L. Jawalkar, S. Jiang, X. Jo, H. S. Joo, K. Kalantarians, N. Keith, C. Keller, D. Khandaker, M. Kim, A. Kim, W. Klein, A. Klein, F. J. Koirala, S. Kubarovsky, V. Kuhn, S. E. Kuleshov, S. V. Lenisa, P. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Markov, N. Mayer, M. McKinnon, B. Meekins, D. Mineeva, T. Mirazita, M. Mokeev, V. Montgomery, R. A. Moutarde, H. Movsisyan, A. Munevar, E. Camacho, C. Munoz Nadel-Turonski, P. Niccolai, S. Niculescu, G. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Pappalardo, L. L. Paremuzyan, R. Park, K. Peng, P. Phillips, J. J. Pierce, J. Pisano, S. Pogorelko, O. Pozdniakov, S. Price, J. W. Procureur, S. Protopopescu, D. Puckett, A. J. R. Raue, B. A. Rimal, D. Ripani, M. Rizzo, A. Rosner, G. Rossi, P. Roy, P. Sabatie, F. Saini, M. S. Salgado, C. Schott, D. Schumacher, R. A. Seder, E. Sharabian, Y. G. Simonyan, A. Smith, C. Smith, G. Sober, D. I. Sokhan, D. Stepanyan, S. S. Stepanyan, S. Strakovsky, I. I. Strauch, S. Sytnik, V. Taiuti, M. Tang, W. Tkachenko, S. Ungaro, M. Vernarsky, B. Vlassov, A. V. Voskanyan, H. Voutier, E. Walford, N. K. Watts, D. P. Weinstein, L. B. Zachariou, N. Zana, L. Zhang, J. Zhao, B. Zhao, Z. W. Zonta, I. TI Precision measurements of g(1) of the proton and of the deuteron with 6 GeV electrons SO PHYSICAL REVIEW C LA English DT Article ID SPIN STRUCTURE; INELASTIC EP; SCATTERING; NUCLEON; CLAS AB The inclusive polarized structure functions of the proton and deuteron, g(1)(p) and g(1)(d) , were measured with high statistical precision using polarized 6 GeV electrons incident on a polarized ammonia target in Hall B at Jefferson Laboratory. Electrons scattered at laboratory angles between 18 and 45 degrees were detected using the CEBAF Large Acceptance Spectrometer (CLAS). For the usual deep inelastic region kinematics, Q(2) > 1 GeV2 and the final-state invariant mass W > 2 GeV, the ratio of polarized to unpolarized structure functions g(1)/F-1 is found to be nearly independent of Q(2) at fixed x. Significant resonant structure is apparent at values of W up to 2.3 GeV. In the framework of perturbative quantum chromodynamics, the high-W results can be used to better constrain the polarization of quarks and gluons in the nucleon, as well as high-twist contributions. C1 [Prok, Y.; Adhikari, K. P.; Adikaram, D.; Amaryan, M. J.; Bultmann, S.; Dodge, G. E.; Guler, N.; Klein, A.; Koirala, S.; Kuhn, S. E.; Mayer, M.; Weinstein, L. B.] Old Dominion Univ, Norfolk, VA 23529 USA. [Prok, Y.; Bosted, P.; Avakian, H.; Brock, J.; Brooks, W. K.; Burkert, V. D.; Carlin, C.; Carman, D. S.; Deur, A.; Doughty, D.; Elouadrhiri, L.; Girod, F. X.; Keith, C.; Kubarovsky, V.; Meekins, D.; Mokeev, V.; Munevar, E.; Nadel-Turonski, P.; Park, K.; Pierce, J.; Raue, B. A.; Rossi, P.; Sharabian, Y. G.; Smith, C.; Stepanyan, S.; Ungaro, M.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Bosted, P.; Fersch, R.; Griffioen, K. A.; Jawalkar, S.; Zhao, B.] Coll William & Mary, Williamsburg, VA 23187 USA. [Kvaltine, N.; Baghdasaryan, H.; Crabb, D.; Hanretty, C.; Kalantarians, N.; Keller, D.; Peng, P.; Tkachenko, S.; Zhao, Z. W.] Univ Virginia, Charlottesville, VA 22901 USA. [Aghasyan, M.; Contalbrigo, M.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.] INFN, Sez Ferrara, I-44100 Ferrara, Italy. [Anderson, M. D.; Ireland, D. G.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Phillips, J. J.; Protopopescu, D.; Rosner, G.; Smith, G.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Pereira, S. Anefalos; De Sanctis, E.; Mirazita, M.; Montgomery, R. A.; Pisano, S.; Rossi, P.] INFN, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ball, J.; Fersch, R.; Garcon, M.; Moutarde, H.; Procureur, S.; Sabatie, F.] CEA, Ctr Saclay, Irfu Serv Phys Nucl0, F-91191 Gif Sur Yvette, France. [Baltzell, N. A.; Dupre, R.; El Alaoui, A.; El Fassi, L.; Hafidi, K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Baltzell, N. A.; Djalali, C.; Fedotov, G.; Gothe, R. W.; Ilieva, Y.; Lu, H. Y.; Park, K.; Strauch, S.; Zachariou, N.] Univ S Carolina, Columbia, SC 29208 USA. [Battaglieri, M.; Celentano, A.; De Vita, R.; Osipenko, M.; Ripani, M.; Taiuti, M.] INFN, Sez Genova, I-16146 Genoa, Italy. [Biselli, A. S.; Fegan, S.] Fairfield Univ, Fairfield, CT 06824 USA. [Bono, J.; Raue, B. A.; Rimal, D.; Schott, D.] Florida Int Univ, Miami, FL 33199 USA. [Briscoe, W. J.; Ilieva, Y.; Schott, D.; Strakovsky, I. I.] George Washington Univ, Washington, DC 20052 USA. [Brooks, W. K.; Kuleshov, S. V.; Sytnik, V.] Univ Tecn Fede Santa Maria, Valparaiso, Chile. [Chandavar, S.; Goetz, J. T.; Hicks, K.; Keller, D.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Colaneri, L.; D'Angelo, A.; Rizzo, A.; Zonta, I.] INFN, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Colaneri, L.; D'Angelo, A.; Rizzo, A.; Zonta, I.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Cole, P. L.; Cortes, O.; Forest, T. A.; Khandaker, M.; Movsisyan, A.] Idaho State Univ, Pocatello, ID 83209 USA. [Crede, V.; Ostrovidov, A. I.; Roy, P.; Saini, M. S.] Florida State Univ, Tallahassee, FL 32306 USA. [Dashyan, N.; Gevorgyan, N.; Ghandilyan, Y.; Paremuzyan, R.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Doughty, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Dupre, R.; Garillon, B.; Guegan, B.; Hattawy, M.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.; Pisano, S.; Sokhan, D.] Inst Phys Nucl, F-91406 Orsay, France. [Fedotov, G.; Ishkhanov, B. S.; Isupov, E. L.; Mokeev, V.] Moscow MV Lomonosov State Univ, Moscow 119234, Russia. [Fleming, J. A.; Watts, D. P.; Zana, L.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Gilfoyle, G. P.] Univ Richmond, Richmond, VA 23173 USA. [Giovanetti, K. L.; Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Gohn, W.; Harrison, N.; Joo, K.; Markov, N.; Mineeva, T.; Puckett, A. J. R.; Seder, E.; Ungaro, M.] Univ Connecticut, Storrs, CT 06269 USA. [Ho, D.; Schumacher, R. A.; Vernarsky, B.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Holtrop, M.; Zana, L.] Univ New Hampshire, Durham, NH 03824 USA. [Jiang, X.; Simonyan, A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Kim, A.; Kim, W.; Stepanyan, S. S.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Klein, F. J.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Kubarovsky, V.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Kubarovsky, V.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Voutier, E.] Univ Grenoble Alpes, LPSC, CNRS IN2P3, INPG, Grenoble, France. RP Prok, Y (reprint author), Old Dominion Univ, Norfolk, VA 23529 USA. EM yprok@jlab.org RI Celentano, Andrea/J-6190-2012; Rizzo, Alessandro/C-6397-2014; Adikaram, Dasuni/D-1539-2016; D'Angelo, Annalisa/A-2439-2012; Adikaram, D/H-7128-2016; Kuleshov, Sergey/D-9940-2013; Schumacher, Reinhard/K-6455-2013; Brooks, William/C-8636-2013; Lu, Haiyun/B-4083-2012; Ireland, David/E-8618-2010; El Alaoui, Ahmed/B-4638-2015; MacGregor, Ian/D-4072-2011; Sabatie, Franck/K-9066-2015; Osipenko, Mikhail/N-8292-2015; Zhang, Jixie/A-1461-2016 OI Celentano, Andrea/0000-0002-7104-2983; Rizzo, Alessandro/0000-0001-5597-8514; D'Angelo, Annalisa/0000-0003-3050-4907; Kuleshov, Sergey/0000-0002-3065-326X; Schumacher, Reinhard/0000-0002-3860-1827; Brooks, William/0000-0001-6161-3570; Ireland, David/0000-0001-7713-7011; Sabatie, Franck/0000-0001-7031-3975; Osipenko, Mikhail/0000-0001-9618-3013; FU U.S. Department of Energy; National Science Foundation; Italian Instituto Nazionale di Fisica Nucleare; French Centre National de la Recherche Scientifique; French Commissariat a l'Energie Atomique; United Kingdom's Science and Technology Facilities Council; Chilean CONICYT; National Research Foundation of Korea; Thomas Jefferson National Accelerator Facility [DE-AC05-06OR23177] FX We would like to acknowledge the outstanding efforts of the staff of the Accelerator and the Physics Divisions at Jefferson Lab that made this experiment possible. This work was supported in part by the U.S. Department of Energy and the National Science Foundation, the Italian Instituto Nazionale di Fisica Nucleare, the French Centre National de la Recherche Scientifique, the French Commissariat a l'Energie Atomique, the United Kingdom's Science and Technology Facilities Council, the Chilean CONICYT, and the National Research Foundation of Korea. The Southeastern Universities Research Association (SURA) operates the Thomas Jefferson National Accelerator Facility for the United States Department of Energy under Contract No. DE-AC05-06OR23177. NR 37 TC 14 Z9 14 U1 0 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 29 PY 2014 VL 90 IS 2 AR 025212 DI 10.1103/PhysRevC.90.025212 PG 18 WC Physics, Nuclear SC Physics GA AO0UL UT WOS:000341027800008 ER PT J AU Bielefeld, J Caldwell, RR Linder, EV AF Bielefeld, Jannis Caldwell, Robert R. Linder, Eric V. TI Dark energy scaling from dark matter to acceleration SO PHYSICAL REVIEW D LA English DT Article ID SOUTH-POLE TELESCOPE; DIGITAL SKY SURVEY; SCALAR FIELD; DATA RELEASE; COSMOLOGY AB The dark sector of the Universe need not be completely separable into distinct dark matter and dark energy components. We consider a model of early dark energy in which the dark energy mimics a dark matter component in both evolution and perturbations at early times. Barotropic aether dark energy scales as a fixed fraction, possibly greater than one, of the dark matter density and has vanishing sound speed at early times before undergoing a transition. This gives signatures not only in cosmic expansion but in sound speed and inhomogeneities, and in number of effective neutrino species. Model parameters describe the timing, sharpness of the transition, and the relative abundance at early times. Upon comparison with current data, we find viable regimes in which the dark energy behaves like dark matter at early times: for transitions well before recombination the dark energy to dark matter fraction can equal or exceed unity, while for transitions near recombination the ratio can only be a few percent. After the transition, dark energy goes its separate way, ultimately driving cosmic acceleration and approaching a cosmological constant in this scenario. C1 [Bielefeld, Jannis; Caldwell, Robert R.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. [Linder, Eric V.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Linder, Eric V.] Univ Calif Berkeley, Berkeley Lab, Berkeley, CA 94720 USA. [Linder, Eric V.] Ewha Womans Univ, Inst Early Universe WCU, Seoul 120750, South Korea. RP Bielefeld, J (reprint author), Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. OI Caldwell, Robert/0000-0001-7490-7463 FU DOE at Dartmouth [DE-SC0010386]; DOE at Berkeley [DE-SC-0007867]; Office of Science, Office of High Energy Physics, of the U. S. Department of Energy [DE-AC02-05CH11231]; Korea World Class University [R32-2009-000-10130] FX R. R. C. thanks the IEU for hospitality during part of this work. This work has been supported by DOE Grants No. DE-SC0010386 at Dartmouth, No. DE-SC-0007867 at Berkeley, and the Director, Office of Science, Office of High Energy Physics, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231, and Korea World Class University Grant No. R32-2009-000-10130. NR 41 TC 5 Z9 5 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 29 PY 2014 VL 90 IS 4 AR 043015 DI 10.1103/PhysRevD.90.043015 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO1MY UT WOS:000341077800002 ER PT J AU Lang, CB Leskovec, L Mohler, D Prelovsek, S Woloshyn, RM AF Lang, C. B. Leskovec, Luka Mohler, Daniel Prelovsek, Sasa Woloshyn, R. M. TI D-s mesons with DK and D * K scattering near threshold SO PHYSICAL REVIEW D LA English DT Article ID QUANTUM-FIELD THEORIES; LATTICE GAUGE-THEORY; VOLUME DEPENDENCE; ENERGY-SPECTRUM; FINITE-VOLUME; STATES; SPECTROSCOPY; MATRIX; SCALAR; QCD AB D-s mesons are studied in three quantum channels (J(P) = 0(+), 1(+) and 2(+)), where experiments have identified the very narrow D-s0* (2317), D-s1 (2460) and narrow D-s1 (2536), D-s2* (2573). We explore the effect of nearby DK and D*K thresholds on the subthreshold states using lattice QCD. Our simulation is done on two very different ensembles of gauge configurations (2 or 2 + 1 dynamical quarks, Pion mass of 266 or 156 MeV, lattice size 16(3) x 32 or 32(3) x 64). In addition to (q) over barq operators we also include meson-meson interpolators in the correlation functions. This clarifies the identification of the states above and below the scattering thresholds. The ensemble with m(pi) similar or equal to 156 MeV renders the D-s1 (2460) as a strong interaction bound state 44(10) MeV below D*K threshold, which is in agreement with the experiment. The D-s0* (2317) is found 37(17) MeV below DK threshold, close to the experiment value of 45 MeV. The narrow resonances D-s1 (2536) and D-s2* (2573) are also found close to the experimental masses. C1 [Lang, C. B.] Graz Univ, Inst Phys, A-8010 Graz, Austria. [Leskovec, Luka; Prelovsek, Sasa] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Mohler, Daniel] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Prelovsek, Sasa] Univ Ljubljana, Dept Phys, Ljubljana 1000, Slovenia. [Woloshyn, R. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. RP Lang, CB (reprint author), Graz Univ, Inst Phys, A-8010 Graz, Austria. EM christian.lang@uni-graz.at; luka.leskovec@ijs.si; dmohler@fnal.gov; sasa.prelovsek@ijs.si; rwww@triumf.ca OI Mohler, Daniel/0000-0003-1852-9562 FU Austrian Science Fund (FWF) [I1313-N27]; Slovenian Research Agency ARRS project [N1-0020]; Natural Sciences and Engineering Research Council of Canada; United States Department of Energy [De-AC02-07CH11359] FX We thank Anna Hasenfratz and the PACS-CS Collaboration for providing gauge configurations and Martin Luscher for making his DD-HMC software available. D. M. would like to thank E. Eichten, F.-K. Guo, M. Hansen, A. Kronfeld, Y. Liu and J. Simone for insightful discussions. The calculations were performed on computing clusters at TRIUMF, the University of Graz and at Jozef Stefan Institute. This work is supported in part by the Austrian Science Fund (FWF):[I1313-N27], by the Slovenian Research Agency ARRS project N1-0020 and by the Natural Sciences and Engineering Research Council of Canada. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. De-AC02-07CH11359 with the United States Department of Energy. Special thanks to the Institute for Nuclear Theory (University of Washington) for hospitality. NR 68 TC 44 Z9 44 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 29 PY 2014 VL 90 IS 3 AR 034510 DI 10.1103/PhysRevD.90.034510 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO1MW UT WOS:000341077600006 ER PT J AU Ligeti, Z Tackmann, FJ AF Ligeti, Zoltan Tackmann, Frank J. TI Precise predictions for B -> X-c tau(nu)over-bar decay distributions SO PHYSICAL REVIEW D LA English DT Article ID INCLUSIVE SEMILEPTONIC-B; LEPTON SPECTRUM; QCD CORRECTIONS; NONPERTURBATIVE CORRECTIONS; MASS AB We derive precise standard model predictions for the dilepton invariant mass and the tau energy distributions in inclusive B -> X-c tau(nu) over bar decay. We include Lambda(2)(QCD)/m(b)(2) and alpha(s) corrections using the 1S short-distance mass scheme, and estimate shape function effects near maximal tau energy. These results can improve the sensitivity of b -> c tau(nu) over bar related observables to beyond standard model physics. C1 [Ligeti, Zoltan] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tackmann, Frank J.] Deutsch Elektronen Synchrotron DESY, Theory Grp, D-22607 Hamburg, Germany. RP Ligeti, Z (reprint author), Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. FU Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; DFG Emmy-Noether [TA 867/1-1] FX We thank Phillip Urquijo for helpful discussions. This work was supported in part by the Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (Z. L.) and by the DFG Emmy-Noether Grant No. TA 867/1-1 (F. T.). NR 34 TC 4 Z9 4 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 29 PY 2014 VL 90 IS 3 AR 034021 DI 10.1103/PhysRevD.90.034021 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO1MW UT WOS:000341077600002 ER PT J AU Miao, HY Sangster, MY Livingstone, AM Hilchey, SP Zhang, L Topham, DJ Mosmann, TR Holden-Wiltse, J Perelson, AS Wu, HL Zand, MS AF Miao, Hongyu Sangster, Mark Y. Livingstone, Alexandra M. Hilchey, Shannon P. Zhang, Le Topham, David J. Mosmann, Tim R. Holden-Wiltse, Jeanne Perelson, Alan S. Wu, Hulin Zand, Martin S. TI Modeling the Dynamics and Migratory Pathways of Virus-Specific Antibody-Secreting Cell Populations in Primary Influenza Infection SO PLOS ONE LA English DT Article ID ANTIGEN PRESENTATION; LYMPHOID-TISSUE; CUTTING EDGE; T-CELLS; MICE; RESPONSES; MEMORY; LUNG; IDENTIFIABILITY; COMPARTMENTS AB The B cell response to influenza infection of the respiratory tract contributes to viral clearance and establishes profound resistance to reinfection by related viruses. Numerous studies have measured virus-specific antibody-secreting cell (ASC) frequencies in different anatomical compartments after influenza infection and provided a general picture of the kinetics of ASC formation and dispersion. However, the dynamics of ASC populations are difficult to determine experimentally and have received little attention. Here, we applied mathematical modeling to investigate the dynamics of ASC growth, death, and migration over the 2-week period following primary influenza infection in mice. Experimental data for model fitting came from high frequency measurements of virus-specific IgM, IgG, and IgA ASCs in the mediastinal lymph node (MLN), spleen, and lung. Model construction was based on a set of assumptions about ASC gain and loss from the sampled sites, and also on the directionality of ASC trafficking pathways. Most notably, modeling results suggest that differences in ASC fate and trafficking patterns reflect the site of formation and the expressed antibody class. Essentially all early IgA ASCs in the MLN migrated to spleen or lung, whereas cell death was likely the major reason for IgM and IgG ASC loss from the MLN. In contrast, the spleen contributed most of the IgM and IgG ASCs that migrated to the lung, but essentially none of the IgA ASCs. This finding points to a critical role for regional lymph nodes such as the MLN in the rapid generation of IgA ASCs that seed the lung. Results for the MLN also suggest that ASC death is a significant early feature of the B cell response. Overall, our analysis is consistent with accepted concepts in many regards, but it also indicates novel features of the B cell response to influenza that warrant further investigation. C1 [Miao, Hongyu; Zhang, Le; Holden-Wiltse, Jeanne; Wu, Hulin] Univ Rochester, Med Ctr, Dept Biostat & Computat Biol, Rochester, NY 14642 USA. [Sangster, Mark Y.; Livingstone, Alexandra M.; Topham, David J.; Mosmann, Tim R.] Univ Rochester, Med Ctr, Dept Microbiol & Immunol, David H Smith Ctr Vaccine Biol & Immunol, Rochester, NY 14642 USA. [Hilchey, Shannon P.; Zand, Martin S.] Univ Rochester, Med Ctr, Dept Med, Rochester, NY 14642 USA. [Perelson, Alan S.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Zand, MS (reprint author), Univ Rochester, Med Ctr, Dept Med, Rochester, NY 14642 USA. EM martin_zand@urmc.rochester.edu RI Zand, Martin/A-8612-2015; OI Zand, Martin/0000-0002-7095-8682 FU National Institute of Allergy and Infectious Diseases [HHSN272201000055C, R01 AI069351] FX This work was funded by the National Institute of Allergy and Infectious Diseases contract HHSN272201000055C and R01 AI069351 (MZ). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 45 TC 1 Z9 1 U1 0 U2 10 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 29 PY 2014 VL 9 IS 8 AR e104781 DI 10.1371/journal.pone.0104781 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AO2EE UT WOS:000341127500022 PM 25171166 ER PT J AU Lax, S Smith, DP Hampton-Marcell, J Owens, SM Handley, KM Scott, NM Gibbons, SM Larsen, P Shogan, BD Weiss, S Metcalf, JL Ursell, LK Vazquez-Baeza, Y Van Treuren, W Hasan, NA Gibson, MK Colwell, R Dantas, G Knight, R Gilbert, JA AF Lax, Simon Smith, Daniel P. Hampton-Marcell, Jarrad Owens, Sarah M. Handley, Kim M. Scott, Nicole M. Gibbons, Sean M. Larsen, Peter Shogan, Benjamin D. Weiss, Sophie Metcalf, Jessica L. Ursell, Luke K. Vazquez-Baeza, Yoshiki Van Treuren, Will Hasan, Nur A. Gibson, Molly K. Colwell, Rita Dantas, Gautam Knight, Rob Gilbert, Jack A. TI Longitudinal analysis of microbial interaction between humans and the indoor environment SO SCIENCE LA English DT Article ID HUMAN SKIN MICROBIOTA; DIVERSITY; HOUSE; BACTERIA; SURFACES; SPREAD; FUNGI; TIME AB The bacteria that colonize humans and our built environments have the potential to influence our health. Microbial communities associated with seven families and their homes over 6 weeks were assessed, including three families that moved their home. Microbial communities differed substantially among homes, and the home microbiome was largely sourced from humans. The microbiota in each home were identifiable by family. Network analysis identified humans as the primary bacterial vector, and a Bayesian method significantly matched individuals to their dwellings. Draft genomes of potential human pathogens observed on a kitchen counter could be matched to the hands of occupants. After a house move, the microbial community in the new house rapidly converged on the microbial community of the occupants' former house, suggesting rapid colonization by the family's microbiota. C1 [Lax, Simon; Smith, Daniel P.; Hampton-Marcell, Jarrad; Handley, Kim M.; Scott, Nicole M.; Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Lax, Simon; Smith, Daniel P.; Hampton-Marcell, Jarrad; Owens, Sarah M.; Handley, Kim M.; Scott, Nicole M.; Gibbons, Sean M.; Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Smith, Daniel P.] Baylor Coll Med, Dept Mol Virol & Microbiol, Alkek Ctr Metagen & Microbiome Res, Houston, TX 77030 USA. [Owens, Sarah M.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Gibbons, Sean M.; Gilbert, Jack A.] Univ Chicago, Grad Program Biophys Sci, Chicago, IL 60637 USA. [Larsen, Peter] Argonne Natl Lab, Dept Biosci, Argonne, IL 60439 USA. [Larsen, Peter] Univ Illinois, Dept Bioengn, Chicago, IL 60607 USA. [Shogan, Benjamin D.] Univ Chicago Med, Dept Surg, Chicago, IL 60637 USA. [Weiss, Sophie; Metcalf, Jessica L.; Ursell, Luke K.; Vazquez-Baeza, Yoshiki; Van Treuren, Will; Knight, Rob] Univ Colorado, Biofrontiers Inst, Boulder, CO 80304 USA. [Weiss, Sophie] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80304 USA. [Ursell, Luke K.; Vazquez-Baeza, Yoshiki; Knight, Rob] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80304 USA. [Vazquez-Baeza, Yoshiki] Univ Colorado, Dept Comp Sci, Boulder, CO 80304 USA. [Hasan, Nur A.; Colwell, Rita] CosmosID, College Pk, MD 20742 USA. [Hasan, Nur A.; Colwell, Rita] Univ Maryland, Inst Adv Comp Studies, Ctr Bioinformat & Computat Biol, College Pk, MD 20742 USA. [Gibson, Molly K.; Dantas, Gautam] Washington Univ, Sch Med, Ctr Genome Sci & Syst Biol, St Louis, MO 63108 USA. [Gibson, Molly K.; Dantas, Gautam] Washington Univ, Sch Med, Dept Pathol & Immunol, St Louis, MO 63110 USA. [Gibson, Molly K.; Dantas, Gautam] Washington Univ, Dept Biomed Engn, St Louis, MO 63130 USA. [Knight, Rob] Univ Colorado, Howard Hughes Med Inst, Boulder, CO 80309 USA. RP Gilbert, JA (reprint author), Univ Chicago, Dept Ecol & Evolut, 1101 E 57th St, Chicago, IL 60637 USA. EM gilbertjack@anl.gov RI Knight, Rob/D-1299-2010; OI Handley, Kim/0000-0003-0531-3009; Colwell, Rita R./0000-0001-5432-1502; Gibbons, Sean/0000-0002-8724-7916; Dantas, Gautam/0000-0003-0455-8370 FU Alfred P. Sloan Foundation's Microbiology of the Built Environment Program; NIH Director's New Innovator Award [DP2-DK-098089]; U.S. Environmental Protection Agency STAR Fellowship; NSF [DGE-11143954]; U.S. Department of Energy [DE-AC02-06CH11357]; University of Chicago Research Computing Center FX This work was supported by the Alfred P. Sloan Foundation's Microbiology of the Built Environment Program and a NIH Director's New Innovator Award (DP2-DK-098089) to G. D. S. M. G was supported by a U.S. Environmental Protection Agency STAR Fellowship. M. K. G. is a NSF graduate research fellow (award DGE-11143954). This work was supported in part by the U.S. Department of Energy under contract DE-AC02-06CH11357. We acknowledge the University of Chicago Research Computing Center for support of this work. All sequence data were submitted to the European Bioinformatics Institute's database under accession no. ERP005806. NR 19 TC 120 Z9 125 U1 19 U2 162 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 29 PY 2014 VL 345 IS 6200 BP 1048 EP 1052 DI 10.1126/science.1254529 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN8RE UT WOS:000340870900039 PM 25170151 ER PT J AU Carneiro, M Rubin, CJ Di Palma, F Albert, FW Alfoldi, J Barrio, AM Pielberg, G Rafati, N Sayyab, S Turner-Maier, J Younis, S Afonso, S Aken, B Alves, JM Barrell, D Bolet, G Boucher, S Burbano, HA Campos, R Chang, JL Duranthon, V Fontanesi, L Garreau, H Heiman, D Johnson, J Mage, RG Peng, Z Queney, G Rogel-Gaillard, C Ruffier, M Searle, S Villafuerte, R Xiong, AQ Young, S Forsberg-Nilsson, K Good, JM Lander, ES Ferrand, N Lindblad-Toh, K Andersson, L AF Carneiro, Miguel Rubin, Carl-Johan Di Palma, Federica Albert, Frank W. Alfoeldi, Jessica Barrio, Alvaro Martinez Pielberg, Gerli Rafati, Nima Sayyab, Shumaila Turner-Maier, Jason Younis, Shady Afonso, Sandra Aken, Bronwen Alves, Joel M. Barrell, Daniel Bolet, Gerard Boucher, Samuel Burbano, Hernan A. Campos, Rita Chang, Jean L. Duranthon, Veronique Fontanesi, Luca Garreau, Herve Heiman, David Johnson, Jeremy Mage, Rose G. Peng, Ze Queney, Guillaume Rogel-Gaillard, Claire Ruffier, Magali Searle, Steve Villafuerte, Rafael Xiong, Anqi Young, Sarah Forsberg-Nilsson, Karin Good, Jeffrey M. Lander, Eric S. Ferrand, Nuno Lindblad-Toh, Kerstin Andersson, Leif TI Rabbit genome analysis reveals a polygenic basis for phenotypic change during domestication SO SCIENCE LA English DT Article ID SELECTION; GENETICS; SWEEPS AB The genetic changes underlying the initial steps of animal domestication are still poorly understood. We generated a high-quality reference genome for the rabbit and compared it to resequencing data from populations of wild and domestic rabbits. We identified more than 100 selective sweeps specific to domestic rabbits but only a relatively small number of fixed (or nearly fixed) single-nucleotide polymorphisms (SNPs) for derived alleles. SNPs with marked allele frequency differences between wild and domestic rabbits were enriched for conserved noncoding sites. Enrichment analyses suggest that genes affecting brain and neuronal development have often been targeted during domestication. We propose that because of a truly complex genetic background, tame behavior in rabbits and other domestic animals evolved by shifts in allele frequencies at many loci, rather than by critical changes at only a few domestication loci. C1 [Carneiro, Miguel; Afonso, Sandra; Alves, Joel M.; Campos, Rita; Ferrand, Nuno] Univ Porto, CIBIO InBIO, Ctr Invest Biodiversidade & Recursos Genet, P-4485661 Vairao, Portugal. [Rubin, Carl-Johan; Barrio, Alvaro Martinez; Pielberg, Gerli; Rafati, Nima; Younis, Shady; Lindblad-Toh, Kerstin; Andersson, Leif] Uppsala Univ, Dept Med Biochem & Microbiol, Sci Life Lab Uppsala, Uppsala, Sweden. [Di Palma, Federica; Alfoeldi, Jessica; Turner-Maier, Jason; Chang, Jean L.; Heiman, David; Johnson, Jeremy; Young, Sarah; Lander, Eric S.; Lindblad-Toh, Kerstin] Broad Inst Harvard & Massachusetts Inst Technol, Cambridge, MA 02142 USA. [Di Palma, Federica] Genome Anal Ctr, Norwich, Norfolk, England. [Albert, Frank W.; Burbano, Hernan A.; Good, Jeffrey M.] Max Planck Inst Evolutionary Anthropol, Dept Evolutionary Genet, Leipzig, Germany. [Sayyab, Shumaila; Andersson, Leif] Swedish Univ Agr Sci, Dept Anim Breeding & Genet, Uppsala, Sweden. [Younis, Shady] Ain Shams Univ, Dept Anim Prod, Cairo, Egypt. [Aken, Bronwen; Barrell, Daniel; Ruffier, Magali; Searle, Steve] Wellcome Trust Sanger Inst, Hinxton, Cambs, England. [Aken, Bronwen; Barrell, Daniel; Ruffier, Magali] European Bioinformat Inst, European Mol Biol Lab, Cambridge CB10 1SD, England. [Alves, Joel M.] Univ Cambridge, Dept Genet, Cambridge CB2 3EH, England. [Bolet, Gerard; Garreau, Herve] INRA, Genet Physiol & Syst Elevage UMR1388, F-31326 Castanet Tolosan, France. [Boucher, Samuel] Labovet Conseil, F-85505 Les Herbiers, France. [Duranthon, Veronique] INRA, Biol Dev & Reprod UMR1198, F-78350 Jouy En Josas, France. [Fontanesi, Luca] Univ Bologna, Div Anim Sci, Dept Agr & Food Sci, I-40127 Bologna, Italy. [Mage, Rose G.] NIAID, Lab Immunol, NIH, Bethesda, MD 20892 USA. [Peng, Ze] US Dept Energy Joint Genome Inst, Lawrence Berkeley Natl Lab, Walnut Creek, CA 94598 USA. [Queney, Guillaume] ANTAGENE, Anim Genom Lab, Lyon, France. [Rogel-Gaillard, Claire] INRA, Genet Anim & Biol Integrat UMR1313, F-78350 Jouy En Josas, France. [Villafuerte, Rafael] IESA CSIC Campo Santo Martires 7, Inst Estudios Sociales Avanzados, Cordoba, Spain. [Xiong, Anqi; Forsberg-Nilsson, Karin] Uppsala Univ, Sci Life Lab, Dept Immunol Genet & Pathol, Uppsala, Sweden. [Good, Jeffrey M.] Univ Montana, Div Biol Sci, Missoula, MT 59812 USA. [Ferrand, Nuno] Univ Porto, Fac Ciencias, Dept Biol, P-4169007 Oporto, Portugal. [Andersson, Leif] Texas A&M Univ, Coll Vet Med & Biomed Sci, Dept Vet Integrat Biosci, College Stn, TX 77843 USA. RP Lindblad-Toh, K (reprint author), Uppsala Univ, Dept Med Biochem & Microbiol, Sci Life Lab Uppsala, Uppsala, Sweden. EM kersli@broadinstitute.org; leif.andersson@imbim.uu.se RI Fontanesi, Luca/L-1770-2014; Ferrand, Nuno /E-6085-2014; Afonso, Sandra/M-5702-2013; Carneiro, Miguel/L-7864-2013; OI Fontanesi, Luca/0000-0001-7050-3760; Ferrand, Nuno /0000-0002-2408-4195; Campos, Rita/0000-0003-4184-3269; Aken, Bronwen/0000-0002-3032-4095; Afonso, Sandra/0000-0001-7212-991X; Carneiro, Miguel/0000-0001-9882-7775; Ruffier, Magali/0000-0002-8386-1580; Burbano, Hernan A./0000-0003-3433-719X FU National Human Genome Research Institute [U54 HG003067]; European Research Council; Wellcome Trust [WT095908, WT098051]; NIH, NIAID; European Molecular Biology Laboratory; European Social Fund; Portuguese Ministerio da Ciencia, Tecnologia e Ensino Superior [SFRH/BPD/72343/2010, SFRH/BPD/64365/2009, SFRH/BD/72381/2010]; NSF [OISE-0754461]; FEDER through COMPETE program; Fundacao para a Ciencia e a Tecnologia [PTDC/CVT/122943/2010, PTDC/BIA-EVF/115069/2009, PTDC/BIA-BDE/72304/2006, PTDC/BIA-BDE/72277/2006]; project "Genomics and Evolutionary Biology" - North Portugal Regional Operational Programme (ON.2 - O Novo Norte) under National Strategic Reference Framework; project "Genomics Applied to Genetic Resources" - North Portugal Regional Operational Programme (ON.2 - O Novo Norte) under National Strategic Reference Framework; European Regional Development Fund (COST Action) [TD1101]; Higher Education Commission in Pakistan FX This work was supported by grants from the National Human Genome Research Institute (U54 HG003067 to E. S. L.), European Research Council project BATESON to L. A., the Wellcome Trust (grants WT095908 and WT098051), the intramural research program of the NIH, NIAID (R. G. M.), the European Molecular Biology Laboratory, Programa Operacional Potencial Humano-Quadro de Referencia Estrategica Nacional funds from the European Social Fund and Portuguese Ministerio da Ciencia, Tecnologia e Ensino Superior [postdoc grants to M. C. (SFRH/BPD/72343/2010) and R. C. (SFRH/BPD/64365/2009) and Ph.D. grant to J.M.A. (SFRH/BD/72381/2010)], a NSF international postdoctoral fellowship to J.M.G. (OISE-0754461), FEDER funds through the COMPETE program and Portuguese national funds through the Fundacao para a Ciencia e a Tecnologia (PTDC/CVT/122943/2010, PTDC/BIA-EVF/115069/2009, PTDC/BIA-BDE/72304/2006, and PTDC/BIA-BDE/72277/2006), the projects "Genomics and Evolutionary Biology" and "Genomics Applied to Genetic Resources" cofinanced by North Portugal Regional Operational Programme 2007/2013 (ON.2 - O Novo Norte) under the National Strategic Reference Framework and the European Regional Development Fund, travel grants to M. C. (COST Action TD1101), and Higher Education Commission in Pakistan (support for Sh.S.). We are grateful to L. Gaffney for assistance with figure preparation, P. C. Alves and S. Mills for providing the snowshoe hare sample, and S. Paabo for hosting M. C., S. A., and R. C. Sequencing was performed by the Broad Institute Genomics Platform. Computer resources were supplied by BITS and UPPNEX at Science for Life Laboratory. The O. cuniculus genome assembly has been deposited in GenBank under the accession number AAGW02000000. The RNA sequencing data have been deposited in GenBank under the bioproject PRJNA78323, the rabbit genome resequencing data under the bioproject PRJNA242290, and the sequence capture data under the bioproject PRJNA221358. NR 18 TC 49 Z9 51 U1 12 U2 93 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 29 PY 2014 VL 345 IS 6200 BP 1074 EP 1079 DI 10.1126/science.1253714 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN8RE UT WOS:000340870900046 PM 25170157 ER PT J AU Li, NB Ren, J AF Li, Nianbei Ren, Jie TI Non-Reciprocal Geometric Wave Diode by Engineering Asymmetric Shapes of Nonlinear Materials SO SCIENTIFIC REPORTS LA English DT Article ID STATE THERMAL RECTIFIER; OPTICAL DIODE; RECTIFICATION; TRANSPORT AB Unidirectional nonreciprocal transport is at the heart of many fundamental problems and applications in both science and technology. Here we study the novel design of wave diode devices by engineering asymmetric shapes of nonlinear materials to realize the function of non-reciprocal wave propagations. We first show analytical results revealing that both nonlinearity and asymmetry are necessary to induce such non-reciprocal (asymmetric) wave propagations. Detailed numerical simulations are further performed for a more realistic geometric wave diode model with typical asymmetric shape, where good non-reciprocal wave diode effect is demonstrated. Finally, we discuss the scalability of geometric wave diodes. The results open a flexible way for designing wave diodes efficiently simply through shape engineering of nonlinear materials, which may find broad implications in controlling energy, mass and information transports. C1 [Li, Nianbei] Tongji Univ, Sch Phys Sci & Engn, Ctr Phonon & Thermal Energy Sci, Shanghai 200092, Peoples R China. [Ren, Jie] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ren, Jie] MIT, Dept Chem, Cambridge, MA 02139 USA. RP Ren, J (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM jieren@mit.edu RI Li, Nianbei/B-6055-2011; Ren, Jie/G-5314-2010 OI Li, Nianbei/0000-0002-9151-7675; Ren, Jie/0000-0003-2806-7226 FU Shanghai Supercomputer Center; National Natural Science Foundation of China [11205114]; Shanghai Rising-Star Program [13QA1403600]; National Nuclear Security Administration of the U.S. DOE at LANL through the LDRD Program [DE-AC52-06NA25396]; Center for Excitonics (MIT) - US Department of Energy, Office of Basic Energy Sciences [DE-SC0001088] FX N.L. acknowledges the supports from Shanghai Supercomputer Center, the National Natural Science Foundation of China, Grant No. 11205114, and Shanghai Rising-Star Program with Grant No. 13QA1403600. J.R. thanks the support by the National Nuclear Security Administration of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396 through the LDRD Program. Jie is also partially supported by the Center for Excitonics (MIT) funded by the US Department of Energy, Office of Basic Energy Sciences (DE-SC0001088). NR 46 TC 5 Z9 5 U1 4 U2 39 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 29 PY 2014 VL 4 AR 6228 DI 10.1038/srep06228 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AO0SU UT WOS:000341023000001 PM 25169668 ER PT J AU Roux, S Hawley, AK Beltran, MT Scofield, M Schwientek, P Stepanauskas, R Woyke, T Hallam, SJ Sullivan, MB AF Roux, Simon Hawley, Alyse K. Beltran, Monica Torres Scofield, Melanie Schwientek, Patrick Stepanauskas, Ramunas Woyke, Tanja Hallam, Steven J. Sullivan, Matthew B. TI Ecology and evolution of viruses infecting uncultivated SUP05 bacteria as revealed by single-cell- and meta- genomics SO ELIFE LA English DT Article DE SUP05; bacteriophages; viruses; single cell genomics; oxygen minimum zones; viral dark matter ID OXYGEN-MINIMUM ZONES; DISSIMILATORY SULFITE REDUCTASE; MARINE VIRUSES; DARK OCEAN; PHOTOSYNTHESIS GENES; DNA VIRUSES; WATERS; SEA; COMMUNITIES; RESISTANCE AB Viruses modulate microbial communities and alter ecosystem functions. However, due to cultivation bottlenecks specific virus-host interaction dynamics remain cryptic. Here we examined 127 single-cell amplified genomes (SAGs) from uncultivated SUP05 bacteria isolated from a marine oxygen minimum zone (OMZ) to identify 69 viral contigs representing five new genera within dsDNA Caudovirales and ssDNA Microviridae. Infection frequencies suggest that similar to 1/3 of SUP05 bacteria are viral-infected, with higher infection frequency where oxygen-deficiency was most severe. Observed Microviridae clonality suggests recovery of bloom-terminating viruses, while systematic co-infection between dsDNA and ssDNA viruses posits previously unrecognized cooperation modes. Analyses of 186 microbial and viral metagenomes revealed that SUP05 viruses persisted for years, but remained endemic to the OMZ. Finally, identification of virus-encoded dissimilatory sulfite reductase suggests SUP05 viruses reprogram their host's energy metabolism. Together these results demonstrate closely coupled SUP05 virus-host co-evolutionary dynamics with potential to modulate biogeochemical cycling in climate-critical and expanding OMZs. C1 [Roux, Simon; Sullivan, Matthew B.] Univ Arizona, Tucson, AZ 85721 USA. [Hawley, Alyse K.; Beltran, Monica Torres; Scofield, Melanie; Hallam, Steven J.] Univ British Columbia, Dept Microbiol & Immunol, Vancouver, BC V5Z 1M9, Canada. [Schwientek, Patrick; Woyke, Tanja] DOE Joint Genome Inst, Walnut Creek, CA USA. [Stepanauskas, Ramunas] Bigelow Lab Ocean Sci, East Boothbay, ME USA. [Hallam, Steven J.] Univ British Columbia, Grad Program Bioinformat, Vancouver, BC V5Z 1M9, Canada. RP Sullivan, MB (reprint author), Life Sci South, Off LSS246, Lab LSS203 LSS207, Ecol & Evolutionary Biol Dept, 1007 East Lowell St, Tucson, AZ 85721 USA. EM shallam@mail.ubc.ca; mbsulli@email.arizona.edu RI Sullivan, Matthew/H-3256-2011 OI Sullivan, Matthew/0000-0003-4040-9831 FU U.S. Department of Energy Joint Genome Institute - Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; G. Unger Vetlesen Foundation; Ambrose Monell Foundation; Tula Foundation - Centre for Microbial Diversity and Evolution; Natural Sciences and Engineering Research Council (NSERC) of Canada; Canada Foundation for Innovation (CFI); Canadian Institute for Advanced Research (CIFAR); BIO5, NSF [OCE-0961947]; Gordon and Betty Moore Foundation [3790]; NSF [OCE-821374, OCE-1019242]; State of Maine Technology Institute FX We thank the crew aboard the MSV John Strickland for logistical and sampling support in Saanich Inlet and Melanie Scofield, Jody Wright, Evan Durno, and Elena Zaikova in the Hallam lab for technical assistance. We also thank the Joint Genome Institute, including IMG and GOLD teams and Sussanah Tringe, Stephanie Malfatti and Tijana Glavina del Rio for technical and project management assistance. This work was performed under the auspices of the U.S. Department of Energy Joint Genome Institute supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231; the G. Unger Vetlesen and Ambrose Monell Foundations and the Tula Foundation funded Centre for Microbial Diversity and Evolution, Natural Sciences and Engineering Research Council (NSERC) of Canada, Canada Foundation for Innovation (CFI), and the Canadian Institute for Advanced Research (CIFAR) through grants awarded to S.J.H; and BIO5, NSF (OCE-0961947) and the Gordon and Betty Moore Foundation (#3790) through grants awarded to M. B. S. Single cell genomics instrumentation at Bigelow Laboratory for Ocean Sciences was supported by NSF grants OCE-821374 and OCE-1019242 to R. S. and by the State of Maine Technology Institute. The single cell genome sequences and annotations can be accessed via IMG (img.jgi.doe.gov, SAG Ids are listed in Supplementary file 4). Viral contigs and defective prophages identified in the SUP05 SAG are available on the Metavir webserver (http://metavir-meb.univ-bpclermont.fr/), as virome "SUP05_viral_sequences" in project "SUP05_SAGs". The web servers hosting viral and microbial metagenome sequences used here are listed in Supplementary file 5. NR 100 TC 41 Z9 41 U1 3 U2 42 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD AUG 29 PY 2014 VL 3 AR e03125 DI 10.7554/eLife.03125 PG 39 WC Biology SC Life Sciences & Biomedicine - Other Topics GA AO3TF UT WOS:000341258100005 PM 25171894 ER PT J AU Malaspina, DM Andersson, L Ergun, RE Wygant, JR Bonnell, JW Kletzing, C Reeves, GD Skoug, RM Larsen, BA AF Malaspina, D. M. Andersson, L. Ergun, R. E. Wygant, J. R. Bonnell, J. W. Kletzing, C. Reeves, G. D. Skoug, R. M. Larsen, B. A. TI Nonlinear electric field structures in the innermagnetosphere SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE Dipolarizations; Nonlinear Electric Fields; Inner Magnetosphere; Radiation Belts ID POLAR OBSERVATIONS; SOLITARY WAVES; DOUBLE-LAYERS; ACCELERATION; PLASMA AB Van Allen Probes observations are presented which demonstrate the presence of nonlinear electric field structures in the inner terrestrial magnetosphere (<6 R-E). A range of structures are observed, including phase space holes and double layers. These structures are observed over several Earth radii in radial distance and over a wide range of magnetic local times. They are observed in the dusk, midnight, and dawn sectors, with the highest concentration premidnight. Some nonlinear electric field structures are observed to coincide with dipolarizations of the magnetic field and increases in electron energy flux for energies between 1 keV and 30 keV. Nonlinear electric field structures possess isolated impulsive electric fields, often with a significant component parallel to the ambient magnetic field, providing a mechanism for nonadiabatic wave-particle interactions in the inner magnetosphere. C1 [Malaspina, D. M.; Andersson, L.; Ergun, R. E.] Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. [Wygant, J. R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Bonnell, J. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Kletzing, C.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Reeves, G. D.; Skoug, R. M.; Larsen, B. A.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Malaspina, DM (reprint author), Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. EM David.Malaspina@colorado.edu RI Larsen, Brian/A-7822-2011; Reeves, Geoffrey/E-8101-2011; OI Larsen, Brian/0000-0003-4515-0208; Reeves, Geoffrey/0000-0002-7985-8098; Kletzing, Craig/0000-0002-4136-3348 FU NASA [NAS5-01072]; Van Allen Probes team; EFW team; EMFISIS team; HOPE team FX The authors thank the Van Allen Probes team, especially the EFW, EMFISIS, and HOPE teams for their support. This work was funded by NASA award NAS5-01072. All data used in this work is available from the EFW, EMFISIS, and HOPE teams. NR 31 TC 26 Z9 26 U1 0 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2014 VL 41 IS 16 BP 5693 EP 5701 DI 10.1002/2014GL061109 PG 9 WC Geosciences, Multidisciplinary SC Geology GA AQ4HT UT WOS:000342755400001 ER PT J AU Chen, LJ Thorne, RM Bortnik, J Li, W Horne, RB Reeves, GD Kletzing, CA Kurth, WS Hospodarsky, GB Spence, HE Blake, JB Fennell, JF AF Chen, Lunjin Thorne, Richard M. Bortnik, Jacob Li, Wen Horne, Richard B. Reeves, G. D. Kletzing, C. A. Kurth, W. S. Hospodarsky, G. B. Spence, H. E. Blake, J. B. Fennell, J. F. TI Generation of unusually low frequency plasmaspheric hiss SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE plasmaspheric hiss; ray tracing; chorus; generation ID DISCRETE CHORUS EMISSIONS; ORIGIN; MAGNETOSPHERE; RADIATION AB It has been reported from Van Allen Probe observations that plasmaspheric hiss intensification in the outer plasmasphere, associated with a substorm injection on 30 September 2012, occurred with a peak frequency near 100 Hz, well below the typical plasmaspheric hiss frequency range, extending down to approximate to 20 Hz. We examine this event of unusually low frequency plasmaspheric hiss to understand its generation mechanism. Quantitative analysis is performed by simulating wave raypaths via the HOTRAY ray tracing code with measured plasma density and calculating raypath-integrated wave gain evaluated using the measured energetic electron distribution. We demonstrate that the growth rate due to substorm-injected electrons is positive but rather weak, leading to small wave gain (approximate to 10 dB) during a single equatorial crossing. Propagation characteristics aided by the sharp density gradient associated with the plasmapause, however, can enable these low-frequency waves to undergo cyclic raypaths, which return to the unstable region leading to repeated amplification to yield sufficient net wave gain (>40 dB) to allow waves to grow from the thermal noise. C1 [Chen, Lunjin] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Thorne, Richard M.; Bortnik, Jacob; Li, Wen] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA USA. [Horne, Richard B.] NERC, British Antarct Survey, Cambridge, England. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Kletzing, C. A.; Kurth, W. S.; Hospodarsky, G. B.] Univ Iowa, Dept Phys & Astron, Iowa City, IA USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Blake, J. B.; Fennell, J. F.] Aerosp Corp, Los Angeles, CA 90009 USA. RP Chen, LJ (reprint author), Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. EM lunjin.chen@gmail.com RI Reeves, Geoffrey/E-8101-2011; OI Reeves, Geoffrey/0000-0002-7985-8098; Horne, Richard/0000-0002-0412-6407; Kletzing, Craig/0000-0002-4136-3348; Kurth, William/0000-0002-5471-6202; Hospodarsky, George/0000-0001-9200-9878 FU NSF [GEM-1405041, AGS-0840178]; NASA LWS grant [NNX13AI61G]; JHU/APL under NASA [967399, 921647, NAS5-01072]; EMFISIS subaward [1001057397:01]; ECT [13-041] FX We acknowledge the Van Allen Probes data from the EMFISIS instrument obtained from https://emfisis.physics.uiowa.edu/data/index and from the MagEIS instrument obtained from http://www.rbsp-ect.lanl.gov/data_pub/. This work was supported by NSF GEM-1405041 and AGS-0840178, NASA LWS grant NNX13AI61G and JHU/APL contracts 967399 and 921647 under NASA's prime contract NAS5-01072. The analysis at UCLA was supported by the EMFISIS subaward 1001057397:01 and by the ECT subaward 13-041. NR 32 TC 11 Z9 11 U1 1 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2014 VL 41 IS 16 BP 5702 EP 5709 DI 10.1002/2014GL060628 PG 8 WC Geosciences, Multidisciplinary SC Geology GA AQ4HT UT WOS:000342755400002 ER PT J AU Johnson, JR Wing, S AF Johnson, Jay R. Wing, Simon TI External versus internal triggering of substorms: An information-theoretical approach SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE substorm; external triggering; information theory; conditional redundancy ID INTERPLANETARY MAGNETIC-FIELD; MAGNETOSPHERIC SUBSTORMS; NORTHWARD TURNINGS; CURRENT DISRUPTION; GEOMAGNETIC TAIL; ONSETS AB The role of external triggering of substorms through northward turning of the interplanetary magnetic field has been examined in a number of recent studies. While Hsu and McPherron (2002, 2004) argue that the strong association between external triggers defined by Lyons et al. (1997) and substorm onsets could be responsible for most substorms, Morley and Freeman (2007) argue that the association between northward interplanetary magnetic field (IMF) turnings and substorm onsets are coincidental rather than causal, because the same external triggers are also closely associated with an artificial list of substorm onsets generated with the Minimal Substorm Model, which has no requirement of northward IMF turning. We examine an expanded list of substorms using conditional redundancy, an entropy-based measure of conditional dependency, to examine whether northward IMF turning as an external trigger provides any additional information about substorm onset beyond knowing that there has been a period of sustained loading of energy flux (southward IMF). Our analysis reveals that only a few percent additional information is provided by the northward turning criterion, which is consistent with the statistics of surrogate data sets of external triggers constructed to coincide with 2% of substorms. We therefore conclude that northward turning of the IMF is, in general, coincidentally, rather than causally, associated with substorm onsets. C1 [Johnson, Jay R.] Princeton Univ, Plasma Phys Lab, Princeton, NJ 08544 USA. [Wing, Simon] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. RP Johnson, JR (reprint author), Princeton Univ, Plasma Phys Lab, Princeton, NJ 08544 USA. EM jrj@pppl.gov FU NSF [AGS-1058456, ATM-0802715, ATM0902730, AGS-1203299]; NASA [NNX13XAE12G, NNH09AM53I, NNH09AK63I, NNH11AR07I]; DOE [DE-AC02-09CH11466] FX Simon Wing acknowledges NSF grants AGS-1058456 and ATM-0802715; and NASA grant NNX13XAE12G. Jay R. Johnson acknowledges support from NASA grants (NNH09AM53I, NNH09AK63I, and NNH11AR07I), NSF grant ATM0902730, AGS-1203299, and DOE contract DE-AC02-09CH11466 as well as participation in the STORM FP7 project. We thank James M. Weygand for the solar wind data processing. The raw solar wind data from ACE, Wind, IMP8, ISEE1, and ISEE3 were obtained from NASA CDAW and NSSDC. Finally, we thank Frey and Mende for their substorm list. NR 26 TC 3 Z9 3 U1 2 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2014 VL 41 IS 16 BP 5748 EP 5754 DI 10.1002/2014GL060928 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AQ4HT UT WOS:000342755400008 ER PT J AU Lanza, NL Fischer, WW Wiens, RC Grotzinger, J Ollila, AM Cousin, A Anderson, RB Clark, BC Gellert, R Mangold, N Maurice, S Le Mouelic, S Nachon, M Schmidt, M Berger, J Clegg, SM Forni, O Hardgrove, C Melikechi, N Newsom, HE Sautter, V AF Lanza, Nina L. Fischer, Woodward W. Wiens, Roger C. Grotzinger, John Ollila, Ann M. Cousin, Agnes Anderson, Ryan B. Clark, Benton C. Gellert, Ralf Mangold, Nicolas Maurice, Sylvestre Le Mouelic, Stephane Nachon, Marion Schmidt, Mariek Berger, Jeffrey Clegg, Samuel M. Forni, Olivier Hardgrove, Craig Melikechi, Noureddine Newsom, Horton E. Sautter, Violaine TI High manganese concentrations in rocks at Gale crater, Mars SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE Mars; oxidation; manganese; chemical weathering ID INDUCED BREAKDOWN SPECTROSCOPY; CHEMCAM INSTRUMENT SUITE; GUSEV CRATER; SPIRIT ROVER; MARTIAN SOIL; MERIDIANI-PLANUM; MN(II) OXIDATION; CURIOSITY ROVER; IRON-FORMATION; CHEMISTRY AB The surface of Mars has long been considered a relatively oxidizing environment, an idea supported by the abundance of ferric iron phases observed there. However, compared to iron, manganese is sensitive only to high redox potential oxidants, and when concentrated in rocks, it provides a more specific redox indicator of aqueous environments. Observations from the ChemCam instrument on the Curiosity rover indicate abundances of manganese in and on some rock targets that are 1-2 orders of magnitude higher than previously observed on Mars, suggesting the presence of an as-yet unidentified manganese-rich phase. These results show that the Martian surface has at some point in time hosted much more highly oxidizing conditions than has previously been recognized. C1 [Lanza, Nina L.; Wiens, Roger C.; Cousin, Agnes; Clegg, Samuel M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Fischer, Woodward W.; Grotzinger, John] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Ollila, Ann M.; Newsom, Horton E.] Univ New Mexico, Inst Meteorit, Albuquerque, NM 87131 USA. [Anderson, Ryan B.] US Geol Survey, Flagstaff, AZ 86001 USA. [Clark, Benton C.] Space Sci Inst, Boulder, CO USA. [Gellert, Ralf] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Mangold, Nicolas; Le Mouelic, Stephane; Nachon, Marion] Univ Nantes, Lab Planetol & Geodynam, Nantes, France. [Maurice, Sylvestre; Forni, Olivier] Univ Toulouse 3, Inst Rech Astrophys & Planetol, F-31062 Toulouse, France. [Schmidt, Mariek] Brock Univ, Dept Earth Sci, St Catharines, ON L2S 3A1, Canada. [Berger, Jeffrey] Univ Western Ontario, Dept Earth Sci, London, ON, Canada. [Hardgrove, Craig] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ USA. [Melikechi, Noureddine] Delaware State Univ, Dept Phys & Engn, Dover, DE USA. [Sautter, Violaine] Museum Natl Hist Nat, F-75231 Paris, France. RP Lanza, NL (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM nlanza@lanl.gov OI Clegg, Sam/0000-0002-0338-0948 FU NASA's Mars Program Office; Centre National d'Etudes Spatiales (CNES) in France FX The data reported here are archived at the Planetary Data System, available at http://pds-geosciences.wustl.edu/missions/msl/index.htm. This research was carried out with funding from NASA's Mars Program Office and the Centre National d'Etudes Spatiales (CNES) in France. We are grateful to Bradley Tebo and an anonymous reviewer for providing valuable feedback. NR 66 TC 15 Z9 15 U1 4 U2 38 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2014 VL 41 IS 16 BP 5755 EP 5763 DI 10.1002/2014GL060329 PG 9 WC Geosciences, Multidisciplinary SC Geology GA AQ4HT UT WOS:000342755400009 ER PT J AU Fyke, JG Vizcaino, M Lipscomb, WH AF Fyke, Jeremy G. Vizcaino, Miren Lipscomb, William H. TI The pattern of anthropogenic signal emergence in Greenland Ice Sheet surface mass balance SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE Greenland; surface mass balance; anthropogenic signal; climate change; cryosphere ID EARTH SYSTEM MODEL; SEA-LEVEL RISE; ATMOSPHERIC CIRCULATION; CLIMATE VARIABILITY; MELT; ACCUMULATION; PROJECTIONS AB Surface mass balance (SMB) trends influence observed Greenland Ice Sheet (GrIS) mass loss, but the component of these trends related to anthropogenic forcing is unclear. Here we study the simulated spatial pattern of emergence of an anthropogenically derived GrIS SMB signal between 1850 and 2100 using the Community Earth System Model. We find emergence timing heterogeneity, with a bimodal structure reflecting interior snowfall increases against a background of low SMB variability, and peripheral surface melting increases against a backdrop of high SMB variability. We also find a nonemerging intermediate region. We conclude that (1) a bimodal pattern of GrIS SMB change will unambiguously reflect the impact of anthropogenic forcing; (2) present-day peripheral and interior SMB trends likely have an underlying anthropogenically forced component; (3) local emergence occurs well before emergence of a spatially integrated signal; and (4) the GrIS summit region may be an ideal location for monitoring regional/global climate change. C1 [Fyke, Jeremy G.; Lipscomb, William H.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Vizcaino, Miren] Delft Univ Technol, Delft, Netherlands. RP Fyke, JG (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM fyke@lanl.gov FU U.S. Department of Energy Office of Science; Delft Technology Fellowship; National Science Foundation; U.S. Department of Energy FX We thank William J. Sacks for technical support. J. G. Fyke and W. H. Lipscomb are supported by the Regional and Global Climate Modeling and Earth System Modeling programs within the U.S. Department of Energy Office of Science. M. Vizcaino is supported by the Delft Technology Fellowship. The CESM project is supported by the National Science Foundation and the U.S. Department of Energy. We used computing resources at the National Center for Atmospheric Research and Oak Ridge National Laboratory. Model data are archived and available upon request to J. Fyke. NR 32 TC 3 Z9 3 U1 3 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2014 VL 41 IS 16 BP 6002 EP 6008 DI 10.1002/2014GL060735 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AQ4HT UT WOS:000342755400041 ER PT J AU Garfinkel, CI Benedict, JJ Maloney, ED AF Garfinkel, Chaim I. Benedict, James J. Maloney, Eric D. TI Impact of the MJO on the boreal winter extratropical circulation SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE MJO; polar vortex; NAO; stratosphere-troposphere coupling ID MADDEN-JULIAN OSCILLATION; SUDDEN STRATOSPHERIC WARMINGS; NORTH-ATLANTIC OSCILLATION; ARCTIC OSCILLATION; WEATHER REGIMES; WAVE ACTIVITY; LIFE-CYCLE; TROPOSPHERE; VARIABILITY; PREDICTION AB The effect of the Madden-Julian Oscillation (MJO) on the Northern Hemisphere wintertime stratospheric polar vortex is evaluated using a meteorological reanalysis data set and a modern atmospheric general circulation model. The MJO influences the tropospheric North Pacific; and in particular, it modulates the heat flux that is in phase with the climatological planetary waves in both the troposphere and stratosphere. The phase of the MJO in which convection is propagating into the tropical central Pacific leads to a weakened vortex, while suppressed MJO convection in this region is associated with a stronger vortex. Subsequently, the MJO modulates the phase of the tropospheric North Atlantic Oscillation (also known as the Arctic Oscillation or the Northern Annular Mode). While the responses in the model and in the reanalysis data differ in some respects, they both indicate that the MJO can remotely impact the extratropical tropospheric circulation via the stratosphere. C1 [Garfinkel, Chaim I.] Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. [Benedict, James J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Maloney, Eric D.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. RP Garfinkel, CI (reprint author), Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. EM chaim.garfinkel@mail.huji.ac.il RI Maloney, Eric/A-9327-2008; garfinkel, chaim/H-6215-2012; Benedict, James/M-5824-2013 OI Maloney, Eric/0000-0002-2660-2611; garfinkel, chaim/0000-0001-7258-666X; Benedict, James/0000-0001-5115-5131 FU Hebrew University of Jerusalem; Israel Science Foundation [1558/14]; Climate and Large-Scale Dynamics Program of the National Science Foundation [AGS-1025584] FX C.I. Garfinkel was supported by a start-up grant from the Hebrew University of Jerusalem and by the Israel Science Foundation (grant 1558/14). E. D. M. was supported by the Climate and Large-Scale Dynamics Program of the National Science Foundation under grant AGS-1025584. The authors thank Dargan Frierson and Dennis L. Hartmann for allowing us to extend the AM3 simulations discussed in Benedict et al. [2013] for an additional 20 years. NR 43 TC 10 Z9 10 U1 1 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2014 VL 41 IS 16 BP 6055 EP 6062 DI 10.1002/2014GL061094 PG 8 WC Geosciences, Multidisciplinary SC Geology GA AQ4HT UT WOS:000342755400048 ER PT J AU Khan, EH Langford, SC Dickinson, JT Boatner, LA AF Khan, Enamul H. Langford, S. C. Dickinson, J. T. Boatner, L. A. TI The interaction of 193 nm excimer laser radiation with single-crystal zinc oxide: Generation of long lived highly excited particles with evidence of Zn Rydberg formation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID POSITIVE-ION EMISSION; FIELD-IONIZATION; ELECTRIC-FIELD; ATOMS; IRRADIATION; ABLATION; PLASMA; MGO AB In past studies, we have observed copious emissions of ionic and atomic Zn from single-crystal ZnO accompanying irradiation of single-crystal ZnO with 193-nm excimer laser irradiation at fluences below the onset of optical breakdown. The Zn+ and ground state Zn degrees are studied using time-of-flight techniques and are mass selected using a quadrupole mass spectrometer. Simultaneously, we have observed emitted particles that are detectable with a Channeltron electron multiplier but cannot be mass selected. It is a reasonable hypothesis that these particles correspond to a neutral atom or molecule in highly excited long lived states. We provide strong evidence that they correspond to high lying Rydberg states of atomic Zn. We propose a production mechanism involving laser excitation via a two photon resonance excitation of Zn degrees. (C)2014 AIP Publishing LLC. C1 [Khan, Enamul H.; Langford, S. C.; Dickinson, J. T.] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. [Boatner, L. A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Dickinson, JT (reprint author), Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. EM jtd@wsu.edu RI Boatner, Lynn/I-6428-2013 OI Boatner, Lynn/0000-0002-0235-7594 FU U.S. Department of Energy [DE-FG02-04ER-15618] FX This work was partially supported by the U.S. Department of Energy under Contract No. DE-FG02-04ER-15618. NR 32 TC 0 Z9 0 U1 2 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 28 PY 2014 VL 116 IS 8 AR 083711 DI 10.1063/1.4892847 PG 5 WC Physics, Applied SC Physics GA AQ5CP UT WOS:000342821600038 ER PT J AU Pham, HH Taylor, CD Henson, NJ AF Pham, Hieu H. Taylor, Christopher D. Henson, Neil J. TI Acidity constants and its dependence on solvent selection from first-principles calculations using cluster-continuum models SO CHEMICAL PHYSICS LETTERS LA English DT Article ID POTENTIOMETRIC PH MEASUREMENTS; DENSITY-FUNCTIONAL THEORY; DISSOCIATION-CONSTANTS; CARBOXYLIC-ACIDS; PK(A) VALUES; ACETIC-ACID; THEORETICAL CALCULATION; THERMODYNAMIC CYCLES; AQUEOUS-SOLUTION; BENZOIC-ACIDS AB Dissociation constants of selected carboxylic acids in aqueous and organic solvents were calculated at quantum chemical level. We considered cases in which trace quantities of water may be present, as well as cases in which water was entirely absent. In the latter cases, alternative proton acceptors need to be considered. For aqueous solvent, short-range solvation effects are considered by adding explicit water molecules as the first solvent shell. In the absence of water, corresponding organic solvents are used directly as the proton acceptors and the resulted pK(a) are quite comparable to those obtained from previous case of aqueous solvent. (C) 2014 Elsevier B.V. All rights reserved. C1 [Pham, Hieu H.; Taylor, Christopher D.; Henson, Neil J.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Pham, HH (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87544 USA. EM hpham@berkeley.edu RI Pham, Hieu/C-6436-2015; OI Henson, Neil/0000-0002-1842-7884 FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX The authors acknowledge the use of high performance computing resources through the Institutional Computing Program at LANL for the completion of this research. The Los Alamos National Laboratory is operated by Los Alamos National Security LLC for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 41 TC 3 Z9 3 U1 0 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD AUG 28 PY 2014 VL 610 BP 141 EP 147 DI 10.1016/j.cplett.2014.07.017 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AQ1FO UT WOS:000342527500027 ER PT J AU Aguiar, JA Zhuo, MJ Bi, ZX Fu, EG Wang, YQ Dholabhai, PP Misra, A Jia, QX Uberuaga, BP AF Aguiar, Jeffery A. Zhuo, Mujin Bi, Zhenxing Fu, Engang Wang, Yongqiang Dholabhai, Pratik P. Misra, Amit Jia, Quanxi Uberuaga, Blas P. TI Orientation-specific amorphization and intercalated recrystallization at ion-irradiated SrTiO3/MgO interfaces SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID STRONTIUM-TITANATE; RADIATION-DAMAGE; BARIUM-TITANATE; NANOCOMPOSITE; BEHAVIOR; OXIDES; FILMS; CRYSTALLIZATION; COMPOSITES; STABILITY AB Oxide composites are a class of materials with potential uses for nuclear, space, and coating applications. Exploiting their promise, however, requires a detailed understanding of their interfacial structure and chemistry. Using analytical microscopy, we have examined the radiation damage behavior at the interface of a model oxide bilayer, SrTiO3/MgO. The as-synthesized SrTiO3 thin film contained both (100) and (110) oriented domains. We found that after ion beam implantation the (110) domains amorphized at a lower radiation fluence than the (100) domains. Further, a persistent crystalline layer of SrTiO3 forms at the interface even as the rest of the SrTiO3 film amorphizes. We hypothesize that the enhanced amorphization susceptibility of the (110) domains is a consequence of how charged irradiation-induced defects at the interfaces interact with the charged planes of the (110) domains. These results demonstrate the complex relationship between interfacial structure and radiation damage evolution at oxide interfaces. C1 [Aguiar, Jeffery A.; Fu, Engang; Wang, Yongqiang; Dholabhai, Pratik P.; Uberuaga, Blas P.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Zhuo, Mujin; Bi, Zhenxing; Misra, Amit; Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Aguiar, JA (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM jeffery.aguiar@lanl.gov RI Dholabhai, Pratik/A-2366-2015; Misra, Amit/H-1087-2012; OI Aguiar, Jeffery/0000-0001-6101-4762 FU Center for Materials at Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center (EFRC) - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the Center for Materials at Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center (EFRC) funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number 2008LANL1026. The work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. We acknowledge Dorothy Coffey at ORNL for fabricating our FIB foils and Yun Xu for depositing our films. JAA acknowledges access to the ORNL's ShaRE User Facility, which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy, where part of the TEM work was performed in collaboration with Miaofang Chi and the LeRoy Eyring Center for Solid State Science at ASU, where part of the TEM work was performed in collaboration with Toshihiro Aoki and Jiangtao Zhu. We also acknowledge helpful discussions and editorial support from Terence Mitchell, Maulik Patel, and Michelle Hanenburg. NR 52 TC 2 Z9 2 U1 2 U2 13 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD AUG 28 PY 2014 VL 29 IS 16 BP 1699 EP 1710 DI 10.1557/jmr.2014.217 PG 12 WC Materials Science, Multidisciplinary SC Materials Science GA AP6PI UT WOS:000342199300002 ER PT J AU Cotton, SJ Igumenshchev, K Miller, WH AF Cotton, Stephen J. Igumenshchev, Kirill Miller, William H. TI Symmetrical windowing for quantum states in quasi-classical trajectory simulations: Application to electron transfer SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article AB It has recently been shown [S.J. Cotton and W.H. Miller, J. Chem. Phys. 139, 234112 (2013)] that a symmetrical windowing quasi-classical (SQC) approach [S.J. Cotton and W.H. Miller, J. Phys. Chem. A 117, 7190 (2013)] applied to the Meyer-Miller model [H.-D. Meyer and W.H. Miller, J. Chem. Phys. 70, 3214 (1979)] for the electronic degrees of freedom in electronically non-adiabatic dynamics is capable of quantitatively reproducing quantum mechanical results for a variety of test applications, including cases where "quantum" coherence effects are significant. Here we apply this same SQC methodology, within a flux-side correlation function framework, to calculate thermal rate constants corresponding to several proposed models of electron transfer processes [P. Huo, T.F. Miller III, and D.F. Coker, J. Chem. Phys. 139, 151103 (2013); A.R. Menzeleev, N. Ananth, and T.F. Miller III, J. Chem. Phys. 135, 074106 (2011)]. Good quantitative agreement with Marcus Theory is obtained over several orders of magnitude variation in non-adiabatic coupling. Moreover, the "inverted regime" in thermal rate constants (with increasing bias) known from Marcus Theory is also reproduced with good accuracy by this very simple classical approach. The SQC treatment is also applied to a recent model of photoinduced proton coupled electron transfer [C. Venkataraman, A. V. Soudackov, and S. Hammes-Schiffer, J. Chem. Phys. 131, 154502 (2009)] and population decay of the photoexcited donor state is found to be in reasonable agreement with results calculated via reduced density matrix theory. (C) 2014 AIP Publishing LLC. C1 [Miller, William H.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Miller, WH (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM millerwh@berkeley.edu FU National Science Foundation [CHE-1148645]; Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Science Foundation Grant No. CHE-1148645 and by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy under Contract No. DE-AC02-05CH11231.; This research utilized computation resources provided by the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 13 TC 17 Z9 18 U1 6 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2014 VL 141 IS 8 AR 084104 DI 10.1063/1.4893345 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AP3OY UT WOS:000341987600008 PM 25173002 ER PT J AU Mitra, C Meyer, T Lee, HN Reboredo, FA AF Mitra, Chandrima Meyer, Tricia Lee, Ho Nyung Reboredo, Fernando A. TI Oxygen diffusion pathways in brownmillerite SrCoO2.5: Influence of structure and chemical potential SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; ION MIGRATION; SADDLE-POINTS; OXIDE; MOBILITY AB To design and discover new materials for next-generation energy materials such as solid-oxide fuel cells (SOFCs), a fundamental understanding of their ionic properties and behaviors is essential. The potential applicability of a material for SOFCs is critically determined by the activation energy barrier of oxygen along various diffusion pathways. In this work, we investigate interstitial-oxygen (O-i) diffusion in brownmillerite oxide SrCoO2.5, employing a first-principles approach. Our calculations indicate highly anisotropic ionic diffusion pathways, which result from its anisotropic crystal structure. The one-dimensional-ordered oxygen vacancy channels are found to provide the easiest diffusion pathway with an activation energy barrier height of 0.62 eV. The directions perpendicular to the vacancy channels have higher energy barriers for O-int diffusion. In addition, we have studied migration barriers for oxygen vacancies that could be present as point defects within the material. This in turn could also facilitate the transport of oxygen. Interestingly, for oxygen vacancies, the lowest barrier height was found to occur within the octahedral layer with an energy of 0.82 eV. Our results imply that interstitial migration would be highly one-dimensional in nature. Oxygen vacancy transport, on the other hand, could preferentially occur in the two-dimensional octahedral plane. (C) 2014 AIP Publishing LLC. C1 [Mitra, Chandrima; Meyer, Tricia; Lee, Ho Nyung; Reboredo, Fernando A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Mitra, C (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RI Lee, Ho Nyung/K-2820-2012 OI Lee, Ho Nyung/0000-0002-2180-3975 FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 28 TC 5 Z9 5 U1 6 U2 47 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2014 VL 141 IS 8 AR 084710 DI 10.1063/1.4893950 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AP3OY UT WOS:000341987600039 PM 25173033 ER PT J AU Schacht, M Schauer, MM AF Schacht, M. Schauer, M. M. TI Shelving and probe efficiency in trapped ion experiments SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE ion trap; coherent control; quantum jumps; pump/probe ID PARITY NONCONSERVATION; FREQUENCY-COMB; SPECTROSCOPY AB A generalized probe sequence typical of trapped ion experiments using shelving is studied. Detection efficiency is analyzed for finite shelved state lifetimes and using multi-modal count distributions. Multi-modal distributions are more appropriate for measurements that use a small number of ions than the simple Poisson counting statistics usually considered and have a larger variance that may be significant in determining uncertainties and in making weighted fits. Optimal probe times and the resulting state detection efficiency and sensitivity are determined for arbitrary cooling rates, initial states, and shelved state lifetimes in terms of a probe coherence time tau(p). A universal optimal probe time of t(p) approximate to 0.43 tau(p) is shown to give close to the optimal probe sensitivity for most systems. C1 [Schacht, M.; Schauer, M. M.] Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA. RP Schacht, M (reprint author), Los Alamos Natl Lab, Div Phys, P-23,Mail Stop H803, Los Alamos, NM 87545 USA. EM schauer@lanl.gov RI Schacht, Mike/J-4441-2015 OI Schacht, Mike/0000-0002-5139-1369 FU Laboratory Directed Research and Development program at Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work was supported by the Laboratory Directed Research and Development program at Los Alamos National Laboratory, operated by Los Alamos National Security, LLC, for the NNSA US Department of Energy under contract No. DE-AC52-06NA25396. NR 17 TC 1 Z9 1 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD AUG 28 PY 2014 VL 47 IS 16 AR 165002 DI 10.1088/0953-4075/47/16/165002 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AP3KS UT WOS:000341975500003 ER PT J AU Marino, R Mininni, PD Rosenberg, DL Pouquet, A AF Marino, R. Mininni, P. D. Rosenberg, D. L. Pouquet, A. TI Large-scale anisotropy in stably stratified rotating flows SO PHYSICAL REVIEW E LA English DT Article ID BREAKING INTERNAL WAVES; KINETIC-ENERGY SPECTRUM; 2-DIMENSIONAL TURBULENCE; SOLAR-WIND; 3-DIMENSIONAL TURBULENCE; LIMITING DYNAMICS; INVERSE CASCADES; FROUDE-NUMBER; CHANNEL FLOW; FLUID AB We present results from direct numerical simulations of the Boussinesq equations in the presence of rotation and/or stratification, both in the vertical direction. The runs are forced isotropically and randomly at small scales and have spatial resolutions of up to 1024(3) grid points and Reynolds numbers of approximate to 1000. We first show that solutions with negative energy flux and inverse cascades develop in rotating turbulence, whether or not stratification is present. However, the purely stratified case is characterized instead by an early-time, highly anisotropic transfer to large scales with almost zero net isotropic energy flux. This is consistent with previous studies that observed the development of vertically sheared horizontal winds, although only at substantially later times. However, and unlike previous works, when sufficient scale separation is allowed between the forcing scale and the domain size, the kinetic energy displays a perpendicular (horizontal) spectrum with power-law behavior compatible with similar to k(perpendicular to)(-5/3), including in the absence of rotation. In this latter purely stratified case, such a spectrum is the result of a direct cascade of the energy contained in the large-scale horizontal wind, as is evidenced by a strong positive flux of energy in the parallel direction at all scales including the largest resolved scales. C1 [Marino, R.; Pouquet, A.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Marino, R.] Inst Chem Phys Proc, I-87036 Arcavacata Di Rende, CS, Italy. [Marino, R.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Mininni, P. D.] Univ Buenos Aires, Fac Ciencias Exactas & Nat, Dept Fis, RA-1428 Buenos Aires, DF, Argentina. [Mininni, P. D.] Consejo Nacl Invest Cient & Tecn, IFIBA, RA-1428 Buenos Aires, DF, Argentina. [Rosenberg, D. L.] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Pouquet, A.] Univ Colorado, Atmospher & Space Phys Lab, Boulder, CO 80309 USA. RP Marino, R (reprint author), Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. RI Marino, Raffaele/M-5130-2015 OI Marino, Raffaele/0000-0002-7372-8620 FU NSF/CMG [1025183]; NSF through the University Corporation for Atmospheric Research on behalf of the National Center for Atmospheric Research (NCAR); UBACYT [20020110200359]; PICT [2011-1529, 2011-1626]; PIP [11220090100825]; LASP; Marie Curie Project FP7 [PIRSES-2010-269297] FX This work was supported by NSF/CMG Grant No. 1025183; it was also sponsored by an NSF cooperative agreement through the University Corporation for Atmospheric Research on behalf of the National Center for Atmospheric Research (NCAR). Computer time was provided on NSF/XSEDE TG-PHY100029 and 110044 and NCAR/ASD on Yellowstone. P. D. M. acknowledges support from UBACYT Grant No. 20020110200359, PICT Grants No. 2011-1529 and No. 2011-1626, and PIP Grant No. 11220090100825. A. P. acknowledges support from LASP and, in particular, Bob Ergun. R. M. acknowledges the Regional Operative Program Calabria ESF 2007/2013 and the Marie Curie Project FP7 PIRSES-2010-269297 "Turboplasmas." NR 77 TC 10 Z9 10 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD AUG 28 PY 2014 VL 90 IS 2 AR 023018 DI 10.1103/PhysRevE.90.023018 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AO4EV UT WOS:000341289900010 PM 25215831 ER PT J AU Yoo, J Yamada, M Ji, HT Jara-Almonte, J Myers, CE Chen, LJ AF Yoo, Jongsoo Yamada, Masaaki Ji, Hantao Jara-Almonte, Jonathan Myers, Clayton E. Chen, Li-Jen TI Laboratory Study of Magnetic Reconnection with a Density Asymmetry across the Current Sheet SO PHYSICAL REVIEW LETTERS LA English DT Article ID REGION; PLASMA; FIELD AB The effects of a density asymmetry across the current sheet on anti-parallel magnetic reconnection are studied systematically in a laboratory plasma. Despite a significant density ratio of up to 10, the in-plane magnetic field profile is not significantly changed. On the other hand, the out-of-plane Hall magnetic field profile is considerably modified; it is almost bipolar in structure with the density asymmetry, as compared to quadrupolar in structure with the symmetric configuration. Moreover, the ion stagnation point is shifted to the low-density side, and the electrostatic potential profile also becomes asymmetric with a deeper potential well on the low-density side. Nonclassical bulk electron heating together with electromagnetic fluctuations in the lower hybrid frequency range is observed near the low-density-side separatrix. The dependence of the ion outflow and reconnection electric field on the density asymmetry is measured and compared with theoretical expectations. The measured ion outflow speeds are about 40% of the theoretical values. C1 [Yoo, Jongsoo; Yamada, Masaaki; Ji, Hantao; Jara-Almonte, Jonathan; Myers, Clayton E.] Princeton Plasma Phys Lab, Ctr Magnet Self Org Lab & Astrophys Plasmas, Princeton, NJ 08543 USA. [Chen, Li-Jen] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. RP Yoo, J (reprint author), Princeton Plasma Phys Lab, Ctr Magnet Self Org Lab & Astrophys Plasmas, POB 451, Princeton, NJ 08543 USA. EM jyoo@pppl.gov OI Yoo, Jongsoo/0000-0003-3881-1995; Myers, Clayton/0000-0003-4539-8406 FU CMSO; DOE [DE-AC0209CH11466]; NASA program for the MMS mission [NNH11AQ45I]; NSF [AGS-1202537] FX This work is supported by CMSO, DOE Contract No. DE-AC0209CH11466, the NASA program for the MMS mission under the Grant No. NNH11AQ45I, and the NSF Grant No. AGS-1202537. The authors thank J. Drake, V. Roytershteyn, M. Shay, and W. Daughton for valuable discussions, and R. Cutler for technical support. NR 40 TC 10 Z9 10 U1 2 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 28 PY 2014 VL 113 IS 9 AR 095002 DI 10.1103/PhysRevLett.113.095002 PG 5 WC Physics, Multidisciplinary SC Physics GA AO4FX UT WOS:000341292800010 PM 25215989 ER PT J AU Pena-Castillo, L Mercer, RG Gurinovich, A Callister, SJ Wright, AT Westbye, AB Beatty, JT Lang, AS AF Pena-Castillo, Lourdes Mercer, Ryan G. Gurinovich, Anastasia Callister, Stephen J. Wright, Aaron T. Westbye, Alexander B. Beatty, J. Thomas Lang, Andrew S. TI Gene co-expression network analysis in Rhodobacter capsulatus and application to comparative expression analysis of Rhodobacter sphaeroides SO BMC GENOMICS LA English DT Article DE Comparative transcriptomics; Module preservation; Gene-protein expression conservation; Rhodobacter capsulatus; Rhodobacter sphaeroides ID TRANSFER AGENT RCGTA; QUORUM-SENSING REGULATION; HYDROGEN-PEROXIDE; R-PACKAGE; DATA SETS; TRANSCRIPTOME; REGULATOR; BACTERIAL; RESPONSES; DATABASE AB Background: The genus Rhodobacter contains purple nonsulfur bacteria found mostly in freshwater environments. Representative strains of two Rhodobacter species, R. capsulatus and R. sphaeroides, have had their genomes fully sequenced and both have been the subject of transcriptional profiling studies. Gene co-expression networks can be used to identify modules of genes with similar expression profiles. Functional analysis of gene modules can then associate co-expressed genes with biological pathways, and network statistics can determine the degree of module preservation in related networks. In this paper, we constructed an R. capsulatus gene co-expression network, performed functional analysis of identified gene modules, and investigated preservation of these modules in R. capsulatus proteomics data and in R. sphaeroides transcriptomics data. Results: The analysis identified 40 gene co-expression modules in R. capsulatus. Investigation of the module gene contents and expression profiles revealed patterns that were validated based on previous studies supporting the biological relevance of these modules. We identified two R. capsulatus gene modules preserved in the protein abundance data. We also identified several gene modules preserved between both Rhodobacter species, which indicate that these cellular processes are conserved between the species and are candidates for functional information transfer between species. Many gene modules were non-preserved, providing insight into processes that differentiate the two species. In addition, using Local Network Similarity (LNS), a recently proposed metric for expression divergence, we assessed the expression conservation of between-species pairs of orthologs, and within-species gene-protein expression profiles. Conclusions: Our analyses provide new sources of information for functional annotation in R. capsulatus because uncharacterized genes in modules are now connected with groups of genes that constitute a joint functional annotation. We identified R. capsulatus modules enriched with genes for ribosomal proteins, porphyrin and bacteriochlorophyll anabolism, and biosynthesis of secondary metabolites to be preserved in R. sphaeroides whereas modules related to RcGTA production and signalling showed lack of preservation in R. sphaeroides. In addition, we demonstrated that network statistics may also be applied within-species to identify congruence between mRNA expression and protein abundance data for which simple correlation measurements have previously had mixed results. C1 [Pena-Castillo, Lourdes; Mercer, Ryan G.; Lang, Andrew S.] Mem Univ Newfoundland, Dept Biol, St John, NF A1B 3X5, Canada. [Pena-Castillo, Lourdes; Gurinovich, Anastasia] Mem Univ Newfoundland, Dept Comp Sci, St John, NF A1B 3X5, Canada. [Callister, Stephen J.; Wright, Aaron T.] Pacific NW Natl Lab, Biol Sci Div, Richland, WA 99352 USA. [Westbye, Alexander B.; Beatty, J. Thomas] Univ British Columbia, Dept Microbiol & Immunol, Vancouver, BC V5Z 1M9, Canada. RP Pena-Castillo, L (reprint author), Mem Univ Newfoundland, Dept Biol, St John, NF A1B 3X5, Canada. EM lourdes@mun.ca; aslang@mun.ca OI Wright, Aaron/0000-0002-3172-5253; Lang, Andrew/0000-0002-4510-7683; Pena Castillo, Lourdes/0000-0002-0643-2547 FU Natural Sciences and Engineering Research Council (NSERC); Newfoundland and Labrador Research & Development Corporation (NL RDC); NSERC; NL RDC; Canada Foundation for Innovation; Government of Newfoundland and Labrador; Memorial University; Department of Energy Office of Biological and Environmental Research (OBER) Genome Sciences Program under the Pan-omics project; DOE OBER; DOE [DE-AC05-76RLO01830]; Canadian Institutes of Health Research [93779] FX The research in L.P-C's laboratory was supported by a Discovery Grant from the Natural Sciences and Engineering Research Council (NSERC), and an IgniteR&D grant from the Newfoundland and Labrador Research & Development Corporation (NL RDC). The research in A.S.L.'s laboratory was supported by grants from NSERC, NL RDC, the Canada Foundation for Innovation, and the Industrial Research and Innovation Fund from the Government of Newfoundland and Labrador. R. G. M. was supported by fellowships from Memorial University and NSERC. A. G. was partially supported by a fellowship from Memorial University. A portion of the research described in this paper was funded by the Department of Energy Office of Biological and Environmental Research (OBER) Genome Sciences Program under the Pan-omics project, and was performed in part in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE OBER and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated by Battelle for the DOE under contract DE-AC05-76RLO01830. A. B. W. was supported by a Canadian Institutes of Health Research grant (#93779) awarded to J.T.B. NR 69 TC 3 Z9 3 U1 3 U2 17 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD AUG 28 PY 2014 VL 15 AR 730 DI 10.1186/1471-2164-15-730 PG 14 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA AO4RF UT WOS:000341328000001 PM 25164283 ER PT J AU Kranzusch, PJ Lee, ASY Wilson, SC Solovykh, MS Vance, RE Berger, JM Doudna, JA AF Kranzusch, Philip J. Lee, Amy S. Y. Wilson, Stephen C. Solovykh, Mikhail S. Vance, Russell E. Berger, James M. Doudna, Jennifer A. TI Structure-Guided Reprogramming of Human cGAS Dinucleotide Linkage Specificity SO CELL LA English DT Article ID CYCLIC GMP-AMP; INNATE IMMUNE-RESPONSE; DNA SENSOR; 2ND-MESSENGER; SYNTHASE; REVEALS; PATHWAY; COMPLEX; CYCLASE; MODEL AB Cyclic dinucleotides (CDNs) play central roles in bacterial pathogenesis and innate immunity. The mammalian enzyme cGAS synthesizes a unique cyclic dinucleotide (cGAMP) containing a 2'-5' phosphodiester linkage essential for optimal immune stimulation, but the molecular basis for linkage specificity is unknown. Here, we show that the Vibrio cholerae pathogenicity factor DncV is a prokaryotic cGAS-like enzyme whose activity provides a mechanistic rationale for the unique ability of cGAS to produce 2'-5' cGAMP. Three high-resolution crystal structures show that DncV and human cGAS generate CDNs in sequential reactions that proceed in opposing directions. We explain 2' and 3' linkage specificity and test this model by reprogramming the human cGAS active site to produce 3'-5' cGAMP, leading to selective stimulation of alternative STING adaptor alleles in cells. These results demonstrate mechanistic homology between bacterial signaling and mammalian innate immunity and explain how active site configuration controls linkage chemistry for pathway-specific signaling. C1 [Kranzusch, Philip J.; Lee, Amy S. Y.; Solovykh, Mikhail S.; Vance, Russell E.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Lee, Amy S. Y.; Doudna, Jennifer A.] Univ Calif Berkeley, Ctr RNA Syst Biol, Berkeley, CA 94720 USA. [Berger, James M.] Johns Hopkins Univ, Sch Med, Dept Biophys, Baltimore, MD 21205 USA. [Kranzusch, Philip J.; Vance, Russell E.; Doudna, Jennifer A.] Univ Calif Berkeley, HHMI, Berkeley, CA 94720 USA. [Wilson, Stephen C.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Berger, JM (reprint author), Johns Hopkins Univ, Sch Med, Dept Biophys, Baltimore, MD 21205 USA. EM jmberger@jhmi.edu; doudna@berkeley.edu FU HHMI; G. Harold and Leila Y. Mathers Foundation; National Cancer Institutes [CA077373]; National Institutes of Health [AI063302, AI080749, AI103817]; NIGMS Center for RNA Systems Biology; Life Sciences Research Foundation; American Cancer Society [PF-14-108-01-RMC] FX X-ray data were collected at Beamline 8.3.1 of the Lawrence Berkeley National Lab Advanced Light Source (ALS) and Beamlines 11.1 and 12.2 of the Stanford Synchrotron Radiation Lightsource (SSRL). The authors are grateful to J. Holton and G. Meigs (ALS); T. Doukov, S. Russi, and A. Gonzalez (SSRL) for technical assistance with data collection and processing; R. Nichiporuk (QB3 Mass Spectrometry Facility) for assistance with product determination; J. Cate, Y. Bai, S. Floor, R. Wilson, and members of the Doudna and Berger labs for helpful comments and discussion. This work was funded by HHMI (R.E.V. and J.A.D.); the G. Harold and Leila Y. Mathers Foundation (J.M.B.); National Cancer Institutes Grant CA077373 (J.M.B.); National Institutes of Health Grants AI063302, AI080749, and AI103817 (R.E.V.); and the NIGMS Center for RNA Systems Biology (A.S.Y.L. and J.A.D.). P.J.K. is supported as an HHMI Fellow of the Life Sciences Research Foundation, and A.S.Y.L. is supported as an American Cancer Society Postdoctoral Fellow (PF-14-108-01-RMC). R.E.V. and J.A.D. are HHMI Investigators. NR 33 TC 21 Z9 23 U1 3 U2 16 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD AUG 28 PY 2014 VL 158 IS 5 BP 1011 EP 1021 DI 10.1016/j.cell.2014.07.028 PG 11 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA AN9RI UT WOS:000340945000008 PM 25131990 ER PT J AU Chuong, CM Bhat, R Widelitz, RB Bissell, MJ AF Chuong, Cheng-Ming Bhat, Ramray Widelitz, Randall B. Bissell, Mina J. TI SnapShot: Branching Morphogenesis SO CELL LA English DT Editorial Material ID MAMMARY-GLAND C1 [Chuong, Cheng-Ming; Widelitz, Randall B.] Univ So Calif, Dept Pathol, Los Angeles, CA 90033 USA. [Bhat, Ramray; Bissell, Mina J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Chuong, Cheng-Ming] Cheng Kung Univ, Ctr Wound Repair & Regenerat, Tainan, Taiwan. RP Chuong, CM (reprint author), Univ So Calif, Dept Pathol, Los Angeles, CA 90033 USA. FU NIAMS NIH HHS [R01 AR042177, R01 AR047364, R01 AR060306] NR 5 TC 8 Z9 8 U1 1 U2 11 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD AUG 28 PY 2014 VL 158 IS 5 BP 1212 EP U265 AR 1212.e1 DI 10.1016/j.cell.2014.08.019 PG 2 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA AN9RI UT WOS:000340945000026 PM 25171418 ER PT J AU Alexeev, Y Fedorov, DG Shvartsburg, AA AF Alexeev, Yuri Fedorov, Dmitri G. Shvartsburg, Alexandre A. TI Effective Ion Mobility Calculations for Macromolecules by Scattering on Electron Clouds SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MOLECULAR-ORBITAL METHOD; PROJECTION APPROXIMATION ALGORITHM; COLLISION CROSS-SECTION; GAS-PHASE; MASS-SPECTROMETRY; STRUCTURAL INFORMATION; TRANSPORT-COEFFICIENTS; ACCURATE COMPUTATION; PROTEIN COMPLEXES; POLYATOMIC IONS AB Broad commercialization and increasing resolving power of ion mobility spectrometry/mass spectrometry (IMS/MS) platforms have engendered an explosion of IMS applications to structural characterization of gas-phase biomolecules. That has renewed interest in more accurate and rapid ion mobility calculations that are needed to elicit ion geometries from the measurements. An approach based on scattering on electron density isosurfaces (SEDI) that mirrors the physics of molecular collisions was proven superior to the common methods involving atomic coordinates a decade ago but has remained impractical for large ions because of extreme computational demands. Here, we accelerate SEDI by up to similar to 500 times using the fragment molecular orbital approach for surface generation and the multiplexed scattering algorithm in conjunction with the new grid extrapolation procedure for cross section evaluations. Parallelization of the code on a supercomputer has produced major further speed gains, allowing SEDI calculations for proteins (defined by over a million surface points) with a precision of <0.1% in 1 min. Initial tests reveal the anticipated dependence of mobility on the ion charge state and lower cross sections in view of reduced surface roughness. Present developments are expected to lead to broad application of SEDI in IMS studies of macromolecules, enabling more accurate and reliable structural assignments. C1 [Alexeev, Yuri] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. [Fedorov, Dmitri G.] Natl Inst Adv Ind Sci & Technol, Nanosyst Res Inst, Tsukuba, Ibaraki 3058568, Japan. [Shvartsburg, Alexandre A.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99354 USA. RP Shvartsburg, AA (reprint author), Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99354 USA. EM aas996@yahoo.com FU Next Generation Super Computing Project and Nanoscience Program (MEXT, Japan); Strategic Programs for Innovative Research (SPIRE, Japan) at AIST; PNNL Technology Commercialization Office; U.S. DOE Office of Science [DE-AC02-06CH11357] FX This work was supported by the Next Generation Super Computing Project and Nanoscience Program (MEXT, Japan), Strategic Programs for Innovative Research (SPIRE, Japan) at AIST, and PNNL Technology Commercialization Office. This research used resources of the Argonne Leadership Computing Facility at ANL, supported by the U.S. DOE Office of Science under contract DE-AC02-06CH11357, and the Environmental Molecular Sciences Laboratory, a DOE national scientific user facility at PNNL. NR 83 TC 13 Z9 13 U1 1 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD AUG 28 PY 2014 VL 118 IS 34 BP 6763 EP 6772 DI 10.1021/jp505012c PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AO2BR UT WOS:000341121000004 PM 25137627 ER PT J AU Aguirre, JC Ferreira, A Ding, H Jenekhe, SA Kopidakis, N Asta, M Pilon, L Rubin, Y Tolbert, SH Schwartz, BJ Dunn, B Ozolins, V AF Aguirre, Jordan C. Ferreira, Amy Ding, Hong Jenekhe, Samson A. Kopidakis, Nikos Asta, Mark Pilon, Laurent Rubin, Yves Tolbert, Sarah H. Schwartz, Benjamin J. Dunn, Bruce Ozolins, Vidvuds TI Panoramic View of Electrochemical Pseudocapacitor and Organic Solar Cell Research in Molecularly Engineered Energy Materials (MEEM) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOUBLE-LAYER CAPACITORS; NEXT-GENERATION SUPERCAPACITORS; POLYMER PHOTOVOLTAIC CELLS; HYDROUS RUTHENIUM OXIDES; CHARGE STORAGE MECHANISM; TRANSITION-METAL OXIDES; BULK-HETEROJUNCTION; MESOPOROUS MATERIALS; CONJUGATED POLYELECTROLYTES; SEMICONDUCTING POLYMERS AB Our program on capacitive energy storage is a comprehensive one that combines experimental and computational components to achieve a fundamental understanding of charge storage processes in redox-based materials, specifically transition metal oxides. Some of the highlights of this program are the identification of intercalation pseudocapacitance in Nb2O5, which enables high energy density to be achieved at high rates, and the development of a new route for synthesizing mesoporous films in which preformed nanocrystal building blocks are used in combination with polymer templating. The resulting material architectures have large surface areas and enable electrolyte access to the redox active pore walls, while the interconnected mesoporous film provides good electronic conductivity. Select first-principles density-functional theory studies of prototypical pseudocapacitor materials are reviewed, providing insight into the key physical and chemical features involved in charge transfer and ion diffusion. Rigorous multiscale physical models and numerical tools have been developed and used to reproduce electrochemical properties of carbon-based electrochemical capacitors with the ultimate objective of facilitating the optimization of electrode design. For the organic photovoltaic (OPV) program, our focus has been ongoing beyond the trial-and-error Edisonian approaches that have been responsible for the increase in power conversion efficiency of blend-cast (BC) bulk heterojunction blends of polymers and fullerenes. Our first approach has been to use molecular self-assembly to create the ideal nanometer-scale architecture using thermodynamics rather than relying on the kinetics of spontaneous phase segregation. We have created fullerenes that self-assemble into one-dimensional stacks and have shown that use of these self-assembled fullerenes lead to dramatically enhanced OPV performance relative to fullerenes that do not assemble. We also have created self-assembling conjugated polymers that form gels based on electrically continuous cross-linked micelles in solution, opening the possibility for water-processable "green" production of OPVs based on these materials. Our second approach has been to avoid kinetic control over phase separation by using a sequential processing (SqP) technique to deposit the polymer and fullerene materials in separate deposition steps. The polymer layer is deposited first, using solvents and deposition conditions that optimize the polymer crystallinity for swelling and hole mobility. The fiillerene layer is then deposited in a second step from a solvent that swells the polymer but does not dissolve it, allowing the fullerene to penetrate into the polymer underlayer to the desired degree. Careful comparison of composition- and thickness-matched BC and SqP devices shows that SqP not only produces more efficient devices but also leads to devices that behave more consistently. C1 [Aguirre, Jordan C.; Ferreira, Amy; Rubin, Yves; Tolbert, Sarah H.; Schwartz, Benjamin J.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Ding, Hong; Asta, Mark] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Jenekhe, Samson A.] Univ Washington, Dept Chem Engn, Seattle, WA 98195 USA. [Jenekhe, Samson A.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Kopidakis, Nikos] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Pilon, Laurent] Univ Calif Los Angeles, Mech & Aerosp Engn Dept, Los Angeles, CA 90095 USA. [Dunn, Bruce; Ozolins, Vidvuds] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. RP Schwartz, BJ (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. EM schwartz@chem.ucla.edu; bdunn@ucla.edu; vidvuds@ucla.edu RI Pilon, Laurent/B-3497-2008; Kopidakis, Nikos/N-4777-2015; Tolbert, Sarah/L-2321-2016; OI Pilon, Laurent/0000-0001-9459-8207; Schwartz, Benjamin/0000-0003-3257-9152 FU Molecularly Engineered Energy Materials, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001342] FX This work was supported as part of the Molecularly Engineered Energy Materials, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award Number DE-SC0001342. NR 139 TC 6 Z9 6 U1 10 U2 77 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19505 EP 19523 DI 10.1021/jp501047j PG 19 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200001 ER PT J AU Kobayashi, T Gupta, S Caporini, MA Pecharsky, VK Pruski, M AF Kobayashi, Takeshi Gupta, Shalabh Caporini, Marc A. Pecharsky, Vitalij K. Pruski, Marek TI Mechanism of Solid-State Thermolysis of Ammonia Borane: A N-15 NMR Study Using Fast Magic-Angle Spinning and Dynamic Nuclear Polarization SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CHEMICAL HYDROGEN STORAGE; N-H COMPOUNDS; THERMAL-DECOMPOSITION; BORON-NITRIDE; SENSITIVITY ENHANCEMENT; COMPLEX HYDRIDES; HIGH-FREQUENCY; SPENT FUEL; MAS-NMR; SPECTROSCOPY AB The solid-state thermolysis of ammonia borane (NH3BH3, AB) was explored using state-of-the-art N-15 solid-state NMR spectroscopy, including 2D indirectly detected H-1{N-15} heteronuclear correlation and dynamic nuclear polarization (DNP)-enhanced N-15{H-1} cross-polarization experiments as well as B-11 NMR The complementary use of N-15 and B-11 NMR experiments, supported by density functional theory calculations of the chemical shift tensors, provided insights into the dehydrogenation mechanism of AB-insights that have not been available by B-11 NMR alone. Specifically, highly branched polyaminoborane derivatives were shown to form from AB via oligomerization in the "head-to-tail" manner, which then transform directly into hexagonal boron nitride analog through the dehydrocyclization reaction, bypassing the formation of polyiminoborane. C1 [Kobayashi, Takeshi; Gupta, Shalabh; Pecharsky, Vitalij K.; Pruski, Marek] US DOE, Ames Lab, Ames, IA 50011 USA. [Caporini, Marc A.] Bruker BioSpin Corp, Billerica, MA 01821 USA. [Pecharsky, Vitalij K.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Kobayashi, T (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM takeshi@iastate.edu; itkp@amelab.gov; mpruski@iastate.edu FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under contract no. DE-AC02-07CH11358. NR 57 TC 9 Z9 9 U1 4 U2 68 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19548 EP 19555 DI 10.1021/jp504328x PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200005 ER PT J AU Chen, T Skinner, B Xie, W Shklovskii, BI Kortshagen, UR AF Chen, Ting Skinner, Brian Xie, Wei Shklovskii, B. I. Kortshagen, Uwe R. TI Carrier Transport in Films of Alkyl-Ligand-Terminated Silicon Nanocrystals SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PLASMA SYNTHESIS; SURFACE PASSIVATION; SI NANOCRYSTALS; QUANTUM DOTS; THIN-FILMS; CONDUCTIVITY AB Silicon nanocrystals (Si NCs) have shown great promise for electroluminescent and photoluminescent applications. In order to optimize the properties of Si NC devices, however, electronic transport in Si NC films needs to be thoroughly understood. Here we present a systematic study of the temperature and electric field dependence of conductivity in films of alkyl-ligand-terminated Si NCs, which to date have shown the highest potential for device applications. Our measurements suggest that the conductivity is limited by the ionization of rare NCs containing donor impurities. At low bias, this ionization is thermally activated, with an ionization energy equal to twice the NC charging energy. As the bias is increased, the ionization energy is reduced by the electric field, as determined by the Poole-Frenkel effect. At large bias and sufficiently low temperature, we observe cold ionization of electrons from donor-containing NCs, with a characteristic tunneling length of about 1 nm. The temperature- and electric-field-dependent conductance measurements presented here provide a systematic and comprehensive picture for electron transport in lightly doped nanocrystal films. C1 [Chen, Ting; Xie, Wei] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [Skinner, Brian; Shklovskii, B. I.] Univ Minnesota, Fine Theoret Phys Inst, Minneapolis, MN 55455 USA. [Skinner, Brian] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Kortshagen, Uwe R.] Univ Minnesota, Dept Mech Engn, Minneapolis, MN 55455 USA. RP Shklovskii, BI (reprint author), Univ Minnesota, Fine Theoret Phys Inst, Minneapolis, MN 55455 USA. EM shklovsk@physics.umn.edu; Kortshagen@umn.edu RI Kortshagen, Uwe/B-8744-2016; OI Kortshagen, Uwe/0000-0001-5944-3656; Skinner, Brian/0000-0003-0774-3563 FU National Science Foundation through the University of Minnesota MRSEC [DMR-0819885]; NSF through the UMN MRSEC program; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We are grateful to K. V. Reich for valuable comments. This work was supported primarily by the National Science Foundation through the University of Minnesota MRSEC under Award No. DMR-0819885. Part of this work was carried out in the College of Science and Engineering Characterization Facility, University of Minnesota, which has received capital equipment funding from the NSF through the UMN MRSEC program. Work at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 35 TC 11 Z9 11 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19580 EP 19588 DI 10.1021/jp5051723 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200009 ER PT J AU McDowell, MT Lichterman, MF Spurgeon, JM Hu, S Sharp, ID Brunschwig, BS Lewis, NS AF McDowell, Matthew T. Lichterman, Michael F. Spurgeon, Joshua M. Hu, Shu Sharp, Ian D. Brunschwig, Bruce S. Lewis, Nathan S. TI Improved Stability of Polycrystalline Bismuth Vanadate Photoanodes by Use of Dual-Layer Thin TiO2/Ni Coatings SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PHOTOELECTROCHEMICAL WATER OXIDATION; VISIBLE-LIGHT IRRADIATION; OXYGEN EVOLUTION REACTION; BIVO4 PHOTOELECTRODES; SILICON PHOTOANODES; HYDROGEN-PRODUCTION; EFFICIENT; CATALYST; ELECTROCATALYSTS; METAL AB Ultrathin dual layers of TiO2 and Ni have been used to stabilize polycrystalline BiVO4 photoanodes against photocorrosion in an aqueous alkaline (pH = 13) electrolyte. Conformal, amorphous TiO2 layers were deposited on BiVO4 thin films by atomic-layer deposition, with Ni deposited onto the TiO2 by sputtering. Under simulated air mass 1.5 illumination, the dual-layer coating extended the lifetime of the BiVO4 photoanodes during photoelectrochernical water oxidation from minutes, for bare BiVO4, to hours, for the modified electrodes. X-ray photoelectron spectroscopy showed that these layers imparted chemical stability to the semiconductor/electrolyte interface. Transmission electron microscopy revealed the structure and morphology of the polycrystalline BiVO4 film as well as of the thin coating layers. This work demonstrates that protection schemes based on ultrathin corrosion-resistant overlayers can be applied beneficially to polycrystalline photoanode materials under conditions relevant to efficient solar-driven water-splitting systems. C1 [McDowell, Matthew T.; Lichterman, Michael F.; Spurgeon, Joshua M.; Hu, Shu; Lewis, Nathan S.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [McDowell, Matthew T.; Lichterman, Michael F.; Spurgeon, Joshua M.; Hu, Shu; Lewis, Nathan S.] CALTECH, Joint Ctr Artificial Photosynthesis, Pasadena, CA 91125 USA. [Brunschwig, Bruce S.; Lewis, Nathan S.] CALTECH, Beckman Inst, Pasadena, CA 91125 USA. [Lewis, Nathan S.] CALTECH, Kavli Nanosci Inst, Pasadena, CA 91125 USA. [Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynthesis, Berkeley, CA 94720 USA. RP Lewis, NS (reprint author), CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. EM nslewis@caltech.edu RI Sharp, Ian/I-6163-2015; Hu, Shu/B-8120-2013 OI Sharp, Ian/0000-0001-5238-7487; FU Office of Science of the U.S. Department of Energy [DE-SC0004993] FX This material is based upon work performed at the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award DE-SC0004993. XPS data were collected at the Molecular Materials Research Center of the Beckman Institute of the California Institute of Technology. NR 50 TC 46 Z9 46 U1 14 U2 136 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19618 EP 19624 DI 10.1021/jp506133y PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200013 ER PT J AU Shkrob, IA Marin, TW Zhu, Y Abraham, DP AF Shkrob, Ilya A. Marin, Timothy W. Zhu, Ye Abraham, Daniel P. TI Why Bis(fluorosulfonyl)imide Is a "Magic Anion" for Electrochemistry SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-ION BATTERIES; SOLID-ELECTROLYTE INTERFACE; SPIN-HAMILTONIAN ENERGIES; LITHIUM DENDRITE GROWTH; INDUCED REDOX REACTIONS; LIQUID ELECTROLYTES; RECHARGEABLE BATTERIES; DEGRADATION-PRODUCTS; RADIATION-CHEMISTRY; ALUMINUM CORROSION AB Ionic liquids consisting of bis(fluorosulfonyl)imide (FSI-) anion show promise as electrolytes for Li-ion-based electric storage devices, as they exhibit relatively low viscosity, high chemical stability, and form robust solid electrolyte interphase (SET) protecting liquid electrolyte from further breakdown on the electrode. These ionic liquids have been reported to inhibit dendrite formation on lithium metal and lithiated graphite electrodes, which also relates to the unusual SEI properties. In this study, we examine the chemistry aspects that may account for this behavior. Radiolysis was used to induce redox reactions of FSI- anions in model systems, and matrix isolation electron paramagnetic resonance was used to identify radical (ion) intermediates generated in these reactions. Our results suggest that qualitative differences between such ionic liquid electrolytes versus common carbonate electrolytes reflect ease of mineralization of the reduced anion without the concurrent generation of organic radicals and/or elimination of gaseous products in side reactions of the corresponding radical intermediates. C1 [Shkrob, Ilya A.; Marin, Timothy W.; Zhu, Ye; Abraham, Daniel P.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Marin, Timothy W.] Benedictine Univ, Dept Chem, Lisle, IL 60532 USA. RP Shkrob, IA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM shkrob@anl.gov FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX We thank S. Chemerisov, D. Quigley, and R. Lowers for technical support. We are grateful to W. Henderson (PNNL) and K. Zaghib (Hydro-Quebec) for providing some of the Li FSI salt used in this work. This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Award Number DE-AC02-06CH11357. Programmatic support via a DOE SISGR grant "An Integrated Basic Research Program for Advanced Nuclear Energy Separations Systems Based on Ionic Liquids" is gratefully acknowledged. NR 83 TC 24 Z9 24 U1 14 U2 106 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19661 EP 19671 DI 10.1021/jp506567p PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200018 ER PT J AU Chialvo, AA Vlcek, L Cummings, PT AF Chialvo, Ariel A. Vlcek, Lukas Cummings, Peter T. TI Surface Strain Effects on the Water-Graphene Interfacial and Confinement Behavior SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; NANOSCOPIC HYDROPHOBIC SOLUTES; MEAN FORCE; NEUTRON-SCATTERING; SUPERCOOLED WATER; THERMAL-EXPANSION; WETTABILITY; EVAPORATION; NANOSCALE; ROUGHNESS AB We studied via molecular dynamics the link between the strain-driven hydration free-energy changes in the association process involving finite-size graphene surfaces, the resulting water graphene interfacial tension, and the combined effect of the surface strain and confinement on the thermodynamic response functions and the dynamics of confined water. We found that an in-plane biaxial tensile strain epsilon = 10% enhances significantly not only the water graphene hydrophobicity with respect to that of the unstrained counterpart but also the confinement effect on the thermodynamic response functions and slowing down of the dynamics of water over those of the corresponding bulk counterpart. The interfacial behavior of water in contact with strained-graphene plates resembles that observed for "pp" corrugated-plate configuration, as reported earlier [Chialvo et al. J. Phys. Chem. C 2013, 117, 23875], exibiting a significant enhancement of the fluid surface hydrophobicity and response functions relative to those of the unstrained surface. In contrast, the slowing down of the dynamics of the confined water does not show any differentiation with respect to the type of surface. C1 [Chialvo, Ariel A.; Vlcek, Lukas] Oak Ridge Natl Lab, Chem Sci Div, Geochem & Interfacial Sci Grp, Oak Ridge, TN 37831 USA. [Vlcek, Lukas] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. [Cummings, Peter T.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. RP Chialvo, AA (reprint author), Oak Ridge Natl Lab, Chem Sci Div, Geochem & Interfacial Sci Grp, Oak Ridge, TN 37831 USA. EM chialvoaa@ornl.gov RI Vlcek, Lukas/N-7090-2013; OI Vlcek, Lukas/0000-0003-4782-7702; Chialvo, Ariel/0000-0002-6091-4563 FU Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This research was supported as part of the Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 67 TC 11 Z9 11 U1 4 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19701 EP 19711 DI 10.1021/jp501776m PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200022 ER PT J AU Stoerzinger, KA Hong, WT Crumlin, EJ Bluhm, H Biegalski, MD Shao-Horn, Y AF Stoerzinger, Kelsey A. Hong, Wesley T. Crumlin, Ethan J. Bluhm, Hendrik Biegalski, Michael D. Shao-Horn, Yang TI Water Reactivity on the LaCoO3 (001) Surface: An Ambient Pressure X-ray Photoelectron Spectroscopy Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PEROVSKITE-TYPE OXIDES; FUNDAMENTAL-ASPECTS; SOLID-SURFACES; METAL-OXIDES; FUEL-CELLS; XPS; ADSORPTION; FILMS; PHOTOEMISSION; PRINCIPLES AB The reactivity of water with the (001)(pc) surface of epitaxial LaCoO3 (LCO) thin films was investigated as a function of relative humidity (RH) by ambient pressure X-ray photoelectron spectroscopy. Specifically, water isobars (pH(2)O = 100 mTorr) were performed cooling from 300 to 25 degrees C, reaching a final RH of similar to 0.3%. Significant changes were found in the O 1s and C is core-level spectra at different RHs, which were deconvoluted to yield new insights into the hydroxylation and hydration of the LCO surface. Surface hydroxyl groups were found dominant, which were accompanied by minor components including (bi)carbonates, adsorbed water, and undercoordinated/surface-dipole-influenced oxygen sites on the perovskite surface. A multilayer model was used to quantify the coverage of each species, from which the LCO (001)(pc) surface was found to exhibit three different regimes upon increasing RH. The water reactivity with the LCO surface proceeded by surface hydroxylatation to reach saturation (up to similar to 0.5 ML), after which carbonates were found to displace hydroxyl groups, and then adsorption of water molecules. C1 [Stoerzinger, Kelsey A.; Hong, Wesley T.; Shao-Horn, Yang] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Shao-Horn, Yang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Crumlin, Ethan J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Stoerzinger, KA (reprint author), MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. EM kastoerz@mit.edu; shaohorn@mit.edu OI Stoerzinger, Kelsey/0000-0002-3431-8290 FU MRSEC Program of the National Science Foundation [DMR-0819762]; Skoltech-MIT Center for Electrochemical Energy; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US Department of Energy at the Lawrence Berkeley National Laboratory [DE- AC02-05CH11231]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation [DGE-1122374] FX We give many thanks to Andrey Shavorskiy for assistance with AP-XPS measurements. This work was supported in part by the MRSEC Program of the National Science Foundation under award number DMR-0819762 and the Skoltech-MIT Center for Electrochemical Energy. The ALS and the MES beamline 11.0.2 are supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US Department of Energy at the Lawrence Berkeley National Laboratory under Contract No. DE- AC02-05CH11231. The PLD preparation performed was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. K.A.S. was supported by the National Science Foundation Graduate Research Fellowship under grant no. DGE-1122374. NR 63 TC 11 Z9 11 U1 5 U2 94 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19733 EP 19741 DI 10.1021/jp502970r PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200025 ER PT J AU McCarty, KF Monti, M Nie, S Siegel, DA Starodub, E El Gabaly, F McDaniel, AH Shavorskiy, A Tyliszczak, T Bluhm, H Bartelt, NC de la Figuera, J AF McCarty, Kevin F. Monti, Matteo Nie, Shu Siegel, David A. Starodub, Elena El Gabaly, Farid McDaniel, Anthony H. Shavorskiy, Andrey Tyliszczak, Tolek Bluhm, Hendrik Bartelt, Norman C. de la Figuera, Juan TI Oxidation of Magnetite(100) to Hematite Observed by in Situ Spectroscopy and Microscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; WATER-GAS SHIFT; IRON-OXIDES; RAMAN MICROSPECTROSCOPY; ELECTRONIC-STRUCTURE; THIN-FILMS; SURFACE; NANOPARTICLES; ALPHA-FE2O3; OXYGEN AB We study where and how hematite (alpha-Fe2O3) nucleates and grows during the oxidation of magnetite(100) single crystals. Hematite inclusions grow along < 110 > directions of the magnetite (Fe3O4), leading to a biaxial array of hematite slabs in an electrically conducting matrix of magnetite. The slab arrays form in both bulk single crystals and thin films of magnetite. Atomic force microscopy reveals that the surface growth of magnetite that accompanies hematite formation is faster adjacent to the hematite slabs. In situ X-ray photoelectron and X-ray absorption spectroscopies at 600 degrees C in an oxygen environment reveal that the conversion of the Fe2+ in magnetite to Fe3+ in hematite occurs without the formation of the metastable phase maghemite (gamma-Fe2O3). We offer an explanation of why Fe3O4(100) oxidizes faster than Fe3O4(111). C1 [McCarty, Kevin F.; Nie, Shu; Siegel, David A.; Starodub, Elena; El Gabaly, Farid; McDaniel, Anthony H.; Bartelt, Norman C.] Sandia Natl Labs, Livermore, CA 94550 USA. [Monti, Matteo; de la Figuera, Juan] CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain. [Shavorskiy, Andrey; Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP McCarty, KF (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM mccarty@sandia.gov RI de la Figuera, Juan/E-7046-2010; OI de la Figuera, Juan/0000-0002-7014-4777; Monti, Matteo/0000-0003-3595-4472 FU Divisions of Materials and Engineering Sciences [DE-AC04-94AL85000]; Chemical Sciences, Geosciences, and Biosciences of the Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; Spanish Ministry of Science and Innovation [MAT2012-38045-C04-01]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX Our research was supported by the Divisions of Materials and Engineering Sciences (under Contract DE-AC04-94AL85000 for SNL) and Chemical Sciences, Geosciences, and Biosciences (under Contract DE-AC02-05CH11231 for LBNL) of the Office of Basic Energy Sciences, U.S. Department of Energy, and the Spanish Ministry of Science and Innovation through Project MAT2012-38045-C04-01. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. H.B. acknowledges support from the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the U.S. Department of Energy under Contract DE-AC02-05CH11231. We thank the group of Marta Castillejo at the Instituto Quimica-Fisica "Rocasolano", Spain, for providing the magnetite film on SrTiO3:Nb sample and Prof. Gareth Parkinson for lending us a synthetic magnetite crystal. NR 62 TC 9 Z9 9 U1 11 U2 85 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19768 EP 19777 DI 10.1021/jp5037603 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200028 ER PT J AU Sanchez-Camacho, P Romero-Ibarra, IC Duan, YH Pfeiffer, H AF Sanchez-Camacho, Pedro Romero-Ibarra, Issis C. Duan, Yuhua Pfeiffer, Heriberto TI Thermodynamic and Kinetic Analyses of the CO2 Chemisorption Mechanism on Na2TiO3: Experimental and Theoretical Evidences SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CARBON-DIOXIDE SORPTION; NANOCRYSTALLINE LITHIUM ZIRCONATE; ENHANCED HYDROGEN-PRODUCTION; DOPED LI2ZRO3 SORBENTS; HIGH-TEMPERATURE; CAPTURE PROPERTIES; LI4SIO4-BASED SORBENTS; ABSORPTION PROPERTIES; SODIUM TITANATE; PARTICLE-SIZE AB Sodium metatitanate (Na2TiO3) was successfully synthesized via a solid-state reaction. The Na2TiO3 structure and microstructure were characterized using X-ray diffraction, scanning and transmission electron microscopy, and N-2 adsorption. Then, the CO2 chemisorption mechanism on Na2TiO3 was systematically analyzed to determine the influence of temperature. The CO2 chemisorption capacity of Na2TiO3 was evaluated both dynamically and isothermally, and the products were reanalyzed to elucidate the Na2TiO3-CO2 reaction mechanism. Different chemical species (Na2CO3, Na2O, and Na4Ti5O12 or Na16Ti10O28) were identified during the CO2 capture process in Na2TiO3. In addition, some CO2 chemisorption kinetic parameters were determined. The Delta H double dagger was found to be 140.9 kJ/mol, to the Na2TiO3-CO2 system, between 600 and 780 degrees C. Results evidenced that CO2 chemisorption on Na2TiO3 highly depends on the reaction temperature. Furthermore, the experiments were theoretically supported by different thermodynamic calculations. The calculated thermodynamic properties of CO2 capture reactions by (Na2TiO3, Na4Ti5O12, and Na16Ti10O28) sodium titanates were fully investigated. C1 [Sanchez-Camacho, Pedro; Romero-Ibarra, Issis C.; Pfeiffer, Heriberto] Univ Nacl Autonoma Mexico, Inst Invest Mat, Mexico City 04510, DF, Mexico. [Duan, Yuhua] US DOE, Natl Energy Technol Lab, Pittsburgh, PA USA. RP Pfeiffer, H (reprint author), Univ Nacl Autonoma Mexico, Inst Invest Mat, Circuito Exterior S-N,Cd Univ, Mexico City 04510, DF, Mexico. EM pfeiffer@iim.unam.mx RI Duan, Yuhua/D-6072-2011; OI Duan, Yuhua/0000-0001-7447-0142; Pfeiffer, Heriberto/0000-0002-6217-3420 FU SENER-CONACYT [150358]; CONACYT FX This work was financially supported by the project SENER-CONACYT 150358. P. Sanchez-Camacho thanks CONACYT for financial support. The authors thank to Adriana Tejeda, Omar Novelo and Carlos Flores for technical help. NR 98 TC 12 Z9 12 U1 5 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19822 EP 19832 DI 10.1021/jp504922e PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200034 ER PT J AU Salas, G Camarero, J Cabrera, D Takacs, H Varela, M Ludwig, R Dahring, H Hilger, I Miranda, R Morales, MD Teran, FJ AF Salas, Gorka Camarero, Julio Cabrera, David Takacs, Helene Varela, Maria Ludwig, Robert Daehring, Heidi Hilger, Ingrid Miranda, Rodolfo del Puerto Morales, Maria Jose Teran, Francisco TI Modulation of Magnetic Heating via Dipolar Magnetic Interactions in Monodisperse and Crystalline Iron Oxide Nanoparticles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID BIOMEDICAL APPLICATIONS; HYPERTHERMIA RESPONSE; PARTICLES; FIELD; NANOCRYSTALS; EFFICIENCY; MEDIATORS; FLUIDS; SIZE; SPIN AB In the pursuit of controlling the heat exposure mediated by magnetic nanoparticles, we provide new guidelines for tailoring magnetic relaxation processes via dipolar interactions. For this purpose, highly crystalline and monodisperse magnetic iron oxide nanocrystals whose sizes range from 7 to 22 nm were synthesized by thermal decomposition of iron organic precursors in 1-octadecene. The as-synthesized nanoparticles are soft nanomagnets, showing superparamagnetic-like behavior and SAR values which progressively increase with particle size, field frequency, and amplitude up to 3.6 kW/g(Fe). Our data show the influence of media viscosity, particle size, and concentration on dipolar interactions and consequently on the magnetic relaxation processes related to the heat release. Understanding the role of dipolar interactions is of great importance toward the use of iron oxide nanoparticles as efficient hyperthermia mediators. C1 [Salas, Gorka; Camarero, Julio; Cabrera, David; Takacs, Helene; Miranda, Rodolfo; Jose Teran, Francisco] IMDEA Nanociencia, Madrid 28049, Spain. [Salas, Gorka; Takacs, Helene; del Puerto Morales, Maria] Inst Ciencia Mat Madrid CSIC, Madrid 28049, Spain. [Camarero, Julio; Miranda, Rodolfo] Univ Autonoma Madrid, Dept Fis Mat Condensada, E-28049 Madrid, Spain. [Camarero, Julio; Miranda, Rodolfo] Univ Autonoma Madrid, Inst Nicolas Cabrera, E-28049 Madrid, Spain. [Varela, Maria] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Varela, Maria] Univ Complutense Madrid, Dept Fis Aplicada 3, E-28040 Madrid, Spain. [Varela, Maria] Univ Complutense Madrid, Inst Pluridisciplinar, E-28040 Madrid, Spain. [Ludwig, Robert; Daehring, Heidi; Hilger, Ingrid] Univ Jena, Jena Univ Hosp, Inst Diagnost & Intervent Radiol 1, D-07740 Jena, Germany. [Jose Teran, Francisco] Unidad Asociada Nanobiotecnol CNB CSIC, Madrid 28049, Spain. [Jose Teran, Francisco] IMDEA Nanociencia, Madrid 28049, Spain. RP Teran, FJ (reprint author), IMDEA Nanociencia, Campus Univ Cantoblanco, Madrid 28049, Spain. EM francisco.teran@imdea.org RI Salas, Gorka/F-6503-2011; Teran, Francisco/F-1285-2010; Morales Herrero, Maria del Puerto/A-4558-2011; Camarero, Julio/C-4375-2014; Varela, Maria/E-2472-2014; OI Salas, Gorka/0000-0002-1196-8813; Morales Herrero, Maria del Puerto/0000-0002-7290-7029; Varela, Maria/0000-0002-6582-7004; Camarero De Diego, Julio/0000-0003-0078-7280 FU European Commission (MULTIFUN) [262943]; Spanish Ministry of Economy and Competitiveness [MAT2010-21822-C02-01, MAT2011-23641, MAT2013-47395-C4-3-R]; Madrid Regional Government (NANOBIOMAGNET) [S2009/MAT-1726]; European Research Council Starting Investigator Award STEMOX [239739]; U.S. Department of Energy (DOE), Basic Energy Sciences (BES), Materials Sciences and Engineering Division; ORNL's Shared Research Equipment (ShaRE) User Program; DOE-BES; Ramon y Cajal subprogram [RYC-2011-09617] FX This work has been partially supported by European Commission (MULTIFUN, no. 262943), Spanish Ministry of Economy and Competitiveness (MAT2010-21822-C02-01, MAT2011-23641, MAT2013-47395-C4-3-R), Madrid Regional Government (NANOBIOMAGNET, S2009/MAT-1726), and the European Research Council Starting Investigator Award STEMOX # 239739. Research at ORNL was supported by the U.S. Department of Energy (DOE), Basic Energy Sciences (BES), Materials Sciences and Engineering Division, and through a user project supported by ORNL's Shared Research Equipment (ShaRE) User Program, which is also sponsored by DOE-BES. F.J.T. acknowledges financial support from Ramon y Cajal subprogram (RYC-2011-09617). We thank C. Casado, R. Amaro, and L. de la Cueva for technical support and Dr. David Serantes for fruitful discussions. NR 51 TC 21 Z9 21 U1 3 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 28 PY 2014 VL 118 IS 34 BP 19985 EP 19994 DI 10.1021/jp5041234 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AO2CD UT WOS:000341122200050 ER PT J AU Haxton, W AF Haxton, Wick TI NEUTRINO PHYSICS what makes the Sun shine SO NATURE LA English DT Editorial Material C1 [Haxton, Wick] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Haxton, Wick] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Haxton, W (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM haxton@berkeley.edu NR 12 TC 1 Z9 1 U1 2 U2 4 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 28 PY 2014 VL 512 IS 7515 BP 378 EP 380 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN8GC UT WOS:000340840600020 PM 25164744 ER PT J AU Brown, JB Boley, N Eisman, R May, GE Stoiber, MH Duff, MO Booth, BW Wen, JY Park, S Suzuki, AM Wan, KH Yu, C Zhang, DY Carlson, JW Cherbas, L Eads, BD Miller, D Mockaitis, K Roberts, J Davis, CA Frise, E Hammonds, AS Olson, S Shenker, S Sturgill, D Samsonova, AA Weiszmann, R Robinson, G Hernandez, J Andrews, J Bickel, PJ Carninci, P Cherbas, P Gingeras, TR Hoskins, RA Kaufman, TC Lai, EC Oliver, B Perrimon, N Graveley, BR Celniker, SE AF Brown, James B. Boley, Nathan Eisman, Robert May, Gemma E. Stoiber, Marcus H. Duff, Michael O. Booth, Ben W. Wen, Jiayu Park, Soo Suzuki, Ana Maria Wan, Kenneth H. Yu, Charles Zhang, Dayu Carlson, Joseph W. Cherbas, Lucy Eads, Brian D. Miller, David Mockaitis, Keithanne Roberts, Johnny Davis, Carrie A. Frise, Erwin Hammonds, Ann S. Olson, Sara Shenker, Sol Sturgill, David Samsonova, Anastasia A. Weiszmann, Richard Robinson, Garret Hernandez, Juan Andrews, Justen Bickel, Peter J. Carninci, Piero Cherbas, Peter Gingeras, Thomas R. Hoskins, Roger A. Kaufman, Thomas C. Lai, Eric C. Oliver, Brian Perrimon, Norbert Graveley, Brenton R. Celniker, Susan E. TI Diversity and dynamics of the Drosophila transcriptome SO NATURE LA English DT Article ID GENOME-WIDE ANALYSIS; LONG NONCODING RNAS; MELANOGASTER GENOME; EXPRESSION ANALYSIS; ENDOGENOUS SIRNAS; GENE-EXPRESSION; CAP-ANALYSIS; IDENTIFICATION; LANDSCAPE; COMPLEX AB Animal transcriptomes are dynamic with each cell type, tissue and organ system expressing an ensemble of transcript forms that give rise to substantial diversity. Here we have identified new genes, transcripts and proteins using poly(A)(+) RNA sequencing from Drosophila melanogaster in cultured cell lines, dissected organ systems and under environmental perturbations. We found that a small set of mostly neural-specific genes has the potential to encode thousands of transcripts each through extensive alternative promoter usage and RNA splicing. The magnitudes of splicing changes are larger between tissues than between developmental stages, and most sex-specific splicing is gonad-specific. Gonads express hundreds of previously unknown coding and long non-coding RNAs (lncRNAs), some of which are antisense to protein-coding genes and produce short regulatory RNAs. Furthermore, previously identified pervasive intergenic transcription occurs primarily within newly identified introns. The fly transcriptome is substantially more complex than previously recognized, with this complexity arising from combinatorial usage of promoters splice sites and polyaclenylation sites. C1 [Brown, James B.; Boley, Nathan; Stoiber, Marcus H.; Robinson, Garret; Hernandez, Juan; Bickel, Peter J.] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. [Brown, James B.; Booth, Ben W.; Park, Soo; Wan, Kenneth H.; Yu, Charles; Carlson, Joseph W.; Frise, Erwin; Hammonds, Ann S.; Weiszmann, Richard; Hoskins, Roger A.; Celniker, Susan E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. [Eisman, Robert; Cherbas, Lucy; Eads, Brian D.; Miller, David; Mockaitis, Keithanne; Andrews, Justen; Cherbas, Peter; Kaufman, Thomas C.] Indiana Univ, Dept Biol, Bloomington, IN 47405 USA. [May, Gemma E.; Duff, Michael O.; Olson, Sara; Graveley, Brenton R.] Univ Connecticut, Ctr Hlth, Inst Syst Genom, Dept Genet & Dev Biol, Farmington, CT 06030 USA. [Wen, Jiayu; Shenker, Sol; Lai, Eric C.] Sloan Kettering Inst, Rockefeller Res Labs 1017C, New York, NY 10065 USA. [Suzuki, Ana Maria; Carninci, Piero] RIKEN Omics Sci Ctr, Yokohama, Kanagawa 2300045, Japan. [Suzuki, Ana Maria; Carninci, Piero] RIKEN Ctr Life Sci Technol, Div Genom Technol, Yokohama, Kanagawa 2300045, Japan. [Zhang, Dayu; Roberts, Johnny; Cherbas, Peter] Indiana Univ, Ctr Genom & Bioinformat, Bloomington, IN 47405 USA. [Davis, Carrie A.; Gingeras, Thomas R.] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA. [Sturgill, David; Oliver, Brian] NIDDK, Sect Dev Genom, Lab Cellular & Dev Biol, NIH, Bethesda, MD 20892 USA. [Samsonova, Anastasia A.; Perrimon, Norbert] Harvard Univ, Sch Med, Dept Genet, Boston, MA 02115 USA. [Samsonova, Anastasia A.; Perrimon, Norbert] Harvard Univ, Sch Med, Howard Hughes Med Inst, Boston, MA 02115 USA. RP Brown, JB (reprint author), Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. EM benbrownofberkeley@gmail.com; graveley@neuron.uchc.edu; celniker@fruitfly.org RI Brown, James/H-2971-2015; Carninci, Piero/K-1568-2014; Samsonova, Anastasia/Q-7591-2016; OI Carninci, Piero/0000-0001-7202-7243; Samsonova, Anastasia/0000-0002-9353-9173; Gingeras, Thomas/0000-0001-9106-3573; Graveley, Brenton/0000-0001-5777-5892 FU National Human Genome Research Institute; Department of Energy [U01 HG004271, U54 HG006944, R01 GM076655, DE-AC02-05CH11231]; NHGRI [K99 HG006698]; modENCODE DAC sub-award [5710003102, 1U01HG007031-01]; ENCODE DAC [5U01HG004695-04]; Indiana METACyt Initiative of Indiana University - Lilly Endowment; [U01-HG004261]; [RC2-HG005639] FX We thank the members of the modENCODE transcription consortium, especially J. Landolin and J. Sandler for their early contributions to these studies. We also thank A. Kundaje and H. Huang for helpful discussions. This work was funded by a contract from the National Human Genome Research Institute modENCODE Project, contract U01 HG004271 and U54 HG006944, to S.E.C. (principal investigator) and P.C., T.R.G., R.A.H. and B.R.G. (co-principal investigators) with additional support from R01 GM076655 (S.E.C.) both under Department of Energy contract no. DE-AC02-05CH11231. J.B.B.'s work was supported by NHGRI K99 HG006698. Work in P.J.B.'s group was supported by the modENCODE DAC sub-award 5710003102, 1U01HG007031-01 and the ENCODE DAC 5U01HG004695-04. Work in Bloomington was supported in part by the Indiana METACyt Initiative of Indiana University, funded by an award from the Lilly Endowment. Work in E.C.L.'s group was supported by U01-HG004261 and RC2-HG005639. NR 50 TC 126 Z9 128 U1 15 U2 92 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 28 PY 2014 VL 512 IS 7515 BP 393 EP 399 DI 10.1038/nature12962 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN8GC UT WOS:000340840600025 PM 24670639 ER PT J AU Gerstein, MB Rozowsky, J Yan, KK Wang, DF Cheng, C Brown, JB Davis, CA Hillier, L Sisu, C Li, JJ Pei, BK Harmanci, AO Duff, MO Djebali, S Alexander, RP Alver, BH Auerbach, R Bell, K Bickel, PJ Boeck, ME Boley, NP Booth, BW Cherbas, L Cherbas, P Di, C Dobins, A Drenkows, J Ewing, B Fang, G Fastucas, M Feingold, EA Frankish, A Gao, GJ Good, PJ Guigo, R Hammonds, A Harrow, J Hoskins, RA Howald, C Hu, L Huang, HY Hubbard, TJP Huynh, C Jhas, S Kasper, D Kato, M Kaufman, TC Kitchen, RR Ladewig, E Lagarde, J Lai, E Leng, L Lu, Z MacCoss, M May, G McWhirter, R Merrihew, G Miller, DM Mortazavi, A Murad, R Oliver, B Olson, S Park, PJ Pazin, MJ Perrimon, N Pervouchine, D Reinke, V Reymond, A Robinson, G Samsonova, A Saunders, GI Schlesingers, F Sethi, A Slack, FJ Spencer, WC Stoiber, MH Strasbourger, P Tanzer, A Thompson, OA Wan, KH Wang, GL Wang, H Watkins, KL Wen, JY Wen, KJ Xue, CH Yang, L Yip, K Zaleskis, C Zhang, Y Zheng, H Brenner, SE Graveley, BR Ceniker, SE Gingeras, TR Waterston, R AF Gerstein, Mark B. Rozowsky, Joel Yan, Koon-Kiu Wang, Daifeng Cheng, Chao Brown, James B. Davis, Carrie A. Hillier, LaDeana Sisu, Cristina Li, Jingyi Jessica Pei, Baikang Harmanci, Arif O. Duff, Michael O. Djebali, Sarah Alexander, Roger P. Alver, Burak H. Auerbach, Raymond Bell, Kimberly Bickel, Peter J. Boeck, Max E. Boley, Nathan P. Booth, Benjamin W. Cherbas, Lucy Cherbas, Peter Di, Chao Dobins, Alex Drenkows, Jorg Ewing, Brent Fang, Gang Fastucas, Megan Feingold, Elise A. Frankish, Adam Gao, Guanjun Good, Peter J. Guigo, Roderic Hammonds, Ann Harrow, Jen Hoskins, Roger A. Howald, Cedric Hu, Long Huang, Haiyan Hubbard, Tim J. P. Huynh, Chau Jhas, Sonali Kasper, Dionna Kato, Masaomi Kaufman, Thomas C. Kitchen, Robert R. Ladewig, Erik Lagarde, Julien Lai, Eric Leng, Ling Lu, Zhi MacCoss, Michael May, Gemma McWhirter, Rebecca Merrihew, Gennifer Miller, David M. Mortazavi, Ali Murad, Rabi Oliver, Brian Olson, Sara Park, Peter J. Pazin, Michael J. Perrimon, Norbert Pervouchine, Dmitri Reinke, Valerie Reymond, Alexandre Robinson, Garrett Samsonova, Anastasia Saunders, Gary I. Schlesingers, Felix Sethi, Anurag Slack, Frank J. Spencer, William C. Stoiber, Marcus H. Strasbourger, Pnina Tanzer, Andrea Thompson, Owen A. Wan, Kenneth H. Wang, Guilin Wang, Huaien Watkins, Kathie L. Wen, Jiayu Wen, Kejia Xue, Chenghai Yang, Li Yip, Kevin Zaleskis, Chris Zhang, Yan Zheng, Henry Brenner, Steven E. Graveley, Brenton R. Ceniker, Susan E. Gingeras, Thomas R. Waterston, Robert TI Comparative analysis of the transcriptome across distant species SO NATURE LA English DT Article ID GENE-EXPRESSION; LANDSCAPE; EVOLUTION; TISSUES; GENOME; CELLS AB The transcriptome is the readout of the genome. Identifying common features in it across distant species can reveal fundamental principles. To this end, the ENCODE and modENCODE consortia have generated large amounts of matched RNA-sequencing data for human, worm and fly. Uniform processing and comprehensive annotation of these data allow comparison across metazoan phyla, extending beyond earlier within-phylum transcriptome comparisons and revealing ancient, conserved features(1-6). Specifically, we discover co-expression modules shared across animals, many of which are enriched in developmental genes. Moreover, we use expression patterns to align the stages in worm and fly development and find a novel pairing between worm embryo and fly pupae, in addition to the embryo-to-embryo and larvae-to-larvae pairings. Furthermore, we find that the extent of non-canonical, non-coding transcription is similar in each organism, per base pair. Finally, we find in all three organisms that the gene-expression levels, both coding and non-coding, can be quantitatively predicted from chromatin features at the promoter using a 'universal model' based on a single set of organism-independent parameters. C1 [Gerstein, Mark B.; Rozowsky, Joel; Yan, Koon-Kiu; Wang, Daifeng; Sisu, Cristina; Pei, Baikang; Harmanci, Arif O.; Alexander, Roger P.; Auerbach, Raymond; Fang, Gang; Kitchen, Robert R.; Leng, Ling; Mortazavi, Ali; Sethi, Anurag; Zhang, Yan; Zheng, Henry] Yale Univ, Program Computat Biol & Bioinformat, New Haven, CT 06520 USA. [Gerstein, Mark B.; Rozowsky, Joel; Yan, Koon-Kiu; Wang, Daifeng; Sisu, Cristina; Pei, Baikang; Harmanci, Arif O.; Alexander, Roger P.; Auerbach, Raymond; Fang, Gang; Kitchen, Robert R.; Leng, Ling; Mortazavi, Ali; Sethi, Anurag; Zhang, Yan; Zheng, Henry] Yale Univ, Dept Mol Biophys & Biochem, New Haven, CT 06520 USA. [Gerstein, Mark B.] Yale Univ, Dept Comp Sci, New Haven, CT 06511 USA. [Cheng, Chao] Geisel Sch Med Dartmouth, Dept Genet, Hanover, NH 03755 USA. [Cheng, Chao] Geisel Sch Med Dartmouth, Inst Quantitat Biomed Sci, Norris Cotton Canc Ctr, Lebanon, NH 03766 USA. [Brown, James B.; Boley, Nathan P.; Booth, Benjamin W.; Hammonds, Ann; Hoskins, Roger A.; Stoiber, Marcus H.; Wan, Kenneth H.; Ceniker, Susan E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. [Brown, James B.; Li, Jingyi Jessica; Bickel, Peter J.; Huang, Haiyan; Robinson, Garrett] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. [Davis, Carrie A.; Bell, Kimberly; Dobins, Alex; Drenkows, Jorg; Fastucas, Megan; Jhas, Sonali; Schlesingers, Felix; Wang, Huaien; Xue, Chenghai; Zaleskis, Chris; Gingeras, Thomas R.] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA. [Hillier, LaDeana; Boeck, Max E.; Ewing, Brent; Huynh, Chau; MacCoss, Michael; Merrihew, Gennifer; Strasbourger, Pnina; Thompson, Owen A.; Waterston, Robert] Dept Genome Sci, Seattle, WA 98195 USA. [Hillier, LaDeana; Boeck, Max E.; Ewing, Brent; Huynh, Chau; MacCoss, Michael; Merrihew, Gennifer; Strasbourger, Pnina; Thompson, Owen A.; Waterston, Robert] Univ Washington, Sch Med, Seattle, WA 98195 USA. [Li, Jingyi Jessica] Univ Calif Los Angeles, Dept Stat, Los Angeles, CA 90095 USA. [Li, Jingyi Jessica] Univ Calif Los Angeles, Dept Human Genet, Los Angeles, CA 90095 USA. [Duff, Michael O.; May, Gemma; Olson, Sara; Yang, Li; Graveley, Brenton R.] Univ Connecticut, Ctr Hlth, Inst Syst Genom, Dept Genet & Dev Biol, Farmington, CT 06030 USA. [Djebali, Sarah; Guigo, Roderic; Lagarde, Julien; Pervouchine, Dmitri] Ctr Genom Regulat, Barcelona 08003, Catalonia, Spain. [Djebali, Sarah; Guigo, Roderic; Lagarde, Julien; Pervouchine, Dmitri] Univ Pompeu Fabra, Dept Ciencies Expt Salut, Barcelona 08003, Catalonia, Spain. [Alver, Burak H.; Park, Peter J.] Harvard Univ, Sch Med, Ctr Biomed Informat, Boston, MA 02115 USA. [Boley, Nathan P.; Stoiber, Marcus H.] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. [Cherbas, Lucy; Cherbas, Peter; Kaufman, Thomas C.] Indiana Univ, Dept Biol, Bloomington, IN 47405 USA. [Cherbas, Lucy; Cherbas, Peter] Indiana Univ, Ctr Genom & Bioinformat, Bloomington, IN 47405 USA. [Di, Chao; Gao, Guanjun; Hu, Long; Lu, Zhi; Wen, Kejia] Tsinghua Univ, Sch Life Sci, MOE Key Lab Bioinformat, Beijing 100084, Peoples R China. [Feingold, Elise A.; Good, Peter J.; Pazin, Michael J.] NHGRI, NIH, Bethesda, MD 20892 USA. [Frankish, Adam; Harrow, Jen; Hubbard, Tim J. P.; Saunders, Gary I.] Wellcome Trust Sanger Inst, Cambridge CB10 1SA, England. [Howald, Cedric; Reymond, Alexandre] Univ Lausanne, Ctr Integrat Genom, CH-1015 Lausanne, Switzerland. [Howald, Cedric] Swiss Inst Bioinformat, CH-1015 Lausanne, Switzerland. [Hubbard, Tim J. P.] Kings Coll London, London WC2R 2LS, England. [Kasper, Dionna; Reinke, Valerie; Wang, Guilin] Yale Univ, Sch Med, Dept Genet, New Haven, CT 06520 USA. [Kato, Masaomi; Slack, Frank J.] Yale Univ, Dept Mol Cellular & Dev Biol, New Haven, CT 06520 USA. [Ladewig, Erik; Lai, Eric; Wen, Jiayu] Sloan Kettering Inst, New York, NY 10065 USA. [May, Gemma] Carnegie Mellon Univ, Dept Biol Sci, Pittsburgh, PA 15213 USA. [McWhirter, Rebecca; Miller, David M.; Spencer, William C.; Watkins, Kathie L.] Vanderbilt Univ, Dept Cell & Dev Biol, Nashville, TN 37232 USA. [Mortazavi, Ali; Murad, Rabi] Univ Calif Irvine, Irvine, CA 92697 USA. [Mortazavi, Ali; Murad, Rabi] Univ Calif Irvine, Ctr Complex Biol Syst, Irvine, CA 92697 USA. [Oliver, Brian] NIDDK, Sect Dev Genom, Lab Cellular & Dev Biol, NIH, Bethesda, MD 20892 USA. [Perrimon, Norbert; Samsonova, Anastasia] Harvard Univ, Sch Med, Dept Genet, Boston, MA 02115 USA. [Perrimon, Norbert; Samsonova, Anastasia] Harvard Univ, Sch Med, Drosophila RNAi Screening Ctr, Boston, MA 02115 USA. [Perrimon, Norbert; Samsonova, Anastasia] Harvard Univ, Sch Med, Howard Hughes Med Inst, Boston, MA 02115 USA. [Saunders, Gary I.] European Bioinformat Inst, Hinxton CB10 1SD, England. [Tanzer, Andrea] Univ Pompeu Fabra, Ctr Genom Regulat, Bioinformat & Genom Programme, Barcelona 08003, Catalonia, Spain. [Tanzer, Andrea] Univ Vienna, Theoret Biochem Grp TBI, Inst Theoret Chem, A-1090 Vienna, Austria. [Yang, Li] Chinese Acad Sci, Shanghai Inst Biol Sci, CAS MPG Partner Inst Computat Biol, Key Lab Computat Biol, Shanghai 200031, Peoples R China. [Yip, Kevin] Chinese Univ Hong Kong, Hong Kong Bioinformat Ctr, Shatin, Hong Kong, Peoples R China. [Yip, Kevin] Chinese Univ Hong Kong, CUHK BGI Innovat Inst Trans Omics 5, Shatin, Hong Kong, Peoples R China. [Brenner, Steven E.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Brenner, Steven E.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. RP Gerstein, MB (reprint author), Yale Univ, Program Computat Biol & Bioinformat, Bass 432,266 Whitney Ave, New Haven, CT 06520 USA. EM cmptxn@gersteinlab.org RI Djebali, Sarah/O-9817-2014; Di, Chao/G-1130-2015; Brown, James/H-2971-2015; Pervouchine, Dmitri/H-5252-2015; Guigo, Roderic/D-1303-2010; Hubbard, Tim/C-2567-2008; Tanzer, Andrea/L-3147-2015; Brenner, Steven/A-8729-2008; Samsonova, Anastasia/Q-7591-2016; OI Djebali, Sarah/0000-0002-0599-1267; Pervouchine, Dmitri/0000-0003-0543-9760; Guigo, Roderic/0000-0002-5738-4477; Hubbard, Tim/0000-0002-1767-9318; Tanzer, Andrea/0000-0003-2873-4236; Brenner, Steven/0000-0001-7559-6185; Samsonova, Anastasia/0000-0002-9353-9173; Sisu, Cristina/0000-0001-9371-0797; Saunders, Gary/0000-0002-7468-0008; Gerstein, Mark/0000-0002-9746-3719; Graveley, Brenton/0000-0001-5777-5892; Slack, Frank/0000-0001-8263-0409; Rozowsky, Joel/0000-0002-3565-0762; Alver, Burak/0000-0002-5019-7652; Pazin, Michael/0000-0002-7561-3640 FU NHGRI; ENCODE; modENCODE project; National Human Genome Research Institute modENCODE Project under Department of Energy [U01 HG004271, U54 HG006944]; Department of Energy [R01 GM076655, DE-AC02-05CH11231, U54 HG007005]; NHGRI [K99 HG006698]; DOE [DE-AC02-05CH11231]; modENCODE DAC sub award [5710003102, 1 U01HG007031-01]; ENCODE DAC [5U01HG004695-04]; NIH [HG007000, HG007355]; Indiana METACyt Initiative of Indiana University - Lilly Endowment, Inc.; National Institutes of Health [U01HG004258, 5U54HG004555]; Wellcome Trust [WT098051]; Spanish Ministry of Education [BIO2011-26205]; [U01-HG004261]; [RC2-HG005639]; [U01 HG 004263] FX The authors thank the NHGRI and the ENCODE and modENCODE projects for support. In particular, this work was funded by a contract from the National Human Genome Research Institute modENCODE Project, contract U01 HG004271 and U54 HG006944, to S.E.C. (principal investigator) and P.C., T.R.G., R.A.H. and B.R.G. (co-principal investigators) with additional support from R01 GM076655 (S.E.C.) both under Department of Energy contract no. DE-AC02-05CH11231, and U54 HG007005 to B.R.G. J.B.B.'s work was supported by NHGRI K99 HG006698 and DOE DE-AC02-05CH11231. Work in P.J.B.'s group was supported by the modENCODE DAC sub award 5710003102, 1 U01HG007031-01 and the ENCODE DAC 5U01HG004695-04. Work in M.B.G.'s group was supported by NIH grants HG007000 and HG007355. Work in Bloomington was supported in part by the Indiana METACyt Initiative of Indiana University, funded by an award from the Lilly Endowment, Inc. Work in E.C.L.'s group was supported by U01-HG004261 and RC2-HG005639. P.J.P. acknowledges support from the National Institutes of Health (grant no. U01HG004258). We thank the HAVANA team for providing annotation of the human reference genome, whose work is supported by National Institutes of Health (grant no. 5U54HG004555), the Wellcome Trust (grant no. WT098051). R.G. acknowledges support from the Spanish Ministry of Education (grant BIO2011-26205). We also acknowledge use of the Yale University Biomedical High Performance Computing Center. R.W.'s lab was supported by grant no. U01 HG 004263. NR 19 TC 69 Z9 69 U1 11 U2 102 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 28 PY 2014 VL 512 IS 7515 BP 445 EP + DI 10.1038/nature13424 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN8GC UT WOS:000340840600037 PM 25164755 ER PT J AU Ho, JWK June, YL Liu, T Alver, BH Lee, S Ikegami, K Sohn, KA Minoda, A Tolstorukov, MY Appert, A Parker, SCJ Gu, TT Kundaje, A Riddle, NC Bishop, E Egelhofer, TA Hu, SS Alekseyenko, AA Rechtsteiner, A Asker, D Belsky, JA Bowmanm, SK Chens, QB Chen, RAJ Day, DS Dong, Y Dose, AC Duan, XK Epstein, CB Ercan, S Feingold, EA Ferrari, F Garrigues, JM Gehlenborg, N Good, PJ Haseley, P He, D Herrmann, M Hoffman, MM Jeffers, TE Kharchenko, PV Kolasinska-Zwierz, P Kotwaliwale, CV Kumar, N Langley, SA Larschan, EN Latorre, I Libbrecht, MW Lin, XQ Park, R Pazin, MJ Pham, HN Plachetka, A Qin, B Schwartz, YB Shoresh, N Stempor, P Vielle, A Wang, CY Whittle, CM Xue, HL Kingstonm, RE Kim, JH Bernstein, BE Dernburg, AF Pirrotta, V Kuroda, MI Noble, WS Tullius, TD Kellis, M MacAlpine, DM Strome, S Elgin, SCR Liu, XS Lieb, JD Ahringer, J Karpen, GH Park, PJ AF Ho, Joshua W. K. June, Youngsook L. Liu, Tao Alver, Burak H. Lee, Soohyun Ikegami, Kohta Sohn, Kyung-Ah Minoda, Aki Tolstorukov, Michael Y. Appert, Alex Parker, Stephen C. J. Gu, Tingting Kundaje, Anshul Riddle, Nicole C. Bishop, Eric Egelhofer, Thea A. Hu, Sheng'en Shawn Alekseyenko, Artyom A. Rechtsteiner, Andreas Asker, Dalal Belsky, Jason A. Bowmanm, Sarah K. Chens, Q. Brent Chen, Ron A. -J. Day, Daniel S. Dong, Yan Dose, Andrea C. Duan, Xikun Epstein, Charles B. Ercan, Sevinc Feingold, Elise A. Ferrari, Francesco Garrigues, Jacob M. Gehlenborg, Nils Good, Peter J. Haseley, Psalm He, Daniel Herrmann, Moritz Hoffman, Michael M. Jeffers, Tess E. Kharchenko, Peter V. Kolasinska-Zwierz, Paulina Kotwaliwale, Chitra V. Kumar, Nischay Langley, Sasha A. Larschan, Erica N. Latorre, Isabel Libbrecht, Maxwell W. Lin, Xueqiu Park, Richard Pazin, Michael J. Pham, Hoang N. Plachetka, Annette Qin, Bo Schwartz, Yuri B. Shoresh, Noam Stempor, Przemyslaw Vielle, Anne Wang, Chengyang Whittle, Christina M. Xue, Huiling Kingstonm, Robert E. Kim, Ju Han Bernstein, Bradley E. Dernburg, Abby F. Pirrotta, Vincenzo Kuroda, Mitzi I. Noble, William S. Tullius, Thomas D. Kellis, Manolis MacAlpine, David M. Strome, Susan Elgin, Sarah C. R. Liu, Xiaole Shirley Lieb, Jason D. Ahringer, Julie Karpen, Gary H. Park, Peter J. TI Comparative analysis of metazoan chromatin organization SO NATURE LA English DT Article ID CENTROMERIC CHROMATIN; DROSOPHILA GENOME; MODENCODE; ELEMENTS; ELEGANS; STATE; TRANSCRIPTION; METHYLATION; DOMAINS; ENCODE AB Genome function is dynamically regulated in part by chromatin, which consists of the histones, non-histone proteins and RNA molecules that package DNA. Studies in Caenorhabditis elegans and Drosophila melanogaster have contributed substantially to our understanding of molecular mechanisms of genome function in humans, and have revealed conservation of chromatin components and mechanisms(1-3). Nevertheless, the three organisms have markedly different genome sizes, chromosome architecture and gene organization. On human and fly chromosomes, for example, pericentric heterochromatin flanks single centromeres, whereas worm chromosomes have dispersed heterochromatin-like regions enriched in the distal chromosomal 'arms', and centromeres distributed along their lengths(4,5). To systematically investigate chromatin organization and associated gene regulation across species, we generated and analysed a large collection of genome-wide chromatin data sets from cell lines and developmental stages in worm, fly and human. Here we present over 800 new data sets from our ENCODE and modENCODE consortia, bringing the total to over 1,400. Comparison of combinatorial patterns of histone modifications, nuclear lamina-associated domains, organization of large-scale topological domains, chromatin environment at promoters and enhancers, nucleosome positioning, and DNA replication patterns reveals many conserved features of chromatin organization among the three organisms. We also find notable differences in the composition and locations of repressive chromatin. These data sets and analyses provide a rich resource for comparative and species-specific investigations of chromatin composition, organization and function. C1 [Ho, Joshua W. K.; June, Youngsook L.; Alver, Burak H.; Lee, Soohyun; Tolstorukov, Michael Y.; Bishop, Eric; Day, Daniel S.; Ferrari, Francesco; Gehlenborg, Nils; Haseley, Psalm; Kharchenko, Peter V.; Park, Richard; Xue, Huiling; Park, Peter J.] Harvard Univ, Sch Med, Ctr Biomed Informat, Boston, MA 02115 USA. [Ho, Joshua W. K.; June, Youngsook L.; Tolstorukov, Michael Y.; Alekseyenko, Artyom A.; Haseley, Psalm; Plachetka, Annette; Xue, Huiling; Kuroda, Mitzi I.; Park, Peter J.] Harvard Univ, Brigham & Womens Hosp, Sch Med, Div Genet,Dept Med, Boston, MA 02115 USA. [Liu, Tao; Liu, Xiaole Shirley] Dana Farber Canc Inst, Ctr Funct Canc Epigenet, Boston, MA 02215 USA. [Liu, Tao; Liu, Xiaole Shirley] Dana Farber Canc Inst, Dept Biostat & Computat Biol, Boston, MA 02215 USA. [Liu, Tao; Liu, Xiaole Shirley] Harvard Univ, Sch Publ Hlth, Boston, MA 02215 USA. [Ikegami, Kohta; Chens, Q. Brent; Ercan, Sevinc; Jeffers, Tess E.; Lieb, Jason D.] Univ N Carolina, Dept Biol, Chapel Hill, NC 27599 USA. [Ikegami, Kohta; Chens, Q. Brent; Ercan, Sevinc; Jeffers, Tess E.; Lieb, Jason D.] Univ N Carolina, Carolina Ctr Genome Sci, Chapel Hill, NC 27599 USA. [Sohn, Kyung-Ah] Ajou Univ, Dept Informat & Comp Engn, Suwon 443749, South Korea. [Sohn, Kyung-Ah; Kim, Ju Han] Seoul Natl Univ, Coll Med, Syst Biomed Informat Res Ctr, Seoul 110799, South Korea. [Minoda, Aki; Langley, Sasha A.; Pham, Hoang N.; Vielle, Anne; Dernburg, Abby F.; Karpen, Gary H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Dept Genome Dynam, Berkeley, CA 94720 USA. [Minoda, Aki; He, Daniel; Kotwaliwale, Chitra V.; Langley, Sasha A.; Pham, Hoang N.; Whittle, Christina M.; Dernburg, Abby F.; Karpen, Gary H.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Tolstorukov, Michael Y.; Bowmanm, Sarah K.; Kingstonm, Robert E.] Massachusetts Gen Hosp, Dept Mol Biol, Boston, MA 02114 USA. [Tolstorukov, Michael Y.; Bowmanm, Sarah K.; Kingstonm, Robert E.; Bernstein, Bradley E.] Harvard Univ, Sch Med, Boston, MA 02114 USA. [Appert, Alex; Chen, Ron A. -J.; Dong, Yan; Herrmann, Moritz; Kolasinska-Zwierz, Paulina; Latorre, Isabel; Stempor, Przemyslaw; Vielle, Anne; Ahringer, Julie] Univ Cambridge, Gurdon Inst, Cambridge CB2 1QN, England. [Appert, Alex; Chen, Ron A. -J.; Dong, Yan; Herrmann, Moritz; Kolasinska-Zwierz, Paulina; Latorre, Isabel; Stempor, Przemyslaw; Vielle, Anne; Ahringer, Julie] Univ Cambridge, Dept Genet, Cambridge CB2 1QN, England. [Parker, Stephen C. J.] NIGMS, NIH, Bethesda, MD 20892 USA. [Parker, Stephen C. J.; Feingold, Elise A.; Good, Peter J.; Pazin, Michael J.] NHGRI, NIH, Bethesda, MD 20892 USA. [Gu, Tingting; Riddle, Nicole C.; Elgin, Sarah C. R.] Washington Univ, Dept Biol, St Louis, MO 63130 USA. [Kundaje, Anshul; Kumar, Nischay; Kellis, Manolis] MIT, Comp Sci & Artificial Intelligence Lab, Cambridge, MA 02139 USA. [Alver, Burak H.; Kundaje, Anshul; Epstein, Charles B.; Gehlenborg, Nils; Kumar, Nischay; Shoresh, Noam; Vielle, Anne; Bernstein, Bradley E.; Kellis, Manolis; Liu, Xiaole Shirley] Broad Inst, Cambridge, MA 02141 USA. [Bishop, Eric; Park, Richard; Tullius, Thomas D.] Boston Univ, Program Bioinformat, Boston, MA 02215 USA. [Egelhofer, Thea A.; Rechtsteiner, Andreas; Garrigues, Jacob M.; Strome, Susan] Univ Calif Santa Cruz, Dept Mol Cell & Dev Biol, Santa Cruz, CA 95064 USA. [Hu, Sheng'en Shawn; Duan, Xikun; Lin, Xueqiu; Qin, Bo; Wang, Chengyang] Tongji Univ, Sch Life Sci & Technol, Dept Bioinformat, Shanghai 200092, Peoples R China. [Alekseyenko, Artyom A.; Plachetka, Annette; Kuroda, Mitzi I.] Harvard Univ, Sch Med, Dept Genet, Boston, MA 02115 USA. [Asker, Dalal; Schwartz, Yuri B.; Pirrotta, Vincenzo] Rutgers State Univ, Dept Mol Biol & Biochem, Piscataway, NJ 08854 USA. [Asker, Dalal] Univ Alexandria, Fac Agr, Food Sci & Technol Dept, Alexandria 21545, Egypt. [Belsky, Jason A.; MacAlpine, David M.] Duke Univ, Med Ctr, Dept Pharmacol & Canc Biol, Durham, NC 27710 USA. [Day, Daniel S.] Harvard Mit Div Hlth Sci & Technol, Cambridge, MA 02139 USA. [Dose, Andrea C.] Univ Calif Davis, Dept Anat Physiol & Cell Biol, Davis, CA 95616 USA. [Ercan, Sevinc] NYU, Dept Biol, Ctr Genom & Syst Biol, New York, NY 10003 USA. [Hoffman, Michael M.] Princess Margaret Canc Ctr, Toronto, ON M6G 1L7, Canada. [Kotwaliwale, Chitra V.; Pham, Hoang N.; Whittle, Christina M.; Bernstein, Bradley E.; Dernburg, Abby F.] Howard Hughes Med Inst, Chevy Chase, MD 20815 USA. [Larschan, Erica N.] Brown Univ, Dept Mol Biol Cellular Biol & Biochem, Providence, RI 02912 USA. [Libbrecht, Maxwell W.; Noble, William S.] Univ Washington, Dept Comp Sci & Engn, Seattle, WA 98195 USA. [Schwartz, Yuri B.] Umea Univ, Dept Mol Biol, S-90187 Umea, Sweden. [Kim, Ju Han] Seoul Natl Univ, Coll Med, Div Biomed Informat, Seoul Natl Univ Biomed Informat, Seoul 110799, South Korea. [Bernstein, Bradley E.] Massachusetts Gen Hosp, Dept Pathol, Boston, MA 02114 USA. [Noble, William S.] Univ Washington, Dept Genome Sci, Seattle, WA 98195 USA. [Tullius, Thomas D.] Boston Univ, Dept Chem, Boston, MA 02215 USA. [Park, Peter J.] Childrens Hosp, Informat Program, Boston, MA 02215 USA. RP MacAlpine, DM (reprint author), Duke Univ, Med Ctr, Dept Pharmacol & Canc Biol, Durham, NC 27710 USA. EM david.macalpine@duke.edu; sstrome@ucsc.edu; selgin@biology2.wustl.edu; xsliu@jimmy.harvard.edu; jdlieb@uchicago.edu; ja219@cam.ac.uk; ghkarpen@lbl.gov; peter_park@hms.harvard.edu RI Tullius, Thomas/A-9685-2008; Liu, Tao/G-3585-2010; Hoffman, Michael/I-1924-2012; Ferrari, Francesco/H-5007-2012; Asker, Dalal/B-5722-2009; Minoda, Aki/D-5335-2017; OI Stempor, Przemyslaw/0000-0002-9464-7475; Jeffers, Tess/0000-0003-4908-0796; Alver, Burak/0000-0002-5019-7652; Gehlenborg, Nils/0000-0003-0327-8297; Pazin, Michael/0000-0002-7561-3640; Latorre, Isabel/0000-0003-0638-1783; Tullius, Thomas/0000-0003-4425-796X; Liu, Tao/0000-0002-8818-8313; Hoffman, Michael/0000-0002-4517-1562; Ferrari, Francesco/0000-0002-9811-3753; Minoda, Aki/0000-0002-2927-5791; Belsky, Jason/0000-0003-2945-6282; Chen, Ron/0000-0001-9186-6747; Liu, Tao/0000-0003-0446-9001; Sohn, Kyung-Ah/0000-0001-8941-1188 FU NHGRI [U01HG004258, U01 HG004270, U01HG004279, U54HG004570, U01HG004695, K99HG006259]; NHBIB [5RL9EB008539]; NIGMS; NIH [U54CA121852]; NSF [1122374]; National Natural Science Foundation of China [31028011]; MEST Korea [MHW-2013-HI13C2164]; Wellcome Trust [54523]; [NRF-2012-0000994] FX This project was mainly funded by NHGRI U01HG004258 (G.H.K., S.C.R.E., M.I.K., P.J.P., V.P.), U01 HG004270 (J.D.L., J.A., A.F.D., X.S.L., S.S.), U01HG004279 (D.M.M.), U54HG004570 (B.E.B.) and U01HG004695 (W.S.N.). It is also supported by NHBIB 5RL9EB008539 (J.W.K.H.), NHGRI K99HG006259 (M.M.H.), NIGMS fellowships (S.C.J.P., E.N.L.), NIH U54CA121852 (T.D.T.), NSF 1122374 (D.S.D.), National Natural Science Foundation of China 31028011 (X.S.L.), MEST Korea MHW-2013-HI13C2164 (J.H.K.), NRF-2012-0000994 (K-AS.), and Wellcome Trust 54523 (J.A.). We thank D. Acevedo and C. Kennedy for technical assistance. NR 24 TC 79 Z9 81 U1 1 U2 57 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 28 PY 2014 VL 512 IS 7515 BP 449 EP U507 DI 10.1038/nature13415 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN8GC UT WOS:000340840600038 PM 25164756 ER PT J AU Anand, VK Quirinale, DG Lee, Y Harmon, BN Furukawa, Y Ogloblichev, VV Huq, A Abernathy, DL Stephens, PW McQueeney, RJ Kreyssig, A Goldman, AI Johnston, DC AF Anand, V. K. Quirinale, D. G. Lee, Y. Harmon, B. N. Furukawa, Y. Ogloblichev, V. V. Huq, A. Abernathy, D. L. Stephens, P. W. McQueeney, R. J. Kreyssig, A. Goldman, A. I. Johnston, D. C. TI Crystallography and physical properties of BaCo2As2, Ba0.94K0.06Co2As2, and Ba0.78K0.22Co2As2 SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; MAGNETIC-PROPERTIES; TERNARY ARSENIDES AB The crystallographic and physical properties of polycrystalline and single-crystal samples of BaCo2As2 and K-doped Ba1-xKxCo2As2 (x = 0.06,0.22) are investigated by x-ray and neutron powder diffraction, magnetic susceptibility chi, magnetization, heat capacity C-p, As-75 nuclear magnetic resonance (NMR), and electrical resistivity rho measurements versus temperature T. The crystals were grown using both Sn flux and CoAs self-flux, where the Sn-grown crystals contain 1.6-2.0 mol% Sn. All samples crystallize in the tetragonal ThCr2Si2-type structure (space group I4/mmm). For BaCo2As2, powder neutron diffraction data show that the c-axis lattice parameter exhibits anomalous negative thermal expansion from 10 K to 300 K, whereas the a axis lattice parameter and the unit cell volume show normal positive thermal expansion over this T range. No transitions in BaCo2As2 were found in this T range from any of the measurements. Below 40-50 K, we find rho alpha T-2, indicating a Fermi liquid ground state. A large density of states at the Fermi energy D(E-F) approximate to 18 states/(eV f.u.) for both spin directions is found from low-T C-p(T) measurements, whereas the band-structure calculations give D(EF) = 8.23 states/(eV f.u.). The enhancement of the former value above the latter is inferred to arise from electron-electron correlations and the electron-phonon interaction. The derived intrinsic chi(T) monotonically increases with decreasing T, with anisotropy chi(ab) > chi c. The As-75-NMR shift data versus T have the same T dependence as the derived chi(T) data, demonstrating that the derived chi(T) data are intrinsic. The observed As-75 nuclear spin dynamics rule out the presence of Neel-type antiferromagnetic electronic spin fluctuations, but are consistent with the presence of ferromagnetic and/or stripe-type antiferromagnetic spin fluctuations. The crystals of Ba0.78K0.22Co2As2 were grown in Sn flux and show properties very similar to those of undoped BaCo2As2. On the other hand, the crystals from two batches of Ba0.94K0.06Co2As2 grown in CoAs self-flux show evidence of weak ferromagnetism at T less than or similar to 10 K with small ordered moments at 1.8 K of approximate to 0.007 and 0.03 mu B per formula unit, respectively. C1 [Anand, V. K.; Quirinale, D. G.; Lee, Y.; Harmon, B. N.; Furukawa, Y.; McQueeney, R. J.; Kreyssig, A.; Goldman, A. I.; Johnston, D. C.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Anand, V. K.; Quirinale, D. G.; Lee, Y.; Harmon, B. N.; Furukawa, Y.; McQueeney, R. J.; Kreyssig, A.; Goldman, A. I.; Johnston, D. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Ogloblichev, V. V.] Russian Acad Sci, Ural Div, Inst Met Phys, Ekaterinburg 620990, Russia. [Huq, A.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37890 USA. [Abernathy, D. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Stephens, P. W.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Anand, VK (reprint author), Helmholtz Zentrum Berlin Mat & Energie, Hahn Meitner Pl 1, D-14109 Berlin, Germany. EM johnston@ameslab.gov RI Anand, Vivek Kumar/J-3381-2013; Ogloblichev, Vasily/K-3399-2013; Abernathy, Douglas/A-3038-2012; Huq, Ashfia/J-8772-2013; McQueeney, Robert/A-2864-2016 OI Anand, Vivek Kumar/0000-0003-2023-7040; Ogloblichev, Vasily/0000-0003-0520-7521; Abernathy, Douglas/0000-0002-3533-003X; Huq, Ashfia/0000-0002-8445-9649; McQueeney, Robert/0000-0003-0718-5602 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358]; Russian Foundation for Basic Research [12-02-31814]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX We thank Abhishek Pandey for experimental assistance and for many helpful discussions. The research at Ames Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. V.V.O. thanks the Ames Laboratory-USDOE for providing the opportunity to be a visiting scientist at the Laboratory and also thanks the Russian Foundation for Basic Research (Grant No. 12-02-31814) for support. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. Research at the Spallation Neutron Source at Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 75 TC 7 Z9 7 U1 10 U2 64 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 28 PY 2014 VL 90 IS 6 AR 064517 DI 10.1103/PhysRevB.90.064517 PG 21 WC Physics, Condensed Matter SC Physics GA AO3WL UT WOS:000341267600004 ER PT J AU Cai, L Toulouse, J Luo, HS Tian, W AF Cai, Ling Toulouse, Jean Luo, Haosu Tian, Wei TI Anisotropic phonon coupling in the relaxor ferroelectric (Na1/2Bi1/2)TiO3 near its high-temperature phase transition SO PHYSICAL REVIEW B LA English DT Article ID INELASTIC NEUTRON-SCATTERING; LATTICE-DYNAMICS; SINGLE-CRYSTAL; SOFT MODES; BATIO3; NA0.5BI0.5TIO3; DISPERSION; BEHAVIOR; NA1/2BI1/2TIO3; PEROVSKITES AB The lead free relaxor Na1/2Bi1/2TiO3 (NBT) undergoes a structural cubic-to-tetragonal transition near 800 K which is caused by the cooperative rotations of O-6 octahedra. These rotations are also accompanied by the displacements of the cations and the formation of the polar nanodomains (PNDs) that are responsible for the characteristic dielectric dispersion of relaxor ferroelectrics. Because of their intrinsic properties, spontaneous polarization, and lack of inversion symmetry, these PNDs are also piezoelectric and can mediate an interaction between polarization and strain or couple the optic and acoustic phonons. Because PNDs introduce a local tetragonal symmetry, the phonon coupling they mediate is found to be anisotropic. In this paper we present inelastic neutron scattering results on coupled transverse acoustic (TA) and transverse optic (TO) phonons in the [110] and [001] directions and across the cubic-tetragonal phase transition at T-C similar to 800 K. The phonon spectra are analyzed using a mode coupling model. In the [110] direction, as in other relaxors and some ferroelectric perovskites, a precipitous drop of the TO phonon into the TA branch or "waterfall" is observed at a certain q(wf) similar to 0.14 r.l.u. In the [001] direction, the highly overdamped line shape can be fitted with closely positioned bare mode energies which are largely overlapping along the dispersion curves. Two competing lattice coupling mechanism are proposed to explain these observations. C1 [Cai, Ling; Toulouse, Jean] Lehigh Univ, Dept Phys, Bethlehem, PA 18015 USA. [Luo, Haosu] Chinese Acad Sci, Shanghai Inst Ceram, Shanghai 201800, Peoples R China. [Tian, Wei] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Cai, L (reprint author), Lehigh Univ, Dept Phys, Bldg 16, Bethlehem, PA 18015 USA. RI Tian, Wei/C-8604-2013 OI Tian, Wei/0000-0001-7735-3187 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX We thank D. Viehland for suggesting this study of NBT and are grateful to P. Gehring, S. Vakhrushev, and B. Hennion for helpful discussions. The neutron scattering experiments conducted at ORNL's High Flux Isotope Reactor were sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 38 TC 1 Z9 1 U1 1 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 28 PY 2014 VL 90 IS 5 AR 054118 DI 10.1103/PhysRevB.90.054118 PG 9 WC Physics, Condensed Matter SC Physics GA AO3WB UT WOS:000341266400001 ER PT J AU Wang, YP Han, XF Fry, JN Krause, JL Zhang, XG Cheng, HP AF Wang, Yun-Peng Han, Xiu-Feng Fry, James N. Krause, Jeffrey L. Zhang, X. -G. Cheng, Hai-Ping TI Deposition of cobalt atoms onto Alq(3) films: A molecular dynamics study SO PHYSICAL REVIEW B LA English DT Article ID SELF-ASSEMBLED MONOLAYERS; AUGMENTED-WAVE METHOD; ALKANETHIOLATE MONOLAYERS; PENETRATION PATHWAYS; VAPOR-DEPOSITION; BOND INSERTION; FORCE-FIELD; SPIN-VALVE; ALUMINUM; SIMULATIONS AB The charge and spin injections into semiconductors are determined by the quality of the electrode/semiconductor interface. The latter is defined by the atomic penetration depth when growing metal electrodes on organic semiconductor thin films by the physical deposition method. Although the interfaces between top electrodes and a typical organic material, tris(8-hydroxyquinoline) aluminum (Alq(3)) thin films, have been intensively investigated by several groups, their results on the atomic penetration depth into Alq(3) film diverged from each other. In this paper we study the deposition of cobalt atoms onto Alq(3) thin films using the molecular dynamics method. The intermixing between Co and Alq(3) is calculated to be limited to the first Alq(3) layer for low Co initial kinetic energies, but spread to a few layers for high initial energies. The results of our calculation indicate that a proper deposition method with low injection energy helps to reduce the amount of intermixing at interfaces and improve the magnetoresistance of an organic-based magnetic junction. C1 [Wang, Yun-Peng; Han, Xiu-Feng] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Fry, James N.; Krause, Jeffrey L.; Cheng, Hai-Ping] Univ Florida, Quantum Theory Project, Gainesville, FL 32611 USA. [Fry, James N.; Krause, Jeffrey L.; Cheng, Hai-Ping] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Zhang, X. -G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Zhang, X. -G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Wang, YP (reprint author), Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. FU State Key Project of Fundamental Research of the Ministry of Science and Technology [2010CB934401]; National Natural Science Foundation of China [11374351, 51229101]; US DOE/BES [DE-FG02-02ER45995]; K. C. Wong Education Foundation, Hong Kong; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The project was supported by the State Key Project of Fundamental Research of the Ministry of Science and Technology (Grant No. 2010CB934401), the National Natural Science Foundation of China (Grants No. 11374351 and No. 51229101), the US DOE/BES Grant No. DE-FG02-02ER45995 (H.-P.C., J.N.F., and J.L.K.), and the partial support from the K. C. Wong Education Foundation, Hong Kong. The calculations were performed on NERSC computers. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 41 TC 0 Z9 0 U1 1 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 28 PY 2014 VL 90 IS 7 AR 075311 DI 10.1103/PhysRevB.90.075311 PG 7 WC Physics, Condensed Matter SC Physics GA AO3WW UT WOS:000341268900006 ER PT J AU del Campo, A Goold, J Paternostro, M AF del Campo, A. Goold, J. Paternostro, M. TI More bang for your buck: Super-adiabatic quantum engines SO SCIENTIFIC REPORTS LA English DT Article ID FREE-ENERGY DIFFERENCES; HEAT ENGINES; FINITE-TIME; EFFICIENCY; SHORTCUTS; ENTROPY; POWER AB The practical untenability of the quasi-static assumption makes any realistic engine intrinsically irreversible and its operating time finite, thus implying friction effects at short cycle times. An important technological goal is thus the design of maximally efficient engines working at the maximum possible power. We show that, by utilising shortcuts to adiabaticity in a quantum engine cycle, one can engineer a thermodynamic cycle working at finite power and zero friction. Our findings are illustrated using a harmonic oscillator undergoing a quantum Otto cycle. C1 [del Campo, A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [del Campo, A.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Goold, J.] Abdus Salam Int Ctr Theoret Phys, I-34014 Trieste, Italy. [Paternostro, M.] Queens Univ, Ctr Theoret Atom Mol & Opt Phys, Sch Math & Phys, Belfast BT7 1NN, Antrim, North Ireland. RP Paternostro, M (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM m.paternostro@qub.ac.uk RI del Campo, Adolfo/B-8439-2009; Goold, John/M-4181-2014; OI del Campo, Adolfo/0000-0003-2219-2851; Goold, John/0000-0001-6264-2728; Goold, John/0000-0001-6702-1736; Paternostro, Mauro/0000-0001-8870-9134 FU U.S. Department of Energy through the LANL/LDRD Program; LANL J. Robert Oppenheimer fellowship; IRCSET through a Marie Curie International Mobility fellowship; UK EPSRC for a Career Acceleration Fellowship under "New Directions for EPSRC Research Leaders'' initiative [EP/G004579/1]; John Templeton Foundation [43467]; EU Collaborative project TherMiQ [618074]; COST Action [MP1209] FX We are grateful to G. De Chiara, B. Damski, S. Deffner, R. Dorner, R. Fazio, C. Jarzynski, E. Passemar and N. Sinitsyn for discussions and comments on this work. AdC is supported by the U.S. Department of Energy through the LANL/LDRD Program and a LANL J. Robert Oppenheimer fellowship. JG acknowledges funding from IRCSET through a Marie Curie International Mobility fellowship. MP thanks the UK EPSRC for a Career Acceleration Fellowship and a grant under the "New Directions for EPSRC Research Leaders'' initiative (EP/G004579/1) the John Templeton Foundation (grant 43467), the EU Collaborative project TherMiQ (Grant Agreement 618074), and the COST Action MP1209. NR 37 TC 43 Z9 43 U1 2 U2 19 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 28 PY 2014 VL 4 AR 6208 DI 10.1038/srep06208 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN9OF UT WOS:000340935700001 PM 25163421 ER PT J AU Wang, P Hudak, MR Lerner, A Grubbs, RK Wang, SM Zhang, Z Karapetrova, E Hickmott, D Majewski, J AF Wang, Peng Hudak, Michael R. Lerner, Allan Grubbs, Robert K. Wang, Shanmin Zhang, Zhan Karapetrova, Evguenia Hickmott, Donald Majewski, Jaroslaw TI X-ray scattering of calcite thin films deposited by atomic layer deposition: Studies in air and in calcite saturated water solution SO THIN SOLID FILMS LA English DT Article DE Calcite; Atomic layer deposition (ALD); Thin films; X-ray scattering; Diffraction; Reflectivity ID MOLECULAR-DYNAMICS SIMULATIONS; IN-SITU; CRYSTALLIZATION ENERGETICS; (104)-WATER INTERFACE; CRYSTAL TRUNCATION; SURFACE SPECIATION; CARBONATE MINERALS; HIGH-PRESSURES; REFLECTIVITY; GROWTH AB Carbonates are one of the most abundant groups of minerals in earth systems and are important in many geological settings and industrial processes. Calcite (CaCO3) thin films produced by atomic layer deposition offer a method to evaluate the surficial properties of carbonates as well as interactions at the carbonate-fluid interface. Using synchrotron X-ray reflectivity and X-ray diffraction, these films are observed to be porous, polycrystalline, and have crystallites oriented with the major (104) calcite cleavage plane parallel to the surface of the z-cut single crystal quartz substrate. An Al2O3 buffer layer, present between quartz and the calcite film, does not affect the as-deposited film, but does influence how the films reorganize in contact with fluid. Without a buffer layer, calcite reorients its crystallites to have populations of (006) and (030) parallel to the substrate, while those with an Al2O3 buffer layer become more amorphous. Amorphous films may represent an analog to amorphous calcium carbonate and provide insights into that material's thermophysical behavior. Due to a higher percentage of pore spaces available for fluid infiltration, films deposited at higher temperature make the calcite thin films more susceptible to amorphization. These films are chemically similar, but structurally dissimilar to bulk natural calcite. Nevertheless, they can be a complementary system to traditional single crystal X-ray surface scattering studies on carbonates, particularly for important but less common minerals, to evaluate mineral-fluid interfacial interactions. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wang, Peng; Wang, Shanmin; Majewski, Jaroslaw] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Hudak, Michael R.; Lerner, Allan; Hickmott, Donald] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Grubbs, Robert K.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Zhang, Zhan; Karapetrova, Evguenia] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Majewski, J (reprint author), Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, POB 1663, Los Alamos, NM 87545 USA. EM jarek@lanl.gov RI Zhang, Zhan/A-9830-2008 OI Zhang, Zhan/0000-0002-7618-6134 FU DOE Office of Basic Energy Sciences; Los Alamos National Laboratory (LANL) under DOE [DE-AC52-06NA25396]; LANL's Laboratory Directed Research and Development Program; U.S. Department of Energy [DEAC02-06CH11357] FX The Manuel Lujan Jr. Neutron Scattering Center at LANSCE is funded by the DOE Office of Basic Energy Sciences and Los Alamos National Laboratory (LANL) under DOE Contract DE-AC52-06NA25396. The funding for this research is provided by LANL's Laboratory Directed Research and Development Program. Work at the Advanced Photon Source is supported by the U.S. Department of Energy under grant No. DEAC02-06CH11357. NR 56 TC 0 Z9 0 U1 1 U2 19 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD AUG 28 PY 2014 VL 565 BP 277 EP 284 DI 10.1016/j.tsf.2014.06.032 PG 8 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA AO1EJ UT WOS:000341054600042 ER PT J AU Pan, X Zhu, K Ren, GF Islam, N Warzywoda, J Fan, ZY AF Pan, Xuan Zhu, Kai Ren, Guofeng Islam, Nazifah Warzywoda, Juliusz Fan, Zhaoyang TI Electrocatalytic properties of a vertically oriented graphene film and its application as a catalytic counter electrode for dye-sensitized solar cells SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID CHARGE-COLLECTION EFFICIENCIES; DOPED GRAPHENE; PERFORMANCE; ARRAYS; OXIDE; FOAM AB Vertically oriented graphene (VOG), with graphene sheets perpendicular to the substrate, exhibits meritorious electrocatalytic properties due to the fully exposed graphene (or graphitic) edges and other plasma introduced defects, even without any heteroatom functionalization. We report the growth and electrocatalytic properties of VOG by plasma-enhanced chemical vapor deposition using methane and nitrogen as source gases. Nitrogen was adopted as plasma ancillary gas to obtain a higher plasma temperature that promotes VOG growth with better electrocatalytic performance, as comparative studies demonstrated. Electron transfer dynamics measurement using a Fe(CN)(6)(3-/4-) redox couple found reduction and oxidation peak-to-peak separation as low as 70 mV, indicating rapid electron-transfer kinetics. The electrocatalytic activity of the VOG electrode on an I-/I-3(-) redox couple was found approaching that of platinum. Using VOG as the counter electrode for dye-sensitized solar cells (DSSCs), a promising power conversion efficiency of 7.63% was demonstrated. Electrochemical impedance spectroscopic study further discloses the impact of VOG properties on DSSC performance. C1 [Pan, Xuan; Ren, Guofeng; Islam, Nazifah; Fan, Zhaoyang] Texas Tech Univ, Dept Elect & Comp Engn, Lubbock, TX 79409 USA. [Pan, Xuan; Ren, Guofeng; Islam, Nazifah; Fan, Zhaoyang] Texas Tech Univ, Nano Tech Ctr, Lubbock, TX 79409 USA. [Zhu, Kai] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. [Warzywoda, Juliusz] Texas Tech Univ, Whitacre Coll Engn, Ctr Mat Characterizat, Lubbock, TX 79409 USA. RP Fan, ZY (reprint author), Texas Tech Univ, Dept Elect & Comp Engn, Lubbock, TX 79409 USA. EM kai.zhu@nrel.gov; zhaoyang.fan@ttu.edu RI Pan, Xuan/K-8545-2014; Ren, Guofeng/P-8362-2015 OI Pan, Xuan/0000-0002-7770-7974; FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX K.Z. acknowledges the support by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy, under contract no. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 33 TC 13 Z9 13 U1 2 U2 47 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 EI 2050-7496 J9 J MATER CHEM A JI J. Mater. Chem. A PD AUG 28 PY 2014 VL 2 IS 32 BP 12746 EP 12753 DI 10.1039/c4ta02028f PG 8 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA AN1MJ UT WOS:000340347700016 ER PT J AU Huang, YQ Fang, J Omenya, F O'Shea, M Chernova, NA Zhang, RB Wang, Q Quackenbush, NF Piper, LFJ Scanlon, DO Whittingham, MS AF Huang, Yiqing Fang, Jin Omenya, Fredrick O'Shea, Martin Chernova, Natasha A. Zhang, Ruibo Wang, Qi Quackenbush, Nicholas F. Piper, Louis F. J. Scanlon, David O. Whittingham, M. Stanley TI Understanding the stability of MnPO4 SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID DENSITY-FUNCTIONAL THEORY; LI-ION BATTERIES; LITHIUM BATTERIES; ELECTRODE MATERIALS; CATHODE MATERIALS; THERMAL-STABILITY; AB-INITIO; LIMNPO4; MN; FE AB We have revealed the critical role of carbon coating in the stability and thermal behaviour of olivine MnPO4 obtained by chemical delithiation of LiMnPO4. (Li)MnPO4 samples with various particle sizes and carbon contents were studied.. Carbon-free LiMnPO4 obtained by solid state synthesis in O-2 becomes amorphous upon delithiation. Small amounts of carbon (0.3 wt%) help to stabilize the olivine structure, so that completely delithiated crystalline olivine MnPO4 can be obtained. Larger amount of carbon (2 wt%) prevents full delithiation. Heating in air, O-2, or N-2 results in structural disorder (<300 degrees C), formation of an intermediate sarcopside Mn-3(PO4)(2) phase (350-450 degrees C), and complete decomposition to Mn2P2O7 on extended heating at 400 degrees C. Carbon coating protects MnPO4 from reacting with environmental water, which is detrimental to its structural stability. C1 [Huang, Yiqing; Fang, Jin; Omenya, Fredrick; Chernova, Natasha A.; Zhang, Ruibo; Wang, Qi; Whittingham, M. Stanley] SUNY Binghamton, Binghamton, NY 13902 USA. [O'Shea, Martin] SUNY Coll Geneseo, Geneseo, NY 14454 USA. [Wang, Qi] Brookhaven Natl Lab, Upton, NY 11973 USA. [Quackenbush, Nicholas F.; Piper, Louis F. J.] SUNY Binghamton, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. [Scanlon, David O.] Univ London Univ Coll, Dept Chem, Kathleen Lonsdale Mat Chem, London WC1H 0AJ, England. [Scanlon, David O.] Diamond Light Source Ltd, Didcot OX11 0DE, Oxon, England. [Whittingham, M. Stanley] SUNY Stony Brook, Northeastern Ctr Chem Energy Storage, Dept Chem, Stony Brook, NY 11794 USA. RP Whittingham, MS (reprint author), SUNY Binghamton, Binghamton, NY 13902 USA. EM stanwhit@gmail.com RI Scanlon, David/B-1516-2008; Zhang, Ruibo/B-4659-2015; Piper, Louis/C-2960-2011 OI Scanlon, David/0000-0001-9174-8601; Piper, Louis/0000-0002-3421-3210 FU Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC001294]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-AC02-06CH11357]; EPSRC [EP/K000144/1, EP/K000136/1]; ARCHER supercomputer through membership of the UK's HPC Materials Chemistry Consortium - EPSRC [EP/L000202]; NYSERDA [17433, 18500] FX This work was supported by the Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DESC001294. Use of the National Synchrotron Light Source at Brookhaven National Laboratory and Advanced Light Source at Argonne National Laboratory is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contracts DE-AC02-98CH10886 and DE-AC02-06CH11357, respectively. We thank Kevin Smith and David Newby Jr for use of the Boston University endstation at Beamline X1B for supplementary measurements. Acknowledgment is made to the Donors of the American Chemical Society Petroleum Research Fund for the support of the XPS studies. The DFT work presented here made use of the UCL Legion HPC Facility, the IRIDIS cluster provided by the EPSRC funded Centre for Innovation (EP/K000144/1 and EP/K000136/1), and the ARCHER supercomputer through membership of the UK's HPC Materials Chemistry Consortium, which is funded by EPSRC grant (EP/L000202). Support by NYSERDA (Q. W.) under Agreements no. 17433 and 18500 is also acknowledged. NR 35 TC 10 Z9 10 U1 6 U2 91 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 EI 2050-7496 J9 J MATER CHEM A JI J. Mater. Chem. A PD AUG 28 PY 2014 VL 2 IS 32 BP 12827 EP 12834 DI 10.1039/c4ta00434e PG 8 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA AN1MJ UT WOS:000340347700027 ER PT J AU Ghidiu, M Naguib, M Shi, C Mashtalir, O Pan, LM Zhang, B Yang, J Gogotsi, Y Billinge, SJL Barsoum, MW AF Ghidiu, M. Naguib, M. Shi, C. Mashtalir, O. Pan, L. M. Zhang, B. Yang, J. Gogotsi, Y. Billinge, S. J. L. Barsoum, M. W. TI Synthesis and characterization of two-dimensional Nb4C3 (MXene) SO CHEMICAL COMMUNICATIONS LA English DT Article ID TITANIUM CARBIDE; ION BATTERIES; EXFOLIATION; INTERCALATION; FAMILY; ANODE AB We report on the synthesis of a phase-pure, 2-dimensional transition metal carbide Nb4C3, produced by immersing Nb4AlC3 powders in hydrofluoric acid. The structure of this, only second MXene with formula M4X3, was investigated with pair distribution function analysis. The resistivity of a cold-pressed disc was 0.0046 Omega m, rendering this MXene one of the most conductive to date. C1 [Ghidiu, M.; Naguib, M.; Mashtalir, O.; Yang, J.; Gogotsi, Y.; Barsoum, M. W.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Ghidiu, M.; Naguib, M.; Mashtalir, O.; Yang, J.; Gogotsi, Y.; Barsoum, M. W.] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. [Shi, C.; Billinge, S. J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Pan, L. M.; Zhang, B.; Yang, J.] Nanjing Tech Univ, Coll Mat Sci & Engn, Nanjing 210009, Peoples R China. [Billinge, S. J. L.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Yang, J (reprint author), Nanjing Tech Univ, Coll Mat Sci & Engn, Nanjing 210009, Peoples R China. EM jianyang.nj@gmail.com; barsoumw@drexel.edu RI Naguib, Michael/A-7315-2012; shi, chenyang/A-9119-2014 OI Naguib, Michael/0000-0002-4952-9023; FU National Science Foundation grant NSF [DMR-1310245]; Jiangsu Government Scholarship for Overseas Studies; Priority Academic Program Development of Jiangsu Higher Education Institutions (PAID); Program for Changjiang Scholars and Innovative Research Team in University (PCSIRT) [IRT1146]; Columbia University Energy Frontier Research Center (EFRC) - U.S. Department of Energy, Basic Energy Sciences (DOE-BES) [DE-SC0001085]; U.S. Department of Energy, Basic Energy Sciences (DOE-BES) [DE-AC02-98CH10886] FX Work at Drexel University was supported by National Science Foundation grant NSF (DMR-1310245) and Jiangsu Government Scholarship for Overseas Studies, the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAID) and the Program for Changjiang Scholars and Innovative Research Team in University (PCSIRT), IRT1146. Work in the Billinge group was supported by the Columbia University Energy Frontier Research Center (EFRC) funded by the U.S. Department of Energy, Basic Energy Sciences (DOE-BES), under Grant No. DE-SC0001085. NSLS is supported by the U.S. Department of Energy, Basic Energy Sciences (DOE-BES) under grant DE-AC02-98CH10886. We thank Majid Beidaghi for his help in preparing samples for the pair distribution function analysis and Mengqiang Zhao for his help in indexing the SAED patterns. NR 23 TC 55 Z9 58 U1 33 U2 300 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 EI 1364-548X J9 CHEM COMMUN JI Chem. Commun. PD AUG 28 PY 2014 VL 50 IS 67 BP 9517 EP 9520 DI 10.1039/c4cc03366c PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AM9QT UT WOS:000340216800021 PM 25010704 ER PT J AU Feng, XF Song, MK Stolte, WC Gardenghi, D Zhang, D Sun, XH Zhu, JF Cairns, EJ Guo, JH AF Feng, Xuefei Song, Min-Kyu Stolte, Wayne C. Gardenghi, David Zhang, Duo Sun, Xuhui Zhu, Junfa Cairns, Elton J. Guo, Jinghua TI Understanding the degradation mechanism of rechargeable lithium/sulfur cells: a comprehensive study of the sulfur-graphene oxide cathode after discharge-charge cycling SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID LI-S BATTERIES; SOLID-ELECTROLYTE INTERPHASE; RAY-ABSORPTION-SPECTROSCOPY; HIGH SPECIFIC ENERGY; ELECTROCHEMICAL PROPERTIES; GRAPHITE ANODE; PERFORMANCE; ION; SEI; COMPOSITES AB Lithium/sulfur (Li/S) cells have attracted much attention due to their higher theoretical specific capacity and energy compared to those of current lithium-ion cells. However, the application of Li/S cells is still hampered by short cycle life. Sulfur graphene oxide (S-GO) nanocomposites have shown promise as cathode materials for long-life Li/S cells because oxygen-containing functional groups on the surface of graphene oxide were successfully used as sulfur immobilizers by forming weak bonds with sulfur and polysulfides. While S-GO showed much improved cycling performance, the capacity decay still needs to be improved for commercially viable cells. In this study, we attempt to understand the capacity fading mechanism based on an ex situ study of the structural and chemical evolution of S-GO nanocomposite cathodes with various numbers of cycles using scanning electron microscopy (SEM), near edge X-ray absorption fine structure (NEXAFS) and X-ray photoelectron spectroscopy (XPS). It is found that both the surface morphologies and chemical structures of the cathode materials change considerably with increasing number of cycles. These changes are attributed to several unexpected chemical reactions of lithium with S GO nanocomposites occurring during the discharge charge processes with the formation of Li2CO3, Li2SO3, Li2SO4, and COSO2Li species. These reactions result in the loss of recyclable active sulfur on the surface of the electrode, and thus capacity fades while coulombic efficiency is near 100%. Moreover, the reaction products accumulate on the cathode surface, forming a compact blocking insulating layer which may make the diffusion of Li ions into/out of the cathode difficult during the discharge charge process and thus lead to lower utilization of sulfur at higher rates. We think that these two observations are significant contributors to the capacity and rate capability degradation of the Li/S-GO cells. Therefore, for the rechargeable Li/S-GO cells, we suggest that the content of oxygen-containing functional groups on GO should be optimized and more stable functional groups need to be identified for further improvement of the cycling performance. The information we gain from this study may provide general insights into the fundamental understanding of the degradation mechanisms of other rechargeable Li/S cells using similar oxygencontaining functional groups as sulfur immobilizers. C1 [Feng, Xuefei; Zhu, Junfa] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China. [Feng, Xuefei; Zhu, Junfa] Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230029, Peoples R China. [Feng, Xuefei; Stolte, Wayne C.; Gardenghi, David; Zhang, Duo; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Song, Min-Kyu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Song, Min-Kyu; Cairns, Elton J.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Stolte, Wayne C.; Gardenghi, David] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Zhang, Duo; Sun, Xuhui] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China. [Cairns, Elton J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Guo, Jinghua] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. RP Zhu, JF (reprint author), Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China. EM jfzhu@ustc.edu.cn; jguo@lbl.gov RI Foundry, Molecular/G-9968-2014; Zhu, Junfa/E-4020-2010; Cairns, Elton/E-8873-2012 OI Zhu, Junfa/0000-0003-0888-4261; Cairns, Elton/0000-0002-1179-7591 FU National Basic Research Program of China [2010CB9233022013CB834605]; National Natural Science Foundation of China [U1232102]; Specialized Research Fund for the Doctoral Program of Higher Education of Ministiy of Education [20113402110029]; University of California, Office of the President, under the Proof of Concept [12PC247581]; Office of Science, the Office of Basic Energy Sciences; U.S. Department of Energy [DE-AC02-05CH11231] FX J.F.Z. acknowledges the financial support from the National Basic Research Program of China (2010CB923302, 2013CB834605), the National Natural Science Foundation of China (Grant No. U1232102), and the Specialized Research Fund for the Doctoral Program of Higher Education of Ministiy of Education (Grant No. 20113402110029). E.J.C. acknowledges financial support from the University of California, Office of the President, under the Proof of Concept Grant No. 12PC247581. The work at the Advanced Light Source is supported by the Office of Science, the Office of Basic Energy Sciences and the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 56 TC 31 Z9 31 U1 10 U2 166 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD AUG 28 PY 2014 VL 16 IS 32 BP 16931 EP 16940 DI 10.1039/c4cp01341g PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN1OK UT WOS:000340353000008 PM 24781200 ER PT J AU Yao, SY Xu, WQ Johnston-Peck, AC Zhao, FZ Liu, ZY Luo, S Senanayake, SD Martinez-Arias, A Liu, WJ Rodriguez, JA AF Yao, S. Y. Xu, W. Q. Johnston-Peck, A. C. Zhao, F. Z. Liu, Z. Y. Luo, S. Senanayake, S. D. Martinez-Arias, A. Liu, W. J. Rodriguez, J. A. TI Morphological effects of the nanostructured ceria support on the activity and stability of CuO/CeO2 catalysts for the water-gas shift reaction SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; EXPOSED FACE PRESENT; IN-SITU; NO REDUCTION; EXCESS H-2; PREFERENTIAL OXIDATION; HYDROGEN-PRODUCTION; NANOSCALE CERIA; CEO2 SUPPORT; CO OXIDATION AB Three CuO/CeO2 catalyst with different morphologies of ceria, namely nanospheres, nanorods and nanocubes, were synthesized and used to catalyze the water-gas shift (WGS) reaction. The reactivity tests showed that the Cu supported on the ceria nanospheres exhibited both the highest activity and superior stability when compared with the nanocube and nanorod ceria catalysts. Operando X-ray diffraction (XRD). X-ray absorption fine structure (XAFS) and diffuse reflectance Fourier transform infrared spectroscopy (DRIFTS) methods were used to characterize these catalysts in their working state. High resolution electron microscopy (HRTEM, STEM) was used to look at the local atomic structure and nano-scale morphology. Our results show that the morphology of the ceria support, which can involve different crystal faces and concentrations of defects and imperfections, has a critical impact on the catalytic properties and influences: (1) the dispersion of CuO in the as-synthesized catalyst; (2) the particle size of metallic Cu upon reduction during the WGS reaction, (3) the stability of the metallic Cu upon variations of temperature, and (4) the dissociation of water on the ceria support. The nanosphere ceria catalyst showed an excellent water dissociation capability, the best dispersion of Cu and a strong Cu-Ce interaction, therefore delivering the best performance among the three WGS catalysts. The metallic Cu, which is the active species during the WGS reaction, was more stabilized on the nanospheres than on the nanorods and nanocubes and thus led to a better stability of the nanosphere catalyst than the other two architectures. Each catalyst exhibited a distinctive line-shape in the 800-1600 cm(-1) region of the DRIFTS spectra, pointing to the existence of different types of carbonate or carboxylate species as surface intermediates for the WGS. C1 [Yao, S. Y.; Liu, W. J.] Peking Univ, Ctr Computat Sci & Engn, Beijing 100871, Peoples R China. [Yao, S. Y.; Liu, W. J.] Peking Univ, Green Chem Ctr, Beijing 100871, Peoples R China. [Yao, S. Y.; Xu, W. Q.; Zhao, F. Z.; Liu, Z. Y.; Luo, S.; Senanayake, S. D.; Rodriguez, J. A.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Johnston-Peck, A. C.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Liu, Z. Y.; Luo, S.; Rodriguez, J. A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11749 USA. [Martinez-Arias, A.] CSIC, Inst Catalisis & Petr Quim, E-28049 Madrid, Spain. RP Liu, WJ (reprint author), Peking Univ, Ctr Computat Sci & Engn, Beijing 100871, Peoples R China. EM liuwj@pku.edu.cn; rodrigez@bnl.gov RI Senanayake, Sanjaya/D-4769-2009; COST, CM1104/I-8057-2015; Liu, Wenjian/N-7575-2016 OI Senanayake, Sanjaya/0000-0003-3991-4232; Liu, Wenjian/0000-0002-1630-3466 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-98CH10886]; China Scholarship Council [201206010107]; MINECO [CTQ2012-32928]; EU COST [CM1104] FX The research carried out at the Chemistry Department, the National Synchrotron Light Source (NSLS) and the Center for Functional Nanomaterials (CFN), at Brookhaven National Laboratory (BNL) was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy (DE-AC02-98CH10886) contract. The financial support from China Scholarship Council (File No. 201206010107) is gratefully acknowledged. Financial support from MINECO (Plan National project CTQ2012-32928) and EU COST CM1104 action is also acknowledged. Thanks are also due to ICP-CSIC Unidad de Apoyo for SBET measurements. NR 59 TC 28 Z9 29 U1 18 U2 184 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD AUG 28 PY 2014 VL 16 IS 32 BP 17183 EP 17195 DI 10.1039/c4cp02276a PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN1OK UT WOS:000340353000034 PM 25012908 ER PT J AU Kim, S Chang, KJ Park, JS AF Kim, Sunghyun Chang, K. J. Park, Ji-Sang TI Finite-size supercell correction scheme for charged defects in one-dimensional systems SO PHYSICAL REVIEW B LA English DT Article ID AUGMENTED-WAVE METHOD; SILICON NANOWIRES; STABILITY AB We propose a finite-size correction scheme for the formation energy of charged defects and impurities in one-dimensional systems within density functional theory. The energy correction in a supercell geometry is obtained by solving the Poisson equation in a continuum model which is described by an anisotropic permittivity tensor, with the defect charge distribution derived from first-principles calculations. We implement our scheme to study impurities and dangling bonds in silicon nanowires and demonstrate that the formation energy of charged defects rapidly converges with the supercell size. C1 [Kim, Sunghyun; Chang, K. J.] Korea Adv Inst Sci & Technol, Dept Phys, Taejon 305701, South Korea. [Park, Ji-Sang] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Kim, S (reprint author), Korea Adv Inst Sci & Technol, Dept Phys, Taejon 305701, South Korea. EM kjchang@kaist.ac.kr RI Chang, Kee Joo/C-1989-2011; Park, Ji-Sang/F-9944-2010; OI Park, Ji-Sang/0000-0002-1374-8793; Kim, Sunghyun/0000-0001-5072-6801 FU National Research Foundation of Korea [NRF-2005-0093845]; Supercomputing Center/Korea Institute of Science and Technology Information [KSC-2013-C1-035] FX This work was supported by the National Research Foundation of Korea under Grant No. NRF-2005-0093845 and by the Supercomputing Center/Korea Institute of Science and Technology Information with supercomputing resources including technical support (KSC-2013-C1-035). NR 30 TC 1 Z9 1 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 27 PY 2014 VL 90 IS 8 AR 085435 DI 10.1103/PhysRevB.90.085435 PG 7 WC Physics, Condensed Matter SC Physics GA AU5GS UT WOS:000345635700006 ER PT J AU Xi, XX He, XG Guan, F Liu, ZX Zhong, RD Schneeloch, JA Liu, TS Gu, GD Du, X Chen, Z Hong, XG Ku, W Carr, GL AF Xi, Xiaoxiang He, Xu-Gang Guan, Fen Liu, Zhenxian Zhong, R. D. Schneeloch, J. A. Liu, T. S. Gu, G. D. Du, X. Chen, Z. Hong, X. G. Ku, Wei Carr, G. L. TI Bulk Signatures of Pressure-Induced Band Inversion and Topological Phase Transitions in Pb1-xSnxSe SO PHYSICAL REVIEW LETTERS LA English DT Article ID CRYSTALLINE INSULATOR; LASER-EMISSION; ALLOYS; TERNARY; SNTE AB The characteristics of topological insulators are manifested in both their surface and bulk properties, but the latter remain to be explored. Here we report bulk signatures of pressure-induced band inversion and topological phase transitions in Pb1-xSnxSe (x = 0.00, 0.15, and 0.23). The results of infrared measurements as a function of pressure indicate the closing and the reopening of the band gap as well as a maximum in the free carrier spectral weight. The enhanced density of states near the band gap in the topological phase gives rise to a steep interband absorption edge. The change of density of states also yields a maximum in the pressure dependence of the Fermi level. Thus, our conclusive results provide a consistent picture of pressure-induced topological phase transitions and highlight the bulk origin of the novel properties in topological insulators. C1 [Xi, Xiaoxiang; Carr, G. L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [He, Xu-Gang; Zhong, R. D.; Schneeloch, J. A.; Liu, T. S.; Gu, G. D.; Ku, Wei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [He, Xu-Gang; Guan, Fen; Du, X.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Liu, Zhenxian] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Liu, T. S.] North Univ China, Sch Chem Engn & Environm, Taiyuan 030051, Peoples R China. [Chen, Z.; Hong, X. G.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. RP Xi, XX (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. RI Zhong, Ruidan/D-5296-2013; OI Zhong, Ruidan/0000-0003-1652-9454; Schneeloch, John/0000-0002-3577-9574 FU U.S. Department of Energy [DE-AC02-98CH10886]; NSF (COMPRES) [DMR-0805056, EAR 06-49658]; DOE/NNSA (CDAC) [DE-FC03-03N00144] FX We are grateful for helpful discussions with C. C. Homes. This work was supported by the U.S. Department of Energy through Contract No. DE-AC02-98CH10886 at BNL. The use of U2A and X17C beamlines was supported by NSF (DMR-0805056; EAR 06-49658, COMPRES) and DOE/NNSA (DE-FC03-03N00144, CDAC). NR 36 TC 14 Z9 14 U1 5 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 27 PY 2014 VL 113 IS 9 AR 096401 DI 10.1103/PhysRevLett.113.096401 PG 5 WC Physics, Multidisciplinary SC Physics GA AS8BB UT WOS:000344474300002 PM 25215996 ER PT J AU Pressel, KG Collins, WD Desai, AR AF Pressel, Kyle G. Collins, William D. Desai, Ankur R. TI The spatial scale dependence of water vapor variability inferred from observations from a very tall tower SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID DETRENDED FLUCTUATION ANALYSIS; WAVE-NUMBER SPECTRA; PACIFIC EXPLORATORY MISSIONS; LIQUID WATER; COMMERCIAL AIRCRAFT; TAYLOR HYPOTHESIS; CARBON-DIOXIDE; TRACE GASES; TIME-SERIES; TEMPERATURE AB Recent studies have established that atmospheric water vapor fields exhibit spatial spectra that take the form of power laws and hence can be compactly characterized by scaling exponents. The power law scaling exponents have been shown to exhibit substantial vertical variability. In this work, Taylor's frozen turbulence hypothesis is used to infer the first-order spatial structure function and generalized detrended fluctuation function scaling exponents for scales between 1 km and 100 km. Both methods are used to estimate the Hurst exponent (H) using 10 Hz time series of water vapor measured at 396 m altitude from an Ameriflux tower in Wisconsin. Due to the diurnal cycle in the boundary layer height at the 396 m observational level, H may be estimated for both the daytime convective mixed layer and the nocturnal residual layer. Values of H approximate to 1/3 are obtained for the convective mixed layer, while values of H > 1/2 apply in the nocturnal residual layer. The results are shown to be remarkably consistent with a similar analysis from satellite-based observations as reported in Pressel and Collins (2012). C1 [Pressel, Kyle G.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Pressel, Kyle G.; Collins, William D.] Lawrence Orlando Berkeley Natl Lab, Climate Sci Dept, Berkeley, CA USA. [Pressel, Kyle G.; Collins, William D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Desai, Ankur R.] Univ Wisconsin, Dept Atmospher & Ocean Sci, Madison, WI USA. RP Pressel, KG (reprint author), CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. EM pressel@caltech.edu RI Collins, William/J-3147-2014; Desai, Ankur/A-5899-2008 OI Collins, William/0000-0002-4463-9848; Desai, Ankur/0000-0002-5226-6041 FU Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC02-05CH11231]; Terrestrial Hazard Observation and Reporting (THOR) Center at Caltech; National Science Foundation [ARC-1107795] FX This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy under contract DE-AC02-05CH11231 as part of their Regional and Global Climate Modeling Program. Observations at the WLEF Park Falls Ameriflux site are supported by National Science Foundation (NSF) DEB-0845166, the Department of Energy Lawrence Berkeley National Lab Ameriflux Network Management Project, and NOAA Earth Systems Research Lab. These observations were made with the assistance of Jonathan Thom, University of Wisconsin-Madison; Arlyn Andrews, NOAA ESRL; Jonathan Kofler, NOAA ESRL; and Dan Buamann, U.S. Geological Survey. We are grateful for support by the Terrestrial Hazard Observation and Reporting (THOR) Center at Caltech and by the National Science Foundation (grant ARC-1107795). The flux and meteorological data from the WLEF tower are free, fair use, and available online at http://flux.aos.wisc.edu/twiki/bin/view/Main/ChEASData and also archived at the Fluxnet/Ameriflux repository. The high-frequency WLEF tower observations used in this study are available online at http://flux.aos.wisc.edu/data/wlef/2013JD021141. NR 46 TC 0 Z9 0 U1 1 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 27 PY 2014 VL 119 IS 16 BP 9822 EP 9837 DI 10.1002/2013JD021141 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AP3RF UT WOS:000341994000015 ER PT J AU Kulkarni, G Sanders, C Zhang, K Liu, XH Zhao, C AF Kulkarni, Gourihar Sanders, Cassandra Zhang, Kai Liu, Xiaohong Zhao, Chun TI Ice nucleation of bare and sulfuric acid-coated mineral dust particles and implication for cloud properties SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID ATMOSPHERE MODEL CAM5; AQUEOUS-SOLUTIONS; HETEROGENEOUS NUCLEATION; DEPOSITION NUCLEATION; SURFACE MODIFICATION; WATER ACTIVITY; ACTIVE-SITES; SULFATE; IMMERSION; AEROSOLS AB Ice nucleation properties of atmospherically relevant dust minerals coated with soluble materials are not yet well understood. We determined ice nucleation ability of bare and sulfuric acid-coated mineral dust particles as a function of temperature (-25 to -35 degrees C) and relative humidity with respect to water (RHw; 75 to 110%) for five different mineral dust types: (1) Arizona test dust, (2) illite, (3) montmorillonite, (4) K-feldspar, and (5) quartz. The particles were dry dispersed and size selected at 200 nm, and we determined the fraction of dust particles nucleating ice at various temperatures and RHw. Under water-subsaturated conditions, compared to bare dust particles, we found that coated particles showed a reduction in their ice nucleation ability. Under water-supersaturated conditions, however, we did not observe a significant coating effect (i.e., the bare and coated dust particles had nearly similar nucleating properties). X-ray diffraction patterns of the coated particles indicated that acid treatment altered the crystalline nature of the surface and caused structural disorder; thus, we concluded that the lack of such structured order reduced the ice nucleation efficiency of the coated particles in deposition ice nucleation mode. In addition, our single column model results show that coated particles significantly modify cloud properties such as ice crystal number concentration and ice water content compared to bare particles in water-subsaturated conditions. However, in water-supersaturated conditions, cloud properties differ only at warmer temperatures. These modeling results imply that future aged dust particle simulations should implement coating parameterizations to accurately predict cloud properties. C1 [Kulkarni, Gourihar; Zhang, Kai; Zhao, Chun] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Sanders, Cassandra] Washington State Univ, Richland, WA USA. [Liu, Xiaohong] Univ Wyoming, Dept Atmospher Sci, Laramie, WY 82071 USA. RP Kulkarni, G (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM Gourihar.Kulkarni@pnnl.gov RI Liu, Xiaohong/E-9304-2011; Zhao, Chun/A-2581-2012; Zhang, Kai/F-8415-2010 OI Liu, Xiaohong/0000-0002-3994-5955; Zhao, Chun/0000-0003-4693-7213; Zhang, Kai/0000-0003-0457-6368 FU Office of Science of the U.S. Department of Energy (DOE) as part of the Atmospheric System Research Program; U.S. DOE Community College Internship program; Battelle Memorial Institute [DE-AC05-76RL0 1830] FX The work was supported by the Office of Science of the U.S. Department of Energy (DOE) as part of the Atmospheric System Research Program. Support for Cassandra Sanders was provided by the U.S. DOE Community College Internship program. We thank Jerome Fast and Elaine King, respectively, for their support of this study. We are grateful for the technical support provided by Danny Nelson. We thank Tamas Varga for performing XRD analysis at Environmental Molecular Sciences Laboratory, which is a national scientific user facility located at Pacific Northwest National Laboratory in Richland, Washington. We also thank three anonymous reviewers for their time and efforts in reviewing this paper. Data supporting sections 2.1, 3.1, 3.2, and 3.4 and Figure 7 are available in the supporting information. This research was performed at the Atmospheric Measurement Laboratory, an atmospheric sciences laboratory at Pacific Northwest National Laboratory (PNNL). PNNL is operated by the U.S. DOE by Battelle Memorial Institute under contract DE-AC05-76RL0 1830. NR 83 TC 9 Z9 9 U1 3 U2 40 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 27 PY 2014 VL 119 IS 16 BP 9993 EP 10011 DI 10.1002/2014JD021567 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AP3RF UT WOS:000341994000025 ER PT J AU Bai, Y Tambe, A Zhou, KH Doudna, JA AF Bai, Yun Tambe, Akshay Zhou, Kaihong Doudna, Jennifer A. TI RNA-guided assembly of Rev-RRE nuclear export complexes SO ELIFE LA English DT Article ID HUMAN-IMMUNODEFICIENCY-VIRUS; SELECTIVE 2'-HYDROXYL ACYLATION; SECONDARY STRUCTURE PREDICTION; SINGLE-NUCLEOTIDE RESOLUTION; RESPONSE ELEMENT; HIV-1 REV; MESSENGER-RNA; VIRION EXPRESSION; SHAPE CHEMISTRY; GENE-EXPRESSION AB HIV replication requires nuclear export of unspliced and singly spliced viral transcripts. Although a unique RNA structure has been proposed for the Rev-response element (RRE) responsible for viral mRNA export, how it recruits multiple HIV Rev proteins to form an export complex has been unclear. We show here that initial binding of Rev to the RRE triggers RNA tertiary structural changes, enabling further Rev binding and the rapid formation of a viral export complex. Analysis of the Rev-RRE assembly pathway using SHAPE-Seq and small-angle X-ray scattering (SAXS) reveals two major steps of Rev-RRE complex formation, beginning with rapid Rev binding to a pre-organized region presenting multiple Rev binding sites. This step induces long-range remodeling of the RNA to expose a cryptic Rev binding site, enabling rapid assembly of additional Rev proteins into the RNA export complex. This kinetic pathway may help maintain the balance between viral replication and maturation. C1 [Bai, Yun; Tambe, Akshay; Zhou, Kaihong; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Zhou, Kaihong; Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM doudna@berkeley.edu FU National Institute of General Medical Sciences, The HARC Center [P50GM82250]; Howard Hughes Medical Institute FX National Institute of General Medical Sciences; The HARC Center, P50GM82250; Howard Hughes Medical Institute NR 65 TC 26 Z9 26 U1 0 U2 18 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD AUG 27 PY 2014 VL 3 AR e03656 DI 10.7554/eLife.03656 PG 17 WC Biology SC Life Sciences & Biomedicine - Other Topics GA AO3SW UT WOS:000341257200002 PM 25163983 ER PT J AU Kirner, JT Stracke, JJ Gregg, BA Finke, RG AF Kirner, Joel T. Stracke, Jordan J. Gregg, Brian A. Finke, Richard G. TI Visible-Light-Assisted Photoelectrochemical Water Oxidation by Thin Films of a Phosphonate-Functionalized Perylene Diimide Plus CoOx Cocatalyst SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE photoelectrochemical; catalysis; water oxidation; perylene diimide; cobalt oxide; molecular semiconductor; organic thin film ID INDUCED DIOXYGEN EVOLUTION; OXYGEN-EVOLVING CATALYST; BIS(PHENETHYLIMIDE) FILMS; HYDROGEN-PRODUCTION; TIN OXIDE; SOLAR; SEMICONDUCTOR; CELL; SPECTROSCOPY; PHOTOANODES AB A novel perylene diimide dye functionalized with phosphonate groups, N,N'-bis(phosphonomethyl)-3,4,9,10-perylenediimide (PMPDI), is synthesized and characterized. Thin films of PMPDI spin-coated onto indium tin oxide (ITO) substrates are further characterized, augmented by photoelectrochemically depositing a CoOx catalyst, and then investigated as photoanodes for water oxidation. These ITO/PMPDI/CoOx electrodes show visible-light-assisted water oxidation with photocurrents in excess of 150 mu A/cm(2) at 1.0 V applied bias vs. Ag/AgCl. Water oxidation is confirmed by the direct detection of O-2, with a faradaic efficiency of 80 +/- 15% measured under 900 mV applied bias vs. Ag/AgCl. Analogous photoanodes prepared with another PDI derivative with alkyl groups in place of PMPDI's phosphonate groups do not function, providing evidence that PMPDI's phosphonate groups may be important for efficient coupling between the inorganic CoOx catalyst and the organic dye. Our ITO/PMPDI/CoOx anodes achieve internal quantum efficiencies for water oxidation similar to 1%, and for hydroquinone oxidation of up to similar to 6%. The novelty of our system is that, to the best of our knowledge, it is the first device to achieve photoelectrochemically driven water oxidation by a single-layer molecular organic semiconductor thin film coupled to a water-oxidation catalyst. C1 [Kirner, Joel T.; Stracke, Jordan J.; Finke, Richard G.] Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA. [Gregg, Brian A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Gregg, BA (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM brian.gregg@nrel.gov; rfinke@lamar.colostate.edu FU Department of Energy, Office of Science, Graduate Fellowship Program; Oak Ridge Associated Universities under DOE [DE-AC05-06OR23100]; U.S. Department of Energy, Office of Science, Basic Energy Science, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC36-08GO28308]; NSF [CHE-1057723] FX This research was supported in part by an award to J.J.S. from the Department of Energy, Office of Science, Graduate Fellowship Program, which was made possible in part by the American Recovery and Reinvestment Act of 2009 and is administered for the Department of Energy by the Oak Ridge Institute for Science and Education, managed by Oak Ridge Associated Universities under DOE Contract DE-AC05-06OR23100. This work was supported in part at the National Renewable Energy Laboratory (NREL) by the U.S. Department of Energy, Office of Science, Basic Energy Science, Division of Chemical Sciences, Geosciences and Biosciences, under Contract DE-AC36-08GO28308. This work was performed primarily at Colorado State University when it was supported by NSF Grant CHE-1057723 (to R.G.F.). We thank Prof. C.M. Elliott and his research group for helpful discussion and for the use of their photovoltaic testing apparatus. NR 49 TC 29 Z9 29 U1 6 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 27 PY 2014 VL 6 IS 16 BP 13367 EP 13377 DI 10.1021/am405598w PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AO2CB UT WOS:000341122000010 PM 24654796 ER PT J AU Zhou, H Wang, HQ Li, YP Li, YY Kang, JY Zheng, JC Jiang, Z Huang, YY Wu, LJ Zhang, LH Kisslinger, K Zhu, YM AF Zhou, Hua Wang, Hui-Qiong Li, Yaping Li, Kongyi Kang, Junyong Zheng, Jin-Cheng Jiang, Zheng Huang, Yuying Wu, Lijun Zhang, Lihua Kisslinger, Kim Zhu, Yimei TI Evolution of Wurtzite ZnO Films on Cubic MgO (001) Substrates: A Structural, Optical, and Electronic Investigation of the Misfit Structures SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE ZnO; MgO; interface; transmission electron microscopy; X-ray absorption fine structure ID RAY-ABSORPTION SPECTROSCOPY; THIN-FILMS; ORIENTATION; GROWTH; SURFACE; TEMPERATURE; DEPOSITION; ROUGHNESS; NANORODS; IFEFFIT AB We investigated the interface between hexagonal ZnO films and cubic MgO (001) substrates, fabricated via molecular beam epitaxy. X-ray diffraction and (scanning) transmission electron microscopy revealed that growth follows the single [0001] direction when the temperature of the substrate is above 200 degrees C, while when the substrate temperature is below 150 degrees C, growth initially is along [0001] and then mainly changes to [0- 332] variants beyond a thickness of similar to 10 nm. Interestingly, a double-domain feature with a rotational angle of 30 degrees appears during growth along [0001] regardless of the temperature, experimentally demonstrating the theoretical predictions for the occurrence of double rotational domains in such a heteroepitaxy [Grundmann et mutation of growth directions, stimulated by the bond-length modulations, as we determined from X-ray absorption spectra at Zn K edge. These results also showed the evolution of the 4p(xy), and 4p(z) states in the conduction band with the rise in the temperature for growth. We consider that our findings may well promote the applications of ZnO in advanced optoelectronics for which its integration with other materials of different phases is desirable. C1 [Zhou, Hua; Wang, Hui-Qiong; Li, Yaping; Li, Kongyi; Kang, Junyong; Zheng, Jin-Cheng] Xiamen Univ, Dept Phys, Key Lab Semicond & Applicat Fujian Prov, Xiamen 361005, Peoples R China. [Jiang, Zheng; Huang, Yuying] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201800, Peoples R China. [Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Zhang, Lihua; Kisslinger, Kim] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Wang, HQ (reprint author), Xiamen Univ, Dept Phys, Key Lab Semicond & Applicat Fujian Prov, Xiamen 361005, Peoples R China. EM hqwang@xmu.edu.cn RI Kisslinger, Kim/F-4485-2014; Zhang, Lihua/F-4502-2014; Zheng, JC/G-3383-2010; Wang, Hui-Qiong/H-4690-2011 OI Zheng, JC/0000-0002-6292-3236; FU Natural Science Foundation of China [11204253, U1232110, U1332105, 61227009, 91321102]; Specialized Research Fund for the Doctoral Program of Higher Education [20120121110021]; Fundamental Research Funds for Central Universities [2012121012, 2013SH001]; National High-Tech R&D Program of China (863 Program) [2013AA050901]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by Natural Science Foundation of China (Grant Nos. 11204253, U1232110, U1332105, 61227009, and 91321102), the Specialized Research Fund for the Doctoral Program of Higher Education (Grant No. 20120121110021), the Fundamental Research Funds for Central Universities (Grant Nos. 2012121012, 2013SH001), and the National High-Tech R&D Program of China (863 Program, No. 2013AA050901). Research carried out (in part) at Condensed Matter Physics and Materials Science Department and the Center for Functional Nanomaterials, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 49 TC 3 Z9 3 U1 3 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 27 PY 2014 VL 6 IS 16 BP 13823 EP 13832 DI 10.1021/am503256p PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AO2CB UT WOS:000341122000063 PM 25055030 ER PT J AU Nasybulin, EN Xu, W Mehdi, BL Thomsen, E Engelhard, MH Masse, RC Bhattacharya, P Gu, M Bennett, W Nie, ZM Wang, CM Browning, ND Zhang, JG AF Nasybulin, Eduard N. Xu, Wu Mehdi, B. Layla Thomsen, Edwin Engelhard, Mark H. Masse, Robert C. Bhattacharya, Priyanka Gu, Meng Bennett, Wendy Nie, Zimin Wang, Chongmin Browning, Nigel D. Zhang, Ji-Guang TI Formation of Interfacial Layer and Long-Term Cyclability of Li-O-2 Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE Li-O-2 battery; rechargeability; carbon nanotubes; Li2O2; cyclability ID X-RAY PHOTOELECTRON; LITHIUM-OXYGEN BATTERY; WALLED CARBON NANOTUBES; LI-AIR BATTERIES; SPECTROSCOPY; LI2O2; ELECTROLYTE; STABILITY; NANOPARTICLES; PERFORMANCE AB The long-term operation of Li-O-2 batteries under full discharge/charge conditions is investigated in a glyme-based electrolyte. The formation of stable interfacial layer on the electrode surface during the initial cycling stabilizes reaction products at subsequent cycling stages as demonstrated by quantitative analyses of the discharge products and the gases released during charging. There is a quick switch from the predominant formation of Li2O2 to the predominant formation of side products during the first few cycles. However, after the formation of the stable interfacial layer, the yield of Li2O2 in the reaction products is stabilized at about 33-40%. Extended cycling under full discharge/charge conditions is achievable upon selection of appropriate electrode materials (carbon source and catalyst) and cycling protocol. Further investigation on the interfacial layer, which in situ forms on air electrode, may increase the long-term yield of Li2O2 during the cycling and enable highly reversible Li-O-2 batteries required for practical applications. C1 [Nasybulin, Eduard N.; Xu, Wu; Thomsen, Edwin; Masse, Robert C.; Bhattacharya, Priyanka; Bennett, Wendy; Nie, Zimin; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Mehdi, B. Layla; Browning, Nigel D.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99354 USA. [Engelhard, Mark H.; Gu, Meng; Wang, Chongmin] Pacific NW Natl Lab, Wiliam R Wiley Environm & Mol Sci Lab, Richland, WA 99354 USA. [Masse, Robert C.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. RP Xu, W (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. EM wu.xu@pnnl.gov; jiguang.zhang@pnnl.gov RI Bhattacharya, Priyanka/E-1652-2011; Masse, Robert /M-8025-2014; Gu, Meng/B-8258-2013; OI Bhattacharya, Priyanka/0000-0003-0368-8480; Masse, Robert /0000-0002-0929-5509; Engelhard, Mark/0000-0002-5543-0812; Browning, Nigel/0000-0003-0491-251X FU Joint Center for Energy Storage Research, an Energy Innovation Hub - DOE's Office of Science, Basic Energy Sciences; DOE's Office of Biological and Environmental Research FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, of the U.S. Department of Energy (DOE). The microscopic analysis in this work was supported by the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by DOE's Office of Science, Basic Energy Sciences, and was performed in the William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 50 TC 20 Z9 20 U1 1 U2 87 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 27 PY 2014 VL 6 IS 16 BP 14141 EP 14151 DI 10.1021/am503390q PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AO2CB UT WOS:000341122000099 PM 25068384 ER PT J AU Pham, VH Dickerson, JH AF Viet Hung Pham Dickerson, James H. TI Superhydrophobic Silanized Melamine Sponges as High Efficiency Oil Absorbent Materials SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE superhydrophobicity; melamine sponge; oil absorbent; silanization; oil spill cleanup ID CARBON NANOTUBE SPONGES; SPILL RECOVERY; POLYURETHANE SPONGE; WATER; ABSORPTION; ULTRALIGHT; SEPARATION; CLEANUP; EMISSIONS; VERSATILE AB Superhydrophobic sponges and sponge-like materials have attracted great attention recently as potential sorbent materials for oil spill cleanup due to their excellent sorption capacity and high selectivity. A major challenge to their broad use is the fabrication of superhydrophobic sponges with superior recydability, good mechanical strength, low cost, and manufacture scalability. In this study, we demonstrate a facile, cost-effective, and scalable method to fabricate robust, superhydrophobic sponges through the silanization of commercial melamine sponges via a solution-immersion process. The silanization was achieved through secondary amine groups on the surface of the sponge skeletons with alkylsilane compounds, forming self-assembled monolayers on the surface of sponge skeletons. This resulted in our ability to tune the surface properties of the sponges from being hydrophilic to superhydrophobic with a water contact angle of 151.0 degrees. The superhydrophobic silanized melamine sponge exhibited excellent sorption capacity for a wide range of organic solvents and oils, from 82 to 163 times its own weight, depending on the polarity and density of the employed organic solvents and oils, and high selectivity and outstanding recyclability with an absorption capacity retention greater than 90% after 1000 cycles. These findings offer an effective approach for oil spill containment and environmental remediation. C1 [Viet Hung Pham; Dickerson, James H.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Dickerson, JH (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM jdickerson@bnl.gov FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We thank Dr. Thomas Butcher and Dr. Christopher Brown for supplying the No. 2 home heating oil and biodiesel. We thank Dr. Xiao Tong for assistance with the XPS measurement and Dr. Antonio Checco for use of the OCA 15+ goniometer for the water contact angle measurements. We thank Dr. Tesfaye Gebre for fruitful discussions. This work was performed at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 34 TC 50 Z9 50 U1 22 U2 153 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 27 PY 2014 VL 6 IS 16 BP 14181 EP 14188 DI 10.1021/am503503m PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AO2CB UT WOS:000341122000104 PM 25039789 ER PT J AU Du, YG Gu, M Varga, T Wang, CM Bowden, ME Chambers, SA AF Du, Yingge Gu, Meng Varga, Tamas Wang, Chongmin Bowden, Mark E. Chambers, Scott A. TI Strain Accommodation by Facile WO6 Octahedral Distortion and Tilting during WO3 Heteroepitaxy on SrTiO3(001) SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE WO3; epitaxy; tungsten oxide; octahedral distortion; SrTiO3 ID TUNGSTEN-OXIDE; THIN-FILMS; PHOTOELECTRON-SPECTROSCOPY; GROWTH; FERROELECTRICITY; TRIOXIDE; PEROVSKITES; COALESCENCE; TRANSITION; EVOLUTION AB In this work, we demonstrate that WO6 octahedra in tungsten trioxide (WO3) undergo an unusually large degree of distortion and tilting to accommodate interfacial strain. This motion strongly impacts nucleation, structure, and defect formation during the epitaxial growth of WO3 on SrTiO3(001). A metastable tetragonal phase can be stabilized by heteroepitaxy and a thickness-dependent phase transition (tetragonal to monoclinic) is observed. In contrast to misfit dislocation formation, facile WO6 octahedral deformation gives rise to three types of planar defects. The thicknesses of affected regions can range from several to tens of nanometers with graded lattice parameters, allowing the strain from interfacial lattice mismatch to be relieved gradually. These atomically resolved, unique interfacial defects may significantly alter the electronic, electrochromic, and mechanical properties of WO3 epitaxial films. C1 [Du, Yingge; Gu, Meng; Varga, Tamas; Wang, Chongmin; Bowden, Mark E.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Chambers, Scott A.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Du, YG (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. EM yingge.du@pnnl.gov RI Gu, Meng/B-8258-2013 FU Department of Energy's Office of Biological and Environmental Research at Pacific Northwest National Laboratory; EMSL's Intramural Research and Capability Development Program; Office of Basic Energy Sciences, Division of Materials Science and Engineering [10122]; Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX The work was performed using the Environmental Molecular Sciences Laboratory, a national scientific user facility, sponsored by the Department of Energy's Office of Biological and Environmental Research, located at Pacific Northwest National Laboratory. Y.D. gratefully acknowledges support by EMSL's Intramural Research and Capability Development Program. A portion of the work was supported by the Office of Basic Energy Sciences, Division of Materials Science and Engineering under Award 10122. M.G. and C.W. are thankful for the support by the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The authors thank Ping Yang, Tim Droubay, and Kelvin H. L. Zhang for many insightful discussions. NR 35 TC 7 Z9 7 U1 2 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 27 PY 2014 VL 6 IS 16 BP 14253 EP 14258 DI 10.1021/am5035686 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AO2CB UT WOS:000341122000113 PM 25058665 ER PT J AU Qiao, L Li, W Xiao, HY Meyer, HM Liang, XL Nguyen, NV Weber, WJ Biegalski, MD AF Qiao, Liang Li, Wei Xiao, Haiyan Meyer, Harry M. Liang, Xuelei Nguyen, N. V. Weber, William J. Biegalski, Michael D. TI Electronic Structure and Band Alignment at an Epitaxial Spinel/Perovskite Heterojunction SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE spinel/perovskite heterojunction; electronic structure; band alignment; photoemission ID RAY PHOTOEMISSION SPECTRA; THIN-FILMS; PRECISE DETERMINATION; COBALT OXIDES; CORE-LEVEL; SRTIO3; CO3O4; INTERFACE; SURFACES; OFFSETS AB The electronic properties of solid solid interfaces play critical roles in a variety of technological applications. Recent advances of film epitaxy and characterization techniques have demonstrated a wealth of exotic phenomena at interfaces of oxide materials, which are critically dependent on the alignment of their energy bands across the interface. Here we report a combined photoemission and electrical investigation of the electronic structures across a prototypical spinel/perovskite heterojunction. Energy-level band alignment at an epitaxial Co3O4/SrTiO3(001) heterointerface indicates a chemically abrupt, type I heterojunction without detectable band bending at both the film and substrate. The unexpected band alignment for this typical p-type semiconductor on SrTiO3 is attributed to its intrinsic d-d interband excitation, which significantly narrows the fundamental band gap between the top of the valence band and the bottom of the conduction band. The formation of the type I heterojunction with a flat-band state results in a simultaneous confinement of both electrons and holes inside the Co3O4 layer, thus rendering the epitaxial Co3O4/SrTiO3(001) heterostructure to be a very promising material for high-efficiency luminescence and optoelectronic device applications. C1 [Qiao, Liang; Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Meyer, Harry M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Li, Wei; Nguyen, N. V.] NIST, Semicond & Dimens Metrol Div, Gaithersburg, MD 20899 USA. [Xiao, Haiyan] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. [Xiao, Haiyan; Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Li, Wei; Liang, Xuelei] Peking Univ, Key Lab Phys & Chem Nanodevices, Beijing 100871, Peoples R China. [Li, Wei; Liang, Xuelei] Peking Univ, Dept Elect, Beijing 100871, Peoples R China. RP Qiao, L (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM qiaol@ornl.gov; biegalskim@ornl.gov RI Weber, William/A-4177-2008; Qiao, Liang/A-8165-2012; Liang, Xuelei/C-4690-2013 OI Weber, William/0000-0002-9017-7365; FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; University of Electronic Science and Technology of China [Y02002010401085]; NSAF Joint Foundation of China [U1330103]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX This research was conducted at the Center for Nanophase Materials Sciences and SHaRE User Facility, which are sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors would like to thank the NIST Center for Nanoscale Science and Technology's Nanofab Facility for device fabrication support. H. Y. Xiao acknowledges the support of scientific research starting funding from University of Electronic Science and Technology of China (Grant No. Y02002010401085) and NSAF Joint Foundation of China (Grant No. U1330103). W. J. Weber was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 50 TC 2 Z9 2 U1 9 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 27 PY 2014 VL 6 IS 16 BP 14338 EP 14344 DI 10.1021/am5036219 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AO2CB UT WOS:000341122000123 PM 25075939 ER PT J AU Gharachorlou, A Detwiler, MD Nartova, AV Lei, Y Lu, JL Elam, JW Delgass, WN Ribeiro, FH Zemlyanov, DY AF Gharachorlou, Amir Detwiler, Michael D. Nartova, Anna V. Lei, Yu Lu, Junling Elam, Jeffrey W. Delgass, W. Nicholas Ribeiro, Fabio H. Zemlyanov, Dmitry Y. TI Palladium Nanoparticle Formation on TiO2(110) by Thermal Decomposition of Palladium(II) Hexafluoroacetylacetonate SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE X-ray photoelectron spectroscopy; scanning tunneling microscopy; atomic layer deposition; Pd(hfac)(2); TiO2(110); nucleation delay; surface science; heterogeneous catalysis ID ATOMIC LAYER DEPOSITION; CHEMICAL-VAPOR-DEPOSITION; PHOTOIONIZATION CROSS-SECTIONS; THIN-FILM GROWTH; PD NANOPARTICLES; RUTILE TIO2(110); COPPER SURFACES; OXIDATION; CATALYSTS; BIS(HEXAFLUOROACETYLACETONATO)PALLADIUM(II) AB Palladium nanoparticles were synthesized by thermal decomposition of palladium(II) hexafluoroacetylacetonate (Pd(hfac)(2)), an atomic layer deposition (ALD) precursor, on a TiO2(110) surface. According to X-ray photoelectron spectroscopy (XPS), Pd(hfac)(2) adsorbs on TiO2(110) dissociatively yielding Pd(hfac)(ads), hfac(ads), and adsorbed fragments of the hfac ligand at 300 K. A (2 x 1) surface overlayer was observed by scanning tunneling microscopy (STM), indicating that hfac adsorbs in a bidentate bridging fashion across two Ti 5-fold atoms and Pd(hfac) adsorbs between two bridging oxygen atoms on the surface. Annealing of the Pd(hfac)(ads) and hfac(ads) species at 525 K decomposed the adsorbed hfac ligands, leaving PdO-like species and/or Pd atoms or clusters. Above 575 K, the XPS Pd 3d peaks shift toward lower binding energies and Pd nanoparticles are observed by STM. These observations point to the sintering of Pd atoms and clusters to Pd nanoparticles. The average height of the Pd nanopartides was 1.2 +/- 0.6 nm at 575 K and increased to 1.7 +/- 0.5 nm following annealing at 875 K. The Pd coverage was estimated from XPS and STM data to be 0.05 and 0.03 monolayers (ML), respectively, after the first adsorption/decomposition cycle. The amount of palladium deposited on the TiO2(110) surface increased linearly with the number of adsorption/decomposition cycles with a growth rate of 0.05 ML or 0.6 angstrom per cycle. We suggest that the removal of the hfac ligand and fragments eliminates the nucleation inhibition of Pd nanopartides previously observed for the Pd(hfac)(2) precursor on TiO2. C1 [Gharachorlou, Amir; Detwiler, Michael D.; Nartova, Anna V.; Delgass, W. Nicholas; Ribeiro, Fabio H.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Nartova, Anna V.] Boreskov Inst Catalysis, Novosibirsk 630090, Russia. [Nartova, Anna V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Lei, Yu; Lu, Junling; Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Zemlyanov, Dmitry Y.] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. RP Zemlyanov, DY (reprint author), Purdue Univ, Birck Nanotechnol Ctr, 1205 W State St, W Lafayette, IN 47906 USA. EM dzemlian@purdue.edu RI Lu, Junling/F-3791-2010 OI Lu, Junling/0000-0002-7371-8414 FU Institute for Atom-efficient Chemical Transformations (TACT), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This material is based upon work supported as part of the Institute for Atom-efficient Chemical Transformations (TACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Use of the Center for Nanoscale Materials (CNM) was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The support of Dr. Nathan Guisinger at CNM during the STM experiments is greatly appreciated. The authors acknowledge Lukas Mayr for his contribution to the figures in this text. NR 42 TC 17 Z9 17 U1 9 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 27 PY 2014 VL 6 IS 16 BP 14702 EP 14711 DI 10.1021/am504127k PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AO2CB UT WOS:000341122000166 PM 25093626 ER PT J AU Chen, HP Hsiao, YC Hu, B Dadmun, M AF Chen, Huipeng Hsiao, Yu-Che Hu, Bin Dadmun, Mark TI Tuning the Morphology and Performance of Low Bandgap Polymer: Fullerene Heterojunctions via Solvent Annealing in Selective Solvents SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID ANGLE NEUTRON-SCATTERING; COPOLYMER THIN-FILMS; SOLAR-CELLS; ORGANIC PHOTOVOLTAICS; CONJUGATED POLYMER; BLENDS; EFFICIENCY; POLY(3-HEXYLTHIOPHENE); METHANOFULLERENES; ORGANIZATION AB Low bandgap polymer (LBG): fullerene mixtures are some of the most promising organic photovoltaic active layers. Unfortunately, there are no post-deposition treatments available to rationally improve the morphology and performance of as-cast LBG: fullerene OPV active layers, where thermal annealing usually fails. Therefore, there is a glaring need to develop post-deposition methods to guide the morphology of LBG: fullerene bulk heterojunctions towards targeted structures and performance. In this paper, the structural evolution of PCPDTBT:PCBM mixtures with solvent annealing (SA) is examined, focusing on the effect of solvent quality of the fullerene and polymer in the annealing vapor on morphological evolution and device performance. The results indicate that exposure of this active layer to the solvent vapor controls the ordering of PCPDTBT and PCBM phase separation very effectively, presumably by inducing component mobility as the solvent plasticizes the mixture. These results also unexpectedly indicate that solvent annealing in a selective solvent provides a method to invert the morphology of the LBG: fullerene mixture from a polymer aggregate dispersed in a polymer: fullerene matrix to fullerene aggregates dispersed in a polymer: fullerene matrix. The judicious choice of solvent vapor, therefore, provides a unique method to exquisitely control and optimize the morphology of LBG conjugated polymer/fullerene mixtures. C1 [Chen, Huipeng; Dadmun, Mark] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Chen, Huipeng] Fuzhou Univ, Inst Optoelect Display, Fuzhou 350002, Peoples R China. [Dadmun, Mark] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Hsiao, Yu-Che; Hu, Bin] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Chen, HP (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM Dad@utk.edu RI Hu, Bin/A-2954-2015 OI Hu, Bin/0000-0002-1573-7625 FU Sustainable Energy Education Research Center; Joint Institute for Neutron Sciences at the University of Tennessee; National Science Foundation [DMR-1005987, DMR-0944772]; Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy - Oak Ridge National Laboratory High Flux Isotope Reactor; National Institute of Standards and Technology, US Department of Commerce FX The authors wish to acknowledge the Sustainable Energy Education Research Center and the Joint Institute for Neutron Sciences at the University of Tennessee, as well as the National Science Foundation (DMR-1005987) for support of this project. MDD also acknowledges the support of the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The support of the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy, who sponsors the Oak Ridge National Laboratory High Flux Isotope Reactor is gratefully acknowledged. This work also utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-0944772. We acknowledge the support of the National Institute of Standards and Technology, US Department of Commerce, in providing the neutron research facilities used in this work. NR 39 TC 15 Z9 16 U1 3 U2 102 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD AUG 27 PY 2014 VL 24 IS 32 BP 5129 EP 5136 DI 10.1002/adfm.201400552 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AO2ID UT WOS:000341142100013 ER PT J AU Lin, YP Chomvong, KL Acosta-Sampson, L Estrela, R Galazka, JM Kim, SR Jin, YS Cate, JHD AF Lin, Yuping Chomvong, Kulika Acosta-Sampson, Ligia Estrela, Raissa Galazka, Jonathan M. Kim, Soo Rin Jin, Yong-Su Cate, Jamie H. D. TI Leveraging transcription factors to speed cellobiose fermentation by Saccharomyces cerevisiae SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Cellobiose; Glycolysis; Systems biology; Transcription factor; Metabolic engineering; Biofuels ID CO-FERMENTATION; STEROL UPTAKE; CATABOLITE REPRESSION; GLUCONEOGENIC GENES; REGULATORY NETWORKS; SIGNALING PATHWAYS; XYLOSE CONSUMPTION; BIOFUEL PRODUCTION; SHUTTLE VECTORS; PROTEIN-KINASE AB Background: Saccharomyces cerevisiae, a key organism used for the manufacture of renewable fuels and chemicals, has been engineered to utilize non-native sugars derived from plant cell walls, such as cellobiose and xylose. However, the rates and efficiencies of these non-native sugar fermentations pale in comparison with those of glucose. Systems biology methods, used to understand biological networks, hold promise for rational microbial strain development in metabolic engineering. Here, we present a systematic strategy for optimizing non-native sugar fermentation by recombinant S. cerevisiae, using cellobiose as a model. Results: Differences in gene expression between cellobiose and glucose metabolism revealed by RNA deep sequencing indicated that cellobiose metabolism induces mitochondrial activation and reduces amino acid biosynthesis under fermentation conditions. Furthermore, glucose-sensing and signaling pathways and their target genes, including the cAMP-dependent protein kinase A pathway controlling the majority of glucose-induced changes, the Snf3-Rgt2-Rgt1 pathway regulating hexose transport, and the Snf1-Mig1 glucose repression pathway, were at most only partially activated under cellobiose conditions. To separate correlations from causative effects, the expression levels of 19 transcription factors perturbed under cellobiose conditions were modulated, and the three strongest promoters under cellobiose conditions were applied to fine-tune expression of the heterologous cellobiose-utilizing pathway. Of the changes in these 19 transcription factors, only overexpression of SUT1 or deletion of HAP4 consistently improved cellobiose fermentation. SUT1 overexpression and HAP4 deletion were not synergistic, suggesting that SUT1 and HAP4 may regulate overlapping genes important for improved cellobiose fermentation. Transcription factor modulation coupled with rational tuning of the cellobiose consumption pathway significantly improved cellobiose fermentation. Conclusions: We used systems-level input to reveal the regulatory mechanisms underlying suboptimal metabolism of the non-glucose sugar cellobiose. By identifying key transcription factors that cause suboptimal cellobiose fermentation in engineered S. cerevisiae, and by fine-tuning the expression of a heterologous cellobiose consumption pathway, we were able to greatly improve cellobiose fermentation by engineered S. cerevisiae. Our results demonstrate a powerful strategy for applying systems biology methods to rapidly identify metabolic engineering targets and overcome bottlenecks in performance of engineered strains. C1 [Lin, Yuping; Acosta-Sampson, Ligia; Estrela, Raissa; Galazka, Jonathan M.; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Chomvong, Kulika; Cate, Jamie H. D.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Kim, Soo Rin; Jin, Yong-Su] Univ Illinois, Dept Food Sci & Human Nutr, Urbana, IL 61801 USA. [Kim, Soo Rin; Jin, Yong-Su] Univ Illinois, Inst Genom Biol, Urbana, IL 61801 USA. RP Cate, JHD (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. EM jcate@lbl.gov OI Kim, Soo Rin/0000-0001-5855-643X FU Energy Biosciences Institute FX We thank Mara Bryan, Stefan Bauer, Ana Belen Ibanez for technical assistance and Crystal Chan for ordering common supplies. We thank Owen Ryan, Xin Li and Mitchell Altschuler for discussion and comments on results. This work was supported by funding from Energy Biosciences Institute to Jamie H. D. Cate, Soo Rin Kim, and Yong-Su Jin. NR 97 TC 9 Z9 10 U1 0 U2 22 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD AUG 27 PY 2014 VL 7 AR 126 DI 10.1186/s13068-014-0126-6 PG 15 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AO0UK UT WOS:000341027700001 PM 25435910 ER PT J AU Nakouzi, GA Nadeau, JH AF Nakouzi, Ghunwa A. Nadeau, Joseph H. TI Does dietary folic acid supplementation in mouse NTD models affect neural tube development or gamete preference at fertilization? SO BMC GENETICS LA English DT Article DE Neural tube defects; Mouse models; Folic acid; Apob; Vangl2; Embryonic lethality; Polyamines; Fertilization; Gametes; Sperm; Oocyte; Epigenetics ID ONE-CARBON METABOLISM; ORNITHINE-DECARBOXYLASE; DEFECTS; FOLATE; MICE; EXPRESSION; GENE; ABNORMALITIES; EPIGENETICS; INFERTILITY AB Background: Neural tube defects (NTDs) are the second most common birth defect in humans. Dietary folic acid (FA) supplementation effectively and safely reduces the incidence of these often debilitating congenital anomalies. FA plays an established role in folate and homocysteine metabolism, but the means by which it suppresses occurrence of NTDs is not understood. In addition, many cases remain resistant to the beneficial effects of folic acid supplementation. To better understand the molecular, biochemical and developmental mechanisms by which FA exerts its effect on NTDs, characterized mouse models are needed that have a defined genetic basis and known response to dietary supplementation. Results: We examined the effect of FA supplementation, at 5-fold the level in the control diet, on the NTD and vertebral phenotypes in Apob(tm1Unc) and Vangl2(lp) mice, hereafter referred to as Apob and Lp respectively. The FA supplemented diet did not reduce the incidence or severity of NTDs in Apob or Lp mutant homozygotes or the loop-tail phenotype in Lp mutant heterozygotes, suggesting that mice with these mutant alleles are resistant to FA supplementation. Folic acid supplementation also did not affect the rate of resorptions or the size of litters, but instead skewed the embryonic genotype distribution in favor of wild-type alleles. Conclusion: Similar genotypic biases have been reported for several NTD models, but were interpreted as diet-induced increases in the incidence and severity of NTDs that led to increased embryonic lethality. Absence of differences in resorption rates and litter sizes argue against induced embryonic lethality. We suggest an alternative interpretation, namely that FA supplementation led to strongly skewed allelic inheritance, perhaps from disturbances in polyamine metabolism that biases fertilization in favor of wild-type gametes. C1 [Nakouzi, Ghunwa A.; Nadeau, Joseph H.] Case Western Reserve Univ, Sch Med, Dept Genet, Cleveland, OH 44106 USA. RP Nadeau, JH (reprint author), Pacific Northwest Res Inst, 720 Broadway, Seattle, WA 98122 USA. EM jnadeau@pnri.org FU NIH [NS058979, DP1HD075624] FX NIH grants NS058979 and DP1HD075624 supported this work. We thank Mary Ann Handel, Marisa Bartolomei, Jacquetta Trasler, Betsy Ross, Lee Niswander, the Nadeau lab for thoughtful discussions of these problems, and the reviewers for their helpful comments and suggestions. NR 58 TC 6 Z9 6 U1 1 U2 14 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2156 J9 BMC GENET JI BMC Genet. PD AUG 27 PY 2014 VL 15 AR 91 DI 10.1186/s12863-014-0091-x PG 9 WC Genetics & Heredity SC Genetics & Heredity GA AO1YT UT WOS:000341112200001 PM 25154628 ER PT J AU Monazam, ER Breault, RW Siriwardane, R AF Monazam, Esmail R. Breault, Ronald W. Siriwardane, Ranjani TI Kinetics of Magnetite (Fe3O4) Oxidation to Hematite (Fe2O3) in Air for Chemical Looping Combustion SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID OXYGEN CARRIERS AB Thermogravimetric analysis (TGA) of magnetite (Fe3O4) oxidation was conducted at temperatures ranging from 750 to 900 degrees C over 10 oxidation cycles. Oxidation experiments were carried out in a continuous stream of air for period of 30 min. The oxidized magnetite (Fe3O4), which resulted in formation of hematite (Fe2O3), was then reduced by using continuous stream of CO (5% and 10%) with N-2 balance. The rate of oxidation was determined by the oxygen weight gain. Analysis of the data indicated that the oxidation behavior followed a two-stage process. The initial oxidation, which was very fast, took place in 2 min and was described using nucleation and growth processes with a low activation energy of about 4.21 +/- 0.45 kJ/mol. As the reaction developed within the surface, oxygen transport through the product layer become the rate-controlling step with activation energy of 53.58 +/- 3.56 kJ/mol. C1 [Breault, Ronald W.; Siriwardane, Ranjani] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Monazam, Esmail R.] REM Engn Serv PLLC, Morgantown, WV 26505 USA. RP Breault, RW (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM ronald.breault@netl.doe.gov OI Breault, Ronald/0000-0002-5552-4050 FU Department of Energy through the office of Fossil Energy's Gasification Technology and Advanced Research funding programs FX We acknowledge the Department of Energy for funding the research through the office of Fossil Energy's Gasification Technology and Advanced Research funding programs. Special thanks go to Duane D. Miller, Hanjing Tian, and Thomas Simonyi of URS Energy & Construction, Inc. for their assistance with experimental work and data. NR 20 TC 12 Z9 13 U1 3 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD AUG 27 PY 2014 VL 53 IS 34 BP 13320 EP 13328 DI 10.1021/ie501536s PG 9 WC Engineering, Chemical SC Engineering GA AO0IJ UT WOS:000340992000011 ER PT J AU Bhagi-Damodaran, A Petrik, ID Marshall, NM Robinson, H Lu, Y AF Bhagi-Damodaran, Ambika Petrik, Igor D. Marshall, Nicholas M. Robinson, Howard Lu, Yi TI Systematic Tuning of Heme Redox Potentials and Its Effects on O-2 Reduction Rates in a Designed Oxidase in Myoglobin SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CYTOCHROME-C-OXIDASE; COPPER OXIDASES; ELECTRON-TRANSFER; BINDING; SITE; PROTEINS; ENZYMES; MODELS AB Cytochrome c Oxidase (CcO) is known to catalyze the reduction of O-2 to H2O efficiently with a much lower overpotential than most other O-2 reduction catalysts. However, methods by which the enzyme fine-tunes the reduction potential (E degrees) of its active site and the corresponding influence on the O-2 reduction activity are not well understood. In this work, we report systematic tuning of the heme E degrees in a functional model of CcO in myoglobin containing three histidines and one tyrosine in the distal pocket of heme. By removing hydrogen-bonding interactions between Ser92 and the proximal His ligand and a heme propionate, and increasing hydrophobicity of the heme pocket through Ser92Ala mutation, we have increased the heme E degrees from 95 +/- 2 to 123 +/- 3 mV. Additionally, replacing the native heme b in the CcO mimic with heme a analogs, diacetyl, monoformyl, and diformyl hemes, that posses electron-withdrawing groups, resulted in higher E degrees values of 175 +/- 5, 210 +/- 6, and 320 +/- 10 mV, respectively. Furthermore, O-2 consumption studies on these CcO mimics revealed a strong enhancement in O-2 reduction rates with increasing heme E degrees. Such methods of tuning the heme E degrees through a combination of secondary sphere mutations and heme substitutions can be applied to tune E degrees of other heme proteins, allowing for comprehensive investigations of the relationship between E degrees and enzymatic activity. C1 [Bhagi-Damodaran, Ambika; Petrik, Igor D.; Marshall, Nicholas M.; Lu, Yi] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Robinson, Howard] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Lu, Y (reprint author), Univ Illinois, Dept Chem, 1209 W Calif St, Urbana, IL 61801 USA. EM yi-lu@illinois.edu RI Lu, Yi/B-5461-2010 OI Lu, Yi/0000-0003-1221-6709 FU US National Institute of Health [GM062211] FX We thank Anoop R. Damodaran and Prof. Robert B. Gennis for helpful discussions. This report is based on work supported by the US National Institute of Health (GM062211). NR 38 TC 23 Z9 23 U1 3 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 27 PY 2014 VL 136 IS 34 BP 11882 EP 11885 DI 10.1021/ja5054863 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AO0IX UT WOS:000340993400008 PM 25076049 ER PT J AU Schmidt, AC Heinemann, FW Lukens, WW Meyer, K AF Schmidt, Anna-Corina Heinemann, Frank W. Lukens, Wayne W., Jr. Meyer, Karsten TI Molecular and Electronic Structure of Dinuclear Uranium Bis-mu-Oxo Complexes with Diamond Core Structural Motifs SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID VALENT ORGANOURANIUM COMPLEXES; BRIDGED DIURANIUM COMPLEXES; CATION-CATION INTERACTIONS; F-ELEMENT COMPLEXES; PENTAVALENT URANIUM; MAGNETIC-PROPERTIES; DIOXYGEN ACTIVATION; FUNCTIONAL-GROUPS; HALIDE-COMPLEXES; URANYL-ION AB In a multiple-bond metathesis reaction, the triazacydononane (tacn)-anchored methyl- and neopentyl (nP)-substituted tris(aryloxide) U-III complex [(((ArO)-Ar-nP,Me)(3)tacn)U-III] (1) reacts with mesityl azide and CO2 to form mesityl isocyanate and the dinuclear bis(mu-oxo)-bridged U-V/U-V complex [{(((ArO)-Ar-nP,Me)(3)tacn)U-V}(2)(mu-O)(2)] (3). This reaction proceeds via the mononuclear U-V imido intermediate [(((ArO)-Ar-nP,Me)(3)tacn)U-V(NMes)] (2), which has been synthesized and fully characterized independently. The dimeric U-V oxo species shows rich redox behavior: complex 3 can be reduced by one and two electrons, respectively, yielding the mixed-valent U-IV/U-V bis(mu-oxo) complex [K(crypt)][{(((ArO)-Ar-nP,Me)(3)tacn)U-IV/V}(2)(mu-O)(2)] (7) and the U-IV/U-IV bis(mu-oxo) complex K-2[{(((ArO)-Ar-nP,Me)(3)tacn)U-IV}(2)(mu-O)(2)] (6). In addition, complex 3 can be oxidized to provide the mononuclear uranium(VI) oxo complexes [(((ArO)-Ar-nP,Me)(3)tacn)U-VI(O)(eq)(OTf)(ax)] (8) and [(((ArO)-Ar-nP,Me)(3)tacn)U-VI(O)(eq)]SbF6 (9). The unique series of bis(mu-oxo) complexes also shows notable magnetic behavior, which was investigated in detail by UV/vis/NIR and EPR spectroscopy as well as SQUID magnetization studies. In order to understand possible magnetic exchange phenomena, the mononuclear terminal oxo complexes [(((ArO)-Ar-nP,Me)(3)tacn)U-V(O)(O-pyridine)] (4) and [(((ArO)-Ar-nP,Me)(3)tacn)U-V(PO)(O-NMe3)] (5) were synthesized and fully characterized. The magnetic study revealed an unusually strong antiferromagnetic exchange coupling between the two U-V ions in 3. Examination of the O-18-labeled bis(mu-oxo)-bridged dinuclear complexes 3, 6, and 7 allowed for the first time the unambiguous assignment of the vibrational signature of the [U(mu-O)(2)U] diamond core structural motif. C1 [Schmidt, Anna-Corina; Heinemann, Frank W.; Meyer, Karsten] Univ Erlangen Nurnberg, Dept Chem & Pharm, D-91058 Erlangen, Germany. [Lukens, Wayne W., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Lukens, WW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, MS 70A-1150, Berkeley, CA 94720 USA. EM wwlukens@lbl.gov; karsten.meyer@fau.de RI Meyer, Karsten/G-2570-2012 OI Meyer, Karsten/0000-0002-7844-2998 FU Bundesministerium fur Bildung and Forschung (BMBF) [02NUK012B]; FAU Erlangen-Nurnberg; COST Action [CM1006]; U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Biosciences, and Geo-sciences Division, Heavy Element Chemistry Program; Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX Dedicated to the memory of Dr. Lester R. Morss for his friendship and encouragement. Support from the Bundesministerium fur Bildung and Forschung (BMBF 2020+, 02NUK012B), the FAU Erlangen-Nurnberg, and COST Action CM1006 is acknowledged. Portions of this work were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Biosciences, and Geo-sciences Division, Heavy Element Chemistry Program and were performed at Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. We thank Dr. A. K. Abdul-Sada and Prof. F. Geoffrey N. Cloke for performing mass spectrometry experiments. Furthermore, we gratefully acknowledge Prof. Dr. Dirk M. Gulch for use of his Raman spectrometer and Dipl. Chem. Tobias Engesser and Prof. Dr. Ingo Krossing for kindly providing Ag[Al(OC(CF3)3)4] and NO[Al(OC(CF3)3)4]. NR 83 TC 21 Z9 21 U1 6 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 27 PY 2014 VL 136 IS 34 BP 11980 EP 11993 DI 10.1021/ja504528n PG 14 WC Chemistry, Multidisciplinary SC Chemistry GA AO0IX UT WOS:000340993400027 PM 24937106 ER PT J AU Hadler, AB Yannello, VJ Bi, WL Alp, EE Fredrickson, DC AF Hadler, Amelia B. Yannello, Vincent J. Bi, Wenli Alp, E. Ercan Fredrickson, Daniel C. TI pi-Conjugation in Gd13Fe10C13 and Its Oxycarbide: Unexpected Connections between Complex Carbides and Simple Organic Molecules SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRANSITION-METAL CARBIDES; ALUMINUM-SILICON OXYCARBIDE; INITIO STRUCTURE SOLUTION; TERNARY RARE-EARTH; CRYSTAL-STRUCTURE; MAGNETIC-PROPERTIES; SOLID-STATE; STRUCTURAL-CHARACTERIZATION; ORGANOMETALLIC POLYMER; CHEMICAL FRUSTRATION AB Carbometalates are a diverse family of solid state structures formed from transition metal (TM)-carbon polyanionic frameworks whose charges are balanced by rare earth (RE) cations. Remarkable structural features, such as transition metal clusters, are often encountered in these phases, and a pressing challenge is to explain how such features emerge from the competing interaction types (RE-M, TM-TM, TM-C, etc.) in these systems. In this Article, we describe a joint experimental and theoretical investigation of two compounds, Gd13Fe10C13 and its oxycarbide Gd13Fe10C13-xOx (x approximate to 1), which add a new dimension to the structural chemistry of carbometalates: pi-conjugation through both TM-C and TM-TM multiple bonds. The crystal structures of both compounds are built from layers of Fe-centered Gd prisms stacked along c and surrounded by an Fe-C network, and differ chiefly in the stacking sequence of these layers. The phases' identical local structures have two types of Fe environment: trigonal planar FeC3 sites and H-shaped Fe2C4 sites, with unusually short Fe-Fe and Fe-C bonds. Fe-57 Mossbauer spectroscopy and DFT-calibrated Huckel calculations on Gd13Fe10C13 build a picture of covalent Fe-C sigma bonds and conjugated pi systems for which Lewis structures can be drawn. Using the reversed approximation Molecular Orbital approach, we can draw isolobal analogies between the Fe centers of this compound and molecular TM complexes: 18-electron configurations could be achieved through sigma and pi bonds with 18 electrons/Fe for the FeC3 site and 18-n (n = 2 for an Fe=Fe double bond) electrons/Fe for the Fe2C4 site. In this way, the vision of a unified bonding scheme of carbometalates and organometallics proffered by earlier studies is realized in a visual manner, directly from the 1-electron wave functions of the Huckel model. The bonding analysis predicts that Gd13Fe10C13 is one electron/formula unit short of an ideal electron count, explaining the tendency of the system toward a small degree of oxygen substitution. Analogies between the pi bonding in Gd13Fe10C13 and that of the allyl anion help rationalize the presence of trigonal planar Fe and linear C units in the structure. The isolobal analogy between Gd13Fe10C13 and an 18-electron coordination complex is expected to apply to carbometalates as a whole, and will be extended to other examples in our future work. C1 [Hadler, Amelia B.; Yannello, Vincent J.; Fredrickson, Daniel C.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Bi, Wenli; Alp, E. Ercan] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Fredrickson, DC (reprint author), Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53706 USA. EM danny@chem.wisc.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Department of Energy Office of Science Early Career Research Program through the Office of Basic Energy Sciences [DE-SC0003947] FX We thank Dr. Chris Ceccarelli at Agilent Technologies for collecting a data set on Gd13Fe10C13-xOx using an Agilent Super Nova A diffractometer. We thank Prof. John Berry for useful discussions about metal-metal and metal-carbon bonding and Mossbauer spectroscopy. Prof. Huifang Xu and Dr. John Fournelle of the UW-Madison Department of Geoscience provided assistance with the powder X-ray diffraction measurements on the Rigaku Rapid II instrument and the SEM/EDS measurements, respectively. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We gratefully acknowledge financial support from the Department of Energy Office of Science Early Career Research Program (DE-SC0003947), through the Office of Basic Energy Sciences. NR 66 TC 5 Z9 5 U1 4 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 27 PY 2014 VL 136 IS 34 BP 12073 EP 12084 DI 10.1021/ja505868w PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA AO0IX UT WOS:000340993400038 PM 25093267 ER PT J AU Kapelewski, MT Geier, SJ Hudson, MR Stuck, D Mason, JA Nelson, JN Xiao, DJ Hulvey, Z Gilmour, E FitzGerald, SA Head-Gordon, M Brown, CM Long, JR AF Kapelewski, Matthew T. Geier, Stephen J. Hudson, Matthew R. Stueck, David Mason, Jarad A. Nelson, Jocienne N. Xiao, Dianne J. Hulvey, Zeric Gilmour, Elizabeth FitzGerald, Stephen A. Head-Gordon, Martin Brown, Craig M. Long, Jeffrey R. TI M-2(m-dobdc) (M = Mg, Mn, Fe, Co, Ni) Metal-Organic Frameworks Exhibiting Increased Charge Density and Enhanced H-2 Binding at the Open Metal Sites SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IRON(II) COORDINATION SITES; CARBON-DIOXIDE CAPTURE; HYDROGEN-STORAGE; METHANE STORAGE; FUNCTIONAL THEORY; ROOM-TEMPERATURE; HIGH-CAPACITY; HYDROCARBON SEPARATIONS; GAS-ADSORPTION; SPECTROSCOPY AB The well-known frameworks of the type M-2(dobdc) (dobdc(4-) = 2,5-dioxido-1,4-benzenedicarboxylate) have numerous potential applications in gas storage and separations, owing to their exceptionally high concentration of coordinatively unsaturated metal surface sites, which can interact strongly with small gas molecules such as H-2 center dot Employing a related meta-functionalized linker that is readily obtained from resorcinol, we now report a family of structural isomers of this framework, M-2(m-dobdc) (M = Mg, Mn, Fe, Co, Ni; m-dobdc(4-) = 4,6-dioxido-1,3-benzenedicarboxylate), featuring exposed M-2 cation sites with a higher apparent charge density. The regioisomeric linker alters the symmetry of the ligand field at the metal sites, leading to increases of 0.4-1.5 kJ/mol in the H-2 binding enthalpies relative to M-2(dobdc). A variety of techniques, including powder X-ray and neutron diffraction, inelastic neutron scattering, infrared spectroscopy, and first-principles electronic structure calculations, are applied in elucidating how these subtle structural and electronic differences give rise to such increases. Importantly, similar enhancements can be anticipated for the gas storage and separation properties of this new family of robust and potentially inexpensive metal-organic frameworks. C1 [Kapelewski, Matthew T.; Geier, Stephen J.; Stueck, David; Mason, Jarad A.; Xiao, Dianne J.; Head-Gordon, Martin; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hudson, Matthew R.; Hulvey, Zeric; Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Nelson, Jocienne N.; Gilmour, Elizabeth; FitzGerald, Stephen A.] Oberlin Coll, Dept Phys, Oberlin, OH 44074 USA. [Hulvey, Zeric] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Brown, Craig M.] Univ Delaware, Newark, DE 19716 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu RI Brown, Craig/B-5430-2009 OI Brown, Craig/0000-0002-9637-9355 FU Department of Energy, Office of Energy Efficiency and Renewable Energy (DOE-EERE), Fuel Cell Technologies Office and through the Department of Energy, Office of Science Graduate Fellowship Program (DOE SCGF); ORISE-ORAU [DE-AC05-06OR23100]; NSF [CHE-1111896]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF; Camille and Henry Dreyfus Postdoctoral Program in Environmental Chemistry; NSERC of Canada; NIST National Research Council FX Research at Berkeley and NIST was supported through the Department of Energy, Office of Energy Efficiency and Renewable Energy (DOE-EERE), Fuel Cell Technologies Office and through the Department of Energy, Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under contract no. DE-AC05-06OR23100. Efforts at Oberlin College were funded through NSF Grant CHE-1111896. We thank the 11-BM staff at the Advanced Photon Source at Argonne National Laboratory for assisting with powder X-ray diffraction experiments. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. We thank the NSF for providing graduate fellowship support for J.A.M. and M.T.K., the Camille and Henry Dreyfus Postdoctoral Program in Environmental Chemistry and the NSERC of Canada for fellowship support of S.J.G., and the NIST National Research Council for a Postdoctoral Fellowship award to M.R.H. In addition, we are grateful to Dr. Greg Haider for help with the diffraction data collection on 17-BM-B at the APS, Dr. Trudy Bolin for the use of the helium glovebox in APS Sector 9, Paul Horn for assistance with the energy decomposition analysis, and Eric Bloch and Rebecca Triano for helpful discussions. NR 95 TC 39 Z9 40 U1 13 U2 160 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 27 PY 2014 VL 136 IS 34 BP 12119 EP 12129 DI 10.1021/ja506230r PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA AO0IX UT WOS:000340993400043 PM 25130365 ER PT J AU Shirokov, AM Negoita, AG Vary, JP Bogner, SK Mazur, AI Mazur, EA Gogny, D AF Shirokov, A. M. Negoita, A. G. Vary, J. P. Bogner, S. K. Mazur, A. I. Mazur, E. A. Gogny, D. TI Properties of nuclear matter within the JISP16 N N interaction SO PHYSICAL REVIEW C LA English DT Article ID LOW-MOMENTUM INTERACTIONS; EQUATION-OF-STATE; BINDING-ENERGY; PARTIAL-WAVES; LIGHT-NUCLEI; SPECTROSCOPY; POTENTIALS AB Saturation properties of the JISP16 N N interaction are studied in symmetric nuclear matter calculations, with special attention paid to the convergence properties with respect to the number of partial waves. We also present results of pure neutron matter calculations with the JISP16 interaction. C1 [Shirokov, A. M.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. [Shirokov, A. M.; Negoita, A. G.; Vary, J. P.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Shirokov, A. M.; Mazur, A. I.; Mazur, E. A.] Pacific Natl Univ, Khabarovsk 680035, Russia. [Negoita, A. G.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 76900, Romania. [Bogner, S. K.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48844 USA. [Bogner, S. K.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Gogny, D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Shirokov, AM (reprint author), Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. RI Shirokov, Andrey/D-7054-2012 FU US DOE [DE-FG02-87ER40371, DE-AC52-07NA27344, DESC0008485]; US National Science Foundation [PHY-0758125, PHY-1068648, PHY 0904782]; Ministry of Education and Science of the Russian Federation [P521, 14.V37.21.1297] FX We gratefully acknowledge discussions with Fritz Coester. This work was supported by the US DOE Grant Nos. DE-FG02-87ER40371, DE-AC52-07NA27344 and DESC0008485 (SciDAC-3/NUCLEI), by the US National Science Foundation under Grant Nos. PHY-0758125, PHY-1068648 and PHY 0904782, and by the Ministry of Education and Science of the Russian Federation under Contract Nos. P521 and 14.V37.21.1297. NR 40 TC 3 Z9 3 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 27 PY 2014 VL 90 IS 2 AR 024324 DI 10.1103/PhysRevC.90.024324 PG 5 WC Physics, Nuclear SC Physics GA AO3UK UT WOS:000341261400001 ER PT J AU Wang, SQ Wu, XG Brodsky, SJ AF Wang, Sheng-Quan Wu, Xing-Gang Brodsky, Stanley J. TI Reanalysis of the higher order perturbative QCD corrections to hadronic Z decays using the principle of maximum conformality SO PHYSICAL REVIEW D LA English DT Article ID SCALE AB A complete calculation of the O(alpha(4)(s)) perturbative quantum chromodynamics (pQCD) corrections to the hadronic decay width of the Z boson has recently been performed by Baikov et al. [Phys. Rev. Lett. 108, 222003 (2012)]. In their analysis, Baikov et al. relied on the conventional practice of simply guessing the renormalization scale and taking an arbitrary range to estimate the pQCD uncertainties. This procedure inevitably introduces an arbitrary, scheme-dependent theoretical systematic error in the predictions. In this paper, we show that the renormalization scale uncertainties for hadronic Z decays can be greatly reduced by applying the principle of maximum conformality (PMC), a rigorous extension of the Brodsky-Lepage-Mackenzie method. The PMC prediction is independent of the choice of renormalization scheme; i.e., it respects renormalization group invariance, and thus it provides an optimal and theoretically rigorous method for setting the renormalization scale. We show that the convergence of the pQCD prediction for the Z hadronic width is greatly improved using the PMC since the divergent renormalon series does not appear. The magnitude of the high-order corrections quickly approach a steady point. The PMC predictions also have the property that any residual dependence on the choice of initial scale is highly suppressed, even for low-order predictions. Thus, one obtains optimal fixed-order predictions for the Z-boson hadronic decay rates thus enabling high precision tests of the Standard Model. C1 [Wang, Sheng-Quan; Wu, Xing-Gang] Chongqing Univ, Dept Phys, Chongqing 401331, Peoples R China. [Brodsky, Stanley J.] Stanford Univ, Stanford Linear Accelerator Ctr, Natl Accelerator Lab, Stanford, CA 94309 USA. RP Wang, SQ (reprint author), Chongqing Univ, Dept Phys, Chongqing 401331, Peoples R China. EM sqwang@cqu.edu.cn; wuxg@cqu.edu.cn; sjbth@slac.stanford.edu RI wu, xing-gang/F-2096-2011 OI wu, xing-gang/0000-0002-7343-1907 FU Natural Science Foundation of China [11275280]; Fundamental Research Funds for the Central Universities [CQDXWL-2012-Z002]; Department of Energy [DE-AC02-76SF00515] FX This work was supported in part by Natural Science Foundation of China under Grant No. 11275280, the Fundamental Research Funds for the Central Universities under Grant No. CQDXWL-2012-Z002, and the Department of Energy Contract No. DE-AC02-76SF00515. NR 18 TC 13 Z9 13 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 27 PY 2014 VL 90 IS 3 AR 037503 DI 10.1103/PhysRevD.90.037503 PG 4 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO3VF UT WOS:000341263800003 ER PT J AU Khare, A Christov, IC Saxena, A AF Khare, Avinash Christov, Ivan C. Saxena, Avadh TI Successive phase transitions and kink solutions in phi(8), phi(10), and phi(12) field theories SO PHYSICAL REVIEW E LA English DT Article ID STATISTICAL-MECHANICS; MODEL; POTENTIALS; DYNAMICS; EQUATION; WAVES AB We obtain exact solutions for kinks in phi(8), phi(10), and phi(12) field theories with degenerate minima, which can describe a second-order phase transition followed by a first-order one, a succession of two first-order phase transitions and a second-order phase transition followed by two first-order phase transitions, respectively. Such phase transitions are known to occur in ferroelastic and ferroelectric crystals and in meson physics. In particular, we find that the higher-order field theories have kink solutions with algebraically decaying tails and also asymmetric cases with mixed exponential-algebraic tail decay, unlike the lower-order phi(4) and phi(6) theories. Additionally, we construct distinct kinks with equal energies in all three field theories considered, and we show the coexistence of up to three distinct kinks (for a phi(12) potential with six degenerate minima). We also summarize phonon dispersion relations for these systems, showing that the higher-order field theories have specific cases in which only nonlinear phonons are allowed. For the phi(10) field theory, which is a quasiexactly solvable model akin to phi(6), we are also able to obtain three analytical solutions for the classical free energy as well as the probability distribution function in the thermodynamic limit. C1 [Khare, Avinash] Indian Inst Sci Educ & Res, Pune 411021, Maharashtra, India. [Christov, Ivan C.; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Christov, Ivan C.; Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Khare, A (reprint author), Indian Inst Sci Educ & Res, Pune 411021, Maharashtra, India. EM khare@iiserpune.ac.in; christov@lanl.gov; avadh@lanl.gov RI Christov, Ivan/B-9418-2008 OI Christov, Ivan/0000-0001-8531-0531 FU U.S. Department of Energy through the LANL/LDRD Program; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX A. K. acknowledges the hospitality of the Center for Nonlinear Studies and the Theoretical Division at LANL. We gratefully acknowledge the support of the U.S. Department of Energy through the LANL/LDRD Program for this work, specifically a Richard P. Feynman fellowship to I. C. C. LANL is operated by Los Alamos National Security, L. L. C., for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 43 TC 4 Z9 4 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD AUG 27 PY 2014 VL 90 IS 2 AR 023208 DI 10.1103/PhysRevE.90.023208 PG 23 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AO3WG UT WOS:000341267000012 PM 25215844 ER PT J AU Borysov, SS Balatsky, AV AF Borysov, Stanislav S. Balatsky, Alexander V. TI Cross-Correlation Asymmetries and Causal Relationships between Stock and Market Risk SO PLOS ONE LA English DT Article ID FINANCIAL-MARKETS; EQUITY MARKETS; TIME-SERIES; VOLATILITY; FLUCTUATIONS; NETWORKS; GRAPHS; TREES AB We study historical correlations and lead-lag relationships between individual stock risk (volatility of daily stock returns) and market risk (volatility of daily returns of a market-representative portfolio) in the US stock market. We consider the cross-correlation functions averaged over all stocks, using 71 stock prices from the Standard & Poor's 500 index for 1994-2013. We focus on the behavior of the cross-correlations at the times of financial crises with significant jumps of market volatility. The observed historical dynamics showed that the dependence between the risks was almost linear during the US stock market downturn of 2002 and after the US housing bubble in 2007, remaining at that level until 2013. Moreover, the averaged cross-correlation function often had an asymmetric shape with respect to zero lag in the periods of high correlation. We develop the analysis by the application of the linear response formalism to study underlying causal relations. The calculated response functions suggest the presence of characteristic regimes near financial crashes, when the volatility of an individual stock follows the market volatility and vice versa. C1 [Borysov, Stanislav S.; Balatsky, Alexander V.] KTH Royal Inst Technol, NORDITA, Stockholm, Sweden. [Borysov, Stanislav S.; Balatsky, Alexander V.] Stockholm Univ, S-10691 Stockholm, Sweden. [Borysov, Stanislav S.] KTH Royal Inst Technol, Stockholm, Sweden. [Borysov, Stanislav S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM USA. RP Borysov, SS (reprint author), KTH Royal Inst Technol, NORDITA, Stockholm, Sweden. EM borysov@kth.se FU Swedish Research Council [VR VCB 621-2012-2983] FX The host institution was Nordita, http://www.nordita.org/. This work was supported by Swedish Research Council grant VR VCB 621-2012-2983, http://www.vr.se/. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 64 TC 3 Z9 3 U1 1 U2 14 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 27 PY 2014 VL 9 IS 8 AR e105874 DI 10.1371/journal.pone.0105874 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN8UR UT WOS:000340880900055 PM 25162697 ER PT J AU Liu, SY Akbashev, AR Yang, XH Liu, XH Li, WL Zhao, L Li, X Couzis, A Han, MG Zhu, YM Krusin-Elbaum, L Li, J Huang, LM Billinge, SJL Spanier, JE O'Brien, S AF Liu, Shuangyi Akbashev, Andrew R. Yang, Xiaohao Liu, Xiaohua Li, Wanlu Zhao, Lukas Li, Xue Couzis, Alexander Han, Myung-Geun Zhu, Yimei Krusin-Elbaum, Lia Li, Jackie Huang, Limin Billinge, Simon J. L. Spanier, Jonathan E. O'Brien, Stephen TI Hollandites as a new class of multiferroics SO SCIENTIFIC REPORTS LA English DT Article ID ROOM-TEMPERATURE; THIN-FILMS; METAL-OXIDES; PEROVSKITE; FERROELECTRICITY; NANOPARTICLES AB Discovery of new complex oxides that exhibit both magnetic and ferroelectric properties is of great interest for the design of functional magnetoelectrics, in which research is driven by the technologically exciting prospect of controlling charges by magnetic fields and spins by applied voltages, for sensors, 4-state logic, and spintronics. Motivated by the notion of a tool-kit for complex oxide design, we developed a chemical synthesis strategy for single-phase multifunctional lattices. Here, we introduce a new class of multiferroic hollandite Ba-Mn-Ti oxides not apparent in nature. BaMn3Ti4O14.25, designated BMT-134, possesses the signature channel-like hollandite structure, contains Mn4+ and Mn3+ in a 1 : 1 ratio, exhibits an antiferromagnetic phase transition (T-N similar to 120 K) with a weak ferromagnetic ordering at lower temperatures, ferroelectricity, a giant dielectric constant at low frequency and a stable intrinsic dielectric constant of similar to 200 (1-100 MHz). With evidence of correlated antiferromagnetic and ferroelectric order, the findings point to an unexplored family of structures belonging to the hollandite supergroup with multifunctional properties, and high potential for developing new magnetoelectric materials. C1 [Liu, Shuangyi; Liu, Xiaohua; Li, Wanlu; Huang, Limin; O'Brien, Stephen] CUNY City Coll, Dept Chem, New York, NY 10031 USA. [Akbashev, Andrew R.; Spanier, Jonathan E.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Yang, Xiaohao; Billinge, Simon J. L.] Columbia Univ, Fu Fdn Sch Engn & Appl Sci, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Zhao, Lukas; Krusin-Elbaum, Lia] CUNY City Coll, Dept Phys, New York, NY 10031 USA. [Li, Xue; Couzis, Alexander] CUNY City Coll, Grove Sch Engn, Dept Chem Engn, New York, NY 10031 USA. [Han, Myung-Geun; Zhu, Yimei; Billinge, Simon J. L.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Li, Jackie] CUNY City Coll, Grove Sch Engn, Dept Engn Mech, New York, NY 10031 USA. [Huang, Limin] South Univ Sci & Technol China, Dept Chem, Shenzhen 518500, Peoples R China. [Spanier, Jonathan E.] Drexel Univ, AJ Drexel Inst Energy & Environm, Philadelphia, PA 19104 USA. [Liu, Shuangyi; Couzis, Alexander; O'Brien, Stephen] CUNY City Coll, Energy Inst, New York, NY 10031 USA. RP O'Brien, S (reprint author), CUNY City Coll, Dept Chem, Marshak Bldg,160 Convent Ave, New York, NY 10031 USA. EM sobrien@ccny.cuny.edu RI O'Brien, Stephen/D-7682-2013; Huang, Limin/J-6211-2014; Akbashev, Andrew/A-7533-2010; OI Spanier, Jonathan/0000-0002-3096-2644 FU Advanced Research Project Agency for Energy (ARPA-e), ADEPT [DE-AR0000114]; National Science Foundation under NSF IDR [1014777]; NSF MIRT [1122594]; Center for Exploitation of Nanostructures in Sensors and Energy Systems under NSF [0833180]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (U.S. DOE-BES) [DE-AC02-98CH10886]; Energy Frontier Research Center (EFRC) - U.S. DOE-BES [DE-SC0001085]; U.S. Army Research Office [W911NF-08-1-0067]; NSF/SRC [DMR 1124696] FX This work was supported by the Advanced Research Project Agency for Energy (ARPA-e), ADEPT DE-AR0000114, and the National Science Foundation under award NSF IDR #1014777. Support is also acknowledged from NSF MIRT #1122594 and the Center for Exploitation of Nanostructures in Sensors and Energy Systems under NSF Cooperative Agreement #0833180. Microscopy work at BNL and use of the National Synchrotron Light Source, Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (U.S. DOE-BES), under Contract No. DE-AC02-98CH10886. X-ray analysis at Columbia University was supported as part of the Energy Frontier Research Center (EFRC) funded by the U.S. DOE-BES under Award Number DE-SC0001085. J.E.S. acknowledges support from the U.S. Army Research Office (W911NF-08-1-0067) and the NSF/SRC-sponsored Nanoelectronics in 2020 and Beyond Program (DMR 1124696). NR 58 TC 10 Z9 10 U1 3 U2 99 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 27 PY 2014 VL 4 AR 6203 DI 10.1038/srep06203 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN9NN UT WOS:000340933700001 PM 25160888 ER PT J AU Agrawal, P Chacko, Z Verhaaren, C AF Agrawal, Prateek Chacko, Zackaria Verhaaren, Christopher B. TI Leptophilic dark matter and the anomalous magnetic moment of the muon SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Phenomenological Models ID ELECTRON-BEAM-DUMP; ELECTROMAGNETIC PROPERTIES; MAJORANA NEUTRINOS; PARTICLES; CONSTRAINTS; SEARCH; MASSES; ANNIHILATION; MODEL; G-2 AB We consider renormalizable theories such that the scattering of dark matter off leptons arises at tree level, but scattering off nuclei only arises at loop. In this framework, the various dark matter candidates can be classified by their spins and by the forms of their interactions with leptons. We determine the corrections to the anomalous magnetic moment of the muon that arise from its interactions with dark matter. We then consider the implications of these results for a set of simplified models of leptophilic dark matter. When a dark matter candidate reduces the existing tension between the standard model prediction of the anomalous magnetic moment and the experimental measurement, the region of parameter space favored to completely remove the discrepancy is highlighted. Conversely, when agreement is worsened, we place limits on the parameters of the corresponding simplified model. These bounds and favored regions are compared against the experimental constraints on the simplified model from direct detection and from collider searches. Although these constraints are severe, we find there do exist limited regions of parameter space in these simple theories that can explain the observed anomaly in the muon magnetic moment while remaining consistent with all experimental bounds. C1 [Agrawal, Prateek] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Chacko, Zackaria; Verhaaren, Christopher B.] Univ Maryland, Dept Phys, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. RP Agrawal, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM prateek@fnal.gov; zchacko@umd.edu; cver@umd.edu OI Agrawal, Prateek/0000-0001-9947-0632; Verhaaren, Christopher/0000-0001-6798-804X FU National Science Foundation [PHYS-1066293, PHY-0968854]; Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy FX We would like to thank Brian Batell, Patrick Fox, Brian Hamilton and Samuel McDermott for useful discussions. PA would like to acknowledge support by the National Science Foundation under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics, where a part of this work was completed. ZC and CV are supported by the NSF grant PHY-0968854. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 114 TC 21 Z9 21 U1 1 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 26 PY 2014 IS 8 AR 147 DI 10.1007/JHEP08(2014)147 PG 37 WC Physics, Particles & Fields SC Physics GA AO6CO UT WOS:000341436300001 ER PT J AU Satow, D AF Satow, Daisuke TI Nonlinear electromagnetic response in quark-gluon plasma SO PHYSICAL REVIEW D LA English DT Article ID STRONG MAGNETIC-FIELD; HEAVY-ION COLLISIONS; HOT GAUGE-THEORIES; HARD THERMAL LOOPS; ELECTRICAL-CONDUCTIVITY; HIGH-TEMPERATURE; DAMPING RATE; QCD PLASMA; EXCITATIONS; AMPLITUDES AB We perform the first systematic study of the nonlinear electromagnetic currents induced by the external electromagnetic field in quark-gluon plasma, in cases where the inhomogeneity of the electromagnetic field is small (large) so that the collision effect is important (negligible). In the former case, we list and classify possible components of the currents in a systematic way and make an order estimate of each component by using the Boltzmann equation in the relaxation time approximation. In the latter case, we explicitly calculate the quadratic current by using the Vlasov equation, and we find that the current generated by the chiral magnetic effect and the quadratic current can have the same order of magnitude by using the Kadanoff-Baym equation. We also demonstrate this property by using a possible configuration of the electromagnetic field realized in a heavy ion collision. C1 [Satow, Daisuke] RIKEN, Nishina Ctr, Theoret Res Div, Wako, Saitama 3510198, Japan. [Satow, Daisuke] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Satow, D (reprint author), RIKEN, Nishina Ctr, Theoret Res Div, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. EM daisuke.sato@riken.jp OI satow, daisuke/0000-0003-4398-1606 FU JSPS Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation [R2411] FX The author thanks M. Hongo, D. Kharzeev, J. Liao, L. Mclerran, and A. Monnai for inspiring and fruitful discussions. He is indebted to N. Yamamoto for collaboration in the beginning of this project and for the valuable comments. He is supported by the JSPS Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation (Grant No. R2411). NR 65 TC 4 Z9 4 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 26 PY 2014 VL 90 IS 3 AR 034018 DI 10.1103/PhysRevD.90.034018 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO4IM UT WOS:000341300700002 ER PT J AU Wu, QL Liu, YZ Johnson, CS Li, YX Dees, DW Lu, WQ AF Wu, Qingliu Liu, Yuzi Johnson, Christopher S. Li, Yangxing Dees, Dennis W. Lu, Wenquan TI Insight into the Structural Evolution of a High-Voltage Spinel for Lithium-Ion Batteries SO CHEMISTRY OF MATERIALS LA English DT Article ID OXYGEN VACANCIES; LINI0.5MN1.5O4; CATHODES; LIMN1.5NI0.5O4; ELECTRODE; PERFORMANCE; P4(3)32; OXIDES AB With a high operating voltage and three-dimensional lithium (Li)-ion diffusion pathways, LixNi0.5Mn1.5O4 (high-voltage [HV] spinel) is considered to be a promising high-energy and high-power density cathode material for Li-ion batteries. Here, we extensively investigate the structural dependence of the spinel cathode on the stoichiometry of the cation/anion ratio through an unprecedented overstoichiometric Li intercalation. This material undergoes the well-known cubic phase transition with one Li insertion from a fully delithiated state. The further overstoichiometric Li intercalation results in a cubic-to-tetragonal phase transition when x reaches 3. When x is electrochemically pushed to similar to 4, the coexistence of a rock-salt structure with a layered component is observed. The parent spinel structure is reformed upon complete deintercalation. This reversibility underscores the fact that the HV spinel has a distinct memory of its original form. The resultant phases and morphologies are identified by X-ray diffraction (XRD) and microscopy methods. C1 [Wu, Qingliu; Johnson, Christopher S.; Dees, Dennis W.; Lu, Wenquan] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Liu, Yuzi] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Li, Yangxing] FMC Corp, Lithium Div, Bessemer City, NC 28016 USA. RP Lu, WQ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM luw@anl.gov RI Liu, Yuzi/C-6849-2011 FU DOE SC [DE-AC02-06CH11357] FX Support from David Howell and Peter Faguy of the U.S. Department of Energy's (DOE) Office of Energy Efficiency & Renewable Energy (EERE) Vehicle Technologies Office is gratefully acknowledged. This work was performed, in part, at the Electron Microscopy Center for Materials Research, the Center for Nanoscale Materials, and the Advanced Photon Source, facilities of the Office of Science (SC), Basic Energy Sciences, and Office of Science User Facilities operated for DOE SC by Argonne National Laboratory under contract no. DE-AC02-06CH11357. We would like to thank Drs. Chikai Lin, Zonghai Chen, and Yang Ren for XRD data collection. A valuable discussion with Dr. Michael Thackeray is also acknowledged. NR 22 TC 8 Z9 8 U1 5 U2 106 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 26 PY 2014 VL 26 IS 16 BP 4750 EP 4756 DI 10.1021/cm5015288 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AO0IS UT WOS:000340992900011 ER PT J AU Peng, HW Perkins, JD Lany, S AF Peng, Haowei Perkins, John D. Lany, Stephan TI Multivalency of Group 15 Dopants in SnO2 SO CHEMISTRY OF MATERIALS LA English DT Article ID AUGMENTED-WAVE METHOD; THIN-FILMS; LONE-PAIR; MOSSBAUER-SPECTROSCOPY; ELECTRICAL-PROPERTIES; SMALL POLARONS; OXIDE; POLARIZATION; DEPOSITION; ENERGY AB The multivalent behavior of group 15 elements P, As, Sb, and Bi, on the cation site in SnO2 has been studied via first-principles calculations. Through accurate calculation of the energy position of the defect transition energy levels with respect to the host conduction band minimum using a combination of hybrid functional and GW calculations, we found that As and Bi will change their oxidation state from +5 to +3 when the Fermi level approaches the conduction band minimum, while P and Sb will stay in the +5 state until the Fermi level rises to an energy well above the conduction band minimum The change of the oxidation state is associated with the occupation of an electron-compensating defect state resulting from the antibonding s-p hybridization between the group 15 dopant and the ligands. Thus, only P and Sb are good electron-dopants (donors). As is a borderline case allowing only limited n-type doping, whereas Bi is a deep defect that pins the Fermi level within the band gap and causes insulating behavior. We discuss the chemical trends with the atomic energy of the valence s state and the ionic radii of the dopants. C1 [Peng, Haowei; Perkins, John D.; Lany, Stephan] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Peng, HW (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Haowei.Peng@nrel.gov; Stephan.Lany@nrel.gov RI Peng, Haowei/K-4654-2012; OI Peng, Haowei/0000-0002-6502-8288; Lany, Stephan/0000-0002-8127-8885 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, (SunShot initiative) [DE-AC36-08GO28308] FX This work was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, (SunShot initiative), under Contract No. DE-AC36-08GO28308 to NREL. The high performance computing resources of the National Energy Research Scientific Computing Center and of NREL's Computational Science Center are gratefully acknowledged. NR 50 TC 3 Z9 3 U1 1 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 26 PY 2014 VL 26 IS 16 BP 4876 EP 4881 DI 10.1021/cm502411g PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AO0IS UT WOS:000340992900027 ER PT J AU Johnson, MA Seifert, S Petrache, HI Kimbe-Hill, AC AF Johnson, Merrell A. Seifert, Soenke Petrache, Horia I. Kimbe-Hill, Ann C. TI Phase Coexistence in Single-Lipid Membranes Induced by Buffering Agents SO LANGMUIR LA English DT Article ID BILAYERS; PROTEINS; SALT; PHOSPHOLIPIDS; STABILIZATION; SEPARATION; REPULSION; OSMOLYTES AB Recent literature has shown that buffers affect the interaction between lipid bilayers through a mechanism that involves van der Waals forces, electrostatics, hydration forces and membrane bending rigidity. This letter shows an additional peculiar effect of buffers on the mixed chain 1-palmitoyl-2-oleoyl-sn-glycero-3-phosphocholine (POPC) lipid bilayers, namely phase coexistence similar to what was reported by Rappolt et al. for alkali chlorides. The data presented suggest that one phase appears to dehydrate below the value in pure water, while the other phase swells as the concentration of buffer is increased. However, since the two phases must be in osmotic equilibrium with one another, this behavior challenges theoretical models of lipid interactions. C1 [Johnson, Merrell A.; Petrache, Horia I.] Indiana Univ Purdue Univ, Dept Phys, Indianapolis, IN 46202 USA. [Seifert, Soenke] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Kimbe-Hill, Ann C.] Indiana Univ Sch Med, Dept Biochem & Mol Biol, Indianapolis, IN 46202 USA. RP Kimbe-Hill, AC (reprint author), Indiana Univ Sch Med, Dept Biochem & Mol Biol, MS 4053,635 Barnhill Dr, Indianapolis, IN 46202 USA. EM ankimble@umail.iu.edu FU U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357]; National Institutes of Health [K01-CA169078-01]; Indiana University FX Results shown in this Letter are derived from work performed at Argonne National Laboratory, X-ray Science Division at the Advanced Photon Source. Argonne is operated by UChicago Argonne, LLC, for the U.S. Department of Energy, Office of Biological and Environmental Research under Contract DE-AC02-06CH11357. The authors would like to thank Dr. Bruce Ray for discussion regarding the protonation state of buffers used in this study. This work was supported, in whole or in part, by National Institutes of Health Grants K01-CA169078-01 (to A.K.H.) and Indiana University Collaborative Research Grants (to H.I.P.). NR 34 TC 3 Z9 3 U1 1 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD AUG 26 PY 2014 VL 30 IS 33 BP 9880 EP 9885 DI 10.1021/la5018938 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AO0IV UT WOS:000340993200002 PM 25102340 ER PT J AU Legg, BA Zhu, MQ Comolli, LR Gilbert, B Banfield, JF AF Legg, Benjamin A. Zhu, Mengqiang Comolli, Luis R. Gilbert, Benjamin Banfield, Jillian F. TI Determination of the Three-Dimensional Structure of Ferrihydrite Nanoparticle Aggregates SO LANGMUIR LA English DT Article ID FRACTAL DIMENSION; SYSTEMS; TRANSFORMATION; SCATTERING; GROWTH AB Aggregation impacts the reactivity, colloidal stability, and transport behavior of nanomaterials, yet methods to characterize basic structural features of aggregates are limited. Here, cryo-transmission electron microscope (cryo-TEM) based tomography is utilized as a method for directly imaging fragile aggregates of nanoparticles in aqueous suspension and an approach for extracting quantitative fractal dimensions from the resulting three-dimensional structural models is introduced. The structural quantification approach is based upon the mass autocorrelation function, and is directly comparable with small-angle X-ray scattering (SAXS) models. This enables accurate characterization of aggregate structure, even in suspensions where the aggregate cluster size is highly polydisperse and traditional SAXS modeling is not reliable. This technique is applied to study real suspensions of ferrihydrite nanoparticles. By comparing tomographic measurements with SAXS-based measurements, we infer that certain suspensions contain polydisperse aggregate size distributions. In other suspensions, fractal-type structures are identified with low intrinsic fractal dimensions. The fractal dimensions are lower than would be predicted by simple models of particle aggregation, and this low dimensionality enables large, low-density aggregates to exist in stable colloidal suspension. C1 [Legg, Benjamin A.; Banfield, Jillian F.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Zhu, Mengqiang; Gilbert, Benjamin; Banfield, Jillian F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Comolli, Luis R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Legg, BA (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. RI Gilbert, Benjamin/E-3182-2010 FU Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank Alexander Hexemer, Steven A. Alvarez, and Eric Schaible for the support with SAXS data acquisition. SAXS experiments were performed at the Advanced Light Source, a user facility at Lawrence Berkeley National Laboratory supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 33 TC 12 Z9 12 U1 7 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD AUG 26 PY 2014 VL 30 IS 33 BP 9931 EP 9940 DI 10.1021/la502128d PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AO0IV UT WOS:000340993200008 PM 25079430 ER PT J AU Melnichenko, YB Lavrik, NV Popov, E Bahadur, J He, L Kravchenko, II Smith, G Pipich, V Szekely, NK AF Melnichenko, Yuri B. Lavrik, N. V. Popov, E. Bahadur, J. He, L. Kravchenko, I. I. Smith, G. Pipich, V. Szekely, N. K. TI Cavitation on Deterministically Nanostructured Surfaces in Contact with an Aqueous Phase: A Small-Angle Neutron Scattering Study SO LANGMUIR LA English DT Article ID NUCLEATION SITE DENSITY; NANOPATTERNED SURFACES; CONDENSATION; SILICA; WATER AB The structure of deterministically nanopatterned surfaces created using a combination of electron beam lithography and reactive ion etching was evaluated using small-angle neutron scattering (SANS). Samples exhibit 2D neutron scattering patterns that confirm the presence of ordered nanoscale cavities consistent with the targeted morphologies as well as with SEM data analysis. Comparison of SANS intensities obtained from samples in air and in contact with an aqueous phase (pure deuterium oxide, D2O, or a contrast matched mixture of D2O + H2O) reveals formation of stable gaseous nanobubbles trapped inside the cavities. The relative volume of nanobubbles depends strongly on the hydrophobicity of the cavity walls. In the case of hydrophobic surfaces, nanobubbles occupy up to 87% of the total cavity volume. The results demonstrate the high degree of sensitivity of SANS measurements for detecting and characterizing nano- and mesoscale bubbles with the volume fraction as low as similar to 10(-6). C1 [Melnichenko, Yuri B.; Bahadur, J.; He, L.; Smith, G.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Lavrik, N. V.; Kravchenko, I. I.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Popov, E.] Oak Ridge Natl Lab, Reactor & Nucl Syst Div, Oak Ridge, TN 37831 USA. [Pipich, V.; Szekely, N. K.] Forschungszentrum Julich GmbH, JCNS, MLZ, D-85747 Garching, Germany. RP Melnichenko, YB (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. EM melnichenkoy@ornl.gov RI Kravchenko, Ivan/K-3022-2015; Szekely, Noemi Kinga/B-4315-2010; Lavrik, Nickolay/B-5268-2011; OI Kravchenko, Ivan/0000-0003-4999-5822; Szekely, Noemi Kinga/0000-0001-6125-4758; Lavrik, Nickolay/0000-0002-9543-5634; He, Lilin/0000-0002-9560-8101 FU Laboratory Directed Research and Development Program; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; ORNL; European Commission [283883] FX The research at Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Laboratory Directed Research and Development Program and the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Preparation of nanostructured surface was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This research was supported in part by the ORNL Postdoctoral Research Associates Program, administered jointly by the ORNL and the Oak Ridge Institute for Science and Education. This research project has been supported in part by the European Commission under the seventh Framework Programme through the 'Research Infrastructures' action of the 'Capacities' Programme, NMI3-II Grant number 283883. NR 30 TC 0 Z9 0 U1 2 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD AUG 26 PY 2014 VL 30 IS 33 BP 9985 EP 9990 DI 10.1021/la500963q PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AO0IV UT WOS:000340993200014 PM 25084807 ER PT J AU Wang, X Thelen, JL Teran, AA Chintapalli, M Nakamura, I Wang, ZG Newstein, MC Balsara, NP Garetz, BA AF Wang, Xin Thelen, Jacob L. Teran, Alexander A. Chintapalli, Mahati Nakamura, Issei Wang, Zhen-Gang Newstein, Maurice C. Balsara, Nitash P. Garetz, Bruce A. TI Evolution of Grain Structure during Disorder-to-Order Transitions in a Block Copolymer/Salt Mixture Studied by Depolarized Light Scattering SO MACROMOLECULES LA English DT Article ID MICROPHASE SEPARATION; PHASE-BEHAVIOR; POLYMER ELECTROLYTES; IONIC-CONDUCTIVITY; SALT; GROWTH; MELTS; THERMODYNAMICS; ORIENTATION; MORPHOLOGY AB Block copolymer/lithium salt mixtures are promising materials for lithium battery electrolytes. The growth of ordered lamellar grains after a block copolymer electrolyte was quenched from the disordered state to the ordered state was studied by depolarized light scattering. Three quench depths below the order-to-disorder transition temperature were studied: 6, 12, and 24 degrees C. Regardless of quench depth, elongated ellipsoidal grains with aspect ratios between six and eight were formed during the initial stage of order formation. This was followed by a rapid reduction in aspect ratio; at long times, isotropic grains with aspect ratios in the vicinity of unity were obtained. Unusual grain growth kinetics were observed at all quench depths: (1) The average grain volume decreased with time after the early stage of grain growth. To our knowledge, a decrease in grain size has never been observed before in any quenched block copolymer system. (2) The volume fraction occupied by ordered grains of the shallowest quenched sample (quench depth of 6 degrees C) was significantly less than unity even after waiting times approaching 400 min. This is consistent with recent theoretical and experimental work indicating the presence of a coexistence window between ordered and disordered phases due to the partitioning of the salt into the ordered domains. At quench depths of 12 and 24 degrees C, which are outside the coexistence window, the grain volume fraction increases monotonically with time, and ordered grains occupy the entire sample at long times. C1 [Wang, Xin; Garetz, Bruce A.] NYU Polytech Sch Engn, Dept Chem & Biomol Engn, Brooklyn, NY 11201 USA. [Thelen, Jacob L.; Teran, Alexander A.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Thelen, Jacob L.; Teran, Alexander A.; Chintapalli, Mahati; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Chintapalli, Mahati] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Nakamura, Issei; Wang, Zhen-Gang] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [Newstein, Maurice C.] NYU Polytech Sch Engn, Dept Elect & Comp Engn, Brooklyn, NY 11201 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Garetz, BA (reprint author), NYU Polytech Sch Engn, Dept Chem & Biomol Engn, Brooklyn, NY 11201 USA. EM bgaretz@nyu.edu FU National Science Foundation [DMR-0966626, DMR-0966765, CBET-0965812] FX The authors acknowledge the generous support of the National Science Foundation through Award Numbers DMR-0966626, DMR-0966765, and CBET-0965812. Any opinions, findings, and conclusions or recommendations expressed in this paper are those of the authors and do not necessarily reflect the views of the National Science Foundation. The assistance of Mr. Hao-Chun Chiang in solving some programming problems is also appreciated NR 40 TC 4 Z9 4 U1 3 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD AUG 26 PY 2014 VL 47 IS 16 BP 5784 EP 5792 DI 10.1021/ma501166p PG 9 WC Polymer Science SC Polymer Science GA AO0IQ UT WOS:000340992700037 ER PT J AU Zhang, Z Carrillo, JMY Ahn, SK Wu, B Hong, KL Smith, GS Do, C AF Zhang, Zhe Carrillo, Jan-Michael Y. Ahn, Suk-kyun Wu, Bin Hong, Kunlun Smith, Gregory S. Do, Changwoo TI Atomistic Structure of Bottlebrush Polymers: Simulations and Neutron Scattering Studies SO MACROMOLECULES LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; COARSE-GRAINED SIMULATIONS; POOR-SOLVENT CONDITIONS; SIDE-CHAIN LENGTH; BRUSH MACROMOLECULES; CYLINDRICAL BRUSHES; CONFORMATION; COPOLYMERS; SCALE; AMBER AB We have used small angle neutron scattering (SANS) measurement and atomistic molecular dynamics (MD) simulations to investigate the conformation of bottlebrush polymers with poly(norbornene) (PNB) backbone and different sizes of poly(lactide) (PLA) side chains (PNB25-g-PLA(5), PNB25-g-PLA(10), and PNB25-g-PLA(19)). At early stage of simulations, stretched side chains with visible spatial-correlations of about 30 angstrom were observed. The experimentally measured SANS data, on the other hand, does not exhibit any correlation peaks in the corresponding length scale indicating a compact form rather than a stretched-hairy polymer conformation. As the simulation continued, the spatial correlations between side chains disappeared after about 40 ns of chain relaxation, and the scattering intensity calculated for the simulated structure becomes reasonably close to the measured one. Statistical approach is used to overcome the time scale limitation and search for optimal conformation space, which also provides a good agreement with the experimental data. Further coarse-grained simulation results suggest that the side chain conformation strongly depends on the solubility competition among side chain, backbone, and solvent. Significant changes of backbone dynamics due to the side chain encapsulation have been revealed and discussed. C1 [Zhang, Zhe; Smith, Gregory S.; Do, Changwoo] Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Carrillo, Jan-Michael Y.] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Ahn, Suk-kyun; Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Wu, Bin] Univ Tennessee, Joint Inst Neutron Sci, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Do, C (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. EM doc1@ornl.gov RI Zhang, Zhe/J-9434-2014; Carrillo, Jan-Michael/K-7170-2013; Hong, Kunlun/E-9787-2015; Smith, Gregory/D-1659-2016; Do, Changwoo/A-9670-2011 OI Zhang, Zhe/0000-0002-1952-5726; Carrillo, Jan-Michael/0000-0001-8774-697X; Hong, Kunlun/0000-0002-2852-5111; Smith, Gregory/0000-0001-5659-1805; Do, Changwoo/0000-0001-8358-8417 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Energy Division; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; Office of Advanced Scientific Computing Research; U.S. Department of Energy; UT-Battelle, LLC [DE-AC05-00OR22725]; EPSRC [EP/K039121/1]; NSF [CHE-1265821] FX The research at Oak Ridge National Laboratory's Spallation Neutron Source and Center for Nanophase Materials Sciences was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Research presented in this work is also supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Energy Division. This research used resources of the Leadership Computing Facility at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. J -M.C.'s contribution was sponsored by the Office of Advanced Scientific Computing Research; U.S. Department of Energy and performed at the Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725. The authors thank Dr. Joseph Curtis for a discussion and guide on SASSIE and Dr. Wei-Ren Chen for scientific discussions. This work benefitted from CCP-SAS software developed through a joint EPSRC (EP/K039121/1) and NSF (CHE-1265821) grant. NR 46 TC 9 Z9 9 U1 6 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD AUG 26 PY 2014 VL 47 IS 16 BP 5808 EP 5814 DI 10.1021/ma500613c PG 7 WC Polymer Science SC Polymer Science GA AO0IQ UT WOS:000340992700040 ER PT J AU Furrer, A Podlesnyak, A Frontzek, M Sashin, I Embs, JP Mitberg, E Pomjakushina, E AF Furrer, A. Podlesnyak, A. Frontzek, M. Sashin, I. Embs, J. P. Mitberg, E. Pomjakushina, E. TI Crystal-field interaction and oxygen stoichiometry effects in strontium-doped rare-earth cobaltates SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-PROPERTIES; PEROVSKITE-TYPE; ELECTRIC-FIELD; PR; CHEMISTRY; EU; SM; DY; ND; LN AB Inelastic neutron scattering was employed to study the crystal-field interaction in the strontium-doped rare-earth compounds RxSr1-xCoO3-z (R = Pr, Nd, Ho, and Er). Particular emphasis is laid on the effect of oxygen deficiencies that naturally occur in the synthesis of these compounds. The observed energy spectra are found to be the result of a superposition of crystal fields with different nearest-neighbor oxygen coordination at the R sites. The experimental data are interpreted in terms of crystal-field parameters, which behave in a consistent manner through the rare-earth series, thereby allowing a reliable extrapolation for rare-earth ions not considered in the present work. C1 [Furrer, A.; Frontzek, M.; Embs, J. P.] Paul Scherrer Inst, Lab Neutron Scattering, CH-5232 Villigen, Switzerland. [Podlesnyak, A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Sashin, I.] Joint Inst Nucl Res, Dubna 141980, Moscow Region, Russia. [Mitberg, E.] RAS, Inst Solid State Chem, Ekaterinburg 620219, Russia. [Pomjakushina, E.] Paul Scherrer Inst, Lab Dev & Methods, CH-5232 Villigen, Switzerland. RP Furrer, A (reprint author), Paul Scherrer Inst, Lab Neutron Scattering, CH-5232 Villigen, Switzerland. EM albert.furrer@psi.ch RI Instrument, CNCS/B-4599-2012; Podlesnyak, Andrey/A-5593-2013; Frontzek, Matthias/C-5146-2012 OI Podlesnyak, Andrey/0000-0001-9366-6319; Frontzek, Matthias/0000-0001-8704-8928 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Part of this work was performed at the Swiss Spallation Neutron Source, Paul Scherrer Institut, Villigen, Switzerland. Research at the Oak Ridge National Laboratory Spallation Neutron Source Oak Ridge, Tennessee, USA, was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 31 TC 1 Z9 1 U1 0 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 26 PY 2014 VL 90 IS 6 AR 064426 DI 10.1103/PhysRevB.90.064426 PG 8 WC Physics, Condensed Matter SC Physics GA AO4HZ UT WOS:000341299400005 ER PT J AU Adare, AM McCumber, MP Nagle, JL Romatschke, P AF Adare, A. M. McCumber, M. P. Nagle, J. L. Romatschke, P. TI Examination whether heavy quarks carry information on the early-time coupling of the quark-gluon plasma SO PHYSICAL REVIEW C LA English DT Article ID SENSITIVE PROBE; THERMALIZATION; MATTER AB The redistribution in momentum space of heavy quarks via their interactions in the quark-gluon plasma is an excellent probe of the heavy quark coupling strength to the medium. We utilize a Monte Carlo Langevin calculation for tracking heavy quark-antiquark pairs embedded in a viscous hydrodynamic space-time evolution. We find that the nuclear modification factor (R-AA) for charm quarks is relatively insensitive to the coupling to the quark-gluon plasma at early times where the highest temperatures are achieved. In contrast the azimuthal angular correlation of charm and anticharm quarks is extremely sensitive to the early time evolution. For beauty quarks the situation is reversed in terms of sensitivity. This work identifies the kinematic distributions of the heavy quarks with the greatest sensitivity, and must be followed by tests of whether they survive hadronization, in particular if recombination is dominant. C1 [Adare, A. M.; Nagle, J. L.; Romatschke, P.] Univ Colorado, Boulder, CO 80309 USA. [McCumber, M. P.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Adare, AM (reprint author), Univ Colorado, Boulder, CO 80309 USA. FU United States Department of Energy (DOE) Division of Nuclear Physics [DE-FG02-00ER41152]; DOE [DE-SC0008027]; Sloan [BR2012-038]; Los Alamos National Laboratory LDRD project [20120775PRD4] FX We gratefully acknowledge useful discussions with Jocrg Aichelin, Steffen Bass, Shanshan Cao, Matt Luzum, and Krishna Rajagopal. A.M.A. and J.L.N. acknowledge support from the United States Department of Energy (DOE) Division of Nuclear Physics (Grant No. DE-FG02-00ER41152). P.R. acknowledges support from DOE Grant No. DE-SC0008027 and Sloan Grant No. BR2012-038. M.P.M. acknowledges support from the Los Alamos National Laboratory LDRD Project No. 20120775PRD4. NR 30 TC 4 Z9 4 U1 4 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 26 PY 2014 VL 90 IS 2 AR 024911 DI 10.1103/PhysRevC.90.024911 PG 6 WC Physics, Nuclear SC Physics GA AO4IL UT WOS:000341300600005 ER PT J AU Myers, LS Ahmed, MW Feldman, G Kafkarkou, A Kendellen, DP Mazumdar, I Mueller, JM Sikora, MH Weller, HR Zimmerman, WR AF Myers, L. S. Ahmed, M. W. Feldman, G. Kafkarkou, A. Kendellen, D. P. Mazumdar, I. Mueller, J. M. Sikora, M. H. Weller, H. R. Zimmerman, W. R. TI Compton scattering from Li-6 at 86 MeV SO PHYSICAL REVIEW C LA English DT Article ID NUCLEONS AB Cross sections for Li-6(gamma,gamma)Li-6 have been measured at the High Intensity Gamma-Ray Source (HI (gamma) over right arrowS) and the sensitivity of these cross sections to the nucleon isoscalar polarizabilities was studied. Data were collected using a quasimonoenergetic 86-MeV photon beam at photon scattering angles of 40 degrees- 160 degrees. These results are an extension of a previous measurement at a lower energy. The earlier work indicated that the Li-6(gamma,gamma)Li-6 reaction at 60 MeV provides a means of extracting the nucleon polarizabilities; this work demonstrates that the sensitivity of the cross section to the polarizabilities is increased at 86 MeV. A full theoretical treatment is needed to verify this conclusion and produce values of the polarizabilities. C1 [Myers, L. S.; Ahmed, M. W.; Kafkarkou, A.; Kendellen, D. P.; Mueller, J. M.; Weller, H. R.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Myers, L. S.; Ahmed, M. W.; Kafkarkou, A.; Kendellen, D. P.; Mueller, J. M.; Sikora, M. H.; Weller, H. R.; Zimmerman, W. R.] Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Ahmed, M. W.] N Carolina Cent Univ, Dept Math & Phys, Durham, NC 27707 USA. [Feldman, G.; Sikora, M. H.] George Washington Univ, Dept Phys, Washington, DC 20052 USA. [Mazumdar, I.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. RP Myers, LS (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. FU U.S. Department of Energy, Office of Science [DE-FG02-97ER41033, DE-FG02-06ER41422] FX The authors would like to acknowledge the contributions of the staff at the HI (gamma) over right arrowS facility for the production of the gamma-ray beam used in this experiment. This work was supported in part by the U.S. Department of Energy, Office of Science, Grants No. DE-FG02-97ER41033 and No. DE-FG02-06ER41422. NR 11 TC 2 Z9 2 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 26 PY 2014 VL 90 IS 2 AR 027603 DI 10.1103/PhysRevC.90.027603 PG 4 WC Physics, Nuclear SC Physics GA AO4IL UT WOS:000341300600010 ER PT J AU Stetcu, I Talou, P Kawano, T Jandel, M AF Stetcu, I. Talou, P. Kawano, T. Jandel, M. TI Properties of prompt-fission gamma rays SO PHYSICAL REVIEW C LA English DT Article ID THERMAL-NEUTRON FISSION; STATISTICAL-MODEL; NUCLEAR-REACTIONS; CF-252; FRAGMENTS; EMISSION; SPECTRUM; RATIOS; U-235 AB In a Monte Carlo Hauser-Feshbach statistical framework, we describe spectra, average multiplicities, average energy, and multiplicity distributions of the prompt. gamma rays produced in the thermal neutron-induced fission of U-235 and Pu-239, and the spontaneous fission of Cf-252. Comparisons against recent experimental data show reasonable agreement in all cases investigated, after adjustment of the initial spin distribution in the fission fragments. In particular, when we include in the calculation the Doppler broadening we obtain a qualitatively good description of the measured low-energy spectra, where contributions from collective discrete transitions in specific fragments can be identified. At higher energies, both the calculated neutron and gamma-ray spectra are softer than experimental data. The impact of selected model parameters on the prompt neutron and gamma-ray spectra is analyzed. Finally, we present the prompt gamma spectrum and multiplicity distribution for the neutron-induced fission of U-235 for 5.5 MeV neutron incident energy, just below the threshold for second-chance fission. C1 [Stetcu, I.; Talou, P.; Kawano, T.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Jandel, M.] Los Alamos Natl Lab, C NR, Los Alamos, NM 87545 USA. RP Stetcu, I (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. FU U.S. Department of Energy through the LANL/LDRD Program; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; U.S. Department of Energy, Office of Science, Nuclear Physics under the Early Career Award [LANL20135009] FX We thank S. Oberstedt, A. Oberstedt, and R. Billnert for providing their data on 252Cf(sf) and 235U(nth, f), and John Ullmann for useful discussions. We gratefully acknowledge the support of the U.S. Department of Energy through the LANL/LDRD Program. This work was performed at Los Alamos National Laboratory, under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. Work by M.J. was supported by the U.S. Department of Energy, Office of Science, Nuclear Physics under the Early Career Award No. LANL20135009. NR 54 TC 17 Z9 17 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 26 PY 2014 VL 90 IS 2 AR 024617 DI 10.1103/PhysRevC.90.024617 PG 13 WC Physics, Nuclear SC Physics GA AO4IL UT WOS:000341300600002 ER PT J AU Dodelson, S Park, S AF Dodelson, Scott Park, Sohyun TI Nonlocal gravity and structure in the Universe SO PHYSICAL REVIEW D LA English DT Article ID COSMIC ACCELERATION; GENERAL-RELATIVITY; DARK ENERGY; GROWTH AB The observed acceleration of the Universe can be explained by modifying general relativity. One such attempt is the nonlocal model of Deser and Woodard. Here we fix the background cosmology using results from the Planck satellite and examine the predictions of nonlocal gravity for the evolution of structure in the Universe, confronting the model with three tests: gravitational lensing, redshift space distortions, and an estimator of gravity E-G that combines spectroscopic information with lensing. Current data favor general relativity (GR) over nonlocal gravity: fixing primordial cosmology with the best fit parameters from Planck leads to weak lensing results favoring GR by 6.8 sigma; redshift space distortions measurements of the growth rate preferring GR by 7.8 sigma; and the single measurement of E-G favoring GR, but by less than 1 sigma. The significance holds up even after the parameters are allowed to vary within Planck limits. The larger lesson is that a successful modified gravity model will likely have to suppress the growth of structure compared to general relativity. C1 [Dodelson, Scott] Fermilab Natl Accelerator Lab, Fermilab Ctr Particle Astrophys, Batavia, IL 60510 USA. [Dodelson, Scott] Univ Chicago, Enrico Fermi Inst, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Dodelson, Scott] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Park, Sohyun] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. RP Dodelson, S (reprint author), Fermilab Natl Accelerator Lab, Fermilab Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. FU U.S. Department of Energy [DE-FG02-95ER40896]; Pennsylvania State University FX We thank Sarah Bridle, Catherine Heymans, Beth Reid, Fabian Schmidt, Sarah Shandera, Fergus Simpson, Constantinos Skordis, Masahiro Takada, and Richard Woodard for useful suggestions and conversations. S. D. is supported by the U.S. Department of Energy, including Grant No. DE-FG02-95ER40896. S. P. is supported by the Eberly Research Funds of The Pennsylvania State University. NR 34 TC 15 Z9 15 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 26 PY 2014 VL 90 IS 4 AR 043535 DI 10.1103/PhysRevD.90.043535 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AN8XU UT WOS:000340890100002 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Anson, CD Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Balewski, J Banerjee, A Barnovska, Z Beavis, DR Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bichsel, H Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Brandin, AV Brovko, SG Bultmann, S Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Cebra, D Cendejas, R Cervantes, MC Chaloupka, P Chang, Z Chattopadhyay, S Chen, HF Chen, JH Chen, L Cheng, J Cherney, M Chikanian, A Christie, W Chwastowski, J Codrington, MJM Corliss, R Cramer, JG Crawford, HJ Cui, X Das, S Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD Dhamija, S di Ruzza, B Didenko, L Dilks, C Ding, F Djawotho, P Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Engle, KS Eppley, G Eun, L Evdokimov, O Fatemi, R Fazio, S Fedorisin, J Filip, P Finch, E Fisyak, Y Flores, CE Gagliardi, CA Gangadharan, DR Garand, D Geurts, F Gibson, A Girard, M Gliske, S Grosnick, D Guo, Y Gupta, A Gupta, S Guryn, W Haag, B Hajkova, O Hamed, A Han, LX Haque, R Harris, JW Hays-Wehle, JP Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, HZ Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Kesich, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Koetke, DD Kollegger, T Konzer, J Koralt, I Korsch, W Kotchenda, L Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Leight, W LeVine, MJ Li, C Li, W Li, X Li, X Li, Y Li, ZM Lima, LM Lisa, MA Liu, F Ljubicic, T Llope, WJ Longacre, RS Luo, X Ma, GL Ma, YG Don, DMMDM Mahapatra, DP Majka, R Margetis, S Markert, C Masui, H Matis, HS McDonald, D McShane, TS Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Munhoz, MG Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nelson, JM Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Oliveira, RAN Pachr, M Page, BS Pal, SK Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Peryt, W Peterson, A Pile, P Planinic, M Pluta, J Plyku, D Poljak, N Porter, J Poskanzer, AM Pruthi, NK Przybycien, M Pujahari, PR Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Riley, CK Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ross, JF Roy, A Ruan, L Rusnak, J Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandacz, A Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Singaraju, RN Skoby, MJ Smirnov, D Smirnov, N Solanki, D Sorensen, P Desouza, UG Spinka, HM Srivastava, B Stanislaus, TDS Stevens, JR Stock, R Strikhanov, M Stringfellow, B Suaide, AAP Sumbera, M Sun, X Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM de Toledo, AS Takahashi, J Tang, AH Tang, Z Tarnowsky, T Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Trzeciak, BA Tsai, OD Turnau, J Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Vossen, A Wada, M Walker, M Wang, F Wang, G Wang, H Wang, JS Wang, XL Wang, Y Wang, Y Webb, G Webb, JC Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, H Xu, N Xu, QH Xu, Y Xu, Z Yan, W Yang, C Yang, Y Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Zawisza, Y Zbroszczyk, H Zha, W Zhang, JB Zhang, S Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhu, X Zhu, YH Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Anson, C. D. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Balewski, J. Banerjee, A. Barnovska, Z. Beavis, D. R. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bichsel, H. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Brandin, A. V. Brovko, S. G. Bueltmann, S. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. Sanchez, M. Calderon de la Barca Cebra, D. Cendejas, R. Cervantes, M. C. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Christie, W. Chwastowski, J. Codrington, M. J. M. Corliss, R. Cramer, J. G. Crawford, H. J. Cui, X. Das, S. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. de Souza, R. Derradi Dhamija, S. di Ruzza, B. Didenko, L. Dilks, C. Ding, F. Djawotho, P. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Engle, K. S. Eppley, G. Eun, L. Evdokimov, O. Fatemi, R. Fazio, S. Fedorisin, J. Filip, P. Finch, E. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Gangadharan, D. R. Garand, D. Geurts, F. Gibson, A. Girard, M. Gliske, S. Grosnick, D. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hajkova, O. Hamed, A. Han, L-X. Haque, R. Harris, J. W. Hays-Wehle, J. P. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, H. Z. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kesich, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Korsch, W. Kotchenda, L. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Leight, W. LeVine, M. J. Li, C. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lima, L. M. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Longacre, R. S. Luo, X. Ma, G. L. Ma, Y. G. Don, D. M. M. D. Madagodagettige Mahapatra, D. P. Majka, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. McShane, T. S. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Munhoz, M. G. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nelson, J. M. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Oliveira, R. A. N. Pachr, M. Page, B. S. Pal, S. K. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Peryt, W. Peterson, A. Pile, P. Planinic, M. Pluta, J. Plyku, D. Poljak, N. Porter, J. Poskanzer, A. M. Pruthi, N. K. Przybycien, M. Pujahari, P. R. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Riley, C. K. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ross, J. F. Roy, A. Ruan, L. Rusnak, J. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandacz, A. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Singaraju, R. N. Skoby, M. J. Smirnov, D. Smirnov, N. Solanki, D. Sorensen, P. deSouza, U. G. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Suaide, A. A. P. Sumbera, M. Sun, X. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. de Toledo, A. Szanto Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Trzeciak, B. A. Tsai, O. D. Turnau, J. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Vossen, A. Wada, M. Walker, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, X. L. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, H. Xu, N. Xu, Q. H. Xu, Y. Xu, Z. Yan, W. Yang, C. Yang, Y. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I-K. Zawisza, Y. Zbroszczyk, H. Zha, W. Zhang, J. B. Zhang, S. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zhu, Y. H. Zoulkarneeva, Y. Zyzak, M. TI Beam Energy Dependence of Moments of the Net-Charge Multiplicity Distributions in Au plus Au Collisions at RHIC SO PHYSICAL REVIEW LETTERS LA English DT Article ID STAR; POINT; QCD AB We report the first measurements of the moments-mean (M), variance (sigma(2)), skewness (S), and kurtosis (kappa)-of the net-charge multiplicity distributions at midrapidity in Au + Au collisions at seven energies, ranging from root s(NN) = 7.7 to 200 GeV, as a part of the Beam Energy Scan program at RHIC. The moments are related to the thermodynamic susceptibilities of net charge, and are sensitive to the location of the QCD critical point. We compare the products of the moments, sigma(2)/M, S sigma, and kappa sigma(2), with the expectations from Poisson and negative binomial distributions (NBDs). The S sigma values deviate from the Poisson baseline and are close to the NBD baseline, while the kappa sigma(2) values tend to lie between the two. Within the present uncertainties, our data do not show nonmonotonic behavior as a function of collision energy. These measurements provide a valuable tool to extract the freeze-out parameters in heavy-ion collisions by comparing with theoretical models. C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, Krakow, Poland. [Gliske, S.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Nelson, J. M.] Univ Birmingham, Birmingham, W Midlands, England. [Arkhipkin, D.; Aschenauer, E. C.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Fazio, S.; Fisyak, Y.; Guryn, W.; Huang, B.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Wang, H.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Brovko, S. G.; Sanchez, M. Calderon de la Barca; Cebra, D.; Ding, F.; Draper, J. E.; Flores, C. E.; Haag, B.; Kesich, A.; Romero, J. L.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Huang, H. Z.; Igo, G.; Landry, K. D.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [de Souza, R. Derradi; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, Sao Paulo, Brazil. [Chen, L.; Huck, P.; Ke, H. W.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Wu, Y. F.; Yang, Y.; Zhang, J. B.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Wang, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Chwastowski, J.; Kycia, R. A.] Cracow Univ Technol, Krakow, Poland. [Cherney, M.; Don, D. M. M. D. Madagodagettige; McShane, T. S.; Ross, J. F.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Hajkova, O.; Pachr, M.] Czech Tech Univ, FNSPE, Prague 11519, Czech Republic. [Barnovska, Z.; Bielcikova, J.; Rusnak, J.; Sumbera, M.; Tlusty, D.; Vertesi, R.] Nucl Phys Inst AS CR, Rez 25068, Czech Republic. [Kisel, I.; Kollegger, T.; Kulakov, I.; Stock, R.; Zyzak, M.] Frankfurt Inst Adv Studies FIAS, Frankfurt, Germany. [Das, S.; Mahapatra, D. P.; Sahu, P. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Pujahari, P. R.; Sarkar, A.; Varma, R.] Indian Inst Technol, Mumbai 400076, Maharashtra, India. [Dhamija, S.; Jacobs, W. W.; Page, B. S.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Kalinkin, D.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow, Russia. [Bhasin, A.; Gupta, A.; Gupta, S.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Dubna Joint Nucl Res Inst, Dubna 141980, Russia. [Alford, J.; Bouchet, J.; Keane, D.; Margetis, S.; Quintero, A.; Shanmuganathan, P. V.; Vanfossen, J. A., Jr.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Korsch, W.; Ramachandran, S.; Webb, G.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Inst Sci & Technol Informat, Taejon, South Korea. [Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.] Inst Modern Phys, Lanzhou, Peoples R China. [Dong, X.; Eun, L.; Masui, H.; Matis, H. S.; Odyniec, G.; Porter, J.; Poskanzer, A. M.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Shi, S. S.; Sichtermann, E. P.; Sun, X.; Sun, X. M.; Symons, T. J. M.; Thomas, J. H.; Wieman, H.; Xu, N.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Balewski, J.; Corliss, R.; Hays-Wehle, J. P.; Leight, W.; Stevens, J. R.; van Nieuwenhuizen, G.; Walker, M.] MIT, Cambridge, MA 02139 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Haque, R.; Kumar, L.; Mohanty, B.; Nasim, Md.] Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. [Anson, C. D.; Gangadharan, D. R.; Humanic, T. J.; Lisa, M. A.; Peterson, A.] Ohio State Univ, Columbus, OH 43210 USA. [Bueltmann, S.; Koralt, I.; Plyku, D.] Old Dominion Univ, Norfolk, VA 23529 USA. [Pawlik, B.; Turnau, J.] Inst Nucl Phys PAN, Krakow, Poland. [Aggarwal, M. M.; Bhati, A. K.; Pruthi, N. K.; Sharma, B.] Panjab Univ, Chandigarh 160014, India. [Cendejas, R.; Dilks, C.; Heppelmann, S.] Penn State Univ, University Pk, PA 16802 USA. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino, Russia. [Garand, D.; Hirsch, A.; Kikola, D. P.; Konzer, J.; Li, X.; Mustafa, M. K.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I-K.] Pusan Natl Univ, Pusan 609735, South Korea. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Llope, W. J.; McDonald, D.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Lima, L. M.; Munhoz, M. G.; Oliveira, R. A. N.; deSouza, U. G.; Suaide, A. A. P.; de Toledo, A. Szanto] Univ Sao Paulo, Sao Paulo, Brazil. [Chen, H. F.; Cui, X.; Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Yang, C.; Zawisza, Y.; Zha, W.; Zhang, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Han, L-X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Zhang, S.; Zhao, J.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Borowski, W.; Kabana, S.] SUBATECH, Nantes, France. [Li, X.; Surrow, B.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Djawotho, P.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Codrington, M. J. M.; Leyva, A. Davila; Hoffmann, G. W.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; De Silva, L. C.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Yan, W.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Engle, K. S.; Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Pal, S. K.; Roy, A.; Sahoo, N. R.; Singaraju, R. N.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kisiel, A.; Pawlak, T.; Peryt, W.; Pluta, J.; Sandacz, A.; Trzeciak, B. A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Bichsel, H.; Cramer, J. G.] Univ Washington, Seattle, WA 98195 USA. [Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Horvat, S.; Majka, R.; Ohlson, A.; Riley, C. K.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, Krakow, Poland. RI Sumbera, Michal/O-7497-2014; Strikhanov, Mikhail/P-7393-2014; Takahashi, Jun/B-2946-2012; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; XIAO, Zhigang/C-3788-2015; Fazio, Salvatore /G-5156-2010; Kumar, Lokesh/A-6154-2010; Aparecido Negrao de Oliveira, Renato/G-9133-2015; Kycia, Radoslaw/J-4397-2015; Chaloupka, Petr/E-5965-2012; Derradi de Souza, Rafael/M-4791-2013; Suaide, Alexandre/L-6239-2016; Yi, Li/Q-1705-2016; Alekseev, Igor/J-8070-2014; Svirida, Dmitry/R-4909-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; OI Sumbera, Michal/0000-0002-0639-7323; Strikhanov, Mikhail/0000-0003-2586-0405; Takahashi, Jun/0000-0002-4091-1779; Kumar, Lokesh/0000-0002-2746-9840; Kycia, Radoslaw/0000-0002-6390-4627; Derradi de Souza, Rafael/0000-0002-2084-7001; Suaide, Alexandre/0000-0003-2847-6556; Yi, Li/0000-0002-7512-2657; Alekseev, Igor/0000-0003-3358-9635; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Sorensen, Paul/0000-0001-5056-9391; Thomas, James/0000-0002-6256-4536 FU Offices of NP and HEP within the U.S. DOE Office of Science; U.S. NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation; GA of the Czech Republic; FIAS of Germany; DAE; DST; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia; MSMT of the Czech Republic; RHIC Operations Group; RCF at BNL; NERSC Center at LBNL; KISTI Center in Korea; Open Science Grid consortium FX We thank M. Asakawa, R. Gavai, S. Gupta, F. Karsch, V. Koch, S. Mukherjee, K. Rajagopal, K. Redlich, and M. A. Stephanov for discussions related to this work. We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3, FAPESP CNPq of Brazil, the Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST and MoE of China, the Korean Research Foundation, GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and CSIR of India, the National Science Centre of Poland, National Research Foundation (NRF-2012004024), the Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. NR 43 TC 76 Z9 76 U1 2 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 26 PY 2014 VL 113 IS 9 AR 092301 DI 10.1103/PhysRevLett.113.092301 PG 7 WC Physics, Multidisciplinary SC Physics GA AO4IX UT WOS:000341301800002 ER PT J AU Zhao, L Klopf, JM Reece, CE Kelley, MJ AF Zhao, Liang Klopf, J. Michael Reece, Charles E. Kelley, Michael J. TI Laser polishing of niobium for superconducting radio-frequency accelerator applications SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID SURFACE AB Interior surfaces of niobium cavities used in superconducting radio frequency accelerators are now obtained by buffered chemical polish and/or electropolish. Laser polishing is a potential alternative, having advantages of speed, freedom from noxious chemistry and availability of in-process inspection. We studied the influence of the laser power density and laser beam raster rate on the surface topography. These two factors need to be combined carefully to smooth the surface without damage. Computational modeling was used to estimate the surface temperature and gain insight into the mechanism of laser polishing. Power spectral density analysis of surface topography measurements shows that laser polishing can produce smooth topography similar to that obtained by electropolish. This is a necessary first step toward introducing laser polishing as an alternative to the currently practiced chemical polishing. C1 [Zhao, Liang; Klopf, J. Michael; Kelley, Michael J.] Coll William & Mary, Dept Appl Sci, Williamsburg, VA 23187 USA. [Zhao, Liang; Reece, Charles E.; Kelley, Michael J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Kelley, MJ (reprint author), Coll William & Mary, Dept Appl Sci, Williamsburg, VA 23187 USA. EM mkelley@jlab.org OI Reece, Charles/0000-0003-1939-8699 FU Office of High Energy Physics of the U.S. Department of Energy [SC0007907]; Jefferson Science Associates, LLC under U.S. DOE [DE-AC05-06OR23177] FX We gratefully acknowledge the support of the Office of High Energy Physics of the U.S. Department of Energy under Grant No. SC0007907 to the College of William & Mary. The experiments were conducted at Jefferson Lab. This work was partly authored by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177. Thanks to staff at the College of William and Mary characterization lab, especially Olga Trofimova for the AFM images. Thanks to Chen Xu for the PSD program, and Ari Palczewski for helping with the CBP samples. We thank Professor Peter Schaaf of Gottingen for providing the computer code used for the model calculations. NR 29 TC 2 Z9 3 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD AUG 26 PY 2014 VL 17 IS 8 AR 083502 DI 10.1103/PhysRevSTAB.17.083502 PG 9 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AO4IZ UT WOS:000341302000001 ER PT J AU Landau, P Guo, Q Hosemann, P Wang, YQ Greer, JR AF Landau, Peri Guo, Qiang Hosemann, Peter Wang, Yongqiang Greer, Julia R. TI Deformation of as-fabricated and helium implanted 100 nm-diameter iron nano-pillars SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Nanoscale plasticity; Tension test; Compression test; Iron; Helium implantation ID DISLOCATION DYNAMICS SIMULATIONS; FERRITIC-MARTENSITIC STEEL; BCC TRANSITION-METALS; SINGLE-CRYSTALS; MECHANICAL-PROPERTIES; PLASTIC-DEFORMATION; COPPER NANOPILLARS; IRRADIATION DAMAGE; SCREW DISLOCATIONS; TENSILE PROPERTIES AB < 101 >-oriented cylindrical single crystalline Fe samples with diameters of 100 nm and heights of 1 mu m were implanted with 0.36 +/- 0.06 at% helium throughout their gauge sections. Uniaxial deformation experiments revealed a 40% higher yield and ultimate strengths in tension and a 25% higher yield strength and flow stress at 10% plastic strain in compression for implanted samples compared with as-fabricated ones. Observed tension-compression asymmetry in implanted pillars was attributed to the non-planarity of screw dislocation cores and to twinning-antitwinning deformation typical of bcc metals and the interaction between dislocations and He bubbles. Compressive stress-strain data in both sets of samples had three distinct regimes: (1) elastic loading followed by (2) discrete strain bursts during plastic flow with significant hardening up to strains of 5%, and (3) "steady state" discrete plasticity characterized by nearly-constant average flow stress. Each regime is discussed and explained in terms of competition in the rates of dislocation multiplication and dislocation annihilation. (C) 2014 Elsevier B.V. All rights reserved. C1 [Landau, Peri; Guo, Qiang; Greer, Julia R.] CALTECH, Dept Mat Sci & Appl Phys, Pasadena, CA 91125 USA. [Guo, Qiang] Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Shanghai 200240, Peoples R China. [Hosemann, Peter] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Wang, Yongqiang] Los Alamos Natl Lab, Ion Beam Mat Lab, Los Alamos, NM 87545 USA. [Greer, Julia R.] CALTECH, Kavli Nanosci Inst, Pasadena, CA 91125 USA. RP Landau, P (reprint author), CALTECH, Dept Mat Sci & Appl Phys, 1200 East Calif Blvd, Pasadena, CA 91125 USA. EM landperi@gmail.com RI Guo, Qiang/D-6389-2012; OI Hosemann, Peter/0000-0003-2281-2213 FU U.S. Department of Energy, Office of Basic Energy Sciences through JRG's Early Career grant [DE-FOA-00003951]; Kavli Nanoscience Institute (KNI); Center for Integrated Nanotechnologies (CINT); DOE nanoscience center FX The authors gratefully acknowledge the financial support of the U.S. Department of Energy, Office of Basic Energy Sciences through JRG's Early Career grant DE-FOA-00003951. The authors also acknowledge support and infrastructure provided by the Kavli Nanoscience Institute (KNI). Helium implantation was supported by Center for Integrated Nanotechnologies (CINT), a DOE nanoscience center jointly operated by Los Alamos and Sandia National Laboratories. NR 82 TC 7 Z9 7 U1 3 U2 45 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD AUG 26 PY 2014 VL 612 BP 316 EP 325 DI 10.1016/j.msea.2014.06.052 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AN1GS UT WOS:000340331300040 ER PT J AU Das, S Dubey, M Roelofs, A AF Das, Saptarshi Dubey, Madan Roelofs, Andreas TI High gain, low noise, fully complementary logic inverter based on bi-layer WSe2 field effect transistors SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILM-TRANSISTOR; MOS2 TRANSISTORS; MULTILAYER MOS2; TRANSPARENT; CONTACTS AB In this article, first, we show that by contact work function engineering, electrostatic doping and proper scaling of both the oxide thickness and the flake thickness, high performance p- and n-type WSe2 field effect transistors (FETs) can be realized. We report record high drive current of 98 mu A/mu m for the electron conduction and 110 mu A/mu m for the hole conduction in Schottky barrier WSe2 FETs. Then, we combine high performance WSe2 PFET with WSe2 NFET in double gated transistor geometry to demonstrate a fully complementary logic inverter. We also show that by adjusting the threshold voltages for the NFET and the PFET, the gain and the noise margin of the inverter can be significantly enhanced. The maximum gain of our chemical doping free WSe2 inverter was found to be similar to 25 and the noise margin was close to its ideal value of similar to 2.5V for a supply voltage of V-DD = 5.0 V. (C) 2014 AIP Publishing LLC. C1 [Das, Saptarshi; Roelofs, Andreas] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Dubey, Madan] US Army, Res Lab, Adelphi, MD 20783 USA. RP Das, S (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Roelofs, Andreas/H-1742-2011 OI Roelofs, Andreas/0000-0003-4141-3082 FU DOE Office of High Energy Physics under DoE Contract [DE-AC02-06CH11357]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors acknowledge the Army Research laboratory. This work was supported by the DOE Office of High Energy Physics under DoE Contract No. DE-AC02-06CH11357. Use of the Center for Nanoscale Materials was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 19 TC 23 Z9 23 U1 3 U2 54 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 25 PY 2014 VL 105 IS 8 AR 083511 DI 10.1063/1.4894426 PG 5 WC Physics, Applied SC Physics GA AQ4HE UT WOS:000342753500099 ER PT J AU Donovan, BF Foley, BM Ihlefeld, JF Maria, JP Hopkins, PE AF Donovan, Brian F. Foley, Brian M. Ihlefeld, Jon F. Maria, Jon-Paul Hopkins, Patrick E. TI Spectral phonon scattering effects on the thermal conductivity of nano-grained barium titanate SO APPLIED PHYSICS LETTERS LA English DT Article ID DIELECTRIC-PROPERTIES; CERAMIC CAPACITORS; THIN-FILMS; SIZE; BATIO3; HEAT AB We study the effect of grain size on thermal conductivity of thin film barium titanate over temperatures ranging from 200 to 500 K. We show that the thermal conductivity of Barium Titanate (BaTiO3) decreases with decreasing grain size as a result of increased phonon scattering from grain boundaries. We analyze our results with a model for thermal conductivity that incorporates a spectrum of mean free paths in BaTiO3. In contrast to the common gray mean free path assumption, our findings suggest that the thermal conductivity of complex oxide perovskites is driven by a spectrum of phonons with varying mean free paths. (C) 2014 AIP Publishing LLC. C1 [Donovan, Brian F.] Univ Virginia, Dept Mat Sci & Engn, Charlottesville, VA 22904 USA. [Foley, Brian M.; Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Ihlefeld, Jon F.] Sandia Natl Labs, Elect Opt & Nanomat Dept, Albuquerque, NM 87185 USA. [Maria, Jon-Paul] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. RP Ihlefeld, JF (reprint author), Sandia Natl Labs, Elect Opt & Nanomat Dept, POB 5800, Albuquerque, NM 87185 USA. EM jihlefe@sandia.gov; phopkins@virginia.cdu FU National Science Foundation [CBET-1339436]; Army Research Office [W911NF-13-1-0378]; Air Force Office of Scientific Research [FA9550-14-1-0067, 5010-UV-AFOSR-0067]; Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to acknowledge Bonnie McKenzie at Sandia National Labs for her help materials characterization and electron microscopy, as well as Christopher T. Shelton for help with the atomic force micrographs seen in the Supporting Material. We appreciate funding from the National Science Foundation (CBET-1339436). the Army Research Office, Grant No. W911NF-13-1-0378, and the Air Force Office of Scientific Research under AFOSR Award No FA9550-14-1-0067 (Subaward No. 5010-UV-AFOSR-0067). This work was also supported, in part, by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 35 TC 8 Z9 8 U1 3 U2 27 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 25 PY 2014 VL 105 IS 8 AR 082907 DI 10.1063/1.4893920 PG 5 WC Physics, Applied SC Physics GA AQ4HE UT WOS:000342753500058 ER PT J AU Hong, XG Ehm, L Duffy, TS AF Hong, Xinguo Ehm, Lars Duffy, Thomas S. TI Polyhedral units and network connectivity in GeO2 glass at high pressure: An X-ray total scattering investigation SO APPLIED PHYSICS LETTERS LA English DT Article ID RUTILE-TYPE; DIFFRACTION; SIO2; CRYSTALLINE; SILICA; LIQUID AB We report a pressure-induced dense tetrahedral intermediate state via Ge-O-Ge rotation formed at 3-5GPa and the polyhedral relations in GeO2 glass up to 17.5GPa using in situ X-ray total scattering and X-ray absorption (XAFS) techniques. It was found that the nearest-neighbor Ge-Ge correlations show a decrease reaching a minimum between 4 and 6GPa, and exhibit negative compression behavior at 7-17.5GPa. The Ge-Ge distance determined by XAFS shows a substantial reduction, i.e., normal compression behavior, at 7-17.5GPa. The comparison with the theoretical g(r) function for rutile-type GeO2 (16.1GPa) indicates that the negative compression of intermediate range order reflects the direct formation of GeO6 octahedral units. Results of coordination number analysis show that GeO2 glass undergoes a transition from tetrahedral GeO4, to GeO5 units (possibly triangular bipyramidal), and finally to octahedral GeO6 units. The present investigation provides the structural details of the polyhedral units and their relationships in GeO2 glass at high pressure. (C) 2014 AIP Publishing LLC. C1 [Hong, Xinguo; Ehm, Lars] SUNY Stony Brook, Inst Mineral Phys, Stony Brook, NY 11794 USA. [Ehm, Lars] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Duffy, Thomas S.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. RP Hong, XG (reprint author), SUNY Stony Brook, Inst Mineral Phys, Stony Brook, NY 11794 USA. EM xhong@bnl.gov RI Duffy, Thomas/C-9140-2017 OI Duffy, Thomas/0000-0002-5357-1259 FU COMPRES under NSF [EAR 11-57758] FX We thank D. Weidner for useful discussions, and M. Newville, X. M. Yu, Z. Zhong, L. P. Huang, and S. Lin for assistance. This research was partially supported by COMPRES under NSF Cooperative Agreement EAR 11-57758. NR 29 TC 9 Z9 9 U1 3 U2 25 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 25 PY 2014 VL 105 IS 8 AR 081904 DI 10.1063/1.4894103 PG 5 WC Physics, Applied SC Physics GA AQ4HE UT WOS:000342753500025 ER PT J AU Lam, NQ AF Lam, Nghi Q. TI Editorial: Reflections on my tenure as Editor-in-Chief of Applied Physics Letters SO APPLIED PHYSICS LETTERS LA English DT Editorial Material C1 Argonne Natl Lab, Argonne, IL 60439 USA. RP Lam, NQ (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. NR 0 TC 0 Z9 0 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 25 PY 2014 VL 105 IS 8 AR 080401 DI 10.1063/1.4894755 PG 2 WC Physics, Applied SC Physics GA AQ4HE UT WOS:000342753500001 ER PT J AU McBride, PM Yan, QM Van de Walle, CG AF McBride, Patrick M. Yan, Qimin Van de Walle, Chris G. TI Effects of In profile on simulations of InGaN/GaN multi-quantum-well light-emitting diodes SO APPLIED PHYSICS LETTERS LA English DT Article ID POLARIZATION AB We investigate the impact of incorporating realistic In profiles in simulations of c-plane InGaN/GaN light-emitting diodes. Simulations based on a drift-diffusion model typically overestimate the onset voltage, but have usually been based on the assumption of ideal quantum wells with a square In profile. We demonstrate that more realistic profiles lead to significant modifications of currentdensity-versus-voltage characteristics, and explain the effects based on changes in the band diagram and carrier overlap. (C) 2014 AIP Publishing LLC. C1 [McBride, Patrick M.; Yan, Qimin; Van de Walle, Chris G.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Yan, Qimin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP McBride, PM (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. RI Yan, Qimin/B-2147-2014 FU Bonderson Fellowship; UCSB's Institute for Energy Efficiency Holbrook Foundation Fellowship; UCSB Solid State Lighting and Energy Center; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0010689]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; SiLENSe FX We thank Sergey Karpov for discussions and support with SiLENSe. P.M.M. gratefully acknowledges support of a Bonderson Fellowship and of UCSB's Institute for Energy Efficiency Holbrook Foundation Fellowship. Q.Y. was supported by the UCSB Solid State Lighting and Energy Center. C.G.V.dW. was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award # DE-SC0010689. Computational resources were provided by the Center for Scientific Computing at the CNSI and MRL (an NSF MRSEC, DMR-1121053). (NSF CNS-0960316), and by NERSC which is supported by the National Energy Research Scientific Computing Center (NERSC) which is a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 20 TC 7 Z9 7 U1 3 U2 24 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 25 PY 2014 VL 105 IS 8 AR 083507 DI 10.1063/1.4894464 PG 3 WC Physics, Applied SC Physics GA AQ4HE UT WOS:000342753500095 ER PT J AU Woolf, D Hensley, J Cederberg, JG Bethke, DT Grine, AD Shaner, EA AF Woolf, D. Hensley, J. Cederberg, J. G. Bethke, D. T. Grine, A. D. Shaner, E. A. TI Heterogeneous metasurface for high temperature selective emission SO APPLIED PHYSICS LETTERS LA English DT Article ID THERMOPHOTOVOLTAIC ENERGY-CONVERSION; CELLS; EFFICIENCY; SURFACE; GROWTH; SINGLE AB We demonstrate selective emission from a heterogeneous metasurface that can survive repeated temperature cycling at 1300 K. Simulations, fabrication, and characterization were performed for a cross-over-a-backplane metasurface consisting of platinum and alumina layers on a sapphire substrate. The structure was stabilized for high temperature operation by an encapsulating alumina layer. The geometry was optimized for integration into a thermophotovoltaic (TPV) system, and was designed to have its emissivity matched to the external quantum efficiency spectrum of 0.6 eV InGaAs TPV material. We present spectral measurements of the metasurface that result in a predicted 22% optical-to-electrical power conversion efficiency in a simplified model at 1300 K. Furthermore, this broadly adaptable selective emitter design can be easily integrated into full-scale TPV systems. (C) 2014 AIP Publishing LLC. C1 [Woolf, D.; Hensley, J.] Phys Sci Inc, New England Business Ctr 20, Andover, MA 01810 USA. [Cederberg, J. G.; Bethke, D. T.; Grine, A. D.; Shaner, E. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Woolf, D (reprint author), Phys Sci Inc, New England Business Ctr 20, Andover, MA 01810 USA. EM dwoolf@psicorp.com FU Office of Naval Research (ONR) [N00014-13-P-1190]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported by the Office of Naval Research (ONR) under Contract No, N00014-13-P-1190. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the ONR. This work was performed, in part, at the Center for Integrated Nanotechnologies (CINT), an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 28 TC 12 Z9 12 U1 0 U2 35 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 25 PY 2014 VL 105 IS 8 AR 081110 DI 10.1063/1.4893742 PG 5 WC Physics, Applied SC Physics GA AQ4HE UT WOS:000342753500011 ER PT J AU Zhang, H Talapin, DV AF Zhang, Hao Talapin, Dmitri V. TI Thermoelectric Tin Selenide: The Beauty of Simplicity SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Editorial Material DE bond anharmonicity; materials science; thermal conductivity; thermoelectrics; tin selenide ID PERFORMANCE BULK THERMOELECTRICS; FIGURE; MERIT; EFFICIENCY C1 [Zhang, Hao; Talapin, Dmitri V.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Zhang, Hao; Talapin, Dmitri V.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Talapin, Dmitri V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Talapin, DV (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM dvtalapin@uchicago.edu NR 15 TC 13 Z9 13 U1 7 U2 112 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 25 PY 2014 VL 53 IS 35 BP 9126 EP 9127 DI 10.1002/anie.201405683 PG 2 WC Chemistry, Multidisciplinary SC Chemistry GA AQ3FT UT WOS:000342676100001 PM 25044424 ER PT J AU Tappan, BC Dirmyer, MR Risha, GA AF Tappan, Bryce C. Dirmyer, Matthew R. Risha, Grant A. TI Evidence of a Kinetic Isotope Effect in Nanoaluminum and Water Combustion SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE aluminum; deuterium; kinetics; metal combustion; nanoparticles ID ALUMINUM PARTICLES; LIQUID WATER; HYDROGEN; PROPELLANTS; TRANSITION; DEUTERIUM; MIXTURES; TIME AB The normally innocuous combination of aluminum and water becomes violently reactive on the nanoscale. Research in the field of the combustion of nanoparticulate aluminum has important implications in the design of molecular aluminum clusters, hydrogen storage systems, as well as energetic formulations which could use extraterrestrial water for space propulsion. However, the mechanism that controls the reaction speed is poorly understood. While current models for micron-sized aluminum water combustion reactions place heavy emphasis on diffusional limitations, as reaction scales become commensurate with diffusion lengths (approaching the nanoscale) reaction rates have long been suspected to depend on chemical kinetics, but have never been definitely measured. The combustion analysis of nanoparticulate aluminum with H2O or D2O is presented. Different reaction rates resulting from the kinetic isotope effect are observed. The current study presents the first-ever observed kinetic isotope effect in a metal combustion reaction and verifies that chemical reaction kinetics play a major role in determining the global burning rate. C1 [Tappan, Bryce C.; Dirmyer, Matthew R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Risha, Grant A.] Penn State Univ, Altoona Coll, Force Technol Ctr 203, Altoona, PA 16601 USA. RP Tappan, BC (reprint author), Los Alamos Natl Lab, MS C920, Los Alamos, NM 87545 USA. EM btappan@lanl.gov FU U.S. Department of Energy through the LANL/LDRD Program; United States Department of Energy [DE-AC52-06A25396] FX We gratefully acknowledge the support of the U.S. Department of Energy through the LANL/LDRD Program for this work and in part to Dr. Bill Wilson of the DTRA-AEI. The Los Alamos National Laboratory is operated by LANS, LLC, for the United States Department of Energy under contract DE-AC52-06A25396. Special thanks go to Prof. Richard A. Yetter and Terrence Connell for their assistance in conducting some of the strand burner experiments. For helpful edits and comments we also thank Drs. Owen Summerscales, David Chavez, Susan Hanson, Virginia Manner, Doug Tasker, and Geoffrey Brown, as well as Caroline Spaeth and Kelly Parker for technical editing and artwork. NR 31 TC 4 Z9 5 U1 5 U2 25 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 25 PY 2014 VL 53 IS 35 BP 9218 EP 9221 DI 10.1002/anie.201404962 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AQ3FT UT WOS:000342676100015 PM 24943658 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Brito, L Martins, MC Pol, ME Teles, PR Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM De Jesus Damiao, D De Oliveira Martins, C De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Yang, D Zhang, L Zou, W Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sauvan, J Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H Rurua, L Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Garcia, JG Geiser, A Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G Hempel, M Horton, D Jung, H Kasemann, M Katsas, P Kieseler, J Kleinwort, C Kramer, M Krucker, D Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Ntomari, E Perrey, H Petrukhin, A Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Riedl, C Ron, E Sahin, M Salfeld-Nebgen, J Saxena, P Schmidt, R Schoerner-Sadenius, T Schroder, M Stein, M Trevino, ADRV Walsh, R Wissing, C Martin, MA Blobel, V Vignali, MC Enderle, H Erfle, J Garutti, E Goebel, K Gorner, M Gosselink, M Haller, J Hoing, RS Kirschenmann, H Klanner, R Kogler, R Lange, J Lapsien, T Lenz, T Marchesini, I Ott, J Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A 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Duric, S. Friis, E. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Woods, N. CA CMS Collaboration TI Search for WW gamma and WZ gamma production and constraints on anomalous quartic gauge couplings in pp collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID CROSS-SECTION; LIMITS; LEP AB A search for WV gamma triple vector boson production is presented based on events containing a W boson decaying to a muon or an electron and a neutrino, a second V (W or Z) boson, and a photon. The data correspond to an integrated luminosity of 19.3 fb(-1) collected in 2012 with the CMS detector at the LHC in pp collisions at root s = 8 TeV. An upper limit of 311 fb on the cross section for the WV gamma production process is obtained at 95% confidence level for photons with a transverse energy above 30 GeV and with an absolute value of pseudorapidity of less than 1.44. This limit is approximately a factor of 3.4 larger than the standard model predictions that are based on next-to-leading order QCD calculations. Since no evidence of anomalous WW gamma gamma or WWZ gamma quartic gauge boson couplings is found, this paper presents the first experimental limits on the dimension-eight parameter f(T,0) and the CP-conserving WWZ gamma parameters kappa(W)(0) and kappa(W)(C). Limits are also obtained for the WW gamma gamma parameters a(0)(W) and a(C)(W). C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Ero, J.; Fabjan, C.; Friedl, M.; Fruhwirth, R.; Ghete, V. M.; Hartl, C.; Hormann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knunz, V.; Krammer, M.; Kratschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schofbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Suarez Gonzalez, J.] Nat Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Bansal, M.; Bansal, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Luyckx, S.; Ochesanu, S.; Roland, B.; Rougny, R.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Heracleous, N.; Kalogeropoulos, A.; Keaveney, J.; Kim, T. J.; Lowette, S.; Maes, M.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Velde, C. Vander; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Crucy, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.; Adiguzel, A.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Komm, M.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, Louvain, Belgium. 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L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; Hamel de Monchenault, G.; Jarry, P.; Locci, E.; Malcles, J.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sauvan, J.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.; Bernet, C.; Winn, D.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Bloch, D.; Brom, J. -M.; Chabert, E. 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[Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 3, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Guth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thuer, S.; Weber, M.] Rhein Westfal TH Aachen, Inst Phys A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Flugge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Inst Phys B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Kramer, M.; Krucker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Ntomari, E.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M.; Salfeld-Nebgen, J.; Saxena, P.; Schmidt, R.; Schoerner-Sadenius, T.; Schroder, M.; Stein, M.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] Deutsch Elekt Synchrotron, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Vignali, M. Centis; Enderle, H.; Erfle, J.; Garutti, E.; Goebel, K.; Gorner, M.; Gosselink, M.; Haller, J.; Hoing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbruck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Barth, C.] Univ Hamburg, Hamburg, Germany. [Baus, C.; Berger, J.; Boser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Muller, T.; Niegel, M.; Nurnberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Rocker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.; Bhardwaj, A.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Jones, J.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Sphicas, P.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kalsi, A. K.; Kaur, M.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, A.; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Mumbai, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dewanjee, R. K.; Dugad, S.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.; Zito, G.; Adair, A.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.; Albergo, S.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.; Albergo, S.] Univ Bologna, Bologna, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Tuve, C.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Moroni, L.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Galanti, M.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Ventura, S.; Zotto, P.; Zucchetta, A.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sez Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; Cruz-Burelo, E. De La; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.; Carrillo Moreno, S.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Popov, A.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potos, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.] Univ Canterbury, Christchurch 1, New Zealand. [Reucroft, S.; Ahmad, A.; Ahmad, M.; Asghar, M. I.; Butt, J.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Golutvin, I.; Gorbunov, I.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Y.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] Ctr Invest Energet & Medioambient CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Fabjan, C.; Fruhwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.; Dias, F. A.; Abdulsalam, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Gomez-Reino Garrido, R.; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Loureno, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schafer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Wohri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Radi, A.; Abdulsalam, A.; Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Konig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Nageli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Dunser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Nageli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Simili, E.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Caudron, A.; Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Ctr Nat Sci, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pesaresi, J. Pela M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Richardson, C.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; De La Barca Sanchez, M. Calderon; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.; Apresyan, A.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wurthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stockli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Sanders, D. A.; Summers, D.] Univ Mississippi, Minneapolis, MN USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. 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Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012 OI Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Gerosa, Raffaele/0000-0001-8359-3734; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Russ, James/0000-0001-9856-9155; Dudko, Lev/0000-0002-4462-3192; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Codispoti, Giuseppe/0000-0003-0217-7021; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Levchenko, Petr/0000-0003-4913-0538; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia) [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS program of Foundation for Polish Science - EU, Regional Development Fund; Thalis program - EU-ESF; Aristeia program - Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS program of Foundation for Polish Science, cofinanced by the EU, Regional Development Fund; and the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF. NR 59 TC 8 Z9 8 U1 3 U2 72 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 25 PY 2014 VL 90 IS 3 AR 032008 DI 10.1103/PhysRevD.90.032008 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO3WM UT WOS:000341267700001 ER PT J AU Yiu, Y Bonfa, P Sanna, S De Renzi, R Carretta, P McGuire, MA Huq, A Nagler, SE AF Yiu, Yuen Bonfa, Pietro Sanna, Samuele De Renzi, Roberto Carretta, Pietro McGuire, Michael A. Huq, Ashfia Nagler, Stephen E. TI Tuning the magnetic and structural phase transitions of PrFeAsO via Fe/Ru spin dilution SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTIVITY; NEUTRON AB Neutron diffraction and muon spin relaxation measurements are used to obtain a detailed phase diagram of PrFe1-xRuxAsO. The isoelectronic substitution of Ru for Fe acts effectively as spin dilution, suppressing both the structural and magnetic phase transitions. The temperature T-S of the tetragonal-orthorhombic structural phase transition decreases gradually as a function of x. Slightly below T-S, coherent precessions of the muon spin are observed corresponding to static magnetism, possibly reflecting a significant magnetoelastic coupling in the FeAs layers. Short-range order in both the Fe and Pr moments persists for higher levels of x. The static magnetic moments disappear at a concentration coincident with that expected for percolation of the J(1)-J(2) square-lattice model. C1 [Yiu, Yuen; Nagler, Stephen E.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Bonfa, Pietro; De Renzi, Roberto] Univ Parma, Dept Phys & Earth Sci, I-43124 Parma, Italy. [Sanna, Samuele; Carretta, Pietro] Univ Pavia, Dept Phys, I-27100 Pavia, Italy. [McGuire, Michael A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Huq, Ashfia] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Nagler, Stephen E.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Nagler, Stephen E.] Univ Tennessee, CIRE, Knoxville, TN 37996 USA. RP Yiu, Y (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM yyiu@utk.edu RI McGuire, Michael/B-5453-2009; Nagler, Stephen/E-4908-2010; Huq, Ashfia/J-8772-2013; Yiu, Yuen/A-4353-2010; De Renzi, Roberto/F-9182-2011 OI McGuire, Michael/0000-0003-1762-9406; Nagler, Stephen/0000-0002-7234-2339; Huq, Ashfia/0000-0002-8445-9649; Yiu, Yuen/0000-0002-1466-6191; De Renzi, Roberto/0000-0002-5015-0061 FU Scientific User Facilities Division of the Office of Science, Basic Energy Sciences, U. S. Department of Energy (BES DOE); Scientific User Facilities Division of BES DOE; Materials Sciences and Engineering Division of BES DOE; Fondazione Cariplo [2011-0266]; BES DOE, through the EPSCoR [DE-FG02-08ER46528]; [2012X3YFZ2] FX The research reported here utilized the mu SR facilities at the Paul Scherrer Institute, Villigen, Switzerland, and neutron scattering facilities at the Spallation Neutron Source, Oak Ridge National Laboratory (ORNL), which is sponsored by the Scientific User Facilities Division of the Office of Science, Basic Energy Sciences, U. S. Department of Energy (BES DOE). We are grateful to A. Amato and H. Luetkens of the Swiss Muon Source group for technical support. We would like to thank A. A. Aczel and T. J. Williams of ORNL for valuable conversations. A.H. and S.E.N. were supported by the Scientific User Facilities Division of BES DOE. M.A.M. was supported by the Materials Sciences and Engineering Division of BES DOE. S.S. and P.C. acknowledge the financial support of Fondazione Cariplo (Research Grant No. 2011-0266). R.D.R., P.B., P.C., and S.S. acknowledge partial support of PRIN2012 Project No. 2012X3YFZ2. Y.Y. was supported by the BES DOE, through the EPSCoR, Grant No. DE-FG02-08ER46528. NR 42 TC 4 Z9 4 U1 0 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 25 PY 2014 VL 90 IS 6 AR 064515 DI 10.1103/PhysRevB.90.064515 PG 8 WC Physics, Condensed Matter SC Physics GA AO3UY UT WOS:000341263000007 ER PT J AU Zou, Y Shao, ZH Peng, JH Li, FD Gong, DS Wang, CY Zuo, XB Zhang, ZY Wu, JH Shi, YY Gong, QG AF Zou, Yang Shao, Zhenhua Peng, Junhui Li, Fudong Gong, Deshun Wang, Chongyuan Zuo, Xiaobing Zhang, Zhiyong Wu, Jihui Shi, Yunyu Gong, Qingguo TI Crystal structure of triple-BRCT-domain of ECT2 and insights into the binding characteristics to CYK-4 SO FEBS LETTERS LA English DT Article DE The epithelial cell transforming protein 2; Triple-BRCT-domain; Auto-inhibition; Binding pocket; Phospho-peptide ID DNA-DAMAGE REPAIR; GTP-BOUND RHOA; CONTRACTILE RING; EXCHANGE FACTOR; MULTISITE PHOSPHORYLATION; CYTOKINESIS; PROTEIN; ACCUMULATION; RECOGNITION; REGION AB Homo sapiens ECT2 is a cell cycle regulator that plays critical roles in cytokinesis. ECT2 activity is restrained during interphase via intra-molecular interactions that involve its N-terminal triple-BRCT-domain and its C-terminal DH-PH domain. At anaphase, this self-inhibitory mechanism is relieved by Plk1-phosphorylated CYK-4, which directly engages the ECT2 BRCT domain. To provide a structural perspective for this auto-inhibitory property, we solved the crystal structure of the ECT2 triple-BRCT-domain. In addition, we systematically analyzed the interaction between the ECT2 BRCT domains with phospho-peptides derived from its binding partner CYK-4, and have identified Ser164 as the major phospho-residue that links CYK-4 to the second ECT2 BRCT domain. Structured summary of protein interactions: ECT2 and CYK-4 bind by isothermal titration calorimetry (1, 2, 3, 4, 5, 6, 7) (C) 2014 Federation of European Biochemical Societies. Published by Elsevier B.V. All rights reserved. C1 [Zou, Yang; Shao, Zhenhua; Peng, Junhui; Li, Fudong; Gong, Deshun; Wang, Chongyuan; Zhang, Zhiyong; Wu, Jihui; Shi, Yunyu; Gong, Qingguo] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Zou, Yang; Shao, Zhenhua; Peng, Junhui; Li, Fudong; Gong, Deshun; Wang, Chongyuan; Zhang, Zhiyong; Wu, Jihui; Shi, Yunyu; Gong, Qingguo] Univ Sci & Technol China, Sch Life Sci, Hefei 230026, Anhui, Peoples R China. [Zuo, Xiaobing] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60349 USA. RP Gong, QG (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. EM qgg@ustc.edu.cn OI Zuo, Xiaobing/0000-0002-0134-4804 FU National Basic Research Program of China (973 Program) [2011CB911104, 2013CB910200]; Chinese National Natural Science Foundation [31170693, 31330018, 31270760]; Chinese Academy of Sciences; Fundamental Research Funds for the Central Universities [WK2070000020] FX The National Basic Research Program of China (973 Program) [Grants 2011CB911104 and 2013CB910200]; Chinese National Natural Science Foundation [Grants 31170693, 31330018, 31270760]; "Outstanding Technical Talent'' project of the Chinese Academy of Sciences. Fundamental Research Funds for the Central Universities [WK2070000020]. NR 51 TC 4 Z9 4 U1 5 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0014-5793 EI 1873-3468 J9 FEBS LETT JI FEBS Lett. PD AUG 25 PY 2014 VL 588 IS 17 BP 2911 EP 2920 DI 10.1016/j.febslet.2014.07.019 PG 10 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA AN8VI UT WOS:000340882900022 PM 25068414 ER PT J AU Naulleau, PP Anderson, CN Anderson, EH Andreson, N Chao, WL Choi, C Goldberg, KA Gullikson, EM Kim, SS Lee, D Miyakawa, R Park, J Rekawa, S Salmassi, F AF Naulleau, Patrick P. Anderson, Christopher N. Anderson, Erik H. Andreson, Nord Chao, Weilun Choi, Changhoon Goldberg, Kenneth A. Gullikson, Eric M. Kim, Seong-Sue Lee, Donggun Miyakawa, Ryan Park, Jongju Rekawa, Seno Salmassi, Farhad TI Electro-optical system for scanning microscopy of extreme ultraviolet masks with a high harmonic generation source SO OPTICS EXPRESS LA English DT Article ID OPTICS; LIGHT; LASER; EUV AB A self-contained electro-optical module for scanning extreme ultraviolet (EUV) reflection microscopy at 13.5 nm wavelength has been developed. The system has been designed to work with stand-alone commercially available EUV high harmonic generation (HHG) sources through the implementation of narrowband harmonic selecting multilayers and off-axis elliptical short focal length zoneplates. The module has been successfully integrated into an EUV mask scanning microscope achieving diffraction limited imaging performance (84 nm point spread function). (C) 2014 Optical Society of America C1 [Naulleau, Patrick P.; Anderson, Christopher N.; Anderson, Erik H.; Andreson, Nord; Chao, Weilun; Goldberg, Kenneth A.; Gullikson, Eric M.; Miyakawa, Ryan; Rekawa, Seno; Salmassi, Farhad] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. [Choi, Changhoon; Kim, Seong-Sue; Lee, Donggun; Park, Jongju] Samsung Elect Co Ltd, Hwasung 445701, Gyeonggi, South Korea. RP Naulleau, PP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM pnaulleau@lbl.gov RI Anderson, Christopher/H-9526-2015 OI Anderson, Christopher/0000-0002-2710-733X FU Samsung Semiconductor through the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by Samsung Semiconductor through the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 26 TC 2 Z9 2 U1 1 U2 3 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD AUG 25 PY 2014 VL 22 IS 17 BP 20144 EP 20154 DI 10.1364/OE.22.020144 PG 11 WC Optics SC Optics GA AN6PJ UT WOS:000340717300049 PM 25321224 ER PT J AU Luk, TS Fofang, NT Cruz-Campa, JL Frank, I Campione, S AF Luk, Ting S. Fofang, Nche T. Cruz-Campa, Jose L. Frank, Ian Campione, Salvatore TI Surface plasmon polariton enhanced ultrathin nano-structured CdTe solar cell SO OPTICS EXPRESS LA English DT Article ID ABSORPTION ENHANCEMENT; SCATTERING; EFFICIENCY; GROWTH; ANTIREFLECTION; NANOPARTICLES; GRATINGS; (211)SI AB We demonstrate numerically that two-dimensional arrays of ultrathin CdTe nano-cylinders on Ag can serve as an effective broadband anti-reflection structure for solar cell applications. Such devices exhibit strong absorption properties, mainly in the CdTe semiconductor regions, and can produce short-circuit current densities of 23.4 mA/cm(2), a remarkable number in the context of solar cells given the ultrathin dimensions of our nano-cylinders. The strong absorption is enabled via excitation of surface plasmon polaritons (SPPs) under plane wave incidence. In particular, we identified the key absorption mechanism as enhanced fields of the SPP standing waves residing at the interface of CdTe nano-cylinders and Ag. We compare the performance of Ag, Au, and Al substrates, and observe significant improvement when using Ag, highlighting the importance of using low-loss metals. Although we use CdTe here, the proposed approach is applicable to other solar cell materials with similar absorption properties. (C) 2014 Optical Society of America C1 [Luk, Ting S.; Fofang, Nche T.; Frank, Ian; Campione, Salvatore] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Luk, Ting S.; Fofang, Nche T.; Cruz-Campa, Jose L.; Frank, Ian; Campione, Salvatore] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Luk, TS (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM tsluk@sandia.gov RI Campione, Salvatore/A-2349-2015 OI Campione, Salvatore/0000-0003-4655-5485 FU Sandia National Laboratory Directed Research Development; Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge fruitful discussion with Dr. Igal Brener. This work was supported by Sandia National Laboratory Directed Research Development and, in part, by the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 42 TC 4 Z9 4 U1 2 U2 45 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD AUG 25 PY 2014 VL 22 IS 17 BP A1372 EP A1379 DI 10.1364/OE.22.0A1372 PG 8 WC Optics SC Optics GA AN6PJ UT WOS:000340717300018 PM 25322192 ER PT J AU Perl, EE McMahon, WE Bowers, JE Friedman, DJ AF Perl, Emmett E. McMahon, William E. Bowers, John E. Friedman, Daniel J. TI Design of antireflective nanostructures and optical coatings for next-generation multijunction photovoltaic devices SO OPTICS EXPRESS LA English DT Article ID SOLAR-CELLS; EFFICIENCY; INDEX AB The successful development of multijunction photovoltaic devices with four or more subcells has placed additional importance on the design of high-quality broadband antireflection coatings. Antireflective nanostructures have shown promise for reducing reflection loss compared to the best thin-film interference coatings. However, material constraints make nanostructures difficult to integrate without introducing additional absorption or electrical losses. In this work, we compare the performance of various nanostructure configurations with that of an optimized multilayer antireflection coating. Transmission into a four-junction solar cell is computed for each antireflective design, and the corresponding cell efficiency is calculated. We find that the best performance is achieved with a hybrid configuration that combines nanostructures with a multilayer thin-film optical coating. This approach increases transmitted power into the top subcell by 1.3% over an optimal thin-film coating, corresponding to an increase of approximately 0.8% in the modeled cell efficiency. (C)2014 Optical Society of America C1 [Perl, Emmett E.; Bowers, John E.] Univ Calif Santa Barbara, Dept Elect & Comp Engn, Santa Barbara, CA 93106 USA. [McMahon, William E.; Friedman, Daniel J.] Natl Renewable Energy Lab, Concentrated Photovolta Grp, Golden, CO 80401 USA. RP Perl, EE (reprint author), Univ Calif Santa Barbara, Dept Elect & Comp Engn, Santa Barbara, CA 93106 USA. EM emmettperl@ece.ucsb.edu FU Center for Energy Efficient Materials, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001009]; National Science Foundation Graduate Research Fellowship [DGE-1144085] FX This material is based upon work supported by the Center for Energy Efficient Materials, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001009. Emmett E. Perl is supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE-1144085. NR 34 TC 6 Z9 7 U1 3 U2 40 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD AUG 25 PY 2014 VL 22 IS 17 BP A1243 EP A1256 DI 10.1364/OE.22.0A1243 PG 14 WC Optics SC Optics GA AN6PJ UT WOS:000340717300005 PM 25322179 ER PT J AU Kogan, VG Prozorov, R AF Kogan, V. G. Prozorov, R. TI Anisotropic criteria for the type of superconductivity SO PHYSICAL REVIEW B LA English DT Article ID INTERCALATION COMPOUNDS; CRITICAL-FIELD; TEMPERATURE; DEPENDENCE; EQUATIONS; STABILITY AB The classical criterion for classification of superconductors as type I or type II based on the isotropic Ginzburg-Landau theory is generalized to arbitrary temperatures for materials with anisotropic Fermi surfaces and order parameters. We argue that the relevant quantity for this classification is the ratio of the upper and thermodynamic critical fields H-c2/H-c, rather than the traditional ratio of the penetration depth and the coherence length lambda/xi. Even in the isotropic case, H-c2/H-c coincides with root 2 lambda/xi only at the critical temperature T-c and they differ as T decreases, the long-known fact. Anisotropies of Fermi surfaces and order parameters may amplify this difference and render false the criterion based on the value of kappa = lambda/xi. C1 [Kogan, V. G.] Iowa State Univ, Ames Lab DOE, Ames, IA 50011 USA. Iowa State Univ, Dept Phys, Ames, IA 50011 USA. RP Kogan, VG (reprint author), Iowa State Univ, Ames Lab DOE, Ames, IA 50011 USA. EM kogan@ameslab.gov; prozorov@ameslab.gov FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; Iowa State University [DE-AC02-07CH11358] FX The authors are grateful to M. A. Tanatar for helpful discussions. This work was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The work was done at the Ames Laboratory, which is operated for the US DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 31 TC 3 Z9 3 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 25 PY 2014 VL 90 IS 5 AR 054516 DI 10.1103/PhysRevB.90.054516 PG 8 WC Physics, Condensed Matter SC Physics GA AO3UT UT WOS:000341262500005 ER PT J AU Pastore, S Wiringa, RB Pieper, SC Schiavilla, R AF Pastore, S. Wiringa, R. B. Pieper, Steven C. Schiavilla, R. TI Quantum Monte Carlo calculations of electromagnetic transitions in Be-8 with meson-exchange currents derived from chiral effective field theory SO PHYSICAL REVIEW C LA English DT Article ID LIGHT-NUCLEI; A=8 AB We report quantum Monte Carlo calculations of electromagnetic transitions in Be-8. The realistic Argonne upsilon(18) two-nucleon and Illinois-7 three-nucleon potentials are used to generate the ground state and nine excited states, with energies that are in excellent agreement with experiment. A dozen M1 and eight E2 transition matrix elements between these states are then evaluated. The E2 matrix elements are computed only in impulse approximation, with those transitions from broad resonant states requiring special treatment. The M1 matrix elements include two-body meson-exchange currents derived from chiral effective field theory, which typically contribute 20%-30% of the total expectation value. Many of the transitions are between isospin-mixed states; the calculations are performed for isospin-pure states and then combined with empirical mixing coefficients to compare to experiment. Alternate mixings are also explored. In general, we find that transitions between states that have the same dominant spatial symmetry are in reasonable agreement with experiments, but transitions between different spatial symmetries are often underpredicted. C1 [Pastore, S.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Wiringa, R. B.; Pieper, Steven C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Schiavilla, R.] Jefferson Lab, Theory Ctr, Newport News, VA 23606 USA. [Schiavilla, R.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. RP Pastore, S (reprint author), Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. EM pastores@mailbox.sc.edu; wiringa@anl.gov; spieper@anl.gov; schiavil@jlab.org RI Wiringa, Robert/M-4970-2015 FU National Science Foundation [PHY-1068305]; US Department of Energy, Office of Nuclear Physics [DE-FG02-09ER41621, DE-AC02-06CH11357, DE-AC05-06OR23177]; NUCLEI SciDAC-3 grant FX The many-body calculations were performed on the parallel computers at the Laboratory Computing Resource Center, Argonne National Laboratory. This work was supported by the National Science Foundation, Grant No. PHY-1068305 (S.P.), and by the US Department of Energy, Office of Nuclear Physics, under Contracts No. DE-FG02-09ER41621 (S.P.), No. DE-AC02-06CH11357 (S.C.P. and R.B.W.) and No. DE-AC05-06OR23177 (R.S.) and under the NUCLEI SciDAC-3 grant. NR 34 TC 7 Z9 7 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 25 PY 2014 VL 90 IS 2 AR 024321 DI 10.1103/PhysRevC.90.024321 PG 12 WC Physics, Nuclear SC Physics GA AO3VY UT WOS:000341266100002 ER PT J AU Robinson, DJ Tsai, Y AF Robinson, Dean J. Tsai, Yuhsin TI Dynamical framework for KeV Dirac neutrino warm dark matter SO PHYSICAL REVIEW D LA English DT Article ID RAY-LINE SIGNAL; STERILE NEUTRINOS; REIONIZATION; MODELS; SCALE; MECHANISM; SPECTRUM; UNIVERSE; POWER AB If the source of the reported 3.5 keV x-ray line is a sterile neutrino, comprising an O(1) fraction of the dark matter (DM), then it exhibits the property that its mass times mixing angle is similar to few x 10(-2) eV, a plausible mass scale for the active neutrinos. This property is a common feature of Dirac neutrino mixing. We present a framework that dynamically produces light active and keV sterile Dirac neutrinos, with appropriate mixing angles to be the x-ray line source. The central idea is that the right-handed active neutrino is a composite state, while elementary sterile neutrinos gain keV masses similarly to the quarks in extended technicolor. The entire framework is fixed by just two dynamical scales and may automatically exhibit a warm dark matter (WDM) production mechanism-dilution of thermal relics from late decays of a heavy composite neutrino-such that the keV neutrinos may comprise an O(1) fraction of the DM. In this framework, the WDM is typically quite cool and within structure formation bounds, with temperature similar to few x 10(-2)T(v) and free-streaming length similar to few kpc. A toy model that exhibits the central features of the framework is also presented. C1 [Robinson, Dean J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Robinson, Dean J.] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tsai, Yuhsin] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. RP Robinson, DJ (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM djrobinson@berkeley.edu; yhtsai@ucdavis.edu OI Tsai, Yuhsin/0000-0001-7847-225X FU U.S. National Science Foundation [PHY-1002399]; Department of Energy [DE-FG02-91ER40674]; hospitality of the Center for Future High Energy Physics in Beijing, China FX The authors thank Simone Alioli, Tom Banks, Francesco D'Eramo, Howie Haber, Zoltan Ligeti, Joel Primack, Joshua Ruderman and Jon Walsh for helpful discussions. We particularly thank Duccio Pappadopulo for providing valuable comments during the preparation of this work. The work of D. R. is supported by the U.S. National Science Foundation under Grant No. PHY-1002399. The work of Y. T. is supported by the Department of Energy under Grant No. DE-FG02-91ER40674. The work of Y.T. was also supported by the hospitality of the Center for Future High Energy Physics in Beijing, China. NR 67 TC 20 Z9 20 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 25 PY 2014 VL 90 IS 4 AR 045030 DI 10.1103/PhysRevD.90.045030 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO3WS UT WOS:000341268400012 ER PT J AU Morgado, L Lourenco, S Londer, YY Schiffer, M Pokkuluri, PR Salgueiro, CA AF Morgado, Leonor Lourenco, Silvia Londer, Yuri Y. Schiffer, Marianne Pokkuluri, P. Raj Salgueiro, Carlos A. TI Dissecting the Functional Role of Key Residues in Triheme Cytochrome PpcA: A Path to Rational Design of G-sulfurreducens Strains with Enhanced Electron Transfer Capabilities SO PLOS ONE LA English DT Article ID C-TYPE CYTOCHROME; GEOBACTER-SULFURREDUCENS; THERMODYNAMIC CHARACTERIZATION; DESULFOVIBRIO-VULGARIS; ESCHERICHIA-COLI; C(7); FAMILY; PHYSIOLOGY; REDUCTION; PROTEINS AB PpcA is the most abundant member of a family of five triheme cytochromes c(7) in the bacterium Geobacter sulfurreducens (Gs) and is the most likely carrier of electrons destined for outer surface during respiration on solid metal oxides, a process that requires extracellular electron transfer. This cytochrome has the highest content of lysine residues (24%) among the family, and it was suggested to be involved in e(-)/H+ energy transduction processes. In the present work, we investigated the functional role of lysine residues strategically located in the vicinity of each heme group. Each lysine was replaced by glutamine or glutamic acid to evaluate the effects of a neutral or negatively charged residue in each position. The results showed that replacing Lys(9) (located near heme IV), Lys(18) (near heme I) or Lys(22) (between hemes I and III) has essentially no effect on the redox properties of the heme groups and are probably involved in redox partner recognition. On the other hand, Lys(43) (near heme IV), Lys(52) (between hemes III and IV) and Lys(60) (near heme III) are crucial in the regulation of the functional mechanism of PpcA, namely in the selection of microstates that allow the protein to establish preferential e(-)/H+ transfer pathways. The results showed that the preferred e(-)/H+ transfer pathways are only established when heme III is the last heme to oxidize, a feature reinforced by a higher difference between its reduction potential and that of its predecessor in the order of oxidation. We also showed that K43 and K52 mutants keep the mechanistic features of PpcA by establishing preferential e(-)/H+ transfer pathways at lower reduction potential values than the wild-type protein, a property that can enable rational design of Gs strains with optimized extracellular electron transfer capabilities. C1 [Morgado, Leonor; Lourenco, Silvia; Salgueiro, Carlos A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Quim, Requimte,CQFB, Caparica, Portugal. [Londer, Yuri Y.; Schiffer, Marianne; Pokkuluri, P. Raj] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Salgueiro, CA (reprint author), Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Quim, Requimte,CQFB, Caparica, Portugal. EM csalgueiro@fct.unl.pt RI Salgueiro, Carlos/A-4522-2013; Morgado, Leonor/D-7387-2013 OI Salgueiro, Carlos/0000-0003-1136-809X; Morgado, Leonor/0000-0002-3760-5180 FU Fundacao para a Cieancia e a Tecnologia (FCT), Portugal [PEst-C/EQB/LA0006/2013]; Fundacao para a Cieancia e a Tecnologia [RECI/BBB-BQB/0230/2012]; division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy program [DE-AC02-06CH11357]; [PTDC/BBB-BEP/0753/2012] FX This work was supported by project grant PTDC/BBB-BEP/0753/2012 (to CAS) and the strategic grant PEst-C/EQB/LA0006/2013 (to REQUIMTE Laboratorio Associado) from Fundacao para a Cieancia e a Tecnologia (FCT), Portugal. The NMR spectrometers are part of The National NMR Facility, supported by Fundacao para a Cieancia e a Tecnologia (RECI/BBB-BQB/0230/2012). PRP is partially supported by the division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy program under contract no. DE-AC02-06CH11357 (URL:http://www.fct.pt). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 30 TC 6 Z9 6 U1 1 U2 5 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 25 PY 2014 VL 9 IS 8 AR e105566 DI 10.1371/journal.pone.0105566 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN9TR UT WOS:000340952200061 PM 25153891 ER PT J AU Liu, XG Mao, DQ Cole, JM Xu, ZC AF Liu, Xiaogang Mao, Deqi Cole, Jacqueline M. Xu, Zhaochao TI Temperature insensitive fluorescence intensity in a coumarin monomer-aggregate coupled system SO CHEMICAL COMMUNICATIONS LA English DT Article ID LASER-INDUCED FLUORESCENCE; PERYLENE BISIMIDE DYES; INDUCED EMISSION; PROBES; THERMOMETRY; BIOLOGY; STATE; WATER; FIELD AB The emission intensities of a fluorescent monomer-aggregate coupled system, based on 7-(dimethylamino)-coumarin-3-carbaldehyde, exhibit ultra-low temperature dependence with a low temperature coefficient of only 0.05% per degrees C, by judicious selection of the excitation wavelength. This finding has significant implications to temperature-sensitive fluorescent applications. C1 [Liu, Xiaogang; Cole, Jacqueline M.] Univ Cambridge, Dept Phys, Cavendish Lab, Cambridge CB3 0HE, England. [Mao, Deqi; Xu, Zhaochao] Chinese Acad Sci, Dalian Inst Chem Phys, Key Lab Separat Sci Analyt Chem, Dalian 116023, Peoples R China. [Mao, Deqi; Xu, Zhaochao] Dalian Univ Technol, State Key Lab Fine Chem, Dalian 116012, Peoples R China. [Cole, Jacqueline M.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Cole, JM (reprint author), Univ Cambridge, Dept Phys, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England. EM jmc61@cam.ac.uk; zcxu@dicp.ac.cn RI Cole, Jacqueline/C-5991-2008; Liu, Xiaogang/H-2189-2011 OI Liu, Xiaogang/0000-0002-2553-2068 FU EPSRC UK National Service for Computational Chemistry Software (NSCCS), at Imperial College London; Argonne National Laboratory; DOE Office of Science, Office of Basic Energy Sciences [DE-ACO2-06CH11357]; National Natural Science Foundation of China [21276251]; Ministry of Human Resources and Social Security of PRC; 100 Talents Program - Chinese Academy of Sciences, State Key Laboratory of Fine Chemicals of China [KF1105]; Singapore Economic Development Board FX The authors wish to thank the EPSRC UK National Service for Computational Chemistry Software (NSCCS), based at Imperial College London, for supporting this work. X.L. is indebted to the Singapore Economic Development Board for a Clean Energy Scholarship. J.M.C. thanks the Fulbright Commission for a UK-US Fulbright Scholar Award hosted by Argonne National Laboratory where work done was supported by DOE Office of Science, Office of Basic Energy Sciences, under Contract No. DE-ACO2-06CH11357. Z.X. is supported by the National Natural Science Foundation of China (21276251), Ministry of Human Resources and Social Security of PRC, the 100 Talents Program funded by Chinese Academy of Sciences, State Key Laboratory of Fine Chemicals of China (KF1105). NR 31 TC 3 Z9 3 U1 6 U2 60 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 EI 1364-548X J9 CHEM COMMUN JI Chem. Commun. PD AUG 25 PY 2014 VL 50 IS 66 BP 9329 EP 9332 DI 10.1039/c4cc04245j PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AN1ON UT WOS:000340353300023 PM 25000229 ER PT J AU Farmer, JM Boatner, LA Chakoumakos, BC Du, MH Lance, MJ Rawn, CJ Bryan, JC AF Farmer, J. Matt Boatner, Lynn A. Chakoumakos, Bryan C. Du, Mao-Hua Lance, Michael J. Rawn, Claudia J. Bryan, Jeff C. TI Structural and crystal chemical properties of rare-earth titanate pyrochlores SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Rare earth compounds; Pyrochlores; Single crystal X-ray diffraction; Crystal growth; Thermal expansion; Density functional theory ID OXIDE PYROCHLORES; IMMOBILIZATION; A(2)B(2)O(7); SPECTROSCOPY; MINERALS; GD2TI2O7; DAMAGE AB Rare-earth titanates, RE2Ti2O7 (where RE = a rare-earth) with the pyrochlore structure continue to be investigated for use as potential stable host materials for nuclear and actinide-rich wastes. Accordingly, the present work is directed towards the elucidation of the fundamental structural, physical, and thermochemical properties of this class of compounds. Single-crystals of the rare earth pyrochlores were synthesized using a high-temperature flux technique and were subsequently characterized using single-crystal X-ray diffraction. The cubic lattice parameters display an approximately linear correlation with the RE-site cation radius. Theoretical calculations of the lattice constants and bond lengths of the subject materials were carried out using density functional theory, and the results are compared to the experimental values. The Sm and Eu titanates exhibit a covalency increase between the REO8 and TiO6 polyhedral resulting in a deviation from the increasing linear lattice parameter through the transition series. Gd2Ti2O7 with the 4f(7) half-filled f-orbital Gd3+ sub-shell exhibits the lowest 48f oxygen positional parameter. The coefficient of thermal expansion for the rare-earth titanate series is approximately linear, and it has a range of 10.1-11.2 x 10 (6) degrees C (1). Raman spectroscopy indicated that the similar to 530 cm (1) peak associated with the Ti-O stretching mode follows a general trend of decreasing frequency with increasing RE reduced mass. (C) 2014 Elsevier B.V. All rights reserved. C1 [Farmer, J. Matt; Boatner, Lynn A.; Du, Mao-Hua; Lance, Michael J.; Rawn, Claudia J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Boatner, Lynn A.; Du, Mao-Hua] Oak Ridge Natl Lab, ORNL Ctr Radiat Detect Mat & Syst, Oak Ridge, TN 37831 USA. [Chakoumakos, Bryan C.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Rawn, Claudia J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Bryan, Jeff C.] Univ Wisconsin, Dept Chem & Biochem, La Crosse, WI 54601 USA. RP Boatner, LA (reprint author), 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM boatnerla@ornl.gov RI Boatner, Lynn/I-6428-2013; Lance, Michael/I-8417-2016; Du, Mao-Hua/B-2108-2010; Chakoumakos, Bryan/A-5601-2016; Farmer, Matt/C-2571-2016 OI Boatner, Lynn/0000-0002-0235-7594; Lance, Michael/0000-0001-5167-5452; Du, Mao-Hua/0000-0001-8796-167X; Chakoumakos, Bryan/0000-0002-7870-6543; Farmer, Matt/0000-0002-7279-1847 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX Research at the Oak Ridge National Laboratory was sponsored by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. The contributions of Sandra Salmen and Allison Gray to the preparation of the manuscript are gratefully acknowledged. NR 37 TC 13 Z9 13 U1 15 U2 91 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD AUG 25 PY 2014 VL 605 BP 63 EP 70 DI 10.1016/j.jallcom.2014.03.153 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AH2CE UT WOS:000335927500010 ER PT J AU Ermanoski, I AF Ermanoski, Ivan TI Cascading pressure thermal reduction for efficient solar fuel production SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen; Thermochemical; Solar fuels; Carbon dioxide ID WATER; HYDROGEN; SYSTEM; OXYGEN; CERIA; HEAT AB Efficient two-step solar-thermochemical fuel production requires vacuum pumping or inert gas sweeping to lower the oxygen pressure in the thermal reduction step. Pumping is hampered by large oxygen volumetric flows, whereas sweeping is energy-intensive, requiring heat recovery at high temperature, and a dedicated inert gas purification plant. A novel pumping approach-using a cascade of chambers at successively lower pressures-is analyzed and shown to lead to over an order of magnitude pressure decrease compared to a single-chambered design. The resulting efficiency gains are substantial, and represent an important step toward practical and efficient solar fuel production on a large scale. Copyright (C) 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ermanoski, I (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM iermano@sandia.gov FU U.S. Department of Energy Fuel Cell Technologies Program via the Solar Thermochemical Hydrogen (STCH) directive; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the U.S. Department of Energy Fuel Cell Technologies Program via the Solar Thermochemical Hydrogen (STCH) directive. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 14 TC 10 Z9 10 U1 0 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD AUG 22 PY 2014 VL 39 IS 25 BP 13114 EP 13117 DI 10.1016/j.ijhydene.2014.06.143 PG 4 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA AO4WX UT WOS:000341343200007 ER PT J AU Chylek, LA Akimov, V Dengjel, J Rigbolt, KTG Hu, B Hlavacek, WS Blagoev, B AF Chylek, Lily A. Akimov, Vyacheslav Dengjel, Joern Rigbolt, Kristoffer T. G. Hu, Bin Hlavacek, William S. Blagoev, Blagoy TI Phosphorylation Site Dynamics of Early T-cell Receptor Signaling SO PLOS ONE LA English DT Article ID WISKOTT-ALDRICH-SYNDROME; PROTEIN-TYROSINE KINASE; TERMINAL SRC KINASE; QUANTITATIVE PHOSPHOPROTEOMIC ANALYSIS; PROLINE-RICH SEQUENCE; TANDEM SH2 DOMAINS; RULE-BASED MODELS; ANTIGEN RECEPTOR; ADAPTER PROTEIN; PHOSPHOLIPASE C-GAMMA-1 AB In adaptive immune responses, T-cell receptor (TCR) signaling impacts multiple cellular processes and results in T-cell differentiation, proliferation, and cytokine production. Although individual protein-protein interactions and phosphorylation events have been studied extensively, we lack a systems-level understanding of how these components cooperate to control signaling dynamics, especially during the crucial first seconds of stimulation. Here, we used quantitative proteomics to characterize reshaping of the T-cell phosphoproteome in response to TCR/CD28 co-stimulation, and found that diverse dynamic patterns emerge within seconds. We detected phosphorylation dynamics as early as 5 s and observed widespread regulation of key TCR signaling proteins by 30 s. Development of a computational model pointed to the presence of novel regulatory mechanisms controlling phosphorylation of sites with central roles in TCR signaling. The model was used to generate predictions suggesting unexpected roles for the phosphatase PTPN6 (SHP-1) and shortcut recruitment of the actin regulator WAS. Predictions were validated experimentally. This integration of proteomics and modeling illustrates a novel, generalizable framework for solidifying quantitative understanding of a signaling network and for elucidating missing links. C1 [Chylek, Lily A.; Hu, Bin; Hlavacek, William S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Chylek, Lily A.; Hlavacek, William S.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Chylek, Lily A.] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY USA. [Akimov, Vyacheslav; Blagoev, Blagoy] Univ Southern Denmark, Dept Biochem & Mol Biol, Odense M, Denmark. [Dengjel, Joern; Rigbolt, Kristoffer T. G.] Univ Freiburg, ZBSA Ctr Biol Syst Anal, BIOSS Ctr Biol Signalling Studies, Freiburg Inst Adv Studies FRIAS,Med Ctr,Dept Derm, D-79106 Freiburg, Germany. [Hu, Bin; Hlavacek, William S.] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. RP Hlavacek, WS (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM wish@lanl.gov; bab@bmb.sdu.dk OI Blagoev, Blagoy/0000-0002-3596-0066; Hlavacek, William/0000-0003-4383-8711 FU National Institutes of Health/National Institute of General Medical Sciences (NIH/NIGMS) [P50GM085273, R01GM076570]; US Department of Energy [DE-AC52-06NA25396]; Excellence Initiative of the German Federal and State Governments through the Freiburg Institute for Advanced Studies (FRIAS) in the School of Life Sciences-LifeNet; Center for Biological Signalling Studies (BIOSS); Danish Council for Independent Research/Natural Sciences; Lundbeck Foundation FX This work was supported by National Institutes of Health/National Institute of General Medical Sciences (NIH/NIGMS) grants P50GM085273 and R01GM076570; US Department of Energy Contract DE-AC52-06NA25396 through the Los Alamos Center for Nonlinear Studies and the Laboratory-directed Research and Development (LDRD) Program; the Excellence Initiative of the German Federal and State Governments through the Freiburg Institute for Advanced Studies (FRIAS) in the School of Life Sciences-LifeNet, and the Center for Biological Signalling Studies (BIOSS); the Danish Council for Independent Research/Natural Sciences; and the Lundbeck Foundation. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 221 TC 13 Z9 13 U1 0 U2 15 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 22 PY 2014 VL 9 IS 8 AR e104240 DI 10.1371/journal.pone.0104240 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AO3LL UT WOS:000341230600012 PM 25147952 ER PT J AU Lee, SW Geller, JT Torok, T Wu, CH Singer, M Reid, FC Tarjan, DR Hazen, TC Arkin, AP Hillson, NJ AF Lee, Sangwon Geller, Jil T. Torok, Tamas Wu, Cindy H. Singer, Mary Reid, Francine C. Tarjan, Daniel R. Hazen, Terry C. Arkin, Adam P. Hillson, Nathan J. TI Characterization of Wastewater Treatment Plant Microbial Communities and the Effects of Carbon Sources on Diversity in Laboratory Models SO PLOS ONE LA English DT Article ID SYNTHETIC-BIOLOGY; SUBSTRATE-SPECIFICITY; PSEUDOMONAS-PUTIDA; BACTERIA; GENE; DEHALOGENASE; BIOCHEMISTRY; DATABASE; INSIGHT; ENZYMES AB We are developing a laboratory-scale model to improve our understanding and capacity to assess the biological risks of genetically engineered bacteria and their genetic elements in the natural environment. Our hypothetical scenario concerns an industrial bioreactor failure resulting in the introduction of genetically engineered bacteria to a downstream municipal wastewater treatment plant (MWWTP). As the first step towards developing a model for this scenario, we sampled microbial communities from the aeration basin of a MWWTP at three seasonal time points. Having established a baseline for community composition, we investigated how the community changed when propagated in the laboratory, including cell culture media conditions that could provide selective pressure in future studies. Specifically, using PhyloChip 16S-rRNA-gene targeting microarrays, we compared the compositions of sampled communities to those of inocula propagated in the laboratory in simulated wastewater conditionally amended with various carbon sources (glucose, chloroacetate, D-threonine) or the ionic liquid 1-ethyl-3-methylimidazolium chloride ([C2mim]Cl). Proteobacteria, Bacteroidetes, and Actinobacteria were predominant in both aeration basin and laboratory-cultured communities. Laboratory-cultured communities were enriched in gamma-Proteobacteria. Enterobacteriaceae, and Aeromonadaceae were enriched by glucose, Pseudomonadaceae by chloroacetate and D-threonine, and Burkholderiacea by high (50 mM) concentrations of chloroacetate. Microbial communities cultured with chloroacetate and D-threonine were more similar to sampled field communities than those cultured with glucose or [C2mim]Cl. Although observed relative richness in operational taxonomic units (OTUs) was lower for laboratory cultures than for field communities, both flask and reactor systems supported phylogenetically diverse communities. These results importantly provide a foundation for laboratory models of industrial bioreactor failure scenarios. C1 [Lee, Sangwon; Tarjan, Daniel R.; Arkin, Adam P.; Hillson, Nathan J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Geller, Jil T.; Torok, Tamas; Wu, Cindy H.; Singer, Mary; Reid, Francine C.; Hazen, Terry C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Hillson, NJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM njhillson@lbl.gov RI Arkin, Adam/A-6751-2008; Hazen, Terry/C-1076-2012 OI Arkin, Adam/0000-0002-4999-2931; Hazen, Terry/0000-0002-2536-9993 FU Office of Science, Office of Biological and Environmental Research, of the United States Department of Energy [DE-AC02-05CH11231] FX This work, performed in part at the Joint BioEnergy Institute, was supported by the Office of Science, Office of Biological and Environmental Research, of the United States Department of Energy (http://science.energy.gov/ber/) under Contract No. DE-AC02-05CH11231 to Lawrence Berkeley National Laboratory (to TCH, APA, and NJH). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 41 TC 0 Z9 0 U1 5 U2 24 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 22 PY 2014 VL 9 IS 8 AR e105689 DI 10.1371/journal.pone.0105689 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AO3LL UT WOS:000341230600070 PM 25148472 ER PT J AU Gilbert, JA Jansson, JK Knight, R AF Gilbert, Jack A. Jansson, Janet K. Knight, Rob TI The Earth Microbiome project: successes and aspirations SO BMC BIOLOGY LA English DT Editorial Material ID DIVERSITY; SOILS C1 [Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Lemont, IL 60439 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Gilbert, Jack A.] Zhejiang Univ, Coll Environm & Resource Sci, Hangzhou 310058, Zhejiang, Peoples R China. [Jansson, Janet K.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Knight, Rob] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Knight, Rob] Univ Colorado, BioFrontiers Inst, Boulder, CO 80309 USA. [Knight, Rob] Univ Colorado, Howard Hughes Med Inst, Boulder, CO 80309 USA. RP Knight, R (reprint author), Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. EM rob.knight@colorado.edu RI Knight, Rob/D-1299-2010 NR 21 TC 90 Z9 93 U1 14 U2 90 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1741-7007 J9 BMC BIOL JI BMC Biol. PD AUG 22 PY 2014 VL 12 AR 69 DI 10.1186/s12915-014-0069-1 PG 4 WC Biology SC Life Sciences & Biomedicine - Other Topics GA AN9IG UT WOS:000340919300001 PM 25184604 ER PT J AU Anisovich, AV Beck, R Burkert, V Klempt, E McCracken, ME Nikonov, VA Sarantsev, AV Schumacher, RA Thoma, U AF Anisovich, A. V. Beck, R. Burkert, V. Klempt, E. McCracken, M. E. Nikonov, V. A. Sarantsev, A. V. Schumacher, R. A. Thoma, U. TI Energy-independent PWA of the reaction gamma p -> K+Lambda SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID MESON PHOTOPRODUCTION; BARYON RESONANCES; SPIN OBSERVABLES; TRANSITION; LAMBDA; MODEL; PION; SIGMA(0); ETA AB Using all recent data on the differential cross sections and spin observables for the reaction gamma p -> K+Lambda, an energy-independent partial-wave analysis is performed for center-of-mass energies from 1.462 to 1.662 GeV. The analysis requires multipoles up to L = 2; there is no evidence that the fit requires multipoles with L = 3. At present the available data allow us to extract the dominant multipoles only. These are compatible with the multipoles obtained in the energy-dependent fit. This result supports the reliability of the Bonn-Gatchina energy-dependent results. C1 [Anisovich, A. V.; Beck, R.; Klempt, E.; Nikonov, V. A.; Sarantsev, A. V.; Thoma, U.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, Bonn, Germany. [Anisovich, A. V.; Nikonov, V. A.; Sarantsev, A. V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Burkert, V.] Jefferson Lab, Newport News, VA USA. [McCracken, M. E.] Washington & Jefferson Coll, Washington, PA USA. [McCracken, M. E.; Schumacher, R. A.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. RP Anisovich, AV (reprint author), Univ Bonn, Helmholtz Inst Strahlen & Kernphys, Bonn, Germany. EM klempt@hiskp.uni-bonn.de RI Schumacher, Reinhard/K-6455-2013 OI Schumacher, Reinhard/0000-0002-3860-1827 NR 38 TC 3 Z9 3 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD AUG 22 PY 2014 VL 50 IS 8 AR 129 DI 10.1140/epja/i2014-14129-3 PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AN9QJ UT WOS:000340942200001 ER PT J AU Lindmaa, A Mattsson, AE Armiento, R AF Lindmaa, A. Mattsson, A. E. Armiento, R. TI Quantum oscillations in the kinetic energy density: Gradient corrections from the Airy gas SO PHYSICAL REVIEW B LA English DT Article ID INHOMOGENEOUS ELECTRON-GAS; THOMAS-FERMI APPROXIMATION; SURFACE AB We derive a closed-form expression for the quantum corrections to the kinetic energy density in the Thomas-Fermi limit of a linear potential model system in three dimensions (the Airy gas). The universality of the expression is tested numerically in a number of three-dimensional model systems: (i) jellium surfaces, (ii) confinement in a hydrogenlike potential (the Bohr atom), (iii) particles confined by a harmonic potential in one and (iv) all three dimensions, and (v) a system with a cosine potential (the Mathieu gas). Our results confirm that the usual gradient expansion of extended Thomas-Fermi theory does not describe the quantum oscillations for systems that incorporate surface regions where the electron density drops off to zero. We find that the correction derived from the Airy gas is universally applicable to relevant spatial regions of systems of types (i), (ii), and (iv), but somewhat surprisingly not (iii). We discuss possible implications of our findings to the development of functionals for the kinetic energy density. C1 [Lindmaa, A.; Armiento, R.] Linkoping Univ, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden. [Mattsson, A. E.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Lindmaa, A (reprint author), Linkoping Univ, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden. EM alexander.lindmaa@liu.se; aematts@sandia.gov; rickard.armiento@liu.se RI Armiento, Rickard/E-1413-2011 OI Armiento, Rickard/0000-0002-5571-0814 FU Swedish Research Council (VR) [621-2011-4249]; Linnaeus Environment at Linkoping on Nanoscale Functional Materials (LiLi-NFM) - VR; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We acknowledge support from the Swedish Research Council (VR), Grant No. 621-2011-4249, as well as the Linnaeus Environment at Linkoping on Nanoscale Functional Materials (LiLi-NFM) funded by VR. A.L. thanks Dr. Olle Hellman for valuable input on the presentation. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 41 TC 5 Z9 5 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 22 PY 2014 VL 90 IS 7 AR 075139 DI 10.1103/PhysRevB.90.075139 PG 15 WC Physics, Condensed Matter SC Physics GA AO3NO UT WOS:000341238200002 ER PT J AU Moriarty, JA Haskins, JB AF Moriarty, John A. Haskins, Justin B. TI Efficient wide-range calculation of free energies in solids and liquids using reversible-scaling molecular dynamics SO PHYSICAL REVIEW B LA English DT Article ID STRUCTURAL PHASE-STABILITY; EQUATION-OF-STATE; TRANSITION-METALS; INTERATOMIC POTENTIALS; HIGH-PRESSURE; ATOMISTIC SIMULATION; TANTALUM; MAGNESIUM; THERMODYNAMICS; ALUMINUM AB We elaborate a novel and efficient method to obtain multiphase Helmholtz free energies from molecular dynamics (MD) simulations over wide ranges of volume and temperature in materials that can be described by temperature-independent ion forces, with both higher accuracy and order-of-magnitude cost savings compared to direct thermodynamic-integration techniques. Our method leverages and significantly extends the technique of reversible-scaling molecular dynamics (RSMD) proposed by de Koning et al. [Phys. Rev. Lett. 83, 3973 (1999)], which allows a free-energy difference in a given phase at constant volume to be calculated as a function of temperature from a single MD simulation. In mechanically stable solid phases, our approach carefully combines quasiharmonic lattice dynamics at low temperatures with an accurate and fully isolated RSMD simulation of the anharmonic vibrational free energy at high temperatures to produce a seamless free energy from zero temperature to above melt along constant-volume isochores. In the liquid, we combine a unique calculation of the free energy along a high-temperature reference isotherm with isochoric RSMD simulations from that temperature to below melt. In metastable solid phases that are mechanically unstable at low temperature, we use two-phase MD melt simulations together with the liquid free energy to obtain the solid free energy along the solidus melt line and then perform isochoric RSMD simulations to temperatures above and below that point. While our free-energy method is general, we have specifically adapted it here to the case of metals in which the ion forces are well described by model generalized pseudopotential theory (MGPT) multi-ion interatomic potentials, and additive electron-thermal free-energy contributions can be included. Then using refined Ta6.8x MGPT potentials, we have converged total free energies and their components to very high and unprecedented sub-milli-Rydberg (mRy) numerical accuracy in the stable-bcc, liquid, and metastable-fcc phases of tantalum for volumes ranging from up to 26% expansion to nearly twofold compression and for temperatures to 25 000 K. In turn, we have successfully used the free energies so obtained to calculate physically accurate thermodynamic properties and gain new insight into their behavior, including sensitive thermodynamic derivatives, bcc and fcc melt curves, and a multiphase equation of state for tantalum (Ta) over the same temperature range and for pressures as high as 600 GPa. We show that the anharmonic free-energy component in the bcc solid, although only 1-5 mRy in magnitude for Ta, can have a significant (15%-20%) effect on thermal expansivity, the Gruneisen parameter, and melt temperatures. We further show that the electron-thermal free-energy component can similarly impact the specific heat and thermal expansivity in both the solid and the liquid, while only minimally affecting (to <= 3%) the bcc and fcc melt curves. C1 [Moriarty, John A.] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94551 USA. [Haskins, Justin B.] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. RP Moriarty, JA (reprint author), Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94551 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE SciDAC [DE-FC02-06ER25788] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. J.B.H. acknowledges support as a summer student at LLNL in 2011 from DOE SciDAC Grant No. DE-FC02-06ER25788, during which time some of this work was begun. NR 59 TC 2 Z9 2 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 22 PY 2014 VL 90 IS 5 AR 054113 DI 10.1103/PhysRevB.90.054113 PG 19 WC Physics, Condensed Matter SC Physics GA AO3NI UT WOS:000341237600002 ER PT J AU Singh, S Fitzsimmons, MR Lookman, T Jeen, H Biswas, A AF Singh, Surendra Fitzsimmons, M. R. Lookman, T. Jeen, H. Biswas, A. TI Elastically controlled manipulation of the magnetic order parameter and the metal-insulator transition in a manganite thin film SO PHYSICAL REVIEW B LA English DT Article ID COLOSSAL MAGNETORESISTANCE; PERCOLATION-THRESHOLD; ELECTRONIC PHASE; STRAIN; SEPARATION; LATTICE; STRESS AB We measured the temperature dependence of the saturation magnetization (M-s) of a (La1-xPrx)(1-y)CayMnO3 (x similar to 0.60, y similar to 0.33) film as a function of applied bending stress. Stress producing a compressive strain of -0.01% along the magnetic easy axis increased the Curie temperature by similar to 6 K and the metal-insulator transition by similar to 4 K. Regardless of whether or not stress is applied to the film, magnetic ordering occurs at temperatures significantly higher than the metal-insulator-transition temperature. The magnetization of the sample at the temperature of the metal-insulator transition is approximately the site percolation threshold for a two-dimensional spin lattice. C1 [Singh, Surendra] Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. [Fitzsimmons, M. R.; Lookman, T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Jeen, H.; Biswas, A.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Jeen, H.] Pusan Natl Univ, Dept Phys, Pusan 609735, South Korea. RP Singh, S (reprint author), Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. EM surendra@barc.gov.in FU Office of Basic Energy Science (BES), U.S. Department of Energy (DOE), National Science Foundation [DMR-0804452]; Los Alamos National Security LLC under DOE [DE-AC52-06NA25396] FX This work was supported by the Office of Basic Energy Science (BES), U.S. Department of Energy (DOE), the National Science Foundation (Grant No. DMR-0804452) (H.J. and A. B.). Discussions with Professor S. K. Sinha, Professor Ivan K. Schuller, Dr. S. Guenon, Dr. G. Ramirez, and Dr. T. Saerbeck are gratefully acknowledged. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract No. DE-AC52-06NA25396. NR 34 TC 2 Z9 2 U1 1 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 22 PY 2014 VL 90 IS 6 AR 060407 DI 10.1103/PhysRevB.90.060407 PG 5 WC Physics, Condensed Matter SC Physics GA AO3NL UT WOS:000341237900001 ER PT J AU Kim, EH Johnson, JR AF Kim, E. -H. Johnson, J. R. TI Comment on "Mode Conversion of Waves in the Ion-Cyclotron Frequency Range in Magnetospheric Plasmas" SO PHYSICAL REVIEW LETTERS LA English DT Editorial Material C1 [Kim, E. -H.; Johnson, J. R.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Kim, EH (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM ehkim@pppl.gov; jrj@pppl.gov NR 3 TC 3 Z9 3 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 22 PY 2014 VL 113 IS 8 AR 089501 DI 10.1103/PhysRevLett.113.089501 PG 1 WC Physics, Multidisciplinary SC Physics GA AO3QE UT WOS:000341247600009 PM 25192130 ER PT J AU Gomez, LF Ferguson, KR Cryan, JP Bacellar, C Tanyag, RMP Jones, C Schorb, S Anielski, D Belkacem, A Bernando, C Boll, R Bozek, J Carron, S Chen, G Delmas, T Englert, L Epp, SW Erk, B Foucar, L Hartmann, R Hexemer, A Huth, M Kwok, J Leone, SR Ma, JHS Maia, FRNC Malmerberg, E Marchesini, S Neumark, DM Poon, B Prell, J Rolles, D Rudek, B Rudenko, A Seifrid, M Siefermann, KR Sturm, FP Swiggers, M Ullrich, J Weise, F Zwart, P Bostedt, C Gessner, O Vilesov, AF AF Gomez, Luis F. Ferguson, Ken R. Cryan, James P. Bacellar, Camila Tanyag, Rico Mayro P. Jones, Curtis Schorb, Sebastian Anielski, Denis Belkacem, Ali Bernando, Charles Boll, Rebecca Bozek, John Carron, Sebastian Chen, Gang Delmas, Tjark Englert, Lars Epp, Sascha W. Erk, Benjamin Foucar, Lutz Hartmann, Robert Hexemer, Alexander Huth, Martin Kwok, Justin Leone, Stephen R. Ma, Jonathan H. S. Maia, Filipe R. N. C. Malmerberg, Erik Marchesini, Stefano Neumark, Daniel M. Poon, Billy Prell, James Rolles, Daniel Rudek, Benedikt Rudenko, Artem Seifrid, Martin Siefermann, Katrin R. Sturm, Felix P. Swiggers, Michele Ullrich, Joachim Weise, Fabian Zwart, Petrus Bostedt, Christoph Gessner, Oliver Vilesov, Andrey F. TI Shapes and vorticities of superfluid helium nanodroplets SO SCIENCE LA English DT Article ID LIQUID-HELIUM; STABILITY; DROP AB Helium nanodroplets are considered ideal model systems to explore quantum hydrodynamics in self-contained, isolated superfluids. However, exploring the dynamic properties of individual droplets is experimentally challenging. In this work, we used single-shot femtosecond x-ray coherent diffractive imaging to investigate the rotation of single, isolated superfluid helium-4 droplets containing similar to 10(8) to 10(11) atoms. The formation of quantum vortex lattices inside the droplets is confirmed by observing characteristic Bragg patterns from xenon clusters trapped in the vortex cores. The vortex densities are up to five orders of magnitude larger than those observed in bulk liquid helium. The droplets exhibit large centrifugal deformations but retain axially symmetric shapes at angular velocities well beyond the stability range of viscous classical droplets. C1 [Gomez, Luis F.; Tanyag, Rico Mayro P.; Jones, Curtis; Seifrid, Martin; Vilesov, Andrey F.] Univ Southern Calif USC, Dept Chem, Los Angeles, CA 90089 USA. [Ferguson, Ken R.; Schorb, Sebastian; Bozek, John; Carron, Sebastian; Swiggers, Michele; Bostedt, Christoph] SLAC Natl Accelerator Lab, Linac Coherent Light Source LCLS, Menlo Pk, CA 94025 USA. [Cryan, James P.; Bacellar, Camila; Belkacem, Ali; Leone, Stephen R.; Ma, Jonathan H. S.; Neumark, Daniel M.; Siefermann, Katrin R.; Sturm, Felix P.; Weise, Fabian; Gessner, Oliver] Lawrence Berkeley Natl Lab LBNL, Ultrafast X Ray Sci Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Bacellar, Camila; Leone, Stephen R.; Neumark, Daniel M.; Prell, James] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Anielski, Denis; Boll, Rebecca; Epp, Sascha W.; Erk, Benjamin; Rudek, Benedikt; Rudenko, Artem; Ullrich, Joachim] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Anielski, Denis; Boll, Rebecca; Epp, Sascha W.; Erk, Benjamin; Foucar, Lutz; Rolles, Daniel; Rudek, Benedikt; Rudenko, Artem; Ullrich, Joachim] Ctr Free Electron Laser Sci CFEL, Max Planck Adv Study Grp, D-22607 Hamburg, Germany. [Bernando, Charles; Vilesov, Andrey F.] USC, Dept Phys & Astron, Los Angeles, CA 90089 USA. [Boll, Rebecca; Erk, Benjamin; Rolles, Daniel] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany. [Chen, Gang; Hexemer, Alexander; Marchesini, Stefano] LBNL, Adv Light Source, Berkeley, CA 94720 USA. [Delmas, Tjark] DESY, CFEL, D-22607 Hamburg, Germany. [Englert, Lars] Max Planck Inst Extraterr Phys, D-85741 Garching, Germany. [Foucar, Lutz; Rolles, Daniel] Max Planck Inst Med Res, D-69120 Heidelberg, Germany. [Hartmann, Robert; Huth, Martin] PNSensor GmbH, D-81739 Munich, Germany. [Kwok, Justin] USC, Mork Family Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ma, Jonathan H. S.] Chinese Univ Hong Kong, Dept Phys, Hong Kong, Peoples R China. [Maia, Filipe R. N. C.] LBNL, Natl Energy Res Sci Comp Ctr, Berkeley, CA 94720 USA. [Malmerberg, Erik; Poon, Billy; Zwart, Petrus] LBNL, Phys Biosci Div, Berkeley, CA 94720 USA. [Malmerberg, Erik] Univ Calfornia Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Marchesini, Stefano] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Rudenko, Artem] Kansas State Univ, Dept Phys, James R Macdonald Lab, Manhattan, KS 66506 USA. [Bostedt, Christoph] Stanford Univ, PULSE Inst, Menlo Pk, CA 94025 USA. [Bostedt, Christoph] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Bostedt, C (reprint author), SLAC Natl Accelerator Lab, Linac Coherent Light Source LCLS, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM bostedt@slac.stanford.edu; ogessner@lbl.gov; vilesov@usc.edu RI Rudenko, Artem/C-7412-2009; Neumark, Daniel/B-9551-2009; Bozek, John/E-9260-2010; Rudek, Benedikt/A-5100-2017; OI Rudenko, Artem/0000-0002-9154-8463; Neumark, Daniel/0000-0002-3762-9473; Bozek, John/0000-0001-7486-7238; Rocha Neves Couto Maia, Filipe/0000-0002-2141-438X; Epp, Sascha/0000-0001-6366-9113; Boll, Rebecca/0000-0001-6286-4064 FU NSF [CHE-1112391]; U.S. Department of Energy (DOE), Office of Basic Energy Sciences (OBES), Chemical Sciences, Geosciences and Biosciences Division [DE-AC02-05CH11231]; Max Planck Society; U.S. DOE OBES [L549]; Office of the Secretary of Defense, National Security Science and Engineering Faculty Fellowship; PULSE Institute at SLAC National Accelerator Laboratory - U.S. DOE OBES [DE-AC02-76SF00515]; USC; Center for Applied Mathematics for Energy Research Applications (CAMERA); NSF; USC Dornsife College of Letters, Arts and Sciences; Alexander von Humboldt Foundation FX This work was supported by NSF grant CHE-1112391 (A. F. V.) at USC; the U.S. Department of Energy (DOE), Office of Basic Energy Sciences (OBES), Chemical Sciences, Geosciences and Biosciences Division through contract no. DE-AC02-05CH11231; and the Max Planck Society by funding the development and operation of the CFEL Advanced Study Group (ASG) Multi-Purpose (CAMP) instrument. Portions of this research were carried out at the LCLS, a national user facility operated by Stanford University on behalf of the U.S. DOE OBES under beam-time grant L549: Imaging of quantum vortices in superfluid helium droplets. S. R. L. and J. P. acknowledge support from the Office of the Secretary of Defense, National Security Science and Engineering Faculty Fellowship. C. B. was partially supported through the PULSE Institute at SLAC National Accelerator Laboratory funded by the U.S. DOE OBES under contract no. DE-AC02-76SF00515. J. K. was supported by the USC Undergraduate Research Associates Program. S. M. was supported by the Center for Applied Mathematics for Energy Research Applications (CAMERA). A. R. was supported by the NSF. M. Seifrid was supported by the USC Dornsife College of Letters, Arts and Sciences Student Opportunities for Academic Research and Summer Undergraduate Research Fund fellowships. K. R. S. was supported by the Alexander von Humboldt Foundation. NR 27 TC 47 Z9 48 U1 6 U2 109 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 22 PY 2014 VL 345 IS 6199 BP 906 EP 909 DI 10.1126/science.1252395 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN3YL UT WOS:000340524700039 PM 25146284 ER PT J AU Azubel, M Koivisto, J Malola, S Bushnell, D Hura, GL Koh, AL Tsunoyama, H Tsukuda, T Pettersson, M Hakkinen, H Kornberg, RD AF Azubel, Maia Koivisto, Jaakko Malola, Sami Bushnell, David Hura, Greg L. Koh, Ai Leen Tsunoyama, Hironori Tsukuda, Tatsuya Pettersson, Mika Hakkinen, Hannu Kornberg, Roger D. TI Electron microscopy of gold nanoparticles at atomic resolution SO SCIENCE LA English DT Article ID CRYSTAL-STRUCTURE; PROTECTED AU-25; NANOCLUSTERS; CLUSTER AB Structure determination of gold nanoparticles (AuNPs) is necessary for understanding their physical and chemical properties, but only one AuNP larger than 1 nanometer in diameter [a 102-gold atom NP (Au102NP)] has been solved to atomic resolution. Whereas the Au102NP structure was determined by x-ray crystallography, other large AuNPs have proved refractory to this approach. Here, we report the structure determination of a Au68NP at atomic resolution by aberration-corrected transmission electron microscopy, performed with the use of a minimal electron dose, an approach that should prove applicable to metal NPs in general. The structure of the Au68NP was supported by small-angle x-ray scattering and by comparison of observed infrared absorption spectra with calculations by density functional theory. C1 [Azubel, Maia; Bushnell, David; Kornberg, Roger D.] Stanford Univ, Sch Med, Dept Struct Biol, Stanford, CA 94305 USA. [Koivisto, Jaakko; Pettersson, Mika; Hakkinen, Hannu] Univ Jyvaskyla, Nanosci Ctr, Dept Chem, FI-40014 Jyvaskyla, Finland. [Malola, Sami; Hakkinen, Hannu] Univ Jyvaskyla, Nanosci Ctr, Dept Phys, FI-40014 Jyvaskyla, Finland. [Hura, Greg L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Koh, Ai Leen] Stanford Univ, Stanford Nanocharacterizat Lab, Stanford, CA 94305 USA. [Tsunoyama, Hironori; Tsukuda, Tatsuya] Hokkaido Univ, Catalysis Res Ctr, Sapporo, Hokkaido 060, Japan. RP Kornberg, RD (reprint author), Stanford Univ, Sch Med, Dept Struct Biol, Stanford, CA 94305 USA. EM kornberg@stanford.edu RI Tsukuda, Tatsuya/G-4979-2014; Tsunoyama, Hironori/D-7124-2014 OI Tsukuda, Tatsuya/0000-0002-0190-6379; Tsunoyama, Hironori/0000-0002-0332-5324 FU Human Frontier Science Program Organization; NIH [AI-21144]; Academy of Finland; National Graduate School in Computational Chemistry and Spectroscopy LASKEMO; U.S. Department of Energy [DE-AC02-05CH11231] FX The work at Stanford University was supported by the Human Frontier Science Program Organization (M. A.) and NIH grant AI-21144 (R. D. K). The work at the University of Jyvaskyla was supported by the Academy of Finland (H. H. and M. P.) and the National Graduate School in Computational Chemistry and Spectroscopy LASKEMO (J. K.). G. L. H was supported by U.S. Department of Energy Biological and Environmental Research grant DE-AC02-05CH11231 under Integrated Diffraction Analysis Technologies. We thank P. Robinson for assistance with EM processing and helpful discussions and E. Hulkko and P. A. Clayborne for help with spectroscopic experiments and preliminary computations, respectively. NR 23 TC 84 Z9 85 U1 19 U2 207 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 22 PY 2014 VL 345 IS 6199 BP 909 EP 912 DI 10.1126/science.1251959 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN3YL UT WOS:000340524700040 PM 25146285 ER PT J AU Liao, HG Zherebetskyy, D Xin, HL Czarnik, C Ercius, P Elmlund, H Pan, M Wang, LW Zheng, HM AF Liao, Hong-Gang Zherebetskyy, Danylo Xin, Huolin Czarnik, Cory Ercius, Peter Elmlund, Hans Pan, Ming Wang, Lin-Wang Zheng, Haimei TI Facet development during platinum nanocube growth SO SCIENCE LA English DT Article ID ELECTRON-MICROSCOPY; GOLD NANOPARTICLES; NANOCRYSTALS; LIQUID; SHAPE; CHEMISTRY AB An understanding of how facets of a nanocrystal develop is critical for controlling nanocrystal shape and designing novel functional materials. However, the atomic pathways of nanocrystal facet development are mostly unknown because of the lack of direct observation. We report the imaging of platinum nanocube growth in a liquid cell using transmission electron microscopy with high spatial and temporal resolution. The growth rates of all low index facets are similar until the {100} facets stop growth. The continuous growth of the rest facets leads to a nanocube. Our calculation shows that the much lower ligand mobility on the {100} facets is responsible for the arresting of {100} growing facets. These findings shed light on nanocrystal shape-control mechanisms and future design of nanomaterials. C1 [Liao, Hong-Gang; Zherebetskyy, Danylo; Xin, Huolin; Wang, Lin-Wang; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Czarnik, Cory; Pan, Ming] Gatan Inc, Pleasanton, CA 94588 USA. [Ercius, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Elmlund, Hans] Stanford Univ, Sch Med, Dept Biol Struct, Stanford, CA 94305 USA. [Zheng, Haimei] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Zheng, HM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM hmzheng@lbl.gov RI Zherebetskyy, Danylo/B-3404-2015; Liao, hong-gang/M-2476-2015; Foundry, Molecular/G-9968-2014; Xin, Huolin/E-2747-2010 OI Xin, Huolin/0000-0002-6521-868X FU U.S. Department of Energy (DOE) Office of Basic Energy Sciences [DE-AC02-05CH11231]; DOE Office of Science FX We thank B. Sadtler for useful comments on the manuscript. Part of the in situ experiments was performed at Gatan, Incorporated using a Tecnai equipped with a K2-IS camera. We also used FEI Titan, Tecnai UT20, JOEL3010, and TEAM0.5 microscopes at the National Center for Electron Microscopy of Lawrence Berkeley National Laboratory, which is supported by the U.S. Department of Energy (DOE) Office of Basic Energy Sciences under contract no. DE-AC02-05CH11231. H. Z. was a residency faculty member of SinBeRise program of BEARS at University of California, Berkeley, during July 2013 to January 2014 and thanks the DOE Office of Science Early Career Research Program for support. NR 21 TC 82 Z9 82 U1 35 U2 228 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 22 PY 2014 VL 345 IS 6199 BP 916 EP 919 DI 10.1126/science.1253149 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN3YL UT WOS:000340524700042 PM 25146287 ER PT J AU Wang, YN Su, ZH Wu, W Nie, S Lu, XH Wang, HY McCarty, K Pei, SS Robles-Hernandez, F Hadjiev, VG Bao, JM AF Wang, Yanan Su, Zhihua Wu, Wei Nie, Shu Lu, Xinghua Wang, Haiyan McCarty, Kevin Pei, Shin-shem Robles-Hernandez, Francisco Hadjiev, Viktor G. Bao, Jiming TI Four-fold Raman enhancement of 2D band in twisted bilayer graphene: evidence for a doubly degenerate Dirac band and quantum interference SO NANOTECHNOLOGY LA English DT Article DE twisted bilayer graphene; Raman scattering; quantum interference ID SCATTERING; SUPERLATTICES; SPECTROSCOPY; FERMIONS; MODES AB We report the observation of a strong 2D band Raman in twisted bilayer graphene (tBLG) with large rotation angles under 638 nm and 532 nm visible laser excitations. The 2D band Raman intensity increased four-fold as opposed to the two-fold increase observed in single-layer graphene. The same tBLG samples also exhibited rotation-dependent G-line resonances and folded phonons under 364 nm UV laser excitation. We attribute this 2D band Raman enhancement to the constructive interference between two double-resonance Raman pathways, which were enabled by a nearly degenerate Dirac band in the tBLG Moire superlattices. C1 [Wang, Yanan; Su, Zhihua; Wu, Wei; Pei, Shin-shem; Bao, Jiming] Univ Houston, Dept Elect & Comp Engn, Houston, TX 77204 USA. [Wu, Wei; Pei, Shin-shem; Bao, Jiming] Univ Houston, Ctr Adv Mat, Houston, TX 77204 USA. [Nie, Shu; McCarty, Kevin] Sandia Natl Labs, Livermore, CA 94550 USA. [Lu, Xinghua] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Wang, Haiyan] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Robles-Hernandez, Francisco] Univ Houston, Coll Engn Technol, Houston, TX 77204 USA. [Hadjiev, Viktor G.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Hadjiev, Viktor G.] Univ Houston, Dept Mech Engn, Houston, TX 77204 USA. RP Wang, YN (reprint author), Univ Houston, Dept Elect & Comp Engn, Houston, TX 77204 USA. EM jbao@uh.edu RI Wang, Haiyan/P-3550-2014; Hadjiev, Viktor/A-7069-2008; OI Wang, Haiyan/0000-0002-7397-1209; Hadjiev, Viktor/0000-0001-8579-9357; ROBLES HERNANDEZ, FRANCISCO/0000-0001-5587-0802 FU Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the US DOE [DE-AC04-94AL85000]; Delta Electronics Foundation; UH CAM; National Science Foundation [ECCS-1240510]; Robert A Welch Foundation [E-1728]; State of Texas through the Texas Center for Superconductivity at the University of Houston FX The work at Sandia National Laboratories was supported by the Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the US DOE under contract No. DE-AC04-94AL85000. SSP, JMB and WW acknowledge support from the Delta Electronics Foundation and the UH CAM. JMB acknowledges support from the National Science Foundation (Career Award ECCS-1240510, monitored by Anupama Kaul; DMR-0907336, monitored by Charles Ying) and from the Robert A Welch Foundation (E-1728). VGH work was supported by the State of Texas through the Texas Center for Superconductivity at the University of Houston. We thank Nicholas Padula for proofreading the manuscript. NR 44 TC 4 Z9 4 U1 1 U2 35 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD AUG 22 PY 2014 VL 25 IS 33 AR 335201 DI 10.1088/0957-4484/25/33/335201 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA AM1NQ UT WOS:000339613600003 PM 25073903 ER PT J AU Rideout, JR He, Y Navas-Molina, JA Walters, WA Ursell, LK Gibbons, SM Chase, J McDonald, D Gonzalez, A Robbins-Pianka, A Clemente, JC Gilbert, JA Huse, SM Zhou, HW Knight, R Caporaso, JG AF Rideout, Jai Ram He, Yan Navas-Molina, Jose A. Walters, William A. Ursell, Luke K. Gibbons, Sean M. Chase, John McDonald, Daniel Gonzalez, Antonio Robbins-Pianka, Adam Clemente, Jose C. Gilbert, Jack A. Huse, Susan M. Zhou, Hong-Wei Knight, Rob Caporaso, J. Gregory TI Subsampled open-reference clustering creates consistent, comprehensive OTU definitions and scales to billions of sequences SO PEERJ LA English DT Article DE OTU picking; Microbial ecology; Microbiome; Qiime; Bioinformatics ID GREENGENES; QIIME AB We present a performance-optimized algorithm, subsampled open-reference OTU picking, for assigning marker gene (e.g., 16S rRNA) sequences generated on next-generation sequencing platforms to operational taxonomic units (OTUs) for microbial community analysis. This algorithm provides benefits over de novo OTU picking (clustering can be performed largely in parallel, reducing runtime) and close-dreference OTU picking (all reads are clustered, not only those that match a reference database sequence with high similarity). Because more of our algorithm can be run in parallel relative to "classic" open-reference OTU picking, it makes open-reference OTU picking tractable on massive amplicon sequence data sets (though on smaller data sets, "classic" open-reference OTU clustering is often faster). We illustrate that here by applying it to the first 15,000 samples sequenced for the Earth Microbiome Project (1.3 billion V4 16S rRNA amplicons). To the best of our knowledge, this is the largest OTU picking run ever performed, and we estimate that our new algorithm runs in less than 1/5 the time than would be required of "classic" open reference OTU picking. We show that subsampled open-reference OTU picking yields results that are highly correlated with those generated by "classic" open-reference OTU picking through comparisons on three well-studied datasets. An implementation of this algorithm is provided in the popular QIIME software package, which uses uclust for read clustering. All analyses were performed using QIIME's uclust wrappers, though we provide details (aided by the open-source code in our GitHub repository) that will allow implementation of subsampled open-reference OTU picking independently of QIIME (e.g., in a compiled programming language, where runtimes should be further reduced). Our analyses should generalize to other implementations of these OTU picking algorithms. Finally, we present a comparison of parameter settings in QIIME's OTU picking workflows and make recommendations on settings for these free parameters to optimize runtime without reducing the quality of the results. These optimized parameters can vastly decrease the runtime of uclust-based OTU picking in QIIME. C1 [Rideout, Jai Ram; Caporaso, J. Gregory] No Arizona Univ, Ctr Microbial Genet & Gen, Flagstaff, AZ 86011 USA. [Rideout, Jai Ram; Clemente, Jose C.] Icahn Sch Med Mt Sinai, Dept Genet & Genom Sci, New York, NY 10029 USA. [He, Yan; Zhou, Hong-Wei] Southern Med Univ, Sch Publ Hlth & Trop Med, State Key Lab Organ Failure Prevent, Guangzhou, Guangdong, Peoples R China. [He, Yan; Zhou, Hong-Wei] Southern Med Univ, Sch Publ Hlth & Trop Med, Dept Environm Hlth, Guangzhou, Guangdong, Peoples R China. [Navas-Molina, Jose A.; McDonald, Daniel; Robbins-Pianka, Adam] Univ Colorado, Dept Comp Sci, Boulder, CO 80309 USA. [Walters, William A.] Univ Colorado, Dept Mol Cellular & Dev Biol, Boulder, CO 80309 USA. [Ursell, Luke K.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Gibbons, Sean M.] Univ Chicago, Grad Program Biophys Sci, Chicago, IL 60637 USA. [Chase, John; Caporaso, J. Gregory] No Arizona Univ, Dept Biol Sci, Flagstaff, AZ 86011 USA. [McDonald, Daniel; Gonzalez, Antonio; Robbins-Pianka, Adam; Knight, Rob] Univ Colorado, BioFrontiers Inst, Boulder, CO 80309 USA. [Gibbons, Sean M.; Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Lemont, IL USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Huse, Susan M.] Brown Univ, Warren Alpert Med Sch, Dept Pathol & Lab Sci, Providence, RI 02912 USA. [Knight, Rob] Univ Colorado, Howard Hughes Med Inst, Boulder, CO 80309 USA. RP Caporaso, JG (reprint author), No Arizona Univ, Ctr Microbial Genet & Gen, Flagstaff, AZ 86011 USA. EM gregcaporaso@gmail.com RI Knight, Rob/D-1299-2010 FU EPA STAR Graduate Fellowship; NSF IGERT [1144807]; Arizona's Technology and Research Initiative Fund; Alfred P. Sloan Foundation [2012-5-42 MBRP] FX SMG was supported by an EPA STAR Graduate Fellowship. DM was supported in part by NSF IGERT (award number: 1144807). This work was partially supported by a grant from Arizona's Technology and Research Initiative Fund to JGC, and by a grant from the Alfred P. Sloan Foundation to JGC and RK (award number: 2012-5-42 MBRP). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 19 TC 65 Z9 66 U1 11 U2 39 PU PEERJ INC PI LONDON PA 341-345 OLD ST, THIRD FLR, LONDON, EC1V 9LL, ENGLAND SN 2167-8359 J9 PEERJ JI PeerJ PD AUG 21 PY 2014 VL 2 AR e545 DI 10.7717/peerj.545 PG 25 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY5NB UT WOS:000347618000003 PM 25177538 ER PT J AU Garcia, I Geisz, JF France, RM Kang, J Wei, SH Ochoa, M Friedman, DJ AF Garcia, I. Geisz, J. F. France, R. M. Kang, J. Wei, S. -H. Ochoa, M. Friedman, D. J. TI Metamorphic Ga0.76In0.24As/GaAs0.75Sb0.25 tunnel junctions grown on GaAs substrates SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID QUASI-RANDOM STRUCTURES; EPITAXIAL-GROWTH; BEAM EPITAXY; BAND OFFSETS; ALLOYS; GAAS1-XSBX; LAYERS; SEMICONDUCTORS; GAAS0.5SB0.5; DIODES AB Lattice-matched and pseudomorphic tunnel junctions have been developed in the past for application in a variety of semiconductor devices, including heterojunction bipolar transistors, vertical cavity surface-emitting lasers, and multijunction solar cells. However, metamorphic tunnel junctions have received little attention. In 4-junction Ga0.51In0.49P/GaAs/Ga0.76In0.24As/Ga0.47In0.53As inverted-metamorphic solar cells (4J-IMM), a metamorphic tunnel junction is required to series connect the 3rd and 4th junctions. We present a tunnel junction based on a metamorphic Ga0.76In0.24As/GaAs0.75Sb0.25 structure for this purpose. This tunnel junction is grown on a metamorphic Ga0.76In0.24As template on a GaAs substrate. The band offsets in the resulting type-II heterojunction are calculated using the first-principles density functional method to estimate the tunneling barrier height and assess the performance of this tunnel junction against other material systems and compositions. The effect of the metamorphic growth on the performance of the tunnel junctions is analyzed using a set of metamorphic templates with varied surface roughness and threading dislocation density. Although the metamorphic template does influence the tunnel junction performance, all tunnel junctions measured have a peak current density over 200 A/cm(2). The tunnel junction on the best template has a peak current density over 1500 A/cm(2) and a voltage drop at 15 A/cm(2) (corresponding to operation at 1000 suns) lower than 10mV, which results in a nearly lossless series connection of the 4th junction in the 4J-IMM structure. (C) 2014 AIP Publishing LLC. C1 [Garcia, I.; Geisz, J. F.; France, R. M.; Kang, J.; Wei, S. -H.; Ochoa, M.; Friedman, D. J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Garcia, I.; Ochoa, M.] Univ Politecn Madrid, Inst Energia Solar, E-28040 Madrid, Spain. RP Garcia, I (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. RI Garcia, Ivan/L-1547-2014 OI Garcia, Ivan/0000-0002-9895-2020 FU People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme under REA [299878]; U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX The authors thankfully acknowledge the invaluable support by W. Olavarria and M. Young growing and processing the semiconductor devices. I. Garcia holds an IOF grant from the People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme (FP7/2007-2013) under REA grant agreement No. 299878. This work is supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 37 TC 4 Z9 4 U1 0 U2 21 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2014 VL 116 IS 7 AR 074508 DI 10.1063/1.4892773 PG 6 WC Physics, Applied SC Physics GA AO2XB UT WOS:000341189400059 ER PT J AU Yu, XB Wang, XX Zhang, QL Li, JC Liu, JF AF Yu, Xiaobai Wang, Xiaoxin Zhang, Qinglin Li, Juchuan Liu, Jifeng TI Oxidation-resistant, solution-processed plasmonic Ni nanochain-SiOx (x < 2) selective solar thermal absorbers SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MICRO-RAMAN SPECTROSCOPY; HYDROGEN SILSESQUIOXANE; NICKEL SILICIDES; HSQ FILMS; COATINGS; NANOPARTICLES; SILICON; XPS AB Metal oxidation at high temperatures has long been a challenge in cermet solar thermal absorbers, which impedes the development of atmospherically stable, high-temperature, high-performance concentrated solar power (CSP) systems. In this work, we demonstrate solution-processed Ni nanochain-SiOx (x < 2) and Ni nanochain-SiO2 selective solar thermal absorbers that exhibit a strong anti-oxidation behavior up to 600 degrees C in air. The thermal stability is far superior to previously reported Ni nanoparticle-Al2O3 selective solar thermal absorbers, which readily oxidize at 450 degrees C. The SiOx (x < 2) and SiO2 matrices are derived from hydrogen silsesquioxane and tetraethyl orthosilicate precursors, respectively, which comprise Si-O cage-like structures and Si-O networks. Fourier transform infrared spectroscopy shows that the dissociation of Si-O cage-like structures and Si-O networks at high temperatures have enabled the formation of new bonds at the Ni/SiOx interface to passivate the surface of Ni nanoparticles and prevent oxidation. X-ray photoelectron spectroscopy and Raman spectroscopy demonstrate that the excess Si in the SiOx (x < 2) matrices reacts with Ni nanostructures to form silicides at the interfaces, which further improves the anti-oxidation properties. As a result, Ni-SiOx (x < 2) systems demonstrate better anti-oxidation performance than Ni-SiO2 systems. This oxidation-resistant Ni nanochain-SiOx (x < 2) cermet coating also exhibits excellent high-temperature optical performance, with a high solar absorptance of similar to 90% and a low emittance similar to 18% measured at 300 degrees C. These results open the door towards atmospheric stable, high temperature, high-performance solar selective absorber coatings processed by low-cost solution-chemical methods for future generations of CSP systems. (C) 2014 AIP Publishing LLC. C1 [Yu, Xiaobai; Wang, Xiaoxin; Liu, Jifeng] Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA. [Zhang, Qinglin] Univ Kentucky, Dept Chem & Mat Engn, Lexington, KY 40506 USA. [Li, Juchuan] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Liu, JF (reprint author), Dartmouth Coll, Thayer Sch Engn, 14 Engn Dr, Hanover, NH 03755 USA. EM Jifeng.Liu@dartmouth.edu RI Zhang, Qinglin/D-9258-2013; Li, Juchuan/A-2992-2009 OI Zhang, Qinglin/0000-0001-5933-4361; Li, Juchuan/0000-0002-6587-5591 FU National Science Foundation (NSF) Small Business Innovation Research (SBIR) Program via Norwich Technologies, Inc. [1315245] FX This work has been supported by National Science Foundation (NSF) Small Business Innovation Research (SBIR) Program under the contract number 1315245 via the subcontract from Norwich Technologies, Inc. We would also like to thank Ms. Veronika Stelmakh and Dr. Jay Senkevich at MIT and Mr. Emil Cashin at Norwich Technologies for their help with the high-temperature emittance measurements. NR 28 TC 3 Z9 3 U1 2 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2014 VL 116 IS 7 AR 073508 DI 10.1063/1.4893656 PG 8 WC Physics, Applied SC Physics GA AO2XB UT WOS:000341189400013 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Aielli, G Aring;kesson, TPA Akimoto, G Akimov, AV Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Ask, S Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Betancourt, C Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Calkins, R Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, B Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Christidi, IA Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirkovic, P Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Coggeshall, J Cole, B Cole, S Colijn, AP Collins-Tooth, C Collot, J Colombo, T Colon, G Compostella, G Muino, PC Coniavitis, E Conidi, MC Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Cuciuc, CM Almenar, CC Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Daniells, AC Hoffmann, MD Dao, V Darbo, G Darlea, GL Darmora, S Dassoulas, JA Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S de Graat, J De Groot, N de Jong, P De la Torre, H De 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Dos Anjos, A Dova, MT Doyle, AT Dris, M Dubbert, J Dube, S Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Dudziak, F Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Dwuznik, M Dyndal, M Ebke, J Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellert, M Elles, S Ellinghaus, F Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Engelmann, R Erdmann, J Ereditato, A Eriksson, D Ernis, G Ernst, J Ernst, M Ernwein, J Errede, D Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Favareto, A Fayard, L Federic, P Fedin, OL Fedorko, W Fehling-Kaschek, M Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Perez, SF Ferrag, S Ferrando, J Ferrari, A Ferrari, 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CA ATLAS Collaboration TI Light-quark and gluon jet discrimination in collisions at root s=7 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID Z-DECAYS; DEPENDENCE; MULTIPLICITY AB A likelihood-based discriminant for the identification of quark- and gluon-initiated jets is built and validated using 4.7 fb of proton-proton collision data at collected with the ATLAS detector at the LHC. Data samples with enriched quark or gluon content are used in the construction and validation of templates of jet properties that are the input to the likelihood-based discriminant. The discriminating power of the jet tagger is established in both data and Monte Carlo samples within a systematic uncertainty of 10-20 %. In data, light-quark jets can be tagged with an efficiency of while achieving a gluon-jet mis-tag rate of in a range between and for jets in the acceptance of the tracker. 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[Ahmad, A.; Alexopoulos, T.; Aloisio, A.; Annovi, A.; Antonov, A.; Byszewski, M.; Dris, M.; Iakovidis, G.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pacheco Pages, A.; Padilla Aranda, C.; Portell Bueso, X.; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pacheco Pages, A.; Padilla Aranda, C.; Portell Bueso, X.; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Dimitrievska, A.; Krstic, J.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Agatonovic-Jovin, T.; Bozovic-Jelisavcic, I.; Cirkovic, P.; Mamuzic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Latour, B. Martin Dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ovcharova, A.; Pagan Griso, S.; Polifka, R.; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Ahmad, A.; Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ovcharova, A.; Pagan Griso, S.; Polifka, R.; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Ahmad, A.; Kuutmann, E. Bergeaas; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mclaughlan, T.; Mudd, R. D.; Murillo Quijada, J. A.; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Yau Wong, K. H.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Okawa, H.; Oliveira Damazio, D.; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Metcalfe, J.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Banfi, D.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. 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Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Paredes Hernandez, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Paredes Hernandez, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Paredes Hernandez, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Perez Reale, V.; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Coll Cosenza, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Monig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Monig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Olivares Pino, S. A.; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagaova, M.; Parzefall, U.; Rave, T. C.; Ruhr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Testa, M.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Vu Anh, T.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Ahmad, A.; Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Oropeza Barrera, C.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Moreno Llacer, M.; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Vazquez Schroeder, T.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimares; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; Zevi della Porta, G.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Sliwa, K.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Morettini, P.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Morettini, P.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Ahmad, A.; Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisck, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Ahmad, A.; Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisck, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Sandbach, R. L.; Snidero, G.; Teixeira Dias Castanheira, M.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Panduro Vazquez, J. G.; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Ahmad, A.; Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schafer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Iturbe Ponce, J. M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Ahmad, A.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Ahmad, A.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Nunes Hanninger, G.; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Parkville, Vic 3052, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Physk, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Ahmad, A.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Ahmad, A.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vranjes Milosavljevic, M.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vranjes Milosavljevic, M.; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Ahmad, A.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Annovi, A.; Antonov, A.; Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Fac Ciencias & Tecnol, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Webster, J. S.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Morgenstern, M.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Safai Tehrani, F.; Sidoti, A.; Solfaroli Camillocci, E.; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Morgenstern, M.; Solfaroli Camillocci, E.; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Commissariat Energie Atom & Energies Alternative, Inst Recherches Lois Fondament Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Sales De Bruin, P. H.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Vickey Boeriu, O. E.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Ahmad, A.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Ahmad, A.; Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Santoyo Castillo, I.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Annovi, A.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Davies, M.; Etzion, E.; Gershon, A.; Guttman, N.; Sadeh, I.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Annovi, A.; Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Torrence, E.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Savard, P.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Savard, P.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Oram, C. J.; Perez Codina, E.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Annovi, A.; Antonov, A.; Artamonov, A.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Alhroob, M.; De Sanctis, U.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torr Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torr Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torr Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torr Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torr Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maetig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Apolle, R.; Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Chen, L.; Gao, J.] Aix Marseille Univ, CPPM, Marseille, France. [Chen, L.; Gao, J.] CNRS, IN2P3, Marseille, France. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Ottawa, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Jenni, P.] CERN, Geneva, Switzerland. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Korol, A. A.; Maximov, D. A.; Rezanova, O. L.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, K.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Liu, K.] Univ Paris Diderot, Paris, France. [Liu, K.] CNRS, IN2P3, Paris, France. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Messina, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tamsett, M. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Tikhomirov, V. O.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Li, Liang/O-1107-2015; Garcia, Jose /H-6339-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Villa, Mauro/C-9883-2009; Staroba, Pavel/G-8850-2014; Alexa, Calin/F-6345-2010; Warburton, Andreas/N-8028-2013; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Nepomuceno, Andre/M-9190-2014; Gabrielli, Alessandro/H-4931-2012; Lokajicek, Milos/G-7800-2014; Turra, Ruggero/N-2374-2014; Castro, Nuno/D-5260-2011; Moraes, Arthur/F-6478-2010; Brooks, William/C-8636-2013; Lei, Xiaowen/O-4348-2014; Doyle, Anthony/C-5889-2009; Di Domenico, Antonio/G-6301-2011; de Groot, Nicolo/A-2675-2009; Wemans, Andre/A-6738-2012; Nemecek, Stanislav/G-5931-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; White, Ryan/E-2979-2015; Bosman, Martine/J-9917-2014; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Marti-Garcia, Salvador/F-3085-2011; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Vranjes Milosavljevic, Marija/F-9847-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Solfaroli Camillocci, Elena/J-1596-2012; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Snesarev, Andrey/H-5090-2013; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015 OI Monzani, Simone/0000-0002-0479-2207; Li, Liang/0000-0001-6411-6107; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Gabrielli, Alessandro/0000-0001-5346-7841; Castro, Nuno/0000-0001-8491-4376; Moraes, Arthur/0000-0002-5157-5686; Brooks, William/0000-0001-6161-3570; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; White, Ryan/0000-0003-3589-5900; Bosman, Martine/0000-0002-7290-643X; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM; Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 58 TC 4 Z9 4 U1 8 U2 105 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 21 PY 2014 VL 74 IS 8 AR 3023 DI 10.1140/epjc/s10052-014-3023-z PG 29 WC Physics, Particles & Fields SC Physics GA AN9SJ UT WOS:000340948500001 ER PT J AU Berkelbach, TC Hybertsen, MS Reichman, DR AF Berkelbach, Timothy C. Hybertsen, Mark S. Reichman, David R. TI Microscopic theory of singlet exciton fission. III. Crystalline pentacene SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CHARGE-TRANSFER TRANSITIONS; ENERGY-TRANSFER DYNAMICS; ELECTRONIC-STRUCTURE; MOLECULAR-DYNAMICS; POLYCRYSTALLINE PENTACENE; BORN-OPPENHEIMER; 1ST PRINCIPLES; LHCII COMPLEX; DIPOLE-MOMENT; HIGHER-PLANTS AB We extend our previous work on singlet exciton fission in isolated dimers to the case of crystalline materials, focusing on pentacene as a canonical and concrete example. We discuss the proper interpretation of the character of low-lying excited states of relevance to singlet fission. In particular, we consider a variety of metrics for measuring charge-transfer character, conclusively demonstrating significant charge-transfer character in the low-lying excited states. The impact of this electronic structure on the subsequent singlet fission dynamics is assessed by performing real-time master-equation calculations involving hundreds of quantum states. We make direct comparisons with experimental absorption spectra and singlet fission rates, finding good quantitative agreement in both cases, and we discuss the mechanistic distinctions that exist between small isolated aggregates and bulk systems. (C) 2014 AIP Publishing LLC. C1 [Berkelbach, Timothy C.; Reichman, David R.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Hybertsen, Mark S.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Berkelbach, TC (reprint author), Columbia Univ, Dept Chem, 3000 Broadway, New York, NY 10027 USA. EM tcb2112@columbia.edu; mhyberts@bnl.gov; drr2103@columbia.edu OI Hybertsen, Mark S/0000-0003-3596-9754 FU Center for Re-Defining Photovoltaic Efficiency through Molecule Scale Control, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001085]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF); ORISE-ORAU [DE-AC05-06OR23100] FX We thank Jeff Neaton, Pierre Darancet, Sahar Sharifzadeh, Joe Subotnik, Garnet Chan, and Eran Rabani for helpful conversations. This work was supported in part by the Center for Re-Defining Photovoltaic Efficiency through Molecule Scale Control, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001085. This work was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-98CH10886 (M. S. H). T. C. B. was supported in part by the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under Contract No. DE-AC05-06OR23100. NR 84 TC 39 Z9 39 U1 7 U2 90 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2014 VL 141 IS 7 AR 074705 DI 10.1063/1.4892793 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OP UT WOS:000340714600039 PM 25149804 ER PT J AU Bhaskaran-Nair, K Kowalski, K Moreno, J Jarrell, M Shelton, WA AF Bhaskaran-Nair, Kiran Kowalski, Karol Moreno, Juana Jarrell, Mark Shelton, William A. TI Equation of motion coupled cluster methods for electron attachment and ionization potential in fullerenes C-60 and C-70 SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; CONNECTED TRIPLE EXCITATIONS; SYMMETRY-ADAPTED-CLUSTER; EXCITED-STATES; CONFIGURATION-INTERACTION; BASIS-SETS; OPEN-SHELL; PHOTOELECTRON-SPECTROSCOPY; RESPONSE FUNCTIONS; MOLECULAR SYSTEMS AB In both molecular and periodic solid-state systems there is a need for the accurate determination of the ionization potential and the electron affinity for systems ranging from light harvesting polymers and photocatalytic compounds to semiconductors. The development of a Green's function approach based on the coupled cluster (CC) formalism would be a valuable tool for addressing many properties involving many-body interactions along with their associated correlation functions. As a first step in this direction, we have developed an accurate and parallel efficient approach based on the equation of motion-CC technique. To demonstrate the high degree of accuracy and numerical efficiency of our approach we calculate the ionization potential and electron affinity for C-60 and C-70. Accurate predictions for these molecules are well beyond traditional molecular scale studies. We compare our results with experiments and both quantum Monte Carlo and GW calculations. (C) 2014 AIP Publishing LLC. C1 [Bhaskaran-Nair, Kiran; Moreno, Juana; Jarrell, Mark] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70802 USA. [Bhaskaran-Nair, Kiran; Moreno, Juana; Jarrell, Mark; Shelton, William A.] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Bhaskaran-Nair, Kiran; Shelton, William A.] Louisiana State Univ, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. [Kowalski, Karol] Pacific NW Natl Lab, Battelle, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. RP Bhaskaran-Nair, K (reprint author), Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70802 USA. EM karol.kowalski@pnnl.gov RI Moreno, Juana/D-5882-2012 FU National Science Foundation under the NSF EPSCoR from the Louisiana Board of Regents [EPS-1003897]; Department of Energy Office of Biological and Environmental Research; U.S. Department of Energy by the Battelle Memorial Institute [DE-AC06.76RLO-1830] FX This work is supported by the National Science Foundation under the NSF EPSCoR Cooperative Agreement No. EPS-1003897 with additional support from the Louisiana Board of Regents. The calculations have been performed using the Environmental Molecular Sciences Laboratory and Pacific Northwest National Laboratory (PNNL) Institutional Computing, both resources located at PNNL, which is sponsored by the Department of Energy Office of Biological and Environmental Research. The PNNL is operated for the U.S. Department of Energy by the Battelle Memorial Institute under Contract No. DE-AC06.76RLO-1830. A small portion of this research has used the high performance computational resources provided by Louisiana State University (http://www.hpc.lsu.edu). NR 98 TC 6 Z9 6 U1 3 U2 30 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2014 VL 141 IS 7 AR 074304 DI 10.1063/1.4891934 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OP UT WOS:000340714600018 PM 25149783 ER PT J AU Carrillo, JMY Sumpter, BG AF Carrillo, Jan-Michael Y. Sumpter, Bobby G. TI Structure and dynamics of confined flexible and unentangled polymer melts in highly adsorbing cylindrical pores SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS; NANOPORES; NANOCOMPOSITE; CHAINS AB Coarse-grained molecular dynamics simulations are used to probe the dynamic phenomena of polymer melts confined in nanopores. The simulation results show excellent agreement in the values obtained for the normalized coherent single chain dynamic structure factor, S(Q, Delta t)/S(Q, 0). In the bulk configuration, both simulations and experiments confirm that the polymer chains follow Rouse dynamics. However, under confinement, the Rouse modes are suppressed. The mean-square radius of gyration < R-g(2)> and the average relative shape anisotropy of the conformation of the polymer chains indicate a pancake-like conformation near the surface and a bulk-like conformation near the center of the confining cylinder. This was confirmed by direct visualization of the polymer chains. Despite the presence of these different conformations, the average form factor of the confined chains still follows the Debye function which describes linear ideal chains, which is in agreement with small angle neutron scattering experiments (SANS). The experimentally inaccessible mean-square displacement (MSD) of the confined monomers, calculated as a function of radial distance from the pore surface, was obtained in the simulations. The simulations show a gradual increase of the MSD from the adsorbed, but mobile layer, to that similar to the bulk far away from the surface. (C) 2014 AIP Publishing LLC. C1 [Carrillo, Jan-Michael Y.] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Sumpter, Bobby G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Carrillo, JMY (reprint author), Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. EM carrillojy@ornl.gov RI Carrillo, Jan-Michael/K-7170-2013; Sumpter, Bobby/C-9459-2013 OI Carrillo, Jan-Michael/0000-0001-8774-697X; Sumpter, Bobby/0000-0001-6341-0355 FU Office of Advanced Scientific Computing Research, U.S. Department of Energy [DE-AC05-00OR22725]; Office of Science, U.S. Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX We thank A. V. Dobrynin, L. Noirez, and C. Do for useful discussions. M. Krutyeva, A. Wischnewski, and D. Richter for substantial guidance that led to the formulation of this manuscript. E. Hubner for performing the calculations of the polymer-surface interaction. J.-M.Y.C. acknowledges support from the Office of Advanced Scientific Computing Research, Office of Science, U.S. Department of Energy under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. B. G. S. was supported by U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. We acknowledge support for aspects of code development from ORNL Laboratory Directed Research and Development. This research used resources of the Leadership Computing Facility at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. NR 40 TC 2 Z9 2 U1 0 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2014 VL 141 IS 7 AR 074904 DI 10.1063/1.4893055 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OP UT WOS:000340714600049 PM 25149814 ER PT J AU Liu, XJ Wang, CZ Lin, HQ Ho, KM AF Liu, Xiaojie Wang, Cai-Zhuang Lin, Hai-Qing Ho, Kai-Ming TI Magnetic Moment Enhancement for Mn-7 Cluster on Graphene SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; BASIS-SET; INITIO; DEFECTS; METALS AB Mn-7 cluster on graphene with different structural motifs and magnetic orders are investigated systematically by first-principles calculations. The calculations show that Mn-7 on graphene prefers a two-layer motif and exhibits a ferrimagnetic coupling. The magnetic moment of the Mn-7 cluster increases from 5.0 mu(B) at its freestanding state to about 6.0 mu(B) upon adsorption on graphene. Mn-7 cluster also induces about 0.3 mu(B) of magnetic moment in the graphene layer, leading to an overall enhancement of 1.3 mu(B) magnetic moment for Mn-7 on graphene. Detail electron transfer and bonding analysis have been carried out to investigate the origin of the magnetic enhancement. C1 [Liu, Xiaojie; Lin, Hai-Qing] Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. [Liu, Xiaojie; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Liu, Xiaojie; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Wang, CZ (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM wangcz@ameslab.gov; haiqing0@csrc.ac.cn FU U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358]; National Natural Science Foundation of China [11204013]; China Postdoctoral Science Foundation [2013T60056] FX Work at Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, including a grant of computer time at the National Energy Research Scientific Computing Centre (NERSC) in Berkeley, CA, under Contract DE-AC02-07CH11358. X.L. also acknowledges the support by the National Natural Science Foundation of China under Grant 11204013 and the China Postdoctoral Science Foundation under Grant 2013T60056. NR 25 TC 4 Z9 4 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 21 PY 2014 VL 118 IS 33 BP 19123 EP 19128 DI 10.1021/jp504329c PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN7VR UT WOS:000340809600033 ER PT J AU Chlistunoff, J Sansinena, JM AF Chlistunoff, Jerzy Sansinena, Jose-Maria TI Effects of Axial Coordination of the Metal Center on the Activity of Iron Tetraphenylporphyrin as a Nonprecious Catalyst for Oxygen Reduction SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PYROLYTIC-GRAPHITE ELECTRODES; AEROGEL CARBON ELECTRODES; FE-BASED CATALYSTS; FUEL-CELL CATHODE; SEMIEMPIRICAL METHODS; PORPHYRINS; COBALT; O-2; LIGAND; ELECTROREDUCTION AB Effects of axial coordination of the metal center on oxygen reduction catalyzed by iron tetraphenylporphyrin have been studied using spectroelectrochemical and rotating ring disk electrode techniques. Among numerous ligands studied, the strongest complexation of the metal center was observed for imidazole and some substituted imidazole ligands. Around 300 mV positive shift of the oxygen reduction potential in 0.5 M H2SO4 was observed when the catalyst support (high surface area carbon Vulcan XC72) was impregnated with polyvinylimidazole. A smaller 200 mV shift of the reduction potential was recorded when graphene modified with 1-(3-aminopropyl)imidazole was used as the catalyst support instead of Vulcan. In both cases, the catalyst selectivity for four-electron reduction was also substantially improved. The effects of iron complexation on oxygen reduction kinetics and mechanism result from both a positive shift of the potential of the first porphyrin reduction and an increase of the electron density on the iron center through the so-called "push effect". The observed phenomena are discussed in relation to heat-treated Fe/N/C catalysts for oxygen reduction. C1 [Chlistunoff, Jerzy; Sansinena, Jose-Maria] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Chlistunoff, J (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM jerzy@lanl.gov FU University of California [12-LR-237440] FX Financial support from the University of California (grant 12-LR-237440) is gratefully acknowledged. NR 49 TC 9 Z9 10 U1 6 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 21 PY 2014 VL 118 IS 33 BP 19139 EP 19149 DI 10.1021/jp5044249 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN7VR UT WOS:000340809600035 ER PT J AU Asara, GG Roldan, A Ricart, JM Rodriguez, JA Illas, F de Leeuw, NH AF Asara, Gian Giacomo Roldan, Alberto Ricart, Josep M. Rodriguez, Jose A. Illas, Francesc de Leeuw, Nora H. TI New Insights into the Structure of the C-Terminated beta-Mo2C (001) Surface from First-Principles Calculations SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; MOLYBDENUM CARBIDE CATALYSTS; AUGMENTED-WAVE METHOD; WATER-GAS SHIFT; DISSOCIATION; DENSITY; HYDROGENATION; AU/TIC(001); SIMULATION; OXYGEN AB Periodic density functional theory (DFT) calculations have been used to study the stability of five different C-terminations of the Mo2C(001) surface in the most stable orthorhombic (beta) phase of this important material. The different terminations all have similar values of the work function or atomic charges, indicating a similar electronic structure, although the analysis of the cleavage energy suggests that the non polar C-terminated surfaces will be the extended terminations seen under thermodynamic equilibrium. Nevertheless, the calculated DFT cleavage energy values together with statistical arguments indicate that different C-terminated motifs are likely to coexist even at temperatures just below annealing conditions. C1 [Asara, Gian Giacomo; Roldan, Alberto; de Leeuw, Nora H.] UCL, Dept Chem, London WC1H 0AJ, England. [Asara, Gian Giacomo; Roldan, Alberto; de Leeuw, Nora H.] Univ Barcelona, Thomas Young Ctr Theory & Simulat Mat, E-08028 Barcelona, Spain. [Asara, Gian Giacomo; Ricart, Josep M.] Univ Rovira & Virgili, Dept Quim Fis & Inorgan, E-43007 Tarragona, Spain. [Asara, Gian Giacomo; Illas, Francesc] Univ Barcelona, Dept Quim Fis, E-08028 Barcelona, Spain. [Asara, Gian Giacomo; Illas, Francesc] Univ Barcelona, IQTCUB, E-08028 Barcelona, Spain. [Rodriguez, Jose A.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Illas, F (reprint author), Univ Barcelona, Dept Quim Fis, C Marti & Franques 1, E-08028 Barcelona, Spain. EM francesc.illas@ub.edu RI Ricart, Josep/K-9802-2014; Illas, Francesc /C-8578-2011 OI Ricart, Josep/0000-0002-2610-5535; Illas, Francesc /0000-0003-2104-6123 FU Spanish MINECO [CTQ2012-30751]; Generalitat de Catalunya [2014SGR97]; XRQTC; Universitat Rovira i Virgili; London Thomas Young Centre; UCL Industrial Doctorate Centre for Molecular Modelling and Materials Science; Ramsay Memorial Trust; University College London; ICREA Academia award; Red Espanola de Supercomputacion FX This work has been supported by the Spanish MINECO grant CTQ2012-30751 grant and, in part, by Generalitat de Catalunya grants 2014SGR97 and XRQTC. G.G.A. thanks the Universitat Rovira i Virgili for supporting his predoctoral research and the London Thomas Young Centre and the UCL Industrial Doctorate Centre for Molecular Modelling and Materials Science for funding. A.R. is grateful to the Ramsay Memorial Trust and University College London for the provision of a Ramsay Fellowship. F.I. acknowledges additional support through the ICREA Academia award for excellence in research. Computational time at the MARENOSTRUM supercomputer has been generously provided by the Barcelona Supercomputing Centre through a grant from Red Espanola de Supercomputacion. NR 40 TC 1 Z9 1 U1 5 U2 61 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 21 PY 2014 VL 118 IS 33 BP 19224 EP 19231 DI 10.1021/jp505847g PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN7VR UT WOS:000340809600045 ER PT J AU Svedruzic, D Gregg, BA AF Svedruzic, Drazenka Gregg, Brian A. TI Mechano-Electrochemistry and Fuel-Forming Mechano-Electrocatalysis on Spring Electrodes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENERGY LANDSCAPE; TENSILE STRAIN; KINETICS; PHOTOSYNTHESIS; DYNAMICS; LAYER AB Each material, in principle, possesses a continuum of electrochemical and electrocatalytic properties that can be reversibly tuned by mechanical stress over its elastic range. As an initial test of this hypothesis we investigate stainless steel extension springs as electrodes. Stretching the springs reversibly doubles the heterogeneous rate constant for electron transfer to a redox species in solution, Ru(NH3)(6)Cl-3, while the charge transfer rate through a surface film of Ni(II/III) oxy-hydroxide increases similar to 4-fold. Straining the springs near their elastic limit in 1 M NaOH increases the electrcatalytic hydrogen evolution current by similar to 50% and the oxygen evolution current by similar to 300%. Thus, even the small elastic strain (similar to 0.1% lattice deformation) that can be applied by stretching a spring leads to significant and reversible increases in the rates of: 1) electron transfer to a redox couple in solution, 2) charge transport through a surface film, and 3) electrocatalysis. C1 [Svedruzic, Drazenka; Gregg, Brian A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Svedruzic, D (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM drazenka.svedruzic@nrel.gov FU U.S. Department of Energy, Office of Science, Basic Energy Science, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC36-08GO28308] FX This work was funded by the U.S. Department of Energy, Office of Science, Basic Energy Science, Division of Chemical Sciences, Geosciences and Biosciences, under Contract No. DE-AC36-08GO28308 to NREL. NR 38 TC 2 Z9 2 U1 4 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 21 PY 2014 VL 118 IS 33 BP 19246 EP 19251 DI 10.1021/jp506279q PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN7VR UT WOS:000340809600048 ER PT J AU Tenney, SA Lu, DY He, F Levy, N Perera, UGE Starr, DE Muller, K Bluhm, H Sutter, P AF Tenney, Samuel A. Lu, Deyu He, Feng Levy, Niv Perera, Uduwanage G. E. Starr, David E. Mueller, Kathrin Bluhm, Hendrik Sutter, Peter TI Key Structure-Property Relationships in CO2 Capture by Supported Alkanolamines SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; CARBON-DIOXIDE CAPTURE; AUGMENTED-WAVE METHOD; ALIPHATIC-ALCOHOLS; SOLID SORBENTS; BASIS-SET; SURFACE; ADSORPTION; TIO2(110); TIO2 AB Heterogeneous interfaces exhibit remarkable material properties resulting from their structural motifs, the judicious placement of functional chemical groups, etc. It has been a long-standing challenge to manipulate and design interface structures at the atomic level to achieve new functionalities. Here, we demonstrate that by modifying the length of the backbone in alkanolamines one can control the packing density of organic monolayers adsorbed on rutile TiO2 and the interaction strength between their amine functional group and the substrate. As a result, we observed strikingly different activities in CO2 capture by the amine functional group of different alkanolamines on TiO2(110). Synchrotron photoelectron spectroscopy at near-ambient CO2 pressures showed that adsorbed 2-amino-1-ethanol (monoethanolamine, MEA) is inactive, whereas the amine group in 3-amino-1-propanol (3AP)/TiO2(110) readily reacts with and captures CO2. Our results suggest that the geometry of the interface plays a decisive role in the reactivity of adsorbed functionalized organic molecules, such as solid-supported alkanolamines for CO2 capture. C1 [Tenney, Samuel A.; Lu, Deyu; Levy, Niv; Perera, Uduwanage G. E.; Starr, David E.; Mueller, Kathrin; Sutter, Peter] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [He, Feng] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Sutter, P (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM psutter@bnl.gov RI Muller, Kathrin/H-1902-2011; Lu, Deyu/O-4418-2016 OI Lu, Deyu/0000-0003-4351-6085 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX Research carried out in part at the Center for Functional Nanomaterials and the National Synchrotron Light Source, Brookhaven National Laboratory, supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. D.L. acknowledges the computational resources at the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The ALS and beamline 11.0.2 are supported by the Director, Office of Science, Office of Basic Energy Sciences, and by the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. NR 45 TC 4 Z9 4 U1 3 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 21 PY 2014 VL 118 IS 33 BP 19252 EP 19258 DI 10.1021/jp507205t PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN7VR UT WOS:000340809600049 ER PT J AU Remsing, RC Baer, MD Schenter, GK Mundy, CJ Weeks, JD AF Remsing, Richard C. Baer, Marcel D. Schenter, Gregory K. Mundy, Christopher J. Weeks, John D. TI The Role of Broken Symmetry in Solvation of a Spherical Cavity in Classical and Quantum Water Models SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; DENSITY-FUNCTIONAL THEORY; FREE-ENERGIES; ELECTROSTATIC POTENTIALS; HYDROPHOBIC HYDRATION; MOLECULAR-DYNAMICS; CHARGED MOLECULES; ION HYDRATION; LIQUID WATER; POLAR AB Insertion of a hard sphere cavity in liquid water breaks translational symmetry and generates an electrostatic potential difference between the region near the cavity and the bulk. Here, we clarify the physical interpretation of this potential and its calculation. We also show that the electrostatic potential in the center of small, medium, and large cavities depends very sensitively on the form of the assumed molecular interactions for different classical simple point-charge models and quantum mechanical DFT-based interaction potentials, as reflected in their description of donor and acceptor hydrogen bonds near the cavity. These differences can significantly affect the magnitude of the scalar electrostatic potential. We argue that the result of these studies will have direct consequences toward our understanding of the thermodynamics of ion solvation through the cavity charging process. C1 [Remsing, Richard C.; Weeks, John D.] Univ Maryland, Inst Phys Sci & Technol, College Pk, MD 20742 USA. [Weeks, John D.] Univ Penn, Dept Chem & Biochem, Philadelphia, PA 19104 USA. [Baer, Marcel D.; Schenter, Gregory K.; Mundy, Christopher J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99354 USA. RP Remsing, RC (reprint author), Univ Penn, Dept Chem & Biomol Engn, Philadelphia, PA 19104 USA. EM rremsing@umd.edu; chris.mundy@pnnl.gov; jdw@umd.edu FU National Science Foundation [CHE0848574, CHE1300993]; U.S. Department of Energy's (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory (PNNL); Linus Pauling Distinguished Postdoctoral Fellowship Program at PNNL; National Energy Research Scientific Computing Center - Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX JDW and RCR are financially supported by the National Science Foundation (Grants CHE0848574 and CHE1300993). CJM and GKS are financially supported by the U.S. Department of Energy's (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory (PNNL) is operated for the Department of Energy by Battelle. MDB is grateful for the support of the Linus Pauling Distinguished Postdoctoral Fellowship Program at PNNL. We acknowledge illuminating discussions and sharing of ideas and preprints with Dr. Shawn M. Kathmann, Dr. Bernhard Sellner, and Prof. Tom Beck. The DFT simulations used resources provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Additional computing resources were generously allocated by PNNL's Institutional Computing program. NR 62 TC 22 Z9 22 U1 3 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 21 PY 2014 VL 5 IS 16 BP 2767 EP 2774 DI 10.1021/jz501067w PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AN7US UT WOS:000340807100001 PM 26278076 ER PT J AU Bolmatov, D Zav'yalov, D Gao, M Zhernenkov, M AF Bolmatov, Dima Zav'yalov, D. Gao, M. Zhernenkov, Mikhail TI Structural Evolution of Supercritical CO2 across the Frenkel Line SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID DYNAMICS; LIQUIDS; GLASS; DISORDER; METALS; MATTER; WATER; ORDER AB Here, we study structural properties of the supercritical carbon dioxide and discover the existence of persistent medium-range order correlations, which make supercritical carbon dioxide nonuniform and heterogeneous on an intermediate length scale. We report on the CO2 heterogeneity shell structure where, in the first shell, both carbon and oxygen atoms experience gas-like-type interactions with short-range order correlations while within the second shell, oxygen atoms essentially exhibit a liquid-like type of interactions due to localization of transverse-like phonon packets. Importantly, we highlight a catalytic role of atoms inside of the nearest-neighbor heterogeneity shell in providing a mechanism for diffusion and proving the existence of an additional thermodynamic boundary in the supercritical carbon dioxide on an intermediate length scale. Finally, we discuss important implications for answering the intriguing question whether Venus may have had CO2 oceans and urge for an experimental detection of this persistent local-order heterogeneity. C1 [Bolmatov, Dima] Cornell Univ, Baker Lab, Ithaca, NY 14853 USA. [Zav'yalov, D.] Volgograd State Tech Univ, Volgograd 400005, Russia. [Gao, M.] Queen Mary Univ London, London E1 4NS, England. [Zhernenkov, Mikhail] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Bolmatov, D (reprint author), Cornell Univ, Baker Lab, Ithaca, NY 14853 USA. EM d.bolmatov@gmail.com RI Zavyalov, Dmitriy/N-7609-2015; OI Zhernenkov, Mikhail/0000-0003-3604-0672 FU Cornell University; U.S. D.O.E. [DE-AC02-98CH10886]; NASA/HQ FX D.B. thanks Ben Widom and Cornell University for support. M.G. thanks Martin Dove for intermolecular potential modelling assistance. Brookhaven National Laboratory is supported under U.S. D.O.E. Grant No. DE-AC02-98CH10886. We are grateful to Ben Widom, Neil Ashcroft, Martin Dove, Zeb Kramer, and Colin Wilson for fruitful discussions. We acknowledge the use of data products or imagery from the Magellan Venus Explorer system operated by the NASA with funding provided by NASA/HQ. NR 41 TC 6 Z9 6 U1 0 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 21 PY 2014 VL 5 IS 16 BP 2785 EP 2790 DI 10.1021/jz5012127 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AN7US UT WOS:000340807100004 PM 26278079 ER PT J AU Hucker, M Christensen, NB Holmes, AT Blackburn, E Forgan, EM Liang, RX Bonn, DA Hardy, WN Gutowski, O von Zimmermann, M Hayden, SM Chang, J AF Huecker, M. Christensen, N. B. Holmes, A. T. Blackburn, E. Forgan, E. M. Liang, Ruixing Bonn, D. A. Hardy, W. N. Gutowski, O. v Zimmermann, M. Hayden, S. M. Chang, J. TI Competing charge, spin, and superconducting orders in underdoped YBa2Cu3Oy SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTOR; UPPER CRITICAL-FIELD; T-C SUPERCONDUCTOR; CUPRATE SUPERCONDUCTORS; STRIPE ORDER; FERMI-SURFACE; MAGNETIC-FIELD; ANTIFERROMAGNETIC CORRELATIONS; QUANTUM OSCILLATIONS; TRANSPORT-PROPERTIES AB To explore the doping dependence of the recently discovered charge-density-wave (CDW) order in YBa2Cu3Oy, we present a bulk-sensitive high-energy x-ray study for several oxygen concentrations, including strongly underdoped YBa2Cu3O6.44. Combined with previous data around the so-called 1/8 doping, we show that bulk CDW order exists at least for hole concentrations (p) in the CuO2 planes of 0.078 less than or similar to p less than or similar to 0.132. This implies that CDW order exists in close vicinity to the quantum critical point for spin-density-wave (SDW) order. In contrast to the pseudogap temperature T*, the onset temperature of CDW order decreases with underdoping to T-CDW similar to 90 K in YBa2Cu3O6.44. Together with a weakened order parameter this suggests a competition between CDW and SDW orders. In addition, the CDW order in YBa2Cu3O6.44 shows the same type of competition with superconductivity as a function of temperature and magnetic field as samples closer to p = 1/8. At low p the CDW incommensurability continues the previously reported linear increasing trend with underdoping. In the entire doping range the in-plane correlation length of the CDW order in b axis direction depends only very weakly on the hole concentration, and appears independent of the type and correlation length of the oxygen-chain order. The onset temperature of the CDW order is remarkably close to a temperature T-dagger that marks the maximum of 1/(T1T) in planar Cu-63 NQR/NMR experiments, potentially indicating a response of the spin dynamics to the formation of the CDW. Our discussion of these findings includes a detailed comparison to the charge stripe order in La2-xBaxCuO4. C1 [Huecker, M.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Christensen, N. B.] Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark. [Holmes, A. T.; Blackburn, E.; Forgan, E. M.] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Liang, Ruixing; Bonn, D. A.; Hardy, W. N.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Liang, Ruixing; Bonn, D. A.; Hardy, W. N.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. [Gutowski, O.; v Zimmermann, M.] DESY, D-22603 Hamburg, Germany. [Hayden, S. M.] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England. [Chang, J.] Ecole Polytech Lausanna EPFL, Inst Mat Complexe, CH-1015 Lausanne, Switzerland. RP Hucker, M (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RI Chang, Johan/F-1506-2014; Holmes, Alexander/B-5485-2013; Hayden, Stephen/F-4162-2011; Christensen, Niels/A-3947-2012 OI Chang, Johan/0000-0002-4655-1516; Holmes, Alexander/0000-0002-3069-3069; Hayden, Stephen/0000-0002-3209-027X; Christensen, Niels/0000-0001-6443-2142 FU Office of Basic Energy Sciences (BES), Division of Materials Science and Engineering, U.S. Department of Energy (DOE) [DE-AC02-98CH10886]; Danish Agency for Science, Technology and Innovation under DANSCATT; EPSRC [EP/G027161/1, EP/J015423/1, EP/J016977/1]; Wolfson Foundation; Royal Society; Swiss National Science Foundation through NCCR-MaNEP [PZ00P2-142434]; U.S. DOE [DE-AC02-06CH11357] FX We acknowledge fruitful discussions with J. M. Tranquada, S. A. Kivelson, L. Taillefer, H.-J. Grafe, A. J. Achkar, and W. Ku. This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Science and Engineering, U.S. Department of Energy (DOE), under Contract No. DE-AC02-98CH10886; the Danish Agency for Science, Technology and Innovation under DANSCATT; the EPSRC (Grants No. EP/G027161/1, No. EP/J015423/1, and No. EP/J016977/1); the Wolfson Foundation; the Royal Society; and the Swiss National Science Foundation through NCCR-MaNEP and Grant No. PZ00P2-142434. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. DOE Office of Science by Argonne National Laboratory, was supported by the U. S. DOE under Contract No. DE-AC02-06CH11357. NR 110 TC 62 Z9 62 U1 3 U2 56 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 21 PY 2014 VL 90 IS 5 AR 054514 DI 10.1103/PhysRevB.90.054514 PG 11 WC Physics, Condensed Matter SC Physics GA AO2OD UT WOS:000341163200005 ER PT J AU Zarkevich, NA Johnson, DD AF Zarkevich, Nikolai A. Johnson, Duane D. TI Stable atomic structure of NiTi austenite SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; MARTENSITIC-TRANSFORMATION; CRYSTAL-STRUCTURES; TINI; DENSITY; ALLOY AB Nitinol (NiTi), the most widely used shape-memory alloy, exhibits an austenite phase that has yet to be identified. The usually assumed austenitic structure is cubic B2, which has imaginary phonon modes, hence it is unstable. We suggest a stable austenitic structure that "on average" has B2 symmetry (observed by x-ray and neutron diffraction), but it exhibits finite atomic displacements from the ideal B2 sites. The proposed structure has a phonon spectrum that agrees with that from neutron scattering, has diffraction spectra in agreement with x-ray diffraction, and has an energy relative to the ground state that agrees with calorimetry data. C1 [Zarkevich, Nikolai A.; Johnson, Duane D.] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. [Johnson, Duane D.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Zarkevich, NA (reprint author), Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. EM zarkev@ameslab.gov; ddj@ameslab.gov RI Zarkevich, Nikolai/A-3261-2013; OI Zarkevich, Nikolai/0000-0003-1919-0177; Johnson, Duane/0000-0003-0794-7283 FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; Iowa State University [DE-AC02-07CH11358] FX We thank Dario Alfe, Brent Fultz, and Graeme Henkelman for helpful discussions. This work was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 29 TC 6 Z9 6 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 21 PY 2014 VL 90 IS 6 AR 060102 DI 10.1103/PhysRevB.90.060102 PG 4 WC Physics, Condensed Matter SC Physics GA AO2OQ UT WOS:000341164800001 ER PT J AU Huo, P Jia, JY Mohapatra, S AF Huo, Peng Jia, Jiangyong Mohapatra, Soumya TI Elucidating the event-by-event flow fluctuations in heavy-ion collisions via the event-shape selection technique SO PHYSICAL REVIEW C LA English DT Article ID RELATIVISTIC NUCLEAR COLLISIONS; INITIAL GEOMETRY FLUCTUATIONS; PLANE CORRELATIONS; ROOT-S(NN)=2.76 TEV; PB COLLISIONS AB The presence of large event-by-event flow fluctuations in heavy ion collisions at the Relativistic Heavy Ion Collider (RHIC) and the Large Hadron Collider (LHC) provides an opportunity to study a broad class of flow observables. This paper explores the correlations among harmonic flow coefficients upsilon(n) and their phases Phi(n), as well as the rapidity fluctuation of upsilon(n). The study is carried out using the Pb + Pb events generated by the multiphase transport (AMPT) model with fixed impact parameter. The overall ellipticity or triangularity of events is varied by selecting on the eccentricities epsilon(n) or the magnitudes of the flow vector q(n) in a subevent for n = 2 and 3, respectively. The responses of the harmonic coefficients, the event-plane correlations, and the rapidity fluctuations to the change in epsilon(n) and q(n) are then systematized. Strong positive correlations are observed among all even harmonics upsilon(2), upsilon(4), and upsilon(6) (all increase with q(2)), between upsilon(2) and upsilon(5) (both increase with q(2)), and between upsilon(3) and upsilon(5) (both increase with q(3)), consistent with the effects of nonlinear collective response. In contrast, an anticorrelation is observed between upsilon(2) and upsilon(3) similar to that seen between epsilon(2) and epsilon(3). These correlation patterns are found to be independent of whether selecting on q(n) or epsilon(n), validating the ability of q(n) in selecting the initial geometry. A forward/backward asymmetry of upsilon(n) (eta) is observed for events selected on q(n) but not on epsilon(n), reflecting dynamical fluctuations exposed by the q(n) selection. Many event-plane correlators show good agreement between q(n) and epsilon(n) selections, suggesting that their variations with q(n) are controlled by the change of epsilon(n) in the initial geometry. Hence these correlators may serve as promising observables for disentangling the fluctuations generated in various stages of the evolution of the matter created in heavy ion collisions. C1 [Huo, Peng; Jia, Jiangyong; Mohapatra, Soumya] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Jia, Jiangyong] Brookhaven Natl Lab, Dept Phys, Upton, NY 11796 USA. RP Jia, JY (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM jjia@bnl.gov FU NSF [PHY-1019387, PHY-1305037] FX This research is supported by NSF under Grants No. PHY-1019387 and No. PHY-1305037. NR 44 TC 19 Z9 19 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 21 PY 2014 VL 90 IS 2 AR 024910 DI 10.1103/PhysRevC.90.024910 PG 13 WC Physics, Nuclear SC Physics GA AO2PG UT WOS:000341166600004 ER PT J AU Pei, JC Fann, GI Harrison, RJ Nazarewicz, W Shi, Y Thornton, S AF Pei, J. C. Fann, G. I. Harrison, R. J. Nazarewicz, W. Shi, Yue Thornton, S. TI Adaptive multi-resolution 3D Hartree-Fock-Bogoliubov solver for nuclear structure SO PHYSICAL REVIEW C LA English DT Article ID HARMONIC-OSCILLATOR BASIS; AXIALLY DEFORMED SOLUTION; GROUND-STATE PROPERTIES; BOGOLYUBOV EQUATIONS; DRIP-LINE; PROGRAM; VERSION; FIELD; SEPARATION; BASES AB Background: Complex many-body systems, such as triaxial and reflection-asymmetric nuclei, weakly bound halo states, cluster configurations, nuclear fragments produced in heavy-ion fusion reactions, cold Fermi gases, and pasta phases in neutron star crust, are all characterized by large sizes and complex topologies in which many geometrical symmetries characteristic of ground-state configurations are broken. A tool of choice to study such complex forms of matter is an adaptive multi-resolution wavelet analysis. This method has generated much excitement since it provides a common framework linking many diversified methodologies across different fields, including signal processing, data compression, harmonic analysis and operator theory, fractals, and quantum field theory. Purpose: To describe complex superfluid many-fermion systems, we introduce an adaptive pseudospectral method for solving self-consistent equations of nuclear density functional theory in three dimensions, without symmetry restrictions. Methods: The numerical method is based on the multi-resolution and computational harmonic analysis techniques with a multi-wavelet basis. The application of state-of-the-art parallel programming techniques include sophisticated object-oriented templates which parse the high-level code into distributed parallel tasks with a multi-thread task queue scheduler for each multi-core node. The internode communications are asynchronous. The algorithm is variational and is capable of solving coupled complex-geometric systems of equations adaptively, with functional and boundary constraints, in a finite spatial domain of very large size, limited by existing parallel computer memory. For smooth functions, user-defined finite precision is guaranteed. Results: The new adaptive multi-resolution Hartree-Fock-Bogoliubov (HFB) solver MADNESS-HFB is bench-marked against a two-dimensional coordinate-space solver HFB-AX that is based on the B-spline technique and a three-dimensional solver HFODD that is based on the harmonic-oscillator basis expansion. Several examples are considered, including the self-consistent HFB problem for spin-polarized trapped cold fermions and the Skyrme-Hartree-Fock (+BCS) problem for triaxial deformed nuclei. Conclusions: The new MADNESS-HFB framework has many attractive features when applied to nuclear and atomic problems involving many-particle superfluid systems. Of particular interest are weakly bound nuclear configurations close to particle drip lines, strongly elongated and dinuclear configurations such as those present in fission and heavy-ion fusion, and exotic pasta phases that appear in neutron star crust. C1 [Pei, J. C.] Peking Univ, Sch Phys, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Pei, J. C.; Nazarewicz, W.; Shi, Yue] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Pei, J. C.; Shi, Yue] Oak Ridge Natl Lab, Joint Inst Nucl Phys & Applicat, Oak Ridge, TN 37831 USA. [Fann, G. I.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Harrison, R. J.; Thornton, S.] SUNY Stony Brook, Inst Adv Computat Sci, Stony Brook, NY 11794 USA. [Harrison, R. J.] Brookhaven Natl Lab, Computat Sci Ctr, Upton, NY 11973 USA. [Nazarewicz, W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Nazarewicz, W.] Univ Warsaw, Inst Theoret Phys, Fac Phys, PL-00681 Warsaw, Poland. RP Pei, JC (reprint author), Peking Univ, Sch Phys, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. FU US Department of Energy (DOE) [DE-AC05-00OR22725, DE-FG02-96ER40963, DE-SC0008499, DE-FG02-13ER42025]; National Natural Science Foundation of China [11375016, 11235001] FX Useful discussions with N. Hinohara, J. Sheikh, and N. Schunck are gratefully acknowledged. This work was supported by the US Department of Energy (DOE) under Contracts No. DE-AC05-00OR22725 (ORNL), No. DE-FG02-96ER40963(University of Tennessee), No. DE-SC0008499 (NUCLEI SciDAC Collaboration), No. DE-FG02-13ER42025 (China-US Theory Institute for Physics with Exotic Nuclei), and by the National Natural Science Foundation of China under Grants No. 11375016 and No. 11235001. An award of computer time was provided by the National Institute for Computational Sciences (NICS) and the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program using resources of the OLCF and ALCF facilities. NR 47 TC 11 Z9 12 U1 3 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 21 PY 2014 VL 90 IS 2 AR 024317 DI 10.1103/PhysRevC.90.024317 PG 8 WC Physics, Nuclear SC Physics GA AO2PG UT WOS:000341166600002 ER PT J AU Haxhimali, T Rudd, RE Cabot, WH Graziani, FR AF Haxhimali, Tomorr Rudd, Robert E. Cabot, William H. Graziani, Frank R. TI Diffusivity in asymmetric Yukawa ionic mixtures in dense plasmas SO PHYSICAL REVIEW E LA English DT Article ID ONE-COMPONENT-PLASMA; MOLECULAR-DYNAMICS SIMULATIONS; EQUATION-OF-STATE; VELOCITY AUTOCORRELATION FUNCTION; STATISTICAL-MECHANICAL THEORY; TRANSPORT-COEFFICIENTS; SELF-DIFFUSION; IRREVERSIBLE PROCESSES; COHERENT APPROACH; KINETIC-THEORY AB In this paper we present molecular dynamics (MD) calculations of the interdiffusion coefficient for asymmetric mixed plasma for thermodynamic conditions relevant to astrophysical and inertial confinement fusion plasmas. Specifically, we consider mixtures of deuterium and argon at temperatures of 100-500 eV and a number density similar to 10(25) ions/cm(3). The motion of 30 000-120 000 ions is simulated in which the ions interact via the Yukawa (screened Coulomb) potential. The electric field of the electrons is included in this effective interaction; the electrons are not simulated explicitly. The species diffusivity is then calculated using the Green-Kubo approach using an integral of the interdiffusion current autocorrelation function, a quantity calculated in the equilibrium MD simulations. Our MD simulation results show that a widely used expression relating the interdiffusion coefficient with the concentration-weighted sum of self-diffusion coefficients overestimates the interdiffusion coefficient. We argue that this effect due to cross-correlation terms in velocities is characteristic of asymmetric mixed plasmas. Comparison of the MD results with predictions of kinetic theories also shows a discrepancy with MD giving effectively a larger Coulomb logarithm. C1 [Haxhimali, Tomorr; Rudd, Robert E.; Cabot, William H.; Graziani, Frank R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Haxhimali, T (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM haxhimali1@llnl.gov FU Laboratory Directed Research and Development Program at LLNL [12-SI-005, 10-ERD-004]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors gratefully acknowledge fruitful discussions with John Castor, Kyle Caspersen, Jeff Greenough, A. Bruce Langdon, Paul Miller, and Heather Whitley. We also thank Michael Murillo for use of his average atom Thomas-Fermi code for the ionization level in mixture, as well as Phil Sterne for his detailed table of Thomas-Fermi results. T.H. acknowledges helpful discussions with Jerome Daligault and Prof. Mark Asta at the initial stage of this work. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. The work was funded by the Laboratory Directed Research and Development Program at LLNL under project tracking codes 12-SI-005 and 10-ERD-004. We gratefully acknowledge supercomputer resources provided through the Institutional Computing Grand Challenge Program at LLNL. NR 88 TC 15 Z9 15 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD AUG 21 PY 2014 VL 90 IS 2 AR 023104 DI 10.1103/PhysRevE.90.023104 PG 16 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AO3TE UT WOS:000341258000009 PM 25215836 ER PT J AU Bruce, R Assmann, RW Boccone, V Bracco, C Brugger, M Cauchi, M Cerutti, F Deboy, D Ferrari, A Lari, L Marsili, A Mereghetti, A Mirarchi, D Quaranta, E Redaelli, S Robert-Demolaize, G Rossi, A Salvachua, B Skordis, E Tambasco, C Valentino, G Weiler, T Vlachoudis, V Wollmann, D AF Bruce, R. Assmann, R. W. Boccone, V. Bracco, C. Brugger, M. Cauchi, M. Cerutti, F. Deboy, D. Ferrari, A. Lari, L. Marsili, A. Mereghetti, A. Mirarchi, D. Quaranta, E. Redaelli, S. Robert-Demolaize, G. Rossi, A. Salvachua, B. Skordis, E. Tambasco, C. Valentino, G. Weiler, T. Vlachoudis, V. Wollmann, D. TI Simulations and measurements of beam loss patterns at the CERN Large Hadron Collider SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID LHC AB The CERN Large Hadron Collider (LHC) is designed to collide proton beams of unprecedented energy, in order to extend the frontiers of high-energy particle physics. During the first very successful running period in 2010-2013, the LHC was routinely storing protons at 3.5-4 TeV with a total beam energy of up to 146 MJ, and even higher stored energies are foreseen in the future. This puts extraordinary demands on the control of beam losses. An uncontrolled loss of even a tiny fraction of the beam could cause a superconducting magnet to undergo a transition into a normal-conducting state, or in the worst case cause material damage. Hence a multistage collimation system has been installed in order to safely intercept high-amplitude beam protons before they are lost elsewhere. To guarantee adequate protection from the collimators, a detailed theoretical understanding is needed. This article presents results of numerical simulations of the distribution of beam losses around the LHC that have leaked out of the collimation system. The studies include tracking of protons through the fields of more than 5000 magnets in the 27 km LHC ring over hundreds of revolutions, and Monte Carlo simulations of particle-matter interactions both in collimators and machine elements being hit by escaping particles. The simulation results agree typically within a factor 2 with measurements of beam loss distributions from the previous LHC run. Considering the complex simulation, which must account for a very large number of unknown imperfections, and in view of the total losses around the ring spanning over 7 orders of magnitude, we consider this an excellent agreement. Our results give confidence in the simulation tools, which are used also for the design of future accelerators. C1 [Bruce, R.; Boccone, V.; Bracco, C.; Brugger, M.; Cauchi, M.; Cerutti, F.; Deboy, D.; Ferrari, A.; Lari, L.; Marsili, A.; Mereghetti, A.; Mirarchi, D.; Quaranta, E.; Redaelli, S.; Rossi, A.; Salvachua, B.; Skordis, E.; Tambasco, C.; Valentino, G.; Weiler, T.; Vlachoudis, V.; Wollmann, D.] CERN, CH-1211 Geneva, Switzerland. [Assmann, R. W.] DESY, D-22607 Hamburg, Germany. [Lari, L.] CSIC UV, IFIC, Valencia 46980, Spain. [Robert-Demolaize, G.] BNL, Upton, NY USA. RP Bruce, R (reprint author), CERN, Geneva 23, CH-1211 Geneva, Switzerland. EM roderik.bruce@cern.ch RI Valentino, Gianluca/I-7518-2016; Assmann, Ralph/L-8457-2016 OI Valentino, Gianluca/0000-0003-3864-7785; FU CERN OP team FX We would like to thank B. Auchmann, R. de Maria, A. Lechner, and F. Schmidt for input and discussions, and the CERN OP team for the support during the loss maps. NR 60 TC 12 Z9 12 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD AUG 21 PY 2014 VL 17 IS 8 AR 081004 DI 10.1103/PhysRevSTAB.17.081004 PG 16 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AO3TW UT WOS:000341259800001 ER PT J AU Stavila, V Talin, AA Allendorf, MD AF Stavila, V. Talin, A. A. Allendorf, M. D. TI MOF-based electronic and optoelectronic devices SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID METAL-ORGANIC FRAMEWORKS; LIQUID-PHASE EPITAXY; POROUS COORDINATION POLYMERS; SECONDARY BUILDING UNITS; BY-STEP ROUTE; THIN-FILMS; CHARGE-TRANSFER; HETEROEPITAXIAL GROWTH; PHOTOVOLTAIC DEVICES; CHEMICAL-DETECTION AB Metal-organic frameworks (MOF5) are a class of hybrid materials with unique Optical and electronic properties arising from rational self-assembly of the organic linkers and metal ions/clusters, yielding myriads of possible structural motifs. The combination of order and chemical tunability, coupled with good environmental stability of MOFs, are prompting many research groups to explore the possibility of incorporating these materials as active components in devices such as solar cells, photodetectors, radiation detectors, and chemical sensors. Although this field is only in its incipiency, many new fundamental insights relevant to integrating MOFs with such devices have already been gained. In this review, we focus our attention on the basic requirements and structural elements needed to fabricate MOF-based devices and summarize the current state of MOF research in the area of electronic, opto-electronic and sensor devices. We summarize various approaches to designing active MOFs, creation of hybrid material systems combining MOFs with other materials, and assembly and integration of MOFs with device hardware. Critical directions of future research are identified, with emphasis on achieving the desired MOF functionality in a device and establishing the structure-property relationships to identify and rationalize the factors that impact device performance. C1 [Stavila, V.; Talin, A. A.; Allendorf, M. D.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Allendorf, MD (reprint author), Sandia Natl Labs, POB 969, Livermore, CA 94551 USA. EM mdallen@sandia.gov FU Laboratory Directed Research and Development Program at Sandia National Laboratories; U.S. DOE Sun Shot Program; U.S. DOE National Nuclear Security Administration [DE-AC04-94AL85000]; Science of Precision Multifunctional Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center - U.S. DOE, Office of Science, Office of Basic Energy Sciences [DESC0001160] FX This work was supported by the Laboratory Directed Research and Development Program at Sandia National Laboratories and the U.S. DOE Sun Shot Program. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. DOE National Nuclear Security Administration under Contract DE-AC04-94AL85000. AAT was supported in part by the Science of Precision Multifunctional Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center funded by the U.S. DOE, Office of Science, Office of Basic Energy Sciences under award DESC0001160. NR 129 TC 232 Z9 232 U1 68 U2 557 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 EI 1460-4744 J9 CHEM SOC REV JI Chem. Soc. Rev. PD AUG 21 PY 2014 VL 43 IS 16 BP 5994 EP 6010 DI 10.1039/c4cs00096j PG 17 WC Chemistry, Multidisciplinary SC Chemistry GA AN3UQ UT WOS:000340514600026 PM 24802763 ER PT J AU Thunga, M Bauer, A Obusek, K Meilunas, R Akinc, M Kessler, MR AF Thunga, Mahendra Bauer, Amy Obusek, Kristine Meilunas, Ray Akinc, Mufit Kessler, Michael R. TI Injection repair of carbon fiber/bismaleimide composite panels with bisphenol E cyanate ester resin SO COMPOSITES SCIENCE AND TECHNOLOGY LA English DT Article DE Polymer-matrix composites (PMCs); Adhesive joints; Thermomechanical properties; Impact behavior; Ultrasonics ID FIBER COMPOSITES; AIRCRAFT; THERMOGRAPHY AB Resin injection of bisphenol E cyanate ester, a low viscosity resin that cures into a high temperature thermoset polymer, is investigated as a reliable repair method to restore strength and stiffness in delaminated carbon fiber/bismaleimide composites used in aircraft panels. The influence of temperature on the viscosity of the uncured resin was measured to optimize the injection conditions for high resin infiltration into the delaminations. The repair efficiency of the resin was evaluated by varying the panel thickness and the method by which the delamination damage was created in the composite specimens. Ultrasonic scanning (C-scan), flash thermography images, and cross-section analysis of repaired panels revealed excellent resin infiltration into the damaged region. Evaluation of mechanical repair efficiency using both bending stiffness and in-plain compressive strength of the composite panels as the repair metrics showed values exceeding 100%. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Thunga, Mahendra; Bauer, Amy; Akinc, Mufit; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA USA. [Thunga, Mahendra; Akinc, Mufit; Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA. [Kessler, Michael R.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Obusek, Kristine] Fleet Readiness Ctr East, Mat Engn Div, Cherry Point, NC USA. [Meilunas, Ray] Naval Air Warfare Ctr, Div Aircraft, Mat Engn Div, Patuxent River, MD USA. RP Kessler, MR (reprint author), Washington State Univ, Sch Mech & Mat Engn, POB 642920, Pullman, WA 99164 USA. EM MichaelR.Kessler@wsu.edu RI Kessler, Michael/C-3153-2008 OI Kessler, Michael/0000-0001-8436-3447 FU ESTCP Program Office [WP-201108] FX The authors would like to acknowledge the funding support by the ESTCP Program Office for this development/validation effort under WP-201108. Special thanks to Dan Barnard and Dr. Steve Holland from the Center for Nondestructive Evaluation, Iowa State University for guidance in C-scan imaging and flash thermography and for providing access to their laboratory facilities. NR 16 TC 6 Z9 8 U1 8 U2 45 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0266-3538 EI 1879-1050 J9 COMPOS SCI TECHNOL JI Compos. Sci. Technol. PD AUG 21 PY 2014 VL 100 BP 174 EP 181 DI 10.1016/j.compscitech.2014.05.024 PG 8 WC Materials Science, Composites SC Materials Science GA AM9SX UT WOS:000340222400024 ER PT J AU Sutter, PM Lavaux, G Wandelt, BD Weinberg, DH Warren, MS Pisani, A AF Sutter, P. M. Lavaux, Guilhem Wandelt, Benjamin D. Weinberg, David H. Warren, Michael S. Pisani, Alice TI Voids in the SDSS DR9: observations, simulations, and the impact of the survey mask SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE methods: data analysis; cosmology: observations; large-scale structure of Universe ID DIGITAL SKY SURVEY; OSCILLATION SPECTROSCOPIC SURVEY; HALO OCCUPATION DISTRIBUTION; EXCURSION SET FORMALISM; DATA RELEASE 7; COSMIC VOIDS; DARK-MATTER; REDSHIFT SURVEY; GALAXY VOIDS; PHOTOMETRIC PROPERTIES AB We present and study cosmic voids identified using the watershed void finder vide in the Sloan Digital Sky Survey Data Release 9, compare these voids to ones identified in mock catalogues, and assess the impact of the survey mask on void statistics such as number functions, ellipticity distributions, and radial density profiles. The nearly 1000 identified voids span three nearly volume-limited samples from redshift z = 0.43 to 0.7. For comparison, we use 98 of the publicly available second-order Lagrangian perturbation theory-based mock galaxy catalogues of Manera et al., and also generate our own mock catalogues by applying a Halo Occupation Distribution model to an N-body simulation. We find that the mask reduces the number density of voids at all scales by a factor of 3 and slightly skews the relative size distributions. This engenders an increase in the mean ellipticity by roughly 30 per cent. However, we find that radial density profiles are largely robust to the effects of the mask. We see excellent agreement between the data and both mock catalogues, and find no tension between the observed void properties and the properties derived from I > colddarkmatter simulations. We have added the void catalogues from both data and mock galaxy populations discussed in this work to the Public Cosmic Void Catalog at ext-link-type="uri" xlink:href="http://www.cosmicvoids.net" xlink:type="simple">http://www.cosmicvoids.net. C1 [Sutter, P. M.; Lavaux, Guilhem; Wandelt, Benjamin D.; Pisani, Alice] Univ Paris 06, Sorbonne Univ, UMR7095, Inst Astrophys Paris, F-75014 Paris, France. [Sutter, P. M.; Lavaux, Guilhem; Wandelt, Benjamin D.; Pisani, Alice] CNRS, UMR7095, Inst Astrophys Paris, F-75014 Paris, France. [Sutter, P. M.; Weinberg, David H.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Sutter, P. M.; Wandelt, Benjamin D.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Lavaux, Guilhem] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada. [Lavaux, Guilhem] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Lavaux, Guilhem] Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. [Wandelt, Benjamin D.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Weinberg, David H.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Warren, Michael S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Sutter, PM (reprint author), Univ Paris 06, Sorbonne Univ, UMR7095, Inst Astrophys Paris, F-75014 Paris, France. EM sutter@iap.fr OI WANDELT, Benjamin/0000-0002-5854-8269; Lavaux, Guilhem/0000-0003-0143-8891 FU NSF [NSF AST 09-08693 ARRA]; ANR Chaire d'Excellence [ANR-10-CEXC-004-01]; UPMC Chaire Internationale in Theoretical Cosmology; NSF grants [AST-0908 902, AST-0708849]; CITA National Fellowship; Government of Canada Post-Doctoral Research Fellowship; Government of Canada through Industry Canada; Province of Ontario through the Ministry of Research and Innovation; NSF Grant [AST-1009505]; French state funds [ANR-10-LABX-63]; ANR within the Investissements d'Avenir programme [ANR-11-IDEX-0004-02] FX PMS and BDW acknowledge support from NSF Grant NSF AST 09-08693 ARRA. BDW acknowledges funding from an ANR Chaire d'Excellence (ANR-10-CEXC-004-01), the UPMC Chaire Internationale in Theoretical Cosmology, and NSF grants AST-0908 902 and AST-0708849. GL acknowledges support from CITA National Fellowship and financial support from the Government of Canada Post-Doctoral Research Fellowship. Research at Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Research and Innovation. DW acknowledges support from NSF Grant AST-1009505. This work made in the ILP LABEX (under reference ANR-10-LABX-63) was supported by French state funds managed by the ANR within the Investissements d'Avenir programme under reference ANR-11-IDEX-0004-02. We would like to thank Nico Hamaus for useful discussions. NR 82 TC 30 Z9 30 U1 0 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD AUG 21 PY 2014 VL 442 IS 4 BP 3127 EP 3137 DI 10.1093/mnras/stu1094 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM5TZ UT WOS:000339924900024 ER PT J AU Braun, H Schmidt, W Niemeyer, JC Almgren, AS AF Braun, H. Schmidt, W. Niemeyer, J. C. Almgren, A. S. TI Large-eddy simulations of isolated disc galaxies with thermal and turbulent feedback SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE turbulence; methods: numerical; stars: formation; galaxies: ISM ID GIANT MOLECULAR CLOUDS; STAR-FORMING GALAXIES; MULTIPHASE INTERSTELLAR-MEDIUM; ACCRETION-DRIVEN TURBULENCE; GAS DEPLETION TIME; NEARBY GALAXIES; GALACTIC DISKS; FORMATION LAW; MILKY-WAY; GRAVITATIONAL-INSTABILITY AB We present a subgrid-scale model for the Multi-phase Interstellar medium, Star formation, and Turbulence (MIST) and explore its behaviour in high-resolution large-eddy simulations of isolated disc galaxies. MIST follows the evolution of a clumpy cold and a diffuse warm component of the gas within a volume element which exchange mass and energy via various cooling, heating and mixing processes. The star formation rate is dynamically computed from the state of the gas in the cold phase. An important feature of MIST is the treatment of unresolved turbulence in the two phases and its interaction with star formation and feedback by supernovae. This makes MIST a particularly suitable model for the interstellar medium in galaxy simulations. We carried out a suite of simulations varying fundamental parameters of our feedback implementation. Several observational properties of galactic star formation are reproduced in our simulations, such as an average star formation efficiency similar to 1 per cent, a typical velocity dispersion around similar to 10 km s(-1) in star-forming regions, and an almost linear relationship between the column densities of star formation and dense molecular gas. C1 [Braun, H.; Schmidt, W.; Niemeyer, J. C.] Univ Gottingen, Inst Astrophys, D-37077 Gottingen, Germany. [Almgren, A. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. RP Braun, H (reprint author), Univ Gottingen, Inst Astrophys, Friedrich Hund Pl 1, D-37077 Gottingen, Germany. EM hbraun@astro.physik.uni-goettingen.de; schmidt@astro.physik.uni-goettingen.de OI Niemeyer, Jens/0000-0002-3063-4325 FU German Research Council [CRC 963]; SciDAC FASTMath Institute-Scientific Discovery through Advanced Computing (SciDAC) program by U.S. Department of Energy; German Research Council FX HB was financially supported by the CRC 963 of the German Research Council. The work of AA was supported by the SciDAC FASTMath Institute, funded by the Scientific Discovery through Advanced Computing (SciDAC) program funded by U.S. Department of Energy. HB, WS and JCN acknowledge financial support by the German Research Council for visits at LBNL. We thank Hsiang-HsuWang for discussions on the initial conditions of idealized IDG. The simulations presented in this article were performed on the SuperMUC of the LRZ (project pr47bi) in Germany. We also acknowledge the yt toolkit by Turk et al. (2011) that was used for our analysis of numerical data. We owe thanks to the referee B. Robertson for a careful and helpful report that helped us to improve this paper. NR 81 TC 6 Z9 6 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD AUG 21 PY 2014 VL 442 IS 4 BP 3407 EP 3426 DI 10.1093/mnras/stu1119 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM5TZ UT WOS:000339924900049 ER PT J AU Callear, SK Ramirez-Cuesta, AJ Kamazawa, K Towata, SI Noritake, T Parker, SF Jones, MO Sugiyama, J Ishikiriyama, M David, WIF AF Callear, Samantha K. Ramirez-Cuesta, Anibal J. Kamazawa, Kazuya Towata, Shin-ichi Noritake, Tatsuo Parker, Stewart F. Jones, Martin O. Sugiyama, Jun Ishikiriyama, Mamoru David, William I. F. TI Understanding composition property relationships in Ti-Cr-V-Mo alloys for optimisation of hydrogen storage in pressurised tanks SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID INELASTIC NEUTRON-SCATTERING; BCT MONOHYDRIDE PHASE; LATTICE-DYNAMICS; H SYSTEM; TRANSITION-METALS; VANADIUM HYDRIDE; SITE OCCUPATION; LOCAL MODES; DIFFUSION; TITANIUM AB The location of hydrogen within Ti-Cr-V-Mo alloys has been investigated during hydrogen absorption and desorption using in situ neutron powder diffraction and inelastic neutron scattering. Neutron powder diffraction identifies a low hydrogen equilibration pressure body-centred tetragonal phase that undergoes a martensitic phase transition to a face-centred cubic phase at high hydrogen equilibration pressures. The average location of the hydrogen in each phase has been identified from the neutron powder diffraction data although inelastic neutron scattering combined with density functional theory calculations show that the local structure is more complex than it appears from the average structure. Furthermore the origin of the change in dissociation pressure and hydrogen trapping on cycling in Ti-Cr-V-Mo alloys is discussed. C1 [Callear, Samantha K.; Ramirez-Cuesta, Anibal J.; Parker, Stewart F.; Jones, Martin O.; David, William I. F.] Rutherford Appleton Lab, STFC, ISIS Facil, Chilton OX11 0QX, Oxon, England. [Ramirez-Cuesta, Anibal J.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Kamazawa, Kazuya; Towata, Shin-ichi; Noritake, Tatsuo; Sugiyama, Jun] Toyota Cent Res & Dev Labs Inc, Nagakute, Aichi 4801192, Japan. [Kamazawa, Kazuya] IBARAKI Quantum Beam Res Ctr IQBRC, CROSS, Tokai, Ibaraki 3191106, Japan. [Ishikiriyama, Mamoru] Toyota Motor Co Ltd, Higashifuji Tech Ctr, Adv Mat Engn Div, Toyota, Aichi, Japan. [David, William I. F.] Univ Oxford, Inorgan Chem Lab, Oxford OX1 3QR, England. [Towata, Shin-ichi] Aichi Synchrotron Radiat Ctr, Aichi Sci & Technol Fdn, Seto, Aichi 4890965, Japan. RP Callear, SK (reprint author), Rutherford Appleton Lab, STFC, ISIS Facil, Chilton OX11 0QX, Oxon, England. EM Sam.Callear@stfc.ac.uk; towata@astf.or.jp RI Ramirez-Cuesta, Timmy/A-4296-2010; Sugiyama, Jun/M-6535-2015; OI Ramirez-Cuesta, Timmy/0000-0003-1231-0068; Sugiyama, Jun/0000-0002-0916-5333; Parker, Stewart/0000-0002-3228-2570 NR 56 TC 0 Z9 0 U1 2 U2 30 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD AUG 21 PY 2014 VL 16 IS 31 BP 16563 EP 16572 DI 10.1039/c4cp01666a PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AM7VB UT WOS:000340075700026 PM 24984893 ER PT J AU Zhang, XM Yu, SS Zheng, WT Liu, P AF Zhang, Xiaoming Yu, Shansheng Zheng, Weitao Liu, Ping TI Stability of Pt near surface alloys under electrochemical conditions: a model study SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID OXYGEN REDUCTION REACTION; DENSITY-FUNCTIONAL THEORY; ELECTRONIC-STRUCTURE; BIMETALLIC SURFACES; SINGLE-CRYSTALS; 1ST PRINCIPLES; ELECTROCATALYSTS; PLATINUM; ADSORPTION; MONOLAYER AB The stability is one of the key requirements for commercializing the fuel cell electrocatalysts in automotive applications. For the widely used Pt-based catalysts, it can be achieved by the formation of a stable Pt skin on the surface. Here, we employed density functional theory (DFT) to explore the stability of monolayer Pt (Pt-ML) on various near surface alloy (NSAs) surfaces, Pt-ML/M-ML/Pt(111) (M = Fe, Co, Ni, Cu; Ru, Rh, Pd, Ag; Os, Ir, Au), under various environmental conditions. Our results show that under the vacuum condition, the alloying M except Ag and Au thermodynamically prefer to stay in the subsurface and the formation of Pt-ML on the surface is thermodynamically favored. A barrier has to be overcome for M to segregate. The situation varies under various electrochemical conditions. Depending on the solutions and the operating reaction pathway, different M should be considered for alloying with Pt to maintain the stability of surface Pt-ML PtRh and PtPd are the only two systems, where the surface Pt-ML is likely to stay intact in perchloric acid (HClO4), sulfuric acid (H2SO4), phosphoric acid (H3PO4) and alkaline solutions as well as under the oxygen reduction reaction (ORR) conditions via different pathways. Ptlr should also be paid attention, which falls only during the ORR via the OOH intermediate. Our results highlight the importance of chemical environments in affecting the stability of the catalysts. C1 [Zhang, Xiaoming; Yu, Shansheng; Zheng, Weitao] Jilin Univ, Dept Mat Sci, Key Lab Mobile Mat, MOE, Changchun 130012, Peoples R China. [Zhang, Xiaoming; Yu, Shansheng; Zheng, Weitao] Jilin Univ, State Key Lab Superhard Mat, Changchun 130012, Peoples R China. [Liu, Ping] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Zheng, WT (reprint author), Jilin Univ, Dept Mat Sci, Key Lab Mobile Mat, MOE, Changchun 130012, Peoples R China. EM wtzheng@jlu.edu.cn; pingliu3@bnl.gov RI Yu, Shansheng/O-8578-2015; OI Yu, Shansheng/0000-0001-9493-6341; zheng, weitao/0000-0002-9028-278X FU US Department of Energy, Office of Science [DE-AC02-98CH10886]; National Natural Science Foundation of China [51372095] FX P.L. would like to thank the funding from the US Department of Energy, Office of Science under Contract No. DE-AC02-98CH10886, and W.T.Z. would like to thank the funding from National Natural Science Foundation of China (No. 51372095). The DFT calculations utilized resources at the Center for Functional Nanomaterials (CFN), Brookhaven National Laboratory and High Performance Computing Center, Jilin University. NR 49 TC 4 Z9 4 U1 10 U2 108 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD AUG 21 PY 2014 VL 16 IS 31 BP 16615 EP 16622 DI 10.1039/c4cp01942c PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AM7VB UT WOS:000340075700031 PM 24994557 ER PT J AU Zhang, L Zhou, TY Tian, J Wang, H Zhang, DW Zhao, X Liu, Y Li, ZT AF Zhang, Liang Zhou, Tian-You Tian, Jia Wang, Hui Zhang, Dan-Wei Zhao, Xin Liu, Yi Li, Zhan-Ting TI A two-dimensional single-layer supramolecular organic framework that is driven by viologen radical cation dimerization and further promoted by cucurbit[8]uril SO POLYMER CHEMISTRY LA English DT Article ID MOLECULAR RECOGNITION; POLYMERS; POLYMERIZATION; CHEMISTRY; WATER; METHYLVIOLOGEN; ASSEMBLIES; NANOSHEETS; INTERFACE; GROWTH AB A two-dimensional supramolecular organic framework has been constructed in water from a rigid water-soluble triangular building block which is driven by the dimerization of three appended viologen radical cation units. Cucurbit[8]uril (CB[8]) further stabilizes the single-layer network by encapsulating the stacking viologen radical cation dimers. The new supramolecular networks have been characterized with UV-vis absorption, electron paramagnetic resonance, dynamic light scattering, solution and solid phase small angle X-ray diffraction, and AFM experiments. The aggregation behaviour is in sharp contrast to that of a triangular control compound, which only forms a discrete dimer or a 2 : 3 encapsulation complex in the absence or presence of CB[8]. C1 [Zhang, Liang; Tian, Jia; Wang, Hui; Zhang, Dan-Wei; Li, Zhan-Ting] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China. [Zhou, Tian-You; Zhao, Xin] Chinese Acad Sci, Shanghai Inst Organ Chem, Shanghai 200032, Peoples R China. [Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Zhang, DW (reprint author), Fudan Univ, Dept Chem, 220 Handan Rd, Shanghai 200433, Peoples R China. EM zhangdw@fudan.edu.cn; yliu@lbl.gov; ztli@fudan.edu.cn RI Liu, yi/A-3384-2008; Tian, Jia/O-2758-2014; Foundry, Molecular/G-9968-2014 OI Liu, yi/0000-0002-3954-6102; Tian, Jia/0000-0001-6793-2804; FU Ministry of Science and Technology [2013CB834501]; Ministry of Education [IRT1117]; National Natural Science Foundation of China [91227108, 21228203, J1103304]; Science and Technology Commission of Shanghai Municipality [13NM1400200]; Molecular Foundry, Lawrence Berkeley National Laboratory; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We are grateful to the Ministry of Science and Technology (2013CB834501), the Ministry of Education (IRT1117), and the National Natural Science Foundation (91227108, 21228203, and J1103304) of China, and Science and Technology Commission of Shanghai Municipality (13NM1400200) for financial support and Shanghai Synchrotron Radiation Facility for providing BL14B1 beamline for collecting the solution-phase synchrotron X-ray diffraction data. Y. L. thanks the support from the Molecular Foundry, Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 64 TC 34 Z9 38 U1 6 U2 64 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1759-9954 EI 1759-9962 J9 POLYM CHEM-UK JI Polym. Chem. PD AUG 21 PY 2014 VL 5 IS 16 BP 4715 EP 4721 DI 10.1039/c4py00139g PG 7 WC Polymer Science SC Polymer Science GA AM5VY UT WOS:000339930300014 ER PT J AU Davidson, SD Zhang, H Sun, JM Wang, Y AF Davidson, Stephen D. Zhang, He Sun, Junming Wang, Yong TI Supported metal catalysts for alcohol/sugar alcohol steam reforming SO DALTON TRANSACTIONS LA English DT Article ID PD-ZN CATALYST; MC FUEL-CELL; HYDROGEN-PRODUCTION; COBALT CATALYSTS; H-2 PRODUCTION; THERMODYNAMIC ANALYSIS; NI CATALYSTS; BIMETALLIC CATALYSTS; MECHANISTIC ASPECTS; CU/ZRO2 CATALYSTS AB Despite extensive studies on hydrogen production via steam reforming of alcohols and sugar alcohols, catalysts typically suffer a variety of issues from poor hydrogen selectivity to rapid deactivation. Here, we summarize recent advances in fundamental understanding of functionality and structure of catalysts for alcohol/sugar alcohol steam reforming, and provide perspectives on further development required to design highly efficient steam reforming catalysts. C1 [Davidson, Stephen D.; Zhang, He; Sun, Junming; Wang, Yong] Washington State Univ, Pullman, WA 99163 USA. [Davidson, Stephen D.; Zhang, He; Sun, Junming; Wang, Yong] Washington State Univ, Sch Chem Engn & Bioengineering, Pullman, WA 99163 USA. [Wang, Yong] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99354 USA. RP Sun, JM (reprint author), Washington State Univ, Pullman, WA 99163 USA. EM Junming.sun@wsu.edu; Yong.wang@pnnl.gov RI Sun, Junming/B-3019-2011 OI Sun, Junming/0000-0002-0071-9635 FU US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences FX We acknowledge the financial support from the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. NR 128 TC 11 Z9 12 U1 1 U2 29 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 EI 1477-9234 J9 DALTON T JI Dalton Trans. PD AUG 21 PY 2014 VL 43 IS 31 BP 11782 EP 11802 DI 10.1039/c4dt00521j PG 21 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AM4YP UT WOS:000339862400001 PM 24687117 ER PT J AU Kumar, N Camaioni, DM Dupuis, M Raugei, S Appel, AM AF Kumar, N. Camaioni, D. M. Dupuis, M. Raugei, S. Appel, A. M. TI Mechanistic insights into hydride transfer for catalytic hydrogenation of CO2 with cobalt cornplexes SO DALTON TRANSACTIONS LA English DT Article ID TRANSITION-METAL HYDRIDES; CARBON-DIOXIDE; FORMIC-ACID; RUTHENIUM(II)-CATALYZED HYDROGENATION; HOMOGENEOUS HYDROGENATION; PINCER COMPLEX; ENERGY; REDUCTION; NI; DIHYDRIDE AB The catalytic hydrogenation of CO2 to formate by Co(dmpe)(2)H can proceed via direct hydride transfer or via CO2 coordination to Co followed by reductive elimination of formate. The different nature of the rate-determining step in the two mechanisms may provide new insights into designing catalysts with improved performance. C1 [Kumar, N.; Camaioni, D. M.; Dupuis, M.; Raugei, S.; Appel, A. M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Raugei, S (reprint author), Pacific NW Natl Lab, POB 999,MS K2-57, Richland, WA 99352 USA. EM simone.raugei@pnnl.gov RI Kumar, Neeraj/M-3279-2015 OI Kumar, Neeraj/0000-0001-6713-2129 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Center for Molecular Electrocatalysis, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science FX The authors thank Dr Jonathan M. Darmon for the preparation of the Cover Artwork. The research by N.K., D.M.C. and A.M.A. was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. The research by S.R. and M.D. was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for the DOE by Battelle. NR 29 TC 24 Z9 24 U1 4 U2 112 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 EI 1477-9234 J9 DALTON T JI Dalton Trans. PD AUG 21 PY 2014 VL 43 IS 31 BP 11803 EP 11806 DI 10.1039/c4dt01551g PG 4 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AM4YP UT WOS:000339862400002 PM 24946902 ER PT J AU Scheinker, A Baily, S Young, D Kolski, JS Prokop, M AF Scheinker, Alexander Baily, Scott Young, Daniel Kolski, Jeffrey S. Prokop, Mark TI In-hardware demonstration of model-independent adaptive tuning of noisy systems with arbitrary phase drift SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Linac; Adaptive control; Feedback control; Model independent control; RF cavity; Phase drift AB In this work, an implementation of a recently developed model-independent adaptive control scheme, for tuning uncertain and time varying systems, is demonstrated on the Los Alamos linear particle accelerator. The main benefits of the algorithm are its simplicity, ability to handle an arbitrary number of components without increased complexity, and the approach is extremely robust to measurement noise, a property which is both analytically proven and demonstrated in the experiments performed. We report on the application of this algorithm for simultaneous tuning of two buncher radio frequency (RF) cavities, in order to maximize beam acceptance into the accelerating electromagnetic field cavities of the machine, with the tuning based only on a noisy measurement of the surviving beam current downstream from the two bunching cavities. The algorithm automatically responds to arbitrary phase shift of the cavity phases, automatically re-tuning the cavity settings and maximizing beam acceptance. Because it is model independent it can be utilized for continuous adaptation to time-variation of a large system, such as due to thermal drift, or damage to components, in which the remaining, functional components would be automatically re-tuned to compensate for the failing ones. We start by discussing the general model-independent adaptive scheme and how it may be digitally applied to a large class of multi-parameter uncertain systems, and then present our experimental results. Published by Elsevier B.V. C1 [Scheinker, Alexander; Baily, Scott; Young, Daniel; Kolski, Jeffrey S.; Prokop, Mark] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Scheinker, A (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM alexscheinker@gmail.com NR 17 TC 4 Z9 4 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD AUG 21 PY 2014 VL 756 BP 30 EP 38 DI 10.1016/j.nima.2014.04.026 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AK3TO UT WOS:000338347800006 ER PT J AU Fisyak, Y Tsai, O Videbaek, F Xu, ZB AF Fisyak, Yuri Tsai, Oleg Videbaek, Flemming Xu, Zhangbu TI Thermal neutron flux measurements in the STAR experimental hall SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Thermal neutrons; Measurements; Simulation ID CALORIMETERS AB We report measurements of thermal neutron fluxes aL different locations in the STAR experimental hall during RHIC Run 13 with proton-proton collisions at root s= 510 GeV. We compare these measurements to calculations based on PYTHlA as a minimum bias event generator, detailed GEANT3 simulation of the STAR detector and experimental hall, and with GCALOR as the neutron transport code. A fairly good agreement was found between simulation and measurements. (C) 2014 Elsevier B.V. All rights reserved. C1 [Fisyak, Yuri; Videbaek, Flemming; Xu, Zhangbu] Brookhaven Natl Lab, Upton, NY 11973 USA. [Tsai, Oleg] Univ Calif Los Angeles, Dept Phys, Los Angeles, CA 90095 USA. RP Fisyak, Y (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM fisyak@bnl.gov OI Fisyak, Yuri/0000-0002-3151-8377 FU Office of NP within the U.S. DOE Office of Science; Office of HEP within the U.S. DOE Office of Science FX We thank Brookhaven National Laboratory Instrumentation Division and, especially, G. Smith and N. Schaknowski, for the He3 detector, and S. Trentalange for a careful reading of this manuscript. We thank the STAR Collaboration, the RHIC Operations Group and RCF at BNL. This work was supported by the Offices of NP and HEP within the U.S. DOE Office of Science. NR 20 TC 3 Z9 3 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD AUG 21 PY 2014 VL 756 BP 68 EP 72 DI 10.1016/j.nima.2014.04.035 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AK3TO UT WOS:000338347800011 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, TD Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA PerezTomei, T Gregores, EM Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Geiser, A Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G Hempel, M Horton, D Jung, H Kasemann, M Katsas, P Kieseler, J Kleinwort, C Kramer, M Krucker, D Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Ntomari, E Perrey, H Petrukhin, A Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Riedl, C Ron, E Sahin, MO Salfeld-Nebgen, J Saxena, P Schmidt, R Schoerner-Sadenius, T Schroder, M Stein, M Trevino, ADRV Walsh, R Wissing, C Martin, MA Blobel, V Enderle, H Erfle, J Garutti, E Goebel, K Gorner, M Gosselink, M Haller, J Hoing, RS Kirschenmann, H Klanner, R Kogler, R Lange, J Lapsien, T Lenz, T Marchesini, I Ott, J Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hartmann, F Hauth, T Held, H Hoffmann, KH Husemann, U Katkov, I Kornmayer, A Kuznetsova, E Pardo, PL Martschei, D Mozer, MU Muller, T Niegel, M Nurnberg, A Oberst, O Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Wolf, R Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Psallidas, A Topsis-Giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Jones, J Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mittal, M Nishu, N Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, S Jain, S Khurana, R Modak, A Mukherjee, S Roy, D Sarkar, S Sharan, M Singh, AP Abdulsalam, A Dutta, D Kailas, S Kumar, V Mohanty, AK Pant, LM Shukla, P Topkar, A Aziz, T Chatterjee, RM Ganguly, S Ghosh, S Guchait, M Gurtu, A Kole, G Kumar, S Maity, M Majumder, G Mazumdar, K Mohanty, GB Parida, B Sudhakar, K Wickramage, N Banerjee, S Dugad, S Arfaei, H Bakhshiansohi, H Behnamian, H Etesami, SM Fahim, A Jafari, A Khakzad, M Najafabadi, MM Naseri, M Mehdiabadi, SP Safarzadeh, B Zeinali, M Grunewald, M Abbrescia, M Barbone, L Calabria, C Chhibra, SS Colaleo, A Creanza, D De Filippis, N De Palma, M Fiore, L Iaselli, G Maggi, G Maggi, M Marangelli, B My, S Nuzzo, S Pacifico, N Pompili, A Pugliese, G Radogna, R Selvaggi, G Silvestris, L Singh, G Venditti, R Verwilligen, P Zito, G Abbiendi, G Benvenuti, AC Bonacorsi, D Braibant-Giacomelli, S Brigliadori, L Campanini, R Capiluppi, P Castro, A Cavallo, FR Codispoti, G Cuffiani, M Dallavalle, GM Fabbri, F Fanfani, A Fasanella, D Giacomelli, P Grandi, C Guiducci, L Marcellini, S Masetti, G Meneghelli, M Montanari, A Navarria, FL Odorici, F Perrotta, A Primavera, F Rossi, AM Rovelli, T Siroli, GP Tosi, N Travaglini, R Albergo, S Cappello, G Chiorboli, M Costa, S Giordano, F Potenza, R Tricomi, A Tuve, C Barbagli, G Ciulli, V Civinini, C D'Alessandro, R Focardi, E Gallo, E Gonzi, S Gori, V Lenzi, P Meschini, M Paoletti, S Sguazzoni, G Tropiano, A Benussi, L Bianco, S Fabbri, F Piccolo, D Fabbricatore, P Ferretti, R Ferro, F Lo Vetere, M Musenich, R Robutti, E Tosi, S Dinardo, ME Fiorendi, S Gennai, S Gerosa, R Ghezzi, A Govoni, P Lucchini, MT Malvezzi, S Manzoni, RA Martelli, A Marzocchi, B Menasce, D Moroni, L Paganoni, M Pedrini, D Ragazzi, S Redaelli, N de Fatis, TT Buontempo, S Cavallo, N Di Guida, S Fabozzi, F Iorio, AOM Lista, L Meola, S Merola, M Paolucci, P Azzi, P 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Panwalkar, S. Park, M. Patel, R. Rekovic, V. Robles, J. Salur, S. Schnetzer, S. Seitz, C. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. Yang, Z. C. York, A. Bouhali, O. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Safonov, A. Sakuma, T. Suarez, I. Tatarinov, A. Toback, D. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wood, J. Gollapinni, S. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Belknap, D. A. Borrello, L. Carlsmith, D. Cepeda, M. Dasu, S. Duric, S. Friis, E. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Woods, N. CA CMS Collaboration TI Search for anomalous production of events with three or more leptons in pp collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID PARTICLE PHYSICS; STANDARD MODEL; SUPERSYMMETRY; SQUARK; LHC; STATES; HIGGS; BOSON AB A search for physics beyond the standard model in events with at least three leptons is presented. The data sample, corresponding to an integrated luminosity of 19.5 fb(-1) of proton-proton collisions with center-of-mass energy root s = 8 TeV, was collected by the CMS experiment at the LHC during 2012. The data are divided into exclusive categories based on the number of leptons and their flavor, the presence or absence of an opposite-sign, same-flavor lepton pair (OSSF), the invariant mass of the OSSF pair, the presence or absence of a tagged bottom-quark jet, the number of identified hadronically decaying tau leptons, and the magnitude of the missing transverse energy and of the scalar sum of jet transverse momenta. The numbers of observed events are found to be consistent with the expected numbers from standard model processes, and limits are placed on new-physics scenarios that yield multilepton final states. In particular, scenarios that predict Higgs boson production in the context of supersymmetric decay chains are examined. We also place a 95% confidence level upper limit of 1.3% on the branching fraction for the decay of a top quark to a charm quark and a Higgs boson (t -> cH), which translates to a bound on the left-and right-handed top-charm flavor-violating Higgs Yukawa couplings, lambda(H)(tc) and lambda(H)(ct), respectively, of root vertical bar lambda(H)(tc)vertical bar(2)+ vertical bar lambda(H)(tc)vertical bar(2) < 0.21. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. 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M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Malek, M.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santaolalla, J.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dias, F. A.; PerezTomei, T.; Novaes, S. F.; Padula, S. S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Genchev, V.; Iaydjiev, P.; Marinov, A.; Piperov, S.; Rodozov, M.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Du, R.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Plestina, R.; Tao, J.; Wang, X.; Wang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, Q.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, CY-1678 Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Mahrous, A.; Radi, A.] Egyptian Network High Energy Phys, Acad Sci Res & Technol Arab Republ Egypt, Cairo, Egypt. [Giammanco, A.; Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.] IN2P3 CNRS, Ecole Polytech, Lab Leprince Ringuet, Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Bloch, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.] Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, Univ Haute Alsace Mulhouse, CNRS IN2P3, Strasbourg, France. [Gadrat, S.] CNRS IN2P3, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Montoya, C. A. Carrillo; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Alvarez, J. D. Ruiz; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.; Leonidov, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Geiser, A.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Kraemer, M.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Ntomari, E.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. O.; Salfeld-Nebgen, J.; Saxena, P.; Schmidt, R.; Schoerner-Sadenius, T.; Schroeder, M.; Stein, M.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Goebel, K.; Gorner, M.; Gosselink, M.; Haller, J.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Mueller, T.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Jones, J.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Plestina, R.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Debrecen Univ Med, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, S.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Mumbai, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, I-40126 Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Asghar, M. I.; Butt, J.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.; Bialkowska, H.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Golutvin, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Tikhonenko, E.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Y.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Contardo, D.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Evangelou, I.; Foudas, C.; Bencze, G.; Mohanty, A. K.; Giordano, F.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; Palla, F.; Pelliccioni, M.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Favaro, C.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Guelmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Guenaydin, Y. O.; Vardarli, F. I.; Yuecel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Richardson, C.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Calderon De La Barca Sanchez, M.; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wurthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Gaz, A.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stockli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. 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[Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Mahrous, A.] Helwan Univ, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. Univ Kansas, Lawrence, KS 66045 USA. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] Ctr Natl Rech Sci CNRS IN2P3, Paris, France. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Bluj, M.] Natl Ctr Nucl Res, Otwock, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Istanbul Univ, Fac Sci, Istanbul, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Guenaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Pioppi, M.] Univ Perugia, INFN Sez Perugia, I-06100 Perugia, Italy. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Benussi, Luigi/O-9684-2014; Lo Vetere, Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Grandi, Claudio/B-5654-2015; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Rovelli, Tiziano/K-4432-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Petrushanko, Sergey/D-6880-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Lazzizzera, Ignazio/E-9678-2015; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013 OI Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Benussi, Luigi/0000-0002-2363-8889; Lo Vetere, Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074; Grandi, Claudio/0000-0001-5998-3070; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Korenkov, Vladimir/0000-0002-2342-7862; Heath, Helen/0000-0001-6576-9740; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Sogut, Kenan/0000-0002-9682-2855; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Longo, Egidio/0000-0001-6238-6787; Gerosa, Raffaele/0000-0001-8359-3734; Covarelli, Roberto/0000-0003-1216-5235; Lazzizzera, Ignazio/0000-0001-5092-7531; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy and the Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, and University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion; Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; U.S. Department of Energy; U.S. National Science Foundation; Marie-Curie program; European Research Council and EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education,Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS program of Foundation for Polish Science; EU, Regional Development Fund; EU-ESF; Greek NSRF; Croatian Science Foundation; National Science Centre, Poland FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent Financing Contract No.; SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the U.S. Department of Energy, and the U.S. National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education,Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS program of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF. NR 73 TC 28 Z9 28 U1 5 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 20 PY 2014 VL 90 IS 3 AR 032006 DI 10.1103/PhysRevD.90.032006 PG 27 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CJ4WI UT WOS:000355488100001 ER PT J AU Yamaoka, H Ikeda, Y Jarrige, I Tsujii, N Zekko, Y Yamamoto, Y Mizuki, J Lin, JF Hiraoka, N Ishii, H Tsuei, KD Kobayashi, TC Honda, F Onuki, Y AF Yamaoka, H. Ikeda, Y. Jarrige, I. Tsujii, N. Zekko, Y. Yamamoto, Y. Mizuki, J. Lin, J. -F. Hiraoka, N. Ishii, H. Tsuei, K. -D. Kobayashi, T. C. Honda, F. Onuki, Y. TI Role of Valence Fluctuations in the Superconductivity of Ce122 Compounds SO PHYSICAL REVIEW LETTERS LA English DT Article ID TEMPERATURE SPECIFIC-HEAT; NEUTRON-SCATTERING; CRYSTAL-FIELD; KONDO-LATTICE; HIGH-PRESSURE; CECU2SI2; CECU2GE2; PHASE; TRANSITION; BEHAVIOR AB Pressure dependence of the Ce valence in CeCu2Ge2 has been measured up to 24 GPa at 300 K and to 17 GPa at 18-20Kusing x-ray absorption spectroscopy in the partial fluorescence yield. Asmooth increase of the Ce valence with pressure is observed across the two superconducting (SC) regions without any noticeable irregularity. The chemical pressure dependence of the Ce valence was also measured in Ce(Cu1-xNix)(2)Si-2 at 20 K. Avery weak, monotonic increase of the valence with x was observed, without any significant change in the two SC regions. Within experimental uncertainties, our results showno evidence for the valence transition with an abrupt change in the valence state near the SC II region, challenging the valence-fluctuation mediated superconductivity model in these compounds at high pressure and low temperature. C1 [Yamaoka, H.] RIKEN, SPring Ctr 8, Sayo, Hyogo 6795148, Japan. [Ikeda, Y.; Kobayashi, T. C.] Okayama Univ, Dept Phys, Okayama 7008530, Japan. [Jarrige, I.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Tsujii, N.] Natl Inst Mat Sci, Quantum Beam Ctr, Tsukuba, Ibaraki 3050047, Japan. [Zekko, Y.; Yamamoto, Y.; Mizuki, J.] Kwansei Gakuin Univ, Grad Sch Sci & Technol, Sanda, Hyogo 6691337, Japan. [Lin, J. -F.] Univ Texas Austin, Dept Geol Sci, Austin, TX 78712 USA. [Lin, J. -F.] Ctr High Pressure Sci & Technol Adv Res HPSTAR, Shanghai 201203, Peoples R China. [Hiraoka, N.; Ishii, H.; Tsuei, K. -D.] Natl Synchrotron Radiat Res Ctr, Hsinchu 30076, Taiwan. [Honda, F.] Tohoku Univ, Inst Mat Res, Oarai, Ibaraki 3111313, Japan. [Onuki, Y.] Univ Ryukyus, Fac Sci, Okinawa 9030213, Japan. RP Yamaoka, H (reprint author), RIKEN, SPring Ctr 8, Sayo, Hyogo 6795148, Japan. RI Lin, Jung-Fu/B-4917-2011; KOBAYASHI, Tatsuo/B-1527-2011; HONDA, Fuminori/D-5578-2015; Ikeda, Yoichi/B-9997-2016; Jarrige, Ignace/M-6371-2016; Tsujii, Naohito/H-2544-2011 OI HONDA, Fuminori/0000-0002-9485-7384; Ikeda, Yoichi/0000-0001-5266-5512; Jarrige, Ignace/0000-0002-1043-5695; Tsujii, Naohito/0000-0002-6181-5911 FU Japan Society for the Promotion of Science; HPSTAR; EFree, an Energy Frontier Research Center - U.S. Department of Energy Office of Science, Office of Basic Energy Sciences [DE-SC0001057] FX The experiments were performed at Taiwan beam line BL12XU (under Proposals No. 2011B4259, No. 2012A4259, No. 2012B4253, No. 2013A4250, and No. 2013A4254), SPring-8. This work is partly supported by a Grant in Aid for Scientific research from the Japan Society for the Promotion of Science. This work at UT Austin was supported by HPSTAR and EFree, an Energy Frontier Research Center funded by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences under Award DE-SC0001057. NR 52 TC 10 Z9 10 U1 3 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 20 PY 2014 VL 113 IS 8 AR 086403 DI 10.1103/PhysRevLett.113.086403 PG 6 WC Physics, Multidisciplinary SC Physics GA AW8IF UT WOS:000346504200009 PM 25192112 ER PT J AU Meinert, M Geisler, MP Schmalhorst, J Heinzmann, U Arenholz, E Hetaba, W Stoger-Pollach, M Hutten, A Reiss, G AF Meinert, Markus Geisler, Manuel P. Schmalhorst, Jan Heinzmann, Ulrich Arenholz, Elke Hetaba, Walid Stoeger-Pollach, Michael Huetten, Andreas Reiss, Guenter TI Experimental realization of a semiconducting full-Heusler compound: Fe2TiSi SO PHYSICAL REVIEW B LA English DT Article ID FE2VAL; MAGNETORESISTANCE; RESISTIVITY; SPECTRA AB Single-phase films of the full-Heusler compound Fe2TiSi have been prepared by magnetron sputtering. The compound is found to be a semiconductor with a gap of 0.4 eV. The electrical resistivity has a logarithmic temperature dependence up to room temperature due to Kondo scattering of a dilute free electron gas off superparamagnetic impurities. The origin of the electron gas is extrinsic due to residual off-stoichiometry. Density functional theory calculations of the electronic structure are in excellent agreement with electron energy loss, optical, and x-ray absorption experiments. Fe2TiSi may find applications as a thermoelectric material. C1 [Meinert, Markus; Geisler, Manuel P.; Schmalhorst, Jan; Hetaba, Walid; Huetten, Andreas; Reiss, Guenter] Univ Bielefeld, Ctr Spinelect Mat & Devices, D-33501 Bielefeld, Germany. [Heinzmann, Ulrich] Univ Bielefeld, Dept Phys, D-33501 Bielefeld, Germany. [Arenholz, Elke] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Hetaba, Walid; Stoeger-Pollach, Michael] Vienna Univ Technol, Univ Serv Ctr Transmiss Electron Microscopy, A-1040 Vienna, Austria. RP Meinert, M (reprint author), Univ Bielefeld, Ctr Spinelect Mat & Devices, D-33501 Bielefeld, Germany. EM meinert@physik.uni-bielefeld.de RI Meinert, Markus/E-8794-2011; Reiss, Gunter/A-3423-2010; Heinzmann, Ulrich/A-6248-2012 OI Meinert, Markus/0000-0002-7813-600X; Reiss, Gunter/0000-0002-0918-5940; FU Ministerium fur Innovation, Wissenschaft, und Forschung des Landes Nordrhein-Westfalen (MIWF NRW); Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank the Ministerium fur Innovation, Wissenschaft, und Forschung des Landes Nordrhein-Westfalen (MIWF NRW) for financial support. We also thank the developers of the ELK code, for their efforts. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 33 TC 5 Z9 5 U1 3 U2 53 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 20 PY 2014 VL 90 IS 8 AR 085127 DI 10.1103/PhysRevB.90.085127 PG 5 WC Physics, Condensed Matter SC Physics GA AS1BO UT WOS:000344011800003 ER PT J AU Skinner, B AF Skinner, Brian TI Coulomb disorder in three-dimensional Dirac systems SO PHYSICAL REVIEW B LA English DT Article ID SEMIMETAL; PHASE AB In three-dimensional materials with a Dirac spectrum, weak short-ranged disorder is essentially irrelevant near the Dirac point. This is manifestly not the case for Coulomb disorder, where the long-ranged nature of the potential produced by charged impurities implies large fluctuations of the disorder potential even when impurities are sparse, and these fluctuations are screened by the formation of electron/hole puddles. In this paper, I present a theory of such nonlinear screening of Coulomb disorder in three-dimensional Dirac systems, and I derive the typical magnitude of the disorder potential, the corresponding density of states, and the size and density of electron/hole puddles. The resulting conductivity is also discussed. C1 Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Skinner, B (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. OI Skinner, Brian/0000-0003-0774-3563 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX I am grateful to R. Nandkishore, S. Gopalakrishnan, J. C. W. Song, B. I. Shklovskii, and E. B. Kolomeisky for helpful discussions and comments. Work at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 30 TC 21 Z9 21 U1 5 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 20 PY 2014 VL 90 IS 6 AR 060202 DI 10.1103/PhysRevB.90.060202 PG 5 WC Physics, Condensed Matter SC Physics GA AS1BL UT WOS:000344011500001 ER PT J AU Pratt, HD Pratt, WR Fang, XK Hudak, NS Anderson, TM AF Pratt, Harry D., III Pratt, William R. Fang, Xikui Hudak, Nicholas S. Anderson, Travis M. TI Mixed-Metal, Structural, and Substitution Effects of Polyoxometalates on Electrochemical Behavior in a Redox Flow Battery SO ELECTROCHIMICA ACTA LA English DT Article DE Flow battery; Polyoxometalates; Iron; Vanadium; Magnetic susceptibility ID MOLECULAR CLUSTER BATTERIES; MULTI-IRON SILICOTUNGSTATES; ENERGY-STORAGE; TRANSPORTATION; CHEMISTRY; SINGLE AB A pair of redox flow batteries containing polyoxometalates was tested as part of an ongoing program in stationary energy storage. The iron-containing dimer, (SiFe3W9(OH)(3)O-34)(2)(OF)(3)(11-), cycled between (SiFe3W9(OH)(3)O-34)(2)(OF)(3)(11-)/(SiFe3W9(OH)(3)O-34)(2)(OH)(3)(14-)and (SiFe3W9(OH)(3)O-34)(2)(OH)(3)(17-)/(SiFe3W9(OH)(3)O-34)(2)(OH)(3)(14-) for the positive and negative electrode, respectively. This compound demonstrated a coulombic efficiency of 83% after 20 cycles with an electrochemical yield (measured discharge capacity as a percentage of theoretical capacity) of 55%. Cyclic voltammetry on the Lindqvist ion, cis-V2W4O194-, showed quasi-reversible vanadium electrochemistry, but tungsten reduction was mostly irreversible. In a flow cell configuration, cis-V(2)W(4)O(19)(4-)had a coulombic efficiency of 45% (for a two-electron process) and an electrochemical yield of 16% after 20 cycles. The poor performance of cis-V(2)W(4)O(19)(4-)was attributed primarily to its higher charge density. Collectively, the results showed that both polyoxometalate size and charge density are both important parameters to consider in battery material performance. Published by Elsevier Ltd. C1 [Pratt, Harry D., III; Pratt, William R.; Hudak, Nicholas S.; Anderson, Travis M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Fang, Xikui] Ames Lab, Ames, IA 50011 USA. RP Anderson, TM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tmander@sandia.gov RI Hudak, Nicholas/D-3529-2011 FU U. S. Department of Energy, Office of Electricity Delivery and Energy Reliability; U. S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Department of Energy, Basic Energy Sciences [DE-AC02-07CH11358] FX We thank the U. S. Department of Energy, Office of Electricity Delivery and Energy Reliability (Dr. Imre Gyuk, Energy Storage Program), for funding. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U. S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The work at Ames Laboratory (magnetic measurements) was supported by the Department of Energy, Basic Energy Sciences under Contract No, DE-AC02-07CH11358. NR 24 TC 2 Z9 2 U1 9 U2 67 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD AUG 20 PY 2014 VL 138 BP 210 EP 214 DI 10.1016/j.electacta.2014.06.110 PG 5 WC Electrochemistry SC Electrochemistry GA AO6LQ UT WOS:000341464000027 ER PT J AU Roller, J Yu, H Vukmirovic, MS Bliznakov, S Kotula, PG Carter, CB Adzic, RR Maric, R AF Roller, J. Yu, H. Vukmirovic, M. S. Bliznakov, S. Kotula, P. G. Carter, C. B. Adzic, R. R. Maric, R. TI Flame-Based Synthesis of Core-Shell Structures Using Pd-Ru and Pd Cores SO ELECTROCHIMICA ACTA LA English DT Article DE Core-shell; Fuel cell; Flame synthesis; Oxygen reduction; Flame processing ID PLATINUM-MONOLAYER ELECTROCATALYSTS; OXYGEN-REDUCTION REACTION; FUEL-CELL ELECTROCATALYSTS; O-2 REDUCTION; NANOPARTICLES; DEPOSITION; CATALYSTS; SURFACES; WATER; HYDROGEN AB Core nanoparticles of Pd, Pd-Ru, and Pd supported on an amorphous carbon are deposited, by a flame-based process, onto glassy carbon rotating disk electrodes and gas diffusion layers. A Pt monolayer was deposited using galvanic displacement of an underpotentially deposited Cu monolayer with Pt. The Pt monolayer is then tested to determine the electrochemical surface area and activity toward the oxygen reduction reaction. Depositions of the Pd core were applied at substrate temperatures of 250 degrees C and 150 degrees C. A Pt-ML/Pd(250 degrees C) has higher Pt mass and specific ORR activities than Pt-ML/Pd(150 degrees C). This is due to smoother surface of Pd (250 degrees C) compared to Pd (150 degrees C). During membrane electrode assembly testing in O-2, the Pt mass activity was 0.532 A/mg(pt) at 0.9 V. The voltage at 1 A/cm(2) was 0.613 V, and a peak power density of 0.93 W/cm(2) was achieved. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Roller, J.; Carter, C. B.; Maric, R.] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Roller, J.; Yu, H.; Maric, R.] Univ Connecticut, Ctr Clean Energy Engn, Storrs, CT 06269 USA. [Yu, H.; Carter, C. B.; Maric, R.] Univ Connecticut, Dept Chem & Biomol Engn, Storrs, CT 06269 USA. [Carter, C. B.; Maric, R.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. [Vukmirovic, M. S.; Bliznakov, S.; Adzic, R. R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Kotula, P. G.] Sandia Natl Labs, Mat Characterizat Dept, Albuquerque, NM 87185 USA. RP Roller, J (reprint author), Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. EM justin.roller@fei.com RI Kotula, Paul/A-7657-2011 OI Kotula, Paul/0000-0002-7521-2759 FU University of Connecticut School of Engineering; NSF CMMI grant [1265893]; United States Department of Energy [DE-AC04-94AL85000]; US Department of Energy, Division of Chemical Sciences, Geosciences, and Biosciences Division [DE-AC02-98CH10886] FX The authors wish to acknowledge the University of Connecticut School of Engineering for partial funding of this work and the NSF CMMI grant #1265893 for funding of the RSDT processing part of the research. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under contract DE-AC04-94AL85000. Work at Brookhaven National Laboratory is supported by the US Department of Energy, Division of Chemical Sciences, Geosciences, and Biosciences Division, under the Contract No. DE-AC02-98CH10886. NR 52 TC 5 Z9 5 U1 5 U2 61 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD AUG 20 PY 2014 VL 138 BP 341 EP 352 DI 10.1016/j.electacta.2014.06.113 PG 12 WC Electrochemistry SC Electrochemistry GA AO6LQ UT WOS:000341464000044 ER PT J AU Chatrchyan, S Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CDO De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Geiser, A Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G Hempel, M Horton, D Jung, H Kasemann, M Katsas, P Kieseler, J Kleinwort, C Kramer, M Krucker, D Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Ntomari, E Perrey, H Petrukhin, A Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Riedl, C Ron, E Sahin, MO Salfeld-Nebgen, J Saxena, P Schmidt, R Schoerner-Sadenius, T Schroder, M Stein, M Trevino, ADRV Walsh, R Wissing, C Martin, MA Blobel, V Enderle, H Erfle, J Garutti, E Goebel, K Gorner, M Gosselink, M Haller, J Hoing, RS Kirschenmann, H Klanner, R Kogler, R Lange, J Lapsien, T Lenz, T Marchesini, I Ott, J Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hartmann, F Hauth, T Held, H Hoffmann, KH Husemann, U Katkov, I Kornmayer, A Kuznetsova, E Pardo, PL Martschei, D Mildner, H Mozer, MU Muller, T Niegel, M Nurnberg, A Oberst, O Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Williamson, S Wolf, R Zeise, M Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Psallidas, A Topsis-Giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Jones, J Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mittal, M Nishu, N Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, S Jain, S Khurana, R Modak, A Mukherjee, S Roy, D Sarkar, S Sharan, M Singh, AP Abdulsalam, A Dutta, D Kailas, S Kumar, V Mohanty, AK Pant, LM Shukla, P Topkar, A Aziz, T Chatterjee, RM Ganguly, S Ghosh, S Guchait, M Gurtu, A Kole, G Kumar, S Maity, M Majumder, G Mazumdar, K Mohanty, GB Parida, B Sudhakar, K Wickramage, N Banerjee, S Dewanjee, RK Dugad, S Arfaei, H Bakhshiansohi, H Behnamian, H Etesami, SM Fahim, A Jafari, A Khakzad, M Najafabadi, MM Naseri, M Mehdiabadi, SP Safarzadeh, B Zeinali, M Grunewald, M Abbrescia, M Barbone, L Calabria, C Chhibra, SS Colaleo, A Creanza, D De Filippis, N De Palma, M Fiore, L Iaselli, G Maggi, G Maggi, M Marangelli, B My, S Nuzzo, S Pacifico, N Pompili, A Pugliese, G Radogna, R Selvaggi, G Silvestris, L Singh, G Venditti, R Verwilligen, P Zito, G Abbiendi, G Benvenuti, AC Bonacorsi, D Braibant-Giacomelli, S Brigliadori, L Campanini, R Capiluppi, P Castro, A 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Lath, A. Panwalkar, S. Park, M. Patel, R. Rekovic, V. Robles, J. Salur, S. Schnetzer, S. Seitz, C. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. Yang, Z. C. York, A. Bouhali, O. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Rose, A. Safonov, A. Sakuma, T. Suarez, I. Tatarinov, A. Toback, D. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wood, J. Gollapinni, S. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Belknap, D. A. Borrello, L. Carlsmith, D. Cepeda, M. Dasu, S. Duric, S. Friis, E. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Woods, N. CA CMS Collaboration TI Measurement of jet multiplicity distributions in t(t)over-bar production in pp collisions at root s=7TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PARTON DISTRIBUTIONS; LHC AB The normalised differential top quark-antiquark production cross section is measured as a function of the jet multiplicity in proton-proton collisions at a centre-of-mass energy of 7 TeV at the LHC with the CMS detector. The measurement is performed in both the dilepton and lepton+jets decay channels using data corresponding to an integrated luminosity of 5.0 fb(-1). Using a procedure to associate jets to decay products of the top quarks, the differential cross section of the t (t) over bar production is determined as a function of the additional jet multiplicity in the lepton+jets channel. Furthermore, the fraction of events with no additional jets is measured in the dilepton channel, as a function of the threshold on the jet transverse momentum. The measurements are compared with predictions from perturbative quantum chromodynamics and no significant deviations are observed. C1 [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Crucy, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Komm, M.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, Louvain La Neuve, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; Correa Martins, M., Jr.; Martins, T.; Souza, M. H. G.; Polatoz, A.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Alda Junior, W. L.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Malek, M.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santaolalla, J.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dias, F. A.; Fernandez Perez Tomei, T. R.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Genchev, V.; Iaydjiev, P.; Marinov, A.; Piperov, S.; Rodozov, M.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Du, R.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Plestina, R.; Tao, J.; Wang, X.; Wang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, Q.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.; Tikvica, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Mahrous, A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J-L; Andrea, J.; Bloch, D.; Brom, J-M; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J-C; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, P.; Le Bihan, A-C; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Montoya, C. A. Carrillo; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Alvarez, J. D. Ruiz; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, Inst Phys Nucl Lyon, CNRS, IN2P3, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.; Tatarinov, A.] Rhein Westfal TH Aachen, Inst Phys 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Geiser, A.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Kraemer, M.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I-A; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Ntomari, E.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. Oe; Salfeld-Nebgen, J.; Saxena, P.; Schmidt, R.; Schoerner-Sadenius, T.; Schroeder, M.; Stein, M.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.; Choudhary, B. C.; Benhabib, L.] DESY, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Gosselink, M.; Haller, J.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mildner, H.; Mozer, M. U.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F-P; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Williamson, S.; Wolf, R.; Zeise, M.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Jones, J.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa; Jain, Sh; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, EHEP, Bombay 400005, Maharashtra, India. [Banerjee, S.; Dewanjee, R. K.; Dugad, S.] Tata Inst Fundamental Res, HECR, Bombay 400005, Maharashtra, India. [Mohammadi, A.; Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Tricomi, A.; Tuve, C.; Potenza, A.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, M.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennaia, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Biasotto, M.; Branca, A.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Galanti, M.; Gasparini, F.; Giubilato, P.; Gozzelino, A.; Gulmini, M.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Maron, G.; Meneguzzo, A. T.; Michelotto, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Sgaravatto, M.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Branca, A.; Galanti, M.; Gasparini, F.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.; Romero, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.; Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Asghar, M. I.; Butt, J.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Bunin, P.; Gavrilenko, M.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Kozlov, G.; Lanev, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Zarubin, A.; Smirnov, I.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Gavrilenko, M.; Epshteyn, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Contardo, D.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Evangelou, I.; Foudas, C.; Bencze, G.; Sharma, A.; Mohanty, A. K.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; Martinez, P.; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Favaro, C.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W-S; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R-S; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Nat Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol BS8 1TH, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A-M; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.; Liu, H.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL 35487 USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Richardson, C.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Longo, E.; Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Grunewald, M.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J-P; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y-J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, D.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. 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[Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Taegu 702701, South Korea. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Gonzalez Caballero, Isidro/E-7350-2010; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Da Silveira, Gustavo Gil/N-7279-2014; Haj Ahmad, Wael/E-6738-2016; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; Michelotto, Michele/A-9571-2013; My, Salvatore/I-5160-2015; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Scodellaro, Luca/K-9091-2014; Cerrada, Marcos/J-6934-2014; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; Lazzizzera, Ignazio/E-9678-2015 OI Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Haj Ahmad, Wael/0000-0003-1491-0446; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; Michelotto, Michele/0000-0001-6644-987X; My, Salvatore/0000-0002-9938-2680; Codispoti, Giuseppe/0000-0003-0217-7021; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIEN-CIAS (Colombia); MSES (Croatia); CSF (Croatia); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie doorWetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU; Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIEN-CIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF(Germany); GSRT(Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie doorWetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 52 TC 4 Z9 4 U1 6 U2 69 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 20 PY 2014 VL 74 IS 8 AR 3014 DI 10.1140/epjc/s10052-014-3014-0 PG 29 WC Physics, Particles & Fields SC Physics GA AN8AV UT WOS:000340824000001 ER PT J AU Duoss, EB Weisgraber, TH Hearon, K Zhu, C Small, W Metz, TR Vericella, JJ Barth, HD Kuntz, JD Maxwell, RS Spadaccini, CM Wilson, TS AF Duoss, Eric B. Weisgraber, Todd H. Hearon, Keith Zhu, Cheng Small, Ward Metz, Thomas R. Vericella, John J. Barth, Holly D. Kuntz, Joshua D. Maxwell, Robert S. Spadaccini, Christopher M. Wilson, Thomas S. TI Three-Dimensional Printing of Elastomeric, Cellular Architectures with Negative Stiffness SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID POISSONS RATIO; MICROVASCULAR NETWORKS; WAVE-GUIDES; METAMATERIALS; SCAFFOLDS; BEHAVIOR; DESIGN AB Three-dimensional printing of viscoelastic inks to create porous, elastomeric architectures with mechanical properties governed by the ordered arrangement of their sub-millimeter struts is reported. Two layouts are patterned, one resembling a "simple cubic" (SC)-like structure and another akin to a "face-centered tetragonal" (FCT) configuration. These structures exhibit markedly distinct load response with directionally dependent behavior, including negative stiffness. More broadly, these findings suggest the ability to independently tailor mechanical response in cellular solids via micro-architected design. Such ordered materials may one day replace random foams in mechanical energy absorption applications. C1 [Duoss, Eric B.; Weisgraber, Todd H.; Hearon, Keith; Zhu, Cheng; Small, Ward; Metz, Thomas R.; Vericella, John J.; Barth, Holly D.; Kuntz, Joshua D.; Maxwell, Robert S.; Spadaccini, Christopher M.; Wilson, Thomas S.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Duoss, EB (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM duoss1@llnl.gov; spadaccini2@llnl.gov; wilson97@llnl.gov RI ZHU, CHENG/J-4692-2016 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Laboratory Directed Research and Development Strategic Initiative program [11-SI-005]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; IM Review [LLNL-JRNL-646053] FX E.B.D. and T. H. W. contributed equally to this work. The authors thank Charles Anderson, Matt Lampe, and Dan Bowen at Kansas City Plant for useful discussions. The authors acknowledge Michael Puso, Ian Darnell, and Robert Ferencz for helpful discussions on implementing the NIKE3D software. The authors acknowledge the photograph in Figure 1 a by Jamie Douglas. The authors thank Mark Pearson for assistance with mechanical testing. The authors also acknowledge Scott Fisher for design and assembly of the in situ compression apparatus for SR mu T imaging. The authors acknowledge the use of the Synchrotron Radiation micro-Tomography beam-line (8.3.2) at the Advanced Light Source (ALS) at Lawrence Berkeley National Laboratory. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors also thank Prof. Duncan J. Maitland at Texas A&M University for volunteering the use of the TA Instruments Q800 Dynamic Mechanical Analyzer for the shear sandwich DMA experiments reported in this study. The authors also thank Sean Kohl and TA Instruments for kindly volunteering the use of the Q800 shear sandwich clamps used in the shear sandwich DMA experiments in this study. This work was funded by the Laboratory Directed Research and Development Strategic Initiative program, 11-SI-005, and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 with IM Review No. LLNL-JRNL-646053. NR 38 TC 22 Z9 22 U1 19 U2 98 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD AUG 20 PY 2014 VL 24 IS 31 BP 4905 EP 4913 DI 10.1002/adfm.201400451 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AN6CW UT WOS:000340682300004 ER PT J AU Srivastava, VK Quinlan, RA Agapov, AL Dunlap, JR Nelson, KM Duranty, E Sokolov, AP Bhat, GS Mays, JW AF Srivastava, Vikram K. Quinlan, Ronald A. Agapov, Alexander L. Dunlap, John R. Nelson, Kimberly M. Duranty, Edward Sokolov, Alexei P. Bhat, Gajanan S. Mays, Jimmy W. TI Macroscopic Properties of Restacked, Redox-Liquid Exfoliated Graphite and Graphite Mimics Produced in Bulk Quantities SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID METAL DICHALCOGENIDE NANOSHEETS; BORON-NITRIDE NANOSHEETS; FEW-LAYER GRAPHENE; MOLYBDENUM-DISULFIDE; ATOMIC LAYERS; ORGANIC FUNCTIONALIZATION; INTERCALATION COMPOUNDS; PHASE EXFOLIATION; SINGLE-LAYER; MOS2 AB The excellent properties exhibited by monolayer graphene have spurred the development of exfoliation techniques using bulk graphite to produce large quantities of pristine monolayer sheets. Development of simple chemistry to exfoliate and intercalate graphite and graphite mimics in large quantities is required for numerous applications. To determine the macroscopic behavior of restacked, exfoliated bulk materials, a systematic approach is presented using a simple, redox-liquid sonication process along to obtain large quantities of 2D and 3D hexagonally layered graphite, molybdenum disulfide, and boron nitride, which are subsequently characterized to observe chemical and structural changes. For MoS2 sonicated with the antioxidant sodium bisulfite, results from Raman spectroscopy, X-ray diffraction, and electron microscopy indicate the presence of distorted phases from different polymorphs, and apparent nanotube structures in the bulk, restacked powder. Furthermore, using thermograviemtric analysis, the antioxidant enhances the resistance to oxidative degradation of MoS2, upon thermal treatment up to 900 degrees C. The addition of the ionic antioxidant decreased dispersion stability in non-polar solvent, suggesting decreased compatibility with non-polar systems. Using simple chemical methods, the ability to generate tailored multidimensional layered materials with unique macroscopic properties is critical for numerous applications, including electrical devices, reinforced polymer composites, lithium-ion capacitors, and chemical sensing. C1 [Srivastava, Vikram K.; Agapov, Alexander L.; Nelson, Kimberly M.; Duranty, Edward; Sokolov, Alexei P.; Mays, Jimmy W.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Sokolov, Alexei P.; Mays, Jimmy W.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Quinlan, Ronald A.] Naval Surface Warfare Ctr, Mat & Power Syst Branch, Carderock Div, West Bethesda, MD 20817 USA. [Dunlap, John R.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Bhat, Gajanan S.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Srivastava, VK (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM vsrivast@utk.edu; jimmymays@utk.edu FU Office of Naval Research [N00014-10-1-0393]; Carderock Division of the Naval Surface Warfare Center's In-house Laboratory Independent Research Program [0601152N]; Division of Materials Science and Engineering, US Department of Energy, Office of Basic Energy Sciences FX This research was supported by the Office of Naval Research (Award No. N00014-10-1-0393). R. A. Q. acknowledges financial support by the Carderock Division of the Naval Surface Warfare Center's In-house Laboratory Independent Research Program administrated under ONR's Program Element 0601152N. A. L. A., K.M.N., A. P. S., and J.W.M. acknowledge partial support from the Division of Materials Science and Engineering, US Department of Energy, Office of Basic Energy Sciences. NR 72 TC 0 Z9 0 U1 7 U2 85 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD AUG 20 PY 2014 VL 24 IS 31 BP 4969 EP 4977 DI 10.1002/adfm.201400484 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AN6CW UT WOS:000340682300012 ER PT J AU Cooper, M AF Cooper, Marcia TI Optically recording velocity interferometer system configurations and impact of target surface reflectance properties [Invited] SO APPLIED OPTICS LA English DT Article ID LIGHT-SCATTERING; ROUGHNESS; DENSITY AB The utility of the optically recording velocity interferometer system (ORVIS) diagnostic to be configured to meet specific experimental needs in terms of line- and surface-imaging modes enabling direct control of the spatial, temporal, and velocity sensitivities is presented along with two case studies of gas gun testing with highly heterogeneous materials. These experiments have successfully coupled two and three ORVIS interferometers onto a single experiment. Light collection from the target reflector is of critical importance to successful test execution. By utilizing the established field of electromagnetic wave scattering from rough surfaces, the reflectance characteristics of several ORVIS reflectors are qualitatively and quantitatively analyzed in terms of the surface roughness statistics, power spectral density, and bidirectional reflectance distribution function. Insights into the impact of the surfaces on ORVIS image records are quantified. Through method development for quantitatively characterizing reflector surfaces, future experimentation can begin with an ability to tailor a reflector to a given test material and experimental arrangement. C1 Sandia Natl Labs, Explos Technol Grp, Albuquerque, NM 87185 USA. RP Cooper, M (reprint author), Sandia Natl Labs, Explos Technol Grp, POB 5800, Albuquerque, NM 87185 USA. EM macoope@sandia.gov FU U. S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The author gratefully acknowledges Wayne Trott for use of his profilometer data, his experiences in surface preparation, and the many fruitful discussions that have contributed significantly to this work. Funding support to conduct the three-interferometer test on the sinusoidal driver is gratefully acknowledged from Tracy Vogler, Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U. S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Approved for unlimited release, SAND2014-3517J. NR 26 TC 1 Z9 1 U1 2 U2 3 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD AUG 20 PY 2014 VL 53 IS 24 BP F21 EP F30 DI 10.1364/AO.53.000F21 PG 10 WC Optics SC Optics GA AN8BE UT WOS:000340825000003 PM 25321138 ER PT J AU Kouri, DP Shields, EA AF Kouri, Drew P. Shields, Eric A. TI Efficient multiframe super-resolution for imagery with lateral shifts SO APPLIED OPTICS LA English DT Article ID REGISTRATION; RESOLUTION; RECONSTRUCTION; ALGORITHMS; QUALITY AB Trade studies used to design optical imaging systems frequently result in systems being undersampled. The resolution of such systems is limited by the finite size of the detector pixels rather than the cutoff spatial frequency of the optical system. Multiframe super-resolution techniques can be used to combine a number of spatially displaced images from such systems into a single, high-resolution image. Nonlinear optimization techniques have frequently been used to solve this problem. Such techniques define an objective function and use numerical optimization methods to obtain a solution. These numerical methods are often more efficient when derivatives of the objective function with respect to the variables can be calculated analytically rather than numerically. We demonstrate for the simple motion model of pure lateral translation that the derivatives of the objective function with respect to the image lateral shifts can be calculated analytically to speed optimization calculations. (C) 2014 Optical Society of America C1 [Kouri, Drew P.; Shields, Eric A.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Shields, EA (reprint author), Sandia Natl Labs, 1515 Eubank Blvd SE, Albuquerque, NM 87123 USA. EM eashiel@sandia.gov FU U. S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U. S. Department of Energy National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 18 TC 3 Z9 3 U1 1 U2 6 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD AUG 20 PY 2014 VL 53 IS 24 BP F1 EP F9 DI 10.1364/AO.53.0000F1 PG 9 WC Optics SC Optics GA AN8BE UT WOS:000340825000002 PM 25321136 ER PT J AU Reichardt, TA Collins, AM McBride, RC Behnke, CA Timlin, JA AF Reichardt, Thomas A. Collins, Aaron M. McBride, Robert C. Behnke, Craig A. Timlin, Jerilyn A. TI Spectroradiometric monitoring for open outdoor culturing of algae and cyanobacteria SO APPLIED OPTICS LA English DT Article ID REMOTE-SENSING REFLECTANCE; INHERENT OPTICAL-PROPERTIES; FLUORESCENCE QUANTUM YIELD; SELF-SHADING CORRECTION; DIEL PATTERNS; CHLOROPHYLL-A; SPIRULINA-PLATENSIS; HYDROGEN-PRODUCTION; SURFACE REFLECTION; COASTAL WATERS AB We assess the measurement of hyperspectral reflectance for outdoor monitoring of green algae and cyanobacteria cultures with a multichannel, fiber-coupled spectroradiometer. Reflectance data acquired over a 4-week period are interpreted via numerical inversion of a reflectance model, in which the above-water reflectance is expressed as a quadratic function of the single backscattering albedo, which is dependent on the absorption and backscatter coefficients. The absorption coefficient is treated as the sum of component spectra consisting of the cultured species (green algae or cyanobacteria), dissolved organic matter, and water (including the temperature dependence of the water absorption spectrum). The backscatter coefficient is approximated as the scaled Hilbert transform of the culture absorption spectrum with a wavelength-independent vertical offset. Additional terms in the reflectance model account for the pigment fluorescence features and the water-surface reflection of sunlight and skylight. For the green algae and cyanobacteria, the wavelength-independent vertical offset of the backscatter coefficient is found to scale linearly with daily dry weight measurements, providing the capability for a nonsampling measurement of biomass in outdoor ponds. Other fitting parameters in the reflectance model are compared with auxiliary measurements and physics-based calculations. The model-derived magnitudes of sunlight and skylight water-surface reflections compare favorably with Fresnel reflectance calculations, while the model-derived quantum efficiency of Chl-alpha fluorescence is found to be in agreement with literature values. Finally, the water temperatures derived from the reflectance model exhibit excellent agreement with thermocouple measurements during the morning hours but correspond to significantly elevated temperatures in the afternoon hours. (C) 2014 Optical Society of America C1 [Reichardt, Thomas A.] Sandia Natl Labs, Remote Sensing & Energet Mat Dept, Livermore, CA 94551 USA. [Collins, Aaron M.; Timlin, Jerilyn A.] Sandia Natl Labs, Bioenergy & Def Technol Dept, Albuquerque, NM 87185 USA. [McBride, Robert C.; Behnke, Craig A.] Sapphire Energy, San Diego, CA 92121 USA. RP Reichardt, TA (reprint author), Sandia Natl Labs, Remote Sensing & Energet Mat Dept, POB 969,MS 9056, Livermore, CA 94551 USA. EM tareich@sandia.gov OI Timlin, Jerilyn/0000-0003-2953-1721 FU U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy (DOE/EERE) Integrated Biorefinery Award [BM0102060-05794-1004173]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We gratefully acknowledge Kathy Alam (Sandia National Laboratories, New Mexico, USA) for guidance on using the spectrophotometer for absorbance measurements. This work was supported by the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy (DOE/EERE) Integrated Biorefinery Award # BM0102060-05794-1004173. Sandia is a multiprogram laboratory operated by the Sandia Corporation, a wholly owned subsidiary of the Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 99 TC 1 Z9 1 U1 4 U2 27 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD AUG 20 PY 2014 VL 53 IS 24 BP F31 EP F45 DI 10.1364/AO.53.000F31 PG 15 WC Optics SC Optics GA AN8BE UT WOS:000340825000004 PM 25321139 ER PT J AU Schrader, KN Subia, SR Myre, JW Summers, KL AF Schrader, Karl N. Subia, Samuel R. Myre, John W. Summers, Kenneth L. TI Ray tracing in a finite-element domain using nodal basis functions SO APPLIED OPTICS LA English DT Article ID GRADIENT-INDEX MEDIA AB A method is presented for tracing rays through a medium discretized as finite-element volumes. The ray-trajectory equations are cast into the local element coordinate frame, and the full finite-element interpolation is used to determine instantaneous index gradient for the ray-path integral equation. The finite-element methodology is also used to interpolate local surface deformations and the surface normal vector for computing the refraction angle when launching rays into the volume, and again when rays exit the medium. The procedure is applied to a finite-element model of an optic with a severe refractive-index gradient, and the results are compared to the closed-form gradient ray-path integral approach. (C) 2014 Optical Society of America C1 [Schrader, Karl N.; Subia, Samuel R.; Myre, John W.; Summers, Kenneth L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Schrader, KN (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM kschrad@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000, SAND2014-2030J] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. (SAND2014-2030J). NR 14 TC 1 Z9 1 U1 1 U2 1 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD AUG 20 PY 2014 VL 53 IS 24 BP F10 EP F20 DI 10.1364/AO.53.000F10 PG 11 WC Optics SC Optics GA AN8BE UT WOS:000340825000001 PM 25321137 ER PT J AU Boye, R AF Boye, Robert TI Sandia National Laboratories Focus Issue: introduction SO APPLIED OPTICS LA English DT Editorial Material AB For more than six decades, Sandia has provided the critical science and technology to address the nation's most challenging issues. Our original nuclear weapons mission has been complemented with work in defense systems, energy and climate, as well as international and homeland security. Our vision is to be a premier science and engineering laboratory for technology solutions to the most challenging problems that threaten peace and freedom for our nation and the globe. (C) 2014 Optical Society of America C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Boye, R (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM rboye@sandia.gov NR 0 TC 0 Z9 0 U1 1 U2 3 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD AUG 20 PY 2014 VL 53 IS 24 BP SL1 EP SL1 DI 10.1364/AO.53.000SL1 PG 1 WC Optics SC Optics GA AN8BE UT WOS:000340825000005 PM 25321140 ER PT J AU McKellar, BHJ Goldman, TJ Stephenson, GJ AF McKellar, Bruce H. J. Goldman, T. J. Stephenson, G. J., Jr. TI Effective masses in a dense fermion background - Applied to neutrinos, dark matter and dark energy SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Article DE Neutrino effective mass; dark matter; dark energy ID ACCELERATING UNIVERSE; SUPERNOVAE; RANGE AB If fermions interact with a scalar field, and there are many fermions present the scalar field may develop an expectation value and generate an effective mass for the fermions. This can lead to the formation of fermion clusters, which could be relevant for neutrino astrophysics and for dark matter astrophysics. Because this system may exhibit negative pressure, it also leads to a model of dark energy. C1 [McKellar, Bruce H. J.] Univ Melbourne, Sch Phys, Australian Res Council, Ctr Excellence Particle Phys Terrascale, Melbourne, Vic 3010, Australia. [Goldman, T. J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Goldman, T. J.; Stephenson, G. J., Jr.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87501 USA. RP McKellar, BHJ (reprint author), Univ Melbourne, Sch Phys, Australian Res Council, Ctr Excellence Particle Phys Terrascale, Melbourne, Vic 3010, Australia. EM bhjm@unimelb.edu.au; tgoldman@lanl.gov; gjs@swcp.com FU Centre of Excellence for Particle Physics at the Terrascale; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; Australian Research Council and his home institutions - the University of Melbourne FX B. H. J. McKellar wishes to express his thanks to the organisers, particularly Harald Fritzsch, for a great conference; the IAS NTU for their hospitality: and the Australian Research Council and his home institutions - the University of Melbourne and the Centre of Excellence for Particle Physics at the Terrascale - for their support.; The work of T. J. Goldman was carried out in part under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 14 TC 0 Z9 0 U1 0 U2 0 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD AUG 20 PY 2014 VL 29 IS 21 SI SI AR 1444010 DI 10.1142/S0217751X14440102 PG 18 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AO0MR UT WOS:000341004300011 ER PT J AU Malmali, M Stickel, JJ Wickramasinghe, SR AF Malmali, Mohammadmahdi Stickel, Jonathan J. Wickramasinghe, S. Ranil TI Sugar concentration and detoxification of clarified biomass hydrolysate by nanofiltration SO SEPARATION AND PURIFICATION TECHNOLOGY LA English DT Article DE Filtration; Acetic acid; Biomass; Fouling; Permeability; Rejection ID ENZYMATIC CELLULOSE HYDROLYSIS; REVERSE-OSMOSIS MEMBRANES; PHYSIOCHEMICAL PROPERTIES; NF MEMBRANES; SEPARATION; REACTOR; COMPONENTS; CHEMISTRY; ACID; PH AB Development of efficient unit operations is critical in order to design economically viable processes for conversion of lignocellulosic biomass into chemicals and fuels. Here the use of nanofiltration membranes for concentration of sugars in a lignocellulosic biomass hydrolysate has been explored. In addition, simultaneous removal of compounds such as acetic acid, 5-(hydroxymethyl)furfural and furfural which are inhibitory to the microorganisms used in the subsequent fermentation step has also been investigated. Dead-end filtration experiments have been used to test a number of commercially available nanofiltration membranes under a range of operating conditions. Model feed streams as well as real hydrolysates have been tested. The results obtained here indicate that both concentration of sugars and removal of hydrolysis degradation products are feasible. However careful selection of the membrane and operating conditions are essential. The introduction of a nanofiltration step for concentration of sugars and removal of hydrolysis degradation products could enable the development of a continuous process for biomass hydrolysis. (C) 2014 Elsevier B.V. All rights reserved. C1 [Malmali, Mohammadmahdi; Wickramasinghe, S. Ranil] Univ Arkansas, Ralph E Martin Dept Chem Engn, Fayetteville, AR 72701 USA. [Stickel, Jonathan J.] Natl Bioenergy Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Wickramasinghe, SR (reprint author), Univ Arkansas, Ralph E Martin Dept Chem Engn, Fayetteville, AR 72701 USA. EM ranil.wickrmasinghe@uark.edu RI Malmali, Mohammadmahdi/N-4441-2015 OI Malmali, Mohammadmahdi/0000-0001-5190-1261 FU Untied States Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory [AFA-1-11658-01] FX This work was funded by the Untied States Department of Energy (Contract No. DE-AC36-08-GO28308) and the National Renewable Energy Laboratory via subcontract AFA-1-11658-01. The authors gratefully acknowledge Dr. Frank Lipnizki from Alfa Laval for providing the Alfa Laval membranes. NR 28 TC 7 Z9 7 U1 2 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1383-5866 EI 1873-3794 J9 SEP PURIF TECHNOL JI Sep. Purif. Technol. PD AUG 20 PY 2014 VL 132 BP 655 EP 665 DI 10.1016/j.seppur.2014.06.014 PG 11 WC Engineering, Chemical SC Engineering GA AN0UX UT WOS:000340300600077 ER PT J AU Ak, NF Brandt, WN Hall, PB Schneider, DP Trump, JR Anderson, SF Hamann, F Myers, AD Paris, I Petitjean, P Ross, NP Shen, Y York, D AF Ak, N. Filiz Brandt, W. N. Hall, P. B. Schneider, D. P. Trump, J. R. Anderson, S. F. Hamann, F. Myers, Adam D. Paris, I. Petitjean, P. Ross, Nicholas P. Shen, Yue York, Don TI THE DEPENDENCE OF C IV BROAD ABSORPTION LINE PROPERTIES ON ACCOMPANYING Si IV AND Al III ABSORPTION: RELATING QUASAR-WIND IONIZATION LEVELS, KINEMATICS, AND COLUMN DENSITIES SO ASTROPHYSICAL JOURNAL LA English DT Article DE quasars: absorption lines ID DIGITAL SKY SURVEY; OSCILLATION SPECTROSCOPIC SURVEY; ACTIVE GALACTIC NUCLEI; DATA RELEASE 9; SDSS-III; DISK WINDS; MULTIYEAR TIMESCALES; EMISSION-LINES; MILKY-WAY; VARIABILITY AB We consider how the profile and multi-year variability properties of a large sample of C IV Broad Absorption Line (BAL) troughs change when BALs from Si IV and/or Al III are present at corresponding velocities, indicating that the line of sight intercepts at least some lower ionization gas. We derive a number of observational results for C IV BALs separated according to the presence or absence of accompanying lower ionization transitions, including measurements of composite profile shapes, equivalent width (EW), characteristic velocities, composite variation profiles, and EW variability. We also measure the correlations between EW and fractional-EW variability for C IV, Si IV, and Al III. Our measurements reveal the basic correlated changes between ionization level, kinematics, and column density expected in accretion-disk wind models; e. g., lines of sight including lower ionization material generally show deeper and broader C IV troughs that have smaller minimum velocities and that are less variable. Many C IV BALs with no accompanying Si IV or Al III BALs may have only mild or no saturation. C1 [Ak, N. Filiz; Brandt, W. N.; Schneider, D. P.; Trump, J. R.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Ak, N. Filiz; Brandt, W. N.; Schneider, D. P.; Trump, J. R.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Ak, N. Filiz] Erciyes Univ, Dept Astron & Space Sci, Fac Sci, TR-38039 Kayseri, Turkey. [Hall, P. B.] York Univ, Dept Phys & Astron, N York, ON M3J 1P3, Canada. [Anderson, S. F.] Univ Washington, Dept Astron, Seattle, WA 98195 USA. [Hamann, F.] Univ Florida, Dept Astron, Gainesville, FL 32611 USA. [Myers, Adam D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [Paris, I.] Univ Chile, Dept Astron, Santiago, Chile. [Petitjean, P.] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Ross, Nicholas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ross, Nicholas P.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Shen, Yue] Carnegie Observ, Pasadena, CA 91101 USA. [York, Don] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [York, Don] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Ak, NF (reprint author), Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. EM nfilizak@astro.psu.edu RI Filiz Ak, Nurten/C-9686-2015; Brandt, William/N-2844-2015 OI Filiz Ak, Nurten/0000-0003-3016-5490; Brandt, William/0000-0002-0167-2453 FU National Science Foundation [AST-1108604]; NSERC; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science FX We gratefully acknowledge financial support from National Science Foundation grant AST-1108604 (N.F.A., W.N.B., D.P.S.) and from NSERC (P.B.H.). We thank N. Arav and M. Eracleous for helpful discussions. We thank D. Proga for allowing us to adapt Figure 2 of Proga et al. (2000) as our Figure 16. We also thank the anonymous referee for constructive feedback.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/. NR 58 TC 9 Z9 9 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2014 VL 791 IS 2 AR 88 DI 10.1088/0004-637X/791/2/88 PG 22 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM7EV UT WOS:000340028400015 ER PT J AU Arevalo, P Bauer, FE Puccetti, S Walton, DJ Koss, M Boggs, SE Brandt, WN Brightman, M Christensen, FE Comastri, A Craig, WW Fuerst, F Gandhi, P Grefenstette, BW Hailey, CJ Harrison, FA Luo, B Madejski, G Madsen, KK Marinucci, A Matt, G Saez, C Stern, D Stuhlinger, M Treister, E Urry, CM Zhang, WW AF Arevalo, P. Bauer, F. E. Puccetti, S. Walton, D. J. Koss, M. Boggs, S. E. Brandt, W. N. Brightman, M. Christensen, F. E. Comastri, A. Craig, W. W. Fuerst, F. Gandhi, P. Grefenstette, B. W. Hailey, C. J. Harrison, F. A. Luo, B. Madejski, G. Madsen, K. K. Marinucci, A. Matt, G. Saez, C. Stern, D. Stuhlinger, M. Treister, E. Urry, C. M. Zhang, W. W. TI THE 2-79 keV X-RAY SPECTRUM OF THE CIRCINUS GALAXY WITH NuSTAR, XMM-Newton, AND CHANDRA: A FULLY COMPTON-THICK ACTIVE GALACTIC NUCLEUS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: individual (Circinus); galaxies: Seyfert; X-rays: galaxies ID STAR-FORMATION RATE; SEYFERT-GALAXIES; NEARBY SEYFERT; RATE INDICATOR; LINE REGION; BEPPOSAX; VIEW; SPECTROSCOPY; ACCRETION; AGN AB The Circinus galaxy is one of the closest obscured active galactic nuclei (AGNs), making it an ideal target for detailed study. Combining archival Chandra and XMM-Newton data with new NuSTAR observations, we model the 2-79 keV spectrum to constrain the primary AGN continuum and to derive physical parameters for the obscuring material. Chandra's high angular resolution allows a separation of nuclear and off-nuclear galactic emission. In the off-nuclear diffuse emission, we find signatures of strong cold reflection, including high equivalent-width neutral Fe lines. This Compton-scattered off-nuclear emission amounts to 18% of the nuclear flux in the Fe line region, but becomes comparable to the nuclear emission above 30 keV. The new analysis no longer supports a prominent transmitted AGN component in the observed band. We find that the nuclear spectrum is consistent with Compton scattering by an optically thick torus, where the intrinsic spectrum is a power law of photon index Gamma = 2.2-2.4, the torus has an equatorial column density of N-H = (6-10) x 10(24) cm(-2), and the intrinsic AGN 2-10 keV luminosity is (2.3-5.1) x10(42) erg s(-1). These values place Circinus along the same relations as unobscured AGNs in accretion rate versus Gamma and L-X versus L-IR phase space. NuSTAR's high sensitivity and low background allow us to study the short timescale variability of Circinus at X-ray energies above 10 keV for the first time. The lack of detected variability favors a Compton-thick absorber, in line with the spectral fitting results. C1 [Arevalo, P.; Bauer, F. E.; Saez, C.] Pontificia Univ Catolica Chile, Fac Fis, Inst Astrofis, Santiago 22, Chile. [Arevalo, P.] Univ Valparaiso, Fac Ciencias, Inst Fis & Astron, Valparaiso, Chile. [Bauer, F. E.] Millennium Inst Astrophys, Boulder, CO 80301 USA. [Bauer, F. E.] Space Sci Inst, Boulder, CO 80301 USA. [Puccetti, S.] ASDC, ASI, I-00133 Rome, Italy. [Puccetti, S.] Osserv Astron Roma, INAF, I-00040 Monte Porzio Catone, RM, Italy. [Walton, D. J.; Fuerst, F.; Grefenstette, B. W.; Harrison, F. A.; Madsen, K. K.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Koss, M.] ETH, Inst Astron, Dept Phys, CH-8093 Zurich, Switzerland. [Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Brandt, W. N.; Luo, B.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Brandt, W. N.; Luo, B.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Brightman, M.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Christensen, F. E.] Danish Tech Univ, Lyngby, Denmark. [Comastri, A.] Osservatorio Astron Bologna, INAF, I-40127 Bologna, Italy. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Gandhi, P.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Hailey, C. J.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Madejski, G.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Marinucci, A.; Matt, G.] Univ Roma Tre, Dipartimento Matemat Fis, I-00146 Rome, Italy. [Saez, C.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Stuhlinger, M.] ESAC, E-28691 Madrid, Spain. [Treister, E.] Univ Concepcion, Dept Astron, Concepcion, Chile. [Urry, C. M.] Yale Univ, Yale Ctr Astron & Astrophys, Dept Phys, New Haven, CT 06520 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Arevalo, P (reprint author), Pontificia Univ Catolica Chile, Fac Fis, Inst Astrofis, Santiago 22, Chile. RI Boggs, Steven/E-4170-2015; Koss, Michael/B-1585-2015; Brandt, William/N-2844-2015; Comastri, Andrea/O-9543-2015; OI Boggs, Steven/0000-0001-9567-4224; Koss, Michael/0000-0002-7998-9581; Brandt, William/0000-0002-0167-2453; Comastri, Andrea/0000-0003-3451-9970; Puccetti, Simonetta/0000-0002-2734-7835; Urry, Meg/0000-0002-0745-9792 FU NASA [NNG08FD60C]; National Aeronautics and Space Administration; Basal-CATA [PFB-06/2007]; CONICYT-Chile FONDECYT [1140304, 1141218, 1120061, Anillo ACT1101]; ASI-INAF grant [I/037/12/0]; Caltech NuSTAR subcontract [44A-1092750]; NASA ADP grant [NNX10AC99G]; Swiss National Science Foundation [PP00P2_138979/1]; STFC [ST/J003697/1] FX We thank the anonymous referee for a thorough review and many useful suggestions that improved this paper. This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). We acknowledge financial support from Basal-CATA PFB-06/2007 (FEB), CONICYT-Chile FONDECYT 1140304 (PA), 1141218 (FEB), 1120061 (ET), and Anillo ACT1101 (PA, FEB, ET). A. C., A. M., and G. M. acknowledge the ASI-INAF grant I/037/12/0. W.N.B. and B. L. acknowledge support from Caltech NuSTAR subcontract 44A-1092750 and NASA ADP grant NNX10AC99G. M. K. gratefully acknowledges support from Swiss National Science Foundation Grant PP00P2_138979/1. P. G. thanks STFC for support (grant reference ST/J003697/1). NR 67 TC 38 Z9 38 U1 2 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2014 VL 791 IS 2 AR 81 DI 10.1088/0004-637X/791/2/81 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM7EV UT WOS:000340028400008 ER PT J AU Schlesinger, KJ Johnson, JA Rockosi, CM Lee, YS Beers, TC Harding, P Prieto, CA Bird, JC Schonrich, R Yanny, B Schneider, DP Weaver, BA Brinkmann, J AF Schlesinger, Katharine J. Johnson, Jennifer A. Rockosi, Constance M. Lee, Young Sun Beers, Timothy C. Harding, Paul Prieto, Carlos Allende Bird, Jonathan C. Schoenrich, Ralph Yanny, Brian Schneider, Donald P. Weaver, Benjamin A. Brinkmann, Jon TI THE VERTICAL METALLICITY GRADIENT OF THE MILKY WAY DISK: TRANSITIONS IN [alpha/Fe] POPULATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE Galaxy: disk; Galaxy: evolution; Galaxy: formation; Galaxy: structure; stars: abundances; surveys ID DIGITAL SKY SURVEY; GENEVA-COPENHAGEN SURVEY; 1ST SPECTROSCOPIC DATA; DARK-MATTER UNIVERSE; GALACTIC THICK DISK; G-DWARF PROBLEM; SOLAR NEIGHBORHOOD; CHEMICAL EVOLUTION; DATA RELEASE; DENSITY DISTRIBUTION AB Using G dwarfs from the Sloan Extension for Galactic Understanding and Exploration (SEGUE) survey, we have determined the vertical metallicity gradient in the Milky Way's disk and examined how this gradient varies for different [alpha/Fe] subsamples. Our sample contains over 40,000 stars with low-resolution spectroscopy over 144 lines of sight. It also covers a significant disk volume, between similar to 0.3 and 1.6 kpc from the Galactic plane, and allows us to examine the disk in situ, whereas previous analyses were more limited in scope. Furthermore, this work does not presuppose a disk structure, whether composed of a single complex population or distinct thin and thick disk components. We employ the SEGUE Stellar Parameter Pipeline to obtain estimates of stellar parameters, [Fe/H], and [alpha/Fe] and extract multiple volume-complete subsamples of approximately 1000 stars each. Based on SEGUE's target-selection algorithm, we adjust each subsample to determine an unbiased picture of disk chemistry; consequently, each individual star represents the properties of many. The metallicity gradient is -0.243(-0.053)(+0.039) dex kpc(-1) for the entire sample, which we compare to various literature results. This gradient stems from the different [alpha/Fe] populations inhabiting different ranges of height above the Galactic plane. Each [alpha/Fe] subsample shows little change in median [Fe/H] with height. If we associate [alpha/Fe] with age, the negligible gradients of our [alpha/Fe] subsamples suggest that stars formed in different epochs exhibit comparable vertical structure, implying similar star formation processes and evolution. C1 [Schlesinger, Katharine J.] Australian Natl Univ, Mt Stromlo Observ, Res Sch Astron & Astrophys, Weston, ACT 2611, Australia. [Johnson, Jennifer A.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Rockosi, Constance M.] Univ Calif Santa Cruz, UCO Lick Observ, Santa Cruz, CA 95064 USA. [Lee, Young Sun] New Mexico State Univ, Dept Astron, Las Cruces, NM 88003 USA. [Beers, Timothy C.] Natl Opt Astron Observ, Tucson, AZ 85737 USA. [Beers, Timothy C.] JINA, E Lansing, MI 48824 USA. [Harding, Paul] Case Western Reserve Univ, Dept Astron, Cleveland, OH 44106 USA. [Prieto, Carlos Allende] Inst Astrofis Canarias, E-38205 Tenerife, Spain. [Prieto, Carlos Allende] Univ La Laguna, Dept Astrofis, E-38206 Tenerife, Spain. [Bird, Jonathan C.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Schoenrich, Ralph] Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England. [Yanny, Brian] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Weaver, Benjamin A.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. [Brinkmann, Jon] Apache Point Observ, Sunspot, NM 88349 USA. RP Schlesinger, KJ (reprint author), Australian Natl Univ, Mt Stromlo Observ, Res Sch Astron & Astrophys, Weston, ACT 2611, Australia. FU NSF [AST-0807997]; Physics Frontiers Center/Joint Institute for Nuclear Astrophysics (JINA) - U.S. National Science Foundation [PHY 08-22648]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science FX We thank M. Hayden and J. Bovy for their helpful discussion on this work. We also thank the anonymous referee for their helpful comments. K.J.S. and J.A.J. acknowledge partial support from NSF grant AST-0807997. Y.S.L. and T.C.B. acknowledge partial support from grant PHY 08-22648: Physics Frontiers Center/Joint Institute for Nuclear Astrophysics (JINA), awarded by the U.S. National Science Foundation.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III Web site is http://www.sdss3.org/. NR 109 TC 11 Z9 11 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2014 VL 791 IS 2 AR 112 DI 10.1088/0004-637X/791/2/112 PG 23 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM7EV UT WOS:000340028400039 ER PT J AU Tendulkar, SP Yang, CW An, HJ Kaspi, VM Archibald, AM Bassa, C Bellm, E Bogdanov, S Harrison, FA Hessels, JWT Janssen, GH Lyne, AG Patruno, A Stappers, B Stern, D Tomsick, JA Boggs, SE Chakrabarty, D Christensen, FE Craig, WW Hailey, CA Zhang, W AF Tendulkar, Shriharsh P. Yang, Chengwei An, Hongjun Kaspi, Victoria M. Archibald, Anne M. Bassa, Cees Bellm, Eric Bogdanov, Slavko Harrison, Fiona A. Hessels, Jason W. T. Janssen, Gemma H. Lyne, Andrew G. Patruno, Alessandro Stappers, Benjamin Stern, Daniel Tomsick, John A. Boggs, Steven E. Chakrabarty, Deepto Christensen, Finn E. Craig, William W. Hailey, Charles A. Zhang, William TI NuSTAR OBSERVATIONS OF THE STATE TRANSITION OF MILLISECOND PULSAR BINARY PSR J1023+0038 SO ASTROPHYSICAL JOURNAL LA English DT Article DE pulsars: general; pulsars: individual (PSR J1023+0038); stars: neutron; X-rays: stars ID X-RAY BINARY; QUASI-PERIODIC OSCILLATIONS; 1ST J102347.6+003841; ACCRETION POWER; XSS J12270-4859; RADIO PULSARS; SPIN-DOWN; SYSTEM; EMISSION; ROTATION AB We report NuSTAR observations of the millisecond pulsar-low-mass X-ray binary (LMXB) transition system PSR J1023+0038 from 2013 June and October, before and after the formation of an accretion disk around the neutron star. Between June 10 and 12, a few days to two weeks before the radio disappearance of the pulsar, the 3-79 keV X-ray spectrum was well fit by a simple power law with a photon index of Gamma = 1.17(-0.07)(+0.08) (at 90% confidence) with a 3-79 keV luminosity of 7.4 +/- 0.4 x 10(32) erg s(-1). Significant orbital modulation was observed with a modulation fraction of 36% +/- 10%. During the October 19-21 observation, the spectrum is described by a softer power law (Gamma = 1.66(-0.05)(+0.06)) with an average luminosity of 5.8 +/- 0.2x10(33) erg s(-1) and a peak luminosity of approximate to 1.2x10(34) erg s(-1) observed during a flare. No significant orbital modulation was detected. The spectral observations are consistent with previous and current multiwavelength observations and show the hard X-ray power law extending to 79 keV without a spectral break. Sharp-edged, flat-bottomed dips are observed with widths between 30 and 1000 s and ingress and egress timescales of 30-60 s. No change in hardness ratio was observed during the dips. Consecutive dip separations are log-normal in distribution with a typical separation of approximately 400 s. These dips are distinct from dipping activity observed in LMXBs. We compare and contrast these dips to observations of dips and state changes in the similar transition systems PSR J1824-2452I and XSS J1227.0-4859 and discuss possible interpretations based on the transitions in the inner disk. C1 [Tendulkar, Shriharsh P.; Bellm, Eric; Harrison, Fiona A.] CALTECH, Pasadena, CA 91125 USA. [Yang, Chengwei; An, Hongjun; Kaspi, Victoria M.] McGill Univ, Dept Phys, Montreal II3A 2T8, PQ, Canada. [Yang, Chengwei] Chinese Acad Sci, Natl Space Sci Ctr, Beijing 100190, Peoples R China. [Archibald, Anne M.; Bassa, Cees; Hessels, Jason W. T.; Janssen, Gemma H.; Patruno, Alessandro] ASTRON, Netherlands Inst Radio Astron, NL-7990 AA Dwingeloo, Netherlands. [Bogdanov, Slavko; Hailey, Charles A.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Hessels, Jason W. T.] Univ Amsterdam, Astron Inst Anton Pannekoek, NL-1090 GE Amsterdam, Netherlands. [Lyne, Andrew G.; Stappers, Benjamin] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Manchester M13 9PL, Lancs, England. [Patruno, Alessandro] Leiden Univ, Leiden Observ, NL-2300 RA Leiden, Netherlands. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Tomsick, John A.; Boggs, Steven E.; Craig, William W.] Univ Calif, Space Sci Lab, Berkeley, CA 94720 USA. [Chakrabarty, Deepto] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Christensen, Finn E.] Tech Univ Denmark, DTU Space, Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Zhang, William] NASA Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. RP Tendulkar, SP (reprint author), CALTECH, 1200 E Calif Blvd,MC 249-17, Pasadena, CA 91125 USA. EM spt@astro.caltech.edu RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bellm, Eric/0000-0001-8018-5348; An, Hongjun/0000-0002-6389-9012; Archibald, Anne/0000-0003-0638-3340 FU NASA [NNG08FD60C]; NuSTAR mission; California Institute of Technology; National Aeronautics and Space Administration; NSERC Discovery Grant; Centre de Recherche en Astrophysique du Quebec, an R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Study; Canada Research Chairs Program; Lorne Trottier Chair in Astrophysics and Cosmology; ERC starting grant DRAGNET; Netherlands Organization for Scientic Research (NWO) Vidi fellowship FX We thank the anonymous referee for detailed suggestions and comments. This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). VMKreceives support from an NSERC Discovery Grant and Accelerator Supplement, from the Centre de Recherche en Astrophysique du Quebec, an R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Study, the Canada Research Chairs Program, and the Lorne Trottier Chair in Astrophysics and Cosmology. J. W. T. H. acknowledges funding for this work from ERC starting grant DRAGNET. A. P. acknowledges support from the Netherlands Organization for Scientic Research (NWO) Vidi fellowship. NR 52 TC 20 Z9 20 U1 1 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2014 VL 791 IS 2 AR 77 DI 10.1088/0004-637X/791/2/77 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AM7EV UT WOS:000340028400004 ER PT J AU Owen, JM AF Owen, J. Michael TI A compatibly differenced total energy conserving form of SPH SO INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN FLUIDS LA English DT Article DE smoothed particle hydrodynamics; meshless methods; energy conservation; compatible discretization ID SMOOTHED PARTICLE HYDRODYNAMICS; ARTIFICIAL VISCOSITY; SIMULATIONS; MAGNETOHYDRODYNAMICS; CONSERVATION; ALGORITHMS; IMPACTS AB describe a modified form of smoothed particle hydrodynamics (SPH) in which the specific thermal energy equation is based on a compatibly differenced formalism, guaranteeing exact conservation of the total energy. We compare the errors and convergence rates of the standard and compatible SPH formalisms on a variety of shock test problems with analytic answers. We find that the new compatible formalism reliably achieves the expected first-order convergence for these analytic shock tests and, in all cases, improves the accuracy of the numerical solution over the standard formalism. We also examine the performance of our new formalism on a more complicated applied problem: the diversion of an asteroid by a kinetic impactor. We find the compatible discretization demonstrates measurable improvement in the convergence of properties such as the deflection velocity in this kind of applied problem as well. Copyright (C) 2014 John Wiley & Sons, Ltd. C1 Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Owen, JM (reprint author), Lawrence Livermore Natl Lab, M-S L-38, Livermore, CA 94550 USA. EM mikeowen@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [W-7405-Eng-48, DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [12-ERD-005] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory in part under Contract W-7405-Eng-48 and in part under Contract DE-AC52-07NA27344. We also acknowledge funding by the Laboratory Directed Research and Development Program at LLNL under tracking code 12-ERD-005. NR 36 TC 9 Z9 9 U1 5 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0271-2091 EI 1097-0363 J9 INT J NUMER METH FL JI Int. J. Numer. Methods Fluids PD AUG 20 PY 2014 VL 75 IS 11 BP 749 EP 774 DI 10.1002/fld.3912 PG 26 WC Computer Science, Interdisciplinary Applications; Mathematics, Interdisciplinary Applications; Mechanics; Physics, Fluids & Plasmas SC Computer Science; Mathematics; Mechanics; Physics GA AL8XF UT WOS:000339422400001 ER PT J AU Lim, YW Cuevas, DA Silva, GGZ Aguinaldo, K Dinsdale, EA Haas, AF Hatay, M Sanchez, SE Wegley-Kelly, L Dutilh, BE Harkins, TT Lee, CC Tom, W Sandin, SA Smith, JE Zgliczynski, B Vermeij, MJA Rohwer, F Edwards, RA AF Lim, Yan Wei Cuevas, Daniel A. Silva, Genivaldo Gueiros Z. Aguinaldo, Kristen Dinsdale, Elizabeth A. Haas, Andreas F. Hatay, Mark Sanchez, Savannah E. Wegley-Kelly, Linda Dutilh, Bas E. Harkins, Timothy T. Lee, Clarence C. Tom, Warren Sandin, Stuart A. Smith, Jennifer E. Zgliczynski, Brian Vermeij, Mark J. A. Rohwer, Forest Edwards, Robert A. TI Sequencing at sea: challenges and experiences in Ion Torrent PGM sequencing during the 2013 Southern Line Islands Research Expedition SO PEERJ LA English DT Article DE Genomics; Sequencing; Expeditions; Metagenomics; Environmental microbiology; Coral reef; Vibrio ID SP-NOV.; GENOME; GENES; METAGENOMICS; GENERATION; IRON AB Genomics and metagenomics have revolutionized our understanding of marine microbial ecology and the importance of microbes in global geochemical cycles. However, the process of DNA sequencing has always been an abstract extension of the research expedition, completed once the samples were returned to the laboratory. During the 2013 Southern Line Islands Research Expedition, we started the first effort to bring next generation sequencing to some of the most remote locations on our planet. We successfully sequenced twenty six marine microbial genomes, and two marine microbial metagenomes using the Ion Torrent PGM platform on the Merchant Yacht Hanse Explorer. Onboard sequence assembly, annotation, and analysis enabled us to investigate the role of the microbes in the coral reef ecology of these islands and atolls. This analysis identified phosphonate as an important phosphorous source for microbes growing in the Line Islands and reinforced the importance of L-serine in marine microbial ecosystems. Sequencing in the field allowed us to propose hypotheses and conduct experiments and further sampling based on the sequences generated. By eliminating the delay between sampling and sequencing, we enhanced the productivity of the research expedition. By overcoming the hurdles associated with sequencing on a boat in the middle of the Pacific Ocean we proved the flexibility of the sequencing, annotation, and analysis pipelines. C1 [Lim, Yan Wei; Aguinaldo, Kristen; Dinsdale, Elizabeth A.; Haas, Andreas F.; Hatay, Mark; Sanchez, Savannah E.; Wegley-Kelly, Linda; Rohwer, Forest; Edwards, Robert A.] San Diego State Univ, Dept Biol, San Diego, CA 92182 USA. [Cuevas, Daniel A.; Silva, Genivaldo Gueiros Z.] San Diego State Univ, Computat Sci Res Ctr, San Diego, CA 92182 USA. [Aguinaldo, Kristen] Thermo Fisher Sci, Ion Torrent Res & Dev Grp, Carlsbad, CA USA. [Dutilh, Bas E.] Radboud Univ Nijmegen Med Ctr, Radboud Inst Mol Life Sci, Ctr Mol & Biomol Informat, Nijmegen, Netherlands. [Dutilh, Bas E.; Edwards, Robert A.] Univ Fed Rio de Janeiro, Inst Biol, Dept Marine Biol, BR-21941 Rio De Janeiro, Brazil. [Harkins, Timothy T.; Lee, Clarence C.; Tom, Warren] Life Technol Inc, Adv Applicat Grp, Beverly, MA USA. [Lee, Clarence C.] Thermo Fisher Sci, Life Sci Grp, San Francisco, CA USA. [Sandin, Stuart A.; Smith, Jennifer E.; Zgliczynski, Brian] Univ Calif San Diego, Scripps Inst Oceanog, Ctr Marine Biodivers & Conservat, La Jolla, CA 92093 USA. [Vermeij, Mark J. A.] Caribbean Res & Management Biodivers CARMABI, Willemstad, Curacao, Neth Antilles. [Vermeij, Mark J. A.] Univ Amsterdam, Inst Biodivers & Ecosyst Dynam, Amsterdam, Netherlands. [Edwards, Robert A.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Edwards, RA (reprint author), San Diego State Univ, Dept Biol, San Diego, CA 92182 USA. EM raedwards@gmail.com RI Dutilh, Bas/B-9719-2011 OI Dutilh, Bas/0000-0003-2329-7890 FU NSF [DEB-1046413, CNS-1305112, MCB-1330800]; Gordon and Betty Moore Foundation [GBMF-3781]; Canadian Institute for Advanced Research (CIFAR) [IMB-ROHW-141679]; CAPES/BRASIL FX This work is partially supported by NSF Dimensions Grant (DEB-1046413; Edwards and Rohwer). This project was also funded in part by the Gordon and Betty Moore Foundation through Grant GBMF-3781 to Rohwer. Additional funding for Yan Wei Lim was provided by the Canadian Institute for Advanced Research (CIFAR; IMB-ROHW-141679). Additional funding for Edwards was provided by NSF grants CNS-1305112, and MCB-1330800. Dutilh was supported by an award from CAPES/BRASIL. The SDSU Vice President of Research, Director's Office of Scripps Institution of Oceanography, Moore Family Foundation, and several private donors provided cruise support. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 44 TC 1 Z9 1 U1 0 U2 15 PU PEERJ INC PI LONDON PA 341-345 OLD ST, THIRD FLR, LONDON, EC1V 9LL, ENGLAND SN 2167-8359 J9 PEERJ JI PeerJ PD AUG 19 PY 2014 VL 2 AR e520 DI 10.7717/peerj.520 PG 23 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY5MY UT WOS:000347617700004 PM 25177534 ER PT J AU Madeo, D Comolli, LR Mocenni, C AF Madeo, Dario Comolli, Luis R. Mocenni, Chiara TI Emergence of microbial networks as response to hostile environments SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE microbial communities; bacterial social networks; evolutionary games; graph theory; evolutive decisions; hostile environmental conditions ID EVOLUTION; COMMUNITY; BACTERIA; BIOFILMS; PHYLA AB The majority of microorganisms live in complex communities under varying conditions. One pivotal question in evolutionary biology is the emergence of cooperative traits and their sustainment in altered environments or in the presence of free-riders. Co-occurrence patterns in the spatial distribution of biofilms can help define species' identities, and systems biology tools are revealing networks of interacting microorganisms. However, networks of inter-dependencies involving micro-organisms in the planktonic phase may be just as important, with the added complexity that they are not bounded in space. An integrated approach linking imaging, "Omics" and modeling has the potential to enable new hypothesis and working models. In order to understand how cooperation can emerge and be maintained without abilities like memory or recognition we use evolutionary game theory as the natural framework to model cell-cell interactions arising from evolutive decisions. We consider a finite population distributed in a spatial domain (biofilm), and divided into two interacting classes with different traits. This interaction can be weighted by distance, and produces physical connections between two elements allowing them to exchange finite amounts of energy and matter. Available strategies to each individual of one class in the population are the propensities or "willingness" to connect any individual of the other class. Following evolutionary game theory, we propose a mathematical model which explains the patterns of connections which emerge when individuals are able to find connection strategies that asymptotically optimize their fitness. The process explains the formation of a network for efficiently exchanging energy and matter among individuals and thus ensuring their survival in hostile environments. C1 [Madeo, Dario; Mocenni, Chiara] Univ Siena, Dept Informat Engn & Math, I-53100 Siena, Italy. [Comolli, Luis R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Struct & Imaging Dept, Div Life Sci, Berkeley, CA 94720 USA. RP Mocenni, C (reprint author), Univ Siena, Dept Informat Engn & Math, Via Roma 56, I-53100 Siena, Italy. EM mocenni@dii.unisi.it FU project "Evolutionary Games on Networks for Modeling Complex Biological and Socio-Economic Phenomena" - CNPq [401795/2013-6] FX The study is partially funded by the project "Evolutionary Games on Networks for Modeling Complex Biological and Socio-Economic Phenomena" financed by CNPq (Program Science without Borders, N. 401795/2013-6). NR 20 TC 4 Z9 4 U1 1 U2 28 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 19 PY 2014 VL 5 AR 407 DI 10.3389/fmicb.2014.00407 PG 13 WC Microbiology SC Microbiology GA AO7VF UT WOS:000341560000001 PM 25191306 ER PT J AU Dettman, JR Cassabaum, AA Saunders, CP Snyder, DL Buscaglia, J AF Dettman, Joshua R. Cassabaum, Alyssa A. Saunders, Christopher P. Snyder, Deanna L. Buscaglia, JoAnn TI Forensic Discrimination of Copper Wire Using Trace Element Concentrations SO ANALYTICAL CHEMISTRY LA English DT Article ID INDUCTIVELY-COUPLED PLASMA; X-RAY-FLUORESCENCE; MASS-SPECTROMETRY; ICP-MS AB Copper may be recovered as evidence in high-profile cases such as thefts and improvised explosive device incidents; comparison of copper samples from the crime scene and those associated with the subject of an investigation can provide probative associative evidence and investigative support. A solution-based inductively coupled plasma mass spectrometry method for measuring trace element concentrations in high-purity copper was developed using standard reference materials. The method was evaluated for its ability to use trace element profiles to statistically discriminate between copper samples considering the precision of the measurement and manufacturing processes. The discriminating power was estimated by comparing samples chosen on the basis of the copper refining and production process to represent the within-source (samples expected to be similar) and between-source (samples expected to be different) variability using multivariate parametric- and empirical-based data simulation models with bootstrap resampling. If the false exclusion rate is set to 5%, >90% of the copper samples can be correctly determined to originate from different sources using a parametric-based model and >87% with an empirical-based approach. These results demonstrate the potential utility of the developed method for the comparison of copper samples encountered as forensic evidence. C1 [Dettman, Joshua R.; Cassabaum, Alyssa A.; Saunders, Christopher P.; Snyder, Deanna L.] Fed Bur Invest, Oak Ridge Inst Sci & Educ, Lab Div, Quantico, VA 22135 USA. [Saunders, Christopher P.] S Dakota State Univ, Dept Math & Stat, Brookings, SD 57007 USA. [Buscaglia, JoAnn] Fed Bur Invest, Lab Div, Counterterrorism & Forens Sci Res Unit, Quantico, VA 22135 USA. RP Buscaglia, J (reprint author), Fed Bur Invest, Lab Div, Counterterrorism & Forens Sci Res Unit, 2501 Invest Pkwy, Quantico, VA 22135 USA. EM joann.buscaglia@ic.fbi.gov NR 39 TC 1 Z9 1 U1 3 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD AUG 19 PY 2014 VL 86 IS 16 BP 8176 EP 8182 DI 10.1021/ac5013514 PG 7 WC Chemistry, Analytical SC Chemistry GA AN6JT UT WOS:000340701500023 PM 25007219 ER PT J AU Wen, B Peng, JH Zuo, XB Gong, QG Zhang, ZY AF Wen, Bin Peng, Junhui Zuo, Xiaobing Gong, Qingguo Zhang, Zhiyong TI Characterization of Protein Flexibility Using Small-Angle X-Ray Scattering and Amplified Collective Motion Simulations SO BIOPHYSICAL JOURNAL LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; ENERGY LANDSCAPE PERSPECTIVE; COARSE-GRAINED SIMULATIONS; NORMAL-MODE ANALYSIS; STRUCTURAL BIOLOGY; REPLICA-EXCHANGE; PROGRAM PACKAGE; T4 LYSOZYME; COMPLEXES; BIOMOLECULES AB Large-scale flexibility within a multidomain protein often plays an important role in its biological function.. Despite its inherent low resolution, small-angle x-ray scattering (SAXS) is well suited to investigate protein flexibility and determine, with the help of computational modeling, what kinds of protein conformations would coexist in solution. In this article, we develop a tool that combines SAXS data with a previously developed sampling technique called amplified collective motions (ACM) to elucidate structures of highly dynamic multidomain proteins in solution. We demonstrate the use of this tool in two proteins, bacteriophage T4 lysozyme and tandem WW domains of the formin-binding protein 21. The ACM simulations can sample the conformational space of proteins much more extensively than standard molecular dynamics (MD) simulations. Therefore, conformations generated by ACM are significantly better at reproducing the SAXS data than are those from MD simulations. C1 [Wen, Bin; Peng, Junhui; Gong, Qingguo; Zhang, Zhiyong] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Wen, Bin; Peng, Junhui; Gong, Qingguo; Zhang, Zhiyong] Univ Sci & Technol China, Sch Life Sci, Hefei 230026, Anhui, Peoples R China. [Zuo, Xiaobing] Argonne Natl Lab, Adv Photon Source, Chicago, IL USA. RP Zhang, ZY (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. EM zzyzhang@ustc.edu.cn OI Zuo, Xiaobing/0000-0002-0134-4804 FU National Key Basic Research Program of China [2013CB910203, 2011CB911104]; National Natural Science Foundation of China [31270760]; Strategic Priority Research Program of the Chinese Academy of Sciences [XDB08030102]; Specialized Research Fund for the Doctoral Program of Higher Education [20113402120013]; Anhui Natural Science Foundation [1208085MC38]; Fundamental Research Funds for the Central Universities [WK2070000020] FX This work is supported by the National Key Basic Research Program of China (grants 2013CB910203 and 2011CB911104), the National Natural Science Foundation of China (grant 31270760), the Strategic Priority Research Program of the Chinese Academy of Sciences (grant XDB08030102), the Specialized Research Fund for the Doctoral Program of Higher Education (grant 20113402120013), Anhui Natural Science Foundation (grant 1208085MC38), and the Fundamental Research Funds for the Central Universities (WK2070000020). NR 59 TC 5 Z9 6 U1 0 U2 19 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD AUG 19 PY 2014 VL 107 IS 4 BP 956 EP 964 DI 10.1016/j.bpj.2014.07.005 PG 9 WC Biophysics SC Biophysics GA AN4SF UT WOS:000340578100020 PM 25140431 ER PT J AU De Santiago, A Longo, AF Ingall, ED Diaz, JM King, LE Lai, B Weber, RJ Russell, AG Oakes, M AF De Santiago, Arlette Longo, Amelia F. Ingall, Ellery D. Diaz, Julia M. King, Laura E. Lai, Barry Weber, Rodney J. Russell, Armistead G. Oakes, Michelle TI Characterization of Selenium in Ambient Aerosols and Primary Emission Sources SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID FLY-ASH; ATMOSPHERIC SELENIUM; IRON SOLUBILITY; TRACE-ELEMENTS; SPECIATION; SPECTROSCOPY; PARTICLES; IDENTIFICATION; COMBUSTION; BARBADOS AB Atmospheric selenium (Se) in aerosols was investigated using X-ray absorption near-edge structure (XANES) spectroscopy and X-ray fluorescence (XRF) microscopy. These techniques were used to determine the oxidation state and elemental associations of Se in common primary emission sources and ambient aerosols collected from the greater Atlanta area. In the majority of ambient aerosol and primary emission source samples, the spectroscopic patterns as well as the absence of elemental correlations suggest Se is in an elemental, organic, or oxide form. XRF microscopy revealed numerous Se-rich particles, or hotspots, accounting on average for,similar to 16% of the total Se in ambient aerosols. Hotspots contained primarily Se-0/Se(-II). However, larger, bulk spectroscopic characterizations revealed Se(IV) as the dominant oxidation state in ambient aerosol, followed by Se-0/Se(-II) and Se(VI). Se(IV) was the only observed oxidation state in gasoline, diesel, and coal fly ash, while biomass burning contained a combination of Se-0/Se(-II) and Se(IV). Although the majority of Se in aerosols was in the most toxic form, the Se concentration is well below the California Environmental Protection Agency chronic exposure limit (similar to 20000 ng/m(3)). C1 [De Santiago, Arlette; Longo, Amelia F.; Ingall, Ellery D.; King, Laura E.; Weber, Rodney J.; Oakes, Michelle] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Diaz, Julia M.] Woods Hole Oceanog Inst, Dept Biol, Woods Hole, MA 02543 USA. [Lai, Barry] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Russell, Armistead G.] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA. RP Ingall, ED (reprint author), Georgia Inst Technol, Sch Earth & Atmospher Sci, 311 Ferst Dr, Atlanta, GA 30332 USA. EM ingall@eas.gatech.edu RI Ingall, Ellery/A-5447-2008 OI Ingall, Ellery/0000-0003-1954-0317 FU National Science Foundation [OCE 1060884, OCE 1357375]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This material is based upon work supported by the National Science Foundation under Grant Nos. OCE 1060884 and OCE 1357375. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation. Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. We thank John Jansen at Southern Co. and Bill Preston at the EPA for providing primary emission source samples. NR 46 TC 5 Z9 5 U1 4 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 8988 EP 8994 DI 10.1021/es500379y PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800008 PM 25075640 ER PT J AU Callagon, E Fenter, P Nagy, KL Sturchio, NC AF Callagon, Erika Fenter, Paul Nagy, Kathryn L. Sturchio, Neil C. TI Incorporation of Pb at the Calcite (104)-Water Interface SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID X-RAY REFLECTIVITY; SOLID-SOLUTION FORMATION; WATER INTERFACE; ADSORPTION COMPLEXES; ABSORPTION SPECTROSCOPY; SORPTION PROCESSES; AQUEOUS-SOLUTIONS; DIVALENT METALS; TRACE-ELEMENTS; IN-SITU AB Lead (Pb) is a common environmental pollutant, and its transport in surface waters and groundwater is controlled in part by sorption and precipitation reactions at mineral surfaces. Using in situ specular and resonant anomalous X-ray reflectivity measurements, we investigated the interaction of the calcite (104) surface with a dilute Pb- and EDTA-bearing solution that is slightly undersaturated with respect to calcite. The X-ray results reveal Pb coherently substituting for Ca in the near-surface layers of strained calcite with Pb/(Pb + Ca) atom fractions as high as 0.28 in the outermost layer. The larger ionic radius of Pb2+ relative to Ca2+ is accommodated in calcite by vertical displacements of Pb relative to the Ca site. In situ atomic force microscopy images obtained during the reaction suggest that Pb incorporation below the surface occurs after initial dissolution followed by regrowth of a strained epitaadal Pb-rich calcite solid-solution at the calcite (104)-water interface. This process could produce a widespread host phase for Pb in groundwater aquifers and soil pore fluids. C1 [Callagon, Erika; Nagy, Kathryn L.; Sturchio, Neil C.] Univ Illinois, Dept Earth & Environm Sci, Chicago, IL 60607 USA. [Fenter, Paul] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Fenter, P (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM fenter@anl.gov FU Geosciences Research Program of the Office of Basic Energy Sciences, U.S. Department of Energy (DOE) [DE-AC02-06CH11357, DE-FG02-03ER15381]; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX This work was supported by the Geosciences Research Program of the Office of Basic Energy Sciences, U.S. Department of Energy (DOE), through contract number DE-AC02-06CH11357 at Argonne National Laboratory and DE-FG02-03ER15381 at UIC. The X-ray data were collected at the X-ray Operations and Research beamline 6-ID-B at the Advanced Photon Source (APS), Argonne National Laboratory. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under contract number DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 42 TC 6 Z9 6 U1 5 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 9263 EP 9269 DI 10.1021/es5014888 PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800040 PM 25007415 ER PT J AU Chang, HS Buettner, SW Seaman, JC Jaffe, PR van Groos, PGK Li, D Peacock, AD Scheckel, KG Kaplan, DI AF Chang, Hyun-shik Buettner, Shea W. Seaman, John C. Jaffe, Peter R. van Groos, Paul G. Koster Li, Dien Peacock, Aaron D. Scheckel, Kirk G. Kaplan, Daniel I. TI Uranium Immobilization in an Iron-Rich Rhizosphere of a Native Wetland Plant from the Savannah River Site under Reducing Conditions SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; CONTAMINATED AQUIFER; MICROBIAL REDUCTION; CHEMICAL SPECIATION; ASTER-TRIPOLIUM; ORYZA-SATIVA; FERRIC-OXIDE; ROOT PLAQUE; FE-PLAQUE; SEDIMENTS AB The hypothesis of this study was that iron plaques formed on the roots of wetland plants and their rhizospheres create environmental conditions favorable for iron reducing bacteria that promote the in situ immobilization of uranium. Greenhouse microcosm studies were conducted using native plants (Sparganium americanum) from a wetland located on the Savannah River Site, Aiken, SC. After iron plaques were established during a 73-day period by using an anoxic Fe(II)-rich nutrient solution, a U(VI) amended nutrient solution was added to the system for an additional two months. Compared to plant-free control microcosms, microcosms containing iron plaques successfully stimulated the growth of targeted iron reducing bacteria, Geobacter spp. Their population continuously increased after the introduction of the U(VI) nutrient solution. The reduction of some of the U(VI) to U(IV) by iron reducing bacteria was deduced based on the observations that the aqueous Fe(II) concentrations increased while the U(VI) concentrations decreased. The Fe(II) produced by the iron reducing bacteria was assumed to be recoddized by the oxygen released from the roots. Advanced spectroscopic analyses revealed that a significant fraction of the U(VI) had been reduced to U(IV) and they were commonly deposited in association with phosphorus on the iron plaque. C1 [Chang, Hyun-shik; Buettner, Shea W.; Seaman, John C.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Jaffe, Peter R.; van Groos, Paul G. Koster] Princeton Univ, Princeton, NJ 08540 USA. [Li, Dien; Kaplan, Daniel I.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Peacock, Aaron D.] Microbial Insights Inc, Rockford, TN 37853 USA. [Scheckel, Kirk G.] US EPA, Cincinnati, OH 45268 USA. RP Kaplan, DI (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA. EM daniel.kaplan@srnl.doe.gov RI Li, Dien/N-6370-2014; OI Scheckel, Kirk/0000-0001-9326-9241 FU Subsurface Biogeochemistry Research Program, within the Climate and Environmental Sciences Division in the Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy [Dr-FG02-08ER64567, ER65222-1038426-0017532]; Department of Energy [DEFC09-07-SR22506]; University of Georgia Research Foundation [DEFC09-07-SR22506]; Natural Sciences and Engineering Research Council of Canada; National Research Council Canada; Canadian Institutes of Health Research; Province of Saskatchewan, Western Economic Diversification Canada; University of Saskatchewan FX This work was supported by Subsurface Biogeochemistry Research Program, within the Climate and Environmental Sciences Division in the Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy, Grants Dr-FG02-08ER64567 and ER65222-1038426-0017532. Portions of this research were supported through a Cooperative Agreement (DEFC09-07-SR22506) between the Department of Energy and the University of Georgia Research Foundation. Although EPA contributed to this article, the research presented was not performed or funded by EPA and was not subject to EPA's quality system requirements. Consequently, the views, interpretations, and conclusions expressed in this article are solely those of the authors and do not necessarily reflect or represent EPA's views or policies. SEM-BSE-EDS images were obtained at the Department of Geology, University of Georgia. The XANES measurements were performed at the Canadian Light Source, supported by the Natural Sciences and Engineering Research Council of Canada, the National Research Council Canada, the Canadian Institutes of Health Research, the Province of Saskatchewan, Western Economic Diversification Canada, and the University of Saskatchewan. NR 62 TC 9 Z9 10 U1 7 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 9270 EP 9278 DI 10.1021/es5015136 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800041 PM 25051143 ER PT J AU Lee, N Sverjensky, DA Hazen, RM AF Lee, Namhey Sverjensky, Dimitri A. Hazen, Robert M. TI Cooperative and Competitive Adsorption of Amino Acids with Ca2+ on Rutile (alpha-TiO2) SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID METAL (HYDR)OXIDE/WATER INTERFACE; SURFACE COMPLEXATION; MINERAL SURFACES; AQUEOUS-SOLUTION; SALT-SOLUTIONS; TIO2; LYSINE; PREDICTION; GOETHITE; EXCHANGE AB The interactions of biomolecules such as amino acids with mineral surfaces in the near-surface environment are an important part of the short and long-term carbon cycles. Amino acid-mineral surface interactions also play an important role in biomineralization, biomedicine, and in assembling the building blocks of life in the prebiotic era. Although the pH effects during adsorption of amino adds onto mineral surfaces have been studied, little is known about the effects of environmentally important divalent cations. In this study, we investigated the adsorption of the oppositely charged amino acids glutamate and lysine with and without the addition of divalent calcium. Without calcium, glutamate shows a maximum in adsorption at a pH of similar to 4 and lysine shows a maximum in adsorption at a pH of similar to 9.4. In comparison, with calcium present, glutamate showed maxima in adsorption at both low and high pH, whereas lysine showed no adsorption at all. These dramatic effects can be described as cooperative adsorption between glutamate and Ca2+ and as competitive adsorption between lysine and Ca2+. The origin of these effects can be attributed to electrostatic phenomena. Adsorption of Ca2+ at high pH makes the rutile surface more positive, which attracts glutamate and repels lysine. Our results indicate that the interactions of biomolecules with mineral surfaces in the environment will be strongly affected by the major dissolved species in natural waters. C1 [Lee, Namhey; Sverjensky, Dimitri A.] Johns Hopkins Univ, Dept Earth & Planetary Sci, Baltimore, MD 21218 USA. [Lee, Namhey; Sverjensky, Dimitri A.; Hazen, Robert M.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. RP Lee, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM namheyl@jhu.edu RI Sverjensky, Dimitri/A-4612-2017 FU NSF [EAR-1023865, EAR-1023889]; DOE [DE-FG02-96ER-14616]; NASA Astrobiology Institute; Carnegie Institution of Washington FX We are extremely grateful for the specially cleaned rutile powder sample provided to them by J. Rosenqvist and D. Wesolowski of Oak Ridge National Laboratory, as well as M. Machesky. We greatly appreciate discussion with and assistance in the laboratory from C. M. Jonsson, C. L. Jonsson, C. F. Estrada, and C. Feuillie. N.L. and D.A.S. greatly appreciate the support of R. J. Hemley during their stay as visiting researchers at the Geophysical Laboratory. This research was conducted with support from the NSF EAR-1023865 (DAS), DOE DE-FG02-96ER-14616 (DAS), NSF EAR-1023889 (RMH), NASA Astrobiology Institute, and the Carnegie Institution of Washington. NR 35 TC 7 Z9 7 U1 4 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 9358 EP 9365 DI 10.1021/es501980y PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800051 PM 25008162 ER PT J AU Choung, S Kim, M Yang, JS Kim, MG Um, W AF Choung, Sungwook Kim, Minkyung Yang, Jung-Seok Kim, Min-Gyu Um, Wooyong TI Effects of Radiation and Temperature on Iodide Sorption by Surfactant-Modified Bentonite SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SAVANNA RIVER SITE; NATURAL ORGANIC-MATTER; RADIOIODINE I-129; MOLECULAR ENVIRONMENT; ADSORPTION; CLAY; ORGANOCLAYS; MINERALS; RADIONUCLIDES; SPECTROSCOPY AB Bentonite, which is used as an engineered barrier in geological repositories, is ineffective for sorbing anionic radionuclides because of its negatively charged surface. This study modified raw bentonite using a cationic surfactant (i.e., hexadecyltrimethylammonium [HDTMA]-Br) to improve its sorption capability for radioactive iodide. The effects of temperature and radiation on the iodide sorption of surfactant-modified bentonite (SMB) were also evaluated under alkaline pH condition similar to that found in repository environments. Different amounts of surfactant, equivalent to the SO, 100, and 200% cation-exchange capacity of the bentonite, were used to produce the HDTMA-SMB for iodide sorption. The sorption reaction of the SMB with iodide reached equilibrium rapidly within 10 min regardless of temperature and radiation conditions. The rate of iodide sorption increased as the amount of the added surfactant was increased and nonlinear sorption behavior was exhibited. However, high temperature and gamma-irradiation (Co-60) resulted in significantly (similar to 2-10 times) lower iodide K-d values for the SMB. The results of FTIR, NMR, and XANES spectroscopy analysis suggested that the decrease in iodide sorption may be caused by weakened physical electrostatic force between the HDTMA and iodide, and by the surfactant becoming detached from the SMB during the heating and irradiation processes. C1 [Choung, Sungwook; Kim, Minkyung; Um, Wooyong] Pohang Univ Sci & Technol POSTECH, Div Adv Nucl Engn, Pohang 790784, South Korea. [Yang, Jung-Seok] KIST, Environm Res Grp, Kangnung 210340, South Korea. [Kim, Min-Gyu] PAL, Pohang 790784, South Korea. [Um, Wooyong] PNNL, Energy & Environm Directorate, Richland, WA 99354 USA. RP Um, W (reprint author), Pohang Univ Sci & Technol POSTECH, Div Adv Nucl Engn, 77 Chongam Ro, Pohang 790784, South Korea. EM Wooyong.um@pnnl.gov RI Kim, Min-Gyu/D-8949-2013 OI Kim, Min-Gyu/0000-0002-2366-6898 FU BK21+ Program through the National Research Foundation of Korea (NRF) - Ministry of Education, Science, and Technology; National Research Foundation of Korea (NRF) - Ministry of Education, Science, and Technology [NRF-2012R1A1A2044287]; KBSI [C34700] FX We especially appreciate the valuable and helpful comments of four anonymous reviewers. This research was supported by the BK21+ Program and Basic Science Research Program (NRF-2012R1A1A2044287) through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science, and Technology. Partial support was also provided by KBSI (Grant No.C34700). The study samples were irradiated at Advanced Technology Radiation Laboratory/KAERI, and the analyses of NMR and FTIR were conducted at KBSI. The XAFS spectra were collected at PAL and experiments at PLS were supported in part by MSIP and POSTECH. NR 43 TC 7 Z9 8 U1 3 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 9684 EP 9691 DI 10.1021/es501661z PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800089 PM 25090368 ER PT J AU Schoen, ME Xue, XB Hawkins, TR Ashbolt, NJ AF Schoen, Mary E. Xue, Xiaobo Hawkins, Troy R. Ashbolt, Nicholas J. TI Comparative Human Health Risk Analysis of Coastal Community Water and Waste Service Options SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ROOF-HARVESTED RAINWATER; DISINFECTION BY-PRODUCTS; DRINKING-WATER; MICROBIAL RISKS; SOUTHEAST QUEENSLAND; CONTROLLED TRIAL; UNITED-STATES; PATHOGENS; QUALITY; SEWAGE AB As a pilot approach to describe adverse human health effects from alternative decentralized community water systems compared to conventional centralized services (business-as-usual [BAUD, selected chemical and microbial hazards were assessed using disability adjusted life years (DALYs) as the common metric. The alternatives included: (1) composting toilets with septic system, (2) urine-diverting toilets with septic system, (3) low flush toilets with blackwater pressure sewer and on-site greywater collection and treatment for nonpotable reuse, and (4) alternative 3 with on-site rainwater treatment and use. Various pathogens (viral, bacterial, and protozoan) and chemicals (disinfection byproducts [DBPs]) were used as reference hazards. The exposure pathways for BAU included accidental ingestion of contaminated recreational water, ingestion of cross-connected sewage to drinking water, and shower exposures to DBPs. The alternative systems included ingestion of treated greywater from garden irrigation, toilet flushing, and crop consumption; and ingestion of treated rainwater while showering. The pathways with the highest health impact included the ingestion of cross-connected drinking water and ingestion of recreational water contaminated by septic seepage. These were also among the most uncertain when characterizing input parameters, particularly the scale of the cross-connection event, and the removal of pathogens during groundwater transport of septic seepage. A comparison of the health burdens indicated potential health benefits by switching from BAU to decentralized water and wastewater systems. C1 [Schoen, Mary E.] Soller Environm Inc, Berkeley, CA 94703 USA. [Xue, Xiaobo] US EPA, Oak Ridge Inst Sci & Educ, Cincinnati, OH 45268 USA. [Hawkins, Troy R.] US EPA, Cincinnati, OH 45268 USA. [Ashbolt, Nicholas J.] Univ Alberta, Edmonton, AB T6G 2G7, Canada. RP Schoen, ME (reprint author), 312 NE 82nd St, Seattle, WA 98115 USA. EM mschoen@sollerenvironmental.com FU U.S. Environmental Protection Agency Office of Research and Development FX This project was supported by the U.S. Environmental Protection Agency Office of Research and Development. NR 52 TC 14 Z9 14 U1 2 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 9728 EP 9736 DI 10.1021/es501262p PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800094 PM 24988142 ER PT J AU Bergesen, JD Heath, GA Gibon, T Suh, S AF Bergesen, Joseph D. Heath, Garvin A. Gibon, Thomas Suh, Sangwon TI Thin-Film Photovoltaic Power Generation Offers Decreasing Greenhouse Gas Emissions and Increasing Environmental Co-benefits in the Long Term SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID LIFE-CYCLE ASSESSMENT; END-OF-LIFE; ELECTRICITY-GENERATION; PV MODULES; ENERGY PAYBACK; WIND POWER; LAND-USE; IMPACTS; TELLURIUM; CADMIUM AB Thin-film photovoltaic (PV) technologies have improved significantly recently, and similar improvements are projected into the future, warranting reevaluation of the environmental implications of PV to update and inform policy decisions. By conducting a hybrid life cycle assessment using the most recent manufacturing data and technology roadmaps, we compare present and projected environmental, human health, and natural resource implications of electricity generated from two common thin-film PV technologies-copper indium gallium selenide (GIGS) and cadmium telluride (CdTe)-in the United States (U.S.) to those of the current U.S. electricity mix. We evaluate how the impacts of thin films can be reduced by likely cost-reducing technological changes: (1) module efficiency increases, (2) module dematerialization, (3) changes in upstream energy and materials production, and (4) end-of-life recycling of balance of system (BOS). Results show comparable environmental and resource impacts for CdTe and GIGS. Compared to the U.S. electricity mix in 2010, both perform at least 90% better in 7 of 12 and at least 50% better in 3 of 12 impact categories, with comparable land use, and increased metal depletion unless BOS recycling is ensured. Technological changes, particularly efficiency increases, contribute to 35-80% reductions in all impacts by 2030. C1 [Bergesen, Joseph D.; Suh, Sangwon] Univ Calif Santa Barbara, Bren Sch Environm Sci & Management, Santa Barbara, CA 93106 USA. [Heath, Garvin A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Gibon, Thomas] Norwegian Univ Sci & Technol NTNU, Dept Energy Proc & Engn, Ind Ecol Programme, NO-7491 Trondheim, Norway. RP Suh, S (reprint author), Univ Calif Santa Barbara, Bren Sch Environm Sci & Management, 2400 Bren Hall, Santa Barbara, CA 93106 USA. EM suh@bren.ucsb.edu OI Gibon, Thomas/0000-0002-2778-8825 FU ConvEne IGERT Program [NSF-DGE 0801627]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy FX We acknowledge Michael Woodhouse and Alan Goodrich of NREL for supplying data and providing review and Anastasiya Lazareva (UCSB) and Patrick O'Donoughue (NREL) for their valuable contributions. Support for J.D.B. was provided by the ConvEne IGERT Program (Grant NSF-DGE 0801627). Support for G.A.H was provided by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy. NR 75 TC 16 Z9 16 U1 3 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 9834 EP 9843 DI 10.1021/es405539z PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800107 PM 24984196 ER PT J AU Kohl, CAK Capo, RC Stewart, BW Wall, AJ Schroeder, KT Hammack, RW Guthrie, GD AF Kohl, Courtney A. Kolesar Capo, Rosemary C. Stewart, Brian W. Wall, Andrew J. Schroeder, Karl T. Hammack, Richard W. Guthrie, George D. TI Strontium Isotopes Test Long-Term Zonal Isolation of Injected and Marcellus Formation Water after Hydraulic Fracturing SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID NATURAL-GAS EXTRACTION; NORTHERN APPALACHIAN BASIN; BARNETT SHALE FORMATION; ACID-MINE DRAINAGE; SOUTHWESTERN PENNSYLVANIA; SURFACE WATERS; WASTE-WATER; WELLS; QUALITY; GEOCHEMISTRY AB One concern regarding unconventional hydrocarbon production from organic-rich shale is that hydraulic fracture stimulation could create pathways that allow injected fluids and deep brines from the target formation or adjacent units to migrate upward into shallow drinking water aquifers. This study presents Sr isotope and geochemical data from a well-constrained site in Greene County, Pennsylvania, in which samples were collected before and after hydraulic fracturing of the Middle Devonian Marcellus Shale. Results spanning a 15-month period indicated no significant migration of Marcellus-derived fluids into Upper Devonian/Lower Mississippian units located 900-1200 m above the lateral Marcellus boreholes or into groundwater sampled at a spring near the site. Monitoring the Sr isotope ratio of water from legacy oil and gas wells or drinking water wells can provide a sensitive early warning of upward brine migration for many years after well stimulation. C1 [Kohl, Courtney A. Kolesar; Capo, Rosemary C.; Stewart, Brian W.; Wall, Andrew J.] Univ Pittsburgh, Dept Geol & Planetary Sci, Pittsburgh, PA 15260 USA. [Kohl, Courtney A. Kolesar; Capo, Rosemary C.; Stewart, Brian W.] Natl Energy Technol Lab Reg Univ Alliance, Pittsburgh, PA 15236 USA. [Wall, Andrew J.; Schroeder, Karl T.; Hammack, Richard W.; Guthrie, George D.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Capo, RC (reprint author), Univ Pittsburgh, Dept Geol & Planetary Sci, Pittsburgh, PA 15260 USA. EM rcapo@pitt.edu; bstewart@pitt.edu FU U.S. Department of Energy, Office of Fossil Energy, under the Office of Oil and Natural Gas; National Energy Technology Laboratory under the RES contract [DE-FE0004000] FX We thank the site operators for access and assistance with sample collection, J. Rodney Diehl and Dennis Stanko for monthly field sampling, and Elizabeth Rowan, Emily Burt, and Thai Phan for assistance with field and analytical work. The comments and suggestions of M. Engle, two anonymous reviewers, and Associate Editor D. Giammar helped clarify and improve this manuscript. This work was supported by the U.S. Department of Energy, Office of Fossil Energy, under the Office of Oil and Natural Gas (Energy Policy Act of 2005, Section 999 Complementary Program Research), as performed through the Oak Ridge Institute for Science and Education at the National Energy Technology Laboratory (A.J.W.) and the National Energy Technology Laboratory's ongoing research under the RES contract DE-FE0004000 (R.C.C. and B.W.S.). NR 44 TC 7 Z9 7 U1 4 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 19 PY 2014 VL 48 IS 16 BP 9867 EP 9873 DI 10.1021/es501099k PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AN6JW UT WOS:000340701800111 PM 25024106 ER PT J AU Kemei, MC Harada, JK Seshadri, R Suchomel, MR AF Kemei, Moureen C. Harada, Jaye K. Seshadri, Ram Suchomel, Matthew R. TI Structural change and phase coexistence upon magnetic ordering in the magnetodielectric spinel Mn3O4 SO PHYSICAL REVIEW B LA English DT Article ID MANGANITES; MAGNETORESISTANCE AB Cooperative Jahn-Teller ordering is well known to drive the cubic Fd (3) over barm to tetragonal I4(1)/amd structural distortion in Mn3O4 at 1170 degrees C. Further structural distortion occurs in Mn3O4 upon magnetic ordering at 42 K. Employing high-resolution variable-temperature synchrotron x-ray diffraction we show that tetragonal I4(1)/amd and orthorhombic Fddd phases coexist with nearly equal fractions below the Neel temperature of Mn3O4. Significant variation in the orthorhombic a and b lattice constants from the tetragonal a lattice constant is observed. Structural phase coexistence in Mn3O4 is attributed to large strains due to the lattice mismatch between the tetragonal I4(1)/amd and the orthorhombic Fddd phases. Strain tensors determined from Rietveld refinement show a highly strained matrix of the I4(1)/amd phase that accommodates the nucleated orthorhombic Fddd phase in the phase coexistence regime. A comparison of the deformation observed in Mn3O4 to structural deformations of other magnetic spinels shows that phase coexistence may be a common theme when structural distortions occur below 50 K. C1 [Kemei, Moureen C.; Harada, Jaye K.; Seshadri, Ram] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Kemei, Moureen C.; Harada, Jaye K.; Seshadri, Ram] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. [Suchomel, Matthew R.] Argonne Natl Lab, X Ray Sci Div, Argonne, IL 60439 USA. RP Kemei, MC (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. EM kemei@mrl.ucsb.edu; jkharada@mrl.ucsb.edu; seshadri@mrl.ucsb.edu; suchomel@aps.anl.gov RI Seshadri, Ram/C-4205-2013; Suchomel, Matthew/C-5491-2015 OI Seshadri, Ram/0000-0001-5858-4027; FU NSF through the DMR [1105301]; Schlumberger Foundation Faculty for the Future fellowship; MRSEC Program of the NSF [DMR 1121053]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We thank Professor Van der Ven for helpful discussions. This project was supported by the NSF through the DMR Grant No. 1105301. M.C.K. was supported by a Schlumberger Foundation Faculty for the Future fellowship. We acknowledge the use of MRL Central Facilities, which are supported by the MRSEC Program of the NSF under Award No. DMR 1121053, a member of the NSF-funded Materials Research Facilities Network (www.mrfn.org). Use of data from the 11-BM beamline at the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Data were also collected on the ID31 beamline at the European Synchrotron Radiation Facility (ESRF), Grenoble, France. We thank A. Fitch and C. Curfs for providing assistance in using beamline ID31. We thank M. Gaultois, Quantum Design staff scientists Dr. N. Dilley and Dr. S. Li, and Quantum Design for high-temperature susceptibility measurements. NR 25 TC 8 Z9 8 U1 3 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 19 PY 2014 VL 90 IS 6 AR 064418 DI 10.1103/PhysRevB.90.064418 PG 8 WC Physics, Condensed Matter SC Physics GA AN6YA UT WOS:000340743500002 ER PT J AU Roberts, BM Stadnik, YV Dzuba, VA Flambaum, VV Leefer, N Budker, D AF Roberts, B. M. Stadnik, Y. V. Dzuba, V. A. Flambaum, V. V. Leefer, N. Budker, D. TI Limiting P-Odd Interactions of Cosmic Fields with Electrons, Protons, and Neutrons SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-ACCURACY CALCULATION; NUCLEAR ANAPOLE MOMENT; MANY-BODY CORRECTIONS; STRONG CP PROBLEM; PARITY NONCONSERVATION; WEAK-INTERACTION; SEARCH; CESIUM; CONSTRAINTS; INVARIANCE AB We propose methods for extracting limits on the strength of P-odd interactions of pseudoscalar and pseudovector cosmic fields with electrons, protons, and neutrons, by exploiting the static and dynamic parity-nonconserving amplitudes and electric dipole moments they induce in atoms. Candidates for such fields are dark matter (including axions) and dark energy, as well as several more exotic sources described by Lorentz-violating standard model extensions. Atomic calculations are performed for H, Li, Na, K, Rb, Cs, Ba+, Tl, Dy, Fr, and Ra+. From these calculations and existing measurements in Dy, Cs, and Tl, we constrain the interaction strengths of the parity-violating static pseudovector cosmic field to be 7 x 10(-15) GeV with an electron, and 3 x 10(-8) GeV with a proton. C1 [Roberts, B. M.; Stadnik, Y. V.; Dzuba, V. A.; Flambaum, V. V.] Univ New S Wales, Sch Phys, Sydney, NSW 2052, Australia. [Flambaum, V. V.] Massey Univ, New Zealand Inst Adv Study, Auckland 0745, New Zealand. [Leefer, N.; Budker, D.] Johannes Gutenberg Univ Mainz, Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Budker, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Budker, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Roberts, BM (reprint author), Univ New S Wales, Sch Phys, Sydney, NSW 2052, Australia. EM b.roberts@unsw.edu.au; y.stadnik@unsw.edu.au RI Roberts, Benjamin/C-1284-2013; Budker, Dmitry/F-7580-2016; Stadnik, Yevgeny/L-4065-2014; OI Roberts, Benjamin/0000-0002-0345-6375; Budker, Dmitry/0000-0002-7356-4814; Leefer, Nathan/0000-0002-4940-8432 FU Australian Research Council; NSF [PHY-1068875]; Perimeter Institute for Theoretical Physics; Government of Canada through Industry Canada; Province of Ontario through the Ministry of Economic Development Innovation; Marie Curie International Incoming Fellowship within the 7th European Community Framework Programme FX The authors would like to thank Michael Hohensee, Iosif B. Khriplovich, Derek Jackson Kimball, V. Alan Kostelecky, Mikhail Kozlov, Maxim Pospelov, Arkady Vainshtein, and Vladimir G. Zelevinsky for valuable discussions. This research was supported in part by the Australian Research Council, by NSF Grant No. PHY-1068875, and by the Perimeter Institute for Theoretical Physics. Research at the Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Economic Development & Innovation. N. Leefer was supported by a Marie Curie International Incoming Fellowship within the 7th European Community Framework Programme. NR 78 TC 27 Z9 27 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 19 PY 2014 VL 113 IS 8 AR 081601 DI 10.1103/PhysRevLett.113.081601 PG 5 WC Physics, Multidisciplinary SC Physics GA AN6ZM UT WOS:000340747900002 PM 25192086 ER PT J AU Wilder, JR Wegener, DT David, MZ Macal, C Daum, R Lauderdale, DS AF Wilder, Jocelyn R. Wegener, Duane T. David, Michael Z. Macal, Charles Daum, Robert Lauderdale, Diane S. TI A National Survey of Skin Infections, Care Behaviors and MRSA Knowledge in the United States SO PLOS ONE LA English DT Article ID RESISTANT STAPHYLOCOCCUS-AUREUS; SOFT-TISSUE INFECTIONS; EMERGENCY-DEPARTMENT; SURVEILLANCE AB A nationally representative sample of approximately 2000 individuals was surveyed to assess SSTI infections over their lifetime and then prospectively over six-months. Knowledge of MRSA, future likelihood to self-treat a SSTI and self-care behaviors was also queried. Chi square tests, linear and multinomial regression were used for analysis. About 50% of those with a reported history of a SSTI typical of MRSA had sought medical treatment. MRSA knowledge was low: 28% of respondents could describe MRSA. Use of protective self-care behaviors that may reduce transmission, such as covering a lesion, differed with knowledge of MRSA and socio-demographics. Those reporting a history of a MRSA-like SSTI were more likely to respond that they would self-treat than those without such a history (OR 2.05 95% CI 1.40, 3.01; p<0.001). Since half of respondents reported not seeking care for past lesions, incidence determined from clinical encounters would greatly underestimate true incidence. MRSA knowledge was not associated with seeking medical care, but was associated with self-care practices that may decrease transmission. C1 [Wilder, Jocelyn R.; David, Michael Z.; Macal, Charles; Daum, Robert; Lauderdale, Diane S.] Univ Chicago, Dept Hlth Studies, Chicago, IL 60637 USA. [Wegener, Duane T.] Ohio State Univ, Dept Psychol, Columbus, OH 43210 USA. [Macal, Charles] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Wilder, JR (reprint author), Univ Chicago, Dept Hlth Studies, Chicago, IL 60637 USA. EM jwilder@uchicago.edu FU Time-Sharing Experiments for the Social Sciences program (TESS; National Science Foundation) [0818839]; National Institute of General Medical Sciences (NIGMS) [U01 Gm087729 MIDAS] FX The survey was supported by Time-Sharing Experiments for the Social Sciences program (TESS; National Science Foundation Grant 0818839; J. Freese and P. S. Visser, principal investigators). Analysis was supported by the National Institute of General Medical Sciences (NIGMS) U01 Gm087729 MIDAS. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 12 TC 5 Z9 5 U1 0 U2 5 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 19 PY 2014 VL 9 IS 8 AR e104277 DI 10.1371/journal.pone.0104277 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN6XM UT WOS:000340742100023 PM 25137061 ER PT J AU Fernandez, CA Martin, PC Schaef, T Bowden, ME Thallapally, PK Dang, L Xu, W Chen, XL McGrail, BP AF Fernandez, Carlos A. Martin, Paul C. Schaef, Todd Bowden, Mark E. Thallapally, Praveen K. Dang, Liem Xu, Wu Chen, Xilin McGrail, B. Peter TI An Electrically Switchable Metal-Organic Framework SO SCIENTIFIC REPORTS LA English DT Article ID IONIC PHASE-TRANSITION; TETRATHIAFULVALENE-CHLORANIL; SPIN-CROSSOVER; COMPLEX; (EDO-TTF)(2)PF6; CU(TCNQ); CRYSTAL; CAPTURE; ENERGY; SALTS AB Crystalline metal organic framework (MOF) materials containing interconnected porosity can be chemically modified to promote stimulus-driven (light, magnetic or electric fields) structural transformations that can be used in a number of devices. Innovative research strategies are now focused on understanding the role of chemical bond manipulation to reversibly alter the free volume in such structures of critical importance for electro-catalysis, molecular electronics, energy storage technologies, sensor devices and smart membranes. In this letter, we study the mechanism for which an electrically switchable MOF composed of Cu(TCNQ) (TCNQ = 7,7,8,8-tetracyanoquinodimethane) transitions from a high-resistance state to a conducting state in a reversible fashion by an applied potential. The actual mechanism for this reversible electrical switching is still not understood even though a number of reports are available describing the application of electric-field-induced switching of Cu(TCNQ) in device fabrication. C1 [Fernandez, Carlos A.; Martin, Paul C.; Xu, Wu; Chen, Xilin; McGrail, B. Peter] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Schaef, Todd; Thallapally, Praveen K.; Dang, Liem] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Bowden, Mark E.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Fernandez, CA (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM carlos.fernandez@pnnl.gov; praveen.thallapally@pnnl.gov; pete.mcgrail@pnnl.gov OI Thallapally, Praveen Kumar/0000-0001-7814-4467; Xu, Wu/0000-0002-2685-8684 FU U.S. Department of Energy; ARPA-E thermal energy storage through High Energy Advanced Thermal Storage (HEATS) program; DOE [DE-AC05-76RL01830] FX This work was performed at Pacific Northwest National Laboratory (PNNL) and was supported by the U.S. Department of Energy, ARPA-E thermal energy storage through High Energy Advanced Thermal Storage (HEATS) program. We thank Dr. James Klausner for programmatic support and helpful discussions throughout the project life cycle. PNNL is operated by Battelle for DOE under contract DE-AC05-76RL01830. NR 33 TC 10 Z9 10 U1 17 U2 139 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 19 PY 2014 VL 4 AR 6114 DI 10.1038/srep06114 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN6NX UT WOS:000340712600001 PM 25135307 ER PT J AU Jeong, DW Choi, WS Okamoto, S Kim, JY Kim, KW Moon, SJ Cho, DY Lee, HN Noh, TW AF Jeong, Da Woon Choi, Woo Seok Okamoto, Satoshi Kim, Jae-Young Kim, Kyung Wan Moon, Soon Jae Cho, Deok-Yong Lee, Ho Nyung Noh, Tae Won TI Dimensionality Control of d-orbital Occupation in Oxide Superlattices SO SCIENTIFIC REPORTS LA English DT Article ID TRANSITION; PRINCIPLES; OCCUPANCY; INTERFACE; LACOO3 AB Manipulating the orbital state in a strongly correlated electron system is of fundamental and technological importance for exploring and developing novel electronic phases. Here, we report an unambiguous demonstration of orbital occupancy control between t(2g) and e(g) multiplets in quasi-two-dimensional transition metal oxide superlattices (SLs) composed of a Mott insulator LaCoO3 and a band insulator LaAlO3. As the LaCoO3 sublayer thickness approaches its fundamental limit (i.e. one unit-cell-thick), the electronic state of the SLs changed from a Mott insulator, in which both t(2g) and e(g) orbitals are partially filled, to a band insulator by completely filling (emptying) the t(2g) (e(g)) orbitals. We found the reduction of dimensionality has a profound effect on the electronic structure evolution, which is, whereas, insensitive to the epitaxial strain. The remarkable orbital controllability shown here offers a promising pathway for novel applications such as catalysis and photovoltaics, where the energy of d level is an essential parameter. C1 [Jeong, Da Woon; Cho, Deok-Yong; Noh, Tae Won] Inst for Basic Sci Korea, Ctr Correlated Electron Syst, Seoul 151747, South Korea. [Jeong, Da Woon; Cho, Deok-Yong; Noh, Tae Won] Seoul Natl Univ, Dept Phys & Astron, Seoul 151747, South Korea. [Choi, Woo Seok; Okamoto, Satoshi; Lee, Ho Nyung] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Choi, Woo Seok] Sungkyunkwan Univ, Dept Phys, Suwon 440746, Gyeonggi D, South Korea. [Kim, Jae-Young] Pohang Univ Sci & Technol, Pohang Accelerator Lab, Pohang 790784, South Korea. [Kim, Kyung Wan] Chungbuk Natl Univ, Dept Phys, Cheongju 361763, South Korea. [Moon, Soon Jae] Hanyang Univ, Dept Phys, Seoul 133791, South Korea. [Cho, Deok-Yong] Chonbuk Natl Univ, Dept Phys, Jeonju 561756, South Korea. RP Cho, DY (reprint author), Inst for Basic Sci Korea, Ctr Correlated Electron Syst, Seoul 151747, South Korea. EM zax@jbnu.ac.kr; hnlee@ornl.gov RI Okamoto, Satoshi/G-5390-2011; Choi, Woo Seok/G-8783-2014; Cho, Deok-Yong/I-4696-2013; Kim, Kyungwan/A-9242-2012; Lee, Ho Nyung/K-2820-2012 OI Okamoto, Satoshi/0000-0002-0493-7568; Cho, Deok-Yong/0000-0001-5789-8286; Kim, Kyungwan/0000-0003-3833-5378; Lee, Ho Nyung/0000-0002-2180-3975 FU Institute for Basic Science (IBS) in Korea; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX We thank G. A. Sawatzky, B. Keimer, V. Hinkov, S. S. A. Seo, S. H. Chang, and R. Eder for helpful discussions. This work was supported by the Institute for Basic Science (IBS) in Korea (x-ray and optical spectroscopy) and by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division (sample design by pulsed laser epitaxy and theory). NR 22 TC 7 Z9 7 U1 4 U2 57 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 19 PY 2014 VL 4 AR 6124 DI 10.1038/srep06124 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN6NZ UT WOS:000340712800003 PM 25134975 ER PT J AU Pan, ZW Lerch, SJL Xu, L Li, XF Chuang, YJ Howe, JY Mahurin, SM Dai, S Hildebrand, M AF Pan, Zhengwei Lerch, Sarah J. L. Xu, Liang Li, Xufan Chuang, Yen-Jun Howe, Jane Y. Mahurin, Shannon M. Dai, Sheng Hildebrand, Mark TI Electronically transparent graphene replicas of diatoms: a new technique for the investigation of frustule morphology SO SCIENTIFIC REPORTS LA English DT Article ID CARBON NANOTUBES; HIGH-QUALITY; SILICON; FILMS AB The morphogenesis of the silica cell walls (called frustules) of unicellular algae known as diatoms is one of the most intriguing mysteries of the diatoms. To study frustule morphogenesis, optical, electron and atomic force microscopy has been extensively used to reveal the frustule morphology. However, since silica frustules are opaque, past observations were limited to outer and fracture surfaces, restricting observations of interior structures. Here we show that opaque silica frustules can be converted into electronically transparent graphene replicas, fabricated using chemical vapor deposition of methane. Chemical vapor deposition creates a continuous graphene coating preserving the frustule's shape and fine, complicated internal features. Subsequent dissolution of the silica with hydrofluoric acid yields a free-standing replica of the internal and external native frustule morphologies. Electron microscopy renders these graphene replicas highly transparent, revealing previously unobserved, complex, three-dimensional, interior frustule structures, which lend new insights into the investigation of frustule morphogenesis. C1 [Pan, Zhengwei; Xu, Liang; Li, Xufan; Chuang, Yen-Jun] Univ Georgia, Coll Engn, Athens, GA 30602 USA. [Pan, Zhengwei] Univ Georgia, Dept Phys & Astron, Athens, GA 30602 USA. [Lerch, Sarah J. L.; Hildebrand, Mark] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Howe, Jane Y.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Mahurin, Shannon M.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Pan, ZW (reprint author), Univ Georgia, Coll Engn, Athens, GA 30602 USA. EM panz@uga.edu; mhildebrand@ucsd.edu RI Howe, Jane/G-2890-2011; Dai, Sheng/K-8411-2015; Li, Xufan/A-8292-2013; OI Dai, Sheng/0000-0002-8046-3931; Li, Xufan/0000-0001-9814-0383; Pan, Zhengwei/0000-0002-3854-958X FU NSF CAREER grant [DMR-0955908]; AFOSR MURI award [RF00965521]; Chemical Sciences, Geosciences and Biosciences Division of Basic Energy Sciences (BES), U.S. Department of Energy (DOE); Division of Scientific User Facilities of BES, U.S. DOE FX Z.W.P. thanks the support of a NSF CAREER grant (DMR-0955908). Work by M.H. and S.L. was supported by an AFOSR MURI award (RF00965521). Work by S.D. and S.M.M. was supported by the Chemical Sciences, Geosciences and Biosciences Division of Basic Energy Sciences (BES), U.S. Department of Energy (DOE). The TEM characterization was conducted at the Oak Ridge National Laboratory ShaRE User Facilities, which is sponsored by the Division of Scientific User Facilities of BES, U.S. DOE. NR 27 TC 6 Z9 7 U1 5 U2 44 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 19 PY 2014 VL 4 AR 6117 DI 10.1038/srep06117 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN6NX UT WOS:000340712600004 PM 25135739 ER PT J AU Linger, JG Vardon, DR Guarnieri, MT Karp, EM Hunsinger, GB Franden, MA Johnson, CW Chupka, G Strathmann, TJ Pienkos, PT Beckham, GT AF Linger, Jeffrey G. Vardon, Derek R. Guarnieri, Michael T. Karp, Eric M. Hunsinger, Glendon B. Franden, Mary Ann Johnson, Christopher W. Chupka, Gina Strathmann, Timothy J. Pienkos, Philip T. Beckham, Gregg T. TI Lignin valorization through integrated biological funneling and chemical catalysis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE biofuels; lignocellulose; biorefinery; aromatic degradation ID PSEUDOMONAS-PUTIDA KT2440; MICROBIAL-DEGRADATION; BIOFUELS PRODUCTION; ESCHERICHIA-COLI; BETA-KETOADIPATE; ACID; BIOMASS; POLYHYDROXYALKANOATES; DEPOLYMERIZATION; BIOSYNTHESIS AB Lignin is an energy-dense, heterogeneous polymer comprised of phenylpropanoid monomers used by plants for structure, water transport, and defense, and it is the second most abundant biopolymer on Earth after cellulose. In production of fuels and chemicals from biomass, lignin is typically underused as a feed-stock and burned for process heat because its inherent heterogeneity and recalcitrance make it difficult to selectively valorize. In nature, however, some organisms have evolved metabolic pathways that enable the utilization of lignin-derived aromatic molecules as carbon sources. Aromatic catabolism typically occurs via upper pathways that act as a "biological funnel" to convert heterogeneous substrates to central intermediates, such as protocatechuate or catechol. These intermediates undergo ring cleavage and are further converted via the beta-ketoadipate pathway to central carbon metabolism. Here, we use a natural aromatic-catabolizing organism, Pseudomonas putida KT2440, to demonstrate that these aromatic metabolic pathways can be used to convert both aromatic model compounds and heterogeneous, lignin-enriched streams derived from pilot-scale biomass pretreatment into medium chain-length polyhydroxyalkanoates (mcl-PHAs). mcl-PHAs were then isolated from the cells and demonstrated to be similar in physicochemical properties to conventional carbohydrate-derived mcl-PHAs, which have applications as bioplastics. In a further demonstration of their utility, mcl-PHAs were catalytically converted to both chemical precursors and fuel-range hydrocarbons. Overall, this work demonstrates that the use of aromatic catabolic pathways enables an approach to valorize lignin by overcoming its inherent heterogeneity to produce fuels, chemicals, and materials. C1 [Linger, Jeffrey G.; Vardon, Derek R.; Guarnieri, Michael T.; Karp, Eric M.; Hunsinger, Glendon B.; Franden, Mary Ann; Johnson, Christopher W.; Pienkos, Philip T.; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Linger, Jeffrey G.; Vardon, Derek R.; Guarnieri, Michael T.; Karp, Eric M.; Franden, Mary Ann; Johnson, Christopher W.; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Adv Biofuels Consortium, Golden, CO 80401 USA. [Chupka, Gina] Natl Renewable Energy Lab, Transportat & Hydrogen Syst Ctr, Golden, CO 80401 USA. [Vardon, Derek R.; Strathmann, Timothy J.] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA. RP Beckham, GT (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. EM gregg.beckham@nrel.gov RI Strathmann, Timothy/K-7606-2012; Vardon, Derek/B-8249-2017 OI Strathmann, Timothy/0000-0002-7299-3115; Vardon, Derek/0000-0002-0199-4524 FU US Department of Energy BioEnergy Technologies Office through the National Advanced Biofuels Consortium; National Science Foundation (NSF) [NSF-CBET-0746453]; NSF Graduate Research Fellowship [NSF-DGE-1144245] FX We thank E. Kuhn and R. Elander for APL; T. VanderWall for conducting the fermentations; M. Resch for running enzymatic hydrolysis; H. Pilath, A. Starace, D. Johnson, and W. Michener for analytical assistance; D. Reuss for analytical assistance and discussions; M. Biddy, T. Foust, and L. Moens for helpful discussions; and B. Knott for comments on the manuscript. We thank the US Department of Energy BioEnergy Technologies Office through the National Advanced Biofuels Consortium for funding. Support for D. R. V. and T.J.S. is also provided by National Science Foundation (NSF) Grant NSF-CBET-0746453 and NSF Graduate Research Fellowship NSF-DGE-1144245 (to D.R.V.). NR 58 TC 97 Z9 97 U1 18 U2 148 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 19 PY 2014 VL 111 IS 33 BP 12013 EP 12018 DI 10.1073/pnas.1410657111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN2TS UT WOS:000340438800039 PM 25092344 ER PT J AU Lemke, RAS Peterson, AC Ziegelhoffer, EC Westphall, MS Tjellstrom, H Coon, JJ Donohue, TJ AF Lemke, Rachelle A. S. Peterson, Amelia C. Ziegelhoffer, Eva C. Westphall, Michael S. Tjellstroem, Henrik Coon, Joshua J. Donohue, Timothy J. TI Synthesis and scavenging role of furan fatty acids SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE radical scavenger; oxygenated fatty acid; fatty acyl methylase ID RHODOBACTER-SPHAEROIDES 2.4.1; SINGLET OXYGEN STRESS; ECF SIGMA-FACTOR; ESCHERICHIA-COLI; RHODOPSEUDOMONAS-SPHAEROIDES; PHOTOOXIDATIVE STRESS; MEMBRANE-LIPIDS; BACTERIA; SYNTHASE; BIOSYNTHESIS AB Fatty acids play important functional and protective roles in living systems. This paper reports on the synthesis of a previously unidentified 19 carbon furan-containing fatty acid, 10,13-epoxy-11-methyl-octadecadienoate (9-(3-methyl-5-pentylfuran-2-yl) nonanoic acid) (19Fu-FA), in phospholipids from Rhodobacter sphaeroides. We show that 19Fu-FA accumulation is increased in cells containing mutations that increase the transcriptional response of this bacterium to singlet oxygen (O-1(2)), a reactive oxygen species generated by energy transfer from one or more light-excited donors to molecular oxygen. We identify a previously undescribed class of S-adenosylmethionine-dependent methylases that convert a phospholipid 18 carbon cis unsaturated fatty acyl chain to a 19 carbon methylated trans unsaturated fatty acyl chain (19M-UFA). We also identify genes required for the O-2-dependent conversion of this 19M-UFA to 19Fu-FA. Finally, we show that the presence of O-1(2) leads to turnover of 19Fu-Fa in vivo. We propose that furan-containing fatty acids like 19Fu-FA can act as a membrane-bound scavenger of O-1(2), which is naturally produced by integral membrane enzymes of the R. sphaeroides photosynthetic apparatus. C1 [Lemke, Rachelle A. S.; Ziegelhoffer, Eva C.; Donohue, Timothy J.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Peterson, Amelia C.; Coon, Joshua J.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Coon, Joshua J.] Univ Wisconsin, Dept Biomol Chem, Madison, WI 53706 USA. [Tjellstroem, Henrik; Coon, Joshua J.; Donohue, Timothy J.] Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. [Westphall, Michael S.] Genome Ctr Wisconsin, Madison, WI 53706 USA. [Tjellstroem, Henrik] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. RP Donohue, TJ (reprint author), Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. EM tdonohue@bact.wisc.edu OI Donohue, Timothy/0000-0001-8738-2467 FU National Institute of General Medical Sciences [GM075273, GM107199]; Department of Energy, Office of Science Great Lakes Bioenergy Research Center [DE-FC02-07ER64494] FX We thank Dr. John Ohlrogge (Michigan State University) for helpful discussions, Dr. John Cronan (University of Illinois) for providing the pAYW19 plasmid, and Becky Ciske for technical assistance early in the project. This work was supported in part by National Institute of General Medical Sciences Grants GM075273 (to T.J.D.) and GM107199 (to J.J.C.) and by Department of Energy, Office of Science Great Lakes Bioenergy Research Center Grant DE-FC02-07ER64494 (to T.J.D.). NR 54 TC 9 Z9 9 U1 1 U2 14 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 19 PY 2014 VL 111 IS 33 BP E3450 EP E3457 DI 10.1073/pnas.1405520111 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN2TS UT WOS:000340438800014 PM 25092314 ER PT J AU Ryan, OW Skerker, JM Maurer, MJ Li, X Tsai, JC Poddar, S Lee, ME DeLoache, W Dueber, JE Arkin, AP Cate, JHD AF Ryan, Owen W. Skerker, Jeffrey M. Maurer, Matthew J. Li, Xin Tsai, Jordan C. Poddar, Snigdha Lee, Michael E. DeLoache, Will Dueber, John E. Arkin, Adam P. Cate, Jamie H. D. TI Selection of chromosomal DNA libraries using a multiplex CRISPR system SO ELIFE LA English DT Article ID SACCHAROMYCES-CEREVISIAE; DIRECTED EVOLUTION; CRYSTAL-STRUCTURE; HIGH-THROUGHPUT; HUMAN-CELLS; RNA; GENOME; YEAST; CAS9; GENES AB The directed evolution of biomolecules to improve or change their activity is central to many engineering and synthetic biology efforts. However, selecting improved variants from gene libraries in living cells requires plasmid expression systems that suffer from variable copy number effects, or the use of complex marker-dependent chromosomal integration strategies. We developed quantitative gene assembly and DNA library insertion into the Saccharomyces cerevisiae genome by optimizing an efficient single-step and marker-free genome editing system using CRISPR-Cas9. With this Multiplex CRISPR (CRISPRm) system, we selected an improved cellobiose utilization pathway in diploid yeast in a single round of mutagenesis and selection, which increased cellobiose fermentation rates by over ten-fold. Mutations recovered in the best cellodextrin transporters reveal synergy between substrate binding and transporter dynamics, and demonstrate the power of CRISPRm to accelerate selection experiments and discoveries of the molecular determinants that enhance biomolecule function. C1 [Ryan, Owen W.; Skerker, Jeffrey M.; Maurer, Matthew J.; Li, Xin; Tsai, Jordan C.; Poddar, Snigdha; Lee, Michael E.; DeLoache, Will; Dueber, John E.; Arkin, Adam P.; Cate, Jamie H. D.] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94704 USA. [Skerker, Jeffrey M.; Lee, Michael E.; DeLoache, Will; Dueber, John E.; Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA USA. [Skerker, Jeffrey M.; Arkin, Adam P.; Cate, Jamie H. D.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA USA. [Tsai, Jordan C.; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Cate, JHD (reprint author), Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94704 USA. EM jcate@lbl.gov RI Arkin, Adam/A-6751-2008; OI Arkin, Adam/0000-0002-4999-2931; Tsai, Jordan/0000-0001-5202-722X; Maurer, Matthew/0000-0002-9150-0240 FU Energy Biosciences Institute FX We thank D. Nunn and J. Doudna for helpful discussions. We thank J. Waters for assistance in phenotype screening assays. This work was supported by funding from the Energy Biosciences Institute. NR 40 TC 55 Z9 56 U1 8 U2 17 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD AUG 19 PY 2014 VL 3 AR e03703 DI 10.7554/eLife.03703 PG 38 WC Biology SC Life Sciences & Biomedicine - Other Topics GA AO3RU UT WOS:000341253500003 ER PT J AU Li, QA Gray, KE Wilkins, SB Fernandez, MG Rosenkranz, S Zheng, H Mitchell, JF AF Li, Qing'an Gray, K. E. Wilkins, S. B. Fernandez, M. Garcia Rosenkranz, S. Zheng, H. Mitchell, J. F. TI Prediction and Experimental Evidence for Thermodynamically Stable Charged Orbital Domain Walls SO PHYSICAL REVIEW X LA English DT Article ID DENSITY-WAVE; DOPED MANGANITES; SUPERCONDUCTIVITY; COEXISTENCE; ORDER AB On theoretical grounds, we show that orbital domain walls (ODWs), which are known to exist in the charge and orbital ordered layered manganite LaSr2Mn2O7, should be partially charged as a result of competition between orbital-induced strain and Coulomb repulsion. This unexpected result provides the necessary condition for the known thermodynamic stability of these ODWs, which are unlike the more typical domain walls that arise only from an external field. We offer experimental data consistent with this theoretical framework through a combined transport and x-ray-diffraction study. In particular, our transport data on this charge and orbital ordered manganite exhibit abrupt transformations to higher conductance at a threshold electric field. As transport phenomena closely resemble effects found for sliding charge-density waves (SCDWs) in pseudo-one-dimensional (1D) materials, a SCDW along such pseudo-1D ODWs provides a natural explanation of our data. Importantly, x-ray-diffraction data eliminate heating and melting of charge order as tenable alternative explanations of our data. C1 [Li, Qing'an; Gray, K. E.; Rosenkranz, S.; Zheng, H.; Mitchell, J. F.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Wilkins, S. B.; Fernandez, M. Garcia] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Li, QA (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM qali@anl.gov OI Rosenkranz, Stephan/0000-0002-5659-0383 FU Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division at Argonne [DE-AC02-06CH11357]; Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division at Brookhaven [DE-AC02-98CH10886] FX The authors would like to acknowledge informative discussions with Peter Littlewood and Ray Osborn and, in particular, with Daniel Khomskii, whose sketch of the ODW orbitals initiated our evaluation of them. This research was funded by the Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division, under Contracts No. DE-AC02-06CH11357 at Argonne and No. DE-AC02-98CH10886 at Brookhaven. NR 19 TC 2 Z9 2 U1 2 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD AUG 18 PY 2014 VL 4 IS 3 AR 031028 DI 10.1103/PhysRevX.4.031028 PG 8 WC Physics, Multidisciplinary SC Physics GA CA7BK UT WOS:000349071800002 ER PT J AU Chen, CY Dawson, S Lewis, IM AF Chen, Chien-Yi Dawson, S. Lewis, I. M. TI Top partners and Higgs boson production SO PHYSICAL REVIEW D LA English DT Article ID VECTOR-LIKE SINGLET; PAIR PRODUCTION; STANDARD MODEL; PP COLLISIONS; ROOT-S=7 TEV; FINAL-STATE; SEARCH; QUARKS; LHC AB The Higgs boson is produced at the LHC through gluon fusion at roughly the Standard Model rate. New colored fermions, which can contribute to gg -> h, must have vectorlike interactions in order not to be in conflict with the experimentally measured rate. We examine the size of the corrections to single and double Higgs production from heavy vectorlike fermions in SU(2)(L) singlets and doublets and search for regions of parameter space where double Higgs production is enhanced relative to the Standard Model prediction. We compare production rates and distributions for double Higgs production from gluon fusion using an exact calculation, the low energy theorem (LET), where the top quark and the heavy vectorlike fermions are taken to be infinitely massive, and an effective theory (EFT) where top mass effects are included exactly and the effects of the heavy fermions are included to O(1/M-X(2)). Unlike the LET, the EFT gives an extremely accurate description of the kinematic distributions for double Higgs production. C1 [Chen, Chien-Yi; Dawson, S.; Lewis, I. M.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Chen, CY (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. OI Dawson, Sally/0000-0002-5598-695X FU U.S. Department of Energy [DE-AC02-98CH10886] FX This work is supported by the U.S. Department of Energy under Grant No. DE-AC02-98CH10886. NR 58 TC 18 Z9 18 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 18 PY 2014 VL 90 IS 3 AR 035016 DI 10.1103/PhysRevD.90.035016 PG 18 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO4DW UT WOS:000341287400012 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Roland, B Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Klein, B Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, TD Pol, ME Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Aleksandrov, A Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Mahmoud, MA Radik, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thur, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Garcia, JG Geiser, A Gunnellini, P Hauk, J Hellwig, G Hempel, M Horton, D Jung, H Kasemann, M Katsas, P Kieseler, J Kleinwort, C Krucker, D Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Ron, E Sahin, MO Salfeld-Nebgen, J Saxena, P Schmidt, R Schoerner-Sadenius, T Schroder, M Spannagel, S Trevino, ADRV Walsh, R Wissing, C Martin, MA Blobel, V Vignali, MC Erfle, J Garutti, E Goebel, K Gorner, M Gosselink, M Haller, J Hoing, RS Kirschenmann, H Klanner, R Kogler, R Lange, J Lapsien, T Lenz, T Marchesini, I Ott, J Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Hartmann, F Hauth, T Husemann, U Katkov, I Kornmayer, A Kuznetsova, E Pardo, PL Mozer, MU Muller, T Nurnberg, A Quast, G Rabbertz, K Ratnikov, F Rocker, S Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Markou, A Markou, C Psallidas, A Topsis-Giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Palinkas, J Szillasi, Z Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kalsi, AK Kaur, M Mittal, M Nishu, N Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Sharma, V Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, S Jain, S Khurana, R Modak, A Mukherjee, S Roy, D Sarkar, S Sharan, M Abdulsalam, A Dutta, D Kailas, S Kumar, V Mohanty, 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CA CMS Collaboration Pereira, AV TI Search for jet extinction in the inclusive jet-p(T) spectrum from proton-proton collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID ATLAS DETECTOR; FINAL-STATES; LHC; DIMENSIONS; SIGNATURES; CMS AB The first search at the LHC for the extinction of QCD jet production is presented, using data collected with the CMS detector corresponding to an integrated luminosity of 10.7 fb-1 of proton-proton collisions at a center-of-mass energy of 8 TeV. The extinction model studied in this analysis is motivated by the search for signatures of strong gravity at the TeV scale (terascale gravity) and assumes the existence of string couplings in the strong-coupling limit. In this limit, the string model predicts the suppression of all high-transverse-momentum standard model processes, including jet production, beyond a certain energy scale. 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[Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Charlot, C.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J-L; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J-M; Chabert, E. C.; Collard, C.; Conte, E.; Fontaine, J-C; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A-C; Van Hove, P.] Univ Haute Alsace Mulhouse, IN2P3, CNRS, Inst Pluridisciplinaire Hubert Curien,Univ Strasb, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Montoya, C. A. Carrillo; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Gunnellini, P.; Hauk, J.; Hellwig, G.; Hempel, M.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I-A; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Ron, E.; Sahin, M. O.; Salfeld-Nebgen, J.; Saxena, P.; Schmidt, R.; Schoerner-Sadenius, T.; Schroeder, M.; Spannagel, S.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Vignali, M. Centis; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Gosselink, M.; Haller, J.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, T.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.; Bhardwaj, A.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kalsi, A. K.; Kaur, M.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iasellia, G.; Maggia, G.; Maggia, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iasellia, G.; Maggia, G.; My, S.; Pugliese, G.; Radogna, R.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castr, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castr, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, Milan, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, I-95124 Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Goria, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropian, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Goria, V.; Lenzi, P.; Tropian, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Dorigo, T.; Galanti, M.; Gasparini, F.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Galanti, M.; Gasparini, F.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Moon, C. S.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.; Roland, G.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.] Univ Turin, Turin, Italy. [Arcidiacono, R.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Park, S.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Y.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubini, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Dordevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Masetti, G.; Giordano, F.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Di Guida, S.; Meola, S.; Paolucci, P.; Spiezia, A.; Palla, F.; Savoy-Navarro, A.; Vernieri, C.; Micheli, F.; Soffi, L.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Roland, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Wardle, N.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W-S; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R-S; Majumder, D.; Petrakou, E.; Shi, X.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A-M; Malik, S.; Marrouche, J.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.; Cooper, S. I.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Richardson, C.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Kennedy, E.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Dittmer, S.; Eggert, N.; Hopkins, W.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Carver, M.; Cheng, T.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida State Univ, Melbourne, FL USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J-P; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y-J; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, England. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Pearson, T.; Planer, M.; Ruchti, R.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Driga, O.; Elmer, P.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.; Kamon, T.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C-E] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.; Radik, A.] British Univ Egypt, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radik, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J-L; Conte, E.; Fontaine, J-C] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.] Eotvos Lorand Univ, Budapest, Hungary. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Bouhali, O.] CNRS, IN2P3, Paris, France. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Roland, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Gonzalez Caballero, Isidro/E-7350-2010; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Scodellaro, Luca/K-9091-2014; Cerrada, Marcos/J-6934-2014; Dahms, Torsten/A-8453-2015; Ferguson, Thomas/O-3444-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Montanari, Alessandro/J-2420-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; OI Gonzalez Caballero, Isidro/0000-0002-8087-3199; Codispoti, Giuseppe/0000-0003-0217-7021; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476; Ferguson, Thomas/0000-0001-5822-3731; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Sogut, Kenan/0000-0002-9682-2855 FU Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of Foundation for Polish Science - European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); and the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF. NR 43 TC 1 Z9 1 U1 5 U2 67 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 18 PY 2014 VL 90 IS 3 AR 032005 DI 10.1103/PhysRevD.90.032005 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO4DW UT WOS:000341287400001 ER PT J AU Cai, S Schaffer, JE Daymond, MR Yu, C Ren, Y AF Cai, S. Schaffer, J. E. Daymond, M. R. Yu, C. Ren, Y. TI Effect of heat treatment temperature on nitinol wire SO APPLIED PHYSICS LETTERS LA English DT Article ID SHAPE-MEMORY ALLOYS; SITU NEUTRON-DIFFRACTION; SUPERELASTIC NITI; R-PHASE; CRYSTAL-STRUCTURE; TIC COMPOSITES; CRACK-TIP; X-RAY; EVOLUTION; STRAIN AB In-situ synchrotron X-ray diffraction has been used to study the influence of the heat treatment temperature on the subsequent micromechanical behavior of nitinol wire. It was found that increase in the heat treatment temperature rotated the austenite texture from the {332}(B2) fiber towards the {111}(B2) fiber, and the texture of the Stress-Induced Martensite phase changed from the ((1) over bar 40)(B19') to the ((1) over bar 20)(B19') fiber accordingly. Heat treatment at a low temperature reduces the internal residual strains in the austenite during super-elastic deformation and therefore improves the materials fatigue performance. The development of internal residual strains in austenite is controlled by transformation induced plasticity and the reversal martensite to austenite transformation. (C) 2014 AIP Publishing LLC. C1 [Cai, S.; Schaffer, J. E.] Ft Wayne Met Res Prod Corp, Ft Wayne, IN 46809 USA. [Daymond, M. R.] Queens Univ, Dept Mech & Mat Engn, Kingston, ON K7L 3N6, Canada. [Yu, C.] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. [Ren, Y.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Cai, S (reprint author), Ft Wayne Met Res Prod Corp, 9609 Ardmore Ave, Ft Wayne, IN 46809 USA. OI Daymond, Mark/0000-0001-6242-7489 FU U.S. Department of Energy, Office of Science [DEAC02-06CH11357] FX Use of the synchrotron X-ray at APS was granted by the U.S. Department of Energy, Office of Science, under Contract No. DEAC02-06CH11357. Data were analyzed by using the FIT2D, Maud, and GSAS software. Cai and Schaffer thank their colleagues C. Myers for making samples, J. Kolhoff for DSC testing and B. Liechty for fatigue testing, and are grateful for the continuous support from Fort Wayne Metals management. NR 38 TC 2 Z9 2 U1 2 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 18 PY 2014 VL 105 IS 7 AR 071904 DI 10.1063/1.4893595 PG 5 WC Physics, Applied SC Physics GA AO2XE UT WOS:000341189800025 ER PT J AU Chapman, BJ Bornstein, AC Ghimire, NJ Mandrus, D Lee, M AF Chapman, Benjamin J. Bornstein, Alexander C. Ghimire, Nirmal J. Mandrus, David Lee, Minhyea TI Spin structure of the anisotropic helimagnet Cr1/3NbS2 in a magnetic field SO APPLIED PHYSICS LETTERS LA English DT Article ID WEAK FERROMAGNETISM; SKYRMION LATTICE; MAGNETORESISTANCE AB In this letter, we describe the ground-state magnetic structure of the highly anisotropic helimagnet Cr1/3NbS2 in a magnetic field. A Heisenberg spin model with Dyzaloshinkii-Moriya interactions and magnetocrystalline anisotropy allows the ground state spin structure to be calculated for magnetic fields of arbitrary strength and direction. Comparison with magnetization measurements shows excellent agreement with the predicted spin structure. (C) 2014 AIP Publishing LLC. C1 [Chapman, Benjamin J.; Bornstein, Alexander C.; Lee, Minhyea] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Ghimire, Nirmal J.; Mandrus, David] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Ghimire, Nirmal J.; Mandrus, David] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Mandrus, David] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Chapman, BJ (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA. EM minhyea.lee@colorado.edu FU US DOE, Basic Energy Sciences, Materials Sciences and Engineering Division (ORNL); CU [DE-SC0006888] FX We thank P. Beale, M. Glaser, and A. Koller for their insight. This work was supported by the US DOE, Basic Energy Sciences, Materials Sciences and Engineering Division (ORNL) and at CU under Award No. DE-SC0006888. NR 22 TC 9 Z9 10 U1 4 U2 31 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 18 PY 2014 VL 105 IS 7 AR 072405 DI 10.1063/1.4893567 PG 4 WC Physics, Applied SC Physics GA AO2XE UT WOS:000341189800048 ER PT J AU Greene, PK Osten, J Lenz, K Fassbender, J Jenkins, C Arenholz, E Endo, T Iwata, N Liu, K AF Greene, Peter K. Osten, Julia Lenz, Kilian Fassbender, Juergen Jenkins, Catherine Arenholz, Elke Endo, Tamio Iwata, Nobuyuki Liu, Kai TI Tuning perpendicular anisotropy gradient in Co/Pd multilayers by ion irradiation SO APPLIED PHYSICS LETTERS LA English DT Article ID 1ST-ORDER REVERSAL CURVES; COUPLED COMPOSITE MEDIA; FILMS; ARRAYS AB The tunability of Ar+ ion irradiation of Co/Pd multilayers has been employed to create depth-dependent perpendicular anisotropy gradients. By adjusting the Ar+ kinetic energy and fluence, the depth and lateral density of the local structural modification are controlled. First-order reversal curve analysis through X-ray magnetic circular dichroism and conventional magnetometry studies shows that the local structural damage weakens the perpendicular anisotropy near the surface, leading to a magnetization tilting towards the in-plane direction. The ion irradiation method is complementary to and may be used in conjunction with, other synthesis approaches to maximize the anisotropy gradient. (C) 2014 AIP Publishing LLC. C1 [Greene, Peter K.; Liu, Kai] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Osten, Julia; Lenz, Kilian; Fassbender, Juergen] Helmholtz Zentrum Dresden Rossendorf, Inst Ion Beam Phys & Mat Res, D-01328 Dresden, Germany. [Osten, Julia; Fassbender, Juergen] Tech Univ Dresden, D-01609 Dresden, Germany. [Jenkins, Catherine; Arenholz, Elke] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Endo, Tamio] Mie Univ, Grad Sch Engn, Tsu, Mie 5148507, Japan. [Iwata, Nobuyuki] Nihon Univ, Dept Elect & Comp Sci, Chiba 2748501, Japan. RP Liu, K (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. EM kailiu@ucdavis.edu RI Liu, Kai/B-1163-2008; Fassbender, Juergen/A-8664-2008 OI Liu, Kai/0000-0001-9413-6782; Fassbender, Juergen/0000-0003-3893-9630 FU U.S. National Science Foundation at UCD [DMR-1007891, ECCS-0925626]; Deutsche Forschungsgemeinschaft at HZDR [FA 314/3-2]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DEAC02-05CH11231] FX This work has been supported by the U.S. National Science Foundation (DMR-1007891 and ECCS-0925626) at UCD and by the Deutsche Forschungsgemeinschaft (Grant No. FA 314/3-2) at HZDR. The work at the ALS was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy (DEAC02-05CH11231). NR 30 TC 3 Z9 3 U1 4 U2 20 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 18 PY 2014 VL 105 IS 7 AR 072401 DI 10.1063/1.4893569 PG 5 WC Physics, Applied SC Physics GA AO2XE UT WOS:000341189800044 ER PT J AU Henry, MD Wolfley, S Monson, T Lewis, R AF Henry, M. David Wolfley, Steve Monson, Todd Lewis, Rupert TI Ga lithography in sputtered niobium for superconductive micro and nanowires SO APPLIED PHYSICS LETTERS LA English DT Article ID FABRICATION; SILICON AB This work demonstrates the use of focused ion beam (FIB) implanted Ga as a lithographic mask for plasma etching of Nb films. Using a highly collimated Ga beam of a FIB, Nb is implanted 12 nm deep with a 14 nm thick Ga layer providing etch selectivity better than 15: 1 with fluorine based etch chemistry. Implanted square test patterns, both 10 mu m by 10 mu m and 100 mu m by 100 mu m, demonstrate that doses above than 7.5 x 10(15) cm(-2) at 30 kV provide adequate mask protection for a 205 nm thick, sputtered Nb film. The resolution of this dry lithographic technique is demonstrated by fabrication of nanowires 75 nm wide by 10 mu m long connected to 50 mu m wide contact pads. The residual resistance ratio of patterned Nb films was 3. The superconducting transition temperature (T-c) = 7.7K was measured using a magnetic properties measurement system. This nanoscale, dry lithographic technique was extended to sputtered TiN and Ta here and could be used on other fluorine etched superconductors such as NbN, NbSi, and NbTi. (C) 2014 AIP Publishing LLC. C1 [Henry, M. David; Wolfley, Steve; Monson, Todd; Lewis, Rupert] Sandia Natl Labs, MESA Facil, Albuquerque, NM 87185 USA. RP Henry, MD (reprint author), Sandia Natl Labs, MESA Facil, POB 5800, Albuquerque, NM 87185 USA. OI Monson, Todd/0000-0002-9782-7084 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The authors acknowledge and thank the staff of Sandia's MESA facility, Travis Young and Michael Wiwi for fabrication and measurement of the films and Charles Pearce for assistance in measurements. NR 18 TC 0 Z9 0 U1 1 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 18 PY 2014 VL 105 IS 7 AR 072601 DI 10.1063/1.4893446 PG 4 WC Physics, Applied SC Physics GA AO2XE UT WOS:000341189800058 ER PT J AU Kumar, A Beyerlein, IJ Wang, J AF Kumar, Anil Beyerlein, Irene J. Wang, Jian TI First-principles study of the structure of Mg/Nb multilayers SO APPLIED PHYSICS LETTERS LA English DT Article ID SEVERE PLASTIC-DEFORMATION; AUGMENTED-WAVE METHOD; MECHANICAL-PROPERTIES; METALLIC MULTILAYERS; ELASTIC CONSTANTS; MAGNESIUM ALLOYS; INTERFACES; STRENGTH; COMPOSITES; NB AB The magnesium (Mg) phase characterized within Mg/Nb multilayers can adopt either a body-centered cubic (bcc-Mg) or hexagonal close packed (hcp-Mg) structure, depending on the Mg layer thickness. Using first-principles density functional theory, we find that bcc-Mg has a similar weight density of hcp-Mg, lower Young's modulus, and higher shear modulus than hcp-Mg, and the same conventional slip systems as the bcc structure. A simple theoretical model is developed to predict the structural stability of both the bcc-Mg/Nb and hcp-Mg/Nb multilayers. It shows that the bcc-Mg/Nb multilayer is energetically favorable when the bcc-Mg layer is less than 4.2 nm. (C) 2014 AIP Publishing LLC. C1 [Kumar, Anil; Wang, Jian] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Wang, J (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. EM wangj6@lanl.gov RI Kumar, Anil /H-4345-2016; Kumar, Anil/A-9834-2013; Wang, Jian/F-2669-2012 OI Kumar, Anil/0000-0002-4901-8987; Wang, Jian/0000-0001-5130-300X FU Los Alamos National Laboratory Directed Research and Development ER Grant [20140348ER]; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences [2014LANLE8C4] FX We would like to thank support from Los Alamos National Laboratory Directed Research and Development ER Grant 20140348ER. J.W. thanks the support from the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Core program under FWP# 2014LANLE8C4. NR 42 TC 3 Z9 3 U1 0 U2 31 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 18 PY 2014 VL 105 IS 7 AR 071602 DI 10.1063/1.4893700 PG 5 WC Physics, Applied SC Physics GA AO2XE UT WOS:000341189800014 ER PT J AU Paulauskas, T Buurma, C Colegrove, E Guo, Z Sivananthan, S Chan, MKY Klie, RF AF Paulauskas, T. Buurma, C. Colegrove, E. Guo, Z. Sivananthan, S. Chan, M. K. Y. Klie, R. F. TI Atomic-resolution characterization of the effects of CdCl2 treatment on poly-crystalline CdTe thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID CDS/CDTE SOLAR-CELLS; EFFICIENCY AB Poly-crystalline CdTe thin films on glass are used in commercial solar-cell superstrate devices. It is well known that post-deposition annealing of the CdTe thin films in a CdCl2 environment significantly increases the device performance, but a fundamental understanding of the effects of such annealing has not been achieved. In this Letter, we report a change in the stoichiometry across twin boundaries in CdTe and propose that native point defects alone cannot account for this variation. Upon annealing in CdCl2, we find that the stoichiometry is restored. Our experimental measurements using atomic-resolution high-angle annular dark field imaging, electron energy-loss spectroscopy, and energy dispersive X-ray spectroscopy in a scanning transmission electron microscope are supported by first-principles density functional theory calculations. (C) 2014 AIP Publishing LLC. C1 [Paulauskas, T.; Buurma, C.; Colegrove, E.; Guo, Z.; Sivananthan, S.; Klie, R. F.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Chan, M. K. Y.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Paulauskas, T (reprint author), Univ Illinois, Dept Phys, 845 W Taylor St M-C 273, Chicago, IL 60607 USA. EM tpaula2@uic.edu FU U.S. Department of Energy Sunshot Program [DOE-EE00005956]; MRI-R2 from National Science Foundation [DMR-0959470]; UIC Research Resources Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by a grant from the U.S. Department of Energy Sunshot Program (No. DOE-EE00005956). The acquisition of the UIC JEOL JEMARM200CF was supported by a MRI-R2 grant from the National Science Foundation [No. DMR-0959470]. Support from the UIC Research Resources Center is also acknowledged. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 32 TC 5 Z9 5 U1 5 U2 30 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 18 PY 2014 VL 105 IS 7 AR 071910 DI 10.1063/1.4893727 PG 5 WC Physics, Applied SC Physics GA AO2XE UT WOS:000341189800031 ER PT J AU Bhattacharya, T Buchoff, MI Christ, NH Ding, HT Gupta, R Jung, C Karsch, F Lin, ZJ Mawhinney, RD McGlynn, G Mukherjee, S Murphy, D Petreczky, P Renfrew, D Schroeder, C Soltz, RA Vranas, PM Yin, HT AF Bhattacharya, Tanmoy Buchoff, Michael I. Christ, Norman H. Ding, H. -T. Gupta, Rajan Jung, Chulwoo Karsch, F. Lin, Zhongjie Mawhinney, R. D. McGlynn, Greg Mukherjee, Swagato Murphy, David Petreczky, P. Renfrew, Dwight Schroeder, Chris Soltz, R. A. Vranas, P. M. Yin, Hantao TI QCD Phase Transition with Chiral Quarks and Physical Quark Masses SO PHYSICAL REVIEW LETTERS LA English DT Article ID CHROMODYNAMICS AB We report on the first lattice calculation of the QCD phase transition using chiral fermions with physical quark masses. This calculation uses 2 + 1 quark flavors, spatial volumes between (4 fm)(3) and (11 fm)(3) and temperatures between 139 and 196 MeV. Each temperature is calculated at a single lattice spacing corresponding to a temporal Euclidean extent of N-t = 8. The disconnected chiral susceptibility, chi(disc) shows a pronounced peak whose position and height depend sensitively on the quark mass. We find no metastability near the peak and a peak height which does not change when a 5 fm spatial extent is increased to 10 fm. Each result is strong evidence that the QCD "phase transition" is not first order but a continuous crossover for m(pi) = 135 MeV. The peak location determines a pseudocritical temperature T-c = 155(1)(8) MeV, in agreement with earlier staggered fermion results. However, the peak height is 50% greater than that suggested by previous staggered results. Chiral SU(2)(L) x SU(2)(R) symmetry is fully restored above 164 MeV, but anomalous U(1)A symmetry breaking is nonzero above T-c and vanishes as T is increased to 196 MeV. C1 [Bhattacharya, Tanmoy; Gupta, Rajan] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. [Buchoff, Michael I.; Schroeder, Chris; Soltz, R. A.; Vranas, P. M.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Buchoff, Michael I.] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Christ, Norman H.; Lin, Zhongjie; Mawhinney, R. D.; McGlynn, Greg; Murphy, David; Renfrew, Dwight; Yin, Hantao] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Ding, H. -T.] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Ding, H. -T.] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Jung, Chulwoo; Karsch, F.; Mukherjee, Swagato; Petreczky, P.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Karsch, F.] Univ Bielefeld, Fak Phys, D-33615 Bielefeld, Germany. RP Bhattacharya, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. EM nhc@phys.columbia.edu RI Bhattacharya, Tanmoy/J-8956-2013; OI Bhattacharya, Tanmoy/0000-0002-1060-652X; Mukherjee, Swagato/0000-0002-3824-1008; Gupta, Rajan/0000-0003-1784-3058; Murphy, David/0000-0002-8538-815X; Ding, Heng-Tong/0000-0003-0590-081X FU LLNL [LDRD13-ERD-023]; U.S. Department of Energy [DE-AC52-07NA27344]; DOE [DE-FG02-92ER40699, DE-KA-1401020, DE-AC02-98CH10886, DE-FG02-00ER41132]; Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Nuclear Physics FX Computing support for this work on the LLNL Vulcan Blue Gene/Q supercomputer came from the Lawrence Livermore National Laboratory (LLNL) Institutional Computing Grand Challenge program. We gratefully acknowledge the high-performance Blue Gene/Q code created and provided by Peter Boyle and thank LLNL for funding from LDRD13-ERD-023. This work has been supported by the U.S. Department of Energy under Contract No. DE-AC52-07NA27344 (LLNL). N. H. C., Z. L., R. D. M., G. M., D. M., and H. Y. were supported in part by DOE Grant No. DE-FG02-92ER40699. T. B. and R. G. were supported in part by DOE Grant No. DE-KA-1401020. H.-T.D., F. K., S. M., and P. P. were supported in part by DOE Grant No. DE-AC02-98CH10886. M. I. B. was supported in part by DOE Grant No. DE-FG02-00ER41132. This work, and the development of software used in this work, has been supported in part through the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Nuclear Physics. NR 19 TC 81 Z9 81 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 18 PY 2014 VL 113 IS 8 AR 082001 DI 10.1103/PhysRevLett.113.082001 PG 4 WC Physics, Multidisciplinary SC Physics GA AO4FT UT WOS:000341292300002 PM 25192088 ER PT J AU Chen, YP Sun, YY Wang, H West, D Xie, Y Zhong, J Meunier, V Cohen, ML Zhang, SB AF Chen, Yuanping Sun, Y. Y. Wang, H. West, D. Xie, Yuee Zhong, J. Meunier, V. Cohen, Marvin L. Zhang, S. B. TI Carbon Kagome Lattice and Orbital-Frustration-Induced Metal-Insulator Transition for Optoelectronics SO PHYSICAL REVIEW LETTERS LA English DT Article ID SPIN LIQUIDS; CYCLOPROPANE; PINWHEEL; ICE AB A three-dimensional elemental carbon kagome lattice, made of only fourfold-coordinated carbon atoms, is proposed based on first-principles calculations. Despite the existence of 60 degrees bond angles in the triangle rings, widely perceived to be energetically unfavorable, the carbon kagome lattice is found to display exceptional stability comparable to that of C-60. The system allows us to study the effects of triangular frustration on the electronic properties of realistic solids, and it demonstrates a metal-insulator transition from that of graphene to a direct gap semiconductor in the visible blue region. By minimizing s-p orbital hybridization, which is an intrinsic property of carbon, not only the band edge states become nearly purely frustrated p states, but also the band structure is qualitatively different from any known bulk elemental semiconductors. For example, the optical properties are similar to those of direct-gap semiconductors GaN and ZnO, whereas the effective masses are comparable to or smaller than those of Si. C1 [Chen, Yuanping; Sun, Y. Y.; Wang, H.; West, D.; Meunier, V.; Zhang, S. B.] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. [Chen, Yuanping; Xie, Yuee; Zhong, J.] Xiangtan Univ, Dept Phys, Xiangtan 411105, Hunan, Peoples R China. [Cohen, Marvin L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Cohen, Marvin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhang, SB (reprint author), Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. EM zhangs9@rpi.edu RI Meunier, Vincent/F-9391-2010; Zhang, Shengbai/D-4885-2013; West, Damien/F-8616-2012; Sun, Yi-Yang/H-4029-2014 OI Meunier, Vincent/0000-0002-7013-179X; Zhang, Shengbai/0000-0003-0833-5860; West, Damien/0000-0002-4970-3968; FU National Natural Science Foundation of China [51176161, 51376005, 11204262]; U.S. DOE [DE-SC0002623]; DOE [DE-AC02-05CH11231]; NSF [DMRIO-1006184]; Theory Program at the Lawrence Berkeley National Laboratory through the Office of Basic Energy Science, U.S. Department of Energy [DE-AC02-05CH11231] FX Work in China was supported by the National Natural Science Foundation of China (Grants No. 51176161, No. 51376005, and No. 11204262). Work at RPI was supported by U.S. DOE under Grant No. DE-SC0002623. The supercomputer time was provided by NERSC under DOE Contract No. DE-AC02-05CH11231 and the CCI at RPI. M. L. C. was supported by NSF Grant No. DMRIO-1006184 and the Theory Program at the Lawrence Berkeley National Laboratory through the Office of Basic Energy Science, U.S. Department of Energy under Contract No. DE-ac02-05ch11231. We thank Susumu Saito and Yuki Sakai for useful discussions. NR 42 TC 14 Z9 14 U1 0 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 18 PY 2014 VL 113 IS 8 AR 085501 DI 10.1103/PhysRevLett.113.085501 PG 5 WC Physics, Multidisciplinary SC Physics GA AO4FT UT WOS:000341292300004 ER PT J AU Zhang, J Sarovar, M AF Zhang, Jun Sarovar, Mohan TI Quantum Hamiltonian Identification from Measurement Time Traces SO PHYSICAL REVIEW LETTERS LA English DT Article AB Precise identification of parameters governing quantum processes is a critical task for quantum information and communication technologies. In this Letter, we consider a setting where system evolution is determined by a parametrized Hamiltonian, and the task is to estimate these parameters from temporal records of a restricted set of system observables (time traces). Based on the notion of system realization from linear systems theory, we develop a constructive algorithm that provides estimates of the unknown parameters directly from these time traces. We illustrate the algorithm and its robustness to measurement noise by applying it to a one-dimensional spin chain model with variable couplings. C1 [Zhang, Jun] Shanghai Jiao Tong Univ, Joint Inst UM, Shanghai 200240, Peoples R China. [Zhang, Jun] Shanghai Jiao Tong Univ, Key Lab Syst Control & Informat Proc MOE, Shanghai 200240, Peoples R China. [Sarovar, Mohan] Sandia Natl Labs, Dept Scalable & Secure Syst Res 08961, Livermore, CA 94550 USA. RP Zhang, J (reprint author), Shanghai Jiao Tong Univ, Joint Inst UM, Shanghai 200240, Peoples R China. EM mnsarov@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSFC [61174086]; State Key Laboratory of Precision Spectroscopy, ECNU, China; National Science Foundation [NSF PHY11-25915] FX M. S. thanks Akshat Kumar for information on techniques for solving multivariate polynomial systems. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. J. Z. acknowledges financial support from NSFC under Grant No. 61174086, and State Key Laboratory of Precision Spectroscopy, ECNU, China. The authors are grateful for the hospitality of KITP at UCSB, where this work was initiated. This research was supported in part by the National Science Foundation under Grant No. NSF PHY11-25915. NR 24 TC 6 Z9 6 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 18 PY 2014 VL 113 IS 8 AR 080401 DI 10.1103/PhysRevLett.113.080401 PG 5 WC Physics, Multidisciplinary SC Physics GA AO4FT UT WOS:000341292300001 PM 25192077 ER PT J AU Asaba, T Han, TH Lawson, BJ Yu, F Tinsman, C Xiang, Z Li, G Lee, YS Li, L AF Asaba, Tomoya Han, Tian-Heng Lawson, B. J. Yu, F. Tinsman, C. Xiang, Z. Li, G. Lee, Young S. Li, Lu TI High-field magnetic ground state in S=1/2 kagome lattice antiferromagnet ZnCu3(OH)(6)Cl-2 SO PHYSICAL REVIEW B LA English DT Article ID HEISENBERG-ANTIFERROMAGNET; SUPERCONDUCTIVITY; INSULATOR; LIQUIDS; PHASE AB Herbertsmithite ZnCu3(OH)(6)Cl-2 is a kagome lattice antiferromagnet with spin-1/2 and has been demonstrated to be a likely candidate of spin liquid by a number of recent experiments. The high-field magnetization of the kagome lattice is complicated due to the presence of a few percent of extra Cu impurities sitting on the interlayer metallic sites. To determine the magnetic ground state of the kagome lattice, we measured the magnetization of a single crystalline ZnCu3(OH)(6)Cl-2 using torque magnetometry down to the base temperatures 20 mK in intense magnetic field as high as 31 T. The high-field intrinsic magnetization from the kagome lattice turns out to be linear with magnetic field, and the magnetic susceptibility is independent of temperature at 20 mK <= T <= 5 K. Moreover, below 2 K, several field-induced anomalies are observed in between 7 T and 15 T. C1 [Asaba, Tomoya; Lawson, B. J.; Yu, F.; Tinsman, C.; Xiang, Z.; Li, G.; Li, Lu] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Han, Tian-Heng; Lee, Young S.] MIT, Cambridge, MA 02139 USA. [Han, Tian-Heng] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Han, Tian-Heng] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Han, Tian-Heng] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Xiang, Z.] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China. RP Li, L (reprint author), Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. EM luli@umich.edu RI Li, Gang/E-3033-2015 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0008110]; U.S. Department of Energy [DE-FG02-07ER46134]; Nakajima Foundation; Grainger Fellowship from the Department of Physics, University of Chicago; National Science Foundation Graduate Fellowship [F031543]; NSF [DMR-084173]; State of Florida; DOE FX This work at the University of Michigan is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Grant No. DE-SC0008110. The work at MIT is supported by the U.S. Department of Energy under Grant No. DE-FG02-07ER46134. T.A. acknowledges the support from the Nakajima Foundation. T.-H.H. acknowledges the support by the Grainger Fellowship from the Department of Physics, University of Chicago during data analysis and manuscript writing. B.J.L. acknowledges the support from the National Science Foundation Graduate Fellowship Grant No. F031543. We are grateful for the discussions with P.A. Lee, S. Sachdev, and Kai Sun. The high-field experiments were performed at the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement No. DMR-084173, by the State of Florida, and by the DOE. NR 31 TC 4 Z9 4 U1 3 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 18 PY 2014 VL 90 IS 6 AR 064417 DI 10.1103/PhysRevB.90.064417 PG 5 WC Physics, Condensed Matter SC Physics GA AO3WK UT WOS:000341267500004 ER PT J AU DeGottardi, W AF DeGottardi, Wade TI Topological insulating phases of non-Abelian anyonic chains SO PHYSICAL REVIEW B LA English DT Article ID CONFORMAL-INVARIANCE; CRITICAL-BEHAVIOR; FIELD-THEORY; ISING-MODEL; BOUNDARY; BULK AB Boundary conformal field theory is brought to bear on the study of topological insulating phases of non-Abelian anyonic chains. These phases display protected anyonic end modes. We consider spin-1/2 su(2)(k) chains at any level k, focusing on the most prominent examples: the case k = 2 describes Ising anyons (equivalent to Majorana fermions) and k = 3 corresponds to Fibonacci anyons. The method we develop is quite general and rests on a deep connection between boundary conformal field theory and topological symmetry. This method tightly constrains the nature of the topological insulating phases of these chains for general k. Emergent anyons which arise at domain walls are shown to have the same braiding properties as the physical quasiparticles. This suggests a "solid-state" topological quantum computation scheme in which emergent anyons are braided by tuning the couplings of non-Abelian quasiparticles in a fixed network. C1 Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP DeGottardi, W (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. FU US Department of Energy, Office of Science, Materials Sciences and Engineering Division FX The work was supported by the US Department of Energy, Office of Science, Materials Sciences and Engineering Division. I would like to thank Diptiman Sen, Smitha Vishveshwara, Konstantin Matveev, Brian Skinner, and Ivar Martin for their insightful comments and suggestions. NR 39 TC 1 Z9 1 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 18 PY 2014 VL 90 IS 7 AR 075129 DI 10.1103/PhysRevB.90.075129 PG 8 WC Physics, Condensed Matter SC Physics GA AO3WU UT WOS:000341268600001 ER PT J AU Kim, J Kim, K Kang, CJ Kim, S Choi, HC Kang, JS Denlinger, JD Min, BI AF Kim, Junwon Kim, Kyoo Kang, Chang-Jong Kim, Sooran Choi, Hong Chul Kang, J. -S. Denlinger, J. D. Min, B. I. TI Termination-dependent surface in-gap states in a potential mixed-valent topological insulator: SmB6 SO PHYSICAL REVIEW B LA English DT Article AB We have investigated the surface states of a potential mixed-valent topological insulator SmB6 based on first-principles density functional theory slab band structure analysis. We have found that metallic surface states are formed in the bulk band gap region, providing evidence for the topological insulating nature of SmB6. The obtained surface in-gap states are quite different from those in existing reports in that they are formed differently depending on the Sm or B-6 surface termination, and are composed of mainly the Sm 4f state indicating the essentiality of including f electrons in describing the surface states. We have obtained the spin chiral structures of the Fermi surfaces, which are also in accordance with the topological insulating nature of SmB6. C1 [Kim, Junwon; Kim, Kyoo; Kang, Chang-Jong; Kim, Sooran; Choi, Hong Chul; Min, B. I.] Pohang Univ Sci & Technol, PCTP, Dept Phys, Pohang 790784, South Korea. [Kang, J. -S.] Catholic Univ Korea, Dept Phys, Puchon 420743, South Korea. [Denlinger, J. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Kim, J (reprint author), Pohang Univ Sci & Technol, PCTP, Dept Phys, Pohang 790784, South Korea. EM bimin@postech.ac.kr OI Kim, Kyoo/0000-0002-7305-8786 FU NRF [2009-0079947, 2011-0025237, 2011-0022444]; POSTECH BSRI grant; KISTI supercomputing center [KSC-2012-C3-055]; U.S. DOE [DE-AC02-05CH11231] FX We would like to thank Jinwoong Kim and J. H. Shim for helpful discussions. This work was supported by the NRF (Grants No. 2009-0079947 and No. 2011-0025237), a POSTECH BSRI grant, and the KISTI supercomputing center (Grant No. KSC-2012-C3-055). J. S. K. acknowledges support by the NRF (Grant No. 2011-0022444). J. D. D. is supported by the U.S. DOE (Grant No. DE-AC02-05CH11231). NR 28 TC 13 Z9 13 U1 2 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 18 PY 2014 VL 90 IS 7 AR 075131 DI 10.1103/PhysRevB.90.075131 PG 6 WC Physics, Condensed Matter SC Physics GA AO3WU UT WOS:000341268600003 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, TDR Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CDO De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA 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CA CMS Collaborat TI Measurement of jet fragmentation in PbPb and pp collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW C LA English DT Article ID ENERGY AB The jet fragmentation function of inclusive jets with transverse momentum p(T) above 100 GeV/c in PbPb collisions has been measured using reconstructed charged particles with p(T) above 1 GeV/c in a cone of radius 0.3 around the jet axis. A data sample of PbPb collisions collected in 2011 at a nucleon-nucleon center-of-mass energy of root s(NN) = 2.76 TeV corresponding to an integrated luminosity of 150 mu b(-1) is used. The results for PbPb collisions as a function of collision centrality and jet transverse momentum are compared to reference distributions based on pp data collected at the same center-of-mass energy in 2013, with an integrated luminosity of 5.3 pb(-1). A centrality-dependent modification of the fragmentation function is found. 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[Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Biasotto, M.; Bisello, D.; Branca, A.; Checchia, P.; Dorigo, T.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Sgaravatto, M.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. 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Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Fantasia, C.; Heister, A.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sakharov, A.; Sarangi, T.; Savin, A.; Smith, W. H.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Buontempo, S.] Vienna Univ Technol, Vienna, Austria. [Giammanco, A.] NICPB, Tallinn, Estonia. [Chinellato, J.; Tonelli Manganote, E. 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Montanari, Alessandro/J-2420-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Russ, James/P-3092-2014 OI Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Tomei, Thiago/0000-0002-1809-5226; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Gallinaro, Michele/0000-0003-1261-2277; Sogut, Kenan/0000-0002-9682-2855; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Korenkov, Vladimir/0000-0002-2342-7862; Giubilato, Piero/0000-0003-4358-5355; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Codispoti, Giuseppe/0000-0003-0217-7021; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Benussi, Luigi/0000-0002-2363-8889; Calvo Alamillo, Enrique/0000-0002-1100-2963; Montanari, Alessandro/0000-0003-2748-6373; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Russ, James/0000-0001-9856-9155 FU Austrian Federal Ministry of Science, Research, and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian funding agency CNPq; Brazilian funding agency CAPES; Brazilian funding agency FAPERJ; Brazilian funding agency FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian funding agency COLCIENCIAS; Croatian Ministry of Science, Education and Sport and the Croatian Science Foundation; Research Promotion Foundation; Ministry of Education and Research, Estonian Research Council, Cyprus [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland, Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation and National Innovation Office, Hungary; Department of Atomic Energy and the Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran;; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education and University of Malaya (Malaysia); Mexican funding agency CINVESTAV the Ministry of Business, Innovation and Employment, New Zealand; Mexican funding agency, CONACYT the Ministry of Business, Innovation and Employment, New Zealand; Mexican funding agency, SEP the Ministry of Business, Innovation and Employment, New Zealand; Mexican funding agency, UASLP-FAI the Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education and the National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss funding agency ETH Board; Swiss funding agency, ETH Zurich; Swiss funding agency, PSI; Swiss funding agency, SNF; Swiss funding agency, UniZH; Swiss funding agency, Canton Zurich; Swiss funding agency, SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme and the European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formationa la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science - European Union, Regional Development Fund; Compagnia di San Paolo (Torino); EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research, and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique and Fonds voor Wetenschappelijk Onderzoek; the Brazilian funding agencies CNPq, CAPES, FAPERJ, and FAPESP; the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian funding agency COLCIENCIAS; the Croatian Ministry of Science, Education and Sport and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education and University of Malaya (Malaysia); the Mexican funding agencies CINVESTAV, CONACYT, SEP, and UASLP-FAI) the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss funding agencies ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER; the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, and the Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey and the Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine and the State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; and the US Department of Energy and the US National Science Foundation. Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formationa la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of Foundation for Polish Science, cofinanced by the European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 35 TC 24 Z9 24 U1 7 U2 76 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 18 PY 2014 VL 90 IS 2 AR 024908 DI 10.1103/PhysRevC.90.024908 PG 20 WC Physics, Nuclear SC Physics GA AO3XT UT WOS:000341271300005 ER PT J AU Luo, Y Fischer, W Blaskiewicz, M Brennan, JM Kling, N Mernick, K Roser, T AF Luo, Y. Fischer, W. Blaskiewicz, M. Brennan, J. M. Kling, N. Mernick, K. Roser, T. TI Burn-off dominated uranium and asymmetric copper-gold operation in RHIC SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB In 2012 the Relativistic Heavy Ion Collider collided uranium-uranium ions with a particle energy of 96.4 GeV/nucleon and copper-gold (Cu-Au) ions at 100 GeV/nucleon for the first time. 3-dimensional stochastic cooling became operational for the first time and greatly enhanced the luminosity. Together with a new lattice configuration, we achieved a burn-off dominated uranium beam lifetime at physics stores. In the asymmetric Cu-Au collision, we observed an increased Cu beam loss stemming from different intrabeam-scattering and cooling rates between the Au and Cu ion bunches. By intentionally slowing down the cooling rate for the Au beam at the beginning of store, we reduced the Cu beam loss and maximized the integrated luminosity. C1 [Luo, Y.; Fischer, W.; Blaskiewicz, M.; Brennan, J. M.; Kling, N.; Mernick, K.; Roser, T.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Luo, Y (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM yluo@bnl.gov NR 51 TC 3 Z9 2 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD AUG 18 PY 2014 VL 17 IS 8 AR 081003 DI 10.1103/PhysRevSTAB.17.081003 PG 15 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AO4GE UT WOS:000341293500002 ER PT J AU Kistler, JD Chotigkrai, N Xu, PH Enderle, B Praserthdam, P Chen, CY Browning, ND Gates, BC AF Kistler, Joseph D. Chotigkrai, Nutchapon Xu, Pinghong Enderle, Bryan Praserthdam, Piyasan Chen, Cong-Yan Browning, Nigel D. Gates, Bruce C. TI A Single-Site Platinum CO Oxidation Catalyst in Zeolite KLTL: Microscopic and Spectroscopic Determination of the Locations of the Platinum Atoms SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE electron microscopy; EXAFS; platinum; single-site catalysts; zeolites ID ALKALI-METAL; NAX; DECOMPOSITION; TEMPERATURES; PARTICLES; LIGANDS; CATIONS; COMPLEX; AMMONIA AB A stable site-isolated mononuclear platinum catalyst with a well-defined structure is presented. Platinum complexes supported in zeolite KLTL were synthesized from [Pt(NH3)(4)](NO3)(2), oxidized at 633 K, and used to catalyze CO oxidation. IR and X-ray absorption spectra and electron micrographs determine the structures and locations of the platinum complexes in the zeolite pores, demonstrate the platinum-support bonding, and show that the platinum remained site isolated after oxidation and catalysis. C1 [Kistler, Joseph D.; Chotigkrai, Nutchapon; Xu, Pinghong; Enderle, Bryan; Chen, Cong-Yan; Gates, Bruce C.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Chen, Cong-Yan] Chevron Energy Technol Co, Richmond, CA 94802 USA. [Browning, Nigel D.] Pacific Northwest Natl Lab, Fundamental & Computat Sci Div, Richland, WA 99352 USA. [Chotigkrai, Nutchapon; Praserthdam, Piyasan] Chulalongkorn Univ, Dept Chem Engn, Ctr Excellence Catalysis & Catalyt React Engn, Bangkok, Thailand. RP Gates, BC (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, One Shields Ave, Davis, CA 95616 USA. EM bcgates@ucdavis.edu OI Browning, Nigel/0000-0003-0491-251X FU Department of Energy (DOE) Basic Energy Science [FG02-04ER15513, DE-SC0005822]; Royal Golden Jubilee PhD program of the Thailand research fund; DOE, Office of Science, Basic Energy Sciences [DE-AC02-76SF00515]; Laboratory Directed Research and Development Program Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL); Environmental Molecular Sciences Laboratory; DOE's Office of Biological and Environmental Research at PNNL; DOE [DE-AC05-76L01830] FX This work was supported by the Department of Energy (DOE) Basic Energy Science Grants FG02-04ER15513 and DE-SC0005822 and the Royal Golden Jubilee PhD program of the Thailand research fund. We acknowledge beam time and support of beamline 4-1 at the Stanford Synchrotron Radiation Lightsource (SSRL), supported by DOE, Office of Science, Basic Energy Sciences, Contract DE-AC02-76SF00515. We acknowledge support through the Laboratory Directed Research and Development Program Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL) and the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research at PNNL. PNNL is a multiprogram national laboratory operated by Battelle for DOE under Contract DE-AC05-76L01830. NR 23 TC 28 Z9 28 U1 34 U2 189 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 18 PY 2014 VL 53 IS 34 BP 8904 EP 8907 DI 10.1002/anie.201403353 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AN3ZC UT WOS:000340526400011 PM 24986134 ER PT J AU Yang, ZQ Yin, LC Lee, J Ren, WC Cheng, HM Ye, HQ Pantelides, ST Pennycook, SJ Chisholm, MF AF Yang, Zhiqing Yin, Lichang Lee, Jaekwang Ren, Wencai Cheng, Hui-Ming Ye, Hengqiang Pantelides, Sokrates T. Pennycook, Stephen J. Chisholm, Matthew F. TI Direct Observation of Atomic Dynamics and Silicon Doping at a Topological Defect in Graphene SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE density functional calculations; doping; electron microscopy; graphene; silicon ID SINGLE-MOLECULE; GROWTH; STABILITY; MEMBRANES; FILMS; MOTOR; GAS AB Chemical decoration of defects is an effective way to functionalize graphene and to study mechanisms of their interaction with environment. We monitored dynamic atomic processes during the formation of a rotary Si trimer in monolayer graphene using an aberration-corrected scanning-transmission electron microscope. An incoming Si atom competed with and replaced a metastable C dimer next to a pair of Si substitutional atoms at a topological defect in graphene, producing a Si trimer. Other atomic events including removal of single C atoms, incorporation and relocation of a C dimer, reversible C C bond rotation, and vibration of Si atoms occurred before the final formation of the Si trimer. Theoretical calculations indicate that it requires 2.0 eV to rotate the Si trimer. Our real-time results provide insight with atomic precision for reaction dynamics during chemical doping at defects in graphene, which have implications for defect nanoengineering of graphene. C1 [Yang, Zhiqing; Yin, Lichang; Ren, Wencai; Cheng, Hui-Ming; Ye, Hengqiang] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China. [Lee, Jaekwang; Chisholm, Matthew F.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Pantelides, Sokrates T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Pennycook, Stephen J.; Chisholm, Matthew F.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Yang, ZQ (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China. EM yangzq@imr.ac.cn; chisholmmf@ornl.gov RI Yang, Zhiqing/E-5188-2011; Cheng, Hui-Ming/B-8682-2012 OI Yang, Zhiqing/0000-0003-2017-6583; FU U.S. Department of Energy, Basic Energy Science, Materials Science and Engineering Division, a ShaRE User program; DOE-BES, NSF of China [51171189, 51172240, 51221264, 51290273, 51371178, 51390473, 51325205]; MoST [2012AA030303]; CAS [KGZD-EW-303-1] FX Z.Q.Y. and M.F.C. conceived the study. Z.Q.Y. performed experiments and wrote the manuscript. J.L. and L.C.Y. performed density functional calculations. W.C.R. and H.M.C. prepared graphene samples. This research was supported by the U.S. Department of Energy, Basic Energy Science, Materials Science and Engineering Division, a ShaRE User program sponsored by DOE-BES, NSF of China (51171189, 51172240, 51221264, 51290273, 51371178, 51390473, 51325205), MoST 2012AA030303, and CAS (KGZD-EW-303-1, Shenyang Supercomputing Center). NR 41 TC 7 Z9 7 U1 5 U2 100 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 18 PY 2014 VL 53 IS 34 BP 8908 EP 8912 DI 10.1002/anie.201403382 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA AN3ZC UT WOS:000340526400012 PM 24981312 ER PT J AU Yu, HJ Ren, Y Xiao, DD Guo, SH Zhu, YB Qian, YM Gu, L Zhou, HS AF Yu, Haijun Ren, Yang Xiao, Dongdong Guo, Shaohua Zhu, Yanbei Qian, Yumin Gu, Lin Zhou, Haoshen TI An Ultrastable Anode for Long-Life Room-Temperature Sodium-Ion Batteries SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE anode materials; electrochemistry; sodium-ion batteries; sodium storage ID CATHODE MATERIAL; ENERGY-STORAGE; ELECTROCHEMICAL NA; CYCLE LIFE; LOW-COST; INTERCALATION; STABILITY; COMPOSITE; INSERTION; ELECTRODE AB Sodium-ion batteries are important alternative energy storage devices that have recently come again into focus for the development of large-scale energy storage devices because sodium is an abundant and low-cost material. However, the development of electrode materials with long-term stability has remained a great challenge. A novel negative-electrode material, a P2-type layered oxide with the chemical composition Na2/3Co1/3Ti2/3O2, exhibits outstanding cycle stability (ca. 84.84 % capacity retention for 3000 cycles, very small decrease in the volume (0.046 %) after 500 cycles), good rate capability (ca. 41 % capacity retention at a discharge/charge rate of 10 C), and a usable reversible capacity of about 90 mAh g(-1) with a safe average storage voltage of approximately 0.7 V in the sodium half-cell. This P2-type layered oxide is a promising anode material for sodium-ion batteries with a long cycle life and should greatly promote the development of room-temperature sodium-ion batteries. C1 [Yu, Haijun; Guo, Shaohua; Qian, Yumin; Zhou, Haoshen] Natl Inst Adv Ind Sci & Technol, Energy Technol Res Inst, Tsukuba, Ibaraki 3058568, Japan. [Zhou, Haoshen] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Zhou, Haoshen] Nanjing Univ, Dept Energy Sci & Engn, Nanjing 210093, Jiangsu, Peoples R China. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Xiao, Dongdong; Gu, Lin] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Zhu, Yanbei] Natl Inst Adv Ind Sci & Technol, Natl Metrol Inst Japan, Tsukuba, Ibaraki 3058568, Japan. RP Gu, L (reprint author), Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. EM l.gu@iphy.ac.cn; hs.zhou@aist.go.jp RI Yu, Haijun/J-4981-2014; Gu, Lin/D-9631-2011; 郭, 少华/R-8504-2016 OI Yu, Haijun/0000-0003-0204-9943; Gu, Lin/0000-0002-7504-031X; 郭, 少华/0000-0003-0818-8354 FU Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST Program); U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was partially supported by the Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST Program). We thank Dr. Matthew Suchomel for help with the high. resolution synchrotron powder diffraction measurements, and Dr. Zhiping Song for help with the cover picture design. The use of the Advanced Photon Source at Argonne National Laboratory was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DE-AC02-06CH11357). NR 38 TC 40 Z9 40 U1 27 U2 285 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 18 PY 2014 VL 53 IS 34 BP 8963 EP 8969 DI 10.1002/anie.201404549 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA AN3ZC UT WOS:000340526400023 PM 24962822 ER PT J AU Cheng, HC Dobrescu, BA Gu, JY AF Cheng, Hsin-Chia Dobrescu, Bogdan A. Gu, Jiayin TI Higgs mass from compositeness at a multi-TeV scale SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; Beyond Standard Model; Technicolor and Composite Models ID ELECTROWEAK SYMMETRY-BREAKING; TOP-QUARK MASS; GROUP FIXED-POINTS; STANDARD MODEL; VACUUM MISALIGNMENT; GAUGE-THEORIES; BOSON; FLAVOR; PHENOMENOLOGY; LHC AB Within composite Higgs models based on the top seesaw mechanism, we show that the Higgs field can arise as the pseudo Nambu-Goldstone boson of the broken U( 3) L chiral symmetry associated with a vector-like quark and the t-b doublet. As a result, the lightest CP-even neutral state of the composite scalar sector is lighter than the top quark, and can be identified as the newly discovered Higgs boson. Constraints on weak-isospin violation push the chiral symmetry breaking scale above a few TeV, implying that other composite scalars are probably too heavy to be probed at the LHC, but may be within reach at a future hadron collider with center-of-mass energy of about 100TeV. C1 [Cheng, Hsin-Chia; Gu, Jiayin] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Dobrescu, Bogdan A.] Fermilab Natl Accelerator Lab, Div Theoret Phys, Batavia, IL 60510 USA. RP Cheng, HC (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. EM cheng@physics.ucdavis.edu; bdob@fnal.gov; jjjgu@ucdavis.edu FU Department of Energy (DOE) [DE-FG02-91ER40674]; DOE [De-AC02-07CH11359] FX We would like to thank Sekhar Chivukula, Markus Luty and John Terning for useful discussions. H.-C. Cheng and J. Gu are supported by the Department of Energy (DOE) under contract no. DE-FG02-91ER40674. Fermilab is operated by the Fermi Research Alliance under Contract No. De-AC02-07CH11359 with the DOE. H.-C. Cheng would like to acknowledge the hospitality of National Center for Theoretical Sciences (North) in Taiwan where part of this work was done. NR 66 TC 8 Z9 8 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 18 PY 2014 IS 8 AR 095 DI 10.1007/JHEP08(2014)095 PG 26 WC Physics, Particles & Fields SC Physics GA AN3RI UT WOS:000340505800004 ER PT J AU Lu, XC Murayama, H AF Lu, Xiaochuan Murayama, Hitoshi TI Neutrino mass anarchy and the Universe SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM; Neutrino Physics; Statistical Methods ID LEPTOGENESIS; BARYOGENESIS; OSCILLATIONS; TEXTURES AB We study the consequence of the neutrino mass anarchy on cosmology, in particular the total mass of neutrinos and baryon asymmetry through leptogenesis. We require independence of measure in each mass matrix elements in addition to the basis independence, which uniquely picks the Gaussian measure. A simple approximate U(1) flavor symmetry makes leptogenesis highly successful. Correlations between the baryon asymmetry and the light-neutrino quantities are investigated. We also discuss possible implications of recently suggested large total mass of neutrinos by the SDSS/BOSS data. C1 [Lu, Xiaochuan; Murayama, Hitoshi] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lu, Xiaochuan; Murayama, Hitoshi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Murayama, Hitoshi] Univ Tokyo, Kovli Inst Phys & Math Universe WPI, Todai Inst Adv Study, Kashiwa, Chiba 2778583, Japan. RP Lu, XC (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM luxiaochuan123456@berkeley.edu; hitoshi@berkeley.edu OI Lu, Xiaochuan/0000-0001-8821-2574 FU U.S. DOE [DE-AC02-05CH11231]; NSF [PHY-1002399, PHY-1316783]; JSPS [26400241, 26105507]; WPI, MEXT, Japan FX This work was supported by the U.S. DOE under Contract DE-AC02-05CH11231, and by the NSF under grants PHY-1002399 and PHY-1316783. HM was also supported by the JSPS Grant-in-Aid for Scientific Research (C) (No. 26400241), Scientific Research on Innovative Areas (No. 26105507), and by WPI, MEXT, Japan. NR 38 TC 4 Z9 4 U1 1 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. 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CA ATLAS Collaboration TI Search for microscopic black holes and string balls in final states with leptons and jets with the ATLAS detector at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID DIMENSIONS; MILLIMETER; COLLISIONS; HIERARCHY; LHC AB A search for an excess of events with multiple high transverse momentum objects including charged leptons and jets is presented, using 20.3 fb(-1) of proton-proton collision data recorded by the ATLAS detector at the Large Hadron Collider in 2012 at a centre-of-mass energy of root s = 8 TeV. No excess of events beyond Standard Model expectations is observed. Using extra-dimensional models for black hole and string ball production and decay, exclusion contours are determined as a function of the mass threshold for production and the fundamental gravity scale for two, four and six extra dimensions. For six extra dimensions, mass thresholds of 4.8-6.2 TeV are excluded at 95 % confidence level, depending on the fundamental gravity scale and model assumptions. Upper limits on the fiducial cross-sections for non-Standard Model production of these final states are set. C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Chan, K.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey. 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S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan City, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Blaise Pascal, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand 2, Photochim Mol & Macromol Lab, CNRS, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN Grp Collegato Cosenza, Lab Nazl Frascati, I-87036 Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Bruckman de Renstrom, P. A.; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M. F.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M. F.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Moreno Llacer, M.; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimares; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Univ Milan, INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J. -F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C. -L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, INFN Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.; Wolters, H.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Veloso, F.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Univ Roma La Sapienza, INFN Sez Roma, I-00185 Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Univ Roma Tre, INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [Kacimi, M. El; Goujdami, D.; Haddad, N.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Grabas, H. M. X.; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J. -P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Sterzo, F. Lo; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Leisos, A.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; De Sanctis, U.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Lin, S. C.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Castillo, L. R. Flores] Chinese Univ Hong Kong, Hong Kong, Hong Kong, Peoples R China. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Korol, A. A.; Maximov, D. A.; Rezanova, O. L.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Tikhomirov, Vladimir/M-6194-2015; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; De, Kaushik/N-1953-2013; Vanadia, Marco/K-5870-2016; Cavalli-Sforza, Matteo/H-7102-2015; Fabbri, Laura/H-3442-2012; Li, Liang/O-1107-2015; Staroba, Pavel/G-8850-2014; Warburton, Andreas/N-8028-2013; Solfaroli Camillocci, Elena/J-1596-2012; Gabrielli, Alessandro/H-4931-2012; Mitsou, Vasiliki/D-1967-2009; Ippolito, Valerio/L-1435-2016; Di Domenico, Antonio/G-6301-2011; Villa, Mauro/C-9883-2009; Livan, Michele/D-7531-2012; Brooks, William/C-8636-2013; Ferrer, Antonio/H-2942-2015; Maneira, Jose/D-8486-2011; Vykydal, Zdenek/H-6426-2016; Boyko, Igor/J-3659-2013; Gladilin, Leonid/B-5226-2011; Gauzzi, Paolo/D-2615-2009; Garcia, Jose /H-6339-2015; Solodkov, Alexander/B-8623-2017; Moraes, Arthur/F-6478-2010; messina, andrea/C-2753-2013; Cabrera Urban, Susana/H-1376-2015; Petrucci, Fabrizio/G-8348-2012; Tartarelli, Giuseppe Francesco/A-5629-2016; Korol, Aleksandr/A-6244-2014; la rotonda, laura/B-4028-2016; Capua, Marcella/A-8549-2015; Fassi, Farida/F-3571-2016 OI Tikhomirov, Vladimir/0000-0002-9634-0581; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; De, Kaushik/0000-0002-5647-4489; Vanadia, Marco/0000-0003-2684-276X; Fabbri, Laura/0000-0002-4002-8353; Li, Liang/0000-0001-6411-6107; Warburton, Andreas/0000-0002-2298-7315; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Gabrielli, Alessandro/0000-0001-5346-7841; Mitsou, Vasiliki/0000-0002-1533-8886; Ippolito, Valerio/0000-0001-5126-1620; Di Domenico, Antonio/0000-0001-8078-2759; Villa, Mauro/0000-0002-9181-8048; Livan, Michele/0000-0002-5877-0062; Brooks, William/0000-0001-6161-3570; Ferrer, Antonio/0000-0003-0532-711X; Maneira, Jose/0000-0002-3222-2738; Vykydal, Zdenek/0000-0003-2329-0672; Boyko, Igor/0000-0002-3355-4662; Gladilin, Leonid/0000-0001-9422-8636; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Moraes, Arthur/0000-0002-5157-5686; Smestad, Lillian/0000-0002-0244-8736; Giorgi, Filippo Maria/0000-0003-1589-2163; Di Micco, Biagio/0000-0002-4067-1592; Petrucci, Fabrizio/0000-0002-5278-2206; Doria, Alessandra/0000-0002-5381-2649; Osculati, Bianca Maria/0000-0002-7246-060X; Coccaro, Andrea/0000-0003-2368-4559; Giordani, Mario/0000-0002-0792-6039; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Korol, Aleksandr/0000-0001-8448-218X; la rotonda, laura/0000-0002-6780-5829; Capua, Marcella/0000-0002-2443-6525; Fassi, Farida/0000-0002-6423-7213 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES , Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 81 TC 4 Z9 4 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 18 PY 2014 IS 8 AR 103 DI 10.1007/JHEP08(2014)103 PG 48 WC Physics, Particles & Fields SC Physics GA AO1VS UT WOS:000341104200001 ER PT J AU Moss, WC King, MJ Blackman, EG AF Moss, William C. King, Michael J. Blackman, Eric G. TI Towards reducing impact-induced brain injury: lessons from a computational study of army and football helmet pads SO COMPUTER METHODS IN BIOMECHANICS AND BIOMEDICAL ENGINEERING LA English DT Article DE helmet; pad; head injury; traumatic brain injury; head injury criterion; impact AB We use computational simulations to compare the impact response of different football and U. S. Army helmet pad materials. We conduct experiments to characterise the material response of different helmet pads. We simulate experimental helmet impact tests performed by the U. S. Army to validate our methods. We then simulate a cylindrical impactor striking different pads. The acceleration history of the impactor is used to calculate the head injury criterion for each pad. We conduct sensitivity studies exploring the effects of pad composition, geometry and material stiffness. We find that (1) the football pad materials do not outperform the currently used military pad material in militarily relevant impact scenarios; (2) optimal material properties for a pad depend on impact energy and (3) thicker pads perform better at all velocities. Although we considered only the isolated response of pad materials, not entire helmet systems, our analysis suggests that by using larger helmet shells with correspondingly thicker pads, impact-induced traumatic brain injury may be reduced. C1 [Moss, William C.] Lawrence Livermore Natl Lab, Weap & Complex Integrat Directorate, Livermore, CA 94551 USA. [King, Michael J.] Lawrence Livermore Natl Lab, Engn Directorate, Livermore, CA 94551 USA. [Blackman, Eric G.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. RP Moss, WC (reprint author), Lawrence Livermore Natl Lab, Weap & Complex Integrat Directorate, 7000 East Ave,L-99, Livermore, CA 94551 USA. EM wmoss@llnl.gov; king74@llnl.gov; Blackman@pas.rochester.edu FU U.S. Army; U.S. Army and the Joint IED Defeat Organization [JIEDDO] through COL R. Todd Dombroski, DO, JIEDDO Surgeon; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We acknowledge funding from the U.S. Army and the Joint IED Defeat Organization [JIEDDO] through COL R. Todd Dombroski, DO, JIEDDO Surgeon. We thank LLNL staff members B. Cracchiola for loaning us his ACH helmet, D. Urabe for performing the compression tests on the manufacturer supplied pads and component foams and W. Brown for CT scanning the ACH helmet and post-processing the files. We also thank N. Kraemer (Riddell), S. Reynolds (Xenith), R. Szalkowski (Team Wendy) and T. Erickson (Oregon Aero) for supplying pad and foam samples used in this study. We thank the U.S. Army Aeromedical Research Laboratory [USAARL] for providing us data from impact tests on infantry helmets. This study was carried out under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 11 TC 3 Z9 3 U1 2 U2 42 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1025-5842 EI 1476-8259 J9 COMPUT METHOD BIOMEC JI Comput. Methods Biomech. Biomed. Eng. PD AUG 18 PY 2014 VL 17 IS 11 BP 1173 EP 1184 DI 10.1080/10255842.2012.739162 PG 12 WC Computer Science, Interdisciplinary Applications; Engineering, Biomedical SC Computer Science; Engineering GA AE5HO UT WOS:000334018600002 PM 23244512 ER PT J AU Shuster, JR Chen, LJ Daughton, WS Lee, LC Lee, KH Bessho, N Torbert, RB Li, G Argall, MR AF Shuster, J. R. Chen, L. -J. Daughton, W. S. Lee, L. C. Lee, K. H. Bessho, N. Torbert, R. B. Li, G. Argall, M. R. TI Highly structured electron anisotropy in collisionless reconnection exhausts SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE collisionless magnetic reconnection; electron distribution function; electron anisotropy; Cluster observation; reconnection exhaust ID MAGNETIC RECONNECTION; ACCELERATION AB Results from two-dimensional particle-in-cell simulations of collisionless magnetic reconnection with zero guide field discussed in this paper reveal that around the time when the reconnection rate peaks, electron velocity distributions become highly structured in magnetic islands and open exhausts. Rings, arcs, and counterstreaming beams are generic and lasting components of the exhaust electron distributions. The temporal dependence of electron distributions provides a perspective to explain an outstanding discrepancy concerning the degree of electron anisotropy in reconnection exhausts and enables inference of the reconnection phase based on observed anisotropic electron distributions. Some of the structures predicted by our simulations are confirmed by measurements from the Cluster spacecraft during its encounter with reconnection exhausts in the magnetotail. C1 [Shuster, J. R.; Chen, L. -J.; Bessho, N.; Torbert, R. B.; Li, G.; Argall, M. R.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Daughton, W. S.] Los Alamos Natl Lab, Los Alamos, NM USA. [Lee, L. C.; Lee, K. H.] Acad Sinica, Inst Earth Sci, Taipei 115, Taiwan. RP Shuster, JR (reprint author), Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. EM jrf63@wildcats.unh.edu RI Lee, Lou-Chuang/I-2588-2013; Daughton, William/L-9661-2013; NASA MMS, Science Team/J-5393-2013 OI Lee, Lou-Chuang/0000-0003-4012-991X; NASA MMS, Science Team/0000-0002-9504-5214 FU NSF [PHY-0903923, AGS-1202537]; NASA [NNX11AH03G]; NASA's Heliophysics Theory Program; National Science Council, Taiwan FX The work at UNH was supported in part by NSF grants PHY-0903923 and AGS-1202537 and NASA grant NNX11AH03G. The contribution from W. Daughton was supported by NASA's Heliophysics Theory Program. Contributions from L. Lee and K.-H. Lee were supported by the National Science Council, Taiwan. The simulation data are available upon request from the authors, and the spacecraft data are available at the Cluster Active Archive website. NR 17 TC 11 Z9 11 U1 3 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2014 VL 41 IS 15 BP 5389 EP 5395 DI 10.1002/2014GL060608 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AP0BI UT WOS:000341725200010 ER PT J AU Ripoll, JF Zinn, J Jeffery, CA Colestock, PL AF Ripoll, Jean-Francois Zinn, John Jeffery, Christopher A. Colestock, Patrick L. TI On the dynamics of hot air plasmas related to lightning discharges: 1. Gas dynamics SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID COLLISION CROSS SECTIONS; NITRIC-OXIDE PRODUCTION; II FLIGHT EXPERIMENT; RETURN STROKES; TRANSPORT COEFFICIENTS; NUMERICAL-CALCULATION; OPTICAL RADIATION; ATMOSPHERIC-PRESSURE; ENERGY-DISSIPATION; NITROGEN-OXIDES AB In this paper, we first study the dynamics of hot shocks in air in cylindrical geometry coupled to multiband radiation transport and detailed air chemistry. The wide energy and length scale ranges which are covered herein includes and exceeds the ones of first and subsequent return strokes happening during lightning discharges. An emphasis is put on the NOx production and the optical power emitted by strong shocks as the ones generated by Joule heating of the air from intense current flows. The production rate of NOx, which is useful for atmospheric global modeling, is found to be between 4.5 x 10(16) and 8.6 x 10(16) molecules/J for all computed cases, which is in agreement with the literature. Two different radiation transport methods are used to characterize the variability of the results according to the radiation transport method. With the exact radiation solver, we show that between 15 and 40% of the energy is lost by radiation, with a percentage between 20 and 25% for averaged lightning energies. The maximal visible peak is between 7 x 10(8) W/m and 3 x 10(7) W/m obtained for, respectively, a 19 kJ/cm and a 28 J/cm energy input. The mean radiated powers in the visible range are found between 9 x 10(6) W/m and 2 x 10(5) W/m for the energies just mentioned. We discuss the agreement of these values with previous studies. C1 [Ripoll, Jean-Francois; Zinn, John; Jeffery, Christopher A.; Colestock, Patrick L.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Ripoll, JF (reprint author), CEA, DAM, DIF, Arpajon, France. EM jean-francois.ripoll@cea.fr NR 98 TC 5 Z9 5 U1 1 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 16 PY 2014 VL 119 IS 15 BP 9196 EP 9217 DI 10.1002/2013JD020067 PG 22 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AO2ZK UT WOS:000341197400002 ER PT J AU Ripoll, JF Zinn, J Colestock, PL Jeffery, CA AF Ripoll, Jean-Francois Zinn, John Colestock, Patrick L. Jeffery, Christopher A. TI On the dynamics of hot air plasmas related to lightning discharges: 2. Electrodynamics SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID COLLISION CROSS SECTIONS; RETURN STROKES; TRANSPORT COEFFICIENTS; NUMERICAL-CALCULATION; ENERGY-DISSIPATION; OPTICAL RADIATION; DART LEADERS; PEAK CURRENT; SHOCK-WAVES; SATELLITE AB In this paper, we develop a model of electrical discharge in air for the simulation of some of the electrical processes involved in lightning discharges, as in lightning return strokes and dart leaders. The discharge is initiated by a vertical electrical field and modeled using a nonlinear R-L-C circuit model, with which we attempt to simulate initiation, growth, radial expansion, and decay of electrical discharges related to lightning. This gas dynamic type model includes also both detailed air chemistry and accurate air radiation transport, as described in the first part of this article. For certain parameter configurations, our first lightning-related discharge simulations compare well with lightning observations and actual knowledge in terms of chronology, charge and energy depleted, current created, electron concentration, temperature, pressure, and optical signature. We also discuss the difficulties to obtain fully consistent results due to the wide parameter variability, their uncertainty, and the complexity of the physics involved. C1 [Ripoll, Jean-Francois; Zinn, John; Colestock, Patrick L.; Jeffery, Christopher A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ripoll, Jean-Francois] CEA, DAM, DIF, Arpajon, France. RP Ripoll, JF (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM jean-francois.ripoll@cea.fr NR 67 TC 6 Z9 6 U1 0 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 16 PY 2014 VL 119 IS 15 BP 9218 EP 9235 DI 10.1002/2013JD020068 PG 18 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AO2ZK UT WOS:000341197400003 ER PT J AU Collow, TW Robock, A Wu, W AF Collow, Thomas W. Robock, Alan Wu, Wei TI Influences of soil moisture and vegetation on convective precipitation forecasts over the United States Great Plains SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID LAND-COVER DATA; EQUIVALENT TEMPERATURE; DEEP CONVECTION; NORTH-AMERICA; ETA-MODEL; MESOSCALE; IMPACT; SATELLITE; SIMULATIONS; SENSITIVITY AB This study investigates the influences of soil moisture and vegetation on 30 h convective precipitation forecasts using the Weather Research and Forecasting model over the United States Great Plains with explicit treatment of convection. North American Regional Reanalysis (NARR) data were used as initial and boundary conditions. We also used an adjusted soil moisture (uniformly adding 0.10 m(3)/m(3) over all soil layers based on NARR biases) to determine whether using a simple observationally based adjustment of soil moisture forcing would provide more accurate simulations and how the soil moisture addition would impact meteorological parameters for different vegetation types. Current and extreme (forest and barren) land covers were examined. Compared to the current vegetation cover, the complete removal of vegetation produced substantially less precipitation, while conversion to forest led to small differences in precipitation. Adding 0.10 m(3)/m(3) to the soil moisture with the current vegetation cover lowered the near surface temperature and increased the humidity to a similar degree as using a fully forested domain with no soil moisture adjustment. However, these temperature and humidity effects on convective available potential energy and moist enthalpy nearly canceled each other out, resulting in a limited precipitation response. Although no substantial changes in precipitation forecasts were found using the adjusted soil moisture, the similarity found between temperature and humidity forecasts using the increased soil moisture and those with a forested domain highlights the sensitivity of the model to soil moisture changes, reinforcing the need for accurate soil moisture initialization in numerical weather forecasting models. C1 [Collow, Thomas W.; Robock, Alan] Rutgers State Univ, Dept Environm Sci, New Brunswick, NJ 08903 USA. [Wu, Wei] Brookhaven Natl Lab, Environm & Climate Sci Dept, Upton, NY 11973 USA. RP Collow, TW (reprint author), INNOVIM LLC, NOAA NWS NCEP Climate Predict Ctr, College Pk, MD USA. EM tcollow@envsci.rutgers.edu RI Robock, Alan/B-6385-2016 FU NASA [NNX09AJ99G]; Brookhaven National Laboratory (BNL) Laboratory Directed Research and Development Program; National Science Foundation FX This work has been supported by NASA grant NNX09AJ99G and the Brookhaven National Laboratory (BNL) Laboratory Directed Research and Development Program. Calculations were performed at the NCAR Wyoming Supercomputing Center, which is supported by the National Science Foundation. NARR data used in this study are available for download at http://rda.ucar.edu/datasets/ds608.0/. We thank Martin Schoonen (BNL) and Peter Daum (BNL) for carefully reading and editing this manuscript, Benjamin Lintner (Rutgers University) for his valuable suggestions on the analysis, and Jeffrey Basara from the University of Oklahoma for providing us with the Oklahoma Mesonet soil moisture data. We finally thank four anonymous reviewers for their feedback on earlier versions of this manuscript. NR 68 TC 4 Z9 5 U1 0 U2 21 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 16 PY 2014 VL 119 IS 15 BP 9338 EP 9358 DI 10.1002/2014JD021454 PG 21 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AO2ZK UT WOS:000341197400010 ER PT J AU Linville, JL Rodriguez, M Brown, SD Mielenz, JR Cox, CD AF Linville, Jessica L. Rodriguez, Miguel, Jr. Brown, Steven D. Mielenz, Jonathan R. Cox, Chris D. TI Transcriptomic analysis of Clostridium thermocellum Populus hydrolysate-tolerant mutant strain shows increased cellular efficiency in response to Populus hydrolysate compared to the wild type strain SO BMC MICROBIOLOGY LA English DT Article DE Clostridium thermocellum; Populus hydrolysate; Inhibitor tolerance; Gene expression; Transcriptomic; RNA-seq; Consolidated bioprocessing ID ACIDOGENIC CHEMOSTAT CELLS; BEIJERINCKII NCIMB 8052; BACILLUS-SUBTILIS; ATCC 27405; RNA-SEQ; SACCHAROMYCES-CEREVISIAE; N-BUTANOL; ACETOBUTYLICUM; FERMENTATION; STRESS AB Background: The thermophilic, anaerobic bacterium, Clostridium thermocellum is a model organism for consolidated processing due to its efficient fermentation of cellulose. Constituents of dilute acid pretreatment hydrolysate are known to inhibit C. thermocellum and other microorganisms. To evaluate the biological impact of this type of hydrolysate, a transcriptomic analysis of growth in hydrolysate-containing medium was conducted on 17.5% v/v Populus hydrolysate-tolerant mutant (PM) and wild type (WT) strains of C. thermocellum. Results: In two levels of Populus hydrolysate medium (0% and 10% v/v), the PM showed both gene specific increases and decreases of gene expression compared to the wild-type strain. The PM had increased expression of genes in energy production and conversion, and amino acid transport and metabolism in both standard and 10% v/v Populus hydrolysate media. In particular, expression of the histidine metabolism increased up to 100 fold. In contrast, the PM decreased gene expression in cell division and sporulation (standard medium only), cell defense mechanisms, cell envelope, cell motility, and cellulosome in both media. The PM downregulated inorganic ion transport and metabolism in standard medium but upregulated it in the hydrolysate media when compared to the WT. The WT differentially expressed 1072 genes in response to the hydrolysate medium which included increased transcription of cell defense mechanisms, cell motility, and cellulosome, and decreased expression in cell envelope, amino acid transport and metabolism, inorganic ion transport and metabolism, and lipid metabolism, while the PM only differentially expressed 92 genes. The PM tolerates up to 17.5% v/v Populus hydrolysate and growth in it elicited 489 genes with differential expression, which included increased expression in energy production and conversion, cellulosome production, and inorganic ion transport and metabolism and decreased expression in transcription and cell defense mechanisms. Conclusion: These results suggest the mechanisms of tolerance for the Populus hydrolysate-tolerant mutant strain of C. thermocellum are based on increased cellular efficiency caused apparently by downregulation of non-critical genes and increasing the expression of genes in energy production and conversion rather than tolerance to specific hydrolysate components. The wild type, conversely, responds to hydrolysate media by down-regulating growth genes and up-regulating stress response genes. C1 [Linville, Jessica L.; Cox, Chris D.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Linville, Jessica L.; Rodriguez, Miguel, Jr.; Brown, Steven D.; Mielenz, Jonathan R.; Cox, Chris D.] Oak Ridge Natl Lab, Bioenergy Sci Ctr, Oak Ridge, TN USA. [Rodriguez, Miguel, Jr.; Brown, Steven D.; Mielenz, Jonathan R.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Cox, Chris D.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37932 USA. RP Cox, CD (reprint author), Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. EM ccox9@utk.edu RI Brown, Steven/A-6792-2011 OI Brown, Steven/0000-0002-9281-3898 FU Office of Science [DE-AC02-05CH11231]; BioEnergy Science Center, a Department of Energy Bioenergy Research Center - Office of Biological and Environmental Research in the Department of Energy Office of Science; Institute for a Secure and Sustainable Environment at the University of Tennessee; DOE [DE-AC05-00OR22725] FX The authors thank Dawn M. Klingeman and Courtney M. Johnson for assistance with RNA purification; Dawn M. Klingeman and Charlotte M. Wilson for qPCR and PCR preparation and analysis and Qiang He and Chris Hemme for assistance with transcriptome analysis. RNA-Seq data was generated by the U.S. Department of Energy (DOE) Joint Genome Institute, which is supported by the Office of Science of the under contract no. DE-AC02-05CH11231. This research was supported by the BioEnergy Science Center, a Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the Department of Energy Office of Science. Additional support was provided by the Institute for a Secure and Sustainable Environment at the University of Tennessee. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the DOE under Contract DE-AC05-00OR22725. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 57 TC 2 Z9 2 U1 1 U2 25 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2180 J9 BMC MICROBIOL JI BMC Microbiol. PD AUG 16 PY 2014 VL 14 AR 215 DI 10.1186/s12866-014-0215-5 PG 17 WC Microbiology SC Microbiology GA AO3EK UT WOS:000341211300001 PM 25128475 ER PT J AU Tsai, CL Shi, Y Tainer, JA AF Tsai, Chi-Lin Shi, Yang Tainer, John A. TI How substrate specificity is imposed on a histone demethylase-lessons from KDM2A SO GENES & DEVELOPMENT LA English DT Article DE histone demethylase; KDM2A; mechanism; substrate specificity ID STRUCTURAL BASIS; TRIMETHYLLYSINE; RECOGNITION; JMJD2A; FAMILY AB Histone lysine methylation and demethylation regulate histone methylation dynamics, which impacts chromatin structure and function. To read and erase the methylated histone residues, lysine demethylases must specifically recognize the histone sequences and methylated sites and discriminate the degree of these methylations. In this issue of Genes & Development, Cheng and colleagues (pp. 1758-1771) determine a crystal structure of histone lysine demethylase KDM2A that specifically targets lower degrees of H3K36 methylation. The results reveal the structural basis for H3K36 substrate specificity and suggest mechanisms of Lys36 demethylation. This KDM2A-H3K36 complex structure, coupled with functional studies, provides needed insight into the process and regulation of histone demethylation. C1 [Tsai, Chi-Lin; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Shi, Yang] Harvard Univ, Sch Med, Boston Childrens Hosp, Div Newborn Med, Boston, MA 02115 USA. [Shi, Yang] Harvard Univ, Sch Med, Dept Cell Biol, Boston, MA 02115 USA. [Tainer, John A.] Scripps Res Inst, Skaggs Inst Chem Biol, Dept Integrat Struct & Computat Biol, La Jolla, CA 92037 USA. RP Tainer, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM yang_shi@hms.harvard.edu; jat@scripps.edu OI Tsai, Chi-Lin/0000-0002-0365-2405 FU National Institutes of Health (NIH) [P01 CA092584]; National Cancer Institute [CA118487]; NIH [MH096066] FX C.-L.T.'s and J.A.T.'s efforts are supported in part by National Institutes of Health (NIH) grant P01 CA092584. Research in the Shi laboratory is supported in part by grants from the National Cancer Institute (CA118487) and the NIH (MH096066). Y.S. is an American Cancer Society Research Professor. NR 11 TC 2 Z9 2 U1 0 U2 3 PU COLD SPRING HARBOR LAB PRESS, PUBLICATIONS DEPT PI COLD SPRING HARBOR PA 1 BUNGTOWN RD, COLD SPRING HARBOR, NY 11724 USA SN 0890-9369 EI 1549-5477 J9 GENE DEV JI Genes Dev. PD AUG 15 PY 2014 VL 28 IS 16 BP 1735 EP 1738 DI 10.1101/gad.249755.114 PG 4 WC Cell Biology; Developmental Biology; Genetics & Heredity SC Cell Biology; Developmental Biology; Genetics & Heredity GA AO1KN UT WOS:000341071100001 PM 25128493 ER PT J AU Goetsch, RJ Anand, VK Johnston, DC AF Goetsch, R. J. Anand, V. K. Johnston, D. C. TI Helical antiferromagnetic ordering in Lu1-xScxMnSi SO PHYSICAL REVIEW B LA English DT Article ID DIFFRACTION; CRYSTAL AB Polycrystalline samples of Lu1-xScxMnSi (x = 0, 0.25, 0.5) are studied using powder x-ray diffraction, heat capacity C-p, magnetization, magnetic susceptibility chi, and electrical resistivity rho measurements versus temperature T and magnetic field H. This system crystallizes in the primitive orthorhombic TiNiSi-type structure (space group Pnma) as previously reported. The rho(T) data indicate metallic behavior. The C-p(T), chi(T), and rho(T) measurements consistently indicate long-range antiferromagnetic (AF) transitions with AF ordering temperatures T-N = 246, 215, and 188 K for x = 0, 0.25, and 0.5, respectively. A second transition is observed at somewhat lower T for each sample from the chi(T) and rho(T) measurements, which we speculate are due to spin reorientation transitions; these second transitions are completely suppressed in H = 5.5 T. The C-p data below 10 K for each composition indicate an enhanced Sommerfeld electronic heat capacity coefficient for the series in the range gamma = 24-29 mJ/mol K-2. The chi(T) measurements up to 1000 K were fitted by local-moment Curie-Weiss behaviors which indicate a low Mn spin S similar to 1. The chi data below T-N are analyzed using the Weiss molecular field theory for a planar noncollinear cycloidal AF structure with a composition-dependent pitch, following the previous neutron diffraction work of Venturini et al. [J. Alloys Compd. 256, 65 (1997)]. Within this model, the fits indicate a turn angle between Mn ordered moments along the cycloid axis of similar to 100 degrees or similar to 145 degrees, either of which indicate dominant AF interactions between the Mn spins in the Lu1-xScxMnSi series of compounds. C1 [Goetsch, R. J.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Goetsch, RJ (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM johnston@ameslab.gov RI Anand, Vivek Kumar/J-3381-2013 OI Anand, Vivek Kumar/0000-0003-2023-7040 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Iowa State University [DE-AC02-07CH11358] FX We thank Srinivasa Thimmaiah for measuring the powder XRD pattern for LuMnSi. The work at Ames Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 12 TC 4 Z9 4 U1 4 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 15 PY 2014 VL 90 IS 6 AR 064415 DI 10.1103/PhysRevB.90.064415 PG 11 WC Physics, Condensed Matter SC Physics GA AO3TA UT WOS:000341257600001 ER PT J AU Dai, LY Pennington, MR AF Dai, Ling-Yun Pennington, M. R. TI Comprehensive amplitude analysis of gamma gamma -> pi(+)pi(-),pi(0)pi(0) and (K)over-barK below 1.5 GeV SO PHYSICAL REVIEW D LA English DT Article ID PHOTON-PHOTON COLLISIONS; PI-PI; SCALAR MESONS; LOW-ENERGY; DISPERSION-RELATIONS; 2-PHOTON PRODUCTION; PAIR PRODUCTION; FINAL-STATE; GEV-C; DECAYS AB In this paper we perform an amplitude analysis of essentially all published pion and kaon pair production data from two-photon collisions below 1.5 GeV. This includes all the high statistics results from Belle, as well as older data from Mark II at SLAC, CELLO at DESY, and Crystal Ball at SLAC. The purpose of this analysis is to provide as close to a model-independent determination of the gamma gamma to meson pair amplitudes as possible. Having data with limited angular coverage, typically vertical bar cos theta vertical bar < 0.6-0.8, and no polarization information for reactions in which spin is an essential complication, the determination of the underlying amplitudes might appear an intractable problem. However, imposing the basic constraints required by analyticity, unitarity, and crossing symmetry makes up for the experimentally missing information. Above 1.5 GeV multimeson production channels become important, and we have too little information to resolve the amplitudes. Nevertheless, below 1.5 GeV the two-photon production of hadron pairs serves as a paradigm for the application of S-matrix techniques. Final state interactions among the meson pairs are critical to this analysis. To fix these, we include the latest pi pi -> pi pi, <(K)over bar>K scattering amplitudes given by dispersive analyses, supplemented in the (K) over barK threshold region by the recent precision Dalitz plot analysis from BABAR. With these hadronic amplitudes built into unitarity, we can constrain the overall description of gamma gamma -> pi pi and (K) over barK data sets, both integrated and differential cross sections, including the high statistics charged and neutral pion, as well as KsKs, data from Belle. Since this analysis invokes coupled hadronic channels, having data on both pp and (K) over barK reduces the solution space to essentially a single form in the region where these channels saturate unitarity. For the pi pi channel, the separation of isospin-0 and -2 and helicity-0 and -2 components is complete. We present the partial wave amplitudes, show how well they fit all the available data, and give the two-photon couplings of scalar and tensor resonances that appear. These partial waves are important inputs into forthcoming dispersive calculations of hadronic light-by-light scattering. C1 [Dai, Ling-Yun; Pennington, M. R.] Thomas Jefferson Natl Accelerator Facil, Ctr Theory, Newport News, VA 23606 USA. RP Dai, LY (reprint author), Thomas Jefferson Natl Accelerator Facil, Ctr Theory, Newport News, VA 23606 USA. EM lingyun@jlab.org; michaelp@jlab.org FU Jefferson Science Associates, LLC, under U.S. DOE [DE-AC05-06OR23177] FX M. R. P. thanks Belle colleagues, Yasushi Watanabe and Sadaharu Uehara, for access to the Belle pi0pi0 data and for previous discussions on the systematic uncertainties involved. We would like to thank Han-Qing Zheng and David Wilson for helpful discussions. This paper has been authored by Jefferson Science Associates, LLC, under U.S. DOE Contract No. DE-AC05-06OR23177. NR 100 TC 8 Z9 8 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 15 PY 2014 VL 90 IS 3 AR 036004 DI 10.1103/PhysRevD.90.036004 PG 34 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO3UZ UT WOS:000341263100007 ER PT J AU Bandoro, J Solomon, S Donohoe, A Thompson, DWJ Santer, BD AF Bandoro, Justin Solomon, Susan Donohoe, Aaron Thompson, David W. J. Santer, Benjamin D. TI Influences of the Antarctic Ozone Hole on Southern Hemispheric Summer Climate Change SO JOURNAL OF CLIMATE LA English DT Article ID STRATOSPHERIC POLAR VORTEX; BREWER-DOBSON CIRCULATION; ANNULAR MODE; INTERANNUAL VARIABILITY; ATMOSPHERIC CIRCULATION; DYNAMICAL MECHANISMS; AUSTRALIAN RAINFALL; GLOBAL ENERGY; EL-NINO; TEMPERATURE AB Over the past three decades, Antarctic surface climate has undergone pronounced changes. Many of these changes have been linked to stratospheric ozone depletion. Here linkages between Antarctic ozone loss, the accompanying circulation changes, and summertime Southern Hemisphere (SH) midlatitude surface temperatures are explored. Long-term surface climate changes associated with ozone-driven changes in the southern annular mode (SAM) at SH midlatitudes in summer are not annular in appearance owing to differences in regional circulation and precipitation impacts. Both station and reanalysis data indicate a trend toward cooler summer temperatures over southeast and south-central Australia and inland areas of the southern tip of Africa. It is also found that since the onset of the ozone hole, there have been significant shifts in the distributions of both the seasonal mean and daily maximum-summertime temperatures in the SH midlatitude regions between high and low ozone years. Unusually hot summer extremes are associated with anomalously high ozone in the previous November, including the recent very hot austral summer of 2012/13. If the relationship found in the past three decades continues to hold, the level of late springtime ozone over Antarctica has the potential to be part of a useful predictor set for the following summer's conditions. The results herein suggest that skillful predictions may be feasible for both the mean seasonal temperature and the frequency of extreme hot events in some SH midlatitude regions of Australia, Africa, and South America. C1 [Bandoro, Justin; Solomon, Susan; Donohoe, Aaron] MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA 02139 USA. [Thompson, David W. J.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Santer, Benjamin D.] Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA USA. RP Bandoro, J (reprint author), MIT, Dept Earth Atmospher & Planetary Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM jbandoro@mit.edu RI Thompson, David/F-9627-2012; Santer, Benjamin/F-9781-2011 FU NSF FESD project on the impact of the ozone hole on the Southern Hemisphere climate; NSERC postgraduate scholarship FX We would like to acknowledge and thank the following centers and agencies for access to and use of their datasets in this study: the NASA Global Modeling and Assimilation Office (GMAO), the European Centre for Medium-Range Weather Forecasts (ECMWF), the Scientific Committee on Antarctic Research (SCAR), the National Climatic Data Center (NCDC), the Met Office Hadley Centre, the Australian Bureau of Meteorology, and the Global Energy and Water Exchanges Project. JB and SS obtained partial support from an NSF FESD project on the impact of the ozone hole on the Southern Hemisphere climate and an NSERC postgraduate scholarship. NR 105 TC 4 Z9 4 U1 6 U2 46 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD AUG 15 PY 2014 VL 27 IS 16 BP 6245 EP 6264 DI 10.1175/JCLI-D-13-00698.1 PG 20 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AN0YV UT WOS:000340310800009 ER PT J AU Maloney, ED Jiang, XA Xie, SP Benedict, JJ AF Maloney, Eric D. Jiang, Xianan Xie, Shang-Ping Benedict, James J. TI Process-Oriented Diagnosis of East Pacific Warm Pool Intraseasonal Variability SO JOURNAL OF CLIMATE LA English DT Article ID MADDEN-JULIAN OSCILLATION; MOIST STATIC ENERGY; TEMPERATURE-GRADIENT APPROXIMATION; BOREAL SUMMER; TROPICAL CIRCULATION; SIMPLE-MODEL; NORTHWARD PROPAGATION; CONVECTION FEEDBACKS; ATMOSPHERE MODEL; CLOUD-RADIATION AB June-October east Pacific warm pool intraseasonal variability (ISV) is assessed in eight atmospheric general circulation simulations. Complex empirical orthogonal function analysis is used to document the leading mode of 30-90-day precipitation variability in the models and Tropical Rainfall Measuring Mission observations. The models exhibit a large spread in amplitude of the leading mode about the observed amplitude. Little relationship is demonstrated between the amplitude of the leading mode and the ability of models to simulate observed north-northeastward propagation. Several process-oriented diagnostics are explored that attempt to distinguish why some models produce superior ISV. A diagnostic based on the difference in 500-850-hPa averaged relative humidity between the top 5% and the bottom 10% of precipitation events exhibits a significant correlation with leading mode amplitude. Diagnostics based on the vertically integrated moist entropy budget also demonstrate success at discriminating models with strong and weak variability. In particular, the vertical component of gross moist stability exhibits a correlation with amplitude of -0.9, suggesting that models in which convection and associated divergent circulations are less efficient at discharging moisture from the column are better able to sustain strong ISV. Several other diagnostics are tested that show no significant relationship with leading mode amplitude, including the warm pool mean surface zonal wind, the strength of surface flux feedbacks, and 500-850-hPa averaged relative humidity for the top 1% of rainfall events. Vertical zonal wind shear and 850-hPa zonal wind do not appear to be good predictors of model success at simulating the observed northward propagation pattern. C1 [Maloney, Eric D.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Jiang, Xianan] Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA USA. [Xie, Shang-Ping] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Benedict, James J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Maloney, ED (reprint author), Colorado State Univ, Dept Atmospher Sci, 1371 Campus Delivery, Ft Collins, CO 80523 USA. EM emaloney@atmos.colostate.edu RI Xie, Shang-Ping/C-1254-2009; Maloney, Eric/A-9327-2008; Benedict, James/M-5824-2013 OI Xie, Shang-Ping/0000-0002-3676-1325; Maloney, Eric/0000-0002-2660-2611; Benedict, James/0000-0001-5115-5131 FU NOAA MAPP program [NA12OAR4310077, NA12OAR4310075]; Climate and Large-Scale Dynamics Program of the National Science Foundation [AGS-0946911, AGS-1025584, AGS-1228302]; NASA CYGNSS program [NNX13AQ50G] FX Two reviewers provided excellent comments that led to significant improvements in the manuscript. The authors thank Cristiana Stan and Charlotte DeMott for making the SP-CCSM data available, and Mark Branson for help in running the CAM and SP-CAM simulations. This work was supported by the NOAA MAPP program under Grant NA12OAR4310077 (EDM and SPX) and NA12OAR4310075 (XJ), by the Climate and Large-Scale Dynamics Program of the National Science Foundation under Grants AGS-0946911, AGS-1025584 (EDM), and AGS-1228302 (XJ) and by the NASA CYGNSS program under Grant NNX13AQ50G (EDM). The statements, findings, conclusions, and recommendations do not necessarily reflect the views of NASA, NSF, NOAA, or the Department of Commerce. NR 78 TC 8 Z9 8 U1 0 U2 11 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD AUG 15 PY 2014 VL 27 IS 16 BP 6305 EP 6324 DI 10.1175/JCLI-D-14-00053.1 PG 20 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AN0YV UT WOS:000340310800012 ER PT J AU Westphal, AJ Stroud, RM Bechtel, HA Brenker, FE Butterworth, AL Flynn, GJ Frank, DR Gainsforth, Z Hillier, JK Postberg, F Simionovici, AS Sterken, VJ Nittler, LR Allen, C Anderson, D Ansari, A Bajt, S Bastien, RK Bassim, N Bridges, J Brownlee, DE Burchell, M Burghammer, M Changela, H Cloetens, P Davis, AM Doll, R Floss, C Gruen, E Heck, PR Hoppe, P Hudson, B Huth, J Kearsley, A King, AJ Lai, B Leitner, J Lemelle, L Leonard, A Leroux, H Lettieri, R Marchant, W Ogliore, R Ong, WJ Price, MC Sandford, SA Tresseras, JAS Schmitz, S Schoonjans, T Schreiber, K Silversmit, G Sole, VA Srama, R Stadermann, F Stephan, T Stodolna, J Sutton, S Trieloff, M Tsou, P Tyliszczak, T Vekemans, B Vincze, L Von Korff, J Wordsworth, N Zevin, D Zolensky, ME AF Westphal, Andrew J. Stroud, Rhonda M. Bechtel, Hans A. Brenker, Frank E. Butterworth, Anna L. Flynn, George J. Frank, David R. Gainsforth, Zack Hillier, Jon K. Postberg, Frank Simionovici, Alexandre S. Sterken, Veerle J. Nittler, Larry R. Allen, Carlton Anderson, David Ansari, Asna Bajt, Sasa Bastien, Ron K. Bassim, Nabil Bridges, John Brownlee, Donald E. Burchell, Mark Burghammer, Manfred Changela, Hitesh Cloetens, Peter Davis, Andrew M. Doll, Ryan Floss, Christine Gruen, Eberhard Heck, Philipp R. Hoppe, Peter Hudson, Bruce Huth, Joachim Kearsley, Anton King, Ashley J. Lai, Barry Leitner, Jan Lemelle, Laurence Leonard, Ariel Leroux, Hugues Lettieri, Robert Marchant, William Ogliore, Ryan Ong, Wei Jia Price, Mark C. Sandford, Scott A. Tresseras, Juan-Angel Sans Schmitz, Sylvia Schoonjans, Tom Schreiber, Kate Silversmit, Geert Sole, Vicente A. Srama, Ralf Stadermann, Frank Stephan, Thomas Stodolna, Julien Sutton, Stephen Trieloff, Mario Tsou, Peter Tyliszczak, Tolek Vekemans, Bart Vincze, Laszlo Von Korff, Joshua Wordsworth, Naomi Zevin, Daniel Zolensky, Michael E. CA 30714 Stardust Home Dusters TI Evidence for interstellar origin of seven dust particles collected by the Stardust spacecraft SO SCIENCE LA English DT Article ID COMET 81P/WILD 2; SOLAR-SYSTEM; INTERPLANETARY DUST; SIZE DISTRIBUTION; GRAINS; IMPACTS; AEROGEL; EVENTS; WILD-2; RETURN AB Seven particles captured by the Stardust Interstellar Dust Collector and returned to Earth for laboratory analysis have features consistent with an origin in the contemporary interstellar dust stream. More than 50 spacecraft debris particles were also identified. The interstellar dust candidates are readily distinguished from debris impacts on the basis of elemental composition and/or impact trajectory. The seven candidate interstellar particles are diverse in elemental composition, crystal structure, and size. The presence of crystalline grains and multiple iron-bearing phases, including sulfide, in some particles indicates that individual interstellar particles diverge from any one representative model of interstellar dust inferred from astronomical observations and theory. C1 [Westphal, Andrew J.; Butterworth, Anna L.; Gainsforth, Zack; Anderson, David; Lettieri, Robert; Marchant, William; Stodolna, Julien; Von Korff, Joshua; Zevin, Daniel] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Stroud, Rhonda M.; Bassim, Nabil] Naval Res Lab, Mat Sci & Technol Div, Washington, DC USA. [Bechtel, Hans A.; Tyliszczak, Tolek] Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA USA. [Brenker, Frank E.; Schmitz, Sylvia] Goethe Univ Frankfurt, Geosci Inst, D-60054 Frankfurt, Germany. [Flynn, George J.] SUNY Coll Plattsburgh, Plattsburgh, NY 12901 USA. [Frank, David R.; Bastien, Ron K.] NASA Johnson Space Ctr JSC, Jacobs Technol ESCG, Houston, TX USA. [Hillier, Jon K.; Postberg, Frank; Trieloff, Mario] Heidelberg Univ, Inst Geowissensch, D-69115 Heidelberg, Germany. [Simionovici, Alexandre S.] Observ Sci Univers Grenoble, Inst Sci Terre, Grenoble, France. [Sterken, Veerle J.] Univ Stuttgart, Inst Raumfahrtsyst IRS, D-70174 Stuttgart, Germany. [Sterken, Veerle J.] TU Braunschweig, IGEP, Braunschweig, Germany. [Sterken, Veerle J.; Gruen, Eberhard] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Sterken, Veerle J.; Heck, Philipp R.] Int Space Sci Inst, Bern, Switzerland. [Nittler, Larry R.] Carnegie Inst Sci, Washington, DC USA. [Allen, Carlton; Zolensky, Michael E.] NASA JSC, Houston, TX USA. [Ansari, Asna] Field Museum Nat Hist, Chicago, IL 60605 USA. [Bajt, Sasa] DESY, Hamburg, Germany. [Bridges, John] Univ Leicester, Space Res Ctr, Leicester, Leics, England. [Brownlee, Donald E.] Univ Washington, Dept Astron, Seattle, WA 98195 USA. [Burchell, Mark; Price, Mark C.] Univ Kent, Canterbury, Kent, England. [Burghammer, Manfred; Schoonjans, Tom; Silversmit, Geert; Vekemans, Bart; Vincze, Laszlo] Univ Ghent, B-9000 Ghent, Belgium. [Changela, Hitesh] Univ New Mexico, Albuquerque, NM 87131 USA. [Cloetens, Peter; Tresseras, Juan-Angel Sans; Sole, Vicente A.] ESRF, Grenoble, France. [Davis, Andrew M.; King, Ashley J.; Stephan, Thomas] Univ Chicago, Chicago, IL 60637 USA. [Doll, Ryan; Floss, Christine; Leonard, Ariel; Ong, Wei Jia; Schreiber, Kate; Stadermann, Frank] Washington Univ, St Louis, MO USA. [Hoppe, Peter; Huth, Joachim; Leitner, Jan] Max Planck Inst Chem, D-55128 Mainz, Germany. [Kearsley, Anton] Nat Hist Museum, London SW7 5BD, England. [Lai, Barry; Sutton, Stephen] Argonne Natl Lab, Adv Photon Source, Lemont, IL USA. [Lemelle, Laurence] Ecole Normale Super Lyon, F-69364 Lyon, France. [Leroux, Hugues] Univ Lille 1, F-59655 Villeneuve Dascq, France. [Ogliore, Ryan] Univ Hawaii Manoa, Honolulu, HI 96822 USA. [Sandford, Scott A.] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. [Srama, Ralf] Univ Stuttgart, IRS, D-70174 Stuttgart, Germany. [Tsou, Peter] CALTECH, Jet Prop Lab, Pasadena, CA USA. [Wordsworth, Naomi] Wexbury, Stoke Poges, Bucks, England. RP Westphal, AJ (reprint author), Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. EM westphal@ssl.berkeley.edu RI Sans Tresserras, Juan Angel/J-9362-2014; Leitner, Jan/A-7391-2015; Hoppe, Peter/B-3032-2015; Bajt, Sasa/G-2228-2010; Stroud, Rhonda/C-5503-2008; OI Sans Tresserras, Juan Angel/0000-0001-9047-3992; Leitner, Jan/0000-0003-3655-6273; Hoppe, Peter/0000-0003-3681-050X; Stroud, Rhonda/0000-0001-5242-8015; Burchell, Mark/0000-0002-2680-8943 FU NASA [NNX09AC36G, NNX09AC63G, NNH11AQ61I, NNX11AC21G, NNX11AE15G]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; U.S. DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; U.S. DOE [DE-AC02-06CH11357]; Klaus Tschira foundation; Tawani Foundation; Science and Technology Facilities Council (UK); German Science Foundation (DFG) [SPP1385]; Funds for Scientific Research (FWO), Flanders, Belgium [G.0395.11, G.0257.12N, G.0C12.13] FX We are deeply grateful to the Stardust@home dusters (list at http://stardustathome.ssl.berkeley.edu/sciencedusters), whose tremendous efforts were critically important to the success of this project. The ISPE consortium gratefully acknowledges the NASA Discovery Program for Stardust, the fourth NASA Discovery mission. NASA grants supported the following authors: NNX09AC36G-A.J.W., A. L. B., Z.G., R. L., D.Z., W. M., and J.V.K.; NNX09AC63G-C.F., R. D., A. L., W.J.O., K. S., and F.J.S.; NNH11AQ61I-R.M.S., H. C. G., and N.D.B.; NNX11AC21G-A.M.D., A.J.K., and T. S.; NNX11AE15G-G.J.F. The Advanced Light Source and the National Center for Electron Microscopy are supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) under contract no. DE-AC02-05CH11231. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. DOE, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-98CH10886. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U. S. DOE Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under contract no. DE-AC02-06CH11357. M. T. and F. P. acknowledge support by Klaus Tschira foundation. A. A. and P. R. H. were supported by the Tawani Foundation. M.J.B. and M. C. P. are supported by Science and Technology Facilities Council (UK). F. E. B., J.K.H., P. H., J.L., F. P., S. S., R. S., and M. T. were supported by funding of the German Science Foundation (DFG) within SPP1385: the first ten million years of the solar system-a planetary materials approach. The ESRF ID13 measurements were performed in the framework of ESRF LTP EC337, with financial support by the Funds for Scientific Research (FWO), Flanders, Belgium (contract nr. G.0395.11, G.0257.12N and Big Science program G.0C12.13). G. Silversmit was postdoctoral fellow of the FWO during the ISPE investigations. Data presented in this paper are described in the supplementary materials and in references (9-20). NR 43 TC 39 Z9 39 U1 5 U2 67 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 15 PY 2014 VL 345 IS 6198 BP 786 EP 791 DI 10.1126/science.1252496 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN4XM UT WOS:000340593100038 PM 25124433 ER PT J AU Reichhardt, CJO Lin, SZ Ray, D Reichhardt, C AF Reichhardt, C. J. Olson Lin, S. Z. Ray, D. Reichhardt, C. TI Comparing the dynamics of skyrmions and superconducting vortices SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE Superconducting vortex; Skyrmion; Pinning; Ratchet ID PINNING CENTERS; VORTEX LATTICES; CHIRAL MAGNET; DEFECTS; DENSITY; ARRAYS; MOTION; PHASES; FILMS; TEMPERATURE AB Vortices in type-II superconductors have attracted enormous attention as ideal systems in which to study nonequilibrium collective phenomena, since the self-ordering of the vortices competes with quenched disorder and thermal effects. Dynamic effects found in vortex systems include depinning, nonequilibrium phase transitions, creep, structural order-disorder transitions, and melting. Understanding vortex dynamics is also important for applications of superconductors which require the vortices either to remain pinned or to move in a controlled fashion. Recently, topological defects called skyrmions have been realized experimentally in chiral magnets. Here we highlight similarities and differences between skyrmion dynamics and vortex dynamics. Many of the previous ideas and experimental setups that have been applied to superconducting vortices can also be used to study skyrmions. We also discuss some of the differences between the two systems, such as the potentially large contribution of the Magnus force in the skyrmion system that can dramatically alter the dynamics and transport properties. (C) 2014 Elsevier B.V. All rights reserved. C1 [Reichhardt, C. J. Olson; Lin, S. Z.; Ray, D.; Reichhardt, C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ray, D.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. RP Reichhardt, CJO (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM cjrx@lanl.gov RI Lin, Shi-Zeng/B-2906-2008 OI Lin, Shi-Zeng/0000-0002-4368-5244 FU NNSA of the U.S. DoE at LANL [DE-AC52-06NA25396] FX This work was carried out under the auspices of the NNSA of the U.S. DoE at LANL under Contract No. DE-AC52-06NA25396. NR 58 TC 2 Z9 2 U1 2 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 EI 1873-2143 J9 PHYSICA C JI Physica C PD AUG 15 PY 2014 VL 503 BP 52 EP 57 DI 10.1016/j.physc.2014.03.029 PG 6 WC Physics, Applied SC Physics GA AM7TC UT WOS:000340070600011 ER PT J AU Ray, D Reichhardt, C Reichhardt, CJO Janko, B AF Ray, D. Reichhardt, C. Reichhardt, C. J. Olson Janko, B. TI Vortex transport and pinning in conformal pinning arrays SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE Vortex; Conformal pinning; Dynamics ID SUPERCONDUCTING FILMS; COLLOIDAL MONOLAYERS; PERIODIC ARRAYS; VORTICES; STATES; DYNAMICS; LATTICES; DEFECTS; CENTERS; PHASES AB We examine the current driven dynamics for vortices interacting with conformal crystal pinning arrays and compare to the dynamics of vortices driven over random pinning arrays. We find that the pinning is enhanced in the conformal arrays for field densities less than 2.5 times the matching field. At higher fields, the effectiveness of the pinning in the moving vortex state is enhanced in the random arrays compared to the conformal arrays, leading to crossing of the velocity force curves. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ray, D.; Janko, B.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Ray, D.; Reichhardt, C.; Reichhardt, C. J. Olson] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reichhardt, CJO (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM cjrx@lanl.gov FU NNSA of the U.S. DoE at LANL [DE-AC52-06NA25396] FX This work was carried out under the auspices of the NNSA of the U.S. DoE at LANL under Contract No. DE-AC52-06NA25396. NR 49 TC 3 Z9 3 U1 1 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 EI 1873-2143 J9 PHYSICA C JI Physica C PD AUG 15 PY 2014 VL 503 BP 123 EP 127 DI 10.1016/j.physc.2014.04.038 PG 5 WC Physics, Applied SC Physics GA AM7TC UT WOS:000340070600025 ER PT J AU Mathew, KJ Essex, RM Hasozbek, A Orlowicz, G Soriano, M AF Mathew, K. J. Essex, R. M. Hasozbek, A. Orlowicz, G. Soriano, M. TI Uranium isotope-amount ratios in certified reference material 116-A-Uranium (enriched) metal assay and isotopic standard SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE Uranium; Certified reference materials; Nuclear safeguards; Thermal ionization mass spectrometry; Traceability ID SECONDARY-ELECTRON MULTIPLIERS; IONIZATION MASS-SPECTROMETRY; TRACEABILITY; TIMS; UNCERTAINTY; LINEARITY; SAMPLES AB Certified reference material (CRM) 116-A, uranium (enriched) metal assay and isotopic standard, was analyzed using TRITON and MAT261 thermal ionization mass spectrometer (TIMS) instruments to characterize the uranium isotope-amount ratios. The certified n(U-238)/n(U-235) "major" ratio in CRM 116-A was determined using a combination of two analytical techniques: total evaporation (TE) and modified total evaporation (MTE). The "minor" isotope-amount ratios n (U-234)/n(U-235) and n(U-235)/n(U-235) in CRM 116-A were characterized using a combination of MTE and conventional analysis techniques. For the n (U-234)/n(U-235) and n(U-236)/n(U-235) ratios, both the MTE and conventional analysis routines incorporate an internal mass bias correction using the measured n(U-238)/n(U-235) ratio as well as corrections for peak tailing from U-235 to U-238. The abundance of U-233, present in CRM 116-A at trace levels, was characterized using a conventional analysis technique that incorporates a secondary electron multiplier (SEM) equipped with an energy filter. CRM 116-A isotope-amount ratios are traceable to the national measurement base and to the International System of Units (S.I.). The measurements leading to the certification of the uranium isotopic abundances in CRM 116-A are discussed. Published by Elsevier B.V. C1 [Mathew, K. J.; Essex, R. M.; Hasozbek, A.; Orlowicz, G.; Soriano, M.] US DOE, New Brunswick Lab, Argonne, IL 60439 USA. RP Mathew, KJ (reprint author), US DOE, New Brunswick Lab, 9800 South Cass Ave,Bldg 350, Argonne, IL 60439 USA. EM kattathu.mathew@ch.doe.gov NR 33 TC 7 Z9 7 U1 0 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD AUG 15 PY 2014 VL 369 BP 48 EP 58 DI 10.1016/j.ijms.2014.06.001 PG 11 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA AM0LG UT WOS:000339536500008 ER PT J AU Pina-Hernandez, C Koshelev, A Digianantonio, L Dhuey, S Polyakov, A Calafiore, G Goltsov, A Yankov, V Babin, S Cabrini, S Peroz, C AF Pina-Hernandez, Carlos Koshelev, Alexander Digianantonio, Lucas Dhuey, Scott Polyakov, Aleksandr Calafiore, Giuseppe Goltsov, Alexander Yankov, Vladimir Babin, Sergey Cabrini, Stefano Peroz, Christophe TI Printable planar lightwave circuits with a high refractive index SO NANOTECHNOLOGY LA English DT Article DE nanoimprint; photonic integrated circuits; titanium dioxide; nanofabrication ID WAVE-GUIDES; NANOIMPRINT LITHOGRAPHY; IMPRINT LITHOGRAPHY; PHOTONIC CHIP; TIO2; RESONATORS; RESOLUTION; DEVICES; NM AB We report a novel nanofabrication method to fabricate printable integrated circuits with a high refractive index working in the visible wavelength range. The printable planar ligthwave circuits are directly imprinted by ultra-violet nanoimprinting into functional TiO2-based resist on the top of planar waveguide core films. The printed photonic circuits are composed of several elementary components including ridge waveguides, light splitters and digital planar holograms. Multi-mode ridge waveguides with propagation losses around 40 dB cm(-1) at 660 nm wavelength, and, on-chip demultiplexers operated in the visible range with 100 channels and a spectral channel spacing around 0.35 nm are successfully demonstrated. C1 [Pina-Hernandez, Carlos; Calafiore, Giuseppe; Babin, Sergey; Peroz, Christophe] aBeam Technol, Hayward, CA 94541 USA. [Koshelev, Alexander; Goltsov, Alexander; Yankov, Vladimir] NanoOpt Devices, Santa Clara, CA 95054 USA. [Digianantonio, Lucas; Dhuey, Scott; Polyakov, Aleksandr; Cabrini, Stefano] Mol Foundry, LBNL, Berkeley, CA 94702 USA. RP Pina-Hernandez, C (reprint author), aBeam Technol, 22290 Foothill Blvd,St 2, Hayward, CA 94541 USA. EM cp@abeamtech.com RI Koshelev, Alexander/J-2574-2014; Foundry, Molecular/G-9968-2014 FU Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DE-AC02-05CH11231]; Air Force Office of Scientific Research (AFOSR), Air Force Material Command, USAF [FA9550-14-C-0020] FX The authors would like to thank S Sassolini and E Wood for their technical support. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under contract DE-AC02-05CH11231. Efforts were sponsored by the Air Force Office of Scientific Research (AFOSR), Air Force Material Command, USAF, under grant/contract number FA9550-14-C-0020. NR 35 TC 4 Z9 4 U1 5 U2 37 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD AUG 15 PY 2014 VL 25 IS 32 AR 325302 DI 10.1088/0957-4484/25/32/325302 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA AM1NO UT WOS:000339613400006 PM 25060823 ER PT J AU Rajewski, DA Takle, ES Lundquist, JK Prueger, JH Pfeiffer, RL Hatfield, JL Spoth, KK Doorenbos, RK AF Rajewski, Daniel A. Takle, Eugene S. Lundquist, Julie K. Prueger, John H. Pfeiffer, Richard L. Hatfield, Jerry L. Spoth, Kristopher K. Doorenbos, Russell K. TI Changes in fluxes of heat, H2O, and CO2 caused by a large wind farm SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Surface fluxes; Wind turbines; Turbulence; Crop microclimate; Spectral analysis ID LAND-SURFACE TEMPERATURE; BOUNDARY-LAYER; TURBINE WAKES; ATMOSPHERIC STABILITY; SONIC ANEMOMETER; ENERGY-BALANCE; IMPACTS; MODEL; SHELTERBELTS; TUNNEL AB The Crop Wind-Energy Experiment (CWEX) provides a platform to investigate the effect of wind turbines and large wind farms on surface fluxes of momentum, heat, moisture, and carbon dioxide (CO2). In 2010 and 2011, eddy covariance flux stations were installed between two lines of turbines at the southwest edge of a large Iowa wind farm from late June to early September. We report changes in fluxes of momentum, sensible heat, latent heat, and CO2 above a corn canopy after surface air had passed through a single line of turbines. In 2010, our flux stations were placed within a field with homogeneous land management practices (same tillage, cultivar, chemical treatments). We stratify the data according to wind direction, diurnal condition, and turbine operational status. Within these categories, the downwind-upwind flux differences quantify turbine influences at the crop surface. Flux differences were negligible in both westerly wind conditions and when the turbines were non operational. When the flow is perpendicular (southerly) or slightly oblique (southwesterly) to the row of turbines during the day, fluxes of CO2 and water (H2O) are enhanced by a factor of five in the lee of the turbines (from three to five turbine diameter distances downwind from the tower) as compared to a west wind. However, we observe a smaller CO2 flux increase of 30-40% for these same wind directions when the turbines are off. In the nighttime, there is strong statistical significance that turbine wakes enhance upward CO2 fluxes and entrain sensible heat toward the crop. The direction of the scalar flux perturbation seems closely associated to the differences in canopy friction velocity. Spectra and co-spectra of momentum components and co-spectra of heat also demonstrate nighttime influence of the wind turbine turbulence at the downwind station. (C) 2014 The Authors. Published by Elsevier BM. C1 [Rajewski, Daniel A.; Takle, Eugene S.; Spoth, Kristopher K.; Doorenbos, Russell K.] Iowa State Univ, Dept Agron, Ames, IA 50011 USA. [Lundquist, Julie K.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. [Lundquist, Julie K.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Prueger, John H.; Pfeiffer, Richard L.; Hatfield, Jerry L.] Natl Lab Agr & Environm, Ames, IA 50011 USA. RP Rajewski, DA (reprint author), Iowa State Univ, 3132 Agronomy Hall, Ames, IA 50011 USA. EM drajewsk@iastate.edu OI Rajewski, Daniel/0000-0002-9609-2303; LUNDQUIST, JULIE/0000-0001-5490-2702 FU National Renewable Energy Laboratory under Professor Lundquist's Joint Appointment; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy; Ames Laboratory (DOE); Center for Global and Regional Environmental Research at the University of Iowa; NSF Research Experience for Undergraduates program [1063048]; National Science Foundation under the State of Iowa EPSCoR [1101284] FX This work was supported in part by the National Renewable Energy Laboratory under Professor Lundquist's Joint Appointment. NREL is a national laboratory of the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, operated by the Alliance for Sustainable Energy, LLC. Partial funding for CWEX-10 was provided by the Ames Laboratory (DOE) and the Center for Global and Regional Environmental Research at the University of Iowa. Surface flux stations for CWEX-11 were provided by NCAR Earth Observing Laboratory under an instrumentation deployment, and undergraduate student participation was supplemented by funding from an NSF Research Experience for Undergraduates program under grant 1063048. We recognize Tom Horst, Steve Oncley, and Gordon MacLean from NCAR EOL for their assistance in data-post processing and analysis techniques. The authors also recognize assistance in interpretation of the results from James Brache, Thomas Sauer, Fernando Miguez, and Sotirios Archontoulis. We also recognize Michael Rhodes from CU for editing contributions of the manuscript. Data analysis was supported in part by the National Science Foundation under the State of Iowa EPSCoR Grant 1101284. The authors also acknowledge the wind farm manager and land owners/operators cooperation in conducting CWEX. NR 57 TC 6 Z9 7 U1 3 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD AUG 15 PY 2014 VL 194 BP 175 EP 187 DI 10.1016/j.agrformet.2014.03.023 PG 13 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA AL4UX UT WOS:000339131400016 ER PT J AU Watkins, JM Liang, Y Richter, F Ryerson, FJ DePaolo, DJ AF Watkins, James M. Liang, Yan Richter, Frank Ryerson, Frederick J. DePaolo, Donald J. TI Diffusion of multi-isotopic chemical species in molten silicates SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID MULTICOMPONENT DIFFUSION; GEOLOGICAL APPLICATIONS; MELTS; FRACTIONATION; MGO-AL2O3-SIO2; CAO-AL2O3-SIO2; LIQUIDS; MATRIX; SYSTEM; SR AB Diffusion experiments in a simplified Na2O-CaO-SiO2 liquid system are used to develop a general formulation for the fractionation of Ca isotopes during liquid-phase diffusion. Although chemical diffusion is a well-studied process, the mathematical description of the effects of diffusion on the separate isotopes of a chemical element is surprisingly underdeveloped and uncertain. Kinetic theory predicts a mass dependence on isotopic mobility, but it is unknown how this translates into a mass dependence on effective binary diffusion coefficients, or more generally, the chemical diffusion coefficients that are housed in a multicomponent diffusion matrix. Our experiments are designed to measure Ca mobility, effective binary diffusion coefficients, the multicomponent diffusion matrix, and the effects of chemical diffusion on Ca isotopes in a liquid of single composition. We carried out two chemical diffusion experiments and one self-diffusion experiment, all at 1250 degrees C and 0.7 GPa and using a bulk composition for which other information is available from the literature. The self-diffusion experiment is used to determine the mobility of Ca in the absence of diffusive fluxes of other liquid components. The chemical diffusion experiments are designed to determine the effect on Ca isotope fractionation of changing the counter-diffusing component from fast-diffusing Na2O to slow-diffusing SiO2. When Na2O is the main counter-diffusing species, CaO diffusion is fast and larger Ca isotopic effects are generated. When SiO2 is the main counter-diffusing species, CaO diffusion is slow and smaller Ca isotopic effects are observed. In both experiments, the liquid is initially isotopically homogeneous, and during the experiment Ca isotopes become fractionated by diffusion. The results are used as a test of a new general expression for the diffusion of isotopes in a multicomponent liquid system that accounts for both self diffusion and the effects of counter-diffusing species. Our results show that (1) diffusive isotopic fractionations depend on the direction of diffusion in composition space, (2) diffusive isotopic fractionations scale with effective binary diffusion coefficient, as previously noted by Watkins et al. (2011), (3) self-diffusion is not decoupled from chemical diffusion, (4) self diffusion can be faster than or slower than chemical diffusion and (5) off-diagonal terms in the chemical diffusion matrix have isotopic mass-dependence. The results imply that relatively large isotopic fractionations can be generated by multicomponent diffusion even in the absence of large concentration gradients of the diffusing element. The new formulations for isotope diffusion can be tested with further experimentation and provide an improved framework for interpreting mass-dependent isotopic variations in natural liquids. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Watkins, James M.] Univ Oregon, Dept Geol Sci, Eugene, OR 97403 USA. [Liang, Yan] Brown Univ, Dept Geol Sci, Providence, RI 02912 USA. [Richter, Frank] Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA. [Ryerson, Frederick J.] Lawrence Livermore Natl Lab, Livermore, CA USA. [DePaolo, Donald J.] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. RP Watkins, JM (reprint author), Univ Oregon, Dept Geol Sci, Eugene, OR 97403 USA. EM watkins4@uoregon.edu RI Liang, Yan/G-2241-2016 OI Liang, Yan/0000-0002-9569-840X FU National Science Foundation [EAR-1050000, EAR-1220076]; U.S. Department of Energy Grant [DE-FG02-01ER15254] FX Ben Jacobsen contributed the SIMS measurements shown in Fig. 2. This research was supported by National Science Foundation Grants EAR-1050000 to D.J.D. and EAR-1220076 to Y.L., and U.S. Department of Energy Grant DE-FG02-01ER15254 to F.M.R. NR 24 TC 7 Z9 7 U1 5 U2 42 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2014 VL 139 BP 313 EP 326 DI 10.1016/j.gca.2014.04.039 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AL5LY UT WOS:000339176400017 ER PT J AU Vetter, L Kozdon, R Valley, JW Mora, CI Spero, HJ AF Vetter, Lael Kozdon, Reinhard Valley, John W. Mora, Claudia I. Spero, Howard J. TI SIMS measurements of intrashell delta C-13 in the cultured planktic foraminifer Orbulina universa SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID CARBON ISOTOPIC COMPOSITION; WESTERN NORTH-ATLANTIC; ION MASS-SPECTROMETRY; EQUATORIAL PACIFIC; OXYGEN ISOTOPES; VERTICAL-DISTRIBUTION; MEDITERRANEAN SEA; ICP-MS; TEMPERATURE; TESTS AB In this study, we present experimental results from the planktic foraminifer Orbulina universa, cultured in the laboratory. We demonstrate that the delta C-13 of shell calcite precipitated in (13) C-labeled seawater for 24 h can be resolved and accurately measured using Secondary Ion Mass Spectrometry (SIMS). Specimens maintained at 20 degrees C were transferred from ambient seawater (delta C-13(DIC) = +1.3 parts per thousand) into seawater with delta C-13(DIC) = +51.5 parts per thousand and enriched [Ba2+] for 24 h. Specimens were then transferred into ambient seawater with elevated [Sr-87] for 6-9 h of calcification, followed by a transfer back into unlabeled ambient seawater until gametogenesis. This technique produced O. universa shells with calcite layers of distinct geochemical signatures. We quantify the spatial positions of trace element labels in the shells using laser ablation ICP-MS depth profiling. Using fragments from the same shells, we quantify intrashell delta C-13(calcite) using SIMS with a 6 or 8 mu m spot (2 SD range +/- 0.5 parts per thousand to 1.7 parts per thousand). Measured delta C-13(calcite) values in O. universa shell layers precipitated in ambient seawater are within 2 parts per thousand of predicted delta C-13(calcite) values. In (13) C-labeled bands of calcite, 6 mu m SIMS spot measurements are within 2 parts per thousand of predicted delta C-13(calcite) values, whereas 8 mu m SIMS spots yield intermediate, mixed values. The spatial agreement between trace element and carbon isotope data suggests that (13) C and cation tracers are synchronously incorporated into shell calcite. These results demonstrate the ability of SIMS delta C-13 measurements to resolve similar to 10 mu m features in foraminifer shell calcite using a 6 mu m spot, and highlight the potential of this technique for addressing questions about ecology, biomineralization, and paleoceanography. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Vetter, Lael; Spero, Howard J.] Univ Calif Davis, Dept Earth & Planetary Sci, Davis, CA 95616 USA. [Kozdon, Reinhard; Valley, John W.] Univ Wisconsin, Dept Geosci, WiscSIMS Lab, Madison, WI 53706 USA. [Mora, Claudia I.] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. RP Vetter, L (reprint author), Tulane Univ, Dept Earth & Environm Sci, New Orleans, LA 70118 USA. EM laelvetter@laelvetter.com RI Kozdon, Reinhard/J-9468-2014; Mora, Claudia/B-5511-2017; OI Kozdon, Reinhard/0000-0001-6347-456X; Mora, Claudia/0000-0003-2042-0208; Vetter, Lael/0000-0003-4240-353X FU UC Davis Durrell Fund for graduate research; NSF [OCE-0550703, OCE1061676, EAR-0946297]; Los Alamos National Laboratory [IGPP:09-RFP-008]; NSF-EAR [0319230, 1053466] FX We gratefully acknowledge the field assistance of A. Russell, J. Fehrenbacher, A. Gagnon, J. Snyder, K. Holland, and B. Wagman; and the staff of the Wrigley Marine Science Center on Catalina Island. We also thank N. Kita and J. Kern at WiscSIMS for analytical support, and D. C. Kelly provided assistance with sample preparation and logistics. This work benefited greatly from the careful and experienced sample preparation of B. Hess, and we thank him for his efforts on Superbowl Sunday. Collection equipment for culturing experiments was partially funded by the UC Davis Durrell Fund for graduate research. This research was supported by NSF awards OCE-0550703, OCE1061676, and EAR-0946297 (H. J. S.), and Los Alamos National Laboratory award IGPP:09-RFP-008 (C. I. M. and H. J. S.). WiscSIMS is partially supported by NSF-EAR (0319230, 1053466). NR 64 TC 4 Z9 4 U1 2 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2014 VL 139 BP 527 EP 539 DI 10.1016/j.gca.2014.04.049 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AL5LY UT WOS:000339176400029 ER PT J AU Joshi, TH Sangiorgio, S Mozin, V Norman, EB Sorensen, P Foxe, M Bench, G Bernstein, A AF Joshi, T. H. Sangiorgio, S. Mozin, V. Norman, E. B. Sorensen, P. Foxe, M. Bench, G. Bernstein, A. TI Design and demonstration of a quasi-monoenergetic neutron source SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Neutron source; Neutron filter; Li-7 (p,n)Be-7 reaction; Nuclear recoil ID NUCLEAR RECOILS; NEAR-THRESHOLD; GE-73 ATOMS; IONIZATION; DETECTOR AB The design of a neutron source capable of producing 24 and 70 keV neutron beams with narrow energy spread is presented. The source exploits near-threshold kinematics of the Li-7 (p,n)Be-7 reaction while taking advantage of the interference 'notches' found in the scattering cross-sections of iron. The design was implemented and characterized at the Center for Accelerator Mass Spectrometry at Lawrence Livermore National Laboratory. Alternative filters such as vanadium and manganese are also explored and the possibility of studying the response of different materials to low-energy nuclear recoils using the resultant neutron beams is discussed. (C) 2014 Elsevier B.V. All rights reserved. C1 [Joshi, T. H.; Norman, E. B.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Joshi, T. H.; Sangiorgio, S.; Mozin, V.; Norman, E. B.; Sorensen, P.; Foxe, M.; Bench, G.; Bernstein, A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Foxe, M.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. RP Joshi, TH (reprint author), Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. EM thjoshi@berkeley.edu FU Lawrence Scholars Program at LLNL; Department of Homeland Security; U.S. Department of Homeland Security; Domestic Nuclear Detection Office; U.S. Department of Defense, Defense Threat Reduction Agency; LDRD program at LLNL [LDRD 13-FS-005]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; [LLNL-JRNL-651154] FX The authors would like to thank Vincent Meot for production of the Li targets, Sergey Kucheyev for Rutherford Backscatter measurements of the lithium targets, Jason Burke for his help with the experimental effort, and Tom Brown for his assistance at CAMS. T.H. Joshi would like to acknowledge the funding of the Lawrence Scholars Program at LLNL and the Department of Homeland Security. A portion of M. Foxe's research was performed under the Nuclear Forensics Graduate Fellowship Program, which is sponsored by the U.S. Department of Homeland Security, Domestic Nuclear Detection Office and the U.S. Department of Defense, Defense Threat Reduction Agency. We gratefully acknowledge the LDRD program (LDRD 13-FS-005) at LLNL. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. LLNL-JRNL-651154 NR 23 TC 0 Z9 0 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD AUG 15 PY 2014 VL 333 BP 6 EP 11 DI 10.1016/j.nimb.2014.04.008 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AL4XH UT WOS:000339137600002 ER PT J AU Halford, E Winter, B Mills, MD Thompson, SP Parr, V John, JJ Nomerotski, A Vallance, C Turchetta, R Brouard, M AF Halford, E. Winter, B. Mills, M. D. Thompson, S. P. Parr, V. John, J. J. Nomerotski, A. Vallance, C. Turchetta, R. Brouard, M. TI Modifications to a commercially available linear mass spectrometer for mass-resolved microscopy with the pixel imaging mass spectrometry (PImMS) camera SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID ASSISTED LASER-DESORPTION; VELOCITY DISTRIBUTIONS; MOLECULAR-IONS; MATRIX; IONIZATION; RESOLUTION; TIME; DETECTOR; DESORPTION/IONIZATION; EXTRACTION AB RATIONALE: Imaging mass spectrometry is a powerful analytical technique capable of accessing a large volume of spatially resolved, chemical data from two-dimensional samples. Probing the entire surface of a sample simultaneously requires a detector with high spatial and temporal resolutions, and the ability to observe events relating to different mass-to-charge ratios. METHODS: A commercially available time-of-flight mass spectrometer, designed for matrix-assisted laser desorption/ionization (MALDI) analysis, was combined with the novel pixel imaging mass spectrometry (PImMS) camera in order to perform multi-mass, microscope-mode imaging experiments. A number of minor modifications were made to the spectrometer hardware and ion optics so that spatial imaging was achieved for a number of small molecules. RESULTS: It was shown that a peak width of Delta m(50%) < 1 m/z unit across the range 200 <= m/z <= 800 can be obtained while also achieving an optimum spatial resolution of 25 mu m. It was further shown that these data were obtained simultaneously for all analytes present without the need to scan the experimental parameters. CONCLUSIONS: This work demonstrates the capability of multi-mass, microscope-mode imaging to reduce the acquisition time of spatially distributed analytes such as multi-arrays or biological tissue sections. It also shows that such an instrument can be commissioned by effecting relatively minor modifications to a conventional commercial machine. Copyright (C) 2014 John Wiley & Sons, Ltd. C1 [Halford, E.; Winter, B.; Brouard, M.] Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, Oxford OX1 3QZ, England. [Mills, M. D.; Thompson, S. P.; Parr, V.] SAI Ltd, Manchester M16 9FE, Lancs, England. [John, J. J.] Univ Oxford, Dept Phys, Oxford OX1 3RH, England. [Nomerotski, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Vallance, C.] Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England. [Turchetta, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. RP Brouard, M (reprint author), Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, South Parks Rd, Oxford OX1 3QZ, England. EM mark.brouard@chem.ox.ac.uk RI Nomerotski, Andrei/A-5169-2010; OI John, Jaya/0000-0001-6831-6501 FU STFC [ST/J002895/1]; EPSRC [EP/L005913/1]; EU [238671] FX The support of the STFC through the Mini-IPS grant ST/J002895/1, the EPSRC via Programme grant No. EP/L005913/1, and the EU through grant FP7 ITN "ICONIC" (238671) is gratefully acknowledged. Elements of the work described here are detailed in the US Patent Application No. 20100294924 A1. NR 39 TC 1 Z9 1 U1 2 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0951-4198 EI 1097-0231 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD AUG 15 PY 2014 VL 28 IS 15 BP 1649 EP 1657 DI 10.1002/rcm.6940 PG 9 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA AK9SP UT WOS:000338767300002 PM 24975244 ER PT J AU Ovchinnikova, OS Bhandari, D Lorenz, M Van Berkel, GJ AF Ovchinnikova, Olga S. Bhandari, Deepak Lorenz, Matthias Van Berkel, Gary J. TI Transmission geometry laser ablation into a non-contact liquid vortex capture probe for mass spectrometry imaging SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID THIN-LAYER-CHROMATOGRAPHY; SURFACE SAMPLING PROBE; DESORPTION/IONIZATION; MATRICES; EMITTER AB RATIONALE: Capture of material from a laser ablation plume into a continuous flow stream of solvent provides the means for uninterrupted sampling, transport and ionization of collected material for coupling with mass spectral analysis. Reported here is the use of vertically aligned transmission geometry laser ablation in combination with a new non-contact liquid vortex capture probe coupled with electrospray ionization for spot sampling and chemical imaging with mass spectrometry. METHODS: A vertically aligned continuous flow liquid vortex capture probe was positioned directly underneath a sample surface in a transmission geometry laser ablation (355 nm, 10 Hz, 7 ns pulse width) set up to capture into solution the ablated material. The outlet of the vortex probe was coupled to the Turbo V (TM) ion source of an AB SCIEX TripleTOF 5600+ mass spectrometer. System operation and performance metrics were tested using inked patterns and thin tissue sections. Glass slides and slides designed especially for laser capture microdissection, viz., DIRECTOR (R) slides and PEN 1.0 (polyethylene naphthalate) membrane slides, were used as sample substrates. RESULTS: The estimated capture efficiency of laser-ablated material was 24%, which was enabled by the use of a probe with large liquid surface area (similar to 2.8 mm(2)) and with gravity to help direct ablated material vertically down towards the probe. The swirling vortex action of the liquid surface potentially enhanced capture and dissolution not only of particulates, but also of gaseous products of the laser ablation. The use of DIRECTOR (R) slides and PEN 1.0 (polyethylene naphthalate) membrane slides as sample substrates enabled effective ablation of a wide range of sample types (basic blue 7, polypropylene glycol, insulin and cyctochrome c) without photodamage using a UV laser. Imaging resolution of about 6 m was demonstrated for stamped ink on DIRECTOR (R) slides based on the ability to distinguish features present both in the optical and in the chemical image. This imaging resolution was 20 times better than the previous best reported results with laser ablation/liquid sample capture mass spectrometry imaging. Using thin sections of brain tissue the chemical image of a selected lipid was obtained with an estimated imaging resolution of about 50 mu m. CONCLUSIONS: A vertically aligned, transmission geometry laser ablation liquid vortex capture probe, electrospray ionization mass spectrometry system provides an effective means for spatially resolved spot sampling and imaging with mass spectrometry. Published in 2014. This article is a U.S. Government work and is in the public domain in the USA. C1 [Ovchinnikova, Olga S.; Bhandari, Deepak; Lorenz, Matthias; Van Berkel, Gary J.] Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. RP Van Berkel, GJ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. EM vanberkelgj@ornl.gov RI Lorenz, Matthias/F-8273-2016 OI Lorenz, Matthias/0000-0003-0867-8548 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; U.S. Government [DE-AC05-00OR22725] FX The authors thank Justin Wiseman (Prosolia, Inc.) for providing the mouse brain thin-tissue section. Instrumental implementation, fundamental, and metric studies were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. The tissue imaging work was supported by, and the TripleTOF (R) 5600+ mass spectrometer used in this work was provided on loan by, AB Sciex through a Cooperative Research and Development Agreement (CRADA NFE-10-02966). This manuscript has been authored by a contractor of the U.S. Government under contract DE-AC05-00OR22725. Accordingly, the U.S. Government retains a paid-up, nonexclusive, irrevocable, worldwide license to publish or reproduce the published form of this contribution, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, or allow others to do so, for U.S. Government purposes. NR 23 TC 11 Z9 11 U1 1 U2 35 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0951-4198 EI 1097-0231 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD AUG 15 PY 2014 VL 28 IS 15 BP 1665 EP 1673 DI 10.1002/rcm.6946 PG 9 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA AK9SP UT WOS:000338767300004 PM 24975246 ER PT J AU Garrett, CK Li, RC AF Garrett, C. Kristopher Li, Ren-Cang TI GIP integrators for Matrix Riccati Differential Equations SO APPLIED MATHEMATICS AND COMPUTATION LA English DT Article DE Matrix Riccati Differential Equation; Singularity; GIP integrator; Runge-Kutta; Generalized Inverse Property ID BOUNDARY-VALUE-PROBLEMS; SOLVING LINEAR BVPS; NUMERICAL-INTEGRATION; TRANSFORMATION METHOD; ALGEBRAIC SYSTEMS; SDIRK METHODS; ALGORITHMS; ODES AB Matrix Riccati Differential Equations (MRDEs) are initial value problems of the form: X' = A(21) - XA(11) + A(22)X - XA(12)X; X(0) = X-0. These equations arise frequently throughout applied mathematics, science, and engineering. It can happen that even when the A(ij) are smooth functions of t or constant, the solution X may have a singularity or even infinitely many singularities. This paper shows several classes of numerical algorithms, which we call GIP integrators, that can solve for X past its singularities. Furthermore, none of the algorithms require knowledge of the placement or even existence of singularities in X. Also, it is shown how embedded Runge-Kutta methods can be used to construct GIP integrators to not only approximate X past singularities but also provide for error estimation to allow efficient time stepping. Finally, several examples are shown to validate the theory. (C) 2014 Elsevier Inc. All rights reserved. C1 [Garrett, C. Kristopher] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Li, Ren-Cang] Univ Texas Arlington, Dept Math, Arlington, TX 76019 USA. RP Li, RC (reprint author), Univ Texas Arlington, Dept Math, POB 19408, Arlington, TX 76019 USA. EM garrettck@ornl.gov; rcli@uta.edu FU NSF [DMS-0810506, DMS-1115834] FX Supported in part by NSF Grant DMS-0810506.; Supported in part by NSF Grant DMS-0810506 and DMS-1115834. NR 49 TC 0 Z9 1 U1 2 U2 6 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0096-3003 EI 1873-5649 J9 APPL MATH COMPUT JI Appl. Math. Comput. PD AUG 15 PY 2014 VL 241 BP 283 EP 297 DI 10.1016/j.amc.2014.05.014 PG 15 WC Mathematics, Applied SC Mathematics GA AK9GD UT WOS:000338734700028 ER PT J AU Nikolaev, AG Yushkov, GY Oks, EM Oztarhan, A Akpek, A Hames-Kocabas, E Urkac, ES Brown, IG AF Nikolaev, A. G. Yushkov, G. Yu. Oks, E. M. Oztarhan, A. Akpek, A. Hames-Kocabas, E. Urkac, E. S. Brown, I. G. TI Modification of anti-bacterial surface properties of textile polymers by vacuum arc ion source implantation SO APPLIED SURFACE SCIENCE LA English DT Article; Proceedings Paper CT 18th International Conference on Surface Modification of Materials by Ion Beams (SMMIB) CY SEP 15-20, 2013 CL Kusadasi, TURKEY DE Ion implantation; Mevva; Antibacterial; Neuron growth; Ag; Nanoparticle ID UHMWPE AB Ion implantation provides an important technology for the modification of material surface properties. The vacuum arc ion source is a unique instrument for the generation of intense beams of metal ions as well as gaseous ions, including mixed metal gas beams with controllable metal:gas ion ratio. Here we describe our exploratory work on the application of vacuum arc ion source-generated ion beams for ion implantation into polymer textile materials for modification of their biological cell compatibility surface properties. We have investigated two specific aspects of cell compatibility: (i) enhancement of the antibacterial characteristics (we chose to use Staphylococcus aureus bacteria) of ion implanted polymer textile fabric, and (ii) the "inverse" concern of enhancement of neural cell growth rate (we chose Rat B-35 neuroblastoma cells) on ion implanted polymer textile. The results of both investigations were positive, with implantation-generated antibacterial efficiency factor up to about 90%, fully comparable to alternative conventional (non-implantation) approaches and with some potentially important advantages over the conventional approach; and with enhancement of neural cell growth rate of up to a factor of 3.5 when grown on suitably implanted polymer textile material. (C) 2014 Elsevier B.V. All rights reserved. C1 [Nikolaev, A. G.; Yushkov, G. Yu.; Oks, E. M.] Russian Acad Sci, Siberian Branch, Inst High Current Elect, Tomsk 634055, Russia. [Oztarhan, A.] Izmir Univ, TR-35140 Izmir, Turkey. [Akpek, A.; Hames-Kocabas, E.; Urkac, E. S.] Ege Univ, Dept Bioengn, TR-35100 Izmir, Turkey. [Brown, I. G.] Lawrence Berkeley Natl Lab, Berkeley, CA 94708 USA. RP Nikolaev, AG (reprint author), Russian Acad Sci, Siberian Branch, Inst High Current Elect, Tomsk 634055, Russia. EM nik@opee.hcei.tsc.ru RI Yushkov, Georgy/O-8024-2015; Nikolaev, Alexey/R-2154-2016; OI Yushkov, Georgy/0000-0002-7615-6058; Nikolaev, Alexey/0000-0003-2724-3697; Oks, Efim/0000-0002-9323-0686 NR 13 TC 2 Z9 4 U1 3 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD AUG 15 PY 2014 VL 310 SI SI BP 51 EP 55 DI 10.1016/j.apsusc.2014.04.002 PG 5 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AL0GQ UT WOS:000338805800009 ER PT J AU Salvadori, MC Teixeira, FS Sgubin, LG Cattani, M Brown, IG AF Salvadori, M. C. Teixeira, F. S. Sgubin, L. G. Cattani, M. Brown, I. G. TI Surface modification by metal ion implantation forming metallic nanoparticles in an insulating matrix SO APPLIED SURFACE SCIENCE LA English DT Article; Proceedings Paper CT 18th International Conference on Surface Modification of Materials by Ion Beams (SMMIB) CY SEP 15-20, 2013 CL Kusadasi, TURKEY DE Surface modification; Nanocomposites; Nanoparticles; Ion implantation ID DYNAMIC COMPOSITION CHANGES; GOLD NANOPARTICLES; PLASMON RESONANCE; PERCOLATION; SIMULATION; POLYMER; TRIDYN AB There is special interest in the incorporation of metallic nanoparticles in a surrounding dielectric matrix for obtaining composites with desirable characteristics such as for surface plasmon resonance, which can be used in photonics and sensing, and controlled surface electrical conductivity. We have investigated nanocomposites produced by metal ion implantation into insulating substrates, where the implanted metal self-assembles into nanoparticles. The nanoparticles nucleate near the maximum of the implantation depth profile (projected range), which can be estimated by computer simulation using the TRIDYN code. TRIDYN is a Monte Carlo simulation program based on the TRIM (Transport and Range of Ions in Matter) code that takes into account compositional changes in the substrate due to two factors: previously implanted dopant atoms, and sputtering of the substrate surface. Our study show that the nanopartides form a bidimentional array buried a few nanometers below the substrate surface. We have studied Au/PMMA (polymethylmethacrylate), Pt/PMMA, Ti/alumina and Au/alumina systems. Transmission electron microscopy of the implanted samples show that metallic nanoparticles form in the insulating matrix. These nanocomposites have been characterized by measuring the resistivity of the composite layer as a function of the implantation dose. The experimental results are compared with a model based on percolation theory, in which electron transport through the composite is explained by conduction through a random resistor network formed by the metallic nanoparticles. Excellent agreement is found between the experimental results and the predictions of the theory. We conclude in that the conductivity process is due only to percolation (when the conducting elements are in geometric contact) and that the contribution from tunneling conduction is negligible. (C) 2014 Elsevier B.V. All rights reserved. C1 [Salvadori, M. C.; Teixeira, F. S.; Sgubin, L. G.; Cattani, M.] Univ Sao Paulo, Inst Phys, BR-05314970 Sao Paulo, Brazil. [Brown, I. G.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Salvadori, MC (reprint author), Univ Sao Paulo, Inst Phys, CP 66318, BR-05314970 Sao Paulo, Brazil. EM mcsalvadori@if.usp.br RI Salvadori, Maria Cecilia/A-9379-2013 NR 33 TC 4 Z9 5 U1 5 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD AUG 15 PY 2014 VL 310 SI SI BP 158 EP 163 DI 10.1016/j.apsusc.2014.03.145 PG 6 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AL0GQ UT WOS:000338805800026 ER PT J AU Sadat, ME Patel, R Bud'ko, SL Ewing, RC Zhang, JM Xue, H Mast, DB Shi, DL AF Sadat, M. E. Patel, Ronak Bud'ko, Sergey L. Ewing, Rodney C. Zhang, Jiaming Xue, Hong Mast, David B. Shi, Donglu TI Dipole-interaction mediated hyperthermia heating mechanism of nanostructured Fe3O4 composites SO MATERIALS LETTERS LA English DT Article DE Magnetism; Cancer therapy; Magnetic nanoparticle; Superparamagnetism ID ALTERNATING MAGNETIC-FIELD; NANOPARTICLES; FLUID; THERAPY AB A correlation between the DC magnetization and hyperthermia heating rate in high frequency magnetic fields was established for two distinctively different magnetic nanoparticle (MNP) systems: (1) polystyrene (PS)/Fe3O4 based composites, consisting of 10 nm diameter Fe3O4 nanoparticles embedded in the matrix of polystyrene (PS) spheres (similar to 100 nm), and (2) similar Fe3O4 nanoparticles coated with polyacrylic acid (PAA) and dispersed in water. Due to physical confinement of Fe3O4 nanoparticles in the former, the PS/Fe3O4 composite exhibited much lower magnetic hyperthermia heating compared to the latter. The reduced magnetic hyperthermia heating in the polystyrene (PS)/Fe3O4 based composites was found to be associated with strong dipolar interactions. (C) 2014 Elsevier B.V. All rights reserved. C1 [Sadat, M. E.; Mast, David B.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Patel, Ronak; Shi, Donglu] Univ Cincinnati, Dept Mech & Mat Engn, Coll Engn & Appl Sci, Cincinnati, OH 45221 USA. [Bud'ko, Sergey L.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Bud'ko, Sergey L.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Ewing, Rodney C.; Zhang, Jiaming] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. [Xue, Hong] Shanghai Jiao Tong Univ, Med X Inst, Shanghai 200030, Peoples R China. [Shi, Donglu] Tongji Univ, Sch Med, Inst Biomed Engn & Nano Sci, Shanghai East Hosp, Shanghai 200120, Peoples R China. RP Shi, DL (reprint author), Univ Cincinnati, Coll Engn & Appl Sci, 493 Rhodes Hall,ML72, Cincinnati, OH 45221 USA. EM donglu.shi@uc.edu FU Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; National Science Foundation (NSF) [NSF (1343568)]; Shanghai Nanotechnology Promotion Center [12nm0501201, 11nm0506100]; National Natural Science Foundation of China [51173135] FX Work at the Ames Laboratory was supported by the Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering under contract no. DE-AC02-07CH11358. The work at University of Cincinnati was supported by a National Science Foundation (NSF) grant under contract no. NSF (1343568). The work at Tongji University was supported by grants from Shanghai Nanotechnology Promotion Center (12nm0501201, 11nm0506100) and the National Natural Science Foundation of China (51173135). NR 12 TC 5 Z9 6 U1 2 U2 48 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-577X EI 1873-4979 J9 MATER LETT JI Mater. Lett. PD AUG 15 PY 2014 VL 129 BP 57 EP 60 DI 10.1016/j.matlet.2014.05.001 PG 4 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AL0LQ UT WOS:000338818800016 ER PT J AU Sarkar, M Kumar, A Tumuluru, JS Patil, KN Bellmer, DD AF Sarkar, Madhura Kumar, Ajay Tumuluru, Jaya Shankar Patil, Krushna N. Bellmer, Danielle D. TI Gasification performance of switchgrass pretreated with torrefaction and densification SO APPLIED ENERGY LA English DT Article DE Torrefaction; Densification; Gasification; Efficiency; Switchgrass; Biofuels ID FLUIDIZED-BED GASIFICATION; HYDROGEN-RICH GAS; OIL PALM FRONDS; BIOMASS GASIFICATION; STEAM GASIFICATION; SYNGAS PRODUCTION; PILOT-SCALE; GASIFIER; AIR; WOOD AB The purpose of this study was to investigate gasification performance of four switchgrass pretreatments (torrefaction at 230 and 270 degrees C, densification, and combined torrefaction and densification) and three gasification temperatures (700, 800 and 900 degrees C). Gasification was performed in a fixed-bed externally heated reactor with air as an oxidizing agent. Switchgrass pretreatment and gasification temperature had significant effects on gasification performance such as gas yields, syngas lower heating value (LHV), and carbon conversion and cold gas efficiencies. With an increase in the gasification temperature, yields of H-2 and CO, syngas LHV, and gasifier efficiencies increased whereas CH4, CO2 and N-2 yields decreased. Among all switchgrass pretreatments, gasification performance of switchgrass with combined torrefaction and densification was the best followed by that of densified, raw and torrefied switchgrass. Gasification of combined torrefied and densified switchgrass resulted in the highest yields of H-2 (0.03 kg/ kg biomass) and CO (0.72 kg/kg biomass), highest syngas LHV (5.08 MJ m(-3)), CCE (92.53%), and CGE (68.40%) at the gasification temperature of 900 degrees C. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Sarkar, Madhura; Kumar, Ajay; Patil, Krushna N.; Bellmer, Danielle D.] Oklahoma State Univ, Dept Biosyst & Agr Engn, Stillwater, OK 74078 USA. [Tumuluru, Jaya Shankar] Idaho Natl Lab, Biofuels & Renewable Energy Div, Idaho Falls, ID 83415 USA. RP Kumar, A (reprint author), 228 Agr Hall, Stillwater, OK 74078 USA. EM ajay.kumar@okstate.edu FU South Central Sun Grant Center FX This project was funded by the South Central Sun Grant Center. The authors appreciate assistance from Mr. Wayne Kiner and his group, for their help in building the reactor. Authors would like to thank Micheal C. Clark and Craig C. Conner of Idaho National Laboratory for supporting the torrefaction and pelleting work. NR 54 TC 24 Z9 25 U1 4 U2 36 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD AUG 15 PY 2014 VL 127 BP 194 EP 201 DI 10.1016/j.apenergy.2014.04.027 PG 8 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AJ7DX UT WOS:000337858500019 ER PT J AU Liu, B Braiman, Y Nair, N Lu, Y Guo, Y Colet, P Wardlaw, M AF Liu, B. Braiman, Y. Nair, N. Lu, Y. Guo, Y. Colet, P. Wardlaw, M. TI Nonlinear dynamics and synchronization of an array of single mode laser diodes in external cavity subject to current modulation SO OPTICS COMMUNICATIONS LA English DT Article DE Diode laser array; Nonlinear dynamics; Synchronization ID WEAK PERIODIC PERTURBATIONS; SEMICONDUCTOR-LASERS; HIGH-POWER; OPTICAL FEEDBACK; TALBOT CAVITY; COHERENT ADDITION; PHASE-LOCKING; CHAOS; INJECTION; DISORDER AB We study the dynamics of an array of single mode laser diodes subject to filtered feedback provided by an external reflection grating. Our numerical simulations show that by modulating the injection current the array can be phase synchronized leading to high power coherent emission. The output peak power density can be varied by tuning the modulation frequency and can be resonantly enhanced once the frequency matches the inverse of external cavity round trip time and mode-locking behavior is realized. Both non-resonant and resonant injection current modulation results in an excellent degree of phase synchronization and coherence at certain modulation amplitudes and frequencies that is manifested by coherent enhancement of far-field optical intensity. (C) 2014 Elsevier B.V. All rights reserved. C1 [Liu, B.; Braiman, Y.; Nair, N.] Oak Ridge Natl Lab, Ctr Engn Sci Adv Res, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Liu, B.; Braiman, Y.; Nair, N.] Univ Tennessee, Dept Mechan Aerosp & Biomed Engn, Knoxville, TN 37996 USA. [Lu, Y.; Guo, Y.] Stevens Inst Technol, Dept Elect & Comp Engn, Hoboken, NJ 07030 USA. [Colet, P.] CSIC UIB, IFISC, E-07122 Palma de Mallorca, Spain. [Wardlaw, M.] Off Naval Res, Maritime Sensing, Arlington, VA 22203 USA. RP Braiman, Y (reprint author), Oak Ridge Natl Lab, Ctr Engn Sci Adv Res, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. EM braimany@ornl.gov RI Colet, Pere/A-2472-2011 OI Colet, Pere/0000-0002-5992-6292 FU Office of Naval Research, National Science Foundation [EFRI 1024660]; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, U.S. Department of Energy [DE-AC05-00OR22725]; MINECO, Spain; FEDER [F152012-30634, TEC2012-36335]; Comunitat Autonoma de les Illes Balears FX This research was supported in parts by the Office of Naval Research, National Science Foundation under grant EFRI#1024660, and the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725, PC acknowledges financial support from MINECO, Spain, and FEDER under Projects F152012-30634 (INTENSE@COSYP) and TEC2012-36335 (TRIPHOP) and by Comunitat Autonoma de les Illes Balears. NR 50 TC 1 Z9 1 U1 3 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0030-4018 EI 1873-0310 J9 OPT COMMUN JI Opt. Commun. PD AUG 15 PY 2014 VL 324 BP 301 EP 310 DI 10.1016/j.optcom.2014.03.001 PG 10 WC Optics SC Optics GA AI6GC UT WOS:000336969100050 ER PT J AU Berryman, JG AF Berryman, James G. TI Computing elastic constants for random polycrystals of orthotropic MgSiO3, related polymorphs, and CaIrO3 analogs SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Hashin-Shtrikman bounds; Self-sonsistent estimates; Elastic constants of random polycrystals ID HASHIN-SHTRIKMAN BOUNDS; DETERMINING EFFECTIVE MODULI; TETRAGONAL SYMMETRIES; VARIATIONAL METHOD; PHASE; CONDUCTIVITY; PEROVSKITE; BULK AB Recent advances in methods for computing both Hashin-Shtrikman bounds and related self-consistent (i.e., coherent potential approximation, or CPA) estimates of the geomechanical constants for polycrystals composed of randomly oriented crystals have been successfully applied to orthotropic MgSiO3-perovskite, post-perovskite, and some related CaIrO3 analogs. In particular, Hashin-Shtrikman bounds provide significantly tighter constraints on the average polycrystal behavior than do the traditional Voigt and Reuss bounds. Self-consistent estimates of effective bulk and shear moduli always lie inside the Hashin-Shtrikman (HS) bounds, unlike the Voigt-Reuss-Hill estimates which might lie inside the HS bounds for some examples, but more typically lie outside these same HashinShtrikman bounds. The discrepancies observed between Voigt-Reuss-Hill estimators and the self-consistent, geometric mean, or Hashin-Shtrikman estimates are nevertheless often small in the examples treated here, being on the order of about 1 percent or less - for both the effective bulk and shear moduli. Percentage discrepancies are also observed to be typically less for the effective shear modulus than for the bulk modulus. This result presumably follows from the method's implicit averaging over five distinct shear-like modes, including three true shear modes (due to twisting excitations) and two quasi-shear modes related to shearing action of uniaxially applied stress or strain. (C) 2013 Published by Elsevier Inc. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Berryman, JG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Road MS74R316C, Berkeley, CA 94720 USA. EM jgberryman@lbl.gov NR 43 TC 2 Z9 2 U1 2 U2 21 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD AUG 15 PY 2014 VL 271 BP 379 EP 396 DI 10.1016/j.jcp.2013.06.038 PG 18 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AI1NW UT WOS:000336618800020 ER PT J AU Xue, TY Cui, XQ Guan, WM Wang, QY Liu, C Wang, HT Qi, K Singh, DJ Zheng, WT AF Xue, Tianyu Cui, Xiaoqiang Guan, Weiming Wang, Qiyu Liu, Chang Wang, Haitao Qi, Kun Singh, D. J. Zheng, Weitao TI Surface plasmon resonance technique for directly probing the interaction of DNA and graphene oxide and ultra-sensitive biosensing SO BIOSENSORS & BIOELECTRONICS LA English DT Article DE DNA; Graphene oxide; Hydrogen bond; Surface plasmon resonance; Au nanoparticles ID LABEL-FREE DETECTION; AU NANOPARTICLES; MULTILAYER FILMS; NUCLEIC-ACIDS; LIVING CELLS; FLUORESCENCE; MICROARRAYS; NANOPROBE; STRATEGY; SWITCH AB The binding of DNA with graphene oxide (GO) is important for applications in disease diagnosis, genetic screening, and drug discovery. The standard assay methods are mainly limited to indirect observation via fluorescence labeling. Here we report the use of surface plasmon resonance for direct sensing of DNA/GO binding. We show that this can be used for ultra-sensitive detection of single-stranded DNA (ssDNA). Furthermore, the results provide a more direct probe of DNA/GO binding abilities and confirm that hydrogen bonding plays a key role in the interaction between GO and ssDNA. This enables to a novel biosensor for highly sensitive and selective detection of ssDNA based on indirect competitive inhibition assay (ICIA). We report development of such a sensor with a linear dynamic range of 10(-14)-10(-6) M a detection limit of 10 fM and a high level of stability during repeated regeneration. (C) 2014 Elsevier B.V. All rights reserved. C1 [Xue, Tianyu; Cui, Xiaoqiang; Wang, Qiyu; Liu, Chang; Wang, Haitao; Qi, Kun; Zheng, Weitao] Jilin Univ, Dept Mat Sci, Key Lab Automobile Mat MOE, Changchun 130012, Peoples R China. [Xue, Tianyu; Cui, Xiaoqiang; Wang, Qiyu; Liu, Chang; Wang, Haitao; Qi, Kun; Zheng, Weitao] Jilin Univ, Dept Mat Sci, State Key Lab Superhard Mat, Changchun 130012, Peoples R China. [Guan, Weiming] State Key Lab Adv Technol Comprehens Utilizat Pla, Kunming 650106, Peoples R China. [Singh, D. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Cui, XQ (reprint author), Jilin Univ, Dept Mat Sci, Key Lab Automobile Mat MOE, Changchun 130012, Peoples R China. EM xqcui@jlu.edu.cn; wtzheng@jlu.edu.cn OI zheng, weitao/0000-0002-9028-278X FU National Natural Science Foundation of China [21275064, 21075051, 51372095]; Program for New Century Excellent Talents in University [NCET-10-0433]; State Key Laboratory of Advanced Technologies for Comprehensive Utilization of Platinum Metals [SKL-SPM-201207]; Fundamental Research Funds for the Jilin University [200903020]; 211 Project of Jilin University, China; Department of Energy, Basic Energy Sciences, Materials Sciences and Technology Division; 985 Project of Jilin University, China FX This work was financially supported by the National Natural Science Foundation of China (Nos. 21275064, 21075051, and 51372095), Program for New Century Excellent Talents in University (NCET-10-0433), the State Key Laboratory of Advanced Technologies for Comprehensive Utilization of Platinum Metals (SKL-SPM-201207), the Fundamental Research Funds for the Jilin University (Grant no. 200903020), and the "211" and "985" Projects of Jilin University, China. Work at ORNL was supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Technology Division. NR 56 TC 25 Z9 25 U1 11 U2 195 PU ELSEVIER ADVANCED TECHNOLOGY PI OXFORD PA OXFORD FULFILLMENT CENTRE THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0956-5663 EI 1873-4235 J9 BIOSENS BIOELECTRON JI Biosens. Bioelectron. PD AUG 15 PY 2014 VL 58 BP 374 EP 379 DI 10.1016/j.bios.2014.03.002 PG 6 WC Biophysics; Biotechnology & Applied Microbiology; Chemistry, Analytical; Electrochemistry; Nanoscience & Nanotechnology SC Biophysics; Biotechnology & Applied Microbiology; Chemistry; Electrochemistry; Science & Technology - Other Topics GA AH4PG UT WOS:000336109900055 PM 24686149 ER PT J AU Wang, ZH Fu, YB Zhang, ZC Yuan, SW Amine, K Battaglia, V Liu, G AF Wang, Zhihui Fu, Yanbao Zhang, Zhengcheng Yuan, Shengwen Amine, Khalil Battaglia, Vincent Liu, Gao TI Application of Stabilized Lithium Metal Powder (SLMP (R)) in graphite anode - A high efficient prelithiation method for lithium-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Stabilized Lithium Metal Powder; Prelithiation; Graphite anode; Solid electrolyte interface formation; Lithium-ion battery ID PERFORMANCE; CATHODE AB Stabilized Lithium Metal Powder (SLMP (R)) was applied in graphite anode and the effects of this prelithiation method to cell performance were investigated. Performance of prelithiated cells was compared with that of regular graphite based cells. The first cycle capacity loss of SLMP prelithiated cell was largely reduced and the corresponding first cycle Coulombic efficiency was significantly improved. The graphite/NMC cell with SLMP prelithiation but without any standard cell formation process showed better cycle performance than that of none SLMP containing cell with standard formation process. Prelithiation of graphite electrode with SLMP promote stable solid electrolyte interface (SEI) formation on the surface of graphite anode. Application of SLMP in lithium-ion battery thus provides an effective method to enhance capacity, and promises a low cost SEI formation process. This also implies the potential use of other promising anode materials, such as Si and Sn that have large first cycle capacity loss, in commercial lithium-ion batteries. Published by Elsevier B.V. C1 [Wang, Zhihui; Fu, Yanbao; Battaglia, Vincent; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Zhang, Zhengcheng; Yuan, Shengwen; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM gliu@lbl.gov RI Fu, Yanbao/F-9583-2011 OI Fu, Yanbao/0000-0001-7752-680X FU Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy under the Industry-Laboratory Integrated Research Program (ILIRP); Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231] FX This research was funded by the Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy under the Industry-Laboratory Integrated Research Program (ILIRP) and Batteries for Advanced Transportation Technologies (BATT) Program under the contract no. DE-AC02-05CH11231. FMC-Lithium Co. is a partner of this project. NR 12 TC 20 Z9 20 U1 25 U2 159 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 15 PY 2014 VL 260 BP 57 EP 61 DI 10.1016/j.jpowsour.2014.02.112 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AG7VG UT WOS:000335626300009 ER PT J AU Shadike, Z Zhou, YN Ding, F Sang, L Nam, KW Yang, XQ Fu, ZW AF Shadike, Zulipiya Zhou, Yong-Ning Ding, Fei Sang, Lin Nam, Kyung-Wan Yang, Xiao-Qing Fu, Zheng-Wen TI The new electrochemical reaction mechanism of Na/FeS2 cell at ambient temperature SO JOURNAL OF POWER SOURCES LA English DT Article DE FeS2; Sodium ion battery; Charge reaction mechanism; Hydrothermal synthesis ID X-RAY-ABSORPTION; LITHIUM BATTERIES; ROOM-TEMPERATURE; IRON FLUORIDE; FES2; CATHODE; XAFS AB FeS2 synthesized by hydrothermal method was used for sodium batteries for the first time. A large initial discharge capacity of 771 mAh g(-1) and a high reversible capacity of 521 mAh g(-1) were obtained. The reaction mechanism of electrochemical de-sodiation (charge) was investigated after the initial discharge. Our results have demonstrated that the composition and structure of electrode after the charging to 3.0 V could not recover its original state of FeS2 and a new phase of NaFeS2 was revealed. This should be responsible to the large irreversible capacity in the first cycle and the high discharge and charge plateaus after the initial cycle. (C) 2014 Elsevier B.V. All rights reserved. C1 [Shadike, Zulipiya; Fu, Zheng-Wen] Fudan Univ, Dept Chem, Shanghai Key Lab Mol Catalysts & Innovat Mat, Shanghai 200433, Peoples R China. [Shadike, Zulipiya; Fu, Zheng-Wen] Fudan Univ, Laser Chem Inst, Shanghai 200433, Peoples R China. [Zhou, Yong-Ning; Nam, Kyung-Wan; Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Ding, Fei; Sang, Lin] Tianjin Inst Power Sources, Natl Key Lab Sci & Technol Power Sources, Tianjin 300384, Peoples R China. RP Fu, ZW (reprint author), Fudan Univ, Dept Chem, Shanghai Key Lab Mol Catalysts & Innovat Mat, Shanghai 200433, Peoples R China. EM xyang@bnl.gov; zwfu@fudan.edu.cn RI Zhou, Yong-Ning/I-9579-2014; Nam, Kyung-Wan/B-9029-2013; Nam, Kyung-Wan/E-9063-2015; Fu, Zheng-wen/I-5880-2016 OI Nam, Kyung-Wan/0000-0001-6278-6369; Nam, Kyung-Wan/0000-0001-6278-6369; FU National Foundation of China [B1120132029]; U.S. Department of Energy; Assistant Secretary for Energy Efficiency and Renewable Energy; Office of Vehicle Technologies under Contract [DE-ACO2-98CH10886]; 973 Program of China [2011CB933300]; Science & Technology Commission of Shanghai Municipality [08DZ2270500, 11JC1400500] FX This work was financially supported by 973 Program (No. 2011CB933300) of China, Science & Technology Commission of Shanghai Municipality (08DZ2270500 and 11JC1400500), and National Foundation of China (No. B1120132029). The work at Brookhaven National Laboratory was supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies under Contract Number DE-ACO2-98CH10886. The authors acknowledge technical supports by the beamline scientists at X14A and X19A at NSLS, BNL. NR 13 TC 18 Z9 18 U1 21 U2 175 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 15 PY 2014 VL 260 BP 72 EP 76 DI 10.1016/j.jpowsour.2014.03.011 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AG7VG UT WOS:000335626300011 ER PT J AU Tulio, AZ Jablonski, JE Jackson, LS Chang, C Edirisinghe, I Burton-Freeman, B AF Tulio, Artemio Z., Jr. Jablonski, Joseph E. Jackson, Lauren S. Chang, Claire Edirisinghe, Indika Burton-Freeman, Britt TI Phenolic composition, antioxidant properties, and endothelial cell function of red and white cranberry fruits (Retracted article. See vol. 166, pg. 514, 2015) SO FOOD CHEMISTRY LA English DT Article; Retracted Publication DE Cranberry; Phenolic compounds; Antioxidants; Anthocyanins; Proanthocyanidins; Flavonols; Phenolic acids; Endothelial cell function; p-Akt; Cell migration; Tube formation ID FIMBRIATED ESCHERICHIA-COLI; DEPENDENT RELAXATION; VACCINIUM-MACROCARPON; INHIBIT ADHERENCE; CAPACITY; EXTRACT; PROANTHOCYANIDINS; ANTHOCYANINS; PROCYANIDINS; VALIDATION AB The effects of phenolic constituents in red cranberry extracts (RCE) and white cranberry extracts (WCE) on the endothelial cell function were investigated. Peonidin-3-O-galactoside, cyanidin-3-O-arabinoside, and cyanidin-3-O-galactoside were the predominant anthocyanins characterized, whereas a procyanidin tetramer was the predominant proanthocyanidin identified. The antioxidant properties of RCE and WCE were not significantly different regardless of antioxidant assays (DPPH, FRAP, and TEAC) used. Both RCE and WCE induced the phosphorylation of Akt in vitro in human umbilical endothelial cells (HUVEC), resulting in the phosphorylation of endothelial nitric oxide synthase, cell migration, and tube formation. The enhanced phosphorylation of PI3/Akt kinase in HUVEC, endothelial cell wound healing, and tube formation elicited by RCE and WCE suggest that overall phenolic constituents rather than individual phenolic compounds within the cranberry matrix may be responsible for these biological effects. Published by Elsevier Ltd. C1 [Tulio, Artemio Z., Jr.; Jablonski, Joseph E.; Jackson, Lauren S.; Chang, Claire] US FDA, Ctr Food Safety & Appl Nutr, Bedford Pk, IL 60501 USA. [Chang, Claire] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA. [Edirisinghe, Indika; Burton-Freeman, Britt] IIT, Inst Food Safety & Hlth, Bedford Pk, IL 60501 USA. RP Tulio, AZ (reprint author), US FDA, Ctr Food Safety & Appl Nutr, 6502 South Archer Rd, Bedford Pk, IL 60501 USA. EM artemio.tulio@fda.hhs.gov NR 29 TC 4 Z9 4 U1 3 U2 78 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0308-8146 EI 1873-7072 J9 FOOD CHEM JI Food Chem. PD AUG 15 PY 2014 VL 157 BP 540 EP 552 DI 10.1016/j.foodchem.2014.02.047 PG 13 WC Chemistry, Applied; Food Science & Technology; Nutrition & Dietetics SC Chemistry; Food Science & Technology; Nutrition & Dietetics GA AF8NT UT WOS:000334973600073 PM 24679816 ER PT J AU Ma, SG Liaw, PK Gao, MC Qiao, JW Wang, ZH Zhang, Y AF Ma, S. G. Liaw, P. K. Gao, M. C. Qiao, J. W. Wang, Z. H. Zhang, Y. TI Damping behavior of AlxCoCrFeNi high-entropy alloys by a dynamic mechanical analyzer SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE High-entropy alloy; Dynamical mechanical property; Damping behavior; Modulus ID BULK METALLIC GLASSES; FE-AL ALLOYS; MULTICOMPONENT ALLOYS; PHASE-FORMATION; SOLID-SOLUTION; MICROSTRUCTURE; RELAXATION; ELEMENTS; DESIGN; SYSTEM AB For the first time, the damping behavior of high-entropy alloys was studied using the dynamic-mechanical analyzer, over a continuous heating temperature from room temperature to 773 K, at a given frequency range from 1 to 16 Hz in model alloys AlxCoCrFeNi (x = 0, 0.25, 0.5, 0.75, and 1). The experimental results reveal that the Al-rich alloys have a much smaller elastic storage- modulus amplitude over the temperature and thus a larger resistance to structural relaxation, while the Al-free and Al-lean alloys exhibit a much higher loss tangent and thus a much higher damping capability. Overall the elastic storage modulus decreases while the loss tangent increases with increasing the temperature, but little dependence was observed for the frequency. Several visible internal-friction peaks were presented in the face-centered cubic alloys, whose positions and heights are independent of the frequency. The damping capability of these alloys can be comparable to or even overwhelm the conventional Fe-Al alloys. The damping behavior above was proposed to be agreeable with the level of ordering (eta) of alloys characterized by two proposed parameters (the relative-entropy effect, Omega, and the atomic-size difference, delta). (C) 2014 Elsevier B.V. All rights reserved. C1 [Ma, S. G.; Wang, Z. H.] Taiyuan Univ Technol, Inst Appl Mech & Biomed Engn, Taiyuan 030024, Peoples R China. [Liaw, P. K.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Gao, M. C.] Natl Energy Technol Lab, Albany, OR 97321 USA. [Gao, M. C.] USR Corp, Albany, OR 97321 USA. [Qiao, J. W.] Taiyuan Univ Technol, Coll Mat Sci & Technol, Lab Appl Phys & Mech Adv Mat, Taiyuan 030024, Peoples R China. [Zhang, Y.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. RP Ma, SG (reprint author), Taiyuan Univ Technol, Inst Appl Mech & Biomed Engn, Taiyuan 030024, Peoples R China. EM mashengguo@tyut.edu.cn; drzhangy@ustb.edu.cn RI ZHANG, Yong/B-7928-2009 OI ZHANG, Yong/0000-0002-6355-9923 FU National Natural Science Foundation of China [51101110, 51371122, 11390362]; Shanxi Scholarship Council of China [2012-032]; US National Science Foundation [DMR-0909037, CMMI-0900271, CMMI-1100080]; Department of Energy Office of Nuclear Energy's University Programs (NEUP) [00119262]; Innovative Processing and Technologies Program of the National Energy Technology Laboratory's (NETL) Strategic Center for Coal under the RES contract [DE-FE-0004000]; Top Young Academic Leaders of Shanxi; Outstanding Innovative Teams of Higher Learning Institutions of Shanxi FX J.W. Qiao would like to acknowledge the financial support of the National Natural Science Foundation of China (No. 51101110 and No. 51371122) and Research Project supported by Shanxi Scholarship Council of China (No. 2012-032). P. K. Liaw appreciates the support from the US National Science Foundation (DMR-0909037, CMMI-0900271, and CMMI-1100080) and the Department of Energy Office of Nuclear Energy's University Programs (NEUP) 00119262. M.C. Gao acknowledges the support of the Innovative Processing and Technologies Program of the National Energy Technology Laboratory's (NETL) Strategic Center for Coal under the RES contract DE-FE-0004000. Z.H. Wang would like to acknowledge the financial support of the National Natural Science Foundation of China (No. 11390362), the Top Young Academic Leaders of Shanxi and the Outstanding Innovative Teams of Higher Learning Institutions of Shanxi. NR 51 TC 14 Z9 14 U1 15 U2 102 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD AUG 15 PY 2014 VL 604 BP 331 EP 339 DI 10.1016/j.jallcom.2014.03.050 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AG6CH UT WOS:000335505600051 ER PT J AU Bassiri-Gharb, N Kalinin, SV Valanoor, N AF Bassiri-Gharb, Nazanin Kalinin, Sergei V. Valanoor, Nagarajan TI Preface to Special Topic: Piezoresponse force microscopy and nanoscale phenomena in polar materials SO JOURNAL OF APPLIED PHYSICS LA English DT Editorial Material ID THIN-FILMS; FERROELECTRIC SURFACES; MULTIFERROICS; BIFEO3; HETEROSTRUCTURES; NANOSTRUCTURES; RESOLUTION; PROSPECTS; MEMORIES; DYNAMICS C1 [Bassiri-Gharb, Nazanin] Georgia Inst Technol, GW Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Kalinin, Sergei V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN USA. [Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Valanoor, Nagarajan] Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia. RP Valanoor, N (reprint author), Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia. EM sergei2@ornl.gov; nagarajan@unsw.edu.au RI valanoor, nagarajan/B-4159-2012; Bassiri-Gharb, Nazanin/F-1783-2011; Kalinin, Sergei/I-9096-2012 OI Bassiri-Gharb, Nazanin/0000-0002-0183-5160; Kalinin, Sergei/0000-0001-5354-6152 NR 69 TC 1 Z9 1 U1 2 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 14 PY 2014 VL 116 IS 6 AR 066701 DI 10.1063/1.4891444 PG 5 WC Physics, Applied SC Physics GA AO2TR UT WOS:000341179400078 ER PT J AU Monfared, SK Oro, DM Grover, M Hammerberg, JE LaLone, BM Pack, CL Schauer, MM Stevens, GD Stone, JB Turley, WD Buttler, WT AF Monfared, S. K. Oro, D. M. Grover, M. Hammerberg, J. E. LaLone, B. M. Pack, C. L. Schauer, M. M. Stevens, G. D. Stone, J. B. Turley, W. D. Buttler, W. T. TI Experimental observations on the links between surface perturbation parameters and shock-induced mass ejection SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INDUCED POLYMORPHIC TRANSITION; PARTICLE-SIZE DISTRIBUTIONS; LOADED SN; TIN; METALS AB We have assembled together our ejecta measurements from explosively shocked tin acquired over a period of about ten years. The tin was cast at 0.99995 purity, and all of the tin targets or samples were shocked to loading pressures of about 27 GPa, allowing meaningful comparisons. The collected data are markedly consistent, and because the total ejected mass scales linearly with the perturbations amplitudes they can be used to estimate how much total Sn mass will be ejected from explosively shocked Sn, at similar loading pressures, based on the surface perturbation parameters of wavelength and amplitude. Most of the data were collected from periodic isosceles shapes that approximate sinusoidal perturbations. Importantly, however, we find that not all periodic perturbations behave similarly. For example, we observed that sawtooth (right triangular) perturbations eject more mass than an isosceles perturbation of similar depth and wavelength, demonstrating that masses ejected from irregular shaped perturbations cannot be normalized to the cross-sectional areas of the perturbations. (C) 2014 AIP Publishing LLC. C1 [Monfared, S. K.; Oro, D. M.; Hammerberg, J. E.; Pack, C. L.; Schauer, M. M.; Stone, J. B.; Buttler, W. T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Grover, M.; LaLone, B. M.; Stevens, G. D.; Turley, W. D.] Natl Secur Technol, Special Technol Lab, Santa Barbara, CA 93117 USA. RP Monfared, SK (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. FU U.S. Department of Energy; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX By acceptance of this article, the publisher recognizes that the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or to allow others to do so, for U. S. Government purposes. Los Alamos National Laboratory requests that the publisher identify this article as work performed under the auspices of the U.S. Department of Energy.; Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 44 TC 11 Z9 11 U1 5 U2 16 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 14 PY 2014 VL 116 IS 6 AR 063504 DI 10.1063/1.4891449 PG 11 WC Physics, Applied SC Physics GA AO2TR UT WOS:000341179400013 ER PT J AU Morozovska, AN Eliseev, EA Ievlev, AV Varenyk, OV Pusenkova, AS Chu, YH Shur, VY Strikha, MV Kalinin, SV AF Morozovska, Anna N. Eliseev, Eugene A. Ievlev, Anton V. Varenyk, Olexander V. Pusenkova, Anastasiia S. Chu, Ying-Hao Shur, Vladimir Ya Strikha, Maksym V. Kalinin, Sergei V. TI Ferroelectric domain triggers the charge modulation in semiconductors (invited) SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DEVICES; FILMS AB We consider a typical heterostructure "domain patterned ferroelectric film-ultra-thin dielectric layer-semiconductor," where the semiconductor can be an electrolyte, paraelectric or multi-layered graphene. Unexpectedly, we have found that the space charge modulation profile and amplitude in the semiconductor, that screens the spontaneous polarization of a 180-deg domain structure of ferroelectric, depends on the domain structure period, dielectric layer thickness and semiconductor screening radius in a rather non-trivial nonlinear way. Multiple size effects appearance and manifestation are defined by the relationship between these three parameters. In addition, we show that the concept of effective gap can be introduced in a simple way only for a single-domain limit. Obtained analytical results open the way for understanding of current-AFM maps of contaminated ferroelectric surfaces in ambient atmosphere as well as explore the possibilities of conductivity control in ultra-thin semiconductor layers. (C) 2014 AIP Publishing LLC. C1 [Morozovska, Anna N.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Morozovska, Anna N.; Strikha, Maksym V.] Natl Acad Sci Ukraine, Inst Semicond Phys, UA-03028 Kiev, Ukraine. [Eliseev, Eugene A.] Natl Acad Sci Ukraine, Inst Problems Mat Sci, UA-03142 Kiev, Ukraine. [Ievlev, Anton V.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Ievlev, Anton V.; Shur, Vladimir Ya] Ural Fed Univ, Ekaterinburg 620000, Russia. [Varenyk, Olexander V.] Taras Shevchenko Kyiv Natl Univ, Radiophys Fac, UA-03022 Kiev, Ukraine. [Pusenkova, Anastasiia S.] Taras Shevchenko Kyiv Natl Univ, Fac Phys, UA-03022 Kiev, Ukraine. [Chu, Ying-Hao] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu, Taiwan. [Chu, Ying-Hao] Acad Sinica, Inst Phys, Taipei 105, Taiwan. RP Shur, VY (reprint author), Ural Fed Univ, 51 Lenina Ave, Ekaterinburg 620000, Russia. EM vladimir.shur@urfu.ru; maksym_strikha@hotmail.com; sergei2@ornl.gov RI Kalinin, Sergei/I-9096-2012; Ievlev, Anton/H-3678-2012; Ying-Hao, Chu/A-4204-2008; OI Kalinin, Sergei/0000-0001-5354-6152; Ievlev, Anton/0000-0003-3645-0508; Ying-Hao, Chu/0000-0002-3435-9084; Strikha, Maksym/0000-0002-2380-0305 FU bilateral SFFR-NSF project (U.S. National Science Foundation) [NSF-DMR-1210588]; bilateral SFFR-NSF project (State Fund of Fundamental Research of Ukraine) [UU48/002]; National Academy of Sciences of Ukraine [35-02-14]; State Fund of Fundamental Research of Ukraine [53.2/006]; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Russian Foundation of Basic Research [14-02-92709 Ind-a] FX A.N.M. and E. A. E. acknowledge the support via bilateral SFFR-NSF project (U.S. National Science Foundation under NSF-DMR-1210588 and State Fund of Fundamental Research of Ukraine, Grant No. UU48/002) and National Academy of Sciences of Ukraine (Grant No. 35-02-14). M. V. S. acknowledges State Fund of Fundamental Research of Ukraine, Grant No. 53.2/006. The part of research (A. V. I. and S. V. K.) was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. S. V. K. acknowledges Office of Basic Energy Sciences, U.S. Department of Energy. Y.H.C acknowledge the National Science Council, R.O.C. (NSC-101-2119-M-009-003-MY2), Ministry of Education (MOE-ATU 101W961), and Center for Interdisciplinary Science of National Chiao Tung University. V.Y.S. acknowledges the Russian Foundation of Basic Research (Grant No. 14-02-92709 Ind-a). NR 46 TC 5 Z9 5 U1 6 U2 34 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 14 PY 2014 VL 116 IS 6 AR 066817 DI 10.1063/1.4891310 PG 11 WC Physics, Applied SC Physics GA AO2TR UT WOS:000341179400095 ER PT J AU Morozovska, AN Eliseev, EA Varenyk, OV Kim, Y Strelcov, E Tselev, A Morozovsky, NV Kalinin, SV AF Morozovska, Anna N. Eliseev, Eugene A. Varenyk, Olexandr V. Kim, Yunseok Strelcov, Evgheni Tselev, Alexander Morozovsky, Nicholas V. Kalinin, Sergei V. TI Nonlinear space charge dynamics in mixed ionic-electronic conductors: Resistive switching and ferroelectric-like hysteresis of electromechanical response SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INTERCALATION-INDUCED STRESS; PHASE-TRANSITION PATHWAYS; BATTERY CATHODE; NANOSCALE; TRANSPORT; PARTICLES; EVOLUTION; MEMRISTOR; DEVICES; MOTION AB We performed self-consistent modelling of nonlinear electrotransport and electromechanical response of thin films of mixed ionic-electronic conductors (MIEC) allowing for steric effects of mobile charged defects (ions, protons, or vacancies), electron degeneration, and Vegard stresses. We establish correlations between the features of the nonlinear space-charge dynamics, current-voltage, and bending-voltage curves for different types of the film electrodes. A pronounced ferroelectric-like hysteresis of the bending-voltage loops and current maxima on the double hysteresis current-voltage loops appear for the electron-transport electrodes. The double hysteresis loop with pronounced humps indicates a memristor-type resistive switching. The switching occurs due to the strong nonlinear coupling between the electronic and ionic subsystems. A sharp meta-stable maximum of the electron density appears near one open electrode and moves to another one during the periodic change of applied voltage. Our results can explain the nonlinear nature and correlation of electrical and mechanical memory effects in thin MIEC films. The analytical expression proving that the electrically induced bending of MIEC films can be detected by interferometric methods is derived. (C) 2014 AIP Publishing LLC. C1 [Morozovska, Anna N.; Morozovsky, Nicholas V.] NAS Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Eliseev, Eugene A.] NAS Ukraine, Inst Problems Mat Sci, UA-03028 Kiev, Ukraine. [Varenyk, Olexandr V.] Taras Shevchenko Kyiv Natl Univ, Radiophys Fac 4, UA-03022 Kiev, Ukraine. [Kim, Yunseok] Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, Suwon 440746, South Korea. [Kim, Yunseok; Strelcov, Evgheni; Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Morozovska, AN (reprint author), NAS Ukraine, Inst Phys, 46 Pr Nauki, UA-03028 Kiev, Ukraine. RI Strelcov, Evgheni/H-1654-2013; Tselev, Alexander/L-8579-2015; Kalinin, Sergei/I-9096-2012 OI Tselev, Alexander/0000-0002-0098-6696; Kalinin, Sergei/0000-0001-5354-6152 FU bilateral SFFR-NSF project (US National Science Foundation) [NSF-DMR-1210588]; bilateral SFFR-NSF project (State Fund of Fundamental of Fundamental Research of Ukraine) [UU48/002]; Center for Nanophase Materials Sciences, Oak Ridge National Laboratory [CNMS2013-293]; Office of Basic Energy Sciences, U.S. Department of Energy FX A.N.M. and E.A.E. are grateful to Professor Long-Qing Chen for useful remarks. A.N.M. and E. A. E. acknowledge the support via bilateral SFFR-NSF project (US National Science Foundation under NSF-DMR-1210588 and State Fund of Fundamental of Fundamental Research of Ukraine, Grant UU48/002). S. V. K., E. S., and A. T acknowledge the Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, user agreement CNMS2013-293 and S. V. K. and A. T. acknowledges the Office of Basic Energy Sciences, U.S. Department of Energy. NR 59 TC 4 Z9 4 U1 5 U2 54 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 14 PY 2014 VL 116 IS 6 AR 066808 DI 10.1063/1.4891346 PG 11 WC Physics, Applied SC Physics GA AO2TR UT WOS:000341179400086 ER PT J AU Mundoor, H Lee, T Gann, DG Ackerman, PJ Senyuk, B van de Lagemaat, J Smalyukh, II AF Mundoor, Haridas Lee, Taewoo Gann, Derek G. Ackerman, Paul J. Senyuk, Bohdan van de Lagemaat, Jao Smalyukh, Ivan I. TI Optically and elastically assembled plasmonic nanoantennae for spatially resolved characterization of chemical composition in soft matter systems using surface enhanced spontaneous and stimulated Raman scattering SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LIQUID-CRYSTALS; GOLD NANOPARTICLES; SPECTROSCOPY; SERS; MICROSCOPY; MOLECULES; DIMERS; RANGE AB We present a method to locally probe spatially varying chemical composition of soft matter systems by use of optically controlled and elastically self-assembled plasmonic nanoantennae. Disc-shaped metal particles with sharp irregular edges are optically trapped, manipulated, and assembled into small clusters to provide a strong enhancement of the Raman scattering signal coming from the sample regions around and in-between these particles. As the particles are reassembled and spatially translated by computer-controlled laser tweezers, we probe chemical composition as a function of spatial coordinates. This allows us to reliably detect tiny quantities of organic molecules, such as capping ligands present on various nanoparticles, as well as to probe chemical composition of the interior of liquid crystal defect cores that can be filled with, for example, polymer chains. The strong electromagnetic field enhancement of optically manipulated nanoparticles' rough surfaces is demonstrated in different forms of spectroscopy and microscopy, including enhanced spontaneous Raman scattering, coherent anti-Stokes Raman scattering, and stimulated Raman scattering imaging modes. (C) 2014 AIP Publishing LLC. C1 [Mundoor, Haridas; Lee, Taewoo; Gann, Derek G.; Ackerman, Paul J.; Senyuk, Bohdan; Smalyukh, Ivan I.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [van de Lagemaat, Jao; Smalyukh, Ivan I.] Natl Renewable Energy Lab, Renewable & Sustainable Energy Inst, Boulder, CO 80309 USA. [van de Lagemaat, Jao; Smalyukh, Ivan I.] Univ Colorado, Boulder, CO 80309 USA. [van de Lagemaat, Jao] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Smalyukh, Ivan I.] Univ Colorado, Dept Elect Comp & Energy Engn, Boulder, CO 80309 USA. [Smalyukh, Ivan I.] Univ Colorado, Mat Sci Engn Program, Boulder, CO 80309 USA. RP van de Lagemaat, J (reprint author), Natl Renewable Energy Lab, Renewable & Sustainable Energy Inst, Boulder, CO 80309 USA. EM Jao.vandeLagemaat@nrel.gov; ivan.smalyukh@colorado.edu RI van de Lagemaat, Jao/J-9431-2012; Senyuk, Bohdan/M-3185-2014; Smalyukh, Ivan/C-2955-2011; Mundoor, Haridas/L-9948-2016 OI Senyuk, Bohdan/0000-0002-0004-3161; Smalyukh, Ivan/0000-0003-3444-1966; Mundoor, Haridas/0000-0001-6589-6475 FU Institute for Complex Adaptive Matter; NSF [DMR-0847782, DMR-0844115]; Office of Basic Energy Sciences of the US Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX This work was supported by the branch contributions of the Institute for Complex Adaptive Matter (H. M.), the NSF grants DMR-0847782 (T. L., B. S., and I. I. S.) and DMR-0844115 (H. M. and I. I. S.), and by the Office of Basic Energy Sciences of the US Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory (J.v.d.L., P.J.A., and H.M.). NR 21 TC 3 Z9 3 U1 3 U2 27 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 14 PY 2014 VL 116 IS 6 AR 063511 DI 10.1063/1.4892932 PG 7 WC Physics, Applied SC Physics GA AO2TR UT WOS:000341179400020 ER PT J AU Varley, JB Lordi, V AF Varley, J. B. Lordi, V. TI Intermixing at the absorber-buffer layer interface in thin-film solar cells: The electronic effects of point defects in Cu(In,Ga)(Se,S)(2) and Cu2ZnSn(Se,S)(4) devices SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID II-VI COMPOUNDS; DETECTED MAGNETIC-RESONANCE; BATH DEPOSITION PROCESS; FAST DIFFUSERS; CDS; CU(IN,GA)SE-2; EFFICIENCY; ZNS; CU; CUINSE2 AB We investigate point defects in the buffer layers CdS and ZnS that may arise from intermixing with Cu(In,Ga)(S,Se)(2) (CIGS) or Cu2ZnSn(S,Se)(4) (CZTS) absorber layers in thin-film photovoltaics. Using hybrid functional calculations, we characterize the electrical and optical behavior of Cu, In, Ga, Se, Sn, Zn, Na, and K impurities in the buffer. We find that In and Ga substituted on the cation site act as shallow donors in CdS and tend to enhance the prevailing n-type conductivity at the interface facilitated by Cd incorporation in CIGS, whereas they are deep donors in ZnS and will be less effective dopants. Substitutional In and Ga can favorably form complexes with cation vacancies (A-centers) which may contribute to the "red kink" effect observed in some CIGS-based devices. For CZTS absorbers, we find that Zn and Sn defects substituting on the buffer cation site are electrically inactive in n-type buffers and will not supplement the donor doping at the interface as in CIGS/CdS or ZnS devices. Sn may also preferentially incorporate on the S site as a deep acceptor in n-type ZnS, which suggests possible concerns with absorber-related interfacial compensation in CZTS devices with ZnS-derived buffers. Cu, Na, and K impurities are found to all have the same qualitative behavior, most favorably acting as compensating acceptors when substituting on the cation site. Our results suggest one beneficial role of K and Na incorporation in CIGS or CZTS devices is the partial passivation of vacancy-related centers in CdS and ZnS buffers, rendering them less effective interfacial hole traps and recombination centers. (C) 2014 AIP Publishing LLC. C1 [Varley, J. B.; Lordi, V.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Varley, JB (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. OI Lordi, Vincenzo/0000-0003-2415-4656 FU U.S. Department of Energy at Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE office of Energy Efficiency and Renewable Energy (EERE) through the SunShot Bridging Research Interactions through collaborative Development Grants in Energy (BRIDGE) program FX We gratefully acknowledge useful discussions with G. Brown, K. Demirkan, N. Mackie, J. L. Lyons, X. He, and A. Rockett. This work was performed under the auspices of the U.S. Department of Energy at Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, funded by the DOE office of Energy Efficiency and Renewable Energy (EERE) through the SunShot Bridging Research Interactions through collaborative Development Grants in Energy (BRIDGE) program. NR 72 TC 7 Z9 7 U1 8 U2 86 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 14 PY 2014 VL 116 IS 6 AR 063505 DI 10.1063/1.4892407 PG 9 WC Physics, Applied SC Physics GA AO2TR UT WOS:000341179400014 ER PT J AU Lin, KH Holian, BL Germann, TC Strachan, A AF Lin, Keng-Hua Holian, Brad Lee Germann, Timothy C. Strachan, Alejandro TI Mesodynamics with implicit degrees of freedom SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DISSIPATIVE PARTICLE DYNAMICS; MOLECULAR-DYNAMICS; ENERGY-CONSERVATION; DETONATION-WAVES; REDUCED MODEL; HEAT; PHASE; DECOMPOSITION; SIMULATION; SHOCK AB Mesoscale phenomena-involving a level of description between the finest atomistic scale and the macroscopic continuum-can be studied by a variation on the usual atomistic-level molecular dynamics (MD) simulation technique. In mesodynamics, the mass points, rather than being atoms, are mesoscopic in size, for instance, representing the centers of mass of polycrystalline grains or molecules. In order to reproduce many of the overall features of fully atomistic MD, which is inherently more expensive, the equations of motion in mesodynamics must be derivable from an interaction potential that is faithful to the compressive equation of state, as well as to tensile decohesion that occurs along the boundaries of the mesoscale units. Moreover, mesodynamics differs from Newton's equations of motion in that dissipation-the exchange of energy between mesoparticles and their internal degrees of freedom (DoFs)-must be described, and so should the transfer of energy between the internal modes of neighboring mesoparticles. We present a formulation where energy transfer between the internal modes of a mesoparticle and its external center-of-mass DoFs occurs in the phase space of mesoparticle coordinates, rather than momenta, resulting in a Galilean invariant formulation that conserves total linear momentum and energy (including the energy internal to the mesoparticles). We show that this approach can be used to describe, in addition to mesoscale problems, conduction electrons in atomic-level simulations of metals, and we demonstrate applications of mesodynamics to shockwave propagation and thermal transport. (C) 2014 AIP Publishing LLC. C1 [Lin, Keng-Hua; Strachan, Alejandro] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Lin, Keng-Hua; Strachan, Alejandro] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Holian, Brad Lee; Germann, Timothy C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, KH (reprint author), Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. OI Germann, Timothy/0000-0002-6813-238X FU ASC Materials and Physics Modeling Program at Los Alamos National Laboratory; U.S. National Science Foundation (NSF) [ECCS-1028667] FX K.-H.L. and A. S. acknowledge the insightful comments from Dr. Edwin Antillon. This work was supported by the ASC Materials and Physics Modeling Program at Los Alamos National Laboratory and by the U.S. National Science Foundation (NSF), Grant No. ECCS-1028667. NR 55 TC 8 Z9 8 U1 2 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2014 VL 141 IS 6 AR 064107 DI 10.1063/1.4891308 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OH UT WOS:000340713700009 PM 25134551 ER PT J AU Manaa, MR Kuo, IFW Fried, LE AF Manaa, M. Riad Kuo, I-Feng W. Fried, Laurence E. TI First-principles high-pressure unreacted equation of state and heat of formation of crystal 2,6-diamino-3, 5-dinitropyrazine-1-oxide (LLM-105) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; ELECTRONIC-STRUCTURE; AB-INITIO; TATB; DYNAMICS; 2,6-DIAMINO-3,5-DINITROPYRAZINE-1-OXIDE; 1,3,5-TRIAMINO-2,4,6-TRINITROBENZENE; PSEUDOPOTENTIALS; TRANSFORMATION; PERFORMANCE AB We report dispersion-corrected density functional theoretical calculations of the unreacted equation of state (EOS) of crystal 2,6-diamino-3, 5-dinitropyrazine-1-oxide (LLM-105) under hydrostatic compression of up to 45 GPa. Convergence tests for k-points sampling in the Brillouin zone show that a 3 x 1 x 2 mesh is required to reproduce the X-ray crystal structure at ambient conditions, and we confirm our finding with a separate supercell calculation. Our high-pressure EOS yields a bulk modulus of 19.2 GPa, and indicates a tendency towards anisotropic compression along the b lattice vector due to molecular orientations within the lattice. We find that the electronic energy band gap decreases from a semiconductor type of 1.3 eV at 0 GPa to quasi-metallic type of 0.6 eV at 45 GPa. The extensive intermolecular hydrogen bonds involving the oxide (-NO) and dioxide (-NO2) interactions with the amine (-NH2) group showed enhanced interactions with increasing pressure that should be discernible in the mid IR spectral region. We do not find evidence for structural phase transitions or chemically induced transformations within the pressure range of our study. The gas phase heat of formation is calculated at the G4 level of theory to be 22.48 kcal/mol, while we obtain 25.92 kcal/mol using the ccCA-PS3 method. Density functional theory calculations of the crystal and the gas phases provided an estimate for the heat of sublimation of 32.4 kcal/mol. We thus determine the room-temperature solid heat of formation of LLM-105 to be -9.9 or -6.5 kcal/mol based on the G4 or ccCA-PS3 methods, respectively. (C) 2014 AIP Publishing LLC. C1 [Manaa, M. Riad; Kuo, I-Feng W.; Fried, Laurence E.] Lawrence Livermore Natl Lab, Energet Mat Ctr, Livermore, CA 94551 USA. RP Manaa, MR (reprint author), Lawrence Livermore Natl Lab, Energet Mat Ctr, Livermore, CA 94551 USA. EM manaa1@llnl.gov RI Fried, Laurence/L-8714-2014 OI Fried, Laurence/0000-0002-9437-7700 FU U.S. Department of Energy Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Advanced Scientific Computation (ASC) program FX This work is performed under the auspices of the U.S. Department of Energy Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Support from the Advanced Scientific Computation (ASC) program and computational resources via the Computational Grand Challenge Program are greatly appreciated. NR 57 TC 3 Z9 4 U1 4 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2014 VL 141 IS 6 AR 064702 DI 10.1063/1.4891933 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OH UT WOS:000340713700043 PM 25134585 ER PT J AU Shepard, R Gidofalvi, G Brozell, SR AF Shepard, Ron Gidofalvi, Gergely Brozell, Scott R. TI The multifacet graphically contracted function method. I. Formulation and implementation SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MATRIX RENORMALIZATION-GROUP; CORRELATED MOLECULAR CALCULATIONS; NONLINEAR-WAVE FUNCTIONS; UNITARY-GROUP APPROACH; GAUSSIAN-BASIS SETS; DOUBLE-ZETA BASIS; CONFIGURATION-INTERACTION; PROGRAM SYSTEM; QUANTUM-CHEMISTRY; FULL CI AB The basic formulation for the multifacet generalization of the graphically contracted function (MFGCF) electronic structure method is presented. The analysis includes the discussion of linear dependency and redundancy of the arc factor parameters, the computation of reduced density matrices, Hamiltonian matrix construction, spin-density matrix construction, the computation of optimization gradients for single-state and state-averaged calculations, graphical wave function analysis, and the efficient computation of configuration state function and Slater determinant expansion coefficients. Timings are given for Hamiltonian matrix element and analytic optimization gradient computations for a range of model problems for full-CI Shavitt graphs, and it is observed that both the energy and the gradient computation scale as O(N(2)n(4)) for N electrons and n orbitals. The important arithmetic operations are within dense matrix-matrix product computational kernels, resulting in a computationally efficient procedure. An initial implementation of the method is used to present applications to several challenging chemical systems, including N-2 dissociation, cubic H-8 dissociation, the symmetric dissociation of H2O, and the insertion of Be into H-2. The results are compared to the exact full-CI values and also to those of the previous single-facet GCF expansion form. (C) 2014 AIP Publishing LLC. C1 [Shepard, Ron; Brozell, Scott R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Gidofalvi, Gergely] Gonzaga Univ, Dept Chem & Biochem, Spokane, WA 99258 USA. RP Shepard, R (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. FU Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy [DE-AC02-06CH11357]; Research Corporation for Science Advancement; Howard Hughes Medical Institute through the Undergraduate Science Education Program FX This work was supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy, under Contract No. DE-AC02-06CH11357. G. G. was supported by an award from the Research Corporation for Science Advancement and a grant to Gonzaga University from the Howard Hughes Medical Institute through the Undergraduate Science Education Program. S. R. B. acknowledges the use of computational facilities at the Ohio Supercomputer Center. NR 50 TC 11 Z9 11 U1 0 U2 7 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2014 VL 141 IS 6 AR 064105 DI 10.1063/1.4890734 PG 26 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OH UT WOS:000340713700007 PM 25134549 ER PT J AU Shepard, R Gidofalvi, G Brozell, SR AF Shepard, Ron Gidofalvi, Gergely Brozell, Scott R. TI The multifacet graphically contracted function method. II. A general procedure for the parameterization of orthogonal matrices and its application to arc factors SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID OPTIMIZATION; ALGORITHMS AB Practical algorithms are presented for the parameterization of orthogonal matrices Q is an element of R (mxn) in terms of the minimal number of essential parameters {phi}. Both square n = m and rectangular n < m situations are examined. Two separate kinds of parameterizations are considered, one in which the individual columns of Q are distinct, and the other in which only Span(Q) is significant. The latter is relevant to chemical applications such as the representation of the arc factors in the multifacet graphically contracted function method and the representation of orbital coefficients in SCF and DFT methods. The parameterizations are represented formally using products of elementary Householder reflector matrices. Standard mathematical libraries, such as LAPACK, may be used to perform the basic low-level factorization, reduction, and other algebraic operations. Some care must be taken with the choice of phase factors in order to ensure stability and continuity. The transformation of gradient arrays between the Q and {phi} parameterizations is also considered. Operation counts for all factorizations and transformations are determined. Numerical results are presented which demonstrate the robustness, stability, and accuracy of these algorithms. (C) 2014 AIP Publishing LLC. C1 [Shepard, Ron; Brozell, Scott R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Gidofalvi, Gergely] Gonzaga Univ, Dept Chem & Biochem, Spokane, WA 99258 USA. RP Shepard, R (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. FU Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy [DE-AC02-06CH11357]; Research Corporation for Science Advancement; Howard Hughes Medical Institute through the Undergraduate Science Education Program FX This work was supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy, under Contract No. DE-AC02-06CH11357. G. G. was supported by an award from the Research Corporation for Science Advancement and a grant to Gonzaga University from the Howard Hughes Medical Institute through the Undergraduate Science Education Program. S.R.B. acknowledges the use of computational facilities at the Ohio Supercomputer Center. NR 18 TC 5 Z9 5 U1 0 U2 6 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2014 VL 141 IS 6 AR 064106 DI 10.1063/1.4890735 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OH UT WOS:000340713700008 PM 25134550 ER PT J AU Werhahn, JC Akase, D Xantheas, SS AF Werhahn, Jasper C. Akase, Dai Xantheas, Sotiris S. TI Universal scaling of potential energy functions describing intermolecular interactions. II. The halide-water and alkali metal-water interactions SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID EFFECTIVE IONIC-RADII; BASIS-SETS; WAVE-FUNCTIONS; PSEUDOPOTENTIALS; SPECTROSCOPY; COMPLEXES; HYDRATION; CRYSTALS; ATOMS; HYDROGEN AB The scaled versions of the newly introduced [S. S. Xantheas and J. C. Werhahn, J. Chem. Phys. 141, 064117 (2014)] generalized forms of some popular potential energy functions (PEFs) describing intermolecular interactions - Mie, Lennard-Jones, Morse, and Buckingham exponential-6 - have been used to fit the ab initio relaxed approach paths and fixed approach paths for the halide-water, X-(H2O), X = F, Cl, Br, I, and alkali metal-water, M+ (H2O), M = Li, Na, K, Rb, Cs, interactions. The generalized forms of those PEFs have an additional parameter with respect to the original forms and produce fits to the ab initio data that are between one and two orders of magnitude better in the chi(2) than the original PEFs. They were found to describe both the long-range, minimum and repulsive wall of the respective potential energy surfaces quite accurately. Overall the 4-parameter extended Morse (eM) and generalized Buckingham exponential-6 (gBe-6) potentials were found to best fit the ab initio data for these two classes of ion-water interactions. The fitted values of the parameter of the (eM) and (gBe-6) PEFs that control the repulsive wall of the potential correlate remarkably well with the ionic radii of the halide and alkali metal ions. (C) 2014 AIP Publishing LLC. C1 [Werhahn, Jasper C.] Tech Univ Munich, Phys Dept E11, D-85748 Garching, Germany. [Akase, Dai] Hiroshima Univ, Ctr Quantum Life Sci, Higashihiroshima 7398526, Japan. [Akase, Dai] Hiroshima Univ, Grad Sch Sci, Dept Chem, Higashihiroshima 7398526, Japan. [Xantheas, Sotiris S.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Xantheas, SS (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999,MS K1-83, Richland, WA 99352 USA. EM sotiris.xantheas@pnnl.gov RI Xantheas, Sotiris/L-1239-2015; OI Xantheas, Sotiris/0000-0002-6303-1037 FU International Max Planck Research School on Advanced Photon Science; U.S. Department of Energy; Japan Society for the Promotion of Science (JSPS) through the Strategic Young Researcher Overseas Visits Program; Technische Universitat Munchen at Garching-Institute for Advanced Study; German Excellence Initiative; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Department of Energy's Office of Biological and Environmental Research; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX J.C.W. thanks the International Max Planck Research School on Advanced Photon Science for a graduate fellowship and the U.S. Department of Energy for additional financial support during his visit to PNNL. D. A. acknowledges support from the Japan Society for the Promotion of Science (JSPS) through the Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation. S. S. X. acknowledges the support, via a Visiting Fellowship, of the Technische Universitat Munchen at Garching-Institute for Advanced Study, funded by the German Excellence Initiative and Professor A. Laubereau for his hospitality. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. A portion of this research was performed using the Molecular Science Computing Facility (MSCF) in EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. This research also used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 7 Z9 7 U1 1 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2014 VL 141 IS 6 AR 064118 DI 10.1063/1.4891820 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OH UT WOS:000340713700020 PM 25134562 ER PT J AU Xantheas, SS Werhahn, JC AF Xantheas, Sotiris S. Werhahn, Jasper C. TI Universal scaling of potential energy functions describing intermolecular interactions. I. Foundations and scalable forms of new generalized Mie, Lennard-Jones, Morse, and Buckingham exponential-6 potentials SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID STATISTICAL-MECHANICS; CORRESPONDING STATES; CONDENSING SYSTEMS; THERMODYNAMIC PROPERTIES; REACTION SURFACE; CYCLOPROPYLIDENE; VAPORIZATION; FEATURES; EQUATION; LIQUIDS AB Based on the formulation of the analytical expression of the potential V(r) describing intermolecular interactions in terms of the dimensionless variables r* = r/r(m) and epsilon* = V/epsilon, where r(m) is the separation at the minimum and e the well depth, we propose more generalized scalable forms for the commonly used Mie, Lennard-Jones, Morse, and Buckingham exponential-6 potential energy functions. These new generalized forms have an additional parameter from the original forms and revert to the original ones for some choice of that parameter. In this respect, the original forms of those potentials can be considered as special cases of the more general forms that are introduced. We also propose a scalable, non-revertible to the original one, 4-parameter extended Morse potential. (C) 2014 AIP Publishing LLC. C1 [Xantheas, Sotiris S.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Werhahn, Jasper C.] Tech Univ Munich, Phys Dept E11, D-85748 Garching, Germany. RP Xantheas, SS (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999,MS K1-83, Richland, WA 99352 USA. EM sotiris.xantheas@pnnl.gov RI Xantheas, Sotiris/L-1239-2015; OI Xantheas, Sotiris/0000-0002-6303-1037 FU Technische Universitat Munchen at Garching Institute for Advanced Study - German Excellence Initiative; International Max Planck Research School on Advanced Photon Science; U.S. Department of Energy; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences FX S.S.X. acknowledges the support, via a Visiting Fellowship, of the Technische Universitat Munchen at Garching Institute for Advanced Study, funded by the German Excellence Initiative and Professor A. Laubereau for his hospitality. J.C.W. thanks the International Max Planck Research School on Advanced Photon Science for a graduate fellowship and the U.S. Department of Energy for additional financial support during his visit to PNNL. We wish to thank Dr. Soohaeng YooWillow for helpful discussions. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. NR 27 TC 9 Z9 9 U1 0 U2 30 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2014 VL 141 IS 6 AR 064117 DI 10.1063/1.4891819 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN6OH UT WOS:000340713700019 PM 25134561 ER PT J AU Bulaevskii, LN Lin, SZ AF Bulaevskii, Lev N. Lin, Shi-Zeng TI Dissipation in Josephson tunneling junctions at low temperatures SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM DYNAMICS AB It is important to know the decoherence mechanism of a qubit based on Josephson junctions. At low temperatures, as quasiparticle concentration becomes exponentially small, one needs to consider energy transfer from tunneling electrons to other degrees of freedom to find dissipation in Josephson junctions and decoherence in qubits. Here we discuss the energy transfer to two-level systems, i.e., the transitions between two different configurations of ions inside an insulating layer separated by a potential barrier. We derive a general equation of motion for the phase difference between two superconducting electrodes and we find a retarded dissipation term due to electromagnetic mechanism and also contribution due to electron tunneling mechanism. Using the equation of motion we calculate the decay of Rabi oscillations and frequency shift in qubits due to the presence of the two-level systems. In the long-time limit our results coincide with those obtained by Martinis et al. [Martinis et al., Phys. Rev. Lett. 95, 210503 (2005)] within the Fermi's Golden Rule approach up to a numerical factor. C1 [Bulaevskii, Lev N.; Lin, Shi-Zeng] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Bulaevskii, LN (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008 OI Lin, Shi-Zeng/0000-0002-4368-5244 FU NNSA of the US DOE at LANL [DE-AC52-06NA25396] FX We acknowledge helpful discussions with V. B. Geshkenbein, G. Blatter, J. Martinis, L. Ioffe, A. Golubov, A. Ustinov, V. Ryazanov, and D. Khmel'nitskii. L.N.B. thanks the Pauli Center, ETH, Zurich, for their hospitality. The work was carried out under the auspices of the NNSA of the US DOE at LANL under Contract No. DE-AC52-06NA25396. NR 17 TC 0 Z9 0 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 14 PY 2014 VL 90 IS 5 AR 054509 DI 10.1103/PhysRevB.90.054509 PG 5 WC Physics, Condensed Matter SC Physics GA AO3SM UT WOS:000341256000004 ER PT J AU Kemper, AF Sentef, MA Moritz, B Freericks, JK Devereaux, TP AF Kemper, A. F. Sentef, M. A. Moritz, B. Freericks, J. K. Devereaux, T. P. TI Effect of dynamical spectral weight redistribution on effective interactions in time-resolved spectroscopy SO PHYSICAL REVIEW B LA English DT Article ID CHARGE-DENSITY-WAVE AB The redistribution of electrons in an ultrafast pump-probe experiment causes significant changes to the spectral distribution of the retarded interaction between electrons and bosonic modes. We study the influence of these changes on pump-probe photoemission spectroscopy for a model electron-phonon coupled system using the nonequilibrium Keldysh formalism. We show that spectral rearrangement due to the driving field preserves an overall sum rule for the electronic self-energy, but modifies the effective electron-phonon scattering as a function of energy. Experimentally, this pump-modified scattering can be tracked by analyzing the fluence or excitation energy dependence of population decay rates and transient changes in dispersion kinks. C1 [Kemper, A. F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Sentef, M. A.; Moritz, B.; Devereaux, T. P.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Moritz, B.] Univ N Dakota, Dept Phys & Astrophys, Grand Forks, ND 58202 USA. [Freericks, J. K.] Georgetown Univ, Dept Phys, Washington, DC 20057 USA. [Devereaux, T. P.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. RP Kemper, AF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM afkemper@lbl.gov RI Sentef, Michael/L-5717-2013; Moritz, Brian/D-7505-2015; Kemper, Alexander/F-8243-2016; OI Sentef, Michael/0000-0002-7946-0282; Moritz, Brian/0000-0002-3747-8484; Kemper, Alexander/0000-0002-5426-5181; Freericks, James/0000-0002-6232-9165 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (DMSE) [DE-AC02-76SF00515, DE-FG02-08ER46542, DE-SC0007091]; U.S. Department of Energy, Office of Science [DE-AC02-05CH11231]; McDevitt bequest at Georgetown FX We would like to thank P. Kirchmann, J. Sobota, and S. Yang for helpful discussions. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (DMSE), under Contracts No. DE-AC02-76SF00515 (Stanford/SIMES), No. DE-FG02-08ER46542 (Georgetown), and No. DE-SC0007091 (for the collaboration). Computational resources were provided by the National Energy Research Scientific Computing Center supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-05CH11231. J.K.F. was supported by the McDevitt bequest at Georgetown. NR 28 TC 19 Z9 19 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 14 PY 2014 VL 90 IS 7 AR 075126 DI 10.1103/PhysRevB.90.075126 PG 7 WC Physics, Condensed Matter SC Physics GA AO3SR UT WOS:000341256600003 ER PT J AU Nefkens, BMK Prakhov, S Aguar-Bartolome, P Annand, JRM Arends, HJ Bantawa, K Beck, R Bekrenev, V Berghauser, H Braghieri, A Briscoe, WJ Brudvik, J Cherepnya, S Codling, RFB Collicott, C Costanza, S Danilkin, IV Denig, A Demissie, B Dieterle, M Downie, EJ Drexler, P Fil'kov, LV Fix, A Garni, S Glazier, DI Gregor, R Hamilton, D Heid, E Hornidge, D Howdle, D Jahn, O Jude, TC Kashevarov, VL Kaser, A Keshelashvili, I Kondratiev, R Korolija, M Kotulla, M Koulbardis, A Kruglov, S Krusche, B Lisin, V Livingston, K MacGregor, IJD Maghrbi, Y Mancel, J Manley, DM McNicoll, EF Mekterovic, D Metag, V Mushkarenkov, A Nikolaev, A Novotny, R Oberle, M Ortega, H Ostrick, M Ott, P Otte, PB Oussena, B Pedroni, P Polonski, A Robinson, J Rosner, G Rostomyan, T Schumann, S Sikora, MH Starostin, A Strakovsky, II Strub, T Suarez, IM Supek, I Tarbert, CM Thiel, M Thomas, A Unverzagt, M Watts, DP Werthmuller, D Witthauer, L AF Nefkens, B. M. K. Prakhov, S. Aguar-Bartolome, P. Annand, J. R. M. Arends, H. J. Bantawa, K. Beck, R. Bekrenev, V. Berghaeuser, H. Braghieri, A. Briscoe, W. J. Brudvik, J. Cherepnya, S. Codling, R. F. B. Collicott, C. Costanza, S. Danilkin, I. V. Denig, A. Demissie, B. Dieterle, M. Downie, E. J. Drexler, P. Fil'kov, L. V. Fix, A. Garni, S. Glazier, D. I. Gregor, R. Hamilton, D. Heid, E. Hornidge, D. Howdle, D. Jahn, O. Jude, T. C. Kashevarov, V. L. Kaeser, A. Keshelashvili, I. Kondratiev, R. Korolija, M. Kotulla, M. Koulbardis, A. Kruglov, S. Krusche, B. Lisin, V. Livingston, K. MacGregor, I. J. D. Maghrbi, Y. Mancel, J. Manley, D. M. McNicoll, E. F. Mekterovic, D. Metag, V. Mushkarenkov, A. Nikolaev, A. Novotny, R. Oberle, M. Ortega, H. Ostrick, M. Ott, P. Otte, P. B. Oussena, B. Pedroni, P. Polonski, A. Robinson, J. Rosner, G. Rostomyan, T. Schumann, S. Sikora, M. H. Starostin, A. Strakovsky, I. I. Strub, T. Suarez, I. M. Supek, I. Tarbert, C. M. Thiel, M. Thomas, A. Unverzagt, M. Watts, D. P. Werthmueller, D. Witthauer, L. CA A2 Collaboration MAMI TI New measurement of the rare decay eta -> pi(0)gamma gamma with the Crystal Ball/TAPS detectors at the Mainz Microtron SO PHYSICAL REVIEW C LA English DT Article ID TAGGED PHOTON SPECTROMETER; MAMI; TAPS AB A new measurement of the rare, doubly radiative decay eta -> pi(0)gamma gamma was conducted with the Crystal Ball and TAPS multiphoton spectrometers together with the photon tagging facility at the Mainz Microtron MAMI. New data on the dependence of the partial decay width, Gamma(eta -> pi(0)gamma gamma), on the two-photon invariant-mass squared, m(2)(gamma gamma), as well as a new, more precise value for the decay width, Gamma(eta -> pi(0)gamma gamma) = (0.33 +/- 0.03(tot)) eV, are based on analysis of 1.2 x 10(3) eta -> pi(0)gamma gamma decays from a total of 6 x 10(7) eta. mesons produced in the gamma p -> eta p reaction. The present results for d Gamma(eta -> pi(0)gamma gamma)/dm(2)(gamma gamma) are in good agreement with previous measurements and recent theoretical calculations for this dependence. C1 [Nefkens, B. M. K.; Prakhov, S.; Brudvik, J.; Starostin, A.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Prakhov, S.; Aguar-Bartolome, P.; Arends, H. J.; Denig, A.; Downie, E. J.; Heid, E.; Jahn, O.; Kashevarov, V. L.; Ortega, H.; Ostrick, M.; Ott, P.; Otte, P. B.; Oussena, B.; Schumann, S.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Briscoe, W. J.; Demissie, B.; Downie, E. J.; Heid, E.; Strakovsky, I. I.] George Washington Univ, Washington, DC 20052 USA. [Annand, J. R. M.; Codling, R. F. B.; Glazier, D. I.; Hamilton, D.; Howdle, D.; Livingston, K.; MacGregor, I. J. D.; Mancel, J.; Robinson, J.; Rosner, G.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Bantawa, K.; Manley, D. M.] Kent State Univ, Kent, OH 44242 USA. [Beck, R.; Nikolaev, A.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Bekrenev, V.; Koulbardis, A.; Kruglov, S.] Petersburg Nucl Phys Inst, petnuc-, Gatchina 188350, Russia. [Berghaeuser, H.; Drexler, P.; Gregor, R.; Kotulla, M.; Metag, V.; Novotny, R.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Braghieri, A.; Costanza, S.; Mushkarenkov, A.; Pedroni, P.] INFN Ses Pavia, I-27100 Pavia, Italy. [Cherepnya, S.; Fil'kov, L. V.; Kashevarov, V. L.] PN Lebedev Phys Inst, Moscow 119991, Russia. [Collicott, C.] Dalhousie Univ, Halifax, NS B3H 4R2, Canada. [Collicott, C.] St Marys Univ, Halifax, NS B3H 3C3, Canada. [Danilkin, I. V.] Jefferson Lab, Newport News, VA 23606 USA. [Dieterle, M.; Garni, S.; Kaeser, A.; Keshelashvili, I.; Krusche, B.; Maghrbi, Y.; Oberle, M.; Rostomyan, T.; Strub, T.] Univ Basel, Dept Phys, CH-4056 Basel, Switzerland. [Fix, A.] Tomsk Polytech Univ, Phys Math Lab, Tomsk 634050, Russia. [Glazier, D. I.; Jude, T. C.; Sikora, M. H.] Univ Edinburgh, Sch Phys, SUPA, Edinburgh EH9 3JZ, Midlothian, Scotland. [Hornidge, D.] Mt Allison Univ, Sackville, NB E4L 1E6, Canada. [Kondratiev, R.; Lisin, V.; Polonski, A.] Inst Nucl Res, Moscow 125047, Russia. [Korolija, M.; Mekterovic, D.] Rudjer Boskovic Inst, HR-10000 Zagreb, Croatia. RP Nefkens, BMK (reprint author), Univ Calif Los Angeles, Los Angeles, CA 90095 USA. EM prakhov@ucla.edu RI MacGregor, Ian/D-4072-2011; Fil'kov, Lev/M-8648-2015; Kashevarov, Victor/O-2260-2015; Cherepnya, Sergey/N-2636-2015 FU Deutsche Forschungsgemeinschaft [SFB443, SFB/TR16, SFB1044]; DFG-RFBR [09-02-91330]; European Community-Research Infrastructure Activity [RII3-CT-2004-506078]; Schweizerischer National fonds; UK Science and Technology Facilities Council [STFC 57071/1, 50727/1]; U.S. Department of Energy; National Science Foundation; INFN (Italy); NSERC (Canada); U.S. Department of Energy [DE-AC05-06OR23177]; Russian Federation federal program "Kadry" [P691]; MSE Program "Nauka" [1.604.2011] FX Entries The authors are indebted to the late B.M.K. Nefkens for bringing the Crystal Ball to MAMI and for setting up an extensive program of photo-induced meson-decay experiments. Without this, the present measurement of eta -> pi0gamma gamma would not have been possible. The authors wish to acknowledge the excellent support of the accelerator group and operators of MAMI. This work was supported by the Deutsche Forschungsgemeinschaft (SFB443, SFB/TR16, and SFB1044), DFG-RFBR (Grant No. 09-02-91330), the European Community-Research Infrastructure Activity under the FP6 "Structuring the European Research Area" program (Hadron Physics, Contract No. RII3-CT-2004-506078), Schweizerischer National fonds, the UK Science and Technology Facilities Council (Grant No. STFC 57071/1, 50727/1), the U.S. Department of Energy and National Science Foundation, INFN (Italy), and NSERC (Canada). The work of I.V. Danilkin is supported by the U.S. Department of Energy (Contract No. DE-AC05-06OR23177). A. Fix acknowledges additional support from the Russian Federation federal program "Kadry" (Contract No. P691) and the MSE Program "Nauka" (Contract No. 1.604.2011). We thank the undergraduate students of Mount Allison University and The George Washington University for their assistance. NR 23 TC 1 Z9 1 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 14 PY 2014 VL 90 IS 2 AR 025206 DI 10.1103/PhysRevC.90.025206 PG 9 WC Physics, Nuclear SC Physics GA AO3SU UT WOS:000341256900003 ER PT J AU Betz, B Gyulassy, M AF Betz, Barbara Gyulassy, Miklos TI Constraints on the path-length dependence of jet quenching in nuclear collisions at RHIC and LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jets; Heavy Ion Phenomenology ID PB-PB COLLISIONS; P(T) AZIMUTHAL ASYMMETRY; TRANSVERSE-MOMENTUM; ENERGY-LOSS; ROOT-S(NN)=2.76 TEV; FLOW; A+A; HADRONS; LIGHT; PQCD AB Recent data on the high-p T pion nuclear modification factor, R-AA (pT), and its elliptic azimuthal asymmetry, v(2) (pT), from RHIC/BNL and LHC/CERN are analyzed in terms of a wide class of jet-energy loss models coupled to different (2+1)d transverse plus Bjorken expanding hydrodynamic fields. We test the consistency of each model by demanding a simultaneous account of the azimuthal, the transverse momentum, and the centrality dependence of the data at both 0.2 and 2.76 ATeV energies. We find a rather broad class of jet-energy independent energy-loss models dE/dx = kappa(T)x(z)T(2+z)zeta q that, when coupled to bulk constrained temperature fields T(x, t), can account for the current data at the chi(2)/d.o.f. <2 level with different temperature-dependent jet-medium couplings, kappa(T), and path-length dependence exponents 0 <= z <= 2. We extend previous studies by including a generic term, 0 < zeta(q) < 2 + q, to test different scenarios of energy-loss fluctuations. While a previously proposed AdS/CFT jet-energy loss model with a temperature-independent jet-medium coupling as well as a near-T-c dominated, pQCD-inspired energy-loss scenario are shown to be inconsistent with the LHC data, once the parameters are constrained by fitting to RHIC results, we find several new solutions with a temperature-dependent kappa(T). We conclude that the current level of statistical and systematic uncertainties of the measured data does not allow a constraint on the path-length exponent z to a range narrower than [0 -2]. C1 [Betz, Barbara] Goethe Univ Frankfurt, Inst Theoret Phys, D-60438 Frankfurt, Germany. [Gyulassy, Miklos] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Gyulassy, Miklos] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Gyulassy, Miklos] HAS, Wigner RCP, Inst Particle & Nucl Phys, H-1121 Budapest, Hungary. RP Betz, B (reprint author), Goethe Univ Frankfurt, Inst Theoret Phys, D-60438 Frankfurt, Germany. EM betz@th.physik.uni-frankfurt.de; gyulassy@phys.columbia.edu FU Helmholtz International Centre for FAIR; US-DOE [DE-FG02-93ER40764, DE-AC02-05CH11231]; MTA Wigner RCP, Budapest FX We are especially grateful to P. Romatschke, U. Heinz, and C. Shen for making their hydrodynamic field grids available. Discussions with J. Xu, A. Ficnar, A. Buzzatti, W. Horowitz, J. Liao, D. Molnar, and X.-N. Wang in the JET Collaboration have been particularly valuable. BB acknowledges financial support received from the Helmholtz International Centre for FAIR within the framework of the LOEWE program (Landesoffensive zur Entwicklung Wissenschaftlich-Okonomischer Exzellenz) launched by the State of Hesse. MG acknowledges support from the US-DOE Nuclear Science Grant No. DE-FG02-93ER40764 and No. DE-AC02-05CH11231 within the framework of the JET Topical Collaboration [6]. The authors also thank the Yukawa Institute for Theoretical Physics, Kyoto University, where part of this work was completed during the YITP-T-13-05 on "New Frontiers in QCD". MG is grateful for partial support from the MTA Wigner RCP, Budapest, during the second half of his sabbatical leave in 2014, where this work was finalized. NR 63 TC 12 Z9 12 U1 0 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 14 PY 2014 IS 8 AR 090 DI 10.1007/JHEP08(2014)090 PG 25 WC Physics, Particles & Fields SC Physics GA AN3MD UT WOS:000340491300004 ER PT J AU Armstrong, MR Zaug, JM Grant, CD Crowhurst, JC Bastea, S AF Armstrong, Michael R. Zaug, Joseph M. Grant, Christian D. Crowhurst, Jonathan C. Bastea, Sorin TI Ultrafast Shock Compression of an Oxygen-Balanced Mixture of Nitromethane and Hydrogen Peroxide SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID EQUATION-OF-STATE; LIQUID NITROMETHANE; PHASE-TRANSITION; SIMULATIONS; CHEMISTRY AB We apply ultrafast optical interferometry to measure the Hugoniot of an oxygen-balanced mixture of nitromethane and hydrogen peroxide (NM/HP) and compare with Hugoniot data for pure nitromethane (NM) and a 90% hydrogen peroxide/water mixture (HP), as well as theoretical predictions. We observe a 2.1% percent mean pairwise difference between the measured shockwave speed (at the measured piston speed) in unreacted NM/HP and the corresponding "universal" liquid Hugoniot, which is larger than the average standard deviation of our data, 1.4%. Unlike the Hugoniots of both HP and NM, in which measured shock speeds deviate to values greater than the unreacted Hugoniot for piston speeds larger than the respective reaction thresholds, in the NM/HP mixture we observe shock speed deviations to values lower than the unreacted Hugoniot well below the von Neumann pressure (approximate to 28 GPa). Although the trend should reverse for high enough piston speeds, the initial behavior is unexpected. Possible explanations range from mixing effects to a complex index of refraction in the reacted solution. If this is indeed a signature of chemical initiation, it would suggest that the process may not be kinetically limited (on a similar to 100 ps time scale) between the initiation threshold and the von Neumann pressure. C1 [Armstrong, Michael R.; Zaug, Joseph M.; Grant, Christian D.; Crowhurst, Jonathan C.; Bastea, Sorin] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Armstrong, MR (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. EM armstrong30@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development grant [11ERD067] FX We acknowledge useful conversations with L. E. Fried, C. Tarver, D. Dlott, and R Manaa. This research was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and it was funded by Laboratory Directed Research and Development grant 11ERD067 with S.B. as principal investigator. NR 33 TC 2 Z9 2 U1 2 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD AUG 14 PY 2014 VL 118 IS 32 BP 6148 EP 6153 DI 10.1021/jp502891p PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AN2TX UT WOS:000340439800002 PM 25012762 ER PT J AU Laurence, TA Ly, S Bourguet, F Fischer, NO Coleman, MA AF Laurence, Ted A. Ly, Sonny Bourguet, Feliza Fischer, Nicholas O. Coleman, Matthew A. TI Fluorescence Correlation Spectroscopy at Micromolar Concentrations without Optical Nanoconfinement SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID CROSS-CORRELATION SPECTROSCOPY; STATISTICAL ACCURACY; FLUCTUATIONS; DIFFUSION; VOLUMES AB Fluorescence correlation spectroscopy (FCS) is an important technique for studying biochemical interactions dynamically that may be used in vitro and in cell-based studies. It is generally claimed that FCS may only be used at nM concentrations. We show that this general consensus is incorrect and that the limitation to nM concentrations is not fundamental but due to detector limits as well as laser fluctuations. With a high count rate detector system and applying laser fluctuation corrections, we demonstrate FCS measurements up to 38 mu M with the same signal-to-noise as at lower concentrations. Optical nanoconfinement approaches previously used to increase the concentration range of FCS are not necessary, and further increases above 38 mu M may be expected using detectors and detector arrays with higher saturation rates and better laser fluctuation corrections. This approach greatly widens the possibilities of dynamic measurements of biochemical interactions using FCS at physiological concentrations. C1 [Laurence, Ted A.; Ly, Sonny; Bourguet, Feliza; Fischer, Nicholas O.; Coleman, Matthew A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Coleman, Matthew A.] Univ Calif Davis, Dept Radiat Oncol, Sacramento, CA 95817 USA. RP Laurence, TA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM laurence2@llnl.gov; ly2@llnl.gov OI Coleman, Matthew/0000-0003-1389-4018 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 within the LDRD program. NR 21 TC 6 Z9 6 U1 1 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 14 PY 2014 VL 118 IS 32 BP 9662 EP 9667 DI 10.1021/jp505881z PG 6 WC Chemistry, Physical SC Chemistry GA AN2VC UT WOS:000340443100013 PM 25060197 ER PT J AU Zhang, F Wood, BC Wang, Y Wang, CZ Ho, KM Chou, MY AF Zhang, Feng Wood, Brandon C. Wang, Yan Wang, Cai-Zhuang Ho, Kai-Ming Chou, Mei-Yin TI Ultrafast Bulk Diffusion of AlHx in High-Entropy Dehydrogenation Intermediates of NaAlH4 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID REVERSIBLE HYDROGEN STORAGE; GENERALIZED GRADIENT APPROXIMATION; ELASTIC NEUTRON-SCATTERING; DENSITY-FUNCTIONAL THEORY; TOTAL-ENERGY CALCULATIONS; POINT-DEFECT DYNAMICS; TI-DOPED NAALH4; WAVE BASIS-SET; SODIUM ALANATE; ALUMINUM HYDRIDES AB Using first-principles molecular dynamics (FPMD) and total-energy calculations, we demonstrate low-barrier bulk diffusion of Al-bearing species in gamma-NaAlH4, a recently proposed high-entropy polymorph of NaAlH4. For charged AlH4- and neutral AlH3 vacancies, the computed barriers for diffusion are <0.1 eV, and we directly observe the predicted diffusive pathways in FPMD simulations at picosecond time scales. In contrast, such diffusion in the alpha phase is inaccessible to FPMD, consistent with much higher barriers. The transport behavior of gamma-NaAlH4, in addition to key dynamical and structural signatures, is consistent with experimental observations of high-mobility species, strongly supporting the idea that an intermediate transition from the alpha phase to a high-entropy polymorph facilitates the hydrogen-releasing decomposition of NaAlH4. Our results provide an answer to longstanding questions regarding the responsible agent for the experimentally observed efficient Al transport during dehydrogenation and suggest that mass transport and phase transformation kinetics are coupled. Implications for understanding the (de)hydrogenation of undoped and catalyzed NaAlH4 are discussed. C1 [Zhang, Feng; Wang, Yan; Chou, Mei-Yin] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Zhang, Feng; Wang, Cai-Zhuang; Ho, Kai-Ming] US DOE, Ames Lab, Ames, IA 50011 USA. [Wood, Brandon C.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Chou, Mei-Yin] Acad Sinica, Inst Atom & Mol Sci, Taipei 10617, Taiwan. RP Chou, MY (reprint author), Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. EM meiyin.chou@physics.gatech.edu RI Chou, Mei-Yin/D-3898-2012 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-97ER45632]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Sampling of the potential energy surface was performed at Georgia Institute of Technology, supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-FG02-97ER45632. These computationally intensive calculations used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy Under Contract No. DE-AC02-05CH11231. Analysis was primarily performed at Ames Laboratory, supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358. The molecular dynamics simulations were performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 46 TC 0 Z9 0 U1 2 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 14 PY 2014 VL 118 IS 32 BP 18356 EP 18361 DI 10.1021/jp504550m PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN2VQ UT WOS:000340444500009 ER PT J AU Seo, DM Boyle, PD Allen, JL Han, SD Jonsson, E Johansson, P Henderson, WA AF Seo, Daniel M. Boyle, Paul D. Allen, Joshua L. Han, Sang-Don Jonsson, Erlendur Johansson, Patrik Henderson, Wesley A. TI Solvate Structures and Computational/Spectroscopic Characterization of LiBF4 Electrolytes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LOW-TEMPERATURE PERFORMANCE; DENSITY-FUNCTIONAL THEORY; LI-ION CELLS; LITHIUM TETRAFLUOROBORATE; FT-RAMAN; CROWN-ETHER; CRYSTAL-STRUCTURES; APROTIC-SOLVENTS; ASSOCIATION; CARBONATE AB Crystal structures have been determined for both LiBF4 and HBF4 solvates: (acetonitrile)(2):LiBF4, (ethylene glycol diethyl ether)(1):LiBF4, (diethylene glycol diethyl ether)(1):LiBF4, (tetrahydrofuran)(1):LiBF4, (methyl methoxyacetate)(1):LiBF4, (succinonitrile)(1):LiBF4, (N,N,N',N '',N ''-pentamethyldiethylenetriamine)(1):HBF4, (N,N,N',N'-tetramethylethylenediamine)(3/2):HBF4, and (phenanthroline)(2):HBF4. These, as well as other known LiBF4 solvate structures, have been characterized by Raman vibrational spectroscopy to unambiguously assign the anion Raman band positions to specific forms of BF4-center dot center dot center dot Li+ cation coordination. In addition, complementary DFT calculations of BF4-center dot center dot center dot Li+ cation complexes have provided additional insight into the challenges associated with accurately interpreting the anion interactions from experimental Raman spectra. This information provides a crucial tool for the characterization of the ionic association interactions within electrolytes. C1 [Seo, Daniel M.; Allen, Joshua L.; Han, Sang-Don; Henderson, Wesley A.] N Carolina State Univ, Dept Chem & Biomol Engn, Ion Liquids & Electrolytes Energy Technol ILEET L, Raleigh, NC 27695 USA. [Boyle, Paul D.] N Carolina State Univ, Dept Chem, Xray Struct Facil, Raleigh, NC 27695 USA. [Jonsson, Erlendur; Johansson, Patrik] Chalmers, Dept Appl Phys, SE-41296 Gothenburg, Sweden. [Henderson, Wesley A.] Pacific NW Natl Lab, Electrochem Mat & Syst Grp, Energy & Environm Directorate, Richland, WA 99352 USA. RP Henderson, WA (reprint author), N Carolina State Univ, Dept Chem & Biomol Engn, Ion Liquids & Electrolytes Energy Technol ILEET L, Raleigh, NC 27695 USA. EM Wesley.Henderson@pnnl.gov RI Johansson, Patrik/A-7660-2010 OI Johansson, Patrik/0000-0002-9907-117X FU U.S. Department of Energy (DOE) Office of Basic Energy Science-Division of Materials Sciences and Engineering [DE-SC0002169]; Swedish Energy Agency via VR/STEM grant FX The authors wish to express their gratitude to the U.S. Department of Energy (DOE) Office of Basic Energy Science-Division of Materials Sciences and Engineering which fully supported the experimental research under Award DE-SC0002169. EJ and PJ would like to thank the Swedish Energy Agency for funding via a VR/STEM grant and SNIC for the allocation of computational resources. NR 61 TC 8 Z9 8 U1 1 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 14 PY 2014 VL 118 IS 32 BP 18377 EP 18386 DI 10.1021/jp5046782 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN2VQ UT WOS:000340444500012 ER PT J AU Gandhiraman, RP Nordlund, D Javier, C Koehne, JE Chen, B Meyyappan, M AF Gandhiraman, Ram P. Nordlund, Dennis Javier, Cristina Koehne, Jessica E. Chen, Bin Meyyappan, M. TI X-ray Absorption Study of Graphene Oxide and Transition Metal Oxide Nanocomposites SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INNER-SHELL EXCITATION; FINE-STRUCTURE SPECTRA; LITHIUM ION BATTERIES; ELECTROPHORETIC DEPOSITION; ELECTROCHEMICAL CAPACITORS; SUPERCAPACITOR ELECTRODES; THIN-FILM; SPECTROSCOPY; ENERGY; PERFORMANCE AB The surface properties of the electrode materials play a crucial role in determining the performance and efficiency of energy storage devices. Graphene oxide and nanostructures of 3d transition metal oxides were synthesized for construction of electrodes in supercapacitors, and the electronic structure and oxidation states were probed using near-edge X-ray absorption fine structure. Understanding the chemistry of graphene oxide would provide valuable insight into its reactivity and properties as the graphene oxide transformation to reduced-graphene oxide is a key step in the synthesis of the electrode materials. Polarized behavior of the synchrotron X-rays and the angular dependency of the near-edge X-ray absorption fine structures (NEXAFS) have been utilized to study the orientation of the sigma and pi bonds of the graphene oxide and graphene oxide-metal oxide nanocomposites. The core-level transitions of individual metal oxides and that of the graphene oxide nanocomposite showed that the interaction of graphene oxide with the metal oxide nanostructures has not altered the electronic structure of either of them. As the restoration of the pi network is important for good electrical conductivity, the C K edge NEXAFS spectra of reduced graphene oxide nanocomposites confirms the same through increased intensity of the sp(2)-derived unoccupied states pi* band. A pronounced angular dependency of the reduced sample and the formation of excitonic peaks confirmed the formation of extended conjugated network. C1 [Gandhiraman, Ram P.; Javier, Cristina; Koehne, Jessica E.; Chen, Bin; Meyyappan, M.] NASA, Ames Res Ctr, Mountain View, CA 94035 USA. [Nordlund, Dennis] Stanford Linear Accelerator Ctr, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. RP Gandhiraman, RP (reprint author), NASA, Ames Res Ctr, Mountain View, CA 94035 USA. EM ramprasad.gandhiraman@nasa.gov RI Gandhiraman, Ram Prasad/B-7004-2013; Nordlund, Dennis/A-8902-2008 OI Gandhiraman, Ram Prasad/0000-0001-8957-7938; Nordlund, Dennis/0000-0001-9524-6908 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE Office of Biological and Environmental Research; National Institutes of Health, National Institute of General Medical Sciences [P41GM103393] FX R.P.G. is with Universities Space Research Association subcontracted to NASA Ames Research Center under NASA cooperative agreement. The beam time for synchrotron measurements was awarded to the authors through the peer-reviewed SLAC research proposal No. 2163. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research and by the National Institutes of Health, National Institute of General Medical Sciences (including P41GM103393). The contents of this publication are solely the responsibility of the authors and do not necessarily represent the official views of NIGMS or NIH. NR 58 TC 7 Z9 7 U1 7 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 14 PY 2014 VL 118 IS 32 BP 18706 EP 18712 DI 10.1021/jp503941t PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN2VQ UT WOS:000340444500051 PM 25152800 ER PT J AU Lopez-Bezanilla, A AF Lopez-Bezanilla, Alejandro TI Substitutional Doping Widens Silicene Gap SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID FIELD-EFFECT TRANSISTORS; ELECTRONIC-PROPERTIES; CARBON NANOTUBES; CHARGE-TRANSPORT; GRAPHENE; CONDUCTANCE; NANOWIRES AB A numerical study of electronic transport properties of doped silicene is presented. By means of ab initio calculations, a self-consistent scattering potential is derived for boron, nitrogen, aluminum, and phosphorus substitutions in silicene, and the quantum-mechanical Landauer-Buttiker approach is used to evaluate the conductivities of doped silicene ribbons with various impurity concentrations. An individual defect introduces asymmetric electron-hole conductivities that depend on both the type of doping and the position of the foreign atom with respect to the edges. Quantum interference effects at zero temperature are modeled to show that randomly distributed defects over 1 mu m long and realistically wide silicon nanoribbons widen the intrinsic electronic gap that arises from quantum confinement. Mobility gaps created at low doping rates may lead to greater efficiency in the design of new silicon-based devices, providing the ability for suitable control of silicon ribbons band gap. C1 Argonne Natl Lab, Lemont, IL 60439 USA. RP Lopez-Bezanilla, A (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Lemont, IL 60439 USA. EM alejandrolb@gmail.com RI Lopez-Bezanilla, Alejandro/B-9125-2015 OI Lopez-Bezanilla, Alejandro/0000-0002-4142-2360 FU DOE-BES [DE-AC02-06CH11357]; DOE (FWP) [70081] FX I gratefully acknowledge the computing resources provided on Blues high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. Work at Argonne is supported by DOE-BES under Contract No. DE-AC02-06CH11357. I acknowledge Glue funding from DOE (FWP#70081). NR 28 TC 9 Z9 9 U1 2 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 14 PY 2014 VL 118 IS 32 BP 18788 EP 18792 DI 10.1021/jp5060809 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AN2VQ UT WOS:000340444500061 ER PT J AU Wanner, C Sonnenthal, EL Liu, XM AF Wanner, Christoph Sonnenthal, Eric L. Liu, Xiao-Ming TI Seawater delta Li-7: A direct proxy for global CO2 consumption by continental silicate weathering? SO CHEMICAL GEOLOGY LA English DT Article DE Li isotopic fractionation; Seawater delta Li-7; Silicate weathering; Reactive transport modeling; CO2 consumption ID LITHIUM ISOTOPIC COMPOSITION; PHANEROZOIC TIME; MACKENZIE BASIN; ATMOSPHERIC CO2; CARBON-DIOXIDE; CLAY-MINERALS; REVISED MODEL; MG ISOTOPES; LI; FRACTIONATION AB The fractionation of stable Li isotopes (Li-6, Li-7) has become a promising proxy for assessing changes related to continental silicate weathering patterns. Recently, the first complete record of Cenozoic seawater Li isotopic composition (delta Li-7) was reported (Misra and Froelich, 2012, Science 335, 818-821) showing a stepwise increase of +9 parts per thousand over the last 56 Ma. This increase was attributed to a general change in continental silicate weathering behavior caused by tectonic uplift. In particular, the low global average riverine delta Li-7 inferred for the Paleocene-Eocene boundary was explained by congruent silicate weathering of primary silicate minerals, which is inconsistent with the stoichiometry of secondary minerals and the resultant water chemistry. In this study, we present a novel reactive transport modeling approach that explicitly includes Li isotopic fractionation to assess alternative geochemically-constrained interpretations that do not rely on congruent weathering. Simulations show that riverine delta Li-7 is mainly controlled by the subsurface residence time, the corresponding weathering intensity, and the concentration of a river's suspended load. Based on these factors, we suspect that the low delta Li-7 observed at the Paleocene-Eocene boundary was inherited from a high weathering intensity with predominant weathering of previously formed secondary mineral phases (e.g., clays, oxides) having low delta Li-7 values. Moreover, we conclude that the Cenozoic delta Li-7 increase was caused by an increasing amount of primary silicate mineral dissolution inherited from an increasing suspended river load concentration and a decreasing weathering intensity both likely induced by tectonic uplift. In contrast, Cenozoic cooling and corresponding pCO(2) and precipitation variations do not seem to have a distinct control on the Cenozoic delta Li-7 record. Finally, our simulations revealed a close relation between delta Li-7 and CO2 consumption by silicate weathering implying that the Cenozoic seawater delta Li-7 record could be potentially used to quantify such CO2 consumption through time. However, more experimental and modeling work is required to quantify the correlation between seawater delta Li-7 and global CO2 consumption by silicate weathering. Key parameters are the temperature-dependent thermodynamic properties of specific Li-bearing primary and secondary minerals (e.g., crystallographic Li substitution reaction, maximum Li substitution, Li solubility, Li isotopic fractionation factor) as well as the determination of global average subsurface and river discharges through time. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wanner, Christoph; Sonnenthal, Eric L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Liu, Xiao-Ming] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Liu, Xiao-Ming] Univ Maryland, Dept Geol, College Pk, MD 20742 USA. RP Wanner, C (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM cwanner@lbl.gov RI Sonnenthal, Eric/A-4336-2009; Liu, Xiaoming/F-5571-2010; OI Wanner, Christoph/0000-0003-3488-8602 FU U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office [GT-480010-12]; Carnegie Institution of Washington FX This work was supported by the U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office, award no. GT-480010-12. Postdoctoral fellowship support was provided to X-ML by the Carnegie Institution of Washington. The manuscript significantly benefited from a helpful editorial handling by Michael Bottcher, and very constructive comments by Philip Pogge von Strandmann and an additional, anonymous reviewer. NR 76 TC 20 Z9 20 U1 3 U2 40 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD AUG 14 PY 2014 VL 381 BP 154 EP 167 DI 10.1016/j.chemgeo.2014.05.005 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AM9NO UT WOS:000340208500014 ER PT J AU Barker, AJ Douglas, TA Jacobson, AD McClelland, JW Ilgen, AG Khosh, MS Lehn, GO Trainor, TP AF Barker, Amanda J. Douglas, T. A. Jacobson, A. D. McClelland, J. W. Ilgen, A. G. Khosh, M. S. Lehn, G. O. Trainor, T. P. TI Late season mobilization of trace metals in two small Alaskan arctic watersheds as a proxy for landscape scale permafrost active layer dynamics SO CHEMICAL GEOLOGY LA English DT Article DE Trace metals; Arctic; Surface waters; Permafrost; Active layer; Geochemistry ID NORTHERN ALASKA; ORGANIC-CARBON; THERMAL STATE; LENA RIVER; RUSSIA; GEOCHEMISTRY; ENVIRONMENT; SPECIATION; HYDROLOGY; DISCHARGE AB Increasing air temperatures in the Arctic have the potential to degrade permafrost and promote the downward migration of the seasonally thawed active layer into previously frozen material. This may expose frozen soils to mineral weathering that could affect the geochemical composition of surface waters. Determining watershed system responses to drivers such as a changing climate relies heavily on understanding seasonal controls on freshwater processes. The majority of studies on elemental concentrations in Arctic river systems have focused on sampling only from spring snowmelt to the summer season. Consequently, there remains a limited understanding of surface water geochemistry, particularly with respect to trace metals, during late fall and early winter. To examine the variability of metal concentrations as a function of seasonality, we measured trace metal concentrations from spring melt to fall freeze-up in 2010 in two high Arctic watersheds: Imnavait Creek, North Slope, Alaska and Roche Mountanee Creek, Brooks Range, Alaska. We focused on aluminum (Al), barium (Ba), iron (Fe), manganese (Mn), nickel (Ni) and zinc (Zn). Concentrations of 'dissolved' (<0.45 mu m) Al, Ba, Fe, and Mn in Imnavait Creek waters and Ba in Roche Mountanee waters were highest in late fall/early winter. To link observed surface water concentrations at Imnavait Creek to parent soil material we analyzed the elemental composition of a soil core from the watershed and tracked the soil temperatures as a function of time and depth. The results from this study show a distinct seasonal signature of trace metal concentrations in late fall that correlates with the depth of the thawed active layer. Published by Elsevier B. V. C1 [Barker, Amanda J.; Douglas, T. A.] US Army Cold Reg Res & Engn Lab, Ft Wainwright, AK 99703 USA. [Barker, Amanda J.; Trainor, T. P.] Univ Alaska Fairbanks, Dept Chem & Biochem, Fairbanks, AK 99775 USA. [Jacobson, A. D.; Lehn, G. O.] Northwestern Univ, Dept Earth & Planetary Sci, Evanston, IL 60208 USA. [McClelland, J. W.; Khosh, M. S.] Univ Texas Austin, Inst Marine Sci, Port Aransas, TX 78373 USA. [Ilgen, A. G.] Sandia Natl Labs, Dept Geochem, Albuquerque, NM 87185 USA. RP Barker, AJ (reprint author), Dept Chem & Biochem, 900 Yukon Dr Rm 194, Fairbanks, AK 99775 USA. EM ajbarker@alaska.edu RI Jacobson, Andrew/I-6102-2015; McClelland, James/C-5396-2008; OI McClelland, James/0000-0001-9619-8194; Khosh, Matthew/0000-0002-5457-7724; Barker, Amanda/0000-0003-0703-2702 FU U.S. National Science Foundation, Office of Polar Programs to [0806714, 0806643, 0806827]; National Science Foundation [1023052]; SnowNET Project through a collaboration; Matthew Sturm (CRREL-Alaska, now at the University of Alaska Fairbanks) FX Funding for this project was from the U.S. National Science Foundation, Office of Polar Programs to Douglas (# 0806714), Jacobson (# 0806643) and McClelland (# 0806827). Toolik Field Station of the University of Alaska Fairbanks-Institute of Arctic Biology and CH2MHill Polar Field Services provided logistical support. Numerous students and collaborators are acknowledged on this project for field and laboratory assistance. Soil horizon profiles were provided as part of a field workshop on Arctic Soils offered by the University of Alaska Fairbanks taught by Dr. Chien-Lu Ping and Dr. Gary Michaelson of the Palmer Research Center, School of Natural Resources and Agriculture Sciences, University of Alaska Fairbanks. Air temperature data are courtesy of the National Science Foundation funded (award # 1023052) SnowNET Project through a collaboration with Matthew Sturm (CRREL-Alaska, now at the University of Alaska Fairbanks). Toolik area precipitation data were provided by Jessie Cherry of the University of Alaska Fairbanks. Soil characterization and metal analysis (XRD, XRF and ICP-MS instrumentation) were accomplished at the University of Alaska FairbanksAdvanced Instrumentation Laboratory with the assistance of Karen Spaleta, Maciej Sliwinski and Ken Severin. We alsowish to acknowledge the editor and anonymous reviewers for their feedback, which greatly strengthened the article. NR 52 TC 3 Z9 4 U1 3 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD AUG 14 PY 2014 VL 381 BP 180 EP 193 DI 10.1016/j.chemgeo.2014.05.012 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AM9NO UT WOS:000340208500016 ER PT J AU Kimball, JB Dunbar, RB Guilderson, TP AF Kimball, Justine B. Dunbar, Robert B. Guilderson, Thomas P. TI Oxygen and carbon isotope fractionation in calcitic deep-sea corals: Implications for paleotemperature reconstruction SO CHEMICAL GEOLOGY LA English DT Article DE Calcite-water fractionation; Oxygen isotope fractionation; "Lines" method; Deep-sea coral; Paleotemperature proxy; Biomineralization ID GROWTH-RATES; BIOLOGICAL CARBONATES; SYNTHETIC ARAGONITE; NEW-ZEALAND; REEF CORAL; WATER; TEMPERATURE; OCTOCORALLIA; ATLANTIC; CLIMATE AB Inhabiting areas of the ocean where paleoenvironmental records are sparse, deep-sea corals represent valuable yet largely untapped Holocene records of intermediate and deep ocean variability. delta O-18 and delta C-13 were analyzed in nine live-collected deep-sea gorgonian corals (Isididae and Coralliidae) in order to further develop the " lines" paleotemperature method. Least squares linear regression analysis for full lifespan delta O-18 vs. delta C-13 (corrected for delta O-18(water) and delta C-13(DIC)) was utilized to yield equations of the form y = mx + b. delta O-18 and intercept values were found to be a function of temperature, and to approximate calcite delta O-18 equilibrium. The corals in this study extend the previously reported calibration (Hill et al., 2011) over a broader range of temperatures from 5 degrees C to 11.2 degrees C. When combined with the data from Hill et al. (2011), a new expression for the relationship between the delta O-18(intercept) value and temperature is proposed: T (degrees C) = -4: 12 +/- 0: 38 (delta O-18(intercept)) + 12: 33 +/- 0: 75 (R-2 = 0: 90; p value<0: 0001) Error estimates are 0.7 C for corals living at cold temperatures (2 degrees C), 1.4 degrees C in warmer waters (11 degrees C), and +/- 0.5 degrees C at the mean water temperature of the data set (4.6 degrees C). The first multi-specimen verification of the " lines" method was performed on three co-located bamboo (Isididae) corals and found to give nearly coincident delta O-18 intercepts. Detailed intraspecimen sampling reveals delta O-18 and delta C-13 isotopic variabilitywithin coeval portions of the skeleton. In one specimen, "lines" method analysis was utilized on multiple samples taken from the same temporal increment of the skeleton, yieldingmultiple delta O-18 intercepts. Calculated temperatures using the calibration proposed here describe a temperature range of 7.9 to 10.3 degrees C, which approaches the temperature range of 11.1 +/- 0.7 degrees C at the coral collection location. (C) 2014 Elsevier B. V. All rights reserved. C1 [Kimball, Justine B.; Dunbar, Robert B.] Stanford Univ, Dept Environm Earth Syst Sci, Stanford, CA 94025 USA. [Guilderson, Thomas P.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. RP Kimball, JB (reprint author), Stanford Univ, Dept Environm Earth Syst Sci, Stanford, CA 94025 USA. EM jkimball@stanford.edu; dunbar@stanford.edu; tguilderson@llnl.gov FU NOAA's Climate Program Office [NA05OAR4310021, NA05OAR4310017]; NSF Graduate Research Fellowship; U.S. Department of Energy [W-7405-Eng-48, DE-AC52-07NA27344] FX Many thanks to DaveMucciarone for his assistance in gathering and understanding the data. We thank the captains and crews of the RV Atlantis, RV Ka'imikai-o-Kanaloa, and DSRV's Alvin, Pisces V, and Pisces IV for their professional and able assistance in acquiring the specimens for this research. This research was supported by NOAA's Climate Program Office under awards NA05OAR4310021 (RBD) and NA05OAR4310017 (TPG) and an NSF Graduate Research Fellowship to JBK. A portion of this work was performed under the auspices of the U. S. Department of Energy (contract W-7405-Eng-48 and DE-AC52-07NA27344). Thanks to Frank Parrish for his generous help in providing the additional samples, Tessa Hill for the use of a micromill aswell as for the helpful discussions, Bob Jones for the electron microprobe operation and Paul Quay for generously answering questions regarding d13CDIC at HOTS. We would like to thank Aradhna Tripati and Brendan Roark for numerous discussions and advice. Additionally, themanuscript was greatly helped by the comments of two anonymous reviewers. NR 55 TC 5 Z9 5 U1 2 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD AUG 14 PY 2014 VL 381 BP 223 EP 233 DI 10.1016/j.chemgeo.2014.05.008 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AM9NO UT WOS:000340208500019 ER PT J AU Roubeau, O Lorusso, G Teat, SJ Evangelisti, M AF Roubeau, O. Lorusso, G. Teat, S. J. Evangelisti, M. TI Cryogenic magneto-caloric effect and magneto-structural correlations in carboxylate-bridged Gd(III) compounds SO DALTON TRANSACTIONS LA English DT Article ID GADOLINIUM COMPLEX COMPOUND; METAL-ORGANIC FRAMEWORK; CRYSTAL-STRUCTURE; MOLECULAR COOLERS; BEHAVIOR; REFRIGERATION; ACETATE; ACID; DERIVATIVES; POLYMERS AB Two new infinite coordination chain compounds [Gd(CH3CO2)(3)(dmf)](infinity) (1) and {[Gd(HO(CH2)(3)CO2)(3)-(H2O)]center dot H2O}(infinity) (2) have been obtained attempting to modify a prototype molecular cooler. The structures of both compounds as determined by single-crystal X-ray diffraction are reported, together with a detailed study of their magnetic and thermal properties, describing for both compounds a large magneto-caloric effect. The dominant ferromagnetic interaction present in 2 clearly favours this material at low applied magnetic fields, with respect to 1 that exhibits antiferromagnetic interactions. Magneto-structural correlations of the sign and strength of the magnetic interactions are derived for carboxylato-bridged Gd(III) systems. C1 [Roubeau, O.; Lorusso, G.; Evangelisti, M.] CSIC, ICMA, Zaragoza 50009, Spain. [Roubeau, O.; Lorusso, G.; Evangelisti, M.] Univ Zaragoza, Zaragoza 50009, Spain. [Teat, S. J.] Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Roubeau, O (reprint author), CSIC, ICMA, Plaza San Francisco S-N, Zaragoza 50009, Spain. EM roubeau@unizar.es RI Evangelisti, Marco/B-5878-2011; Roubeau, Olivier/A-6839-2010; Lorusso, Giulia/L-9211-2013 OI Evangelisti, Marco/0000-0002-8028-9064; Roubeau, Olivier/0000-0003-2095-5843; Lorusso, Giulia/0000-0002-4078-6808 FU Spanish MINECO; FEDER [MAT2011-24284, MAT2012-38318-C03-01]; EU Marie Curie IEF [PIEF-GA-2011-299356]; Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work has been supported by the Spanish MINECO and FEDER through grants MAT2011-24284 and MAT2012-38318-C03-01 and by an EU Marie Curie IEF (PIEF-GA-2011-299356 to G. L.). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 49 TC 8 Z9 8 U1 1 U2 28 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 EI 1477-9234 J9 DALTON T JI Dalton Trans. PD AUG 14 PY 2014 VL 43 IS 30 BP 11502 EP 11509 DI 10.1039/c4dt00697f PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AM0LY UT WOS:000339538300010 PM 24840855 ER PT J AU Hawkins, CA Bustillos, CG Copping, R Scott, BL May, I Nilsson, M AF Hawkins, C. A. Bustillos, C. G. Copping, R. Scott, B. L. May, I. Nilsson, M. TI Challenging conventional f-element separation chemistry - reversing uranyl(VI)/lanthanide(III) solvent extraction selectivity SO CHEMICAL COMMUNICATIONS LA English DT Article ID SCHIFF-BASE COMPLEXES; URANYL-NITRATE; TRIVALENT ACTINIDES; MOLECULAR-STRUCTURE; CONJUGATE ADDITION; NITRIC-ACID; SALOPHEN; CRYSTAL; LANTHANIDES; WATER AB The water soluble tetradentate Schiff base, N,N'-bis(5-sulfonatosalicylidene)-diaminoethane (H(2)salen-SO3), will readily coordinate to the uranyl(VI) cation, but not to the same extent to trivalent lanthanide cations. This allows for the reversal of conventional solvent extraction properties and opens the possibility for novel separation processes. C1 [Hawkins, C. A.; Bustillos, C. G.; Nilsson, M.] Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92617 USA. [Bustillos, C. G.; Copping, R.; Scott, B. L.; May, I.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Nilsson, M (reprint author), Univ Calif Irvine, Dept Chem Engn & Mat Sci, 916 Engn Tower, Irvine, CA 92617 USA. EM nilssonm@uci.edu RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 FU University of California under the UCOP [12-LF-237294] FX This work was supported by the University of California under the UCOP Grant ID# 12-LF-237294. NR 53 TC 4 Z9 4 U1 1 U2 40 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 EI 1364-548X J9 CHEM COMMUN JI Chem. Commun. PD AUG 14 PY 2014 VL 50 IS 63 BP 8670 EP 8673 DI 10.1039/c4cc03031a PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AL9OF UT WOS:000339469900011 PM 24958394 ER PT J AU Zhang, GH Li, J Deng, Y Miller, JT Kropf, AJ Bunel, EE Lei, AW AF Zhang, Guanghui Li, Jing Deng, Yi Miller, Jeffrey T. Kropf, A. Jeremy Bunel, Emilio E. Lei, Aiwen TI Structure-kinetic relationship study of organozinc reagents SO CHEMICAL COMMUNICATIONS LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; EXAFS; ZN; TRANSMETALATION; STEP AB Phenylzinc reagents prepared from various zinc halides show distinct kinetic features in the palladium-catalyzed Negishi-type oxidative coupling reaction, in which the phenylzinc reagent prepared from ZnI2 gives the highest rate. In situ infrared and X-ray absorption spectroscopy studies show that the higher reaction rate was observed for longer Zn-C bond distances. C1 [Zhang, Guanghui; Li, Jing; Deng, Yi; Kropf, A. Jeremy; Lei, Aiwen] Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Hubei, Peoples R China. [Zhang, Guanghui; Deng, Yi; Miller, Jeffrey T.; Bunel, Emilio E.; Lei, Aiwen] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Lei, Aiwen] Chinese Acad Sci, Shanghai Inst Organ Chem, State Key Lab Organometall Chem, Shanghai 200032, Peoples R China. RP Lei, AW (reprint author), Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Hubei, Peoples R China. EM aiwenlei@whu.edu.cn RI Zhang, Guanghui/C-4747-2008; BM, MRCAT/G-7576-2011; ID, MRCAT/G-7586-2011; OI Zhang, Guanghui/0000-0002-5854-6909; Lei, Aiwen/0000-0001-8417-3061 FU 973 Program [2012CB725302]; National Natural Science Foundation of China [21390400, 21025206, 21272180, 21302148]; Research Fund for the Doctoral Program of Higher Education of China [20120141130002]; Program for Changjiang Scholars and Innovative Research Team in University [IRT1030]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Department of Energy; MRCAT FX This work was supported by the 973 Program (2012CB725302), the National Natural Science Foundation of China (21390400, 21025206, 21272180 and 21302148), the Research Fund for the Doctoral Program of Higher Education of China (20120141130002) and the Program for Changjiang Scholars and Innovative Research Team in University (IRT1030). Use of the Advanced Photon Source was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. MRCAT operations were supported by the Department of Energy and the MRCAT member institutions. NR 27 TC 7 Z9 7 U1 4 U2 51 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 EI 1364-548X J9 CHEM COMMUN JI Chem. Commun. PD AUG 14 PY 2014 VL 50 IS 63 BP 8709 EP 8711 DI 10.1039/c4cc01135j PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA AL9OF UT WOS:000339469900021 PM 24964262 ER PT J AU Dobrescu, BA Peterson, AD AF Dobrescu, Bogdan A. Peterson, Andrea D. TI W' signatures with odd Higgs particles SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Higgs Physics; Gauge Symmetry ID DARK-MATTER; GAUGE-MODEL; PHENOMENOLOGY; BOSONS AB We point out that W' bosons may decay predominantly into Higgs particles associated with their broken gauge symmetry. We demonstrate this in a renormalizable model where the W' and W couplings to fermions differ only by an overall normalization. This "meta-sequential" W' boson decays into a scalar pair, with the charged one subsequently decaying into a W boson and a neutral scalar. These scalars are odd under a parity of the Higgs sector, which consists of a complex bidoublet and a doublet. The W' and Z' bosons have the same mass and branching fractions into scalars, and may show up at the LHC in final states involving one or two electroweak bosons and missing transverse energy. C1 [Dobrescu, Bogdan A.; Peterson, Andrea D.] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Peterson, Andrea D.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. RP Dobrescu, BA (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. EM bdob@fnal.gov; adpeterson2@wisc.edu FU Fermilab Fellowship in Theoretical Physics; Fermi Research Alliance, LLC [DE-AC02-07CH11359] FX We would like to thank Calin Alexa, Yang Bai, Vernon Barger, Patrick Fox, Adam Jinaru, Sudhir Malik, Caroline Milstene and Liantao Wang for stimulating conversations. A.P. is supported by the Fermilab Fellowship in Theoretical Physics. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the US Department of Energy. NR 35 TC 3 Z9 3 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 13 PY 2014 IS 8 AR 078 DI 10.1007/JHEP08(2014)078 PG 20 WC Physics, Particles & Fields SC Physics GA AY9TI UT WOS:000347892900001 ER PT J AU Sarntivijai, S Lin, Y Xiang, ZS Meehan, TF Diehl, AD Vempati, UD Schurer, SC Pang, C Malone, J Parkinson, H Liu, Y Takatsuki, T Saijo, K Masuya, H Nakamura, Y Brush, MH Haendel, MA Zheng, J Stoeckert, CJ Peters, B Mungall, CJ Carey, TE States, DJ Athey, BD He, YQ AF Sarntivijai, Sirarat Lin, Yu Xiang, Zuoshuang Meehan, Terrence F. Diehl, Alexander D. Vempati, Uma D. Schuerer, Stephan C. Pang, Chao Malone, James Parkinson, Helen Liu, Yue Takatsuki, Terue Saijo, Kaoru Masuya, Hiroshi Nakamura, Yukio Brush, Matthew H. Haendel, Melissa A. Zheng, Jie Stoeckert, Christian J. Peters, Bjoern Mungall, Christopher J. Carey, Thomas E. States, David J. Athey, Brian D. He, Yongqun TI CLO: The cell line ontology SO JOURNAL OF BIOMEDICAL SEMANTICS LA English DT Article DE Cell line; Cell line cell; Immortal cell line cell; Mortal cell line cell; Cell line cell culturing; Anatomy AB Background: Cell lines have been widely used in biomedical research. The community-based Cell Line Ontology (CLO) is a member of the OBO Foundry library that covers the domain of cell lines. Since its publication two years ago, significant updates have been made, including new groups joining the CLO consortium, new cell line cells, upper level alignment with the Cell Ontology (CL) and the Ontology for Biomedical Investigation, and logical extensions. Construction and content: Collaboration among the CLO, CL, and OBI has established consensus definitions of cell line-specific terms such as 'cell line', 'cell line cell', 'cell line culturing', and 'mortal' vs. 'immortal cell line cell'. A cell line is a genetically stable cultured cell population that contains individual cell line cells. The hierarchical structure of the CLO is built based on the hierarchy of the in vivo cell types defined in CL and tissue types (from which cell line cells are derived) defined in the UBERON cross-species anatomy ontology. The new hierarchical structure makes it easier to browse, query, and perform automated classification. We have recently added classes representing more than 2,000 cell line cells from the RIKEN BRC Cell Bank to CLO. Overall, the CLO now contains similar to 38,000 classes of specific cell line cells derived from over 200 in vivo cell types from various organisms. Utility and discussion: The CLO has been applied to different biomedical research studies. Example case studies include annotation and analysis of EBI ArrayExpress data, bioassays, and host-vaccine/pathogen interaction. CLO's utility goes beyond a catalogue of cell line types. The alignment of the CLO with related ontologies combined with the use of ontological reasoners will support sophisticated inferencing to advance translational informatics development. C1 [Sarntivijai, Sirarat] US FDA, Silver Spring, MD 20993 USA. [Sarntivijai, Sirarat; Lin, Yu; Xiang, Zuoshuang; Liu, Yue; Carey, Thomas E.; Athey, Brian D.; He, Yongqun] Univ Michigan, Ann Arbor, MI 48109 USA. [Meehan, Terrence F.; Malone, James; Parkinson, Helen] EMBL EBI, European Mol Biol Lab, Hinxton, Oxon, England. [Diehl, Alexander D.] SUNY Buffalo, Buffalo, NY 14260 USA. [Vempati, Uma D.; Schuerer, Stephan C.] Univ Miami, Miami, FL USA. [Pang, Chao] Univ Groningen, Univ Med Ctr Groningen, NL-9713 AV Groningen, Netherlands. [Takatsuki, Terue; Saijo, Kaoru; Masuya, Hiroshi; Nakamura, Yukio] RIKEN, BioResource Ctr, Tsukuba, Ibaraki, Japan. [Brush, Matthew H.; Haendel, Melissa A.] Oregon Hlth & Sci Univ, Portland, OR USA. [Zheng, Jie; Stoeckert, Christian J.] Univ Penn, Philadelphia, PA 19104 USA. [Peters, Bjoern] La Jolla Inst Allergy & Immunol, La Jolla, CA USA. [Mungall, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [States, David J.] OncProTech LLC, Ann Arbor, MI USA. RP Sarntivijai, S (reprint author), US FDA, Silver Spring, MD 20993 USA. EM siiraa@umich.edu; yongqunh@med.umich.edu RI Zheng, Jie/M-1191-2015; Nakamura, Yukio/A-5263-2016; Masuya, Hiroshi/A-6442-2016; Diehl, Alexander/G-9883-2016; OI Zheng, Jie/0000-0002-2999-0103; Masuya, Hiroshi/0000-0002-3392-466X; Diehl, Alexander/0000-0001-9990-8331; Athey, Brian/0000-0002-9793-535X; Parkinson, Helen/0000-0003-3035-4195; He, Yongqun/0000-0001-9189-9661; Sarntivijai, Sirarat/0000-0002-2548-641X; Meehan, Terrence/0000-0003-1980-3228; Carey, Thomas/0000-0002-5202-7518 FU National Institutes of Health (NIH) [1R01AI081062]; National Institute of Allergy and Infectious Diseases (NIAID) [U54 DA021519]; NIH Office of the Director [1R24OD011883]; NIH [1R01GM093132-01, HHSN272201200010C, U01HL111561]; National Human Genome Research Institute (NHGRI) [RC2HG005668]; European Molecular Biology Laboratory (EMBL-EBI) core funds; EC [200754]; National Bioscience Database Center (NBDC) of the Japan Science and Technology Agency (JST) FX The work described is funded in part by the National Institutes of Health (NIH) grants 1R01AI081062 (YH) from the National Institute of Allergy and Infectious Diseases (NIAID), U54 DA021519 for the National Center for Integrative Biomedical Informatics (BDA), 1R24OD011883 from the NIH Office of the Director (MAH and MHB), NIH grant 1R01GM093132-01 (JZ and CJS), NIH contract HHSN272201200010C (BP), U01HL111561 (SCS) as part of the Library of Integrated Network-based Cellular Signatures (LINCS) program, and RC2HG005668 (SCS) supported by the National Human Genome Research Institute (NHGRI), European Molecular Biology Laboratory (EMBL-EBI) core funds (HP, JM), EC FP7 Funds Grant number: 200754 Gen2Phen (CP), and funding from the National Bioscience Database Center (NBDC) of the Japan Science and Technology Agency (JST) for BRC [21]. The content of this paper is solely the responsibility of the author and does not necessarily represent the official views of the NIAID, NHGRI, the NIH or other funding organizations. The article-processing charge for this article was paid by a discretionary fund from Dr. Robert Dysko, the director of the Unit for Laboratory Animal Medicine (ULAM) in the University of Michigan. NR 22 TC 8 Z9 8 U1 0 U2 1 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 2041-1480 J9 J BIOMED SEMANT JI J. Biomed. Semant. 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CA CMS Collaboration TI Measurement of the muon charge asymmetry in inclusive pp -> W plus X production at root s=7 TeV and an improved determination of light parton distribution functions SO PHYSICAL REVIEW D LA English DT Article ID 3-LOOP SPLITTING FUNCTIONS; HADRON COLLIDERS; LEADING-ORDER; BOSON PRODUCTION; LHC; QCD; SCATTERING; EVOLUTION; DENSITIES; TEVATRON AB Measurements of the muon charge asymmetry in inclusive pp -> W + X production at root s = 7 TeV are presented. The data sample corresponds to an integrated luminosity of 4.7 fb(-1) recorded with the CMS detector at the LHC. With a sample of more than 20 million W -> mu nu events, the statistical precision is greatly improved in comparison to previous measurements. These new results provide additional constraints on the parton distribution functions of the proton in the range of the Bjorken scaling variable x from 10(-3) to 10(-1). These measurements and the recent CMS measurement of associated W + charm production are used together with the cross sections for inclusive deep inelastic e(+/-) p scattering at HERA in a next-to-leading-order QCD analysis. The determination of the valence quark distributions is improved, and the strange-quark distribution is probed directly through the leading-order process g + s -> W + c in proton-proton collisions at the LHC. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.; Radi, A.] Inst Hochenergiephys OeAW, Vienna, Austria. 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S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Mueller, T.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Psallidas, A.; Topsis-giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Jones, J.; Kokkas, P.; Manthos, N.; Papadopoulos, I.] Univ Ioannina, GR-45110 Ioannina, Greece. [Paradas, E.; Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Radi, A.; Karancsi, J.; Raics, P.; Ujvari, B.; Fasanella, D.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay, Maharashtra, India. [Radi, A.; Abdulsalam, A.; Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.; Manzoni, R. A.; Martelli, A.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.; Riccardi, C.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Radi, A.; Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Radi, A.; Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Torassa, E.; Tosi, M.; Triossi, A.; Vanini, S.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.; Biasini, M.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Boccali, T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Radi, A.; Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Radi, A.; Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Sacchi, R.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.; Solano, A.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya Jabatan Fizik, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de la Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.; Ryutin, R.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Radi, A.; Bialkowska, H.; Bluj, M.; Boimska, B.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Wrochna, G.] Natl Ctr Nucl Res, Otwock, Poland. [Zalewski, P.; Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Bunin, P.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Y.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernyndez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Pelayo, J. Puerta; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Radi, A.; Contardo, D.; Lingemann, J.; Mohanty, A. K.; Giordano, F.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; Pelliccioni, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Loureno, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rojo, J.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.; Starodumov, A.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duesner, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tauscher, L.; Theofilatos, K.; Treille, D.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Radi, A.; Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Favaro, C.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Ctr Nat Sci, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Anastassov, A.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.; Askew, A.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.; Baarmand, M. M.] Florida State Univ, Tallahassee, FL 32306 USA. [Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Chinellato, J.; Tonelli Manganote, E. J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.; De Benedetti, A.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Adiguzel, A.; Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.; Bhatti, A.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sakharov, A.; Sarangi, T.; Savin, A.; Smith, W. H.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Abdelalim, A. A.; Elgammal, S.] Zewail City Sci & Technol, Zewail, Egypt. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. British Univ Egypt, Cairo, Egypt. Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bell, A. J.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.] Eotvos Lorand Univ, Budapest, Hungary. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Castaldi, R.; Grippo, M. T.; Squillacioti, P.; Seixas, J.; Chamizo Llatas, M.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Heredia-de la Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Istanbul Univ, Fac Sci, Istanbul, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Popov, A.; Zhukov, V.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Flix, Josep/G-5414-2012; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Montanari, Alessandro/J-2420-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Gonzalez Caballero, Isidro/E-7350-2010; Codispoti, Giuseppe/F-6574-2014; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Yazgan, Efe/A-4915-2015; Scodellaro, Luca/K-9091-2014; Cerrada, Marcos/J-6934-2014; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014 OI Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Flix, Josep/0000-0003-2688-8047; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Russ, James/0000-0001-9856-9155; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Codispoti, Giuseppe/0000-0003-0217-7021; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087 FU Austrian Federal Ministry of Science and Research; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy and the Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria a de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, UK; U.S. Department of Energy; U.S. National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria a de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, UK; the U.S. Department of Energy, and the U.S. National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 71 TC 22 Z9 22 U1 6 U2 62 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 13 PY 2014 VL 90 IS 3 AR 032004 DI 10.1103/PhysRevD.90.032004 PG 33 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AO1WG UT WOS:000341105600001 ER PT J AU Hudson, CM Lau, BY Williams, KP AF Hudson, Corey M. Lau, Britney Y. Williams, Kelly P. TI Ends of the line for tmRNA-SmpB SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE tmRNA; SmpB; trans-translation; Carsonella; Mycoplasma ID TRANSFER-MESSENGER-RNA; PEPTIDYL-TRANSFER-RNA; RIBOSOME-RESCUE; ESCHERICHIA-COLI; NUCLEOTIDE-SEQUENCES; STALLED RIBOSOMES; TRANS-TRANSLATION; PROTEIN; SYSTEM; DATABASE AB Genes for the RNA tmRNA and protein SmpB, partners in the trans-translation process that rescues stalled ribosomes, have previously been found in all bacteria and some organelles. During a major update of The tmRNA Website (relocated to http://bioinformatics.sandia.gov/tmrna), including addition of an SmpB sequence database, we found some bacteria that lack functionally significant regions of SmpB. Three groups with reduced genomes have lost the central loop of SmpB, which is thought to improve alanylation and EF-Tu activation: Carsonella, Hodgkinia, and the hemoplasmas (hemotropic Mycoplasma). Carsonella has also lost the SmpB C-terminal tail, thought to stimulate the decoding center of the ribosome. We validate recent identification of tmRNA homologs in oomycete mitochondria by finding partner genes from oomycete nuclei that target SmpB to the mitochondrion. We have moreover identified through exhaustive search a small number of complete, but often highly derived, bacterial genomes that appear to lack a functional copy of either the tmRNA or SmpB gene (but not both). One Carsonella isolate exhibits complete degradation of the tmRNA gene sequence yet its smpB shows no evidence for relaxed selective constraint, relative to other genes in the genome. After loss of the SmpB central loop in the hemoplasmas, one subclade apparently lost tmRNA. Carsonella also exhibits gene overlap such that tmRNA maturation should produce a non-stop smpB mRNA. At least some of the tmRNA/SmpB-deficient strains appear to further lack the ArfA and ArfB backup systems for ribosome rescue. The most frequent neighbors of smpB are the tmRNA gene, a ratA/mfH unit, and the gene for RNaseR, a known physical and functional partner of tmRNA-SmpB. C1 [Hudson, Corey M.; Lau, Britney Y.; Williams, Kelly P.] Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94550 USA. RP Williams, KP (reprint author), Sandia Natl Labs, Dept Syst Biol, 7011 East Ave, Livermore, CA 94550 USA. EM kpwilli@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We thank Daniel Sloan (Yale U.) for detailed data on Carsonella dN/dS values. This research was fully supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 41 TC 9 Z9 9 U1 1 U2 4 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 13 PY 2014 VL 5 AR 421 DI 10.3389/fmicb.2014.00421 PG 9 WC Microbiology SC Microbiology GA AO7GM UT WOS:000341520500001 PM 25165464 ER PT J AU Keating, DH Zhang, YP Ong, IM McIlwain, S Morales, EH Grass, JA Tremaine, M Bothfeld, W Higbee, A Ulbrich, A Balloon, AJ Westphall, MS Aldrich, J Lipton, MS Kim, J Moskvin, OV Bukhman, YV Coon, JJ Kiley, PJ Bates, DM Landick, R AF Keating, David H. Zhang, Yaoping Ong, Irene M. McIlwain, Sean Morales, Eduardo H. Grass, Jeffrey A. Tremaine, Mary Bothfeld, William Higbee, Alan Ulbrich, Arne Balloon, Allison J. Westphall, Michael S. Aldrich, Josh Lipton, Mary S. Kim, Joonhoon Moskvin, Oleg V. Bukhman, Yury V. Coon, Joshua J. Kiley, Patricia J. Bates, Donna M. Landick, Robert TI Aromatic inhibitors derived from ammonia-pretreated lignocellulose hinder bacterial ethanologenesis by activating regulatory circuits controlling inhibitor efflux and detoxification SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE Escherichia coli; lignocellulosic hydrolysate; aromatic inhibitors; transcriptomics; RNAseq; proteomics; ethanol; biofuels ID ESCHERICHIA-COLI KO11; GENE-EXPRESSION; FURFURAL TOLERANCE; XYLOSE METABOLISM; MASS-SPECTROMETRY; STATIONARY-PHASE; LON PROTEASE; ROB; FERMENTATION; ETHANOL AB Efficient microbial conversion of lignocellulosic hydrolysates to biofuels is a key barrier to the economically viable deployment of lignocellulosic biofuels. A chief contributor to this barrier is the impact on microbial processes and energy metabolism of lignocellulose-derived inhibitors, including phenolic carboxylates, phenolic amides (for ammonia-pretreated biomass), phenolic aldehydes, and furfurals. To understand the bacterial pathways induced by inhibitors present in ammonia-pretreated biomass hydrolysates, which are less well studied than acid-pretreated biomass hydrolysates, we developed and exploited synthetic mimics of ammonia-pretreated corn stover hydrolysate (ACSH). To determine regulatory responses to the inhibitors normally present in ACSH, we measured transcript and protein levels in an Escherichia coli ethanologen using RNA-seq and quantitative proteomics during fermentation to ethanol of synthetic hydrolysates containing or lacking the inhibitors. Our study identified four major regulators mediating these responses, the MarA/SoxS/Rob network, AaeR, FrmR, and YqhC. Induction of these regulons was correlated with a reduced rate of ethanol production, buildup of pyruvate, depletion of ATP and NAD(P)H, and an inhibition of xylose conversion. The aromatic aldehyde inhibitor 5-hydroxymethylfurfural appeared to be reduced to its alcohol form by the ethanologen during fermentation, whereas phenolic acid and amide inhibitors were not metabolized. Together, our findings establish that the major regulatory responses to lignocellulose-derived inhibitors are mediated by transcriptional rather than translational regulators, suggest that energy consumed for inhibitor efflux and detoxification may limit biofuel production, and identify a network of regulators for future synthetic biology efforts. C1 [Keating, David H.; Zhang, Yaoping; Ong, Irene M.; McIlwain, Sean; Morales, Eduardo H.; Grass, Jeffrey A.; Tremaine, Mary; Bothfeld, William; Higbee, Alan; Kim, Joonhoon; Moskvin, Oleg V.; Bukhman, Yury V.; Coon, Joshua J.; Kiley, Patricia J.; Bates, Donna M.; Landick, Robert] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. [Morales, Eduardo H.; Westphall, Michael S.; Coon, Joshua J.; Kiley, Patricia J.] Univ Wisconsin, Dept Biomol Chem, Madison, WI 53726 USA. [Grass, Jeffrey A.; Landick, Robert] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA. [Ulbrich, Arne; Balloon, Allison J.; Westphall, Michael S.; Coon, Joshua J.] Univ Wisconsin, Dept Chem, Madison, WI 53726 USA. [Aldrich, Josh; Lipton, Mary S.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kim, Joonhoon] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53726 USA. [Landick, Robert] Univ Wisconsin, Dept Bacteriol, Madison, WI 53726 USA. RP Bates, DM (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Wisconsin Energy Inst 4119, 1552 Univ Ave, Madison, WI 53726 USA. EM dbates@glbrc.wisc.edu; landick@biochem.wisc.edu RI Moskvin, Oleg/C-5916-2015; Kim, Joonhoon/E-6253-2012; Lipton, Mary/H-3913-2012; OI Moskvin, Oleg/0000-0003-1499-8900; Kim, Joonhoon/0000-0002-7425-1828; Bukhman, Yury/0000-0002-8111-7651 FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494]; DOE [DE-AC05-76RLO01830] FX The authors thank Trey Sato and Jeff Piotrowski for critical reading of the manuscript, Fachuang Lu and John Ralph for advice on synthesis of feruloyl and coumaroyl amide, and Christa Pennacchio and colleagues at the Joint Genome Institute for cDNA library preparation and sequencing. This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494). Portions of this research were enabled by the DOE GSP under the Pan-omics project. Work was performed in the Environmental Molecular Science Laboratory, a U.S. Department of Energy (DOE) national scientific user facility at Pacific Northwest National Laboratory (PNNL) in Richland, WA. Battelle operates PNNL for the DOE under contract DE-AC05-76RLO01830. NR 67 TC 9 Z9 9 U1 2 U2 32 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 13 PY 2014 VL 5 AR UNSP 402 DI 10.3389/fmicb.2014.00402 PG 17 WC Microbiology SC Microbiology GA AO7GL UT WOS:000341520400001 PM 25177315 ER PT J AU Avila, JR DeMarco, EJ Emery, JD Farha, OK Pellin, MJ Hupp, JT Martinson, ABF AF Avila, Jason R. DeMarco, Erica J. Emery, Jonathan D. Farha, Omar K. Pellin, Michael J. Hupp, Joseph T. Martinson, Alex B. F. TI Real-Time Observation of Atomic Layer Deposition Inhibition: Metal Oxide Growth on Self-Assembled Alkanethiols SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE atomic layer deposition; self-assembled monolayers; quartz crystal microbalance; alkanethiol; in situ; analytical methods ID TITANIUM-OXIDE; ALUMINUM-OXIDE; MONOLAYERS; TEMPERATURE; FILMS; SURFACES; TIO2; NANOPARTICLES; NUCLEATION; DIOXIDE AB Through in situ quartz crystal microbalance (QCM) monitoring, we resolve the growth of a self-assembled monolayer (SAM) and subsequent metal oxide deposition with high resolution. We introduce the fitting of mass deposited during each atomic layer deposition (ALD) cycle to an analytical island-growth model that enables quantification of growth inhibition, nucleation density, and the uninhibited ALD growth rate. A long-chain alkanethiol was self-assembled as a monolayer on gold-coated quartz crystals in order to investigate its effectiveness as a barrier to ALD. Compared to solution-loading, vapor-loading is observed to produce a SAM with equal or greater inhibition ability in minutes vs days. The metal oxide growth temperature and the choice of precursor also significantly affect the nucleation density, which ranges from 0.001 to 1 sites/nm(2). Finally, we observe a minimum 100 cycle inhibition of an oxide ALD process, ZnO, under moderately optimized conditions. C1 [Avila, Jason R.; DeMarco, Erica J.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Emery, Jonathan D.; Pellin, Michael J.; Martinson, Alex B. F.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Farha, Omar K.] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah, Saudi Arabia. RP Martinson, ABF (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. EM martinson@anl.gov RI Pellin, Michael/B-5897-2008; Faculty of, Sciences, KAU/E-7305-2017; OI Pellin, Michael/0000-0002-8149-9768; Martinson, Alex/0000-0003-3916-1672 FU ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; U.S. Department of Energy, Office of Science, Laboratory by UChicago Argonne, LLC. [DE-AC02-06CH11357]; NSFNSEC; NSF-MRSEC; KECK Foundation; state of Illinois; Northwestern University FX This work was supported as part of the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001059. A portion of the research was performed at Argonne National Laboratory, a U.S. Department of Energy, Office of Science, Laboratory operated under Contract DE-AC02-06CH11357 by UChicago Argonne, LLC. Addition electron microscopy was performed in the EPIC and KECKII facilities of the NUANCE Center at Northwestern University. The NUANCE center is supported by NSFNSEC, NSF-MRSEC, the KECK Foundation, the state of Illinois, and Northwestern University. NR 37 TC 10 Z9 10 U1 6 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 13 PY 2014 VL 6 IS 15 BP 11891 EP 11898 DI 10.1021/am503008j PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AN2WI UT WOS:000340446300014 PM 25046585 ER PT J AU McCarthy, RF Weimer, MS Emery, JD Hock, AS Martinson, ABF AF McCarthy, Robert F. Weimer, Matthew S. Emery, Jonathan D. Hock, Adam S. Martinson, Alex B. F. TI Oxygen-Free Atomic Layer Deposition of Indium Sulfide SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE Atomic layer deposition; indium sulfide; in situ measurements; surface reactions; indium(III) amidinate; photovoltaics ID CU(IN,GA)SE-2 SOLAR-CELLS; IN2O3 THIN-FILMS; HYDROGEN-SULFIDE; BUFFER LAYERS; AMIDINATE COMPLEXES; VAPOR-DEPOSITION; TANTALUM OXIDE; IN2S3; GROWTH; EPITAXY AB Atomic layer deposition (ALD) of indium sulfide (In2S3) films was achieved using a newly synthesized indium precursor and hydrogen sulfide. We obtain dense and adherent thin films free from halide and oxygen impurities. Self-limiting half-reactions are demonstrated at temperatures up to 225 degrees C, where oriented crystalline thin films are obtained without further annealing. Low-temperature growth of 0.89 angstrom/cycle is observed at 150 degrees C, while higher growth temperatures gradually reduce the per-cycle growth rate. Rutherford backscattering spectroscopy (RBS) together with depth-profiling Auger electron spectroscopy (AES) reveal a S/In ratio of 1.5 with no detectable carbon, nitrogen, halogen, or oxygen impurities. The resistivity of thin films prior to air exposure decreases with increasing deposition temperature, reaching <1 Omega.cm for films deposited at 225 degrees C. Hall measurements reveal n-type conductivity due to free electron concentrations up to 10(18) cm(-3) and mobilities of order 1 cm(2)/(V.s). The digital synthesis of In2S3 via ALD at temperatures up to 225 degrees C may allow high quality thin films to be leveraged in optoelectronic devices including photovoltaic absorbers, buffer layers, and intermediate band materials. C1 [McCarthy, Robert F.; Weimer, Matthew S.; Emery, Jonathan D.; Martinson, Alex B. F.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Hock, Adam S.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Weimer, Matthew S.; Hock, Adam S.] IIT, Dept Biol & Chem Sci, Chicago, IL 60616 USA. RP Martinson, ABF (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 South Cass Ave, Argonne, IL 60439 USA. EM martinson@anl.gov RI Hock, Adam/D-7660-2012; OI Hock, Adam/0000-0003-1440-1473; Martinson, Alex/0000-0003-3916-1672 FU U.S. Department of Energy [DE-AC02-06CH11357]; UChicago Argonne, LLC [DE-AC02-06CH11357]; Department of Education GAANN Fellowship [P200A090137]; Department of Energy; Illinois Institute of Technology FX Argonne National Laboratory's work was supported under U.S. Department of Energy contract DE-AC02-06CH11357. The electron microscopy was accomplished at the Electron Microscopy Center at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. M.S.W. would like to thank the Department of Education GAANN Fellowship under grant #P200A090137. We also wish to thank Dr. Shannon C. Riha for useful discussions and Paul A. Fenter for access to the atomic force microscope. A.S.H. would like to thank the Department of Energy and the Illinois Institute of Technology for funding and startup support. NR 53 TC 5 Z9 5 U1 5 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 13 PY 2014 VL 6 IS 15 BP 12137 EP 12145 DI 10.1021/am501331w PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AN2WI UT WOS:000340446300041 PM 25061915 ER PT J AU Elshobaki, M Anderegg, J Chaudhary, S AF Elshobaki, Moneim Anderegg, James Chaudhary, Sumit TI Efficient Polymer Solar Cells Fabricated on Poly(3,4-ethylenedioxythiophene):Poly(styrenesulfonate)-Etched Old Indium Tin Oxide Substrates SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE indium tin oxide; PEDOT:PSS; etching; polymer solar cells; transparent electrode ID LIGHT-EMITTING-DIODES; WORK FUNCTION; LAYER; CONDUCTIVITY; FILMS AB In organic electronic devices, indium tin oxide (ITO) and poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) are the most common transparent electrode and anodic buffer layer materials, respectively. A widespread concern is that PEDOT:PSS is acidic and etches ITO. We show that this issue is not serious: only a few nanometers of ITO are etched in typical device processing conditions and storage thereafter; conductivity losses are affordable; and optical transmission gains further offset these losses. Organic photovoltaic (OPV) devices fabricated on old ITO (with PEDOT:PSS history) were similar or higher in efficiency than devices on fresh ITO. Poly[[4,8-bis[(2-ethylhexyl)oxy]benzo[1,2b:4,5-b']dithiophene-2,6-diyl][3-fluoro-2-[(2-ethylhexyl)carbonyl]thieno[3,4-b]thiophenediyl]] (PTB7) devices on old ITO showed efficiencies up to 9.24% compared to 8.72% efficient devices on fresh ITO. This reusability of ITO can be impactful for economics of organic electronics because ITO accounts for almost 90% of energy embedded in devices, such as OPVs. C1 [Elshobaki, Moneim; Chaudhary, Sumit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Anderegg, James] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Chaudhary, Sumit] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Elshobaki, Moneim] Mansoura Univ, Dept Phys, Mansoura 35516, Egypt. RP Chaudhary, S (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM sumitc@iastate.edu OI Elshobaki, Moneim/0000-0003-2125-0394 FU U.S. National Science Foundation [CBET 1236839]; Egyptian government [GM915] FX This work was supported by the U.S. National Science Foundation (Award CBET 1236839). Moneim Elshobaki thanks the fellowship support from the Egyptian government under Contract GM915. The authors gratefully acknowledge John Carr, Max Noack, and Joydeep Bhattacharya for the fruitful discussions and help with providing old ITO substrates. NR 20 TC 4 Z9 4 U1 3 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 13 PY 2014 VL 6 IS 15 BP 12196 EP 12202 DI 10.1021/am5037884 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AN2WI UT WOS:000340446300047 PM 25046352 ER PT J AU Williams, VO DeMarco, EJ Katz, MJ Libera, JA Riha, SC Kim, DW Avila, JR Martinson, ABF Elam, JW Pellin, MJ Farha, OK Hupp, JT AF Williams, Vennesa O. DeMarco, Erica J. Katz, Michael J. Libera, Joseph A. Riha, Shannon C. Kim, Dong Wook Avila, Jason R. Martinson, Alex B. F. Elam, Jeffrey W. Pellin, Michael J. Farha, Omar K. Hupp, Joseph T. TI Fabrication of Transparent-Conducting-Oxide-Coated Inverse Opals as Mesostructured Architectures for Electrocatalysis Applications: A Case Study with NiO SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE nickel oxide; water oxidation; atomic-layer deposition; inverse opals; catalysis; electrochemistry ID ATOMIC LAYER DEPOSITION; SENSITIZED SOLAR-CELLS; OXYGEN EVOLUTION; THIN-FILMS; NANOPOROUS MATERIALS; ALKALINE-SOLUTION; TIO2 PHOTOANODES; SIO2; ELECTRODES; TIN AB Highly ordered, and conductive inverse opal arrays were made with silica and subsequently coated with tin-doped indium oxide (ITO) via atomic layer deposition (ALD). We demonstrate the utility of the resulting mesostructured electrodes by further coating them with nickel oxide via ALD. The NiO-coated arrays are capable of efficiently electrochemically evolving oxygen from water. These modular, crack-free, transparent, high surface area, and conducting structures show promise for many applications including electrocatalysis, photocatalysis, and dye-sensitized solar cells. C1 [Williams, Vennesa O.; DeMarco, Erica J.; Katz, Michael J.; Kim, Dong Wook; Avila, Jason R.; Pellin, Michael J.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Williams, Vennesa O.; DeMarco, Erica J.; Katz, Michael J.; Kim, Dong Wook; Avila, Jason R.; Pellin, Michael J.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Argonne Northwestern Solar Energy Res Ctr ANSER, Evanston, IL 60208 USA. [Williams, Vennesa O.; DeMarco, Erica J.; Riha, Shannon C.; Martinson, Alex B. F.; Pellin, Michael J.; Hupp, Joseph T.] Argonne Natl Lab, Mat Sci Div, Argonne, IL 60439 USA. [Libera, Joseph A.; Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Hupp, Joseph T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Farha, Omar K.] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah, Saudi Arabia. RP Farha, OK (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM o-farha@northwestern.edu; j-hupp@northwestern.edu RI Pellin, Michael/B-5897-2008; Faculty of, Sciences, KAU/E-7305-2017; OI Pellin, Michael/0000-0002-8149-9768; Katz, Michael/0000-0002-7744-3956; Martinson, Alex/0000-0003-3916-1672 FU ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059] FX This work was supported as part of the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001059. NR 44 TC 16 Z9 16 U1 3 U2 104 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 13 PY 2014 VL 6 IS 15 BP 12290 EP 12294 DI 10.1021/am501910n PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AN2WI UT WOS:000340446300057 PM 25033088 ER PT J AU Zhang, PF Gong, YT Wei, ZZ Wang, J Zhang, ZY Li, HR Dai, S Wang, Y AF Zhang, Pengfei Gong, Yutong Wei, Zhongzhe Wang, Jing Zhang, Zhiyong Li, Haoran Dai, Sheng Wang, Yong TI Updating Biomass into Functional Carbon Material in Ionothermal Manner SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE porous carbon; nitrogen-doped carbon; biomass; ionothermal synthesis; soft template; ionic liquid ID IONIC LIQUIDS; MESOPOROUS CARBON; HYDROTHERMAL CARBONIZATION; PLATINUM NANOPARTICLES; DOPED CARBON; OXIDATION; CELLULOSE; NITRIDE; WATER; TEMPERATURE AB The development of meaningful ways to transfer biomass into useful materials, more efficient energy carriers, and/or carbon storage deposits is a profound challenge of our days. Herein, an ionothermal carbonization (ITC) method, via treating natural resources (glucose, cellulose, and sugar cane bagesse) in nonmetal ionic liquids (ILs) at similar to 200 degrees C, is established for the fabrication of porous heteroatom-doped carbon materials with high yield. Commercial ELs with bulky bis(trifluoromethylsulfonyl)imide anion or cross-linkable nitrile group were found to be efficient and recyclable templates for porosity control, leading to exciting nanoarchitectures with promising performance in oxygen reduction reaction. The optimized Its (12 mL) can dissolve and directly convert up to 15 g of glucose into porous carbon materials (S-BET: 272 m(2)/g) one time. This ITC method relies on the synergistic use of structure-directing effect, good biomass solubility, and excellent thermal stability of ILs, and provides a sustainable strategy for exploiting biomass. C1 [Zhang, Pengfei; Gong, Yutong; Wei, Zhongzhe; Wang, Jing; Li, Haoran; Wang, Yong] Zhejiang Univ, Dept Chem, Carbon Nano Mat Grp, Ctr Chem High Performance & Novel Mat, Hangzhou 310028, Zhejiang, Peoples R China. [Zhang, Pengfei; Zhang, Zhiyong; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Wang, Y (reprint author), Zhejiang Univ, Dept Chem, Carbon Nano Mat Grp, Ctr Chem High Performance & Novel Mat, Hangzhou 310028, Zhejiang, Peoples R China. EM chemwy@zju.edu.cn RI Wang, Yong/B-8892-2013; Dai, Sheng/K-8411-2015; Zhang, Pengfei/I-5484-2013; Zhang, Zhiyong/H-5611-2012 OI Wang, Yong/0000-0001-8043-5757; Dai, Sheng/0000-0002-8046-3931; Zhang, Zhiyong/0000-0001-7936-9510 FU National Natural Science Foundation of China [21376208, U1162124]; Zhejiang Provincial Natural Science Foundation for Distinguished Young Scholars of China [LR13B030001]; Specialized Research Fund for the Doctoral Program of Higher Education [J20130060]; Fundamental Research Funds for the Central Universities; Program for Zhejiang Leading Team of ST Innovation; Partner Group Program of the Zhejiang University; Max-Planck Society; Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [ERKCC61] FX Financial support from the National Natural Science Foundation of China (21376208 and U1162124), the Zhejiang Provincial Natural Science Foundation for Distinguished Young Scholars of China (LR13B030001), the Specialized Research Fund for the Doctoral Program of Higher Education (J20130060), the Fundamental Research Funds for the Central Universities, the Program for Zhejiang Leading Team of S&T Innovation, the Partner Group Program of the Zhejiang University, and the Max-Planck Society is greatly appreciated. P. Zhang and S. Dai. were supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number ERKCC61. NR 53 TC 28 Z9 28 U1 8 U2 119 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 13 PY 2014 VL 6 IS 15 BP 12515 EP 12522 DI 10.1021/am5023682 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AN2WI UT WOS:000340446300083 PM 25001196 ER PT J AU Lin, CK Piao, Y Kan, YC Bareno, J Bloom, I Ren, Y Amine, K Chen, ZH AF Lin, Chi-kai Piao, Ying Kan, Yongchun Bareno, Javier Bloom, Ira Ren, Yang Amine, Khalil Chen, Zonghai TI Probing Thermally Induced Decomposition of Delithiated Li1.2-xNi0.15Mn0.55Co0.1O2 by in Situ High-Energy X-ray Diffraction SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE safety; thermal stability; cathode; X-ray diffraction; lithium-ion battery ID LITHIUM-ION BATTERIES; STRUCTURAL-CHANGES; CATHODE MATERIALS; STABILITY; OXIDE; SAFETY; XRD AB Safety of lithium-ion batteries has been a major barrier to large-scale applications. For better understanding the failure mechanism of battery materials under thermal abuse, the decomposition of a delithiated high energy cathode material, Li1.2-xNi0.15Mn0.66Co0.1O2, in the stainless-steel high pressure capsules was investigated by in situ high energy X-ray diffraction. The data revealed that the thermally induced decomposition of the delithiated transition metal (TM) oxide was strongly influenced by the presence of electrolyte components. When there was no electrolyte, the layered structure for the delithiated TM oxide was changed to a disordered Li1-xM2O4-type spinel, which started at ca. 266 degrees C. The disordered Li1-xM2O4-type spinel was decomposed to a disordered M3O4-type spinel phase, which started at ca. 327 degrees C. In the presence of organic solvent, the layered structure was decomposed to a disordered M3O4-type spinel phase, and the onset temperature of the decomposition was ca. 216 degrees C. When the LiPF6 salt was also present, the onset temperature of the decomposition was changed to ca. 249 degrees C with the formation of MnF2 phase. The results suggest that a proper optimization of the electrolyte component, that is, the organic solvent and the lithium salt, can alter the decomposition pathway of delithiated cathodes, leading to improved safety of lithium-ion batteries. C1 [Lin, Chi-kai; Piao, Ying; Kan, Yongchun; Bareno, Javier; Bloom, Ira; Amine, Khalil; Chen, Zonghai] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Piao, Ying] Jilin Univ, Coll Phys, Key Lab Phys & Technol Adv Batteries, Minist Educ, Changchun 130012, Peoples R China. [Kan, Yongchun] Univ Sci & Technol China, State Key Lab Fire Sci, Hefei 230026, Anhui, Peoples R China. RP Chen, ZH (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zonghai.chen@anl.gov RI Chen, Zonghai/F-1067-2015; OI Chen, Zonghai/0000-0001-5371-9463; Bareno, Javier/0000-0003-1230-9278 FU U.S. Department of Energy (DOE), Office of Vehicle Technologies; U.S. DOE by UChicago Argonne, LLC [DE-AC02-06CH11357]; U.S. DOE, Office of Science, Office of Basic Energy Sciences; DOE Vehicle Technologies Program (VTP) of the Applied Battery Research (ABR) for Transportation Program FX Research at Argonne National Laboratory was funded by U.S. Department of Energy (DOE), Office of Vehicle Technologies. Argonne National Laboratory is operated for the U.S. DOE by UChicago Argonne, LLC, under Contract No. DE-AC02-06CH11357. The authors also acknowledge the use of the Advanced Photon Source of Argonne National Laboratory supported by the U.S. DOE, Office of Science, Office of Basic Energy Sciences. The cathodes were produced at the U.S. DOE Cell Analysis, Modeling and Prototyping (CAMP) facility, Argonne National Laboratory. The CAMP facility at Argonne is fully supported by the DOE Vehicle Technologies Program (VTP) within the core funding of the Applied Battery Research (ABR) for Transportation Program. NR 28 TC 10 Z9 10 U1 6 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 13 PY 2014 VL 6 IS 15 BP 12692 EP 12697 DI 10.1021/am502689f PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AN2WI UT WOS:000340446300104 PM 24977645 ER PT J AU Rao, SG Karim, A Schwartz, J Antler, N Schenkel, T Siddiqi, I AF Rao, Saleem G. Karim, Altaf Schwartz, Julian Antler, Natania Schenkel, Thomas Siddiqi, Irfan TI Directed Assembly of Nanodiamond Nitrogen-Vacancy Centers on a Chemically Modified Patterned Surface SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE nitrogen-vacancy center nanodiamond; directed self-assembly; self-assembled monolayer ID SINGLE-ELECTRON TRANSISTOR; CARBON NANOTUBES; NANOWIRES; NANOSTRUCTURES; DIAMOND; METALS; ARRAYS; FILMS AB Nitrogen-vacancy (NV) centers in nanodiamond (ND) particles are an attractive material for photonic, quantum information, and biological sensing technologies due to their optical properties-bright single photon emission and long spin coherence time. To harness these features in practical devices, it is essential to realize efficient methods to assemble and pattern NDs at the micro-/nanoscale. In this work, we report the large scale patterned assembly of NDs on a Au surface by creating hydrophobic and hydrophilic regions using self-assembled monolayer (SAM). Hydrophobic regions are created using a methyl (-CH3) terminated SAM of octadecanethiol molecules. Evaporating a water droplet suspension of NDs on the SAM patterned surface assembles the NDs in the bare Au, hydrophilic regions. Using this procedure, we successfully produced a ND structures in the shape of dots, lines, and rectangles. Subsequent photoluminescence imaging of the patterned NDs confirmed the presence of optically active NV centers. Experimental evidence in conjunction with computational analysis indicates that the surface wettability of the SAM modified Au surface plays a dominant role in the assembly of NDs as compared to van der Waals and other substrate - ND interactions. C1 [Rao, Saleem G.] King Fahd Univ Petr & Minerals, Dept Phys, Dhahran 31261, Saudi Arabia. [Karim, Altaf] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Enviornm Energy Technol Div, Berkeley, CA 94720 USA. [Schwartz, Julian; Schenkel, Thomas] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. [Schwartz, Julian] Tech Univ Ilmenau, Inst Micro & Nanoelect, Dept Micro & Nanoelect Syst, D-98684 Ilmenau, Germany. [Antler, Natania; Siddiqi, Irfan] Univ Calif Berkeley, Dept Phys, Quantum Nanoelect Lab, Berkeley, CA 94709 USA. RP Rao, SG (reprint author), King Fahd Univ Petr & Minerals, Dept Phys, Dhahran 31261, Saudi Arabia. EM saleemg@kfupm.edu.sa RI Siddiqi, Irfan/E-5548-2015 FU KFUPM department of physics; Deanship of Scientific Research King Fahd University of Petroleum and Minerals [RG1103-1,2] FX Support from the KFUPM department of physics is gratefully acknowledged. This work was supported by the Deanship of Scientific Research King Fahd University of Petroleum and Minerals grant no. RG1103-1,2. NR 45 TC 4 Z9 4 U1 3 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 13 PY 2014 VL 6 IS 15 BP 12893 EP 12900 DI 10.1021/am5027665 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AN2WI UT WOS:000340446300129 PM 25029262 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovinb, T Aguilar-Saavedraa, A Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexaa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, PA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Bangert, A Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertolucci, F Besana, I Besjes, GJ Bessidskaia, O Besson, N Betancourt, C Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De 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Zevi Zhang, D. Zhang, F. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, L. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the centrality and pseudorapidity dependence of the integrated elliptic flow in lead-lead collisions at root S-NN=2.76 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; NUCLEAR COLLISIONS; COLLABORATION; PERSPECTIVE AB The integrated elliptic flow of charged particles produced in Pb+Pb collisions at root S-NN = 2.76 TeV has been measured with the ATLAS detector using data collected at the Large Hadron Collider. 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M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, CH-1211 Geneva 23, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Tskhadadze, E. G.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA, Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E-E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripian, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripian, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Sandbach, R. L.; Snidero, G.; Castanheir, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, London, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Hsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Parkville, Vic 3052, Australia. [Amidei, D.; Cheng, H. C.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Harper, D.; Levin, D.; McCarn, A.; Neal, H. A.; Qian, J.; Wilson, A.; Xu, L.; Zhang, D.; Zhou, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F; Asbah, N.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Gjelsten, K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, I-56010 Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedraa, A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedraa, A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedraa, A.] Univ Granada, CAFPE, Granada, Spain. [Do Valle Wemans, A.] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, V.; Sopko, B.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P. P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, L. S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. 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R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. 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E.; Jon-And, K.; Khandanyan, H.; Kim, H. Y.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H. Y.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G-Y.; Saavedra, A. F.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskour, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Savard, P.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Savard, P.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vartapetian, A.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Alhroob, M.; De Sanctis, U.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Buszello, C. P.; Ferrari, A.; Isaksson, C.; Madsen, A.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.; Pasztor, G.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Gormley, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Korol, A. A.; Rezanova, O. L.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Nessi, M.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Moraes, Arthur/F-6478-2010; Ferrando, James/A-9192-2012; Bosman, Martine/J-9917-2014; Villa, Mauro/C-9883-2009; Warburton, Andreas/N-8028-2013; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Nepomuceno, Andre/M-9190-2014; Gabrielli, Alessandro/H-4931-2012; Lokajicek, Milos/G-7800-2014; Turra, Ruggero/N-2374-2014; Castro, Nuno/D-5260-2011; Li, Liang/O-1107-2015; Garcia, Jose /H-6339-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Delgado, Angel/L-8545-2014; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Smirnova, Oxana/A-4401-2013; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Marti-Garcia, Salvador/F-3085-2011; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Staroba, Pavel/G-8850-2014; Brooks, William/C-8636-2013; Lei, Xiaowen/O-4348-2014; Doyle, Anthony/C-5889-2009; Di Domenico, Antonio/G-6301-2011; de Groot, Nicolo/A-2675-2009; Wemans, Andre/A-6738-2012; Nemecek, Stanislav/G-5931-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009 OI Moraes, Arthur/0000-0002-5157-5686; Ferrando, James/0000-0002-1007-7816; Bosman, Martine/0000-0002-7290-643X; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Gabrielli, Alessandro/0000-0001-5346-7841; Castro, Nuno/0000-0001-8491-4376; Li, Liang/0000-0001-6411-6107; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Delgado, Angel/0000-0003-1843-5750; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Brooks, William/0000-0001-6161-3570; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 35 TC 6 Z9 6 U1 8 U2 107 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 13 PY 2014 VL 74 IS 8 AR 2982 DI 10.1140/epjc/s10052-014-2982-4 PG 25 WC Physics, Particles & Fields SC Physics GA AN4RB UT WOS:000340574300001 ER PT J AU Abelev, B Adam, J Adamova, D Aggarwal, MM Agnello, M Agostinelli, A Agrawal, N Ahammed, Z Ahmad, N Masoodi, AA Ahmed, I Ahn, SU Ahn, SA Aimo, I Aiola, S Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alexandre, D Alici, A Alkin, A Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Augustinus, A Averbeck, R Awes, TC Azmi, MD Bach, M Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, PC Baumann, C Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I 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Zhu, X. Zichichi, A. Zimmermann, A. Zimmermann, M. B. Zinovjev, G. Zoccarato, Y. Zynovyev, M. Zyzak, M. CA ALICE Collaboration TI Measurement of quarkonium production at forward rapidity in collisions at TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PP COLLISIONS; ROOT-S=7 TEV; P(P)OVER-BAR COLLISIONS; HADRONIC PRODUCTION; UPSILON-PRODUCTION; J/PSI PRODUCTION; CROSS-SECTIONS; PSI; HADROPRODUCTION; ALICE AB The inclusive production cross sections at forward rapidity of , , (1S) and (2S) are measured in collisions at with the ALICE detector at the LHC. The analysis is based on a data sample corresponding to an integrated luminosity of 1.35 pb. Quarkonia are reconstructed in the dimuon-decay channel and the signal yields are evaluated by fitting the invariant mass distributions. The differential production cross sections are measured as a function of the transverse momentum and rapidity , over the ranges GeV/c for , GeV/c for all other resonances and for . The measured cross sections integrated over and , and assuming unpolarized quarkonia, are: b, b, nb and nb, where the first uncertainty is statistical and the second one is systematic. The results are compared to measurements performed by other LHC experiments and to theoretical models. C1 CERN, CH-1211 Geneva 23, Switzerland. [Grigoryan, A.; Gulkanyan, H.; Papikyan, V.] Yerevan Phys Inst, AI Alikhanyan Natl Sci Lab, Yerevan 375036, Armenia. [Cortes Maldonado, I.; Fernandez Tellez, A.; Martinez, M. I.; Rodriguez Cahuantzi, M.; Tejeda Munoz, G.; Vargas, A.; Vergara Limon, S.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Alkin, A.; Chelnokov, V.; Grinyov, B.; Ivanytskyi, O.; Martynov, Y.; Trubnikov, V.; Zinovjev, G.; Zynovyev, M.] Bogolyubov Inst Theoret Phys, Kiev, Ukraine. [Das, S.; Ghosh, S. K.; Raha, S.] Bose Inst, Dept Phys, Kolkata, India. [Das, S.; Ghosh, S. K.; Raha, S.] Bose Inst, CAPSS, Kolkata, India. [Pestov, Y.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. 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[Milosevic, J.] Univ Wroclaw, Inst Theoret Phys, PL-50138 Wroclaw, Poland. [Oh, S. K.] Konkuk Univ, Seoul, South Korea. [Redlich, K.] Aligarh Muslim Univ, Dept Appl Phys, Aligarh, Uttar Pradesh, India. [Takaki, J. D. Tapia] Univ Kansas, Lawrence, KS 66045 USA. RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Suaide, Alexandre/L-6239-2016; Castillo Castellanos, Javier/G-8915-2013; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; feofilov, grigory/A-2549-2013; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Guber, Fedor/I-4271-2013; Zarochentsev, Andrey/J-6253-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Graczykowski, Lukasz/O-7522-2015; Janik, Malgorzata/O-7520-2015; Cosentino, Mauro/L-2418-2014; Bregant, Marco/I-7663-2012; Kovalenko, Vladimir/C-5709-2013; Bearden, Ian/M-4504-2014; Yang, Hongyan/J-9826-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Takahashi, Jun/B-2946-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Kucera, Vit/G-8459-2014; Krizek, Filip/G-8967-2014; Sevcenco, Adrian/C-1832-2012; Bielcikova, Jana/G-9342-2014; Vajzer, Michal/G-8469-2014; Wagner, Vladimir/G-5650-2014; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Usai, Gianluca/E-9604-2015; Ahmed, Ijaz/E-9144-2015; Salgado, Carlos A./G-2168-2015; Barnby, Lee/G-2135-2010; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014 OI Fiore, Enrichetta Maria/0000-0002-3548-2690; Suaide, Alexandre/0000-0003-2847-6556; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; feofilov, grigory/0000-0003-3700-8623; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Guber, Fedor/0000-0001-8790-3218; Zarochentsev, Andrey/0000-0002-3502-8084; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Janik, Malgorzata/0000-0002-3356-3438; Cosentino, Mauro/0000-0002-7880-8611; Kovalenko, Vladimir/0000-0001-6012-6615; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Takahashi, Jun/0000-0002-4091-1779; Sevcenco, Adrian/0000-0002-4151-1056; Peitzmann, Thomas/0000-0002-7116-899X; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Barnby, Lee/0000-0001-7357-9904; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461 FU Worldwide LHC Computing Grid (WLCG) collaboration; State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy of the Government of India; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT; DGAPA, Mexico; ALFA-EC; EPLANET Program (European Particle Physics Latin American Network) Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics; CNCS-UEFISCDI-Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN; Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut AMP; Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio FX We are grateful to M. Butenschoen, K.-T. Chao, R. L. Kisslinger and J.-P. Lansberg for providing us model calculations and for intensive discussions. The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration. The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German BMBF and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC and the EPLANET Program (European Particle Physics Latin American Network) Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and CNCS-UEFISCDI-Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 56 TC 27 Z9 28 U1 0 U2 84 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. 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Dias, FA Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, 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Mesropian, C. Arora, S. Barker, A. Chou, J. P. Contreras-Campana, C. Contreras-Campana, E. Duggan, D. Ferencek, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Lath, A. Panwalkar, S. Park, M. Patel, R. Rekovic, V. Robles, J. Salur, S. Schnetzer, S. Seitz, C. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. Yang, Z. C. York, A. Bouhali, O. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Rose, A. Safonov, A. Sakuma, T. Suarez, I. Tatarinov, A. Toback, D. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wood, J. Gollapinni, S. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Belknap, D. A. Borrello, L. Carlsmith, D. Cepeda, M. Dasu, S. Duric, S. Friis, E. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Woods, N. CA CMS Collaboration TI Search for invisible decays of Higgs bosons in the vector boson fusion and associated ZH production modes SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID DARK-MATTER; LHC; DETECTOR; PARTICLE; LEP AB A search for invisible decays of Higgs bosons is performed using the vector boson fusion and associated ZH production modes. In the ZH mode, the Z boson is required to decay to a pair of charged leptons or a bb quark pair. The searches use the 8TeV pp collision dataset collected by the CMS detector at the LHC, corresponding to an integrated luminosity of up to 19.7 fb(-1). Certain channels include data from 7TeV collisions corresponding to an integrated luminosity of 4.9 fb(-1).The searches are sensitive to non-standardmodel invisible decays of the recently observed Higgs boson, as well as additional Higgs bosons with similar production modes and large invisible branching fractions. In all channels, the observed data are consistent with the expected standard model backgrounds. Limits are set on the production cross section times invisible branching fraction, as a function of the Higgs boson mass, for the vector boson fusion and ZH production modes. By combining all channels, and assuming standard model Higgs boson cross sections and acceptances, the observed (expected) upper limit on the invisible branching fraction at m(H) = 125GeV is found to be 0.58 (0.44) at 95% confidence level. We interpret this limit in terms of a Higgs-portal model of dark matter interactions. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. 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G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Komm, M.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; Correa Martins Junior, M.; Martins, T.; Pol, M. E.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Alda Junior, W. L.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Malek, M.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santaolalla, J.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dias, F. A.; Fernandez Perez Tomei, T. R.; Novaes, S. 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T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Pioppi, M.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Asghar, M. I.; Butt, J.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Golutvin, I.; Gorbunov, I.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Contardo, D.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Evangelou, I.; Foudas, C.; Bencze, G.; Sharma, A.; Mohanty, A. K.; Giordano, F.; Meola, S.; Paolucci, P.; Galanti, M.; Palla, F.; Pelliccioni, M.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Srimanobhas, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Richardson, C.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Mahrous, A.] Helwan Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] CNRS IN2P3, Paris, France. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Bluj, M.] Natl Ctr Nucl Res, Otwock, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Istanbul Univ, Fac Sci, Istanbul, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [CMS Collaboration] CERN, Geneva, Switzerland. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI de la Cruz, Begona/K-7552-2014; Gonzalez Caballero, Isidro/E-7350-2010; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Montanari, Alessandro/J-2420-2012; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Scodellaro, Luca/K-9091-2014; Cerrada, Marcos/J-6934-2014; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Popov, Andrey/E-1052-2012; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; OI Gonzalez Caballero, Isidro/0000-0002-8087-3199; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Russ, James/0000-0001-9856-9155; Codispoti, Giuseppe/0000-0003-0217-7021; Scodellaro, Luca/0000-0002-4974-8330; Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Popov, Andrey/0000-0002-1207-0984; Kasemann, Matthias/0000-0002-0429-2448; Barbieri, Richard/0000-0002-7945-005X; Landsberg, Greg/0000-0002-4184-9380; Blekman, Freya/0000-0002-7366-7098; Marzocchi, Badder/0000-0001-6687-6214; Costa, Salvatore/0000-0001-9919-0569; Gerosa, Raffaele/0000-0001-8359-3734; Malik, Sudhir/0000-0002-6356-2655; Staiano, Amedeo/0000-0003-1803-624X; Tonelli, Guido Emilio/0000-0003-2606-9156; Abbiendi, Giovanni/0000-0003-4499-7562; WANG, MIN-ZU/0000-0002-0979-8341; Rizzi, Andrea/0000-0002-4543-2718; Gershtein, Yuri/0000-0002-4871-5449; Androsov, Konstantin/0000-0003-2694-6542; HSIUNG, YEE/0000-0003-4801-1238; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Tosi, Nicolo/0000-0002-0474-0247; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Margaroli, Fabrizio/0000-0002-3869-0153; Tricomi, Alessia Rita/0000-0002-5071-5501; Martinez Ruiz del Arbol, Pablo/0000-0002-7737-5121; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Fiorendi, Sara/0000-0003-3273-9419; Toback, David/0000-0003-3457-4144; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Vidal Marono, Miguel/0000-0002-2590-5987; Goldstein, Joel/0000-0003-1591-6014; Korenkov, Vladimir/0000-0002-2342-7862; Heath, Helen/0000-0001-6576-9740; Grassi, Marco/0000-0003-2422-6736; ORTONA, Giacomo/0000-0001-8411-2971; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Ulrich, Ralf/0000-0002-2535-402X; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Sogut, Kenan/0000-0002-9682-2855; Jacob, Jeson/0000-0001-6895-5493 FU Austrian Federal Ministry of Science and Research; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland, Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education and University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science by EU, Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the royal patronage of H. R. H. Princess Maha Chakri Sirindhorn of Thailand. NR 78 TC 45 Z9 45 U1 10 U2 95 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 13 PY 2014 VL 74 IS 8 AR 2980 DI 10.1140/epjc/s10052-014-2980-6 PG 35 WC Physics, Particles & Fields SC Physics GA AN4QY UT WOS:000340574000001 ER PT J AU Klebanoff, LE Breit, J Roe, GS Damberger, T Erbel, T Wingert, S Coleman, B Radley, CJ Oros, JM Schuttinger, P Woolley, R Ghotb, H Prey, S Velinsky, S White, W Saunders, R Saunders, C Drake, R Rea, G Fliess, D Hooson, R Elrick, WT Hamilton, J Skradski, T Brown, G Chao, B Zelinsky, M Sorkin, A McGlaughlin, R Moreland, G Hanley, RC Koonce, M Johnson, TA AF Klebanoff, L. E. Breit, Js. Roe, G. S. Damberger, T. Erbel, T. Wingert, S. Coleman, B. Radley, C. J. Oros, J. M. Schuttinger, P. Woolley, R. Ghotb, H. Prey, S. Velinsky, S. White, W. Saunders, R. Saunders, C. Drake, R. Rea, G. Fliess, D. Hooson, R. Elrick, W. T. Hamilton, J. Skradski, T. Brown, G. Chao, B. Zelinsky, M. Sorkin, A. McGlaughlin, R. Moreland, G. Hanley, R. C. Koonce, M. Johnson, T. A. TI Fuel cell mobile lighting: A fuel cell market transformation project SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Fuel cell; Market transformation; Mobile lighting; Construction equipment; Ground support equipment AB We report the results of a project aimed to introduce proton exchange membrane (PEM) hydrogen fuel cell technology into aviation ground support equipment (GSE) and rental construction equipment. The purpose of the project was to design, build, field-test and then commercialize fuel cell equipment that is superior to its diesel counterpart. The commercializing of this hydrogen-based technology will help to start the process of displacing diesel fuel use in aviation GSE and in mobile construction equipment. We describe a hydrogen fuel cell mobile lighting tower (H2LT) that combines hydrogen stored as a high pressure gas, PEM fuel cell technology, and advanced lighting into a single unit with uses in aviation and construction. We assembled a project team of 15 institutional partners combining new technology expertise (hydrogen, fuel cells), equipment mass manufacturing capability (mobile light towers, lighting) and influential end-users to field test the H2LT in real-world use in diverse environments. Seed funding provided by Boeing enabled additional funding from the U.S. Department of Energy (DOE) and a preponderance of in-kind contributions from the industrial partners. Prototype units were constructed and field tested in the entertainment industry, at the San Francisco International Airport, at the NASA Kennedy Space Center, with the California Department of Transportation (Caltrans), and with the Connecticut Department of Transportation. The goals of these approximately year-long field tests were to assess operation of the H2LT technology in a wide variety of potentially corrosive environments (cold, wet, hot, humid, salty air) performing a wide variety of tasks, to reduce diesel emissions at these locations, and to help promote hydrogen PEM technology in new influential markets. The H2LT proved to be exceptionally durable in these diverse environments, demonstrating the compatibility of PEM fuel cells and high-pressure hydrogen storage with the construction equipment application. Results from the field tests are discussed, including system performance (efficiency, duration, durability) and the efficacy of refueling the system by different methods (H-2 stations, mobile refueling). The H2LT system is compared directly to a comparable diesel-fueled light tower with regard to size, performance and emissions savings. Overall, end users were pleased with the performance of the H2LT, noting the lack of emissions and exceptionally low noise level. Recommendations for improvement were also collected and will be discussed. Two types of lighting used on the H2LT (plasma, LED) were characterized by U.C. Davis in collaboration with Caltrans. LED lighting was found to be the most energy efficient and robust lighting technology for the highly mobile H2LT application. The technical "lessons-learned" are reviewed, along with the plans for commercialization of the H2LT technology by Multiquip Inc. Finally, the benefits to the industrial participants of the project organization are described. Copyright (C) 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Klebanoff, L. E.; Johnson, T. A.] Sandia Natl Labs, Livermore, CA 94551 USA. [Breit, Js.; Roe, G. S.] Boeing Commercial Airplanes, Syst Concept Ctr, Everett, WA 98203 USA. [Damberger, T.] Golden State Energy, Carson City, NV 89703 USA. [Erbel, T.; Wingert, S.; Coleman, B.] Multiquip Inc, Carson, CA 90746 USA. [Radley, C. J.; Oros, J. M.; Schuttinger, P.] Altergy Syst, Folsom, CA 95630 USA. [Woolley, R.; Ghotb, H.; Prey, S.] Caltrans Div Res, Innovat & Syst Informat Technol Applicat Off, Irvine, CA 92612 USA. [Velinsky, S.; White, W.] Univ Calif Davis, Dept Mech & Aerosp Engn, Davis, CA 95616 USA. [Saunders, R.; Saunders, C.] Saunders Elect Inc, Arleta, CA 91331 USA. [Drake, R.; Rea, G.] Stray Light Opt Technol Inc, Scottsburg, IN 47170 USA. [Fliess, D.; Hooson, R.] San Francisco Int Airport, City & Cty San Francisco, San Francisco, CA 94128 USA. [Elrick, W. T.; Hamilton, J.] Calif Fuel Cell Partnership, West Sacramento, CA 95691 USA. [Skradski, T.] Lumenworks, Oakland, CA 94610 USA. [Brown, G.] Luxirn Corp, Santa Clara, CA 95054 USA. [Chao, B.; Zelinsky, M.] Ovon Hydrogen Syst, Rochester Hills, MI 48309 USA. [Sorkin, A.; McGlaughlin, R.] NASA, TEERM Principal Ctr, Kennedy Space Ctr, FL 32899 USA. [Moreland, G.] SRA Int, Latham, NY USA. [Hanley, R. C.] Connecticut Dept Transportat, Newington, CT 06131 USA. [Koonce, M.] IGX Grp Inc, San Francisco, CA 94102 USA. RP Klebanoff, LE (reprint author), Sandia Natl Labs, POB 969,MS 9161,7011 East Ave, Livermore, CA 94551 USA. EM lekleba@sandia.gov FU Boeing Company [SC02/1651.14.00]; Fuel Cell Market Transformation Program at the U.S. DOE Fuel Cell Technologies Office; DOE; Division of Research and Innovation at Caltrans (under the direction of Larry Orcutt); U.C. Davis AHMCT; NASA KSC; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Partial funding from the Boeing Company is gratefully acknowledged via the Boeing/Sandia CRADA SC02/1651.14.00. Funding from the Fuel Cell Market Transformation Program (led by Pete Devlin) at the U.S. DOE Fuel Cell Technologies Office was critical, making the broader and stronger development project possible, and specifically allowing the construction and field testing of five additional H2LT units. In addition to funding, we appreciate the encouragement of Pete and his colleagues Nancy Garland and John Christensen in the Market Transformation program. Special thanks to Sunita Satyapal at DOE for supporting this work. The authors thank Tien Nguyen of DOE for providing an analysis of GHG emissions for the H2LT technology, with the hydrogen derived from either steam reforming of natural gas, or wind-based electrolysis of water.; The project would not have been successful without the participation of Caltrans. We thank Randy Iwasaki, former director of Caltrans, for providing wonderful encouragement and support of the work in its early phases, and offering resources of the Division of Research and Innovation at Caltrans (under the direction of Larry Orcutt) to be applied in support of the project. Larry Orcutt directed Nancy Chinlund of Caltrans to become involved. Nancy was very proactive in launching the project from a Caltrans perspective, which led directly to Randy Woolley's involvement in the project. The Caltrans partners aggressively challenged the project to build a prototype in a few months' time to be shown at the 2009 AASHTO meeting.; Caltrans provided considerable in-kind support through the donation of its own technical expertise and through its support of the U.C. Davis AHMCT for characterizing the lighting options for the H2LT as well as supervising the Caltrans District 3 field test. We acknowledge the contributions of Gonzalo Gomez of Caltrans for discussions of lighting technology options for the H2LT. Ben Creed, Lauren Miller, Sean Donohoe and Matt Jones at U.C. Davis provided many hours of night work characterizing the illumination provided by the candidate plasma, LED and MH lighting options. In a related activity, Ty Larson of Boeing performed checks that the glass covering the plasma lights was sufficiently absorbing UV radiation, which was very helpful.; The staff at Saunders Electric, including Ron Brewer, Frank Soggiu and Pat Hess were instrumental in the 3-year field tests of the Alpha and Beta H2LT units used for the Los Angeles entertainment award shows and elsewhere in the entertainment industry.; The field test of the unit at the NASA KSC was an excellent example of cooperation between government agencies. We thank Chuck Griffin for providing local supervision of the project from the NASA KSC end, along with a lot of help from Melissa Clevenger of the propellants group and Ray Davis from operations. The KSC staff were extremely professional and helpful. We thank Pattie Lewis Burford (ITB Inc.) and Jerry Curran (EASI) for providing corrosion inspection of the Beta unit that was field tested at the NASA KSC for a year, and Randy Morris for extensive coordination.; Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 9 TC 3 Z9 3 U1 0 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD AUG 13 PY 2014 VL 39 IS 24 BP 12948 EP 12972 DI 10.1016/j.ijhydene.2014.05.180 PG 25 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA AN6FI UT WOS:000340689900058 ER PT J AU Das, S Rastogi, A Wu, LJ Zheng, JC Hossain, Z Zhu, YM Budhani, RC AF Das, Shubhankar Rastogi, A. Wu, Lijun Zheng, Jin-Cheng Hossain, Z. Zhu, Yimei Budhani, R. C. TI Kondo scattering in delta-doped LaTiO3/SrTiO3 interfaces: Renormalization by spin-orbit interactions SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-FIELD; THIN-FILMS; MAGNETORESISTANCE; ELECTRONS; TITANATE; SYSTEMS; ALLOYS; TIME AB We present a study of delta doping at the LaTiO3/SrTiO3 interface with isostructural antiferromagnetic perovskite LaCrO3 that dramatically alters the properties of the two-dimensional electron gas at the interface. The effects include a reduction in sheet-carrier density, prominence of the low-temperature resistivity minimum, enhancement of weak antilocalization below 10 K, and observation of a strong anisotropic magnetoresistance (MR). The positive and negative MR for out-of-plane and in-plane fields, respectively, and the field and temperature dependencies of MR suggest Kondo scattering by localized Ti3+ moments renormalized by spin-orbit interaction at T < 10 K, with the increased delta-layer thickness. Electron-energy-loss spectroscopy and density functional calculations provide convincing evidence of blocking of electron transfer from LTO to STO by the delta layer. C1 [Das, Shubhankar; Rastogi, A.; Hossain, Z.; Budhani, R. C.] Indian Inst Technol, Dept Phys, Condensed Matter Low Dimens Syst Lab, Kanpur 208016, Uttar Pradesh, India. [Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Zheng, Jin-Cheng] Xiamen Univ, Dept Phys, Xiamen 361005, Peoples R China. [Zheng, Jin-Cheng] Xiamen Univ, Fujian Prov Key Lab Theoret & Computat Chem, Xiamen 361005, Peoples R China. [Budhani, R. C.] CSIR, Natl Phys Lab, New Delhi 110012, India. RP Das, S (reprint author), Indian Inst Technol, Dept Phys, Condensed Matter Low Dimens Syst Lab, Kanpur 208016, Uttar Pradesh, India. EM rcb@iitk.ac.in RI Rastogi, Ankur/G-5311-2010; Rastogi, Ankur/O-4979-2014; Zheng, JC/G-3383-2010 OI Rastogi, Ankur/0000-0002-4056-9088; Rastogi, Ankur/0000-0002-4056-9088; Zheng, JC/0000-0002-6292-3236 FU Department of Science and Technology, India; IIT Kanpur; CSIR; CSIR-India; US Department of Energy, Office of Basic Energy Science [DE-AC02-98CH10886]; NSF of China [U1232110] FX We thank P. C. Joshi for technical support. R.C.B. acknowledges a J. C. Bose National Fellowship from the Department of Science and Technology, India. S. D. and A. R. thank IIT Kanpur and CSIR for financial support. This research has been funded by CSIR-India and IIT Kanpur. Work at BNL was supported by the US Department of Energy, Office of Basic Energy Science, under Contract No. DE-AC02-98CH10886. J.C.Z. acknowledge the support of the NSF of China (Grant No. U1232110). NR 36 TC 5 Z9 5 U1 8 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 13 PY 2014 VL 90 IS 8 AR 081107 DI 10.1103/PhysRevB.90.081107 PG 5 WC Physics, Condensed Matter SC Physics GA AO1VZ UT WOS:000341104900002 ER PT J AU Spataru, CD Leonard, F AF Spataru, Catalin D. Leonard, Francois TI Fermi-level pinning, charge transfer, and relaxation of spin-momentum locking at metal contacts to topological insulators SO PHYSICAL REVIEW B LA English DT Article ID AUGMENTED-WAVE METHOD; SINGLE DIRAC CONE; SURFACE; BI2TE3 AB Topological insulators are of interest for many applications in electronics and optoelectronics, but harnessing their unique properties requires detailed understanding and control of charge injection at electrical contacts. Here we present large-scale ab initio calculations of the electronic properties of Au, Ni, Pt, Pd, and graphene contacts to Bi2Se3. We show that regardless of the metal, the Fermi level is located in the conduction band, leading to n-type Ohmic contact to the first quintuplet. Furthermore, we find strong charge transfer and band bending in the first few quintuplets, with no Schottky barrier for charge injection even when the topological insulator is undoped. Our calculations indicate that Au and graphene leave the spin-momentum locking mostly unaltered, but on the other hand, Ni, Pd, and Pt strongly hybridize with Bi2Se3 and relax spin-momentum locking. Our results indicate that judicious choice of the contact metal is essential to reveal the unique surface features of topological insulators. C1 [Spataru, Catalin D.; Leonard, Francois] Sandia Natl Labs, Livermore, CA 94551 USA. RP Spataru, CD (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM cdspata@sandia.gov FU Office of Naval Research [N0001413IP20091]; Laboratory Directed Research and Development Program at Sandia National Laboratories; United States Department of Energy [DEAC01-94-AL85000] FX We thank Peter Sharma, Michael Shaughnessy, and Thomas Beechem for useful discussions. This work was supported by the Electromagnetic Materials program of the Office of Naval Research under Agreement No. N0001413IP20091 and the Laboratory Directed Research and Development Program at Sandia National Laboratories, a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Co., for the United States Department of Energy under Contract No. DEAC01-94-AL85000. NR 27 TC 0 Z9 0 U1 4 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 13 PY 2014 VL 90 IS 8 AR 085115 DI 10.1103/PhysRevB.90.085115 PG 6 WC Physics, Condensed Matter SC Physics GA AO1VZ UT WOS:000341104900004 ER PT J AU Ying, T Mondaini, R Sun, XD Paiva, T Fye, RM Scalettar, RT AF Ying, T. Mondaini, R. Sun, X. D. Paiva, T. Fye, R. M. Scalettar, R. T. TI Determinant quantum Monte Carlo study of d-wave pairing in the plaquette Hubbard hamiltonian SO PHYSICAL REVIEW B LA English DT Article ID EXACT-DIAGONALIZATION; NUMERICAL-SIMULATION; HOLE DYNAMICS; MODEL; BINDING; SUPERCONDUCTORS; CLUSTERS; SYSTEMS AB Determinant quantum Monte Carlo (DQMC) is used to determine the pairing and magnetic response for a Hubbard model built up from four-site clusters-a two-dimensional square lattice consisting of elemental 2 x 2 plaquettes with hopping t and on-site repulsion U coupled by an interplaquette hopping t' <= t. Superconductivity in this geometry has previously been studied by a variety of analytic and numeric methods, with differing conclusions concerning whether the pairing correlations and transition temperature are raised near half filling by the inhomogeneous hopping or not. For U/t = 4, DQMC indicates an optimal t'/t approximate to 0.4 at which the pairing vertex is most attractive. The optimal t'/t increases with U/t. We then contrast our results for this plaquette model with a hamiltonian which instead involves a regular pattern of site energies whose large site energy limit is the three-band CuO2 model; we show that there the inhomogeneity rapidly, and monotonically, suppresses pairing. C1 [Ying, T.; Sun, X. D.] Harbin Inst Technol, Dept Phys, Harbin 150001, Peoples R China. [Mondaini, R.] Penn State Univ, Dept Phys, Davey Lab 104, University Pk, PA 16802 USA. [Mondaini, R.; Scalettar, R. T.] Univ Calif Davis, Phys Dept, Davis, CA 95616 USA. [Paiva, T.] Univ Fed Rio de Janeiro, Inst Fis, BR-21941972 Rio De Janeiro, RJ, Brazil. [Fye, R. M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ying, T (reprint author), Harbin Inst Technol, Dept Phys, Harbin 150001, Peoples R China. RI Paiva, Thereza/B-9778-2013; Mondaini, Rubem/A-9433-2013 OI Paiva, Thereza/0000-0002-4199-3809; Mondaini, Rubem/0000-0001-8005-2297 FU National Key Basic Research Program of China [2013CB328702]; DOE [DE-NA0001842-0]; Office of the President of the University of California; CNPq; FAPERJ FX This work was supported by the National Key Basic Research Program of China, Grant No. 2013CB328702, by DOE DE-NA0001842-0, and by the Office of the President of the University of California. Support from CNPq and FAPERJ (TP and RM) is gratefully acknowledged. NR 44 TC 4 Z9 4 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 13 PY 2014 VL 90 IS 7 AR 075121 DI 10.1103/PhysRevB.90.075121 PG 11 WC Physics, Condensed Matter SC Physics GA AO1VY UT WOS:000341104800001 ER PT J AU Bedlinskiy, I Kubarovsky, V Niccolai, S Stoler, P Adhikari, KP Anderson, MD Pereira, SA Avakian, H Ball, J Baltzell, NA Battaglieri, M Batourine, V Biselli, AS Boiarinov, S Bono, J Briscoe, WJ Brooks, WK Burkert, VD Carman, DS Celentano, A Chandavar, S Colaneri, L Cole, PL Contalbrigo, M Cortes, O Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Doughty, D Dupre, R Egiyan, H El Alaoui, A El Fassi, L Elouadrhiri, L Eugenio, P Fedotov, G Fegan, S Fleming, JA Forest, TA Garillon, B Garcon, M Gavalian, G Gevorgyan, N Ghandilyan, Y Gilfoyle, GP Giovanetti, KL Girod, FX Golovatch, E Gothe, RW Griffioen, KA Guegan, B Guidal, M Guo, L Hafidi, K Hakobyan, H Harrison, N Hattawy, M Hicks, K Holtrop, M Ireland, DG Ishkhanov, BS Isupov, EL Jenkins, D Jo, HS Joo, K Keller, D Khandaker, M Kim, A Kim, W Klein, A Klein, FJ Koirala, S Kuhn, SE Kuleshov, SV Lenisa, P Levine, WI Livingston, K Lu, HY MacGregor, IJD Markov, N Mayer, M McKinnon, B Mirazita, M Mokeev, V Montgomery, RA Moody, CI Moutarde, H Movsisyan, A Camacho, CM Nadel-Turonski, P Niculescu, I Osipenko, M Ostrovidov, AI Pappalardo, LL Park, K Park, S Pasyuk, E Phelps, E Phelps, W Phillips, JJ Pisano, S Pogorelko, O Price, JW Prok, Y Protopopescu, D Procureur, S Puckett, AJR Raue, BA Ripani, M Ritchie, BG Rizzo, A Rossi, P Roy, P Sabatie, F Salgado, C Schott, D Schumacher, RA Seder, E Senderovich, I Sharabian, YG Simonyan, A Smith, GD Sober, DI Sokhan, D Stepanyan, SS Strauch, S Sytnik, V Tang, W Tian, Y Ungaro, M Vlassov, AV Voskanyan, H Voutier, E Walford, NK Watts, D Wei, X Weinstein, LB Yurov, M Zachariou, N Zana, L Zhang, J Zhao, ZW Zonta, I AF Bedlinskiy, I. Kubarovsky, V. Niccolai, S. Stoler, P. Adhikari, K. P. Anderson, M. D. Pereira, S. Anefalos Avakian, H. Ball, J. Baltzell, N. A. Battaglieri, M. Batourine, V. Biselli, A. S. Boiarinov, S. Bono, J. Briscoe, W. J. Brooks, W. K. Burkert, V. D. Carman, D. S. Celentano, A. Chandavar, S. Colaneri, L. Cole, P. L. Contalbrigo, M. Cortes, O. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Doughty, D. Dupre, R. Egiyan, H. El Alaoui, A. El Fassi, L. Elouadrhiri, L. Eugenio, P. Fedotov, G. Fegan, S. Fleming, J. A. Forest, T. A. Garillon, B. Garcon, M. Gavalian, G. Gevorgyan, N. Ghandilyan, Y. Gilfoyle, G. P. Giovanetti, K. L. Girod, F. X. Golovatch, E. Gothe, R. W. Griffioen, K. A. Guegan, B. Guidal, M. Guo, L. Hafidi, K. Hakobyan, H. Harrison, N. Hattawy, M. Hicks, K. Holtrop, M. Ireland, D. G. Ishkhanov, B. S. Isupov, E. L. Jenkins, D. Jo, H. S. Joo, K. Keller, D. Khandaker, M. Kim, A. Kim, W. Klein, A. Klein, F. J. Koirala, S. Kuhn, S. E. Kuleshov, S. V. Lenisa, P. Levine, W. I. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Markov, N. Mayer, M. McKinnon, B. Mirazita, M. Mokeev, V. Montgomery, R. A. Moody, C. I. Moutarde, H. Movsisyan, A. Camacho, C. Munoz Nadel-Turonski, P. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Pappalardo, L. L. Park, K. Park, S. Pasyuk, E. Phelps, E. Phelps, W. Phillips, J. J. Pisano, S. Pogorelko, O. Price, J. W. Prok, Y. Protopopescu, D. Procureur, S. Puckett, A. J. R. Raue, B. A. Ripani, M. Ritchie, B. G. Rizzo, A. Rossi, P. Roy, P. Sabatie, F. Salgado, C. Schott, D. Schumacher, R. A. Seder, E. Senderovich, I. Sharabian, Y. G. Simonyan, A. Smith, G. D. Sober, D. I. Sokhan, D. Stepanyan, S. S. Strauch, S. Sytnik, V. Tang, W. Tian, Ye Ungaro, M. Vlassov, A. V. Voskanyan, H. Voutier, E. Walford, N. K. Watts, D. Wei, X. Weinstein, L. B. Yurov, M. Zachariou, N. Zana, L. Zhang, J. Zhao, Z. W. Zonta, I. CA CLAS Collaboration TI Exclusive pi(0) electroproduction at W > 2 GeV with CLAS SO PHYSICAL REVIEW C LA English DT Article ID PION ELECTROPRODUCTION; PARTON DISTRIBUTIONS; MESONS; TRANSVERSITY; SYSTEM AB Exclusive neutral-pion electroproduction (ep -> e'p'pi(0)) was measured at Jefferson Lab with a 5.75-GeV electron beam and the CLAS detector. Differential cross sections d(4)sigma/dtdQ(2)dx(B)d phi(pi) and structure functions sigma(T) + sigma(L), sigma(TT), and sigma(LT) as functions of t were obtained over a wide range of Q(2) and x(B). The data are compared with Regge and handbag theoretical calculations. Analyses in both frameworks find that a large dominance of transverse processes is necessary to explain the experimental results. For the Regge analysis it is found that the inclusion of vector meson rescattering processes is necessary to bring the magnitude of the calculated and measured structure functions into rough agreement. In the handbag framework, there are two independent calculations, both of which appear to roughly explain the magnitude of the structure functions in terms of transversity generalized parton distributions. C1 [Baltzell, N. A.; El Alaoui, A.; Hafidi, K.; Moody, C. I.] Argonne Natl Lab, Argonne, IL 60439 USA. [Ritchie, B. G.; Senderovich, I.] Arizona State Univ, Tempe, AZ 85287 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Levine, W. I.; Schumacher, R. A.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Klein, F. J.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Ball, J.; Garcon, M.; Girod, F. X.; Moutarde, H.; Procureur, S.; Sabatie, F.] CEA, Ctr Saclay, Irfu Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Doughty, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Harrison, N.; Joo, K.; Kim, A.; Markov, N.; Puckett, A. J. R.; Seder, E.; Ungaro, M.] Univ Connecticut, Storrs, CT 06269 USA. [Biselli, A. S.] Fairfield Univ, Fairfield, CT 06824 USA. [Bono, J.; Guo, L.; Phelps, W.; Raue, B. A.] Florida Int Univ, Miami, FL 33199 USA. [Crede, V.; Eugenio, P.; Ostrovidov, A. I.; Park, S.; Roy, P.] Florida State Univ, Tallahassee, FL 32306 USA. [Niccolai, S.; Briscoe, W. J.; Nadel-Turonski, P.; Schott, D.; Strauch, S.] George Washington Univ, Washington, DC 20052 USA. [Cole, P. L.; Cortes, O.; Forest, T. A.; Khandaker, M.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Pereira, S. Anefalos; De Sanctis, E.; Mirazita, M.; Montgomery, R. A.; Pisano, S.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Colaneri, L.; D'Angelo, A.; Rizzo, A.; Zonta, I.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Niccolai, S.; Dupre, R.; Garillon, B.; Guegan, B.; Guidal, M.; Hattawy, M.; Jo, H. S.; Camacho, C. Munoz; Sokhan, D.] Inst Phys Nucl ORSAY, Orsay, France. [Bedlinskiy, I.; Kuleshov, S. V.; Pogorelko, O.; Vlassov, A. V.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Giovanetti, K. L.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Batourine, V.; Kim, W.; Park, K.; Stepanyan, S. S.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Voutier, E.] Univ Grenoble 1, CNRS, LPSC, INPG,IN2P3, Grenoble, France. [Egiyan, H.; Holtrop, M.; Zana, L.] Univ New Hampshire, Durham, NH 03824 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Chandavar, S.; Hicks, K.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Adhikari, K. P.; El Fassi, L.; Gavalian, G.; Klein, A.; Koirala, S.; Kuhn, S. E.; Mayer, M.; Prok, Y.; Weinstein, L. B.; Zhang, J.] Old Dominion Univ, Norfolk, VA 23529 USA. [Kubarovsky, V.; Stoler, P.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Gilfoyle, G. P.] Univ Richmond, Richmond, VA 23173 USA. [D'Angelo, A.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Fedotov, G.; Golovatch, E.; Ishkhanov, B. S.; Isupov, E. L.; Mokeev, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119234, Russia. [Baltzell, N. A.; Djalali, C.; Fedotov, G.; Gothe, R. W.; Lu, H. Y.; Phelps, E.; Strauch, S.; Tian, Ye; Zachariou, N.; Zhao, Z. W.] Univ S Carolina, Columbia, SC 29208 USA. [Kubarovsky, V.; Avakian, H.; Batourine, V.; Boiarinov, S.; Brooks, W. K.; Burkert, V. D.; Carman, D. S.; Deur, A.; Doughty, D.; Egiyan, H.; Elouadrhiri, L.; Girod, F. X.; Guo, L.; Mokeev, V.; Nadel-Turonski, P.; Park, K.; Pasyuk, E.; Prok, Y.; Raue, B. A.; Rossi, P.; Sharabian, Y. G.; Ungaro, M.; Wei, X.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Brooks, W. K.; Hakobyan, H.; Kuleshov, S. V.; Sytnik, V.] Univ Tecn Federico Santa Maria, Region, Chile. [Fleming, J. A.; Smith, G. D.; Zana, L.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Anderson, M. D.; Ireland, D. G.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Phillips, J. J.; Protopopescu, D.; Sokhan, D.; Watts, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Jenkins, D.] Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. [Keller, D.; Prok, Y.; Yurov, M.; Zhao, Z. W.] Univ Virginia, Charlottesville, VA 22901 USA. [Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Dashyan, N.; Gevorgyan, N.; Ghandilyan, Y.; Hakobyan, H.; Simonyan, A.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Bedlinskiy, I (reprint author), Inst Theoret & Expt Phys, Moscow 117218, Russia. RI Kuleshov, Sergey/D-9940-2013; D'Angelo, Annalisa/A-2439-2012; Celentano, Andrea/J-6190-2012; Rizzo, Alessandro/C-6397-2014; Schumacher, Reinhard/K-6455-2013; Brooks, William/C-8636-2013; Lu, Haiyun/B-4083-2012; Ireland, David/E-8618-2010; El Alaoui, Ahmed/B-4638-2015; MacGregor, Ian/D-4072-2011; Sabatie, Franck/K-9066-2015; Osipenko, Mikhail/N-8292-2015; Zhang, Jixie/A-1461-2016 OI Bono, Jason/0000-0002-3018-714X; Kuleshov, Sergey/0000-0002-3065-326X; D'Angelo, Annalisa/0000-0003-3050-4907; Celentano, Andrea/0000-0002-7104-2983; Rizzo, Alessandro/0000-0001-5597-8514; Schumacher, Reinhard/0000-0002-3860-1827; Brooks, William/0000-0001-6161-3570; Ireland, David/0000-0001-7713-7011; Sabatie, Franck/0000-0001-7031-3975; Osipenko, Mikhail/0000-0001-9618-3013; FU US Department of Energy and National Science Foundation; French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique; French-American Cultural Exchange (FACE); Italian Istituto Nazionale di Fisica Nucleare; Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT); National Research Foundation of Korea; UK Science and Technology Facilities Council (STFC); Jefferson Science Associates (JSA) [DE-AC05-06OR23177] FX We thank the staff of the Accelerator and Physics Divisions at Jefferson Lab for making the experiment possible. We also thank G. Goldstein, S. Goloskokov, P. Kroll, J. M. Laget, and S. Liuti for many informative discussions and clarifications of their work and making available the results of their calculations. This work was supported in part by the US Department of Energy and National Science Foundation, the French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique, the French-American Cultural Exchange (FACE), the Italian Istituto Nazionale di Fisica Nucleare, the Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT), the National Research Foundation of Korea, and the UK Science and Technology Facilities Council (STFC). The Jefferson Science Associates (JSA) operates the Thomas Jefferson National Accelerator Facility for the United States Department of Energy under Contract No. DE-AC05-06OR23177. NR 37 TC 8 Z9 8 U1 2 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 13 PY 2014 VL 90 IS 2 AR 025205 DI 10.1103/PhysRevC.90.025205 PG 26 WC Physics, Nuclear SC Physics GA AO1WC UT WOS:000341105200007 ER PT J AU Abraham, DB Maciolek, A Vasilyev, O AF Abraham, D. B. Maciolek, A. Vasilyev, O. TI Emergent Long-Range Couplings in Arrays of Fluid Cells SO PHYSICAL REVIEW LETTERS LA English DT Article ID 2-DIMENSIONAL ISING MODEL; TRANSITIONS AB We present a system exhibiting extraordinarily long-range cooperative effects, on a length scale far exceeding the bulk correlation length. We give a theoretical explanation of these phenomena based on the mesoscopic picture of phase coexistence in finite systems, which is confirmed by Monte Carlo simulation studies. Our work demonstrates that such action at a distance can occur in classical systems involving simple or complex fluids, such as colloid-polymer mixtures or ferromagnets. C1 [Abraham, D. B.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Abraham, D. B.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Maciolek, A.; Vasilyev, O.] Max Planck Inst Intelligente Syst, D-70569 Stuttgart, Germany. [Maciolek, A.; Vasilyev, O.] Univ Stuttgart, Inst Theoret Phys 4, D-70569 Stuttgart, Germany. [Maciolek, A.] Polish Acad Sci, Inst Phys Chem, PL-01224 Warsaw, Poland. RP Abraham, DB (reprint author), Univ Oxford, Dept Phys, 1 Keble Rd, Oxford OX1 3NP, England. NR 13 TC 2 Z9 2 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 13 PY 2014 VL 113 IS 7 AR 077204 DI 10.1103/PhysRevLett.113.077204 PG 4 WC Physics, Multidisciplinary SC Physics GA AO2AA UT WOS:000341115700024 PM 25170731 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Anson, CD Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Balewski, J Banerjee, A Beavis, DR Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bichsel, H Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Brandin, AV Brovko, SG Bultmann, S Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Campbell, JM Cebra, D Cendejas, R Cervantes, MC Chaloupka, P Chang, Z Chattopadhyay, S Chen, HF Chen, JH Chen, L Cheng, J Cherney, M Chikanian, A Christie, W Chwastowski, J Codrington, MJM Contin, G Cramer, JG Crawford, HJ Cui, X Das, S Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD Dhamija, S di Ruzza, B Didenko, L Dilks, C Ding, F Djawotho, P Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Engle, KS Eppley, G Eun, L Evdokimov, O Eyser, O Fatemi, R Fazio, S Fedorisin, J Filip, P Finch, E Fisyak, Y Flores, CE Gagliardi, CA Gangadharan, DR Garand, D Geurts, F Gibson, A Girard, M Gliske, S Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, A Gupta, S Guryn, W Haag, B Hamed, A Han, LX Haque, R Harris, JW Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, HZ Huang, X Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Kesich, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Koetke, DD Kollegger, T Konzer, J Koralt, I Kosarzewski, LK Kotchenda, L Kraishan, AF Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH LeVine, MJ Li, C Li, W Li, X Li, X Li, Y Li, ZM Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, GL Ma, YG Don, DMMDM Mahapatra, DP Majka, R Margetis, S Markert, C Masui, H Matis, HS McDonald, D McShane, TS Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nelson, JM Nigmatkulov, G Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Olvitt, DL Pachr, M Page, BS Pal, SK Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Peryt, W Pile, P Planinic, M Pluta, J Poljak, N Poniatowska, K Porter, J Poskanzer, AM Pruthi, NK Przybycien, M Pujahari, PR Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Riley, CK Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ross, JF Roy, A Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Singaraju, RN Skoby, MJ Smirnov, D Smirnov, N Solanki, D Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stevens, JR Stock, R Strikhanov, M Stringfellow, B Sumbera, M Sun, X Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM Szelezniak, MA Takahashi, J Tang, AH Tang, Z Tarnowsky, T Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Trzeciak, BA Tsai, OD Turnau, J Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vandenbroucke, M Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Vossen, A Wada, M Wang, F Wang, G Wang, H Wang, JS Wang, XL Wang, Y Wang, Y Webb, G Webb, JC Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, H Xu, J Xu, N Xu, QH Xu, Y Xu, Z Yan, W Yang, C Yang, Y Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zawisza, Y Zbroszczyk, H Zha, W Zhang, JB Zhang, JL Zhang, S Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhu, X Zhu, YH Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Anson, C. D. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Balewski, J. Banerjee, A. Beavis, D. R. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bichsel, H. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Brandin, A. V. Brovko, S. G. Bueltmann, S. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. Sanchez, M. Calderon de la Barca Campbell, J. M. Cebra, D. Cendejas, R. Cervantes, M. C. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Christie, W. Chwastowski, J. Codrington, M. J. M. Contin, G. Cramer, J. G. Crawford, H. J. Cui, X. Das, S. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. Derradi de Souza, R. Dhamija, S. di Ruzza, B. Didenko, L. Dilks, C. Ding, F. Djawotho, P. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Engle, K. S. Eppley, G. Eun, L. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Fedorisin, J. Filip, P. Finch, E. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Gangadharan, D. R. Garand, D. Geurts, F. Gibson, A. Girard, M. Gliske, S. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hamed, A. Han, L. -X. Haque, R. Harris, J. W. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, H. Z. Huang, X. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kesich, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Kosarzewski, L. K. Kotchenda, L. Kraishan, A. F. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. LeVine, M. J. Li, C. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, G. L. Ma, Y. G. Don, D. M. M. D. Madagodagettige Mahapatra, D. P. Majka, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. McShane, T. S. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nelson, J. M. Nigmatkulov, G. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Olvitt, D. L., Jr. Pachr, M. Page, B. S. Pal, S. K. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Peryt, W. Pile, P. Planinic, M. Pluta, J. Poljak, N. Poniatowska, K. Porter, J. Poskanzer, A. M. Pruthi, N. K. Przybycien, M. Pujahari, P. R. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Riley, C. K. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ross, J. F. Roy, A. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Singaraju, R. N. Skoby, M. J. Smirnov, D. Smirnov, N. Solanki, D. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Sun, X. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szelezniak, M. A. Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Trzeciak, B. A. Tsai, O. D. Turnau, J. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vandenbroucke, M. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Vossen, A. Wada, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, X. L. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, H. Xu, J. Xu, N. Xu, Q. H. Xu, Y. Xu, Z. Yan, W. Yang, C. Yang, Y. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I. -K. Yu, N. Zawisza, Y. Zbroszczyk, H. Zha, W. Zhang, J. B. Zhang, J. L. Zhang, S. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zhu, Y. H. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Measurement of Longitudinal Spin Asymmetries for Weak Boson Production in Polarized Proton-Proton Collisions at RHIC SO PHYSICAL REVIEW LETTERS LA English DT Article ID FLAVOR ASYMMETRY; NUCLEON SEA; ELECTROMAGNETIC CALORIMETER; PARTON DISTRIBUTIONS; QUARK DISTRIBUTIONS; SYMMETRY-BREAKING; GOTTFRIED SUM AB We report measurements of single- and double-spin asymmetries for W-+/- and Z/gamma* boson production in longitudinally polarized p + p collisions at root s = 510 GeV by the STAR experiment at RHIC. The asymmetries for W-+/- were measured as a function of the decay lepton pseudorapidity, which provides a theoretically clean probe of the proton's polarized quark distributions at the scale of the W mass. The results are compared to theoretical predictions, constrained by polarized deep inelastic scattering measurements, and show a preference for a sizable, positive up antiquark polarization in the range 0.05 < x < 0.2. C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, PL-30059 Krakow, Poland. [Gliske, S.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Nelson, J. M.] Univ Birmingham, Birmingham B15 2TT, W Midlands, England. [Arkhipkin, D.; Aschenauer, E. C.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Eyser, O.; Fazio, S.; Fisyak, Y.; Guryn, W.; Huang, B.; Ke, H. W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Wang, H.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Brovko, S. G.; Sanchez, M. Calderon de la Barca; Cebra, D.; Ding, F.; Draper, J. E.; Flores, C. E.; Haag, B.; Kesich, A.; Romero, J. L.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Huang, H. Z.; Igo, G.; Landry, K. D.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, BR-13131 Sao Paulo, Brazil. [Chen, L.; Huck, P.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Wu, Y. F.; Xu, J.; Yang, Y.; Yu, N.; Zhang, J. B.; Zhao, J.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Wang, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Chwastowski, J.; Kycia, R. A.] Cracow Univ Technol, PL-31155 Krakow, Poland. [Cherney, M.; De Silva, L. C.; Don, D. M. M. D. Madagodagettige; McShane, T. S.; Ross, J. F.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Pachr, M.; Rusnakova, O.; Trzeciak, B. 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V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino 142281, Russia. [Garand, D.; Hirsch, A.; Konzer, J.; Li, X.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Llope, W. J.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Chen, H. F.; Cui, X.; Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Yang, C.; Zawisza, Y.; Zha, W.; Zhang, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.; Zhang, J. L.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Han, L. -X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Zhang, S.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Borowski, W.; Kabana, S.] SUBATECH, F-44307 Nantes, France. [Gunarathne, D. S.; Kraishan, A. F.; Li, X.; Olvitt, D. L., Jr.; Surrow, B.; Vandenbroucke, M.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Djawotho, P.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Sahoo, N. R.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Codrington, M. J. M.; Leyva, A. Davila; Hoffmann, G. W.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; McDonald, D.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Huang, X.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Yan, W.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Engle, K. S.; Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Pal, S. K.; Roy, A.; Singaraju, R. N.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kikola, D. P.; Kisiel, A.; Kosarzewski, L. K.; Pawlak, T.; Peryt, W.; Pluta, J.; Poniatowska, K.; Zbroszczyk, H.] Warsaw Univ Technol, PL-00661 Warsaw, Poland. [Bichsel, H.; Cramer, J. G.] Univ Washington, Seattle, WA 98195 USA. [Putschke, J.] Wayne State Univ, Detroit, MI 48201 USA. [Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Horvat, S.; Majka, R.; Ohlson, A.; Riley, C. K.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, PL-30059 Krakow, Poland. RI Yi, Li/Q-1705-2016; Alekseev, Igor/J-8070-2014; Svirida, Dmitry/R-4909-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017; Yip, Kin/D-6860-2013; Derradi de Souza, Rafael/M-4791-2013; Xin, Kefeng/O-9195-2016; Sumbera, Michal/O-7497-2014; Strikhanov, Mikhail/P-7393-2014; Takahashi, Jun/B-2946-2012; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; XIAO, Zhigang/C-3788-2015; Fazio, Salvatore /G-5156-2010; Kumar, Lokesh/A-6154-2010; Kycia, Radoslaw/J-4397-2015; Chaloupka, Petr/E-5965-2012; Huang, Bingchu/H-6343-2015 OI Yi, Li/0000-0002-7512-2657; Alekseev, Igor/0000-0003-3358-9635; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418; Yip, Kin/0000-0002-8576-4311; Fisyak, Yuri/0000-0002-3151-8377; Ke, Hongwei/0000-0003-1463-7291; Sorensen, Paul/0000-0001-5056-9391; Thomas, James/0000-0002-6256-4536; Derradi de Souza, Rafael/0000-0002-2084-7001; Xin, Kefeng/0000-0003-4853-9219; Sumbera, Michal/0000-0002-0639-7323; Strikhanov, Mikhail/0000-0003-2586-0405; Takahashi, Jun/0000-0002-4091-1779; Kumar, Lokesh/0000-0002-2746-9840; Kycia, Radoslaw/0000-0002-6390-4627; Huang, Bingchu/0000-0002-3253-3210 FU RHIC Operations Group; RCF at BNL; NERSC Center at LBNL; KISTI Center in Korea; Open Science Grid consortium; Office of NP within the U.S. DOE Office of Science; Office of HEP within the U.S. DOE Office of Science; U.S. NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation, GA; MSMT of the Czech Republic, FIAS of Germany; DAE; DST; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia FX We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. We are grateful to M. Stratmann for useful discussions. This work was supported in part by the Offices of NP and HEP within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3, FAPESP CNPq of Brazil, the Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST and MoE of China, the Korean Research Foundation, GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and CSIR of India, the National Science Centre of Poland, National Research Foundation (NRF-2012004024), the Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. NR 36 TC 21 Z9 21 U1 0 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 13 PY 2014 VL 113 IS 7 AR 072301 DI 10.1103/PhysRevLett.113.072301 PG 7 WC Physics, Multidisciplinary SC Physics GA AO2AA UT WOS:000341115700005 ER PT J AU Chernikov, A Berkelbach, TC Hill, HM Rigosi, A Li, YL Aslan, OB Reichman, DR Hybertsen, MS Heinz, TF AF Chernikov, Alexey Berkelbach, Timothy C. Hill, Heather M. Rigosi, Albert Li, Yilei Aslan, Ozgur Burak Reichman, David R. Hybertsen, Mark S. Heinz, Tony F. TI Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID VALLEY POLARIZATION; MOS2; WSE2; PHOTOLUMINESCENCE; SEMICONDUCTOR; SHEETS; FILMS AB We have experimentally determined the energies of the ground and first four excited excitonic states of the fundamental optical transition in monolayer WS2, a model system for the growing class of atomically thin two-dimensional semiconductor crystals. From the spectra, we establish a large exciton binding energy of 0.32 eV and a pronounced deviation from the usual hydrogenic Rydberg series of energy levels of the excitonic states. We explain both of these results using a microscopic theory in which the nonlocal nature of the effective dielectric screening modifies the functional form of the Coulomb interaction. These strong but unconventional electron-hole interactions are expected to be ubiquitous in atomically thin materials. C1 [Chernikov, Alexey; Hill, Heather M.; Rigosi, Albert; Li, Yilei; Aslan, Ozgur Burak; Heinz, Tony F.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Chernikov, Alexey; Hill, Heather M.; Rigosi, Albert; Li, Yilei; Aslan, Ozgur Burak; Heinz, Tony F.] Columbia Univ, Dept Elect Engn, New York, NY 10027 USA. [Berkelbach, Timothy C.; Reichman, David R.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Hybertsen, Mark S.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Chernikov, A (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. EM aac2183@columbia.edu; tony.heinz@columbia.edu RI Heinz, Tony/K-7797-2015; OI Heinz, Tony/0000-0003-1365-9464; Aslan, Ozgur Burak/0000-0002-0925-3026; Hybertsen, Mark S/0000-0003-3596-9754 FU Center for Re-Defining Photovoltaic Efficiency through Molecule Scale Control, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001085]; National Science Foundation [DMR-1122594, DMR-1124894]; Alexander von Humboldt Foundation within the Feodor-Lynen Fellowship Program; U.S. Department of Energy, Office of Science [DE-AC05-06OR23100]; NSF [DGE-1069240]; NSF; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported in part by the Center for Re-Defining Photovoltaic Efficiency through Molecule Scale Control, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0001085. Support for the reflection contrast measurements was also provided by the National Science Foundation through Grants No. DMR-1122594 and No. DMR-1124894. A. C. gratefully acknowledges funding from the Alexander von Humboldt Foundation within the Feodor-Lynen Fellowship Program. T. C. B. was supported in part by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC05-06OR23100. H. M. H. and A. R. were supported by the NSF through an IGERT Fellowship (Grant No. DGE-1069240) and through a Graduate Research Fellowship, respectively. This work was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886 (M. S. H). NR 48 TC 290 Z9 291 U1 44 U2 191 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 13 PY 2014 VL 113 IS 7 AR 076802 DI 10.1103/PhysRevLett.113.076802 PG 5 WC Physics, Multidisciplinary SC Physics GA AO2AA UT WOS:000341115700020 PM 25170725 ER PT J AU Gopalakrishnan, S Martin, I Demler, EA AF Gopalakrishnan, S. Martin, I. Demler, E. A. TI Comment on "Quantum Quasicrystals of Spin-Orbit-Coupled Dipolar Bosons" Reply SO PHYSICAL REVIEW LETTERS LA English DT Editorial Material ID CHARGE-DENSITY WAVES C1 [Gopalakrishnan, S.; Demler, E. A.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Martin, I.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Gopalakrishnan, S (reprint author), Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. NR 14 TC 2 Z9 2 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 13 PY 2014 VL 113 IS 7 AR 079603 DI 10.1103/PhysRevLett.113.079603 PG 2 WC Physics, Multidisciplinary SC Physics GA AO2AA UT WOS:000341115700031 PM 25170739 ER PT J AU Hazra, DK Shafieloo, A Smoot, GF Starobinsky, AA AF Hazra, Dhiraj Kumar Shafieloo, Arman Smoot, George F. Starobinsky, Alexei A. TI Inflation with Whip-Shaped Suppressed Scalar Power Spectra SO PHYSICAL REVIEW LETTERS LA English DT Article ID PROBE WMAP OBSERVATIONS; MICROWAVE; UNIVERSE AB Motivated by the idea that inflation occurs at the grand unified theory symmetry breaking scale, in this Letter we construct a new class of large field inflaton potentials where the inflaton starts with a power law potential; after an initial period of relatively fast roll that lasts until after a few e folds inside the horizon it transits to the attractor of the slow roll part of the potential with a lower power. Because of the initial fast roll stages of inflation, we find a suppression in scalar primordial power at large scales and at the same time the choice of the potential can provide us a tensor primordial spectrum with a high amplitude. This suppression in scalar power with a large tensor-to-scalar ratio helps us to reconcile the Planck and BICEP2 data in a single framework. We find that a transition from a cubic to quadratic form of inflaton potential generates an appropriate suppression in the power of the scalar primordial spectrum that provides a significant improvement in fit compared to the power law model when compared with Planck and BICEP2 data together. We calculate the extent of non-Gaussianity, specifically, the bispectrum for the best fit potential, and show that it is consistent with Planck bispectrum constraints. C1 [Hazra, Dhiraj Kumar; Shafieloo, Arman] Asia Pacific Ctr Theoret Phys, Pohang 790784, Gyeongbuk, South Korea. [Shafieloo, Arman] POSTECH, Dept Phys, Pohang 790784, Gyeongbuk, South Korea. [Smoot, George F.] Univ Paris 10, Univ Sorbonne Paris Cite, Lab APC PCCP, F-75205 Paris 13, France. [Smoot, George F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Smoot, George F.] Univ Calif Berkeley, LBNL, Berkeley, CA 94720 USA. [Starobinsky, Alexei A.] RAS, Landau Inst Theoret Phys, Moscow 119334, Russia. RP Hazra, DK (reprint author), Asia Pacific Ctr Theoret Phys, Pohang 790784, Gyeongbuk, South Korea. EM dhiraj@apctp.org; arman@apctp.org; gfsmoot@lbl.gov; alstar@landau.ac.ru OI Starobinsky, Alexei/0000-0002-8946-9088 FU Korea Ministry of Education, Science and Technology; Gyeongsangbuk-Do and Pohang City for Independent Junior Research Groups at the Asia Pacific Center for Theoretical Physics; National Research Foundation of Korea [NRF-2013R1A1A2013795]; Chaire d'Excellence Universite Sorbonne Paris Cite; UNIVEARTHS LABEX program at Universite Sorbonne Paris Cite [ANR-10-LABX-0023, ANR-11-IDEX-0005-02]; [RFBR 14-02-00894] FX D. K. H. and A. S. wish to acknowledge support from the Korea Ministry of Education, Science and Technology, Gyeongsangbuk-Do and Pohang City for Independent Junior Research Groups at the Asia Pacific Center for Theoretical Physics. We also acknowledge the use of publicly available CAMB and COSMOMC in our analysis. The authors would like to thank Antony Lewis for providing us the new COSMOMC package that takes into account the recent BICEP2 data. We acknowledge the use of WMAP-9 data and from the Legacy Archive for Microwave Background Data Analysis (LAMBDA) [39], Planck data and likelihood from the Planck Legacy Archive (PLA) [40], and BICEP2 data from [41]. A. S. would like to acknowledge the support of the National Research Foundation of Korea (NRF-2013R1A1A2013795). G. F. S. acknowledges support through his Chaire d'Excellence Universite Sorbonne Paris Cite and the financial support of the UNIVEARTHS LABEX program at Universite Sorbonne Paris Cite (ANR-10-LABX-0023 and ANR-11-IDEX-0005-02). A. A. S. thanks Professor E. Guendelman for hospitality in the Ben-Gurion University, Beer-Sheva, Israel, during the period when this Letter was finished. A. A. S. was also partially supported by Grant No. RFBR 14-02-00894. NR 50 TC 25 Z9 25 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 13 PY 2014 VL 113 IS 7 AR 071301 DI 10.1103/PhysRevLett.113.071301 PG 6 WC Physics, Multidisciplinary SC Physics GA AO2AA UT WOS:000341115700003 PM 25170696 ER PT J AU Ren, YF Hansen, SF Ebert, B Lau, J Scheller, HV AF Ren, Yanfang Hansen, Sara Fasmer Ebert, Berit Lau, Jane Scheller, Henrik Vibe TI Site-Directed Mutagenesis of IRX9, IRX9L and IRX14 Proteins Involved in Xylan Biosynthesis: Glycosyltransferase Activity Is Not Required for IRX9 Function in Arabidopsis SO PLOS ONE LA English DT Article ID GLUCURONOXYLAN BIOSYNTHESIS; COMPLEX; REVEALS; MEMBERS; GENES; GT43; ELONGATION; BACKBONE; RESIDUES AB Xylans constitute the main non-cellulosic polysaccharide in the secondary cell walls of plants. Several genes predicted to encode glycosyltransferases are required for the synthesis of the xylan backbone even though it is a homopolymer consisting entirely of beta-1,4-linked xylose residues. The putative glycosyltransferases IRX9, IRX14, and IRX10 (or the paralogs IRX9L, IRX14L, and IRX10L) are required for xylan backbone synthesis in Arabidopsis. To investigate the function of IRX9, IRX9L, and IRX14, we identified amino acid residues known to be essential for catalytic function in homologous mammalian proteins and generated modified cDNA clones encoding proteins where these residues would be mutated. The mutated gene constructs were used to transform wild-type Arabidopsis plants and the irx9 and irx14 mutants, which are deficient in xylan synthesis. The ability of the mutated proteins to complement the mutants was investigated by measuring growth, determining cell wall composition, and microscopic analysis of stem cross-sections of the transgenic plants. The six different mutated versions of IRX9 and IRX9-L were all able to complement the irx9 mutant phenotype, indicating that residues known to be essential for glycosyltransferases function in homologous proteins are not essential for the biological function of IRX9/IRX9L. Two out of three mutated IRX14 complemented the irx14 mutant, including a mutant in the predicted catalytic amino acid. A IRX14 protein mutated in the substrate-binding DxD motif did not complement the irx14 mutant. Thus, substrate binding is important for IRX14 function but catalytic activity may not be essential for the function of the protein. The data indicate that IRX9/IRX9L have an essential structural function, most likely by interacting with the IRX10/IRX10L proteins, but do not have an essential catalytic function. Most likely IRX14 also has primarily a structural role, but it cannot be excluded that the protein has an important enzymatic activity. C1 [Ren, Yanfang; Hansen, Sara Fasmer; Ebert, Berit; Lau, Jane; Scheller, Henrik Vibe] Lawrence Berkeley Natl Lab, Joint Bioenergy Inst, Berkeley, CA 94720 USA. [Ren, Yanfang] Guizhou Univ, Coll Agr, Guiyang, Peoples R China. [Ebert, Berit] Univ Copenhagen, Fac Sci, Dept Plant & Environm Sci, Frederiksberg, Denmark. [Scheller, Henrik Vibe] Univ Calif, Dept Plant & Microbial Biol, Berkeley, CA USA. RP Scheller, HV (reprint author), Lawrence Berkeley Natl Lab, Joint Bioenergy Inst, Berkeley, CA 94720 USA. EM hscheller@lbl.gov RI Ebert, Berit/F-1856-2016; Scheller, Henrik/A-8106-2008 OI Ebert, Berit/0000-0002-6914-5473; Scheller, Henrik/0000-0002-6702-3560 FU U.S. Department of Energy, Office of Science (science.energy.gov), Office of Biological and Environmental Research [DE-AC02-05CH11231]; Lawrence Berkeley National Laboratory; China Scholarship Council [2010852564]; Carlsberg Foundation [2010_01_0509] FX This work was funded by the U.S. Department of Energy, Office of Science (science.energy.gov), Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 with Lawrence Berkeley National Laboratory. YR was supported by China Scholarship Council (www.csc.edu.cn) grant 2010852564. SFH was supported by a fellowship from The Carlsberg Foundation (www.carlsbergfondet.dk) contract 2010_01_0509. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 31 TC 12 Z9 12 U1 3 U2 16 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 13 PY 2014 VL 9 IS 8 AR e105014 DI 10.1371/journal.pone.0105014 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AN9BM UT WOS:000340900600112 PM 25118690 ER PT J AU Kusoglu, A Kushner, D Paul, DK Karan, K Hickner, MA Weber, AZ AF Kusoglu, Ahmet Kushner, Douglas Paul, Devproshad K. Karan, Kunal Hickner, Michael A. Weber, Adam Z. TI Impact of Substrate and Processing on Confinement of Nafion Thin Films SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID X-RAY-SCATTERING; CELL CATALYST LAYERS; PERFLUOROSULFONIC ACID IONOMERS; PROTON CONDUCTION MECHANISM; ELECTROLYTE FUEL-CELLS; WATER-UPTAKE; SCHROEDERS-PARADOX; MONOLAYER FILMS; ADSORBED NAFION; MEMBRANES AB Thin films of ion-conducting polymers are an important area of study due to their function in many electrochemical devices and as analogues for interfacial phenomena that occur in bulk films. In this paper, the properties of Nafion, a prototypical ionomer, are investigated as thin films (4 to 300 nm) on carbon, gold, and platinum substrates that are fabricated using different casting methods and thermal histories. Specifically, water uptake, swelling, and morphology are investigated by quartz-crystal microbalance, ellipsometry, and grazing-incidence X-ray scattering to develop structure/property/ processing relationships. For all substrates, as the films' thickness decreased, there is an initial decrease in swelling followed by a subsequent increase for film thicknesses below approximate to 20 nm due to a disordering of the film hydrophilic/hydrophobic structure. Decreased swelling and less structural order is observed on gold for spin-cast films compared to self-assembled films; the opposite effect is observed for films on carbon. The presented systematic data set and analyses represent a thorough study of the behavior of Nafion thin films on model substrates of interest in metal catalyst/carbon electrodes, and these insights help to elucidate the underlying polymer physics and confinement effects in these and related systems. C1 [Kusoglu, Ahmet; Weber, Adam Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Kushner, Douglas; Hickner, Michael A.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Paul, Devproshad K.; Karan, Kunal] Queens Univ, Dept Chem Engn, Kingston, ON K7L 3N6, Canada. RP Kusoglu, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM azweber@lbl.gov OI Kusoglu, Ahmet/0000-0002-2761-1050 FU Fuel Cell Technologies Office, of the U. S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, the Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office through General Motors Corporation [DE-EE0000470]; Natural Sciences and Engineering Research Council of Canada (NSERC); Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank Dr. Miguel Modestino for helpful discussions and preparation of the Pt substrates. The authors also thank Dr. Alex Hexemer for helpful discussions and facilitating the use of equipment at the Advanced Light Source (ALS) in Berkeley Lab. A. K. and A.Z.W. were supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office, of the U. S. Department of Energy under contract number DE-AC02-05CH11231; D. K. and M. A. H. acknowledge the support of the U.S. Department of Energy, the Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office through a subcontract from General Motors Corporation under Grant DE-EE0000470; D. K. P. and K. K. acknowledge financial support from Natural Sciences and Engineering Research Council of Canada (NSERC). This work made use of facilities at the Advanced Light Source (ALS) beamline 7.3.3, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (Contract No. DE-AC02-05CH11231). NR 73 TC 30 Z9 30 U1 7 U2 76 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD AUG 13 PY 2014 VL 24 IS 30 BP 4763 EP 4774 DI 10.1002/adfm.201304311 PG 12 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AN4IB UT WOS:000340549900005 ER PT J AU Keller, AM Ghosh, Y DeVore, MS Phipps, ME Stewart, MH Wilson, BS Lidke, DS Hollingsworth, JA Werner, JH AF Keller, Aaron M. Ghosh, Yagnaseni DeVore, Matthew S. Phipps, Mary E. Stewart, Michael H. Wilson, Bridget S. Lidke, Diane S. Hollingsworth, Jennifer A. Werner, James H. TI 3-Dimensional Tracking of Non-blinking 'Giant' Quantum Dots in Live Cells SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID SINGLE-PARTICLE TRACKING; MOLECULE TRACKING; SHELL-THICKNESS; MULTIFUNCTIONAL LIGANDS; AUGER RECOMBINATION; SUPPRESSED BLINKING; DIFFUSION; MEMBRANE; RECEPTOR; TIME AB While semiconductor quantum dots (QDs) have been used successfully in numerous single particle tracking (SPT) studies due to their high photoluminescence efficiency, photostability, and broad palette of emission colors, conventional QDs exhibit fluorescence intermittency or 'blinking,' which causes ambiguity in particle trajectory analysis and limits tracking duration. Here, non-blinking 'giant' quantum dots (gQDs) are exploited to study IgE-Fc epsilon RI receptor dynamics in live cells using a confocal-based 3D SPT microscope. There is a 7-fold increase in the probability of observing IgE-Fc epsilon RI for longer than 1 min using the gQDs compared to commercially available QDs. A time-gated photon-pair correlation analysis is implemented to verify that selected SPT trajectories are definitively from individual gQDs and not aggregates. The increase in tracking duration for the gQDs allows the observation of multiple changes in diffusion rates of individual IgE-Fc epsilon RI receptors occurring on long (>1 min) time scales, which are quantified using a time-dependent diffusion coefficient and hidden Markov modeling. Non-blinking gQDs should become an important tool in future live cell 2D and 3D SPT studies, especially in cases where changes in cellular dynamics are occurring on the time scale of several minutes. C1 [Keller, Aaron M.; Ghosh, Yagnaseni; DeVore, Matthew S.; Phipps, Mary E.; Hollingsworth, Jennifer A.; Werner, James H.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Stewart, Michael H.] US Naval Res Lab, Opt Sci Div, Washington, DC 20375 USA. [Wilson, Bridget S.; Lidke, Diane S.] Univ New Mexico, Hlth Sci Ctr, Dept Pathol, Albuquerque, NM 87131 USA. [Wilson, Bridget S.; Lidke, Diane S.] Univ New Mexico, Hlth Sci Ctr, Canc Res & Treatment Ctr, Albuquerque, NM 87131 USA. RP Keller, AM (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM jenn@lanl.gov; jwerner@lanl.gov FU National Institutes of Health [5R01AI097154-02]; NIH-NIGMS Grant [1R01GM084702-01]; Los Alamos National Laboratory Directed Research and Development Program; National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396]; New Mexico Spatiotemporal Modeling Center [P50GM0852673]; NIH [R01GM100114]; [P50 GM065794]; [R01AI051575] FX This work was supported by the National Institutes of Health (5R01AI097154-02) JHW. JAH also acknowledges partial support by NIH-NIGMS Grant 1R01GM084702-01. YG was supported in part by the Los Alamos National Laboratory Directed Research and Development Program. This work was performed at the Center for Integrated Nanotechnologies, a US Department of Energy, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. Collaborative efforts were also supported by P50 GM065794 and R01AI051575 (BSW), the New Mexico Spatiotemporal Modeling Center (P50GM0852673) and NIH R01GM100114 (DSL). We thank Jennifer Martinez for advice on bioconjugation and general use of laboratory resources, Peter Goodwin for assistance with AFM measurements, Patrick Cutler and Cedric Cleyrat for advice on handling and labeling the RBL-2H3 mast cells, Darrick Williams for advice on QD water solubilization via ligand exchange, Han Htoon for advice on assessing the number of gQD particles using time-gated PPC, and Pengfei Zhang for assistance with the PPC analysis. NR 58 TC 9 Z9 9 U1 9 U2 47 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD AUG 13 PY 2014 VL 24 IS 30 BP 4796 EP 4803 DI 10.1002/adfm.201400349 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AN4IB UT WOS:000340549900009 PM 25798080 ER PT J AU Vautard, F Grappe, H Ozcan, S AF Vautard, Frederic Grappe, Hippolyte Ozcan, Soydan TI Engineered Interface Chemistry to Improve the Strength of Carbon Fiber Composites Cured by Electron Beam SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID ADHESION STRENGTH; SURFACE; EPOXY; OXIDATION; PLASMA; BULK AB A reactive sizing was designed to achieve high levels of interfacial adhesion and improved mechanical properties with a carbon fiber acrylate system cured by electron beam (EB). The sizing was made of a partially cured epoxy sizing with a high density of pendant functional groups (acrylate functionality) to facilitate covalent bonding with the matrix. The interlaminar shear strength improved from 61 to 81 MPa (+33%) without postprocessing, reaching a shear strength similar to that of the same system cured by a thermal treatment. Observation of the fracture profiles clearly highlighted a change in the fracture mechanism from a purely adhesive failure to a cohesive failure. To the best of our knowledge, such improvements of the mechanical properties of carbon fiber composites cured by EB, without any postcure, have not been reported previously. This constitutes a breakthrough for the industrial development of EB curing of composites. C1 [Vautard, Frederic; Grappe, Hippolyte; Ozcan, Soydan] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Vautard, F (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM vautard@msu.edu OI Ozcan, Soydan/0000-0002-3825-4589 FU U.S. Department of Energy [DE-AC05-00OR22725]; Shared Research Equipment (ShaRE) User Facility FX This manuscript was authored by UT-Battelle, LLC, under Contract DE-AC05-00OR22725 with the U.S. Department of Energy. The U.S. government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. government retains, a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. government purposes. This research was supported in part by the Shared Research Equipment (ShaRE) User Facility operated for the U.S. Department of Energy Office of Science by the Oak Ridge National Laboratory. Cytec Industries Inc. is sincerely thanked for providing Ebecryl 600. Huntsman Advanced Materials and Momentive are gratefully acknowledged for providing Araldite MY 721 and Epon 828, respectively. Bayer Material Science LLC is sincerely thanked for providing Desmolux D 100. NR 26 TC 4 Z9 4 U1 1 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD AUG 13 PY 2014 VL 53 IS 32 BP 12729 EP 12736 DI 10.1021/ie501678j PG 8 WC Engineering, Chemical SC Engineering GA AN2UI UT WOS:000340441000019 ER PT J AU Liu, J Fernandez, CA Martin, PF Thallapally, PK Strachan, DM AF Liu, Jian Fernandez, Carlos A. Martin, Paul F. Thallapally, Praveen K. Strachan, Denis M. TI A Two-Column Method for the Separation of Kr and Xe from Process Off-Gases SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID METAL-ORGANIC FRAMEWORK; COORDINATION SITES; ADSORPTION SITES; SURFACE-AREA; NOBLE-GASES; STORAGE; PORES; XENON AB Radioactive isotopes of xenon (Xe) and krypton (Kr) exist in the off-gases from the reprocessing of nuclear fuels. To meet regulations, at least the Kr needs to be removed from these off-gas streams. Two metal organic framework (MOF) materials were investigated to determine the removal efficiency and capacity of MOF materials for krypton recovery from air at noncryogenic temperatures. Our two-column breakthrough measurements on nickel dioxobenzenodicarboxylic acid and a partially fluorinated MOF with copper indicate that these materials can capture and separate parts per million levels of Xe and Kr from air. In a two-column system, the removal efficiency and adsorption capacity for Kr on these two MOFs were further increased upon removal of Xe on the first bed. These results show that there is a promising future for the use of MOFs for the removal of noble gas radionuclides from process off-gases during reactor operation or reprocessing of irradiated nuclear fuels. C1 [Liu, Jian; Fernandez, Carlos A.; Martin, Paul F.; Strachan, Denis M.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Thallapally, Praveen K.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Thallapally, PK (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM Praveen.Thallapally@pnnl.gov RI Liu, Jian/C-4707-2011; Liu, Jian/D-3393-2009; OI Liu, Jian/0000-0001-5329-7408; Liu, Jian/0000-0001-5329-7408; Thallapally, Praveen Kumar/0000-0001-7814-4467 FU U.S. Department of Energy (DOE), Office of Nuclear Energy; U.S. Department of Energy by Battelle Memorial Institute [DE-AC05-76RL01830] FX The authors would like to thank the U.S. Department of Energy (DOE), Office of Nuclear Energy for their support, in particular, Dr. James Bresee who has direct project oversight responsibilities. The authors would also like to thank Dr. Terry Todd (Idaho National Laboratory) and Dr. Robert Jubin (Oak Ridge National Laboratory) for their continued programmatic support and guidance. Pacific Northwest National Laboratory is a multiprogram national laboratory operated for the U.S. Department of Energy by Battelle Memorial Institute under Contract DE-AC05-76RL01830. NR 31 TC 8 Z9 8 U1 7 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD AUG 13 PY 2014 VL 53 IS 32 BP 12893 EP 12899 DI 10.1021/ie502156h PG 7 WC Engineering, Chemical SC Engineering GA AN2UI UT WOS:000340441000037 ER PT J AU Fedin, I Talapin, DV AF Fedin, Igor Talapin, Dmitri V. TI Probing the Surface of Colloidal Nanomaterials with Potentiometry in Situ SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CDTE QUANTUM DOTS; CDSE NANOCRYSTALS; GROWTH; LIGANDS; GOLD AB Colloidal nanomaterials represent an important branch of modem chemistry. However, we have very little understanding of molecular processes that occur at the nanocrystal (NC) surface during synthesis and post-synthetic modifications. Here we show that potentiometry can be used to study the surface of colloidal NCs under realistic reaction conditions. Potentiometric titrations of CdSe and InP nanostructures provide information on the active surface area, the affinity of ligands to the NC surface, and the surface reaction kinetics. These studies can be carried out at different temperatures in polar and nonpolar media for NCs of different sizes and shapes. In situ potentiometry can provide real-time feedback during synthesis of core-shell nanostructures. C1 [Fedin, Igor; Talapin, Dmitri V.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Fedin, Igor; Talapin, Dmitri V.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Talapin, Dmitri V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Talapin, DV (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM dvtalapin@uchicago.edu FU NSF [DMR-1310398]; DOD ONR [N00014-13-1-0490]; David and Lucie Packard Foundation; Keck Foundation; NSF MRSEC Program [DMR 08-20054]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We thank Sandrine Ithurria for advice on NC synthesis, J. Matthew Kurley for help with the experimental setup, and Dmitriy S. Dolzhnikov for advice on the electrode preparation. This work was supported by NSF under Award No. DMR-1310398 and by DOD ONR under Award No. N00014-13-1-0490. D.V.T. also thanks the David and Lucie Packard Foundation and Keck Foundation for support. This work used facilities supported by NSF MRSEC Program Award No. DMR 08-20054. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 29 TC 5 Z9 5 U1 4 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 13 PY 2014 VL 136 IS 32 BP 11228 EP 11231 DI 10.1021/ja503866w PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AN2UY UT WOS:000340442700006 PM 25066770 ER PT J AU Qiao, ZA Zhang, PF Chai, SH Chi, MF Veith, GM Gallego, NC Kidder, M Dai, S AF Qiao, Zhen-An Zhang, Pengfei Chai, Song-Hai Chi, Miaofang Veith, Gabriel M. Gallego, Nidia C. Kidder, Michelle Dai, Sheng TI Lab-in-a-Shell: Encapsulating Metal Clusters for Size Sieving Catalysis SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SOLVENT-FREE OXIDATION; HETEROGENEOUS CATALYST; SELECTIVE OXIDATION; NANOPARTICLE CATALYSTS; ALCOHOL OXIDATION; AEROBIC OXIDATION; PD NANOPARTICLES; CO OXIDATION; CARBON; GOLD AB Here we describe a lab-in-a-shell strategy for the preparation of multifunctional core shell nano-spheres consisting of a core of metal clusters and an outer microporous silica shell. Various metal clusters (e.g., Pd and Pt) were encapsulated and confined in the void space mediated by the entrapped polymer dots inside hollow silica nanospheres acting first as complexing agent for metal ions and additionally as encapsulator for dusters, limiting growth and suppressing the sintering. The Pd clusters encapsulated in hybrid core shell structures exhibit exceptional size-selective catalysis in allylic oxidations of substrates with the same reactive site but different molecular size (cyclohexene similar to 0.5 nm, cholesteryl acetate similar to 1.91 nm). The solvent-free aerobic oxidation of diverse hydrocarbons and alcohols was further carried out to illustrate the benefits of such an architecture in catalysis. High activity, outstanding thermal stability and good recyclability were observed over the core shell nanocatalyst. C1 [Qiao, Zhen-An; Zhang, Pengfei; Chai, Song-Hai; Kidder, Michelle; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Chi, Miaofang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Veith, Gabriel M.; Gallego, Nidia C.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Zhang, PF (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM chemistryzpf@163.com; dais@ornl.gov RI Chai, Song-Hai/A-9299-2012; Dai, Sheng/K-8411-2015; Zhang, Pengfei/I-5484-2013; Chi, Miaofang/Q-2489-2015; OI Chai, Song-Hai/0000-0002-4152-2513; Dai, Sheng/0000-0002-8046-3931; Chi, Miaofang/0000-0003-0764-1567; Qiao, Zhen-An/0000-0001-6064-9360; Gallego, Nidia/0000-0002-8252-0194 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. NR 36 TC 53 Z9 53 U1 26 U2 298 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 13 PY 2014 VL 136 IS 32 BP 11260 EP 11263 DI 10.1021/ja505903r PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AN2UY UT WOS:000340442700014 PM 25075561 ER EF